WorldWideScience

Sample records for atomic beam diffraction

  1. Diffraction of helium atom beams from a micro-structured reflection grating

    Energy Technology Data Exchange (ETDEWEB)

    Zhao, Bum Suk; Meijer, Gerard; Schoellkopf, Wieland [Fritz-Haber-Institut der Max-Planck-Gesellschaft, Berlin (Germany); Schulz, Stephan [Universitaet Ulm (Germany). Institut fuer Quanteninformationsverarbeitung

    2008-07-01

    We have observed high-resolution diffraction patterns of a thermal-energy helium-atom beam reflected from a micro-structured surface grating at grazing incidence. The grating has a periodicity of 20 {mu}m and consists of 10-{mu}m-wide Cr stripes patterned on a quartz substrate. Fully-resolved diffraction peaks up to the 7-th order are observed at grazing incidence angles up to 20 mrad. With changes in de Broglie wavelength or incidence angle the relative diffraction intensities show significant variations which are attributed to the atom-surface Casimir-van der Waals potential. In addition, the overall probability of coherent reflection is found to increase with increasing de Broglie wavelength and decreasing incidence angle. We discuss whether this behavior indicates quantum reflection at the long-range attractive branch of the atom-surface potential.

  2. Fast atom diffraction inside a molecular beam epitaxy chamber, a rich combination

    Science.gov (United States)

    Debiossac, M.; Atkinson, P.; Zugarramurdi, A.; Eddrief, M.; Finocchi, F.; Etgens, V. H.; Momeni, A.; Khemliche, H.; Borisov, A. G.; Roncin, P.

    2017-01-01

    Two aspects of the contribution of grazing incidence fast atom diffraction (GIFAD) to molecular beam epitaxy (MBE) are reviewed here: the ability of GIFAD to provide in-situ a precise description of the atomic-scale surface topology, and its ability to follow larger-scale changes in surface roughness during layer-by-layer growth. Recent experimental and theoretical results obtained for the He atom beam incident along the highly corrugated [ 1 1 bar 0 ] direction of the β2(2 × 4) reconstructed GaAs(001) surface are summarized. We also discuss the measurements and calculations for the beam incidence along the weakly corrugated [010] direction where a periodicity twice smaller than expected is observed. The combination of the experiment, quantum scattering matrix calculations, and semiclassical analysis allows structural characteristics of the surface to be revealed. For the in situ measurements of GIFAD during molecular beam epitaxy of GaAs on GaAs surface we analyze the change in elastic and inelastic contributions in the scattered beam, and the variation of the diffraction pattern in polar angle scattering. This analysis outlines the robustness, the simplicity and the richness of the GIFAD as a technique to monitor the layer-by-layer epitaxial growth.

  3. Diffracted field distribution from a knife-edge truncated semi- Gaussian beam as an atomic (molecular) mirror

    Institute of Scientific and Technical Information of China (English)

    Zheng Ping; Gao Wei-Jian; Yin Jian-Ping

    2006-01-01

    We investigate the diffraction characteristics of an incident Gaussian beam cut by a straight edge bounding a semi-infinite opaque plane using Kirchhoff scalar wave theory in the Fresnel limit, and propose a new and simple mirror scheme to reflect atoms by using the intensity gradient induced by a blue-detuned semi-Gaussian laser beam. The optical potential of the diffracted light of the knife-cut semi-Gaussian beam for 85Rb atom and its spontaneous emission probability are calculated and compared with the performance of the evanescent-wave mirror. Our study shows that the optical potential of the diffracted light of the semi-Gaussian beam is far higher than that of the evanescent light wave, and the maximum normal velocity of the incident atoms can be far greater than that of the evanescent light wave under the same parameters, so the blue-detuned semi-Gaussian beam, as a novel atomic mirror, can be used to efficiently reflect cold atoms with a normal velocity of greater than 1 m/s. However, the intensity gradient (force) of the diffracted light of the semi-Gaussian-beam is much smaller than that of the evanescent light wave, so its spontaneous emission probability is greater than that from the evanescent-wave when the normal velocity of incident atoms is greater.

  4. Double diffraction in an atomic gravimeter

    CERN Document Server

    Malossi, Nicola; Merlet, Sébastien; Landragin, Arnaud; Santos, Franck Pereira Dos

    2009-01-01

    We demonstrate the realization of a new scheme for cold atom gravimetry based on the use of double diffraction beamsplitters recently demonstrated in \\cite{Leveque}, where the use of two retro-reflected Raman beams allows symmetric diffraction in $\\pm \\hbar k_{eff}$ momenta. Though in principle restricted to the case of zero Doppler shift, for which the two pairs of Raman beams are simultaneously resonant, we demonstrate that such diffraction pulses can remain efficient on atoms with non zero velocity, such as in a gravimeter, when modulating the frequency of one of the two Raman laser sources. We use such pulses to realize an interferometer insensitive to laser phase noise and some of the dominant systematics. This reduces the technical requirements and would allow the realization of a simple atomic gravimeter. We demonstrate a sensitivity of $1.2\\times10^{-7}g$ per shot.

  5. Tunable Beam Diffraction in Infiltrated Microstructured Fibers

    DEFF Research Database (Denmark)

    Rosberg, Christian Romer; Bennet, Francis H.; Neshev, Dragomir N.;

    We experimentally study beam propagation in two dimensional photonic lattices in microstructured optical fibers infiltrated with high index liquids. We demonstrate strongly tunable beam diffraction by dynamically varying the coupling between individual lattice sites....

  6. Relation between reflection high-energy electron diffraction specular beam intensity and the surface atomic structure/surface morphology of GaAs(111)B

    Energy Technology Data Exchange (ETDEWEB)

    Chen, P.; Rajkumar, K.C.; Madhukar, A. (Univ. of Southern California, Los Angeles (United States))

    The intensity behavior of the specular beam in reflection high-energy electron diffraction (RHEED) from GaAs(111)B grown by molecular-beam epitaxy (MBE) is investigated for various growth and diffraction conditions. The temporal behavior during the initial growth of a buffer layer is examined at a fixed diffraction condition. Intensity increase is observed during and after the initial stages of buffer layer growth and found to saturate after about 80 monolayer growth. Intensity oscillations are seen starting at different moments of initial growth, the earliest observed after only 14 monolayer growth. These results are used to guide and control GaAs(111)B growths with mirrorlike surface morphology.

  7. Atoms in static fields Chaos or Diffraction?

    CERN Document Server

    Dando, P A

    1998-01-01

    A brief review of the manifestations of classical chaos observed in atomic systems is presented. Particular attention is paid to the analysis of atomic spectra by periodic orbit-type theories. For diamagnetic non-hydrogenic Rydberg atoms, the dynamical explanation for observed spectral features has been disputed. By building on our previous work on the photoabsorption spectrum, we show how, by the addition of diffractive terms, the spectral fluctuations in the energy level spectrum of general Rydberg atoms can be obtained with remarkable precision from the Gutzwiller trace formula. This provides further evidence that non-hydrogenic systems are most naturally described in terms of diffraction rather than classical chaos.

  8. Atomic laser-beam finder.

    Science.gov (United States)

    Viering, Kirsten; Medellin, David; Mo, Jianyong; Raizen, Mark G

    2012-11-05

    We report on an experimental method to align a laser beam to a cloud of atoms trapped in a magneto-optical trap (MOT). We show how balanced lock-in detection leads to a very sensitive method to align the laser beam to the atoms in the plane perpendicular to the propagation direction. This provides a very reliable and fast way of aligning laser beams to atoms trapped in a MOT.

  9. Atom Lithography with a Chromium Atomic Beam

    Institute of Scientific and Technical Information of China (English)

    ZHANG Wen-Tao; LI Tong-Bao

    2006-01-01

    @@ Direct write atom lithography is a new technique in which resonant light is used to pattern an atomic beam and the nanostructures are formed when the atoms deposit on the substrate. We design an experiment setup to fabricate chromium nanolines by depositing an atomic beam of 52 Cr through an off-resonant laser standing wave with the wavelength of 425.55 nm onto a silicon substrate. The resulting nanolines exhibit a period of 215 ± 3 nm with height of 1 nm.

  10. Studies on coherence and decoherence in Fast Atom Diffraction

    Energy Technology Data Exchange (ETDEWEB)

    Seifert, J.; Lienemann, J. [Institut für Physik der Humboldt-Universität zu Berlin, Newtonstraße 15, D-12489 Berlin (Germany); Schüller, A. [Physikalisch-Technische Bundesanstalt (PTB), AG 6.21, Bundesallee 100, D-38116 Braunschweig (Germany); Winter, H., E-mail: winter@physik.hu-berlin.de [Institut für Physik der Humboldt-Universität zu Berlin, Newtonstraße 15, D-12489 Berlin (Germany)

    2015-05-01

    A few years ago, quantum effects were observed for the scattering of fast atoms from surfaces under a grazing angle of incidence. We discuss basic features of Fast Atom Diffraction (FAD) which adds a further powerful method to the established tools in ion beam analysis and surface science. Attractive features of FAD in studies on the structure of surfaces comprise negligible radiation damage, cost effective operation of the complete setup, no charging effects in studies with insulators, and an extreme sensitivity to the topmost layer of surface atoms. The observation of diffraction patterns is based on the quantum coherence which is preserved during the scattering process with the target surface. We will discuss basic features of the coherence phenomena and its role for the observation of quantum effects in the angular distributions for grazingly scattered atoms. In a comparison of data obtained for H and He atoms we demonstrate that two different mechanisms for decoherence are important.

  11. Flat hat glass diffractive optical beam shaper

    Science.gov (United States)

    Reichel, Steffen; Petzold, Uwe; Biertuempfel, Ralf; Vogt, Helge

    2009-02-01

    Many laser applications need a homogeneous - so called flat hat - light distribution in the application area. However, many laser emit Gaussian shaped light. The technology of diffractive optical elements (DOE) can be used to shape the Gaussian beam into a flat hat beam at a compact length. SCHOTT presents a DOE design of a flat hat DOE beam shaper made out of optical glass. Here the material glass has the significant advantage of high laser durability, low scattering losses, high resistance to temperature, moisture, and chemicals compared to polymer DOEs. Simulations and measurements on different DOEs for different wavelength, laser beam width, and laser divergence are presented. Surprisingly the flat hat DOE beam shaper depends only weakly on wavelength and beam width but strongly on laser divergence. Based on the good agreement between simulation and measurement an improved flat hat DOE beam shaper is also presented.

  12. When fast atom diffraction turns 3D

    Energy Technology Data Exchange (ETDEWEB)

    Zugarramurdi, Asier; Borisov, Andrei G., E-mail: andrei.borissov@u-psud.fr

    2013-12-15

    Fast atom diffraction at surfaces (FAD) in grazing incidence geometry is characterized by the slow motion in the direction perpendicular to the surface and fast motion parallel to the surface plane along a low index direction. It is established experimentally that for the typical surfaces the FAD reveals the 2D diffraction patterns associated with exchange of the reciprocal lattice vector perpendicular to the direction of fast motion. The reciprocal lattice vector exchange along the direction of fast motion is negligible. The usual approximation made in the description of the experimental data is then to assume that the effective potential leading to the diffraction results from the averaging of the 3D surface potential along the atomic strings forming the axial channel. In this work we use full quantum wave packet propagation calculations to study theoretically the possibility to observe the 3D diffraction in FAD experiments. We show that for the surfaces with large unit cell, such as can be the case for reconstructed or vicinal surfaces, the 3D diffraction can be observed. The reciprocal lattice vector exchange along the direction of fast motion leads to several Laue circles in the diffraction pattern.

  13. A multibeam atom laser: coherent atom beam splitting from a single far detuned laser

    OpenAIRE

    Dugué, J.; Dennis, G.; Jeppesen, M.; Johnsson, M. T.; Figl, C.; Robins, N. P.; Close, J. D.

    2007-01-01

    We report the experimental realisation of a multibeam atom laser. A single continuous atom laser is outcoupled from a Bose-Einstein condensate (BEC) via an optical Raman transition. The atom laser is subsequently split into up to five atomic beams with slightly different momenta, resulting in multiple, nearly co-propagating, coherent beams which could be of use in interferometric experiments. The splitting process itself is a novel realization of Bragg diffraction, driven by each of the optic...

  14. Image processing for grazing incidence fast atom diffraction

    Science.gov (United States)

    Debiossac, Maxime; Roncin, Philippe

    2016-09-01

    Grazing incidence fast atom diffraction (GIFAD, or FAD) has developed as a surface sensitive technique. Compared with thermal energies helium diffraction (TEAS or HAS), GIFAD is less sensitive to thermal decoherence but also more demanding in terms of surface coherence, the mean distance between defects. Such high quality surfaces can be obtained from freshly cleaved crystals or in a molecular beam epitaxy (MBE) chamber where a GIFAD setup has been installed allowing in situ operation. Based on recent publications by Atkinson et al. (2014) and Debiossac et al. (2014), the paper describes in detail the basic steps needed to measure the relative intensities of the diffraction spots. Care is taken to outline the underlying physical assumptions.

  15. Design and fabrication of diffractive atom chips for laser cooling and trapping

    CERN Document Server

    Cotter, J P; Griffin, P F; Rabey, I M; Docherty, K; Riis, E; Arnold, A S; Hinds, E A

    2016-01-01

    It has recently been shown that optical reflection gratings fabricated directly into an atom chip provide a simple and effective way to trap and cool substantial clouds of atoms [1,2]. In this article we describe how the gratings are designed and micro-fabricated and we characterise their optical properties, which determine their effectiveness as a cold atom source. We use simple scalar diffraction theory to understand how the morphology of the gratings determines the power in the diffracted beams.

  16. Optical generation of non-diffracting beams via photorefractive holography

    CERN Document Server

    Vieira, Tarcio A; Gesualdi, Marcos R R; Zamboni-Rached, Michel

    2015-01-01

    This work presents, for the first time the optical generation of non-diffracting beams via photorefractive holography. Optical generation of non-diffracting beams using conventional optics components is difficult and, in some instances, unfeasible, as it is wave fields given by superposition of non-diffracting beams. It is known that computer generated holograms and spatial light modulators (SLMs) successfully generate such beams. With photorefractive holography technique, the hologram of a non-diffracting beam is constructed (recorded) and reconstructed (reading) optically in a nonlinear photorefractive medium. The experimental realization of a non-diffracting beam was made in a photorefractive holography setup using a photorefractive Bi12SiO20 (BSO) crystal as the holographic recording medium, where the non-diffracting beams, the Bessel beam arrays and superposition of co-propagating Bessel beams (Frozen Waves) were obtained experimentally. The experimental results are in agreement with the theoretically pr...

  17. Femtosecond Electron Diffraction: Next generation electron sources for atomically resolved dynamics

    OpenAIRE

    Hirscht, Julian

    2015-01-01

    Three instruments for femtosecond electron diffraction (FED) experiments were erected, partially commissioned and used for first diffraction experiments. The Relativistic Electron Gun for Atomic Exploration (REGAE) was completed by beamline elements including supports, a specimen chamber and dark current or electron beam collimating elements such that the commissioning process, including first diffraction experiments in this context, could be started. The temporal resolution of this machine i...

  18. Improved accuracy in nano beam electron diffraction

    Energy Technology Data Exchange (ETDEWEB)

    Beche, A; Rouviere, J-L [CEA, INAC, SP2M, LEMMA, 17 rue des Martyrs, F-38054 Grenoble Cedex 9 (France); Clement, L, E-mail: armand.beche@cea.f, E-mail: jean-luc.rouviere@cea.f [ST Microelectronics, 850 rue Jean Monnet, F-38920 Crolles (France)

    2010-02-01

    Nano beam electron diffraction (NBD or NBED) is applied on a well controlled sample in order to evaluate the limit of the technique to measure strain. Measurements are realised on a 27nm thick Si{sub 0.7}Ge{sub 0.3} layer embedded in a silicon matrix, with a TITAN microscope working at 300kV. Using a standard condenser aperture of 50{mu}m, a probe size diameter of 2.7 nm is obtained and a strain accuracy of 6x10{sup -4} (mean root square, rms) is achieved. NBED patterns are acquired along a [110] direction and the bidimensionnal strain in the (110) plane is measured. Finite element simulations are carried out to check experimental results and reveal that strain relaxation and probe averaging in a 170nm thick TEM lamella reduces strain by 15%.

  19. Imaging an atomic beam using fluorescence

    Institute of Scientific and Technical Information of China (English)

    Ming He(何明); Jin Wang(王谨); Mingsheng Zhan(詹明生)

    2003-01-01

    A fluorescence detection scheme is applied to image an atomic beam. Using two laser diodes as the sources of detection light and pumping light respectively, the fluorescence image of the atomic beam is then observed by a commercial CCD-camera, which is corresponding to the atomic state and velocity distribution. The detection scheme has a great utilization in the experiments of cold atoms and atomic optics.

  20. Design and Analysis of Diffractive Axicons for Gaussian Beam Illumination

    Institute of Scientific and Technical Information of China (English)

    PU Jixiong; Shojiro Nemoto

    2001-01-01

    The diffractive axicon for the illumination with Gaussian beams is designed. The stationary phase method and the numerical calculation are used to analyze the diffraction integral describing the diffraction field. It is shown that with the Gaussian beam illumination of a smaller beam radius, the axicon can produces the uniform-axial-intensity with the lower oscillation frequency and the smaller oscillation amplitude. In addition, with the Gaussian beam illumination of a suitable beam radius, we can achieve the more uniform central-core width.

  1. Diffraction-free beams in fractional Schr\\"odinger equation

    CERN Document Server

    Zhang, Yiqi; Belić, Milivoj R; Ahmed, Noor; Zhang, Yanpeng; Xiao, Min

    2015-01-01

    We consider the propagation of one-dimensional and two-dimensional (1D, 2D) Gaussian beams in FSE without a potential, analytically and numerically. Without chirp, a 1D Gaussian beam splits into two nondiffracting Gaussian beams during propagation, while a 2D Gaussian beam undergoes conical diffraction. When a Gaussian beam carries linear chirp, the 1D beam deflects along the trajectories $z=\\pm2(x-x_0)$, which are independent of the chirp. In the case of 2D Gaussian beam, the propagation is also deflected, but the trajectories align along the diffraction cone $z=2r$ and the direction is determined by the chirp. Both 1D and 2D Gaussian beams are diffractionless and display uniform propagation. The nondiffracting property discovered in this model applies to other beams as well. Based on this nondiffracting and splitting property, we introduce the Talbot effect of diffractionless beams in FSE.

  2. Nonparaxial diffraction analysis of Airy and SAiry beams.

    Science.gov (United States)

    Carretero, Luis; Acebal, Pablo; Blaya, Salvador; García, Celia; Fimia, Antonio; Madrigal, Roque; Murciano, Angel

    2009-12-07

    We theoretically analyze Airy beams by solving the exact vectorial Helmholtz equation using boundary conditions at a diffraction aperture. As result, the diffracted beams are obtained in the whole space; thus, we demonstrate that the parabolic trajectories are larger than those previously reported, showing that the Airy beams start to form before the Fourier plane. We also demonstrate the possibility of using a new type of Airy beams (SAiry beams) with finite energy that can be generated at the focal plane of the lens due to diffraction by a circular aperture of a spherical wave modified by a cubic phase. The finite energy ensured by the principle of conservation of energy of a diffracted beam.

  3. Quantum reflection of helium atom beams from a microstructured grating

    OpenAIRE

    Zhao, Bum Suk; Schulz, Stephan A.; Meek, Samuel A.; Meijer, Gerard; Schöllkopf, Wieland

    2008-01-01

    We observe high-resolution diffraction patterns of a thermal-energy helium-atom beam reflected from a microstructured surface grating at grazing incidence. The grating consists of 10-$\\mu$m-wide Cr strips patterned on a quartz substrate and has a periodicity of 20 $\\mu$m. Fully-resolved diffraction peaks up to the $7^{\\rm th}$ order are observed at grazing angles up to 20 mrad. With changes in de Broglie wavelength or grazing angle the relative diffraction intensities show significant variati...

  4. Atomic resolution 3D electron diffraction microscopy

    Energy Technology Data Exchange (ETDEWEB)

    Miao, Jianwei; Ohsuna, Tetsu; Terasaki, Osamu; O' Keefe, Michael A.

    2002-03-01

    Electron lens aberration is the major barrier limiting the resolution of electron microscopy. Here we describe a novel form of electron microscopy to overcome electron lens aberration. By combining coherent electron diffraction with the oversampling phasing method, we show that the 3D structure of a 2 x 2 x 2 unit cell nano-crystal (framework of LTA [Al12Si12O48]8) can be ab initio determined at the resolution of 1 Angstrom from a series of simulated noisy diffraction pattern projections with rotation angles ranging from -70 degrees to +70 degrees in 5 degrees increments along a single rotation axis. This form of microscopy (which we call 3D electron diffraction microscopy) does not require any reference waves, and can image the 3D structure of nanocrystals, as well as non-crystalline biological and materials science samples, with the resolution limited only by the quality of sample diffraction.

  5. Extension of Friedel's law to Vortex Beam Diffraction

    CERN Document Server

    Juchtmans, Roeland; Verbeeck, Jo

    2016-01-01

    Friedel's law states that the modulus of the Fourier transform of real functions is centrosymmetric, while the phase is antisymmetric. As a consequence of this, elastic scattering of plane wave photons or electrons within the first-order Born-approximation as well as Fraunhofer diffraction on any aperture, is bound to result in centrosymmetric diffraction patterns. Friedel's law, however, does not apply for vortex beams, and centrosymmetry in general is not present in their diffraction patterns. In this work we extend Friedel's law for vortex beams by showing that the diffraction patterns of vortex beams with opposite topological charge, scattered on the same two dimensional potential, always are centrosymmetric to one another, regardless of the symmetry of the scattering object. We verify our statement by means of numerical simulations and experimental data. Our research provides deeper understanding in vortex beam diffraction and can be used to design new experiments to measure the topological charge of vor...

  6. A cold 87Rb atomic beam

    Institute of Scientific and Technical Information of China (English)

    Wang Xiao-Jia; Feng Yan-Ying; Xue Hong-Bo; Zhou Zhao-Ying; Zhang Wen-Dong

    2011-01-01

    We demonstrate an experimental setup for the production of a beam source of cold 87Rb atoms.The atoms are extracted from a trapped cold atomic cloud in an unbalanced three-dimensional magneto-optical trap.Via a radiation pressure difference generated by a specially designed leak tunnel along one trapping laser beam,the atoms are pushed out continuously with low velocities and a high flux.The most-probable velocity in the beam is varied from 9 m/s to 19 m/s by varying the detuning of the trapping laser beams in the magneto-optical trap and the flux can be tuned up to 4× 109 s-1 by increasing the intensity of the trapping beams.We also present a simple model for describing the dependence of the beam performance on the magneto-optical trap trapping laser intensity and the detuning.

  7. Atoms in parallel fields: Analysis with diffractive periodic orbits

    Science.gov (United States)

    Owen, S. M.; Monteiro, T. S.; Dando, P. A.

    2000-11-01

    We show that fluctuations in the density of states of nonhydrogenic atoms in parallel fields are strongly influenced by diffractive periodic orbits. Unlike typical systems with a diffractive point scatterer, the atomic core of small atoms like lithium and helium is best understood as a combined geometric and diffractive scatterer. Each Gutzwiller (geometric) periodic orbit is paired with a diffractive orbit of the same action. We investigate, particularly, amplitudes for contributions from repetitions, and multiple scattering orbits. We find that periodic orbit repetitions are described by ``hybrid'' orbits, combining both diffractive and geometric core scatters, and that by including all possible permutations we can obtain excellent agreement between the semiclassical model and accurate fully quantal calculations. For high repetitions, we find even one-scatter diffractive contributions become of the same order as those of the geometric periodic orbit for repetition numbers n~ħ-1/2. Although the contribution of individual diffractive orbits is suppressed by O(ħ1/2) relative to the geometric periodic orbits, the proliferation of diffractive orbits with increasing period means that the diffractive effect for the atom can persist in the ħ-->0 limit.

  8. Novel Atomic Mirror with a Blue-Detuned Semi-Gaussian Beam

    Institute of Scientific and Technical Information of China (English)

    郑萍; 高伟建; 印建平

    2003-01-01

    A novel and simple atomic mirror composed of a blue-detuned semi-Gaussian beam is proposed. From the Fresnel diffraction theory, the intensity distributions of a collimated GaUssian laser beam diffracted by the straight edge of a semi-infinite opaque plate are studied. The optical potential of the semi-Gaussian beam for 85 Rb atoms and its spontaneous emission probability are calculated and compared with the performance of the evanescent-wave mirror. Our study shows that the blue-detuned semi-Gaussian beam, as a novel atomic mirror, can be used to reflect atomic beam efliciently, and under the same beam parameters and lower normal atomic velocity, the performance of the semi-Gaussian-beam mirror is better than that of the evanescent-wave mirror.

  9. Manipulation and analysis of atomic and molecular beams using transmission gratings and Fresnel zone plates

    Energy Technology Data Exchange (ETDEWEB)

    Grisenti, R.E.

    2000-06-01

    In this thesis experimental results on the diffraction of rare gas atoms (He, Ne, Ar, Kr) and molecular (D{sub 2}) beams by a 100 nm period transmission grating and on the focusing of a helium atom beam through a Fresnel zone plate have been reported. (orig.)

  10. Atomic scattering from an adsorbed monolayer solid with a helium beam that penetrates to the substrate

    DEFF Research Database (Denmark)

    Hansen, Flemming Yssing; Bruch, L.W.; Dammann, Bernd

    2013-01-01

    Diffraction and one-phonon inelastic scattering of a thermal energy helium atomic beam are evaluated in the situation that the target monolayer lattice is so dilated that the atomic beam penetrates to the interlayer region between the monolayer and the substrate. The scattering is simulated...

  11. Tailoring non-diffractive beams from amorphous light speckles

    Science.gov (United States)

    Di Battista, D.; Ancora, D.; Leonetti, M.; Zacharakis, G.

    2016-09-01

    Bessel beams are non-diffracting light structures, which maintain their spatial features after meters of propagation and are realized with simple optical elements such as axicon lenses, spatial filters, and lasers. In this paper, we demonstrate a method for generating non diffractive Bessel-like beams through a heavily scattering system, exploiting wavefronts shaped by a spatial light modulator. With the proposed method starting from amorphous speckle patterns, it is possible to produce at user defined positions configurable and non-diffracting light distributions which can improve depth-of-field in speckled illumination microscopy.

  12. Quantum reflection of helium atom beams from a microstructured grating

    Science.gov (United States)

    Zhao, Bum Suk; Schulz, Stephan A.; Meek, Samuel A.; Meijer, Gerard; Schöllkopf, Wieland

    2008-07-01

    We observe high-resolution diffraction patterns of a thermal-energy helium atom beam reflected from a microstructured surface grating at grazing incidence. The grating consists of 10-μm -wide Cr strips patterned on a quartz substrate and has a periodicity of 20μm . Fully resolved diffraction peaks up to the seventh order are observed at grazing angles up to 20mrad . With changes in de Broglie wavelength or grazing angle the relative diffraction intensities show significant variations which shed light on the nature of the atom-surface interaction potential. The observations are explained in terms of quantum reflection at the long-range attractive Casimir-van der Waals potential.

  13. Quantum reflection of helium atom beams from a microstructured grating

    CERN Document Server

    Zhao, Bum Suk; Meek, Samuel A; Meijer, Gerard; Schöllkopf, Wieland

    2008-01-01

    We observe high-resolution diffraction patterns of a thermal-energy helium-atom beam reflected from a microstructured surface grating at grazing incidence. The grating consists of 10-$\\mu$m-wide Cr strips patterned on a quartz substrate and has a periodicity of 20 $\\mu$m. Fully-resolved diffraction peaks up to the $7^{\\rm th}$ order are observed at grazing angles up to 20 mrad. With changes in de Broglie wavelength or grazing angle the relative diffraction intensities show significant variations which shed light on the nature of the atom-surface interaction potential. The observations are explained in terms of quantum reflection at the long-range attractive Casimir-van der Waals potential.

  14. Suppressing Ghost Diffraction in E-Beam-Written Gratings

    Science.gov (United States)

    Wilson, Daniel; Backlund, Johan

    2009-01-01

    A modified scheme for electron-beam (E-beam) writing used in the fabrication of convex or concave diffraction gratings makes it possible to suppress the ghost diffraction heretofore exhibited by such gratings. Ghost diffraction is a spurious component of diffraction caused by a spurious component of grating periodicity as described below. The ghost diffraction orders appear between the main diffraction orders and are typically more intense than is the diffuse scattering from the grating. At such high intensity, ghost diffraction is the dominant source of degradation of grating performance. The pattern of a convex or concave grating is established by electron-beam writing in a resist material coating a substrate that has the desired convex or concave shape. Unfortunately, as a result of the characteristics of electrostatic deflectors used to control the electron beam, it is possible to expose only a small field - typically between 0.5 and 1.0 mm wide - at a given fixed position of the electron gun relative to the substrate. To make a grating larger than the field size, it is necessary to move the substrate to make it possible to write fields centered at different positions, so that the larger area is synthesized by "stitching" the exposed fields.

  15. Diffraction control of subwavelength structured light beams in Kapitza media.

    Science.gov (United States)

    Huang, Changming; Ye, Fangwei; Chen, Xianfeng

    2015-05-18

    Kapitza tandem structures, consisting of thin alternating layers with opposite signs of the dielectric permittivity, have been recently predicted to afford diffraction arrest of focused microwave radiation [Phys. Rev. Lett. 110, 143901 (2013)]. Here we study the applicability of the Kapitza effect to control the propagation of structured subwavelength light beams. We show that a sufficiently deep modulation of the dielectric permittivity allows a nearly complete diffraction cancellation of multiple-peak subwavelength beams, and we study how the degree of diffraction cancellation decreases as the spatial spectrum of the input beam broadens. We also find that subwavelength light beams can be steered by varying the depth of the permittivity modulation. In particular, a sufficiently large permittivity modulation is shown to cause otherwise titled inputs to propagate always along the direction of modulation.

  16. Phase effects due to beam misalignment on diffraction gratings

    CERN Document Server

    Lodhia, Deepali; Brueckner, Frank; Carbone, Ludovico; Fulda, Paul; Kokeyama, Keiko; Freise, Andreas

    2013-01-01

    All-reflective interferometer configurations have been proposed for the next generation of gravitational wave detectors, with diffractive elements replacing transmissive optics. However, an additional phase noise creates more stringent conditions for alignment stability. A framework for alignment stability with the use of diffractive elements was required using a Gaussian model. We successfully create such a framework involving modal decomposition to replicate small displacements of the beam (or grating) and show that the modal model does not contain the phase changes seen in an otherwise geometric planewave approach. The modal decomposition description is justified by verifying experimentally that the phase of a diffracted Gaussian beam is independent of the beam shape, achieved by comparing the phase change between a zero-order and first-order mode beam. To interpret our findings we employ a rigorous time-domain simulation to demonstrate that the phase changes resulting from a modal decomposition are correc...

  17. Diffraction grating characterisation for cold-atom experiments

    CERN Document Server

    McGilligan, James P; Riis, Erling; Arnold, Aidan S

    2016-01-01

    We have studied the optical properties of gratings micro-fabricated into semiconductor wafers, which can be used for simplifying cold-atom experiments. The study entailed characterisation of diffraction efficiency as a function of coating, periodicity, duty cycle and geometry using over 100 distinct gratings. The critical parameters of experimental use, such as diffraction angle and wavelength are also discussed, with an outlook to achieving optimal ultracold experimental conditions.

  18. Polar POLICRYPS diffractive structures generate cylindrical vector beams

    Energy Technology Data Exchange (ETDEWEB)

    Alj, Domenico; Caputo, Roberto, E-mail: roberto.caputo@fis.unical.it; Umeton, Cesare [Department of Physics and CNR-NANOTEC University of Calabria, I-87036 Rende (CS) (Italy); Paladugu, Sathyanarayana [Soft Matter Lab, Department of Physics, Bilkent University, Ankara 06800 (Turkey); Volpe, Giovanni [Soft Matter Lab, Department of Physics, Bilkent University, Ankara 06800 (Turkey); UNAM-National Nanotechnology Research Center, Bilkent University, Ankara 06800 (Turkey)

    2015-11-16

    Local shaping of the polarization state of a light beam is appealing for a number of applications. This can be achieved by employing devices containing birefringent materials. In this article, we present one such enables converting a uniformly circularly polarized beam into a cylindrical vector beam (CVB). This device has been fabricated by exploiting the POLICRYPS (POlymer-LIquid CRYstals-Polymer-Slices) photocuring technique. It is a liquid-crystal-based optical diffraction grating featuring polar symmetry of the director alignment. We have characterized the resulting CVB profile and polarization for the cases of left and right circularly polarized incoming beams.

  19. Relativistic atomic beam spectroscopy II

    Energy Technology Data Exchange (ETDEWEB)

    NONE

    1991-12-31

    We are requesting support for a postdoctoral person to participate in H{sup -} studies at Los Alamos. In addition, we are requesting funding for a state-of-the-art YAG laser system that would allow us to obtain data at three times our present rate with improved beam quality.

  20. Gaussian beam diffraction in weakly anisotropic inhomogeneous media

    Energy Technology Data Exchange (ETDEWEB)

    Kravtsov, Yu.A., E-mail: kravtsov@am.szczecin.p [Institute of Physics, Maritime University of Szczecin, Szczecin 70-500 (Poland); Space Research Institute, Russian Academy of Science, Moscow 117 997 (Russian Federation); Berczynski, P., E-mail: pawel.berczynski@ps.p [Institute of Physics, West Pomeranian University of Technology, Szczecin 70-310 (Poland); Bieg, B., E-mail: b.bieg@am.szczecin.p [Institute of Physics, Maritime University of Szczecin, Szczecin 70-500 (Poland)

    2009-08-10

    Combination of quasi-isotropic approximation (QIA) of geometric optics with paraxial complex geometric optics (PCGO) is suggested, which allows describing both diffraction and polarization evolution of Gaussian electromagnetic beams in weakly anisotropic inhomogeneous media. Combination QIA/PCGO reduces Maxwell equations to the system of the ordinary differential equations of the first order and radically simplifies solution of various problems, related to microwave plasma diagnostics, including plasma polarimetry, interferometry and refractometry in thermonuclear reactors. Efficiency of the method is demonstrated by the example of electromagnetic beam diffraction in a linear layer of magnetized plasma with parameters, modeling tokamak plasma in the project ITER.

  1. Non-diffracting speckles of a perfect vortex beam

    Science.gov (United States)

    Gangi Reddy, Salla; P, Chithrabhanu; Vaity, Pravin; Aadhi, A.; Prabhakar, Shashi; Singh, R. P.

    2016-05-01

    We generate perfect optical vortex (POV) beams, whose intensity distribution is independent of the order, and scatter them through a rough surface. We show that the size of produced speckles is independent of the order of the POV and their Fourier transform gives the random non-diffracting fields. The invariant size of speckles over the free space propagation verifies their non-diffracting or non-diverging nature. The size of speckles can be easily controlled by changing the axicon parameter, used to generate the Bessel-Gauss beams whose Fourier transform provides the POV. These results may be useful in applications of POV for authentication in cryptography.

  2. Diffractive beam parameters of LP01 mode of fiber

    Institute of Scientific and Technical Information of China (English)

    Lianhuang Li; Fuyuan Guo

    2009-01-01

    The diffractive beam parameters of LP01 mode of fiber are analyzed in detail. Based on solving linear equations, two formulas for two kinds of mode-field radii as functions of normalized frequency are presented, and relations between angular radius of far-field divergence, beam propagation factor, and normalized frequency are given. Numerical calculation indicates that the maximal relative error is smaller than 1% within a reasonable parameter range.

  3. Demodulation for multi vortex beams based on composite diffraction hologram

    Science.gov (United States)

    Zhang, Weibin; Li, Yingchun; Sun, Tengfen; Shao, Wei; Zhu, Fuquan; Wang, YingYing

    2016-12-01

    While projecting a Gaussian beam onto the spatial light modulator (SLM) which has loaded a composite hologram, several vortex beams can be generated at one time. On the contrary, while projecting the corresponding vortex beam onto the hologram, the Gaussian beam can be restored, realizing the demodulation of vortex beam. In traditional optical communication systems, a hologram can only demodulate one incident vortex beam. In this paper, a vortex beam demodulation method based on composite diffraction hologram is proposed, which can demodulate several incident vortex beams with only one hologram. An experimental system is set up in this paper which achieves the generation, transmission and demodulation experiments of vortex beams with 64QAM-OFDM signals. After a series of offline processing on the demodulated Gaussian beam, constellation and bit error rates (BER) of each subcarrier for OFDM signals are acquired. The experimental results show that good system performance can be achieved with this method as the BERs of all subcarriers are under the FEC threshold.

  4. Higher-order harmonics of general limited diffraction Bessel beams

    Science.gov (United States)

    Ding, De-Sheng; Huang, Jin-Huang

    2016-12-01

    In this paper, we extensively study the higher-order harmonic generation of the general limited diffraction m-th-order Bessel beam. The analysis is based on successive approximations of the Khokhlov-Zabolotskaya-Kuznetsov (KZK) equation. Asymptotic expansions are presented for higher-order harmonic Bessel beams in near and far fields. The validity of asymptotic approximation is also analyzed. The higher-order harmonic of the Bessel beam with the lowest zero-order is taken as a special example. Project supported by the National Natural Science Foundation of China (Grant Nos. 11074038 and 11374051).

  5. Controlling the Multiport Nature of Bragg Diffraction in Atom Interferometry

    CERN Document Server

    Parker, Richard H; Estey, Brian; Zhong, Weicheng; Huang, Eric; Müller, Holger

    2016-01-01

    Bragg diffraction has been used in atom interferometers because it allows signal enhancement through multiphoton momentum transfer and suppression of systematics by not changing the internal state of atoms. Its multi-port nature, however, can lead to parasitic interferometers, allows for intensity-dependent phase shifts in the primary interferometers, and distorts the ellipses used for phase extraction. We study and suppress these unwanted effects. Specifically, phase extraction by ellipse fitting and the resulting systematic phase shifts are calculated by Monte Carlo simulations. Phase shifts arising from the thermal motion of the atoms are controlled by spatial selection of atoms and an appropriate choice of Bragg intensity. In these simulations, we found that Gaussian Bragg pulse shapes yield the smallest systematic shifts. Parasitic interferometers are suppressed by a "magic" Bragg pulse duration. The sensitivity of the apparatus was improved by the addition of AC Stark shift compensation, which permits d...

  6. Femtosecond electron diffraction: heralding the era of atomically resolved dynamics

    Science.gov (United States)

    Sciaini, Germán; Miller, R. J. Dwayne

    2011-09-01

    One of the great dream experiments in Science is to directly observe atomic motions as they occur. Femtosecond electron diffraction provided the first 'light' of sufficient intensity to achieve this goal by attaining atomic resolution to structural changes on the relevant timescales. This review covers the technical progress that made this new level of acuity possible and gives a survey of the new insights gained from an atomic level perspective of structural dynamics. Atomic level views of the simplest possible structural transition, melting, are discussed for a number of systems in which both thermal and purely electronically driven atomic displacements can be correlated with the degree of directional bonding. Optical manipulation of charge distributions and effects on interatomic forces/bonding can be directly observed through the ensuing atomic motions. New phenomena involving strongly correlated electron-lattice systems are also discussed in which optically induced changes in the potential energy landscape lead to ballistic structural changes. Concepts such as the structural order parameters are now directly observable at the atomic level of inspection to give a remarkable view of the extraordinary degree of cooperativity involved in strongly correlated electron-lattice systems. These recent examples, in combination with time-resolved real space imaging now possible with electron probes, are truly defining an emerging field that holds great promise to make a significant impact in how we understand structural dynamics. This article is dedicated to the memory of Professor David John Hugh Cockayne, a world leader in electron microscopy, who sadly passed away in December.

  7. Low-kilovolt coherent electron diffractive imaging instrument based on a single-atom electron source

    Energy Technology Data Exchange (ETDEWEB)

    Lin, Chun-Yueh [Department of Physics, National Taiwan University, Taipei 10617, Taiwan (China); Chang, Wei-Tse; Chen, Yi-Sheng; Hwu, En-Te; Chang, Chia-Seng; Hwang, Ing-Shouh, E-mail: ishwang@phys.sinica.edu.tw [Institute of Physics, Academia Sinica, Nankang, Taipei 11529, Taiwan (China); Hsu, Wei-Hao [Department of Materials Science and Engineering, National Tsing Hua University, Hsinchu 30013, Taiwan (China)

    2016-03-15

    In this work, a transmission-type, low-kilovolt coherent electron diffractive imaging instrument was constructed. It comprised a single-atom field emitter, a triple-element electrostatic lens, a sample holder, and a retractable delay line detector to record the diffraction patterns at different positions behind the sample. It was designed to image materials thinner than 3 nm. The authors analyzed the asymmetric triple-element electrostatic lens for focusing the electron beams and achieved a focused beam spot of 87 nm on the sample plane at the electron energy of 2 kV. High-angle coherent diffraction patterns of a suspended graphene sample corresponding to (0.62 Å){sup −1} were recorded. This work demonstrated the potential of coherent diffractive imaging of thin two-dimensional materials, biological molecules, and nano-objects at a voltage between 1 and 10 kV. The ultimate goal of this instrument is to achieve atomic resolution of these materials with high contrast and little radiation damage.

  8. Amplitude and phase characterization by diffracted beam interferometry: blind dbi

    Energy Technology Data Exchange (ETDEWEB)

    Lopez Lago, E; Gonzalez Nunez, H; De la Fuente, R, E-mail: elena.lopez.lago@usc.es [Departamento de Fisica Aplicada, Escuela Universitaria de Optica y Optometria, Campus Vida, Universidade of Santiago de Compostela, E-15782 Santiago de Compostela, Galicia (Spain)

    2011-01-01

    Diffracted beam interferometry is a self referenced method characterization technique whose operation principle is based on the reconstruction of the phase of a beam starting from the interference data between the beam and its diffracted copy. The phase is recovered indirectly by means of an iterative algorithm that relates the irradiances of the interfering beams and its phase difference. The first experimental demonstration of DBI was implemented on a Mach-Zehnder interferometer which incorporated an afocal imaging system in each arm, in order to form an image of a common object in different planes at the output of the interferometer. The irradiance data as well as the phase difference data were picked up from one of the image planes and they were introduced in the iterative algorithm. In this work we discuss a modification of the algorithm that allows to reconstruct simultaneously the amplitude and phase of the wavefront starting from, exclusively, the phase difference between the two waves that interfere in one of the image planes. This new algorithm improves the reconstruction process because the data acquisition process is faster and consequently the method is less influenced by environment disturbances. The method has been applied successfully to the characterization of phase plates and laser beams as well as to the local characterization of ophthalmic lenses.

  9. On the Angular Width of Diffractive Beam in Anisotropic Media

    CERN Document Server

    Lock, Edwin H

    2011-01-01

    2-D diffraction patterns arising in the far-field region were investigated theoretically for the case, when the plane wave with non collinear group and phase velocities is incident on the wide slit in opaque screen with arbitrary orientation. This investigation was carried out by consideration as an example of magnetostatic surface wave diffraction in tangentially magnetized ferrite slab. It was deduced the universal analytical formula, which one can use to calculate the angular width of diffractive beam in any 2-D anisotropic geometries for the waves of various nature. It was shown, that in 2-D anisotropic geometries this width may be not only more or less then the value L/D (L - wavelength of incident wave, D - length of slit), but it also may be equal to zero in certain conditions.

  10. Many-beam dynamical simulation of electron backscatter diffraction patterns

    Energy Technology Data Exchange (ETDEWEB)

    Winkelmann, Aimo [Max-Planck-Institut fuer Mikrostrukturphysik, Weinberg 2, D-06120 Halle (Germany)], E-mail: winkelm@mpi-halle.mpg.de; Trager-Cowan, Carol; Sweeney, Francis [Department of Physics, University of Strathclyde, Glasgow G4 ONG, Scotland (United Kingdom); Day, Austin P. [Aunt Daisy Scientific Ltd., Dixton Rd., Monmouth, Gwent, NP25 3PP (United Kingdom); Parbrook, Peter [EPSRC National Centre for III-V Technologies, University of Sheffield (United Kingdom)

    2007-04-15

    We present an approach for the simulation of complete electron backscatter diffraction (EBSD) patterns where the relative intensity distributions in the patterns are accurately reproduced. The Bloch wave theory is applied to describe the electron diffraction process. For the simulation of experimental patterns with a large field of view, a large number of reflecting planes has to be taken into account. This is made possible by the Bethe perturbation of weak reflections. Very good agreement is obtained for simulated and experimental patterns of gallium nitride GaN{l_brace}0001{r_brace} at 20 kV electron energy. Experimental features like zone-axis fine structure and higher-order Laue zone rings are accurately reproduced. We discuss the influence of the diffraction of the incident beam in our experiment.

  11. Optimization of a constrained linear monochromator design for neutral atom beams.

    Science.gov (United States)

    Kaltenbacher, Thomas

    2016-04-01

    A focused ground state, neutral atom beam, exploiting its de Broglie wavelength by means of atom optics, is used for neutral atom microscopy imaging. Employing Fresnel zone plates as a lens for these beams is a well established microscopy technique. To date, even for favorable beam source conditions a minimal focus spot size of slightly below 1μm was reached. This limitation is essentially given by the intrinsic spectral purity of the beam in combination with the chromatic aberration of the diffraction based zone plate. Therefore, it is important to enhance the monochromaticity of the beam, enabling a higher spatial resolution, preferably below 100nm. We propose to increase the monochromaticity of a neutral atom beam by means of a so-called linear monochromator set-up - a Fresnel zone plate in combination with a pinhole aperture - in order to gain more than one order of magnitude in spatial resolution. This configuration is known in X-ray microscopy and has proven to be useful, but has not been applied to neutral atom beams. The main result of this work is optimal design parameters based on models for this linear monochromator set-up followed by a second zone plate for focusing. The optimization was performed for minimizing the focal spot size and maximizing the centre line intensity at the detector position for an atom beam simultaneously. The results presented in this work are for, but not limited to, a neutral helium atom beam.

  12. Small angle scatter imaging from wide beam diffraction patterns

    Energy Technology Data Exchange (ETDEWEB)

    Wilkinson, Steven J [Department of Materials and Medical Sciences, Cranfield University, Shrivenham, Swindon, Wiltshire SN6 8LA (United Kingdom); Rogers, Keith D [Department of Materials and Medical Sciences, Cranfield University, Shrivenham, Swindon, Wiltshire SN6 8LA (United Kingdom); Hall, Chris J [School of Physics, Monash University, Victoria 3800 (Australia); Round, Adam R [EMBL c/o DESY, Building 25a, Notkestrasse 85, 22603 Hamburg (Germany)

    2007-05-07

    In this paper we report on the extension of the technique of mapping small angle x-ray scatter (SAXS) across a soft material specimen several millimetres square. In the conventional SAXS mapping technique a pencil beam of x-rays is raster scanned over the specimen with the scatter pattern recorded from each point in the raster. In our technique a wide, parallel beam is used, speeding up the data collection time considerably. An image processing algorithm is used to separate the scatter pattern features from individual points along the line of the beam. To test the efficacy of the technique a phantom was constructed using gelatin and rat tail tendon collagen. Collagen fibres in the phantom were arranged in quarters horizontally, diagonally and vertically leaving one quarter with just gelatin. The phantom was used to collect both raster scanned sets of SAXS patterns spaced at 0.25 mm horizontally and vertically and also a wide beam data set. The width of the beam in this case was approximately 7 mm. Using the third-order diffraction of rat tail tendon intensity data were gathered from each SAXS pattern and used to construct a map. Data from the raster scan image and that from the wide beam are compared. Finally using a phantom made from dehydrated rat tail tendon and paraffin wax a tomographic slice constructed using data from SAXS patterns is shown.

  13. Correlating Atom Probe Crystallographic Measurements with Transmission Kikuchi Diffraction Data.

    Science.gov (United States)

    Breen, Andrew J; Babinsky, Katharina; Day, Alec C; Eder, K; Oakman, Connor J; Trimby, Patrick W; Primig, Sophie; Cairney, Julie M; Ringer, Simon P

    2017-03-14

    Correlative microscopy approaches offer synergistic solutions to many research problems. One such combination, that has been studied in limited detail, is the use of atom probe tomography (APT) and transmission Kikuchi diffraction (TKD) on the same tip specimen. By combining these two powerful microscopy techniques, the microstructure of important engineering alloys can be studied in greater detail. For the first time, the accuracy of crystallographic measurements made using APT will be independently verified using TKD. Experimental data from two atom probe tips, one a nanocrystalline Al-0.5Ag alloy specimen collected on a straight flight-path atom probe and the other a high purity Mo specimen collected on a reflectron-fitted instrument, will be compared. We find that the average minimum misorientation angle, calculated from calibrated atom probe reconstructions with two different pole combinations, deviate 0.7° and 1.4°, respectively, from the TKD results. The type of atom probe and experimental conditions appear to have some impact on this accuracy and the reconstruction and measurement procedures are likely to contribute further to degradation in angular resolution. The challenges and implications of this correlative approach will also be discussed.

  14. Wavefront aberrations of x-ray dynamical diffraction beams.

    Science.gov (United States)

    Liao, Keliang; Hong, Youli; Sheng, Weifan

    2014-10-01

    The effects of dynamical diffraction in x-ray diffractive optics with large numerical aperture render the wavefront aberrations difficult to describe using the aberration polynomials, yet knowledge of them plays an important role in a vast variety of scientific problems ranging from optical testing to adaptive optics. Although the diffraction theory of optical aberrations was established decades ago, its application in the area of x-ray dynamical diffraction theory (DDT) is still lacking. Here, we conduct a theoretical study on the aberration properties of x-ray dynamical diffraction beams. By treating the modulus of the complex envelope as the amplitude weight function in the orthogonalization procedure, we generalize the nonrecursive matrix method for the determination of orthonormal aberration polynomials, wherein Zernike DDT and Legendre DDT polynomials are proposed. As an example, we investigate the aberration evolution inside a tilted multilayer Laue lens. The corresponding Legendre DDT polynomials are obtained numerically, which represent balanced aberrations yielding minimum variance of the classical aberrations of an anamorphic optical system. The balancing of classical aberrations and their standard deviations are discussed. We also present the Strehl ratio of the primary and secondary balanced aberrations.

  15. High sensitivity, low-systematics atom interferometers using Bragg diffraction and Bloch oscillations

    CERN Document Server

    Estey, Brian; Müller, Holger; Kuan, Pei-Chen; Lan, Shau-Yu

    2014-01-01

    We describe a new scheme for atom interferometry based on both large-momentum transfer Bragg beam splitters and Bloch oscillations. Combining the advantages of previous approaches to recoil-sensitive interferometers, we increase the signal and suppress a systematic phase shift caused by Bragg diffraction at least 60-fold, matching experiment to theory; the systematic shift can be eliminated from Mach-Zehnder interferometers. We demonstrate high contrast, interference with up to 4.4 million radians of phase difference between freely evolving matter waves, and a resolution of $\\delta \\alpha/\\alpha=0.33\\,$ppb$\\sqrt{\\rm 6h}$ available to measurements of the fine structure constant.

  16. Universal diffraction of atoms and molecules from a quantum reflection grating.

    Science.gov (United States)

    Zhao, Bum Suk; Zhang, Weiqing; Schöllkopf, Wieland

    2016-03-01

    Since de Broglie's work on the wave nature of particles, various optical phenomena have been observed with matter waves of atoms and molecules. However, the analogy between classical and atom/molecule optics is not exact because of different dispersion relations. In addition, according to de Broglie's formula, different combinations of particle mass and velocity can give the same de Broglie wavelength. As a result, even for identical wavelengths, different molecular properties such as electric polarizabilities, Casimir-Polder forces, and dissociation energies modify (and potentially suppress) the resulting matter-wave optical phenomena such as diffraction intensities or interference effects. We report on the universal behavior observed in matter-wave diffraction of He atoms and He2 and D2 molecules from a ruled grating. Clear evidence for emerging beam resonances is observed in the diffraction patterns, which are quantitatively the same for all three particles and only depend on the de Broglie wavelength. A model, combining secondary scattering and quantum reflection, permits us to trace the observed universal behavior back to the peculiar principles of quantum reflection.

  17. Fully vectorial accelerating diffraction-free Helmholtz beams.

    Science.gov (United States)

    Aleahmad, Parinaz; Miri, Mohammad-Ali; Mills, Matthew S; Kaminer, Ido; Segev, Mordechai; Christodoulides, Demetrios N

    2012-11-16

    We show that new families of diffraction-free nonparaxial accelerating optical beams can be generated by considering the symmetries of the underlying vectorial Helmholtz equation. Both two-dimensional transverse electric and magnetic accelerating wave fronts are possible, capable of moving along elliptic trajectories. Experimental results corroborate these predictions when these waves are launched from either the major or minor axis of the ellipse. In addition, three-dimensional spherical nondiffracting field configurations are presented along with their evolution dynamics. Finally, fully vectorial self-similar accelerating optical wave solutions are obtained via oblate-prolate spheroidal wave functions. In all occasions, these effects are illustrated via pertinent examples.

  18. Fast character projection electron beam lithography for diffractive optical elements

    Science.gov (United States)

    Harzendorf, Torsten; Fuchs, Frank; Banasch, Michael; Zeitner, Uwe D.

    2014-05-01

    Electron beam lithography becomes attractive also for the fabrication of large scale diffractive optical elements by the use of the character projection (CP) technique. Even in the comparable fast variable shaped beam (VSB) exposure approach for conventional electron beam writers optical nanostructures may require very long writing times exceeding 24 hours per wafer because of the high density of features, as required by e.g. sub-wavelength nanostructures. Using character projection, the writing time can be reduced by more than one order of magnitude, due to the simultaneous exposure of multiple features. The benefit of character projection increases with increasing complexity of the features and decreasing period. In this contribution we demonstrate the CP technique for a grating of hexagonal symmetry at 350nm period. The pattern is designed to provide antireflective (AR) properties, which can be adapted in their spectral and angular domain for applications from VIS to NIR by changing the feature size and the etching depth of the nanostructure. This AR nanostructure can be used on the backside of optical elements e.g. gratings, when an AR coating stack could not be applied for the reason of climatic conditions or wave front accuracy.

  19. Energy-filtered electron-diffracted beam holography

    Energy Technology Data Exchange (ETDEWEB)

    Herring, R.A. [Center for Advanced Materials and Related Technology, Department of Mechanical Engineering, University of Victoria, P.O. Box. 3055, STN CSC, Victoria, BC, V8N 4T6 (Canada)]. E-mail: rherring@uvic.ca

    2005-10-15

    A method of energy-filtered electron holography is described where any two electron-diffracted beams can be interfered using an electron biprism. A Gatan image filter is used to select the energy loss of the electrons produced in the holograms. Gallium arsenide is used as the TEM specimen. This method of microscopy confirms that fringes extending beyond a limiting aperture were due to inelastically scattered electrons and specifically electrons scattered from the bulk plasmon. The degree of coherence of the zero-loss and energy-loss electrons were high and measured to be {approx}0.3, which was maintained even for the high energy-loss electrons up to 100 eV. Future systematic studies using this method should help understand the Stobbs factor and contribute to the development of quantitative high-resolution electron microscopy.

  20. Energy-filtered electron-diffracted beam holography.

    Science.gov (United States)

    Herring, R A

    2005-10-01

    A method of energy-filtered electron holography is described where any two electron-diffracted beams can be interfered using an electron biprism. A Gatan image filter is used to select the energy loss of the electrons produced in the holograms. Gallium arsenide is used as the TEM specimen. This method of microscopy confirms that fringes extending beyond a limiting aperture were due to inelastically scattered electrons and specifically electrons scattered from the bulk plasmon. The degree of coherence of the zero-loss and energy-loss electrons were high and measured to be approximately 0.3, which was maintained even for the high energy-loss electrons up to 100 eV. Future systematic studies using this method should help understand the Stobbs factor and contribute to the development of quantitative high-resolution electron microscopy.

  1. Dual-Beam Atom Laser Driven by Spinor Dynamics

    Science.gov (United States)

    Thompson, Robert; Lundblad, Nathan; Maleki, Lute; Aveline, David

    2007-01-01

    An atom laser now undergoing development simultaneously generates two pulsed beams of correlated Rb-87 atoms. (An atom laser is a source of atoms in beams characterized by coherent matter waves, analogous to a conventional laser, which is a source of coherent light waves.) The pumping mechanism of this atom laser is based on spinor dynamics in a Bose-Einstein condensate. By virtue of the angular-momentum conserving collisions that generate the two beams, the number of atoms in one beam is correlated with the number of atoms in the other beam. Such correlations are intimately linked to entanglement and squeezing in atomic ensembles, and atom lasers like this one could be used in exploring related aspects of Bose-Einstein condensates, and as components of future sensors relying on atom interferometry. In this atom-laser apparatus, a Bose-Einstein condensate of about 2 x 10(exp 6) Rb-87 atoms at a temperature of about 120 micro-K is first formed through all-optical means in a relatively weak singlebeam running-wave dipole trap that has been formed by focusing of a CO2-laser beam. By a technique that is established in the art, the trap is loaded from an ultrahigh-vacuum magnetooptical trap that is, itself, loaded via a cold atomic beam from an upstream two-dimensional magneto-optical trap that resides in a rubidium-vapor cell that is differentially pumped from an adjoining vacuum chamber, wherein are performed scientific observations of the beams ultimately generated by the atom laser.

  2. Atom Interferometry with up to 24-Photon-Momentum-Transfer Beam Splitters

    CERN Document Server

    Mueller, Holger; Long, Quan; Herrmann, Sven; Chu, Steven

    2007-01-01

    We present multi- (up to 24-)photon Bragg diffraction as beam splitter to achieve the largest splitting in momentum space in any light-pulse atom interferometer thus far. Relative to the 2-photon processes used in the most sensitive present interferometers, these large momentum transfer beam splitters increase the phase shift 12-fold for Mach-Zehnder and 144-fold for Ramsey-Borde geometries. As the atom's internal state is not changed, important systematic effects can cancel. This dramatic increase in sensitivity and precision opens the door to improved measurements of the fine-structure constant, inertial forces, and tests of relativity and quantum electrodynamics.

  3. Theoretical analysis of a collimated hollow-laser-beam generated by a single axicon using diffraction integral

    Institute of Scientific and Technical Information of China (English)

    Yong Qian(钱勇); Yuzhu Wang(王育竹)

    2004-01-01

    A novel method to generate a collimated hollow-laser-beam (HLB) by only a single axicon is proposed. With some reasonable assumptions, the radial light intensity distribution is calculated in detail by diffraction integral theory. The result of numerical simulation shows that this method is valid. Compared with other methods of generating HLB, this scheme is extraordinarily simple in principle and can be utilized experimentally to construct a light trap in atomic fountain for convenience.

  4. X-ray topography using the forward transmitted beam under multiple-beam diffraction conditions.

    Science.gov (United States)

    Tsusaka, Y; Takeda, S; Takano, H; Yokoyama, K; Kagoshima, Y; Matsui, J

    2016-02-01

    X-ray topographs are taken for a sapphire wafer with the [0001] surface normal, as an example, by forward transmitted synchrotron x-ray beams combined with two-dimensional electronic arrays in the x-ray detector having a spatial resolution of 1 μm. They exhibit no shape deformation and no position shift of the dislocation lines on the topographs. Since the topography is performed under multiple-beam diffraction conditions, the topographic images of a single diffraction (two-wave approximation condition) or plural diffractions (six-wave approximation condition) can be recorded without large specimen position changes. As usual Lang topographs, it is possible to determine the Burgers vector of each dislocation line. Because of high parallelism of the incoming x-rays and linear sensitivity of the electronic arrays to the incident x-rays, the present technique can be used to visualize individual dislocations in single crystals of the dislocation density as high as 1 × 10(5) cm(-2).

  5. PYRAMIDAL-HOLLOW-BEAM DIPOLE TRAP FOR ALKALI ATOMS

    Institute of Scientific and Technical Information of China (English)

    YIN JIAN-PING; GAO WEI-JIAN; WANG YU-ZHU; ZHU YI-FU; WANG YI-QIU

    2000-01-01

    We propose a dark gravito-optical dipole trap, for alkali atoms, consisting of a blue-detuned, pyramidal-hollow laser beam propagating upward and the gravity field. When cold atoms from a magneto-optical trap are loaded into the pyramidal-hollow beam and bounce inside the pyramidal-hollow beam, they experience efficient Sisyphus cooling and geometric cooling induced by the pyramidal-hollow beam and the weak repumping beam propagating downward. Our study shows that an ultracold and dense atomic sample with an equilibrium 3D momentum of ~ 3hk and an atomic density above the point of Bose-Einstein condensation may be obtained in this pure optical trap.

  6. A Compact, High-Flux Cold Atom Beam Source

    Science.gov (United States)

    Kellogg, James R.; Kohel, James M.; Thompson, Robert J.; Aveline, David C.; Yu, Nan; Schlippert, Dennis

    2012-01-01

    The performance of cold atom experiments relying on three-dimensional magneto-optical trap techniques can be greatly enhanced by employing a highflux cold atom beam to obtain high atom loading rates while maintaining low background pressures in the UHV MOT (ultra-high vacuum magneto-optical trap) regions. Several techniques exist for generating slow beams of cold atoms. However, one of the technically simplest approaches is a two-dimensional (2D) MOT. Such an atom source typically employs at least two orthogonal trapping beams, plus an additional longitudinal "push" beam to yield maximum atomic flux. A 2D atom source was created with angled trapping collimators that not only traps atoms in two orthogonal directions, but also provides a longitudinal pushing component that eliminates the need for an additional push beam. This development reduces the overall package size, which in turn, makes the 2D trap simpler, and requires less total optical power. The atom source is more compact than a previously published effort, and has greater than an order of magnitude improved loading performance.

  7. An Atomic Lens Using a Focusing Hollow Beam

    Institute of Scientific and Technical Information of China (English)

    夏勇; 印建平; 王育竹

    2003-01-01

    We propose a new method to generate a focused hollow laser beam by using an azimuthally distributed 2π-phase plate and a convergent thin lens, and calculate the intensity distribution of the focused hollow beam in free propagation space. The relationship between the waist w0 of the incident collimated Gaussian beam and the dark spot size of the focused hollow beam at the focal point, and the relationship between the focal length f of the thin lens and the dark spot size are studied respectively. The optical potential of the blue-detuned focused hollow beam for 85Rb atoms is calculated. Our study shows that when the larger waist w of the incident Gaussian beam and the shorter focal length f of the lens are chosen, we can obtain an extremely small dark spot size of the focused hollow beam, which can be used to form an atomic lens with a resolution of several angstroms.

  8. An introduction to Bragg diffraction-based cold atom interferometry gravimeter

    Institute of Scientific and Technical Information of China (English)

    HU; Qingqing; YANG; Jun; LUO; Yukun; JIA; Aiai; WEI; Chunhua; LI; Zehuan

    2015-01-01

    This paper presents a new type of cold atom interferometry gravimeter based on Bragg diffraction,w hich is able to increase the gravity m easurem ent sensitivity and stability of com m on Ram an atom gravim eters significantly. By com paring w ith Ram an transition,the principles and advantages of Bragg diffraction-based atom gravim eters have been introduced. The theoretical m odel for a tim e-dom ain Bragg atom gravim eter has been constructed. Som e key technical requirem ents for an n-order Bragg diffraction-based atom gravim eter have been deduced,including the tem perature of atom cloud,the diam eter,curvature radius,frequency,intensity,and tim ing sequence of Bragg lasers,etc. The analysis results are verified by the existing experim ental data in discussion. The present study provides a good reference for the understanding and construction of a Bragg atom gravim eter.

  9. Precision atomic beam density characterization by diode laser absorption spectroscopy

    Science.gov (United States)

    Oxley, Paul; Wihbey, Joseph

    2016-09-01

    We provide experimental and theoretical details of a simple technique to determine absolute line-of-sight integrated atomic beam densities based on resonant laser absorption. In our experiments, a thermal lithium beam is chopped on and off while the frequency of a laser crossing the beam at right angles is scanned slowly across the resonance transition. A lock-in amplifier detects the laser absorption signal at the chop frequency from which the atomic density is determined. The accuracy of our experimental method is confirmed using the related technique of wavelength modulation spectroscopy. For beams which absorb of order 1% of the incident laser light, our measurements allow the beam density to be determined to an accuracy better than 5% and with a precision of 3% on a time scale of order 1 s. Fractional absorptions of order 10-5 are detectable on a one-minute time scale when we employ a double laser beam technique which limits laser intensity noise. For a lithium beam with a thickness of 9 mm, we have measured atomic densities as low as 5 × 104 atoms cm-3. The simplicity of our technique and the details we provide should allow our method to be easily implemented in most atomic or molecular beam apparatuses.

  10. Production of Dynamic Frozen Waves: Controlling shape, location (and speed) of diffraction-resistant beams

    CERN Document Server

    Vieira, Tárcio A; Zamboni-Rached, Michel; Recami, Erasmo

    2015-01-01

    In recent times, we experimentally realized a quite efficient modeling of the shape of diffraction-resistant optical beams; thus generating for the first time the so-called Frozen Waves (FW), whose longitudinal intensity pattern can be arbitrarily chosen, within a prefixed space interval of the propagation axis. Such waves possess a host of potential applications: in medicine, biomedical optics, optical tweezers, atom guiding, remote sensing, tractor beams, optical communications or metrology, and other topics in photonic areas. In this work, we extend our theory of FWs -- which led to beams endowed with a static envelope -- through a dynamic modeling of the FWs, whose shape is now allowed to evolve in time in a predetermined way. And we experimentally create such dynamic FWs in Optics, via a computational holographic technique and a spatial light modulator. Experimental results are here presented for two cases of dynamic FWs, one of the zeroth and the other of higher order, the last one being the most intere...

  11. Intense Atomic and Molecular Beams via Neon Buffer Gas Cooling

    CERN Document Server

    Patterson, David; Doyle, John M

    2008-01-01

    We realize a continuous guided beam of cold deuterated ammonia with a flux of 3e11 ND3 molecules/s and a continuous free-space beam of cold potassium with a flux of 1e16 K atoms/s. A novel feature of the buffer gas source used to produce these beams is cold neon, which, due to intermediate Knudsen number beam dynamics, produces a forward velocity and low-energy tail that is comparable to much colder helium-based sources. We expect this source to be trivially generalizable to a very wide range of atomic and molecular species with significant vapor pressure below 1000 K. This source has properties that make it a good starting point for laser cooling of molecules or atoms, cold collision studies, trapping, or nonlinear optics in buffer-gas-cooled atomic or molecular gases.

  12. Investigation of accelerated neutral atom beams created from gas cluster ion beams

    Energy Technology Data Exchange (ETDEWEB)

    Kirkpatrick, A., E-mail: akirkpatrick@exogenesis.us [Exogenesis Corporation, 20 Fortune Drive, Billerica, MA 01821 (United States); Kirkpatrick, S.; Walsh, M.; Chau, S.; Mack, M.; Harrison, S.; Svrluga, R.; Khoury, J. [Exogenesis Corporation, 20 Fortune Drive, Billerica, MA 01821 (United States)

    2013-07-15

    A new concept for ultra-shallow processing of surfaces known as accelerated neutral atom beam (ANAB) technique employs conversion of energetic gas cluster ions produced by the gas cluster ion beam (GCIB) method into intense collimated beams of coincident neutral gas atoms having controllable average energies from less than 10 eV per atom to beyond 100 eV per atom. A beam of accelerated gas cluster ions is first produced as is usual in GCIB, but conditions within the source ionizer and extraction regions are adjusted such that immediately after ionization and acceleration the clusters undergo collisions with non-ionized gas atoms. Energy transfer during these collisions causes the energetic cluster ions to release many of their constituent atoms. An electrostatic deflector is then used to eliminate charged species, leaving the released neutral atoms to still travel collectively at the same velocities they had as bonded components of their parent clusters. Upon target impact, the accelerated neutral atom beams produce effects similar to those normally associated with GCIB, but to shallower depths, with less surface damage and with superior subsurface interfaces. The paper discusses generation and characterization of the accelerated neutral atom beams, describes interactions of the beams with target surfaces, and presents examples of ongoing work on applications for biomedical devices.

  13. Theoretical tools for atom-laser-beam propagation

    OpenAIRE

    Riou, Jean-Félix; Le Coq, Yann; Impens, François; Guerin, William; Bordé, Christian,; Aspect, Alain; Bouyer, Philippe

    2008-01-01

    We present a theoretical model for the propagation of non self-interacting atom laser beams. We start from a general propagation integral equation, and we use the same approximations as in photon optics to derive tools to calculate the atom laser beam propagation. We discuss the approximations that allow to reduce the general equation whether to a Fresnel-Kirchhoff integral calculated by using the stationary phase method, or to the eikonal. Within the paraxial approximation, we also introduce...

  14. Direct observation of ultrafast atomic motion using time-resolved X-ray diffraction

    Energy Technology Data Exchange (ETDEWEB)

    Shymanovich, U.

    2007-11-13

    This thesis is dedicated to the study of the atomic motion in laser irradiated solids on a picosecond to subpicosecond time-scale using the time-resolved X-ray diffraction technique. In the second chapter, the laser system, the laser-plasma based X-ray source and the experimental setup for optical pump / X-ray probe measurements were presented. Chapter 3 is devoted to the characterization and comparison of different types of X-ray optics. Chapter 4 presented the time-resolved X-ray diffraction experiments performed for this thesis. The first two sections of this chapter discuss the measurements of initially unexpected strain-induced transient changes of the integrated reflectivity of the X-ray probe beam. The elimination of the strain-induced transient changes of the integrated reflectivity represented an important prerequisite to perform the study of lattice heating in Germanium after femtosecond optical excitation by measuring the transient Debye-Waller effect. The third section describes the investigations of acoustic waves upon ultrafast optical excitation and discusses the two different pressure contributions driving them: the thermal and the electronic ones. (orig.)

  15. Neutron Diffraction Studies of the Atomic Vibrations of Bulk and Surface Atoms of Nanocrystalline SiC

    Science.gov (United States)

    Stelmakh, S.; Grzanka, E.; Zhao, Y.; Palosz, W.; Palosz, B.

    2004-01-01

    Thermal atomic motions of nanocrystalline Sic were characterized by two temperature atomic factors B(sub core), and B(sub shell). With the use of wide angle neutron diffraction data it was shown that at the diffraction vector above 15A(exp -1) the Wilson plots gives directly the temperature factor of the grain interior (B(sub core)). At lower Q values the slope of the Wilson plot provides information on the relative amplitudes of vibrations of the core and shell atoms.

  16. Cold atom dynamics in crossed laser beam waveguides

    CERN Document Server

    Torrontegui, E; Ruschhaupt, A; Guéry-Odelin, D; Muga, J G

    2010-01-01

    We study the dynamics of neutral cold atoms in an $L$-shaped crossed-beam optical waveguide formed by two perpendicular red-detuned lasers of different intensities and a blue-detuned laser at the corner. Complemented with a vibrational cooling process this setting works as a one-way device or "atom diode".

  17. Single- and double-slit collimating effects on fast-atom diffraction spectra

    Science.gov (United States)

    Gravielle, M. S.; Miraglia, J. E.

    2016-09-01

    Diffraction patterns produced by fast He atoms grazingly impinging on a LiF(0 0 1) surface are investigated focusing on the influence of the beam collimation. Single- and double-slit collimating devices situated in front of the beam source are considered. To describe the scattering process we use the Surface Initial Value Representation (SIVR) approximation, which is a semi-quantum approach that incorporates a realistic description of the initial wave packet in terms of the collimating parameters. Our initial wave-packet model is based on the Van Cittert-Zernike theorem. For a single-slit collimation the width of the collimating aperture controls the shape of the azimuthal angle distribution, making different interference mechanisms visible, while the length of the slit affects the polar angle distribution. Additionally, we found that by means of a double-slit collimation it might be possible to obtain a wide polar angle distribution, which is associated with a large spread of the initial momentum perpendicular to the surface, derived from the uncertainty principle. It might be used as a simple way to probe the surface potential for different normal energies.

  18. Low-Dose, Low-Temperature Convergent-Beam Electron Diffraction and Multiwavelength Analysis of Hydrocarbon Films by Electron Diffraction

    Science.gov (United States)

    Wu, Jinsong; Spence, John C. H.

    2003-10-01

    Aromatic hydrocarbon (perylene, coronene) and tetracontane films are shown to produce useful convergent-beam electron diffraction (CBED) patterns under low-dose and low-temperature conditions. These were obtained using a Zeiss LEO-921 electron microscope with an omega energy filter at liquid helium and nitrogen temperatures. The usefulness of patterns showing CBED disks of constant intensity (“blank disks,” indicating kinematic scattering) for structure analysis is investigated, with the aim of avoiding film-bending artifacts. Using CBED patterns from thicker areas, sample thickness was experimentally determined using either two-beam or three-beam patterns. Koehler mode illumination (a new form of SAD pattern offering smaller areas) was also used, and the possibility of obtaining structure factor moduli using the kinematic and two-beam approximations was investigated by comparing measured diffraction intensities with experimental ones for these known structures. The commonly used approximation |F| [similar] Ig (intended to account for bending) was found to be a worse approximation than the two-beam approximation with well-defined excitation error for these microdiffraction experiments. A new multiwavelength method of retrieving structure factor moduli and thickness from microdiffraction patterns using two-beam theory is demonstrated for tetracontane.

  19. Diffraction properties of four-petal Gaussian beams in uniaxially anisotropic crystal

    Institute of Scientific and Technical Information of China (English)

    Bin Tang; Yi Jin; Meiping Jiang; Xingfang Jiang

    2008-01-01

    @@ Propagation properties of polarized four-petal Gaussian beams along the optical axis of uniaxially anisotropic crystals were investigated. Based on the paraxially vectorial theory of beam propagation, analytic expressions of the diffraction light field were obtained. The effects of the anisotropy on the polarization properties of the diffracted four-petal Gaussian beams have also been explained by numerical method. The results elucidate that the linear polarization state and the symmetry of the incident beams cannot be kept during propagation in anisotropic crystals.

  20. Femtosecond electron diffraction. Next generation electron sources for atomically resolved dynamics

    Energy Technology Data Exchange (ETDEWEB)

    Hirscht, Julian

    2015-08-15

    Three instruments for femtosecond electron diffraction (FED) experiments were erected, partially commissioned and used for first diffraction experiments. The Relativistic Electron Gun for Atomic Exploration (REGAE) was completed by beamline elements including supports, a specimen chamber and dark current or electron beam collimating elements such that the commissioning process, including first diffraction experiments in this context, could be started. The temporal resolution of this machine is simulated to be 25 fs (fwhm) short, while a transverse coherence length of 30 nm (fwhm) is feasible to resolve proteins on this scale. Whether this machine is capable of meeting these predictions or whether the dynamics of the electron beam will stay limited by accelerator components, is not finally determined by the end of this work, because commissioning and improvement of accelerator components is ongoing. Simultaneously, a compact DC electron diffraction apparatus, the E-Gun 300, designed for solid and liquid specimens and a target electron energy of 300 keV, was built. Fundamental design issues of the high potential carrying and beam generating components occurred and are limiting the maximum potential and electron energy to 120 keV. Furthermore, this is limiting the range of possible applications and consequently the design and construction of a brand new instrument began. The Femtosecond Electron Diffraction CAmera for Molecular Movies (FED-CAMM) bridges the performance problems of very high electric potentials and provides optimal operational conditions for all applied electron energies up to 300 keV. The variability of gap spacings and optimized manufacturing of the high voltage electrodes lead to the best possible electron pulse durations obtainable with a compact DC setup, that does not comprise of rf-structures. This third apparatus possesses pulse durations just a few tenth femtoseconds apart from the design limit of the highly relativistic REGAE and combines the

  1. Particle manipulation beyond the diffraction limit using structured super-oscillating light beams

    CERN Document Server

    Singh, Brijesh Kumar; Roichman, Yael; Arie, Ady

    2016-01-01

    The diffraction limited resolution of light focused by a lens was derived in 1873 by Ernst Abbe. Later in 1952, a method to reach sub-diffraction light spots was proposed by modulating the wavefront of the focused beam. In a related development, super-oscillating functions, i.e. band limited functions that locally oscillate faster than their highest Fourier component, were introduced and experimentally applied for super-resolution microscopy. Up till now, only simple Gaussian-like sub-diffraction spots were used. Here we show that the amplitude and phase profile of these sub-diffraction spots can be arbitrarily controlled. In particular we utilize Hermite-Gauss, Laguerre-Gauss and Airy functions to structure super-oscillating beams with sub-diffraction lobes. These structured beams are then used for high resolution trapping and manipulation of nanometer-sized particles. The trapping potential provides unprecedented localization accuracy and stiffness, significantly exceeding those provided by standard diffrac...

  2. Field Ionization detection of supersonic helium atom beams

    Science.gov (United States)

    Doak, R. B.

    2003-10-01

    Field ionization detectors (FID) may offer near-unity detection efficiency and nanoscale spatial resolution. To date, FID detection of molecular beams has been limited to effusive beams of broad Maxwellian velocity distributions. We report FID measurements on monoenergetic helium beams, including intensity measurements and time-of-flight measurements. The FID tips were carefully prepared and characterized in a field ionization microscope prior to use. With the supersonic helium beam we find a much smaller effective detection area ( 50 sq. nm) than was reported in the effusive helium beam experiments ( 200,000 sq. nm). This suggests that the FID ionization yield depends strongly on energy loss by the impinging atom during its initial collision with the FID surface: Our thermal energy, monoenergetic helium beam atoms likely lose little or no energy upon scattering from the clean tungsten FID surface, allowing the scattered atoms to escape the FID polarization field and therby reducing the ionization yield. To improve signal levels, inelastic scattering might be enhanced by use of lower beam velocities (present in the tails of a Maxwellian) or by adsorbing an overlayer on the FID tip (present at cryogenic tip temperatures). These factors likely explain the higher detection yields measured in the effusive beam experiments.

  3. Robust population transfer in atomic beams induced by Doppler shifts

    Science.gov (United States)

    Unanyan, R. G.

    2016-10-01

    The influence of photon momentum recoil on adiabatic population transfer in an atomic three-level lambda system is studied. It is shown that the Doppler frequency shifts, due to atomic motion, can play an important role in adiabatic population transfer processes of atomic internal states by a pair of laser fields. For the limiting case of slow atoms (Doppler shift much smaller than the photon recoil energy), the atoms occupy the same target state regardless of the order of switching of laser fields, while for the case of fast atoms interacting with the intuitive sequence of pulses, the target state is the intermediate atomic state. Furthermore, it is shown that this novel technique for adiabatic population transfer is related to a level crossing in the bright-intermediate state basis (rather than in the original atomic basis). It is shown that these processes are robust with respect to parameter fluctuations, such as the laser pulse area and the relative spatial offset (delay) of the laser beams. The obtained results can be used for the control of temporal evolution of atomic populations in cold atomic beams by externally adjustable Doppler shifts.

  4. A Novel Controllable Beam Splitter for Guided Atoms

    Institute of Scientific and Technical Information of China (English)

    刘南春; 高伟建; 印建平

    2003-01-01

    We propose a novel atomic beamsplitter for guided atoms composed of a U-shaped current carrying conductor and an additional bias magnetic field, and study the dynamic process of atomic beam splitting in the beamsplitter by Monte Carlo simulations. Our study shows that the splitting ratio of the beamsplitter can be continuously adjusted from 0 to 1by changing the additional bias field. In addition, the transverse temperature of guided atoms at the outlets of the beamsplitter are also estimated and explained qualitatively.

  5. Single-Shot Electron Diffraction using a Cold Atom Electron Source

    CERN Document Server

    Speirs, Rory W; Nugent, Keith A; Sparkes, Benjamin M; Scholten, Robert E

    2015-01-01

    Cold atom electron sources are a promising alternative to traditional photocathode sources for use in ultrafast electron diffraction due to greatly reduced electron temperature at creation, and the potential for a corresponding increase in brightness. Here we demonstrate single-shot, nanosecond electron diffraction from monocrystalline gold using cold electron bunches generated in a cold atom electron source. The diffraction patterns have sufficient signal to allow registration of multiple single-shot images, generating an averaged image with significantly higher signal-to-noise ratio than obtained with unregistered averaging. Reflection high-energy electron diffraction (RHEED) was also demonstrated, showing that cold atom electron sources may be useful in resolving nanosecond dynamics of nanometre scale near-surface structures.

  6. Diffraction of fast atoms and molecules during grazing scattering from surfaces

    Science.gov (United States)

    Schüller, A.; Busch, M.; Seifert, J.; Wethekam, S.; Winter, H.

    2009-11-01

    Grazing scattering of light atoms and small molecules with energies up to several keV from atomically clean and flat surfaces along low-indexed directions gives rise to diffraction phenomena. The potential of this new method of Fast Atom Diffraction (FAD) as surface analytical tool is discussed. We show that, despite substantial decoherence due to thermal vibrations, nuclear energy loss, and, especially, excitations of the electronic system, FAD is not limited to insulator or semiconductor surfaces. Detailed studies of the geometric structure of insulator surfaces and superstructures on metal surfaces performed using FAD as an efficient virtually non-destructive method are presented.

  7. Quantum diffraction effects on the atomic polarization collision in partially ionized dense plasmas

    Energy Technology Data Exchange (ETDEWEB)

    Jung, Young-Dae, E-mail: ydjung@hanyang.ac.kr [Department of Electrical and Computer Engineering, MC 0407, University of California, San Diego, 9500 Gilman Drive, La Jolla, California 92093-0407, USA and Department of Applied Physics and Department of Bionanotechnology, Hanyang University, Ansan, Kyunggi-Do 426-791 (Korea, Republic of)

    2014-04-15

    The influence of quantum diffraction on the electron-atom polarization collision process is investigated in partially ionized dense plasmas. The pseudopotential model and eikonal method are employed to obtain the eikonal phase shift and eikonal cross section as functions of the impact parameter, collision energy, Debye length, electron de Broglie wavelength, and atomic polarizability. The results show that the eikonal phase shift for the electron-hydrogen atom polarization collision decreases with an increase of the electron de Broglie wavelength. It is important to note that the influence of quantum diffraction produces the repulsive part in the electron-atom polarization interaction. It is also found that the quantum diffraction effect enhances the differential eikonal cross section. Additionally, the total eikonal cross section decreases with increasing electron de Broglie wavelength. The variations of the eikonal cross section due to the influence of finite size of the de Broglie wavelength and Debye radius are also discussed.

  8. Diffraction-resistant scalar beams generated by a parabolic reflector and a source of spherical waves.

    Science.gov (United States)

    Zamboni-Rached, Michel; de Assis, Mariana Carolina; Ambrosio, Leonardo A

    2015-07-01

    In this work, we propose the generation of diffraction-resistant beams by using a parabolic reflector and a source of spherical waves positioned at a point slightly displaced from its focus (away from the reflector). In our analysis, considering the reflector dimensions much greater than the wavelength, we describe the main characteristics of the resulting beams, showing their properties of resistance to the diffraction effects. Due to its simplicity, this method may be an interesting alternative for the generation of long-range diffraction-resistant waves.

  9. Diffraction Resistant Scalar Beams Generated by a Parabolic Reflector and a Source of Spherical Waves

    CERN Document Server

    Zamboni-Rached, Michel; Ambrosio, Leonardo A

    2015-01-01

    In this work, we propose the generation of diffraction resistant beams by using a parabolic reflector and a source of spherical waves positioned at a point slightly displaced from its focus (away from the reflector). In our analysis, considering the reflector dimensions much greater than the wavelength, we describe the main characteristics of the resulting beams, showing their properties of resistance to the diffraction effects. Due to its simplicity, this method may be an interesting alternative for the generation of long range diffraction resistant waves.

  10. Self-focusing of femtosecond diffraction-resistant vortex beams in water.

    Science.gov (United States)

    Shiffler, Stacy; Polynkin, Pavel; Moloney, Jerome

    2011-10-01

    We report experiments on self-focusing of femtosecond diffraction-resistant vortex beams in water. These beams are higher-order Bessel beams with weak azimuthal modulation of the transverse intensity patterns. The modulation overrides the self-focusing dynamics and results in the formation of regular bottlelike filament distributions. The peak-power thresholds for filamentation, at a particular distance, are relatively accurately estimated by the adaptation of the Marburger formula derived earlier for Gaussian beams. The nonlinear conversion of the incident conical waves into the localized spatial wave packets propagating near the beam axis is observed.

  11. Spectral anomalies of diffracted pulsed Hermite-Gaussian beams in dispersive media

    Institute of Scientific and Technical Information of China (English)

    Zhao Zhi-Guo; Pan Liu-Zhan; Lü Bai-Da

    2008-01-01

    This paper derives and uses the recurrence expressions for the power spectra of diffracted pulsed Hermite-Gaussian (HG) beams in dispersive media to study the spectral anomalies of pulsed HG beams in the far field. Numerical results are given to illustrate the dependence of spectral switches on the pulse parameters, truncation parameter and dispersive property of the medium. The potential application of spectral anomalies of ultrashort pulsed beams in information encoding and transmission is discussed.

  12. Modeling laser beam diffraction and propagation by the mode-expansion method.

    Science.gov (United States)

    Snyder, James J

    2007-08-01

    In the mode-expansion method for modeling propagation of a diffracted beam, the beam at the aperture can be expanded as a weighted set of orthogonal modes. The parameters of the expansion modes are chosen to maximize the weighting coefficient of the lowest-order mode. As the beam propagates, its field distribution can be reconstructed from the set of weighting coefficients and the Gouy phase of the lowest-order mode. We have developed a simple procedure to implement the mode-expansion method for propagation through an arbitrary ABCD matrix, and we have demonstrated that it is accurate in comparison with direct calculations of diffraction integrals and much faster.

  13. Discrimination of orbital angular momentum modes of the terahertz vortex beam using a diffractive mode transformer.

    Science.gov (United States)

    Liu, Changming; Wei, Xuli; Niu, Liting; Wang, Kejia; Yang, Zhengang; Liu, Jinsong

    2016-06-13

    We present an efficient method to discriminate orbital angular momentum (OAM) of the terahertz (THz) vortex beam using a diffractive mode transformer. The mode transformer performs a log-polar coordinate transformation of the input THz vortex beam, which consists of two 3D-printed diffractive elements. A following lens separates each transformed OAM mode to a different lateral position in its focal plane. This method enables a simultaneous measurement over multiple OAM modes of the THz vortex beam. We experimentally demonstrate the measurement of seven individual OAM modes and two multiplexed OAM modes, which is in good agreement with simulations.

  14. Simulation of high energy photoelectron diffraction using many-beam dynamical Kikuchi-band theory

    Science.gov (United States)

    Winkelmann, Aimo; Schröter, Bernd; Richter, Wolfgang

    2004-06-01

    We use the many-beam dynamical theory of electron diffraction for the calculation of x-ray photoelectron diffraction (XPD) patterns of the substrate emission. The reciprocity principle is used to apply a Bloch wave model for the diffraction of an incoming plane wave by a three-dimensional crystal. In this way, many-beam dynamical simulations of XPD in the context of Kikuchi-band theory can be carried out. This extends the results of the two-beam theory used so far and leads to quantitative descriptions of XPD patterns in the picture of photoelectrons reflected by lattice planes. The effects of forward scattering directions, substrate polarity, circular structures due to onedimensional diffraction, and emitter specific extinction of Kikuchi lines can be reproduced by Kikuchi-band theory. The results are compared with single scattering cluster calculations. In this way, the equivalence of the cluster approach and the Kikuchi-band picture can be demonstrated completely in both directions

  15. Atomic-Beam Magnetic Resonance Experiments at ISOLDE

    CERN Multimedia

    2002-01-01

    The aim of the atomic-beam magnetic resonance (ABMR) experiments at ISOLDE is to map the nuclear behaviour in wide regions of the nuclear chart by measuring nuclear spins and moments of ground and isomeric states. This is made through an investigation of the atomic hyperfine structure of free, neutral atoms in a thermal atomic-beam using radio-frequency techniques. On-line operation allows the study of short-lived nuclei far from the region of beta-stability.\\\\ \\\\ The ABMR experiments on the |2S^1 ^2 elements Rb, Cs, Au and Fr have been completed, and present efforts are directed towards the elements with an open p-shell and on the rare-earth elements.\\\\ \\\\ The experimental data obtained are compared with results from model calculations, giving information on the single-particle structure and on the nuclear shape parameters.

  16. Characterization of a polychromatic neutron beam diffracted by pyrolytic graphite crystals

    CERN Document Server

    Byun, S H; Choi, H D

    2002-01-01

    The beam spectrum for polychromatic neutrons diffracted by pyrolytic graphite crystals was characterized. The theoretical beam spectrum was obtained using the diffraction model for a mosaic crystal. The lattice vibration effects were included in the calculation using the reported vibration amplitude of the crystal and the measured time-of-flight spectra in the thermal region. The calculated beam spectrum was compared with the results obtained in the absence of thermal motion. The lattice vibration effects became more important for the higher diffraction orders and a large decrease in the neutron flux induced by the vibrations was identified in the epithermal region. The validity of the beam spectrum was estimated by comparing with the effective quantities determined from prompt gamma-ray measurements and Cd-ratios measured both for 1/nu and non-1/nu nuclides.

  17. Fabrication of atomically smooth SrRuO3 thin films by laser molecular beam epitaxy

    Institute of Scientific and Technical Information of China (English)

    2008-01-01

    High-quality SrRuO3 (SRO) thin films and SrTiO3/SRO bilayer were grown epitaxially on SrTiO3 (STO)(001) substrates by laser molecular beam epitaxy. The results of in situ observation of reflection high-energy electron diffraction and ex situ X-ray diffraction θ -2θ scan indicate that the SRO thin films have good crystallinity. The measurements of atomic force microscopy and scan tunneling microscopy reveal that the surface of the SRO thin film is atomically smooth. The resistivity of the SRO thin film is 300 μΩ·cm at room temperature. Furthermore, the transmission electron microscopy study shows that the interfaces of STO/SRO and SRO/STO are very clear and no interfacial reaction layer was observed. The experimental results show that the SRO thin film is an excellent electrode material for devices based on perovskite oxide materials.

  18. Atomic physics experiments with stored cooled heavy ion beams

    Energy Technology Data Exchange (ETDEWEB)

    Datz, S.

    1986-01-01

    The wide ranging interest in the development of heavy ion synchrotrons with electron beam cooling is evident from the number of projects presently under way. Although much of the initial motivation for these rings stemmed from nuclear and particle physics, a considerable amount of atomic physics experimentation is planned. This paper surveys some of the new opportunities in atomic physics which may be made available with storage ring systems. 25 refs., 3 tabs.

  19. A compact atomic beam based system for Doppler-free laser spectroscopy of Strontium atoms

    OpenAIRE

    Verma, Gunjan; Vishwakarma, Chetan; Dharmadhikari, C. V.; Rapol, Umakant D.

    2016-01-01

    We report the construction of a simple, light weight and compact atomic beam spectroscopy cell for Strontium atoms. The cell is built using glass blowing technique and includes a simple Titanium Sublimation Pump for active pumping of the residual and background gases to maintain ultra-high vacuum. Commercially available and electrically heated dispenser source is used to generate the beam of Sr atoms. We perform spectroscopy on the $5s^2\\ ^1S_0\\longrightarrow 5s\\ 5p\\ ^1P_1$ transition to obta...

  20. Molecular Beam Studies of Hot Atom Chemical Reactions: Reactive Scattering of Energetic Deuterium Atoms

    Science.gov (United States)

    Continetti, R. E.; Balko, B. A.; Lee, Y. T.

    1989-02-01

    A brief review of the application of the crossed molecular beams technique to the study of hot atom chemical reactions in the last twenty years is given. Specific emphasis is placed on recent advances in the use of photolytically produced energetic deuterium atoms in the study of the fundamental elementary reactions D + H{sub 2} -> DH + H and the substitution reaction D + C{sub 2}H{sub 2} -> C{sub 2}HD + H. Recent advances in uv laser and pulsed molecular beam techniques have made the detailed study of hydrogen atom reactions under single collision conditions possible.

  1. Sensitive spectroscopy of an ytterbium atomic beam

    CERN Document Server

    Guttridge, A; Kemp, S L; Boddy, D; Freytag, R; Tarbutt, M R; Hinds, E A; Cornish, S L

    2015-01-01

    Experimental studies of ultracold ytterbium atoms generally involve the frequency stabilisation (locking) of lasers to two transitions at 399 and 556 nm in order to implement laser cooling. Here we present a simple and robust apparatus for generation of suitable, narrow fluorescence signals with a high signal to noise ratio at both wavelengths. The design utilises easily acquired vacuum parts, optics and electronics and requires very little laser power. We demonstrate the stability and precision of the frequency stabilisation at 556 nm by presenting sensitive measurements of the gravitational sag of an ytterbium MOT as a function of laser power.

  2. Ion beam polishing for three-dimensional electron backscattered diffraction

    DEFF Research Database (Denmark)

    Saowadee, Nath; Agersted, Karsten; Ubhi, H.S.;

    2013-01-01

    averaging and/or poor 3D-EBSD data quality. In this work a low kV focused ion beam was successfully implemented to automatically polish surfaces during 3D-EBSD of La- and Nb-doped strontium titanate of volume 12.6 × 12.6 × 3.0 μm. The key to achieving this technique is the combination of a defocused low k...

  3. Atomic Beam Laser Spectrometer for In-field Isotopic Analysis

    Energy Technology Data Exchange (ETDEWEB)

    Castro, Alonso [Los Alamos National Lab. (LANL), Los Alamos, NM (United States). Actinide Analytical Chemistry Group

    2016-06-22

    This is a powerpoint presentation for the DTRA quarterly program review that goes into detail about the atomic beam laser spectrometer for in-field isotopic analysis. The project goals are the following: analysis of post-detonation debris, determination of U and Pu isotopic composition, and fieldable prototype: < 2ft3, < 1000W.

  4. Development of atomic beam probe for tokamaks

    Energy Technology Data Exchange (ETDEWEB)

    Berta, M., E-mail: bertam@sze.hu [Széchenyi István University, EURATOM Association, Győr (Hungary); Institute of Plasma Physics AS CR, v.v.i., Prague (Czech Republic); Anda, G.; Aradi, M.; Bencze, A.; Buday, Cs.; Kiss, I.G.; Tulipán, Sz.; Veres, G.; Zoletnik, S. [Wigner – RCP, HAS, EURATOM Association, Budapest (Hungary); Havlícek, J.; Háček, P. [Institute of Plasma Physics AS CR, v.v.i., Prague (Czech Republic); Charles University in Prague, Faculty of Mathematics and Physics (Czech Republic)

    2013-11-15

    Highlights: • ABP is newly developed diagnostic. • Unique measurement method for the determination of plasma edge current variations caused by different transient events such as ELMs. • The design process has been fruitfully supported by the physically motivated computer simulations. • Li-BES system has been modified accordingly to the needs of the ABP. -- Abstract: The concept and development of a new detection method for light alkali ions stemming from diagnostic beams installed on medium size tokamak is described. The method allows us the simultaneous measurement of plasma density fluctuations and fast variations in poloidal magnetic field, therefore one can infer the fast changes in edge plasma current. The concept has been worked out and the whole design process has been done at Wigner RCP. The test detector with appropriate mechanics and electronics is already installed on COMPASS tokamak. General ion trajectory calculation code (ABPIons) has also been developed. Detailed calculations show the possibility of reconstruction of edge plasma current density profile changes with high temporal resolution, and the possibility of density profile reconstruction with better spatial resolution compared to standard Li-BES measurement, this is important for pedestal studies.

  5. Parabolic antennas, and circular slot arrays, for the generation of Non-Diffracting Beams of Microwaves

    CERN Document Server

    Zamboni-Rached, Michel

    2014-01-01

    We propose in detail Antennas for generating Non-Diffracting Beams of Microwaves, for instance with frequencies of the order of 10 GHz, obtaining fair results even when having recourse to realistic apertures endowed with reasonable diameters. Our first proposal refers mainly to sets of suitable annular slits, having in mind various possible applications, including remote sensing. Our second proposal --which constitutes one of the main aims of this paper-- refers to the alternative, rather simple, use of a Parabolic Reflector, illuminated by a spherical wave source located on the paraboloid axis but slightly displaced with respect to the Focus of the Paraboloid. Such a parabolic reflector yields "extended focus" (non-diffracting) beams. [OCIS codes: 999.9999; 070.7545; 050.1120; 280.0280; 050.1755; 070.0070; 200.0200. Keywords: Non-Diffracting Waves; Microwaves; Remote sensing; Annular Arrays; Bessel beams; Extended focus; Reflecting paraboloids; Parabolic reflectors; Parabolic antennas].

  6. An efficient and accurate method for calculating nonlinear diffraction beam fields

    Energy Technology Data Exchange (ETDEWEB)

    Jeong, Hyun Jo; Cho, Sung Jong; Nam, Ki Woong; Lee, Jang Hyun [Division of Mechanical and Automotive Engineering, Wonkwang University, Iksan (Korea, Republic of)

    2016-04-15

    This study develops an efficient and accurate method for calculating nonlinear diffraction beam fields propagating in fluids or solids. The Westervelt equation and quasilinear theory, from which the integral solutions for the fundamental and second harmonics can be obtained, are first considered. A computationally efficient method is then developed using a multi-Gaussian beam (MGB) model that easily separates the diffraction effects from the plane wave solution. The MGB models provide accurate beam fields when compared with the integral solutions for a number of transmitter-receiver geometries. These models can also serve as fast, powerful modeling tools for many nonlinear acoustics applications, especially in making diffraction corrections for the nonlinearity parameter determination, because of their computational efficiency and accuracy.

  7. A STUDY OF HIGH FRAME RATE ULTRASONIC IMAGING WITH LIMITED DIFFRACTION BEAMS

    Institute of Scientific and Technical Information of China (English)

    刘立庄; 卞正中; 姚斌

    2003-01-01

    Objective To investigate a new class of solutions to the isotropic/homogeneous scalar wave equation, which termed limited diffraction beams and realize ultrasonic 3D imaging. Methods Limited diffraction beams were derived. We performed the study of 3D pulse-echo imaging with limited diffraction array beam. To obtain high frame rate images, a single plane wave pulse (broadband) was transmitted with the arrays. Echoes received with the same arrays were processed with Fourier method to construct 3D images. Results Compared with traditional pulse-echo imaging, this method has a larger depth of field, high frame rate, and high signal-to-noise ratio. Conclusion The new method has prospect of high frame rate 3D imaging. In addition, the imaging system based this method is easily implemented and has high quality image.

  8. A single diffractive optical element for implementing spectrum-splitting and beam-concentration functions simultaneously with high diffraction efficiency

    CERN Document Server

    Ye, Jia-Sheng; Huang, Qing-Li; Dong, Bi-Zhen; Zhang, Yan; Yang, Guo-Zhen

    2013-01-01

    In this paper, a novel method is proposed, and employed to design a single diffractive optical element (DOE) for implementing spectrum-splitting and beam-concentration (SSBC) functions simultaneously. We develop an optimization algorithm, through which the SSBC DOE can be optimized within an arbitrary thickness range, according to the limitations of modern photolithography technology. Theoretical simulation results reveal that the designed SSBC DOE has a high optical focusing efficiency. It is expected that the designed SSBC DOE should have practical applications in high-efficiency solar cell systems.

  9. A single diffractive optical element implementing spectrum-splitting and beam-concentration functions simultaneously with high diffraction efficiency

    Institute of Scientific and Technical Information of China (English)

    Ye Jia-Sheng; Wang Jin-Ze; Huang Qing-Li; Dong Bi-Zhen; Zhang Yan; Yang Guo-Zhen

    2013-01-01

    In this paper,a novel method is proposed and employed to design a single diffractive optical element (DOE) for implementing spectrum-splitting and beam-concentration (SSBC) functions simultaneously.We develop an optimization algorithm,through which the SSBC DOE can be optimized within an arbitrary thickness range according to the limitations of modem photolithography technology.Theoretical simulation results reveal that the designed SSBC DOE has a high optical focusing efficiency.It is expected that the designed SSBC DOE should have practical applications in high-efficiency solar cell systems.

  10. Manufacture of refractive and diffractive beam-shaping elements in higher quantities using glass molding technology

    Science.gov (United States)

    Wolz, Michael; Blöcher, Ullrich; Dross, Gerhard; Schmitt, Jana; Bischoff, Christian; Umhofer, Udo

    2015-03-01

    Laser beam shaping elements can be used e.g. for material processing. The results of these processes can be improved when the usually Gaussian profile of the laser is transformed into a top hat profile, which can be circular or rectangular in shape. Another frequently used type of beam-forming devices are beam splitters for parallel processing using only one laser. These types of beam formers can be implemented as diffractive or refractive elements. So far these optics are produced either directly by means of lithography e.g. in glass or in plastic using a hot embossing process or nanoimprint technology. Elements produced in this way have either the disadvantage of high costs or they are limited in temperature range, laser power or wavelength. A newly developed molding process for glass allows the manufacture of larger numbers of optics with reduced cost. The production of molds for refractive top hat beam shaping devices requires very high precision of the applied grinding process. Form deviations below 100 nm are necessary to obtain a homogeneous illumination. Measurements of the surface topography of gauss to top hat beam shaping elements using white light interferometry are presented as well as results of optical measurements of the beam profile using a camera. Continuous diffractive beam shaping elements for beam splitting applications are designed to generate several sub-beams each carrying the same energy. In order to achieve this, form deviations of less than 50 nm are required. Measurements of the surface of a 1 x 5 beam splitter are compared with ideal beam splitter profiles. The resulting beam intensity distribution of a molded element is presented.

  11. Genetic algorithms optimization of photonic crystal fibers for half diffraction angle reduction of output beam.

    Science.gov (United States)

    Lu, Jyun-Hong; Cai, Dong-Po; Tsai, Ya-Lun; Chen, Chii-Chang; Lin, Chu-En; Yen, Ta-Jen

    2014-09-22

    In this work, we optimize the structure of the photonic crystal fibers by using genetic algorithms to provide strong light confinement in fiber and small half diffraction angle of output beam. Furthermore, this article shows the potentials of this study, such as optimizing three purposes at the same time and the arbitrary structure design is achieved. We report two optimized results obtained by different optimization conditions. The results show that the half diffraction angle of the output beam of the photonic crystal fibers can be reduced.

  12. Formation of high-order acoustic Bessel beams by spiral diffraction gratings

    CERN Document Server

    Jiménez, Noé; Sánchez-Morcillo, Víctor; Romero-García, Vicent; García-Raffi, Lluis M; Staliunas, Kestutis

    2016-01-01

    The formation of high-order Bessel beams by a passive acoustic device consisting of an Archimedes' spiral diffraction grating is theoretically, numerically and experimentally reported in this work. These beams are propagation-invariant solutions of the Helmholtz equation and are characterized by an azimuthal variation of the phase along its annular spectrum producing an acoustic vortex in the near field. In our system, the scattering of plane acoustic waves by the spiral grating leads to the formation of the acoustic vortex with zero pressure on-axis and the angular phase dislocations characterized by the spiral geometry. The order of the generated Bessel beam and, as a consequence, the size of the generated vortex can be fixed by the number of arms in the spiral diffraction grating. The obtained results allow to obtain Bessel beams with controllable vorticity by a passive device, which has potential applications in low-cost acoustic tweezers and acoustic radiation force devices.

  13. Formation of high-order acoustic Bessel beams by spiral diffraction gratings

    Science.gov (United States)

    Jiménez, Noé; Picó, R.; Sánchez-Morcillo, V.; Romero-García, V.; García-Raffi, L. M.; Staliunas, K.

    2016-11-01

    The formation of high-order Bessel beams by a passive acoustic device consisting of an Archimedes' spiral diffraction grating is theoretically, numerically, and experimentally reported in this paper. These beams are propagation-invariant solutions of the Helmholtz equation and are characterized by an azimuthal variation of the phase along its annular spectrum producing an acoustic vortex in the near field. In our system, the scattering of plane acoustic waves by the spiral grating leads to the formation of the acoustic vortex with zero pressure on axis and the angular phase dislocations characterized by the spiral geometry. The order of the generated Bessel beam and, as a consequence, the size of the generated vortex can be fixed by the number of arms in the spiral diffraction grating. The obtained results allow for obtaining Bessel beams with controllable vorticity by a passive device, which has potential applications in low-cost acoustic tweezers and acoustic radiation force devices.

  14. Noninvasive measurement of micron electron beam size of high energy using diffraction radiation

    CERN Document Server

    Naumenko, G A

    2003-01-01

    Treatments of the usage of diffraction radiation from the relativistic electrons moving though a conductive slit for the transverse beam size measurement encounter hard limitation of the method sensitivity for the electron energy larger than 1 GeV. We consider in this article a possibility of application of the artificial phase shift, which can take place when transverse electron position varies. This allows us to realize the measurements of transverse size of supper-relativistic electron beams with the small emittance.

  15. A prompt gamma neutron activation analysis facility using a diffracted beam

    Science.gov (United States)

    Harling, Otto K.; Chabeuf, Jean-Michel; Lambert, Frédérique; Yasuda, Gopika

    1993-12-01

    A prompt gamma neutron activation analysis facility has been constructed at the MIT Research Reactor using a diffracted beam from a multilayered graphite monochromator. A beam of 0.0143 eV neutrons of intensity 6 × 10 6{n}/{cm 2}s is available at the sample position. Backgrounds are low due to the use of the diffracted beam and are further improved by a sapphire crystal in the beam line. This design allowed the Ge detecting crystal to be placed close to the sample position, 4 cm, with a resultant high detection efficiency. The sensitivity of the facility is reported for several representative pure elements. The major impetus for the construction of this facility was the need for accurate analyses of 10B in biological samples for neutron capture therapy research. Detailed results for this type of analysis are provided. The sensitivity of this diffracted beam facility currently exceeds that of two representative direct beam facilities using reactors of twice the power of the MITR-II. Possible major improvements in sensitivity, more than an order of magnitude, and in background levels are outlined for future development.

  16. Beam Size Measurement by Optical Diffraction Radiation and Laser System for Compton Polarimeter

    Energy Technology Data Exchange (ETDEWEB)

    Liu, Chuyu [Peking Univ., Beijing (China)

    2012-12-31

    Beam diagnostics is an essential constituent of any accelerator, so that it is named as "organs of sense" or "eyes of the accelerator." Beam diagnostics is a rich field. A great variety of physical effects or physical principles are made use of in this field. Some devices are based on electro-magnetic influence by moving charges, such as faraday cups, beam transformers, pick-ups; Some are related to Coulomb interaction of charged particles with matter, such as scintillators, viewing screens, ionization chambers; Nuclear or elementary particle physics interactions happen in some other devices, like beam loss monitors, polarimeters, luminosity monitors; Some measure photons emitted by moving charges, such as transition radiation, synchrotron radiation monitors and diffraction radiation-which is the topic of the first part of this thesis; Also, some make use of interaction of particles with photons, such as laser wire and Compton polarimeters-which is the second part of my thesis. Diagnostics let us perceive what properties a beam has and how it behaves in a machine, give us guideline for commissioning, controlling the machine and indispensable parameters vital to physics experiments. In the next two decades, the research highlight will be colliders (TESLA, CLIC, JLC) and fourth-generation light sources (TESLA FEL, LCLS, Spring 8 FEL) based on linear accelerator. These machines require a new generation of accelerator with smaller beam, better stability and greater efficiency. Compared with those existing linear accelerators, the performance of next generation linear accelerator will be doubled in all aspects, such as 10 times smaller horizontal beam size, more than 10 times smaller vertical beam size and a few or more times higher peak power. Furthermore, some special positions in the accelerator have even more stringent requirements, such as the interaction point of colliders and wigglor of free electron lasers. Higher performance of these accelerators increases the

  17. The effect of laser beam size in a zig-zag collimator on transverse cooling of a krypton atomic beam

    Indian Academy of Sciences (India)

    Vivek Singh; V B Tiwari; S Singh; S R Mishra; H S Rawat

    2014-07-01

    The effect of size of a cooling laser beam in a zig-zag atomic beam collimator on transverse cooling of a krypton atomic beam is investigated. The simulation results show that discreteness in the interaction between the cooling laser beam and atomic beam, arising due to finite size and incidence angle of the cooling laser beam, significantly reduces the value of transverse velocity capture range of the collimator. The experimental observations show the trend similar to that obtained from simulations. Our study can be particularly useful where a small zig-zag collimator is required.

  18. Theoretical study of precision and accuracy of strain analysis by nano-beam electron diffraction

    Energy Technology Data Exchange (ETDEWEB)

    Mahr, Christoph, E-mail: mahr@ifp.uni-bremen.de; Müller-Caspary, Knut; Grieb, Tim; Schowalter, Marco; Mehrtens, Thorsten; Krause, Florian F.; Zillmann, Dennis; Rosenauer, Andreas

    2015-11-15

    Measurement of lattice strain is important to characterize semiconductor nanostructures. As strain has large influence on the electronic band structure, methods for the measurement of strain with high precision, accuracy and spatial resolution in a large field of view are mandatory. In this paper we present a theoretical study of precision and accuracy of measurement of strain by convergent nano-beam electron diffraction. It is found that the accuracy of the evaluation suffers from halos in the diffraction pattern caused by a variation of strain within the area covered by the focussed electron beam. This effect, which is expected to be strong at sharp interfaces between materials with different lattice plane distances, will be discussed for convergent-beam electron diffraction patterns using a conventional probe and for patterns formed by a precessing electron beam. Furthermore, we discuss approaches to optimize the accuracy of strain measured at interfaces. The study is based on the evaluation of diffraction patterns simulated for different realistic structures that have been investigated experimentally in former publications. These simulations account for thermal diffuse scattering using the frozen-lattice approach and the modulation-transfer function of the image-recording system. The influence of Poisson noise is also investigated. - Highlights: • Theoretical study of precision and accuracy of strain analysis by nano-beam electron diffraction. • Evaluation of simulations for exact knowledge of the actual strain. • Improvement of precision using electron beam precession. • Explanation of artefacts in the measurement close to interfaces. • Theoretical solution for the improvement of the accuracy at interfaces.

  19. High-resolution diffraction microscopy using the plane-wave field of a nearly diffraction limited focused x-ray beam

    OpenAIRE

    Takahashi, Yukio; Nishino, Yoshinori; Tsutsumi, Ryosuke; Kubo, Hideto; Furukawa, Hayato; Mimura, Hidekazu; MATSUYAMA, Satoshi; Zettsu, Nobuyuki; Matsubara, Eiichiro; Ishikawa, Tetsuya; Yamauchi, Kazuto

    2009-01-01

    X-ray waves in the center of the beam waist of nearly diffraction limited focused x-ray beams can be considered to have amplitude and phase that are both almost uniform, i.e., they are x-ray plane waves. Here we report the results of an experimental demonstration of high-resolution diffraction microscopy using the x-ray plane wave of the synchrotron x-ray beam focused using Kirkpatrik-Baez mirrors. A silver nanocube with an edge length of ∼100 nm is illuminated with the x-ray beam focused to ...

  20. Surface symmetry of monolayer titanium oxide on Mo(1 1 2) studied via fast atom diffraction

    Energy Technology Data Exchange (ETDEWEB)

    Seifert, J., E-mail: jan.seifert@physik.hu-berlin.de; Winter, H.

    2013-11-15

    In studies on titanium oxide thin films we demonstrate the potential of Fast Atom Diffraction (FAD) and triangulation methods to derive the surface unit cell with enhanced surface sensitivity. Helium atoms with energies of 1–2 keV are scattered from the surface along low indexed surface directions under grazing angles of incidence. From the observed diffraction patterns, the lateral periodicity of the surface structures is derived. For low TiO{sub x} coverages a well-ordered c(2 × 4) superstructure and for higher coverage a p(8 × 2) film is observed. Based on FAD and triangulation methods for azimuthal rotation of the target the arrangement of topmost atoms in smaller sub-unit cells is revealed.

  1. Overview of non-intercepting beam-size monitoring with optical diffraction radiation

    CERN Document Server

    Lumpkin, Alex H

    2012-01-01

    The initial demonstrations over the last several years of the use of optical diffraction radiation (ODR) as non-intercepting electron-beam-parameter monitors are reviewed. Developments in both far-field imaging and near-field imaging are addressed for ODR generated by a metal plane with a slit aperture, a single metal plane, and two-plane interferences. Polarization effects and sensitivities to beam size, divergence, and position will be discussed as well as a proposed path towards monitoring 10-micron beam sizes at 25 GeV.

  2. Overview of nonintercepting beam-size monitoring with optical diffraction radiation

    Energy Technology Data Exchange (ETDEWEB)

    Lumpkin, Alex H.; /Fermilab

    2010-08-01

    The initial demonstrations over the last several years of the use of optical diffraction radiation (ODR) as nonintercepting electron-beam-parameter monitors are reviewed. Developments in both far-field imaging and near-field imaging are addressed for ODR generated by a metal plane with a slit aperture, a single metal plane, and two-plane interferences. Polarization effects and sensitivities to beam size, divergence, and position will be discussed as well as a proposed path towards monitoring 10-micron beam sizes at 25 GeV.

  3. Image processing for grazing incidence fast atom diffraction: the $\\beta_2$(2x4) reconstruction of the GaAs(001) surface

    CERN Document Server

    Debiossac, Maxime

    2015-01-01

    Grazing incidence fast atom diffraction (GIFAD, or FAD) has developed as a very sensitive technique most suited for well ordered crystalline surfaces. Such high quality surfaces are routinely fabricated in molecular beam epitaxy (MBE) chamber and a GIFAD setup has been installed allowing in situ operation. Focusing here on static condition, i.e. before or after the growth process, the paper describes in details the few steps needed to measure the relative intensities of the diffraction spots. Care is taken to outline the underlying physical assumptions.

  4. Quantitative strain analysis for advanced CMOS technology by Nano Beam Diffraction

    KAUST Repository

    Wang, Qingxiao

    2010-07-01

    Nano Beam Diffraction has been used to analyze the local strain distribution in MOS transistors. The influence of wafer process on the channel strain has been systematically analyzed in this paper. The source/drain implantation can cause a little strain loss but the silicidation step is the key process in which dramatic strain loss has been found. © 2010 IEEE.

  5. Neutral atom beam technique enhances bioactivity of PEEK

    Energy Technology Data Exchange (ETDEWEB)

    Khoury, Joseph, E-mail: jkhoury@exogenesis.us [Exogenesis Corporation, Billerica, MA 01821 (United States); Kirkpatrick, Sean R.; Maxwell, Melissa; Cherian, Raymond E.; Kirkpatrick, Allen; Svrluga, Richard C. [Exogenesis Corporation, Billerica, MA 01821 (United States)

    2013-07-15

    Polyetheretherketone (PEEK) is currently gaining popularity in orthopedic and spinal applications but has potential drawbacks in use. PEEK is biocompatible, similar in elasticity to bone, and radiolucent; however, it has been shown to be inert and does not integrate well with bone. Recent efforts have focused on increasing the bioactivity of PEEK by modifying the surface to improve the bone-implant interface. We have employed a novel Accelerated Neutral Atom Beam technique (ANAB) to enhance the bioactivity of PEEK. ANAB employs an intense beam of cluster-like packets of accelerated unbonded neutral argon (Ar) gas atoms. These beams are created by first producing a highly energetic Gas Cluster Ion Beam (GCIB) comprised of van der Waals bonded Ar atoms, then transferring energy to the clusters so as to cause release of most of the interatomic bonds, and finally deflecting away the remaining electrically charged cluster cores of still bonded atoms. We identified that ANAB treatment of PEEK results in nanometer scale surface modifications as well as increased surface hydrophilicity. Human osteoblasts seeded onto the surface of ANAB-treated PEEK exhibited enhanced growth as compared to control PEEK as evidenced by cell proliferation assays and microscopy. This increase in bioactivity resulted in cell proliferation levels comparable to native titanium. An in vivo study using a rat calvarial critical size defect model revealed enhanced osseointegration where bone tissue formation was evident only on the ANAB treated PEEK. Taken together, these data suggest that ANAB treatment of PEEK has the potential to enhance its bioactivity, resulting in bone formation and significantly decreasing osseointegration time of orthopedic and spinal implants.

  6. Optical phase conjugation in atomic beams and vapors

    Science.gov (United States)

    Donoghue, John James

    1997-07-01

    Optical phase conjugation in atomic beams and vapors using alkali metal atoms as the nonlinear medium is examined. The significance of the sodium system is that the nonlinear gain is high due to the hyperfine system, which behaves as a Raman system. The gains observed were larger than 100 in cases involving two separate pump lasers. The gain is also seen to be more complicated than a Raman system. The frequency of the beams is examined for three separate configurations. We examine a self pumped configuration, an externally pumped configuration consisting of two pump lasers and a probe, and a ring configuration. The observed gain in a self pumped configuration is a result of a mixture of a three level Mollow type gain and a Raman gain. The initial cavity laser is a result of the Mollow gain, and the conjugate produced is seen to arise from the interaction of the cavity beams with the initial pump beam to produce the conjugate. In the externally pumped scheme, the gain is due to Coherent Population Trapping (CPT) in a double-Λ Raman system. There is an equilibrium that is obtained that is responsible for the high gains observed in this particular setup. The bandwidth of the ground state two photon induced coherence is less than the natural lifetime, indicating CPT as the gain mechanism. In the ring configuration, we observed two separate gains. There is a forward and a backward gain. These two oscillations occur together for a 430 MHZ bandwidth which coincides with the observed width of the phase conjugate oscillation. The design of our vapor cells is discussed in depth. The heat pipe configuration, necessary to successfully conduct these experiments is shown in detail. The design of our atomic beams is also discussed.

  7. Classical simulation of atomic beam focusing and deposition for atom lithography

    Institute of Scientific and Technical Information of China (English)

    Xianzhong Chen(陈献忠); Hanmin Yao(姚汉民); Xunan Chen(陈旭南)

    2004-01-01

    We start from the intensity distribution of a standing wave (SW) laser field and deduce the classical equation of atomic motion. The image distortion is analyzed using transfer function approach. Atomic flux density distribution as a function of propagation distance is calculated based on Monte-Carlo scheme and trajectory tracing method. Simulation results have shown that source imperfection, especially beam spread, plays an important role in broadening the feature width, and the focus depth of atom lens for real atomic source is longer than that for perfect source. The ideal focal plane can be easily determined by the variation of atomic density at the minimal potential of the laser field as a function of traveling distance.

  8. Half-plane diffraction of Gaussian beams carrying two vortices of equal charges

    Institute of Scientific and Technical Information of China (English)

    He De; Gao Zeng-Hui; Lü Bai-Da

    2011-01-01

    This paper derives explicit expressions for the propagation of Ganssian beams carrying two vortices of equal charges m =±1 diffracted at a half-plane screen,which enables the study of the dynamic evolution of vortices in the diffraction field.It shows that there may be no vortices,a pair or several pairs of vortices of opposite charges m =+l,-1 in the diffraction field.Pair creation,annihilation and motion of vortices may appear upon propagation.The off-axis distance additionally affects the evolutionary behaviour.In the process the total topological charge is equal to zero,which is unequal to that of the vortex beam at the source plane.A comparison with the free-space propagation of two vortices of equal charges and a further extension are made.

  9. Modern Focused-Ion-Beam-Based Site-Specific Specimen Preparation for Atom Probe Tomography.

    Science.gov (United States)

    Prosa, Ty J; Larson, David J

    2017-02-06

    Approximately 30 years after the first use of focused ion beam (FIB) instruments to prepare atom probe tomography specimens, this technique has grown to be used by hundreds of researchers around the world. This past decade has seen tremendous advances in atom probe applications, enabled by the continued development of FIB-based specimen preparation methodologies. In this work, we provide a short review of the origin of the FIB method and the standard methods used today for lift-out and sharpening, using the annular milling method as applied to atom probe tomography specimens. Key steps for enabling correlative analysis with transmission electron-beam backscatter diffraction, transmission electron microscopy, and atom probe tomography are presented, and strategies for preparing specimens for modern microelectronic device structures are reviewed and discussed in detail. Examples are used for discussion of the steps for each of these methods. We conclude with examples of the challenges presented by complex topologies such as nanowires, nanoparticles, and organic materials.

  10. On-line laser spectroscopy with thermal atomic beams

    CERN Document Server

    Thibault, C; De Saint-Simon, M; Duong, H T; Guimbal, P; Huber, G; Jacquinot, P; Juncar, P; Klapisch, Robert; Liberman, S; Pesnelle, A; Pillet, P; Pinard, J; Serre, J M; Touchard, F; Vialle, J L

    1981-01-01

    On-line high resolution laser spectroscopy experiments have been performed in which the light from a CW tunable dye laser interacts at right angles with a thermal atomic beam. /sup 76-98/Rb, /sup 118-145 /Cs and /sup 208-213/Fr have been studied using the ionic beam delivered by the ISOLDE on-line mass separator at CERN while /sup 30-31/Na and /sup 38-47/K have been studied by setting the apparatus directly on-line with the PS 20 GeV proton beam. The principle of the method is briefly explained and some results concerning nuclear structure are given. The hyperfine structure, spins and isotope shifts of the alkali isotopes and isomers are measured. (8 refs).

  11. Coherent and non coherent atom optics experiment with an ultra-narrow beam of metastable rare gas atoms; Experiences d'optique atomique coherente ou non avec un jet superfin d'atomes metastables de gaz rares

    Energy Technology Data Exchange (ETDEWEB)

    Grucker, J

    2007-12-15

    In this thesis, we present a new type of atomic source: an ultra-narrow beam of metastable atoms produced by resonant metastability exchange inside a supersonic beam of rare gas atoms. We used the coherence properties of this beam to observe the diffraction of metastable helium, argon and neon atoms by a nano-transmission grating and by micro-reflection-gratings. Then, we evidenced transitions between Zeeman sublevels of neon metastable {sup 3}P{sub 2} state due to the quadrupolar part of Van der Waals potential. After we showed experimental proofs of the observation of this phenomenon, we calculated the transition probabilities in the Landau - Zener model. We discussed the interest of Van der Waals - Zeeman transitions for atom interferometry. Last, we described the Zeeman cooling of the supersonic metastable argon beam ({sup 3}P{sub 2}). We have succeeded in slowing down atoms to speeds below 100 m/s. We gave experimental details and showed the first time-of-flight measurements of slowed atoms.

  12. Toward atomic resolution diffractive imaging of isolated molecules with x-ray free-electron lasers

    CERN Document Server

    Stern, Stephan; Filsinger, Frank; Rouzée, Arnaud; Rudenko, Artem; Johnsson, Per; Martin, Andrew V; Barty, Anton; Bostedt, Christoph; Bozek, John D; Coffee, Ryan N; Epp, Sascha; Erk, Benjamin; Foucar, Lutz; Hartmann, Robert; Kimmel, Nils; Kühnel, Kai-Uwe; Maurer, Jochen; Messerschmidt, Marc; Rudek, Benedikt; Starodub, Dmitri G; Thøgersen, Jan; Weidenspointner, Georg; White, Thomas A; Stapelfeldt, Henrik; Rolles, Daniel; Chapman, Henry N; Küpper, Jochen

    2014-01-01

    We give a detailed account of the theoretical analysis and the experimental results of an x-ray-diffraction experiment on quantum-state selected and strongly laser-aligned gas-phase ensembles of the prototypical large asymmetric rotor molecule 2,5-diiodobenzonitrile, performed at the Linac Coherent Light Source [Phys. Rev. Lett. 112, 083002 (2014)]. This experiment is the first step toward coherent diffractive imaging of structures and structural dynamics of isolated molecules at atomic resolution, i. e., picometers and femtoseconds, using x-ray free-electron lasers.

  13. Interaction of Photon Vortex Beams with Atomic Matter

    Science.gov (United States)

    Solyanik, Maria; Afanasev, Andrei; Carlson, Carl E.

    2017-01-01

    In our work we consider helical Bessel beams' (BB's) propagation and interaction with isotropic matter. Dynamical properties of the beams with non-zero orbital angular momentum (OAM), which are determined by spatial degrees of freedom and polarization, modify the fundamental processes in light-matter interactions. Circular dichroism of BBs propagating in hydrogen gas was considered within the frame of studying the vortex beams' attenuation due to photoabsorption in hydrogen gas. In this case, the phenomenon is due to the topology of the wave front, contrary to the zero OAM case, when the change in polarization state is due to matter inhomogeneity. The effect of circular dichroism has been predicted by calculating the beam ellipticity evolution when traversing an isotropic target. According to our results, the BBs' transverse ellipticity profile has a structure of concentric circular maxima which correspond to minima of the intensity. The characteristic polarization singularity arises on the beam axis as the result of interaction with matter. It is shown, that even for the case of the paraxial approximation the effect of circular dichroism takes place. These signatures can be used for theoretical and experimental analysis of the interactions of optical vortices with atomic matter.

  14. Performance predictions of a focused ion beam from a laser cooled and compressed atomic beam

    Energy Technology Data Exchange (ETDEWEB)

    Haaf, G. ten; Wouters, S. H. W.; Vredenbregt, E. J. D.; Mutsaers, P. H. A. [Department of Applied Physics, Eindhoven University of Technology, P.O. Box 513, 5600 MB Eindhoven (Netherlands); Geer, S. B. van der [Department of Applied Physics, Eindhoven University of Technology, P.O. Box 513, 5600 MB Eindhoven (Netherlands); Pulsar Physics, Burghstraat 47, 5614 BC Eindhoven (Netherlands)

    2014-12-28

    Focused ion beams are indispensable tools in the semiconductor industry because of their ability to image and modify structures at the nanometer length scale. Here, we report on performance predictions of a new type of focused ion beam based on photo-ionization of a laser cooled and compressed atomic beam. Particle tracing simulations are performed to investigate the effects of disorder-induced heating after ionization in a large electric field. They lead to a constraint on this electric field strength which is used as input for an analytical model which predicts the minimum attainable spot size as a function of, amongst others, the flux density of the atomic beam, the temperature of this beam, and the total current. At low currents (I < 10 pA), the spot size will be limited by a combination of spherical aberration and brightness, while at higher currents, this is a combination of chromatic aberration and brightness. It is expected that a nanometer size spot is possible at a current of 1 pA. The analytical model was verified with particle tracing simulations of a complete focused ion beam setup. A genetic algorithm was used to find the optimum acceleration electric field as a function of the current. At low currents, the result agrees well with the analytical model, while at higher currents, the spot sizes found are even lower due to effects that are not taken into account in the analytical model.

  15. Intermolecular orientations in liquid acetonitrile: new insights based on diffraction measurements and all-atom simulations

    CERN Document Server

    Pothoczki, Szilvia

    2016-01-01

    Intermolecular correlations in liquid acetonitrile (CH3CN) have been revisited by calculating orientational correlation functions. In the present approach, hydrogen atoms are included, so that a concept applicable for molecules of (nearly) tetrahedral shape can be exploited. In this way molecular arrangements are elucidated not only for closest neighbours but also extending well beyond the first coordination sphere. Thus a complementary viewpoint is provided to the more popular dipole-dipole correlations. Our calculations are based on large structural models that were obtained by applying diffraction data and partial radial distribution functions from potential-based (all-atom) molecular dynamics simulation simultaneously, within the framework of the Reverse Monte Carlo method.

  16. Plasmas and atom beam activation of the surface of polymers

    Energy Technology Data Exchange (ETDEWEB)

    Lopez-Santos, C; Yubero, F; Cotrino, J; Barranco, A; Gonzalez-Elipe, A R [Instituto de Ciencia de Materiales de Sevilla (CSIC-Univ. Sevilla), Avda Americo Vespucio 49, E-41092 Sevilla (Spain)], E-mail: arge@icmse.csic.es

    2008-11-21

    Wetting properties of polyethylene terephthalate (PET) and low-density polyethylene polymers have been investigated after treatment with a microwave (MW) plasma discharge at low pressure and a dielectric barrier discharge at atmospheric pressure. Experiments have also been carried out in situ with an atom source installed in an x-ray photoemission spectrometer (XPS). The water contact angle measured on both polymers experienced a significant decrease after activation, but a progressive recovery up to different values after ageing. Standard chemical analysis by XPS showed that the plasma and oxygen beam treatments produced an increase in the concentration of -C(O){sub x} functional groups at the outermost surface layers of the treated polymers. Besides, the oxygen distribution between the topmost surface layer and the bulk has been obtained by non-destructive XPS peak shape analysis. Atomic force microscopy analysis of the surface topography showed that, except for PET treated with the MW plasma and the atom beam, the surface roughness increased after the plasma treatments. Wetting angle variations, oxygen content and distribution, surface roughness and evolution of these properties with time are comparatively discussed by taking into account the basic processes that each type of activation procedure induces in the outmost surface layers of the treated polymers.

  17. New view on the diffraction discovered by Grimaldi and Gaussian beams

    CERN Document Server

    Yurkin, Alexander V

    2013-01-01

    In offered work short historical excursus to the classical theory of light is presented: Grimaldi, Fermat, Newton, Huygens, Young, Fresnel, Fraunhofer, and Gauss. The ray analog of wave model of light and Huygens-Fresnel's elementary waves on the basis of consideration of geometrical model is offered. New geometrical properties of Gaussian beams are analyzed. The new, generalized interpretation of a corner of diffraction divergence of beams of light is given. Difference of geometrical properties of wave fronts of infinite and finite length is shown. Examples of possible application of our geometrical model in various areas are given.

  18. Diffractive-optics-based beam combination of a phase-locked fiber laser array.

    Science.gov (United States)

    Cheung, Eric C; Ho, James G; Goodno, Gregory D; Rice, Robert R; Rothenberg, Josh; Thielen, Peter; Weber, Mark; Wickham, Michael

    2008-02-15

    A diffractive optical element (DOE) is used as a beam combiner for an actively phase-locked array of fiber lasers. Use of a DOE eliminates the far-field sidelobes and the accompanying loss of beam quality typically observed in tiled coherent laser arrays. Using this technique, we demonstrated coherent combination of five fiber lasers with 91% efficiency and M2=1.04. Combination efficiency and phase locking is robust even with large amplitude and phase fluctuations on the input laser array elements. Calculations and power handling measurements suggest that this approach can scale to both high channel counts and high powers.

  19. Scattering of diffracting beams of electron cyclotron waves by random density fluctuations in inhomogeneous plasmas

    Science.gov (United States)

    Weber, Hannes; Maj, Omar; Poli, Emanuele

    2015-03-01

    The physics and first results of the new WKBeam code for electron cyclotron beams in tokamak plasmas are presented. This code is developed on the basis of a kinetic radiative transfer model which is general enough to account for the effects of diffraction and density fluctuations on the beam. Our preliminary numerical results show a significant broadening of the power deposition profile in ITER due to scattering from random density fluctuations at the plasma edge, while such scattering effects are found to be negligible in medium-size tokamaks like ASDEX upgrade.

  20. Preserving a diffraction-limited beam in Ho:YAG laser using coherent polarization locking.

    Science.gov (United States)

    Tan, L H; Chua, C F; Phua, P B

    2012-11-15

    We overcome several thermal issues present in Ho:YAG lasers by distributing the gain over a larger volume and achieve a diffraction-limited beam using coherent polarization locking. Increased single-pass absorption, suppression of output power saturation, and improvement in beam quality were shown using the coherent polarization locking technique as compared to a conventional Ho:YAG laser cavity with the same pump and cavity configuration. Ten watts of CW Ho:YAG laser power was generated with >96% coherent combining efficiency.

  1. Matter-wave beam splitter on an atom chip for a portable atom-interferometer

    CERN Document Server

    Kim, S J; Gang, S T; Kim, J B

    2016-01-01

    We construct a matter-wave beam splitter using 87Rb Bose-Einstein condensate on an atom chip. Through the use of radio-frequency-induced double-well potentials, we were able to split a BEC into two clouds separated by distances ranging from 2.8 {\\mu}m to 57 {\\mu}m. Interference between these two freely expanding BECs has been observed. By varying the rf-field amplitude, frequency, or polarization, we investigate behaviors of the beam-splitter. From the perspective of practical use, our BEC manipulation system is suitable for application to interferometry since it is compact and the repetition rate is high due to the anodic bonded atom chip on the vacuum cell. The portable system occupies a volume of 0.5 m3 and operates at a repetition rate as high as ~0.2 Hz.

  2. Diffraction control in PT-symmetric photonic lattices: from beam rectification to dynamic localization

    CERN Document Server

    Kartashov, Yaroslav V; Konotop, Vladimir V; Torner, Lluis

    2016-01-01

    We address the propagation of light beams in longitudinally modulated PT-symmetric lattices, built as arrays of couplers with periodically varying separation between their channels, and show a number of possibilities for efficient diffraction control available in such non-conservative structures. The dynamics of light in such lattices crucially depends on the ratio of the switching length for the straight segments of each coupler and the longitudinal lattice period. Depending on the longitudinal period, one can achieve either beam rectification, when the input light propagates at a fixed angle across the structure without diffractive broadening, or dynamic localization, when the initial intensity distribution is periodically restored after each longitudinal period. Importantly, the transition between these two different propagation regimes can be achieved by tuning only gain and losses acting in the system, provided that the PT-symmetry remains unbroken. The impact of Kerr nonlinearity is also discussed.

  3. Cold beam of isotopically pure Yb atoms by deflection using 1D-optical molasses

    Science.gov (United States)

    Rathod, K. D.; Singh, P. K.; Natarajan, Vasant

    2014-09-01

    We demonstrate generation of an isotopically pure beam of laser-cooled Yb atoms by deflection using 1D-optical molasses. Atoms in a collimated thermal beam are first slowed using a Zeeman Slower. They are then subjected to a pair of molasses beams inclined at $45^\\circ$ with respect to the slowed atomic beam. The slowed atoms are deflected and probed at a distance of 160 mm. We demonstrate selective deflection of the bosonic isotope $^{174}$Yb, and the fermionic isotope $^{171}$Yb. Using a transient measurement after the molasses beams are turned on, we find a longitudinal temperature of 41 mK.

  4. Cold beam of isotopically pure Yb atoms by deflection using 1D-optical molasses

    Indian Academy of Sciences (India)

    K D Rathod; P K Singh; Vasant Natarajan

    2014-09-01

    We demonstrate the generation of an isotopically pure beam of laser-cooled Yb atoms by deflection using 1D-optical molasses. Atoms in a collimated thermal beam are first slowed using a Zeeman slower. They are then subjected to a pair of molasses beams inclined at 45° with respect to the slowed atomic beam. The slowed atoms are deflected and probed at a distance of 160 mm. We demonstrate the selective deflection of the bosonic isotope 174Yb and the fermionic isotope 171Yb. Using a transient measurement after the molasses beams are turned on, we find a longitudinal temperature of 41 mK.

  5. One Atomic Beam as a Detector of Classical Harmonic Vibrations with Micro Amplitudes and Low Frequencies

    CERN Document Server

    Wong, Werner

    2013-01-01

    We propose a simplest detector of harmonic vibrations with micro amplitudes and low frequencies, i.e. the detector consisting of one atomic beam. Here the atomic beam is induced by a plane harmonic wave and has a classical collective harmonic vibrations, which vibrant directions are perpendicular to the wave vectors of atomic beam. Compared with the detector consisting of atomic Mach-Zehnder interferometer, the new detector has two advantages: (1) it is suitable for the detection of the harmonic vibrations induced either by a longitudinal plane harmonic wave or by a transverse plane harmonic wave; (2) the quantum noise fluctuation of the atomic beam is exactly zero.

  6. Diffraction efficiency of plasmonic gratings fabricated by electron beam lithography using a silver halide film

    Science.gov (United States)

    Sudheer, Porwal, S.; Bhartiya, S.; Rao, B. T.; Tiwari, P.; Srivastava, Himanshu; Sharma, T. K.; Rai, V. N.; Srivastava, A. K.; Naik, P. A.

    2016-07-01

    The silver nanoparticle surface relief gratings of ˜10 μm period are fabricated using electron beam lithography on the silver halide film substrate. Morphological characterization of the gratings shows that the period, the shape, and the relief depth in the gratings are mainly dependent on the number of lines per frame, the spot size, and the accelerating voltage of electron beam raster in the SEM. Optical absorption of the silver nanoparticle gratings provides a broad localized surface plasmon resonance peak in the visible region, whereas the intensity of the peaks depends on the number density of silver nanoparticles in the gratings. The maximum efficiency of ˜7.2% for first order diffraction is observed for the grating fabricated at 15 keV. The efficiency is peaking at 560 nm with ˜380 nm bandwidth. The measured profiles of the diffraction efficiency for the gratings are found in close agreement with the Raman-Nath diffraction theory. This technique provides a simple and efficient method for the fabrication of plasmonic nanoparticle grating structures with high diffraction efficiency having broad wavelength tuning.

  7. Matrix isolation sublimation: An apparatus for producing cryogenic beams of atoms and molecules

    Energy Technology Data Exchange (ETDEWEB)

    Sacramento, R. L.; Alves, B. X.; Silva, B. A.; Wolff, W.; Cesar, C. L. [Instituto de Física, Universidade Federal do Rio de Janeiro, Caixa Postal 68528, 21941-972 Rio de Janeiro, RJ (Brazil); Oliveira, A. N. [Instituto de Física, Universidade Federal do Rio de Janeiro, Caixa Postal 68528, 21941-972 Rio de Janeiro, RJ (Brazil); INMETRO, Av. Nossa Senhora das Graças, 50 25250-020 Duque de Caxias, RJ (Brazil); Li, M. S. [Instituto de Física de São Carlos, Universidade de São Paulo, Ave. Trabalhador São Carlense, 400, 13565-590 São Carlos, SP (Brazil)

    2015-07-15

    We describe the apparatus to generate cryogenic beams of atoms and molecules based on matrix isolation sublimation. Isolation matrices of Ne and H{sub 2} are hosts for atomic and molecular species which are sublimated into vacuum at cryogenic temperatures. The resulting cryogenic beams are used for high-resolution laser spectroscopy. The technique also aims at loading atomic and molecular traps.

  8. Matrix isolation sublimation: An apparatus for producing cryogenic beams of atoms and molecules.

    Science.gov (United States)

    Sacramento, R L; Oliveira, A N; Alves, B X; Silva, B A; Li, M S; Wolff, W; Cesar, C L

    2015-07-01

    We describe the apparatus to generate cryogenic beams of atoms and molecules based on matrix isolation sublimation. Isolation matrices of Ne and H2 are hosts for atomic and molecular species which are sublimated into vacuum at cryogenic temperatures. The resulting cryogenic beams are used for high-resolution laser spectroscopy. The technique also aims at loading atomic and molecular traps.

  9. Combined experimental and theoretical study of fast atom diffraction on the β2(2×4) reconstructed GaAs(001) surface

    Science.gov (United States)

    Debiossac, M.; Zugarramurdi, A.; Khemliche, H.; Roncin, P.; Borisov, A. G.; Momeni, A.; Atkinson, P.; Eddrief, M.; Finocchi, F.; Etgens, V. H.

    2014-10-01

    A grazing incidence fast atom diffraction (GIFAD or FAD) setup, installed on a molecular beam epitaxy chamber, has been used to characterize the β2(2×4) reconstruction of a GaAs(001) surface at 530∘C under an As4 overpressure. Using a 400-eV 4He beam, high-resolution diffraction patterns with up to eighty well-resolved diffraction orders are observed simultaneously, providing a detailed fingerprint of the surface structure. Experimental diffraction data are in good agreement with results from quantum scattering calculations based on an ab initio projectile-surface interaction potential. Along with exact calculations, we show that a straightforward semiclassical analysis allows the features of the diffraction chart to be linked to the main characteristics of the surface reconstruction topography. Our results demonstrate that GIFAD is a technique suitable for measuring in situ the subtle details of complex surface reconstructions. We have performed measurements at very small incidence angles, where the kinetic energy of the projectile motion perpendicular to the surface can be reduced to less than 1 meV. This allowed the depth of the attractive van der Waals potential well to be estimated as -8.7 meV in very good agreement with results reported in literature.

  10. Focused Azimuthally E-Polarized Vector Beam and Spatial Magnetic Resolution below the Diffraction Limit

    CERN Document Server

    Veysi, Mehdi; Capolino, Filippo

    2016-01-01

    An azimuthally E-polarized vector beam (AEVB) has a salient feature that it contains a magnetic-dominant region within which electric field has a null and longitudinal magnetic field is maximum. Fresnel diffraction theory and plane-wave spectral (PWS) calculations are applied to quantify the field features of such a beam upon focusing through a lens. The diffraction-limited full width at half maximum (FWHM) of the beams longitudinal magnetic field intensity profile and complementary FWHM (CFWHM) of the beam's annular-shaped total electric field intensity profile are calculated at the lens's focal plane as a function of the lens's paraxial focal distance. Subsequently, we demonstrate, for the first time, that a very high resolution magnetic field at optical frequency with the total magnetic field FWHM of 0.23{\\lambda}(magnetic field spot size of 0.04{\\lambda}^2) can be achieved by placing a subwavelength dense dielectric Mie scatterer in the minimum-waist plane of a self-standing converging AEVB. The theory sh...

  11. Optimizations in angular dispersive neutron powder diffraction using divergent beam geometries

    Science.gov (United States)

    Buchsteiner, Alexandra; Stüßer, Norbert

    2009-01-01

    Angular dispersive neutron powder diffractometers are usually built using beam divergencies defined by Soller type collimators. To account for the needs of resolution for crystal structure refinement a good in-pile collimation α1, a high take-off angle above 90∘ at the monochromator and a good collimation α3 in front of the detector bank are chosen whereas the value of α2 for the collimation between monochromator and sample is less crucial. During the last years new strategies were developed at our institute using wide divergent beam geometries defined by fan collimators or slit-type diaphragms which correlate ray direction and wavelength within the beam. Here we present the performance of a newly developed fan collimator, which enables one to adjust the opening of the collimator channels on both sides independently. This fan collimator is positioned in front of the monochromator at the instrument E6 at the Helmholtz Centre Berlin (formerly Hahn-Meitner-Institut Berlin). It will be shown that control of the beam divergency allows optimization of the resolution in a large angular diffraction range. Hence the resolution and intensity can be adapted to the needs of powder diffraction. Monte Carlo simulations using McStas are used to check and prove the optimal setting of the instrument. We obtain a very good agreement between experimental and simulated data and demonstrate the superior outcome of the new instrument configuration with respect to Soller type instruments.

  12. Optimizations in angular dispersive neutron powder diffraction using divergent beam geometries

    Energy Technology Data Exchange (ETDEWEB)

    Buchsteiner, Alexandra [Helmholtz Centre Berlin for Materials and Energy, Glienicker Str. 100, D-14109 Berlin (Germany)], E-mail: buchsteiner@helmholtz-berlin.de; Stuesser, Norbert [Helmholtz Centre Berlin for Materials and Energy, Glienicker Str. 100, D-14109 Berlin (Germany)

    2009-01-11

    Angular dispersive neutron powder diffractometers are usually built using beam divergencies defined by Soller type collimators. To account for the needs of resolution for crystal structure refinement a good in-pile collimation {alpha}{sub 1}, a high take-off angle above 90 deg. at the monochromator and a good collimation {alpha}{sub 3} in front of the detector bank are chosen whereas the value of {alpha}{sub 2} for the collimation between monochromator and sample is less crucial. During the last years new strategies were developed at our institute using wide divergent beam geometries defined by fan collimators or slit-type diaphragms which correlate ray direction and wavelength within the beam. Here we present the performance of a newly developed fan collimator, which enables one to adjust the opening of the collimator channels on both sides independently. This fan collimator is positioned in front of the monochromator at the instrument E6 at the Helmholtz Centre Berlin (formerly Hahn-Meitner-Institut Berlin). It will be shown that control of the beam divergency allows optimization of the resolution in a large angular diffraction range. Hence the resolution and intensity can be adapted to the needs of powder diffraction. Monte Carlo simulations using McStas are used to check and prove the optimal setting of the instrument. We obtain a very good agreement between experimental and simulated data and demonstrate the superior outcome of the new instrument configuration with respect to Soller type instruments.

  13. Focused azimuthally polarized vector beam and spatial magnetic resolution below the diffraction limit

    Science.gov (United States)

    Veysi, Mehdi; Guclu, Caner; Capolino, Filippo

    2016-11-01

    An azimuthally electric-polarized vector beam (APB), with a polarization vortex, has a salient feature that it contains a magnetic-dominant region within which electric field ideally has a null while longitudinal magnetic field is maximum. Fresnel diffraction theory and plane-wave spectral (PWS) calculations are applied to quantify field features of such a beam upon focusing through a lens. The diffraction-limited full width at half maximum (FWHM) of the beam's longitudinal magnetic field intensity profile and complementary FWHM (CFWHM) of the beam's annular-shaped total electric field intensity profile are examined at the lens's focal plane as a function of the lens's paraxial focal distance. Then, we place a subwavelength dense dielectric Mie scatterer in the minimum-waist plane of a self-standing converging APB and demonstrate for the first time that a very high resolution magnetic field at optical frequency is achieved with total magnetic field FWHM of 0.23{\\lambda} (i.e., magnetic field spot area of 0.04{\\lambda}^2) within a magnetic-dominant region. The theory shown here is valuable for development of optical microscopy and spectroscopy systems based on magnetic dipolar transitions which are in general much weaker than their electric counterparts.

  14. Computer simulations of X-ray six-beam diffraction in a perfect silicon crystal. I.

    Science.gov (United States)

    Kohn, V G; Khikhlukha, D R

    2016-05-01

    This paper reports computer simulations of the transmitted-beam intensity distribution for the case of six-beam (000, 220, 242, 044, -224, -202) diffraction of X-rays in a perfect silicon crystal of thickness 1 mm. Both the plane-wave angular dependence and the six-beam section topographs, which are usually obtained in experiments with a restricted beam (two-dimensional slit), are calculated. The angular dependence is calculated in accordance with Ewald's theory. The section topographs are calculated from the angular dependence by means of the fast Fourier transformation procedure. This approach allows one to consider, for the first time, the transformation of the topograph's structure due to the two-dimensional slit sizes and the distance between the slit and the detector. The results are in good agreement with the results of other works and with the experimental data. This method of calculation does not require a supercomputer and it was performed on a standard laptop. A detailed explanation of the main features of the diffraction patterns at different distances between the slit and the detector is presented.

  15. Atomic structure of a single large biomolecule from diffraction patterns of random orientations

    CERN Document Server

    Tegze, Miklós

    2012-01-01

    The short and intense pulses of the new X-ray free electron lasers, now operational or under construction, may make possible diffraction experiments on single molecule-sized objects with high resolution, before radiation damage destroys the sample. In a single molecule imaging (SMI) experiment thousands of diffraction patterns of single molecules with random orientations are recorded. One of the most challenging problems of SMI is how to assemble these noisy patterns of unknown orientations into a consistent single set of diffraction data. Here we present a new method which can solve the orientation problem of SMI efficiently even for large biological molecules and in the presence of noise. We show on simulated diffraction patterns of a large protein molecule, how the orientations of the patterns can be found and the structure to atomic resolution can be solved. The concept of our algorithm could be also applied to experiments where images of an object are recorded in unknown orientations and/or positions lik...

  16. Estimated H-atom anisotropic displacement parameters: a comparison between different methods and with neutron diffraction results

    DEFF Research Database (Denmark)

    Munshi, Parthapratim; Madsen, Anders Ø; Spackman, Mark A;

    2008-01-01

    Anisotropic displacement parameters (ADPs) are compared for H atoms estimated using three recently described procedures, both among themselves and with neutron diffraction results. The results convincingly demonstrate that all methods are capable of giving excellent results for several benchmark...

  17. Measurement of Velocity Distribution in Atomic Beam by Diode Laser with Narrow Line width

    Institute of Scientific and Technical Information of China (English)

    CHEN Jingbiao; WANG Fengzhi; YANG Donghai; WANG YiQiu

    2001-01-01

    In this paper, by using the detecting laser beam interacts with the atomic beam at a sharp angle and the Doppler frequency shift effect, the velocity distribution in cesium atomic beam is measured with a diode laser of narrow linewidth of 1 MHz. The effects of the atomic natural line width and cycling transition detecting factor on the measured results have been analyzed. Finally, the measured results have been compared with the theoretical calculation.

  18. An atomic beam source for fast loading of a magneto-optical trap under high vacuum

    DEFF Research Database (Denmark)

    McDowall, P.D.; Hilliard, Andrew; Grünzweig, T.;

    2012-01-01

    We report on a directional atomic beam created using an alkali metal dispenser and a nozzle. By applying a high current (15 A) pulse to the dispenser at room temperature we can rapidly heat it to a temperature at which it starts dispensing, avoiding the need for preheating. The atomic beam produced...... is capable of loading 90 of a magneto-optical trap (MOT) in less than 7 s while maintaining a low vacuum pressure of 10 -11 Torr. The transverse velocity components of the atomic beam are measured to be within typical capture velocities of a rubidium MOT. Finally, we show that the atomic beam can be turned...

  19. The wave energy flux of high frequency diffracting beams in complex geometrical optics

    Science.gov (United States)

    Maj, Omar; Mariani, Alberto; Poli, Emanuele; Farina, Daniela

    2013-04-01

    We consider the construction of asymptotic solutions of Maxwell's equations for a diffracting wave beam in the high frequency limit and address the description of the wave energy flux transported by the beam. With this aim, the complex eikonal method is applied. That is a generalization of the standard geometrical optics method in which the phase function is assumed to be complex valued, with the non-negative imaginary part accounting for the finite width of the beam cross section. In this framework, we propose an argument which simplifies significantly the analysis of the transport equation for the wave field amplitude and allows us to derive the wave energy flux. The theoretical analysis is illustrated numerically for the case of electron cyclotron beams in tokamak plasmas by using the GRAY code [D. Farina, Fusion Sci. Technol. 52, 154 (2007)], which is based upon the complex eikonal theory. The results are compared to those of the paraxial beam tracing code TORBEAM [E. Poli et al., Comput. Phys. Commun. 136, 90 (2001)], which provides an independent calculation of the energy flow.

  20. The wave energy flux of high frequency diffracting beams in complex geometrical optics

    Energy Technology Data Exchange (ETDEWEB)

    Maj, Omar; Poli, Emanuele [Max Planck Institute for Plasma Physics, EURATOM Association, Boltzmannstr. 2, 85748 Garching (Germany); Mariani, Alberto [Istituto di Fisica del Plasma ' P. Caldirola,' Consiglio Nazionale delle Ricerche, EURATOM-ENEA-CNR Association, via R. Cozzi 53, I-20125 Milano (Italy); Universita degli Studi di Milano, Dipartimento di Fisica, Via Celoria 16, 20133 Milano (Italy); Farina, Daniela [Istituto di Fisica del Plasma ' P. Caldirola,' Consiglio Nazionale delle Ricerche, EURATOM-ENEA-CNR Association, via R. Cozzi 53, I-20125 Milano (Italy)

    2013-04-15

    We consider the construction of asymptotic solutions of Maxwell's equations for a diffracting wave beam in the high frequency limit and address the description of the wave energy flux transported by the beam. With this aim, the complex eikonal method is applied. That is a generalization of the standard geometrical optics method in which the phase function is assumed to be complex valued, with the non-negative imaginary part accounting for the finite width of the beam cross section. In this framework, we propose an argument which simplifies significantly the analysis of the transport equation for the wave field amplitude and allows us to derive the wave energy flux. The theoretical analysis is illustrated numerically for the case of electron cyclotron beams in tokamak plasmas by using the GRAY code [D. Farina, Fusion Sci. Technol. 52, 154 (2007)], which is based upon the complex eikonal theory. The results are compared to those of the paraxial beam tracing code TORBEAM [E. Poli et al., Comput. Phys. Commun. 136, 90 (2001)], which provides an independent calculation of the energy flow.

  1. Neutron diffraction of titanium aluminides formed by continuous electron-beam treatment

    Science.gov (United States)

    Valkov, S.; Neov, D.; Luytov, D.; Petrov, P.

    2016-03-01

    Ti-Al-based alloys were produced by hybrid electron-beam technologies. A composite Ti-Al film was deposited on a Ti substrate by electron-beam evaporation (EBE), followed by electron-beam treatment (EBT) by a continuously scanned electron beam. The speed of the specimens motion during the EBT were V 1 = 1 cm/sec and V 2 = 5 cm/sec, in order to realize two different alloying mechanisms -- by surface melting and by electron-beam irradiation without melting the surface. The samples prepared were characterized by XRD and neutron diffraction to study the crystal structure on the surface and in depth. SEM/EDX analysis was conducted to explore the surface structure and analyze the chemical composition. Nanoindentation measurements were also carried out. No intermetallic phases were registered in the sample treated at velocity V 1, while the sample treated at V 2 exhibited a Ti3Al/TiAl structure on the surface, transformed to Ti/TiAl in depth. The nanoindentation test demonstrated a significant negative hardness gradient from the surface to the depth of the sample.

  2. Convergent beam electron diffraction study on ge-based oxide spinels

    Energy Technology Data Exchange (ETDEWEB)

    Ikeda, S I; Umeyama, N [Nanoelectronics Research Institute, AIST, Tsukuba (Japan); Matsuhata, H [Energy Semiconductor Electronics Research Laboratory, AIST, Tsukuba (Japan); Tominaga, A; Sato, H [Department of Physics, Chuo University, Tokyo (Japan); Hara, S [Art, Science and Technology Center for Cooperative Research, Kyushu University, Fukuoka (Japan); Watanabe, T [Department of Physics, Nihon University, Tokyo (Japan); Tomiyasu, K [IMR, Tohoku University, Sendai (Japan); Crawford, M K, E-mail: ikeda-shin@aist.go.j [DuPont Co., Wilmington, Delaware (United States)

    2009-03-01

    Transition metal oxides with spinel crystal structure exhibit intriguing and non trivial magnetic phenomena owing to magnetic frustration between spins having antiferromagnetic coupling interaction on triangle or kagome lattice. GeCo{sub 2}O{sub 4}(GCO) and GeNi{sub 2}O{sub 4}(GNO), which belong to above category, are very rare normal spinels containing Ge ion. Both reveal antiferromagnetic-like phase transitions at 20 K and 12 K, respectively. According to previous neutron and x-ray diffraction measurements, GNO keeps its cubic structural symmetry down to 2 K which is not natural because such a magnetic transition tends to associate with symmetry breaking structural transitions. In order to know whether the structural transition or symmetry change occur or not at the magnetic transition in detail, convergent beam electron diffraction measurements is employed for the compounds.

  3. Atomic layer deposition ultrathin film origami using focused ion beams

    Science.gov (United States)

    Supekar, O. D.; Brown, J. J.; Eigenfeld, N. T.; Gertsch, J. C.; Bright, V. M.

    2016-12-01

    Focused ion beam (FIB) micromachining is a powerful tool for maskless lithography and in recent years FIB has been explored as a tool for strain engineering. Ion beam induced deformation can be utilized as a means for folding freestanding thin films into complex 3D structures. FIB of high energy gallium (Ga+) ions induces stress by generation of dislocations and ion implantation within material layers, which create creases or folds upon mechanical relaxation enabled by motion of the material layers. One limitation on such processing is the ability to fabricate flat freestanding thin film structures. This capability is limited by the residual stresses formed during processing and fabrication of the films, which can result in initial curvature and deformation of films upon release from a sacrificial fabrication layer. This paper demonstrates folding in freestanding ultrathin films (1:1000) by ion-induced stress relaxation. The ultrathin flat structures are fabricated using atomic layer deposition on sacrificial polyimide. We have demonstrated vertical folding with 30 keV Ga+ ions in structures with lateral dimensions varying from 10 to 50 μm.

  4. Evolution of the phase singularities in edge-diffracted optical-vortex beams

    CERN Document Server

    Bekshaev, Aleksandr; Chernykh, Aleksey; Khoroshun, Anna

    2016-01-01

    We study, both theoretically and by experiment, migration of the amplitude zeros within a fixed cross section of the edge-diffracted optical-vortex beam, when the screen edge performs permanent translation in the transverse plane from the beam periphery towards the axis. Generally, the amplitude zeros (optical-vortex cores) describe spiral-like trajectories. When the screen edge advances uniformly, the motion of the amplitude zeros is not smooth and sometimes shows anomalously high rates, which make an impression of instantaneous "jumps" from one position to another. We analyze the nature, conditions and mechanism of these jumps and show that they are associated with the "birth - annihilation" topological reactions involving the optical vortex dipoles.

  5. Two-dimensional analytic modeling of acoustic diffraction for ultrasonic beam steering by phased array transducers.

    Science.gov (United States)

    Wang, Tiansi; Zhang, Chong; Aleksov, Aleksandar; Salama, Islam; Kar, Aravinda

    2017-04-01

    Phased array ultrasonic transducers enable modulating the focal position of the acoustic waves, and this capability is utilized in many applications, such as medical imaging and non-destructive testing. This type of transducers also provides a mechanism to generate tilted wavefronts in acousto-optic deflectors to deflect laser beams for high precision advanced laser material processing. In this paper, a theoretical model is presented for the diffraction of ultrasonic waves emitted by several phased array transducers into an acousto-optic medium such as TeO2 crystal. A simple analytic expression is obtained for the distribution of the ultrasonic displacement field in the crystal. The model prediction is found to be in good agreement with the results of a numerical model that is based on a non-paraxial multi-Gaussian beam (NMGB) model.

  6. Diffraction Radiation Diagnostics for Moderate to High Energy Charged Particle Beams

    CERN Document Server

    Fiorito, R B

    2001-01-01

    Diffraction radiation (DR) is produced when a charged particle passes throughan aperture or near a discontinuity in the media in which it is traveling. DRis closely related to transition radiation (TR), which is produced when acharged particle traverses the boundary between media with different dielectricconstants. In contrast to TR, which is now extensively used for beam diagnosticpurposes, the potential of DR as a non-interceptive, multi-parameter beamdiagnostic remains largely undeveloped. For diagnostic measurements it isuseful to observe backward reflected DR from an circular aperture or slitinclined with respect to the beam velocity. However, up to now, well foundedequations for the spectral-angular intensities of backward DR from suchapertures have not been available. We present a new derivation of the spectralangular intensity of backward DR produced from an inclined slit for twoorientations of the slit axis, i.e. perpendicular and parallel to the plane ofincidence. Our mathematical approach is genera...

  7. Radiation damage free two-color X-ray ghost diffraction with atomic resolution

    CERN Document Server

    Li, Zheng; Chapman, Henry; Shih, Yanhua

    2015-01-01

    The X-ray free electron lasers (XFEL) can enable diffractive structural determination of protein crystals or single molecules that are too small and radiation-sensitive for conventional X-ray analysis. However the electronic form factor could have been modified during the ultrashort X-ray pulse due to photoionization and electron cascade caused by the intense X-ray pulse. For general X-ray imaging techniques, to minimize radiation damage effect is of major concern to ensure faithful reconstruction of the structure. Here we show that a radiation damage free diffraction can be achieved with an atomic spatial resolution, by using X-ray parametric down-conversion (PDC), and two-color biphoton ghost imaging. We illustrate that formation of the diffractive patterns satisfies a condition analogous to the Bragg equation, with a resolution that could be as fine as the lattice length scale of several Angstrom. Because the samples are illuminated by the optical photons of low energy, they can be free of radiation damage...

  8. Development of atomic-beam resonance method to measure the nuclear moments of unstable nuclei

    Energy Technology Data Exchange (ETDEWEB)

    Sugimoto, T., E-mail: sugimoto@ribf.riken.jp [SPring-8 (Japan); Asahi, K. [Tokyo Institute of Technology, Department of Physics (Japan); Kawamura, H.; Murata, J. [Rikkyo University, Department of Physics (Japan); Nagae, D.; Shimada, K. [Tokyo Institute of Technology, Department of Physics (Japan); Ueno, H.; Yoshimi, A. [RIKEN Nishina Center (Japan)

    2008-01-15

    We have been working on the development of a new technique of atomic-beam resonance method to measure the nuclear moments of unstable nuclei. In the present study, an ion-guiding system to be used as an atomic-beam source have been developed.

  9. Nano-modulated electron beams via electron diffraction and emittance exchange for coherent x-ray generation

    CERN Document Server

    Nanni, Emilio A; Moncton, David E

    2015-01-01

    A new method for generation of relativistic electron beams with current modulations at nanometer scale and below is presented. The current modulation is produced by diffracting relativistic electrons in perfect crystal Si, accelerating the diffracted beam and imaging the crystal structure, then transferring the image into the temporal dimension via emittance exchange. The modulation period can be tuned by adjusting electron optics after diffraction. This tunable longitudinal modulation can have a period as short as a few angstroms, enabling production of coherent hard x-rays from a device based on inverse Compton scattering with total length of a few meters. Electron beam simulations from cathode emission through diffraction, acceleration and image formation with variable magnification are presented along with estimates of the coherent x-ray output properties.

  10. Multiobjective optimizations of a novel cryocooled dc gun based ultrafast electron diffraction beam line

    Science.gov (United States)

    Gulliford, Colwyn; Bartnik, Adam; Bazarov, Ivan

    2016-09-01

    We present the results of multiobjective genetic algorithm optimizations of a single-shot ultrafast electron diffraction beam line utilizing a 225 kV dc gun with a novel cryocooled photocathode system and buncher cavity. Optimizations of the transverse projected emittance as a function of bunch charge are presented and discussed in terms of the scaling laws derived in the charge saturation limit. Additionally, optimization of the transverse coherence length as a function of final rms bunch length at the sample location have been performed for three different sample radii: 50, 100, and 200 μ m , for two final bunch charges: 1 05 electrons (16 fC) and 1 06 electrons (160 fC). Example optimal solutions are analyzed, and the effects of disordered induced heating estimated. In particular, a relative coherence length of Lc ,x/σx=0.27 nm /μ m was obtained for a final bunch charge of 1 05 electrons and final bunch length of σt≈100 fs . For a final charge of 1 06 electrons the cryogun produces Lc ,x/σx≈0.1 nm /μ m for σt≈100 - 200 fs and σx≥50 μ m . These results demonstrate the viability of using genetic algorithms in the design and operation of ultrafast electron diffraction beam lines.

  11. Grazing incidence collisions of ions and atoms with surfaces: from charge exchange to atomic diffraction; Collisions rasantes d'ions ou d'atomes sur les surfaces: de l'echange de charge a la diffraction atomique

    Energy Technology Data Exchange (ETDEWEB)

    Rousseau, P

    2006-09-15

    This thesis reports two studies about the interaction with insulating surfaces of keV ions or atoms under grazing incidence. The first part presents a study of charge exchange processes occurring during the interaction of singly charged ions with the surface of NaCl. In particular, by measuring the scattered charge fraction and the energy loss in coincidence with electron emission, the neutralization mechanism is determined for S{sup +}, C{sup +}, Xe{sup +}, H{sup +}, O{sup +}, Kr{sup +}, N{sup +}, Ar{sup +}, F{sup +}, Ne{sup +} and He{sup +}. These results show the importance of the double electron capture as neutralization process for ions having too much potential energy for resonant capture and not enough for Auger neutralization. We have also studied the ionisation of the projectile and of the surface, and the different Auger-like neutralization processes resulting in electron emission, population of conduction band or excited state. For oxygen scattering, we have measured an higher electron yield in coincidence with scattered negative ion than with scattered atom suggesting the transient formation above the surface of the oxygen doubly negative ion. The second study deals with the fast atom diffraction, a new phenomenon observed for the first time during this work. Due to the large parallel velocity, the surface appears as a corrugated wall where rows interfere. Similarly to the Thermal Atom Scattering the diffraction pattern corresponds to the surface potential and is sensitive to vibrations. We have study the H-NaCl and He-LiF atom-surface potentials in the 20 meV - 1 eV range. This new method offers interesting perspectives for surface characterisation. (author)

  12. The effect of atoms excited by electron beam on metal evaporation

    CERN Document Server

    Xie Guo Feng; Ying Chun Tong

    2002-01-01

    In atomic vapor laser isotope separation (AVLIS), the metal is heated to melt by electron beams. The vapor atoms may be excited by electrons when flying through the electron beam. The excited atoms may be deexcited by inelastic collision during expansion. The electronic energy transfers translational energy. In order to analyse the effect of reaction between atoms and electron beams on vapor physical parameters, such as density, velocity and temperature, direct-simulation Monte Carlo method (DSMC) is used to simulate the 2-D gadolinium evaporation from long and narrow crucible. The simulation results show that the velocity and temperature of vapor increase, and the density decreases

  13. Velocity distribution measurements in atomic beams generated using laser induced back-ablation

    CERN Document Server

    Denning, A; Lee, S; Ammonson, M; Bergeson, S D

    2008-01-01

    We present measurements of the velocity distribution of calcium atoms in an atomic beam generated using a dual-stage laser back-ablation apparatus. Distributions are measured using a velocity selective Doppler time-of-flight technique. They are Boltzmann-like with rms velocities corresponding to temperatures above the melting point for calcium. Contrary to a recent report in the literature, this method does not generate a sub-thermal atomic beam.

  14. The Possibility of Noninvasive Micron High Energy Electron Beam Size Measurement Using Diffraction Radiation

    CERN Document Server

    Naumenko, Gennady; Aryshev, Alexander; Cline, David B; Fukui, Yasuo; Hamatsu, Ryosuke; Hayano, Hitoshi; Karataev, Pavel; Muto, Toshiya; Potylitsyn, Alexander; Ross, Marc; Urakawa, Junji

    2005-01-01

    During the last years a noninvasive method for beam size measurement based on the optical diffraction radiation (ODR) has been in progress (P. Karataev, et al., Physical Review Letters 93, 244802 (2004). However this technique encounters with hard sensitivity limitation for electron energies larger than several GeV. For example, for SLAC conditions the sensitivity of this method is 4 orders smaller than an appropriate one. We suggest to use a "dis-phased" slit target, where two semi-planes are turned with respect to each other at a small "dis-phased" angle. In order to ensure the interference between the diverged radiation beams we use a cylindrical lens. This method has much better sensitivity and resolution. A "dis-phased" angle 10 milliradians gives the optimal sensitivity to 5 microns transversal beam size. The theoretical model for calculating the ODR radiation from such targets (including focusing by cylindrical lens) is presented. It is shown that the sensitivity of this method does not depend on the L...

  15. Atomic structure of "multilayer silicene" grown on Ag(111): Dynamical low energy electron diffraction analysis

    Science.gov (United States)

    Kawahara, Kazuaki; Shirasawa, Tetsuroh; Lin, Chun-Liang; Nagao, Ryo; Tsukahara, Noriyuki; Takahashi, Toshio; Arafune, Ryuichi; Kawai, Maki; Takagi, Noriaki

    2016-09-01

    We have investigated the atomic structure of the "multilayer silicene" grown on the Ag(111) single crystal surface by using low energy electron diffraction (LEED) and scanning tunneling microscopy (STM). We measured the intensity of the LEED spot as a function of the incident electron energy (I-V curve) and analyzed the I-V curve using a dynamical LEED theory. We have found that the Si(111)(√{ 3} ×√{ 3})-Ag model well reproduces the I-V curve whereas the models consisting of the honeycomb structure of Si do not. The bias dependence of the STM image of multilayer silicene agrees with that of the Si(111)(√{ 3} ×√{ 3})-Ag reconstructed surface. Consequently, we have concluded that the multilayer silicene grown on Ag(111) is identical to the Si(111)(√{ 3} ×√{ 3})-Ag reconstructed structure.

  16. Metastable states' population of uranium atoms produced by electron-beam heating

    Energy Technology Data Exchange (ETDEWEB)

    Ohba, Hironori; Shibata, Takemasa [Japan Atomic Energy Research Inst., Tokai, Ibaraki (Japan). Tokai Research Establishment; Nishimura, Akihiko; Ogura, Koichi [Japan Atomic Energy Research Inst., Kansai Research Establishment, Advanced Photon Research Center, Kyoto (Japan)

    2000-08-01

    The metastable states' population densities of uranium atoms produced by electron-beam heating were measured by the laser induced fluorescence method. The atomic excitation temperature derived from the metastable state distribution was lower than the evaporation surface temperature. With increasing deposition rate, the atomic excitation temperature decreased to about 2000 K. (author)

  17. Generation of a cold pulsed beam of Rb atoms by transfer from a 3D magneto-optic trap

    CERN Document Server

    Chanu, Sapam Ranjita; Natarajan, Vasant

    2016-01-01

    We demonstrate a technique for producing a cold pulsed beam of atoms by transferring a cloud of atoms trapped in a three dimensional magneto-optic trap (MOT). The MOT is loaded by heating a getter source of Rb atoms. We show that it is advantageous to transfer with two beams (with a small angle between them) compared to a single beam, because the atoms stop interacting with the beams in the two-beam technique, which results in a Gaussian velocity distribution. The atoms are further cooled in optical molasses by turning off the MOT magnetic field before the transfer beams are turned on.

  18. Quantum coherent tractor beam effect for atoms trapped near a nanowaveguide

    Science.gov (United States)

    Sadgrove, Mark; Wimberger, Sandro; Nic Chormaic, Síle

    2016-01-01

    We propose several schemes to realize a tractor beam effect for ultracold atoms in the vicinity of a few-mode nanowaveguide. Atoms trapped near the waveguide are transported in a direction opposite to the guided mode propagation direction. We analyse three specific examples for ultracold 23Na atoms trapped near a specific nanowaveguide (i.e. an optical nanofibre): (i) a conveyor belt-type tractor beam effect, (ii) an accelerator tractor beam effect, and (iii) a quantum coherent tractor beam effect, all of which can effectively pull atoms along the nanofibre toward the light source. This technique provides a new tool for controlling the motion of particles near nanowaveguides with potential applications in the study of particle transport and binding as well as atom interferometry. PMID:27440516

  19. Development of a prompt gamma activation analysis facility using diffracted polychromatic neutron beam

    CERN Document Server

    Byun, S H; Choi, H D

    2002-01-01

    A prompt gamma activation analysis facility has recently been developed at Hanaro, the 24 MW research reactor in the Korea Atomic Energy Research Institute. Polychromatic thermal neutrons are extracted by setting pyrolytic graphite crystals at a Bragg angle of 45 deg. . The detection system comprises a large single n-type HPGe detector, signal electronics and a fast ADC. Neutron beam characterization was performed both theoretically and experimentally. The neutron flux was measured to be 7.9x10 sup 7 n/cm sup 2 s in a 1x1 cm sup 2 beam area at the sample position with a uniformity of 12%. The corresponding Cd-ratio for gold was found to be 266. The beam quality was compared with other representative thermal neutron prompt gamma activation analysis. The detection efficiency was calibrated up to 11 MeV using a set of radionuclides and the (n,gamma) reactions of N and Cl. Finally, the sensitivities and the detection limits were obtained for several elements.

  20. Fast spatial beam shaping by acousto-optic diffraction for 3D non-linear microscopy.

    Science.gov (United States)

    Akemann, Walther; Léger, Jean-François; Ventalon, Cathie; Mathieu, Benjamin; Dieudonné, Stéphane; Bourdieu, Laurent

    2015-11-01

    Acousto-optic deflection (AOD) devices offer unprecedented fast control of the entire spatial structure of light beams, most notably their phase. AOD light modulation of ultra-short laser pulses, however, is not straightforward to implement because of intrinsic chromatic dispersion and non-stationarity of acousto-optic diffraction. While schemes exist to compensate chromatic dispersion, non-stationarity remains an obstacle. In this work we demonstrate an efficient AOD light modulator for stable phase modulation using time-locked generation of frequency-modulated acoustic waves at the full repetition rate of a high power laser pulse amplifier of 80 kHz. We establish the non-local relationship between the optical phase and the generating acoustic frequency function and verify the system for temporal stability, phase accuracy and generation of non-linear two-dimensional phase functions.

  1. Focusing a beam beyond the diffraction limit using a hyperlens-based device

    Institute of Scientific and Technical Information of China (English)

    Zheng Guo-Xing; Zhang Rui-Ying; Li Song; He Ping-An; Zhou Hui

    2011-01-01

    A super-focusing device composed of a focusing objective and a hyperlens is proposed to focus an incident plane wave into the deep subwavelength dimension. In the device,the objective converts the incident plane wave into a convergent one.The half cylindrical hyperlens can support high wave vector k modes propagating towards its core.So the convergent wave can be focused into an ultrasmall spot beyond the diffraction limit.The layout is proposed for the super-focusing device and its characteristics are investigated theoretically.Numerical simulations verify that the focused beams are confined in a spot with a diameter of 16.3 nm in the focal plane of the focusing objective with a numerical aperture of 0.6,which corresponds to a super-resolution spot of λ0/23 (λ0 is the wavelength in vacuum).The simulations confirm the effectiveness of the proposed device.

  2. Beam shaping for multicolour light-emitting diodes with diffractive optical elements

    KAUST Repository

    Yu, Chao

    2016-10-06

    An improved particle swarm optimization method is proposed for the design of ultra-thin diffractive optical elements (DOEs) enabling multicolour beam shaping functionality. We employ pre-optimized initial structures and adaptive weight strategy in the algorithm to achieve better and identical shaping performance for multiple colours. Accordingly, a DOE for shaping light from green and blue LEDs has been designed and fabricated. Both experiment and numerical simulations have been conducted and the results agree well with each other. 15.66% average root mean square error (RMSE) and 0.22% RMSE difference are achieved. In addition, the parameters closely related to the performance of the optimization are analysed, which can provide insights for future application designs.

  3. Time-Resolved Diffraction Profiles and Atomic Dynamics in Short-Pulse Laser-Induced Structural Transformations: Molecular Dynamics Study

    Science.gov (United States)

    2006-05-16

    clearly reflected in the evolution of the structure function. In just 3–4 ps the peaks characteristic of the fcc structure dis- appear and the structure...apparent in the figure. The diffraction peaks from 111 and 311 atomic planes, present in the original fcc structure , shift in the direction of smaller Q...the fcc crystalline structure. Each peak in Gr corresponds to a specific interatomic distance between a pair of atoms in a perfect fcc structure . For

  4. Superresolution far-field diffraction spot in the free-space laser communication system due to radially polarized beam

    Science.gov (United States)

    Wang, Chao; Jiang, Lun; Hu, Yuan; Liu, Zhuang; Li, Ying-chao; Wang, Le

    2016-10-01

    In the free-space laser communication, there is a strong need for a technology that can decrease the size of the diffraction spot in the receiver port, because a smaller diffraction spot in the receive port makes the transmit data more secure. In this paper, instead of the usage of the larger size aperture lens in the free-space laser communication system, we introduce a diffractive superresolution technology that changing the received information laser beam into radially polarized beam which is focused on the detector array. In the paper, firstly, the conversion method of the information natural light which the optical antenna received to the radially polarized beam is discussed in detail. Then, in the focal plane, the transverse intensity distribution expression near the focal point for the radially polarized laser beam are presented, and the numerical simulation results of the intensity distributions around the focal point on different numerical apertures (NA) are given. The full width at half-maximum (FWHM) values of the main lobe are considered for the standard of the spot size. Through a comparison of the focal point FWHM values with the natural light and radially polarized beam, we judge the superresolution performance of the receiver optical system with radially polarized beam on different NA of 0.4, 0.6 and 0.75. We find that the method of focusing with radially polarized beam generates a smaller spot size than the Airy spot size when the NA is no less than 0.6; when the NA reach to 0.75, the resolution is 1.5 times than the diffraction limit. But it will decrease the light power in the process of natural light converted to radially polarized beam. When the communication laser is polarized laser, the energy loss can be reduced to around 20%. This technology can be applied when the laser energy is not the main concern in the communication.

  5. Development of francium atomic beam for the search of the electron electric dipole moment

    Directory of Open Access Journals (Sweden)

    Sato Tomoya

    2014-03-01

    Full Text Available For the measurement of the electron electric dipole moment using Fr atoms, a Fr ion-atom conversion is one of the most critical process. An ion-atom converter based on the “orthotropic” type of Fr source has been developed. This converter is able to convert a few keV Fr ion beam to a thermal atomic beam using a cycle of the surface ionization and neutralization. In this article, the development of the converter is reported.

  6. Multiobjective optimization design of an rf gun based electron diffraction beam line

    Science.gov (United States)

    Gulliford, Colwyn; Bartnik, Adam; Bazarov, Ivan; Maxson, Jared

    2017-03-01

    Multiobjective genetic algorithm optimizations of a single-shot ultrafast electron diffraction beam line comprised of a 100 MV /m 1.6-cell normal conducting rf (NCRF) gun, as well as a nine-cell 2 π /3 bunching cavity placed between two solenoids, have been performed. These include optimization of the normalized transverse emittance as a function of bunch charge, as well as optimization of the transverse coherence length as a function of the rms bunch length of the beam at the sample location for a fixed charge of 1 06 electrons. Analysis of the resulting solutions is discussed in terms of the relevant scaling laws, and a detailed description of one of the resulting solutions from the coherence length optimizations is given. For a charge of 1 06 electrons and final beam sizes of σx≥25 μ m and σt≈5 fs , we found a relative coherence length of Lc ,x/σx≈0.07 using direct optimization of the coherence length. Additionally, based on optimizations of the emittance as a function of final bunch length, we estimate the relative coherence length for bunch lengths of 30 and 100 fs to be roughly 0.1 and 0.2 nm /μ m , respectively. Finally, using the scaling of the optimal emittance with bunch charge, for a charge of 1 05 electrons, we estimate relative coherence lengths of 0.3, 0.5, and 0.92 nm /μ m for final bunch lengths of 5, 30 and 100 fs, respectively.

  7. Raman - Nath approximation for diffraction of atoms in the laser field taking into account spontaneous emission of atoms for ground and high energy level

    Science.gov (United States)

    Hovhannisayan, L.; Muradyan, A. Zh

    2012-03-01

    The problem of resonant Kapitza - Dirac diffraction is solved in Raman - Nath approximation out of familiar Bessel function approximation (applicable in zero and very large resonance detuning cases). It shows new and promising results for the atom optics and atom interferometry if the atomic momentum state has been prepared in a form of discrete Gaussian distribution. Namely, instead of monotonic broadening within the Bessel function approximation, our formula yields in splitting of initial distribution into two identical peaks, whith preserving form, which symmetrically move away from the distribution center for the interaction time. A table-shaped form for the ultimate momentum distribution also is in frame of new distributions. As to relaxation processes, they have only quantitative influence on the pattern of diffraction.

  8. Summary of informal workshop on state of ion beam facilities for atomic physics research

    Energy Technology Data Exchange (ETDEWEB)

    Jones, K.W.; Cocke, C.L.; Datz, S.; Kostroun, V.

    1984-11-13

    The present state of ion beam facilities for atomic physics research in the United States is assessed by means of a questionnaire and informal workshop. Recommendations for future facilities are given. 3 refs.

  9. Particle beam technology for control of atomic-bonding state in materials

    Energy Technology Data Exchange (ETDEWEB)

    Ishikawa, Junzo [Kyoto Univ. (Japan). Faculty of Engineering

    1997-03-01

    The atomic-bonding state in materials can be controlled through `kinetic bonding` process by energetic particle beams which have a sufficient atomic kinetic energy. In order to clarify the `kinetic bonding` process the negative-ion beam deposition is considered as an ideal method because the negative ion has no additional active energies. Sputter type heavy negative-ion sources can be used for this purpose. Carbon films prepared by carbon negative-ion beam deposition have a strong dependency of the film properties on ion beam kinetic energy and have a quite high thermal conductivity which is comparable to that of the IIb diamond at a kinetic energy of 50-100 eV/atom. It suggests that new or metastable materials could be formed through the `kinetic bonding` process. Negative-ion beams can also be used for ion implantation, in which charging problems are perfectly reduced. (author)

  10. Examination of Short- and Long-Range Atomic Order Nanocrystalline SiC and Diamond by Powder Diffraction Methods

    Science.gov (United States)

    Palosz, B.; Grzanka, E.; Stelmakh, S.; Gierlotka, S.; Weber, H.-P.; Proffen, T.; Palosz, W.

    2002-01-01

    The real atomic structure of nanocrystals determines unique, key properties of the materials. Determination of the structure presents a challenge due to inherent limitations of standard powder diffraction techniques when applied to nanocrystals. Alternate methodology of the structural analysis of nanocrystals (several nanometers in size) based on Bragg-like scattering and called the "apparent lattice parameter" (alp) is proposed. Application of the alp methodology to examination of the core-shell model of nanocrystals will be presented. The results of application of the alp method to structural analysis of several nanopowders were complemented by those obtained by determination of the Atomic Pair Distribution Function, PDF. Based on synchrotron and neutron diffraction data measured in a large diffraction vector of up to Q = 25 Angstroms(exp -1), the surface stresses in nanocrystalline diamond and SiC were evaluated.

  11. Magnetic focusing of cold atomic beam with a 2D array of current-carrying wires

    Institute of Scientific and Technical Information of China (English)

    Yang Liu; Min Yun; Jianping Yin

    2006-01-01

    @@ A new scheme to realize a two-dimensional (2D) array of magnetic micro-lenses for a cold atomic beam,formed by an array of square current-carrying wires,is proposed.We calculate the spatial distributions of the magnetic fields from the array of current-carrying wires and the magnetic focusing potential for cold rubidium atoms,and study the dynamic focusing processes of cold atoms passing through the magnetic micro-lens array and its focusing properties by using Monte-Carlo simulations and trajectory tracing method.The result shows that the proposed micro-lens array can be used to focus effectively a cold atomic beam,even to load ultracold atoms or a BEC sample into a 2D optical lattice formed by blue detuned hollow beams.

  12. A Simulator for Producing of High Flux Atomic Oxygen Beam by Using ECR Plasma Source

    Institute of Scientific and Technical Information of China (English)

    Shuwang DUO; Meishuan LI; Yaming ZHANG

    2004-01-01

    In order to study the atomic oxygen corrosion of spacecraft materials in low earth orbit environment, an atomic oxygen simulator was established. In the simulator, a 2.45 GHz microwave source with maximum power of 600 W was launched into the circular cavity to generate ECR (electron cyclotron resonance) plasma. The oxygen ion beam moved onto a negatively biased Mo plate under the condition of symmetry magnetic mirror field confine, then was neutralized and reflected to form oxygen atom beam. The properties of plasma density, electron temperature, plasma space potential and ion incident energy were characterized. The atomic oxygen beam flux was calibrated by measuring the mass loss rate of Kapton during the atomic 5~30 eV and a cross section of φ80 mm could be obtained under the operating pressure of 10-1~10-3 Pa. Such a high flux source can provide accelerated simulation tests of materials and coatings for space applications.

  13. Several atomic-physics issues connected with the use of neutral beams in fusion experiments

    Energy Technology Data Exchange (ETDEWEB)

    Post, D.E.; Grisham, L.R.; Fonck, R.J.

    1982-08-01

    Energetic neutral beams are used for heating and diagnostics in present magnetic fusion experiments. They are also being considered for use in future large experiments. Atomic physics issues are important for both the production of the neutral beams and the interaction of the beams and the plasma. Interest in neutral beams based on negative hydrogen ions is growing, largely based on advances in producing high current ion sources. An extension of the negative ion approach has been the suggestion to use negative ions of Z > 1 elements, such as carbon and oxygen, to form high power neutral beams for plasma heating.

  14. Neutron diffraction analyses of U-(6-10 wt.%)Mo alloy powders fabricated by centrifugal atomization

    Energy Technology Data Exchange (ETDEWEB)

    Park, Jong Man [Advanced Fuel Technology Development Division, Korea Atomic Energy Research Institute, 150 Deokjin-dong, Yuseong, Daejeon 305-353 (Korea, Republic of); Ryu, Ho Jin, E-mail: hjryu@kaeri.re.k [Advanced Fuel Technology Development Division, Korea Atomic Energy Research Institute, 150 Deokjin-dong, Yuseong, Daejeon 305-353 (Korea, Republic of); Kim, Ki Hwan; Lee, Don Bae; Lee, Yoon Sang [Advanced Fuel Technology Development Division, Korea Atomic Energy Research Institute, 150 Deokjin-dong, Yuseong, Daejeon 305-353 (Korea, Republic of); Lee, Jeong Soo; Seong, Baek Seok [Neutron Science Division, Korea Atomic Energy Research Institute, 150 Deokjin-dong, Yuseong, Daejeon 305-353 (Korea, Republic of); Kim, Chang Kyu [Advanced Fuel Technology Development Division, Korea Atomic Energy Research Institute, 150 Deokjin-dong, Yuseong, Daejeon 305-353 (Korea, Republic of); Cornen, Marilyne [INSA de Rennes, UMR CNRS 6226 Sciences Chimiques de Rennes/Chimie-Metallurgie, 20 Avenue des Buttes de Coesmes, 35043 Rennes Cedex (France)

    2010-02-15

    Lattice parameters of U-(6-10 wt.%)Mo alloy powders fabricated by a centrifugal atomization technique were measured by neutron diffraction analyses. A micro-segregation of Mo at cell boundaries was observed in the centrifugally atomized U-Mo alloy powders with varying Mo content. Lattice parameters of gamma phases decrease linearly with the increasing Mo content. By separating the overlapped diffraction peaks from cell boundaries and cell interior, lattice parameters and Mo contents of each region were calculated. The Mo content at cell boundaries is about 2-5 at.% lower than that in the cell interior and the lattice parameters for the cell boundaries are higher than those for the cell interior of the atomized U-Mo powder.

  15. Neutron diffraction analyses of U-(6-10 wt.%)Mo alloy powders fabricated by centrifugal atomization

    Science.gov (United States)

    Park, Jong Man; Ryu, Ho Jin; Kim, Ki Hwan; Lee, Don Bae; Lee, Yoon Sang; Lee, Jeong Soo; Seong, Baek Seok; Kim, Chang Kyu; Cornen, Marilyne

    2010-02-01

    Lattice parameters of U-(6-10 wt.%)Mo alloy powders fabricated by a centrifugal atomization technique were measured by neutron diffraction analyses. A micro-segregation of Mo at cell boundaries was observed in the centrifugally atomized U-Mo alloy powders with varying Mo content. Lattice parameters of gamma phases decrease linearly with the increasing Mo content. By separating the overlapped diffraction peaks from cell boundaries and cell interior, lattice parameters and Mo contents of each region were calculated. The Mo content at cell boundaries is about 2-5 at.% lower than that in the cell interior and the lattice parameters for the cell boundaries are higher than those for the cell interior of the atomized U-Mo powder.

  16. Effects of focused ion beam milling on electron backscatter diffraction patterns in strontium titanate and stabilized zirconia

    DEFF Research Database (Denmark)

    Saowadee, Nath; Agersted, Karsten; Bowen, Jacob R.

    2012-01-01

    This study investigates the effect of focused ion beam (FIB) current and accelerating voltage on electron backscatter diffraction pattern quality of yttria‐stabilized zirconia (YSZ) and Nb‐doped strontium titanate (STN) to optimize data quality and acquisition time for 3D‐EBSD experiments by FIB...

  17. X-rays diffraction on a new chromium oxide single-crystal thin film prepared by molecular beam epitaxy

    NARCIS (Netherlands)

    Du, X. S.; Hak, S.; Hibma, T.; Rogojanu, O. C.; Struth, B.

    2006-01-01

    Chromium oxide films were prepared on MgO substrates by molecular beam epitaxy. The crystalline structure of the films was characterized by X-ray diffraction (XRD) with conventional as well as synchrotron X-ray sources. The theta-2 theta spectra showed that the film was a new chromium oxide epitaxia

  18. A diffracted-beam monochromator for long linear detectors in X-ray diffractometers with Bragg-Brentano parafocusing geometry

    NARCIS (Netherlands)

    Van der Pers, N.M.; Hendrikx, R.W.A.; Delhez, R.; Böttger, A.J.

    2013-01-01

    A new diffracted-beam monochromator has been developed for Bragg-Brentano X-ray diffractometers equipped with a linear detector. The monochromator consists of a cone-shaped graphite highly oriented pyrolytic graphite crystal oriented out of the equatorial plane such that the parafocusing geometry is

  19. Aspherical-atom modeling of coordination compounds by single-crystal X-ray diffraction allows the correct metal atom to be identified.

    Science.gov (United States)

    Dittrich, Birger; Wandtke, Claudia M; Meents, Alke; Pröpper, Kevin; Mondal, Kartik Chandra; Samuel, Prinson P; Amin Sk, Nurul; Singh, Amit Pratap; Roesky, Herbert W; Sidhu, Navdeep

    2015-02-02

    Single-crystal X-ray diffraction (XRD) is often considered the gold standard in analytical chemistry, as it allows element identification as well as determination of atom connectivity and the solid-state structure of completely unknown samples. Element assignment is based on the number of electrons of an atom, so that a distinction of neighboring heavier elements in the periodic table by XRD is often difficult. A computationally efficient procedure for aspherical-atom least-squares refinement of conventional diffraction data of organometallic compounds is proposed. The iterative procedure is conceptually similar to Hirshfeld-atom refinement (Acta Crystallogr. Sect. A- 2008, 64, 383-393; IUCrJ. 2014, 1,61-79), but it relies on tabulated invariom scattering factors (Acta Crystallogr. Sect. B- 2013, 69, 91-104) and the Hansen/Coppens multipole model; disordered structures can be handled as well. Five linear-coordinate 3d metal complexes, for which the wrong element is found if standard independent-atom model scattering factors are relied upon, are studied, and it is shown that only aspherical-atom scattering factors allow a reliable assignment. The influence of anomalous dispersion in identifying the correct element is investigated and discussed.

  20. Large deflection angle, high-power adaptive fiber optics collimator with preserved near-diffraction-limited beam quality.

    Science.gov (United States)

    Zhi, Dong; Ma, Yanxing; Chen, Zilun; Wang, Xiaolin; Zhou, Pu; Si, Lei

    2016-05-15

    We report on the development of a monolithic adaptive fiber optics collimator, with a large deflection angle and preserved near-diffraction-limited beam quality, that has been tested at a maximal output power at the 300 W level. Additionally, a new measurement method of beam quality (M2 factor) is developed. Experimental results show that the deflection angle of the collimated beam is in the range of 0-0.27 mrad in the X direction and 0-0.19 mrad in the Y direction. The effective working frequency of the device is about 710 Hz. By employing the new measurement method of the M2 factor, we calculate that the beam quality is Mx2=1.35 and My2=1.24, which is in agreement with the result from the beam propagation analyzer and is preserved well with the increasing output power.

  1. Ultrashort pulse laser patterning of indium tin oxide thin films on glass by uniform diffractive beam patterns

    Energy Technology Data Exchange (ETDEWEB)

    Kuang Zheng, E-mail: z.kuang@liv.ac.uk [Laser Group, School of Engineering, University of Liverpool, Brownlow Street, Liverpool L69 3GQ (United Kingdom); Perrie, Walter; Liu Dun; Fitzsimons, Paul; Edwardson, Stuart P.; Fearon, Eamonn; Dearden, Geoff; Watkins, Ken G. [Laser Group, School of Engineering, University of Liverpool, Brownlow Street, Liverpool L69 3GQ (United Kingdom)

    2012-07-15

    In the last decade, indium tin oxide (ITO) has been most commonly employed to create transparent conducting oxides (TCOs) thin films for many industrial applications. It is usually necessary to pattern ITO thin films to create functional structures for specific applications. Direct-write micro-patterning of ITO thin films by ultra-short pulse lasers has demonstrated high quality without requiring multiple processing stations, compared with conventional patterning technologies (e.g. wet-etch lithography). However, the processing efficiency and throughput with a single beam can be insufficient because of the high level of attenuation needed for the output to meet the required 'thermal-free' parameters. In this paper, high throughput surface direct micro-structuring of ITO on glass is demonstrated by parallel processing using diffractive multiple ultrashort pulse laser beams ({lambda} = 1064 nm, {tau}p = 10 ps). By avoiding periodic and symmetrical geometry design, the diffractive multiple beam pattern generated by a spatial light modulator has high uniformity (the energy variation between each diffractive beam is <9%). The ITO thin film is removed by laser ablation of 25 identical beams at the same time without any damage to the glass substrate. Additionally, by synchronizing a scanning galvanometer, the processing demonstrates high flexibility to generate various surface patterns.

  2. New diagnostic technique for Zeeman-compensated atomic beam slowing: technique and results

    NARCIS (Netherlands)

    Molenaar, P.A.; Straten, P. van der; Heideman, H.G.M.; Metcalf, H.

    2001-01-01

    We have developed a new diagnostic tool for the study of Zeeman-compensated slowing of an alkali atomic beam. Our time-of-flight technique measures the longitudinal veloc- ity distribution of the slowed atoms with a resolution below the Doppler limit of 30 cm/s. Furthermore, it can map the position

  3. Self-corrected sensors based on atomic absorption spectroscopy for atom flux measurements in molecular beam epitaxy

    Energy Technology Data Exchange (ETDEWEB)

    Du, Y., E-mail: yingge.du@pnnl.gov, E-mail: scott.chambers@pnnl.gov; Liyu, A. V. [Environmental Molecular Sciences Laboratory, Pacific Northwest National Laboratory, Richland, Washington 99352 (United States); Droubay, T. C.; Chambers, S. A., E-mail: yingge.du@pnnl.gov, E-mail: scott.chambers@pnnl.gov [Fundamental and Computational Sciences Directorate, Pacific Northwest National Laboratory, Richland, Washington 99352 (United States); Li, G. [Energy and Environment Directorate, Pacific Northwest National Laboratory, Richland, Washington 99352 (United States)

    2014-04-21

    A high sensitivity atom flux sensor based on atomic absorption spectroscopy has been designed and implemented to control electron beam evaporators and effusion cells in a molecular beam epitaxy system. Using a high-resolution spectrometer and a two-dimensional charge coupled device detector in a double-beam configuration, we employ either a non-resonant line or a resonant line with low cross section from the same hollow cathode lamp as the reference for nearly perfect background correction and baseline drift removal. This setup also significantly shortens the warm-up time needed compared to other sensor technologies and drastically reduces the noise coming from the surrounding environment. In addition, the high-resolution spectrometer allows the most sensitive resonant line to be isolated and used to provide excellent signal-to-noise ratio.

  4. Self-corrected Sensors Based On Atomic Absorption Spectroscopy For Atom Flux Measurements In Molecular Beam Epitaxy

    Energy Technology Data Exchange (ETDEWEB)

    Du, Yingge; Droubay, Timothy C.; Liyu, Andrey V.; Li, Guosheng; Chambers, Scott A.

    2014-04-24

    A high sensitivity atom flux sensor based on atomic absorption spectroscopy has been designed and implemented to control electron beam evaporators and effusion cells in a molecular beam epitaxy system. Using a high-resolution spectrometer and a two-dimensional charge coupled device (CCD) detector in a double-beam configuration, we employ a non-resonant line or a resonant line with lower absorbance from the same hollow cathode lamp as the reference for nearly perfect background correction and baseline drift removal. This setup also significantly shortens the warm-up time needed compared to other sensor technologies and drastically reduces the noise coming from the surrounding environment. In addition, the high-resolution spectrometer allows the most sensitive resonant line to be isolated and used to provide excellent signal-to-noise ratio.

  5. Self-corrected sensors based on atomic absorption spectroscopy for atom flux measurements in molecular beam epitaxy

    Science.gov (United States)

    Du, Y.; Droubay, T. C.; Liyu, A. V.; Li, G.; Chambers, S. A.

    2014-04-01

    A high sensitivity atom flux sensor based on atomic absorption spectroscopy has been designed and implemented to control electron beam evaporators and effusion cells in a molecular beam epitaxy system. Using a high-resolution spectrometer and a two-dimensional charge coupled device detector in a double-beam configuration, we employ either a non-resonant line or a resonant line with low cross section from the same hollow cathode lamp as the reference for nearly perfect background correction and baseline drift removal. This setup also significantly shortens the warm-up time needed compared to other sensor technologies and drastically reduces the noise coming from the surrounding environment. In addition, the high-resolution spectrometer allows the most sensitive resonant line to be isolated and used to provide excellent signal-to-noise ratio.

  6. X-ray diffraction from bone employing annular and semi-annular beams.

    Science.gov (United States)

    Dicken, A J; Evans, J P O; Rogers, K D; Stone, N; Greenwood, C; Godber, S X; Prokopiou, D; Clement, J G; Lyburn, I D; Martin, R M; Zioupos, P

    2015-08-07

    There is a compelling need for accurate, low cost diagnostics to identify osteo-tissues that are associated with a high risk of fracture within an individual. To satisfy this requirement the quantification of bone characteristics such as 'bone quality' need to exceed that provided currently by densitometry. Bone mineral chemistry and microstructure can be determined from coherent x-ray scatter signatures of bone specimens. Therefore, if these signatures can be measured, in vivo, to an appropriate accuracy it should be possible by extending terms within a fracture risk model to improve fracture risk prediction.In this preliminary study we present an examination of a new x-ray diffraction technique that employs hollow annular and semi-annular beams to measure aspects of 'bone quality'. We present diffractograms obtained with our approach from ex vivo bone specimens at Mo Kα and W Kα energies. Primary data is parameterized to provide estimates of bone characteristics and to indicate the precision with which these can be determined.

  7. Beating the classical limit: A diffraction-limited spectrograph for an arbitrary input beam

    CERN Document Server

    Betters, Christopher H; Robertson, J Gordon; Bland-Hawthorn, Joss

    2013-01-01

    We demonstrate a new approach to classical fiber-fed spectroscopy. Our method is to use a photonic lantern that converts an arbitrary (e.g. incoherent) input beam into N diffraction-limited outputs. For the highest throughput, the number of outputs must be matched to the total number of unpolarized spatial modes on input. This approach has many advantages: (i) after the lantern, the instrument is constructed from 'commercial off the shelf' components; (ii) the instrument is the minimum size and mass configuration at a fixed resolving power and spectral order (~shoebox sized in this case); (iii) the throughput is better than 60% (slit to detector, including detector QE of ~80%); (iv) the scattered light at the detector can be less than 0.1% (total power). Our first implementation operates over 1545-1555 nm (limited by the detector, a 640$\\times$512 array with 20$\\mu$m pitch) with a spectral resolution of 0.055nm (R~30,000) using a 1$\\times$7 (1 multi-mode input to 7 single-mode outputs) photonic lantern. This ...

  8. Four beam interferometer manual: Operating instructions for the INEL diffraction Moire interferometer

    Energy Technology Data Exchange (ETDEWEB)

    Deason, V.A.

    1993-11-01

    Moire interferometry is an interferometric method for measuring changes of in-plane geometry. It is essentially insensitive to out-of-plane topography or changes in that topography. Changes in geometry are referenced to a particular moment in time when the moire` sensor, a diffraction grating, was attached to the specimen. Distortions experienced by the specimen prior to that time are not directly detectable, although they may be inferred from specimen behavior or condition. In its most common form, moire interferometry is not well suited to large (> 50 mm square), curved (< 300 mm diameter) or high temperature (> 200 C) regions. However, various efforts have been made to handle each of these conditions. In general, the moire` process is most straightforward for flat, 25 mm diameter regions of coverage and room temperature. Much smaller or larger regions require more specialized optics, which can become very expensive. This report will discuss various aspects of moire interferometry. In particular, a new four beam (bi-axial) interferometer is described in detail. Issues involved in safety, assembly, calibration and use are fully explained.

  9. A compact design for a magnetic synchrotron to store beams of hydrogen atoms

    CERN Document Server

    van der Poel, Aernout P P; Softley, Timothy P; Bethlem, Hendrick L

    2015-01-01

    We present a design for an atomic synchrotron consisting of 40 hybrid magnetic hexapole lenses arranged in a circle. We show that for realistic parameters, hydrogen atoms with a velocity up to 600 m/s can be stored in a 1-meter diameter ring, which implies that the atoms can be injected in the ring directly from a pulsed supersonic beam source. This ring can be used to study collisions between stored hydrogen atoms and molecular beams of many different atoms and molecules. The advantage of using a synchrotron is two-fold: (i) the collision partners move in the same direction as the stored atoms, resulting in a small relative velocity and thus a low collision energy, and (ii) by storing atoms for many round-trips, the sensitivity to collisions is enhanced by a factor of 100-1000. In the proposed ring, the cross-sections for collisions between hydrogen, the most abundant atom in the universe, with any atom or molecule that can be put in a beam, including He, H$_2$, CO, ammonia and OH can be measured at energies...

  10. Negative optical spin torque wrench of a non-diffracting non-paraxial fractional Bessel vortex beam

    Science.gov (United States)

    Mitri, F. G.

    2016-10-01

    An absorptive Rayleigh dielectric sphere in a non-diffracting non-paraxial fractional Bessel vortex beam experiences a spin torque. The axial and transverse radiation spin torque components are evaluated in the dipole approximation using the radiative correction of the electric field. Particular emphasis is given on the polarization as well as changing the topological charge α and the half-cone angle of the beam. When α is zero, the axial spin torque component vanishes. However, when α becomes a real positive number, the vortex beam induces left-handed (negative) axial spin torque as the sphere shifts off-axially from the center of the beam. The results show that a non-diffracting non-paraxial fractional Bessel vortex beam is capable of inducing a spin reversal of an absorptive Rayleigh sphere placed arbitrarily in its path. Potential applications are yet to be explored in particle manipulation, rotation in optical tweezers, optical tractor beams, and the design of optically-engineered metamaterials to name a few areas.

  11. A blu-ray laser diode based dual-beam interference lithography for fabrication of diffraction gratings for surface encoders

    Science.gov (United States)

    Zhu, Xiangwen; Li, Xinghui; Zhou, Qian; Wang, Xiaohao; Ni, Kai

    2016-11-01

    The paper presents a dual-beam interference lithography technology for fabrication of diffraction gratings for surface encoders by using cost-effective 405 nm blu-ray laser diodes. In this system, an amplitude division interferometer system is employed. A laser beam raying from a blu-ray laser diode is collimated and then divided into two beams by a beam splitter. These two beams are changed their propagation directions and interfere with each other. Generated interference fringes are exposed on the photoresist coated substrate. Grating line spacing d can be adjusted by changing the incident angle between these two beams. Grating width Wc that determines the measurement of the surface encoder is decided by the coherence length Lc of the laser diode and the grating line spacing d. Calculation and simulation were carried out to decide the grating width. Lc was experimentally obtained. A fabrication system was constructed to verify the feasibility of this technology. Diffraction gratings with a 2.5 micron line spacing and a 2.5 mm width was obtained.

  12. Diffraction studies for stoichiometry effects in BaTiO3 grown by molecular beam epitaxy on Ge(001)

    Science.gov (United States)

    Hsu, Min-Hsiang Mark; Merckling, Clement; El Kazzi, Salim; Pantouvaki, Marianna; Richard, Oliver; Bender, Hugo; Meersschaut, Johan; Van Campenhout, Joris; Absil, Philippe; Van Thourhout, Dries

    2016-12-01

    In this work, we present a systematic study of the effect of the stoichiometry of BaTiO3 (BTO) films grown on the Ge(001) substrate by molecular-beam-epitaxy using different characterization methods relying on beam diffraction, including reflection high-energy electron diffraction (RHEED), X-ray diffraction (XRD), and selected-area electron diffraction in transmission electron microscopy. Surprisingly, over a wide range of [Ba]/[Ti] ratios, as measured by the Rutherford backscattering spectrometry, all the BTO layers exhibit the same epitaxial relationship BTO(001)//Ge(001) with the substrate, describing a 45° lattice rotation of the BTO lattice with respect to the Ge lattice. However, varying the [Ba]/[Ti] ratio does change the diffraction behavior. From RHEED patterns, we can derive that excessive [Ba] and [Ti] generate twinning planes and a rougher surface in the non-stoichiometric BTO layers. XRD allows us to follow the evolution of the lattice constants as a function of the [Ba]/[Ti] ratio, providing an option for tuning the tetragonality of the BTO layer. In addition, we found that the intensity ratio of the 3 lowest-order Bragg peaks I(001)/I(002), I(101)/I(002), and I(111)/I(002) derived from ω - 2θ scans characteristically depend on the BTO stoichiometry. To explain the relation between observed diffraction patterns and the stoichiometry of the BTO films, we propose a model based on diffraction theory explaining how excess [Ba] or [Ti] in the layer influences the diffraction response.

  13. Detection of a coherent population trapping resonance in a beam of 87Rb atoms by the Ramsey method

    Science.gov (United States)

    Sokolov, I. M.

    2015-10-01

    Formation of a coherent population trapping (CPT) resonance is studied in the interaction of a beam of 87Rb atoms with two spatially separated domains of the dichromatic field. Various resonance excitation schemes are compared depending on the choice of operation transitions and type of the polarisation scheme. In the case of a single-velocity atomic beam, the dependence of the CPT resonance profile is studied as a function of principal parameters of the system: beam velocity, distance between optical fields, laser beam dimensions and intensities, and applied permanent magnetic field. Influence of the atomic beam angular divergence and residual beam velocity spread on the resonance quality parameter is estimated.

  14. Probing the short range spin dependent interactions by polarized {sup 3}He atom beams

    Energy Technology Data Exchange (ETDEWEB)

    Yan, H. [China Academy of Engineering Physics, Institute of Nuclear Physics and Chemistry, Mianyang, Sichuan (China); Indiana University, Center for Exploration of Energy and Matter, Bloomington, IN (United States); Sun, G.A.; Gong, J.; Pang, B.B.; Wang, Y.; Yang, Y.W.; Zhang, J.; Zhang, Y. [China Academy of Engineering Physics, Institute of Nuclear Physics and Chemistry, Mianyang, Sichuan (China)

    2014-10-15

    Experiments using polarized {sup 3}He atom beams to search for short range spin dependent forces are proposed. High intensity, high polarization, small beam size {sup 3}He atom beams have been successfully produced and used in surface science researches. By incorporating background reduction designs as combination shielding by μ-metal and superconductor and double beam paths, the precision of spin rotation angle per unit length could be improved by a factor of ∝ 10{sup 4}. By this precision, in combination with a high density and low magnetic susceptibility sample source mass, and reversing one beam path if necessary, sensitivities on three different types of spin dependent interactions could be improved by as much as ∝ 10{sup 2} to ∝ 10{sup 8} over the current experiments at the millimeter range. (orig.)

  15. Real-time detection of focal position of workpiece surface during laser processing using diffractive beam samplers

    Science.gov (United States)

    Cao, Binh Xuan; Hoang, PhuongLe; Ahn, Sanghoon; Kim, Jeng-o.; Sohn, Hyonkee; Noh, Jiwhan

    2016-11-01

    The real-time fabrication of microgrooves on a curved surface using a laser beam, without preprogramming their shapes into the machining instructions, is a major challenge in laser processing owing to limitations associated with the real-time detection of the focal position. A new approach using a sampled fraction of the beam from a diffractive beam sampler (DBS) is therefore presented in order to overcome this limitation. By considering the sampled fraction of the beam an analysis of the results allows for precise positioning of the specimen for focal-point identification. This allows for the determination of the focus for a broad variety of laser types and laser powers, thereby providing stringent focusing conditions with high numerical apertures. This approach is easy to implement, inexpensive, independent of the roughness or granularity of the workpieces, and more importantly does not require auxiliary lasers and displacement sensors for real-time measurement during the fabrication process.

  16. The calculation of the diffraction of the laser beams with a phase singularity on the micro-axicons with using high-performance computing

    Science.gov (United States)

    A, Savelyev D.; N, Khonina S.

    2014-03-01

    We analyze the diffraction of the laser beam with a vortex phase singularity on the basis of the finite-difference time-domain method (FDTD). It is shown that, when incident beam has phase singularity, increase of the micro-axicon radius leads to extension of the light needle consisting of longitudinal electric field component. The numerical investigations held of the near-field diffraction for the most common and easily implemented types of polarization of the incident beam - linear and circular.

  17. Reactions of carbon atoms in pulsed molecular beams

    Energy Technology Data Exchange (ETDEWEB)

    Reisler, H. [Univ. of Southern California, Los Angeles (United States)

    1993-12-01

    This research program consists of a broad scope of experiments designed to unravel the chemistry of atomic carbon in its two spin states, P and D, by using well-controlled initial conditions and state-resolved detection of products. Prerequisite to the proposed studies (and the reason why so little is known about carbon atom reactions), is the development of clean sources of carbon atoms. Therefore, in parallel with the studies of its chemistry and reaction dynamics, the authors continuously explore new, state-specific and efficient ways of producing atomic carbon. In the current program, C({sup 3}P) is produced via laser ablation of graphite, and three areas of study are being pursued: (i) exothermic reactions with small inorganic molecules (e.g., O{sub 2}, N{sub 2}O, NO{sub 2}) that can proceed via multiple pathways; (ii) the influence of vibrational and translational energy on endothermic reactions involving H-containing reactants that yield CH products (e.g., H{sub 2}O H{sub 2}CO); (iii) reactions of C({sup 3}P) with free radicals (e.g., HCO, CH{sub 3}O). In addition, the authors plan to develop a source of C({sup 1}D) atoms by exploiting the pyrolysis of diazotetrazole and its salts in the ablation source. Another important goal involves collaboration with theoreticians in order to obtain relevant potential energy surfaces, rationalize the experimental results and predict the roles of translational and vibrational energies.

  18. Optical dipole mirror for cold atoms based on a metallic diffraction grating

    DEFF Research Database (Denmark)

    Kawalec, Tomasz; Bartoszek-Bober, Dobroslawa; Panas, Roman

    2014-01-01

    and numerically determined mirror efficiencies are close to 100%. The intensity of SPPs above a real grating coupler and the atomic trajectories, as well as the momentum dispersion of the atom cloud being reflected, are computed. A suggestion is given as to how the plasmonic mirror might serve as an optical atom...

  19. Wavefront-correction for nearly diffraction-limited focusing of dual-color laser beams to high intensities.

    Science.gov (United States)

    Zhao, Baozhen; Zhang, Jun; Chen, Shouyuan; Liu, Cheng; Golovin, Grigory; Banerjee, Sudeep; Brown, Kevin; Mills, Jared; Petersen, Chad; Umstadter, Donald

    2014-11-03

    We demonstrate wavefront correction of terawatt-peak-power laser beams at two distinct and well-separated wavelengths. Simultaneous near diffraction-limited focusability is achieved for both the fundamental (800 nm) and second harmonic (400 nm) of Ti:sapphire-amplified laser light. By comparing the relative effectiveness of various correction loops, the optimal ones are found. Simultaneous correction of both beams of different color relies on the linear proportionality between their wavefront aberrations. This method can enable two-color experiments at relativistic intensities.

  20. Reflection High-Energy Electron Diffraction Beam-Induced Structural and Property Changes on WO3 Thin Films

    Energy Technology Data Exchange (ETDEWEB)

    Du, Yingge; Zhang, Hongliang; Varga, Tamas; Chambers, Scott A.

    2014-08-08

    Reduction of transition metal oxides can greatly change their physical and chemical properties. Using deposition of WO3 as a case study, we demonstrate that reflection high-energy electron diffraction (RHEED), a surface-sensitive tool widely used to monitor thin-film deposition processes, can significantly affect the cation valence and physical properties of the films through electron-beam induced sample reduction. The RHEED beam is found to increase film smoothness during epitaxial growth of WO3, as well as change the electronic properties of the film through preferential removal of surface oxygen.

  1. Producing acoustic 'Frozen Waves': simulated experiments with diffraction/attenuation resistant beams in lossy media.

    Science.gov (United States)

    Prego-Borges, José L; Zamboni-Rached, Michel; Recami, Erasmo; Costa, Eduardo Tavares

    2014-08-01

    The so-called Localized Waves (LW), and the "Frozen Waves" (FW), have raised significant attention in the areas of Optics and Ultrasound, because of their surprising energy localization properties. The LWs resist the effects of diffraction for large distances, and possess an interesting self-reconstruction -self-healing- property (after obstacles with size smaller than the antenna's); while the FWs, a sub-class of LWs, offer the possibility of arbitrarily modeling the longitudinal field intensity pattern inside a prefixed interval, for instance 0⩽z⩽L, of the wave propagation axis. More specifically, the FWs are localized fields "at rest", that is, with a static envelope (within which only the carrier wave propagates), and can be endowed moreover with a high transverse localization. In this paper we investigate, by simulated experiments, various cases of generation of ultrasonic FW fields, with the frequency of f0=1 MHz in a water-like medium, taking account of the effects of attenuation. We present results of FWs for distances up to L=80 mm, in attenuating media with absorption coefficient α in the range 70⩽α⩽170 dB/m. Such simulated FW fields are constructed by using a procedure developed by us, via appropriate finite superpositions of monochromatic ultrasonic Bessel beams. We pay due attention to the selection of the FW parameters, constrained by the rather tight restrictions imposed by experimental Acoustics, as well as to some practical implications of the transducer design. The energy localization properties of the Frozen Waves can find application even in many medical apparatus, such as bistouries or acoustic tweezers, as well as for treatment of diseased tissues (in particular, for the destruction of tumor cells, without affecting the surrounding tissues; also for kidney stone shuttering, etc.).

  2. LOW ENERGY BEAM-GAS SPECTROSCOPY OF HIGHLY IONISED ATOMS

    OpenAIRE

    Desesquelles, J.; DENIS A.; Druetta, M.; Martin, S.

    1989-01-01

    Features of low energy beam-gas spectroscopic source are reviewed and compared to those of other light sources. Measurement techniques are surveyed. They include the study of wavelength of heavy multiply charged ions in visible and u.v. ranges from normal excited states, doubly excited states, high n levels and doubly excited Rydberg levels.

  3. Efficient sub-Doppler transverse laser cooling of an indium atomic beam

    Energy Technology Data Exchange (ETDEWEB)

    Kim, Jae-Ihn

    2009-07-23

    Laser cooled atomic gases and atomic beams are widely studied samples in experimental research in atomic and optical physics. For the application of ultra cold gases as model systems for e.g. quantum many particle systems, the atomic species is not very important. Thus this field is dominated by alkaline, earthalkaline elements which are easily accessible with conventional laser sources and have convenient closed cooling transition. On the other hand, laser cooled atoms may also be interesting for technological applications, for instance for the creation of novel materials by atomic nanofabrication (ANF). There it will be important to use technologically relevant materials. As an example, using group III atoms of the periodical table in ANF may open a route to generate fully 3D structured composite materials. The minimal requirement in such an ANF experiment is the collimation of an atomic beam which is accessible by one dimensional laser cooling. In this dissertation, I describe transverse laser cooling of an Indium atomic beam. For efficient laser cooling on a cycling transition, I have built a tunable, continuous-wave coherent ultraviolet source at 326 nm based on frequency tripling. For this purpose, two independent high power Yb-doped fiber amplifiers for the generation of the fundamental radiation at {lambda}{sub {omega}} = 977 nm have been constructed. I have observed sub-Doppler transverse laser cooling of an Indium atomic beam on a cycling transition of In by introducing a polarization gradient in the linear-perpendicular-linear configuration. The transverse velocity spread of a laser-cooled In atomic beam at full width at half maximum was achieved to be 13.5{+-}3.8 cm/s yielding a full divergence of only 0.48 {+-} 0.13 mrad. In addition, nonlinear spectroscopy of a 3-level, {lambda}-type level system driven by a pump and a probe beam has been investigated in order to understand the absorption line shapes used as a frequency reference in a previous two

  4. Using a short-pulse diffraction-limited laser beam to probe filamentation of a random phase plate smoothed beam.

    Science.gov (United States)

    Kline, J L; Montgomery, D S; Flippo, K A; Johnson, R P; Rose, H A; Shimada, T; Williams, E A

    2008-10-01

    A short pulse (few picoseconds) laser probe provides high temporal resolution measurements to elucidate details of fast dynamic phenomena not observable with typical longer laser pulse probes and gated diagnostics. Such a short pulse laser probe (SPLP) has been used to measure filamentation of a random phase plate (RPP) smoothed laser beam in a gas-jet plasma. The plasma index of refraction due to driven density and temperature fluctuations by the RPP beam perturbs the phase front of a SPLP propagating at a 90 degree angle with respect to the RPP interaction beam. The density and temperature fluctuations are quasistatic on the time scale of the SPLP (approximately 2 ps). The transmitted near-field intensity distribution from the SPLP provides a measure of the phase front perturbation. At low plasma densities, the transmitted intensity pattern is asymmetric with striations across the entire probe beam in the direction of the RPP smoothed beam. As the plasma density increases, the striations break up into smaller sizes along the direction of the RPP beam propagation. The breakup of the intensity pattern is consistent with self-focusing of the RPP smoothed interaction beam. Simulations of the experiment using the wave propagation code, PF3D, are in qualitative agreement demonstrating that the asymmetric striations can be attributed to the RPP driven density fluctuations. Quantification of the beam breakup measured by the transmitted SPLP could lead to a new method for measuring self-focusing of lasers in underdense plasmas.

  5. Probing the energy flow in Bessel light beams using atomic photoionization

    Science.gov (United States)

    Surzhykov, A.; Seipt, D.; Fritzsche, S.

    2016-09-01

    The growing interest in twisted light beams also requires a better understanding of their complex internal structure. Particular attention is currently being given to the energy circulation in these beams as usually described by the Poynting vector field. In the present study we propose to use the photoionization of alkali-metal atoms as a probe process to measure (and visualize) the energy flow in twisted light fields. Such measurements are possible since the angular distribution of photoelectrons, emitted from a small atomic target, appears sensitive to and is determined by the local direction of the Poynting vector. To illustrate the feasibility of the proposed method, detailed calculations were performed for the ionization of sodium atoms by nondiffractive Bessel beams.

  6. Dynamics of Finite Energy Airy Beams Carrying Orbital Angular Momentum in Multilevel Atomic Vapors

    Science.gov (United States)

    Wu, Zhenkun; Wang, Shun; Hu, Weifei; Gu, Yuzong

    2016-10-01

    We numerically investigate the dynamics of inward circular finite-energy Airy beams carrying different orbital angular momentum (OAM) numbers in a close-Λ three-level atomic vapor with the electromagnetically induced transparency (EIT) window. We report that due to the EIT induced by the microwave field, the transverse intensity distribution properties of Airy beam can be feasibly manipulated and modulated through adjusting OAM numbers l and the frequency detuning, as well as the propagation distance, in the multi-level atomic systems. What's more, the rotation of the beam also can be observed with different positions in atomic ensembles. The investigation may provide a useful tool for studying particle manipulation, signal processing and propagation in graded-index (GRIN) fibers.

  7. Separate determination of the amplitude of thermal vibrations and static atomic displacements in titanium carbide by neutron diffraction

    Energy Technology Data Exchange (ETDEWEB)

    Khidirov, I., E-mail: khidirov@inp.uz; Parpiev, A. S. [Uzbekistan Academy of Sciences, Institute of Nuclear Physics (Uzbekistan)

    2011-05-15

    The amplitude of thermal (dynamic) atomic vibrations and meansquare static atomic displacements in titanium carbide TiC{sub x} (x = 0.97, 0.88, 0.70) have been separately determined by measuring neutron diffraction patterns at two temperatures (T{sub 1} = 300 K and T{sub 2} = 80 K). The static lattice distortions in stoichiometric titanium carbide are experimentally found to be negligible. In the TiC{sub x} homogeneity range, the amplitude {radical}u{sup 2}{sub dyn} of thermal atomic vibrations significantly increases with a decrease in the carbon concentration. The Debye temperature has been determined for the first time in the TiC{sub x} homogeneity range at both room and liquid-nitrogen temperatures.

  8. Radioactive ion beam transportation for the fundamental symmetry study with laser-trapped atoms

    Energy Technology Data Exchange (ETDEWEB)

    Arikawa, Hiroshi, E-mail: arikawa@cyric.tohoku.ac.jp; Ando, S.; Aoki, T.; Ezure, S.; Harada, K.; Hayamizu, T.; Inoue, T.; Ishikawa, T.; Itoh, M.; Kawamura, H.; Kato, K.; Kato, T.; Uchiyama, A.; Sakemi, Y. [Cyclotron and Radioisotope Center, Tohoku University, Miyagi 980-8578 (Japan); Aoki, T. [Graduate School of Arts and Sciences, University of Tokyo, Tokyo 153-8902 (Japan); Furukawa, T. [Department of Physics, Tokyo Metropolitan University, Tokyo 192-0397 (Japan); Hatakeyama, A. [Department of Applied Physics, Tokyo University of Agriculture and Technology, Tokyo 184-8588 (Japan); Hatanaka, K.; Yoshida, H. P. [Research Center for Nuclear Physics, Osaka University, Osaka 606-8502 (Japan); Imai, K. [Advanced Science Research Center, Japan Atomic Energy Agency, Ibaraki 319-1184 (Japan); and others

    2014-02-15

    The search for the violation of the fundamental symmetry in a radioactive atom is the promising candidate for precision tests of the standard model and its possible extensions. The subtle signal arising from the symmetry violation is enhanced in heavy atoms, such as a francium (Fr). To realize high precision measurements, a large amount of radioactive isotopes is required. The Fr is produced via a nuclear fusion reaction using a melted gold target with a {sup 18}O primary beam at Cyclotron and Radioisotope Center, Tohoku University. The maximum extraction efficiency of the Fr ion was achieved at approximately 35%. The beam line consists of an electrostatic deflector, three electrostatic quadrupole triplets to the measurement area at 10 m away from the reaction point, and several beam diagnosis systems. We optimized parameters of the beam line.

  9. Three-dimensionally modulated anisotropic structure for diffractive optical elements created by one-step three-beam polarization holographic photoalignment

    Science.gov (United States)

    Kawai, Kotaro; Sakamoto, Moritsugu; Noda, Kohei; Sasaki, Tomoyuki; Kawatsuki, Nobuhiro; Ono, Hiroshi

    2016-03-01

    A diffractive optical element with a three-dimensional liquid crystal (LC) alignment structure for advanced control of polarized beams was fabricated by a highly efficient one-step photoalignment method. This study is of great significance because different two-dimensional continuous and complex alignment patterns can be produced on two alignment films by simultaneously irradiating an empty glass cell composed of two unaligned photocrosslinkable polymer LC films with three-beam polarized interference beam. The polarization azimuth, ellipticity, and rotation direction of the diffracted beams from the resultant LC grating widely varied depending on the two-dimensional diffracted position and the polarization states of the incident beams. These polarization diffraction properties are well explained by theoretical analysis based on Jones calculus.

  10. An atomic coilgun: using pulsed magnetic fields to slow a supersonic beam

    Energy Technology Data Exchange (ETDEWEB)

    Narevicius, E [Center for Nonlinear Dynamics and Department of Physics, Univesity of Texas at Austin, Austin, TX 78712-1081 (United States); Parthey, C G [Center for Nonlinear Dynamics and Department of Physics, Univesity of Texas at Austin, Austin, TX 78712-1081 (United States); Libson, A [Center for Nonlinear Dynamics and Department of Physics, Univesity of Texas at Austin, Austin, TX 78712-1081 (United States); Narevicius, J [Center for Nonlinear Dynamics and Department of Physics, Univesity of Texas at Austin, Austin, TX 78712-1081 (United States); Chavez, I [Center for Nonlinear Dynamics and Department of Physics, Univesity of Texas at Austin, Austin, TX 78712-1081 (United States); Even, U [Sackler School of Chemistry, Tel-Aviv University, Tel-Aviv (Israel); Raizen, M G [Center for Nonlinear Dynamics and Department of Physics, Univesity of Texas at Austin, Austin, TX 78712-1081 (United States)

    2007-10-15

    We report the experimental demonstration of a novel method to slow atoms and molecules with permanent magnetic moments using pulsed magnetic fields. In our experiments, we observe the slowing of a supersonic beam of metastable neon from 461.0 {+-} 7.7 to 403 {+-} 16 m s{sup -1} in 18 stages, where the slowed peak is clearly separated from the initial distribution. This method has broad applications as it may easily be generalized, using seeding and entrainment into supersonic beams, to all paramagnetic atoms and molecules.

  11. Coherent reflection of He atom beams from rough surfaces at near-grazing incidence

    OpenAIRE

    Zhao, B.; Schewe, C.; Meijer, G.; Schöllkopf, W.

    2010-01-01

    We report coherent reflection of thermal He atom beams from various microscopically rough surfaces at grazing incidence. For a sufficiently small normal component kz of the incident wave- vector of the atom the reflection probability is found to be a function of kz only. This behavior is explained by quantum-reflection at the attractive branch of the Casimir-van der Waals interaction potential. For larger values of kz the overall reflection probability decreases rapidly and is found to also d...

  12. Precision measurement of transverse velocity distribution of a strontium atomic beam

    OpenAIRE

    Gao, F.; H. Liu; Xu, P.; X. Tian; Y. Wang; Ren, J; Haibin Wu; Hong Chang

    2014-01-01

    We measure the transverse velocity distribution in a thermal Sr atomic beam precisely by velocity-selective saturated fluorescence spectroscopy. The use of an ultrastable laser system and the narrow intercombination transition line of Sr atoms mean that the resolution of the measured velocity can reach 0.13 m/s, corresponding to 90$\\mu K$ in energy units. The experimental results are in very good agreement with the results of theoretical calculations. Based on the spectroscopic techniques use...

  13. Nanometer scale period sinusoidal atom gratings produced by a Stern-Gerlach beam splitter

    CERN Document Server

    Dubetsky, B

    2002-01-01

    An atom interferometer based on a Stern-Gerlach beam splitter is proposed. Atom scattering from a combination of magnetic quadrupole and homogeneous magnetic fields is considered. Using Raman transitions, atoms are coherently excited into and de-excited from sublevels having nonzero magnetic quantum numbers. The spatial regions in which the atoms are in such sublevels are small and have magnetic fields designed to have constant gradients. Therefore, the atoms experience position-independent accelerations, and the aberration of the coherently separated and recombined atomic beams remains small. We find that because of these properties it is possible to envision an apparatus producing atomic density gratings with nm-scale periods and large contrasts over 10-100 $\\mu $m. We use a new method of describing the atomic interaction with a pulsed spatially homogeneous field. In our detailed analysis, we calculate corrections caused by the non-linear part of the potential and the finite value of the de-Broglie wave len...

  14. Time-of-flight measurements in atomic beam devices using adiabatic high frequency transitions and sextupole magnets

    CERN Document Server

    Baumgarten, C; Brunn, I; Court, G; Ciullo, G; Ferretti, P; Golendukhin, A; Graw, G; Haeberli, W; Henoch, M; Hertenberger, R; Koch, N; Kolster, H; Lenisa, P; Nass, A; Podyachev, S P; Reggiani, D; Rith, K; Simani, M C; Steffens, E; Stewart, J; Wise, T

    2002-01-01

    Atomic beam devices are frequently equipped with sextupole magnets to focus the beam or to act as spin filters in combination with RF-transitions for manipulating the hyperfine population within the atomic beam. A useful tool for the analysis of sextupole systems, the application of time-of-flight (TOF) measurements is presented. TOF measurements are enabled without mechanical beam chopper by utilizing adiabatic radio frequency transitions to select atoms within a certain time interval. This method is especially interesting for the use in atomic beam devices that are already equipped with RF-transitions and sextupole magnets and where space limitations or the required quality of the vacuum do not allow the installation of a mechanical chopper. The measurements presented here were performed with the atomic beam polarimeter of the HERMES polarized deuterium target and the results have been used to optimize the sextupole system of the polarimeter.

  15. Detection of a coherent population trapping resonance in a beam of {sup 87}Rb atoms by the Ramsey method

    Energy Technology Data Exchange (ETDEWEB)

    Sokolov, I M [Peter the Great St.Petersburg Polytechnic University, St.Petersburg (Russian Federation)

    2015-10-31

    Formation of a coherent population trapping (CPT) resonance is studied in the interaction of a beam of {sup 87}Rb atoms with two spatially separated domains of the dichromatic field. Various resonance excitation schemes are compared depending on the choice of operation transitions and type of the polarisation scheme. In the case of a single-velocity atomic beam, the dependence of the CPT resonance profile is studied as a function of principal parameters of the system: beam velocity, distance between optical fields, laser beam dimensions and intensities, and applied permanent magnetic field. Influence of the atomic beam angular divergence and residual beam velocity spread on the resonance quality parameter is estimated. (atomic beams)

  16. Atomic structure solution of the complex quasicrystal approximant Al77Rh15Ru8 from electron diffraction data.

    Science.gov (United States)

    Samuha, Shmuel; Mugnaioli, Enrico; Grushko, Benjamin; Kolb, Ute; Meshi, Louisa

    2014-12-01

    The crystal structure of the novel Al77Rh15Ru8 phase (which is an approximant of decagonal quasicrystals) was determined using modern direct methods (MDM) applied to automated electron diffraction tomography (ADT) data. The Al77Rh15Ru8 E-phase is orthorhombic [Pbma, a = 23.40 (5), b = 16.20 (4) and c = 20.00 (5) Å] and has one of the most complicated intermetallic structures solved solely by electron diffraction methods. Its structural model consists of 78 unique atomic positions in the unit cell (19 Rh/Ru and 59 Al). Precession electron diffraction (PED) patterns and high-resolution electron microscopy (HRTEM) images were used for the validation of the proposed atomic model. The structure of the E-phase is described using hierarchical packing of polyhedra and a single type of tiling in the form of a parallelogram. Based on this description, the structure of the E-phase is compared with that of the ε6-phase formed in Al-Rh-Ru at close compositions.

  17. Special diffractive elements for optical trapping fabricated on optical fiber tips using the focused ion beam

    Science.gov (United States)

    Rodrigues Ribeiro, R. S.; Guerreiro, A.; Viegas, J.; Jorge, P. A. S.

    2016-05-01

    In this work, spiral phase lenses and Fresnel zone lenses for beam tailoring, fabricated on the tip of optical fibers, are reported. The spiral phase lenses allow tailoring the fundamental guided mode, a Gaussian beam, into a Laguerre - Gaussian profile without using additional optical elements. Whereas, the Fresnel lenses are used as focusing systems. The lenses are fabricated using Focused Ion Beam milling, enabling high resolution in the manufacturing process. The output optical intensity profiles matching the numerical simulations are presented and analyzed.

  18. New diagnostic technique for Zeeman-compensated atomic beam slowing: technique and results

    OpenAIRE

    Molenaar, P.A.; Van Der Straten, P.; Heideman, H.G.M.; Metcalf, H

    2001-01-01

    We have developed a new diagnostic tool for the study of Zeeman-compensated slowing of an alkali atomic beam. Our time-of-flight technique measures the longitudinal veloc- ity distribution of the slowed atoms with a resolution below the Doppler limit of 30 cm/s. Furthermore, it can map the position and velocity distribution of atoms in either ground hyperfine level inside the solenoid without any devices inside the solenoid. The technique reveals the optical pumping ef- fects, and shows in de...

  19. Reaction Mechanism of Oxygen Atoms with Unsaturated Hydrocarbons by the Crossed-Molecular-Beams Method

    Science.gov (United States)

    Buss, R. J.; Baseman, R. J.; Guozhong, H.; Lee, Y. T.

    1982-04-01

    From a series of studies of the reaction of oxygen atoms with unsaturated hydrocarbons using the crossed molecular beam method, the dominant reaction mechanisms were found to be the simple substitution reactions with oxygen atoms replacing H, Cl, Br atom or alkyl groups. Complication due to secondary reaction was avoided by carrying out experiments under single collisions and observing primary products directly. Primary products were identified by measuring the angular and velocity distributions of products at all the mass numbers which could be detected by the mass spectrometer, and from comparison of these distributions, applying the requirement of energy and momentum conservation.

  20. Atomic-scale thermocapillary flow in focused ion beam milling

    Energy Technology Data Exchange (ETDEWEB)

    Das, K.; Johnson, H. T.; Freund, J. B., E-mail: jbfreund@illinois.edu [Mechanical Science and Engineering and Aerospace Engineering, University of Illinois at Urbana–Champaign, 1206 West Green Street MC-244, Urbana, Illinois 61801 (United States)

    2015-05-15

    Focused ion beams provide a means of nanometer-scale manufacturing and material processing, which is used for applications such as forming nanometer-scale pores in thin films for DNA sequencing. We investigate such a configuration with Ga{sup +} bombardment of a Si thin-film target using molecular dynamics simulation. For a range of ion intensities in a realistic configuration, a recirculating melt region develops, which is seen to flow with a symmetrical pattern, counter to how it would flow were it driven by the ion momentum flux. Such flow is potentially important for the shape and composition of the formed structures. Relevant stress scales and estimated physical properties of silicon under these extreme conditions support the importance thermocapillary effects. A flow model with Marangoni forcing, based upon the temperature gradient and geometry from the atomistic simulation, indeed reproduces the flow and thus could be used to anticipate such flows and their influence in applications.

  1. Crossed-molecular-beams reactive scattering of oxygen atoms

    Energy Technology Data Exchange (ETDEWEB)

    Baseman, R.J.

    1982-11-01

    The reactions of O(/sup 3/P) with six prototypical unsaturated hydrocarbons, and the reaction of O(/sup 1/D) with HD, have been studied in high-resolution crossed-molecular-beams scattering experiments with mass-spectrometric detection. The observed laboratory-product angular and velocity distributions unambiguously identify parent-daughter ion pairs, distinguish different neutral sources of the same ion, and have been used to identify the primary products of the reactions. The derived center-of-mass product angular and translational energy distributions have been used to elucidate the detailed reaction dynamics. These results demonstrate that O(/sup 3/P)-unsaturated hydrocarbon chemistry is dominated by single bond cleavages, leading to radical products exclusively.

  2. Generation of Laguerre Gaussian beams using spiral phase diffractive elements fabricated on optical fiber tips using focused ion beam milling

    Science.gov (United States)

    Rodrigues Ribeiro, R. S.; Dahal, P.; Guerreiro, A.; Jorge, P. A. S.; Viegas, J.

    2016-03-01

    In this work, spiral phase lenses fabricated on the tip of single mode optical fibers are reported. This allows tailoring the fundamental guided mode, a Gaussian beam, into a Laguerre - Gaussian profile without using additional optical elements. The lenses are fabricated using Focused Ion Beam milling, enabling high resolution in the manufacturing process. The phase profiles are evaluated and validated using an implementation of the Finite Differences Time Domain. The output optical intensity profiles matching the numerical simulations are presented and analyzed. Finally, results on cell trapping and manipulation are briefly described.

  3. Roles of secondary electrons and sputtered atoms in ion-beam-induced deposition

    NARCIS (Netherlands)

    Chen, P.; Salemink, H.W.M.; Alkemade, P.F.A.

    2009-01-01

    The authors report the results of investigating two models for ion-beam-induced deposition (IBID). These models describe IBID in terms of the impact of secondary electrons and of sputtered atoms, respectively. The yields of deposition, sputtering, and secondary electron emission, as well as the ener

  4. Precision Atomic Physics Techniques for Nuclear Physics with Radioactive Beams

    CERN Document Server

    Blaum, Klaus; Nörtershäuser, Wilfried

    2012-01-01

    Atomic physics techniques for the determination of ground-state properties of radioactive isotopes are very sensitive and provide accurate masses, binding energies, Q-values, charge radii, spins, and electromagnetic moments. Many fields in nuclear physics benefit from these highly accurate numbers. They give insight into details of the nuclear structure for a better understanding of the underlying effective interactions, provide important input for studies of fundamental symmetries in physics, and help to understand the nucleosynthesis processes that are responsible for the observed chemical abundances in the Universe. Penning-trap and and storage-ring mass spectrometry as well as laser spectroscopy of radioactive nuclei have now been used for a long time but significant progress has been achieved in these fields within the last decade. The basic principles of laser spectroscopic investigations, Penning-trap and storage-ring mass measurements of short-lived nuclei are summarized and selected physics results a...

  5. Effects of the spatial frequency composition of the target pattern and the number of quantization levels in diffractive beam shaper design.

    Science.gov (United States)

    Hsu, Ku-Hui; Lin, Hoang Yan

    2012-06-01

    A mathematical model is derived, and numerical simulation is analyzed for laser beam shaping by using multilevel phase-only diffractive optical elements (DOEs). We used the simulated annealing algorithm to design the beam shapers. The result has an essential effect on the diffractive pattern quality caused by the spatial frequency composition of target patterns for the same incident gaussian beam size and target pattern area. The root mean square error between the diffractive and target patterns is smaller for the target patterns with lower spatial frequencies. Moreover, the effect of spatial frequency composition can be relaxed for the cases of larger incident gaussian beam size. In addition, finer quality control of a diffraction pattern can be obtained by increasing the number of quantization levels at the DOEs.

  6. Universal diffraction of atoms and molecules from a quantum reflection grating

    OpenAIRE

    Zhao, B.; W. Zhang; Schöllkopf, W.

    2016-01-01

    Since de Broglie’s work on the wave nature of particles, various optical phenomena have been observed with matter waves of atoms and molecules. However, the analogy between classical and atom/molecule optics is not exact because of different dispersion relations. In addition, according to de Broglie’s formula, different combinations of particle mass and velocity can give the same de Broglie wavelength. As a result, even for identical wavelengths, different molecular properties such as electri...

  7. Spatiospectral transmission of a plane-mirror Fabry-Perot interferometer with nonuniform finite-size diffraction beam illuminations.

    Science.gov (United States)

    Lee, Jae Yong; Hahn, Jae Won; Lee, Hai-Woong

    2002-05-01

    The transmission of a plane-mirror Fabry-Perot (PFP) interferometer is theoretically modeled and investigated by treating the spatial and spectral features in a unified manner. A spatiospectral transfer function is formulated and utilized to describe the beam propagation and the multiple-beam interference occurring in an ideal one-dimensional strip PFP interferometer with no diffraction loss. The spatial-frequency filtration of a finite-size beam input not only determines the transmitted spatial beam profile but also plays a crucial role in affecting the overall spectral transmittance. The inherent deviations of the spectral transmittance from what we know as the standard Airy's formula are revealed in diverse aspects, including the less-than-unity peak transmittance, the displacement of a resonance peak frequency, and the asymmetric detuning profile. Our theoretical analysis extends to the misaligned PFP interferometers, such as the cases in which non-normal-incidence beams or wedge-aligned mirrors are used that could severely degrade the effective interferometer finesse.

  8. Toward atomic resolution diffractive imaging of isolated molecules with x-ray free-electron lasers

    DEFF Research Database (Denmark)

    Stern, Stephan; Holmegaard, Lotte; Filsinger, Frank

    2014-01-01

    We give a detailed account of the theoretical analysis and the experimental results of an x-ray-diffraction experiment on quantum-state selected and strongly laser-aligned gas-phase ensembles of the prototypical large asymmetric rotor molecule 2,5-diiodobenzonitrile, performed at the Linac Cohere...

  9. Coherent and dynamic beam splitting based on light storage in cold atoms

    Science.gov (United States)

    Park, Kwang-Kyoon; Zhao, Tian-Ming; Lee, Jong-Chan; Chough, Young-Tak; Kim, Yoon-Ho

    2016-01-01

    We demonstrate a coherent and dynamic beam splitter based on light storage in cold atoms. An input weak laser pulse is first stored in a cold atom ensemble via electromagnetically-induced transparency (EIT). A set of counter-propagating control fields, applied at a later time, retrieves the stored pulse into two output spatial modes. The high visibility interference between the two output pulses clearly demonstrates that the beam splitting process is coherent. Furthermore, by manipulating the control lasers, it is possible to dynamically control the storage time, the power splitting ratio, the relative phase, and the optical frequencies of the output pulses. With further improvements, the active beam splitter demonstrated in this work might have applications in photonic photonic quantum information and in all-optical information processing. PMID:27677457

  10. Characterization of a SiC/SiC composite by X-ray diffraction, atomic force microscopy and positron spectroscopies

    Energy Technology Data Exchange (ETDEWEB)

    Brauer, G. [Institut fuer Ionenstrahlphysik und Materialforschung, Forschungszentrum Rossendorf e.V., PF 510119, D-01314 Dresden (Germany)]. E-mail: g.brauer@fz-rossendorf.de; Anwand, W. [Institut fuer Ionenstrahlphysik und Materialforschung, Forschungszentrum Rossendorf e.V., PF 510119, D-01314 Dresden (Germany); Eichhorn, F. [Institut fuer Ionenstrahlphysik und Materialforschung, Forschungszentrum Rossendorf e.V., PF 510119, D-01314 Dresden (Germany); Skorupa, W. [Institut fuer Ionenstrahlphysik und Materialforschung, Forschungszentrum Rossendorf e.V., PF 510119, D-01314 Dresden (Germany); Hofer, C. [Institut fuer Physik, Montanuniversitaet Leoben, Franz Josef Str. 18, A-8700 Leoben (Austria); Teichert, C. [Institut fuer Physik, Montanuniversitaet Leoben, Franz Josef Str. 18, A-8700 Leoben (Austria); Kuriplach, J. [Department of Low Temperature Physics, Faculty of Mathematics and Physics, Charles University, V Holesovickach 2, CZ-180 00 Prague (Czech Republic); Cizek, J. [Department of Low Temperature Physics, Faculty of Mathematics and Physics, Charles University, V Holesovickach 2, CZ-180 00 Prague (Czech Republic); Prochazka, I. [Department of Low Temperature Physics, Faculty of Mathematics and Physics, Charles University, V Holesovickach 2, CZ-180 00 Prague (Czech Republic); Coleman, P.G. [Department of Physics, University of Bath, Bath BA2 7 AY (United Kingdom); Nozawa, T. [Metals and Ceramics Division, Oak Ridge National Laboratory, P.O. Box 2008, MS6151, Oak Ridge, TN 37831-6151 (United States); Kohyama, A. [Institute of Advanced Energy, Kyoto University, Gokasho, Uji, Kyoto 611-0011 (Japan)

    2006-02-28

    A SiC/SiC composite is characterized by X-ray diffraction, atomic force microscopy and various positron spectroscopies (slow positron implantation, positron lifetime and re-emission). It is found that besides its main constituent 3C-SiC the composite still must contain some graphite. In order to better interpret the experimental findings of the composite, a pyrolytic graphite sample was also investigated by slow positron implantation and positron lifetime spectroscopies. In addition, theoretical calculations of positron properties of graphite are presented.

  11. 160 W high-power, high-efficiency, near-diffraction-limited beam quality all-fiber picosecond pulse laser

    Science.gov (United States)

    Sun, Chang; Ge, Tingwu; An, Na; Cao, Kang; Wang, Zhiyong

    2016-10-01

    We experimentally demonstrate a high-power, high-efficiency, near-diffraction-limited beam quality all-fiber picosecond pulse laser, which consists of a passively mode-locked seed laser and three-stage master power amplifiers. A repetition frequency multiplier and a high Yb-doped gain fiber with shorter length are utilized in the laser system to suppress the nonlinear effects and reduce the pulse broadening caused by dispersion. Moreover, the homemade light mode controllers based on a coiling and tapering fiber technique and the active fiber of the amplifier with a relatively small mode area are adopted to improve the beam quality. In addition, by experimentally adjusting the active fiber length, the optical conversion efficiency of the overall laser system can be optimized. Eventually, a 160 W high-power, high-efficiency, near-diffraction-limited picosecond pulse fiber laser is obtained, with the beam quality factor M2 at 1.12 and an optical conversion efficiency of the system of 75%.

  12. Radiation forces on a three-level atom in the high-order Bessel beams

    Institute of Scientific and Technical Information of China (English)

    Wang Zheng-Ling; Yin Jian-Ping

    2008-01-01

    The general expressions of the average dissipative and dipole forces acting on a A-configuration three-level atom in an arbitrary light field are derived by means of the optical Bloch equations based on the atomic density matrix elements, and the general properties of the average dissipative and dipole forces on a three-level atom in the linearly-polarized high-order Bessel beams (HBBs) are analysed. We find a resonant property (with two resonant peaks) of the dissipative force and a non-resonant property (with two pairs of non-resonant peaks) of the dipole force on the three-level atom, which are completely different from those on the two-level atom. Meanwhile we find a saturation effect of the average dissipative force in the HBB, which comes from the saturation of the upper-level population. Our study shows that the general expressions of the average dissipative and dipole forces on the three-level atom will be simplified to those of the two-level atom under the approximation of large detuning. Finally, we study the axial and azimuthal Doppler cooling of atoms in 1D optical molasses composed of two counter-propagating HBBs and discuss the azimuthal influence of the HBB on the Doppler cooling limit. We also find that the Doppler limit of atoms in the molasses HBB is slightly below the conventional Doppler limit of hг/(2кB) due to the orbital angular momentum lh of the HBB.

  13. Nonlinear effects in optical pumping of a cold and slow atomic beam

    KAUST Repository

    Porfido, N.

    2015-10-12

    By photoionizing hyperfine (HF) levels of the Cs state 62P3/2 in a slow and cold atom beam, we find how their population depends on the excitation laser power. The long time (around 180μs) spent by the slow atoms inside the resonant laser beam is large enough to enable exploration of a unique atom-light interaction regime heavily affected by time-dependent optical pumping. We demonstrate that, under such conditions, the onset of nonlinear effects in the population dynamics and optical pumping occurs at excitation laser intensities much smaller than the conventional respective saturation values. The evolution of population within the HF structure is calculated by numerical integration of the multilevel optical Bloch equations. The agreement between numerical results and experiment outcomes is excellent. All main features in the experimental findings are explained by the occurrence of “dark” and “bright” resonances leading to power-dependent branching coefficients.

  14. Preparation and Analysis of Atom Probe Tips by Xenon Focused Ion Beam Milling.

    Science.gov (United States)

    Estivill, Robert; Audoit, Guillaume; Barnes, Jean-Paul; Grenier, Adeline; Blavette, Didier

    2016-06-01

    The damage and ion distribution induced in Si by an inductively coupled plasma Xe focused ion beam was investigated by atom probe tomography. By using predefined patterns it was possible to prepare the atom probe tips with a sub 50 nm end radius in the ion beam microscope. The atom probe reconstruction shows good agreement with simulated implantation profiles and interplanar distances extracted from spatial distribution maps. The elemental profiles of O and C indicate co-implantation during the milling process. The presence of small disc-shaped Xe clusters are also found in the three-dimensional reconstruction. These are attributed to the presence of Xe nanocrystals or bubbles that open during the evaporation process. The expected accumulated dose points to a loss of >95% of the Xe during analysis, which escapes undetected.

  15. Atomic-scale thermocapillary flow in focused ion beam milling

    Science.gov (United States)

    Das, Kallol; Johnson, Harley; Freund, Jonathan

    2016-11-01

    Focused ion beams (FIB) offer an attractive tool for nanometer-scale manufacturing and material processing, particularly because they can be focused to a few nanometer diameter spot. This motivates their use for many applications, such as sample preparation for transmission electron microscopy (TEM), forming nanometer scale pores in thin films for DNA sequencing. Despite its widespread use, the specific mechanisms of FIB milling, especially at high ion fluxes for which significant phase change might occur, remains incompletely understood. Here we investigate the process of nanopore fabrication in thin Si films using molecular dynamics simulation where Ga+ ions are used as the focused ions. For a range of ion intensities in a realistic configuration, a recirculating melt region develops, which is seen to flow with a symmetrical pattern, counter to how it would flow were it is driven by the ion momentum flux. Such flow is potentially important for the shape and composition of the formed structures. Relevant stress scales and estimated physical properties of silicon under these extreme conditions support the importance thermocapillary effects. A continuum flow model with Marangoni forcing reproduces the flow.

  16. Diffraction of a Gaussian beam in a three-dimensional smoothly inhomogeneous medium: an eikonal-based complex geometrical-optics approach.

    Science.gov (United States)

    Berczynski, Pawel; Bliokh, Konstantin Yu; Kravtsov, Yuri A; Stateczny, Andrzej

    2006-06-01

    We present an ab initio account of the paraxial complex geometrical optics (CGO) in application to scalar Gaussian beam propagation and diffraction in a 3D smoothly inhomogeneous medium. The paraxial CGO deals with quadratic expansion of the complex eikonal and reduces the wave problem to the solution of ordinary differential equations of the Riccati type. This substantially simplifies the description of Gaussian beam diffraction as compared with full-wave or parabolic (quasi-optics) equations. For a Gaussian beam propagating in a homogeneous medium or along the symmetry axis in a lenslike medium, the CGO equations possess analytical solutions; otherwise, they can be readily solved numerically. As a nontrivial example we consider Gaussian beam propagation and diffraction along a helical ray in an axially symmetric waveguide medium. It is shown that the major axis of the beam's elliptical cross section grows unboundedly; it is oriented predominantly in the azimuthal (binormal) direction and does not obey the parallel-transport law.

  17. The Buffer Gas Beam: An Intense, Cold, and Slow Source for Atoms and Molecules

    CERN Document Server

    Hutzler, Nicholas R; Doyle, John M

    2011-01-01

    Beams of atoms and molecules are stalwart tools for spectroscopy and studies of collisional processes. The supersonic expansion technique can create cold beams of many species of atoms and molecules. However, the resulting beam is typically moving at a speed of 300-600 m/s in the lab frame, and for a large class of species has insufficient flux (i.e. brightness) for important applications. In contrast, buffer gas beams can be a superior method in many cases, producing cold and relatively slow molecules in the lab frame with high brightness and great versatility. There are basic differences between supersonic and buffer gas cooled beams regarding particular technological advantages and constraints. At present, it is clear that not all of the possible variations on the buffer gas method have been studied. In this review, we will present a survey of the current state of the art in buffer gas beams, and explore some of the possible future directions that these new methods might take.

  18. Influence of ion/atom arrival ratio on structure and optical properties of AlN films by ion beam assisted deposition

    Energy Technology Data Exchange (ETDEWEB)

    Meng, Jian-ping [Department of Energy Material and Technology, General Research Institute for Nonferrous Metals, Beijing 100088 (China); School of Engineering and Technology, China University of Geosciences, Beijing 100083 (China); Fu, Zhi-qiang, E-mail: fuzq@cugb.edu.cn [School of Engineering and Technology, China University of Geosciences, Beijing 100083 (China); Liu, Xiao-peng [Department of Energy Material and Technology, General Research Institute for Nonferrous Metals, Beijing 100088 (China); Yue, Wen; Wang, Cheng-biao [School of Engineering and Technology, China University of Geosciences, Beijing 100083 (China)

    2014-10-30

    Highlights: • AlN films were fabricated by dual ion beam sputtering. • Chemical bond status and phase composition of the films were studied by XPS and XRD. • Optical constants were measured by spectroscopic ellipsometry. • Influence of ion/atom arrival ratio on the films was studied. - Abstract: In order to improve the optical properties of AlN films, the influence of the ion/atom arrival ratio on the structure and optical characteristics of AlN films deposited by dual ion beam sputtering was studied by using X-ray diffraction, scanning electron microscopy, X-ray photoelectron spectroscopy, spectroscopic ellipsometry and UV–vis spectroscopy. The films prepared at the ion/atom arrival ratio of 1.4 are amorphous while the crystalline quality is improved with the increase of the ion/atom arrival ratio. The films deposited at the ion/atom arrival ratio of no less than 1.8 have an approximately stoichiometric ratio and mainly consist of aluminum nitride with little aluminum oxynitride, while metallic aluminum component appears in the films deposited at the ion/atom arrival ratio of 1.4. When the ion/atom arrival ratio is not less than 1.8, films are smooth, high transmitting and dense. The films prepared with high ion/atom arrival ratio (≥1.8) display the characteristic of a dielectric. The films deposited at the ion/atom arrival ratio of 1.4 are coarse, opaque and show characteristic of cermet.

  19. Dislocation-based plasticity model and micro-beam Laue diffraction analysis of polycrystalline Ni foil: A forward prediction

    Science.gov (United States)

    Song, Xu; Hofmann, Felix; Korsunsky, Alexander M.

    2010-10-01

    A physically-based, rate and length-scale dependent strain gradient crystal plasticity framework was employed to simulate the polycrystalline plastic deformation at the microscopic level in a large-grained, commercially pure Ni sample. The latter was characterised in terms of the grain morphology and orientation (in the bulk) by micro-beam Laue diffraction experiments carried out on beamline B16 at Diamond Light Source. The corresponding finite element model was developed using a grain-based mesh with the specific grain orientation assignment appropriate for the sample considered. Sample stretching to 2% plastic strain was simulated, and a post-processor was developed to extract the information about the local lattice misorientation (curvature), enabling forward-prediction of the Laue diffraction patterns. The 'streaking' phenomenon of the Laue spots (anisotropic broadening of two-dimensional (2D) diffraction peaks observed on the 2D detector) was correctly captured by the simulation, as constructed by direct superposition of reflections from different integration points within the diffraction gauge volume. Good agreement was found between the images collected from experiments and simulation patterns at various positions in the sample.

  20. Characterization of the Absolute Crystal Polarity across Twin Boundaries in Gallium Phosphide Using Convergent-Beam Electron Diffraction.

    Science.gov (United States)

    Cohen; McKernan; Carter

    1999-05-01

    : The measurement of absolute crystal polarity is crucial to understanding the structural properties of many planar defects in compound semiconductors. Grain boundaries, including twin boundaries, in the sphalerite lattice are uniquely characterized by the crystallographic misorientation of individual grains and the direction of the crystal polarity in domains adjoining the grain boundary. To evaluate crystal polarity in gallium phosphide (GaP), asymmetrical interference contrast in convergent-beam electron-diffraction (CBED) patterns was used to ascertain the nature and direction of polar bonds. The direction of the asymmetry in the electron diffraction reflections was correlated with the crystal polarity of a sample with known polarity. The CBED technique was applied to determine the polar orientation of grains adjoining Sigma = 3 coherent and lateral twin boundaries in polycrystalline GaP.

  1. Consistency of atomic data for the interpretation of beam emission spectra

    Energy Technology Data Exchange (ETDEWEB)

    Delabie, E; Von Hellermann, M G [FOM Institute for Plasma Physics Rijnhuizen, Association EURATOM-FOM, PO Box 1207, 3430 BE Nieuwegein (Netherlands); Brix, M; Giroud, C; Surrey, E; Zastrow, K D [EURATOM/CCFE Association, Culham Science Centre, Abingdon, OX14 3DB (United Kingdom); Jaspers, R J E [Eindhoven University of Technology, Postbus 513, 5600 MB Eindhoven (Netherlands); Marchuk, O [Forschungszentrum Juelich, Association EURATOM-FZJ, 52425, Juelich (Germany); O' Mullane, M G [Department of Physics, University of Strathclyde, 107 Rottenrow, Glasgow G4 0NG (United Kingdom); Ralchenko, Yu, E-mail: e.delabie@fz-juelich.d [Atomic Physics Division, National Institute of Standards and Technology, Gaithersburg, MD 20899-8422 (United States)

    2010-12-15

    Several collisional-radiative (CR) models (Anderson et al 2000 Plasma Phys. Control. Fusion 42 781-806, Hutchinson 2002 Plasma Phys. Control. Fusion 44 71-82, Marchuk et al 2008 Rev. Sci. Instrum. 79 10F532) have been developed to calculate the attenuation and the population of excited states of hydrogen or deuterium beams injected into tokamak plasmas. The datasets generated by these CR models are needed for the modelling of beam ion deposition and (excited) beam densities in current experiments, and the reliability of these data will be crucial to obtain helium ash densities on ITER combining charge exchange and beam emission spectroscopy. Good agreement between the different CR models for the neutral beam (NB) is found, if corrections to the fundamental cross sections are taken into account. First the H{sub {alpha}} and H{sub {beta}} beam emission spectra from JET are compared with the expected intensities. Second, the line ratios within the Stark multiplet are compared with the predictions of a sublevel resolved model. The measured intensity of the full multiplet is {approx}30% lower than expected on the basis of beam attenuation codes and the updated beam emission rates, but apart from the atomic data this could also be due to the characterization of the NB path and line of sight integration and the absolute calibration of the optics. The modelled n = 3 to n = 4 population agrees very well with the ratio of the measured H{sub {alpha}} to H{sub {beta}} beam emission intensities. Good agreement is found as well between the NB power fractions measured with beam emission in plasma and on the JET Neutral Beam Test Bed. The Stark line ratios and {sigma}/{pi} intensity ratio deviate from a statistical distribution, in agreement with the CR model in parabolic states from Marchuk et al (2010 J. Phys. B: At. Mol. Opt. Phys. 43 011002).

  2. In situ x-ray diffraction measurements of the capillary fountain jet produced via ultrasonic atomization

    Science.gov (United States)

    Yano, Yohko F.; Douguchi, Junya; Kumagai, Atsushi; Iijima, Takao; Tomida, Yukinobu; Miyamoto, Toshiaki; Matsuura, Kazuo

    2006-11-01

    In situ x-ray diffraction measurements were carried out for investigating the liquid structure in the ultrasonic fountain jet to consider the mechanism of the "ultrasonic ethanol separation" reported by Sato et al. [J. Chem. Phys. 114, 2382 (2001)]. For pure liquids (water and ethanol), it was found that the high frequency ultrasound does not affect the liquid structure microscopically. For the 20mol% ethanol-water mixture, the estimated ethanol mole fraction in the ultrasonic fountain jet by using the position of the main maximum in the x-ray diffraction profile coincided with that in the reservoir. This result suggests that the ethanol separation is not caused by any distorted liquid structure under the ultrasound irradiation and occurs when or after the generation of the liquid droplet mist.

  3. Third-dimension information retrieval from a single convergent-beam transmission electron diffraction pattern using an artificial neural network

    Science.gov (United States)

    Pennington, Robert S.; Van den Broek, Wouter; Koch, Christoph T.

    2014-05-01

    We have reconstructed third-dimension specimen information from convergent-beam electron diffraction (CBED) patterns simulated using the stacked-Bloch-wave method. By reformulating the stacked-Bloch-wave formalism as an artificial neural network and optimizing with resilient back propagation, we demonstrate specimen orientation reconstructions with depth resolutions down to 5 nm. To show our algorithm's ability to analyze realistic data, we also discuss and demonstrate our algorithm reconstructing from noisy data and using a limited number of CBED disks. Applicability of this reconstruction algorithm to other specimen parameters is discussed.

  4. A diffracted-beam monochromator for long linear detectors in X-ray diffractometers with Bragg-Brentano parafocusing geometry.

    Science.gov (United States)

    van der Pers, N M; Hendrikx, R W A; Delhez, R; Böttger, A J

    2013-04-01

    A new diffracted-beam monochromator has been developed for Bragg-Brentano X-ray diffractometers equipped with a linear detector. The monochromator consists of a cone-shaped graphite highly oriented pyrolytic graphite crystal oriented out of the equatorial plane such that the parafocusing geometry is preserved over the whole opening angle of the linear detector. In our standard setup a maximum wavelength discrimination of 3% is achieved with an overall efficiency of 20% and a small decrease in angular resolution of only 0.02 °2θ. In principle, an energy resolution as low as 1.5% can be achieved.

  5. International Atomic Energy Agency intercomparison of ion beam analysis software

    Science.gov (United States)

    Barradas, N. P.; Arstila, K.; Battistig, G.; Bianconi, M.; Dytlewski, N.; Jeynes, C.; Kótai, E.; Lulli, G.; Mayer, M.; Rauhala, E.; Szilágyi, E.; Thompson, M.

    2007-09-01

    Ion beam analysis (IBA) includes a group of techniques for the determination of elemental concentration depth profiles of thin film materials. Often the final results rely on simulations, fits and calculations, made by dedicated codes written for specific techniques. Here we evaluate numerical codes dedicated to the analysis of Rutherford backscattering spectrometry, non-Rutherford elastic backscattering spectrometry, elastic recoil detection analysis and non-resonant nuclear reaction analysis data. Several software packages have been presented and made available to the community. New codes regularly appear, and old codes continue to be used and occasionally updated and expanded. However, those codes have to date not been validated, or even compared to each other. Consequently, IBA practitioners use codes whose validity, correctness and accuracy have never been validated beyond the authors' efforts. In this work, we present the results of an IBA software intercomparison exercise, where seven different packages participated. These were DEPTH, GISA, DataFurnace (NDF), RBX, RUMP, SIMNRA (all analytical codes) and MCERD (a Monte Carlo code). In a first step, a series of simulations were defined, testing different capabilities of the codes, for fixed conditions. In a second step, a set of real experimental data were analysed. The main conclusion is that the codes perform well within the limits of their design, and that the largest differences in the results obtained are due to differences in the fundamental databases used (stopping power and scattering cross section). In particular, spectra can be calculated including Rutherford cross sections with screening, energy resolution convolutions including energy straggling, and pileup effects, with agreement between the codes available at the 0.1% level. This same agreement is also available for the non-RBS techniques. This agreement is not limited to calculation of spectra from particular structures with predetermined

  6. The polarized H and D atomic beam source for ANKE at COSY-Jülich

    Energy Technology Data Exchange (ETDEWEB)

    Mikirtychyants, M., E-mail: m.mikirtychyants@fz-juelich.de [Institut für Kernphysik, Forschungszentrum Jülich, 52425 Jülich (Germany); High Energy Physics Department, St.Petersburg Nuclear Physics Institute, 188300 Gatchina (Russian Federation); Engels, R. [Institut für Kernphysik, Forschungszentrum Jülich, 52425 Jülich (Germany); Grigoryev, K. [Institut für Kernphysik, Forschungszentrum Jülich, 52425 Jülich (Germany); High Energy Physics Department, St.Petersburg Nuclear Physics Institute, 188300 Gatchina (Russian Federation); Kleines, H. [Zentrallabor für Elektronik, Forschungszentrum Jülich, 52425 Jülich (Germany); Kravtsov, P. [High Energy Physics Department, St.Petersburg Nuclear Physics Institute, 188300 Gatchina (Russian Federation); Lorenz, S. [Physikalisches Institut, Friedrich-Alexander-Universität Erlangen-Nürnberg, 91058 Erlangen (Germany); Nekipelov, M. [Institut für Kernphysik, Forschungszentrum Jülich, 52425 Jülich (Germany); High Energy Physics Department, St.Petersburg Nuclear Physics Institute, 188300 Gatchina (Russian Federation); Nelyubin, V. [High Energy Physics Department, St.Petersburg Nuclear Physics Institute, 188300 Gatchina (Russian Federation); Rathmann, F.; Sarkadi, J. [Institut für Kernphysik, Forschungszentrum Jülich, 52425 Jülich (Germany); and others

    2013-09-01

    A polarized atomic beam source was developed for the polarized internal storage-cell gas target at the magnet spectrometer ANKE of COSY-Jülich. The intensities of the beams injected into the storage cell, measured with a compression tube, are 7.5×10{sup 16} hydrogen atoms/s (two hyperfine states) and 3.9×10{sup 16} deuterium atoms/s (three hyperfine states). For the hydrogen beam the achieved vector polarizations are p{sub z}≈±0.92. For the deuterium beam, the obtained combinations of vector and tensor (p{sub zz}) polarizations are p{sub z}≈±0.90 (with a constant p{sub zz}≈+0.86), and p{sub zz}=+0.90 or p{sub zz}=−1.71 (both with vanishing p{sub z}). The paper includes a detailed technical description of the apparatus and of the investigations performed during the development. This source has been very successfully used for single and double polarization measurements at ANKE as well as for studies of the polarization of recombining hydrogen molecules.

  7. Ultra Stable, Industrial Green Tailored Pulse Fiber Laser with Diffraction-limited Beam Quality for Advanced Micromachining

    Energy Technology Data Exchange (ETDEWEB)

    Deladurantaye, P; Roy, V; Desbiens, L; Drolet, M; Taillon, Y; Galarneau, P, E-mail: pascal.deladurantaye@ino.ca [INO, 2740 rue Einstein, Quebec City, QC, G1P 4S4 (Canada)

    2011-02-01

    We report on a novel pulsed fiber laser platform providing pulse shaping agility at high repetition rates and at a wavelength of 532 nm. The oscillator is based on the direct modulation of a seed laser diode followed by a chain of fiber amplifiers. Advanced Large Mode Area (LMA) fiber designs as well as proprietary techniques to mitigate non-linear effects enable output energy per pulse up to 100 {mu}J at 1064 nm with diffraction-limited beam quality and narrow line widths suitable for efficient frequency conversion. Ultra stable pulses with tailored pulse shapes were demonstrated in the green region of the spectrum at repetition rates higher than 200 kHz. Pulse durations between 2.5 ns and 640 ns are available, as well as pulse to pulse dynamic shape selection at repetition rates up to 1 MHz. The pulse energy stability at 532 nm is better than {+-} 1.5%, 3{sigma}, over 10 000 pulses. Excellent beam characteristics were obtained. The M{sup 2} parameter is lower than 1.05, the beam waist astigmatism and beam waist asymmetry are below 10% and below 8% respectively, with high stability over time. We foresee that the small spot size, high repetition rate and pulse tailoring capability of this platform will provide advantages to practitioners who are developing novel, advanced processes in many industrially important applications.

  8. Atomic ordering and systematics of bonding lengths in the Ti-V omega phase: a neutron diffraction study

    Energy Technology Data Exchange (ETDEWEB)

    Benites, G.M.; Guillermet, A.F. [Consejo Nacional de Investigaciones Cientificas y Tecnicas, Centro Atomico Bariloche (Argentina); Aurelio, G. [Universidad Nacional del Comahue, Buenos Aires 1400, 8300 Neuquen (Argentina); Cuello, G.J.; Bermejo, F.J. [Instituto de Estructura de la Materia, Consejo Superior de Investigaciones Cientificas y Tecnicas, Serrano 123, Madrid E-28006 (Spain)

    1999-03-04

    A new model describing the structural and bonding properties of the omega ({Omega}) phase in Zr-Nb alloys has recently been presented [12]. This model, which was aimed at explaining the composition dependence of the bonding lengths, predicts that the {Omega} phase is ordered, i.e., that some crystallographic sites are preferentially occupied by Zr atoms. Such feature, which should in principle be observed in other, related {Omega} phases, has not yet been tested against direct measurements. This problem has now been studied in the Ti-V system, which is the analogue of Zr-Nb in the 3d-transition series. Neutron diffraction measurements have been performed in quenched Ti-V alloys with V contents between 14 and 17 at.%. The diffraction spectra have been analysed using the Rietveld method, and a systematic analysis is reported here of the possibility of deviations from the random occupation of the two sublattices which are distinguished in the {Omega} structure. In addition, these new diffraction data are used in an evaluation of the shortest interatomic distances which are relevant for a comparison with the predictions of the model of Grad et al. (orig.) 28 refs.

  9. On amplitude beam splitting of tender X-rays (2-8 keV photon energy) using conical diffraction from reflection gratings with laminar profile.

    Science.gov (United States)

    Jark, Werner; Eichert, Diane

    2016-01-01

    Conical diffraction is obtained when a radiation beam impinges onto a periodically ruled surface structure parallel or almost parallel to the ruling. In this condition the incident intensity is diffracted through an arc, away from the plane of incidence. The diffracted intensity thus lies on a cone, which leads to the name `conical diffraction'. In this configuration almost no part of the ruled structure will produce any shadowing effect for the incident or the diffracted beam. Then, compared with a grating in the classical orientation, relatively higher diffraction efficiencies will be observed for fewer diffraction orders. When the incident beam is perfectly parallel to the grooves of a rectangular grating profile, the symmetry of the setup causes diffraction of the intensity symmetrically around the plane of incidence. This situation was previously tested experimentally in the VUV spectral range for the amplitude beam splitting of a radiation beam with a photon energy of 25 eV. In this case the ideally expected beam splitting efficiency of about 80% for the diffraction into the two first orders was confirmed for the optimum combination of groove depth and angle of grazing incidence. The feasibility of the amplitude beam splitting for hard X-rays with 12 keV photon energy by use of the same concept was theoretically confirmed. However, no related experimental data are presented yet, not even for lower energy soft X-rays. The present study reports the first experimental data for the conical diffraction from a rectangular grating profile in the tender X-ray range for photon energies of 4 keV and 6 keV. The expected symmetries are observed. The maximum absolute efficiency for beam splitting was measured to be only about 30%. As the reflectivity of the grating coating at the corresponding angle of grazing incidence was found to be only of the order of 50%, the relative beam splitting efficiency was thus 60%. This is to be compared also here with an ideally

  10. Diffraction Studies of the Atomic Vibrations of Bulk and Surface Atoms in the Reciprocal and Real Spaces of Nanocrystalline SiC

    Science.gov (United States)

    Stelmakh, S.; Grzanka, E.; Weber, H.-P.; Vogel, S.; Palosz, B.; Palosz, B.

    2004-01-01

    To describe and evaluate the vibrational properties of nanoparticles it is necessary to distinguish between the surface and the core of the particles. Theoretical calculations show that vibrational density of states of the inner atoms of nanograins is similar to bulk material but shifted to higher energies which can be explained by the fact that the gain core is stressed (hardened) due to the presence of internal pressure. Theoretical calculations also show that there is a difference between vibrational properties of a crystal lattice of the grain interior in isolated particles and in a dense (sintered) nanocrystalline material. This is probably due to a coupling of the modes inside the grains via the grain boundaries in dense nanocrystalline bodies. We examined strains present in the surface shell based on examination of diamond and Sic nanocrystals in reciprocal (Bragg-type scattering) and real (PDF analysis) space analysis of neutron diffraction data. Recently we examined the atomic thermal motions in nanocrystalline Sic based on the assumption of a simple Einstein model for uncorrelated atomic notions. According to this model, the Bragg intensity is attenuated as a function of scattering angle by the Debye-Waller factor. Based on this assumption overall temperature factors were determined from the Wilson plots.

  11. Ion-beam induced atomic mixing in isotopically controlled silicon multilayers

    Science.gov (United States)

    Radek, M.; Bracht, H.; Liedke, B.; Böttger, R.; Posselt, M.

    2016-11-01

    Implantation of germanium (Ge), gallium (Ga), and arsenic (As) into crystalline and preamorphized isotopically controlled silicon (Si) multilayer structures at temperatures between 153 K and 973 K was performed to study the mechanisms mediating ion-beam induced atomic mixing. Secondary-ion-mass-spectrometry was applied to determine concentration-depth profiles of the stable isotopes before and after ion implantation. The intermixing is analytically described by a depth-dependent displacement function. The maximum displacement is found to depend not only on temperature and microstructure but also on the doping type of the implanted ion. Molecular dynamics calculations evaluate the contribution of cascade mixing, i.e., thermal-spike mixing, to the overall observed atomic mixing. Calculated and experimental results on the temperature dependence of ion-beam mixing in the amorphous and crystalline structures provide strong evidence for ion-beam induced enhanced crystallization and enhanced self-diffusion, respectively. On the other hand, the former process is confirmed by channeling Rutherford backscattering analyses of the amorphous layer thickness remaining after implantation, the latter process is consistently attributed to the formation of highly mobile Si di-interstitials formed under irradiation and in the course of damage annealing. The observed ion-beam mixing in Si is compared to recent results on ion-beam mixing of Ge isotope multilayers that, in contrast to Si, are fully described by thermal-spike mixing only.

  12. Assessment of Shape Memory Alloys - From Atoms To Actuators - Via In Situ Neutron Diffraction

    Science.gov (United States)

    Benafan, Othmane

    2014-01-01

    As shape memory alloys (SMAs) become an established actuator technology, it is important to identify the fundamental mechanisms responsible for their performance by understanding microstructure performance relationships from processing to final form. Yet, microstructural examination of SMAs at stress and temperature is often a challenge since structural changes occur with stress and temperature and microstructures cannot be preserved through quenching or after stress removal, as would be the case for conventional materials. One solution to this dilemma is in situ neutron diffraction, which has been applied to the investigation of SMAs and has offered a unique approach to reveal the fundamental micromechanics and microstructural aspects of bulk SMAs in a non-destructive setting. Through this technique, it is possible to directly correlate the micromechanical responses (e.g., internal residual stresses, lattice strains), microstructural evolutions (e.g., texture, defects) and phase transformation properties (e.g., phase fractions, kinetics) to the macroscopic actuator behavior. In this work, in situ neutron diffraction was systematically employed to evaluate the deformation and transformation behavior of SMAs under typical actuator conditions. Austenite and martensite phases, yield behavior, variant selection and transformation temperatures were characterized for a polycrystalline NiTi (49.9 at. Ni). As the alloy transforms under thermomechanical loading, the measured textures and lattice plane-level variations were directly related to the cyclic actuation-strain characteristics and the dimensional instability (strain ratcheting) commonly observed in this alloy. The effect of training on the shape memory characteristics of the alloy and the development of two-way shape memory effect (TWSME) were also assessed. The final conversion from a material to a useful actuator, typically termed shape setting, was also investigated in situ during constrained heatingcooling and

  13. Discrete Energies of a Weakly Outcoupled Atom Laser Beam Outside the Bose–Einstein Condensate Region

    Directory of Open Access Journals (Sweden)

    Teguh Budi Prayitno

    2014-12-01

    Full Text Available We consider the possibility of a discrete set of energies of a weakly outcoupled atom laser beam to the homogeneous Schrödinger equation with anisotropic harmonic trap in Cartesian coordinates outside the Bose–Einstein condensate region. This treatment is used because working in the cylindrical coordinates is not really possible, even though we implement the cigar-shaped trap case. The Schrödinger equation appears to replace a set of two-coupled Gross– Pitaevskii equations by enabling the weak-coupling assumption. This atom laser can be produced in a simple way that only involves extracting the atoms in a condensate from by using the radio frequency field. We initially present the relation between condensates as sources and atom laser as an output by exploring the previous work of Riou et al. in the case of theoretical work for the propagation of atom laser beams. We also show that even though the discrete energies are obtained by means of an approaching harmonic oscillator, degeneracy is only available in two states because of the anisotropic external potential

  14. Diffractive Combiner of Single-Mode Pump Laser-Diode Beams

    Science.gov (United States)

    Liu, Duncan; Wilson, Daniel; Qiu, Yueming; Forouhar, Siamak

    2007-01-01

    An optical beam combiner now under development would make it possible to use the outputs of multiple single-mode laser diodes to pump a neodymium: yttrium aluminum garnet (Nd:YAG) nonplanar ring oscillator (NPRO) laser while ensuring that the laser operates at only a single desired frequency. Heretofore, an Nd:YAG NPRO like the present one has been pumped by a single multimode laser-diode beam delivered via an optical fiber. It would be desirable to use multiple pump laser diodes to increase reliability beyond that obtainable from a single pump laser diode. However, as explained below, simplistically coupling multiple multimode laser-diode beams through a fiber-optic combiner would entail a significant reduction in coupling efficiency, and lasing would occur at one or more other frequencies in addition to the single desired frequency. Figure 1 schematically illustrates the principle of operation of a laser-diode-pumped Nd:YAG NPRO. The laser beam path is confined in a Nd:YAG crystal by means of total internal reflections on the three back facets and a partial-reflection coating on the front facet. The wavelength of the pump beam - 808 nm - is the wavelength most strongly absorbed by the Nd:YAG crystal. The crystal can lase at a wavelength of either 1,064 nm or 1,319 nm - which one depending on the optical coating on the front facet. A thermal lens effect induced by the pump beam enables stable lasing in the lowest-order transverse electromagnetic mode (the TEM00 mode). The frequency of this laser is very stable because of the mechanical stability of the laser crystal and the unidirectional nature of the lasing. The unidirectionality is a result of the combined effects of (1) a Faraday rotation induced by an externally applied magnetic field and (2) polarization associated with non-normal incidence and reflection on the front facet.

  15. Precision measurement of transverse velocity distribution of a Strontium atomic beam

    CERN Document Server

    Gao, F; Xu, P; Tian, X; Wang, Y; Ren, J; Wu, Haibin; Chang, Hong

    2013-01-01

    We measure precisely the transverse velocity distribution in a thermal Sr atomic beam with a velocity selective saturated fluorescence spectroscopy. By using the ultrastable laser system and narrow intercombination transition line of Sr atoms, the resolution of the velocity measured can be reached 0.13m/s, corresponding to 90$\\mu K$ in energy unit. The experimental results are agreement very well with a theoretical calculation. With the spectroscopic techniques, the absolute frequency of the intercombination transition of $^{88}$Sr is measured by an optical-frequency comb generator referenced to the SI second through an H maser, which is given by 434 829 121 318(10)kHz.

  16. Observation of strong virtual scattering under three-beam (220, 371) X-ray diffraction in TeO{sub 2} single crystal

    Energy Technology Data Exchange (ETDEWEB)

    Blagov, A. E.; Kovalchuk, M. V. [Russian Academy of Sciences, Shubnikov Institute of Crystallography (Russian Federation); Kohn, V. G. [Kurchatov Institute, Russian Research Centre (Russian Federation); Pisarevskii, Yu. V.; Prosekov, P. A., E-mail: aopt@ns.crys.ras.ru [Russian Academy of Sciences, Shubnikov Institute of Crystallography (Russian Federation)

    2010-01-15

    A strong effect of virtual scattering has been experimentally observed when studying the nearly coplanar three-beam (220, 371) X-ray diffraction in a paratellurite single crystal under high-resolution double-crystal X-ray diffraction using MoK{sub {alpha}1} radiation. One characteristic feature of this effect is that the angular dependence of the first (strong) reflection intensity and its shape barely change in the three-beam range of parameters, whereas very strong changes are observed for the second (weak) reflection not only in the three-beam range but also far beyond it, which is related to the variation in the two-beam diffraction parameter due to virtual scattering. The changes observed are asymmetric and make it possible to determine the triplet combination of structure-factor phases.

  17. X-ray diffraction imaging with the Multiple Inverse Fan Beam topology: principles, performance and potential for security screening.

    Science.gov (United States)

    Harding, G; Fleckenstein, H; Kosciesza, D; Olesinski, S; Strecker, H; Theedt, T; Zienert, G

    2012-07-01

    The steadily increasing number of explosive threat classes, including home-made explosives (HMEs), liquids, amorphous and gels (LAGs), is forcing up the false-alarm rates of security screening equipment. This development can best be countered by increasing the number of features available for classification. X-ray diffraction intrinsically offers multiple features for both solid and LAGs explosive detection, and is thus becoming increasingly important for false-alarm and cost reduction in both carry-on and checked baggage security screening. Following a brief introduction to X-ray diffraction imaging (XDI), which synthesizes in a single modality the image-forming and material-analysis capabilities of X-rays, the Multiple Inverse Fan Beam (MIFB) XDI topology is described. Physical relationships obtaining in such MIFB XDI components as the radiation source, collimators and room-temperature detectors are presented with experimental performances that have been achieved. Representative X-ray diffraction profiles of threat substances measured with a laboratory MIFB XDI system are displayed. The performance of Next-Generation (MIFB) XDI relative to that of the 2nd Generation XRD 3500TM screener (Morpho Detection Germany GmbH) is assessed. The potential of MIFB XDI, both for reducing the exorbitant cost of false alarms in hold baggage screening (HBS), as well as for combining "in situ" liquid and solid explosive detection in carry-on luggage screening is outlined.

  18. Crossed beam reactive scattering of oxygen atoms and surface scattering studies of gaseous condensation

    Energy Technology Data Exchange (ETDEWEB)

    Sibener, S.J.

    1979-09-01

    A high pressure, radio frequency discharge nozzle beam source was developed for the production of very intense (greater than or equal to 10/sup 18/ atoms sr/sup -1/ sec/sup -1/) supersonic beams of oxygen atoms. This source is capable of producing seeded beams of ground state O(/sup 3/P/sub J/) atoms when dilute oxygen-argon mixtures are used, with molecular dissociation levels exceeding 80% being realized for operation at pressures up to 350 torr. When dilute oxygen-helium mixtures are employed both ground state O(/sup 3/P/sub J/) and excited state O(/sup 1/D/sub 2/) atoms are present in the terminal beam, with molecular dissociation levels typically exceeding 60% being achieved for operation at pressures up to 200 torr. Atomic oxygen mean translational energies from 0.14 to 0.50 eV were obtained using the seeded beams technique, with Mach numbers as high as 10 (FWHM ..delta.. v/v approx. = 20%) being realized. The IC1, CF/sub 3/I, C/sub 6/H/sub 6/, and C/sub 6/D/sub 6/ reactions are discussed in detail. The IC1 and CF/sub 3/I studies have enabled us to determine an improved value for the bond energy of the IO radical: D/sub o/(IO) = 55 +- 2 kcal/mole. The IO product angular and velocity distributions have been used to generate center-of-mass flux contour maps, which indicate that these two reactions proceed via relatively long-lived collision complexes whose mean lifetimes are slightly shorter than their respective rotational periods. The O(/sup 3/P/sub J/) + C/sub 6/H/sub 6/ and C/sub 6/D/sub 6/ reactions were studied in order to elucidate the reaction mechanism, and, in particular, to identify the primary reaction products produced in these reactions. Finally, a series of beam-surface scattering experiments are described which examined the internal and translational energy dependence of molecular condensation probabilities for collisions involving either CC1/sub 4/ or SF/sub 6/ and their respective condensed phases. 117 references. (JFP)

  19. Generation of neutral atomic beams utilizing photodetachment by high power diode laser stacks

    Science.gov (United States)

    O'Connor, A. P.; Grussie, F.; Bruhns, H.; de Ruette, N.; Koenning, T. P.; Miller, K. A.; Savin, D. W.; Stützel, J.; Urbain, X.; Kreckel, H.

    2015-11-01

    We demonstrate the use of high power diode laser stacks to photodetach fast hydrogen and carbon anions and produce ground term neutral atomic beams. We achieve photodetachment efficiencies of ˜7.4% for H- at a beam energy of 10 keV and ˜3.7% for C- at 28 keV. The diode laser systems used here operate at 975 nm and 808 nm, respectively, and provide high continuous power levels of up to 2 kW, without the need of additional enhancements like optical cavities. The alignment of the beams is straightforward and operation at constant power levels is very stable, while maintenance is minimal. We present a dedicated photodetachment setup that is suitable to efficiently neutralize the majority of stable negative ions in the periodic table.

  20. Applications of beam-foil spectroscopy to atomic collisions in solids

    Science.gov (United States)

    Sellin, I. A.

    1976-01-01

    Some selected papers presented at the Fourth International Conference on Beam-Foil Spectroscopy, whose results are of particular pertinence to ionic collision phenomena in solids, are reviewed. The topics discussed include solid target effects and means of surmounting them in the measurement of excited projectile ion lifetimes for low-energy heavy element ions; the electron emission accompanying the passage of heavy particles through solid targets; the collision broadening of X rays emitted from 100 keV ions moving in solids; residual K-shell excitation in chlorine ions penetrating carbon; comparison between 40 MeV Si on gaseous SiH4 targets at 300 mtorr and 40 MeV Si on Al; and the emergent surface interaction in beam-foil spectroscopy. A distinct overlap of interests between the sciences of beam-foil spectroscopy and atomic collisions in solids is pointed out.

  1. Generation of neutral atomic beams utilizing photodetachment by high power diode laser stacks

    CERN Document Server

    O'Connor, A P; Grussie, F; Koenning, T P; Miller, K A; de Ruette, N; Stützel, J; Savin, D W; Urbain, X; Kreckel, H

    2015-01-01

    We demonstrate the use of high power diode laser stacks to photodetach fast hydrogen and carbon anions and produce ground term neutral atomic beams. We achieve photodetachment efficiencies of $\\sim$7.4\\% for H$^-$ at a beam energy of 10\\,keV and $\\sim$3.7\\% for C$^-$ at 28\\,keV. The diode laser systems used here operate at 975\\,nm and 808\\,nm, respectively, and provide high continuous power levels of up to 2\\,kW, without the need of additional enhancements like optical cavities. The alignment of the beams is straightforward and operation at constant power levels is very stable, while maintenance is minimal. We present a dedicated photodetachment setup that is suitable to efficiently neutralize the majority of stable negative ions in the periodic table.

  2. OPTIMIZATION AND CHARACTERIZATION OF ELECTRON BEAM RESIST USING ATOMIC FORCE MICROSCOPY

    Directory of Open Access Journals (Sweden)

    - Sutikno

    2012-01-01

    Full Text Available Resis negatif ma-N 2403 dan 495 K PMMA memiliki resolusi yang baik untuk aplikasi litografi berkas elektron (EBL. Ketebalanresist optimal memainkan peran penting dalam paparan berkas elektron. Oleh karena itu, dalam penelitian ini, ketebalan darikedua resist yang dioptimalkan menggunakan spincoater dalam jangkauan laju spin 1000-6000 rpm. Semakin laju spin meningkat,ketebalan resist menurun juga. Morfologi permukaan resist dikarakterisasi dengan mikroskop gaya atom. Butir butir resist nampakpanjang. Dalam analisis AFM, permukaan profil resist negatif ma-N 2403 dan 495 K PMMA nampak seperti kerucut. Negative resist ma-N 2403 and 495 K PMMA have good resolution for electron beam lithography (EBL application. The optimumresist thickness plays significant role in e-beam exposure. Therefore, in this research, thicknesses of both resists were optimizedusing spincoater within spin speeds of 1000-6000 rpm. As spin speed increased, resist thickness decreased as well. Morphology ofresist surfaces were characterized using atomic force microscopy (AFM. Grains of resist show long grains. In AFM analyses,surface profiles of negative resist ma-N 2403 and 495 K PMMA show cone peaks.Keywords: e-beam resist; spincoater; e-beam lithography

  3. Intense electron beams from GaAs photocathodes as a tool for molecular and atomic physics

    Energy Technology Data Exchange (ETDEWEB)

    Krantz, Claude

    2009-10-28

    We present cesium-coated GaAs photocathodes as reliable sources of intense, quasi-monoenergetic electron beams in atomic and molecular physics experiments. In long-time operation of the Electron Target of the ion storage ring TSR in Heidelberg, cold electron beams could be realised at steadily improving intensity and reliability. Minimisation of processes degrading the quantum efficiency allowed to increase the extractable current to more than 1mA at usable cathode lifetimes of 24 h or more. The benefits of the cold electron beam with respect to its application to electron cooling and electron-ion recombination experiments are discussed. Benchmark experiments demonstrate the superior cooling force and energy resolution of the photoelectron beam compared to its thermionic counterparts. The long period of operation allowed to study the long-time behaviour of the GaAs samples during multiple usage cycles at the Electron Target and repeated in-vacuum surface cleaning by atomic hydrogen exposure. An electron emission spectroscopy setup has been implemented at the photocathode preparation chamber of the Electron Target. Among others, this new facility opened the way to a novel application of GaAs (Cs) photocathodes as robust, ultraviolet-driven electron emitters. Based on this principle, a prototype of an electron gun, designed for implementation at the HITRAP setup at GSI, has been built and taken into operation successfully. (orig.)

  4. Laser beam diffraction at the edge of a film and application to thin film metrology.

    Science.gov (United States)

    Do, P A; Touaibia, M; Haché, A

    2013-08-20

    The thickness change of a film is measured optically using self-interference of a single laser beam incident at the edge of the film. Theory suggests that when a half-plane phase shift is applied to a Gaussian laser beam, interference fringes appear in the near and far field, in which position varies with the amount of phase shift. By measuring fringe pattern displacement, we demonstrate detection of thickness changes in chitosan films induced by temperature rises of a few degrees centigrade. With a laser at 543 nm, the minimum detectable thickness change is 0.8 nm in ideal conditions (quarter wave films), corresponding with a phase shift of 0.02 rad, and the minimum detectable film thickness is ∼30  nm. Potential use for surface temperature measurements is discussed.

  5. Uniform versus Gaussian Beams: A Comparison of the Effects of Diffraction, Obscuration, and Aberations.

    Science.gov (United States)

    1985-12-16

    beams D0 FOR 1473 UNCLASSIFIED SECURITY CLASSIFICATION OF THIS PAGE (Wen Dese Entered UNCLASSIFIED I[CUmI ’y CL A SSICATION 0 r T "IS P*GC/"h4. DA,. I...plotted on a logarithmic scale (Figs. 3c and 3d ). The positions of maxima and minima and the correspond- ing irradiance and encircled-power values are

  6. Test of Equivalence Principle at $10^{-8}$ Level by a Dual-species Double-diffraction Raman Atom Interferometer

    CERN Document Server

    Zhou, Lin; Tang, Biao; Chen, Xi; Gao, Fen; Peng, Wencui; Duan, Weitao; Zhong, Jiaqi; Xiong, Zongyuan; Wang, Jin; Zhang, Yuanzhong; Zhan, Mingsheng

    2015-01-01

    We report an improved test of the weak equivalence principle by using a simultaneous $^{85}$Rb-$^{87}$Rb dual-species atom interferometer. We propose and implement a four-wave double-diffraction Raman transition scheme for the interferometer, and demonstrate its ability in suppressing common-mode phase noise of Raman lasers after their frequencies and intensity ratios are optimized. The statistical uncertainty of the experimental data for E\\"{o}tv\\"{o}s parameter $\\eta$ is $0.8\\times10^{-8}$ at 3200 s. With various systematic errors corrected the final value is $\\eta=(2.8\\pm3.0)\\times10^{-8}$. The major uncertainty is attributed to the Coriolis effect.

  7. Atomic scattering in the diffraction limit: electron transfer in keV Li+-Na(3s, 3p) collisions

    DEFF Research Database (Denmark)

    Poel, Mike van der; Nielsen, C.V.; Rybaltover, M.;

    2002-01-01

    . This setup yields a momentum resolution of 0.12 an, an order of magnitude better angular resolution than previous measurements on this system. This enables us to clearly resolve Fraunhofer-type diffraction patterns in the angle DCS. In particular, the angular width of the ring structure is given by the ratio...... of the de Broglie wavelength lambda(dB) = 150 fm at a velocity v = 0.20 au and the effective atomic diameter for electron capture 2R = 20 au. Parallel AO and MO semiclassical coupled-channel calculations of the Na(3s, 3p) --> Li(2s, 2p) state-to-state collision amplitudes have been performed, and quantum...

  8. Test of Equivalence Principle at 10(-8) Level by a Dual-Species Double-Diffraction Raman Atom Interferometer.

    Science.gov (United States)

    Zhou, Lin; Long, Shitong; Tang, Biao; Chen, Xi; Gao, Fen; Peng, Wencui; Duan, Weitao; Zhong, Jiaqi; Xiong, Zongyuan; Wang, Jin; Zhang, Yuanzhong; Zhan, Mingsheng

    2015-07-01

    We report an improved test of the weak equivalence principle by using a simultaneous 85Rb-87Rb dual-species atom interferometer. We propose and implement a four-wave double-diffraction Raman transition scheme for the interferometer, and demonstrate its ability in suppressing common-mode phase noise of Raman lasers after their frequencies and intensity ratios are optimized. The statistical uncertainty of the experimental data for Eötvös parameter η is 0.8×10(-8) at 3200 s. With various systematic errors corrected, the final value is η=(2.8±3.0)×10(-8). The major uncertainty is attributed to the Coriolis effect.

  9. Self-referenced coherent diffraction x-ray movie of Angstrom- and femtosecond-scale atomic motion

    CERN Document Server

    Glownia, J M; Cryan, J P; Hartsock, R; Kozina, M; Minitti, M P; Nelson, S; Robinson, J; Sato, T; van Driel, T; Welch, G; Weninger, C; Zhi, D; Bucksbaum, P H

    2016-01-01

    Time-resolved femtosecond x-ray diffraction patterns from laser-excited molecular iodine are used to create a movie of intramolecular motion with time and space resolution of $30~$fs and $0.3$ \\AA . The high spatial fidelity is due to interference between the moving excitation and the static initial charge distribution. This x-ray interference has not been employed to image internal motion in molecules before. The initial state is used as the local oscillator for heterodyne amplification of the excited charge distribution to retrieve real-space movies of atomic motion on \\AA ngstrom and femtosecond scales. Coherent vibrational motion and dispersion, dissociation, and rotational dephasing are all clearly visible in the data, thereby demonstrating the stunning sensitivity of heterodyne methods.

  10. Structured mirror array for two-dimensional collimation of a chromium beam in atom lithography

    Institute of Scientific and Technical Information of China (English)

    Zhang Wan-Jing; Ma Yan; Li Tong-Bao; Zhang Ping-Ping; Deng Xiao; Chen Sheng; Xiao Sheng-Wei

    2013-01-01

    Direct-write atom lithography,one of the potential nanofabrication techniques,is restricted by some difficulties in producing optical masks for the deposition of complex structures.In order to make further progress,a structured mirror array is developed to transversely collimate the chromium atomic beam in two dimensions.The best collimation is obtained when the laser red detunes by natural line-width of transition 7S3 → 7P40 of the chromium atom.The collimation ratio is 0.45 vertically (in x axis),and it is 0.55 horizontally (in y axis).The theoretical model is also simulated,and success of our structured mirror array is achieved.

  11. Reducing aberration effect of Fourier transform lens by modifying Fourier spectrum of diffractive optical element in beam shaping optical system.

    Science.gov (United States)

    Zhang, Fang; Zhu, Jing; Song, Qiang; Yue, Weirui; Liu, Jingdan; Wang, Jian; Situ, Guohai; Huang, Huijie

    2015-10-20

    In general, Fourier transform lenses are considered as ideal in the design algorithms of diffractive optical elements (DOEs). However, the inherent aberrations of a real Fourier transform lens disturb the far field pattern. The difference between the generated pattern and the expected design will impact the system performance. Therefore, a method for modifying the Fourier spectrum of DOEs without introducing other optical elements to reduce the aberration effect of the Fourier transform lens is proposed. By applying this method, beam shaping performance is improved markedly for the optical system with a real Fourier transform lens. The experiments carried out with a commercial Fourier transform lens give evidence for this method. The method is capable of reducing the system complexity as well as improving its performance.

  12. X-ray absorption microtomography (microCT) and small beam diffraction mapping of sea urchin teeth.

    Science.gov (United States)

    Stock, S R; Barss, J; Dahl, T; Veis, A; Almer, J D

    2002-07-01

    Two noninvasive X-ray techniques, laboratory X-ray absorption microtomography (microCT) and X-ray diffraction mapping, were used to study teeth of the sea urchin Lytechinus variegatus. MicroCT revealed low attenuation regions at near the tooth's stone part and along the carinar process-central prism boundary; this latter observation appears to be novel. The expected variation of Mg fraction x in the mineral phase (calcite, Ca(1-x)Mg(x)CO(3)) cannot account for all of the linear attenuation coefficient decrease in the two zones: this suggested that soft tissue is localized there. Transmission diffraction mapping (synchrotron X-radiation, 80.8 keV, 0.1 x 0.1mm(2) beam area, 0.1mm translation grid, image plate area detector) simultaneously probed variations in 3-D and showed that the crystal elements of the "T"-shaped tooth were very highly aligned. Diffraction patterns from the keel (adaxial web) and from the abaxial flange (containing primary plates and the stone part) differed markedly. The flange contained two populations of identically oriented crystal elements with lattice parameters corresponding to x=0.13 and x=0.32. The keel produced one set of diffraction spots corresponding to the lower x. The compositions were more or less equivalent to those determined by others for camarodont teeth, and the high Mg phase is expected to be disks of secondary mineral epitaxially related to the underlying primary mineral element. Lattice parameter gradients were not noted in the keel or flange. Taken together, the microCT and diffraction results indicated that there was a band of relatively high protein content, of up to approximately 0.25 volume fraction, in the central part of the flange and paralleling its adaxial and abaxial faces. X-ray microCT and microdiffraction data used in conjunction with protein distribution data will be crucial for understanding the properties of various biocomposites and their mechanical functions.

  13. Molecular-beam epitaxy growth and structural characterization of semiconductor-ferromagnet heterostructures by grazing incidence X-ray diffraction

    Energy Technology Data Exchange (ETDEWEB)

    Satapathy, D.K.

    2005-12-19

    The present work is devoted to the growth of the ferromagnetic metal MnAs on the semiconductor GaAs by molecular-beam epitaxy (MBE). The MnAs thin films are deposited on GaAs by molecular-beam epitaxy (MBE). Grazing incidence diffraction (GID) and reflection high-energy electron diffraction (RHEED) are used in situ to investigate the nucleation, evolution of strain, morphology and interfacial structure during the MBE growth. Four stages of the nucleation process during growth of MnAs on GaAs(001) are revealed by RHEED azimuthal scans. GID shows that further growth of MnAs films proceed via the formation of relaxed islands at a nominal thickness of 2.5 ML which increase in size and finally coalesce to form a continuous film. Early on, an ordered array of misfit dislocations forms at the interface releasing the misfit strain even before complete coalescence occurs. The fascinating complex nucleation process of MnAs on GaAs(0 0 1) contains elements of both Volmer-Weber and Stranski-Krastanov growth. A nonuniform strain amounting to 0.66%, along the [1 -1 0] direction and 0.54%, along the [1 1 0] direction is demonstrated from x-ray line profile analysis. A high correlation between the defects is found along the GaAs[1 1 0] direction. An extremely periodic array of misfit dislocations with a period of 4.95{+-}0.05 nm is formed at the interface along the [1 1 0] direction which releases the 7.5% of misfit. The inhomogeneous strain due to the periodic dislocations is confined at the interface within a layer of 1.6 nm thickness. The misfit along the [1 -1 0] direction is released by the formation of a coincidence site lattice. (orig.)

  14. Impact of Electron Collision Mixing on the delay times of an electron beam excited Atomic Xenon laser

    NARCIS (Netherlands)

    Peters, Peter J.; Lan, Yun Fu; Ohwa, Mieko; Kushner, Mark J.

    1990-01-01

    The atomic xenon (5d¿6p) infrared laser has been experimentally and theoretically investigated using a short-pulse (30-ns), high-power (1-10-MW/cm3) coaxial electron beam excitation source. In most cases, laser oscillation is not observed during the e-beam current pulse. Laser pulses of hundreds of

  15. High-resolution computational ghost imaging and ghost diffraction through turbulence via a beam-shaping method

    Science.gov (United States)

    Luo, Chun-Ling; Zhuo, Ling-Qing

    2017-01-01

    Imaging through atmospheric turbulence is a topic with a long history and grand challenges still exist in the remote sensing and astro observation fields. In this letter, we try to propose a simple scheme to improve the resolution of imaging through turbulence based on the computational ghost imaging (CGI) and computational ghost diffraction (CGD) setup via the laser beam shaping techniques. A unified theory of CGI and CGD through turbulence with the multi-Gaussian shaped incoherent source is developed, and numerical examples are given to see clearly the effects of the system parameters to CGI and CGD. Our results show that the atmospheric effect to the CGI and CGD system is closely related to the propagation distance between the source and the object. In addition, by properly increasing the beam order of the multi-Gaussian source, we can improve the resolution of CGI and CGD through turbulence relative to the commonly used Gaussian source. Therefore our results may find applications in remote sensing and astro observation.

  16. Ray-tracing simulations of spherical Johann diffraction spectrometer for in-beam X-ray experiments

    Energy Technology Data Exchange (ETDEWEB)

    Jagodziński, P., E-mail: jagodzin@tu.kielce.pl [Department of Physics, Kielce University of Technology, Tysiaclecia PP 7, 25-314 Kielce (Poland); Pajek, M.; Banaś, D. [Institute of Physics, Jan Kochanowski University, Świȩtokrzyska 15, 25-406 Kielce (Poland); Beyer, H.F. [GSI Helmholtzzentrum für Schwerionenforschung, D-64291 Darmstadt (Germany); Trassinelli, M. [Institut des NanoSciences de Paris, Université Pierre et Marie Curie, 4 Place Jussieu, 75015 Paris (France); Stoehlker, Th. [GSI Helmholtzzentrum für Schwerionenforschung, D-64291 Darmstadt (Germany); Helmholtz-Insitut Jena, D-07743 Jena (Germany); Institut für Optic und Quantenelektronik, Friedrich-Schiller-Universität Jena, D-07743 Jena (Germany)

    2014-07-01

    The results of the Monte-Carlo ray-tracing simulations for a Johann-type Bragg spectrometer with spherically curved-crystal designed to detect the X-rays from a fast-moving source are reported. These calculations were performed to optimize the X-ray spectrometer to be used at the gas-target installed at ion storage ring for high-resolution X-ray experiments. In particular, the two-dimensional distributions of detected photons were studied using the Monte-Carlo method both for the stationary and moving X-ray sources, taking into account a detailed description of X-ray source and X-ray diffraction on the crystal as well as a role of the Doppler effect for in-beam experiments. The origin of the asymmetry of observed X-ray profiles was discussed in detail and the procedure to derive a precise (sub-eV) X-ray transition energy for such asymmetric profiles was proposed. The results are important for the investigations of 1s2p{sup 3}P{sub 2}→1s2s{sup 3}S{sub 1} intrashell transition in excited He-like uranium ions in in-beam X-ray experiments.

  17. Theory of longitudinal atomic beam spin echo and parity violating Berry-phases in atoms; Theorie des longitudinalen Atomstrahl-Spinechos und paritaetsverletzende Berry-Phasen in Atomen

    Energy Technology Data Exchange (ETDEWEB)

    Bergmann, T.F.

    2006-07-19

    We present a nonrelativistic theory for the quantum mechanical description of longitudinal atomic beam spin echo experiments, where a beam of neutral atoms is subjected to static electric and magnetic fields. The atomic wave function is the solution of a matrix-valued Schroedinger equation and can be written as superposition of local (atomic) eigenstates of the potential matrix. The position- and time-dependent amplitude function of each eigenstate represents an atomic wave packet and can be calculated in a series expansion with a master formula that we derive. The zeroth order of this series expansion describes the adiabatic limit, whereas the higher order contributions contain the mixing of the eigenstates and the corresponding amplitude functions. We give a tutorial for the theoretical description of longitudinal atomic beam spin echo experiments and for the so-called Fahrplan model, which is a visualisation tool for the propagation of wave packets of different atomic eigenstates. As an example for the application of our theory, we study parity violating geometric (Berry-)phases. In this context, we define geometric flux densities, which for certain field configurations can be used to illustrate geometric phases in a vector diagram. Considering an example with a specific field configuration, we prove the existence of a parity violating geometric phase. (orig.)

  18. Producing acoustic 'Frozen Waves': Simulated experiments with diffraction/attenuation resistant beams, in lossy media

    CERN Document Server

    Prego-Borges, Jose' L; Recami, Erasmo; Tavares-Costa, Eduardo

    2013-01-01

    The so-called Localized Waves (LW), and the "Frozen Waves" (FW), have arisen significant attention in the areas of Optics and Ultrasound, because of their surprising energy localization properties. The LWs resist the effects of diffraction for large distances, and possess an interesting self-reconstruction (self-healing) property, after obstacles with size smaller than the antenna's; while the FWs, a sub-class of theirs, offer the possibility of arbitrarily modeling the field longitudinal intensity pattern inside a prefixed interval, for instance 0 < z < L, of the wave propagation axis. More specifically, the FWs are localized fields "at rest", that is, with a static envelope (within which only the carrier wave propagates), and can be endowed moreover with a high transverse localization. In this paper we investigate by simulated experiments, various cases of generation of ultrasonic FW fields, with frequency f_o = 1 MHz in a water-like medium, taking account of the effects of attenuation. We present res...

  19. ARTICLE Crossed Beams Study on the Dynamics of F Atom Reaction with 1,2-Butadiene

    Science.gov (United States)

    Xiao, Chong-fa; Shen, Guan-lin; Wang, Xiu-yan; Yang, Xue-ming

    2010-12-01

    We have investigated the dynamics of the F+C4H6 reaction using the universal crossed molecular beam method. The C4H5F+H reaction channel was observed in this experiment. Angular resolved time-of-flight spectra have been measured for the C4H5F product. Product angular distributions as well as kinetic energy distributions were determined for this product channel. Experimental results show that the C4H5F product is largely backward scattered with considerable forward scattering signal, relative to the F atom beam direction. This suggests that the reaction channel mainly proceeds via a long-lived complex formation mechanism, with possible contribution from a direct SN2 type mechanism.

  20. Bright focused ion beam sources based on laser-cooled atoms

    CERN Document Server

    McClelland, J J; Knuffman, B; Twedt, K A; Schwarzkopf, A; Wilson, T M

    2015-01-01

    Nanoscale focused ion beams (FIBs) represent one of the most useful tools in nanotechnology, enabling nanofabrication via milling and gas-assisted deposition, microscopy and microanalysis, and selective, spatially resolved doping of materials. Recently, a new type of FIB source has emerged, which uses ionization of laser cooled neutral atoms to produce the ion beam. The extremely cold temperatures attainable with laser cooling (in the range of 100 uK or below) result in a beam of ions with a very small transverse velocity distribution. This corresponds to a source with extremely high brightness that rivals or may even exceed the brightness of the industry standard Ga+ liquid metal ion source. In this review we discuss the context of ion beam technology in which these new ion sources can play a role, their principles of operation, and some examples of recent demonstrations. The field is relatively new, so only a few applications have been demonstrated, most notably low energy ion microscopy with Li ions. Never...

  1. Absorption spectroscopy characterization measurements of a laser-produced Na atomic beam

    Energy Technology Data Exchange (ETDEWEB)

    Ching, C.H.; Bailey, J.E.; Lake, P.W.; Filuk, A.B.; Adams, R.G.; McKenney, J.

    1996-06-01

    This work describes a pulsed Na atomic beam source developed for spectroscopic diagnosis of a high-power ion diode on the Particle Beam Fusion Accelerator II. The goal is to produce a {approximately} 10{sup 12}-cm{sup {minus}3}-density Na atomic beam that can be injected into the diode acceleration gap to measure electric and magnetic fields from the Stark and Zeeman effects through laser-induced-fluorescence or absorption spectroscopy. A {approximately} 10 ns fwhm, 1.06 {micro}m, 0.6 J/cm{sup 2} laser incident through a glass slide heats a Na-bearing thin film, creating a plasma that generates a sodium vapor plume. A {approximately} 1 {micro}sec fwhm dye laser beam tuned to 5,890 {angstrom} is used for absorption measurement of the Na I resonant doublet by viewing parallel to the film surface. The dye laser light is coupled through a fiber to a spectrograph with a time-integrated CCD camera. A two-dimensional mapping of the Na vapor density is obtained through absorption measurements at different spatial locations. Time-of-flight and Doppler broadening of the absorption with {approximately} 0.1 {angstrom} spectral resolution indicate that the Na neutral vapor temperature is about 0.5 to 2 eV. Laser-induced-fluorescence from {approximately} 1 {times} 10{sup 12}-cm{sup {minus}3} Na I 3s-3p lines observed with a streaked spectrograph provides a signal level sufficient for {approximately} 0.06 {angstrom} wavelength shift measurements in a mock-up of an ion diode experiment.

  2. Influence of laser power on deposition of the chromium atomic beam in laser standing wave

    Institute of Scientific and Technical Information of China (English)

    2009-01-01

    One-dimensional deposition of collimated Cr atomic beam focused by a near-resonant Gaussian standing-laser field with wavelength of 425.55 nm is examined from particle-optics approach by using an adaptive step size,fourth-order Runge-Kutta type algorithm.The influence of laser power on deposition of atoms in laser standing wave is discussed and the simulative result shows that the FWHM of nanometer stripe is 102 nm and contrast is 2:1 with laser power equal to 3 mW,the FWHM is 1.2 nm and contrast is 32:1 with laser power equal to 16 mW,but with laser power increase,equal to 50 mW,the nonmeter structure forms the multi-crests and exacerbates.

  3. Coherent reflection of He atom beams from rough surfaces at near-grazing incidence

    CERN Document Server

    Zhao, Bum Suk; Meijer, Gerard; Schöllkopf, Wieland

    2010-01-01

    We here report coherent reflection of thermal He atom beams from various microscopically rough surfaces at grazing incidence. For a sufficiently small normal component $k_z$ of the incident wave-vector of the atom the reflection probability is found to be a function of $k_z$ only. This behavior is explained by quantum-reflection at the attractive branch of the Casimir-van der Waals interaction potential. For larger values of $k_z$ the overall reflection probability decreases rapidly and is found to also depend on the parallel component $k_x$ of the wave-vector. The material specific $k_x$ dependence for this classical reflection at the repulsive branch of the potential is explained qualitatively in terms of the averaging-out of the surface roughness under grazing incidence conditions.

  4. Coherent Reflection of He Atom Beams from Rough Surfaces at Grazing Incidence

    Science.gov (United States)

    Zhao, Bum Suk; Schewe, H. Christian; Meijer, Gerard; Schöllkopf, Wieland

    2010-09-01

    We report coherent reflection of thermal He atom beams from various microscopically rough surfaces at grazing incidence. For a sufficiently small normal component kz of the incident wave vector of the atom the reflection probability is found to be a function of kz only. This behavior is explained by quantum reflection at the attractive branch of the Casimir-van der Waals interaction potential. For larger values of kz the overall reflection probability decreases rapidly and is found to also depend on the parallel component kx of the wave vector. The material specific kx dependence for this classic reflection at the repulsive branch of the potential is discussed in terms of an averaging out of the surface roughness under grazing incidence conditions.

  5. Precision measurement of transverse velocity distribution of a strontium atomic beam

    Science.gov (United States)

    Gao, F.; Liu, H.; Xu, P.; Tian, X.; Wang, Y.; Ren, J.; Wu, Haibin; Chang, Hong

    2014-02-01

    We measure the transverse velocity distribution in a thermal Sr atomic beam precisely by velocity-selective saturated fluorescence spectroscopy. The use of an ultrastable laser system and the narrow intercombination transition line of Sr atoms mean that the resolution of the measured velocity can reach 0.13 m/s, corresponding to 90 μK in energy units. The experimental results are in very good agreement with the results of theoretical calculations. Based on the spectroscopic techniques used here, the absolute frequency of the intercombination transition of 88Sr is measured using an optical-frequency comb generator referenced to the SI second through an H maser, and is given as 434 829 121 318(10) kHz.

  6. Precision measurement of transverse velocity distribution of a strontium atomic beam

    Directory of Open Access Journals (Sweden)

    F. Gao

    2014-02-01

    Full Text Available We measure the transverse velocity distribution in a thermal Sr atomic beam precisely by velocity-selective saturated fluorescence spectroscopy. The use of an ultrastable laser system and the narrow intercombination transition line of Sr atoms mean that the resolution of the measured velocity can reach 0.13 m/s, corresponding to 90 μK in energy units. The experimental results are in very good agreement with the results of theoretical calculations. Based on the spectroscopic techniques used here, the absolute frequency of the intercombination transition of 88Sr is measured using an optical-frequency comb generator referenced to the SI second through an H maser, and is given as 434 829 121 318(10 kHz.

  7. Influence of laser power on deposition of the chromium atomic beam in laser standing wave

    Institute of Scientific and Technical Information of China (English)

    ZHANG WenTao; ZHU BaoHua; ZHANG BaoWu; LI TongBao

    2009-01-01

    One-dimensional deposition of collimated Cr atomic beam focused by a near-resonant Gaussian standing-laser field with wavelength of 425.55 nm is examined from particle-optics approach by using an adaptive step size, fourth-order Runge-Kutta type algorithm. The influence of laser power on depo-sition of atoms in laser standing wave is discussed and the simulative result shows that the FWHM of nanometer stripe is 102 nm and contrast is 2:1 with laser power equal to 3 mW, the FWHM is 1.2 nm and contrast is 32:1 with laser power equal to 16 mW, but with laser power increase, equal to 50 mW, the nonmeter structure forms the multi-crests and exacerbates.

  8. Use of an Atmospheric Atomic Oxygen Beam for Restoration of Defaced Paintings

    Science.gov (United States)

    Banks, Bruce A.; Rutledge, Sharon K.; Karla, Margaret; Norris, Mary Jo; Real, William A.; Haytas, Christy A.

    1999-01-01

    An atmospheric atomic oxygen beam has been found to be effective in removing organic materials through oxidation that are typical of graffiti or other contaminant defacements which may occur to the surfaces of paintings. The technique, developed by the National Aeronautics and Space Administration, is portable and was successfully used at the Carnegie Museum of Art to remove a lipstick smudge from the surface of porous paint on the Andy Warhol painting "Bathtub." This process was also evaluated for suitability to remove felt tip and ball point ink graffiti from paper, gesso on canvas and cotton canvas.

  9. Determination of the Projected Atomic Potential by Deconvolution of the Auto-Correlation Function of TEM Electron Nano-Diffraction Patterns

    Directory of Open Access Journals (Sweden)

    Liberato De Caro

    2016-11-01

    Full Text Available We present a novel method to determine the projected atomic potential of a specimen directly from transmission electron microscopy coherent electron nano-diffraction patterns, overcoming common limitations encountered so far due to the dynamical nature of electron-matter interaction. The projected potential is obtained by deconvolution of the inverse Fourier transform of experimental diffraction patterns rescaled in intensity by using theoretical values of the kinematical atomic scattering factors. This novelty enables the compensation of dynamical effects typical of transmission electron microscopy (TEM experiments on standard specimens with thicknesses up to a few tens of nm. The projected atomic potentials so obtained are averaged on sample regions illuminated by nano-sized electron probes and are in good quantitative agreement with theoretical expectations. Contrary to lens-based microscopy, here the spatial resolution in the retrieved projected atomic potential profiles is related to the finer lattice spacing measured in the electron diffraction pattern. The method has been successfully applied to experimental nano-diffraction data of crystalline centrosymmetric and non-centrosymmetric specimens achieving a resolution of 65 pm.

  10. X-ray diffraction using synchrotron radiation on the G.I.L.D.A. beam line at the E.S.R.F

    Energy Technology Data Exchange (ETDEWEB)

    Balerna, A. [INFN, Laboratori Nazionali di Frascati, Rome (Italy); Meneghini, C. [INFN, Laboratori Nazionali di Frascati, Rome (Italy)]|[INFM, Genoa (Italy); Bordoni, S. [Rome Univ. `Tor Vergata` (Italy). Dip. di Fisica; Mobilio, S. [Rome Univ. III (Italy). Dip. di Fisica `E. Amaldi`

    1996-09-01

    The aim of this lecture is to make a short introduction on Synchrotron radiation, its history and main properties. The main components of a synchrotron radiation beam line will be described. The Italian beam line, General purpose Italian beam line Line for Diffraction and Absorption (G.I.L.D.A.) at the European Synchrotron Radiation Facility (E.S.R.F.) in Grenoble will be used as an example. The G.I.L.D.A. diffractometer will be described in detail reporting also some experimental results.

  11. Adsorption, X-ray Diffraction, Photoelectron, and Atomic Emission Spectroscopy Benchmark Studies for the Eighth Industrial Fluid Properties Simulation Challenge*+

    Science.gov (United States)

    Ross, Richard B.; Aeschliman, David B.; Ahmad, Riaz; Brennan, John K.; Brostrom, Myles L.; Frankel, Kevin A.; Moore, Jonathan D.; Moore, Joshua D.; Mountain, Raymond D.; Poirier, Derrick M.; Thommes, Matthias; Shen, Vincent K.; Schultz, Nathan E.; Siderius, Daniel W.; Smith, Kenneth D.

    2016-01-01

    The primary goal of the eighth industrial fluid properties simulation challenge was to test the ability of molecular simulation methods to predict the adsorption of organic adsorbates in activated carbon materials. The challenge focused on the adsorption of perfluorohexane in the activated carbon standard BAM-P109 (Panne and Thünemann 2010). Entrants were challenged to predict the adsorption of perfluorohexane in the activated carbon at a temperature of 273 K and at relative pressures of 0.1, 0.3, and 0.6. The relative pressure (P/Po) is defined as that relative to the bulk saturation pressure predicted by the fluid model at a given temperature (273 K in this case). The predictions were judged by comparison to a set of experimentally determined values, which are published here for the first time and were not disclosed to the entrants prior to the challenge. Benchmark experimental studies, described herein, were also carried out and provided to entrants in order to aid in the development of new force fields and simulation methods to be employed in the challenge. These studies included argon, carbon dioxide, and water adsorption in the BAM-P109 activated carbon as well as X-ray diffraction, X-ray microtomography, photoelectron spectroscopy, and atomic emission spectroscopy studies of BAM-P109. Several concurrent studies were carried out for the BAM-P108 activated carbon (Panne and Thünemann 2010). These are included in the current manuscript for comparison. PMID:27840543

  12. In situ surface X-ray diffraction studies of the copper-electrolyte interface. Atomic structure and homoepitaxial grwoth

    Energy Technology Data Exchange (ETDEWEB)

    Golks, Frederik

    2011-05-19

    Copper electrodeposition is the predominantly used technique for on-chip wiring in the fabrication of ultra-large scale integrated (ULSI) microchips. In this 'damascene copper electroplating' process, multicomponent electrolytes containing organic additives realize void-free filling of trenches with high aspect ratio ('superconformal deposition'). Despite manifold studies, motivated by the continuous trend to shrink wiring dimensions and thus the demand of optimized plating baths, detailed knowledge on the growth mechanism - in presence and absence of additives - is still lacking. Using a recently developed hanging meniscus X-ray transmission cell, brilliant synchrotron x-rays and a fast, one-dimensional detector system, unique real-time in situ surface X-ray diffraction studies of copper electrodeposition were performed under realistic reaction conditions, approaching rates of technological relevance. Preparatory measurements of the electrochemical dissolution of Au(001) in chloride-containing electrolyte demonstrated the capability of this powerful technique, specifically the possibility to follow atomic-scale deposition or dissolution processes with a time resolution down to five milliseconds. The electrochemical as well as structural characterization of the Cu(001)- and Cu(111)-electrolyte interfaces provided detailed insight into the complex atomic-scale structures in presence of specifically adsorbed chloride on these surfaces. The interface of Cu(001) in chloride-containing electrolyte exhibits a continuous surface phase transition of a disordered Cl adlayer to a c(2 x 2) Cl adlayer with increasing potential. The latter was found to induce a small vertical corrugation of substrate atoms, which can be ascribed to lattice relaxations induced by the presence of coadsorbed water molecules and cations in the outer part of the electrochemical double layer. The study of the specific adsorption of chloride on Cu(111) from acidic aqueous

  13. Optical diffraction into thick slab waveguides: a finite-beam RCWA approach to solve extremely asymmetrical scattering-EAS in slanted holographic gratings

    Science.gov (United States)

    Pietralunga, Silvia M.; Geroldi, Alessandro; Serafini, Mirko

    2012-06-01

    We have implemented a Finite-Beam Rigorous Coupled-Wave Approach (FB-RCWA) to solve for guided-optics propagation in the presence of holographic slanted Bragg gratings, embedded in the core of slab waveguides and operated in Extreme Asymmetrical Scattering (EAS) configuration. In EAS a resonance condition can be established, as proceeding from the design parameters. Diffraction efficiency can be evaluated as the ratio of the flux of diffracted power P1, on a suitably defined cross-section along the propagation of diffracted beam, and input power P0. By FBRCWA, no limitation in the depth of grating modulation is assumed. The first-order diffracted field in resonant Bragg condition propagates along the waveguide. EAS in thick waveguides operating in highly multimodal regime can be investigated, as well as macroscopic volumes and widely extended illuminated regions up to a few millimeters. In thick slabs, η > 90% is demonstrated, for input illuminated apertures of length L >= Lc, where Lc is the optimum coupling length. The effects of detuning from Bragg condition, both in distribution and amplitude of the diffracted field, are quantified. Diffraction efficiency, i.e. optical coupling, bandwidth is evaluated.

  14. On the combination of a low energy hydrogen atom beam with a cold multipole ion trap

    Energy Technology Data Exchange (ETDEWEB)

    Borodi, Gheorghe

    2008-12-09

    The first part of the activities of this thesis was to develop a sophisticated ion storage apparatus dedicated to study chemical processes with atomic hydrogen. The integration of a differentially pumped radical beam source into an existing temperature variable 22- pole trapping machine has required major modifications. Since astrophysical questions have been in the center of our interest, the introduction first gives a short overview of astrophysics and -chemistry. The basics of ion trapping in temperature variable rf traps is well-documented in the literature; therefore, the description of the basic instrument (Chapter 2) is kept rather short. Much effort has been put into the development of an intense and stable source for hydrogen atoms the kinetic energy of which can be changed. Chapter 3 describes this module in detail with emphasis on the integration of magnetic hexapoles for guiding the atoms and special treatments of the surfaces for reducing H-H recombination. Due to the unique sensitivity of the rf ion trapping technique, this instrument allows one to study a variety of reactions of astrochemical and fundamental interest. The results of this work are summarized in Chapter 4. Reactions of CO{sub 2}{sup +} with hydrogen atoms and molecules have been established as calibration standard for in situ determination of H and H{sub 2} densities over the full temperature range of the apparatus (10 K-300 K). For the first time, reactions of H- and D-atoms with the ionic hydrocarbons CH{sup +}, CH{sub 2}{sup +}, and CH{sub 4}{sup +} have been studied at temperatures of interstellar space. A very interesting, not yet fully understood collision system is the interaction of protonated methane with H. The outlook presents some ideas, how to improve the new instrument and a few reaction systems are mentioned which may be studied next. (orig.)

  15. Average Dissipative and Dipole Forces on a Three-Level Atom in a Laguerre-Gaussian Beam

    Institute of Scientific and Technical Information of China (English)

    WANG Zheng-Ling; YIN Jian-Ping

    2005-01-01

    @@ By means of the optical Bloch equations based on the atomic density matrix elements, the general expressions of the average dissipative force, dipole force and the mechanical torque acting on a A-configuration three-level atom in a linearly-polarized Laguerre-Gaussian beam (LGB) with an angular momentum of lh are derived, and the general properties of the average dissipative and dipole force on the three-level atom in the linearly-polarized LGB are analysed. We find a resonant property (with two resonant peaks) of the dissipative force and a non-resonant property (with two pairs of non-resonant peaks) of the dipole force on the three-level atom, which are completely different from those on the two-level atom. Our study also shows that all of general expressions on the three-level atom will be simplified to those on the two-level atom in the approximation of large detuning.

  16. Diffraction to De-Diffraction

    CERN Document Server

    Tamari, V F

    2003-01-01

    De-diffraction (DD), a new procedure to totally cancel diffraction effects from wave-fields is presented, whereby the full field from an aperture is utilized and a truncated geometrical field is obtained, allowing infinitely sharp focusing and non-diverging beams. This is done by reversing a diffracted wave-fields' direction. The method is derived from the wave equation and demonstrated in the case of Kirchhoff's integral. An elementary bow-wavelet is described and the DD process is related to quantum and relativity theories.

  17. Application of Powder Diffraction Methods to the Analysis of the Atomic Structure of Nanocrystals: The Concept of the Apparent Lattice Parameter (ALP)

    Science.gov (United States)

    Palosz, B.; Grzanka, E.; Gierlotka, S.; Stelmakh, S.; Pielaszek, R.; Bismayer, U.; Weber, H.-P.; Palosz, W.; Curreri, Peter A. (Technical Monitor)

    2002-01-01

    The applicability of standard methods of elaboration of powder diffraction data for determination of the structure of nano-size crystallites is analysed. Based on our theoretical calculations of powder diffraction data we show, that the assumption of the infinite crystal lattice for nanocrystals smaller than 20 nm in size is not justified. Application of conventional tools developed for elaboration of powder diffraction data, like the Rietveld method, may lead to erroneous interpretation of the experimental results. An alternate evaluation of diffraction data of nanoparticles, based on the so-called 'apparent lattice parameter' (alp) is introduced. We assume a model of nanocrystal having a grain core with well-defined crystal structure, surrounded by a surface shell with the atomic structure similar to that of the core but being under a strain (compressive or tensile). The two structural components, the core and the shell, form essentially a composite crystal with interfering, inseparable diffraction properties. Because the structure of such a nanocrystal is not uniform, it defies the basic definitions of an unambiguous crystallographic phase. Consequently, a set of lattice parameters used for characterization of simple crystal phases is insufficient for a proper description of the complex structure of nanocrystals. We developed a method of evaluation of powder diffraction data of nanocrystals, which refers to a core-shell model and is based on the 'apparent lattice parameter' methodology. For a given diffraction pattem, the alp values are calculated for every individual Bragg reflection. For nanocrystals the alp values depend on the diffraction vector Q. By modeling different a0tomic structures of nanocrystals and calculating theoretically corresponding diffraction patterns using the Debye functions we showed, that alp-Q plots show characteristic shapes which can be used for evaluation of the atomic structure of the core-shell system. We show, that using a simple

  18. Molecular beam epitaxy of GeTe-Sb{sub 2}Te{sub 3} phase change materials studied by X-ray diffraction

    Energy Technology Data Exchange (ETDEWEB)

    Shayduk, Roman

    2010-05-20

    The integration of phase change materials into semiconductor heterostructures may lead to the development of a new generation of high density non-volatile phase change memories. Epitaxial phase change materials allow to study the detailed structural changes during the phase transition and to determine the scaling limits of the memory. This work is dedicated to the epitaxial growth of Ge-Sb-Te phase change alloys on GaSb(001). We deposit Ge-Sb-Te (GST) films on GaSb(001) substrates by means of molecular beam epitaxy (MBE). The film orientation and lattice constant evolution is determined in real time during growth using grazing incidence X-ray diffraction (GID). The nucleation stage of the growth is studied in situ using reflection high energy electron diffraction (RHEED). Four growth regimes of GST on GaSb(001) were observed: amorphous, polycrystalline, incubated epitaxial and direct epitaxial. Amorphous film grows for substrate temperatures below 100 C. For substrate temperatures in the range 100-160 C, the film grows in polycrystalline form. Incubated epitaxial growth is observed at temperatures from 180 to 210 C. This growth regime is characterized by an initial 0.6nm thick amorphous layer formation, which crystallizes epitaxially as the film thickness increases. The determined lattice constant of the films is 6.01 A, very close to that of the metastable GST phase. The films predominantly possess an epitaxial cube-on-cube relationship. At higher temperatures the films grow epitaxially, however the growth rate is rapidly decreasing with temperature. At temperatures above 270 C the growth rate is zero. The composition of the grown films is close to 2:2:5 for Ge, Sb and Te, respectively. The determined crystal structure of the films is face centered cubic (FCC) with a rhombohedral distortion. The analysis of X-ray peak widths gives a value for the rhombohedral angle of 89.56 . We observe two types of reflections in reciprocal space indicating two FCC sublattices in

  19. Optical Guiding of Trapped Atoms by a Blue-Detuned Hollow Laser Beam in the Horizontal Direction

    Institute of Scientific and Technical Information of China (English)

    JIANG Kai-Jun; LI Ke; WANG Jin; ZHAN Ming-Sheng

    2005-01-01

    @@ Optical guiding of 85 Rb atoms in a magneto-optical trap (MOT) by a blue-detuned horizontal hollow laser beam is demonstrated experimentally. The guiding efficiency and the velocity distribution of the guided atoms are found to have strong dependence on the detuning of the guiding laser. In particular, the optimum guiding occurs when the blue detuning of the hollow laser beam is approximately equal to the hyperfine structure splitting of the 85Rb ground states, in good agreement with the theoretical analysis based on a three-level model.

  20. Atomic layer deposition of an Al2O3 dielectric on ultrathin graphite by using electron beam irradiation

    Institute of Scientific and Technical Information of China (English)

    Jiang Ran; Meng Lingguo; Zhang Xijian; Hyung-Suk Jung; Cheol Seong Hwang

    2012-01-01

    Atomic layer deposition ofan Al2O3 dielectric on ultrathin graphite is studied in order to investigate the integration of a high k dielectric with graphite-based substrates.Electron beam irradiation on the graphite surface is followed by a standard atomic layer deposition of Al2O3.Improvement of the Al2O3 layer deposition morphology was observed when using this radiation exposure on graphite.This result may be attributed to the amorphous change of the graphite layers during electron beam irradiation.

  1. SINGLE CRYSTAL NEUTRON DIFFRACTION.

    Energy Technology Data Exchange (ETDEWEB)

    KOETZLE,T.F.

    2001-03-13

    Single-crystal neutron diffraction measures the elastic Bragg reflection intensities from crystals of a material, the structure of which is the subject of investigation. A single crystal is placed in a beam of neutrons produced at a nuclear reactor or at a proton accelerator-based spallation source. Single-crystal diffraction measurements are commonly made at thermal neutron beam energies, which correspond to neutron wavelengths in the neighborhood of 1 Angstrom. For high-resolution studies requiring shorter wavelengths (ca. 0.3-0.8 Angstroms), a pulsed spallation source or a high-temperature moderator (a ''hot source'') at a reactor may be used. When complex structures with large unit-cell repeats are under investigation, as is the case in structural biology, a cryogenic-temperature moderator (a ''cold source'') may be employed to obtain longer neutron wavelengths (ca. 4-10 Angstroms). A single-crystal neutron diffraction analysis will determine the crystal structure of the material, typically including its unit cell and space group, the positions of the atomic nuclei and their mean-square displacements, and relevant site occupancies. Because the neutron possesses a magnetic moment, the magnetic structure of the material can be determined as well, from the magnetic contribution to the Bragg intensities. This latter aspect falls beyond the scope of the present unit; for information on magnetic scattering of neutrons see Unit 14.3. Instruments for single-crystal diffraction (single-crystal diffractometers or SCDs) are generally available at the major neutron scattering center facilities. Beam time on many of these instruments is available through a proposal mechanism. A listing of neutron SCD instruments and their corresponding facility contacts is included in an appendix accompanying this unit.

  2. Synthesis of atomically thin hexagonal boron nitride films on nickel foils by molecular beam epitaxy

    Energy Technology Data Exchange (ETDEWEB)

    Nakhaie, S.; Wofford, J. M.; Schumann, T.; Jahn, U.; Ramsteiner, M.; Hanke, M.; Lopes, J. M. J., E-mail: lopes@pdi-berlin.de; Riechert, H. [Paul-Drude-Institut für Festkörperelektronik, Hausvogteiplatz 5-7, 10117 Berlin (Germany)

    2015-05-25

    Hexagonal boron nitride (h-BN) is a layered two-dimensional material with properties that make it promising as a dielectric in various applications. We report the growth of h-BN films on Ni foils from elemental B and N using molecular beam epitaxy. The presence of crystalline h-BN over the entire substrate is confirmed by Raman spectroscopy. Atomic force microscopy is used to examine the morphology and continuity of the synthesized films. A scanning electron microscopy study of films obtained using shorter depositions offers insight into the nucleation and growth behavior of h-BN on the Ni substrate. The morphology of h-BN was found to evolve from dendritic, star-shaped islands to larger, smooth triangular ones with increasing growth temperature.

  3. Quantitative measurements of electromechanical response with a combined optical beam and interferometric atomic force microscope

    Energy Technology Data Exchange (ETDEWEB)

    Labuda, Aleksander; Proksch, Roger [Asylum Research an Oxford Instruments Company, Santa Barbara, California 93117 (United States)

    2015-06-22

    An ongoing challenge in atomic force microscope (AFM) experiments is the quantitative measurement of cantilever motion. The vast majority of AFMs use the optical beam deflection (OBD) method to infer the deflection of the cantilever. The OBD method is easy to implement, has impressive noise performance, and tends to be mechanically robust. However, it represents an indirect measurement of the cantilever displacement, since it is fundamentally an angular rather than a displacement measurement. Here, we demonstrate a metrological AFM that combines an OBD sensor with a laser Doppler vibrometer (LDV) to enable accurate measurements of the cantilever velocity and displacement. The OBD/LDV AFM allows a host of quantitative measurements to be performed, including in-situ measurements of cantilever oscillation modes in piezoresponse force microscopy. As an example application, we demonstrate how this instrument can be used for accurate quantification of piezoelectric sensitivity—a longstanding goal in the electromechanical community.

  4. Adiabatic approximation for a two-level atom in a light beam

    CERN Document Server

    Aftalion, Amandine

    2011-01-01

    Following the recent experimental realization of synthetic gauge magnetic forces, Jean Dalibard adressed the question whether the adiabatic ansatz could be math- ematically justified for a model of an atom in 2 internal states, shun by a quasi resonant laser beam. In this paper, we derive rigorously the asymptotic model guessed by the physicists, and show that this asymptotic analysis contains the in- formation about the presence of vortices. Surprisingly the main difficulties do not come from the nonlinear part but from the linear Hamiltonian. More precisely, the analysis of the nonlinear minimization problem and its asymptotic reduction to simpler ones, relies on an accurate partition of low and high frequencies (or mo- menta). This requires to reconsider carefully previous mathematical works about the adiabatic limit. Although the estimates are not sharp, this asymptotic analysis provides a good insight about the validity of the asymptotic picture, with respect to the size of the many parameters initially ...

  5. Silicon dioxide mask by plasma enhanced atomic layer deposition in focused ion beam lithography

    Science.gov (United States)

    Liu, Zhengjun; Shah, Ali; Alasaarela, Tapani; Chekurov, Nikolai; Savin, Hele; Tittonen, Ilkka

    2017-02-01

    In this work, focused ion beam (FIB) lithography was developed for plasma enhanced atomic layer deposited (PEALD) silicon dioxide SiO2 hard mask. The PEALD process greatly decreases the deposition temperature of the SiO2 hard mask. FIB Ga+ ion implantation on the deposited SiO2 layer increases the wet etch resistivity of the irradiated region. A programmed exposure in FIB followed by development in a wet etchant enables the precisely defined nanoscale patterning. The combination of FIB exposure parameters and the development time provides greater freedom for optimization. The developed process provides high pattern dimension accuracy over the tested range of 90–210 nm. Utilizing the SiO2 mask developed in this work, silicon nanopillars with 40 nm diameter were successfully fabricated with cryogenic deep reactive ion etching and the aspect ratio reached 16:1. The fabricated mask is suitable for sub-100 nm high aspect ratio silicon structure fabrication.

  6. Effect of scattering on the dispersion distortions of signals and the diffraction of finite beams in the case of partial reflection from the ionosphere

    Science.gov (United States)

    Gusev, V. D.; Zhidovlenko, I. Iu.; Prikhod'Ko, L. I.

    1987-11-01

    An analysis is made of distortions of pulsed signals and finite radio-wave beams of different shape and duration in a triangular ionospheric layer with small-scale irregularities. The effects of the regular ionospheric gradient and of small-scale irregularities on the distortions are examined. The problem is solved using the method of statistical tests with modeling of the random permittivity of the ionosphere. It is shown that the spreading of the beams due to reflection and scattering significantly exceeds their diffraction divergence.

  7. Atomic Diffusion in Cu/Si (111) and Cu/SiO2/Si (111) Systems by Neutral Cluster Beam Deposition

    Institute of Scientific and Technical Information of China (English)

    CAO Bo; LI Gong-Ping; CHEN Xi-Meng; CHO Seong-Jin; KIM Hee

    2008-01-01

    @@ The Cu films are deposited on two kinds of p-type Si (111) substrates by ionized cluster beam (ICB) technique.The interface reaction and atomic diffusion of Cu/Si (111) and Cu/SiO2/Si (111) systems are studied at different annealing temperatures by x-ray diffraction (XRD) and Rutherford backscattering spectrometry (RBS). Some significant results are obtained: For the Cu/Si (111) samples prepared by neutral clusters, the interdiffusion of Cu and Si atoms occurs when annealed at 230℃. The diffusion coefficients of the samples annealed at 230℃and 500℃ are 8.5 × 10-15 cm2.s-1 and 3.0 × 10-14 cm2.s-1, respectively. The formation of the copper-silicide phase is observed by XRD, and its intensity becomes stronger with the increase of annealing temperature. For the Cu/SiO2/Si (111) samples prepared by neutral clusters, the interdiffusion of Cu and Si atoms occurs and copper silicides are formed when annealed at 450℃. The diffusion coefficients of Cu in Si are calculated to be 6.0 × 10-16 cm2.s-1 at 450℃, due to the fact that the existence of the SiO2 layer suppresses the interdiffusion of Cu and Si.

  8. Light and/or atomic beams to detect ultraweak gravitational effects

    Directory of Open Access Journals (Sweden)

    Tartaglia Angelo

    2014-06-01

    Full Text Available We shall review the opportunities lent by ring lasers and atomic beams interferometry in order to reveal gravitomagnetic effects on Earth. Both techniques are based on the asymmetric propagation of waves in the gravitational field of a rotating mass; actually the times of flight for co- or counter-rotating closed paths turn out to be different. After discussing properties and limitations of the two approaches we shall describe the proposed GINGER experiment which is being developed for the Gran Sasso National Laboratories in Italy. The experimental apparatus will consist of a three-dimensional array of square rings, 6m × 6m, that is planned to reach a sensitivity in the order of 1prad/√Hertz or better. This sensitivity would be one order of magnitude better than the best existing ring, which is the G-ring in Wettzell, Bavaria, and would allow for the terrestrial detection of the Lense-Thirring effect and possibly of deviations from General Relativity. The possibility of using either the ring laser approach or atomic interferometry in a space mission will also be considered. The technology problems are under experimental study using both the German G-ring and the smaller G-Pisa ring, located at the Gran Sasso.

  9. Photoionization Broadening of the 1S-2S Transition in a Beam of Atomic Hydrogen

    CERN Document Server

    Kolachevsky, N; Fischer, M; Haas, M; Herrmann, M; Holzwarth, R; Hänsch, T W; Jentschura, U D; Keitel, C H; Udem, T; Udem, Th.

    2006-01-01

    We consider the excitation dynamics of the two-photon \\sts transition in a beam of atomic hydrogen by 243 nm laser radiation. Specifically, we study the impact of ionization damping on the transition line shape, caused by the possibility of ionization of the $2S$ level by the same laser field. Using a Monte-Carlo simulation, we calculate the line shape of the \\sts transition for the experimental geometry used in the two latest absolute frequency measurements (M. Niering {\\it et al.}, PRL 84, 5496 (2000) and M. Fischer {\\it et al.}, PRL 92, 230802 (2004)). The calculated line shift and line width are in excellent agreement with the experimentally observed values. From this comparison we can verify the values of the dynamic Stark shift coefficient for the \\sts transition for the first time on a level of 15%. We show that the ionization modifies the velocity distribution of the metastable atoms, the line shape of the \\sts transition, and has an influence on the derivation of its absolute frequency.

  10. X-ray diffraction: instrumentation and applications.

    Science.gov (United States)

    Bunaciu, Andrei A; Udriştioiu, Elena Gabriela; Aboul-Enein, Hassan Y

    2015-01-01

    X-ray diffraction (XRD) is a powerful nondestructive technique for characterizing crystalline materials. It provides information on structures, phases, preferred crystal orientations (texture), and other structural parameters, such as average grain size, crystallinity, strain, and crystal defects. X-ray diffraction peaks are produced by constructive interference of a monochromatic beam of X-rays scattered at specific angles from each set of lattice planes in a sample. The peak intensities are determined by the distribution of atoms within the lattice. Consequently, the X-ray diffraction pattern is the fingerprint of periodic atomic arrangements in a given material. This review summarizes the scientific trends associated with the rapid development of the technique of X-ray diffraction over the past five years pertaining to the fields of pharmaceuticals, forensic science, geological applications, microelectronics, and glass manufacturing, as well as in corrosion analysis.

  11. l- and n-changing collisions during interaction of a pulsed beam of Li Rydberg atoms with CO2

    Science.gov (United States)

    Dubreuil, B.; Harnafi, M.

    1989-07-01

    The pulsed Li atomic beam produced in our experiment is based on controlled transversely-excited-atmospheric CO2 laser-induced ablation of a Li metal target. The atomic beam is propagated in vacuum or in CO2 gas at low pressure. Atoms in the beam are probed by laser-induced fluorescence spectroscopy. This allows the determination of time-of-flight and velocity distributions. Li Rydberg states (n=5-13) are populated in the beam by two-step pulsed-laser excitation. The excited atoms interact with CO2 molecules. l- and n-changing cross sections are deduced from the time evolution of the resonant or collision-induced fluorescence following this selective excitation. l-changing cross sections of the order of 104 AṦ are measured; they increase with n as opposed to the plateau observed for Li* colliding with a diatomic molecule. This behavior is qualitatively well explained in the framework of the free-electron model. n-->n' changing processes with large cross sections (10-100 AṦ) are also observed even in the case of large electronic energy change (ΔEnn'>103 cm-1). These results can be interpreted in terms of resonant-electronic to vibrational energy transfers between Li Rydberg states and CO2 vibrational modes.

  12. Detection of slow atoms confined in a Cesium vapor cell by spatially separated pump and probe laser beams

    CERN Document Server

    Todorov, Petko; Maurin, Isabelle; Saltiel, Solomon; Bloch, Daniel

    2013-01-01

    The velocity distribution of atoms in a thermal gas is usually described through a Maxwell-Boltzman distribution of energy, and assumes isotropy. As a consequence, the probability for an atom to leave the surface under an azimuth angle {\\theta} should evolve as cos {\\theta}, in spite of the fact that there is no microscopic basis to justify such a law. The contribution of atoms moving at a grazing incidence towards or from the surface, i.e. atoms with a small normal velocity, here called "slow" atoms, reveals essential in the development of spectroscopic methods probing a dilute atomic vapor in the vicinity of a surface, enabling a sub-Doppler resolution under a normal incidence irradiation. The probability for such "slow" atoms may be reduced by surface roughness and atom-surface interaction. Here, we describe a method to observe and to count these slow atoms relying on a mechanical discrimination, through spatially separated pump and probe beams. We also report on our experimental progresses toward such a g...

  13. Atoms

    Institute of Scientific and Technical Information of China (English)

    刘洪毓

    2007-01-01

    Atoms(原子)are all around us.They are something like the bricks (砖块)of which everything is made. The size of an atom is very,very small.In just one grain of salt are held millions of atoms. Atoms are very important.The way one object acts depends on what

  14. Nondestructive mapping of chemical composition and structural qualities of group III-nitride nanowires using submicron beam synchrotron-based X-ray diffraction

    Energy Technology Data Exchange (ETDEWEB)

    Bonanno, P.L., E-mail: plb2@njit.edu [Georgia Institute of Technology/GTL, UMI 2958 Georgia Tech-CNRS, 57070 Metz (France); Gautier, S. [LMOPS + UMI: Laboratoire Matériaux Optiques, Photonique et micro-nano Systèmes, UMR CNRS 7132, Université de Metz et SUPELEC, 2 rue E. Belin, 57070 Metz, France, UMI 2958 Georgia Tech-CNRS, 57070 Metz (France); Gmili, Y.El.; Moudakir, T. [UMI 2958 Georgia Tech-CNRS, 57070 Metz (France); Sirenko, A.A. [Department of Physics, New Jersey Institute of Technology, Newark, NJ 07102 (United States); Kazimirov, A. [Cornell High Energy Synchrotron Source (CHESS), Cornell University, Ithaca, NY 14853 (United States); Cai, Z.-H. [Advanced Photon Source, 9700 S. Cass Avenue, Argonne, IL 60439 (United States); Martin, J. [LMOPS + UMI: Laboratoire Matériaux Optiques, Photonique et micro-nano Systèmes, UMR CNRS 7132, Université de Metz et SUPELEC, 2 rue E. Belin, 57070 Metz, France, UMI 2958 Georgia Tech-CNRS, 57070 Metz (France); Goh, W.H. [Georgia Institute of Technology/GTL, UMI 2958 Georgia Tech-CNRS, 57070 Metz (France); Martinez, A.; Ramdane, A.; Le Gratiet, L. [Laboratoire de Photonique et de Nanostructures, UPR CNRS 20, Route de Nozay, 91460 Marcoussis (France); Maloufi, N. [Laboratoire d' Etude des Textures et Application aux Matériaux UMR CNRS 7078 Ile du Saulcy 57045 METZ cedex 1 (France); Assouar, M.B. [Laboratoire de Physique des Milieux Ionisés et Applications, Nancy University, CNRS, BP 239, F-54506 Vandoeuvre-lès-Nancy Cédex (France); Ougazzaden, A. [Georgia Institute of Technology/GTL, UMI 2958 Georgia Tech-CNRS, 57070 Metz (France)

    2013-08-31

    Submicron beam synchrotron-based X-ray diffraction (XRD) techniques have been developed and used to accurately and nondestructively map chemical composition and material quality of selectively grown group III-nitride nanowires. GaN, AlGaN, and InGaN multi-quantum-well nanowires have been selectively grown on lattice matched and mismatched substrates, and the challenges associated with obtaining and interpreting submicron beam XRD results are addressed and solved. Nanoscale cathodoluminescence is used to examine exciton behavior, and energy-dispersive X-ray spectroscopy is used to verify chemical composition. Scanning transmission electron microscopy is later used to paint a more complete picture. The advantages of submicron beam XRD over other techniques are discussed in the context of this challenging material system. - Highlights: ► We used nano selective area growth to create nanowires of GaN, AlGaN and InGaN/GaN. ► We characterized them by synchrotron-based submicron beam X-ray diffraction (XRD). ► This technique accurately determined chemical and crystallographic properties. ► Challenges of XRD are addressed in the context of this challenging material system. ► Advantages of XRD over other characterization methods are discussed.

  15. Stress evaluation in thin films: Micro-focus synchrotron X-ray diffraction combined with focused ion beam patterning for d{sub o} evaluation

    Energy Technology Data Exchange (ETDEWEB)

    Baimpas, Nikolaos, E-mail: nikolaos.baimpas@eng.ox.ac.uk [University of Oxford, Dept. of Engineering Science (United Kingdom); Le Bourhis, Eric [University of Poitiers, Institut P' , Laboratoire de Physique des Matériaux, Poitiers (France); Eve, Sophie [ENSICAEN, CRISMAT, Caen (France); Thiaudière, Dominique [Synchrotron SOLEIL, L' Orme des Merisiers Saint-Aubin, Paris (France); Hardie, Christopher [University of Oxford, Materials Department (United Kingdom); Korsunsky, Alexander M. [University of Oxford, Dept. of Engineering Science (United Kingdom)

    2013-12-31

    Nanocrystalline metallic coatings of sub-micron thickness are widely used in modern microelectronic applications. In X-ray diffraction experiments to determine both the residual and applied stresses in nanocrystalline coatings, one difficult challenge that comes up invariably is the determination of the strain-free lattice spacing d{sub o}. The present study addresses this challenge by using the focused ion beam (FIB) to generate a built-in strain-free reference by patterning (milling) a 50 × 50 μm{sup 2} region of the coating to produce an array of small stress-relieved “islands” ∼ 0.8 × 0.8 μm{sup 2} each. Transmission X-ray diffraction setup was used for data collection at DIFFABS beamline (Synchrotron SOLEIL, France). A 150 nm-thick multi-layered W–Cu nano-composite thin film on polyimide (Kapton®) substrate was studied. The samples were loaded incrementally using a compact uniaxial loading device, and micro-beam diffraction data were collected on and away from the reference array. It was shown experimentally that the “island” array remained approximately strain free throughout the experiment, providing an on-board d{sub o} lattice spacing reference. The changing lattice spacing d in the coating was also monitored away from the array, to deduce the elastic strain evolution during deformation. The results and their implications are presented and discussed. - Highlights: • In situ deformation study of laminate polycrystalline W–Cu thin films • Focused ion beam (FIB) patterning of an array of “islands” on thin films surface • X-ray diffraction on island-patterned region • Constant strain on “islands” independently of the deformation of the substrate.

  16. Near-diffraction-limited segmented broad area diode laser based on off-axis spectral beam combining

    DEFF Research Database (Denmark)

    Jensen, O.B.; Thestrup Nielsen, Birgitte; Andersen, Peter E.;

    2006-01-01

    The beam quality of a 500-mu m-wide broad area diode laser with five active segments has been improved beyond the beam quality of the individual segments. The principle of this new laser system is based on off-axis feedback in combination with spectral beam combining. By using a double......-feedback scheme we are able to improve the beam quality of the laser by a factor of 23 from M-2 = 55 for the free-running diode laser to M-2 = 2.4 for the laser with feedback at a drive current of 2.2 A. The improved M-2 value is a factor of 3.4 below M-2 = 8.2 for a single free-running segment. This is the first...... time that the beam quality of a segmented broad area diode laser has been improved beyond the beam quality of the individual segments....

  17. Customized atomic force microscopy probe by focused-ion-beam-assisted tip transfer

    Energy Technology Data Exchange (ETDEWEB)

    Wang, Andrew; Butte, Manish J., E-mail: manish.butte@stanford.edu [Department of Pediatrics, Division of Immunology, Allergy and Rheumatology, Stanford University, Stanford, California 94305 (United States)

    2014-08-04

    We present a technique for transferring separately fabricated tips onto tipless atomic force microscopy (AFM) cantilevers, performed using focused ion beam-assisted nanomanipulation. This method addresses the need in scanning probe microscopy for certain tip geometries that cannot be achieved by conventional lithography. For example, in probing complex layered materials or tall biological cells using AFM, a tall tip with a high-aspect-ratio is required to avoid artifacts caused by collisions of the tip's sides with the material being probed. We show experimentally that tall (18 μm) cantilever tips fabricated by this approach reduce squeeze-film damping, which fits predictions from hydrodynamic theory, and results in an increased quality factor (Q) of the fundamental flexural mode. We demonstrate that a customized tip's well-defined geometry, tall tip height, and aspect ratio enable improved measurement of elastic moduli by allowing access to low-laying portions of tall cells (T lymphocytes). This technique can be generally used to attach tips to any micromechanical device when conventional lithography of tips cannot be accomplished.

  18. Breaking the diffraction-limited resolution barrier in fiber-optical two-photon fluorescence endoscopy by an azimuthally-polarized beam.

    Science.gov (United States)

    Gu, Min; Kang, Hong; Li, Xiangping

    2014-01-10

    Although fiber-optical two-photon endoscopy has been recognized as a potential high-resolution diagnostic and therapeutic procedure in vivo, its resolution is limited by the optical diffraction nature to a few micrometers due to the low numerical aperture of an endoscopic objective. On the other hand, stimulated emission depletion (STED) achieved by a circularly-polarized vortex beam has been used to break the diffraction-limited resolution barrier in a bulky microscope. It has been a challenge to apply the STED principle to a fiber-optical two-photon endoscope as a circular polarization state cannot be maintained due to the birefringence of a fiber. Here, we demonstrate the first fiber-optical STED two-photon endoscope using an azimuthally-polarized beam directly generated from a double-clad fiber. As such, the diffraction-limited resolution barrier of fiber-optical two-photon endoscopy can be broken by a factor of three. Our new accomplishment has paved a robust way for high-resolution in vivo biomedical studies.

  19. Atomic Layer Epitaxy of h-BN(0001) Multilayers on Co(0001) and Molecular Beam Epitaxy Growth of Graphene on h-BN(0001)/Co(0001).

    Science.gov (United States)

    Driver, M Sky; Beatty, John D; Olanipekun, Opeyemi; Reid, Kimberly; Rath, Ashutosh; Voyles, Paul M; Kelber, Jeffry A

    2016-03-22

    The direct growth of hexagonal boron nitride (h-BN) by industrially scalable methods is of broad interest for spintronic and nanoelectronic device applications. Such applications often require atomically precise control of film thickness and azimuthal registry between layers and substrate. We report the formation, by atomic layer epitaxy (ALE), of multilayer h-BN(0001) films (up to 7 monolayers) on Co(0001). The ALE process employs BCl3/NH3 cycles at 600 K substrate temperature. X-ray photoelectron spectroscopy (XPS) and low energy electron diffraction (LEED) data show that this process yields an increase in h-BN average film thickness linearly proportional to the number of BCl3/NH3 cycles, with BN layers in azimuthal registry with each other and with the Co(0001) substrate. LEED diffraction spot profile data indicate an average BN domain size of at least 1900 Å. Optical microscopy data indicate the presence of some domains as large as ∼20 μm. Transmission electron microscopy (TEM) and ambient exposure studies demonstrate macroscopic and microscopic continuity of the h-BN film, with the h-BN film highly conformal to the Co substrate. Photoemission data show that the h-BN(0001) film is p-type, with band bending near the Co/h-BN interface. Growth of graphene by molecular beam epitaxy (MBE) is observed on the surface of multilayer h-BN(0001) at temperatures of 800 K. LEED data indicate azimuthal graphene alignment with the h-BN and Co(0001) lattices, with domain size similar to BN. The evidence of multilayer BN and graphene azimuthal alignment with the lattice of the Co(0001) substrate demonstrates that this procedure is suitable for scalable production of heterojunctions for spintronic applications.

  20. Generations of dark hollow beams and their applications in laser cooling of atoms and all optical-type Bose-Einstein condensation

    Institute of Scientific and Technical Information of China (English)

    印建平; 高伟建; 王海峰; 龙全; 王育竹

    2002-01-01

    We report on a new experimental result to generate dark hollow beams by using a geometric optical method.We propose two new methods to produce focused and localized hollow laser beams by using π-phase plates. UsingMonte-Carlo simulations, we have studied the Sisyphus cooling of alkali atoms in pyramidal hollow beam gravito-opticaltraps. We discuss some potential applications of the dark hollow beams in atom optics and the preparation of an alloptically-cooled and optically-trapped atomic Bose-Einstein condensation (BEC).Our research shows that an ultracoldatomic sample with a temperature of ~ 2μK can be obtained in the pyramidal hollow beam dipole trap and an alloptical-type BEC may be realized in a far blue-detuned, hollow beam trap.

  1. A trapped atom interferometer with ultracold Sr atoms

    CERN Document Server

    Zhang, Xian; Mazzoni, Tommaso; Poli, Nicola; Tino, Guglielmo M

    2016-01-01

    We report on a trapped atom interferometer based on Bragg diffraction and Bloch oscillations with alkaline-earth-metal atoms. We use a Ramsey-Bord\\'e Bragg interferometer with $^{88}$Sr atoms combined with Bloch oscillations to extend the interferometer time. Thanks to a long coherence time for Bloch oscillations of $^{88}$Sr atoms, we observed interference up to 1 s evolution time in the lattice. A detailed study of decoherence sources during the Bloch phase is also presented. While still limited in sensitivity by lattice lifetime and beam inhomogeneity this result opens the way to high contrast trapped interferometers with extended interrogation time.

  2. External Heavy-Atom Effect via Orbital Interactions Revealed by Single-Crystal X-ray Diffraction.

    Science.gov (United States)

    Sun, Xingxing; Zhang, Baicheng; Li, Xinyang; Trindle, Carl O; Zhang, Guoqing

    2016-07-28

    Enhanced spin-orbit coupling through external heavy-atom effect (EHE) has been routinely used to induce room-temperature phosphorescence (RTP) for purely organic molecular materials. Therefore, understanding the nature of EHE, i.e., the specific orbital interactions between the external heavy atom and the luminophore, is of essential importance in molecular design. For organic systems, halogens (e.g., Cl, Br, and I) are the most commonly seen heavy atoms serving to realize the EHE-related RTP. In this report, we conduct an investigation on how heavy-atom perturbers and aromatic luminophores interact on the basis of data obtained from crystallography. We synthesized two classes of molecular systems including N-haloalkyl-substituted carbazoles and quinolinium halides, where the luminescent molecules are considered as "base" or "acid" relative to the heavy-atom perturbers, respectively. We propose that electron donation from a π molecular orbital (MO) of the carbazole to the σ* MO of the C-X bond (π/σ*) and n electron donation to a π* MO of the quinolinium moiety (n/π*) are responsible for the EHE (RTP) in the solid state, respectively.

  3. Performance of an optical encoder based on a nondiffractive beam implemented with a specific photodetection integrated circuit and a diffractive optical element.

    Science.gov (United States)

    Quintián, Fernando Perez; Calarco, Nicolás; Lutenberg, Ariel; Lipovetzky, José

    2015-09-01

    In this paper, we study the incremental signal produced by an optical encoder based on a nondiffractive beam (NDB). The NDB is generated by means of a diffractive optical element (DOE). The detection system is composed by an application specific integrated circuit (ASIC) sensor. The sensor consists of an array of eight concentric annular photodiodes, each one provided with a programmable gain amplifier. In this way, the system is able to synthesize a nonuniform detectivity. The contrast, amplitude, and harmonic content of the sinusoidal output signal are analyzed. The influence of the cross talk among the annular photodiodes is placed in evidence through the dependence of the signal contrast on the wavelength.

  4. Gaussian Schell Source as Model for Slit-Collimated Atomic and Molecular Beams

    CERN Document Server

    McMorran, Ben

    2008-01-01

    We show how to make a Gaussian Schell-model (GSM) beam. Then we compare the intensity profile, the transverse coherence width and the divergence angle of a GSM beam with those same properties of a beam that is collimated with two hard-edged slits. This work offers an intuitive way to understand various interferometer designs, and we compare our results with data.

  5. Development of the negative ion beams relevant to ITER and JT-60SA at Japan Atomic Energy Agency

    Energy Technology Data Exchange (ETDEWEB)

    Hanada, M., E-mail: hanada.masaya@jaea.go.jp; Kojima, A.; Tobari, H.; Nishikiori, R.; Hiratsuka, J.; Kashiwagi, M.; Umeda, N.; Yoshida, M.; Ichikawa, M.; Watanabe, K. [Japan Atomic Energy Agency, 801-1 Mukouyama, Naka-shi, Ibaraki-ken 319-0913 (Japan); Yamano, Y. [Saitama University, Saitama, Saitama-ken 338-8570 (Japan); Grisham, L. R. [Princeton Plasma Physics Laboratory, Princeton, New Jersey 08543 (United States)

    2016-02-15

    In order to realize negative ion sources and accelerators to be applicable to International Thermonuclear Experimental Reactor and JT-60 Super Advanced, a large cesium (Cs)-seeded negative ion source and a multi-aperture and multi-stage electric acceleration have been developed at Japan Atomic Energy Agency (JAEA). Long pulse production and acceleration of the negative ion beams have been independently carried out. The long pulse production of the high current beams has achieved 100 s at the beam current of 15 A by modifying the JT-60 negative ion source. The pulse duration time is increased three times longer than that before the modification. As for the acceleration, a pulse duration time has been also extended two orders of magnitudes from 0.4 s to 60 s. The developments of the negative ion source and acceleration at JAEA are well in progress towards the realization of the negative ion sources and accelerators for fusion applications.

  6. Development of the negative ion beams relevant to ITER and JT-60SA at Japan Atomic Energy Agency.

    Science.gov (United States)

    Hanada, M; Kojima, A; Tobari, H; Nishikiori, R; Hiratsuka, J; Kashiwagi, M; Umeda, N; Yoshida, M; Ichikawa, M; Watanabe, K; Yamano, Y; Grisham, L R

    2016-02-01

    In order to realize negative ion sources and accelerators to be applicable to International Thermonuclear Experimental Reactor and JT-60 Super Advanced, a large cesium (Cs)-seeded negative ion source and a multi-aperture and multi-stage electric acceleration have been developed at Japan Atomic Energy Agency (JAEA). Long pulse production and acceleration of the negative ion beams have been independently carried out. The long pulse production of the high current beams has achieved 100 s at the beam current of 15 A by modifying the JT-60 negative ion source. The pulse duration time is increased three times longer than that before the modification. As for the acceleration, a pulse duration time has been also extended two orders of magnitudes from 0.4 s to 60 s. The developments of the negative ion source and acceleration at JAEA are well in progress towards the realization of the negative ion sources and accelerators for fusion applications.

  7. Atom probe tomography characterisation of a laser diode structure grown by molecular beam epitaxy

    Energy Technology Data Exchange (ETDEWEB)

    Bennett, Samantha E.; Humphreys, Colin J.; Oliver, Rachel A. [Department of Materials Science and Metallurgy, University of Cambridge, Pembroke Street, Cambridge, CB2 3QZ (United Kingdom); Smeeton, Tim M.; Hooper, Stewart E.; Heffernan, Jonathan [Sharp Laboratories of Europe Limited, Edmund Halley Road, Oxford Science Park, Oxford, OX4 4GB (United Kingdom); Saxey, David W.; Smith, George D. W. [Department of Materials, University of Oxford, Parks Road, Oxford, OX1 3PH (United Kingdom)

    2012-03-01

    Atom probe tomography (APT) has been used to achieve three-dimensional characterization of a III-nitride laser diode (LD) structure grown by molecular beam epitaxy (MBE). Four APT data sets have been obtained, with fields of view up to 400 nm in depth and 120 nm in diameter. These data sets contain material from the InGaN quantum well (QW) active region, as well as the surrounding p- and n-doped waveguide and cladding layers, enabling comprehensive study of the structure and composition of the LD structure. Two regions of the same sample, with different average indium contents (18% and 16%) in the QW region, were studied. The APT data are shown to provide easy access to the p-type dopant levels, and the composition of a thin AlGaN barrier layer. Next, the distribution of indium within the InGaN QW was analyzed, to assess any possible inhomogeneity of the distribution of indium (''indium clustering''). No evidence for a statistically significant deviation from a random distribution was found, indicating that these MBE-grown InGaN QWs do not require indium clusters for carrier localization. However, the APT data show steps in the QW interfaces, leading to well-width fluctuations, which may act to localize carriers. Additionally, the unexpected presence of a small amount (x = 0.005) of indium in a layer grown intentionally as GaN was revealed. Finally, the same statistical method applied to the QW was used to show that the indium distribution within a thick InGaN waveguide layer in the n-doped region did not show any deviation from randomness.

  8. Two-color above threshold ionization of atoms and ions in XUV Bessel beams and combined with intense laser light

    CERN Document Server

    Seipt, D; Surzhykov, A; Fritzsche, S

    2016-01-01

    The two-color above-threshold ionization (ATI) of atoms and ions is investigated for a vortex Bessel beam in the presence of a strong near-infrared (NIR) light field. While the photoionization is caused by the photons from the weak but extreme ultra-violet (XUV) vortex Bessel beam, the energy and angular distribution of the photoelectrons and their sideband structure are affected by the plane-wave NIR field. We here explore the energy spectra and angular emission of the photoelectrons in such two-color fields as a function of the size and location of the target (atoms) with regard to the beam axis. In addition, analogue to the circular dichroism in typical two-color ATI experiments with circularly polarized light, we define and discuss seven different dichroism signals for such vortex Bessel beams that arise from the various combinations of the orbital and spin angular momenta of the two light fields. For localized targets, it is found that these dichroism signals strongly depend on the size and position of t...

  9. Diffraction pattern by nanometric thin films under illumination of an orbital angular momentum beam with integer topological charge

    Science.gov (United States)

    Mendoza, J. H.; Díaz, C. F.; Acevedo, C. H.; Torres, Y.

    2016-02-01

    The orbital angular momentum of light has a big contribution in many engineering applications like optical communications, because this physical property allows eigenstates characteristic of the wavefront rotation when the beam is propagated. The nature of these eigenstates allows that information can be encoded and gives immunity to electromagnetic interference, allowing an increase of bandwidth, cadence and capacity of the communication channel. This work shown the methodology using nanometric thin films like Titanium based (TiO2) grown over strontium titanate (SrTiO3) support, to distinguish and discriminate a well- defined integer value of the topological charge of an OAM beam.

  10. High-energy transmission Laue micro-beam X-ray diffraction: a probe for intra-granular lattice orientation and elastic strain in thicker samples.

    Science.gov (United States)

    Hofmann, Felix; Song, Xu; Abbey, Brian; Jun, Tea-Sung; Korsunsky, Alexander M

    2012-05-01

    An understanding of the mechanical response of modern engineering alloys to complex loading conditions is essential for the design of load-bearing components in high-performance safety-critical aerospace applications. A detailed knowledge of how material behaviour is modified by fatigue and the ability to predict failure reliably are vital for enhanced component performance. Unlike macroscopic bulk properties (e.g. stiffness, yield stress, etc.) that depend on the average behaviour of many grains, material failure is governed by `weakest link'-type mechanisms. It is strongly dependent on the anisotropic single-crystal elastic-plastic behaviour, local morphology and microstructure, and grain-to-grain interactions. For the development and validation of models that capture these complex phenomena, the ability to probe deformation behaviour at the micro-scale is key. The diffraction of highly penetrating synchrotron X-rays is well suited to this purpose and micro-beam Laue diffraction is a particularly powerful tool that has emerged in recent years. Typically it uses photon energies of 5-25 keV, limiting penetration into the material, so that only thin samples or near-surface regions can be studied. In this paper the development of high-energy transmission Laue (HETL) micro-beam X-ray diffraction is described, extending the micro-beam Laue technique to significantly higher photon energies (50-150 keV). It allows the probing of thicker sample sections, with the potential for grain-level characterization of real engineering components. The new HETL technique is used to study the deformation behaviour of individual grains in a large-grained polycrystalline nickel sample during in situ tensile loading. Refinement of the Laue diffraction patterns yields lattice orientations and qualitative information about elastic strains. After deformation, bands of high lattice misorientation can be identified in the sample. Orientation spread within individual scattering volumes is

  11. The structures and dynamics of atomic and molecular adsorbates on metal surfaces by scanning tunneling microscopy and low energy electron diffraction

    Energy Technology Data Exchange (ETDEWEB)

    Yoon, Hyungsuk Alexander [Univ. of California, Berkeley, CA (United States)

    1996-12-01

    Studies of surface structure and dynamics of atoms and molecules on metal surfaces are presented. My research has focused on understanding the nature of adsorbate-adsorbate and adsorbate-substrate interactions through surface studies of coverage dependency and coadsorption using both scanning tunneling microscopy (STM) and low energy electron diffraction (LEED). The effect of adsorbate coverage on the surface structures of sulfur on Pt(111) and Rh(111) was examined. On Pt(111), sulfur forms p(2x2) at 0.25 ML of sulfur, which transforms into a more compressed (√3x√3)R30° at 0.33 ML. On both structures, it was found that sulfur adsorbs only in fcc sites. When the coverage of sulfur exceeds 0.33 ML, it formed more complex c(√3x7)rect structure with 3 sulfur atoms per unit cell. In this structure, two different adsorption sites for sulfur atoms were observed - two on fcc sites and one on hcp site within the unit cell.

  12. Creation evidence of the second non-dispersive Zakharenko wave by helium atomic beams in superfluid helium-II at low temperatures

    Indian Academy of Sciences (India)

    A A Zakharenko

    2007-10-01

    In this work, the experimental results of the creation of the second non-dispersive Zakharenko wave (ph = g ≠ 0) in the negative roton branch (the so-called second sound) of the bulk elementary excitations (BEEs) energy spectra are introduced. Several BEE signals detected by a bolometer situated in the isotopically pure liquid helium-II at low temperatures ∼ 100 mK are shown, which give evidence of negative roton creation in the liquid by helium atomic beams striking the liquid surface. The negative roton signals were clearly distinguished by the following ways: the negative roton signal created by helium atomic beams appeared earlier than the positive roton signal created by the beams, and presence of both positive and negative roton signals together. It is natural that the negative roton creation by the beams requires the 4He-atom energies ∼ 12 K, while the positive roton creation by the atomic beams requires energies ∼ 35 K. Therefore, successive increase in the heater power resulting in an increase in the 4He-atom energies gives solid evidence that the negative rotons are first created in the liquid by the helium atomic beams.

  13. Production, formation, and transport of high-brightness atomic hydrogen beam studies for the relativistic heavy ion collider polarized source upgrade

    Energy Technology Data Exchange (ETDEWEB)

    Kolmogorov, A., E-mail: anton.kolmogorov@gmail.com; Stupishin, N. [Budker Institute of Nuclear Physics, Novosibirsk (Russian Federation); Atoian, G.; Ritter, J.; Zelenski, A. [Brookhaven National Laboratory, Upton, New York 11973 (United States); Davydenko, V.; Ivanov, A. [Budker Institute of Nuclear Physics, Novosibirsk (Russian Federation); Novosibirsk State University, Novosibirsk (Russian Federation)

    2014-02-15

    The RHIC polarized H{sup −} ion source had been successfully upgraded to higher intensity and polarization by using a very high brightness fast atomic beam source developed at BINP, Novosibirsk. In this source the proton beam is extracted by a four-grid multi-aperture ion optical system and neutralized in the H{sub 2} gas cell downstream from the grids. The proton beam is extracted from plasma emitter with a low transverse ion temperature of ∼0.2 eV which is formed by plasma jet expansion from the arc plasma generator. The multi-hole grids are spherically shaped to produce “geometrical” beam focusing. Proton beam formation and transport of atomic beam were experimentally studied at test bench.

  14. Test of Equivalence Principle at 1 0-8 Level by a Dual-Species Double-Diffraction Raman Atom Interferometer

    Science.gov (United States)

    Zhou, Lin; Long, Shitong; Tang, Biao; Chen, Xi; Gao, Fen; Peng, Wencui; Duan, Weitao; Zhong, Jiaqi; Xiong, Zongyuan; Wang, Jin; Zhang, Yuanzhong; Zhan, Mingsheng

    2015-07-01

    We report an improved test of the weak equivalence principle by using a simultaneous 85Rb-87Rb dual-species atom interferometer. We propose and implement a four-wave double-diffraction Raman transition scheme for the interferometer, and demonstrate its ability in suppressing common-mode phase noise of Raman lasers after their frequencies and intensity ratios are optimized. The statistical uncertainty of the experimental data for Eötvös parameter η is 0.8 ×1 0-8 at 3200 s. With various systematic errors corrected, the final value is η =(2.8 ±3.0 )×1 0-8. The major uncertainty is attributed to the Coriolis effect.

  15. Atomic substitution effects on the structural and vibrational properties of NixPb1-xTiO3: X-ray diffraction and Raman scattering investigations

    Directory of Open Access Journals (Sweden)

    R. C. da Costa

    2015-07-01

    Full Text Available The effects of the atomic substitution of Pb by Ni in the PbTiO3 ferroelectric perovskite on the vibrational and structural properties was studied using x-ray diffraction and Raman scattering. It was observed that for Ni concentrations between 0.0 and 0.4, there is the formation of a solid solution with reduction of the Raman wavenumber of the E(TO1 soft mode and the tetragonallity factor, which influence directly the temperature of the tetragonal ferroelectric to cubic paraelectric phase transition, the Curie temperature. For concentrations greater than 0.4, it is observed the formation of a PbTiO3 and NiTiO3 composite, denounced by the recovering of the both, tetragonallity factor and the E(TO1 soft mode wavenumber. The values of the Curie temperatures were estimated by the Raman scattering measurements for temperatures ranging from 300 to 950 K.

  16. Surface structures from low energy electron diffraction: Atoms, small molecules and an ordered ice film on metal surfaces

    Energy Technology Data Exchange (ETDEWEB)

    Materer, N.F.

    1995-09-01

    We investigated the surface bonding of various adsorbates (0, S, C{sub 2}H{sub 3} and NO) along with the resulting relaxation of the Pt(111) surface using low energy electron diffiraction (LEED). LEED experiments have been performed on these ordered overlayers along with theoretical structural analysis using automated tensor LEED (ATLEED). The resulting surface structures of these ordered overlayers exhibit similar adsorbate-induced relaxations. In all cases the adsorbate occupies the fcc hollow site and induces an approximately 0.1 A buckling of the metal surface. The three metal atoms directly bonded to the adsorbate are ``pulled`` out of the surface and the metal atom that is not bound to the adsorbate is `pushed`` inward. In order to understand the reliability of such details, we have carried out a comprehensive study of various non-structural parameters used in a LEED computation. We also studied the adsorption of water on the Pt(lll) surface. We ordered an ultra thin ice film on this surface. The film`s surface is found to be the (0001) face of hexagonal ice. This surface is apparently terminated by a full-bilayer, in which the uppermost water molecules have large vibrational amplitudes even at temperatures as low as 90 K. We examined two other metal surfaces besides Pt(111): Ni(111) and Fe(lll). On Ni(111), we have studied the surface under a high coverage of NO. On both Ni(111) and Pt(111) NO molecules occupy the hollow sites and the N-0 bond distances are practically identical. The challenging sample preparation of an Fe(111) surface has been investigated and a successful procedure has been obtained. The small interlayer spacing found on Fe(111) required special treatment in the LEED calculations. A new ATLEED program has been developed to handle this surface.

  17. Production of rare-earth atomic negative ion beams in a cesium-sputter-type negative ion source

    Energy Technology Data Exchange (ETDEWEB)

    Davis, V.T. [Test Support Division, Defense Threat Reduction Agency, West Desert Test Center, Dugway, UT 84022-5000 (United States)]. E-mail: vernon.davis@us.army.mil; Covington, A.M. [Department of Physics, University of Nevada, MS 220, Reno, NV 89557-0058 (United States); Duvvuri, S.S. [Department of Physics, University of Nevada, MS 220, Reno, NV 89557-0058 (United States); Kraus, R.G. [Department of Physics, University of Nevada, MS 220, Reno, NV 89557-0058 (United States); Emmons, E.D. [Department of Physics, University of Nevada, MS 220, Reno, NV 89557-0058 (United States); Kvale, T.J. [Department of Physics and Astronomy, University of Toledo, Toledo, OH (United States); Thompson, J.S. [Department of Physics, University of Nevada, MS 220, Reno, NV 89557-0058 (United States)

    2007-08-15

    The desire to study negative ion structure and negative ion-photon interactions has spurred the development of ion sources for use in research and industry. The many different types of negative ion sources available today differ in their characteristics and abilities to produce anions of various species. Thus the importance of choosing the correct type of negative ion source for a particular research or industrial application is clear. In this study, the results of an investigation on the production of beams composed of negatively-charged rare-earth ions from a cylindrical-cathode-geometry, cesium-sputter-type negative ion source are presented. Beams of atomic anions have been observed for most of the first-row rare-earth elements, with typical currents ranging from hundreds of picoamps to several nanoamps.

  18. Refinement of atomic and magnetic structures using neutron diffraction for synthesized bulk and nano-nickel zinc gallate ferrite

    Energy Technology Data Exchange (ETDEWEB)

    Ata-Allah, S.S. [Reactor Physics Department, NRC, Atomic Energy Authority, P.O. Box 13759, Cairo (Egypt); Balagurov, A.M. [Frank Laboratory of Neutron Physics, JINR, 141980 Dubna, Moscow region (Russian Federation); Hashhash, A. [Reactor Physics Department, NRC, Atomic Energy Authority, P.O. Box 13759, Cairo (Egypt); Bobrikov, I.A. [Frank Laboratory of Neutron Physics, JINR, 141980 Dubna, Moscow region (Russian Federation); Hamdy, Sh. [Reactor Physics Department, NRC, Atomic Energy Authority, P.O. Box 13759, Cairo (Egypt)

    2016-01-15

    The parent NiFe{sub 2}O{sub 4} and Zn/Ga substituted spinel ferrite powders have been prepared by solid state reaction technique. As a typical example, the Ni{sub 0.7}Zn{sub 0.3}Fe{sub 1.5}Ga{sub 0.5}O{sub 4} sample has been prepared by sol–gel auto combustion method with the nano-scale crystallites size. X-ray and Mössbauer studies were carried out for the prepared samples. Structure and microstructure properties were investigated using the time-of-flight HRFD instrument at the IBR-2 pulsed reactor, at a temperatures range 15–473 K. The Rietveld refinement of the neutron diffraction data revealed that all samples possess cubic symmetry corresponding to the space group Fd3m. Cations distribution show that Ni{sup 2+} is a complete inverse spinel ion, while Ga{sup 3+} equally distributed between the two A and B-sublattices. The level of microstrains in bulk samples was estimated as very small while the size of coherently scattered domains is quite large. For nano-structured sample the domain size is around 120 Å.

  19. 高通量冷原子束流的实现与测量%Realization and Measurement of a High-flux Atomic Beam

    Institute of Scientific and Technical Information of China (English)

    张玉驰; 亓鲁; 王同雨; 房建成

    2013-01-01

    A high-flux Cesium atomic beam is produced from a 2D+ Magneto-optical trap (MOT).The cald atomic beam has a flux of about 8.5 × 1010 atoms/s,a mean velocity of about 16 m/s,velocity distribution of 4 m/s and has a divergence of 25 mrad.Phase-sensitive time-of-flight method is used to measure the flux of the atomic beam.It is also investigated that how the atomic beam depends on the background alkali pressure,the power of push beam,and the detuning of the cooling beams of 2D+MOT.%我们在实验上基于铯原子的2D+磁光阱获得了通量为8.5×1010原子/s、平均速度与速度分布分别为16 m/s与4 m/s、空间发散角为25 mrad的冷原子束流,通过相敏的飞行时间法对原子束流的通量进行了准确测量,并对背景原子气压、推送光功率以及冷却光失谐等参量对原子束流的影响进行了实验研究与分析.

  20. Atomic radical abatement of organic impurities from electron beam deposited metallic structures

    NARCIS (Netherlands)

    Wnuk, J.D.; Gorham, J.M.; Rosenberg, S.G.; Madey, T.E.; Hagen, C.W.; Fairbrother, D.H.

    2010-01-01

    Focused electron beam induced processing (FEBIP) of volatile organometallic precursors has become an effective and versatile method of fabricating metal-containing nanostructures. However, the electron stimulated decomposition process responsible for the growth of these nanostructures traps much of

  1. A collimated focused ultrasound beam of high acoustic transmission and minimum diffraction achieved by using a lens with subwavelength structures

    Energy Technology Data Exchange (ETDEWEB)

    Lin, Zhou; Tu, Juan; Cheng, Jianchun [Key Laboratory of Modern Acoustics (MOE), Department of Physics, Collaborative Innovation Center of Advanced Microstructure, Nanjing University, Nanjing 210093 (China); Guo, Xiasheng, E-mail: guoxs@nju.edu.cn, E-mail: dzhang@nju.edu.cn [Key Laboratory of Modern Acoustics (MOE), Department of Physics, Collaborative Innovation Center of Advanced Microstructure, Nanjing University, Nanjing 210093 (China); Department of Engineering Science and Mechanics, The Pennsylvania State University, University Park, Pennsylvania 16802 (United States); Wu, Junru [Department of Physics, University of Vermont, Burlington, Vermont 05405 (United States); Huang, Pingtong [Department of Ultrasound, The Second Affiliated Hospital of Zhejiang University School of Medicine, Hangzhou 310009 (China); Zhang, Dong, E-mail: guoxs@nju.edu.cn, E-mail: dzhang@nju.edu.cn [Key Laboratory of Modern Acoustics (MOE), Department of Physics, Collaborative Innovation Center of Advanced Microstructure, Nanjing University, Nanjing 210093 (China); The State Key Laboratory of Acoustics, Chinese Academy of Science, Beijing 10080 (China)

    2015-09-14

    An acoustic focusing lens incorporated with periodically aligned subwavelength grooves corrugated on its spherical surface has been developed. It is demonstrated theoretically and experimentally that acoustic focusing achieved by using the lens can suppress the relative side-lobe amplitudes, enhance the focal gain, and minimize the shifting of the focus. Use of the lens coupled with a planar ultrasound transducer can generate an ultrasound beam with enhanced acoustic transmission and collimation effect, which offers the capability of improving the safety, efficiency, and accuracy of targeted surgery implemented by high intensity focused ultrasound.

  2. Stochastic growth theory of molecular beam epitaxy with atom correlation effects: A Monte-Carlo master equation method

    Science.gov (United States)

    Nakayama, Hiroshi; Furuichi, Akihisa; Kita, Takashi; Nishino, Taneo

    1997-04-01

    Structural phase transition of epitaxial growing layer is quite important to understand the atomic scale mechanism of molecular beam epitaxy (MBE). GaAs and related alloy semiconductors are typical systems which show variety of such structural transitions during MBE. Structural evolution of surface reconstruction phases and an order-disorder transition in III-V alloy semiconductors are typical cases where such phase transitions appear during epitaxial processes. In this work, a stochastic theory and the Monte-Carlo simulation have been presented to describe the structural evolution of epitaxial growth in binary system. This method, known here as the 'Monte-Carlo master equation (MCME) method', couples a master equation for epitaxial growth kinetics with an Ising Hamiltonian of growing surface. The Monte-Carlo (MC) simulation of binary growing surface with atom-correlation effects has successfully revealed the evolution of atomic structure and the formation of short-range ordering (SRO) during epitaxy. This demonstrates the usefulness of the MCME method in describing the atomic-structural dynamics as compared with a conventional theory of epitaxy based on a diffusion equation and standard nucleation theory.

  3. Measurement of Wigner function via atomic beam deflection in Raman- Nath regime

    CERN Document Server

    Khosa, A H; Khosa, Ashfaq Hussain

    2002-01-01

    We propose a method for the reconstruction of photon statistics and hence the Wigner function of a quantized cavity field. The method is based on the measurement of momentum distribution of two level atoms after atom- field interaction in Raman-Nath regime. We reconstruct the photon statistics of the cavity field both the cases of resonant and off- resonant atom field interaction.. For the measurement of Wigner function we propose to displace the photon statistics of the cavity field. We successfully reconstruct the Wigner function of the Schrodinger-cat state in a straightforward manner by employing the proposed method without much mathematical manipulation of the experimental data.

  4. DESIGNING A DIFFRACTIVE OPTICAL ELEMENT FOR CONTROLLING THE BEAM PROFILE IN A THREE-DIMENSIONAL SPACE USING THE SIMULATED ANNEALING ALGORITHM

    Institute of Scientific and Technical Information of China (English)

    LIANG WEN-XI; ZHANG JING-JUAN; L(U) JUN-FENG; LIAO RUI

    2001-01-01

    We have designed a spatially quantized diffractive optical element (DOE) for controlling the beam profile in a three-dimensional space with the help of the simulated annealing (SA) algorithm. In this paper, we investigate the annealing schedule and the neighbourhood which are the deterministic parameters of the process that warrant the quality of the SA algorithm. The algorithm is employed to solve the discrete stochastic optimization problem of the design of a DOE. The objective function which constrains the optimization is also studied. The computed results demonstrate that the procedure of the algorithm converges stably to an optimal solution close to the global optimum with an acceptable computing time. The results meet the design requirement well and are applicable.

  5. A convergent-beam electron diffraction study of strain homogeneity in severely strained aluminum processed by equal-channel angular pressing

    Energy Technology Data Exchange (ETDEWEB)

    Alhajeri, Saleh N. [Materials Research Group, Faculty of Engineering and the Environment, University of Southampton, Southampton SO17 1BJ (United Kingdom); Department of Manufacturing Engineering, College of Technological Studies, PAAET, PO Box 42325, Shuwaikh 70654 (Kuwait); Fox, Alan G. [Materials Research Group, Faculty of Engineering and the Environment, University of Southampton, Southampton SO17 1BJ (United Kingdom); Mechanical Engineering Department, Asian University, 89 Moo 12, Highway 331, Banglamung, Chon Buri 20260 (Thailand); Langdon, Terence G., E-mail: langdon@usc.edu [Materials Research Group, Faculty of Engineering and the Environment, University of Southampton, Southampton SO17 1BJ (United Kingdom); Departments of Aerospace and Mechanical Engineering and Materials Science, University of Southern California, Los Angeles, CA 90089-1453 (United States)

    2011-11-15

    Aluminum of commercial purity was processed by equal-channel angular pressing (ECAP) through two, four and eight passes at room temperature. A series of [1 1 4] convergent-beam electron diffraction (CBED) zone axis patterns were obtained using an electron probe with a diameter of 20 nm. Observations were recorded both immediately adjacent to the grain boundaries and in the grain interiors. Symmetry breaking of the higher-order Laue zone (HOLZ) lines was observed adjacent to the boundaries after two and four passes but not in the grain interiors. Pattern simulation of the CBED patterns taken from the two- and four-pass samples adjacent to the boundaries revealed a homogeneous strain with compressive and shear components. The presence of these homogeneous strains demonstrates that the internal stresses associated with the deformation of aluminum at room temperature are localized in the close vicinity, to within {approx}20 nm, of the grain boundaries.

  6. Consideration of Wall Reflection and Diffraction in the Room Acoustic Prediction Using the Phased Beam Tracing Method

    DEFF Research Database (Denmark)

    Jeong, Cheol-Ho

    2007-01-01

    of the PBTM gives advantages in the binaural simulation. Particularity in the early part of the impulse response at mid frequency, the binaural simulation result shows an excellent correspondence with the measurement in the application of a conference room. The diffraction phenomenon was incorporated...... and consequently the guidelines were suggested for these parameters. The approximate angle‐dependent/independent reflection coefficients were tested. The angle dependent reflection coefficient can take the angle dependence of the incident wave into account as well as the size effect of the surface. Also, the merit...... of representing the negative real part was discussed. The PBTM result shows a good agreement with the measurement especially in the early part of impulse response and at mid frequency. The new method of ii binaural simulation for the PBTM was suggested. The peculiar feature of frequency domain calculation...

  7. Synchrotron X-ray studies of the keel of the short-spined sea urchin Lytechinus variegatus: absorption microtomography (microCT) and small beam diffraction mapping.

    Science.gov (United States)

    Stock, S R; Barss, J; Dahl, T; Veis, A; Almer, J D; Carlo, F

    2003-05-01

    In sea urchin teeth, the keel plays an important structural role, and this paper reports results of microstructural characterization of the keel of Lytechinus variegatus using two noninvasive synchrotron x-ray techniques: x-ray absorption microtomography (microCT) and x-ray diffraction mapping. MicroCT with 14 keV x-rays mapped the spatial distribution of mineral at the 1.3 microm level in a millimeter-sized fragment of a mature portion of the keel. Two rows of low absorption channels (i.e., primary channels) slightly less than 10 microm in diameter were found running linearly from the flange to the base of the keel and parallel to its sides. The primary channels paralleled the oral edge of the keel, and the microCT slices revealed a planar secondary channel leading from each primary channel to the side of the keel. The primary and secondary channels were more or less coplanar and may correspond to the soft tissue between plates of the carinar process. Transmission x-ray diffraction with 80.8 keV x-rays and a 0.1 mm beam mapped the distribution of calcite crystal orientations and the composition Ca(1-x)Mg(x)CO(3) of the calcite. Unlike the variable Mg concentration and highly curved prisms found in the keel of Paracentrotus lividus, a constant Mg content (x = 0.13) and relatively little prism curvature was found in the keel of Lytechinus variegatus.

  8. Supersonic Fe beam source for chromatic aberration-free laser focusing of atoms

    CERN Document Server

    Bosch, R C M; Van der Straten, P; Leeuwen, K A H

    2002-01-01

    A monochromatic Fe beam is generated by heated supersonic expansion of argon seeded with Fe vapor. At a nozzle temperature of 1930 K and 800 torr argon inlet pressure the Fe beam has an axial velocity spread of 8% and intensity of 3 x 10 sup 1 sup 5 s sup - sup 1 sr sup - sup 1 , corresponding to a deposition rate of 10 nm/h at 150 mm from the nozzle. The two-chamber alumina crucibles are chemically stable for liquid Fe. With 400 mm sup 3 Fe we have operated for more than 200 hours without reloading. The power consumption at 1930 K is 750 W. Temperature stability at constant power (without feedback) is better than 30 K. The source is intended for deposition of nano-structures by laser focusing of the Fe beam. The small axial velocity spread virtually eliminates the increase in focal spot size due to chromatic aberration. (authors)

  9. Diffraction Anomalous Near-Edge Structure

    Science.gov (United States)

    Moltaji, Habib O., Jr.

    1995-11-01

    To determine the atomic structure about atom of an element in a sample of a condensed multicomponent single crystal, contrast radiation is proposed with the use of Diffraction Anomalous Near-Edge Structure (DANES), which combines the long-range order sensitivity of the x-ray diffraction and short-range order of the x-ray absorption near-edge techniques. This is achieved by modulating the photon energy of the x-ray beam incident on the sample over a range of energies near an absorption edge of the selected element. Due to anomalous dispersion, x-ray diffraction, and x-ray absorption, the DANES intensity with respect to the selected element is obtained in a single experiment. I demonstrate that synchrotron DANES measurements for the single crystal of thin film and the powder samples and provide the same local atomic structural information as the x-ray absorption near-edge with diffraction condition and can be used to provide enhanced site selectivity. I demonstrate calculations of DAFS intensity and measurements of polarized DANES and XANES intensity.

  10. Effects of co-implanted oxygen or aluminum atoms on hydrogen migration and damage structure in multiple-beam irradiated Al sub 2 O sub 3

    CERN Document Server

    Katano, Y; Yamamoto, S; Nakazawa, T; Yamaki, D; Noda, K

    2000-01-01

    Depth profiles of implanted H atoms were measured for single crystalline Al sub 2 O sub 3 samples irradiated at 923 K with dual or triple beams of 0.25 MeV H-, 0.6 MeV He-, 2.4 MeV O-ions or 2.6 MeV Al-ions. The peaks occur at 1.55 and 1.45 mu m in the depth profiles measured for the H + Al dual beam irradiation and H + O dual beam case, respectively. The ratio of the peak areas is over 4, which is much larger than the implanted H atom ratio of 1.1, indicating that implanted Al atoms suppress the mobility of H atoms. However, the ratio becomes almost 1 between the triple beam samples with H + He + O-ions and with H + He + Al-ions at comparable doses. The fact demonstrates that implanted He atoms overwhelm the effects of the implanted self-cation/anion excess atoms on the migration behaviors of implanted hydrogen and radiation produced point defects, with the resulting sluggish cavity growth observed.

  11. Fabrication of NIL templates and diffractive optical elements using the new Vistec SB4050 VSB e-beam writer

    Science.gov (United States)

    Butschke, Joerg; Irmscher, Mathias; Koepernik, Corinna; Martens, Stephan; Sailer, Holger; Schnabel, Bernd

    2015-03-01

    Targeting mass production of nanostructures, nanoimprint lithography (NIL) is one of the most cost-effective ways to do so. One of the most critical topics is the pattern quality of the imprint master template. Therefore the new Vistec SB4050 VSB e-beam writer has been evaluated regarding its capability for state-of-the-art NIL template and DOE making. Equipped with a new air bearing stage the tool can expose a wide variety of substrates including large and heavy ones. For 9035 substrates a placement accuracy of 9nm (3sigma) as well as an overlay accuracy of 7nm (3sigma) with a mean error below 2nm has been achieved. Targeting for minimum feature size, a resolution below 30nm has been achieved for both, dense lines and holes pattern even using CAR. In addition, 3D structuring capability has been proved by applying GenISys' Layout Beamer calibrated for an appropriate negative tone resist. Further investigation has been done on shot count optimization regarding circular holes respective pillars. Using a feature size dependent segmentation, writing time reduction could be achieved keeping the original feature shape. Besides screening of typical tool parameter an application driven evaluation has been done by fabricating different type of templates based on silicon and quartz. 2D and 3D features have been realized. Furthermore holograms have been fabricated and proved for their performance by optical measurements.

  12. Development of a compact thermal lithium atom beam source for measurements of electron velocity distribution function anisotropy in electron cyclotron resonance plasmas.

    Science.gov (United States)

    Nishioka, T; Shikama, T; Nagamizo, S; Fujii, K; Zushi, H; Uchida, M; Iwamae, A; Tanaka, H; Maekawa, T; Hasuo, M

    2013-07-01

    The anisotropy of the electron velocity distribution function (EVDF) in plasmas can be deduced from the polarization of emissions induced by anisotropic electron-impact excitation. In this paper, we develop a compact thermal lithium atom beam source for spatially resolved measurements of the EVDF anisotropy in electron cyclotron resonance (ECR) plasmas. The beam system is designed such that the ejected beam has a slab shape, and the beam direction is variable. The divergence and flux of the beam are evaluated by experiments and calculations. The developed beam system is installed in an ECR plasma device with a cusp magnetic field, and the LiI 2s-2p emission (670.8 nm) is observed in low-pressure helium plasma. The two-dimensional distributions of the degree and direction of the polarization in the LiI emission are measured by a polarization imaging system. The evaluated polarization distribution suggests the spatial variation of the EVDF anisotropy.

  13. The atomic structure and chemical composition of HfOx (x < 2) films prepared by ion-beam sputtering deposition

    Science.gov (United States)

    Aliev, V. S.; Gerasimova, A. K.; Kruchinin, V. N.; Gritsenko, V. A.; Prosvirin, I. P.; Badmaeva, I. A.

    2016-08-01

    Non-stoichiometric HfOx films of different chemical composition (x partial pressure in a chamber. An effect of chemical composition on the atomic structure of the films was studied by reflection high-energy electron diffraction, x-ray photoelectron spectroscopy and field emission scanning electron microscopy methods. The films were found to be amorphous, consisting only of three components: Hf-metal clusters, Hf4O7 suboxide and stoichiometric HfO2. The relative concentration of these components varies with changing x. The surface of the films contains the increased oxygen content compared to the bulk. It was found that the Hf4O7 suboxide concentration is maximal at x = 1.8. The concept of hafnium oxide film growth by the IBSD method is proposed to explain the lack of suboxides variety in the films and the instability of HfO2, when annealed at high temperature.

  14. Cylindrical Vector Beams for Rapid Polarization-Dependent Measurements in Atomic Systems

    Science.gov (United States)

    2011-12-05

    optical trapping [11], atom guiding [12], laser machining [13], charged particle acceleration [14,15], and polarimetry [16]. Yet despite numerous...been implemented and demonstrated experimentally. They have been used for probing molecules [3], trapping microspheres [11], generating surface...however, magneto - optic polarization effects could also become important. The azimuthal profiles shown in Fig. 4(a) are sinusoidal, indicating that the

  15. Propagation of Gaussian Schell-model beam in electromagnetically induced transparency atomic vapor%高斯谢尔模型光束在EIT原子气体中的传输特性研究

    Institute of Scientific and Technical Information of China (English)

    许森东; 徐弼军; 陆璇辉

    2013-01-01

    为了研究高斯-谢尔模型(GSM)光束在电磁感应透明(EIT)材料中的传输特性,利用矩阵光学理论、衍射积分理论、相干偏振统一理论推导了GSM光束通过EIT材料的传输交叉谱密度方程的解析表达式。该表达式可以用于计算和研究GSM光束通过EIT原子气体的谱密度和相干度的变化。分析显示GSM光束的谱密度和相干度都可以通过控制光的拉比频率调控。此研究结果提供了一种新的调控光传输的方法和技术,同时该发现也为控制部分相干光的谱密度和相干度提供了一种新方法。%In order to study the propagation characteristics of Gaussian Schell-model (GSM) beams in electromagnetically induced transparency atomic vapor, the analytical expression was obtained for the cross-spectral density function of a Gaussian Schell-model beam passing through the electromagnetically induced transparency atomic vapor based on the matrix optics theory, diffraction integral theory and unified theory of coherence and polarization. The formula can be used in the study of the changes in the spectral density and spectral degree of coherence of the beam through the EIT atomic vapor. Numerical examples show that both the spectral density and the spectral degree of coherence of the GSM beam can be modulated by the Rabi frequency of the control light. The results have been provided a new method and technique for modulation the beam propagation. The findings indicate a new technique for controlling the spectral density and the spectral degree of coherence of the partially coherent light beam.

  16. DIFFRACTION FROM MODEL CRYSTALS

    Science.gov (United States)

    Although calculating X-ray diffraction patterns from atomic coordinates of a crystal structure is a widely available capability, calculation from non-periodic arrays of atoms has not been widely applied to cellulose. Non-periodic arrays result from modeling studies that, even though started with at...

  17. From atomic structure to excess entropy: a neutron diffraction and density functional theory study of CaO-Al2O3-SiO2 melts

    Science.gov (United States)

    Liu, Maoyuan; Jacob, Aurélie; Schmetterer, Clemens; Masset, Patrick J.; Hennet, Louis; Fischer, Henry E.; Kozaily, Jad; Jahn, Sandro; Gray-Weale, Angus

    2016-04-01

    Calcium aluminosilicate \\text{CaO}-\\text{A}{{\\text{l}}2}{{\\text{O}}3}-\\text{Si}{{\\text{O}}2} (CAS) melts with compositions {{≤ft(\\text{CaO}-\\text{Si}{{\\text{O}}2}\\right)}x}{{≤ft(\\text{A}{{\\text{l}}2}{{\\text{O}}3}\\right)}1-x} for x  text{A}{{\\text{l}}2}{{\\text{O}}3}\\right)}x}{{≤ft(\\text{Si}{{\\text{O}}2}\\right)}1-x} for x≥slant 0.5 are studied using neutron diffraction with aerodynamic levitation and density functional theory molecular dynamics modelling. Simulated structure factors are found to be in good agreement with experimental structure factors. Local atomic structures from simulations reveal the role of calcium cations as a network modifier, and aluminium cations as a non-tetrahedral network former. Distributions of tetrahedral order show that an increasing concentration of the network former Al increases entropy, while an increasing concentration of the network modifier Ca decreases entropy. This trend is opposite to the conventional understanding that increasing amounts of network former should increase order in the network liquid, and so decrease entropy. The two-body correlation entropy S 2 is found to not correlate with the excess entropy values obtained from thermochemical databases, while entropies including higher-order correlations such as tetrahedral order, O-M-O or M-O-M bond angles and Q N environments show a clear linear correlation between computed entropy and database excess entropy. The possible relationship between atomic structures and excess entropy is discussed.

  18. Nondestructive atomic compositional analysis of BeMgZnO quaternary alloys using ion beam analytical techniques

    Energy Technology Data Exchange (ETDEWEB)

    Zolnai, Z., E-mail: zolnai.zsolt@ttk.mta.hu [Research Centre for Natural Sciences, Institute of Technical Physics and Materials Science (MFA), Konkoly-Thege M. út 29-33, H-1121 Budapest (Hungary); Toporkov, M. [Department of Electrical and Computer Engineering, Virginia Commonwealth University, 601W Main St, Richmond, VA 23284 (United States); Volk, J. [Research Centre for Natural Sciences, Institute of Technical Physics and Materials Science (MFA), Konkoly-Thege M. út 29-33, H-1121 Budapest (Hungary); Department of Electrical and Computer Engineering, Virginia Commonwealth University, 601W Main St, Richmond, VA 23284 (United States); Demchenko, D.O. [Department of Physics, Virginia Commonwealth University, 701W. Grace St., Richmond, VA 23284 (United States); Okur, S. [Department of Electrical and Computer Engineering, Virginia Commonwealth University, 601W Main St, Richmond, VA 23284 (United States); Szabó, Z. [Research Centre for Natural Sciences, Institute of Technical Physics and Materials Science (MFA), Konkoly-Thege M. út 29-33, H-1121 Budapest (Hungary); Özgür, Ü.; Morkoç, H.; Avrutin, V. [Department of Electrical and Computer Engineering, Virginia Commonwealth University, 601W Main St, Richmond, VA 23284 (United States); Kótai, E. [Wigner Research Centre for Physics, Institute for Particle and Nuclear Physics, Konkoly-Thege M. út 29-33, H-1121 Budapest (Hungary)

    2015-02-01

    Highlights: • BeMgZnO thin layers were grown with plasma-assisted molecular beam epitaxy (MBE). • The Be contents were accurately measured with RBS and proton elastic backscattering. • The Tauc bandgap was measured from optical transmittance experiments. • The bandgap has been varied between 3.26 eV and 4.62 eV via the Be and Mg content. • Experimental and density functional theory calculated bandgaps were in good agreement. - Abstract: The atomic composition with less than 1–2 atom% uncertainty was measured in ternary BeZnO and quaternary BeMgZnO alloys using a combination of nondestructive Rutherford backscattering spectrometry with 1 MeV He{sup +} analyzing ion beam and non-Rutherford elastic backscattering experiments with 2.53 MeV energy protons. An enhancement factor of 60 in the cross-section of Be for protons has been achieved to monitor Be atomic concentrations. Usually the quantitative analysis of BeZnO and BeMgZnO systems is challenging due to difficulties with appropriate experimental tools for the detection of the light Be element with satisfactory accuracy. As it is shown, our applied ion beam technique, supported with the detailed simulation of ion stopping, backscattering, and detection processes allows of quantitative depth profiling and compositional analysis of wurtzite BeZnO/ZnO/sapphire and BeMgZnO/ZnO/sapphire layer structures with low uncertainty for both Be and Mg. In addition, the excitonic bandgaps of the layers were deduced from optical transmittance measurements. To augment the measured compositions and bandgaps of BeO and MgO co-alloyed ZnO layers, hybrid density functional bandgap calculations were performed with varying the Be and Mg contents. The theoretical vs. experimental bandgaps show linear correlation in the entire bandgap range studied from 3.26 eV to 4.62 eV. The analytical method employed should help facilitate bandgap engineering for potential applications, such as solar blind UV photodetectors and

  19. Copper Vapor Laser with One-Beam Radiation of Diffraction Quality and Its Capabilities for Microprocessing of Materials for Electronic Engineering Products

    Directory of Open Access Journals (Sweden)

    N. A. Lyabin

    2014-01-01

    Full Text Available The structure, spatial, time and energy characteristics of copper vapor laser radiation (CVL with optical resonators possessing high spatial selectivity have been investigated: with an unstable resonator (UR with two convex mirrors and telescopic UR, and the conditions to form one-beam radiation with diffraction divergence and high stability of directivity pattern axis have been defined.The most weighty and prospective application of CVL with UR with two convex mirrors is to use it as a driving oscillator (DO in a copper vapor laser system (CVLS of the type: driving oscillator – power amplifier (DO – PA when diffraction beam radiating power and power density in a focused spot of 10-20 µm in diameter increases by 1-2 orders. Using industrial sealed-off active elements (AE of “Kulon” series with an average radiation power of 15-25 W as PAs the peak power density increases up to 1011 W/cm 2 while an application of AE “Crystal” with 30- 50 W power gives up to 1012 W/cm 2 , which is sufficient for efficient and qualitative microprocessing of materials up to 1…2 mm thick. Such a CVLS has become the basis for creating up-to-date automated laser technological installations (ALTI of “Karavella-1” and “Karavella-1M” types to manufacture precision parts of electronic engineering products (EEP of metal up to 0.5 mm thick and of non-metal up to 1.5…1.8 mm thick.CVL with a telescopic UR with an average power of 5-6 W diffraction radiation beam has become the basis for creating industrial ALTI “Karavella-2” and “Karavella-2M” to manufacture precision parts of electronic engineering products (EEP of metal up to 0.3 mm thick and of non-metal up to 0.5 – 0.7 mm thick.Practical work on all types of ALTI “Karavella” has shown a set of significant advantages of a laser way of pulsed microprocessing over the traditional ones, including electro-erosion machining: a wide range of structural metal and non-metal materials to be

  20. Generation of One-Dimensional Array of Focused Hollow-Beam Pipes and Its Surface Microscopic Waveguide for Cold Atoms or Molecules

    Institute of Scientific and Technical Information of China (English)

    JI Xian-Ming; XIA Yong; YIN Jian-Ping

    2004-01-01

    We propose a new scheme to guide cold atoms (or molecules) by using a one-dimensional (1D) array of focused hollow-beam pipes generated by the combination of a binary phase grating and a 1D array of micro-cylindrical lenses on the substrate surface. We also calculate the intensity distribution of the focused hollow-beam pipe array and its optical potential for 85Rb atoms. The result shows that when the blue detuning of the incident beam and its intensity are 10 GHz and 7.0 × 103 W/m2 respectively, the horizontal dark spot size of each focused hollow-beam pipe and the efficient optical potential are 4.4μm and ~ 0.23mK, which is high enough to guide cold 85Rb atoms (~ 20 μK) from a standard optical molasses and then to realize the 1D array of surface atomic waveguides on an atom chip.

  1. Photocorrosion of coupled CdS/CdSe photoelectrodes coated with ZnO. Atomic force microscopy and X-ray diffraction studies

    Energy Technology Data Exchange (ETDEWEB)

    Rincon, M.E.; Sanchez, M. [UNAM, Temixco (Mexico). Centro de Investigacion en Energia; Ruiz-Garcia, J. [UASLP, San Luis Potosi (Mexico). Inst. de Fisica

    1998-10-01

    The stability of photoelectrochemical cells based on chemically deposited CdS/CdSe coupled films has been examined. Changes in surface structure and composition of coated and uncoated CdS{sub 250}/CdSe coupled films as well as CdSe films have been examined by atomic force microscopy and X-ray diffraction. The superior stability at short times of the coupled system, compared to CdSe, is related to the increase in the hexagonal character (stronger bonding) and the smaller recombination rate of the photogenerated carriers. At large operation times, the lower stability of the coupled system is related to band opening, which increases the oxidation rates of the passivating Se/S layer. The recrystallization illuminated CdSe photoanodes, and coupled films working in the dark can be explained by the presence of surface states and back reactions. Stable short-circuit currents were obtained with coupled films coated with a thin layer (350 {angstrom}) of ZnO. It is likely that oxidation and redeposition of the protective ZnO film competes for hole consumption. The rough morphology of the coated photoelectrodes correlated to a substantial increase in surface area that resembles ZnO particulate film electrodes sensitized by CdSe and CdS.

  2. Resonant Formation of $d\\mu t$ Molecules in Deuterium An Atomic Beam Measurement of Muon Catalyzed dt Fusion

    CERN Document Server

    Fujiwara, M C; Bailey, J M; Beer, G A; Beveridge, J L; Faifman, M P; Huber, T M; Kammel, P; Kim, S K; Knowles, P E; Kunselman, A R; Maier, M; Markushin, V E; Marshall, G M; Martoff, C J; Mason, G R; Mulhauser, F; Olin, A; Petitjean, C; Porcelli, T A; Wozniak, J; Zmeskal, J

    2000-01-01

    Resonant formation of $d\\mu t$ molecules in collisions of muonic tritium ($\\mu t$) on D$_2$ was investigated using a beam of $\\mu t$ atoms, demonstrating a new direct approach in muon catalyzed fusion studies. Strong epithermal resonances in $d\\mu t$ formation were directly revealed for the first time. From the time-of-flight analysis of $2036\\pm 116$ $dt$ fusion events, a formation rate consistent with $0.73\\pm (0.16)_{meas} \\pm (0.09)_{model}$ times the theoretical prediction was obtained. For the largest peak at a resonance energy of $0.423 \\pm 0.037$ eV, this corresponds to a rate of $(7.1 \\pm 1.8) \\times 10^9$ s$^{-1}$, more than an order of magnitude larger than those at low energies.

  3. Studies of Compound States of Atomic Negative Ions Using Laser Beams

    Science.gov (United States)

    1984-07-01

    funds for Dr. T. J. Kvale , a postdoctoral fellow from Professor J. T. Park’s laboratory at the University of Missouri. Dr. Kvale joined our group January...Beam are Collinear. RESUME NAME: Thomas Jay Kvale TITLE: Postdoctoral Fellow in Physics EDUCATION: A.B. Gustavus Adolphus College (Cum Laude), 1975 M.S...Photography ___ __’ii Thomas Jay Kvale REFEREED PAPERS 1. J. E. Aldag, J. L. Peacher, P. J. Martin, V. C. Sutcliffe, J. George, E. Redd, T. J. Kvale , D

  4. Efficient focusing of 8 keV X-rays with multilayer Fresnel zone plates fabricated by atomic layer deposition and focused ion beam milling.

    Science.gov (United States)

    Mayer, Marcel; Keskinbora, Kahraman; Grévent, Corinne; Szeghalmi, Adriana; Knez, Mato; Weigand, Markus; Snigirev, Anatoly; Snigireva, Irina; Schütz, Gisela

    2013-05-01

    Fresnel zone plates (FZPs) recently showed significant improvement by focusing soft X-rays down to ~10 nm. In contrast to soft X-rays, generally a very high aspect ratio FZP is needed for efficient focusing of hard X-rays. Therefore, FZPs had limited success in the hard X-ray range owing to difficulties of manufacturing high-aspect-ratio zone plates using conventional techniques. Here, employing a method of fabrication based on atomic layer deposition (ALD) and focused ion beam (FIB) milling, FZPs with very high aspect ratios were prepared. Such multilayer FZPs with outermost zone widths of 10 and 35 nm and aspect ratios of up to 243 were tested for their focusing properties at 8 keV and shown to focus hard X-rays efficiently. This success was enabled by the outstanding layer quality thanks to ALD. Via the use of FIB for slicing the multilayer structures, desired aspect ratios could be obtained by precisely controlling the thickness. Experimental diffraction efficiencies of multilayer FZPs fabricated via this combination reached up to 15.58% at 8 keV. In addition, scanning transmission X-ray microscopy experiments at 1.5 keV were carried out using one of the multilayer FZPs and resolved a 60 nm feature size. Finally, the prospective of different material combinations with various outermost zone widths at 8 and 17 keV is discussed in the light of the coupled wave theory and the thin-grating approximation. Al2O3/Ir is outlined as a promising future material candidate for extremely high resolution with a theoretical efficiency of more than 20% for as small an outermost zone width as 10 nm at 17 keV.

  5. Atom laser dynamics in a tight waveguide

    Energy Technology Data Exchange (ETDEWEB)

    Campo, A del; Lizuain, I; Muga, J G [Departamento de Quimica-Fisica, UPV-EHU, Apartado. 644, Bilbao (Spain); Pons, M [Departamento de Fisica Aplicada I, E.U.I.T. de Minas y Obras Publicas, UPV-EHU, 48901 Barakaldo (Spain); Moshinsky, M [Instituto de Fisica, Universidad Nacional Autonoma de Mexico, Apartado Postal 20-364, 01000 Mexico D.F. (Mexico)], E-mail: adolfo.delcampo@ehu.es

    2008-02-15

    We study the transient dynamics that arise during the formation of an atom laser beam in a tight waveguide. The time dependent density profile develops a series of wiggles which are related to the diffraction in time phenomenon. The apodization of matter waves, which relies on the use of smooth aperture functions, allows to suppress such oscillations in a time interval, after which there is a revival of the diffraction in time. The revival time scale is directly related to the inverse of the harmonic trap frequency for the atom reservoir.

  6. Fabrication and characterization of tunnel barriers in a multi-walled carbon nanotube formed by argon atom beam irradiation

    Energy Technology Data Exchange (ETDEWEB)

    Tomizawa, H. [Advanced Device Laboratory, RIKEN, 2-1 Hirosawa, Wako, Saitama 351-0198 (Japan); Department of Applied Physics, Tokyo University of Science, 6-3-1 Niijuku, Katsushika-ku, Tokyo 125-8585 (Japan); Yamaguchi, T., E-mail: tyamag@riken.jp [Advanced Device Laboratory, RIKEN, 2-1 Hirosawa, Wako, Saitama 351-0198 (Japan); Akita, S. [Department of Physics and Electronics, Osaka Prefecture University, 1-1 Gakuen-cho, Nakaku, Sakai, Osaka 599-8531 (Japan); Ishibashi, K. [Advanced Device Laboratory, RIKEN, 2-1 Hirosawa, Wako, Saitama 351-0198 (Japan); Department of Applied Physics, Tokyo University of Science, 6-3-1 Niijuku, Katsushika-ku, Tokyo 125-8585 (Japan); RIKEN Center for Emergent Matter Science (CEMS), 2-1 Hirosawa, Wako, Saitama 351-0198 (Japan)

    2015-07-28

    We have evaluated tunnel barriers formed in multi-walled carbon nanotubes (MWNTs) by an Ar atom beam irradiation method and applied the technique to fabricate coupled double quantum dots. The two-terminal resistance of the individual MWNTs was increased owing to local damage caused by the Ar beam irradiation. The temperature dependence of the current through a single barrier suggested two different contributions to its Arrhenius plot, i.e., formed by direct tunneling through the barrier and by thermal activation over the barrier. The height of the formed barriers was estimated. The fabrication technique was used to produce coupled double quantum dots with serially formed triple barriers on a MWNT. The current measured at 1.5 K as a function of two side-gate voltages resulted in a honeycomb-like charge stability diagram, which confirmed the formation of the double dots. The characteristic parameters of the double quantum dots were calculated, and the feasibility of the technique is discussed.

  7. High-speed, two-dimensional synchrotron white-beam x-ray radiography of spray breakup and atomization.

    Science.gov (United States)

    Halls, Benjamin R; Radke, Christopher D; Reuter, Benjamin J; Kastengren, Alan L; Gord, James R; Meyer, Terrence R

    2017-01-23

    High-speed, two-dimensional synchrotron x-ray radiography and phase-contrast imaging are demonstrated in propulsion sprays. Measurements are performed at the 7-BM beamline at the Advanced Photon Source user facility at Argonne National Laboratory using a recently developed broadband x-ray white beam. This novel enhancement allows for high speed, high fidelity x-ray imaging for the community at large. Quantitative path-integrated liquid distributions and spatio-temporal dynamics of the sprays were imaged with a LuAG:Ce scintillator optically coupled to a high-speed CMOS camera. Images are collected with a microscope objective at frame rates of 20 kHz and with a macro lens at 120 kHz, achieving spatial resolutions of 12 μm and 65 μm, respectively. Imaging with and without potassium iodide (KI) as a contrast-enhancing agent is compared, and the effects of broadband attenuation and spatial beam characteristics are determined through modeling and experimental calibration. In addition, phase contrast is used to differentiate liquid streams with varying concentrations of KI. The experimental approach is applied to different spray conditions, including quantitative measurements of mass distribution during primary atomization and qualitative visualization of turbulent binary fluid mixing.

  8. The measurement of stress and phase fraction distributions in pre and post-transition Zircaloy oxides using nano-beam synchrotron X-ray diffraction

    Science.gov (United States)

    Swan, H.; Blackmur, M. S.; Hyde, J. M.; Laferrere, A.; Ortner, S. R.; Styman, P. D.; Staines, C.; Gass, M.; Hulme, H.; Cole-Baker, A.; Frankel, P.

    2016-10-01

    Zircaloy-4 oxide stress profiles and tetragonal:monoclinic oxide phase fraction distributions were studied using nano-beam transmission X-ray diffraction. Continuous stress relief and phase transformation during the first cycle of oxide growth was observed. The in-plane monoclinic stress was shown to relax strongly up to each transition, whereas in-plane tetragonal stress-relief (near the metal-oxide interface) was only observed post transition. The research demonstrates that plasticity in the metal and the development of a band of in-plane cracking both relax the monoclinic in-plane stress. The observations are consistent with a model of transition in which in-plane cracking becomes interlinked prior to transition. These cracks, combined with the development of cracks with a through-thickness component (driven primarily by plasticity in the metal) and/or a porous network of fine cracks (associated with phase transformation), form a percolation path through the oxide layer. The oxidising species can then percolate from the oxide surface to the metal/oxide interface, at which stage transition then ensues.

  9. Direct observation of strain in InAs quantum dots and cap layer during molecular beam epitaxial growth using in situ X-ray diffraction

    Energy Technology Data Exchange (ETDEWEB)

    Shimomura, Kenichi; Ohshita, Yoshio; Kamiya, Itaru, E-mail: kamiya@toyota-ti.ac.jp [Toyota Technological Institute, 2-12-1 Hisakata, Tempaku, Nagoya 468-8511 (Japan); Suzuki, Hidetoshi [Faculty of Engineering, University of Miyazaki, 1-1 Gakuen Kibanadai-nishi, Miyazaki 889-2192 (Japan); Sasaki, Takuo; Takahasi, Masamitu [Quantum Beam Science Center, Japan Atomic Energy Agency, Koto 1-1-1, Sayo-cho, Hyogo 679-5148 (Japan)

    2015-11-14

    Direct measurements on the growth of InAs quantum dots (QDs) and various cap layers during molecular beam epitaxy are performed by in situ X-ray diffraction (XRD). The evolution of strain induced both in the QDs and cap layers during capping is discussed based on the XRD intensity transients obtained at various lattice constants. Transients with different features are observed from those obtained during InGaAs and GaAs capping. The difference observed is attributed to In-Ga intermixing between the QDs and the cap layer under limited supply of In. Photoluminescence (PL) wavelength can be tuned by controlling the intermixing, which affects both the strain induced in the QDs and the barrier heights. The PL wavelength also varies with the cap layer thickness. A large redshift occurs by reducing the cap thickness. The in situ XRD observation reveals that this is a result of reduced strain. We demonstrate how such information about strain can be applied for designing and preparing novel device structures.

  10. Improved laser damage threshold performance of calcium fluoride optical surfaces via Accelerated Neutral Atom Beam (ANAB) processing

    Science.gov (United States)

    Kirkpatrick, S.; Walsh, M.; Svrluga, R.; Thomas, M.

    2015-11-01

    Optics are not keeping up with the pace of laser advancements. The laser industry is rapidly increasing its power capabilities and reducing wavelengths which have exposed the optics as a weak link in lifetime failures for these advanced systems. Nanometer sized surface defects (scratches, pits, bumps and residual particles) on the surface of optics are a significant limiting factor to high end performance. Angstrom level smoothing of materials such as calcium fluoride, spinel, magnesium fluoride, zinc sulfide, LBO and others presents a unique challenge for traditional polishing techniques. Exogenesis Corporation, using its new and proprietary Accelerated Neutral Atom Beam (ANAB) technology, is able to remove nano-scale surface damage and particle contamination leaving many material surfaces with roughness typically around one Angstrom. This surface defect mitigation via ANAB processing can be shown to increase performance properties of high intensity optical materials. This paper describes the ANAB technology and summarizes smoothing results for calcium fluoride laser windows. It further correlates laser damage threshold improvements with the smoothing produced by ANAB surface treatment. All ANAB processing was performed at Exogenesis Corporation using an nAccel100TM Accelerated Particle Beam processing tool. All surface measurement data for the paper was produced via AFM analysis on a Park Model XE70 AFM, and all laser damage testing was performed at Spica Technologies, Inc. Exogenesis Corporation's ANAB processing technology is a new and unique surface modification technique that has demonstrated to be highly effective at correcting nano-scale surface defects. ANAB is a non-contact vacuum process comprised of an intense beam of accelerated, electrically neutral gas atoms with average energies of a few tens of electron volts. The ANAB process does not apply mechanical forces associated with traditional polishing techniques. ANAB efficiently removes surface

  11. A short pulse (7 μs FWHM) and high repetition rate (dc-5kHz) cantilever piezovalve for pulsed atomic and molecular beams

    NARCIS (Netherlands)

    Irimia, D.; Dobrikov, D.; Kortekaas, R.; Voet, H.; Ende, D.A. van den; Groen, W.A.; Janssen, M.H.M.

    2009-01-01

    In this paper we report on the design and operation of a novel piezovalve for the production of short pulsed atomic or molecular beams. The high speed valve operates on the principle of a cantilever piezo. The only moving part, besides the cantilever piezo itself, is a very small O-ring that forms t

  12. The NanoBeamBalance: A passive, tensile-test device for the atomic force microscope

    Science.gov (United States)

    Wenger, M. P. E.; Mesquida, P.

    2011-05-01

    An add-on device is presented, which significantly expands the force measurement capabilities of the atomic force microscope (AFM). The device consists of a completely passive mechanism, which translates the vertical motion of the AFM tip in force measurements into a horizontal motion of two sample support pads. The advantage is that it is much easier to deposit microscopic samples from suspension onto flat surfaces than to attach them reliably between tip and a surface. The working-principle and the design of the device is comprehensively described and demonstrated on the example of collagen fibres with a diameter of a few μm. Well-defined tensile measurements in longitudinal direction were performed, showing that the tensile stiffness of collagen fibres from rat tail tendon decreases by a factor of 5 when rehydrated from a dried sample and slowly increases upon cross-linking with glutaraldehyde.

  13. Helium, neon and argon diffraction from Ru(0001).

    Science.gov (United States)

    Minniti, M; Díaz, C; Fernández Cuñado, J L; Politano, A; Maccariello, D; Martín, F; Farías, D; Miranda, R

    2012-09-05

    We present an experimental and theoretical study of He, Ne and Ar diffraction from the Ru(0001) surface. Close-coupling calculations were performed to estimate the corrugation function and the potential well depth in the atom-surface interaction in all three cases. DFT (density functional theory) calculations, including van der Waals dispersion forces, were used to validate the close-coupling results and to further analyze the experimental results. Our DFT calculations indicate that, in the incident energy range 20-150 meV, anticorrugating effects are present in the case of He and Ar diffraction, whereas normal corrugation is observed with Ne beams.

  14. Evanescent Wave Atomic Mirror

    Science.gov (United States)

    Ghezali, S.; Taleb, A.

    2008-09-01

    A research project at the "Laboratoire d'électronique quantique" consists in a theoretical study of the reflection and diffraction phenomena via an atomic mirror. This poster presents the principle of an atomic mirror. Many groups in the world have constructed this type of atom optics experiments such as in Paris-Orsay-Villetaneuse (France), Stanford-Gaithersburg (USA), Munich-Heidelberg (Germany), etc. A laser beam goes into a prism with an incidence bigger than the critical incidence. It undergoes a total reflection on the plane face of the prism and then exits. The transmitted resulting wave out of the prism is evanescent and repulsive as the frequency detuning of the laser beam compared to the atomic transition δ = ωL-ω0 is positive. The cold atomic sample interacts with this evanescent wave and undergoes one or more elastic bounces by passing into backward points in its trajectory because the atoms' kinetic energy (of the order of the μeV) is less than the maximum of the dipolar potential barrier ℏΩ2/Δ where Ω is the Rabi frequency [1]. In fact, the atoms are cooled and captured in a magneto-optical trap placed at a distance of the order of the cm above the prism surface. The dipolar potential with which interact the slow atoms is obtained for a two level atom in a case of a dipolar electric transition (D2 Rubidium transition at a wavelength of 780nm delivered by a Titane-Saphir laser between a fundamental state Jf = l/2 and an excited state Je = 3/2). This potential is corrected by an attractive Van der Waals term which varies as 1/z3 in the Lennard-Jones approximation (typical atomic distance of the order of λ0/2π where λ0 is the laser wavelength) and in 1/z4 if the distance between the atom and its image in the dielectric is big in front of λ0/2π. This last case is obtained in a quantum electrodynamic calculation by taking into account an orthornormal base [2]. We'll examine the role of spontaneous emission for which the rate is inversely

  15. Ab-initio primitive cell parameters from single convergent-beam electron diffraction patterns: a converse route to the identification of microcrystals with electrons.

    Science.gov (United States)

    Le Page, Y

    1992-04-01

    A new method for the ab initio derivation of Buerger-reduced primitive cell parameters from coordinate measurements of spots on single convergent-beam electron diffraction (CBED) patterns is described, which does not involve trial-and-error. The pattern can be taken along any zone axis, and misorientations of the crystallite by as much as a few degrees are taken into account without loss of accuracy. This derivation of cell parameters by least-squares analysis of the measurements has been automated in a program called NRCBED. Present accuracy is about 1% on lengths and 2 degrees on angles, but could be significantly improved by modelling projector lens aberrations, or by using a microscope without a projector lens. With present technology, it is possible to obtain a CBED pattern and a semi-quantitative energy-dispersive X-ray (EDX) analysis simultaneously from a single microcrystal a few hundred Angströms across. It becomes therefore possible to identify the material of the crystal on a single CBED pattern: a cell parameter database for known compounds is searched with the primitive cell parameters obtained in the above way, and with a mask describing the EDX results qualitatively. Feasibility is demonstrated on a crystallite of CeO2 500 Angströms across. With this new approach, trial-and-error should disappear from the solution of other long-standing problems: interpretation of X-ray powder patterns for new compounds in the presence of impurity lines, or in the case of multiple phases should become straight-forward.

  16. Plasmonic properties of Ag nanoparticles embedded in GeO2-SiO2 matrix by atom beam sputtering.

    Science.gov (United States)

    Mohapatra, Satyabrata

    2016-02-01

    Nanocomposite thin films containing Ag nanoparticles embedded in the GeO2-SiO2 matrix were synthesized by the atom beam co-sputtering technique. The structural, optical and plasmonic properties and the chemical composition of the nanocomposite thin films were studied by transmission electron microscopy (TEM) with energy dispersive X-ray spectroscopy (EDX), UV-visible absorption spectroscopy and X-ray photoelectron spectroscopy (XPS). UV-visible absorption studies on Ag-SiO2 nanocomposites revealed the presence of a strong localized surface plasmon resonance (LSPR) peak characteristic of Ag nanoparticles at 413 nm, which showed a blue shift of 26 nm (413 to 387 nm) along with a significant broadening and drastic decrease in intensity with the incorporation of 16 at% of Ge into the SiO2 matrix. TEM studies on Ag-GeO2-SiO2 nanocomposite thin films confirmed the presence of Ag nanoparticles with an average size of 3.8 nm in addition to their aggregates with an average size of 16.2 nm. Thermal annealing in air resulted in strong enhancement in the intensity of the LSPR peak, which showed a regular red shift of 51 nm (from 387 to 438 nm) with the increase in annealing temperature up to 500 °C. XPS studies showed that annealing in air resulted in oxidation of excess Ge atoms in the nanocomposite into GeO2. Our work demonstrates the possibility of controllably tuning the LSPR of Ag nanoparticles embedded in the GeO2-SiO2 matrix by single-step thermal annealing, which is interesting for optical applications.

  17. Neutron diffraction of cell membranes (myelin).

    Science.gov (United States)

    Parsons, D F; Akers, C K

    1969-09-05

    Small-angle neutron diffraction (wavelength 4.05 angstroms) of human and rabbit sciatic nerve has been carried out by means of the Brookhaven high flux beam reactor with an automated slit camera. Most of the free water of the nerves was substituted in order to minimize incoherent scatter of hydrogen atoms. The differences in amplitude and phase shifts between neutrons and x-rays resulted in a neutron diffraction pattern that was completely different from the x-ray pattern. The neutron pattern consisted of a single peak of about 89-angstrom spacing in the region examined (up to 6-angstrom spacing). The strong third, fourth, and fifth order reflections (about 60, 45, and 36 angstroms) seen in the x-ray pattern were suppressed. The neutron data indicated a strong scattering from one portion of the membrane.

  18. Approaching Defect-free Amorphous Silicon Nitride by Plasma-assisted Atomic Beam Deposition for High Performance Gate Dielectric

    Science.gov (United States)

    Tsai, Shu-Ju; Wang, Chiang-Lun; Lee, Hung-Chun; Lin, Chun-Yeh; Chen, Jhih-Wei; Shiu, Hong-Wei; Chang, Lo-Yueh; Hsueh, Han-Ting; Chen, Hung-Ying; Tsai, Jyun-Yu; Lu, Ying-Hsin; Chang, Ting-Chang; Tu, Li-Wei; Teng, Hsisheng; Chen, Yi-Chun; Chen, Chia-Hao; Wu, Chung-Lin

    2016-06-01

    In the past few decades, gate insulators with a high dielectric constant (high-k dielectric) enabling a physically thick but dielectrically thin insulating layer, have been used to replace traditional SiOx insulator and to ensure continuous downscaling of Si-based transistor technology. However, due to the non-silicon derivative natures of the high-k metal oxides, transport properties in these dielectrics are still limited by various structural defects on the hetero-interfaces and inside the dielectrics. Here, we show that another insulating silicon compound, amorphous silicon nitride (a-Si3N4), is a promising candidate of effective electrical insulator for use as a high-k dielectric. We have examined a-Si3N4 deposited using the plasma-assisted atomic beam deposition (PA-ABD) technique in an ultra-high vacuum (UHV) environment and demonstrated the absence of defect-related luminescence; it was also found that the electronic structure across the a-Si3N4/Si heterojunction approaches the intrinsic limit, which exhibits large band gap energy and valence band offset. We demonstrate that charge transport properties in the metal/a-Si3N4/Si (MNS) structures approach defect-free limits with a large breakdown field and a low leakage current. Using PA-ABD, our results suggest a general strategy to markedly improve the performance of gate dielectric using a nearly defect-free insulator.

  19. Spin-to-Orbital Angular Momentum Conversion and Spin-Polarization Filtering in Electron Beams

    CERN Document Server

    Karimi, Ebrahim; Grillo, Vincenzo; Santamato, Enrico; 10.1103/PhysRevLett.108.044801

    2012-01-01

    We propose the design of a space-variant Wien filter for electron beams that induces a spin half-turn and converts the corresponding spin angular momentum variation into orbital angular momentum of the beam itself by exploiting a geometrical phase arising in the spin manipulation. When applied to a spatially coherent input spin-polarized electron beam, such a device can generate an electron vortex beam, carrying orbital angular momentum. When applied to an unpolarized input beam, the proposed device, in combination with a suitable diffraction element, can act as a very effective spin-polarization filter. The same approach can also be applied to neutron or atom beams.

  20. Measurements of radiation near an atomic spectral line from the interaction of a 30 GeV electron beam and a long plasma

    Energy Technology Data Exchange (ETDEWEB)

    Catravas, P.; Chattopadhyay, S.; Esarey, E.; Leemans, W. P.; Assmann, R.; Decker, F.-J.; Hogan, M. J.; Iverson, R.; Siemann, R. H.; Walz, D. (and others)

    2001-10-01

    Emissions produced or initiated by a 30-GeV electron beam propagating through a {approx}1-m long heat pipe oven containing neutral and partially ionized vapor have been measured near atomic spectral lines in a beam-plasma wakefield experiment. The Cerenkov spatial profile has been studied as a function of oven temperature and pressure, observation wavelength, and ionizing laser intensity and delay. The Cerenkov peak angle is affected by the creation of plasma, and estimates of neutral and plasma density have been extracted. Increases in visible background radiation, consistent with increased plasma recombination emissions due to dissipation of wakefields, were simultaneously measured.

  1. Measurements of Radiation Near An Atomic Spectral Line From the Interaction of a 30-GeV Electron Beam And a Long Plasma

    Energy Technology Data Exchange (ETDEWEB)

    Catravas, P.; Chattopadhyay, S.; Esarey, E.; Leemans, W.P.; /LBL, Berkeley; Assmann, R.; Decker, F.J.; Hogan, M.J.; Iverson, R.; Siemann, R.H.; Walz, D.; Whittum, D.; /SLAC; Blue, B.; Clayton, C.; Joshi, C.; Marsh, K.A.; Mori, W.B.; Wang, S.; /UCLA; Katsouleas, T.; Lee, S.; Muggli, P.; /Southern California U.

    2005-09-12

    Emissions produced or initiated by a 30 GeV electron beam propagating through a {approx}1 m long heat pipe oven containing neutral and partially ionized vapor have been measured near atomic spectral lines in a beam-plasma wakefield experiment. The Cerenkov spatial profile has been studied as a function of oven temperature and pressure, observation wavelength, and ionizing laser intensity and delay. The Cerenkov peak angle is affected by the creation of plasma; estimates of plasma and neutral density have been extracted. Increases in visible background radiation consistent with increased plasma recombination emissions due to dissipation of wakefields were simultaneously measured.

  2. Measurements of radiation near an atomic spectral line from the interaction of a 30 GeV electron beam and a long plasma

    Energy Technology Data Exchange (ETDEWEB)

    Catravas, P.E.; Chattopadhyay, S.; Esarey, E.; Leemans, W.P.; Assmann, R.; Decker, F.-J.; Hogan, M.J.; Iverson, R.; Siemann, R.H.; Walz, D.; Whittum, D.; Blue, B.; Clayton, C; Joshi, C.; Marsh, K.A.; Mori, W.B.; Wang, S.; Katsouleas, T.; Lee, S.; Muggli, P.

    2000-10-31

    Emissions produced or initiated by a 30 GeV electron beam propagating through a {approx} 1 m long heat pipe oven containing neutral and partially ionized vapor have been measured near atomic spectral lines in a beam-plasma wakefield experiment. The Cerenkov spatial profile has been studied as a function of oven temperature and pressure, observation wavelength, and ionizing laser intensity and delay. The Cerenkov peak angle is affected by the creating of plasma, and estimates of neutral and plasma density have been extracted. Increases in visible background radiation, consistent with increased plasma recombination emissions due to dissipation of wakefields, were simultaneously measured.

  3. Measurements of radiation near an atomic spectral line from the interaction of a 30 GeV electron beam and a long plasma

    Science.gov (United States)

    Catravas, P.; Chattopadhyay, S.; Esarey, E.; Leemans, W. P.; Assmann, R.; Decker, F.-J.; Hogan, M. J.; Iverson, R.; Siemann, R. H.; Walz, D.; Whittum, D.; Blue, B.; Clayton, C.; Joshi, C.; Marsh, K. A.; Mori, W. B.; Wang, S.; Katsouleas, T.; Lee, S.; Muggli, P.

    2001-10-01

    Emissions produced or initiated by a 30-GeV electron beam propagating through a ~1-m long heat pipe oven containing neutral and partially ionized vapor have been measured near atomic spectral lines in a beam-plasma wakefield experiment. The Cerenkov spatial profile has been studied as a function of oven temperature and pressure, observation wavelength, and ionizing laser intensity and delay. The Cerenkov peak angle is affected by the creation of plasma, and estimates of neutral and plasma density have been extracted. Increases in visible background radiation, consistent with increased plasma recombination emissions due to dissipation of wakefields, were simultaneously measured.

  4. X-Ray Diffraction Apparatus

    Science.gov (United States)

    Blake, David F. (Inventor); Bryson, Charles (Inventor); Freund, Friedmann (Inventor)

    1996-01-01

    An x-ray diffraction apparatus for use in analyzing the x-ray diffraction pattern of a sample is introduced. The apparatus includes a beam source for generating a collimated x-ray beam having one or more discrete x-ray energies, a holder for holding the sample to be analyzed in the path of the beam, and a charge-coupled device having an array of pixels for detecting, in one or more selected photon energy ranges, x-ray diffraction photons produced by irradiating such a sample with said beam. The CCD is coupled to an output unit which receives input information relating to the energies of photons striking each pixel in the CCD, and constructs the diffraction pattern of photons within a selected energy range striking the CCD.

  5. Enhanced high-speed coherent diffraction imaging

    Science.gov (United States)

    Potier, Jonathan; Fricker, Sebastien; Idir, Mourad

    2011-03-01

    Due to recent advances in X-ray microscopy, we are now able to image objects with nanometer resolution thanks to Synchrotron beam lines or Free Electron Lasers (FEL). The PCI (Phase Contrast Imaging) is a robust technique that can recover the wavefront from measurements of only few intensity pictures in the Fresnel diffraction region. With our fast straightforward calculus methods, we manage to provide the phase induced by a microscopic specimen in few seconds. We can therefore obtain high contrasted images from transparent materials at very small scales. To reach atomic resolution imaging and thus make a transition from the near to the far field, the Coherent Diffraction Imaging (CDI) technique finds its roots in the analysis of diffraction patterns to obtain the phase of the altered complex wave. Theoretical results about existence and uniqueness of this retrieved piece of information by both iterative and direct algorithms have already been released. However, performances of algorithms remain limited by the coherence of the X-ray beam, presence of random noise and the saturation threshold of the detector. We will present reconstructions of samples using an enhanced version of HIO algorithm improving the speed of convergence and its repeatability. As a first step toward a practical X-Ray CDI system, initial images for reconstructions are acquired with the laser-based CDI system working in the visible spectrum.

  6. The spectroscopy in the atomic vapour

    Energy Technology Data Exchange (ETDEWEB)

    Lee, Jai Hyung; Chang, Joon Sung; Jhe, Won Ho [Seoul National University, Seoul (Korea)

    1998-04-01

    As spectroscopies in the atomic vapor, we perform experiments on fluorescence in dense atomic vapor, single color two-photon resonant three photon ionization, production of high temperature oven and its spectroscopic application, atomic trap and cold atomic beam. We observe lengthening of lifetime as atomic density increase and compare this result with Holstein equation. Dependence on pressure an d polarization reveals the result is due to collisions between Yb atom and Ar buffer gas. At high atomic density, self-focusing and conical emission are observed. In two-photon resonant three photon ionization scheme, ionization rate is dependent on polarization. From selection rule, we determined the energy level. At higher energy, asymmetry and broadening of ionization linewidth due to AC Stark effect are observed. As the result of numerical simulation of time evolution in the two-photon transition, distortion of time evolution of density is obtained. For spectroscopy of high-melting-point elements, we design and produce high temperature oven. We observe absorption spectra of high-melting-point elements, Er and Sm. As high temperature nonlinear spectroscopies, we perform conical emission and self-diffraction in Sm vapor. We produce magneto-optical trap system and measure fluorescence from trapped atoms and temperature. By trapping Rb isotopes simultaneously, we perform collision experiment at low temperature. Using hollow mirror system, we trap atoms and produce cold atomic beam. (author). 160 refs., 66 figs., 5 tabs.

  7. Diffraction radiation from relativistic particles

    CERN Document Server

    Potylitsyn, Alexander Petrovich; Strikhanov, Mikhail Nikolaevich; Tishchenko, Alexey Alexandrovich

    2010-01-01

    This book deals with diffraction radiation, which implies the boundary problems of electromagnetic radiation theory. Diffraction radiation is generated when a charged particle moves in a vacuum near a target edge. Diffraction radiation of non-relativistic particles is widely used to design intense emitters in the cm wavelength range. Diffraction radiation from relativistic charged particles is important for noninvasive beam diagnostics and design of free electron lasers based on Smith-Purcell radiation which is diffraction radiation from periodic structures. Different analytical models of diffraction radiation and results of recent experimental studies are presented in this book. The book may also serve as guide to classical electrodynamics applications in beam physics and electrodynamics. It can be of great use for young researchers to develop skills and for experienced scientists to obtain new results.

  8. Measurement of the scalar polarizability of the indium $6p_{1/2}$ state using two-step atomic-beam spectroscopy

    CERN Document Server

    Augenbraun, Benjamin L; Rupasinghe, P M; Majumder, P K

    2016-01-01

    We have completed a measurement of the Stark shift within the $^{115}$In $6s_{1/2} \\rightarrow 6p_{1/2}$ excited-state transition using two-step laser spectroscopy in an indium atomic beam. Combining this measurement with recent experimental results we determine the scalar polarizability, $\\alpha_{0}$, of the $6p_{1/2}$ state to be $7683 \\pm43 \\,a_{0}^{3}$ in atomic units, a result which agrees very well with recent theoretical calculations. In this experiment, one laser, stabilized to the $5p_{1/2} \\rightarrow 6s_{1/2}$ 410~nm transition, was directed transversely to the atomic beam, while a second, overlapping laser was scanned across the 1343~nm $6s_{1/2} \\rightarrow 6p_{1/2}$ transition. We utilized two-tone frequency-modulation spectroscopy of the infrared laser beam to measure the second-step absorption in the interaction region, where the optical depth is less than 10$^{-3}$. In the course of our experimental work we also determined the hyperfine splitting within the $6p_{1/2}$ state, improving upon th...

  9. Parabolic scaling beams.

    Science.gov (United States)

    Gao, Nan; Xie, Changqing

    2014-06-15

    We generalize the concept of diffraction free beams to parabolic scaling beams (PSBs), whose normalized intensity scales parabolically during propagation. These beams are nondiffracting in the circular parabolic coordinate systems, and all the diffraction free beams of Durnin's type have counterparts as PSBs. Parabolic scaling Bessel beams with Gaussian apodization are investigated in detail, their nonparaxial extrapolations are derived, and experimental results agree well with theoretical predictions.

  10. QED-based Optical Bloch Equations without electric dipole approximation: A model for a two-level atom interacting with a monochromatic X-ray laser beam

    CERN Document Server

    Zhang, Wen-Zhuo

    2012-01-01

    We derive a set of optical Bloch equations (OBEs) directly from the minimal-coupling Hamiltonian density of the bound-state quantum electrodynamics (bound-state QED). Such optical Bloch equations are beyond the former widely-used ones due to that there is no electric dipole approximation (EDA) on the minimal-coupling Hamiltonian density of the bound-state QED. Then our optical Bloch equations can describe a two-level atom interacting with a monochromatic light of arbitrary wavelength, which are suitable to study the spectroscopy and the Rabi oscillations of two-level atoms in X-ray laser beams since that the wavelength of X-ray is close to an atom to make the electric dipole approximation (EDA) invalid.

  11. Atomic magnetometer

    Science.gov (United States)

    Schwindt, Peter [Albuquerque, NM; Johnson, Cort N [Albuquerque, NM

    2012-07-03

    An atomic magnetometer is disclosed which uses a pump light beam at a D1 or D2 transition of an alkali metal vapor to magnetically polarize the vapor in a heated cell, and a probe light beam at a different D2 or D1 transition to sense the magnetic field via a polarization rotation of the probe light beam. The pump and probe light beams are both directed along substantially the same optical path through an optical waveplate and through the heated cell to an optical filter which blocks the pump light beam while transmitting the probe light beam to one or more photodetectors which generate electrical signals to sense the magnetic field. The optical waveplate functions as a quarter waveplate to circularly polarize the pump light beam, and as a half waveplate to maintain the probe light beam linearly polarized.

  12. On the Use of Wide-Angle Energy-Sensitive Detectors in White-Beam X-Ray Single-Crystal Diffraction

    DEFF Research Database (Denmark)

    Buras, B.; Staun Olsen, J.; Gerward, Leif

    1980-01-01

    The possible applications of multiple-element or large-area semiconductor detectors in single-crystal X-ray diffraction are discussed on the basis of experimental results using Bremsstrahlung as well as synchrotron radiation.......The possible applications of multiple-element or large-area semiconductor detectors in single-crystal X-ray diffraction are discussed on the basis of experimental results using Bremsstrahlung as well as synchrotron radiation....

  13. Atomic structure of glassy Mg60Cu30Y10 investigated with EXAFS, x-ray and neutron diffraction, and reverse Monte Carlo simulations

    DEFF Research Database (Denmark)

    Jovari, P.; Saksl, K.; Pryds, Nini;

    2007-01-01

    Short range order of amorphous Mg60Cu30Y10 was investigated by x-ray and neutron diffraction, Cu and Y K-edge x-ray absorption fine structure measurements, and the reverse Monte Carlo simulation technique. We found that Mg-Mg and Mg-Cu nearest neighbor distances are very similar to values found i...

  14. Atom Skimmers and Atom Lasers Utilizing Them

    Science.gov (United States)

    Hulet, Randall; Tollett, Jeff; Franke, Kurt; Moss, Steve; Sackett, Charles; Gerton, Jordan; Ghaffari, Bita; McAlexander, W.; Strecker, K.; Homan, D.

    2005-01-01

    Atom skimmers are devices that act as low-pass velocity filters for atoms in thermal atomic beams. An atom skimmer operating in conjunction with a suitable thermal atomic-beam source (e.g., an oven in which cesium is heated) can serve as a source of slow atoms for a magneto-optical trap or other apparatus in an atomic-physics experiment. Phenomena that are studied in such apparatuses include Bose-Einstein condensation of atomic gases, spectra of trapped atoms, and collisions of slowly moving atoms. An atom skimmer includes a curved, low-thermal-conduction tube that leads from the outlet of a thermal atomic-beam source to the inlet of a magneto-optical trap or other device in which the selected low-velocity atoms are to be used. Permanent rare-earth magnets are placed around the tube in a yoke of high-magnetic-permeability material to establish a quadrupole or octupole magnetic field leading from the source to the trap. The atoms are attracted to the locus of minimum magnetic-field intensity in the middle of the tube, and the gradient of the magnetic field provides centripetal force that guides the atoms around the curve along the axis of the tube. The threshold velocity for guiding is dictated by the gradient of the magnetic field and the radius of curvature of the tube. Atoms moving at lesser velocities are successfully guided; faster atoms strike the tube wall and are lost from the beam.

  15. Role of neutron beams in understanding the structure of alloys ferroelectrics and semi conductors

    Directory of Open Access Journals (Sweden)

    V. V. Agashe

    1960-04-01

    Full Text Available Our knowledge of materials is advanced to great extent with the help of optical, X-ray and electron beams, yet certain problems like order/disorder in alloys of metals having neighbouring atomic numbers, magnetic moment of magnetic alloys and compounds, position of atoms/ions in ferroelectrics cannot be solved with these techniques alone. Fortunately neutron beams because of their interaction with nuclei, can give us a detailed information about these problems. This paper reviews the experimental technique of neutron diffraction. Certain problems in alloy constitution, ferro-electricity and magnetic moments are discussed in light of the information obtained from neutron diffraction studies.

  16. Reflection high energy electron diffraction studies on Si{sub x}Sn{sub y}Ge{sub 1−x−y} on Si(100) molecular beam epitaxial growth

    Energy Technology Data Exchange (ETDEWEB)

    Nikiforov, A.I., E-mail: nikif@isp.nsc.ru [Rzhanov Institute of Semiconductor Physics, Siberian Branch of the Russian Academy of Sciences, Lavrentjeva 13, 630090 Novosibirsk (Russian Federation); Mashanov, V.I.; Timofeev, V.A.; Pchelyakov, O.P. [Rzhanov Institute of Semiconductor Physics, Siberian Branch of the Russian Academy of Sciences, Lavrentjeva 13, 630090 Novosibirsk (Russian Federation); Cheng, H.-H. [Center for Condensed Matter Sciences and Graduate Institute of Electronic Engineering, National Taiwan University, Taipei, 106, Taiwan, ROC (China)

    2014-04-30

    In situ reflection high energy electron diffraction was used to study the surface micromorphology of Si{sub x}Sn{sub y}Ge{sub 1−x−y} / Si(100) heterostructures obtained by molecular beam epitaxy. The obtained reflection high energy electron diffraction data allowed us to conclude that the epitaxial Si{sub x}Sn{sub y}Ge{sub 1−x−y} films are grown by the Stranski–Krastanov mechanism. It was established that Si{sub x}Sn{sub y}Ge{sub 1−x−y} and Ge{sub 1−z}Sn{sub z} wetting layer thicknesses depend on the substrate temperature. The observed surface superstructures changed during the wetting layer growth. - Highlights: • Stranski–Krastanov mechanism • Wetting layers depend on the temperature • Superstructures change.

  17. The role of phase separation for self-organized surface pattern formation by ion beam erosion and metal atom co-deposition

    Energy Technology Data Exchange (ETDEWEB)

    Hofsaess, H.; Zhang, K.; Pape, A.; Bobes, O.; Broetzmann, M. [Georg-August University Goettingen, II. Institute of Physics, Goettingen (Germany)

    2013-05-15

    We investigate the ripple pattern formation on Si surfaces at room temperature during normal incidence ion beam erosion under simultaneous deposition of different metallic co-deposited surfactant atoms. The co-deposition of small amounts of metallic atoms, in particular Fe and Mo, is known to have a tremendous impact on the evolution of nanoscale surface patterns on Si. In previous work on ion erosion of Si during co-deposition of Fe atoms, we proposed that chemical interactions between Fe and Si atoms of the steady-state mixed Fe{sub x} Si surface layer formed during ion beam erosion is a dominant driving force for self-organized pattern formation. In particular, we provided experimental evidence for the formation of amorphous iron disilicide. To confirm and generalize such chemical effects on the pattern formation, in particular the tendency for phase separation, we have now irradiated Si surfaces with normal incidence 5 keV Xe ions under simultaneous gracing incidence co-deposition of Fe, Ni, Cu, Mo, W, Pt, and Au surfactant atoms. The selected metals in the two groups (Fe, Ni, Cu) and (W, Pt, Au) are very similar regarding their collision cascade behavior, but strongly differ regarding their tendency to silicide formation. We find pronounced ripple pattern formation only for those co deposited metals (Fe, Mo, Ni, W, and Pt), which are prone to the formation of mono and disilicides. In contrast, for Cu and Au co-deposition the surface remains very flat, even after irradiation at high ion fluence. Because of the very different behavior of Cu compared to Fe, Ni and Au compared to W, Pt, phase separation toward amorphous metal silicide phases is seen as the relevant process for the pattern formation on Si in the case of Fe, Mo, Ni, W, and Pt co-deposition. (orig.)

  18. Far-field divergence for Gaussian beam under annular aperture diffraction%圆环孔径衍射高斯光束远场发散角研究

    Institute of Scientific and Technical Information of China (English)

    王超; 董科研; 江伦; 安岩

    2015-01-01

    The simple approximated analytic expression for the far-field divergence angle of Gaussian beam diffracted by an annular aperture was derived based on the Fraunhofer diffraction theory and by the approximate of the diffraction integration kernel function. For diffraction aperture with different diameters and obscuration ratios (OR), the analytic expression was compared by strict Fraunhofer diffraction expression, and the far-field divergences solved by these two expressions were nearly identical. The error was no more than 2.7%. Compared with the traditional method of getting the beam divergence by numerical integration, the troublesome integral was avoided, but a relative high precision was kept through this approximated formula. The analytic formula was effective on condition that the Gaussian beam waist diameter was more than or equal to 3.5 times the obscuration diameter, and less than or equal to the aperture diameter. In an actual engineering application, especially the space laser communication optical antenna with the characteristics of large-aperture and small-OR, the establishing conditions generally are satisfied.%基于夫琅禾费衍射理论,通过对衍射积分的核函数进行近似,推导并得出了简洁的经圆环形孔径衍射的高斯光束远场发散角的近似解析式.在不同衍射孔径外径和不同遮拦比的条件下,将该解析式与严格的夫琅禾费衍射积分进行比较,发现二者求出的远场发散角接近一致,最大误差不超过2.7%.与传统数值积分求取光束发散角相比,该近似解析式在避免繁琐的积分运算同时保持了较高的精度.该解析式成立条件为高斯光束的束腰直径大于等于3.5倍中心遮拦直径,且小于等于孔径直径;在实际工程应用中,特别是具有大口径、小遮拦比特点的空间激光通信光学天线这一应用场景,该条件一般能够被满足.

  19. Atomic structure of glassy Mg60Cu30Y10 investigated with EXAFS, x-ray and neutron diffraction, and reverse Monte Carlo simulations

    DEFF Research Database (Denmark)

    Jovari, P.; Saksl, K.; Pryds, Nini;

    2007-01-01

    Short range order of amorphous Mg60Cu30Y10 was investigated by x-ray and neutron diffraction, Cu and Y K-edge x-ray absorption fine structure measurements, and the reverse Monte Carlo simulation technique. We found that Mg-Mg and Mg-Cu nearest neighbor distances are very similar to values found...... studied by differential scanning calorimetry and in situ x-ray powder diffraction. The alloy shows a glass transition and three crystallization events, the first and dominant one at 456 K corresponding to eutectic crystallization of at least three phases: Mg2Cu and most likely cubic MgY and CuMgY....

  20. Impact of Casimir-Polder interaction on Poisson-spot diffraction at a dielectric sphere

    CERN Document Server

    Hemmerich, Joshua Leo; Reisinger, Thomas; Nimmrichter, Stefan; Fiedler, Johannes; Hahn, Horst; Gleiter, Herbert; Buhmann, Stefan Yoshi

    2016-01-01

    Diffraction of matter-waves is an important demonstration of the fact that objects in nature possess a mixture of particle-like and wave-like properties. Unlike in the case of light diffraction, matter-waves are subject to a vacuum-mediated interaction with diffraction obstacles. Here we present a detailed account of this effect through the calculation of the attractive Casimir-Polder potential between a dielectric sphere and an atomic beam. Furthermore, we use our calculated potential to make predictions about the diffraction patterns to be observed in an ongoing experiment where a beam of indium atoms is diffracted around a silicon dioxide sphere. The result is an amplification of the on-axis bright feature which is the matter-wave analogue of the well-known `Poisson spot' from optics. Our treatment confirms that the diffraction patterns resulting from our complete account of the sphere Casimir-Polder potential are indistinguishable from those found via a large-sphere non-retarded approximation in the discu...

  1. Impact of Casimir-Polder interaction on Poisson-spot diffraction at a dielectric sphere

    Science.gov (United States)

    Hemmerich, Joshua L.; Bennett, Robert; Reisinger, Thomas; Nimmrichter, Stefan; Fiedler, Johannes; Hahn, Horst; Gleiter, Herbert; Buhmann, Stefan Yoshi

    2016-08-01

    Diffraction of matter waves is an important demonstration of the fact that objects in nature possess a mixture of particlelike and wavelike properties. Unlike in the case of light diffraction, matter waves are subject to a vacuum-mediated interaction with diffraction obstacles. Here we present a detailed account of this effect through the calculation of the attractive Casimir-Polder potential between a dielectric sphere and an atomic beam. Furthermore, we use our calculated potential to make predictions about the diffraction patterns to be observed in an ongoing experiment where a beam of indium atoms is diffracted around a silicon-dioxide sphere. The result is an amplification of the on-axis bright feature, which is the matter-wave analog of the well-known "Poisson spot" from optics. Our treatment confirms that the diffraction patterns resulting from our complete account of the sphere Casimir-Polder potential are indistinguishable from those found via a large-sphere nonretarded approximation in the discussed experiments, establishing the latter as an adequate model.

  2. Study of X-Ray and $\\gamma$-Ray Spectra from Antiprotonic Atoms at the Slowly Extracted Antiproton Beam of LEAR

    CERN Multimedia

    2002-01-01

    This experiment will study the X-ray spectra of antiprotonic atoms and the $\\gamma$ spectra of residual nuclei after the antiproton absorption. We intend to begin with measurements on selected isotopically pure targets. Strong interaction effects, the antiproton absorption and the atomic cascade are analysed through the measurement of energies, lineshapes, relative and absolute intensities of all observable lines. The experiments are continued to determine st in resolved fine structure levels and in different isotopes of the same element. Coincidence techniques may be applied. All components of the experimental set-up are already existing from previous experiments and we could begin the measurements with any slowly extracted beam of low energy at LEAR.

  3. Damage effects of {ion}/{atom} beam milling on MNOS (Al/Si 3N 4/SiO 2/Si) capacitors

    Science.gov (United States)

    Bangert, U.; Belson, J.; Wilson, I. H.

    1984-02-01

    Low energy argon ion and atom beams produced by saddle field sources have been used to study changes in CVD Si 3N 4/SiO 2/Si structures after bombardment of the bare nitride at a particle energy of 2.9 keV. Interface state densities Nst and flatband voltages VFB were extracted from high frequency (1.3 MHz) and quasi-static C- V curves. Bombardment was found to induce an increase in Nst and positive and negative charge storage associated with the nitride (or the nitride/oxide interface). The effect was more pronounced under ion bombardment. On the supposition that displacement damage is similar for ion and atom bombardments the differences in charge storage are interpreted in terms of enhanced trapping under the field associated with ion bombardment.

  4. Investigation on the lattice site location of the excess arsenic atoms in GaAs layers grown by low temperature molecular beam epitaxy

    Energy Technology Data Exchange (ETDEWEB)

    Yu, Kin Man; Liliental-Weber, Z.

    1991-11-01

    We have measured the excess As atoms present in gaze layers grown by molecular beam epitaxy at low substrate temperatures using particle induced x-ray emission technique. The amount of excess As atoms in layers grown by MBE at 200{degrees}C were found to be {approximately} 4 {times} 10{sup 20} cm{sup {minus}2}. Subsequent annealing of the layers under As overpressure at 600{degrees}C did not result in any substantial As loss. However, transmission electron microscopy revealed that As precipitates (2-5nm in diameter) were present in the annealed layers. The lattice location of the excess As atoms in the as grown layers was investigated by ion channeling methods. Angular scans were performed in the <110> axis of the crystal. Our results strongly suggest that a large fraction of these excess As atoms are located in an interstitial position close to an As row. These As intersitials'' are located at a site slightly displaced from the tetrahedral site in a diamond cubic lattice. No interstitial As signal is observed in the annealed layers.

  5. Investigation on the lattice site location of the excess arsenic atoms in GaAs layers grown by low temperature molecular beam epitaxy

    Energy Technology Data Exchange (ETDEWEB)

    Yu, Kin Man; Liliental-Weber, Z.

    1991-11-01

    We have measured the excess As atoms present in gaze layers grown by molecular beam epitaxy at low substrate temperatures using particle induced x-ray emission technique. The amount of excess As atoms in layers grown by MBE at 200{degrees}C were found to be {approximately} 4 {times} 10{sup 20} cm{sup {minus}2}. Subsequent annealing of the layers under As overpressure at 600{degrees}C did not result in any substantial As loss. However, transmission electron microscopy revealed that As precipitates (2-5nm in diameter) were present in the annealed layers. The lattice location of the excess As atoms in the as grown layers was investigated by ion channeling methods. Angular scans were performed in the <110> axis of the crystal. Our results strongly suggest that a large fraction of these excess As atoms are located in an interstitial position close to an As row. These As ``intersitials`` are located at a site slightly displaced from the tetrahedral site in a diamond cubic lattice. No interstitial As signal is observed in the annealed layers.

  6. The temperature dependent variation of bulk and surface composition of In(x)Ga(1-x)As on GaAs grown by chemical beam epitaxy studied by RHEED, X-ray diffraction and XPS

    Science.gov (United States)

    Hansen, H. S.; Bensaoula, A.; Tougaard, S.; Zborowski, J.; Ignatiev, A.

    1992-01-01

    The paper investigates the bulk as well as near-surface composition of In(x)Ga(1-x)As epilayers on GaAs grown by chemical beam epitaxy (CBE) as a function of triethylindium flow rate and substrate temperature by reflection high energy electron diffraction (RHEED), X-ray diffraction, and XPS. To clarify whether the bulk stoichiometry of CBE-grown ternaries can be extracted from the growth rate change as determined by the change in the period of RHEED oscillations from binary to ternary compound growth, a systematic study of growth rate change as a function of ternary bulk composition determined by X-ray diffraction was performed at various temperatures. It is shown that for low growth temperatures there is a linear relationship between the two methods of determination, whereas no correlation is found for higher growth temperatures, in contrast to the MBE case where the two methods of determination yield identical results. In the near surface region the epilayer composition is determined in situ by XPS.

  7. 经卡式光学天线发射的高斯光束衍射特性的研究%The Study of Diffraction Characteristics of Gaussian Beam Transmitted by Cassegrain Optical Antenna in Laser Communication

    Institute of Scientific and Technical Information of China (English)

    刘龙飞; 佟首峰; 王超

    2015-01-01

    激光通信发射系统一般都是采用卡塞格林式望远镜作为发射天线,由于激光通信采用的光源波形为高斯光束,卡式光学系统的主次镜光学结构为环形结构,以往对均匀波经圆孔光阑后的衍射特性并不适用于激光通信。对基尔霍夫衍射公式进行了简化,利用数值计算的方法,利用仿真软件得到了高斯光束通过卡式光学天线之后的远场衍射分布特性,并与近场菲涅尔衍射分布特性进行分析比对,给出了卡式光学结构的最佳遮拦比为0.2,理论上可以达到1.5倍的近衍射极限发射束散角,在工程计算中有一定的应用价值。%For laser communication transmitter systems,a Cassegrain telescope is generally used as a transmitting anten-na. As the light wave using in laser communication is a Gaussian light beam, and the optical structure of primary and secondary mirrors of Cassette optical system are ring structures,in the past,the diffractions characteristics that Uniform wave pass through circular aperture are not fit to apply in laser communications. The complicated Kirchhoff diffraction formula is simplified in this paper. The distributed characteristics of far-field diffraction that Gaussian beam pass through Cassette optical antenna are got by using simulation software and compared with the distribution characteristics of near-field Fresnel diffraction. The optimum obscuration ratio of Cassegrain optical structure can be 0.2.Theoretically, a 1.5 times transimitted angle of near diffraction limit can be got. There are some certain values in engineering calculations.

  8. Combined measurement of X-ray photon correlation spectroscopy and diffracted X-ray tracking using pink beam X-rays.

    Science.gov (United States)

    Shinohara, Yuya; Watanabe, Akira; Kishimoto, Hiroyuki; Amemiya, Yoshiyuki

    2013-09-01

    Combined X-ray photon correlation spectroscopy (XPCS) and diffracted X-ray tracking (DXT) measurements of carbon-black nanocrystals embedded in styrene-butadiene rubber were performed. From the intensity fluctuation of speckle patterns in a small-angle scattering region (XPCS), dynamical information relating to the translational motion can be obtained, and the rotational motion is observed through the changes in the positions of DXT diffraction spots. Graphitized carbon-black nanocrystals in unvulcanized styrene-butadiene rubber showed an apparent discrepancy between their translational and rotational motions; this result seems to support a stress-relaxation model for the origin of super-diffusive particle motion that is widely observed in nanocolloidal systems. Combined measurements using these two techniques will give new insights into nanoscopic dynamics, and will be useful as a microrheology technique.

  9. Condensed matter applied atomic collision physics, v.4

    CERN Document Server

    Datz, Sheldon

    1983-01-01

    Applied Atomic Collision Physics, Volume 4: Condensed Matter deals with the fundamental knowledge of collision processes in condensed media.The book focuses on the range of applications of atomic collisions in condensed matter, extending from effects on biological systems to the characterization and modification of solids. This volume begins with the description of some aspects of the physics involved in the production of ion beams. The radiation effects in biological and chemical systems, ion scattering and atomic diffraction, x-ray fluorescence analysis, and photoelectron and Auger spectrosc

  10. Neutron diffraction

    Energy Technology Data Exchange (ETDEWEB)

    Heger, G. [Rheinisch-Westfaelische Technische Hochschule Aachen, Inst. fuer Kristallographie, Aachen (Germany)

    1996-12-31

    X-ray diffraction using conventional laboratory equipment and/or synchrotron installations is the most important method for structure analyses. The purpose of this paper is to discuss special cases, for which, in addition to this indispensable part, neutrons are required to solve structural problems. Even though the huge intensity of modern synchrotron sources allows in principle the study of magnetic X-ray scattering the investigation of magnetic structures is still one of the most important applications of neutron diffraction. (author) 15 figs., 1 tab., 10 refs.

  11. The identification of autoionizing states of atomic chromium for the resonance ionization laser ion source of the ISOLDE radioactive ion beam facility

    Science.gov (United States)

    Day Goodacre, T.; Chrysalidis, K.; Fedorov, D. V.; Fedosseev, V. N.; Marsh, B. A.; Molkanov, P. L.; Rossel, R. E.; Rothe, S.; Seiffert, C.

    2017-03-01

    This paper presents the results of an investigation into autoionizing states of atomic chromium, in the service of the resonance ionization laser ion source (RILIS): the principal ion source of the ISOLDE radioactive ion beam facility based at CERN. The multi-step resonance photo-ionization process enables element selective ionization which, in combination with mass separation, allows isotope specific selectivity in the production of radioactive ion beams at ISOLDE. The element selective nature of the process requires a multi-step "ionization scheme" to be developed for each element. Using the method of in-source resonance ionization spectroscopy, an optimal three-step, three-resonance photo-ionization scheme originating from the 3d5(6S)4s a7S3 atomic ground state has been developed for chromium. The scheme uses an ionizing transition to one of the 15 newly observed autoionizing states reported here. Details of the spectroscopic studies are described and the new ionization scheme is summarized.

  12. Atomic and electronic structure transformations in SnS2 at high pressures: a joint single crystal X-ray diffraction and DFT study.

    Science.gov (United States)

    Filsø, M Ø; Eikeland, E; Zhang, J; Madsen, S R; Iversen, B B

    2016-03-07

    The layered semiconductor SnS2 spurs much interest for both intercalation and optoelectronic applications. Despite the wealth of research in the field of metal dichalcogenides, the structure-property relationship of this compound remains unclear. Here we present a thorough study combining single-crystal X-ray diffraction and DFT calculations on SnS2 in the pressure range 0 band structure calculations. The calculated narrowing of the band gap is supported by a significant, reversible color change of the single crystal. At 20 GPa, the size of the band gap has decreased from 2.15 to 0.88 eV, and band gap closure is predicted to occur at 33 GPa.

  13. Diode-pumped dual-wavelength Nd:LSO laser at 1059 and 1067  nm with nearly diffraction-limited beam quality.

    Science.gov (United States)

    Huang, Xiaoxu; Lan, Jinglong; Lin, Zhi; Wang, Yi; Xu, Bin; Xu, Huiying; Cai, Zhiping; Xu, Xiaodong; Zhang, Jian; Xu, Jun

    2016-04-10

    We report a diode-pumped continuous-wave simultaneous dual-wavelength Nd:LSO laser at 1059 and 1067 nm. By employing a specially coated output coupler with relatively high transmissions at high-gain emission lines of 1075 and 1079 nm, the two low-gain emission lines, 1059 and 1067 nm, can be achieved, for the first time to our knowledge, with maximum output power of 1.27 W and slope efficiency of about 29.2%. The output power is only limited by the available pump power. Output beam quality is also measured to be about 1.19 and 1.21 of the beam propagation factors in the x and y directions, respectively.

  14. ELASTIC AND INELASTIC HELIUM ATOM SCATTERING AT A CLEAVED MICA SHEET

    NARCIS (Netherlands)

    BRUSDEYLINS, G; SCHMICKER, D

    1995-01-01

    A mica sheet has been cleaved in situ in a UHV beam scattering apparatus. The diffraction of the helium atoms shows sharp Bragg peaks. In the [110] and [110] directions of the hexagonal surface the intensities of the Bragg peaks are analysed in terms of a sinusoidal corrugation. With hard wall scatt

  15. Note: Determination of torsional spring constant of atomic force microscopy cantilevers: combining normal spring constant and classical beam theory.

    Science.gov (United States)

    Álvarez-Asencio, R; Thormann, E; Rutland, M W

    2013-09-01

    A technique has been developed for the calculation of torsional spring constants for AFM cantilevers based on the combination of the normal spring constant and plate/beam theory. It is easy to apply and allow the determination of torsional constants for stiff cantilevers where the thermal power spectrum is difficult to obtain due to the high resonance frequency and low signal/noise ratio. The applicability is shown to be general and this simple approach can thus be used to obtain torsional constants for any beam shaped cantilever.

  16. From atomic structure to excess entropy: a neutron diffraction and density functional theory study of CaO-Al₂O₃-SiO₂ melts.

    Science.gov (United States)

    Liu, Maoyuan; Jacob, Aurélie; Schmetterer, Clemens; Masset, Patrick J; Hennet, Louis; Fischer, Henry E; Kozaily, Jad; Jahn, Sandro; Gray-Weale, Angus

    2016-04-06

    Calcium aluminosilicate CaO-Al2O3-SiO2 (CAS) melts with compositions (CaO-SiO2)(x)(Al2O3)(1-x) for x  theory molecular dynamics modelling. Simulated structure factors are found to be in good agreement with experimental structure factors. Local atomic structures from simulations reveal the role of calcium cations as a network modifier, and aluminium cations as a non-tetrahedral network former. Distributions of tetrahedral order show that an increasing concentration of the network former Al increases entropy, while an increasing concentration of the network modifier Ca decreases entropy. This trend is opposite to the conventional understanding that increasing amounts of network former should increase order in the network liquid, and so decrease entropy. The two-body correlation entropy S2 is found to not correlate with the excess entropy values obtained from thermochemical databases, while entropies including higher-order correlations such as tetrahedral order, O-M-O or M-O-M bond angles and Q(N) environments show a clear linear correlation between computed entropy and database excess entropy. The possible relationship between atomic structures and excess entropy is discussed.

  17. Order within disorder: The atomic structure of ion-beam sputtered amorphous tantala (a-Ta2O5

    Directory of Open Access Journals (Sweden)

    Riccardo Bassiri

    2015-03-01

    Full Text Available Amorphous tantala (a-Ta2O5 is a technologically important material often used in high-performance coatings. Understanding this material at the atomic level provides a way to further improve performance. This work details extended X-ray absorption fine structure measurements of a-Ta2O5 coatings, where high-quality experimental data and theoretical fits have allowed a detailed interpretation of the nearest-neighbor distributions. It was found that the tantalum atom is surrounded by four shells of atoms in sequence; oxygen, tantalum, oxygen, and tantalum. A discussion is also included on how these models can be interpreted within the context of published crystalline Ta2O5 and other a-T2O5 studies.

  18. Note: Determination of torsional spring constant of atomic force microscopy cantilevers: Combining normal spring constant and classical beam theory

    DEFF Research Database (Denmark)

    Álvarez-Asencio, R.; Thormann, Esben; Rutland, M.W.

    2013-01-01

    A technique has been developed for the calculation of torsional spring constants for AFM cantilevers based on the combination of the normal spring constant and plate/beam theory. It is easy to apply and allow the determination of torsional constants for stiff cantilevers where the thermal power...

  19. Excitation of the shear horizontal mode in a monolayer by inelastic helium atom scattering

    DEFF Research Database (Denmark)

    Bruch, L. W.; Hansen, Flemming Yssing

    2005-01-01

    Inelastic scattering of a low-energy atomic helium beam (HAS) by a physisorbed monolayer is treated in the one-phonon approximation using a time-dependent wave,packet formulation. The calculations show that modes with shear horizontal polarization can be excited near high symmetry azimuths....... The diffraction and inelastic processes arise from a strong coupling of the incident atom to the target and the calculated results show large departures from expectations based on analogies to inelastic thermal neutron scattering....

  20. Optical diffraction for measurements of nano-mechanical bending

    Science.gov (United States)

    Hermans, Rodolfo I.; Dueck, Benjamin; Ndieyira, Joseph Wafula; McKendry, Rachel A.; Aeppli, Gabriel

    2016-06-01

    We explore and exploit diffraction effects that have been previously neglected when modelling optical measurement techniques for the bending of micro-mechanical transducers such as cantilevers for atomic force microscopy. The illumination of a cantilever edge causes an asymmetric diffraction pattern at the photo-detector affecting the calibration of the measured signal in the popular optical beam deflection technique (OBDT). The conditions that avoid such detection artefacts conflict with the use of smaller cantilevers. Embracing diffraction patterns as data yields a potent detection technique that decouples tilt and curvature and simultaneously relaxes the requirements on the illumination alignment and detector position through a measurable which is invariant to translation and rotation. We show analytical results, numerical simulations and physiologically relevant experimental data demonstrating the utility of the diffraction patterns. We offer experimental design guidelines and quantify possible sources of systematic error in OBDT. We demonstrate a new nanometre resolution detection method that can replace OBDT, where diffraction effects from finite sized or patterned cantilevers are exploited. Such effects are readily generalized to cantilever arrays, and allow transmission detection of mechanical curvature, enabling instrumentation with simpler geometry. We highlight the comparative advantages over OBDT by detecting molecular activity of antibiotic Vancomycin.

  1. Structural effects due to the incorporation of Ar atoms in the lattice of ZrO sub 2 thin films prepared by ion beam assisted deposition

    CERN Document Server

    Holgado, J P; Veen, A V; Schut, H; Hosson, J T M; González-Elipe, A R

    2002-01-01

    Two sets of ZrO sub 2 thin films have been prepared at room temperature by ion beam induced chemical vapour deposition and subsequently annealed up to 1323 K. The two sets of samples have been prepared by using either O sub 2 sup + or mixtures of (O sub 2 sup + +Ar sup +) ions for the decomposition of a volatile metallorganic precursor of zirconium. The structure and microstructure of these two sets of samples have been determined by means of X-ray diffraction, Fourier transform infrared spectroscopy and positron beam analysis (PBA). The samples were very compact and dense and had a very low-surface roughness. After annealing in air at T>=573 K both sets of films were transparent and showed similar refraction indexes. For the (O sub 2 sup + +Ar sup +)-ZrO sub 2 thin films it is shown by X-ray photoelectron spectroscopy and Rutherford back scattering that a certain amount of incorporated Ar (5-6 at.%) remains incorporated within the oxide lattice. No changes were detected in the amount of incorporated Ar even ...

  2. Aluminium incorporation in Al{sub x}Ga{sub 1-x}N/GaN heterostructures: A comparative study by ion beam analysis and X-ray diffraction

    Energy Technology Data Exchange (ETDEWEB)

    Redondo-Cubero, A. [ISOM and Dpt. de Ingenieria Electronica, ETSI Telecomunicacion, Universidad Politecnica de Madrid, E-28040 Madrid (Spain); Centro de Micro-Analisis de Materiales, Universidad Autonoma de Madrid, E-28049 Madrid (Spain); Gago, R. [Centro de Micro-Analisis de Materiales, Universidad Autonoma de Madrid, E-28049 Madrid (Spain)], E-mail: raul.gago@uam.es; Gonzalez-Posada, F. [ISOM and Dpt. de Ingenieria Electronica, ETSI Telecomunicacion, Universidad Politecnica de Madrid, E-28040 Madrid (Spain); Kreissig, U. [Institute of Ion Beam Physics and Materials Research, Forschungszentrum Dresden-Rossendorf, PF 51019, D-01314 Dresden (Germany); Di Forte Poisson, M.-A. [Thales Research and Technology/TIGER 91461 Marcoussis Cedex (France); Brana, A.F.; Munoz, E. [ISOM and Dpt. de Ingenieria Electronica, ETSI Telecomunicacion, Universidad Politecnica de Madrid, E-28040 Madrid (Spain)

    2008-10-01

    The Al content in Al{sub x}Ga{sub 1-x}N/GaN heterostructures has been determined by X-ray diffraction (XRD) and contrasted with absolute measurements from ion beam analysis (IBA) methods. For this purpose, samples with 0.1 < x < 0.3 grown by metal organic chemical vapour deposition on sapphire substrates have been studied. XRD and IBA corroborate the good epitaxial growth of the AlGaN layer, which slightly deteriorates with the incorporation of Al for x > 0.2. The assessment of Al incorporation by XRD is quite reliable regarding the average value along the sample thickness. However, XRD analysis tends to overestimate the Al fraction at low contents, which is attributed to the presence of strain within the layer. For the highest Al incorporation, IBA detects a certain Al in-depth compositional profile that should be considered for better XRD data analysis.

  3. Relativistic atomic beam spectroscopy 2. Appendix A: Progress report, July 1, 1989--June 30, 1992: Final report

    Energy Technology Data Exchange (ETDEWEB)

    Bryant, H.C.

    1992-07-01

    This work supported by the Division of Chemical Sciences, Office of Basic Energy Services, Office of Energy Research, US Department of Energy during the period July 1, 1989 to June 30, 1992, resulted in noteworthy scientific results in three categories which we shall discuss in turn: The spectroscopy of high-lying doubly-excited states of H{sup {minus}}, interactions with thin foils, and multiphoton processes. Radiological safety concerns and slow beam studies are also briefly discussed.

  4. Atom interferometry with lithium atoms: theoretical analysis and design of an interferometer, applications; Interferometrie atomique avec l'atome de lithium: analyse theorique et construction d'un interferometre, applications

    Energy Technology Data Exchange (ETDEWEB)

    Champenois, C

    1999-12-01

    This thesis is devoted to studies which prepared the construction of an atom Mach-Zehnder interferometer. In such an interferometer, the propagating waves are spatially separated, and the internal state of the atom is not modified. The beam-splitters are diffraction gratings, consisting of standing optical waves near-resonant with an atomic transition. We use the Bloch functions to define the atom wave inside the standing wave grating and thus explain the diffraction process in different cases. We developed a nearly all-analytical model for the propagation of an atom wave inside a Mach-Zehnder interferometer. The contrast of the signal is studied for many cases: phase or amplitude gratings, effects of extra paths, effects of the main mismatches, monochromatic or lightly polychromatic sources. Finally, we discuss three interferometric measurements we think very interesting. The first, the index of refraction of gas for atomic waves, is studied in detail, with numerical simulations. The other measures we propose deal with the electrical properties of lithium. We discuss the ultimate limit for the measure of the static electric polarizability of lithium by atomic interferometry. Then, we discuss how one could measure the possible charge of the lithium atom. We conclude that an optically cooled and collimated atom beam would improve precision. (author)

  5. Influence of relative parameters on quality of long distance diffraction-free beam%相关参数对长距离近似无衍射光束质量的影响

    Institute of Scientific and Technical Information of China (English)

    郑维涛; 吴逢铁; 张前安; 程治明

    2012-01-01

    The influence of relative parameters,such as the focal length of the convergence lens and the distance between the convergence lens and the axicon, on the propagation distance of long distance diffraction-free beam generated by two axicons is analyzed using ray-tracing method. Numerical simulation is carried out with Mathcad. The results show that, while other conditions are invariable, the propagation distance of long distance diffraction-free beam decreases as the focal length of the convergence lens increases, and rises with the increasing of the distance between the convergence lens and the axicon. The theory is verified by experiment, and the experimental results are consistent with theoretical analysis.%利用光线追迹法分析了会聚透镜焦距及会聚透镜与轴棱锥的距离等相关参数对双轴棱锥产生的长距离近似无衍射光束传播距离的影响,运用Mathcad对其进行了数值模拟.结果显示:在其他条件不变的情况下,近似无衍射光束的传播距离随会聚透镜焦距的增大而减小,随会聚透镜与轴棱锥之间距离的增大而增大.通过实验对理论进行了验证,所得结果与理论分析相吻合.

  6. “Fast Atom Diffraction” IBA in the regime of quantum scattering

    Energy Technology Data Exchange (ETDEWEB)

    Winter, H., E-mail: winter@physik.hu-berlin.de

    2014-08-01

    Recently, quantum effects were observed for the scattering of fast atoms from surfaces under a grazing angle of incidence. We discuss basic features of Fast Atom Diffraction (FAD) which adds a further powerful method to the established tools in ion beam analysis. Attractive features of FAD in studies on the structure of surfaces comprise negligible radiation damage, no charging effects, and an extreme sensitivity to the topmost layer of surface atoms. Scanning the quantum wavelength associated with the motion of a massive particle by the variation of its kinetic energy allows one to apply interferometric concepts to surface analysis based on the scattering of fast atoms.

  7. Spatial dynamics of laser-induced fluorescence in an intense laser beam: experiment and theory in alkali metal atoms

    CERN Document Server

    Auzinsh, Marcis; Ferber, Ruvin; Gahbauer, Florian; Kalnins, Uldis

    2015-01-01

    We have shown that it is possible to model accurately optical phenomena in intense laser fields by taking into account the intensity distribution over the laser beam. We developed a theoretical model that divided an intense laser beam into concentric regions, each with a Rabi frequency that corresponds to the intensity in that region, and solved a set of coupled optical Bloch equations for the density matrix in each region. Experimentally obtained magneto-optical resonance curves for the $F_g=2\\longrightarrow F_e=1$ transition of the $D_1$ line of $^{87}$Rb agreed very well with the theoretical model up to a laser intensity of around 200 mW/cm$^2$ for a transition whose saturation intensity is around 4.5 mW/cm$^2$. We have studied the spatial dependence of the fluorescence intensity in an intense laser beam experimentally and theoretically. An experiment was conducted whereby a broad, intense pump laser excited the $F_g=4\\longrightarrow F_e=3$ transition of the $D_2$ line of cesium while a weak, narrow probe ...

  8. Average and local atomic-scale structure in BaZrxTi(1-x)O3 (x = 0. 10, 0.20, 0.40) ceramics by high-energy x-ray diffraction and Raman spectroscopy.

    Science.gov (United States)

    Buscaglia, Vincenzo; Tripathi, Saurabh; Petkov, Valeri; Dapiaggi, Monica; Deluca, Marco; Gajović, Andreja; Ren, Yang

    2014-02-12

    High-resolution x-ray diffraction (XRD), Raman spectroscopy and total scattering XRD coupled to atomic pair distribution function (PDF) analysis studies of the atomic-scale structure of archetypal BaZrxTi(1-x)O3 (x = 0.10, 0.20, 0.40) ceramics are presented over a wide temperature range (100-450 K). For x = 0.1 and 0.2 the results reveal, well above the Curie temperature, the presence of Ti-rich polar clusters which are precursors of a long-range ferroelectric order observed below TC. Polar nanoregions (PNRs) and relaxor behaviour are observed over the whole temperature range for x = 0.4. Irrespective of ceramic composition, the polar clusters are due to locally correlated off-centre displacement of Zr/Ti cations compatible with local rhombohedral symmetry. Formation of Zr-rich clusters is indicated by Raman spectroscopy for all compositions. Considering the isovalent substitution of Ti with Zr in BaZrxTi1-xO3, the mechanism of formation and growth of the PNRs is not due to charge ordering and random fields, but rather to a reduction of the local strain promoted by the large difference in ion size between Zr(4+) and Ti(4+). As a result, non-polar or weakly polar Zr-rich clusters and polar Ti-rich clusters are randomly distributed in a paraelectric lattice and the long-range ferroelectric order is disrupted with increasing Zr concentration.

  9. Production of intense beams of mass-selected water cluster ions and theoretical study of atom-water interactions

    CERN Document Server

    Wang, Z P; Reinhard, P -G; Suraud, E; Bruny, G; Montano, C; Feil, S; Eden, S; Abdoul-Carime, H; Farizon, B; Farizon, M; Ouaskit, S; Maerk, T D

    2009-01-01

    The influences of water molecules surrounding biological molecules during irradiation with heavy particles (atoms,ions) are currently a major subject in radiation science on a molecular level. In order to elucidate the underlying complex reaction mechanisms we have initiated a joint experimental and theoretical investigation with the aim to make direct comparisons between experimental and theoretical results. As a first step, studies of collisions of a water molecule with a neutral projectile (C atom) at high velocities (> 0.1 a.u.), and with a charged projectile (proton) at low velocities (< 0.1 a.u.) have been studied within the microscopic framework. In particular, time-dependent density functional theory (TDDFT) was applied to the valence electrons and coupled non-adiabatically to Molecular dynamics (MD) for ionic cores. Complementary experimental developments have been carried out to study projectile interactions with accelerated (< 10 keV) and mass-selected cluster ions. The first size distributio...

  10. Dynamics of bisolitonic matter waves in a Bose-Einstein condensate subjected to an atomic beam splitter and gravity

    CERN Document Server

    Dikande, Alain Moise; Ebobenow, Joseph

    2010-01-01

    A theoretical scheme for an experimental implementation involving bisolitonic matter waves from an attractive Bose-Einstein condensate, is considered within the framework of a non-perturbative approach to the associate Gross-Pitaevskii equation. The model consists of a single condensate subjected to an expulsive harmonic potential creating a double-condensate structure, and a gravitational potential that induces atomic exchanges between the two overlapping post condensates. Using a non-isospectral scattering transform method, exact expressions for the bright-matter-wave bisolitons are found in terms of double-lump envelopes with the co-propagating pulses displaying more or less pronounced differences in their widths and tails depending on the mass of atoms composing the condensate.

  11. 同步辐射高分辨率衍射光束线的设计%Beam line design for high-resolution diffraction at synchrotron radiation sources

    Institute of Scientific and Technical Information of China (English)

    U Pietsch; O H Seeck

    2007-01-01

    The general design of a high-resolution diffraction beamline at a third generation X-ray synchrotron radiation source is presented.For this,we introduce the basics of high resolution diffraction and the optical elements necessary to prepare a nearly parallel but intense X-ray beam with well-defined photon energy for high-resolution application.In particular,the function of double-crystal and four-bounced crystal monochromators is explained in terms of X-ray dynamical theory.As an example,we present the layout of the High Resolution Diffraction(HighRes)beamline at the new synchrotron radiation source PETRA Ⅲ in Hamburg(Germany)which will become operational in 2009.By optimizing the optical components.a resolution in q-space will be achieved down to △q=10-5 nm-1with micron beam size and a flux of more than 10 11 cts/s.%介绍了第三代同步辐射高分辨率X射线衍射光束线的总体设计.给出了高分辨率衍射的基本原理并描述了获得确定光子能量的近平行高强度X射线光束线所必需的光学元件.特别是用X射线动力学理论,解释了双晶及四次反射晶体单色器.作为一个实例,介绍了将于2009年开始在德国汉堡运行的一个新的同步辐射源PETRA Ⅲ的高分辨率衍射(HighRes)光束线的设置情况.通过优化光学部件,对微米尺寸光束,q 空间的分辨减小到△q=10-5 nm-1,光通量大于10 11cts/s.

  12. Atomic Oxygen (ATOX) simulation of Teflon FEP and Kapton H surfaces using a high intensity, low energy, mass selected, ion beam facility

    Science.gov (United States)

    Vered, R.; Grossman, E.; Lempert, G. D.; Lifshitz, Y.

    1994-01-01

    A high intensity (greater than 10(exp 15) ions/sq cm) low energy (down to 5 eV) mass selected ion beam (MSIB) facility was used to study the effects of ATOX on two polymers commonly used for space applications (Kapton H and Teflon FEP). The polymers were exposed to O(+) and Ne(+) fluences on 10(exp 15) - 10(exp 19) ions/sq cm, using 30eV ions. A variety of analytical methods were used to analyze the eroded surfaces including: (1) atomic force microscopy (AFM) for morphology measurements; (2) total mass loss measurements using a microbalance; (3) surface chemical composition using x-ray photoelectron spectroscopy (XPS), and (4) residual gas analysis (RGA) of the released gases during bombardment. The relative significance of the collisional and chemical degradation processes was evaluated by comparing the effects of Ne(+) and O(+) bombardment. For 30 eV ions it was found that the Kapton is eroded via chemical mechanisms while Teflon FEP is eroded via collisional mechanisms. AFM analysis was found very powerful in revealing the evolution of the damage from its initial atomic scale (roughness of approx. 1 nm) to its final microscopic scale (roughness greater than 1 micron). Both the surface morphology and the average roughness of the bombarded surfaces (averaged over 1 micron x 1 micron images by the system's computer) were determined for each sample. For 30 eV a non linear increase of the Kapton roughness with the O(+) fluence was discovered (a slow increase rate for fluences phi less than 5 x 10(exp 17) O(+)/sq cm, and a rapid increase rate for phi greater than 5 x 10(exp 17) O(+)/sq cm). Comparative studies on the same materials exposed to RF and DC oxygen plasmas indicate that the specific details of the erosion depend on the simulation facility emphasizing the advantages of the ion beam facility.

  13. Diffractive Physics

    CERN Document Server

    Martin, A D; Khoze, V A; Krauss, F; Ryskin, M G; Zapp, K

    2012-01-01

    `Soft' high-energy interactions are clearly important in pp collisions. Indeed, these events are dominant by many orders of magnitude, and about 40% are of diffractive origin; that is, due to elastic scattering or proton dissociation. Moreover, soft interactions unavoidably give an underlying component to the rare `hard' events, from which we hope to extract new physics. Here, we discuss how to quantify this contamination. First we present a brief introduction to diffraction. We emphasize the different treatment required for proton dissociation into low- and high-mass systems; the former requiring a multichannel eikonal approach, and the latter the computation of triple-Pomeron diagrams with multi-Pomeron corrections. Then we give an overview of the Pomeron, and explain how the QCD (BFKL-type) Pomeron is the natural object to continue from the `hard' to the `soft' domain. In this way we can obtain a partonic description of soft interactions. We introduce the so-called KMR model, based on this partonic approac...

  14. Electron-Beam Atomic Spectroscopy for In Situ Measurements of Melt Composition for Refractory Metals: Analysis of Fundamental Physics and Plasma Models

    Science.gov (United States)

    Gasper, Paul Joseph; Apelian, Diran

    2015-04-01

    Electron-beam (EB) melting is used for the processing of refractory metals, such as Ta, Nb, Mo, and W. These metals have high value and are critical to many industries, including the semiconductor, aerospace, and nuclear industries. EB melting can also purify secondary feedstock, enabling the recovery and recycling of these materials. Currently, there is no method for measuring melt composition in situ during EB melting. Optical emission spectroscopy of the plasma generated by EB impact with vapor above the melt, a technique here termed electron-beam atomic spectroscopy, can be used to measure melt composition in situ, allowing for analysis of melt dynamics, facilitating improvement of EB melting processes and aiding recycling and recovery of these critical and high-value metals. This paper reviews the physics of the plasma generation by EB impact by characterizing the densities and energies of electrons, ions, and neutrals, and describing the interactions between them. Then several plasma models are introduced and their suitability to this application analyzed. Lastly, a potential method for calibration-free composition measurement is described and the challenges for implementation addressed.

  15. Atomic and Nuclear Analytical Methods XRF, Mössbauer, XPS, NAA and Ion-Beam Spectroscopic Techniques

    CERN Document Server

    Verma, H R

    2007-01-01

    This book is a blend of analytical methods based on the phenomenon of atomic and nuclear physics. It comprises comprehensive presentations about X-ray Fluorescence (XRF), Mössbauer Spectroscopy (MS), X-ray Photoelectron Spectroscopy (XPS), Neutron- Activation Analysis (NAA), Particle Induced X-ray Emission Analysis (PIXE), Rutherford Backscattering Analysis (RBS), Elastic Recoil Detection (ERD), Nuclear Reaction Analysis (NRA), Particle Induced Gamma-ray Emission Analysis (PIGE), and Accelerator Mass Spectrometry (AMS). These techniques are commonly applied in the fields of medicine, biology, environmental studies, archaeology or geology et al. and pursued in major international research laboratories.

  16. A comment on the relation between diffraction and entropy

    CERN Document Server

    Baake, Michael

    2012-01-01

    Diffraction methods are used to detect atomic order in solids. While uniquely ergodic systems with pure point diffraction have zero entropy, the relation between diffraction and entropy is not as straightforward in general. In particular, there exist families of homometric systems, which are systems sharing the same diffraction, with varying entropy. We summarise the present state of understanding by several characteristic examples.

  17. Contactless friction and the {sup 3}He-{sup 4}He dimer. Studies with the atomic-beam spin-echo spectrometer; Kontaktlose Reibung und das {sup 3}He-{sup 4}He-Dimer. Untersuchungen mit dem Atomstrahlspinechospektrometer

    Energy Technology Data Exchange (ETDEWEB)

    Janke, Matthias

    2016-04-20

    In this thesis the time of flight resolved atomic beam spin echo method (SEToF) is applied to a {sup 3}He-beam for the first time and studied systematically. This method is shown to be superior to the usual atomic beam spin echo technique. With SEToF it is possible to almost completely remove unpolarized background and to reach a beam polarisation close to 100%. The SEToF technique is shown to be crucial for the first experimental proof of the existence of the {sup 3}He-{sup 4}He dimer. This dimer is the weakest bound van-der-Waals-molecule known to date. Furthermore, a drag force between an atom and a dielectric surface is detected originating from the fluctuating dipole moment of the atom. Not only the measured friction coefficients match their theoretical predictions perfectly, but our data also shows the correct temperature dependence. A great many technological renewals and improvements were installed in the apparatus during this thesis work. They have become necessary or sensible due to the relocation of the physics institute. A few of them are documented and motivated in this thesis.

  18. Ultracold ordered electron beam

    Energy Technology Data Exchange (ETDEWEB)

    Habs, D.; Kramp, J.; Krause, P.; Matl, K.; Neumann, R.; Schwalm, D.

    1988-01-01

    We have started an experimental program to develop an ultracold electron beam, which can be used together with a standard electron cooling device in the Heidelberg Test Storage Ring TSR. In contrast to the standard-type design using electron beam extraction beam extraction from a heated cathode, the ultracold beam is produced by photoemission of electrons from a cooled semiconductor crystal irradiated with an intense near-infrared laser light beam. Adiabatic acceleration is expected to provide ordering of the electron beam itself. Besides the cooling of ion beams to extremely low temperatures, with the aim of obtaining crystallization, the ultracold beam will constitute an excellent target for atomic physics experiments.

  19. The stereo-dynamics of collisional autoionization of ammonia by helium and neon metastable excited atoms through molecular beam experiments

    Energy Technology Data Exchange (ETDEWEB)

    Falcinelli, Stefano, E-mail: stefano.falcinelli@unipg.it; Vecchiocattivi, Franco [Department of Civil and Environmental Engineering, University of Perugia, Via G. Duranti 93, 06125 Perugia (Italy); Bartocci, Alessio; Cavalli, Simonetta; Pirani, Fernando [Department of Chemistry, Biology, and Biotechnology, University of Perugia, Via Elce di sotto 8, 06123 Perugia (Italy)

    2015-10-28

    A combined analysis of both new (energy spectra of emitted electrons) and previously published (ionization cross sections) experimental data, measured under the same conditions and concerning electronically excited lighter noble gas –NH{sub 3} collisional autoionization processes, is carried out. Such an analysis, performed by exploiting a formulation of the full potential energy surface both in the real and imaginary parts, provides direct information on energetics, structure, and lifetime of the intermediate collision complex over all the configuration space. The marked anisotropy in the attraction of the real part, driving the approach of reagents, and the selective role of the imaginary component, associated to the charge transfer coupling between entrance and exit channels, suggests that reactive events occur almost exclusively in the molecular hemisphere containing the nitrogen lone pair. Crucial details on the stereo-dynamics of elementary collisional autoionization processes are then obtained, in which the open shell nature of the disclosed ionic core of metastable atom plays a crucial role. The same analysis also suggests that the strength of the attraction and the anisotropy of the interaction increases regularly along the series Ne{sup *}({sup 3}P), He{sup *}({sup 3}S), He{sup *}({sup 1}S)–NH{sub 3}. These findings can be ascribed to the strong rise of the metastable atom electronic polarizability (deformability) along the series. The obtained results can stimulate state of the art ab initio calculations focused on specific features of the transition state (energetics, structure, lifetime, etc.) which can be crucial for a further improvement of the adopted treatment and to better understand the nature of the leading interaction components which are the same responsible for the formation of the intermolecular halogen and hydrogen bond.

  20. The stereo-dynamics of collisional autoionization of ammonia by helium and neon metastable excited atoms through molecular beam experiments.

    Science.gov (United States)

    Falcinelli, Stefano; Bartocci, Alessio; Cavalli, Simonetta; Pirani, Fernando; Vecchiocattivi, Franco

    2015-10-28

    A combined analysis of both new (energy spectra of emitted electrons) and previously published (ionization cross sections) experimental data, measured under the same conditions and concerning electronically excited lighter noble gas -NH3 collisional autoionization processes, is carried out. Such an analysis, performed by exploiting a formulation of the full potential energy surface both in the real and imaginary parts, provides direct information on energetics, structure, and lifetime of the intermediate collision complex over all the configuration space. The marked anisotropy in the attraction of the real part, driving the approach of reagents, and the selective role of the imaginary component, associated to the charge transfer coupling between entrance and exit channels, suggests that reactive events occur almost exclusively in the molecular hemisphere containing the nitrogen lone pair. Crucial details on the stereo-dynamics of elementary collisional autoionization processes are then obtained, in which the open shell nature of the disclosed ionic core of metastable atom plays a crucial role. The same analysis also suggests that the strength of the attraction and the anisotropy of the interaction increases regularly along the series Ne*((3)P), He*((3)S), He*((1)S)-NH3. These findings can be ascribed to the strong rise of the metastable atom electronic polarizability (deformability) along the series. The obtained results can stimulate state of the art ab initio calculations focused on specific features of the transition state (energetics, structure, lifetime, etc.) which can be crucial for a further improvement of the adopted treatment and to better understand the nature of the leading interaction components which are the same responsible for the formation of the intermolecular halogen and hydrogen bond.

  1. Free radical hydrogen atom abstraction from saturated hydrocarbons: A crossed-molecular-beams study of the reaction Cl + C{sub 3}H{sub 8} {yields} HCl + C{sub 3}H{sub 7}

    Energy Technology Data Exchange (ETDEWEB)

    Blank, D.A.; Hemmi, N.; Suits, A.G.; Lee, Y.T. [Lawrence Berkeley National Lab., CA (United States)

    1997-04-01

    The abstraction of hydrogen atoms from saturated hydrocarbons are reactions of fundamental importance in combustion as well as often being the rate limiting step in free radical substitution reactions. The authors have begun studying these reactions under single collision conditions using the crossed molecular beam technique on beamline 9.0.2.1, utilizing VUV undulator radiation to selectively ionize the scattered hydrocarbon free radical products (C{sub x}H{sub 2x+1}). The crossed molecular beam technique involves two reactant molecular beams fixed at 90{degrees}. The molecular beam sources are rotatable in the plane defined by the two beams. The scattered neutral products travel 12.0 cm where they are photoionized using the VUV undulator radiation, mass selected, and counted as a function of time. In the authors initial investigations they are using halogen atoms as protypical free radicals to abstract hydrogen atoms from small alkanes. Their first study has been looking at the reaction of Cl + propane {r_arrow} HCl + propyl radical. In their preliminary efforts the authors have measured the laboratory scattering angular distribution and time of flight spectra for the propyl radical products at collision energies of 9.6 kcal/mol and 14.9 kcal/mol.

  2. Multiple annular linear diffractive axicons.

    Science.gov (United States)

    Bialic, Emilie; de la Tocnaye, Jean-Louis de Bougrenet

    2011-04-01

    We propose a chromatic analysis of multiple annular linear diffractive axicons. Large aperture axicons are optical devices providing achromatic nondiffracting beams, with an extended depth of focus, when illuminated by a white light source, due to chromatic foci superimposition. Annular apertures introduce chromatic foci separation, and because chromatic aberrations result in focal segment axial shifts, polychromatic imaging properties are partially lost. We investigate here various design parameters that can be used to achieve color splitting, filtering, and combining using these properties. In order to improve the low-power efficiency of a single annular axicon, we suggest a spatial multiplexing of concentric annular axicons with different sizes and periods we call multiple annular aperture diffractive axicons (MALDAs). These are chosen to maintain focal depths while enabling color imaging with sufficient diffraction efficiency. Illustrations are given for binary phase diffractive axicons, considering technical aspects such as grating design wavelength and phase dependence due to the grating thickness.

  3. Determining the polarization state of an extreme ultraviolet free-electron laser beam using atomic circular dichroism.

    Science.gov (United States)

    Mazza, T; Ilchen, M; Rafipoor, A J; Callegari, C; Finetti, P; Plekan, O; Prince, K C; Richter, R; Danailov, M B; Demidovich, A; De Ninno, G; Grazioli, C; Ivanov, R; Mahne, N; Raimondi, L; Svetina, C; Avaldi, L; Bolognesi, P; Coreno, M; O'Keeffe, P; Di Fraia, M; Devetta, M; Ovcharenko, Y; Möller, Th; Lyamayev, V; Stienkemeier, F; Düsterer, S; Ueda, K; Costello, J T; Kazansky, A K; Kabachnik, N M; Meyer, M

    2014-04-16

    Ultrafast extreme ultraviolet and X-ray free-electron lasers are set to revolutionize many domains such as bio-photonics and materials science, in a manner similar to optical lasers over the past two decades. Although their number will grow steadily over the coming decade, their complete characterization remains an elusive goal. This represents a significant barrier to their wider adoption and hence to the full realization of their potential in modern photon sciences. Although a great deal of progress has been made on temporal characterization and wavefront measurements at ultrahigh extreme ultraviolet and X-ray intensities, only few, if any progress on accurately measuring other key parameters such as the state of polarization has emerged. Here we show that by combining ultra-short extreme ultraviolet free electron laser pulses from FERMI with near-infrared laser pulses, we can accurately measure the polarization state of a free electron laser beam in an elegant, non-invasive and straightforward manner using circular dichroism.

  4. High-contrast process using a positive-tone resist with antistatic coating and high-energy (100-keV) e-beam lithography for fabricating diffractive optical elements (DOE) on quartz

    Science.gov (United States)

    Poli, Louis C.; Kondek, Christine A.; Shoop, Barry L.; McLane, George F.

    1995-06-01

    Diffractive optical elements (DOE) are becoming important as optical signal processing elements in increasingly diverse applications. These elements, fabricated on quartz, may be used as phase shift type masks or as embedded components that implement a transfer function within a processing network. A process is under development for the fabrication of a DOE implementing a Jervis error diffusion kernel for research in half tone image processing. Dry etching is performed after lithography and pattern transfer through a nickel mask. This results in etched areal features on the substrate. An optical diffraction medium is thus created. Lithographic patterning is done by e-beam lithography (EBL) to realize small features, but also offers the important advantage of a large depth of field which relaxes the problem of complex surface topology. The recent availability of high energy (100 KeV) lithography tools provides a capability for precision overlay, small feature resolution, and enhanced image contrast through a lower induced proximity effect. Patterning by EBL on insulating substrates is complicated by the necessity of providing a vehicle for the avoidance of charge buildup on the surface. In a previously presented paper a methodology was shown for the use of TQV-501 (Nitto Chemical) antistatic compound as a final spin on film for use with PMMA and SAL-601 (Shipley). In this current work, a process is described using EBL and a high performance positive resist working with a final film layer of antistatic TQV-501 on a nickel coated wafer. The process may then be reapplied to realize additional lithographic levels in registration, for multilevel DOE components. High energy (100 KeV) EBL is used to provide high quality pattern definition. The e-beam sensitive resist, ZEP-320-37 (Nagase Chemical) in dilution, together with a top film layer of TQV-501 serves as a bilevel resist system and is used for patterning the desired image before definition of the nickel mask through

  5. Study of gamma-ray emission by proton beam interaction with injected Boron atoms for future medical imaging applications

    Science.gov (United States)

    Petringa, G.; Cirrone, G. A. P.; Caliri, C.; Cuttone, G.; Giuffrida, L.; Larosa, G.; Manna, R.; Manti, L.; Marchese, V.; Marchetta, C.; Margarone, D.; Milluzzo, G.; Picciotto, A.; Romano, F.; Romano, F. P.; Russo, A. D.; Russo, G.; Santonocito, D.; Scuderi, V.

    2017-03-01

    In this work an experimental and theoretical study of gamma-prompt emission has been carried out with the main aim being to understand to what extent this approach can be used during a treatment based on proton-boron fusion therapy. An experimental campaign, carried out with a high purity Germanium detector, has been performed to evaluate the gamma emission from two pure 11B and 10B targets. Furthermore, a set of analytical simulations, using the Talys nuclear reaction code has been performed and the calculated spectra compared with the experimental results. These comparisons allowed us to successfully validate Talys which was then used to estimate the gamma emission when a realistic Boron concentration was considered. Both simulations and experimental results suggest that the gamma emission is low at certain proton energies, thus in order to improve the imaging capabilities, while still maintaining the Boron therapeutic role, we propose the addition of natural Copper bound by a dipyrromethene, BodiPy, to boron atoms. Analytical simulations with Talys suggest that the characteristic spectrum of the copper prompt gamma-rays has several peaks in the energetic regions where the background is negligible.

  6. Ultra-fast Coherent Diffraction Imaging of Single Particles, Clusters and Biomolecules

    Energy Technology Data Exchange (ETDEWEB)

    Hajdu, J; Chapman, H

    2006-09-27

    Theoretical studies and simulations predict that with a very short and very intense coherent X-ray pulse a single diffraction pattern may be recorded from a large macromolecule, a virus, or a cell without the need for crystalline periodicity. Measurement of the over-sampled X-ray diffraction pattern permits phase retrieval and hence structure determination. Although individual samples will be destroyed by the very intense X-ray pulse, a three-dimensional data set could be assembled when copies of a reproducible sample are exposed to the beam one by one. The challenges in carrying out such an experiment requires an interdisciplinary approach, drawing upon structural biology, atomic and plasma physics, mathematics, statistics, and XFEL physics. The potential for breakthrough science in this area is great with impact not only in the biological areas but wherever structural information at or near atomic resolution on the nanoscale is valuable.

  7. Ultracold Ordered Electron Beam

    Science.gov (United States)

    Habs, D.; Kramp, J.; Krause, P.; Matl, K.; Neumann, R.; Schwalm, D.

    1988-01-01

    We have started an experimental program to develop an ultracold electron beam, which can be used together with a standard electron cooling device in the Heidelberg Test Storage Ring TSR. In contrast to the standard-type design using electron beam extraction from a heated cathode, the ultracold beam is produced by photoemission of electrons from a cooled semiconductor crystal irradiated with an intense near-infrared laser light beam. Adiabatic acceleration is expected to provide ordering of the electron beam itself. Besides the cooling of ion beams to extremely low temperatures, with the aim of obtaining crystallization, the ultracold beam will constitute an excellent target for atomic physics experiments.

  8. ARTICLE Crossed Beams Study on the Dynamics of CI Atom Reaction with Silane%交叉分子束研究氯原子与硅烷的反应动力学

    Institute of Scientific and Technical Information of China (English)

    肖重发; 沈关林; 王秀岩; 杨学明

    2011-01-01

    The dynamics of the C1+SiH4 reaction has been studied using the universal crossed molecular beam method.Angular resolved time-of-flight spectra have been measured for the channel SiH3Cl+H.Product angular distributions as well as energy distributions in the center-of-mass frame were determined for the channel.Experimental results show that the SiH3Cl product is mainly backward scattered relative to the Cl atom beam direction, suggesting that the channel takes place via a typical SN2 type reaction mechanism.

  9. In Situ Ramp Anneal X-ray Diffraction Study of Atomic Layer Deposited Ultrathin TaN and Ta 1-x Al x N y Films for Cu Diffusion Barrier Applications

    Energy Technology Data Exchange (ETDEWEB)

    Consiglio, S.; Dey, S.; Yu, K.; Tapily, K.; Clark, R. D.; Hasegawa, T.; Wajda, C. S.; Leusink, G. J.; Diebold, A. C.

    2016-01-01

    Ultrathin TaN and Ta1-xAlxNy films with x = 0.21 to 0.88 were deposited by atomic layer deposition (ALD) and evaluated for Cu diffusion barrier effectiveness compared to physical vapor deposition (PVD) grown TaN. Cu diffusion barrier effectiveness was investigated using in-situ ramp anneal synchrotron X-ray diffraction (XRD) on Cu/1.8 nm barrier/Si stacks. A Kissinger-like analysis was used to assess the kinetics of Cu3Si formation and determine the effective activation energy (Ea) for Cu silicidation. Compared to the stack with a PVD TaN barrier, the stacks with the ALD films exhibited a higher crystallization temperature (Tc) for Cu silicidation. The Ea values of Cu3Si formation for stacks with the ALD films were close to the reported value for grain boundary diffusion of Cu whereas the Ea of Cu3Si formation for the stack with PVD TaN is closer to the reported value for lattice diffusion. For 3 nm films, grazing incidence in-plane XRD showed evidence of nanocrystallites in an amorphous matrix with broad peaks corresponding to high density cubic phase for the ALD grown films and lower density hexagonal phase for the PVD grown film further elucidating the difference in initial failure mechanisms due to differences in barrier crystallinity and associated phase.

  10. Single-spin addressing in an atomic Mott insulator

    DEFF Research Database (Denmark)

    Weitenberg, Christof; Endres, Manuel; Sherson, Jacob

    2011-01-01

    with sub-diffraction-limited resolution, well below the lattice spacing. The Mott insulator provided us with a large two-dimensional array of perfectly arranged atoms, in which we created arbitrary spin patterns by sequentially addressing selected lattice sites after freezing out the atom distribution. We......Ultracold atoms in optical lattices provide a versatile tool with which to investigate fundamental properties of quantum many-body systems. In particular, the high degree of control of experimental parameters has allowed the study of many interesting phenomena, such as quantum phase transitions...... and quantum spin dynamics. Here we demonstrate how such control can be implemented at the most fundamental level of a single spin at a specific site of an optical lattice. Using a tightly focused laser beam together with a microwave field, we were able to flip the spin of individual atoms in a Mott insulator...

  11. Transverse electron beam diagnostics at REGAE

    Energy Technology Data Exchange (ETDEWEB)

    Bayesteh, Shima

    2014-12-15

    The use of high-intensity electron and X-ray pulsed sources allows for the direct observation of atomic motions as they occur. While the production of such high coherent, brilliant, short X-ray pulses requires large-scale and costly accelerator facilities, it is feasible to employ a high-intensity source of electrons by exploiting a more compact design. The Relativistic Electron Gun for Atomic Exploration (REGAE) facility is a small linear accelerator at DESY, Hamburg, equipped with a photocathode radio frequency (RF) gun that produces relativistic ultra-short (<100 fs), low charge (<1 pC) electron bunches of high coherence. By means of time-resolved diffraction experiments, such an electron source can probe ultrafast laser-induced atomic structural changes that occur with a temporal resolution of ∝100 fs. A comprehensive characterization of the electron beam, for every pulse, is of fundamental importance to study the atomic motions with the desired resolution and quality. This thesis reports on the transversal diagnostics of the electron beam with an emphasis on a scintillator-based beam profile monitor. The diagnostics is capable of evaluating the beam parameters such as charge, energy, energy spread and transverse profile, at very low charges and on a shot-to-shot basis. A full characterization of the scintillator's emission, the optical setup and the detector (camera) of the profile monitor is presented, from which an absolute charge calibration of the system is derived. The profile monitor is specially developed to accommodate more applications, such as dark current suppression, overlapping the electron probe and the laser pump within 1 ns accuracy, as well as charge and transverse emittance measurements. For the determination of the transverse emittance two techniques were applied. The first one introduces a new method that exploits a diffraction pattern to measure the emittance, while the second one is based on a version of the Pepper-pot technique. A

  12. Effect of structural in-depth heterogeneities on electrical properties of Pb(Zr0.52Ti0.48) O3 thin films as revealed by nano-beam X-ray diffraction

    Science.gov (United States)

    Vaxelaire, N.; Kovacova, V.; Bernasconi, A.; Le Rhun, G.; Alvarez-Murga, M.; Vaughan, G. B. M.; Defay, E.; Gergaud, P.

    2016-09-01

    A direct quantification of a structural in-depth composition in the lead zirconate titanate Pb(Zr,Ti)O3 thin films of morphotropic composition has been conducted using the newly available X-ray nano-pencil beam (i.e., beam size of 100 nm × 1 μm) diffraction approach. We tested two samples with different Zr/Ti chemical gradients. Here, we demonstrate the presence of a significant microstructural gradient between the rhombohedral and tetragonal phases through PbZrxTi1-xO3 (PZT) films with a 100 nm in-depth resolution. The phase gradient extends over around 350 nm, and it is repeated through the PZT film three times, which corresponds to the number of thermal annealings. Moreover, this microstructural gradient is in agreement with the Zr/Ti chemical gradient observed by the secondary ion mass spectroscopy (SIMS). Indeed, the quantity of tetragonal phases rises in the Ti-rich zones as revealed by SIMS, and the quantity of rhombohedral phases rises in the Zr-rich zones. We also demonstrated a huge difference in the in-depth phase variation between the two tested samples. The gradient free sample still contains 4.7% of phase variation through the film and the amplified gradient contains 9.6% of phase variation through the film. Knowing that the gradient free sample shows better electric and piezoelectric coefficients, one can draw a correlation between the chemical composition, crystallographic homogeneity, and electro-mechanical properties of the film. The more close the film is to the morphotropic composition and the more it is crystallographically homogeneous, the higher the piezoelectric coefficients of the PZT are. Finally, the adequate knowledge of phase variation and its relation to the fabrication technique are crucial for the enhancement of the PZT electro-mechanical properties. Our methodology and findings open up new perspectives in establishing a relevant quantitative feedback to reach an ultimate electro-mechanical coupling in the sol-gel PZT thin films.

  13. Characterization of the Plasma Edge for Technique of Atomic Helium Beam in the CIEMAT Fusion Device; Caracterizacion del Borde del Plasma del Dispositivo de Fusion TJ-II del CIEMAT mediante el Diagnostico del Haz Supersonico de Helio

    Energy Technology Data Exchange (ETDEWEB)

    Hidalgo, A.

    2003-07-01

    In this report, the measurement of Electron Temperature and Density in the Boundary Plasma of TJ-II with a Supersonic Helium Beam Diagnostic and work devoted to the upgrading of this technique are described. Also, simulations of Laser Induced Fluorescence (LIF) studies of level populations of electronically excited He atoms are shown. This last technique is now being installed in the CIEMAT fusion device. (Author ) 36 refs.

  14. Atom interferometry experiments with lithium. Accurate measurement of the electric polarizability; Experiences d'interferometrie atomique avec le lithium. Mesure de precision de la polarisabilite electrique

    Energy Technology Data Exchange (ETDEWEB)

    Miffre, A

    2005-06-15

    Atom interferometers are very sensitive tools to make precise measurements of physical quantities. This study presents a measurement of the static electric polarizability of lithium by atom interferometry. Our result, {alpha} = (24.33 {+-} 0.16)*10{sup -30} m{sup 3}, improves by a factor 3 the most accurate measurements of this quantity. This work describes the tuning and the operation of a Mach-Zehnder atom interferometer in detail. The two interfering arms are separated by the elastic diffraction of the atomic wave by a laser standing wave, almost resonant with the first resonance transition of lithium atom. A set of experimental techniques, often complicated to implement, is necessary to build the experimental set-up. After a detailed study of the atom source (a supersonic beam of lithium seeded in argon), we present our experimental atom signals which exhibit a very high fringe visibility, up to 84.5 % for first order diffraction. A wide variety of signals has been observed by diffraction of the bosonic isotope at higher diffraction orders and by diffraction of the fermionic less abundant isotope. The quality of these signals is then used to do very accurate phase measurements. A first experiment investigates how the atom interferometer signals are modified by a magnetic field gradient. An absolute measurement of lithium atom electric polarizability is then achieved by applying a static electric field on one of the two interfering arms, separated by only 90 micrometers. The construction of such a capacitor, its alignment in the experimental set-up and its operation are fully detailed.We obtain a very accurate phase measurement of the induced Lo Surdo - Stark phase shift (0.07 % precision). For this first measurement, the final uncertainty on the electric polarizability of lithium is only 0.66 %, and is dominated by the uncertainty on the atom beam mean velocity, so that a further reduction of the uncertainty can be expected. (author)

  15. Combined crossed molecular beam and ab initio investigation of the multichannel reaction of boron monoxide (BO; X2Σ+) with Propylene (CH3CHCH2; X1A'): competing atomic hydrogen and methyl loss pathways.

    Science.gov (United States)

    Maity, Surajit; Dangi, Beni B; Parker, Dorian S N; Kaiser, Ralf I; An, Yi; Sun, Bing-Jian; Chang, A H H

    2014-10-16

    The reaction dynamics of boron monoxide ((11)BO; X(2)Σ(+)) with propylene (CH(3)CHCH(2); X(1)A') were investigated under single collision conditions at a collision energy of 22.5 ± 1.3 kJ mol(-1). The crossed molecular beam investigation combined with ab initio electronic structure and statistical (RRKM) calculations reveals that the reaction follows indirect scattering dynamics and proceeds via the barrierless addition of boron monoxide radical with its radical center located at the boron atom. This addition takes place to either the terminal carbon atom (C1) and/or the central carbon atom (C2) of propylene reactant forming (11)BOC(3)H(6) intermediate(s). The long-lived (11)BOC(3)H(6) doublet intermediate(s) underwent unimolecular decomposition involving at least three competing reaction mechanisms via an atomic hydrogen loss from the vinyl group, an atomic hydrogen loss from the methyl group, and a methyl group elimination to form cis-/trans-1-propenyl-oxo-borane (CH(3)CHCH(11)BO), 3-propenyl-oxo-borane (CH(2)CHCH(2)(11)BO), and ethenyl-oxo-borane (CH(2)CH(11)BO), respectively. Utilizing partially deuterated propylene (CD(3)CHCH(2) and CH(3)CDCD(2)), we reveal that the loss of a vinyl hydrogen atom is the dominant hydrogen elimination pathway (85 ± 10%) forming cis-/trans-1-propenyl-oxo-borane, compared to the loss of a methyl hydrogen atom (15 ± 10%) leading to 3-propenyl-oxo-borane. The branching ratios for an atomic hydrogen loss from the vinyl group, an atomic hydrogen loss from the methyl group, and a methyl group loss are experimentally derived to be 26 ± 8%:5 ± 3%:69 ± 15%, respectively; these data correlate nicely with the branching ratios calculated via RRKM theory of 19%:5%:75%, respectively.

  16. High-resolution structure of viruses from random diffraction snapshots

    CERN Document Server

    Hosseinizadeh, A; Dashti, A; Fung, R; D'Souza, R M; Ourmazd, A

    2014-01-01

    The advent of the X-ray Free Electron Laser (XFEL) has made it possible to record diffraction snapshots of biological entities injected into the X-ray beam before the onset of radiation damage. Algorithmic means must then be used to determine the snapshot orientations and thence the three-dimensional structure of the object. Existing Bayesian approaches are limited in reconstruction resolution typically to 1/10 of the object diameter, with the computational expense increasing as the eighth power of the ratio of diameter to resolution. We present an approach capable of exploiting object symmetries to recover three-dimensional structure to high resolution, and thus reconstruct the structure of the satellite tobacco necrosis virus to atomic level. Our approach offers the highest reconstruction resolution for XFEL snapshots to date, and provides a potentially powerful alternative route for analysis of data from crystalline and nanocrystalline objects.

  17. Facing the phase problem in Coherent Diffractive Imaging via Memetic Algorithms

    Science.gov (United States)

    Colombo, Alessandro; Galli, Davide Emilio; de Caro, Liberato; Scattarella, Francesco; Carlino, Elvio

    2017-02-01

    Coherent Diffractive Imaging is a lensless technique that allows imaging of matter at a spatial resolution not limited by lens aberrations. This technique exploits the measured diffraction pattern of a coherent beam scattered by periodic and non–periodic objects to retrieve spatial information. The diffracted intensity, for weak–scattering objects, is proportional to the modulus of the Fourier Transform of the object scattering function. Any phase information, needed to retrieve its scattering function, has to be retrieved by means of suitable algorithms. Here we present a new approach, based on a memetic algorithm, i.e. a hybrid genetic algorithm, to face the phase problem, which exploits the synergy of deterministic and stochastic optimization methods. The new approach has been tested on simulated data and applied to the phasing of transmission electron microscopy coherent electron diffraction data of a SrTiO3 sample. We have been able to quantitatively retrieve the projected atomic potential, and also image the oxygen columns, which are not directly visible in the relevant high-resolution transmission electron microscopy images. Our approach proves to be a new powerful tool for the study of matter at atomic resolution and opens new perspectives in those applications in which effective phase retrieval is necessary.

  18. X-ray holography with atomic resolution

    Science.gov (United States)

    Tegze, Miklós; Faigel, Gyula

    1996-03-01

    DIFFRACTION methods for crystallographic structure determination suffer from the so-called 'phase problem'; a diffraction pattern provides intensity but not phase information for the scattered beams, and therefore cannot be uniquely inverted to obtain the crystal structure of a sample. Holographic methods1, on the other hand, offer a means of extracting both intensity and phase information. To be useful for crystallographic applications, holography must be implemented with radiation of sufficiently small wavelength to resolve atomic-scale features2. One method, electron-emission holography3-9, uses electron waves and is a powerful tool for studying surface structure; but it cannot image the internal structure of solids because of complications arising from the highly anisotropic nature of electron scattering processes. A proposed alternative method uses X-rays2,10-13, which scatter more isotropically than electrons. Here we demonstrate the efficacy of atomic-scale X-ray holography by obtaining direct images of the three-dimensional arrangement of strontium atoms in the cubic perovskite SrTiO3. With more intense synchrotron sources for illumination, and with the development of improved X-ray detectors, X-ray holography should become a powerful general technique for unambiguous structure determination in condensed matter systems.

  19. X-ray diffraction imaging of material microstructures

    KAUST Repository

    Varga, Laszlo

    2016-10-20

    Various examples are provided for x-ray imaging of the microstructure of materials. In one example, a system for non-destructive material testing includes an x-ray source configured to generate a beam spot on a test item; a grid detector configured to receive x- rays diffracted from the test object; and a computing device configured to determine a microstructure image based at least in part upon a diffraction pattern of the x-rays diffracted from the test object. In another example, a method for determining a microstructure of a material includes illuminating a beam spot on the material with a beam of incident x-rays; detecting, with a grid detector, x-rays diffracted from the material; and determining, by a computing device, a microstructure image based at least in part upon a diffraction pattern of the x-rays diffracted from the material.

  20. Atom probe tomography today

    Directory of Open Access Journals (Sweden)

    Alfred Cerezo

    2007-12-01

    Full Text Available This review aims to describe and illustrate the advances in the application of atom probe tomography that have been made possible by recent developments, particularly in specimen preparation techniques (using dual-beam focused-ion beam instruments but also of the more routine use of laser pulsing. The combination of these two developments now permits atomic-scale investigation of site-specific regions within engineering alloys (e.g. at grain boundaries and in the vicinity of cracks and also the atomic-level characterization of interfaces in multilayers, oxide films, and semiconductor materials and devices.

  1. Diffraction coherence in optics

    CERN Document Server

    Françon, M; Green, L L

    2013-01-01

    Diffraction: Coherence in Optics presents a detailed account of the course on Fraunhofer diffraction phenomena, studied at the Faculty of Science in Paris. The publication first elaborates on Huygens' principle and diffraction phenomena for a monochromatic point source and diffraction by an aperture of simple form. Discussions focus on diffraction at infinity and at a finite distance, simplified expressions for the field, calculation of the path difference, diffraction by a rectangular aperture, narrow slit, and circular aperture, and distribution of luminous flux in the airy spot. The book th

  2. Use of Reciprocal Lattice Layer Spacing in Electron Backscatter Diffraction Pattern Analysis

    Energy Technology Data Exchange (ETDEWEB)

    Eades, J.A.; Michael, J.R.

    1999-05-10

    In the scanning electron microscope (SEM), using electron backscattered diffraction (EBSD), it is possible to measure the spacing of the layers in the reciprocal lattice. These values are of great use in confirming the identification of phases. The technique derives the layer spacing from the HOLZ rings which appear in patterns from many materials. The method adapts results from convergent-beam electron diffraction (CBED) in the transmission electron microscope (TEM). For many materials the measured layer spacing compares well with the calculated layer spacing. A noted exception is for higher atomic number materials. In these cases an extrapolation procedure is described that requires layer spacing measurements at a range of accelerating voltages. This procedure is shown to improves the accuracy of the technique significantly. The application of layer spacing measurements in EBSD is shown to be of use for the analysis of two polytypes of SiC.

  3. Uniting Electron Crystallography and Powder Diffraction

    CERN Document Server

    Shankland, Kenneth; Meshi, Louisa; Avilov, Anatoly; David, William

    2012-01-01

    The polycrystalline and nanocrystalline states play an increasingly important role in exploiting the properties of materials, encompassing applications as diverse as pharmaceuticals, catalysts, solar cells and energy storage. A knowledge of the three-dimensional atomic and molecular structure of materials is essential for understanding and controlling their properties, yet traditional single-crystal X-ray diffraction methods lose their power when only polycrystalline and nanocrystalline samples are available. It is here that powder diffraction and single-crystal electron diffraction techniques take over, substantially extending the range of applicability of the crystallographic principles of structure determination.  This volume, a collection of teaching contributions presented at the Crystallographic Course in Erice in 2011, clearly describes the fundamentals and the state-of-the-art of powder diffraction and electron diffraction methods in materials characterisation, encompassing a diverse range of discipl...

  4. Diffraction efficiency enhancement of femtosecond laser-engraved diffraction gratings due to CO{sub 2} laser polishing

    Energy Technology Data Exchange (ETDEWEB)

    Choi, Hun-Kook [Gwangju Institute of Science and Technology, Gwangju (Korea, Republic of); Chosun University, Gwangju (Korea, Republic of); Jung, Deok; Sohn, Ik-Bu; Noh, Young-Chul; Lee, Yong-Tak [Gwangju Institute of Science and Technology, Gwangju (Korea, Republic of); Kim, Jin-Tae [Chosun University, Gwangju (Korea, Republic of); Ahsan, Shamim [Khulna University, Khulna (Bangladesh)

    2014-11-15

    This research demonstrates laser-assisted fabrication of high-efficiency diffraction gratings in fused-silica glass samples. Initially, femtosecond laser pulses are used to engrave diffraction gratings on the glass surfaces. Then, these micro-patterned glass samples undergo CO{sub 2} laser polishing process. unpolished diffraction gratings encoded in the glass samples show an overall diffraction efficiency of 18.1%. diffraction gratings imprinted on the glass samples and then polished four times by using a CO{sub 2} laser beam attain a diffraction efficiency of 32.7%. We also investigate the diffraction patterns of the diffraction gratings encoded on fused-silica glass surfaces. The proposed CO{sub 2} laser polishing technique shows great potential in patterning high-efficiency diffraction gratings on the surfaces of various transparent materials.

  5. X-Ray Diffraction.

    Science.gov (United States)

    Smith, D. K.; Smith, K. L.

    1980-01-01

    Reviews applications in research and analytical characterization of compounds and materials in the field of X-ray diffraction, emphasizing new developments in applications and instrumentation in both single crystal and powder diffraction. Cites 414 references. (CS)

  6. GENERALIZED FRESNEL DIFFRACTION INTEGRAL AND ITS APPLICATIONS

    Institute of Scientific and Technical Information of China (English)

    YANG JUN; FAN DIAN-YUAN; WANG SHI-JI; GU YUAN

    2000-01-01

    Within the generalized definition of ABCDGH matrices, the conventional ABCDGH diffraction integral is ex-tended for a misaligned complex paraxial system with a curved optical axis. On this basis the transformation lawfor Gaussian-Schell model beams through an ABCDGH systems is derived, the propagation behavior of the mutualcoherence function through ABCDGH systems in the presence of random media is investigated as well.

  7. A slow gravity compensated atom laser

    DEFF Research Database (Denmark)

    Kleine Büning, G.; Will, J.; Ertmer, W.

    2010-01-01

    We report on a slow guided atom laser beam outcoupled from a Bose–Einstein condensate of 87Rb atoms in a hybrid trap. The acceleration of the atom laser beam can be controlled by compensating the gravitational acceleration and we reach residual accelerations as low as 0.0027 g. The outcoupling me...

  8. Plasma For-Injector of Separable Material Based on the Beam-Plasma Discharge for Ion-Atomic Separation Technologies. Conception

    OpenAIRE

    Skibenko, E. I.; Yu. V. Kovtun; V.B. Yuferov

    2010-01-01

    In the paper, the functional definition of a plasma for-injector of separable material is presented, and the requirements to it are formulated. The version of a device for the material separation into elements based on the beam-plasma discharge is under consideration. The dimensions of a pilot separating device are determined. The following quantities are estimated: the particle concentration per unit length of the separating device, effective length of the beam-plasma interaction (BPI) withi...

  9. Robustness via Diffractal Architectures

    CERN Document Server

    Moocarme, Matthew

    2015-01-01

    When plane waves diffract through fractal-patterned apertures, the resulting far-field profiles or diffractals also exhibit iterated, self-similar features. Here we show that this specific architecture enables robust signal processing and spatial multiplexing: arbitrary parts of a diffractal contain sufficient information to recreate the entire original sparse signal.

  10. Diffractive production of mesons

    Directory of Open Access Journals (Sweden)

    Schicker Rainer

    2014-01-01

    Full Text Available The interest in the study of diffractive meson production is discussed. The description of diffraction within Regge phenomenology is presented, and the QCD-based understanding of diffractive processes is given. Central production is reviewed, and the corresponding main results from the COMPASS experiment and from the experiments at the ISR, RHIC, TEVATRON and LHC collider are summarised.

  11. Diffractive production of mesons

    CERN Document Server

    Schicker, R

    2014-01-01

    The interest in the study of diffractive meson production is discussed. The description of diffraction within Regge phenomenology is presented, and the QCD-based understanding of diffractive processes is given. Central production is reviewed, and the corresponding main results from the COMPASS experiment and from the experiments at the ISR, RHIC, TEVATRON and LHC collider are summarised.

  12. Crossed-beam reaction of carbon atoms with hydrocarbon molecules. V. Chemical dynamics of n-C4H3 formation from reaction of C(3Pj) with allene, H2CCCH2(X 1A1)

    Science.gov (United States)

    Kaiser, R. I.; Mebel, A. M.; Chang, A. H. H.; Lin, S. H.; Lee, Y. T.

    1999-06-01

    The crossed molecular beams technique was employed to investigate the reaction between ground state carbon atoms, C(3Pj), and allene, H2CCCH2(X 1A1), at two averaged collision energies of 19.6 and 38.8 kJ mol-1. Product angular distributions and time-of-flight spectra of C4H3 were recorded. Forward-convolution fitting of the data yields weakly polarized center-of-mass angular flux distributions isotropic at lower, but forward scattered with respect to the carbon beam at a higher collision energy. The maximum translational energy release and the angular distributions combined with ab initio and RRKM calculations are consistent with the formation of the n-C4H3 radical in its electronic ground state. The channel to the i-C4H3 isomer contributes less than 1.5%. Reaction dynamics inferred from the experimental data indicate that the carbon atom attacks the π-orbitals of the allenic carbon-carbon double bond barrierless via a loose, reactant-like transition state located at the centrifugal barrier. The initially formed cyclopropylidene derivative rotates in a plane almost perpendicular to the total angular momentum vector around its C-axis and undergoes ring opening to triplet butatriene. At higher collision energy, the butatriene complex decomposes within 0.6 ps via hydrogen emission to form the n-C4H3 isomer and atomic hydrogen through an exit transition state located 9.2 kJ mol-1 above the products. The explicit identification of the n-C4H3 radical under single collision represents a further example of a carbon-hydrogen exchange in reactions of ground state carbon atoms with unsaturated hydrocarbons. This channel opens a barrierless route to synthesize extremely reactive hydrocarbon radicals in combustion processes, interstellar chemistry, and hydrocarbon-rich atmospheres of Jupiter, Saturn, Titan, as well as Triton.

  13. Diffraction radiation from relativistic heavy ions

    Science.gov (United States)

    Potylitsyna, N. A.

    2001-01-01

    In recent years, the relativistic heavy ion beams at new accelerator facilities are allowed to obtain some new interesting results (see, for instance, Datz et al., Phys. Rev. Lett. 79 (18) (1997) 3355; Ladyrin et al., Nucl. Instr. and Meth. A 404 (1998) 129). The problem of non-destructive heavy ion beam diagnostics at these accelerators is highly pressing. The authors of the papers (Rule et al., Proceedings of the Seventh Beam Instrumentation Workshop, Argonne IL, AIP Conference Proceedings, Vol. 390, NY, 1997; Castellano, Nucl. Instr. and Meth. A 394 (1997) 275) suggested to use diffraction radiation (DR) appearing when a charge moves close to a conducting surface (Bolotovskii and Voskresenskii, Sov. Phys. Usp. 9 (1966) 73) for non-destructive electron beam diagnostics. The DR characteristics are defined by both Lorentz-factor and the particle charge, and do not depend on its mass. The estimation of feasibility of using DR for relativistic ion beam diagnostics is undoubtedly interesting.

  14. Development and characterization of electron sources for diffraction applications

    Energy Technology Data Exchange (ETDEWEB)

    Casandruc, Albert

    2015-12-15

    The dream to control chemical reactions that are essential to life is now closer than ever to gratify. Recent scientific progress has made it possible to investigate phenomena and processes which deploy at the angstroms scale and at rates on the order femtoseconds. Techniques such as Ultrafast Electron Diffraction (UED) are currently able to reveal the spatial atomic configuration of systems with unit cell sizes on the order of a few nanometers with about 100 femtosecond temporal resolution. Still, major advances are needed for structural interrogation of biological systems like protein crystals, which have unit cell sizes of 10 nanometers or larger, and sample sizes of less than one micrometer. For such samples, the performance of these electron-based techniques is now limited by the quality, in particular the brightness, of the electron source. The current Ph.D. work represents a contribution towards the development and the characterization of electron sources which are essential to static and time-resolved electron diffraction techniques. The focus was on electron source fabrication and electron beam characterization measurements, using the solenoid and the aperture scan techniques, but also on the development and maintenance of the relevant experimental setups. As a result, new experimental facilities are now available in the group and, at the same time, novel concepts for generating electron beams for electron diffraction applications have been developed. In terms of existing electron sources, the capability to trigger and detect field emission from single double-gated field emitter Mo tips was successfully proven. These sharp emitter tips promise high brightness electron beams, but for investigating individual such structures, new engineering was needed. Secondly, the influence of the surface electric field on electron beam properties has been systematically performed for flat Mo photocathodes. This study is very valuable especially for state

  15. Dielectric barrier discharge source for supersonic beams

    Energy Technology Data Exchange (ETDEWEB)

    Luria, K.; Lavie, N.; Even, U. [Sackler School of Chemistry, Tel Aviv University, Tel Aviv 69978 (Israel)

    2009-10-15

    We present a new excitation source for pulsed supersonic beams. The excitation is based on dielectric barrier discharge in the beam. It produces cold beams of metastable atoms, dissociated neutral atoms from molecular precursors, and both positive and negative ions with high efficiency and reliability.

  16. Atomic-layer engineering of oxide superconductors

    Science.gov (United States)

    Bollinger, A. T.; Eckstein, J. N.; Dubuis, G.; Pavuna, D.; Božović, I.

    2012-02-01

    Molecular beam epitaxy technique has enabled synthesis of atomically smooth thin films, multilayers, and superlattices of cuprates and other complex oxides. Such heterostructures show high temperature superconductivity and enable novel experiments that probe the basic physics of this phenomenon. For example, it was established that high temperature superconductivity and anti-ferromagnetic phases separate on Ångström scale, while the pseudo-gap state apparently mixes with high temperature superconductivity over an anomalously large length scale (the "Giant Proximity Effect"). We review some recent experiments on such films and superlattices, including X-ray diffraction, atomic force microscopy, angle-resolved time of flight ion scattering and recoil spectroscopy, transport measurements, highresolution transmission electron microscopy, resonant X-ray scattering, low-energy muon spin resonance, and ultrafast photo-induced reflection high energy electron diffraction. The results include an unambiguous demonstration of strong coupling of in-plane charge excitations to out-of-plane lattice vibrations, a discovery of interface high temperature superconductivity that occurs in a single CuO2 plane, evidence for local pairs, and establishing tight limits on the temperature range of superconducting fluctuations.

  17. Atomic-Layer Engineering of Oxide Superconductors

    Energy Technology Data Exchange (ETDEWEB)

    Bozovic I.; Bollinger, A.T.; Eckstein, J.N.; Dubuis, G.; Pavuna, D.

    2012-03-01

    Molecular beam epitaxy technique has enabled synthesis of atomically smooth thin films, multilayers, and superlattices of cuprates and other complex oxides. Such heterostructures show high temperature superconductivity and enable novel experiments that probe the basic physics of this phenomenon. For example, it was established that high temperature superconductivity and anti-ferromagnetic phases separate on Angstrom scale, while the pseudo-gap state apparently mixes with high temperature superconductivity over an anomalously large length scale (the 'Giant Proximity Effect'). We review some recent experiments on such films and superlattices, including X-ray diffraction, atomic force microscopy, angle-resolved time of flight ion scattering and recoil spectroscopy, transport measurements, high resolution transmission electron microscopy, resonant X-ray scattering, low-energy muon spin resonance, and ultrafast photo-induced reflection high energy electron diffraction. The results include an unambiguous demonstration of strong coupling of in-plane charge excitations to out-of-plane lattice vibrations, a discovery of interface high temperature superconductivity that occurs in a single CuO{sub 2} plane, evidence for local pairs, and establishing tight limits on the temperature range of superconducting fluctuations.

  18. Glancing angle x-ray diffraction : A different approach

    NARCIS (Netherlands)

    Brussel, B.A. van; Hosson, J.Th.M. De

    1994-01-01

    This letter describes a novel technique of diffracted beam glancing angle x-ray diffraction by which depth profiles of stresses and transformed phases in structures like implanted materials can be determined. An important feature is that this method may be applied successfully in a standard powder d

  19. Formation of uniform fringe pattern free from diffraction noise at LDA measurement volume using holographic imaging configuration

    Science.gov (United States)

    Ghosh, Abhijit; Nirala, A. K.

    2016-05-01

    In the present study we have proposed a technique for improving fringe quality at laser Doppler anemometry measurement volume in real time using single hololens imaging configuration over conventional imaging configuration with Gaussian beam optics. In order to remove interference fringe gradients as well as higher order diffraction noise formed at measurement volume in the former approach, a combined hololens imaging system has also been proposed. For qualitative as well as quantitative analysis of fringes formed at measurement volume, atomic force microscopy (AFM) analysis has been performed.

  20. Atomic physics

    Energy Technology Data Exchange (ETDEWEB)

    Livingston, A.E.; Kukla, K.; Cheng, S. [Univ. of Toledo, OH (United States)] [and others

    1995-08-01

    In a collaboration with the Atomic Physics group at Argonne and the University of Toledo, the Atomic Physics group at the University of Notre Dame is measuring the fine structure transition energies in highly-charged lithium-like and helium-like ions using beam-foil spectroscopy. Precise measurements of 2s-2p transition energies in simple (few-electron) atomic systems provide stringent tests of several classes of current atomic- structure calculations. Analyses of measurements in helium-like Ar{sup 16+} have been completed, and the results submitted for publication. A current goal is to measure the 1s2s{sup 3}S{sub 1} - 1s2p{sup 3}P{sub 0} transition wavelength in helium-like Ni{sup 26+}. Measurements of the 1s2s{sup 2}S{sub 1/2} - 1s2p{sup 2}P{sub 1/2,3/2} transition wavelengths in lithium-like Kr{sup 33+} is planned. Wavelength and lifetime measurements in copper-like U{sup 63+} are also expected to be initiated. The group is also participating in measurements of forbidden transitions in helium-like ions. A measurement of the lifetime of the 1s2s{sup 3}S{sub 1} state in Kr{sup 34+} was published recently. In a collaboration including P. Mokler of GSI, Darmstadt, measurements have been made of the spectral distribution of the 2E1 decay continuum in helium-like Kr{sup 34+}. Initial results have been reported and further measurements are planned.