WorldWideScience

Sample records for atmospheric pollutants derived

  1. Atmospheric pollution

    International Nuclear Information System (INIS)

    Lambrozo, J.; Guillossou, G.

    2008-01-01

    The atmosphere is the reservoir of numerous pollutants (nitrogen oxides, sulfur oxides, carbon oxides, particulates, volatile organic compounds, polycyclic aromatic hydrocarbons) from natural origin or anthropogenic origin ( industry, transport, agriculture, district heating). With epidemiologic studies the atmospheric pollution is associated with an increase of respiratory and cardiovascular diseases. At the european level, the technological progress, the legislation have allowed a reduction of pollutant emissions, however these efforts have to be continued because the sanitary impact of atmospheric pollution must not be underestimated, even if the risks appear less important that these ones in relation with tobacco, inside pollution or others factors of cardiovascular risks. Indeed, on these last factors an individual action is possible for the exposure to air pollution people have no control. (N.C.)

  2. mathematical modelling of atmospheric dispersion of pollutants

    International Nuclear Information System (INIS)

    Mohamed, M.E.

    2002-01-01

    the main objectives of this thesis are dealing with environmental problems adopting mathematical techniques. in this respect, atmospheric dispersion processes have been investigated by improving the analytical models to realize the realistic physical phenomena. to achieve these aims, the skeleton of this work contained both mathematical and environmental topics,performed in six chapters. in chapter one we presented a comprehensive review study of most important informations related to our work such as thermal stability , plume rise, inversion, advection , dispersion of pollutants, gaussian plume models dealing with both radioactive and industrial contaminants. chapter two deals with estimating the decay distance as well as the decay time of either industrial or radioactive airborne pollutant. further, highly turbulent atmosphere has been investigated as a special case in the three main thermal stability classes namely, neutral, stable, and unstable atmosphere. chapter three is concerned with obtaining maximum ground level concentration of air pollutant. the variable effective height of pollutants has been considered throughout the mathematical treatment. as a special case the constancy of effective height has been derived mathematically and the maximum ground level concentration as well as its location have been established

  3. Mobile Instruments Measure Atmospheric Pollutants

    Science.gov (United States)

    2009-01-01

    As a part of NASA's active research of the Earth s atmosphere, which has included missions such as the Atmospheric Laboratory of Applications and Science (ATLAS, launched in 1992) and the Total Ozone Mapping Spectrometer (TOMS, launched on the Earth Probe satellite in 1996), the Agency also performs ground-based air pollution research. The ability to measure trace amounts of airborne pollutants precisely and quickly is important for determining natural patterns and human effects on global warming and air pollution, but until recent advances in field-grade spectroscopic instrumentation, this rapid, accurate data collection was limited and extremely difficult. In order to understand causes of climate change and airborne pollution, NASA has supported the development of compact, low power, rapid response instruments operating in the mid-infrared "molecular fingerprint" portion of the electromagnetic spectrum. These instruments, which measure atmospheric trace gases and airborne particles, can be deployed in mobile laboratories - customized ground vehicles, typically - to map distributions of pollutants in real time. The instruments must be rugged enough to operate rapidly and accurately, despite frequent jostling that can misalign, damage, or disconnect sensitive components. By measuring quickly while moving through an environment, a mobile laboratory can correlate data and geographic points, revealing patterns in the environment s pollutants. Rapid pollutant measurements also enable direct determination of pollutant sources and sinks (mechanisms that remove greenhouse gases and pollutants), providing information critical to understanding and managing atmospheric greenhouse gas and air pollutant concentrations.

  4. Gas fired boilers and atmospheric pollution

    International Nuclear Information System (INIS)

    Chiaranello, J.M.

    1991-01-01

    A general analysis concerning atmospheric pollution is presented: chemical composition and vertical distribution of atmosphere and pollutants, chemical reactions, ozone destruction and production cycles, COx, NOx and SOx pollutions. The gas fired boiler number and repartition in France are presented and the associated pollution is analyzed (CO2, CO, NOx) and quantified. Various pollution control technics concerning gas fired boiler pollutants are described and a pollution criterion for clean gas fired generators is proposed

  5. Atmospheric pollution: history, science and regulation

    Energy Technology Data Exchange (ETDEWEB)

    Jacobson, M.Z. [Stanford University, Stanford, CA (USA). Dept. of Civil and Environmental Engineering

    2002-07-01

    The book provides an introduction to the history and science of major air pollution issues. It begins with an introduction to the history of discovery of chemicals in the atmosphere, and moves on to a discussion of the evolution of the earth's atmosphere. It then discusses five major atmospheric pollution topics: urban outdoor air pollution, indoor air pollution, acid deposition, stratospheric ozone depletion, and global climate change. The book contains numerous student examples and problems and over 200 color illustrations and photographs.

  6. Lichens and atmospheric pollution

    Energy Technology Data Exchange (ETDEWEB)

    Tallis, J H

    1964-09-01

    The extreme sensitivity of lichens, particularly the larger ones, to industrialization has been recognized for many years. Most people attribute the absence of lichens from urban areas to the atmospheric pollution prevailing, and a few attribute it to climatic dryness, resulting from efficient drainage systems in towns. The two main components of air pollution are solid matter, or soot, and gaseous sulfur dioxide. The main effects of pollution appear to be: a direct reduction of light intensity by smoke haze, a deposit of soot on the plant surface, an acidification of the soil, and direct damage to plants. A body of evidence indicates that SO/sub 2/ may be the main harmful component for lichens. The distribution of lichens thus might be used to determine the limits within which atmospheric pollution is operating. 5 references.

  7. Atmosphere pollutants-their health and environmental effects

    International Nuclear Information System (INIS)

    Issa, Ali Sasi; Ibsaim, Rajab A.

    2006-01-01

    The conducted studies, continuous monitoring and measuring of the atmosphere pollution surrounding the world cities for a decade in the last century demonstrated increased rates of some pollutants, often exceeded the levels which are considered to be safe for health. Most of the dangerous pollutants in the atmosphere are suspended particles, sulfur oxides, nitrogen oxides, ozone troposphere and lead, these are the main responsible pollutant in contaminating the atmosphere leading to increase of death percentage in the major cities. For a duration of nearly a century, atmosphere pollution accidents in cities like London approved that inhaling contaminated air is dangerous and deadly sometimes. In 1880 2200 person from London inhabitants have died when coal smoke with heating and industrial gases have been accumulated to form a toxic smog of sulfur oxide gas and suspended particles in the atmosphere of the city. In this paper we discuss type of atmosphere pollutants and their health and environmental effects on human being, creatures and earth and ways of eliminating that.(Author)

  8. Clean Air Slots Amid Atmospheric Pollution

    Science.gov (United States)

    Hobbs, Peter V.

    2002-01-01

    This article investigates the mechanism for those layers in the atmosphere that are free of air borne pollution even though the air above and below them carry pollutants. Atmospheric subsidence is posed as a mechanism for this phenomenon.

  9. Effect of atmospheric pollution on health

    International Nuclear Information System (INIS)

    Islam, M.S.

    1990-01-01

    In recent years the incidence of smog episodes and their intensity have gone down considerably and difference in atmospheric pollutant levels between urban and rural areas is very small. Even the sudden moderate elevation of atmospheric pollution during winter months affects the pulmonary function adversely and provokes increased respiratory symptomes. The prevalence of rhinitis and allergy is more frequent both in adults and in children in urban townships than in rural areas. It has also been observed that industrial city dwellers have inferior pulmonary function. Very recent results indicate possible interaction between atmospheric pollutant levels and regeneration process following airways infection in yound children. (orig.) [de

  10. Dispersion and transport of atmospheric pollutants

    International Nuclear Information System (INIS)

    Cieslik, S.

    1991-01-01

    This paper presents the physical mechanisms that govern the dispersion and transport of air pollutant; the influence of the state of the 'carrying fluid', i.e. the role of meteorology; and finally, outlines the different techniques of assessing the process. Aspects of physical mechanisms and meteorology covered include: fate of an air pollutant; turbulence and dispersion; transport; wind speed and direction; atmospheric stability; and the role of atmospheric water. Assessment techniques covered are: concentrations measurements; modelling meteorological observations; and tracer releases. It is concluded that the only way to reduce air pollution is to pollute less. 10 refs., 12 figs., 2 tabs

  11. Atmospheric Chemistry and Air Pollution

    Directory of Open Access Journals (Sweden)

    Jeffrey S. Gaffney

    2003-01-01

    Full Text Available Atmospheric chemistry is an important discipline for understanding air pollution and its impacts. This mini-review gives a brief history of air pollution and presents an overview of some of the basic photochemistry involved in the production of ozone and other oxidants in the atmosphere. Urban air quality issues are reviewed with a specific focus on ozone and other oxidants, primary and secondary aerosols, alternative fuels, and the potential for chlorine releases to amplify oxidant chemistry in industrial areas. Regional air pollution issues such as acid rain, long-range transport of aerosols and visibility loss, and the connections of aerosols to ozone and peroxyacetyl nitrate chemistry are examined. Finally, the potential impacts of air pollutants on the global-scale radiative balances of gases and aerosols are discussed briefly.

  12. Modeling of atmospheric pollutant transfers

    International Nuclear Information System (INIS)

    Jourdain, F.

    2007-01-01

    Modeling is today a common tool for the evaluation of the environmental impact of atmospheric pollution events, for the design of air monitoring networks or for the calculation of pollutant concentrations in the ambient air. It is even necessary for the a priori evaluation of the consequences of a pollution plume. A large choice of atmospheric transfer codes exist but no ideal tool is available which allows to model all kinds of situations. The present day approach consists in combining different types of modeling according to the requested results and simulations. The CEA has a solid experience in this domain and has developed independent tools for the impact and safety studies relative to industrial facilities and to the management of crisis situations. (J.S.)

  13. Effects of atmospheric pollutants on lipids

    International Nuclear Information System (INIS)

    Howton, D.R.

    1976-01-01

    Studies on effects of atmospheric pollutants on lipids emphasized effects of nitrogen dioxide on olefinic centers of alveolar fluid surfactant lipids. The finding that NO 2 attacks α-tocopherol much more avidly than olefinic fatty esters indicates that the autoxidation enhancing effects of this atmospheric pollutant may be greatly magnified by destruction of native antioxidants that normally suppress the extensiveness of such lipid oxidation

  14. Remote measurement of atmospheric pollutants

    Science.gov (United States)

    Allario, F.; Hoell, J.; Seals, R. K.

    1979-01-01

    The concentration and vertical distribution of atmospheric ammonia and ozone are remotely sensed, using dual-C02-laser multichannel infrared Heterodyne Spectrometer (1HS). Innovation makes atmospheric pollution measurements possible with nearly-quantum-noise-limited sensitivity and ultrafine spectral resolution.

  15. Atmospheric pollution. From processes to modelling

    International Nuclear Information System (INIS)

    Sportisse, B.

    2008-01-01

    Air quality, greenhouse effect, ozone hole, chemical or nuclear accidents.. All these phenomena are tightly linked to the chemical composition of atmosphere and to the atmospheric dispersion of pollutants. This book aims at supplying the main elements of understanding of 'atmospheric pollutions': stakes, physical processes involved, role of scientific expertise in decision making. Content: 1 - classifications and scales: chemical composition of the atmosphere, vertical structure, time scales (transport, residence); 2 - matter/light interaction: notions of radiative transfer, application to the Earth's atmosphere; 3 - some elements about the atmospheric boundary layer: notion of scales in meteorology, atmospheric boundary layer (ABL), thermal stratification and stability, description of ABL turbulence, elements of atmospheric dynamics, some elements about the urban climate; 4 - notions of atmospheric chemistry: characteristics, ozone stratospheric chemistry, ozone tropospheric chemistry, brief introduction to indoor air quality; 5 - aerosols, clouds and rains: aerosols and particulates, aerosols and clouds, acid rains and leaching; 6 - towards numerical simulation: equation of reactive dispersion, numerical methods for chemistry-transport models, numerical resolution of the general equation of aerosols dynamics (GDE), modern simulation chains, perspectives. (J.S.)

  16. Atmospheric pollution in our environment

    International Nuclear Information System (INIS)

    Tanvir, G.

    1986-01-01

    Air pollution is associated with all the activities of humans. It is becoming a serious problem in coming years so it is relevant to find out how seriously our atmosphere is being polluted and how this pollution affects human and plant life in our environment. Not only the human activities are the source of our pollution but nature causes more pollution. Air pollution that is due to the pressure of foreign substances in air, effects the quality and concentration of air substances. It is not only injurious to property, but also to vegetation and animal life. Air pollution is one of our most serious environmental problems. The sources vary from smoke-stacks and automobiles to noise and foreon containing aerosols. (orig./A.B.)

  17. Students 'Weigh' Atmospheric Pollution.

    Science.gov (United States)

    Caporaloni, Marina

    1998-01-01

    Describes a procedure developed by students that measures the mass concentration of particles in a polluted urban atmosphere. Uses a portable fan and filters of various materials. Compares students' data with official data. (DDR)

  18. Low-technology monitoring of atmospheric metal pollution in central Scotland

    Energy Technology Data Exchange (ETDEWEB)

    Yule, F A; Lloyd, O L

    1984-01-01

    In epidemiological studies covering relationships of disease patterns and patterns of atmospheric pollution, conventional filtering equipment is normally used for monitoring the pollution. For various reasons, however, this type of approach often results in levels of pollution being obtained for only a few sites within an extensive fieldwork area. Hence, alternative monitoring techniques, which allow a high density of sampling sites in an area, have been of interest to an increasing number of investigators. The monitors used, known as low-technology monitors, fall into two main categories; indigenous; and transplants. In the authors surveys of atmospheric metal pollutants in industrial communities in Scotland, the indigenous sample materials have included: Hypnum cupressiforme, Lecanora conizaeoides, Agropyron repens and surface soils. In their transplant surveys a variety of different low-technology samplers have been deployed, the most frequently used being: spherical and flat moss bags, Hypogymnia physodes, Tak (synthetic fabric), and total deposition collectors. The data obtained from the various surveys have been plotted on a variety of types of computer map to minimize any systematic bias resulting from the use of a single technique. The pollution patterns found in one particular town were partly unexpected, in view of the dominant wind direction in the locality concerned. Hence it was decided to carry out a wind tunnel experiment to investigate the situation further. The wind tunnel experiment produced results which were consistent with the patterns of pollution derived from the metal surveys, and revealed that the meteorological dispersal of the pollution was unexpectedly influenced by local topography.

  19. The nitrogen oxides and the atmospheric pollution

    International Nuclear Information System (INIS)

    1990-01-01

    The objective of this document is to bring information on the acid atmospheric pollution, on the researches and studies in progress, on the european directives and the national regulations, on the processus and burners with low emission of nitrogen oxides and on the rule that the gas, fuel without sulphur, generating little nitrogen oxides, plays in the fight against atmospheric pollution. 20 refs., 8 figs., 12 tabs

  20. Atmospheric dispersion of pollutants in an industrial area of Cuba

    International Nuclear Information System (INIS)

    Cruz Monte de Oca, Feliberto de la; Furet Bridon, Norma Raisa; Turtos Carbonell, Leonor; Lorente Vera, Mercedes

    2011-01-01

    Air pollution by different chemicals; take a great connotation in the world, given the adverse effects on ecosystems and particularly human health. The urban development, the modification of the land surface and the climate change, phenomena derived from a world population explosion, are altering the composition of the air. The atmosphere deposits pollutants in the water courses and in land, which harms not only the persons, but also to the animals and the plants of the ecosystem. To know as these pollutants are dispersed in the atmosphere it is very important in the establishment of better urban, regional and world predictions of the air quality. The present study aims to assess the local spread of sulphur dioxide, nitrogen oxides and particulate matter from an industrial zone. The study was done using the pollutant Gaussian Dispersion Models AERMOD. For the evaluation of contaminants were considered two modeling scenarios: urban and rural. The SO 2 concentrations (μg/m 3 ) were obtained for 1 h, 24 h and all period (1 year), exceeding the permissible limits (500, 50 y 20 μg/m 3 ). It was also recorded for each period the number of times SO 2 concentrations exceeded the reference values in each of the scenarios discussed (urban: 39, 61 y 39; rural: 99, 75 y 25). At the end of modeling in the urban setting, 39 recipients exceeded the reference value, occupying an area of 9.75 km 2 and 25 receivers in the case of the rural setting, for an area of 6.25 km 2 . For NOx and particulate matter concentrations estimated values were always below the reference values. The obtained results in this case show the potentiality of AERMOD system for the evaluation of atmospheric dispersion of pollutants

  1. Medical aspects of atmosphere pollution in Tbilisi, Georgia.

    Science.gov (United States)

    Lagidze, Lamzira; Matchavariani, Lia; Tsivtsivadze, Nodar; Khidasheli, Nargiz; Paichadze, Nino; Motsonelidze, Nargiz; Vakhtangishvili, Maia

    2015-01-01

    Climate change and its impact on ecosystems is one of the main problem of 21st century. Increase in green house gas in the atmosphere was regarded as an important cause. Atmospheric composition had significantly changed due to intensive technogenic pollution. Increase in aerosol (solid, liquid and gas) concentration had serious impact on human health and raised the level of risk factors for longevity of life. Despite, global character of climatic change and its intensity in numerous ways was influenced by local specificity of regions, their geographical location and meteorological factors. A study on the atmospheric quality (quantitative and percentage estimation of aerosols) of Georgia was carried out. Also the assessment of impact of meteorological and ecological conditions on human health was made for Tbilisi city. A relation between contaminants and meteorological factors was evaluated, particularly gas pollutants were strongly correlated with each other due to their photochemical activity; positive correlation (0.65; 0.69) between air temperature and pollutants. All the contaminants showed negative correlation with relative humidity, due to hydrolyzing ability. On the basis of multi-factorial statistical analysis, correlation between ambulance call, weather type, atmosphere pollution index, change in ground ozone quantity and earth magnetic field were determined. Atmospheric pollution due to dust, carbon, sulfur and nitrogen oxides, ground ozone quantity in Tbilisi significantly exceeded maximum permissible level, that effected human health.

  2. The influence of combustion derived pollutants on limestone deterioration

    DEFF Research Database (Denmark)

    Johnson, JB; Montgomery, Melanie; Thompson, GE

    1996-01-01

    This study concerns quantification of the relative chemical degradation effects of dry deposition of combustion-derived atmospheric pollutants, HCl, SO2 and NO2, on Portland and Monks Park limestones, employing laboratory exposure chambers for periods of 30 days. Using presentation rates up to 40 x...... 10(-4) mu g cm(-2) s(-1), the pollutants were assessed individually and in various combinations, along with ozone as oxidant, at 84% RH with dry or water-wetted surfaces. The degradation was followed by analysis of exposed stone, for Cl-, SO42- and NO3-, and of run-off solution for Ca2+, in addition...... to the anions. From these data, the total calcium released from limestone to reaction ions and products and the percentages of each pollutant reacted (and so the deposition velocity (V-D)) in each exposure regime were calculated. HCl acted independently of the presence of other pollutants, showed 40 and 100...

  3. Atmospheric pollution and health. An introduction; Pollution atmospherique et sante une introduction

    Energy Technology Data Exchange (ETDEWEB)

    Zmirou, D. [Universite-Faculte de Medecine, 38 - Grenoble (France)

    1996-12-31

    Physiological observations and pollution measurements allowed for the study of short and long term respiratory effects of tropospheric ozone and fine particulate pollution on man, depending on age and health factors. Risk reduction policies towards air quality, and criteria issues for atmospheric pollution control and abatement measures, are discussed

  4. Sampling of Atmospheric Precipitation and Deposits for Analysis of Atmospheric Pollution

    OpenAIRE

    Skarżyńska, K.; Polkowska, Ż; Namieśnik, J.

    2006-01-01

    This paper reviews techniques and equipment for collecting precipitation samples from the atmosphere (fog and cloud water) and from atmospheric deposits (dew, hoarfrost, and rime) that are suitable for the evaluation of atmospheric pollution. It discusses the storage and preparation of samples for analysis and also presents bibliographic information on the concentration ranges of inorganic and organic compounds in the precipitation and atmospheric deposit samples.

  5. Lenticels as indicators of atmospheric smoke pollution

    Energy Technology Data Exchange (ETDEWEB)

    Pesek, F.

    1960-01-01

    The invasion of smoke pollution gets from the atmosphere into the plants only by lenticels and stomata. The most toxic smoke constituents penetrating into the stele are SO/sub 2/, H/sub 2/SiF/sub 6/, H/sub 3/AsO/sub 4/, HCl and C/sub 6/H/sub 5/OH. Lenticels are bark stomata filled with merenchym tissue, which hinders the entrance of mechanical smoke particles into the interior tissues of the stele. In autumn, the lenticels are packed by cork slabs formed by the cork cambium. In spring, this cork slab is broken by a new mechanical tissue. Sambucus nigra L. has a merenchym sensitive to the presence of smoke pollution, and the lenticels may serve, therefore, as indicators of smoke pollution in the atmosphere. The intensity of damage caused by smoke constituents penetrating into the plants through lenticels depends upon a series of exterior and interior factors. They are the number of lenticels per area unit of bark surface in the whole circumference, the pH of the biocomplex near the lenticel in the interior tissues of stele, and the concentration of smoke pollution in the atmosphere. The most effective way of preventing smoke damage is to install pollution control equipment in the industrial works.

  6. A Review of the Effects of Major Atmospheric Pollutants on Pollen Grains, Pollen Content, and Allergenicity

    Directory of Open Access Journals (Sweden)

    Hélène Sénéchal

    2015-01-01

    Full Text Available This review summarizes the available data related to the effects of air pollution on pollen grains from different plant species. Several studies carried out either on in situ harvested pollen or on pollen exposed in different places more or less polluted are presented and discussed. The different experimental procedures used to monitor the impact of pollution on pollen grains and on various produced external or internal subparticles are listed. Physicochemical and biological effects of artificial pollution (gaseous and particulate on pollen from different plants, in different laboratory conditions, are considered. The effects of polluted pollen grains, subparticles, and derived aeroallergens in animal models, in in vitro cell culture, on healthy human and allergic patients are described. Combined effects of atmospheric pollutants and pollen grains-derived biological material on allergic population are specifically discussed. Within the notion of “polluen,” some methodological biases are underlined and research tracks in this field are proposed.

  7. A Review of the Effects of Major Atmospheric Pollutants on Pollen Grains, Pollen Content, and Allergenicity

    Science.gov (United States)

    Sénéchal, Hélène; Visez, Nicolas; Charpin, Denis; Shahali, Youcef; Peltre, Gabriel; Biolley, Jean-Philippe; Lhuissier, Franck; Couderc, Rémy; Yamada, Ohri; Malrat-Domenge, Audrey; Pham-Thi, Nhân; Poncet, Pascal; Sutra, Jean-Pierre

    2015-01-01

    This review summarizes the available data related to the effects of air pollution on pollen grains from different plant species. Several studies carried out either on in situ harvested pollen or on pollen exposed in different places more or less polluted are presented and discussed. The different experimental procedures used to monitor the impact of pollution on pollen grains and on various produced external or internal subparticles are listed. Physicochemical and biological effects of artificial pollution (gaseous and particulate) on pollen from different plants, in different laboratory conditions, are considered. The effects of polluted pollen grains, subparticles, and derived aeroallergens in animal models, in in vitro cell culture, on healthy human and allergic patients are described. Combined effects of atmospheric pollutants and pollen grains-derived biological material on allergic population are specifically discussed. Within the notion of “polluen,” some methodological biases are underlined and research tracks in this field are proposed. PMID:26819967

  8. An assessment of worldwide energy-related atmospheric pollution

    International Nuclear Information System (INIS)

    1989-01-01

    Energy-related emissions of atmospheric pollutants are currently suspected as the source of a number of major environmental problems. Early concerns about local and regional air quality and respiratory health risks, greatly alleviated in the case of sulfur dioxide (SO 2 ) emissions by the use of tall stacks, have been superseded by ''global problems,'' such as acidification of the biosphere, increase in tropospheric ozone (O 3 ), visibility impairment, long-term exposure to toxic pollutants, and buildup of ''greenhouse gases''. Chapter 1 assesses the sources and physical/chemical atmospheric processes of energy-related atmospheric pollution (ERAP). It is not an exhaustive review but rather a documented statement of the state-of-art knowledge on issues critical to effective environmental decision-making. Chapter 2 looks at the effects on man, the environment and materials, and chapter 3 presents an overview and policy options. (author)

  9. Atmospheric pollution: How is it in Morocco?

    International Nuclear Information System (INIS)

    Nejjari, Chakib; Mechakra-Tahiri, S.

    1999-01-01

    The effect of atmospheric pollution is recognised. Risks are defined by toxicological studies on man and animal and by epidemiological studies based on population in industrial countries. Air pollution due to the economical development and the contamination of the atmosphere by chemical substances (gas and aerosols), has been also increasing around the world. The case here is in Morocco. SO 2 emissions has increased from 129 thousand tons per year to 180 tt per year in 1992 and will reach 300 tt per year in 2005. In Morocco today exist a large number of vehicles and industries (chemical industries, refineries, plastic...) emitting pollutants in rural cities and causing toxic products as aerosols and smog. A table concerning the evolution of gas emissions (SO 2 ; NO x ; CO and Ozone) in Morocco per thousand tons per year from 1982 until 2020 is given in details. Projects are settled to increase the air quality and reduce air pollution and its impact on public health

  10. Using an epiphytic moss to identify previously unknown sources of atmospheric cadmium pollution

    Science.gov (United States)

    Geoffrey H. Donovan; Sarah E. Jovan; Demetrios Gatziolis; Igor Burstyn; Yvonne L. Michael; Michael C. Amacher; Vicente J. Monleon

    2016-01-01

    Urban networks of air-quality monitors are often too widely spaced to identify sources of air pollutants, especially if they do not disperse far from emission sources. The objectives of this study were to test the use of moss bio-indicators to develop a fine-scale map of atmospherically-derived cadmium and to identify the sources of cadmium in a complex urban setting....

  11. Atmospheric Metal Pollutants-Archives, Methods, and History

    International Nuclear Information System (INIS)

    Norton, Stephen A.

    2007-01-01

    Pollution of the atmosphere with cadmium (Cd), mercury (Hg), and lead (Pb) is a consequence of human activities. Natural archives are necessary to reconstruct the long-term history of metal deposition because accurate measurement of atmospheric deposition is a recent accomplishment. Reconstructions require: (1) accurate determination of concentrations of elements and isotopes, (2) accurate chronology of archives, and (3) archives that faithfully record atmosphere deposition. The most useful long-term archives are accumulations of ice and snow, peat, and lake sediment. Quantification of Cd deposition is uncommon because of its low concentration and substantial chemical mobility. Nonetheless, trends in peat and lake sediment are similar to those of Hg and Pb since ca. 1800 a.d. Both Hg and Pb are relatively chemically immobile and thus the peat and lake archives are believed to record historic trends of atmospheric deposition. Isotopic and concentration studies of Pb indicate a history of northern hemisphere atmospheric pollution extending back prior to 0 a.d. Although measurements of Hg concentration are now routine, isotopic measurements are in their infancy. Some Hg pollution sources have unique isotopic ratios, thereby contributing unique signals to the total Hg. Maximum accumulation rates of Hg and Pb occur up to 10 years later than for Cd (1970s versus 1960s in eastern North America, perhaps slightly later in Europe). By 2004, deposition of Cd, Hg, and Pb had declined from peak values in eastern North America more than 75, 75, and 90%, respectively

  12. Atmospheric pollution in Lisbon urban atmosphere

    Science.gov (United States)

    Oliveira, C.

    2009-04-01

    Lisbon is the capital city of Portugal with about 565,000 residents in 2008 and a population density of 6,600 inhabitants per square kilometre. Like several other major metropolis, the town is surrounded by satellite cities, forming together a region known as "Lisbon Metropolitan Area" with about 3 million inhabitants, a quarter of the overall Portuguese population. Besides their local residents, it is estimated that more than one million citizens come into the Lisbon area every day from the outskirts, leading to elevated traffic densities and intense traffic jams, with important consequences on air pollution levels and obvious negative impacts on human health. Airborne particulate matter limit values are frequently exceeded, making urgent the existence of consistent programs to monitor and help taking measures to control them. Within the Portuguese project PAHLIS (Polycyclic Aromatic Hydrocarbons Contamination in Lisbon Urban Atmosphere) financed by the Portuguese Science Foundation ("Fundação para a Ciência e a Tecnologia"), an aerosol and vapour phase sampling program is being implemented in the city of Lisbon at two selected contrasting zones, namely a typically busy area with intense road traffic and frequent exceedences of the particulate matter standard for the maximum allowable concentration, and a residential quieter area, thus with a cleaner atmosphere characterised as an urban background site. An one month-long sampling campaign was performed during the summer of 2008, where particulate matter was collected in two fractions (coarse 2.5µmwork are expected to cover a lack of reliable information regarding sources of atmospheric pollutants in Portugal and present, for the first time, systematic data of PAHs levels in Lisbon. Acknowledgement: This work was performed under Project PAHLIS (PTDC/AMB/65699/2006) financed by "Fundação para a Ciência e a Tecnologia". C. Oliveira thanks Project PAHLIS his scholarship.

  13. Application of computational fluid mechanics to atmospheric pollution problems

    Science.gov (United States)

    Hung, R. J.; Liaw, G. S.; Smith, R. E.

    1986-01-01

    One of the most noticeable effects of air pollution on the properties of the atmosphere is the reduction in visibility. This paper reports the results of investigations of the fluid dynamical and microphysical processes involved in the formation of advection fog on aerosols from combustion-related pollutants, as condensation nuclei. The effects of a polydisperse aerosol distribution, on the condensation/nucleation processes which cause the reduction in visibility are studied. This study demonstrates how computational fluid mechanics and heat transfer modeling can be applied to simulate the life cycle of the atmosphereic pollution problems.

  14. [Consequences of atmospheric pollution fluctuations in patients with COPD].

    Science.gov (United States)

    Amiot, N; Tillon, J; Viacroze, C; Aouine, H; Muir, J-F

    2010-10-01

    Fluctuations in atmospheric pollution are responsible for an important morbidity and mortality in the patients suffering from chronic obstructive pulmonary disease (COPD). Epidemiological studies show a significant increase in the mortality and hospitalization rates in COPD patients in relation to moderate increases in atmospheric pollution. In vitro and in vivo studies demonstrate a pro-inflammatory role and an oxidative toxicity of atmospheric particles and secondary morphological and functional changes in the respiratory epithelium and the immune system. An excess of particulate matter, ozone, NO(2), SO(2) and CO is directly correlated to the number of episodes of acute respiratory failure in different countries all over the world. The mechanisms implicated are complex and variable, dependent on the different pollutant agents, climatic variations and inter-individual susceptibility. Further experimental studies are necessary in order to clarify our fundamental understanding and, alongside better control of air quality, to reduce short-term respiratory complications. The consequences of atmospheric pollution fluctuations on the exacerbation rate and therefore on the morbidity and mortality of patients with COPD emphasize the importance of preventive environmental management in the field of public health. Copyright © 2010. Published by Elsevier Masson SAS.

  15. Archives of Atmospheric Lead Pollution

    Science.gov (United States)

    Weiss, Dominik; Shotyk, William; Kempf, Oliver

    Environmental archives such as peat bogs, sediments, corals, trees, polar ice, plant material from herbarium collections, and human tissue material have greatly helped to assess both ancient and recent atmospheric lead deposition and its sources on a regional and global scale. In Europe detectable atmospheric lead pollution began as early as 6000years ago due to enhanced soil dust and agricultural activities, as studies of peat bogs reveal. Increased lead emissions during ancient Greek and Roman times have been recorded and identified in many long-term archives such as lake sediments in Sweden, ice cores in Greenland, and peat bogs in Spain, Switzerland, the United Kingdom, and the Netherlands. For the period since the Industrial Revolution, other archives such as corals, trees, and herbarium collections provide similar chronologies of atmospheric lead pollution, with periods of enhanced lead deposition occurring at the turn of the century and since 1950. The main sources have been industry, including coal burning, ferrous and nonferrous smelting, and open waste incineration until c.1950 and leaded gasoline use since 1950. The greatest lead emissions to the atmosphere all over Europe occurred between 1950 and 1980 due to traffic exhaust. A marked drop in atmospheric lead fluxes found in most archives since the 1980s has been attributed to the phasing out of leaded gasoline. The isotope ratios of lead in the various archives show qualitatively similar temporal changes, for example, the immediate response to the introduction and phasing out of leaded gasoline. Isotope studies largely confirm source assessments based on lead emission inventories and allow the contributions of various anthropogenic sources to be calculated.

  16. Spectral solar irradiance and some optical properties for various polluted atmospheres

    International Nuclear Information System (INIS)

    Jacovides, Constantinos P.; Asimakopoulos, Demosthenis N.; Steven, Michael D.

    2000-01-01

    Using ground-based spectroradiometric measurements taken over the Athens atmosphere during May 1995, the influence of gaseous pollutants and aerosol on the spectral radiant energy distribution was investigated. It was found that spectral measurements exhibited variations based on various polluted urban atmospheric conditions as determined via gaseous pollutants record analysis. The relative attenuations cause by gaseous pollutants and aerosol can exceed 27%, 17% and 16% in the global ultraviolet, visible and near-infrared portions of the solar spectrum respectively, as compared to 'background' values. In contrast, an enhancement of the near-infrared diffuse component by 66%, was observed, while in visible and ultraviolet bands the relative increases reached 54% and 21% respectively. Experimental total Rayleigh-corrected and spectral aerosol optical depths were retrieved, representing differences in polluted air over the Athens atmosphere. The diffuse component accounts for more than 80% of the total radiation field under high polluted atmosphere. The observed differences of solar radiation between the Athens center and at a nearby suburban site are a manifestation of contrasting air properties provided mainly by automotive traffic. (Author)

  17. Atmospheric pollution and its influence on British forests

    Energy Technology Data Exchange (ETDEWEB)

    Lines, R

    1958-01-01

    The two chief sources of atmospheric pollution in Britain are the combustion of fuels and salt spray blown inland from the sea. This paper reviews the research done up to 1958 on both combustion-related air pollution and sea salt deposition in Great Britain.

  18. The Influence of Combustion-derived pollutants on limestone deterioration

    DEFF Research Database (Denmark)

    Johnson, J.B.; Montgomery, Melanie; Thompson, G.E.

    1996-01-01

    The wet deposition of combustion-derived atmospheric pollutant species, on to freshly cut or diesel-smoked Portland and Monks Park limestone and marble samples, was carried out in a laboratory 'wetting and drying' salt spray chamber for 84 days. Along with the effect of CO2-equilibrated de...... limestones, respectively. Thus the water and hydrogen ion loading effects are significant, as well as the limestone type, but the nature of the anion is not, under the given wetting and drying regime. Further work showed that the increased resistance of marble over that of limestone, to calcium loss...

  19. Atmospheric pollutants monitoring by analysis of epiphytic lichens

    International Nuclear Information System (INIS)

    Fuga, Alessandra; Saiki, Mitiko; Marcelli, Marcelo P.; Saldiva, Paulo H.N.

    2008-01-01

    The Canoparmelia texana epiphytic lichenized fungi was used to monitor atmospheric pollution in the Sao Paulo metropolitan region, SP, Brazil. The cluster analysis applied to the element concentration values confirmed the site groups of different levels of pollution due to industrial and vehicular emissions. In the distribution maps of element concentrations, higher concentrations of Ba and Mn were observed in the vicinity of industries and of a petrochemical complex. The highest concentration of Co found in lichens from the Sao Miguel Paulista site is due to the emissions from a metallurgical processing plant that produces this element. For Br and Zn, the highest concentrations could be associated both to vehicular and industrial emissions. Exploratory analyses revealed that the accumulation of toxic elements in C. texana may be of use in evaluating the human risk of cardiopulmonary mortality due to prolonged exposure to ambient levels of air pollution. - Canoparmelia texana lichenized fungi is a valuable biomonitor for atmospheric pollution

  20. Polarimetric Remote Sensing of Atmospheric Particulate Pollutants

    Science.gov (United States)

    Li, Z.; Zhang, Y.; Hong, J.

    2018-04-01

    Atmospheric particulate pollutants not only reduce atmospheric visibility, change the energy balance of the troposphere, but also affect human and vegetation health. For monitoring the particulate pollutants, we establish and develop a series of inversion algorithms based on polarimetric remote sensing technology which has unique advantages in dealing with atmospheric particulates. A solution is pointed out to estimate the near surface PM2.5 mass concentrations from full remote sensing measurements including polarimetric, active and infrared remote sensing technologies. It is found that the mean relative error of PM2.5 retrieved by full remote sensing measurements is 35.5 % in the case of October 5th 2013, improved to a certain degree compared to previous studies. A systematic comparison with the ground-based observations further indicates the effectiveness of the inversion algorithm and reliability of results. A new generation of polarized sensors (DPC and PCF), whose observation can support these algorithms, will be onboard GF series satellites and launched by China in the near future.

  1. The characteristic features of the atmospheric diffusion of pollutants

    International Nuclear Information System (INIS)

    Schultz, H.

    1986-01-01

    The publication facilitates access to the development and effects of air pollution caused by the major emission sources by way of discussing the atmospheric dispersion of pollutants and the processes involved. Apart from the physical ratings of atmospheric pollutants the author focuses on the meteorological parameters determining the dispersion process as well as on the unavoidable statistical variations. Representative realistic maximum and minimum values indicating the relation between emissions from the relevant sources and the resulting air pollution allow an expeditious evaluation of possible environmental impacts classified by the different types of pollutants. The publication not only discusses the direct incorporation, that is the breathing of contaminated air or the absorption of food grown or produced in contaminated regions but also refers to radiation doses which due to the presence of radioactive substances accumulate in the human organism. Comprehensive references are annexed to facilitate access to relevant problems connected with the subject discussed. (orig./HP) [de

  2. Problematic of atmospheric pollution in Lebanon: the better stake is apprehended, the best acts are taken

    International Nuclear Information System (INIS)

    Chehab, Said

    1998-01-01

    The document presents an overview on atmospheric pollution in Lebanon, with an analysis of sources of pollution, their impact on local and global environment and their control.Local causes of pollution are mainly: -Thermal power plants of electric power production which produce 75% SO 2 emission and 60% dust - Industries, especially cement industry - Land transportation which produces 70% NOX emission and 50% CO 2 A description of air pollution caused by these three sectors is revealed. Pollutants derived from fuel combustion are analyzed. It is estimated that in 2010, Co 2 emission will reach 5204450 tons, SO 2 emission will be 136470 tons, NOX emissions 96870 and dust estimated to 4130 tons. CFC consumption and measures of control according to Montreal Protocol are described. Recommendations for control of air pollution in Lebanon within a national policy are presented

  3. Biomagnetic Monitoring of Atmospheric Pollution: A Review of Magnetic Signatures from Biological Sensors.

    Science.gov (United States)

    Hofman, Jelle; Maher, Barbara A; Muxworthy, Adrian R; Wuyts, Karen; Castanheiro, Ana; Samson, Roeland

    2017-06-20

    Biomagnetic monitoring of atmospheric pollution is a growing application in the field of environmental magnetism. Particulate matter (PM) in atmospheric pollution contains readily measurable concentrations of magnetic minerals. Biological surfaces, exposed to atmospheric pollution, accumulate magnetic particles over time, providing a record of location-specific, time-integrated air quality information. This review summarizes current knowledge of biological material ("sensors") used for biomagnetic monitoring purposes. Our work addresses the following: the range of magnetic properties reported for lichens, mosses, leaves, bark, trunk wood, insects, crustaceans, mammal and human tissues; their associations with atmospheric pollutant species (PM, NO x , trace elements, PAHs); the pros and cons of biomagnetic monitoring of atmospheric pollution; current challenges for large-scale implementation of biomagnetic monitoring; and future perspectives. A summary table is presented, with the aim of aiding researchers and policy makers in selecting the most suitable biological sensor for their intended biomagnetic monitoring purpose.

  4. Nonlinear dynamics of the atmospheric pollutants in Mexico City

    Science.gov (United States)

    Muñoz-Diosdado, Alejandro; Barrera-Ferrer, Amilcar; Angulo-Brown, Fernando

    2014-05-01

    The atmospheric pollution in the Metropolitan Zone of Mexico City (MZMC) is a serious problem with social, economical and political consequences, in virtue that it is the region which concentrates both the greatest country population and a great part of commercial and industrial activities. According to the World Health Organization, maximum permissible concentrations of atmospheric pollutants are exceeded frequently. In the MZMC, the environmental monitoring has been limited to criteria pollutants, named in this way due to when their levels are measured in the atmosphere, they indicate in a precise way the air quality. The Automatic Atmospheric Monitoring Network monitors and registers the values of pollutants concentration in air in the MZMC. Actually, it is integrated by approximately 35 automatic-equipped remote stations, which report an every-hour register. Local and global invariant quantities have been widely used to describe the fractal properties of diverse time series. In the study of certain time series, many times it is assumed that they are monofractal, which means that they can be described only with one fractal dimension. But this hypothesis is unrealistic because a lot of time series are heterogeneous and non stationary, so their scaling properties are not the same throughout time and therefore they may require more fractal dimensions for their description. Complexity of the atmospheric pollutants dynamics suggests us to analyze its time series of hourly concentration registers with the multifractal formalism. So, in this work, air concentration time series of MZMC criteria pollutants were studied with the proposed method. The chosen pollutants to perform this analysis are ozone, sulfur dioxide, carbon monoxide, nitrogen dioxide and PM10 (particles less than 10 micrometers). We found that pollutants air concentration time series are multifractal. When we calculate the degree of multifractality for each time series we know that while more

  5. Mortality, fog and atmospheric pollution

    Energy Technology Data Exchange (ETDEWEB)

    Martin, A E; Bradley, W H

    1960-01-01

    A study was made associating climate and atmospheric pollution with excess mortality in greater London during the winter of 1958 and 1959. It was a particularly foggy winter with 6 major episodes, 4 of which resembled previous dangerous smogs. There were two additional periods of high pollution without fog. Excess mortality during these 8 periods ranged from 70 to 230. During one period, a flu epidemic accompanied the fog. In 4 to 6 foggy periods, morbidity (hospital bed demand) also increased. This small number of observations indicates mortality association: on 2/3 of days with high SO/sub 2/ (2.5 pphM) or high particulate soot (10 mg/m/sup 3/), and on all days with thick fog, there was an increase in mortality (20 deaths more than previous day) on that or the following day. Fifteen-day moving mortality index and bronchitis mortality index were significantly correlated with black suspended matter and SO/sub 2/; association with pneumonia was not significant. Also little or no relation between mortality and humidity, mean temperature, or barometric pressure was found. Rapid response of mortality to air pollution may indicate that pollution affects mostly those already ill.

  6. Multi-scale dynamic modeling of atmospheric pollution in urban environment

    International Nuclear Information System (INIS)

    Thouron, Laetitia

    2017-01-01

    Urban air pollution has been identified as an important cause of health impacts, including premature deaths. In particular, ambient concentrations of gaseous pollutants such as nitrogen dioxide (NO 2 ) and particulate matter (PM10 and PM2.5) are regulated, which means that emission reduction strategies must be put in place to reduce these concentrations in places where the corresponding regulations are not respected. Besides, air pollution can contribute to the contamination of other media, for example through the contribution of atmospheric deposition to runoff contamination. The multifactorial and multi-scale aspects of urban make the pollution sources difficult to identify. Indeed, the urban environment is a heterogeneous space characterized by complex architectural structures (old buildings alongside a more modern building, residential, commercial, industrial zones, roads, etc.), non-uniform atmospheric pollutant emissions and therefore the population exposure to pollution is variable in space and time. The modeling of urban air pollution aims to understand the origin of pollutants, their spatial extent and their concentration/deposition levels. Some pollutants have long residence times and can stay several weeks in the atmosphere (PM2.5) and therefore be transported over long distances, while others are more local (NO x in the vicinity of traffic). The spatial distribution of a pollutant will therefore depend on several factors, and in particular on the surfaces encountered. Air quality depends strongly on weather, buildings (canyon-street) and emissions. The aim of this thesis is to address some of these aspects by modeling: (1) urban background pollution with a transport-chemical model (Polyphemus / POLAIR3D), which makes it possible to estimate atmospheric pollutants by type of urban surfaces (roofs, walls and roadways), (2) street-level pollution by explicitly integrating the effects of the building in a three-dimensional way with a multi-scale model of

  7. POLARIMETRIC REMOTE SENSING OF ATMOSPHERIC PARTICULATE POLLUTANTS

    Directory of Open Access Journals (Sweden)

    Z. Li

    2018-04-01

    Full Text Available Atmospheric particulate pollutants not only reduce atmospheric visibility, change the energy balance of the troposphere, but also affect human and vegetation health. For monitoring the particulate pollutants, we establish and develop a series of inversion algorithms based on polarimetric remote sensing technology which has unique advantages in dealing with atmospheric particulates. A solution is pointed out to estimate the near surface PM2.5 mass concentrations from full remote sensing measurements including polarimetric, active and infrared remote sensing technologies. It is found that the mean relative error of PM2.5 retrieved by full remote sensing measurements is 35.5 % in the case of October 5th 2013, improved to a certain degree compared to previous studies. A systematic comparison with the ground-based observations further indicates the effectiveness of the inversion algorithm and reliability of results. A new generation of polarized sensors (DPC and PCF, whose observation can support these algorithms, will be onboard GF series satellites and launched by China in the near future.

  8. Atmospheric Pollution: Its Origins and Prevention.

    Science.gov (United States)

    Meetham, A. R.

    Although atmospheric pollution can be reduced or eliminated in many different ways, each way involves questions of economics, the time factor, availability of materials, priority over other urgent reforms, and individual and social psychology. To provide a basis for consideration of these questions, this book gives information not only about the…

  9. Atmospheric Heavy Metal Pollution - Development of Chronological ...

    Indian Academy of Sciences (India)

    Home; Journals; Resonance – Journal of Science Education; Volume 6; Issue 4. Atmospheric Heavy Metal Pollution - Development of Chronological Records and Geochemical Monitoring. Rohit Shrivastav. General Article Volume 6 Issue 4 April 2001 pp 62-68 ...

  10. Influence of ship emission on atmospheric pollutant concentration around Osaka Bay, Japan

    International Nuclear Information System (INIS)

    Kondo, A.; Yamaguchi, K.; Nishikawa, E.

    1999-01-01

    Marine traffic in Osaka Bay is very intensified and much atmosphere pollutant (SO x and NO x ) from ships is released but there is no regulation about the ship emission. In this paper, we investigated the emission amounts of SO x NO x and HC from car, factory and ships in Osaka bay area and estimated the influence of the ship emission on the atmospheric pollutant concentration, using both the meteorological prediction model and the atmospheric pollutant concentration prediction model including the dry deposition and the chemical reaction. In Osaka bay area, the emission amounts of SO x and NO x from ships were about 30% of the total emission amounts, respectively. Using these emission data, the atmospheric pollutant concentration was simulated on a summer fine day when high oxidant concentration was measured at several observatories and was compared with the observed data. Though some differences were seen between the simulated results and the observed data, the diurnal variation agreed reasonably. The second simulation was carried out except for the ship emission and we estimated the influence of the ship emission on the atmospheric pollutant concentration. It was found that the ship emission raised SO 2 , NO 2 and NO concentration not only in shore area but also in 40km inland. (Author)

  11. Atmospheric dispersion models for environmental pollution applications

    International Nuclear Information System (INIS)

    Gifford, F.A.

    1976-01-01

    Pollutants are introduced into the air by many of man's activities. The potentially harmful effects these can cause are, broadly speaking, of two kinds: long-term, possibly large-scale and wide-spread chronic effects, including long-term effects on the earth's climate; and acute, short-term effects such as those associated with urban air pollution. This section is concerned with mathematical cloud or plume models describing the role of the atmosphere, primarily in relation to the second of these, the acute effects of air pollution, i.e., those arising from comparatively high concentration levels. The need for such air pollution modeling studies has increased spectacularly as a result of the National Environmental Policy Act of 1968 and, especially, two key court decisions; the Calvert Cliffs decision, and the Sierra Club ruling on environmental non-degradation

  12. Prediction on long-term mean and mean square pollutant concentrations in an urban atmosphere

    Energy Technology Data Exchange (ETDEWEB)

    Kumar, S; Lamb, R G; Seinfeld, J H

    1976-01-01

    The general problem of predicting long-term average (say yearly) pollutant concentrations in an urban atmosphere is formulated. The pollutant concentration can be viewed as a random process, the complete description of which requires knowledge of its probability density function, which is unknown. The mean concentration is the first moment of the concentration distribution, and at present there exist a number of models for predicting the long-term mean concentration of an inert pollutant. The second moment, or mean square concentration, indicates additional features of the distribution, such as the level of fluctuations about the mean. In the paper a model proposed by Lamb for the long-term mean concentration is reviewed, and a new model for prediction of the long-term mean square concentration of an inert air pollutant is derived. The properties and uses of the model are discussed, and the equations defining the model are presented in a form for direct application to an urban area.

  13. [Observation on atmospheric pollution in Xianghe during Beijing 2008 Olympic Games].

    Science.gov (United States)

    Pan, Yue-Peng; Wang, Yue-Si; Hu, Bo; Liu, Quan; Wang, Ying-Hong; Nan, Wei-Dong

    2010-01-01

    There is a concern that much of the atmospheric pollution experienced in Beijing is regional in nature and not attributable to local sources. The objective of this study is to examine the contribution of sources outside Beijing to atmospheric pollution levels during Beijing 2008 Olympic Games. The observations of SO2, NO(x), O3, PM2.5 and PM10 were conducted from June 1 to September 30, 2008 in Xianghe, a rural site about 70 km southeast of Beijing. Sources and transportation of atmospheric pollution during the experiment were discussed with surface meteorology data and backward trajectories calculated using HYSPLIT model. The results showed that the daily average maximum (mean +/- standard deviation) concentrations of SO2, NO(x), O3, PM2.5, and PM10 during observation reached 84.4(13.4 +/- 15.2), 43.3 (15.9 +/- 9.1), 230 (82 +/- 38), 184 (76 +/- 42) and 248 (113 +/- 52) microg x m(-3), respectively. In particular, during the pollution episodes from July 20 to August 12, the hourly average concentration of O3 exceeded the National Ambient Air Quality Standard II for 46 h (9%), and the daily average concentration of PM10 exceeded the Standard for 11 d (46%); PM2.5 exceeded the US EPA Standard for 18 d (75%). The daily average concentrations of SO2, NO(x), O3, PM2.5 and PM10 decreased from 27.7, 18.6, 96, 90, 127 microg x m(-3) in June-July to 5.8, 13.2, 80, 60, 106 microg x m(-3) during Olympic Games (August-September), respectively. The typical diurnal variations of NO(x), PM2.5 and PM10 were similar, peaking at 07:00 and 20:00, while the maximum of O3 occurred between 14:00 to 16:00 local time. The findings also suggested that the atmospheric pollution in Xianghe is related to local emission, regional transport as well as the meteorological conditions. Northerly wind and precipitation are favorable for diffusion and wet deposition of pollutants, while sustained south flows make the atmospheric pollution more serious. The lead-lag correlation analysis during the

  14. Stable lead isotopes and lake sediments. A useful combination for the study of atmospheric lead pollution history

    Energy Technology Data Exchange (ETDEWEB)

    Renberg, I.; Braennvall, M.-L.; Bindler, R. [Department of Ecology and Environmental Science, Umea University, SE-901 87 Umea (Sweden); Emteryd, O. [Department of Forest Ecology, Swedish University of Agricultural Sciences, SE-901 83 Umea (Sweden)

    2002-06-20

    Analysis of stable lead isotopes and lead concentrations in lake-sediment deposits, not least in varved (annually-laminated) sediments, is a useful method to study lead pollution history. This paper presents details from a study of 31 lakes in Sweden. Using a strong acid digestion of sediment samples and ICP-MS analyses, we have found that Swedish lake sediments have a high natural (pre-pollution) 206[Pb]/207[Pb] ratio (mean 1.52{+-}0.18, range 1.28-2.01, n=31 lakes). In contrast, atmospheric lead pollution derived from metal smelting processes, coal burning and from alkyl-lead added to petrol has a lower ratio (<1.2). Consequently, when pollution lead deposition began approximately 3500 years ago, the lead isotope ratio of the sediments started to decline, and in modern sediments it is typically <1.2. Using the isotope and concentration values and a mixing model, the relative contribution of pollution and natural lead in sediment samples can be calculated. The pollution lead records of the Swedish lake sediments show a consistent picture of the atmospheric lead pollution history. Some noticeable features are the Roman peak, the large and permanent Medieval increase, peaks at approximately 1200 and 1530 ad, the rapid increase after World War II, the peak in the 1970s, and the large modern decline.

  15. Population-production-pollution nexus based air pollution management model for alleviating the atmospheric crisis in Beijing, China.

    Science.gov (United States)

    Zeng, X T; Tong, Y F; Cui, L; Kong, X M; Sheng, Y N; Chen, L; Li, Y P

    2017-07-15

    In recent years, increscent emissions in the city of Beijing due to expanded population, accelerated industrialization and inter-regional pollutant transportation have led to hazardous atmospheric pollution issues. Although a number of anthropogenic control measures have been put into use, frequent/severe haze events have still challenged regional governments. In this study, a hybrid population-production-pollution nexus model (PPP) is proposed for air pollution management and air quality planning (AMP) with the aim to coordinate human activities and environmental protection. A fuzzy-stochastic mixed quadratic programming method (FSQ) is developed and introduced into a PPP for tackling atmospheric pollution issues with uncertainties. Based on the contribution of an index of population-production-pollution, a hybrid PPP-based AMP model that considers employment structure, industrial layout pattern, production mode, pollutant purification efficiency and a pollution mitigation scheme have been applied in Beijing. Results of the adjustment of employment structure, pollution mitigation scheme, and green gross domestic product under various environmental regulation scenarios are obtained and analyzed. This study can facilitate the identification of optimized policies for alleviating population-production-emission conflict in the study region, as well as ameliorating the hazardous air pollution crisis at an urban level. Copyright © 2017 Elsevier Ltd. All rights reserved.

  16. Effective pollutant emission heights for atmospheric transport modelling based on real-world information.

    Science.gov (United States)

    Pregger, Thomas; Friedrich, Rainer

    2009-02-01

    Emission data needed as input for the operation of atmospheric models should not only be spatially and temporally resolved. Another important feature is the effective emission height which significantly influences modelled concentration values. Unfortunately this information, which is especially relevant for large point sources, is usually not available and simple assumptions are often used in atmospheric models. As a contribution to improve knowledge on emission heights this paper provides typical default values for the driving parameters stack height and flue gas temperature, velocity and flow rate for different industrial sources. The results were derived from an analysis of the probably most comprehensive database of real-world stack information existing in Europe based on German industrial data. A bottom-up calculation of effective emission heights applying equations used for Gaussian dispersion models shows significant differences depending on source and air pollutant and compared to approaches currently used for atmospheric transport modelling.

  17. Atmospheric pollution and its implications in the Eastern Transvaal highveld

    CSIR Research Space (South Africa)

    Tyson, PD

    1988-04-01

    Full Text Available This report is a review of available information on the dispersion climatology, the degree of atmospheric pollution and the various impacts of that pollution on man and environment in the Eastern Transvaal Highveld (ETH) and adjacent regions...

  18. Role of atmospheric circulations in haze pollution in December 2016

    Science.gov (United States)

    Yin, Zhicong; Wang, Huijun

    2017-09-01

    In the east of China, recent haze pollution has been severe and damaging. In addition to anthropogenic emissions, atmospheric circulations and local meteorological conditions were conducive factors. The number of December haze days over North China and the Huanghuai area has increased sharply since 2010 and was greatest in 2016. During 2016, the most aggressive control measures for anthropogenic emissions were implemented from 16 to 21 December, but the most severe haze pollution still occurred, covering approximately 25 % of the land area of China and lasting for 6 days. The atmospheric circulations must play critical roles in the sub-seasonal haze events. Actually, the positive phase of the East Atlantic-West Russia pattern in the middle troposphere strengthened the anomalous anti-cyclone over the NH area that confined vertical motion below. The associated southerly anomalies made the cold air and surface wind speed weaker, but enhanced the humid flow. Thus, the horizontal and vertical dispersion of atmospheric particulates was suppressed and the pollutants gathered within a narrow space. In December 2016, these key indices were strongly beneficial for haze occurrence and combined to result in the severest haze pollution. The influences of the preceding autumn sea surface temperature near the Gulf of Alaska and the subtropical eastern Pacific, October-November snow cover in western Siberia, and associated physical processes on haze pollution are also discussed.

  19. Atmospheric transport of pollution to the Arctic

    International Nuclear Information System (INIS)

    Iversen, T.

    1984-01-01

    If the atmospheric processes are assumed to be nearly adiabatic, the conclusion is that the possible source areas of Arctic air pollution detected at ground level have to be situated in areas with almost the same temperature as observed in the Arctic itself. Sources south of the polar front system can only contribute to high-altitude (or upper level) Arctic pollution. The amplitude and phase of long, planetary waves are important since they determine the position of the polar front, and provide conditions for meridional transport of air at certain longitudes

  20. Using magnetic and chemical measurements to detect atmospherically-derived metal pollution in artificial soils and metal uptake in plants

    International Nuclear Information System (INIS)

    Sapkota, B.; Cioppa, M.T.

    2012-01-01

    Quantification of potential effects of ambient atmospheric pollution on magnetic and chemical properties of soils and plants requires precise experimental studies. A controlled growth experiment assessing magnetic and chemical parameters was conducted within (controls) and outside (exposed) a greenhouse setting. Magnetic susceptibility (MS) measurements showed that while initial MS values were similar for the sample sets, the overall MS value of exposed soil was significantly greater than in controls, suggesting an additional input of Fe-containing particles. Scanning electron microscope images of the exposed soils revealed numerous angular magnetic particles and magnetic spherules typical of vehicular exhaust and combustion processes, respectively. Similarly, chemical analysis of plant roots showed that plants grown in the exposed soil had higher concentrations of Fe and heavy (toxic) metals than controls. This evidence suggests that atmospheric deposition contributed to the MS increase in exposed soils and increased metal uptake by plants grown in this soil. - Highlights: ► Magnetic susceptibility (MS) values increased in exposed soils during the growth. ► MS values in control soils decreased from their initial values during the growth. ► Decrease in MS values due to downwards migration of Fe particles, magnetic mineral transformations and Fe uptake by plants. ► Higher metal uptake in plants grown in exposed soils than those grown in controls. ► Atmospheric particulate deposition isolated as main contributor to these effects. - Variations in atmospheric particulate levels are measurable using magnetic and chemical techniques on soils and plant biomass, and suggest pollutant levels may be higher than previously recognized.

  1. Measurement of atmospheric pollutants

    Energy Technology Data Exchange (ETDEWEB)

    1975-01-01

    Studies of simplified methods of determining various atmospheric pollutants were performed. Measurements with Kitagawa detecting tubes were made in front of Shibuya Station in Tokyo on October 27, 1973. The number of cars that passed the site was counted then the nitrogen dioxide, sulfur dioxide, hydrocarbons and carbon monoxide content was determined. The number of cars was about 7000-12,000 between 9 AM and 6 PM. The heaviest traffic occurred around 10 am, and the least traffic occurred around 1 pm. A simulation experiment of smoking was also performed. A simplified model of smoking indicated that the concentration of CO in the mouth is as high as 10,000-15,000 ppM. The simplified measurement of sulfur dioxide and nitrogen dioxide by the use of a small piece of an alkaline filter was also investigated. A photoelectric colorimeter gave an excellent demonstration of the pollution due to SO/sub 2/ and NO/sub 2/. A simplified determination of NO/sub 2/ by the Saltzman method was also performed.

  2. Observations of atmospheric pollutants at Lhasa during 2014-2015: Pollution status and the influence of meteorological factors.

    Science.gov (United States)

    Duo, Bu; Cui, Lulu; Wang, Zhenzhen; Li, Rui; Zhang, Liwu; Fu, Hongbo; Chen, Jianmin; Zhang, Huifang; Qiong, A

    2018-01-01

    Atmospheric pollutants including SO 2 , NO 2 , CO, O 3 and inhalable particulate matter (PM 2.5 and PM 10 ) were monitored continuously from March 2014 to February 2015 to investigate characteristics of air pollution at Lhasa, Tibetan Plateau. Species exhibited similar seasonal variations except O 3 , with the peaks in winter but low valleys in summer. The maximum O 3 concentration was observed in spring, followed by summer, autumn, and winter. The positive correlation between O 3 and PM 10 in spring indicated similar sources of them, and was assumed to be turbulent transport. Temperature was the dominant meteorological factor for most species in spring. High temperature accelerates O 3 photochemistry, and favors air disturbance which is conductive to dust resuspension in spring. Relative humidity (RH) and atmospheric pressure were the main meteorological factors in summer. RH showed negative correlations with species, while atmospheric pressure posed opposite situation. Wind speed (WS) was the dominant meteorological factor in autumn, the negative correlations between WS and species indicated diffusion by wind. Most species showed non-significant correlations with meteorological factors in winter, indicating the dependence of pollution on source emission rather than restriction by meteorology. Pollution weather character indicated that emissions were from biomass burning and dust suspension, and meteorological factors also played an important role. Air stream injection from the stratosphere was observed during O 3 pollution period. Air parcels from Southwest Asia were observed during air pollution period in winter. An enhancement in air pollutants such as O 3 would be expected in the future, more attention should be given to countermeasures for prevention of air pollution in the future. Copyright © 2017. Published by Elsevier B.V.

  3. The propagation of light pollution in the atmosphere

    Science.gov (United States)

    Cinzano, P.; Falchi, F.

    2012-12-01

    Recent methods to map artificial night-sky brightness and stellar visibility across large territories or their distribution over the entire sky at any site are based on computation of the propagation of light pollution with Garstang models, a simplified solution of the radiative transfer problem in the atmosphere that allows fast computation by reducing it to a ray-tracing approach. They are accurate for a clear atmosphere, when a two-scattering approximation is acceptable, which is the most common situation. We present here up-to-date extended Garstang models (EGM), which provide a more general numerical solution for the radiative transfer problem applied to the propagation of light pollution in the atmosphere. We also present the LPTRAN software package, an application of EGM to high-resolution Defense Meteorological Satellite Program (DMSP) Operational Linescan System (OLS) satellite measurements of artificial light emission and to GTOPO30 (Global 30 Arcsecond) digital elevation data, which provides an up-to-date method to predict the artificial brightness distribution of the night sky at any site in the world at any visible wavelength for a broad range of atmospheric situations and the artificial radiation density in the atmosphere across the territory. EGM account for (i) multiple scattering, (ii) wavelengths from 250 nm to infrared, (iii) the Earth's curvature and its screening effects, (iv) site and source elevation, (v) many kinds of atmosphere with the possibility of custom set-up (e.g. including thermal inversion layers), (vi) a mix of different boundary-layer aerosols and tropospheric aerosols, with the possibility of custom set-up, (vii) up to five aerosol layers in the upper atmosphere, including fresh and aged volcanic dust and meteoric dust, (viii) variations of the scattering phase function with elevation, (ix) continuum and line gas absorption from many species, ozone included, (x) up to five cloud layers, (xi) wavelength-dependent bidirectional

  4. Effective pollutant emission heights for atmospheric transport modelling based on real-world information

    International Nuclear Information System (INIS)

    Pregger, Thomas; Friedrich, Rainer

    2009-01-01

    Emission data needed as input for the operation of atmospheric models should not only be spatially and temporally resolved. Another important feature is the effective emission height which significantly influences modelled concentration values. Unfortunately this information, which is especially relevant for large point sources, is usually not available and simple assumptions are often used in atmospheric models. As a contribution to improve knowledge on emission heights this paper provides typical default values for the driving parameters stack height and flue gas temperature, velocity and flow rate for different industrial sources. The results were derived from an analysis of the probably most comprehensive database of real-world stack information existing in Europe based on German industrial data. A bottom-up calculation of effective emission heights applying equations used for Gaussian dispersion models shows significant differences depending on source and air pollutant and compared to approaches currently used for atmospheric transport modelling. - The comprehensive analysis of real-world stack data provides detailed default parameter values for improving vertical emission distribution in atmospheric modelling

  5. Urban planning and interactions with atmospheric pollution in Arve valley

    Science.gov (United States)

    Langlois de Septenville, William; Cossart, Étienne

    2017-04-01

    Atmospheric pollution is a major concern of urbanised areas and territory managers have to conduct efficient policies to decrease population exposure and vulnerability. Even if pollution peaks are subject to an important mediatisation and to a large part of preventive actions, background pollution remains responsible of the largest sanitary effects. They depend on (1) the concentration and the duration of the exposure and (2) to the kind of pollutants considered. Many sources of pollutants can be identified in urban areas as heating, industry or traffic; and each of them generates specific particles. Currently, the major part of pollution risk studies focuses on modelling particle emissions and their dissemination in the environment. These kinds of studies highlight the hazard intensity and its spatiality, commonly named the hazard exposure. Another part of risk studies, less frequent, considers the vulnerability. Vulnerability is a complex concept that involves a wide range of scales and objects ranging from biophysical parameters to social characteristics. They notably concern accessibility to information, knowledge and perceptions about the risk. The Arve valley (south-east of France) is subject to heavy pollution concentrations. High levels recording in this area have imposed the implementation of an Atmosphere Protection Plan. This type of plan is triggered if a peak occurs and enforces provisional binding measures for polluters, such as highway speed limitation for traffic emissions. These measures are only focused on emissions and have no effect for reducing vulnerability and exposition, for a long- and short-term time scales. An opportunity to ensure this objective is to consider how local urban morphologies can combine exposition and vulnerability situations. Indeed, cities have been planned without taking into account atmospheric pollution and morphologies. This context may conduct to the increase in both of these two risk components and producing

  6. [Respiratory symptoms and atmospheric pollution and respiratory symptoms in the general population].

    Science.gov (United States)

    Simon, I; Charpin, D

    2010-06-01

    Epidemiological studies on air pollution have mainly been interested in the effects of short- or long-term exposure on patients suffering from respiratory illnesses. Fewer studies have addressed the acute effects of air pollution on respiratory symptoms in the general population. We conducted a review of the literature over the last 16years that has addressed the impact of atmospheric pollution on respiratory symptoms in the general population to estimate the magnitude of effect. The majority of studies demonstrated a significant association between exposure to air pollutants and the occurrence of respiratory symptoms, without any threshold. Although a link between atmospheric pollution and respiratory symptoms has been demonstrated, knowledge of the effects of specific air pollutants and the effect of pollution on particular vulnerable groups (infants, young children, the elderly) is still limited. There is a need for further studies in this area. Copyright 2010 SPLF. Published by Elsevier Masson SAS. All rights reserved.

  7. A 700 year record of combustion-derived pollution in northern Spain: Tools to identify the Holocene/Anthropocene transition in coastal environments

    International Nuclear Information System (INIS)

    Leorri, Eduardo; Mitra, Siddhartha; Irabien, María Jesús; Zimmerman, Andrew R.; Blake, William H.; Cearreta, Alejandro

    2014-01-01

    There is an uneven geographical distribution of historic records of atmospheric pollutants from SW Europe and those that exist are very limited in temporal extent. Alternative data source is required to understand temporal trends in human impacts on atmospheric pollution. Polycyclic aromatic hydrocarbons (PAHs), heavy metal content and stable Pb isotopic ratios in a sediment core from a salt marsh in northern Spain were used to reconstruct the regional history of contaminant inputs over the last 700 years. Pre-1800s concentrations of Pb and PAHs represented baseline concentrations, i.e. pre-Industrial, conditions. During the initial stages of the Industrial Revolution, 1800s to 1860s, PAH concentrations increased by a factor of about two above baseline levels in the sediment column. By the 1930s, PAH levels reached ca. 10 times pre-Industrial levels and, along with Pb, reached a peak at ca. 1975 CE. Since then, sedimentary PAH and Pb concentrations decreased significantly. A combination of PAH isomer and Pb stable isotope ratios suggests that the contaminant sources are regional, likely derived partially from wood, but mainly coal used by the metallurgic industry in the Basque country since the 1800s and until the 1970s when leaded petrol saw increased use. This chronology of regional atmosphere-derived pollution expands current southwest Europe emission records and shows coastal salt marsh sediments to be useful in reconstructing the Anthropocene. - Highlights: • Historic records of atmospheric pollutant emissions in SW Europe are needed. • PAH and Pb concentrations and ratios from a north Spain salt marsh core were used. • Atmosphere emissions mainly from regional coal burning increased in the early 1800s. • Emissions associated with leaded gasoline peaked in 1975 CE. • The results suggest 1800 CE as the Holocene/Anthropocene transition

  8. A 700 year record of combustion-derived pollution in northern Spain: Tools to identify the Holocene/Anthropocene transition in coastal environments

    Energy Technology Data Exchange (ETDEWEB)

    Leorri, Eduardo, E-mail: leorrie@ecu.edu [Department of Geological Sciences, East Carolina University, Graham Building 103B, Greenville, NC 27858 (United States); Mitra, Siddhartha, E-mail: mitras@ecu.edu [Department of Geological Sciences, East Carolina University, Graham Building 103B, Greenville, NC 27858 (United States); Irabien, María Jesús, E-mail: mariajesus.irabien@ehu.es [Departamento de Mineralogía y Petrología, Facultad de Ciencia y Tecnología, Universidad del País Vasco UPV/EHU, Apartado 644, 48080 Bilbao (Spain); Zimmerman, Andrew R., E-mail: azimmer@ufl.edu [Department of Geological Sciences, University of Florida, 241 Williamson Hall, P.O. Box 112120, Gainesville, FL 32611 (United States); Blake, William H., E-mail: william.blake@plymouth.ac.uk [Consolidated Radioisotope Facility, University of Plymouth, Plymouth (United Kingdom); Cearreta, Alejandro, E-mail: alejandro.cearreta@ehu.es [Departamento de Estratigrafía y Paleontología, Facultad de Ciencia y Tecnología, Universidad del País Vasco UPV/EHU, Apartado 644, 48080 Bilbao (Spain)

    2014-02-01

    There is an uneven geographical distribution of historic records of atmospheric pollutants from SW Europe and those that exist are very limited in temporal extent. Alternative data source is required to understand temporal trends in human impacts on atmospheric pollution. Polycyclic aromatic hydrocarbons (PAHs), heavy metal content and stable Pb isotopic ratios in a sediment core from a salt marsh in northern Spain were used to reconstruct the regional history of contaminant inputs over the last 700 years. Pre-1800s concentrations of Pb and PAHs represented baseline concentrations, i.e. pre-Industrial, conditions. During the initial stages of the Industrial Revolution, 1800s to 1860s, PAH concentrations increased by a factor of about two above baseline levels in the sediment column. By the 1930s, PAH levels reached ca. 10 times pre-Industrial levels and, along with Pb, reached a peak at ca. 1975 CE. Since then, sedimentary PAH and Pb concentrations decreased significantly. A combination of PAH isomer and Pb stable isotope ratios suggests that the contaminant sources are regional, likely derived partially from wood, but mainly coal used by the metallurgic industry in the Basque country since the 1800s and until the 1970s when leaded petrol saw increased use. This chronology of regional atmosphere-derived pollution expands current southwest Europe emission records and shows coastal salt marsh sediments to be useful in reconstructing the Anthropocene. - Highlights: • Historic records of atmospheric pollutant emissions in SW Europe are needed. • PAH and Pb concentrations and ratios from a north Spain salt marsh core were used. • Atmosphere emissions mainly from regional coal burning increased in the early 1800s. • Emissions associated with leaded gasoline peaked in 1975 CE. • The results suggest 1800 CE as the Holocene/Anthropocene transition.

  9. Atmospheric corrosion in Gran Canaria specifically meteorological and pollution conditions

    International Nuclear Information System (INIS)

    Gonzalez, J.E.G.; Valles, M.L.; Mirza R, J.C.

    1998-01-01

    Carbon steel, copper, zinc and aluminium samples were exposed in different sizes with known ambient parameters in Gran Canaria Island and atmospheric corrosion was investigated. Weight-loss measurements used to determine corrosion damage were complemented with metallographic and XP S determination in order to characterize the structure and morphology of surface corrosion products. The ambient aggressiveness could be well evaluated from meteorological and pollution data. All atmospheric corrosion and environmental data were statistically processed for establishing general corrosion damage functions for carbon steel, copper, aluminium and zinc in terms of Gran Canaria extreme meteorological and pollution parameters. (Author)

  10. Remote measurement of atmospheric pollutants with laser techniques

    Energy Technology Data Exchange (ETDEWEB)

    Corio, W; Querzola, B; Zanzottera, E

    1979-03-01

    Laser techniques for the remote sensing of atmospheric pollutants are reviewed, with attention given to lidars based on Rayleigh and Mie scattering, the Raman effect, or fluorescent scattering. Emphasis is placed on differential absorption lidars, which rely on Rayleigh or Mie scattering for measurements made in the IR or in the visible-UV range, respectively. A comprehensive air pollution monitoring program based on differential absorption lidars, together with systems using fluorescent backscattering and absorption measurements with topographic backscattering, is described.

  11. Natural sources of gaseous pollutants in the atmosphere

    Energy Technology Data Exchange (ETDEWEB)

    Altshuller, A P

    1958-01-01

    Various gaseous pollutants including ozone, nitrous oxide, nitric oxide, nitrogen dioxide, methane, hydrogen, formaldehyde, ammonia, hydrogen sulfide, mercaptans, chlorine compounds and free radicals can be formed by natural processes such as ultraviolet photochemical processes in the upper atmosphere and microbiological processes. The modes of formation and destruction of these gases, especially of their concentrations in the atmosphere, and the various reactions in which these gases can participate with each other are discussed in detail. 114 references.

  12. Usefulness of the infrared heterodyne radiometer in remote sensing of atmospheric pollutants.

    Science.gov (United States)

    Menzies, R. T.; Shumate, M. S.

    1971-01-01

    The application of narrow-band optical receivers to the problem of sensing atmospheric pollution is discussed. The emission/absorption lines of many major atmospheric pollutant molecules overlap the operating frequency bands of CO2 laser and CO laser heterodyne receivers. Several remote pollution sensing systems which are based upon utilization of these spectral overlaps are described, and an analysis of their potential is presented. The possibility of using other lasers (e.g.: the PbSnTe tunable diode laser) as local oscillators is also considered. Results of laboratory experiments with a CO2 laser heterodyne radiometer are presented.

  13. Atmospheric pollution over the eastern Mediterranean during summer - a review

    Science.gov (United States)

    Dayan, Uri; Ricaud, Philippe; Zbinden, Régina; Dulac, François

    2017-11-01

    The eastern Mediterranean (EM) is one of the regions in the world where elevated concentrations of primary and secondary gaseous air pollutants have been reported frequently, mainly in summer. This review discusses published studies of the atmospheric dispersion and transport conditions characterizing this region during the summer, followed by a description of some essential studies dealing with the corresponding concentrations of air pollutants such as ozone, carbon monoxide, total reactive nitrogen, methane, and sulfate aerosols observed there. The interlaced relationship between the downward motion of the subsiding air aloft induced by global circulation systems affecting the EM and the depth of the Persian Trough, a low-pressure trough that extends from the Asian monsoon at the surface controlling the spatiotemporal distribution of the mixed boundary layer during summer, is discussed. The strength of the wind flow within the mixed layer and its depth affect much the amount of pollutants transported and determine the potential of the atmosphere to disperse contaminants off their origins in the EM. The reduced mixed layer and the accompanying weak westerlies, characterizing the summer in this region, led to reduced ventilation rates, preventing an effective dilution of the contaminants. Several studies pointing at specific local (e.g., ventilation rates) and regional peculiarities (long-range transport) enhancing the build-up of air pollutant concentrations are presented. Tropospheric ozone (O3) concentrations observed in the summer over the EM are among the highest over the Northern Hemisphere. The three essential processes controlling its formation (i.e., long-range transport of polluted air masses, dynamic subsidence at mid-tropospheric levels, and stratosphere-to-troposphere exchange) are reviewed. Airborne campaigns and satellite-borne initiatives have indicated that the concentration values of reactive nitrogen identified as precursors in the formation of O

  14. Potential atmospheric pollution from the Invergordon industrial complex

    Energy Technology Data Exchange (ETDEWEB)

    Neustein, S A; Danby, N P

    1971-11-01

    The main atmospheric pollutants from the Invergordon complex will be fluorine and hydrogen fluoride from the aluminum smelter and sulfur dioxide and hydrocarbons from the oil refinery. Both acute and chronic tree damage is expected. The effects of F and SO/sub 2/ on the trees via the soil is expected to be insignificant. Acute tree damage results from high concentrations of pollutants as a result of meteorological conditions or industrial cleansing failure. Chronic tree damage results from long term low level pollution. Broad leaved trees are not regarded as susceptible to chronic pollution. All the conifers are susceptible. Clean air sampling has begun in order to provide before and after comparison. Foliage samplers will be taken for a radius of 16,000 m. A survey of lichens has been completed. Lichenology may assist in discrimination between F and SO/sub 2/ injuries.

  15. Linking Atmospheric Pollution to Cryospheric Changes over the Third Pole

    Science.gov (United States)

    Kang, S.; Zhang, Q.; Ji, Z.; Li, Y.; Chen, J.; Zhang, G.; Li, C.; Cong, Z.; Chen, P.; Guo, J.; Huang, J.; Tripathee, L.; Rupakheti, D.; Li, X.; Zhang, Y.; Panday, A. K.; Rupakheti, M.

    2016-12-01

    Known as "the Third Pole" (TP), the Tibetan Plateau and surrounding mountains hold the largest aggregate of glaciers outside the pole regions. Recent monitoring and projection indicated an accelerated glacier decline and increasing glacier runoff. The long-range transport of South Asian atmospheric pollutants, including light absorbing impurities (LAIs) such as black carbon (BC) and mineral dust (MD), can absorb the solar radiation in the atmosphere and reduce albedo after being deposited onto the cryosphere, thereby promoting glacier and snow melt. A coordinated atmospheric pollution monitoring network has been launched covering the TP with emphasis on trans-Himalayan transects since 2013. TSP were collected for 24h at an interval of 3-6 days. BC/OC, polycyclic aromatic hydrocarbons (PAHs) and heavy metals were measured. Results reveal a consistent decrease in almost all analyzed parameters from south to north across the Himalayas. Geochemical signatures of carbonaceous aerosols indicate dominant sources of biomass burning and vehicle exhaust, in line with results of PAHs. Integrated analysis of satellite images and air mass trajectories suggest that the trans-boundary air pollution occurred episodically and concentrated in pre-monsoon seasons via upper air circulation, through-valley wind, and local convection. Simulation results showed that carbonaceous aerosols produced positive/negative shortwave radiative forcing in the atmosphere/ground surface. Aerosols increased surface air temperatures by 0.1-0.5° over the TP and decreased temperatures in South Asia during the monsoon season. Surface snow/ice samples were collected from benchmark glaciers to estimate the impacts of LAIs on glacier melt with model assistance. BC (37%) and MD (32%) contribute to the summer melting of Laohugou Glacier in the northern TP. MD (38%) contributed more glacier melt than BC (11%) on Zhadang Glacier in the southern TP. In the southeastern TP, BC and MD contribute to 30% of the

  16. On the calculation of atmospheric thermal pollution resulted from a flat area source

    International Nuclear Information System (INIS)

    Perkauskas, D.Ch.; Senuta, K.A.

    1984-01-01

    A spatial distribution of thermal atmospheric pollution from a flat area source - a great city or a lake-cooler of NPP was investigated. The numerical solution obtained lets to evaluate the horizontal and vertical spreading of the thermal atmospheric pollution by the different wind velocities in dependence of the inhomogeneities in humidity of the earth's surface

  17. Effects of atmospheric pollution on vegetation

    Energy Technology Data Exchange (ETDEWEB)

    Metcalfe, C R

    1953-10-10

    In September, 1953, two sections of the British Association (Botany and Forestry) jointly discussed the effects of various components of air pollution. Conclusions reached included the position that the symptoms of ill health in plants that have been subjected to a polluted fog are due not so much to reduction in availability of light as to the presence of toxic substances in the atmosphere. Examples of these symptoms include shedding of flowers and leaves, blackening and death of buds and flowers, scorching of foliage, and complete destruction of more sensitive plants. Sulfur dioxide was identified as one of the more important toxic substances. Practical remedies for the problem were discussed, and the currently-known dose-response relationships (concentrations in excess of 0.5 ppm were known to cause lesions on some plants) were defined. Instances of reduced growth of crop plants and the inhibition of development of lichens and mosses were recounted. The complex relationships between soil condition and air pollution of the growth of plants were discussed.

  18. Mathematical models for atmospheric pollutants. Appendix A. Elements of meteorology. Final report

    International Nuclear Information System (INIS)

    Drake, R.L.; Laulainen, N.S.

    1979-08-01

    The meteorological elements that are important in the transport and fate of airborne pollutants are summarized. The summary consists of descriptions of the thermal, water, kinematic and dynamic structures of the atmosphere, the time and space scale classifications of atmospheric motions, and modifications of pollutant plumes as they pass over nonhomogeneous surface conditions and complex terrain. The discussions consider the atmospheric thermal layers and their stability, formation of clouds and the production of rain and snow, the movement of air masses and weather fronts, the horizontal winds in the planetary boundary layer, and wind profiles over transition zones and complex terrain

  19. A quarter century of biomonitoring atmospheric pollution in the Czech Republic.

    Science.gov (United States)

    Suchara, Ivan; Sucharová, Julie; Holá, Marie

    2017-05-01

    The Czech Republic (CZ) had extremely high emissions and atmospheric deposition of pollutants in the second half of the 1980s. Since the beginning of the 1990s, moss, spruce bark and forest floor humus have been used as bioindicators of air quality. In the first half of the 1990s, seven larger areas were found to be affected by high atmospheric deposition loads. Six of these "hot spots" were caused by industrial pollution sources, mainly situated in coal basins in the NW and NE part of the country, and one large area in the SE was affected by increased deposition loads of eroded soil particles. After restructuring of industry in CZ, these hot spots were substantially reduced or even disappeared between 1995 and 2000. Since 2000, only two larger areas with slightly increased levels of industrial pollutant deposition and a larger area affected by soil dust have repeatedly been identified by biomonitoring. The distribution of lead isotope ratios in moss showed the main deposition zones around important emission sources. Very high SO 2 emissions led to extreme acidity of spruce bark extracts (pH of about 2.3) at the end of the 1980s. The rate of increasing bark pH was strikingly similar to the rate of recovery of acid wet deposition measured at forest stations in CZ. By about 2005, when the median pH value in bark increased to about 3.2, the re-colonisation of trees by several epiphyte lichen species was observed throughout CZ. An increase in the accumulation of Chernobyl-derived 137 Cs in bark was detected at about ten sites affected by precipitation during the time when radioactive plumes crossed CZ (1986). Accumulated deposition loads in forest floor humus corresponded to the position of the moss and bark hot spots.

  20. Study on the total amount control of atmospheric pollutant based on GIS.

    Science.gov (United States)

    Wang, Jian-Ping; Guo, Xi-Kun

    2005-08-01

    To provide effective environmental management for total amount control of atmospheric pollutants. An atmospheric diffusion model of sulfur dioxide on the surface of the earth was established and tested in Shantou of Guangdong Province on the basis of an overall assessment of regional natural environment, social economic state of development, pollution sources and atmospheric environmental quality. Compared with actual monitoring results in a studied region, simulation values fell within the range of two times of error and were evenly distributed in the two sides of the monitored values. Predicted with the largest emission model method, the largest emission of sulfur dioxide would be 54,279.792 tons per year in 2010. The mathematical model established and revised on the basis of GIS is more rational and suitable for the regional characteristics of total amount control of air pollutants.

  1. Spectroradiometric inspection of nuclear pollution in the atmosphere based on photochemical effects

    Science.gov (United States)

    Chistyakova, Liliya K.; Kopytin, Yurii D.

    2005-07-01

    Results of theoretical and experimental investigations of remote monitoring methods based on secondary radioactivity effects including anomalous gaseous fields and their emissions in optical and microwave ranges are discussed. The feasibility of remote registration of secondary emission and absorption spectra from weakly ionized regions in the atmosphere above nuclear power engineering objects, dumps, and tailings dumps of nuclear wastes are examined. Based on the literature data on the excess concentrations of aerosol and gaseous components produced in radiation fields above their background levels, the diffusion parameters of radioactive emissions in the atmosphere are evaluated. The methods under consideration are shown to be promising for ecological monitoring of atmospheric radioactive pollution. High sensitivities of these methods enable pollutants to be detected at long distances. Simultaneous use of passive and active methods gives additional information on the parameters of radioactive pollution.

  2. Concentrations and (delta)13C values of atmospheric CO2 from oceanic atmosphere through time: polluted and non-polluted areas

    International Nuclear Information System (INIS)

    Longinelli, Antonio; Selmo, Enrico; Lenaz, Renzo; Ori, Carlo

    2005-01-01

    CO 2 is one of the primary agents of global climate changes. The increase of atmospheric CO 2 concentration is essentially related to human-induced emissions and, particularly, to the burning of fossil fuel whose (delta) 13 C values are quite negative. Consequently, an increase of the CO 2 concentration in the atmosphere should be paralleled by a decrease of its (delta) 13 C. Continuous and/or spot measurements of CO 2 concentrations were repeatedly carried out during the last decade and in the same period of the year along hemispheric courses from Italy to Antarctica on a vessel of the Italian National Research Program in Antarctica. During these expeditions, discrete air samples were also collected in 4-l Pyrex flasks in order to carry out precise carbon isotope analyses on atmospheric CO 2 from different areas, including theoretically 'clean' open ocean areas, with the main purpose of comparing these open ocean results with the results obtained by the National Oceanic and Atmospheric Administration/World Meteorological Organization (NOAA/WMO) at land-based stations. According to the data obtained for these two variables, a relatively large atmospheric pollution is apparent in the Mediterranean area where the CO 2 concentration has reached the value of 384 ppmv while quite negative (delta) 13 C values have been measured only occasionally. In this area, southerly winds probably help to reduce the effect of atmospheric pollution even though, despite a large variability of CO 2 concentrations, these values are consistently higher than those measured in open ocean areas by a few ppmv to about 10 ppmv. A marked, though non-continuous, pollution is apparent in the area of the Bab-el-Mandeb strait where (delta) 13 C values considerably more negative than in the Central and Southern Red Sea were measured. The concentration of atmospheric CO 2 over the Central Indian Ocean increased from about 361 ppmv at the end of 1996 to about 373 ppmv at the end of 2003 (mean growth

  3. [Characteristics of Winter Atmospheric Mixing Layer Height in Beijing-Tianjin-Hebei Region and Their Relationship with the Atmospheric Pollution].

    Science.gov (United States)

    Li, Meng; Tang, Gui-qian; Huang, Jun; Liu, Zi-rui; An, Jun-lin; Wang, Yue-si

    2015-06-01

    Atmospheric mixing layer height (MLH) is one of the main factors affecting the atmospheric diffusion and plays an important role in air quality assessment and distribution of the pollutants. Based on the ceilometers data, this paper has made synchronous observation on MLH in Beijing-Tianjin-Hebei region (Beijing, Tianjin, Shijiazhuang and Qinhuangdao) in heavy polluted February 2014 and analyzed the respective overall change and its regional features. Results show that in February 2014,the average of mixing layer height in Qinhuangdao is the highest, up to 865 +/- 268 m, and in Shijiazhuang is the lowest (568 +/- 207 m), Beijing's and Tianjin's are in between, 818 +/- 319 m and 834 +/- 334 m respectively; Combined with the meteorological data, we find that radiation and wind speed are main factors of the mixing layer height; The relationship between the particle concentration and mixing layer height in four sites suggests that mixing layer is less than 800 m, concentration of fine particulate matter in four sites will exceed the national standard (GB 3095-2012, 75 microg x m(-3)). During the period of observation, the proportion of days that mixing layer is less than 800 m in Beijing, Tianjin, Shijiazhuang and Qinhuangdao are 50%, 43%, 80% and 50% respectively. Shijiazhuang though nearly formation contaminant concentration is high, within the atmospheric mixed layer pollutant load is not high. Unfavorable atmospheric diffusion conditions are the main causes of heavy pollution in Shijiazhuang for a long time. The results of the study are of great significance for cognitive Beijing-Tianjin-Hebei area pollution distribution, and can provide a scientific reference for reasonable distribution of regional pollution sources.

  4. Tundra uptake of atmospheric elemental mercury drives Arctic mercury pollution.

    Science.gov (United States)

    Obrist, Daniel; Agnan, Yannick; Jiskra, Martin; Olson, Christine L; Colegrove, Dominique P; Hueber, Jacques; Moore, Christopher W; Sonke, Jeroen E; Helmig, Detlev

    2017-07-12

    Anthropogenic activities have led to large-scale mercury (Hg) pollution in the Arctic. It has been suggested that sea-salt-induced chemical cycling of Hg (through 'atmospheric mercury depletion events', or AMDEs) and wet deposition via precipitation are sources of Hg to the Arctic in its oxidized form (Hg(ii)). However, there is little evidence for the occurrence of AMDEs outside of coastal regions, and their importance to net Hg deposition has been questioned. Furthermore, wet-deposition measurements in the Arctic showed some of the lowest levels of Hg deposition via precipitation worldwide, raising questions as to the sources of high Arctic Hg loading. Here we present a comprehensive Hg-deposition mass-balance study, and show that most of the Hg (about 70%) in the interior Arctic tundra is derived from gaseous elemental Hg (Hg(0)) deposition, with only minor contributions from the deposition of Hg(ii) via precipitation or AMDEs. We find that deposition of Hg(0)-the form ubiquitously present in the global atmosphere-occurs throughout the year, and that it is enhanced in summer through the uptake of Hg(0) by vegetation. Tundra uptake of gaseous Hg(0) leads to high soil Hg concentrations, with Hg masses greatly exceeding the levels found in temperate soils. Our concurrent Hg stable isotope measurements in the atmosphere, snowpack, vegetation and soils support our finding that Hg(0) dominates as a source to the tundra. Hg concentration and stable isotope data from an inland-to-coastal transect show high soil Hg concentrations consistently derived from Hg(0), suggesting that the Arctic tundra might be a globally important Hg sink. We suggest that the high tundra soil Hg concentrations might also explain why Arctic rivers annually transport large amounts of Hg to the Arctic Ocean.

  5. Atmospheric pollution history at Linfen (China) uncovered by magnetic and chemical parameters of sediments from a water reservoir

    International Nuclear Information System (INIS)

    Ma, Mingming; Hu, Shouyun; Cao, Liwan; Appel, Erwin; Wang, Longsheng

    2015-01-01

    We studied magnetic and chemical parameters of sediments from sediments of a water reservoir at Linfen (China) in order to quantitatively reconstruct the atmospheric pollution history in this region. The results show that the main magnetic phases are magnetite and maghemite originating from the surrounding catchment and from anthropogenic activities, and there is a significant positive relationship between magnetic concentration parameters and heavy metals concentrations, indicating that magnetic proxies can be used to monitor the anthropogenic pollution. In order to uncover the atmospheric pollution history, we combined the known events of environmental improvement with variations of magnetic susceptibility (χ) and heavy metals along the cores to obtain a detailed chronological framework. In addition, air comprehensive pollution index (ACPI) was reconstructed from regression equation among magnetic and chemical parameters as well as atmospheric monitoring data. Based on these results, the atmospheric pollution history was successfully reconstructed. - Highlights: • Magnetic proxies can be used to monitor the heavy mental pollution in sediments. • Accurate age model was obtained using known events of environmental improvement. • Regression equation was obtained among sediment records and monitoring data. • Atmospheric pollution history was quantitatively reconstructed. - Atmospheric pollution history was quantitatively reconstructed using magnetic and chemical records of reservoir sediments combined with atmospheric monitoring data

  6. The role of forest in mitigating the impact of atmospheric dust pollution in a mixed landscape.

    Science.gov (United States)

    Santos, Artur; Pinho, Pedro; Munzi, Silvana; Botelho, Maria João; Palma-Oliveira, José Manuel; Branquinho, Cristina

    2017-05-01

    Atmospheric dust pollution, especially particulate matter below 2.5 μm, causes 3.3 million premature deaths per year worldwide. Although pollution sources are increasingly well known, the role of ecosystems in mitigating their impact is still poorly known. Our objective was to investigate the role of forests located in the surrounding of industrial and urban areas in reducing atmospheric dust pollution. This was tested using lichen transplants as biomonitors in a Mediterranean regional area with high levels of dry deposition. After a multivariate analysis, we have modeled the maximum pollution load expected for each site taking into consideration nearby pollutant sources. The difference between maximum expected pollution load and the observed values was explained by the deposition in nearby forests. Both the dust pollution and the ameliorating effect of forested areas were then mapped. The results showed that forest located nearby pollution sources plays an important role in reducing atmospheric dust pollution, highlighting their importance in the provision of the ecosystem service of air purification.

  7. Using an epiphytic moss to identify previously unknown sources of atmospheric cadmium pollution

    International Nuclear Information System (INIS)

    Donovan, Geoffrey H.; Jovan, Sarah E.; Gatziolis, Demetrios; Burstyn, Igor; Michael, Yvonne L.; Amacher, Michael C.; Monleon, Vicente J.

    2016-01-01

    Urban networks of air-quality monitors are often too widely spaced to identify sources of air pollutants, especially if they do not disperse far from emission sources. The objectives of this study were to test the use of moss bio-indicators to develop a fine-scale map of atmospherically-derived cadmium and to identify the sources of cadmium in a complex urban setting. We collected 346 samples of the moss Orthotrichum lyellii from deciduous trees in December, 2013 using a modified randomized grid-based sampling strategy across Portland, Oregon. We estimated a spatial linear model of moss cadmium levels and predicted cadmium on a 50 m grid across the city. Cadmium levels in moss were positively correlated with proximity to two stained-glass manufacturers, proximity to the Oregon–Washington border, and percent industrial land in a 500 m buffer, and negatively correlated with percent residential land in a 500 m buffer. The maps showed very high concentrations of cadmium around the two stained-glass manufacturers, neither of which were known to environmental regulators as cadmium emitters. In addition, in response to our findings, the Oregon Department of Environmental Quality placed an instrumental monitor 120 m from the larger stained-glass manufacturer in October, 2015. The monthly average atmospheric cadmium concentration was 29.4 ng/m"3, which is 49 times higher than Oregon's benchmark of 0.6 ng/m"3, and high enough to pose a health risk from even short-term exposure. Both stained-glass manufacturers voluntarily stopped using cadmium after the monitoring results were made public, and the monthly average cadmium levels precipitously dropped to 1.1 ng/m"3 for stained-glass manufacturer #1 and 0.67 ng/m"3 for stained-glass manufacturer #2. - Highlights: • Bio-indicators are a valid method for measuring atmospheric pollutants • We used moss to map atmospheric cadmium in Portland, Oregon • Using a spatial linear model, we identified two stained

  8. Epiphytic lichen diversity on dead and dying conifers under different levels of atmospheric pollution

    International Nuclear Information System (INIS)

    Hauck, Markus

    2005-01-01

    Based on literature data, epiphytic lichen abundance was comparably studied in montane woodlands on healthy versus dead or dying conifers of Europe and North America in areas with different levels of atmospheric pollution. Study sites comprised Picea abies forests in the Harz Mountains and in the northern Alps, Germany, Picea rubens-Abies balsamea forests on Whiteface Mountain, Adirondacks, New York, U.S.A. and Picea engelmannii-Abies lasiocarpa forests in the Salish Mountains, Montana, U.S.A. Detrended correspondence analysis showed that epiphytic lichen vegetation differed more between healthy and dead or dying trees at high- versus low-polluted sites. This is attributed to greater differences in chemical habitat conditions between trees of different vitality in highly polluted areas. Based on these results, a hypothetical model of relative importance of site factors for small-scale variation of epiphytic lichen abundance versus atmospheric pollutant load is discussed. - Epiphytic lichen diversity differs increasingly between healthy and dead or dying conifers with increasing atmospheric pollutant load

  9. Atmospheric particulate pollution in Kenitra (Morocco)

    International Nuclear Information System (INIS)

    Zghaid, Mustapha; Noack, Yves; Boukla, Moussa; Benyaich, Fouad

    2009-01-01

    Cities of Morocco are exposed to a high atmospheric particulate pollution due to automobile traffic, industrialization, but also to soil dusts (in relation with aridity and desert proximity). Monitoring networks and data about air pollution still rare. The present study is a preliminary work about particulate and heavy metals pollution in Kenitra city. Aerosols had been collected with a PM10 sampler (Partisol), a dichotomous sampler (P M2.5 and P M2.5-10 fractions) and stacked filter unit (Gent type) with a fine fraction (below 2.5 um) and a coarse fraction. In summer, the average PM10 concentration is near 80 u g/N m 3 , above the EEC rule and OMS recommendations, but similar to some other african towns. The ratio P M2.5/PM 10 is low (below 0.5), with seasonal variation in relation with meteorology. The lead and nickel concentrations are also very low, in relation with the use of leaded gasoline and the oldness of many vehicles. This preliminary work reveals high levels of pollution (especially PM10, Pb and Ni) in the town of Kenitra. The major sources are traffic, soil dusts and resuspension of deposited particles. It is necessary to develop monitoring network and sanitary and and environmental impact studies in these cities [fr

  10. ROCKY EXTRASOLAR PLANETARY COMPOSITIONS DERIVED FROM EXTERNALLY POLLUTED WHITE DWARFS

    International Nuclear Information System (INIS)

    Klein, B.; Jura, M.; Zuckerman, B.; Koester, D.

    2011-01-01

    We report Keck High Resolution Echelle Spectrometer data and model atmosphere analysis of two helium-dominated white dwarfs, PG1225–079 and HS2253+8023, whose heavy pollutions most likely derive from the accretion of terrestrial-type planet(esimal)s. For each system, the minimum accreted mass is ∼10 22 g, that of a large asteroid. In PG1225–079, Mg, Cr, Mn, Fe, and Ni have abundance ratios similar to bulk Earth values, while we measure four refractory elements, Ca, Sc, Ti, and V, all at a factor of ∼2-3 higher abundance than in the bulk Earth. For HS2253+8023 the swallowed material was compositionally similar to bulk Earth in being more than 85% by mass in the major element species, O, Mg, Si, and Fe, and with abundances in the distinctive proportions of mineral oxides—compelling evidence for an origin in a rocky parent body. Including previous studies we now know of four heavily polluted white dwarfs where the measured oxygen and hydrogen are consistent with the view that the parents' bodies formed with little ice, interior to any snow line in their nebular environments. The growing handful of polluted white dwarf systems with comprehensive abundance measurements form a baseline for characterizing rocky exoplanet compositions that can be compared with bulk Earth.

  11. Atmospheric ventilation corridors and coefficients for pollution plume ...

    African Journals Online (AJOL)

    This study presents a comparative investigation of atmospheric ventilation corridors and coefficients for gaseous pollution plume released from an isolated industrial facility into the ambient air of the host community in Ile-Ife suburb, southwest Nigeria. For the months of September to December in the year 2012 and 2013, ...

  12. Is atmospheric pollution exposure during pregnancy associated with individual and contextual characteristics? A nationwide study in France.

    Science.gov (United States)

    Ouidir, Marion; Lepeule, Johanna; Siroux, Valérie; Malherbe, Laure; Meleux, Frederik; Rivière, Emmanuel; Launay, Ludivine; Zaros, Cécile; Cheminat, Marie; Charles, Marie-Aline; Slama, Rémy

    2017-10-01

    Exposure to atmospheric pollutants is a danger for the health of pregnant mother and children. Our objective was to identify individual (socioeconomic and behavioural) and contextual factors associated with atmospheric pollution pregnancy exposure at the nationwide level. Among 14 921 women from the French nationwide ELFE (French Longitudinal Study of Children) mother-child cohort recruited in 2011, outdoor exposure levels of PM 2.5 , PM 10 (particulate matter atmospheric pollutants with individual (maternal age, body mass index, parity, education level, relationship status, smoking status) and contextual (European Deprivation Index, urbanisation level) factors. Patterns of associations were globally similar across pollutants. For the CART approach, the highest tertile of exposure included mainly women not in a relationship living in urban and socially deprived areas, with lower education level. Linear regression models identified different determinants of atmospheric pollutants exposure according to the residential urbanisation level. In urban areas, atmospheric pollutants exposure increased with social deprivation, while in rural areas a U-shaped relationship was observed. We highlighted social inequalities in atmospheric pollutants exposure according to contextual characteristics such as urbanisation level and social deprivation and also according to individual characteristics such as education, being in a relationship and smoking status. In French urban areas, pregnant women from the most deprived neighbourhoods were those most exposed to health-threatening atmospheric pollutants. © Article author(s) (or their employer(s) unless otherwise stated in the text of the article) 2017. All rights reserved. No commercial use is permitted unless otherwise expressly granted.

  13. Peculiarities of general atmospheric circulation above Kazakhstan and trans-bordering transfer of polluted substances

    International Nuclear Information System (INIS)

    Turulina, G.K.; Muradov, M.A.; Sal'nikov, V.G.; Bogacev, V.P.

    1997-01-01

    Essential information is gathered for analysis and typification of atmospheric processes observed above Kazakhstan during studied period (1964-1986). Peculiarities of atmospheric processes and trans-bordering transfer of polluted substances above Kazakhstan territory are researched. Received data indicate on actuality of the problem for Republic of Kazakhstan and necessity of signing of the International Convention on trans-bordering pollution with purpose of integration in fulfillment of International Program of observation and assessment of spreading of air pollutants in Europe. (author)

  14. Transboundary radioactive and chemical pollution simulation using an atmospheric/marine predicting system

    International Nuclear Information System (INIS)

    Telenta, B.; Antic, D.

    2001-01-01

    The atmospheric models can be used to simulate the transport of contaminants in typical accidental cases and for realistic meteorological conditions. Some numerical models for weather forecast can be used for near to real simulations of propagation of radioactive nuclides or classical chemical pollutants to the atmosphere. The various meteorological parameters are taken into account and various meteorological conditions, even complex ones, can be analyzed. The models can be used for very well assessment of the airborne pollution from energy sources and industrial installations, for comparative studies and for safety analysis. This report describes an proposal for a project of the transboundary pollution simulation, that can be used for the East Mediterranean Region. The project is based on the numerical models developed in the in simulating of the Chernobyl accident and similar hypothetical cases. The study is based on an atmospheric models developed in Euro-Mediterranean Centre on Insular Coastal Dynamics (ICoD), Foundation for International Studies, Valeta, Malta

  15. Ozone and atmospheric pollution at synoptic scale: the monitoring network Paes

    International Nuclear Information System (INIS)

    Gheusi, F.; Chevalier, A.; Delmas, R.; Athier, G.; Bouchou, P.; Cousin, J.M.; Meyerfeld, Y.; Laj, P.; Sellegri, K.; Ancellet, G.

    2007-01-01

    Ozone as an environmental concern extends beyond the questions usually covered by media - stratospheric ozone depletion and urban pollution peaks. Strong expositions to this pollutant are frequent even far from pollution sources, and the background tropospheric content of ozone has been growing fivefold over the last century. In response to this concern at the French national scale, formerly independent monitoring stations have been coordinated since 2004 in a structured network: Paes (French acronym for atmospheric pollution at synoptic scale). The data are put in free access online. (authors)

  16. Terrestrial mosses as biomonitors of atmospheric POPs pollution: a review.

    Science.gov (United States)

    Harmens, H; Foan, L; Simon, V; Mills, G

    2013-02-01

    Worldwide there is concern about the continuing release of persistent organic pollutants (POPs) into the environment. In this study we review the application of mosses as biomonitors of atmospheric deposition of POPs. Examples in the literature show that mosses are suitable organisms to monitor spatial patterns and temporal trends of atmospheric concentrations or deposition of POPs. These examples include polycyclic aromatic hydrocarbons (PAHs), polychlorobiphenyls (PCBs), dioxins and furans (PCDD/Fs), and polybrominated diphenyl ethers (PBDEs). The majority of studies report on PAHs concentrations in mosses and relative few studies have been conducted on other POPs. So far, many studies have focused on spatial patterns around pollution sources or the concentration in mosses in remote areas such as the polar regions, as an indication of long-range transport of POPs. Very few studies have determined temporal trends or have directly related the concentrations in mosses with measured atmospheric concentrations and/or deposition fluxes. Copyright © 2012 Elsevier Ltd. All rights reserved.

  17. Assessment of atmospheric pollution in the city of Naberezhnye ...

    African Journals Online (AJOL)

    By the nature of spatial distribution, two distinctly different groups of pollutants were defined: mainly contained in emissions of industrial enterprises, and coming into the atmospheric air, mainly with emissions from automotive transport. Keywords: emissions fromautomotive transport, maximum permissible concentration, ...

  18. [Atmospheric air pollution: a risk factor for COPD?].

    Science.gov (United States)

    Allain, Y-M; Roche, N; Huchon, G

    2010-04-01

    Tobacco smoking is the leading cause of COPD worldwide but other risk factors have been recognized. Air pollution is one of them, but its exact role in the development of COPD is hard to demonstrate. Its physiological effects on lung function have only been studied since the nineties by long and tedious cohort studies. Difficulties arise from the heterogeneity of air pollution (gas and particles); thus, its respiratory effects have to be examined for every component separately, and in different populations. It is also necessary to analyse the effects of atmospheric pollution in the short and the long term, considering both its physiological, clinical and toxicological effects, from childhood to adulthood. These factors make it difficult to obtain statistically significant results. Nevertheless, most studies seem to point to a role of air pollution in the development of COPD via oxydative stress but further studies are needed to confirm the exact effect of each component of air pollution on the respiratory tract. These studies could lead to improved public health policies and results are awaited that would identify at-risk populations, decide appropriate preventive measures and propose documented thresholds in pollution exposure... thereby limiting the spread of COPD. Copyright 2010 SPLF. Published by Elsevier Masson SAS. All rights reserved.

  19. Evaluation of environmental damage due to atmospheric pollution caused by power economy

    International Nuclear Information System (INIS)

    Burneikis, J.; Shtreimikiene, D.

    1996-01-01

    Methods to evaluate the environmental damage due to atmospheric pollution caused by power economy are presented. The products of burning fossil fuel (CO 2 , SO 2 , NO x and ashes) make the bulk of the pollutants that are being discharged into the atmosphere. To evaluate the damage caused by these pollutants an empirical method is suggested. The direct and analytical methods are used as a basis in collecting data for the empirical evaluation. All the three methods are described and empirical formulas suggested for calculating environmental damage due to burning fossil fuel in thermal power stations. The authors prove the necessity to change the present system of environmental taxes in Lithuania, which are purely symbolic. (author). 8 refs., 9 tabs

  20. Meteorological controls on atmospheric particulate pollution during hazard reduction burns

    Science.gov (United States)

    Di Virgilio, Giovanni; Hart, Melissa Anne; Jiang, Ningbo

    2018-05-01

    Internationally, severe wildfires are an escalating problem likely to worsen given projected changes to climate. Hazard reduction burns (HRBs) are used to suppress wildfire occurrences, but they generate considerable emissions of atmospheric fine particulate matter, which depend upon prevailing atmospheric conditions, and can degrade air quality. Our objectives are to improve understanding of the relationships between meteorological conditions and air quality during HRBs in Sydney, Australia. We identify the primary meteorological covariates linked to high PM2.5 pollution (particulates pollution, the PBLH between 00:00 and 07:00 LT (local time) was 100-200 m higher than days with high pollution. The PBLH was similar during 10:00-17:00 LT for both low and high pollution days, but higher after 18:00 LT for HRB days with low pollution. Cloud cover, temperature and wind speed reflected the above pattern, e.g. mean temperatures and wind speeds were 2 °C cooler and 0.5 m s-1 lower during mornings and evenings of HRB days when air quality was poor. These cooler, more stable morning and evening conditions coincide with nocturnal westerly cold air drainage flows in Sydney, which are associated with reduced mixing height and vertical dispersion, leading to the build-up of PM2.5. These findings indicate that air pollution impacts may be reduced by altering the timing of HRBs by conducting them later in the morning (by a matter of hours). Our findings support location-specific forecasts of the air quality impacts of HRBs in Sydney and similar regions elsewhere.

  1. Atmospheric deposition exposes Qinling pandas to toxic pollutants.

    Science.gov (United States)

    Chen, Yi-Ping; Zheng, Ying-Juan; Liu, Qiang; Song, Yi; An, Zhi-Sheng; Ma, Qing-Yi; Ellison, Aaron M

    2017-03-01

    The giant panda (Ailuropoda melanoleuca) is one of the most endangered animals in the world, and it is recognized worldwide as a symbol for conservation. A previous study showed that wild and captive pandas, especially those of the Qinling subspecies, were exposed to toxicants in their diet of bamboo; the ultimate origin of these toxicants is unknown. Here we show that atmospheric deposition is the most likely origin of heavy metals and persistent organic pollutants (POPs) in the diets of captive and wild Qinling pandas. Average atmospheric deposition was 199, 115, and 49 g·m -2 ·yr -1 in the center of Xi'an City, at China's Shaanxi Wild Animal Research Center (SWARC), and at Foping National Nature Reserve (FNNR), respectively. Atmospheric deposition of heavy metals (As, Cd, Cr, Pb, Hg, Co, Cu, Zn, Mn, and Ni) and POPs was highest at Xi'an City, intermediate at SWARC, and lowest at FNNR. Soil concentrations of the aforementioned heavy metals other than As and Zn also were significantly higher at SWARC than at FNNR. Efforts to conserve Qinling pandas may be compromised by air pollution attendant to China's economic development. Improvement of air quality and reductions of toxic emissions are urgently required to protect China's iconic species. © 2017 by the Ecological Society of America.

  2. Microscale atmospheric pollution of Pogranichny settlement (Primorsky region, Russia)

    Science.gov (United States)

    Kholodov, Aleksei; Ugay, Sergey; Drozd, Vladimir; Agoshkov, Alexander; Golokhvast, Kirill

    2017-10-01

    The paper discusses the study of atmospheric particulate matter in the small urban settlement Pogranichny by means of laser granulometry of snow water. The atmosphere of this settlement is polluted with particles under 10 μm (PM10) to a certain extent. We found microparticles potentially hazardous to health in significant quantities (from 176.3% to 24.9%) in 4 sampling points out of 9. Large particles (sized over 400 μm) dominate on the most territory of the settlement reaching 78.1%.

  3. Terrestrial mosses as biomonitors of atmospheric POPs pollution: A review

    International Nuclear Information System (INIS)

    Harmens, H.; Foan, L.; Simon, V.; Mills, G.

    2013-01-01

    Worldwide there is concern about the continuing release of persistent organic pollutants (POPs) into the environment. In this study we review the application of mosses as biomonitors of atmospheric deposition of POPs. Examples in the literature show that mosses are suitable organisms to monitor spatial patterns and temporal trends of atmospheric concentrations or deposition of POPs. These examples include polycyclic aromatic hydrocarbons (PAHs), polychlorobiphenyls (PCBs), dioxins and furans (PCDD/Fs), and polybrominated diphenyl ethers (PBDEs). The majority of studies report on PAHs concentrations in mosses and relative few studies have been conducted on other POPs. So far, many studies have focused on spatial patterns around pollution sources or the concentration in mosses in remote areas such as the polar regions, as an indication of long-range transport of POPs. Very few studies have determined temporal trends or have directly related the concentrations in mosses with measured atmospheric concentrations and/or deposition fluxes. - Highlights: ► Terrestrial mosses are suitable organisms to monitor deposition of POPs. ► They provide a good indication of spatial patterns and temporal trends. ► Mosses have been used as biomonitors of PAHs, PCBs, PBDEs dioxins and furans. ► Few studies have assessed the relationship between concentrations in air and mosses. - Mosses are suitable biomonitors of persistent organic pollutants (POPs).

  4. The Influence of Meteorological Factors and Atmospheric Pollutants on the Risk of Preterm Birth.

    Science.gov (United States)

    Giorgis-Allemand, Lise; Pedersen, Marie; Bernard, Claire; Aguilera, Inmaculada; Beelen, Rob M J; Chatzi, Leda; Cirach, Marta; Danileviciute, Asta; Dedele, Audrius; van Eijsden, Manon; Estarlich, Marisa; Fernández-Somoano, Ana; Fernández, Mariana F; Forastiere, Francesco; Gehring, Ulrike; Grazuleviciene, Regina; Gruzieva, Olena; Heude, Barbara; Hoek, Gerard; de Hoogh, Kees; van den Hooven, Edith H; Håberg, Siri E; Iñiguez, Carmen; Jaddoe, Vincent W V; Korek, Michal; Lertxundi, Aitana; Lepeule, Johanna; Nafstad, Per; Nystad, Wenche; Patelarou, Evridiki; Porta, Daniela; Postma, Dirkje; Raaschou-Nielsen, Ole; Rudnai, Peter; Siroux, Valérie; Sunyer, Jordi; Stephanou, Euripides; Sørensen, Mette; Eriksen, Kirsten Thorup; Tuffnell, Derek; Varró, Mihály J; Vrijkotte, Tanja G M; Wijga, Alet; Wright, John; Nieuwenhuijsen, Mark J; Pershagen, Göran; Brunekreef, Bert; Kogevinas, Manolis; Slama, Rémy

    2017-02-15

    Atmospheric pollutants and meteorological conditions are suspected to be causes of preterm birth. We aimed to characterize their possible association with the risk of preterm birth (defined as birth occurring before 37 completed gestational weeks). We pooled individual data from 13 birth cohorts in 11 European countries (71,493 births from the period 1994-2011, European Study of Cohorts for Air Pollution Effects (ESCAPE)). City-specific meteorological data from routine monitors were averaged over time windows spanning from 1 week to the whole pregnancy. Atmospheric pollution measurements (nitrogen oxides and particulate matter) were combined with data from permanent monitors and land-use data into seasonally adjusted land-use regression models. Preterm birth risks associated with air pollution and meteorological factors were estimated using adjusted discrete-time Cox models. The frequency of preterm birth was 5.0%. Preterm birth risk tended to increase with first-trimester average atmospheric pressure (odds ratio per 5-mbar increase = 1.06, 95% confidence interval: 1.01, 1.11), which could not be distinguished from altitude. There was also some evidence of an increase in preterm birth risk with first-trimester average temperature in the -5°C to 15°C range, with a plateau afterwards (spline coding, P = 0.08). No evidence of adverse association with atmospheric pollutants was observed. Our study lends support for an increase in preterm birth risk with atmospheric pressure. © The Author 2017. Published by Oxford University Press on behalf of the Johns Hopkins Bloomberg School of Public Health. All rights reserved. For permissions, please e-mail: journals.permissions@oup.com.

  5. Complex Physiological Response of Norway Spruce to Atmospheric Pollution - Decreased Carbon Isotope Discrimination and Unchanged Tree Biomass Increment.

    Science.gov (United States)

    Čada, Vojtěch; Šantrůčková, Hana; Šantrůček, Jiří; Kubištová, Lenka; Seedre, Meelis; Svoboda, Miroslav

    2016-01-01

    Atmospheric pollution critically affects forest ecosystems around the world by directly impacting the assimilation apparatus of trees and indirectly by altering soil conditions, which subsequently also leads to changes in carbon cycling. To evaluate the extent of the physiological effect of moderate level sulfate and reactive nitrogen acidic deposition, we performed a retrospective dendrochronological analysis of several physiological parameters derived from periodic measurements of carbon stable isotope composition ((13)C discrimination, intercellular CO2 concentration and intrinsic water use efficiency) and annual diameter increments (tree biomass increment, its inter-annual variability and correlation with temperature, cloud cover, precipitation and Palmer drought severity index). The analysis was performed in two mountain Norway spruce (Picea abies) stands of the Bohemian Forest (Czech Republic, central Europe), where moderate levels of pollution peaked in the 1970s and 1980s and no evident impact on tree growth or link to mortality has been reported. The significant influence of pollution on trees was expressed most sensitively by a 1.88‰ reduction of carbon isotope discrimination (Δ(13)C). The effects of atmospheric pollution interacted with increasing atmospheric CO2 concentration and temperature. As a result, we observed no change in intercellular CO2 concentrations (Ci), an abrupt increase in water use efficiency (iWUE) and no change in biomass increment, which could also partly result from changes in carbon partitioning (e.g., from below- to above-ground). The biomass increment was significantly related to Δ(13)C on an individual tree level, but the relationship was lost during the pollution period. We suggest that this was caused by a shift from the dominant influence of the photosynthetic rate to stomatal conductance on Δ(13)C during the pollution period. Using biomass increment-climate correlation analyses, we did not identify any clear pollution

  6. Silica nanoparticles capture atmospheric lead: implications in the treatment of environmental heavy metal pollution.

    Science.gov (United States)

    Yang, Xifei; Shen, Zhiguo; Zhang, Bing; Yang, Jianping; Hong, Wen-Xu; Zhuang, Zhixiong; Liu, Jianjun

    2013-01-01

    Lead (Pb) contamination in the air is a severe global problem, most notably in China. Removal of Pb from polluted air remains a significant challenge. It is unclear what potential effects silica nanoparticles (SiNPs) exposure can have on atmospheric Pb. Here we first characterized the features of SiNPs by measuring the particle size, zeta potential and the specific surface area of SiO(2) particles using a Nicomp 380/ZLS submicron particle sizer, the Brunauer-Emmett-Teller (BET) method and transmission electronic microscopy (TEM). We measured the content of the metal Pb adsorbed by SiNPs exposed to two Pb polluted electric battery plants using inductively coupled plasma mass spectrometry (ICP-MS). It is found that SiNPs exposed to two Pb polluted electric battery plants absorb more atmospheric Pb compared to either blank control or micro-sized SiO(2) particles in a time-dependent manner. This is the first study demonstrating that SiNPs exposure can absorb atmospheric Pb in the polluted environment. These novel findings indicate that SiNPs have potential to serve as a significant adsorbent of Pb from industrial pollution, implicating a potentially novel application of SiNPs in the treatment of environmental heavy metal pollution. Copyright © 2012 Elsevier Ltd. All rights reserved.

  7. Aerodynamic modeling of the lower part of the atmospheric boundary layer

    International Nuclear Information System (INIS)

    Mohamed, K.S.

    1992-01-01

    In this thesis , we present a study dealing with the basic meteorology concepts commonly used in air pollution. The pollutant motion in the atmosphere together with its basic mathematical concepts have been reviewed. This review includes; atmospheric forces acting on a particle, atmospheric turbulence, atmospheric stability and the most widely used atmospheric diffusion models. The resistance for pollutant transfer for different atmospheric stability classes has been derived in terms of both wind velocity profile parameters and diffusion coefficients. Therefrom, the residence time of a pollutant in the atmosphere is obtained. The dust particle trajectory and deposition in case of neutral atmosphere is formulated mathematically adopting particle Gaussian distribution. An analytical treatment for the diffusion equation with extension of the boundary conditions to include the ground surface absorption of pollutants and presence of elevated inversion layer, has been presented . The concept of decay distance is introduced and applied in a sample calculation for the dispersion of pollutants over growing wheat field

  8. Using an epiphytic moss to identify previously unknown sources of atmospheric cadmium pollution

    Energy Technology Data Exchange (ETDEWEB)

    Donovan, Geoffrey H., E-mail: gdonovan@fs.fed.us [USDA Forest Service, PNW Research Station, 620 SW Main, Suite 400, Portland, OR 97205 (United States); Jovan, Sarah E., E-mail: sjovan@fs.fed.us [USDA Forest Service, PNW Research Station, 620 SW Main, Suite 400, Portland, OR 97205 (United States); Gatziolis, Demetrios, E-mail: dgatziolis@fs.fed.us [USDA Forest Service, PNW Research Station, 620 SW Main, Suite 400, Portland, OR 97205 (United States); Burstyn, Igor, E-mail: igor.burstyn@drexel.edu [Dornsife School of Public Health, Drexel University, Nesbitt Hall, 3215 Market St, Philadelphia, PA 19104 (United States); Michael, Yvonne L., E-mail: ylm23@drexel.edu [Dornsife School of Public Health, Drexel University, Nesbitt Hall, 3215 Market St, Philadelphia, PA 19104 (United States); Amacher, Michael C., E-mail: mcamacher1@outlook.com [USDA Forest Service, Logan Forest Sciences Laboratory, 860 North 1200 East, Logan, UT 84321 (United States); Monleon, Vicente J., E-mail: vjmonleon@fs.fed.us [USDA Forest Service, PNW Research Station, 3200 SW Jefferson Way, Corvallis, OR 97331 (United States)

    2016-07-15

    Urban networks of air-quality monitors are often too widely spaced to identify sources of air pollutants, especially if they do not disperse far from emission sources. The objectives of this study were to test the use of moss bio-indicators to develop a fine-scale map of atmospherically-derived cadmium and to identify the sources of cadmium in a complex urban setting. We collected 346 samples of the moss Orthotrichum lyellii from deciduous trees in December, 2013 using a modified randomized grid-based sampling strategy across Portland, Oregon. We estimated a spatial linear model of moss cadmium levels and predicted cadmium on a 50 m grid across the city. Cadmium levels in moss were positively correlated with proximity to two stained-glass manufacturers, proximity to the Oregon–Washington border, and percent industrial land in a 500 m buffer, and negatively correlated with percent residential land in a 500 m buffer. The maps showed very high concentrations of cadmium around the two stained-glass manufacturers, neither of which were known to environmental regulators as cadmium emitters. In addition, in response to our findings, the Oregon Department of Environmental Quality placed an instrumental monitor 120 m from the larger stained-glass manufacturer in October, 2015. The monthly average atmospheric cadmium concentration was 29.4 ng/m{sup 3}, which is 49 times higher than Oregon's benchmark of 0.6 ng/m{sup 3}, and high enough to pose a health risk from even short-term exposure. Both stained-glass manufacturers voluntarily stopped using cadmium after the monitoring results were made public, and the monthly average cadmium levels precipitously dropped to 1.1 ng/m{sup 3} for stained-glass manufacturer #1 and 0.67 ng/m{sup 3} for stained-glass manufacturer #2. - Highlights: • Bio-indicators are a valid method for measuring atmospheric pollutants • We used moss to map atmospheric cadmium in Portland, Oregon • Using a spatial linear model, we identified two

  9. Atmospheric pollution and specific tolerance of lichens

    Energy Technology Data Exchange (ETDEWEB)

    De Sloover, J

    1968-01-01

    An ecological method has been designed which allows a quantitative estimation of specific sensitivity of lichens to atmospheric pollution. That method is based on a comparison of the ''cortege moyen specifique'' i.e. the mean number of lichens growing with each species in a given area. Four of the obtained sequences are compared (The Dender valley and the area surrounding Gand, Belgium: the Oslo and the Helsinki areas); they show the order to toxiphoby of the related epiphytic lichens.

  10. Observable Effects of Atmospheric Pollution on Outpatient and Inpatient Morbidity in Bulgaria.

    Science.gov (United States)

    Platikanova, Magdalena; Penkova-Radicheva, Mariana

    2016-04-01

    One of Europe's most well-developed industrial regions is found in the Republic of Bulgaria. The industrialization of the region has a big impact on air pollution. Thermal power plant "Maritza East" (the largest of its kind in southeastern Europe), the army training range, machine manufacturers, household heating and high volume of automobile traffic are all major sources of pollution in the region. A five year study (2009-2013) followed yearly concentrations of principal atmospheric pollutants such as sulfur dioxide, dust, nitrogen dioxide, lead aerosols and hydrogen sulfide, and the way in which those levels had an effect on morbidity (outpatient and inpatient medical care) in the area. Statistical processing of data has been completed to represent and analyze the collected data in nonparametric and alternative format. Atmospheric pollution affects human health directly through pathological changes in the human organism. The registered outpatient care provided for the period 2009-2013 is highest for diseases of the cardiovascular system (11.85%), the respiratory system (17.34%) and the genitourinary system (9.76%). The registered rate of hospitalization for the same period is for diseases of the digestive system (11.90%), the cardiovascular system (11.85%), respiratory system (10.86%) and the genitourinary system (8.88%). The observed period shows a decrease in average yearly concentrations of the principal atmospheric pollutants in the industrial region (Bulgaria) and reflects a decrease in morbidity based on outpatient care and an increase in morbidity by inpatient care (hospitalization). Our findings should be corroborated in future longitudinal studies.

  11. Contribution to the modeling of atmospheric pollution in cities; Contribution a la modelisation de la pollution atmospherique dans les villes

    Energy Technology Data Exchange (ETDEWEB)

    Glockmer, St.

    2000-07-01

    Pollution generated by urban traffic and by industry at its periphery is a serious problem of our cities. Once emitted in the atmosphere, pollutants undergo two types of constraints: on one side they react chemically one with another and, on the other side, they are transported by the wind. We have chosen to work on the dynamical, thermal and chemical aspects of the pollution at different scales of the phenomena: local scale (around a group of buildings) and meso-scale (a whole city). Our ambition is not to realize a complete model but to advance step by step on each aspect. We have contributed to the realization of a numerical tool that will be completed and used for concrete pollution episodes. The first chapter is a description of the atmospheric boundary layer. Chapters two and three present models and results of numerical simulations. We stress on k-{epsilon}, RNG and v{sup 2}-f turbulence models, radiative heat transfer models and dynamical and thermal wall laws that allow to take in consideration surface roughness. The last chapter is dedicated to atmospheric chemistry. We have moreover developed a general solver of any number of transport equations coupled by a stiff chemistry and simplified ozone kinetics. (author)

  12. Ideas in Practice: Studies in Atmospheric Pollution For Science Teachers

    Science.gov (United States)

    Rowe, Donald R.

    1974-01-01

    Describes the content and structure of an enviromental course offered by the Department of Engineering Technology at Western Kentucky University. The course focuses on atmospheric pollution and is designed for science teachers currently teaching in the school system. (JR)

  13. AICE Survey of USSR Air Pollution Literature, Volume 12: Technical Papers from the Leningrad International Symposium on the Meteorological Aspects of Atmospheric Pollution, Part I.

    Science.gov (United States)

    Nuttonson, M. Y.

    Twelve papers dealing with the meteorological aspects of air pollution were translated. These papers were initially presented at an international symposium held in Leningrad during July 1968. The papers are: Status and prospective development of meteorological studies of atmospheric pollution, Effect of the stability of the atmosphere on the…

  14. Atmospheric pollution over the eastern Mediterranean during summer – a review

    Directory of Open Access Journals (Sweden)

    U. Dayan

    2017-11-01

    Full Text Available The eastern Mediterranean (EM is one of the regions in the world where elevated concentrations of primary and secondary gaseous air pollutants have been reported frequently, mainly in summer. This review discusses published studies of the atmospheric dispersion and transport conditions characterizing this region during the summer, followed by a description of some essential studies dealing with the corresponding concentrations of air pollutants such as ozone, carbon monoxide, total reactive nitrogen, methane, and sulfate aerosols observed there. The interlaced relationship between the downward motion of the subsiding air aloft induced by global circulation systems affecting the EM and the depth of the Persian Trough, a low-pressure trough that extends from the Asian monsoon at the surface controlling the spatiotemporal distribution of the mixed boundary layer during summer, is discussed. The strength of the wind flow within the mixed layer and its depth affect much the amount of pollutants transported and determine the potential of the atmosphere to disperse contaminants off their origins in the EM. The reduced mixed layer and the accompanying weak westerlies, characterizing the summer in this region, led to reduced ventilation rates, preventing an effective dilution of the contaminants. Several studies pointing at specific local (e.g., ventilation rates and regional peculiarities (long-range transport enhancing the build-up of air pollutant concentrations are presented. Tropospheric ozone (O3 concentrations observed in the summer over the EM are among the highest over the Northern Hemisphere. The three essential processes controlling its formation (i.e., long-range transport of polluted air masses, dynamic subsidence at mid-tropospheric levels, and stratosphere-to-troposphere exchange are reviewed. Airborne campaigns and satellite-borne initiatives have indicated that the concentration values of reactive nitrogen identified as precursors in

  15. Use of lichens as indicator and test organism for atmospheric pollution

    Energy Technology Data Exchange (ETDEWEB)

    Skye, E

    1969-01-01

    Some species of lichens are very specialized with regard to their substrata, while others grow on almost any substratum. The species that grow on the bark of trees are discussed. Not all kinds of bark are equally desirable to all epiphytic lichen species. Some species occur on bark with a fairly low pH (pH 3-4), while others occur on moderately acid to almost neutral bark (pH 4.5-6-7). Different ways of using lichens as indicators and test plants for atmospheric pollution have been tried. Individual species have served as indicators. In order to get an idea of the zonation around a source of damage, it is possible to use the number of species per tree or group of trees examined. This method is practicable only under certain special conditions. The comparison of the species gives a better indication of the degree and kind of atmospheric pollution than the epiphyte flora. De Sloover and LeBlanc have published a formula, with the aid of which an index of atmospheric purity (IAP) may be produced. This index may then be used in the cartographical representation of zones of air purity. Another formula is based on the degree of cover and poleotolerance in the individual species. Schoenbeck has developed Brodo's transplantation method and uses Hypogymnia physodes as a test organism for atmospheric pollution. The extent of the damage to the lichens is recorded on infra-red-sensitive film. The damaged areas are measured with a planimeter, by which means a numerical value is obtained for the extent of damage.

  16. Control of emissions from stationary combustion sources: Pollutant detection and behavior in the atmosphere

    International Nuclear Information System (INIS)

    Licht, W.; Engel, A.J.; Slater, S.M.

    1979-01-01

    Stationary combustion resources continue to be significant sources of NOx and SOx pollutants in the ambient atmosphere. This volume considers four problem areas: (1) control of emissions from stationary combustion sources, particularly SOx and NOx (2) pollutant behavior in the atmosphere (3) advances in air pollution analysis and (4) air quality management. Topics of interest include carbon slurries for sulfur dioxide abatement, mass transfer in the Kellogg-Weir air quality control system, oxidation/inhibition of sulfite ion in aqueous solution, some micrometeorological methods of measuring dry deposition rates, Spanish moss as an indicator of airborne metal contamination, and air quality impacts from future electric power generation in Texas

  17. Complex Physiological Response of Norway Spruce to Atmospheric Pollution – Decreased Carbon Isotope Discrimination and Unchanged Tree Biomass Increment

    Science.gov (United States)

    Čada, Vojtěch; Šantrůčková, Hana; Šantrůček, Jiří; Kubištová, Lenka; Seedre, Meelis; Svoboda, Miroslav

    2016-01-01

    Atmospheric pollution critically affects forest ecosystems around the world by directly impacting the assimilation apparatus of trees and indirectly by altering soil conditions, which subsequently also leads to changes in carbon cycling. To evaluate the extent of the physiological effect of moderate level sulfate and reactive nitrogen acidic deposition, we performed a retrospective dendrochronological analysis of several physiological parameters derived from periodic measurements of carbon stable isotope composition (13C discrimination, intercellular CO2 concentration and intrinsic water use efficiency) and annual diameter increments (tree biomass increment, its inter-annual variability and correlation with temperature, cloud cover, precipitation and Palmer drought severity index). The analysis was performed in two mountain Norway spruce (Picea abies) stands of the Bohemian Forest (Czech Republic, central Europe), where moderate levels of pollution peaked in the 1970s and 1980s and no evident impact on tree growth or link to mortality has been reported. The significant influence of pollution on trees was expressed most sensitively by a 1.88‰ reduction of carbon isotope discrimination (Δ13C). The effects of atmospheric pollution interacted with increasing atmospheric CO2 concentration and temperature. As a result, we observed no change in intercellular CO2 concentrations (Ci), an abrupt increase in water use efficiency (iWUE) and no change in biomass increment, which could also partly result from changes in carbon partitioning (e.g., from below- to above-ground). The biomass increment was significantly related to Δ13C on an individual tree level, but the relationship was lost during the pollution period. We suggest that this was caused by a shift from the dominant influence of the photosynthetic rate to stomatal conductance on Δ13C during the pollution period. Using biomass increment-climate correlation analyses, we did not identify any clear pollution

  18. The influence of scales of atmospheric motion on air pollution over Portugal

    Science.gov (United States)

    Russo, Ana; Trigo, Ricardo; Mendes, Manuel; Jerez, Sonia; Gouveia, Célia Marina

    2014-05-01

    Air pollution is determined by the combination of different factors, namely, emissions, physical constrains, meteorology and chemical processes [1,2,3]. The relative importance of such factors is influenced by their interaction on diverse scales of atmospheric motion. Each scale depicts different meteorological conditions, which, when combined with the different air pollution sources and photochemistry, result in varying ambient concentrations [2]. Identifying the dominant scales of atmospheric motion over a given airshed can be of great importance for many applications such as air pollution and pollen dispersion or wind energy management [2]. Portugal has been affected by numerous air pollution episodes during the last decade. These episodes are often related to peak emissions from local industry or transport, but can also be associated to regional transport from other urban areas or to exceptional emission events, such as forest fires. This research aims to identify the scales of atmospheric motion which contribute to an increase of air pollution. A method is proposed for differentiating between the scales of atmospheric motion that can be applied on a daily basis from data collected at several wind-measuring sites in a given airshed and to reanalysis datasets. The method is based on the daily mean wind recirculation and the mean and standard deviation between sites. The determination of the thresholds between scales is performed empirically following the approach of Levy et al. [2] and also through a automatic statistical approach computed taking into account the tails of the distributions (e.g. 95% and 99% percentile) of the different wind samples. A comparison is made with two objective approaches: 1) daily synoptic classification for the same period over the region [4] and 2) a 3-D backward trajectory approach [5,6] for specific episodes. Furthermore, the outcomes are expected to support the Portuguese authorities on the implementation of strategies for a

  19. The risks of premature mortality related to atmospheric pollution. Comparison with those related to tobacco and those related to radioactivity

    International Nuclear Information System (INIS)

    Durand, Bernard

    2014-01-01

    Whereas atmospheric pollution is now recognized as one of the most important cause of mortality in the world, this report first notices that these pollutants have mainly an anthropogenic origin. In a first part, the author presents the main harmful atmospheric pollutants, and briefly discusses their origin and their impact on health: carbon monoxide, sulphur oxides, ammonia, nitrogen oxides, persistent organic pollutants, volatile organic compounds, ozone, tars, soot or particles, heavy metals. In a second part, the author discusses the assessment of hazards related to atmospheric pollution, and more particularly the assessment of premature morbidity due to different pollutants according to different organisations and programs. He also discusses health impacts on a short and on a long term, notably in terms of exposure in big cities. In a third part, based on measurements of emissions of primary pollutant, notably primary particles, the author tries to identify the most dangerous sources of atmospheric pollutions

  20. DETECTING INDUSTRIAL POLLUTION IN THE ATMOSPHERES OF EARTH-LIKE EXOPLANETS

    Energy Technology Data Exchange (ETDEWEB)

    Lin, Henry W. [Harvard College, Cambridge, MA 02138 (United States); Abad, Gonzalo Gonzalez; Loeb, Abraham, E-mail: henrylin@college.harvard.edu, E-mail: ggonzalezabad@cfa.harvard.edu, E-mail: aloeb@cfa.harvard.edu [Harvard-Smithsonian Center for Astrophysics, 60 Garden St., Cambridge, MA 02138 (United States)

    2014-09-01

    Detecting biosignatures, such as molecular oxygen in combination with a reducing gas, in the atmospheres of transiting exoplanets has been a major focus in the search for alien life. We point out that in addition to these generic indicators, anthropogenic pollution could be used as a novel biosignature for intelligent life. To this end, we identify pollutants in the Earth's atmosphere that have significant absorption features in the spectral range covered by the James Webb Space Telescope. We focus on tetrafluoromethane (CF{sub 4}) and trichlorofluoromethane (CCl{sub 3}F), which are the easiest to detect chlorofluorocarbons (CFCs) produced by anthropogenic activity. We estimate that ∼1.2 days (∼1.7 days) of total integration time will be sufficient to detect or constrain the concentration of CCl{sub 3}F (CF{sub 4}) to ∼10 times the current terrestrial level.

  1. The Multimedia Environmental Pollutant Assessment System (MEPAS)reg-sign: Atmospheric pathway formulations. Revision

    International Nuclear Information System (INIS)

    Droppo, J.G.; Buck, J.W.

    1996-03-01

    The Multimedia Environmental Pollutant Assessment System (MEPAS) is an integrated software implementation of physics-based fate and transport models for health and environmental risk assessments of both radioactive and hazardous pollutants. This atmospheric component report is one of a series of formulation reports that document the MEPAS mathematical models. MEPAS is a multimedia model; pollutant transport is modeled within, through, and between multiple media (air, soil, groundwater, and surface water). The estimated concentrations in the various media are used to compute exposures and impacts to the environment, to maximum individuals, and to populations. The MEPAS atmospheric component for the air media documented in this report includes models for emission from a source to the air, initial plume rise and dispersion, airborne pollutant transport and dispersion, and deposition to soils and crops. The material in this report is documentation for MEPAS Versions 3.0 and 3.1 and the MEPAS version used in the Remedial Action Assessment System (RAAS) Version 1.0

  2. Correlation study of air pollution and cardio-respiratory diseases through NAA of an atmospheric pollutant biomonitor

    International Nuclear Information System (INIS)

    Saiki, M.; Alves, E.R.; Genezini, F.A.; Santos, J.O.; Marcelli, M.P.; Saldiva, P.H.N.

    2014-01-01

    In this study neutron activation analysis was applied to analyze lichen samples used as atmospheric pollutant biomonitors in order to verify if there is correlation between air pollution and its effects on the cardio respiratory system. Canoparmelia texana lichenized fungii species was chosen for passive biomonitoring of atmospheric pollutants. The population group selected for this study was adults over 45 years. Lichen samples collected in Sao Paulo city were cleaned, freeze-dried and ground for the analyses. Aliquots of samples were irradiated at the IEA-R1 nuclear research reactor for short and long periods along with synthetic element standards. The induced gamma activities of the samples and standards were measured using a gamma ray spectrometer with an HPGe detector and the concentrations of As, Ba, Br, Ca, Cd, Cl, Co, Cr, Cs, Fe, Hf, K, Mg, Mn, Na, Rb, Sb, Sc, Se,Th, V, Zn and lanthanides were determined. For quality control of the results, certified reference materials were analyzed together. Mortality data for the population due to cardio-respiratory diseases were obtained from the database of the Secretariat of Health of the Sao Paulo Municipality for the years 2005-2009. Results obtained point to vehicular and industrial emissions as the origins of pollutants in Sao Paulo city. The statistical treatment of Pearson's correlation applied to the results of lichen element concentrations and mortality rates indicated significant positive correlation for the elements Co, Mn and Zn for adults. (author)

  3. Study of laser monitoring techniques of pollutants in atmosphere

    International Nuclear Information System (INIS)

    Hassan, T. A. A.

    2006-01-01

    There are several techniques used as a tool for monitoring the pollutions in the atmosphere, where the laser radiation sending through the sample of atmosphere to be investigated ether transmission or the scattering of the light, all the way through a variety of different techniques for monitoring the air quality. We are showed in this study the comparison of detection techniques through measuring the light scattered in some particular direction, rather than measuring direction the attenuation due to two type of scattering (Rayieh scattering and Mie scattering) during (optical Radar, Roman backscattering and Resonance fluorescence).(Author)

  4. Atmospheric pollution history at Linfen (China) uncovered by magnetic and chemical parameters of sediments from a water reservoir.

    Science.gov (United States)

    Ma, Mingming; Hu, Shouyun; Cao, Liwan; Appel, Erwin; Wang, Longsheng

    2015-09-01

    We studied magnetic and chemical parameters of sediments from sediments of a water reservoir at Linfen (China) in order to quantitatively reconstruct the atmospheric pollution history in this region. The results show that the main magnetic phases are magnetite and maghemite originating from the surrounding catchment and from anthropogenic activities, and there is a significant positive relationship between magnetic concentration parameters and heavy metals concentrations, indicating that magnetic proxies can be used to monitor the anthropogenic pollution. In order to uncover the atmospheric pollution history, we combined the known events of environmental improvement with variations of magnetic susceptibility (χ) and heavy metals along the cores to obtain a detailed chronological framework. In addition, air comprehensive pollution index (ACPI) was reconstructed from regression equation among magnetic and chemical parameters as well as atmospheric monitoring data. Based on these results, the atmospheric pollution history was successfully reconstructed. Copyright © 2015 Elsevier Ltd. All rights reserved.

  5. Relationship between epiphytic lichens, trace elements and gaseous atmospheric pollutants

    NARCIS (Netherlands)

    Dobben, van H.F.; Wamelink, G.W.W.; Braak, ter C.J.F.

    2001-01-01

    A study was conducted to determine the joint effect of gaseous atmospheric pollutants and trace elements on epiphytic lichens. We used our data to test the hypothesis that lichens are generally insensitive to toxic effects of trace elements, and can therefore be used as accumulator organisms to

  6. Thermal Band Atmospheric Correction Using Atmospheric Profiles Derived from Global Positioning System Radio Occultation and the Atmospheric Infrared Sounder

    Science.gov (United States)

    Pagnutti, Mary; Holekamp, Kara; Stewart, Randy; Vaughan, Ronald D.

    2006-01-01

    This Rapid Prototyping Capability study explores the potential to use atmospheric profiles derived from GPS (Global Positioning System) radio occultation measurements and by AIRS (Atmospheric Infrared Sounder) onboard the Aqua satellite to improve surface temperature retrieval from remotely sensed thermal imagery. This study demonstrates an example of a cross-cutting decision support technology whereby NASA data or models are shown to improve a wide number of observation systems or models. The ability to use one data source to improve others will be critical to the GEOSS (Global Earth Observation System of Systems) where a large number of potentially useful systems will require auxiliary datasets as input for decision support. Atmospheric correction of thermal imagery decouples TOA radiance and separates surface emission from atmospheric emission and absorption. Surface temperature can then be estimated from the surface emission with knowledge of its emissivity. Traditionally, radiosonde sounders or atmospheric models based on radiosonde sounders, such as the NOAA (National Oceanic & Atmospheric Administration) ARL (Air Resources Laboratory) READY (Real-time Environmental Application and Display sYstem), provide the atmospheric profiles required to perform atmospheric correction. Unfortunately, these types of data are too spatially sparse and too infrequently taken. The advent of high accuracy, global coverage, atmospheric data using GPS radio occultation and AIRS may provide a new avenue for filling data input gaps. In this study, AIRS and GPS radio occultation derived atmospheric profiles from the German Aerospace Center CHAMP (CHAllenging Minisatellite Payload), the Argentinean Commission on Space Activities SAC-C (Satellite de Aplicaciones Cientificas-C), and the pair of NASA GRACE (Gravity Recovery and Climate Experiment) satellites are used as input data in atmospheric radiative transport modeling based on the MODTRAN (MODerate resolution atmospheric

  7. Huguangyan Maar Lake (SE China): A solid record of atmospheric mercury pollution history in a non-remote region

    Science.gov (United States)

    Zeng, Yan; Chen, Jingan; Yang, Yongqiong; Wang, Jianxu; Zhu, Zhengjie; Li, Jian

    2017-10-01

    Mercury is a highly toxic metal that can cause harm to environment and human health. As atmospheric deposition is the main source of total Hg input to aquatic system in remote and pristine regions, almost all the studies on atmospheric Hg pollution history concentrated in these areas, while the studies in non-remote areas are much limited, especially for the long history records. In this study, Huguangyan Maar Lake, an undisturbed lake system at low altitude in China, was selected to reconstruct the atmospheric mercury pollution history. Variation patterns of TOC, Hg and non-residual Sr in the sediment core indicated that, compared to the direct atmospheric Hg deposition, the effect of either Hg scavenging from water column by algae or the catchment inputs of previously deposited Hg on the Hg accumulation in the lake sediment was limited. The sediment Hg content in Huguangyan Lake was mainly controlled by the atmospheric Hg deposition, and thus accurately reflected the atmospheric Hg pollution history. The Hga (Hg content from atmospheric deposition) in Huguangyan Lake presented a comparable variation pattern to that in remote sites. It had the same variation trend as the global atmospheric Hg before 1950 CE, which could be attributed to the Industrial Revolution. After that, it was mainly controlled by Hg emissions from Asian countries. The variation of Hga also indicated that atmospheric Hg deposition accelerated significantly since 2000 CE. This study, along with other investigations in remote sites in China, showed that the sediment Hg in Huguangyan Lake responded to the atmospheric Hg pollution more sensitively than in the alpine regions. It should be noted that, the more intensive acceleration of Hg deposition in Huguangyan Lake may imply that the South of China suffered from much more serious atmospheric Hg pollution than previous studies revealed.

  8. Effects of atmospheric transport and trade on air pollution mortality in China

    Science.gov (United States)

    Zhao, Hongyan; Li, Xin; Zhang, Qiang; Jiang, Xujia; Lin, Jintai; Peters, Glen P.; Li, Meng; Geng, Guannan; Zheng, Bo; Huo, Hong; Zhang, Lin; Wang, Haikun; Davis, Steven J.; He, Kebin

    2017-09-01

    Air quality is a major environmental concern in China, where premature deaths due to air pollution have exceeded 1 million people per year in recent years. Here, using a novel coupling of economic, physical and epidemiological models, we estimate the premature mortality related to anthropogenic outdoor PM2.5 air pollution in seven regions of China in 2010 and show for the first time how the distribution of these deaths in China is determined by a combination of economic activities and physical transport of pollution in the atmosphere. We find that 33 % (338 600 premature deaths) of China's PM2.5-related premature mortality in 2010 were caused by pollutants emitted in a different region of the country and transported in the atmosphere, especially from north to south and from east to west. Trade further extended the cross-regional impact; 56 % of (568 900 premature deaths) China's PM2.5-related premature mortality was related to consumption in another region, including 423 800 (42 % of total) and 145 100 (14 %) premature deaths from domestic consumption and international trade respectively. Our results indicate that multilateral and multi-stage cooperation under a regional sustainable development framework is in urgent need to mitigate air pollution and related health impacts, and efforts to reduce the health impacts of air pollution in China should be prioritized according to the source and location of emissions, the type and economic value of the emitting activities, and the related patterns of consumption.

  9. Advection of pollutants by internal solitary waves in oceanic and atmospheric stable stratifications

    Directory of Open Access Journals (Sweden)

    G. W. Haarlemmer

    1998-01-01

    Full Text Available When a pollutant is released into the ocean or atmosphere under turbulent conditions, even a steady release is captured by large eddies resulting in localized patches of high concentration of the pollutant. If such a cloud of pollutant subsequently enters a stable stratification-either a pycnocline or thermocline-then internal waves are excited. Since large solitary internal waves have a recirculating core, pollutants may be trapped in the sclitary wave, and advected large distances through the waveguide provided by the stratification. This paper addresses the mechanisms, through computer and physical simulation, by which a localized release of a dense pollutant results in solitary waves that trap the pollutant or disperse the pollutant faster than in the absence of the waves.

  10. Supplemental mathematical formulations, Atmospheric pathway: The Multimedia Environmental Pollutant Assessment System (MEPAS)

    International Nuclear Information System (INIS)

    Droppo, J.G.; Buck, J.W.

    1996-03-01

    The Multimedia Environmental Pollutant Assessment System (MEPAS) is an integrated software implementation of physics-based fate and transport models for health and environmental risk assessments of both radioactive and hazardous pollutants. This atmospheric component report is one of a series of formulation reports that document the MEPAS mathematical models. MEPAS is a ''multimedia'' model; pollutant transport is modeled within, through, and between multiple media (air, soil, groundwater, and surface water). The estimated concentrations in the various media are used to compute exposures and impacts to the environment, to maximum individuals, and to populations

  11. Essentials of multiangle data-processing methodology for smoke polluted atmospheres

    Science.gov (United States)

    Vladimir Kovalev; A. Petkov; Cyle Wold; Shawn Urbanski; WeiMin Hao

    2011-01-01

    Essentials for investigating smoke plume characteristics with scanning lidar are discussed. Particularly, we outline basic principles for determining dynamics, heights, and optical properties of smoke plumes and layers in wildfire-polluted atmospheres. Both simulated and experimental data obtained in vicinities of wildfires with a two-wavelength scanning lidar are...

  12. Vulnerability to diffuse pollution of European soils and groundwater

    NARCIS (Netherlands)

    Meinardi CR; Beusen AHW; Bollen MJS; Klepper O; LBG; CWM

    1994-01-01

    From the Atlantic Ocean to the Ural Mountains, European soils and groundwater are threatened by diffuse pollution derived from various chemicals used in modern agriculture and by increased atmospheric deposition of pollutants. The investigated vulnerability of soils (including groundwater) to

  13. Atmospheric pollutants in alpine peat bogs record a detailed chronology of industrial and agricultural development on the Australian continent

    International Nuclear Information System (INIS)

    Marx, Samuel K.; Kamber, Balz S.; McGowan, Hamish A.; Zawadzki, Atun

    2010-01-01

    Two peat bogs from remote alpine sites in Australia were found to contain detailed and coherent histories of atmospheric metal pollution for Pb, Zn, Cu, Mo, Ag, As, Cd, Sb, Zn, In, Cr, Ni, Tl and V. Dramatic increases in metal deposition in the post-1850 AD portion of the cores coincide with the onset of mining in Australia. Using both Pb isotopes and metals, pollutants were ascribed to the main atmospheric pollution emitting sources in Australia, namely mining and smelting, coal combustion and agriculture. Results imply mining and metal production are the major source of atmospheric metal pollution, although coal combustion may account for up to 30% of metal pollutants. A novel finding of this study is the increase in the otherwise near-constant Y/Ho ratio after 1900 AD. We link this change to widespread and increased application of marine phosphate fertiliser in Australia's main agricultural area (the Murray Darling Basin). - Detailed records of atmospheric metal pollution accumulation in Australia are presented and are shown to trace the industrial and agricultural development of the continent.

  14. Dispersion of atmospheric air pollution in summer and winter season.

    Science.gov (United States)

    Cichowicz, Robert; Wielgosiński, Grzegorz; Fetter, Wojciech

    2017-11-04

    Seasonal variation of air pollution is associated with variety of seasons and specificity of particular months which form the so-called summer and winter season also known as the "heating" season. The occurrence of higher values of air pollution in different months of a year is associated with the type of climate, and accordingly with different atmospheric conditions in particular months, changing state of weather on a given day, and anthropogenic activity. The appearance of these conditions results in different levels of air pollution characteristic for a given period. The study uses data collected during a seven-year period (2009-2015) in the automatic measuring station of immissions located in Eastern Wielkopolska. The analysis concerns the average and maximum values of air pollution (i.e., particulate matter PM10, sulfur dioxide, nitrogen dioxide, carbon monoxide, and ozone) from the perspective of their occurrence in particular seasons and months or in relation to meteorological actors such as temperature, humidity, and wind speed.

  15. Atmospheric pollutants in peri-urban forests of Quercus ilex: evidence of pollution abatement and threats for vegetation.

    Science.gov (United States)

    García-Gómez, Héctor; Aguillaume, Laura; Izquieta-Rojano, Sheila; Valiño, Fernando; Àvila, Anna; Elustondo, David; Santamaría, Jesús M; Alastuey, Andrés; Calvete-Sogo, Héctor; González-Fernández, Ignacio; Alonso, Rocío

    2016-04-01

    Peri-urban vegetation is generally accepted as a significant remover of atmospheric pollutants, but it could also be threatened by these compounds, with origin in both urban and non-urban areas. To characterize the seasonal and geographical variation of pollutant concentrations and to improve the empirical understanding of the influence of Mediterranean broadleaf evergreen forests on air quality, four forests of Quercus ilex (three peri-urban and one remote) were monitored in different areas in Spain. Concentrations of nitrogen dioxide (NO2), ammonia (NH3), nitric acid (HNO3) and ozone (O3) were measured during 2 years in open areas and inside the forests and aerosols (PM10) were monitored in open areas during 1 year. Ozone was the only air pollutant expected to have direct phytotoxic effects on vegetation according to current thresholds for the protection of vegetation. The concentrations of N compounds were not high enough to directly affect vegetation but could be contributing through atmospheric N deposition to the eutrophization of these ecosystems. Peri-urban forests of Q. ilex showed a significant below-canopy reduction of gaseous concentrations (particularly NH3, with a mean reduction of 29-38%), which indicated the feasibility of these forests to provide an ecosystem service of air quality improvement. Well-designed monitoring programs are needed to further investigate air quality improvement by peri-urban ecosystems while assessing the threat that air pollution can pose to vegetation.

  16. AMFIC Web Data Base - A Satellite System for the Monitoring and Forecasting of Atmospheric Pollution

    Directory of Open Access Journals (Sweden)

    P. Symeonidis

    2008-01-01

    Full Text Available In this work we present the contribution of the Laboratory of Atmospheric Pollution and Pollution Control Engineering of Democritus University of Thrace in the AMFIC-Air Monitoring and Forecasting In China European project. Within the framework of this project our laboratory in co-operation with DRAXIS company will create and manage a web satellite data base. This system will host atmospheric pollution satellite data for China and for the whole globe in general. Atmospheric pollution data with different spatial resolution such as O3 and NO2 total columns and measurements of other important trace gasses from GOME (ERS-2, SCIAMACHY (ENVISAT and OMI (EOS-AURA along with aerosol total load estimates from AATSR (ENVISAT will be brought to a common spatial and temporal resolution and become available to the scientific community in simple ascii files and maps format. Available will also be the results from the validation procedure of the satellite data with the use of ground-based observations and a set of high resolution maps and forecasts emerging from atmospheric pollution models. Data will be available for two geographical clusters. The one cluster includes the greater area of China and the other the whole globe. This integrated satellite system will be fully operational within the next two years and will also include a set of innovative tools that allow easy manipulation and analysis of the data. Automatic detection of features such as plumes and monitoring of their evolution, data covariance analysis enabling the detection of emission signatures of different sources, cluster analysis etc will be possible through those tools. The AMFIC satellite system shares a set of characteristics with its predecessor, AIRSAT. Here, we present some of these characteristics in order to bring out the contribution of such a system in atmospheric sciences.

  17. Atmospheric pollution in an urban environment by tree bark biomonitoring--part I: trace element analysis.

    Science.gov (United States)

    Guéguen, Florence; Stille, Peter; Lahd Geagea, Majdi; Boutin, René

    2012-03-01

    Tree bark has been shown to be a useful biomonitor of past air quality because it accumulates atmospheric particulate matter (PM) in its outermost structure. Trace element concentrations of tree bark of more than 73 trees allow to elucidate the impact of past atmospheric pollution on the urban environment of the cities of Strasbourg and Kehl in the Rhine Valley. Compared to the upper continental crust (UCC) tree barks are strongly enriched in Mn, Ni, Cu, Zn, Cd and Pb. To assess the degree of pollution of the different sites in the cities, a geoaccumulation index I(geo) was applied. Global pollution by V, Ni, Cr, Sb, Sn and Pb was observed in barks sampled close to traffic axes. Cr, Mo, Cd pollution principally occurred in the industrial area. A total geoaccumulation index I(GEO-tot) was defined; it is based on the total of the investigated elements and allows to evaluate the global pollution of the studied environment by assembling the I(geo) indices on a pollution map. Copyright © 2011 Elsevier Ltd. All rights reserved.

  18. A study on the environmental behavior of global air pollutants based on the continuous measurements of atmospheric radon concentrations

    International Nuclear Information System (INIS)

    Iida, Takao; Yamazawa, Hiromi

    2003-01-01

    Radon is a useful natural radioactive tracer of air transportation of atmospheric pollution, since radon is a noble gas and chemically inert. The atmospheric radon concentration is usually measured by a high-sensitivity electrostatic collection method or a two-filter method. The variations of radon concentrations observed over a solitary island and in the upper atmosphere are suitable for comparing with those of air pollutants. Some numerical simulation models were used to study the radon global transport in the atmosphere. In East Asia, atmospheric radon and air pollutants are transported with the air stream from the continent of China to the Northwestern Pacific Ocean. It is necessary to clarify the transport mechanism from both radon observations at various locations and numerical simulation. (author)

  19. Comparative discussion on some measurements of the atmospheric natural radioactivity and pollution with coal smoke particles

    International Nuclear Information System (INIS)

    Zoran, M.

    1977-01-01

    The results of measuring the natural radioactivity and coal smoke pollution are discussed for two sites in an industrial town, as well as for two heights at the same site, in connection with large scale and local atmospheric stability. The effects of the radiation fog upon the radon daughters acumulation near the ground are examined in some detail. By comparing the pollutant diurnal variations during two periods of similar atmospheric stability in autumn, respectively in winter, the contribution from the dwelling coal heating has been estimated to be about half of the total pollution in the town. (author)

  20. Archiving Derived Data with the PDS Atmospheres Node: The Educational Labeling System for Atmospheres (ELSA)

    Science.gov (United States)

    Neakrase, L. D. V.; Hornung, D.; Chanover, N.; Huber, L.; Beebe, R.; Johnson, J.; Sweebe, K.; Stevenson, Z.

    2017-06-01

    The PDS Atmospheres Node is developing an online tool, the Educational Labeling System for Atmospheres (ELSA), to aid in planning and creation of PDS4 bundles and associated labels for archiving derived data.

  1. Atmospheric pollution and human reproduction: Report on the Munich International Workshop

    Czech Academy of Sciences Publication Activity Database

    Slama, R.; Darrow, L.; Parker, J.; Woodruff, T.J.; Strickland, M.; Nieuwenhuijsen, M.; Glinianaia, S.; Hoggatt, J.; Kannan, S.; Hurley, K.; Kalinka, J.; Šrám, Radim; Brauer, M.; Wilhelm, M.; Heinrich, J.; Ritz, B.

    2008-01-01

    Roč. 116, č. 6 (2008), s. 791-798 ISSN 0091-6765 Institutional research plan: CEZ:AV0Z50390512 Keywords : Atmospheric pollution * Birth weight * Exposure assessment Subject RIV: DN - Health Impact of the Environment Quality Impact factor: 6.123, year: 2008

  2. Emission of pollutants in the atmosphere according to oil products quality

    International Nuclear Information System (INIS)

    Denkovska, Jasmina; Dimitrovski, Aleksandar

    1999-01-01

    In this paper the comparison of the environmental protection legal regulations as well as pollutants emission in atmosphere in a most European countries is shown. The air pollution directly depends on both fuel consumption and fuel quality. The fuel quality in Republic of Macedonia gradually is performing and incorporating with anchors European countries. On the other side, energy potentials have no rights to ignore environmental protection, neither environmental protection should be dominated under energy plants. Reciprocal antagonisms should be overtaken through corresponding legislation. (Author)

  3. Influence of weather and atmospheric pollution on physical activity in patients with COPD.

    Science.gov (United States)

    Alahmari, Ayedh D; Mackay, Alex J; Patel, Anant R C; Kowlessar, Beverly S; Singh, Richa; Brill, Simon E; Allinson, James P; Wedzicha, Jadwiga A; Donaldson, Gavin C

    2015-06-13

    Information concerning how climate and atmospheric pollutants affects physical activity in COPD patients is lacking and might be valuable in determining when physical activity should be encouraged. Seventy-three stable COPD patients recorded on daily diary cards worsening of respiratory symptoms, peak expiratory flow rate, hours spent outside the home and the number of steps taken per day. Pedometry data was recorded on 16,478 days, an average of 267 days per patient (range 29-658). Daily data for atmospheric PM10 and ozone (O3) were obtained for Bloomsbury Square, Central London from the Air Quality Information Archive databases. Daily weather data were obtained for London Heathrow from the British Atmospheric Data Archive. Colder weather below 22.5 °C, reduced daily step count by 43.3 steps day per °C (95% CI 2.14 to 84.4; p = 0.039) and activity was lower on rainy than dry days (p = 0.002) and on overcast compared to sunny days (p atmospheric pollution at high levels.

  4. A Regulation for the Control of Atmospheric Pollution, Amended Version.

    Science.gov (United States)

    Puerto Rico Environmental Quality Board, San Juan.

    Nine articles, related to the preservation of the natural quality of the air, and to prevention, elimination and control of atmospheric pollution in the Commonwealth of Puerto Rico, are contained in this document. These articles were written and enacted by the Environmental Quality Board in accordance with Law No. 9, approved June 18, 1970 -…

  5. Source-receptor metrology and modeling of trace amounts of atmospheric pollutants

    International Nuclear Information System (INIS)

    Coddeville, P.

    2005-12-01

    This work deals with acid pollution and with its long distance transport using the metrology of trace amounts of pollutants in rural environment and the identification of the emission sources at the origin of acid atmospheric fallouts. Several French and foreign precipitation collectors have been evaluated and tested on the field. The measurement efficiency and limitations of four sampling systems for gas and particulate sulfur, ammonia and nitrous compounds have been evaluated. The limits of methods and the measurement uncertainties have been determined and calculated. A second aspect concerns the development of oriented receptor-type statistical models with the aim of improving the research of emission sources in smaller size areas defined by the cells of a geographical mesh. The construction of these models combines the pollution data of the sites with the informations about the trajectories of air masses. Results are given as probability or concentration fields revealing the areas potentially at the origin of pollutant emissions. Areas with strong pollutant emissions have been detected at the Polish, Czech and German borders and have been identified as responsible of pollution events encountered in Morvan region. Quantitative source-receptor relations have been also established. The different atmospheric transport profiles, their related frequency and concentration have been also evaluated using a dynamical clouds classification of air mass retro-trajectories. Finally, the first medium-term exploitation results (14 years) of precipitation data from measurement stations allow to perfectly identify the different meteorological regimes of the French territory by establishing a relation with the chemical composition of rainfalls. A west-east oriented increase of rainfall acidity is observed over the French territory. The pluviometry of the north-east area being among the highest of France, it generates more important deposits of acidifying compounds. The analysis

  6. Atmospheric pollution assessment from a mountainous environment in Southern Ghana: case study of Abetifi

    International Nuclear Information System (INIS)

    Palm, Linda Maud Naa-Dedei

    2016-07-01

    In the pursuit to improve man’s livelihood, human activities which include emission of heavy metals from various industries and sectors, as well as the past use of chemicals such as pesticides, polychlorinated biphenyls and flame retardants have often mobilized and redistributed natural substances and anthropogenic pollutants into the atmosphere, predisposing it to relatively high concentrations of such pollutants even in pristine areas in the environment. This study assessed the level of atmospheric pollution, contributing sources and human health exposure risk of persistent organic pollutants (POPs) along with selected heavy metals with focus on Abetifi, one of the highest altitude environments in Ghana. Passive sampling with polyurethane foam (PUF) as adsorbent was employed. Samplers were deployed every 84 days for two years. A total of 65 polyurethane foams were deployed and twelve (12) groups of analytes were considered together with their various isomers. High resolution gas chromatographic technique coupled with high resolution mass spectrometry (HRGC-HRMS) and electron capture detectors (ECD) were used in the analysis of the POPs. Besides, high performance liquid chromatography (HPLC) coupled with MS was employed in analysing the perfluorinated compounds (PFCs) while the heavy metals were analysed using Atomic Absorption Spectrometer (AAS). Principal Component Analysis (PCA) and UNMIX model were used to group pollution source contribution of all analytes (POPs and heavy metals) in this study. Diagnostic isomer and other predictive ratios were also employed for source apportionment of various individual analyte groups. Results revealed that polychlorinated dibenzo-furans gave with the least total mean concentration (0.074 pg/m"3) for the sampling period and polybrominated biphenyls gave the highest (55 pg/m"3). The pesticide group gave values in the order of DRINs (53 pg/m"3) > DDT (41 pg/m"3) > HCHs (28 pg/m"3). Data for perflourinated compounds (PFCs) in

  7. Coupled atmosphere-soil-vegetation modelling for the assessment of the impact of atmospheric releases of heavy metals and of persistent organic pollutants at the European scale

    International Nuclear Information System (INIS)

    Queguiner, Solen

    2008-01-01

    The objective of this research thesis is to couple a model of atmospheric dispersion with a multi-environment model in order to perform impact studies related to atmospheric pollution by heavy metals and POPs (persistent organic pollutants). The author first presents the studied pollutants, their physical and chemical properties, and their effects on health. Then, he addresses the atmospheric modelling with a presentation of the used atmospheric dispersion model (POLAIR3D), and an application to heavy metals. Simulations are performed on a 4-year period in order to try to represent the inter-annual variability of atmospheric lead and cadmium concentrations. The next part reports the modelling of POPs which required the introduction of a soil model to address re-emissions. Results are compared with provided measurements. The fourth part reports the modelling of agricultural environments in the impact model, and more particularly physical processes and parameters proper to heavy metals and POPs. The author finally reports two case studies, one related to heavy metals, and the other to POPs [fr

  8. Atmospheric pollutant outflow from southern Asia: a review

    Science.gov (United States)

    Lawrence, M. G.; Lelieveld, J.

    2010-11-01

    Southern Asia, extending from Pakistan and Afghanistan to Indonesia and Papua New Guinea, is one of the most heavily populated regions of the world. Biofuel and biomass burning play a disproportionately large role in the emissions of most key pollutant gases and aerosols there, in contrast to much of the rest of the Northern Hemisphere, where fossil fuel burning and industrial processes tend to dominate. This results in polluted air masses which are enriched in carbon-containing aerosols, carbon monoxide, and hydrocarbons. The outflow and long-distance transport of these polluted air masses is characterized by three distinct seasonal circulation patterns: the winter monsoon, the summer monsoon, and the monsoon transition periods. During winter, the near-surface flow is mostly northeasterly, and the regional pollution forms a thick haze layer in the lower troposphere which spreads out over millions of square km between southern Asia and the Intertropical Convergence Zone (ITCZ), located several degrees south of the equator over the Indian Ocean during this period. During summer, the heavy monsoon rains effectively remove soluble gases and aerosols. Less soluble species, on the other hand, are lifted to the upper troposphere in deep convective clouds, and are then transported away from the region by strong upper tropospheric winds, particularly towards northern Africa and the Mediterranean in the tropical easterly jet. Part of the pollution can reach the tropical tropopause layer, the gateway to the stratosphere. During the monsoon transition periods, the flow across the Indian Ocean is primarily zonal, and strong pollution plumes originating from both southeastern Asia and from Africa spread across the central Indian Ocean. This paper provides a review of the current state of knowledge based on the many observational and modeling studies over the last decades that have examined the southern Asian atmospheric pollutant outflow and its large scale effects. An outlook

  9. Effects of atmospheric transport and trade on air pollution mortality in China

    Directory of Open Access Journals (Sweden)

    H. Zhao

    2017-09-01

    Full Text Available Air quality is a major environmental concern in China, where premature deaths due to air pollution have exceeded 1 million people per year in recent years. Here, using a novel coupling of economic, physical and epidemiological models, we estimate the premature mortality related to anthropogenic outdoor PM2. 5 air pollution in seven regions of China in 2010 and show for the first time how the distribution of these deaths in China is determined by a combination of economic activities and physical transport of pollution in the atmosphere. We find that 33 % (338 600 premature deaths of China's PM2. 5-related premature mortality in 2010 were caused by pollutants emitted in a different region of the country and transported in the atmosphere, especially from north to south and from east to west. Trade further extended the cross-regional impact; 56 % of (568 900 premature deaths China's PM2. 5-related premature mortality was related to consumption in another region, including 423 800 (42 % of total and 145 100 (14 % premature deaths from domestic consumption and international trade respectively. Our results indicate that multilateral and multi-stage cooperation under a regional sustainable development framework is in urgent need to mitigate air pollution and related health impacts, and efforts to reduce the health impacts of air pollution in China should be prioritized according to the source and location of emissions, the type and economic value of the emitting activities, and the related patterns of consumption.

  10. Atmospheric dispersion modeling of primary pollutants from electric power plants: Application to a coal-fired power plant

    International Nuclear Information System (INIS)

    McIlvaine, C.M.

    1994-01-01

    The normal operation of a power plant generally releases pollutants to the atmosphere. The objective of this paper is to describe a modeling method to estimate the changes in air pollutant concentrations that result from these emissions. This modeling approach is applicable to coal, biomass, oil, and natural gas technologies. As an example, this paper uses a hypothetical 500 megawatt (MW) coal-fired power plant, located at a Southeast Reference site in the U.S. and at a Southwest Reference Site. The pollutants resulting from the operation of the power plant may be classified as primary (emitted directly from the plant) or secondary (formed in the atmosphere from primary pollutants). The primary pollutants of interest in this paper are nitrogen oxides (NO x , sulfur dioxide SO 2 , particulate matter and metals

  11. Biomonitoring of atmospheric pollution (with emphasis on trace elements) - BioMAP. Proceedings of an international workshop

    International Nuclear Information System (INIS)

    2000-06-01

    Some organisms accumulate atmospheric contaminants over certain periods of time and concentrate them, thus allowing reliable analytical measurements if the organisms are suitably chosen. Measurements of contaminants accumulated by such organisms (biomonitors) provide information on the integrated exposure over an extended period of time. They may also be present in remote areas, and no expensive technical equipment is involved in collecting them. Therefore, biomonitoring can be an effective tool for pollutant mapping and trend monitoring by real time and retrospective analysis. The IAEA is making concerted efforts to promote the practical use of nuclear and related analytical techniques in studies of non-radioactive environmental pollutants that may impact human health, and one of the main emphases is on studying air contaminants. The idea of organizing a workshop on biomonitoring atmospheric pollution arose during an IAEA Technical Co-operation Project on Monitoring of Trace Element Air Pollution, carried out at the Instituto Tecnologico e Nuclear (ITN), Portugal, with substantial technical support by the Interfaculty Reactor Institute (IRI) of the Delft University of Technology (TUDelft), Netherlands. The International Workshop on Biomonitoring of Atmospheric Pollution (With Emphasis on Trace Elements) - BioMAP, was held in Lisbon, Portugal, from 21 to 24 September 1997. The meeting was organized in co-operation with the Instituto Tecnologico e Nuclear

  12. Biomonitoring of atmospheric pollution (with emphasis on trace elements) - BioMAP. Proceedings of an international workshop

    Energy Technology Data Exchange (ETDEWEB)

    NONE

    2000-06-01

    Some organisms accumulate atmospheric contaminants over certain periods of time and concentrate them, thus allowing reliable analytical measurements if the organisms are suitably chosen. Measurements of contaminants accumulated by such organisms (biomonitors) provide information on the integrated exposure over an extended period of time. They may also be present in remote areas, and no expensive technical equipment is involved in collecting them. Therefore, biomonitoring can be an effective tool for pollutant mapping and trend monitoring by real time and retrospective analysis. The IAEA is making concerted efforts to promote the practicaluse of nuclear and related analytical techniques in studies of non-radioactive environmental pollutants that may impact human health, and one of the main emphases is on studying air contaminants. The idea of organizing a workshop on biomonitoring atmospheric pollution arose during an IAEA Technical Co-operation Project on Monitoring of Trace Element Air Pollution, carried out at the Instituto Tecnologico e Nuclear (ITN), Portugal, with substantial technical support by the Interfaculty Reactor Institute (IRI) of the Delft University of Technology (TUDelft), Netherlands. The International Workshop on Biomonitoring of Atmospheric Pollution (With Emphasis on Trace Elements) - BioMAP, was held in Lisbon, Portugal, from 21 to 24 September 1997. The meeting was organized in co-operation with the Instituto Tecnologico e Nuclear.

  13. The effects of atmospheric pollutants upon standstone: evidence from real time measurements and analysis of decay features on historic buildings

    Energy Technology Data Exchange (ETDEWEB)

    Halsey, D.P.; Dews, J.; Harris, F.C. [Wolverhampton Univ. (United Kingdom). School of Construction, Engineering and Technology; Mitchell, D.J. [Wolverhampton Univ. (United Kingdom). School of Applied Sciences

    1995-12-31

    Due to the urbanisation and industrialisation of the West Midlands, UK, historic sandstone buildings are exposed to atmospheric pollution. In order to assess the impact of this pollution upon their deterioration, chemical analysis of runoff water, from sandstone and control surfaces, has been carried out. The amount of stone affected by atmospheric pollution has been quantified by surveying selected sandstone buildings. (author)

  14. The effects of atmospheric pollutants upon standstone: evidence from real time measurements and analysis of decay features on historic buildings

    Energy Technology Data Exchange (ETDEWEB)

    Halsey, D P; Dews, J; Harris, F C [Wolverhampton Univ. (United Kingdom). School of Construction, Engineering and Technology; Mitchell, D J [Wolverhampton Univ. (United Kingdom). School of Applied Sciences

    1996-12-31

    Due to the urbanisation and industrialisation of the West Midlands, UK, historic sandstone buildings are exposed to atmospheric pollution. In order to assess the impact of this pollution upon their deterioration, chemical analysis of runoff water, from sandstone and control surfaces, has been carried out. The amount of stone affected by atmospheric pollution has been quantified by surveying selected sandstone buildings. (author)

  15. Atmospheric Heavy Metal Pollution

    Indian Academy of Sciences (India)

    elements which constitute an important class of pollutants. Such pollutants ... spheric transport processes. In rural regions ... response of redox potential: those which are fixed in reducing conditions ... pollution in urban areas of northern Britain in the eighteenth .... adjusting the desired flame condition, the instrument is cali-.

  16. Magnetic particles in atmospheric particulate matter collected at sites with different level of air pollution

    Czech Academy of Sciences Publication Activity Database

    Petrovský, Eduard; Zbořil, R.; Matys Grygar, Tomáš; Kotlík, B.; Novák, J.; Kapička, Aleš; Grison, Hana

    2013-01-01

    Roč. 57, č. 4 (2013), s. 755-770 ISSN 0039-3169 R&D Projects: GA ČR GAP210/10/0554 Institutional support: RVO:67985530 ; RVO:61388980 Keywords : magnetite * atmospheric dust * pollution * rock magnetism Subject RIV: DI - Air Pollution ; Quality Impact factor: 0.752, year: 2013

  17. Atmospheric turbidity parameters in the high polluted site of egypt

    International Nuclear Information System (INIS)

    Shaltout, M.A.M.; Rahoma, U.A.

    1996-01-01

    Monthly variations of Linke, angstrom and Schuepp turbidity coefficients and gamma exponent as well as the influence of climatic factor on them are analysed. For each of these turbidity coefficients; calculated from measurements of broad band filters at Helwan, egypt, desert climate, are reported. A linear regression model fitted to Angstrom's turbidity turbidity coefficient beta and Linke turbidity L for Helwan. The calculation showed that, it is higher values of atmospheric turbidity coefficients due to, both the effect of air pollutants in the Helwan atmosphere from the four cement companies and some of heavy industrial factories, and the effect of the former's desert climate. 6 figs., 2 tabs

  18. Intense atmospheric pollution modifies weather: a~case of mixed biomass burning with fossil fuel combustion pollution in the eastern China

    OpenAIRE

    A. J. Ding; C. B. Fu; X. Q. Yang; J. N. Sun; T. Petäjä; V.-M. Kerminen; T. Wang; Y. N. Xie; E. Herrmann; L. F. Zheng; W. Nie; X. L. Wei; M. Kulmala

    2013-01-01

    The influence of air pollutants, particularly aerosols, on regional and global climate is widely investigated, but only a very limited number of studies reports their impacts on everyday weather. In this work, we present for the first time direct (observational) evidence of a clear effect how a mixed atmospheric pollution changes the weather with a substantial modification in air temperature and rainfall. By using comprehensive measurements in Nanjing, China, we found that mixed agricultural ...

  19. Historical atmospheric pollution trends in Southeast Asia inferred from lake sediment records.

    Science.gov (United States)

    Engels, S; Fong, L S R Z; Chen, Q; Leng, M J; McGowan, S; Idris, M; Rose, N L; Ruslan, M S; Taylor, D; Yang, H

    2018-04-01

    Fossil fuel combustion leads to increased levels of air pollution, which negatively affects human health as well as the environment. Documented data for Southeast Asia (SEA) show a strong increase in fossil fuel consumption since 1980, but information on coal and oil combustion before 1980 is not widely available. Spheroidal carbonaceous particles (SCPs) and heavy metals, such as mercury (Hg), are emitted as by-products of fossil fuel combustion and may accumulate in sediments following atmospheric fallout. Here we use sediment SCP and Hg records from several freshwater lentic ecosystems in SEA (Malaysia, Philippines, Singapore) to reconstruct long-term, region-wide variations in levels of these two key atmospheric pollution indicators. The age-depth models of Philippine sediment cores do not reach back far enough to date first SCP presence, but single SCP occurrences are first observed between 1925 and 1950 for a Malaysian site. Increasing SCP flux is observed at our sites from 1960 onward, although individual sites show minor differences in trends. SCP fluxes show a general decline after 2000 at each of our study sites. While the records show broadly similar temporal trends across SEA, absolute SCP fluxes differ between sites, with a record from Malaysia showing SCP fluxes that are two orders of magnitude lower than records from the Philippines. Similar trends in records from China and Japan represent the emergence of atmospheric pollution as a broadly-based inter-region environmental problem during the 20th century. Hg fluxes were relatively stable from the second half of the 20th century onward. As catchment soils are also contaminated with atmospheric Hg, future soil erosion can be expected to lead to enhanced Hg flux into surface waters. Copyright © 2018 Elsevier Ltd. All rights reserved.

  20. Development of ion-exchange collectors for monitoring atmospheric deposition of inorganic pollutants in Alaska parklands

    Science.gov (United States)

    Brumbaugh, William G.; Arms, Jesse W.; Linder, Greg L.; Melton, Vanessa D.

    2016-09-19

    Between 2010 and 2014, the U.S. Geological Survey completed a series of laboratory and field experiments designed to develop methodology to support the National Park Service’s long-term atmospheric pollutant monitoring efforts in parklands of Arctic Alaska. The goals of this research were to develop passive sampling methods that could be used for long-term monitoring of inorganic pollutants in remote areas of arctic parklands and characterize relations between wet and dry deposition of atmospheric pollutants to that of concentrations accumulated by mosses, specifically the stair-step, splendid feather moss, Hylocomium splendens. Mosses and lichens have been used by National Park Service managers as atmospheric pollutant biomonitors since about 1990; however, additional research is needed to better characterize the dynamics of moss bioaccumulation for various classes of atmospheric pollutants. To meet these research goals, the U.S. Geological Survey investigated the use of passive ionexchange collectors (IECs) that were adapted from the design of Fenn and others (2004). Using a modified IEC configuration, mulitple experiments were completed that included the following: (a) preliminary laboratory and development testing of IECs, (b) pilot-scale validation field studies during 2012 with IECs at sites with instrumental monitoring stations, and (c) deployment of IECs in 2014 at sites in Alaska having known or suspected regional sources of atmospheric pollutants where samples of Hylocomium splendens moss also could be collected for comparison. The targeted substances primarily included ammonium, nitrate, and sulfate ions, and certain toxicologically important trace metals, including cadmium, cobalt, copper, nickel, lead, and zinc.Deposition of atmospheric pollutants is comparatively low throughout most of Alaska; consequently, modifications of the original IEC design were needed. The most notable modification was conversion from a single-stage mixed-bed column to a two

  1. Studies of atmospheric pollutants concentration factors from La Reina reactor

    International Nuclear Information System (INIS)

    Vera, I.; Alegria, E.

    1983-01-01

    Results of an atmospheric diffusion model for pollutant gases re shown, in which the nuclear reactor of the La Reina Nuclear Centre is considered as the emitting source. The model uses a gaussian shape steady state cloud of concentration of pollutants and actual topographical and meteorological statistics data os the zone. Expected and maximum probable concentration factors are computed in a polar lattice in 16 wind directions. It was found that peaks for expected concentration factors and maximum probable concentration factors at ground level fall within the N and ESE directions at distances where hills or mountains reach the emitted cloud. A discussion of the practical value of these calculations is given. (Author)

  2. Studies of atmospheric pollutants concentration factors from La Reina reactor

    Energy Technology Data Exchange (ETDEWEB)

    Vera, I; Alegria, E [Comision Chilena de Energia Nuclear, Santiago. Div. de Seguridade Nuclear y Radioproteccion

    1983-11-01

    Results of an atmospheric diffusion model for pollutant gases are shown, in which the nuclear reactor of the La Reina Nuclear Centre is considered as the emitting source. The model uses a gaussian shape steady state cloud of concentration of pollutants and actual topographical and meteorological statistics data of the zone. Expected and maximum probable concentration factors are computed in a polar lattice in 16 wind directions. It was found that peaks for expected concentration factors and maximum probable concentration factors at ground level fall within the N and ESE directions at distances where hills or mountains reach the emitted cloud. A discussion of the practical value of these calculations is given.

  3. Elevational and Spatial Gradients of Atmospheric Metal Pollution in the North Pacific

    Science.gov (United States)

    Jongebloed, U. A.; Osterberg, E. C.; Kreutz, K. J.; Ferris, D. G.; Campbell, S.; Saylor, P. L.; Winski, D.; Handley, M.

    2017-12-01

    The industrial revolution has led to a several-fold increase in the atmospheric concentrations of heavy metals and metalloids including Pb, Cd, Cu, Zn, Hg and As. Modern emissions inventories identify Asia as the largest emitter of many of these toxic pollutants, which are subsequently transported eastwards across the North Pacific Ocean by prevailing westerly winds in the mid-upper troposphere. Previous ice cores collected from the Yukon Territory in the eastern North Pacific reveal evolution-dependent metal pollution histories; the highest (5300 m elevation) core from Mt. Logan records a nearly pure trans-Pacific Asian pollution record, whereas cores from lower sites like the Eclipse Icefield (3017 m) record a complex combination of Asian and more local North American emission. However, it is unclear if this elevation gradient of pollution sources is found in other regions of the North Pacific. Furthermore, the previous ice core records end in the late 1990's, before efforts by some Asian nations to reduce metal pollution, and it is unknown if North Pacific atmospheric metal concentrations have declined in response to these efforts. Here we investigate metal and metalloid concentrations and sources recorded in ice core and snow pit samples recovered from a vertical transect spanning 2200 - 5242 m within Denali National Park in the Central Alaska Range. We compare these metal concentrations and crustal enrichment factors to data from the Yukon Territory to investigate North Pacific regional metal gradients. We also present preliminary results from a new 60 m ice core from the Eclipse Icefield to evaluate recent trends in metal concentrations since the end of the Mt. Logan and original Eclipse records in 1998, and compare this to the recent metal pollution history recorded in the 2013 Denali Ice Core collected from the summit plateau (3900 m) of Mt. Hunter.

  4. Public Perceptions of How Long Air Pollution and Carbon Dioxide Remain in the Atmosphere.

    Science.gov (United States)

    Dryden, Rachel; Morgan, M Granger; Bostrom, Ann; Bruine de Bruin, Wändi

    2018-03-01

    The atmospheric residence time of carbon dioxide is hundreds of years, many orders of magnitude longer than that of common air pollution, which is typically hours to a few days. However, randomly selected respondents in a mail survey in Allegheny County, PA (N = 119) and in a national survey conducted with MTurk (N = 1,013) judged the two to be identical (in decades), considerably overestimating the residence time of air pollution and drastically underestimating that of carbon dioxide. Moreover, while many respondents believed that action is needed today to avoid climate change (regardless of cause), roughly a quarter held the view that if climate change is real and serious, we will be able to stop it in the future when it happens, just as we did with common air pollution. In addition to assessing respondents' understanding of how long carbon dioxide and common air pollution stay in the atmosphere, we also explored the extent to which people correctly identified causes of climate change and how their beliefs affect support for action. With climate change at the forefront of politics and mainstream media, informing discussions of policy is increasingly important. Confusion about the causes and consequences of climate change, and especially about carbon dioxide's long atmospheric residence time, could have profound implications for sustained support of policies to achieve reductions in carbon dioxide emissions and other greenhouse gases. © 2017 Society for Risk Analysis.

  5. Experiences with the Haertel-Truebungstest at diagnosing injuries to spruce caused by atmospheric pollution

    Energy Technology Data Exchange (ETDEWEB)

    Pelz, E

    1958-01-01

    The Haertel-Truebungstest is based on the observation that spruce needles secrete more wax at the stomata in areas affected by atmospheric pollution than in areas without. The increased secretion of wax is taken for a symptom of injury caused by atmospheric pollution. The wax is extracted in boiling water and, after cooling down, the turbidity of the extract is measured quantitatively in a photometer. Investigations on spruce in Saxony and Thuringia confirm the tendency to increasing turbidity towards the source of smoke. A considerable dispersion of turbidity values however impairs the results of this method, so that a great number of samples must be used in order to find out a trend. The dispersion of turbidity values in spruce forests that are not directly influenced by atmospheric pollution substantially exceeds the dispersion of the +/- 1% of the turbidity value that was found by Haertel. As was stated by Haertel and Papesch, the dispersion of individual turbidity values grows with increasing doses of SO/sub 2/. In Saxony the individual smoke emissions so densely cover one another, that there are scarcely any areas without air pollution and, probably, a relation exists between this continuous influence of smoke and SO/sub 2/ and the dispersion of turbidity values. It may be, however, that the environmental factors have also a certain influence, as, on vast areas of Saxony, spruce is growing on sites that are not its natural habitat.

  6. Intense atmospheric pollution modifies weather: a case of mixed biomass burning with fossil fuel combustion pollution in eastern China

    Science.gov (United States)

    Ding, A. J.; Fu, C. B.; Yang, X. Q.; Sun, J. N.; Petäjä, T.; Kerminen, V.-M.; Wang, T.; Xie, Y.; Herrmann, E.; Zheng, L. F.; Nie, W.; Liu, Q.; Wei, X. L.; Kulmala, M.

    2013-10-01

    The influence of air pollutants, especially aerosols, on regional and global climate has been widely investigated, but only a very limited number of studies report their impacts on everyday weather. In this work, we present for the first time direct (observational) evidence of a clear effect of how a mixed atmospheric pollution changes the weather with a substantial modification in the air temperature and rainfall. By using comprehensive measurements in Nanjing, China, we found that mixed agricultural burning plumes with fossil fuel combustion pollution resulted in a decrease in the solar radiation intensity by more than 70%, a decrease in the sensible heat by more than 85%, a temperature drop by almost 10 K, and a change in rainfall during both daytime and nighttime. Our results show clear air pollution-weather interactions, and quantify how air pollution affects weather via air pollution-boundary layer dynamics and aerosol-radiation-cloud feedbacks. This study highlights cross-disciplinary needs to investigate the environmental, weather and climate impacts of the mixed biomass burning and fossil fuel combustion sources in East China.

  7. Numerical study of the effects of local atmospheric circulations on a pollution event over Beijing-Tianjin-Hebei, China.

    Science.gov (United States)

    Miao, Yucong; Liu, Shuhua; Zheng, Yijia; Wang, Shu; Chen, Bicheng; Zheng, Hui; Zhao, Jingchuan

    2015-04-01

    Currently, the Chinese central government is considering plans to build a trilateral economic sphere in the Bohai Bay area, including Beijing, Tianjin and Hebei (BTH), where haze pollution frequently occurs. To achieve sustainable development, it is necessary to understand the physical mechanism of the haze pollution there. Therefore, the pollutant transport mechanisms of a haze event over the BTH region from 23 to 24 September 2011 were studied using the Weather Research and Forecasting model and the FLEXible-PARTicle dispersion model to understand the effects of the local atmospheric circulations and atmospheric boundary layer structure. Results suggested that the penetration by sea-breeze could strengthen the vertical dispersion by lifting up the planetary boundary layer height (PBLH) and carry the local pollutants to the downstream areas; in the early night, two elevated pollution layers (EPLs) may be generated over the mountain areas: the pollutants in the upper EPL at the altitude of 2-2.5 km were favored to disperse by long-range transport, while the lower EPL at the altitude of 1 km may serve as a reservoir, and the pollutants there could be transported downward and contribute to the surface air pollution. The intensity of the sea-land and mountain-valley breeze circulations played an important role in the vertical transport and distribution of pollutants. It was also found that the diurnal evolution of the PBLH is important for the vertical dispersion of the pollutants, which is strongly affected by the local atmospheric circulations and the distribution of urban areas. Copyright © 2015. Published by Elsevier B.V.

  8. A hydrogeochemical study of rain water to characterize the source of atmospheric pollutants at Jodhpur - desert city of India (abstract)

    International Nuclear Information System (INIS)

    Shrivastava, K.L.; Ojha, S.K.

    1999-01-01

    A study was undertaken has been conducted to determined the physical parameters and chemical species in the first precipitants of the season at desert city of Jodhpur to understand firstly, the degree of pollutants in the atmosphere and secondly to identity the minerals/pollutants of the atmosphere to characterize its possible source of origin. The precipitate samples for cations and other physical and chemical parameters by standard analytical methods. The results obtained on turbidity, conductivity, total dissolved solids and the ratio of total dissolved solids and conductivity, show a moderate degree of pollutants at all the four sites, A, B, C and D but slightly higher at C and D sites. The concentration of various water-soluble chemical species present in the precipitates, specially a balance between acidic and basic constituents decides its pH value. Hydrogen ions are mainly responsible for acidification of rain waters and are derived chiefly from oxidation of SO/sub 2/ and NO/sub 2/ to from H/sub 2/SO/sub 4/ and HNO/sub 3/ respectively. Hence a correlation study carried out between H/sup */and SO/sub 4//sup --/, NO/sub 3/ and Cl. Result shows no strong correlation between H/sup +/ and Cl/up -/. A group of strongly corrected elements Cl, Na/sup +/,K/sup +/ and Mg/sup ++/ were observed representing a similar source of their origin. The atmospheric desert dust components chiefly consist of quartz, mica flakes, clays like illite, kaolinite etc., and especially clays, may neutralize the acidity of precipitates via H/sup +/ exchange. Some minerals like Halite, Gypsum, Dolomite, Calcite may get slightly dissolved in the rainwater to replace H/sup +/ ions and so, impart alkalinity. Thus, it is logical to believe that the cations may have been derived originally from some of the geological source. Some rations like Cl/Na, Mg/Na, Ca/Na are known to have been used in characterization of the source. As expected in the atmosphere of desert city, like Jodhpur, the solid

  9. Atmospheric pollutant outflow from southern Asia: a review

    Directory of Open Access Journals (Sweden)

    M. G. Lawrence

    2010-11-01

    Full Text Available Southern Asia, extending from Pakistan and Afghanistan to Indonesia and Papua New Guinea, is one of the most heavily populated regions of the world. Biofuel and biomass burning play a disproportionately large role in the emissions of most key pollutant gases and aerosols there, in contrast to much of the rest of the Northern Hemisphere, where fossil fuel burning and industrial processes tend to dominate. This results in polluted air masses which are enriched in carbon-containing aerosols, carbon monoxide, and hydrocarbons. The outflow and long-distance transport of these polluted air masses is characterized by three distinct seasonal circulation patterns: the winter monsoon, the summer monsoon, and the monsoon transition periods. During winter, the near-surface flow is mostly northeasterly, and the regional pollution forms a thick haze layer in the lower troposphere which spreads out over millions of square km between southern Asia and the Intertropical Convergence Zone (ITCZ, located several degrees south of the equator over the Indian Ocean during this period. During summer, the heavy monsoon rains effectively remove soluble gases and aerosols. Less soluble species, on the other hand, are lifted to the upper troposphere in deep convective clouds, and are then transported away from the region by strong upper tropospheric winds, particularly towards northern Africa and the Mediterranean in the tropical easterly jet. Part of the pollution can reach the tropical tropopause layer, the gateway to the stratosphere. During the monsoon transition periods, the flow across the Indian Ocean is primarily zonal, and strong pollution plumes originating from both southeastern Asia and from Africa spread across the central Indian Ocean. This paper provides a review of the current state of knowledge based on the many observational and modeling studies over the last decades that have examined the southern Asian atmospheric pollutant outflow and its large scale

  10. Priority pollutant analysis of MHD-derived combustion products

    Science.gov (United States)

    Parks, Katherine D.

    An important factor in developing Magnetohydrodynamics (MHD) for commercial applications is environmental impact. Consequently, an effort was initiated to identify and quantify any possible undesirable minute chemical constituents in MHD waste streams, with special emphasis on the priority pollutant species. This paper discusses how priority pollutant analyses were used to accomplish the following goals at the University of Tennessee Space Institute (UTSI): comparison of the composition of solid combustion products collected from various locations along a prototypical MHD flow train during the firing of Illinois No. 6 and Montana Rosebud coals; comparison of solid waste products generated from MHD and conventional power plant technologies; and identification of a suitable disposal option for various MHD derived combustion products. Results from our ongoing research plans for gas phase sampling and analysis of priority pollutant volatiles, semi-volatiles, and metals are discussed.

  11. Meteorologia e poluição atmosférica Meteorology and atmospheric pollution

    Directory of Open Access Journals (Sweden)

    Davidson Martins Moreira

    2008-06-01

    Full Text Available Neste trabalho apresentam-se os principais aspectos relacionados à meteorologia ligada ao processo de dispersão turbulenta de poluentes atmosféricos. Ressalta-se que a meteorologia desempenha um papel fundamental para o controle da qualidade do ar, pois os eventos meteorológicos guiam a dispersão de poluentes e sua deposição no solo. Discutem-se os recentes melhoramentos da descrição e previsão dos fenômenos que envolvem a poluição atmosférica considerando a melhoria da qualidade de vida da população.This work shows the main aspects related to the meteorology linked to the process of turbulent dispersion of atmospheric pollutants. It is pointed out that meteorology is fundamental to air quality control, and meteorological events guide the pollutant dispersion and its deposition on the soil. Recent improvements on the description and forecast of the phenomena that involve atmospheric pollution, considering the population quality of life, are discussed.

  12. Ozone Atmospheric Pollution and Alzheimer's Disease: From Epidemiological Facts to Molecular Mechanisms.

    Science.gov (United States)

    Croze, Marine L; Zimmer, Luc

    2018-01-01

    Atmospheric pollution is a well-known environmental hazard, especially in developing countries where millions of people are exposed to airborne pollutant levels above safety standards. Accordingly, several epidemiological and animal studies confirmed its role in respiratory and cardiovascular pathologies and identified a strong link between ambient air pollution exposure and adverse health outcomes such as hospitalization and mortality. More recently, the potential deleterious effect of air pollution inhalation on the central nervous system was also investigated and mounting evidence supports a link between air pollution exposure and neurodegenerative pathologies, especially Alzheimer's disease (AD). The focus of this review is to highlight the possible link between ozone air pollution exposure and AD incidence. This review's approach will go from observational and epidemiological facts to the proposal of molecular mechanisms. First, epidemiological and postmortem human study data concerning residents of ozone-severely polluted megacities will be presented and discussed. Then, the more particular role of ozone air pollution in AD pathology will be described and evidenced by toxicological studies in rat or mouse with ozone pollution exposure only. The experimental paradigms used to reproduce in rodent the human exposure to ozone air pollution will be described. Finally, current insights into the molecular mechanisms through which ozone inhalation can affect the brain and play a role in AD development or progression will be recapitulated.

  13. Vegetation fires and air pollution in Vietnam.

    Science.gov (United States)

    Le, Thanh Ha; Thanh Nguyen, Thi Nhat; Lasko, Kristofer; Ilavajhala, Shriram; Vadrevu, Krishna Prasad; Justice, Chris

    2014-12-01

    Forest fires are a significant source of air pollution in Asia. In this study, we integrate satellite remote sensing data and ground-based measurements to infer fire-air pollution relationships in selected regions of Vietnam. We first characterized the active fires and burnt areas at a regional scale from MODIS satellite data. We then used satellite-derived active fire data to correlate the resulting atmospheric pollution. Further, we analyzed the relationship between satellite atmospheric variables and ground-based air pollutant parameters. Our results show peak fire activity during March in Vietnam, with hotspots in the Northwest and Central Highlands. Active fires were significantly correlated with UV Aerosol Index (UVAI), aerosol extinction absorption optical depth (AAOD), and Carbon Monoxide. The use of satellite aerosol optical thickness improved the prediction of Particulate Matter (PM) concentration significantly. Copyright © 2014 Elsevier Ltd. All rights reserved.

  14. Web technologies for rapid assessment of pollution of the atmosphere of the industrial city

    Science.gov (United States)

    Shaparev, N.; Tokarev, A.; Yakubailik, O.; Soldatov, A.

    2018-05-01

    The functionality, architectural features, the user interface of the geoinformation web-system of environmental monitoring of Krasnoyarsk is discussed. This system is created in service-oriented architecture. Data collection from the automated stations to monitor the state of atmospheric air has been implemented. An original device to measure the level of contamination of the atmosphere by fine dust PM2.5 has developed. Assessment of the level of air pollution is based on the quality index AQI atmosphere.

  15. Metallic corrosion in the polluted urban atmosphere of Hong Kong.

    Science.gov (United States)

    Liu, Bo; Wang, Da-Wei; Guo, Hai; Ling, Zhen-Hao; Cheung, Kalam

    2015-01-01

    This study aimed to explore the relationship between air pollutants, particularly acidic particles, and metallic material corrosion. An atmospheric corrosion test was carried out in spring-summer 2012 at a polluted urban site, i.e., Tung Chung in western Hong Kong. Nine types of metallic materials, namely iron, Q235 steel, 20# steel, 16Mn steel, copper, bronze, brass, aluminum, and aluminum alloy, were selected as specimens for corrosion tests. Ten sets of the nine materials were all exposed to ambient air, and then each set was collected individually after exposure to ambient air for consecutive 6, 13, 20, 27, 35, 42, 49, 56, 63, and 70 days, respectively. After the removal of the corrosion products on the surface of the exposed specimens, the corrosion rate of each material was determined. The surface structure of materials was observed using scanning electron microscopy (SEM) before and after the corrosion tests. Environmental factors including temperature, relative humidity, concentrations of gaseous pollutants, i.e., sulfur dioxide (SO₂), nitrogen dioxide (NO₂), carbon monoxide (CO), ozone (O₃), and particulate-phase pollutants, i.e., PM₂.₅ (FSP) and PM₁₀ (RSP), were monitored. Correlation analysis between environmental factors and corrosion rate of materials indicated that iron and carbon steel were damaged by both gaseous pollutants (SO₂ and NO₂) and particles. Copper and copper alloys were mainly corroded by gaseous pollutants (SO₂ and O₃), while corrosion of aluminum and aluminum alloy was mainly attributed to NO₂ and particles.

  16. NATO Advanced Study Institute on Pollutants from Combustion Formation and Impact on Atmospheric Chemistry

    CERN Document Server

    2000-01-01

    This volume is based on the lectures presented at the NATO Advanced Study Institute: (ASI) «Pollutants Formation from Combustion. Formation Mechanisms and Impact on th th Atmospheric Chemistry» held in Maratea, Italy, from 13 to 26 september 1998. Preservation of the environment is of increasing concern in individual countries but also at continental or world scales. The structure of a NATO ASI which involve lecturers and participants of different nationalities was thought as especially well suited to address environmental issues. As combustion is known to substantially contribute to the damaging of the atmosphere, it was natural to concentrate the ASI program on reviewing the currently available knowledge of the formation mechanisms of the main pollutants liberated by combustion systems. In most situations, pollutants are present as trace components and their formation and removal is strongly conditioned by the chemical reactions initiated by fuel consumption. Therefore specific lectures were aimed at defi...

  17. Pollutants transport and atmospheric variability of CO2 over Siberia: contribution of airborne measurements

    International Nuclear Information System (INIS)

    Paris, J.D.

    2008-12-01

    The work presented here intends to characterize the variations of atmospheric concentrations of CO 2 , CO, O 3 and ultrafine particles, over a large scale aircraft transect above Siberia, during three intensive YAK-AEROSIB campaigns in April 2006, September 2006 and August 2007, respectively. Pollutant and greenhouse gases distribution in this poorly studied region is needed to model atmospheric long range transport. I show here that CO concentrations at the time of the campaigns is broadly affected by (1) advection of Chinese pollutants through baro-clinic perturbations, (2) advection (diffuse or not) of European pollutants at various altitudes, (3) and of biomass burning from Central Asia. This set of factors is analyzed through a novel statistical technique based on clustering of backward transport simulated by the FLEXPART Lagrangian model. Large observed CO 2 gradients in summer are matched against vertical mixing in GCM simulated CO 2 . At last I present ultrafine particle measurements, and a possible nucleation summer maximum in the clean, continental mid-troposphere. (author)

  18. Elemental atmospheric pollution assessment via moss-based measurements in Portland, Oregon

    Science.gov (United States)

    Demetrios Gatziolis; Sarah Jovan; Geoffrey Donovan; Michael Amacher; Vicente Monleon

    2016-01-01

    Mosses accumulate pollutants from the atmosphere and can serve as an inexpensive screening tool for mapping air quality and guiding the placement of monitoring instruments. We measured 22 elements using 346 moss samples collected across Portland, Oregon, in December 2013. Our objectives were to develop citywide maps showing concentrations of each element in moss and...

  19. Long-range atmospheric transport of pollutants to the Eastern Mediterranean basin

    International Nuclear Information System (INIS)

    Tuncel, G.; Tuncel, S.

    1994-01-01

    A permanent stations has been established in the Eastern Mediterranean coast of Turkey for continuous monitoring of aerosols and precipitation. The station is part of the MED-POL programme which includes all countries that have coasts in the Mediterranean Sea and attempts to determine the role of the atmospheric fluxes of pollutants on the pollution of the Mediterranea Sea. Aerosol and deposition samples have been collected since early 1992. Concentrations of SO 4 , NO 3 , Cl, Li, Pb, K, Ca, Al, As, Cd, Cr, Cu, Se, Zn and Na were determined by ion chromatography and atomic absorption spectrometry. Daily samples will be screened to select the ones which correspond to transport from Europe and will be analyzed for a larger number of parameters using INAA. Method development took most of the time in 1992, and analysis are still in progress. Available data have shown that concentrations of anthropogenic elements are smaller in the Eastern Mediterranean atmosphere compared to other rural sites in the Europe. (author). 21 refs, 8 figs, 6 tabs

  20. An advanced open-path atmospheric pollution monitor for large areas

    International Nuclear Information System (INIS)

    Taylor, L.

    1995-01-01

    Large amounts of toxic waste materials, generated in manufacturing fuel for nuclear reactors, are stored in tanks buried over large areas at DOE sites. Flammable and hazardous gases are continually generated by chemical reactions in the waste materials. To prevent explosive concentrations of these gases, the gases are automatically vented to the atmosphere when the pressure exceeds a preset value. Real-time monitoring of the atmosphere above the tanks with automatic alarming is needed to prevent exposing workers to unsafe conditions when venting occurs. This project is to design, develop, and test an atmospheric pollution monitor which can measure concentrations of DOE-specified and EPA-specified hazardous gases over ranges as long as 4km. A CO 2 laser to measure absorption spectra and to determine the distance over which the measurements are made, is combined with an acousto-optic tunable filter (AOTF) to measure thermal emission spectra

  1. A landscape-scale approach to examining the fate of atmospherically derived industrial metals in the surficial environment.

    Science.gov (United States)

    Stromsoe, Nicola; Marx, Samuel K; McGowan, Hamish A; Callow, Nikolaus; Heijnis, Henk; Zawadzki, Atun

    2015-02-01

    Industrial metals are now ubiquitous within the atmosphere and their deposition represents a potential source of contamination to surficial environments. Few studies, however, have examined the environmental fate of atmospheric industrial metals within different surface environments. In this study, patterns of accumulation of atmospherically transported industrial metals were investigated within the surface environments of the Snowy Mountains, Australia. Metals, including Pb, Sb, Cr and Mo, were enriched in aerosols collected in the Snowy Mountains by 3.5-50 times pre-industrial concentrations. In sedimentary environments (soils, lakes and reservoirs) metals showed varying degrees of enrichment. Differences were attributed to the relative degree of atmospheric input, metal sensitivity to enrichment, catchment area and metal behaviour following deposition. In settings where atmospheric deposition dominated (ombrotrophic peat mires in the upper parts of catchments), metal enrichment patterns most closely resembled those in collected aerosols. However, even in these environments significant dilution (by 5-7 times) occurred. The most sensitive industrial metals (those with the lowest natural concentration; Cd, Ag, Sb and Mo) were enriched throughout the studied environments. However, in alpine tarn-lakes no other metals were enriched, due to the dilution of pollutant-metals by catchment derived sediment. In reservoirs, which were located lower within catchments, industrial metals exhibited more complex patterns. Particle reactive metals (e.g. Pb) displayed little enrichment, implying that they were retained up catchment, whereas more soluble metals (e.g., Cu and Zn) showed evidence of concentration. These same metals (Cu and Zn) were depleted in soils, implying that they are preferentially transported through catchments. Enrichment of other metals (e.g. Cd) varied between reservoirs as a function of contributing catchment area. Overall this study showed that the fate

  2. Response of protozoan and microbial communities in various coniferous forest soils after transfer to forests with different levels of atmospheric pollution.

    NARCIS (Netherlands)

    Couteaux, M.-M.; Raubuch, M.; Berg, M.P.

    1998-01-01

    During recent decades, forest ecosystems have been exposed to high levels of atmospheric pollution, and it has been argued that this affects the composition and activity of decomposer communities and, subsequently, ecosystem functioning. To investigate the effects of atmospheric pollution on

  3. Laser system for remote sensing monitoring of air pollution and quality control of the atmosphere

    Directory of Open Access Journals (Sweden)

    Belić Ilija

    2012-01-01

    Full Text Available Monitoring of the atmosphere and determination of the types and amounts of pollutants is becoming more important issue in complex and global monitoring of the environment. On the geocomponent and geocomplex level problem of monitoring the environment is attracting the attention of the scientific experts of different profiles (chemists, physicists, geographers, biologists, meteorologists, both in the national and international projects. Because of the general characteristics of the Earth's atmosphere (Dynamically Ballanced Instability DBI and the potential contribution to climate change solutions air-pollution monitoring has become particularly important field of environmental research. Control of aerosol distribution over Europe is enabled by EARLINET systems (European Aerosol Lidar NETwork. Serbia’s inclusion into these European courses needs development of the device, the standardization of methods and direct activity in determining the type, quantity and location of aerosol. This paper is analyzing the first step in the study of air-pollution, which is consisted of the realization of a functional model of LIDAR remote sensing devices for the large particle pollutants.

  4. Numerical models for computation of pollutant-dispersion in the atmosphere

    International Nuclear Information System (INIS)

    Leder, S.M.; Biesemann-Krueger, A.

    1985-04-01

    The report describes some models which are used to compute the concentration of emitted pollutants in the lower atmosphere. A dispersion model, developed at the University of Hamburg, is considered in more detail and treated with two different numerical methods. The convergence of the methods is investigated and a comparison of numerical results and dispersion experiments carried out at the Nuclear Research Center Karlsruhe is given. (orig.) [de

  5. Natural gas and quality of fuels for the reduction of atmospheric pollution

    International Nuclear Information System (INIS)

    Riva, A.; Occhio, L.; Andreetto, B.

    1998-01-01

    The production of atmospheric pollutants in combustion processes depends on plant characteristic, combustion conditions and fuel quality. The influence of fuel quality on the emission of sulphur oxides, nitrogen oxides, carbon monoxide, dust and carbon dioxide and on the emission of some toxic pollutants, such as heavy metals and polycyclic aromatic hydrocarbons, is analysed. The comparison between the emission limits, fixed by the Italian legislation, and the uncontrolled pollutant emissions, produced by fossil fuel combustion in power plants and industrial use, shows that, in order to comply with the limits, a reduction of pollutant emissions is required through the use of abatement systems and cleaner fuels where natural gas has a primary role. The use of cleaner fuels is particularly required in heating plants and appliances for the residential sector, where the development of new gas technologies further increases the environmental advantages of natural gas in comparison with other fuels [it

  6. Inorganic nitrogenous air pollutants, atmospheric nitrogen deposition and their potential ecological impacts in remote areas of western North America (Invited)

    Science.gov (United States)

    Bytnerowicz, A.; Fenn, M. E.; Fraczek, W.; Johnson, R.; Allen, E. B.

    2013-12-01

    Dry deposition of gaseous inorganic nitrogenous (N) air pollutants plays an important role in total atmospheric N deposition and its ecological effects in the arid and semi-arid ecosystems. Passive samplers and denuder/ filter pack systems have been used for determining ambient concentrations of ammonia (NH3), nitric oxide (NO), nitrogen dioxide (NO2), and nitric acid vapor (HNO3) in the topographically complex remote areas of the western United States and Canada. Concentrations of the measured pollutants varied significantly between the monitoring areas. Highest NH3, NO2 and HNO3 levels occurred in southern California areas downwind of the Los Angeles Basin and in the western Sierra Nevada impacted by emissions from the California Central Valley and the San Francisco Bay area. Strong spatial gradients of N pollutants were also present in southeastern Alaska due to cruise ship emissions and in the Athabasca Oil Sands Region in Canada affected by oil exploitation. Distribution of these pollutants has been depicted by maps generated by several geostatistical methodologies within the ArcGIS Geostatistical Analyst (ESRI, USA). Such maps help to understand spatial and temporal changes of air pollutants caused by various anthropogenic activities and locally-generated vs. long range-transported air pollutants. Pollution distribution maps for individual N species and gaseous inorganic reactive nitrogen (Nr) have been developed for the southern portion of the Sierra Nevada, Lake Tahoe Basin, San Bernardino Mountains, Joshua Tree National Park and the Athabasca Oil Sands Region. The N air pollution data have been utilized for estimates of dry and total N deposition by a GIS-based inferential method specifically developed for understanding potential ecological impacts in arid and semi-arid areas. The method is based on spatial and temporal distribution of concentrations of major drivers of N dry deposition, their surface deposition velocities and stomatal conductance values

  7. Aerosol Indices Derived from MODIS Data for Indicating Aerosol-Induced Air Pollution

    Directory of Open Access Journals (Sweden)

    Junliang He

    2014-02-01

    Full Text Available Aerosol optical depth (AOD is a critical variable in estimating aerosol concentration in the atmosphere, evaluating severity of atmospheric pollution, and studying their impact on climate. With the assistance of the 6S radiative transfer model, we simulated apparent reflectancein relation to AOD in each Moderate Resolution Imaging Spectroradiometer (MODIS waveband in this study. The closeness of the relationship was used to identify the most and least sensitive MODIS wavebands. These two bands were then used to construct three aerosol indices (difference, ratio, and normalized difference for estimating AOD quickly and effectively. The three indices were correlated, respectively, with in situ measured AOD at the Aerosol Robotic NETwork (AERONET Lake Taihu, Beijing, and Xianghe stations. It is found that apparent reflectance of the blue waveband (band 3 is the most sensitive to AOD while the mid-infrared wavelength (band 7 is the least sensitive. The difference aerosol index is the most accurate in indicating aerosol-induced atmospheric pollution with a correlation coefficient of 0.585, 0.860, 0.685, and 0.333 at the Lake Taihu station, 0.721, 0.839, 0.795, and 0.629 at the Beijing station, and 0.778, 0.782, 0.837, and 0.643 at the Xianghe station in spring, summer, autumn and winter, respectively. It is concluded that the newly proposed difference aerosol index can be used effectively to study the level of aerosol-induced air pollution from MODIS satellite imagery with relative ease.

  8. Data processing technique for multiangle lidar sounding of poorly stratified polluted atmospheres: Theory and experiment

    Science.gov (United States)

    Cyle E. Wold; Vladimir A. Kovalev; Alexander P. Petkov; Wei Min Hao

    2012-01-01

    Scanning elastic lidar, which can operate in different slant directions, is the most appropriate remote sensing tool for investigating the optical properties of smoke-polluted atmospheres. However, the commonly used methodologies of multiangle measurements are based on the assumption of horizontal stratification of the searched atmosphere1,2. When working in real...

  9. Intense atmospheric pollution modifies weather: a~case of mixed biomass burning with fossil fuel combustion pollution in the eastern China

    Science.gov (United States)

    Ding, A. J.; Fu, C. B.; Yang, X. Q.; Sun, J. N.; Petäjä, T.; Kerminen, V.-M.; Wang, T.; Xie, Y. N.; Herrmann, E.; Zheng, L. F.; Nie, W.; Wei, X. L.; Kulmala, M.

    2013-06-01

    The influence of air pollutants, particularly aerosols, on regional and global climate is widely investigated, but only a very limited number of studies reports their impacts on everyday weather. In this work, we present for the first time direct (observational) evidence of a clear effect how a mixed atmospheric pollution changes the weather with a substantial modification in air temperature and rainfall. By using comprehensive measurements in Nanjing, China, we found that mixed agricultural burning plumes with fossil fuel combustion pollution resulted in a decrease of solar radiation by more than 70%, of sensible heat flux over 85%, a temperature drop by almost 10 K, and a change of rainfall during daytime and nighttime. Our results show clear air pollution - weather interactions, and quantify how air pollution affects weather with the influence of air pollution-boundary layer dynamics and aerosol-radiation-cloudy feedbacks. This study highlights a cross-disciplinary needs to study the environmental, weather and climate impact of the mixed biomass burning and fossil fuel combustion sources in the East China.

  10. Comparing early twentieth century and present-day atmospheric pollution in SW France: A story of lichens

    International Nuclear Information System (INIS)

    Agnan, Y.; Séjalon-Delmas, N.; Probst, A.

    2013-01-01

    Lichens have long been known to be good indicators of air quality and atmospheric deposition. Xanthoria parietina was selected to investigate past (sourced from a herbarium) and present-day trace metal pollution in four sites from South-West France (close to Albi). Enrichment factors, relationships between elements and hierarchical classification indicated that the atmosphere was mainly impacted by coal combustion (as shown by As, Pb or Cd contamination) during the early twentieth century, whereas more recently, another mixture of pollutants (e.g. Sb, Sn, Pb and Cu) from local factories and car traffic has emerged. The Rare Earth Elements (REE) and other lithogenic elements indicated a higher dust content in the atmosphere in the early twentieth century and a specific lithological local signature. In addition to long-range atmospheric transport, local urban emissions had a strong impact on trace element contamination registered in lichens, particularly for contemporary data. - Highlights: ► We compared metal concentrations registered in contemporary and early 1900's lichens. ► In the past, As, Pb and Cd were enriched due to coal combustion. ► Nowadays, a new mixture of enriched contaminants (Sb, Sn, Pb and Cu) was evidenced. ► REE originated from local bedrock and proved an increased dust deposition in the past. ► Lichens recorded both local and long-range atmospheric contamination. - Using lichens registration, past (As, Pb, Cd) and recent (Sb, Sn, Cu) atmospheric pollution from local and long-range transport, as well as dust deposition, was evidenced in SW France.

  11. Analysis of the experimental data of air pollution using atmospheric dispersion modeling and rough set

    International Nuclear Information System (INIS)

    Halfa, I.K.I

    2008-01-01

    This thesis contains four chapters and list of references:In chapter 1, we introduce a brief survey about the atmospheric concepts and the topological methods for data analysis.In section 1.1, we give introduce a general introduction. We recall some of atmospheric fundamentals in Section 1.2. Section 1.3, shows the concepts of modern topological methods for data analysis.In chapter 2, we have studied the properties of atmosphere and focus on concept of Rough set and its properties. This concepts of rough set has been applied to analyze the atmospheric data.In section 2.1, we introduce a general introduction about concept of rough set and properties of atmosphere. Section 2.2 focuses on the concept of rough set and its properties and generalization of approximation of rough set theory by using topological space. In section 2.3 we have studied the stabilities of atmosphere for Inshas location for all seasons using different schemes and compared these schemes using statistical and rough set methods. In section 2.4, we introduce mixing height of plume for all seasons. Section 2.5 introduced seasonal surface layer turbulence processes for Inshas location. Section 2.6 gives a comparison between the seasonal surface layer turbulence processes for Inshas location and for different locations using rough set theory.In chapter 3 we focus on the concept of variable precision rough set (VPRS) and its properties and using it to compare, between the estimated and observed data of the concentration of air pollution for Inshas location. In Section 3.1 we introduce a general introduction about VPRS and air pollution. In Section 3.2 we have focused on the concept and properties of VPRS. In Section 3.3 we have introduced a method to estimate the concentration of air pollution for Inshas location using Gaussian plume model. Section 3.4 has showed the experimental data. The estimated data have been compared with the observed data using statistical methods in Section 3.5. In Section 3

  12. Comparing early twentieth century and present-day atmospheric pollution in SW France: A story of lichens.

    Science.gov (United States)

    Agnan, Y; Séjalon-Delmas, N; Probst, A

    2013-01-01

    Lichens have long been known to be good indicators of air quality and atmospheric deposition. Xanthoria parietina was selected to investigate past (sourced from a herbarium) and present-day trace metal pollution in four sites from South-West France (close to Albi). Enrichment factors, relationships between elements and hierarchical classification indicated that the atmosphere was mainly impacted by coal combustion (as shown by As, Pb or Cd contamination) during the early twentieth century, whereas more recently, another mixture of pollutants (e.g. Sb, Sn, Pb and Cu) from local factories and car traffic has emerged. The Rare Earth Elements (REE) and other lithogenic elements indicated a higher dust content in the atmosphere in the early twentieth century and a specific lithological local signature. In addition to long-range atmospheric transport, local urban emissions had a strong impact on trace element contamination registered in lichens, particularly for contemporary data. Copyright © 2012 Elsevier Ltd. All rights reserved.

  13. AICE Survey of USSR Air Pollution Literature, Volume 13: Technical Papers from the Leningrad International Symposium on the Meteorological Aspects of Atmospheric Pollution, Part 2.

    Science.gov (United States)

    Nuttonson, M. Y., Ed.

    Twelve papers were translated from Russian: Automation of Information Processing Involved in Experimental Studies of Atmospheric Diffusion, Micrometeorological Characteristics of Atmospheric Pollution Conditions, Study of theInfluence of Irregularities of the Earth's Surface on the Air Flow Characteristics in a Wind Tunnel, Use of Parameters of…

  14. Atmospheric dispersion and inverse modelling for the reconstruction of accidental sources of pollutants

    International Nuclear Information System (INIS)

    Winiarek, Victor

    2014-01-01

    Uncontrolled releases of pollutant in the atmosphere may be the consequence of various situations: accidents, for instance leaks or explosions in an industrial plant, or terrorist attacks such as biological bombs, especially in urban areas. In the event of such situations, authorities' objectives are various: predict the contaminated zones to apply first countermeasures such as evacuation of concerned population; determine the source location; assess the long-term polluted areas, for instance by deposition of persistent pollutants in the soil. To achieve these objectives, numerical models can be used to model the atmospheric dispersion of pollutants. We will first present the different processes that govern the transport of pollutants in the atmosphere, then the different numerical models that are commonly used in this context. The choice between these models mainly depends of the scale and the details one seeks to take into account. We will then present several inverse modeling methods to estimate the emission as well as statistical methods to estimate prior errors, to which the inversion is very sensitive. Several case studies are presented, using synthetic data as well as real data such as the estimation of source terms from the Fukushima accident in March 2011. From our results, we estimate the Cesium-137 emission to be between 12 and 19 PBq with a standard deviation between 15 and 65% and the Iodine-131 emission to be between 190 and 380 PBq with a standard deviation between 5 and 10%. Concerning the localization of an unknown source of pollutant, two strategies can be considered. On one hand parametric methods use a limited number of parameters to characterize the source term to be reconstructed. To do so, strong assumptions are made on the nature of the source. The inverse problem is hence to estimate these parameters. On the other hand nonparametric methods attempt to reconstruct a full emission field. Several parametric and nonparametric methods are

  15. L'IIASA and the integrated simulation of the trans-border atmospheric pollution assessment and evaluation

    International Nuclear Information System (INIS)

    Soleille, S.; Brignon, J.M.; Farret, R.; Landrieu, G.; Le Gall, A.C.; Rouil, L.

    2003-09-01

    The RAINS model is an integrated evaluation model for many pollutants and many effects, developed by he IIASA. This model studies the emissions of 4 atmospheric pollutants (nitrogen oxides, sulfur oxides, ammonium and volatile organic compounds) and the necessary costs to reduce them and the dispersion of these pollutants and their effects (tropospheric ozone formation, acidification and eutrophication). The model can be used in activities scenario mode (energy, agriculture, transports...) to calculate the emissions and their effects or in optimization mode to calculate strategies of emissions control from environmental constraints. (A.L.B.)

  16. AICE Survey of USSR Air Pollution Literature, Volume 14: Technical Papers from the Leningrad International Symposium on the Meteorological Aspects of Atmospheric Pollution, Part 3.

    Science.gov (United States)

    Nuttonson, M. Y.

    Fifteen papers were translated: On the removal of impurities from the atmosphere by clouds and precipitation; Some aspects of the adoption of automatic methods of determining atmospheric pollutants; Recording of sulfur dioxide content at the outskirts of a city. Comparison of measurement results for a valley and an elevation; Theoretical and…

  17. Atmospheric pollution and melanic moths in Manchester and its environs

    Energy Technology Data Exchange (ETDEWEB)

    Askew, R R; Cook, L M; Bishop, J A

    1971-01-01

    Samples of moths have been taken in the Manchester area at sites in localities with moderate to extreme atmospheric pollution. The majority of species collected are dark in color, many typically pale species being represented by dark variants. Four species polymorphic for melanic and non-melanic morphs have been examined in more detail. In Biston betularia the melanic frequency is over 93% at all stations, but the frequency of typicals appears to have increased over the past 15 years. This coincides with a period of extensive smoke control zonation. Gondontis bidentata has a higher frequency of melanics than has been recorded elsewhere in the country. There is significant variation between sites, the higher frequencies occurring in the more polluted localities. Non-melanics segregate into a pale and a dark category. In reared samples males exhibit a greater frequency of melanics than females.

  18. Calculations of color and visibility in urban atmospheres polluted by gaseous NO/sub 2/

    Energy Technology Data Exchange (ETDEWEB)

    Hodkinson, J.R.

    1966-01-01

    Calculations are made of the optical effects of persistent gaseous NO/sub 2/ pollution at 0.2-2 ppm in a city atmosphere in both the presence and absence of a polluting aerosol which does not absorb light or NO/sub 2/. It is concluded that the coloring of the horizon sky and of distant white objects would resemble whiskey, tea or cola-drinks, and the visual range would be markedly reduced. 2 references, 3 figures, 1 table.

  19. How and when urban vehicular traffic pollutes the environment

    International Nuclear Information System (INIS)

    Cera, L.; Di Mascio, P.

    1993-01-01

    This paper first compares monitored values of urban traffic air and noise pollution with Italian and European Communities pollution limits to assess the efficacy of current and proposed pollution regulations. The paper then focuses on the environmental impacts of the generation and discharge of waste waters during the construction and use of road surfaces. The related problems discussed include: soil erosion due to the increased exposure of bordering terrestrial ecosystems to damaging atmospheric pollutants; and the reception by roadside land areas of pollutants absorbed in rainfall runoff which has come into contact with road surfaces. Some suggestions are made on how to abate these particular types of traffic derived pollutants

  20. Tillandsia recurvata L. as a bioindicator of sulfur atmospheric pollution

    OpenAIRE

    Graciano, Corina; Fernández, L V; Caldiz, D O

    2003-01-01

    Tillandsia recurvata L. is an epiphyte that absorbs nutrients from the air, so it could be used as a bioindicator of atmospheric sulfur pollution. In order to test this idea, Tillandsia recurvata samples were seasonally collected for two years at three sites of La Plata, Buenos Aires Province, Argentina, in a suburban park and in a rural area 60 km away from the city. Macro- and microscopic observations were carried out and chlorophyll and sulfur concentrations of the tissue were measured to ...

  1. Attenuation of mining-derived pollutants in the hyporheic zone. A review

    International Nuclear Information System (INIS)

    Gandy, C.J.; Jarvis, A.P.; Smith, J.W.N.

    2007-01-01

    Mine water pollution is a major cause of surface- and groundwater pollution in former mining districts throughout Europe. It is a potential barrier to achieving good status water bodies, which is a requirement of the EU Water Framework Directive. In the UK, a concerted effort has been made over the last decade or so to address the scientific and practical challenges relating to the remediation of mine water pollution. However, most of this work has focused on remediation of point sources of pollution (typically arising from abandoned mines and shafts), while the behaviour of mine water at the groundwater-surface water interface (the 'hyporheic zone') has received far less attention in relevant scientific and engineering literature. The extent of mine water pollution and capacity for its attenuation at the hyporheic zone has not been well quantified while, furthermore, the complex chemical and microbial processes occurring there (specifically with reference to mining-derived pollutants) have not been investigated in any depth. The absence of such data may relate, in a large part, to the difficulty in physically measuring volumes and concentrations associated with these river inputs/exports. A far greater body of literature addresses biogeochemical processes at the hyporheic zone (especially relating to manganese), albeit many such articles relate to aqueous metal dynamics in general, rather than mine water specifically. This paper presents a review of the natural attenuation processes that may limit the movement and availability of mining-derived pollutants at the groundwater-surface water (GW-SW) interface, and specifically within the hyporheic zone. A substantial part focuses on precipitation and adsorption processes at the hyporheic zone, as well as discussing the role of microbial processes in governing metal ion mobility. (author)

  2. Attenuation of mining-derived pollutants in the hyporheic zone. A review

    Energy Technology Data Exchange (ETDEWEB)

    Gandy, C.J.; Jarvis, A.P. [Hydrogeochemical Engineering Research and Outreach (HERO), Institute for Research on Environment and Sustainability, Newcastle University, Newcastle upon Tyne, NE1 7RU (United Kingdom); Smith, J.W.N. [Environment Agency, Science Group, Solihull, West Midlands, B92 7HX (United Kingdom); Catchment Science Centre, Sheffield University, Kroto Research Institute, Sheffield, S3 7HQ (United Kingdom)

    2007-02-15

    Mine water pollution is a major cause of surface- and groundwater pollution in former mining districts throughout Europe. It is a potential barrier to achieving good status water bodies, which is a requirement of the EU Water Framework Directive. In the UK, a concerted effort has been made over the last decade or so to address the scientific and practical challenges relating to the remediation of mine water pollution. However, most of this work has focused on remediation of point sources of pollution (typically arising from abandoned mines and shafts), while the behaviour of mine water at the groundwater-surface water interface (the 'hyporheic zone') has received far less attention in relevant scientific and engineering literature. The extent of mine water pollution and capacity for its attenuation at the hyporheic zone has not been well quantified while, furthermore, the complex chemical and microbial processes occurring there (specifically with reference to mining-derived pollutants) have not been investigated in any depth. The absence of such data may relate, in a large part, to the difficulty in physically measuring volumes and concentrations associated with these river inputs/exports. A far greater body of literature addresses biogeochemical processes at the hyporheic zone (especially relating to manganese), albeit many such articles relate to aqueous metal dynamics in general, rather than mine water specifically. This paper presents a review of the natural attenuation processes that may limit the movement and availability of mining-derived pollutants at the groundwater-surface water (GW-SW) interface, and specifically within the hyporheic zone. A substantial part focuses on precipitation and adsorption processes at the hyporheic zone, as well as discussing the role of microbial processes in governing metal ion mobility. (author)

  3. Atmospheric lead and heavy metal pollution records from a Belgian peat bog spanning the last two millenia: Human impact on a regional to global scale

    Energy Technology Data Exchange (ETDEWEB)

    Vleeschouwer, Francois de [URAP, Departement de Geologie, Universite de Liege, Allee du 6 Aout B18 Sart Tilman B4000 - Liege (Belgium)]. E-mail: fdevleeschouwer@student.ulg.ac.be; Gerard, Laetitia [URAP, Departement de Geologie, Universite de Liege, Allee du 6 Aout B18 Sart Tilman B4000 - Liege (Belgium); Goormaghtigh, Catherine [Unite de recherche: ' Isotopes, Petrologie et Environnement' , Departement des Sciences de la Terre et de l' Environnement, CP 160/02 Universite Libre de Bruxelles, Avenue FD. Roosevelt, 50, B-1050 Bruxelles (Belgium); Mattielli, Nadine [Unite de recherche: ' Isotopes, Petrologie et Environnement' , Departement des Sciences de la Terre et de l' Environnement, CP 160/02 Universite Libre de Bruxelles, Avenue FD. Roosevelt, 50, B-1050 Bruxelles (Belgium); Le Roux, Gael [Institute of Environmental Geochemistry, University of Heidelberg, Im Neuenheimer Feld 236 B-69120 Heidelberg (Germany); Fagel, Nathalie [URAP, Departement de Geologie, Universite de Liege, Allee du 6 Aout B18 Sart Tilman B4000 - Liege (Belgium)

    2007-05-15

    Europe has been continuously polluted throughout the last two millennia. During the Roman Empire, these pollutions were mainly from ore extraction and smelting across Europe. Then, during the Middle Ages and the Early times of Industrial revolution (i.e. 1750), these pollutions extended to coal burning and combustion engine. Belgian ombrotrophic peat bogs have proved an effective archive of these pollutants and provide the opportunity to reconstruct the history of atmospheric deposition in NW Europe. The results of recent and past trace metal accumulation and Pb isotopes from a one-meter peat core (in the Misten peat bog) have been derived using XRF and Nu-plasma MC-ICP-MS. Combined with {sup 14}C and {sup 210}Pb dates these data have enabled us to trace fluxes in anthropogenic pollution back to original Roman times. Several periods of well-known Pb pollution events are clearly recorded including the Early and Late Roman Empire, the Middle Ages and the second industrial revolution. Also recorded is the introduction of leaded gasoline, and more recently the introduction of unleaded gasoline. Lead isotopes in this site have also enabled us to fingerprint several regional and global sources of anthropogenic particles.

  4. Atmospheric lead and heavy metal pollution records from a Belgian peat bog spanning the last two millenia. Human impact on a regional to global scale

    Energy Technology Data Exchange (ETDEWEB)

    De Vleeschouwer, Francois; Gerard, Laetitia; Fagel, Nathalie [URAP, Departement de Geologie, Universite de Liege, Allee du 6 Aout B18 Sart Tilman B4000 - Liege (Belgium); Goormaghtigh, Catherine; Mattielli, Nadine [Unite de recherche: ' ' Isotopes, Petrologie et Environnement' ' , Departement des Sciences de la Terre et de l' Environnement, CP 160/02 Universite Libre de Bruxelles, Avenue FD. Roosevelt, 50, B-1050 Bruxelles (Belgium); Le Roux, Gael [Institute of Environmental Geochemistry, University of Heidelberg, Im Neuenheimer Feld 236 B-69120 Heidelberg (Germany)

    2007-05-15

    Europe has been continuously polluted throughout the last two millennia. During the Roman Empire, these pollutions were mainly from ore extraction and smelting across Europe. Then, during the Middle Ages and the Early times of Industrial revolution (i.e. 1750), these pollutions extended to coal burning and combustion engine. Belgian ombrotrophic peat bogs have proved an effective archive of these pollutants and provide the opportunity to reconstruct the history of atmospheric deposition in NW Europe. The results of recent and past trace metal accumulation and Pb isotopes from a one-meter peat core (in the Misten peat bog) have been derived using XRF and Nu-plasma MC-ICP-MS. Combined with {sup 14}C and {sup 210}Pb dates these data have enabled us to trace fluxes in anthropogenic pollution back to original Roman times. Several periods of well-known Pb pollution events are clearly recorded including the Early and Late Roman Empire, the Middle Ages and the second industrial revolution. Also recorded is the introduction of leaded gasoline, and more recently the introduction of unleaded gasoline. Lead isotopes in this site have also enabled us to fingerprint several regional and global sources of anthropogenic particles. (author)

  5. Relationships between removal processes and residence times for atmospheric pollutants

    International Nuclear Information System (INIS)

    Slinn, W.G.N.

    1978-01-01

    This report is concerned with improving estimates for the residence times of atmospheric trace constituents in various atmospheric reservoirs. Residence times are defined only for steady-state conditions; i.e., when the net growth rate vanishes. The most useful case of vanishing net growth rate is when the total growth rate is equal to the decay rate. It is demonstrated that the most important advance towards improving estimates of pollutant residence times is through proper choices of reservoirs. Chosen reservoirs should possess the following features: steady-state conditions, uniform mixing ratio throughout or throughout specified subreservoirs, and subreservoirs chosen in which removal rates can be treated as approximate constants. An example of a poorly mixed reservoir, the stratosphere, is discussed. In another example, it is suggested that commonly used reservoirs for atmospheric CO 2 have been chosen poorly and that a substantial portion of the anthropogenic CO 2 released during the past 50 years may still be mixing into the stratosphere. In another example, it is suggested that determination of the dry deposition velocity for accumulation-mode aerosol particles may not be so important as previously thought. To improve estimates for the atmospheric residence times of these particles, it is important to increase knowledge of what is called the ascension velocity

  6. Exploratory analysis of atmospheric pollution in a coastal forest ecosystem in central Italy

    Directory of Open Access Journals (Sweden)

    Rita Aromolo

    2015-02-01

    Full Text Available Exploratory analysis of atmospheric pollution in a coastal forest ecosystem in central Italy - The study of spatial and temporal distribution of heavy metals in the atmosphere through the continuous assessment of deposition is of great interest for the analysis of anthropogenic pressure on the environment and the potential toxicity to humans and other living organisms. Information based on reliable estimates of heavy metals is therefore crucial for the evaluation of environmental quality. Trends in heavy metal concentration in atmospheric depositions on a coastal forest ecosystem (Castelporziano, Rome are analyzed in the present study based on a three-year monitoring field survey over three sites representative of different woodland characteristics in the area. Our results highlight both the influence of transportation processes in the short and medium distance based on the human pressure reflecting urban expansion and infrastructure development on the fringe of Castelporziano pristine forest. Further studies investigating the latent correlation with meteorological variables at various temporal scales are needed to provide a comprehensive picture of environmental conditions in a forest ecosystem subjected to increasing human pressure. Analysis of runoff water quality and the determination of other heavy metals, such as arsenic, may identify additional sources of pollution impacting soil and forest ecosystem.

  7. Atmospheric pollution and plant growth

    Energy Technology Data Exchange (ETDEWEB)

    Bleasdale, J K.A.

    1952-03-01

    Although sulfur dioxide is the most common and usually the most abundant polluting agent, experiments with this gas have shown that, under the conditions employed, there is no effect on yield unless the concentration is high enough to cause leaf injury. S23 ryegrass was grown in beds in greenhouses. Treatment with purified air gave, with one exception, a dry weight considerably higher than treatment with polluted air. No sign of leaf damage could be detected in the greenhouse with polluted air. This fact would seem to indicate that pollution decreases the growth rate, even in the absence of visible injury.

  8. Natural and anthropogenic pollution of the global atmosphere

    International Nuclear Information System (INIS)

    Jaworowski, Z.

    1999-01-01

    Results of determination of natural radionuclides, fission products and heavy metals in contemporary and pre-industrial ice from 14 glaciers in Southern and Northern Hemisphere, and in aerosols collected during three decades from seven altitudes between 0 and 15 km in the troposphere and atmosphere, were used for determinations of fluxes of man-made and natural pollutants into the global atmosphere. For these determinations 137 Cs from nuclear explosions and natural 210 Pb were used as tracers. Concentration of natural radionuclides and heavy metals in ice deposited before industrial revolution were higher than the contemporary precipitation presented as firn in high mountain and polar glaciers. This is due probably to volcanic activity which was higher before the first part of 20 th century. Man-made contribution to the total atmospheric flux is now 3.5% for 226 Ra, 12% for U, 7.4% for Pb, 011% for Cd, 62% for V and 5.8 for Hg. The mass of annual global wet precipitation, determined for the first time with radioactive tracers, is 5.7·10 1 7 kg. In Poland the lowest concentration of stable lead in human bones is now in highly industrialized southern districts. Lead level in medieval human bones from these districts reached up to 370 μg/g. Its current average level in inhabitants of southern Poland is 3.5 μg/g, i. e. similar as 1800 years ago. (author)

  9. Growing Atmospheric Pollution and Its Relation with Occurrences of Natural Hazards in India

    Science.gov (United States)

    Singh, Ramesh

    In the last three decades, multi satellite remote sensing data have revealed increasing atmospheric pollution. The satellite data have shown spatial distribution of fine and coarse atmospheric particles which impact human health, cloud albedo and atmospheric and meteorological parameters. The long range dusts coming over India travel through Arabian Sea and reach to the Bay of Bengal, such long range transport of dust influences atmospheric and ocean parameters, as a result strong coupling exists between land-ocean-atmosphere. Various kind of natural hazards, such as cyclone, algal bloom, cloud burst, excessive rainfall have been observed apart from the intense fog, haze and smog during winter and post monsoon seasons that have serious impacts on human health of people living in the Indo-Gangetic basin. The long range transport of dust and local anthropogenic emissions also reach to the Himalayan region affecting snow and glaciers of Himalaya and accelerating melting of snow and glaciers which is a threat of flooding of rivers originate from Himalayan region.

  10. The laser absorption spectrometer - A new remote sensing instrument for atmospheric pollution monitoring

    Science.gov (United States)

    Shumate, M. S.

    1974-01-01

    An instrument capable of remotely monitoring trace atmospheric constituents is described. The instrument, called a laser absorption spectrometer, can be operated from an aircraft or spacecraft to measure the concentration of selected gases in three dimensions. This device will be particularly useful for rapid determination of pollutant levels in urban areas.

  11. The effect of nitrogen additions on oak foliage and herbivore communities at sites with high and low atmospheric pollution

    International Nuclear Information System (INIS)

    Eatough Jones, Michele; Paine, Timothy D.; Fenn, Mark E.

    2008-01-01

    To evaluate plant and herbivore responses to nitrogen we conducted a fertilization study at a low and high pollution site in the mixed conifer forests surrounding Los Angeles, California. Contrary to expectations, discriminant function analysis of oak herbivore communities showed significant response to N fertilization when atmospheric deposition was high, but not when atmospheric deposition was low. We hypothesize that longer-term fertilization treatments are needed at the low pollution site before foliar N nutrition increases sufficiently to affect herbivore communities. At the high pollution site, fertilization was also associated with increased catkin production and higher densities of a byturid beetle that feeds on the catkins of oak. Leaf nitrogen and nitrate were significantly higher at the high pollution site compared to the low pollution site. Foliar nitrate concentrations were positively correlated with abundance of sucking insects, leafrollers and plutellids in all three years of the study. - Nitrogen additions at sites impacted by air pollution were associated with altered foliar herbivore communities and increased densities of a catkin-feeding beetle on Quercus kellogii

  12. A four-layer model for calculating the dispersion and chemical conversion of pollutants in the atmosphere

    International Nuclear Information System (INIS)

    Nguyen, T.H.

    1989-01-01

    A four-layer model for the calculation of the propagation and chemical change of emitted pollutants in the ground level troposphere is presented. The following influences on the spreading of pollutants are considered: the height of the mixing layer, the orography, the horizontal and vertical advection, the horizontal and vertical diffusion, the diurnal variation of insolation, the source strength of the emissions of NO x , HC, SO 2 and CO. The knowledge of the wind field is an essential precondition for spreading calculations in the ground level troposphere. For the calculation of the wind field, a wind model is developed with the help of the variation calculation. The propagation and the chemical change of pollutants in the atmosphere in the Upper Rhine Graben are calculated for various atmospheric conditions and emission data. The influences of the wind power orography, the parametrization of the turbulent diffusion and the emission volume on the concentration of the photooxidants are studied in detail. (orig./KW) With 82 figs., 9 tabs [de

  13. Human health risk assessment of lead pollution in atmospheric deposition in Baoshan District, Shanghai.

    Science.gov (United States)

    Chen, Yuanyuan; Wang, Jun; Shi, Guitao; Sun, Xiaojing; Chen, Zhenlou; Xu, Shiyuan

    2011-12-01

    The lead (Pb) content in atmospheric deposition was determined at 42 sampling sites in Baoshan District of Shanghai, China. Based on exposure and dose-response assessments, the health risk caused by Pb exposure in atmospheric deposition was investigated. The results indicated that Pb was significantly accumulated in atmospheric deposition. The spatial distribution of Pb was mapped by geostatistical analysis, and the results showed that pollution hotspots were present at traffic and industrial zones. Ingestion was the main route of Pb exposure in both adults and children. For children the risk value was above 1, whereas it was below 1 for the adult group. Therefore, children belong to the high-risk group for Pb exposure from atmospheric deposition in the observed area of Shanghai, China.

  14. Differential Optical-absorption Spectroscopy (doas) System For Urban Atmospheric-pollution Monitoring

    OpenAIRE

    Edner, H; Ragnarson, P; Spannare, S; Svanberg, Sune

    1993-01-01

    We describe a fully computer-controlled differential optical absorption spectroscopy system for atmospheric air pollution monitoring. A receiving optical telescope can sequentially tune in to light beams from a number of distant high-pressure Xe lamp light sources to cover the area of a medium-sized city. A beam-finding servosystem and automatic gain control permit unattended long-time monitoring. Using an astronomical code, we can also search and track celestial sources. Selected wavelength ...

  15. Atmospheric weighting functions and surface partial derivatives for remote sensing of scattering planetary atmospheres in thermal spectral region: general adjoint approach

    International Nuclear Information System (INIS)

    Ustinov, Eugene A.

    2005-01-01

    An approach to formulation of inversion algorithms for remote sensing in the thermal spectral region in the case of a scattering planetary atmosphere, based on the adjoint equation of radiative transfer (Ustinov (JQSRT 68 (2001) 195; JQSRT 73 (2002) 29); referred to as Papers 1 and 2, respectively, in the main text), is applied to the general case of retrievals of atmospheric and surface parameters for the scattering atmosphere with nadir viewing geometry. Analytic expressions for corresponding weighting functions for atmospheric parameters and partial derivatives for surface parameters are derived. The case of pure atmospheric absorption with a scattering underlying surface is considered and convergence to results obtained for the non-scattering atmospheres (Ustinov (JQSRT 74 (2002) 683), referred to as Paper 3 in the main text) is demonstrated

  16. The development of clean coal technology is the main way to control of atmospheric pollution in China

    Energy Technology Data Exchange (ETDEWEB)

    Wu Lixin; Xu Hong [Clean Coal Engineering & Research Center of Coal Industry (China)

    1999-11-01

    Atmospheric pollution in China and its causes are analysed. Power stations, industrial boilers and kilns and domestic coal combustion are the main pollution sources. Clean coal technologies are urgently needed. Main clean coal technologies which can improve the present situation of industrial coal combustion are coal cleaning, blending and briquetting; boiler retrofitting; advanced technologies to improve combustion efficiency and reduce pollution - fluidized bed combustion and pulverized coal desulfurization; and advanced desulfurization and dedusting technologies and equipment.

  17. The role of catchment vegetation in reducing atmospheric inputs of pollutant aerosols in Ganga river.

    Science.gov (United States)

    Shubhashish, Kumar; Pandey, Richa; Pandey, Jitendra

    2012-08-01

    The role of woody perennials in the Ganga river basin in modifying the run-off quality as influenced by atmospheric deposition of pollutant aerosols was investigated. The concentration of seven nutrients and eight metals were measured in atmospheric deposits as well as in run-off water under the influence of five woody perennials. Nutrient retention was recorded maximum for Bougainvillea spectabilis ranged from 4.30 % to 33.70 %. Metal retention was recorded highest for Ficus benghalensis ranged from 5.15 % to 36.98 %. Although some species showed nutrient enrichment, all the species considered in the study invariably contribute to reduce nutrients and metal concentration in run-off water. Reduction in run off was recorded maximum for B. spectabilis (nutrient 6.48 %-40.66 %; metal 7.86 %-22.85 %) and minimum for Ficus religiosa (nutrient 1.68 %-27.19 %; metal 6.55 %-31.55 %). The study forms the first report on the use of woody perennials in reducing input of atmospheric pollutants to Ganga river and has relevance in formulating strategies for river basin management.

  18. Influence of the characteristics of atmospheric boundary layer on the vertical distribution of air pollutant in China's Yangtze River Delta

    Science.gov (United States)

    Wang, Chenggang; Cao, Le

    2016-04-01

    Air pollution occurring in the atmospheric boundary layer is a kind of weather phenomenon which decreases the visibility of the atmosphere and results in poor air quality. Recently, the occurrence of the heavy air pollution events has become more frequent all over Asia, especially in Mid-Eastern China. In December 2015, the most severe air pollution in recorded history of China occurred in the regions of Yangtze River Delta and Beijing-Tianjin-Hebei. More than 10 days of severe air pollution (Air Quality Index, AQI>200) appeared in many large cities of China such as Beijing, Tianjin, Shijiazhuang and Baoding. Thus, the research and the management of the air pollution has attracted most attentions in China. In order to investigate the formation, development and dissipation of the air pollutions in China, a field campaign has been conducted between January 1, 2015 and January 28, 2015 in Yangtze River Delta of China, aiming at a intensive observation of the vertical structure of the air pollutants in the atmospheric boundary layer during the time period with heavy pollution. In this study, the observation data obtained in the field campaign mentioned above is analyzed. The characteristics of the atmospheric boundary layer and the vertical distribution of air pollutants in the city Dongshan located in the center of Lake Taihu are shown and discussed in great detail. It is indicated that the stability of the boundary layer is the strongest during the nighttime and the early morning of Dongshan. Meanwhile, the major air pollutants, PM2.5 and PM10 in the boundary layer, reach their maximum values, 177.1μg m-3 and 285μg m-3 respectively. The convective boundary layer height in the observations ranges from approximately 700m to 1100m. It is found that the major air pollutants tend to be confined in a relatively shallow boundary layer, which represents that the boundary layer height is the dominant factor for controlling the vertical distribution of the air pollutants. In

  19. Evaluation of atmospheric pollution in Kenitra city (MOROCCO) (Particles and Metals)

    International Nuclear Information System (INIS)

    Zghaid, M.; Noack, Y.; Tahiri, M.; Zahry, F.; Bounakhla, M.; Benyaich, F

    2008-01-01

    Full text: All Recent epidemiological studies show that air pollution in general and especially particulate pollution have a strong influence on human health, particularly on the respiratory and cardio-vascular systems, but also affect the developing fetus. Like developed countries, countries under development are subject to significant air pollution both urban and industrial. The car park is often old, sometimes uncontrolled industrialization, the regulations of atmospheric emissions are infancy and the network monitoring rare. The aim of this work is to focus on the problem of particulate air pollution in Kenitra (50 km north of Rabat, Morocco) by characterizing the pollution in both quantity and quality, to assess the impact potential health and provide decision makers with reliable data. Initial results show that the OMS recommendations, along with European standards on sulfur dioxide as well as PM10 are largely outdated (80 ug / Nm 3 instead of 40 in average). This is also the case for some metals: Lead concentrations are approximately ten times greater than those encountered in urban sites in Europe; nickel is fifteen times higher than the European standard. The metals are mainly present in the thin fraction (particles below 2.5 um). The low proportion of thin particles in the total particles, show the influence of resuspension events and other natural inputs from arid or desert. The SO2 average concentrations are also quite important (60 ug / m 3 ). The concentrations near the site are much higher than those that can be measured on similar sites in Europe. It is more than probable that in this city, the health impacts are not negligible. We will look to continue this work in three aspects: Spatial distribution of particulate pollution in Kenitra; The health impact of air pollution in Kenitra; Cyto-and geno-toxicity of airborne particles in Kenitra [fr

  20. Source apportionment of atmospheric mercury pollution in China using the GEOS-Chem model

    International Nuclear Information System (INIS)

    Wang, Long; Wang, Shuxiao; Zhang, Lei; Wang, Yuxuan; Zhang, Yanxu; Nielsen, Chris; McElroy, Michael B.; Hao, Jiming

    2014-01-01

    China is the largest atmospheric mercury (Hg) emitter in the world. Its Hg emissions and environmental impacts need to be evaluated. In this study, China's Hg emission inventory is updated to 2007 and applied in the GEOS-Chem model to simulate the Hg concentrations and depositions in China. Results indicate that simulations agree well with observed background Hg concentrations. The anthropogenic sources contributed 35–50% of THg concentration and 50–70% of total deposition in polluted regions. Sensitivity analysis was performed to assess the impacts of mercury emissions from power plants, non-ferrous metal smelters and cement plants. It is found that power plants are the most important emission sources in the North China, the Yangtze River Delta (YRD) and the Pearl River Delta (PRD) while the contribution of non-ferrous metal smelters is most significant in the Southwest China. The impacts of cement plants are significant in the YRD, PRD and Central China. - Highlights: • China's anthropogenic mercury emission was 643.1 t in 2007. • GEOS-Chem model well reproduces the background Hg concentrations. • Anthropogenic emissions contribute 35–50% of Hg concentrations in polluted regions. • The priorities for mercury control in polluted regions are identified. - Anthropogenic Hg emissions are updated and their impacts on atmospheric mercury concentrations and depositions are quantified for China

  1. Interception of wet deposited atmospheric pollutants by herbaceous vegetation: Data review and modelling

    Energy Technology Data Exchange (ETDEWEB)

    Gonze, M.-A., E-mail: marc-andre.gonze@irsn.fr; Sy, M.M.

    2016-09-15

    Better understanding and predicting interception of wet deposited pollutants by vegetation remains a key issue in risk assessment studies of atmospheric pollution. We develop different alternative models, following either empirical or semi-mechanistic descriptions, on the basis of an exhaustive dataset consisting of 440 observations obtained in controlled experiments, from 1970 to 2014, for a wide variety of herbaceous plants, radioactive substances and rainfall conditions. The predictive performances of the models and the uncertainty/variability of the parameters are evaluated under Hierarchical Bayesian modelling framework. It is demonstrated that the variability of the interception fraction is satisfactorily explained and quite accurately modelled by a process-based alternative in which absorption of ionic substances onto the foliage surfaces is determined by their electrical valence. Under this assumption, the 95% credible interval of the predicted interception fraction encompasses 81% of the observations, including situations where either plant biomass or rainfall intensity are unknown. This novel approach is a serious candidate to challenge existing empirical relationships in radiological or chemical risk assessment tools. - Highlights: • Literature data on the interception of atmospheric pollutants by herbs were reviewed • Predictive models were developed and evaluated in the Bayesian modelling framework • Sensitivity of interception to environmental conditions was satisfactorily explained • 81% of the observations were satisfactorily predicted by a semi-mechanistic model • This model challenges empirical relationships currently used in risk assessment tools.

  2. Long distance atmospheric pollution: assessment, risks, management and decision. Collection of abstracts of research works. Synthesis of results of researches performed within the framework of the PRIMEQUAL programme

    International Nuclear Information System (INIS)

    Kirchner, Severine; Ramalho, Olivier; Bellanger, Anne-Pauline; Blondeau, Patrice; Bonvallot, Nathalie; Campagna, Dave; Cellier, Pierre; Charles, Lionel; Coddeville, Patrice; Coll, Isabelle; Frejafon, Emeric; Gehin, Evelyne; George, Christian; Glorennec, Philippe; Gros, Valerie; Hecq, Walter; Laj, Paolo; Le Calve, Stephane; Mallet, Cecile; Momas, Isabelle; Mullot, Jean-Ulrich; Plaisance, Herve; Probst, Anne; Seigneur, Christian; Vlassopoulo, Chloe; Weiss, Karine

    2014-11-01

    After a brief presentation of the PRIMEQUAL programme, an inter-agency and institution research programme for a better air quality (275 supported research actions since the programme creation), an introduction presents the context of research works within this programme on long distance pollution. Various research works are then briefly presented. They address three main themes: 1) determining factors and atmospheric processes (role of organic nitrates in nitrogen transport, source and evolution of organic carbonated pollution in the atmosphere, modelling of long distance pollution, a miniature and autonomous station for atmospheric composition monitoring), 2) the regional evidence of pollutants transport (local and long distance pollution in Ile-de-France, pollutant transport and air quality in Mediterranean Sea, measurement and modelling of the deposition of Saharan dusts, relationship between forest fires and air quality), and 3) long term impacts on ecosystems, health and economy (peat lands as markers of atmospheric contamination, 20 years of measurements of atmospheric depositions in France and trends on the long term, vulnerability of ecosystems to atmospheric nitrogen, a cost-benefit approach to the relationship between long distance pollution and climate change). An appendix contains the call for research propositions which resulted in the above-mentioned researches

  3. The Influence of Meteorological Factors and Atmospheric Pollutants on the Risk of Preterm Birth

    NARCIS (Netherlands)

    Giorgis-Allemand, Lise; Pedersen, Marie; Bernard, Claire; Aguilera, Inmaculada; Beelen, Rob M J; Chatzi, Leda; Cirach, Marta; Danileviciute, Asta; Dedele, Audrius; van Eijsden, Manon; Estarlich, Marisa; Fernández-Somoano, Ana; Fernández, Mariana F; Forastiere, Francesco; Gehring, Ulrike; Grazuleviciene, Regina; Gruzieva, Olena; Heude, Barbara; Hoek, Gerard; de Hoogh, Kees; van den Hooven, Edith H; Håberg, Siri E; Iñiguez, Carmen; Jaddoe, Vincent W V; Korek, Michal; Lertxundi, Aitana; Lepeule, Johanna; Nafstad, Per; Nystad, Wenche; Patelarou, Evridiki; Porta, Daniela; Postma, Dirkje; Raaschou-Nielsen, Ole; Rudnai, Peter; Siroux, Valérie; Sunyer, Jordi; Stephanou, Euripides; Sørensen, Mette; Eriksen, Kirsten Thorup; Tuffnell, Derek; Varró, Mihály J; Vrijkotte, Tanja G M; Wijga, Alet; Wright, John; Nieuwenhuijsen, Mark J; Pershagen, Göran; Brunekreef, Bert; Kogevinas, Manolis; Slama, Rémy

    2017-01-01

    Atmospheric pollutants and meteorological conditions are suspected to be causes of preterm birth. We aimed to characterize their possible association with the risk of preterm birth (defined as birth occurring before 37 completed gestational weeks). We pooled individual data from 13 birth cohorts in

  4. The Influence of Meteorological Factors and Atmospheric Pollutants on the Risk of Preterm Birth.

    NARCIS (Netherlands)

    Giorgis-Allemand, Lise; Pedersen, Marie; Bernard, Claire; Aguilera, Inmaculada; Beelen, Rob M J; Chatzi, Leda; Cirach, Marta; Danileviciute, Asta; Dedele, Audrius; van Eijsden, Manon; Estarlich, Marisa; Fernández-Somoano, Ana; Fernández, Mariana F; Forastiere, Francesco; Gehring, Ulrike; Grazuleviciene, Regina; Gruzieva, Olena; Heude, Barbara; Hoek, Gerard; de Hoogh, Kees; van den Hooven, Edith H; Håberg, Siri E; Iñiguez, Carmen; Jaddoe, Vincent W V; Korek, Michal; Lertxundi, Aitana; Lepeule, Johanna; Nafstad, Per; Nystad, Wenche; Patelarou, Evridiki; Porta, Daniela; Postma, Dirkje; Raaschou-Nielsen, Ole; Rudnai, Peter; Siroux, Valérie; Sunyer, Jordi; Stephanou, Euripides; Sørensen, Mette; Eriksen, Kirsten Thorup; Tuffnell, Derek; Varró, Mihály J; Vrijkotte, Tanja G M; Wijga, Alet; Wright, John; Nieuwenhuijsen, Mark J; Pershagen, Göran; Brunekreef, Bert; Kogevinas, Manolis; Slama, Rémy

    2017-01-01

    Atmospheric pollutants and meteorological conditions are suspected to be causes of preterm birth. We aimed to characterize their possible association with the risk of preterm birth (defined as birth occurring before 37 completed gestational weeks). We pooled individual data from 13 birth cohorts in

  5. Severe Pollution in China Amplified by Atmospheric Moisture.

    Science.gov (United States)

    Tie, Xuexi; Huang, Ru-Jin; Cao, Junji; Zhang, Qiang; Cheng, Yafang; Su, Hang; Chang, Di; Pöschl, Ulrich; Hoffmann, Thorsten; Dusek, Uli; Li, Guohui; Worsnop, Douglas R; O'Dowd, Colin D

    2017-11-17

    In recent years, severe haze events often occurred in China, causing serious environmental problems. The mechanisms responsible for the haze formation, however, are still not well understood, hindering the forecast and mitigation of haze pollution. Our study of the 2012-13 winter haze events in Beijing shows that atmospheric water vapour plays a critical role in enhancing the heavy haze events. Under weak solar radiation and stagnant moist meteorological conditions in winter, air pollutants and water vapour accumulate in a shallow planetary boundary layer (PBL). A positive feedback cycle is triggered resulting in the formation of heavy haze: (1) the dispersal of water vapour is constrained by the shallow PBL, leading to an increase in relative humidity (RH); (2) the high RH induces an increase of aerosol particle size by enhanced hygroscopic growth and multiphase reactions to increase particle size and mass, which results in (3) further dimming and decrease of PBL height, and thus further depressing of aerosol and water vapour in a very shallow PBL. This positive feedback constitutes a self-amplification mechanism in which water vapour leads to a trapping and massive increase of particulate matter in the near-surface air to which people are exposed with severe health hazards.

  6. Atmospheric Chemistry Over Southern Africa

    Science.gov (United States)

    Gatebe, Charles K.; Levy, Robert C.; Thompson, Anne M.

    2011-01-01

    During the southern African dry season, regional haze from mixed industrial pollution, biomass burning aerosol and gases from domestic and grassland fires, and biogenic sources from plants and soils is worsened by a semi-permanent atmosphere gyre over the subcontinent. These factors were a driver of several major international field campaigns in the 1990s and early 2000s, and attracted many scientists to the region. Some researchers were interested in understanding fundamental processes governing chemistry of the atmosphere and interaction with climate change. Others found favorable conditions for evaluating satellite-derived measurements of atmospheric properties and a changing land surface. With that background in mind a workshop on atmospheric chemistry was held in South Africa. Sponsored by the International Commission for Atmospheric Chemistry and Global Pollution (ICACGP; http://www.icacgp.org/), the workshop received generous support from the South African power utility, Eskom, and the Climatology Research Group of the University of the Witwatersrand, Johannesburg, South Africa. The purpose of the workshop was to review some earlier findings as well as more recent findings on southern African climate vulnerability, chemical changes due to urbanization, land-use modification, and how these factors interact. Originally proposed by John Burrows, president of ICACGP, the workshop was the first ICACGP regional workshop to study the interaction of air pollution with global chemical and climate change. Organized locally by the University of the Witwatersrand, the workshop attracted more than 60 delegates from South Africa, Mozambique, Botswana, Zimbabwe, France, Germany, Canada, and the United States. More than 30 presentations were given, exploring both retrospective and prospective aspects of the science. In several talks, attention was focused on southern African chemistry, atmospheric pollution monitoring, and climate processes as they were studied in the field

  7. Modeling and evaluation of urban pollution events of atmospheric heavy metals from a large Cu-smelter.

    Science.gov (United States)

    Chen, Bing; Stein, Ariel F; Castell, Nuria; Gonzalez-Castanedo, Yolanda; Sanchez de la Campa, A M; de la Rosa, J D

    2016-01-01

    Metal smelting and processing are highly polluting activities that have a strong influence on the levels of heavy metals in air, soil, and crops. We employ an atmospheric transport and dispersion model to predict the pollution levels originated from the second largest Cu-smelter in Europe. The model predicts that the concentrations of copper (Cu), zinc (Zn), and arsenic (As) in an urban area close to the Cu-smelter can reach 170, 70, and 30 ng m−3, respectively. The model captures all the observed urban pollution events, but the magnitude of the elemental concentrations is predicted to be lower than that of the observed values; ~300, ~500, and ~100 ng m−3 for Cu, Zn, and As, respectively. The comparison between model and observations showed an average correlation coefficient of 0.62 ± 0.13. The simulation shows that the transport of heavy metals reaches a peak in the afternoon over the urban area. The under-prediction in the peak is explained by the simulated stronger winds compared with monitoring data. The stronger simulated winds enhance the transport and dispersion of heavy metals to the regional area, diminishing the impact of pollution events in the urban area. This model, driven by high resolution meteorology (2 km in horizontal), predicts the hourly-interval evolutions of atmospheric heavy metal pollutions in the close by urban area of industrial hotspot.

  8. Atmospheric Concentrations of Persistent Organic Pollutants in the Southern Ocean

    Science.gov (United States)

    Vlahos, P.; Edson, J.; Cifuentes, A.; McGillis, W. R.; Zappa, C.

    2008-12-01

    Long-range transport of persistent organic pollutant (POPs) is a global concern. Remote regions such as the Southern Ocean are greatly under-sampled though critical components in understanding POPs cycling. Over 20 high-volume air samples were collected in the Southern Ocean aboard the RV Brown during the GASEX III experiment between Mar 05 to April 9 2008. The relatively stationary platform (51S,38W) enabled the collection of a unique atmospheric time series at this open ocean station. Air sampling was also conducted across transects from Punto Arenas, Chile and to Montevideo, Uruguay. Samples were collected using glass sleeves packed with poly-urethane foam plugs and C-18 resin in order to collect target organic pollutants (per-fluorinated compounds, currently and historically used pesticides) in this under-sampled region. Here we present POPs concentrations and trends over the sampled period and compare variations with air parcel back trajectories to establish potential origins of their long-range transport.

  9. Annual Patterns of Atmospheric Pollutions and Episodes over Cairo Egypt

    Directory of Open Access Journals (Sweden)

    Y. Aboel Fetouh

    2013-01-01

    Full Text Available The Nile Delta major cities, particularly Cairo, experienced stagnant air pollution episodes, known as Black Cloud, every year over the past decade during autumn. Low-elevated thermal inversion layers play a crucial role in intensifying pollution impacts. Carbon monoxide, ozone, atmospheric temperature, water vapor, and methane measurements from the tropospheric emission spectrometer (TES on board the Aura have been used to assess the dominant component below the inversion layer. In this study, time series analysis, autocorrelations, and cross correlations are performed to gain a better understanding of the connections between those parameters and their local effect. Satellite-based data were obtained for the years 2005–2010. The parameters mentioned were investigated throughout the whole year in order to study the possible episodes that take place in addition to their change from year to year. Ozone and carbon monoxide were the two major indicators to the most basic episodes that occur over Cairo and the Delta region.

  10. Problematic of atmospheric pollution in Lebanon: the better stake is apprehended, the best acts are taken

    International Nuclear Information System (INIS)

    Chehab, Said

    2000-01-01

    The article is an overview on atmospheric pollution in Lebanon. It presents an analysis of sources of pollution in the country and their impacts on local and global environment and describes their control. Air pollution is mainly due to the industrial, electrical and transportation sectors. Pollutants from fuel combustion are analyzed. It is estimated that in 2010, CO 2 emissions will reach 5987250 tons, SO 2 emissions is estimated to be 182950 tons, Nox to 105180 and dusts to 4965 tons. CFC consumption and measures of control according to Montreal protocol are described. Consumption of primary energy, consumption of petroleum products, quantity of petroleum in refineries and production of cement in Lebanon are also presented in tables

  11. Size-differentiated composition of inorganic atmospheric aerosols of both marine and polluted continental origin

    Science.gov (United States)

    Harrison, Roy M.; Pio, Casimiro A.

    Atmospheric aerosols were sampled with a high volume impactor/diffusion battery system and the collected fractions analysed for their major water-soluble inorganic constituents. Sulphate, nitrate and chloride showed bimodal distributions; sulphate and nitrate were mainly associated with NH 4+, having approximately log-normal distributions with modes at 1.0 μm. In unpolluted maritime air, chlorides appeared as salts of sodium and magnesium with average modes at c. 5 μm, whilst in polluted air masses significant concentrations of ammonium chloride sub-μm aerosols were detected. Sodium nitrate and sodium sulphate aerosols having average modes of c. 3.5 μm were observed in mixed maritime/polluted air masses. The dimensions of these particles indicate formation from absorption of H 2SO 4 and HNO 3 at the surface of marine NaCl particles. The concentration of H + was very low, but the possibility of its neutralization by atmospheric ammonia during sampling was ruled out by parallel air sampling using an 'ammonia denuder'.

  12. Data on microscale atmospheric pollution of Bolshoy Kamen town (Primorsky region, Russia)

    Science.gov (United States)

    Kholodov, Aleksei; Ugay, Sergey; Drozd, Vladimir; Maiss, Natalia; Golokhvast, Kirill

    2017-10-01

    The paper discusses the study of atmospheric particulate matter of Bolshoy Kamen town by means of laser granulometry of snow water samples. Snow sampling points were selected close to major enterprises, along the main streets and roads of the town and in the residential area. The near-ground layer of atmospheric air of the town contains particulate matter of three main size classes: under 10 microns, 10-50 microns and over 700 microns. It is shown that the atmosphere of this town is lightly polluted with particles under 10 μm (PM10). Only in 5 sampling points out of 11 we found microparticles potentially hazardous to human health in significant quantities - from 16.2% to 34.6%. On the most territory of the town large particles (over 400 μm) dominate reaching 79.2%. We can conclude that judging by the particle size analysis of snow water samples Bolshoy Kamen town can be considered safe in terms of presence of particles under 10 μm (PM10) in the atmosphere.

  13. Recreational atmospheric pollution episodes: Inhalable metalliferous particles from firework displays

    Science.gov (United States)

    Moreno, Teresa; Querol, Xavier; Alastuey, Andrés; Cruz Minguillón, Mari; Pey, Jorge; Rodriguez, Sergio; Vicente Miró, José; Felis, Carles; Gibbons, Wes

    The use of fireworks creates an unusual and distinctive anthropogenic atmospheric pollution event. We report on aerosol samples collected during Las Fallas in Valencia, a 6-day celebration famous for its firework displays, and add comparative data on firework- and bonfire-contaminated atmospheric aerosol samples collected from elsewhere in Spain (Barcelona, L'Alcora, and Borriana) and during the Guy Fawkes celebrations in London. Specific high-profile official firework events during Las Fallas included the afternoon Mascletà and the nightly aerial displays (especially in the climactic final 2 days of the fiesta) and were accompanied by pollution spikes in suspended particles, NO, SO 2, and the creation and dispersal of an aerosol cloud enriched in a range of metallic elements. Notable metal aerosol concentration increases recorded during Las Fallas were potassium (from 500 to 5900 ng m -3), aluminium (as Al 2O 3 from around 600 to 2200 ng m -3), titanium (from 200 to 700 ng m -3), magnesium (from 100 to 500 ng m -3), lead (from 17 to 379 ng m -3), barium (from 39 to 322 ng m -3), strontium (from 3 to 112 ng m -3), copper (from 12 to 71 ng m -3), and antimony (from 1 to 52 ng m -3). Firework-contaminated aerosols of similarly metalliferous composition were also identified at the other monitoring sites, although different sites show variations attributable to other sources such as bonfires and local industry. Unusual levels of the trace elements Ba, Sr and (to a lesser extent) Cu, always in proportions with Ba dominant, along with strongly enhanced K, Pb, and Sb, are identified as being particularly characteristic of firework aerosols. Although firework-related recreational pollution episodes are transient in nature, they are highly concentrated, contribute significantly to total annual metal emissions, and are on average fine enough to be easily inhaled and a health risk to susceptible individuals.

  14. Regional transport and dilution during high-pollution episodes in southern France: Summary of findings from the Field Experiment to Constraint Models of Atmospheric Pollution and Emissions Transport (ESCOMPTE)

    Science.gov (United States)

    Drobinski, P.; SaïD, F.; Ancellet, G.; Arteta, J.; Augustin, P.; Bastin, S.; Brut, A.; Caccia, J. L.; Campistron, B.; Cautenet, S.; Colette, A.; Coll, I.; Corsmeier, U.; Cros, B.; Dabas, A.; Delbarre, H.; Dufour, A.; Durand, P.; GuéNard, V.; Hasel, M.; Kalthoff, N.; Kottmeier, C.; Lasry, F.; Lemonsu, A.; Lohou, F.; Masson, V.; Menut, L.; Moppert, C.; Peuch, V. H.; Puygrenier, V.; Reitebuch, O.; Vautard, R.

    2007-07-01

    In the French Mediterranean basin the large city of Marseille and its industrialized suburbs (oil plants in the Fos-Berre area) are major pollutant sources that cause frequent and hazardous pollution episodes, especially in summer when intense solar heating enhances the photochemical activity and when the sea breeze circulation redistributes pollutants farther north in the countryside. This paper summarizes the findings of 5 years of research on the sea breeze in southern France and related mesoscale transport and dilution of pollutants within the Field Experiment to Constraint Models of Atmospheric Pollution and Emissions Transport (ESCOMPTE) program held in June and July 2001. This paper provides an overview of the experimental and numerical challenges identified before the ESCOMPTE field experiment and summarizes the key findings made in observation, simulation, and theory. We specifically address the role of large-scale atmospheric circulation to local ozone vertical distribution and the mesoscale processes driving horizontal advection of pollutants and vertical transport and mixing via entrainment at the top of the sea breeze or at the front and venting along the sloped terrain. The crucial importance of the interactions between processes of various spatial and temporal scales is thus highlighted. The advances in numerical modeling and forecasting of sea breeze events and ozone pollution episodes in southern France are also underlined. Finally, we conclude and point out some open research questions needing further investigation.

  15. Regional transport and dilution during high-pollution episodes in southern France: Summary of findings from the Field Experiment to Constraint Models of Atmospheric Pollution and Emissions Transport (ESCOMPTE)

    International Nuclear Information System (INIS)

    Drobinski, P.; Menut, L.; Ancellet, G.; Bastin, S.; Colette, A.; Said, F.; Brut, A.; Campistron, B.; Cros, B.; Durand, P.; Lohou, F.; Moppert, C.; Puygrenier, V.; Arteta, J.; Cautenet, S.; Augustin, P.; Delbarre, H.; Caccia, J.L.; Guenard, V.; Coll, I.; Lasry, F.; Corsmeier, U.; Hasel, M.; Kalthoff, N.; Kottmeier, C.; Dabas, A.; Dufour, A.; Lemonsu, A.; Masson, V.; Peuch, V.H.; Reitebuch, O.; Vautard, R.

    2007-01-01

    In the French Mediterranean basin the large city of Marseille and its industrialized suburbs (oil plants in the Fos-Berre area) are major pollutant sources that cause frequent and hazardous pollution episodes, especially in summer when intense solar heating enhances the photochemical activity and when the sea breeze circulation redistributes pollutants farther north in the countryside. This paper summarizes the findings of 5 years of research on the sea breeze in southern France and related mesoscale transport and dilution of pollutants within the Field Experiment to Constraint Models of Atmospheric Pollution and Emissions Transport (ESCOMPTE) program held in June and July 2001. This paper provides an overview of the experimental and numerical challenges identified before the ESCOMPTE field experiment and summarizes the key findings made in observation, simulation, and theory. We specifically address the role of large-scale atmospheric circulation to local ozone vertical distribution and the mesoscale processes driving horizontal advection of pollutants and vertical transport and mixing via entrainment at the top of the sea breeze or at the front and venting along the sloped terrain. The crucial importance of the interactions between processes of various spatial and temporal scales is thus highlighted. The advances in numerical modeling and forecasting of sea breeze events and ozone pollution episodes in southern France are also underlined. Finally, we conclude and point out some open research questions needing further investigation. (authors)

  16. Regional transport and dilution during high-pollution episodes in southern France: Summary of findings from the Field Experiment to Constraint Models of Atmospheric Pollution and Emissions Transport (ESCOMPTE)

    Energy Technology Data Exchange (ETDEWEB)

    Drobinski, P.; Menut, L. [Ecole Polytechnique, Inst Pierre Simon Laplace, Laboratoire de Meteorologie Dynamique, F-91128 Palaiseau (France); Ancellet, G.; Bastin, S.; Colette, A. [Universite Pierre et Marie Curie, Institut Pierre Simon Laplace, Service d' aeronomie, 4 place Jussieu, F-75252 Paris, (France); Said, F.; Brut, A.; Campistron, B.; Cros, B.; Durand, P.; Lohou, F.; Moppert, C.; Puygrenier, V. [Univ Toulouse, Lab Aerol, F-31400 Toulouse, (France); Arteta, J.; Cautenet, S. [Univ Clermont Ferrand, Lab Meteorol Phys, F-63174 Aubiere, (France); Augustin, P.; Delbarre, H. [Univ Littoral Cote d' Opale, Lab Physicochim Atmosphere, F-59140 Dunkerque, (France); Caccia, J.L.; Guenard, V. [Univ Toulon and Var, Lab Sondages Electromagnet Environm Terr, F-83957 La Garde, (France); Coll, I.; Lasry, F. [Fac Sci and Technol, Lab Interuniv Syst Atmospher, F-94010 Creteil, (France); Corsmeier, U.; Hasel, M.; Kalthoff, N.; Kottmeier, C. [Univ Karlsruhe, Inst Meteorol and Klimaforsch, Forschungszentrum, D-76133 Karlsruhe, (Germany); Dabas, A.; Dufour, A.; Lemonsu, A.; Masson, V.; Peuch, V.H. [Ctr Natl Rech Meteorol, F-31057 Toulouse, (France); Reitebuch, O. [Deutsch Zentrum Luft and Raumfahrt, Inst Atmospher Phys, D-82234 Wessling, (Germany); Vautard, R. [Inst Pierre Simon Laplace, CEA Saclay, Lab Sci Climat and Environm, F-91191 Gif Sur Yvette, (France)

    2007-07-01

    In the French Mediterranean basin the large city of Marseille and its industrialized suburbs (oil plants in the Fos-Berre area) are major pollutant sources that cause frequent and hazardous pollution episodes, especially in summer when intense solar heating enhances the photochemical activity and when the sea breeze circulation redistributes pollutants farther north in the countryside. This paper summarizes the findings of 5 years of research on the sea breeze in southern France and related mesoscale transport and dilution of pollutants within the Field Experiment to Constraint Models of Atmospheric Pollution and Emissions Transport (ESCOMPTE) program held in June and July 2001. This paper provides an overview of the experimental and numerical challenges identified before the ESCOMPTE field experiment and summarizes the key findings made in observation, simulation, and theory. We specifically address the role of large-scale atmospheric circulation to local ozone vertical distribution and the mesoscale processes driving horizontal advection of pollutants and vertical transport and mixing via entrainment at the top of the sea breeze or at the front and venting along the sloped terrain. The crucial importance of the interactions between processes of various spatial and temporal scales is thus highlighted. The advances in numerical modeling and forecasting of sea breeze events and ozone pollution episodes in southern France are also underlined. Finally, we conclude and point out some open research questions needing further investigation. (authors)

  17. [Magnetic Response of Dust-loaded Leaves in Parks of Shanghai to Atmospheric Heavy Metal Pollution].

    Science.gov (United States)

    Liu, Fei; Chu, Hui-min; Zheng, Xiang-min

    2015-12-01

    To reveal the magnetic response to the atmospheric heavy metal pollution in leaves along urban parks, Camphor leaf samples, widely distributed at urban parks, were collected along the year leading wind direction of Shanghai, by setting two vertical and horizontal sections, using rock magnetic properties and heavy metal contents analysis. The results showed that the magnetic minerals of samples were predominated by ferromagnetic minerals, and both the concentration and grain size of magnetite particles gradually decreased with the winter monsoon direction from the main industrial district. A rigorous cleaning of leaves using ultrasonic agitator washer could remove about 63%-90% of low-field susceptibility values of the leaves, and this strongly indicated that the intensity of magnetic signal was mainly controlled by the PMs accumulated on the leaves surfaces. Moreover, there was a significant linear relationship between heavy metals contents (Fe, Mn, Zn, Cu, Cr, V and Pb) and magnetic parameters (0.442 ≤ R ≤ 0.799, P atmospheric heavy metal pollution. The results of multivariate statistical analysis showed that the content of magnetic minerals and heavy metal indust-loaded tree leaves was affected by associated pollution of industry and traffic.

  18. The changing face of urban air pollution

    Science.gov (United States)

    Lewis, Alastair C.

    2018-02-01

    The atmospheric chemistry that leads to photochemical smog and climate-active aerosols requires the presence of volatile organic compounds (VOCs) (1, 2). The VOCs in urban air typically derive from the prevailing energy and transport technologies as well as the use of petrochemical-derived products. On page 760 of this issue, McDonald et al. (3) report that a notable change in emissions may be underway in U.S. cities, with effects on secondary pollutants such as organic aerosols. Shifting from an urban atmosphere dominated by transport-related VOCs to one dominated by VOCs from coatings, adhesives, and consumer products would alter predictions of urban air quality and challenge the existing policy framework for emissions control.

  19. Simulation of trace metals and PAH atmospheric pollution over Greater Paris: Concentrations and deposition on urban surfaces

    Science.gov (United States)

    Thouron, L.; Seigneur, C.; Kim, Y.; Legorgeu, C.; Roustan, Y.; Bruge, B.

    2017-10-01

    Urban areas can be subject not only to poor air quality, but also to contamination of other environmental media by air pollutants. Here, we address the potential transfer of selected air pollutants (two metals and three PAH) to urban surfaces. To that end, we simulate meteorology and air pollution from Europe to a Paris suburban neighborhood, using a four-level one-way nesting approach. The meteorological and air quality simulations use urban canopy sub-models in order to better represent the effect of the urban morphology on the air flow, atmospheric dispersion, and deposition of air pollutants to urban surfaces. This modeling approach allows us to distinguish air pollutant deposition among various urban surfaces (roofs, roads, and walls). Meteorological model performance is satisfactory, showing improved results compared to earlier simulations, although precipitation amounts are underestimated. Concentration simulation results are also satisfactory for both metals, with a fractional bias Paris region. The model simulation results suggest that both wet and dry deposition processes need to be considered when estimating the transfer of air pollutants to other environmental media. Dry deposition fluxes to various urban surfaces are mostly uniform for PAH, which are entirely present in fine particles. However, there is significantly less wall deposition compared to deposition to roofs and roads for trace metals, due to their coarse fraction. Meteorology, particle size distribution, and urban morphology are all important factors affecting air pollutant deposition. Future work should focus on the collection of data suitable to evaluate the performance of atmospheric models for both wet and dry deposition with fine spatial resolution.

  20. Low levels of persistent organic pollutants (POPs) in New Zealand eels reflect isolation from atmospheric sources

    International Nuclear Information System (INIS)

    Holmqvist, Niklas; Stenroth, Patrik; Berglund, Olof; Nystroem, Per; Olsson, Karin; Jellyman, Don; McIntosh, Angus R.; Larsson, Per

    2006-01-01

    Polychlorinated biphenyls (PCBs) and organic pesticides (i.e., DDTs) were measured in long finned eels (Anguilla dieffenbachii) in 17 streams on the west coast of South Island, New Zealand. Very low levels of PCBs and low levels of ppDDE were found. The concentrations of PCBs and ppDDE were not correlated within sites indicating that different processes determined the levels of the two pollutants in New Zealand eels. The PCBs probably originate from atmospheric transport, ppDDE levels are determined by land use and are higher in agriculture areas. The low contamination level of these aquatic systems seems to be a function of a low input from both long and short-range transport as well as few local point sources. No correlation could be found between lipid content and persistent organic pollutants (POPs) concentration (as shown in previous studies) in the eels which could be explained by low and irregular intake of the pollutants. - Low levels of PCBs found in New Zealand eels reflect isolation from atmospheric sources while DDTs levels are determined by land use

  1. Air pollutants and atmospheric pressure increased risk of ED visit for spontaneous pneumothorax.

    Science.gov (United States)

    Park, Joo Hyung; Lee, Sun Hwa; Yun, Seong Jong; Ryu, Seokyong; Choi, Seung Woon; Kim, Hye Jin; Kang, Tae Kyung; Oh, Sung Chan; Cho, Suk Jin

    2018-04-14

    To investigate the impact of short-term exposure to air pollutants and meteorological variation on ED visits for primary spontaneous pneumothorax (PSP). We retrospectively identified PSP cases that presented at the ED of our tertiary center between January 2015 and September 2016. We classified the days into three types: no PSP day (0 case/day), sporadic days (1-2 cases/day), and cluster days (PSP, ≥3 cases/day). Association between the daily incidence of PSP with air pollutants and meteorological data were determined using Poisson generalized-linear-model to calculate incidence rate ratio (IRRs) and the use of time-series (lag-1 [the cumulative air pollution level on the previous day of PSP], lag-2 [two days ago], and lag-3 [three days ago]). Using multivariate logistic regression analysis, O 3 (p = 0.010), NO 2 (p = 0.047), particulate matters (PM) 10 (p = 0.021), and PM 2.5 (p = 0.008) were significant factors of PSP occurrence. When the concentration of O 3 , NO 2 , PM 10 , and PM 2.5 were increased, PSP IRRs increased approximately 15, 16, 3, and 5-fold, respectively. With the time-series analyses, atmospheric pressure in lag-3 was significantly lower and in lag-2, was significantly higher in PSP days compared with no PSP days. Among air pollutant concentrations, O 3 in lag-1 (p = 0.017) and lag-2 (p = 0.038), NO 2 in lag-1 (p = 0.015) and lag-2 (p = 0.009), PM 10 in lag-1 (p = 0.012), and PM 2.5 in lag-1 (p = 0.021) and lag-2 (p = 0.032) were significantly different between no PSP and PSP days. Increased concentrations of air pollutants and abrupt change in atmospheric pressure were significantly associated with increased IRR of PSP. Copyright © 2018 Elsevier Inc. All rights reserved.

  2. Influence of the atmospheric aerosol and air pollution on solar albedo of the earth. Vol. 4

    International Nuclear Information System (INIS)

    Mayhoub, A.B.; Mohamed, K.S.

    1996-01-01

    The effect of increasing atmospheric aerosol and air pollutant concentration on the solar albedo and consequently upon the heat budget near the earth's surface is studied. The magnitude of aerosol absorption coefficient to back-scattering coefficient B ab /B bs is calculated. This study will be used to estimate atmospheric stability categories and other meteorological parameters which are affected by thermal state radiation balance of the atmosphere as mixing and inversion height of Inshas nuclear reactor site. Consequently, concentration distribution of radioactive release from Inshas can be evaluated.. 4 figs., 5 tabs

  3. Influence of the atmospheric aerosol and air pollution on solar albedo of the earth. Vol. 4

    Energy Technology Data Exchange (ETDEWEB)

    Mayhoub, A B; Mohamed, K S [Mathematics and Theoretical Physics Department, Nuclear Research Center, Atomic Energy Auhtority, Cairo, (Egypt)

    1996-03-01

    The effect of increasing atmospheric aerosol and air pollutant concentration on the solar albedo and consequently upon the heat budget near the earth`s surface is studied. The magnitude of aerosol absorption coefficient to back-scattering coefficient B{sub ab}/B{sub bs} is calculated. This study will be used to estimate atmospheric stability categories and other meteorological parameters which are affected by thermal state radiation balance of the atmosphere as mixing and inversion height of Inshas nuclear reactor site. Consequently, concentration distribution of radioactive release from Inshas can be evaluated.. 4 figs., 5 tabs.

  4. Biomonitoring of atmospheric pollution (with emphasis on trace elements) - BioMap II. Proceedings of an international workshop

    International Nuclear Information System (INIS)

    2003-01-01

    Certain types of organisms integrate pollution over time, reducing the need for continuous chemical monitoring, thus avoiding the difficulty of interpreting 'snapshot' measurements and offering the potential of retrospective monitoring. Such organisms enrich the substance to be determined so that the analytical accessibility is improved and the measurement uncertainty reduced. By observing and measuring the changes in an appropriately selected organism, a conclusion as to the kind of pollution, its source, and its intensity can be drawn. The IAEA is making concerted efforts to promote the practical use of nuclear and related analytical techniques in studies of non-radioactive environmental pollutants that may impact on human health, and one of the main emphasis is on studying air contaminants. The IAEA has been systematically supporting biomonitoring atmospheric pollution for 10 years in the framework of its project on Environmental Pollution Monitoring and Research Using Nuclear and Related Analytical Techniques. The objective of this project is to identify the source and evaluate the fate of key non-radioactive environmental contaminants and provide the basis for improved health for human populations. The project has been implemented through a Coordinated Research Project on Validation and Application of Plants as Biomonitors of Trace Element Atmospheric Pollution Analysed by Nuclear and Related Techniques, several technical co-operation projects, and some dedicated analytical quality control activities. Within the scope of these efforts, the Second International Workshop on Biomonitoring of Atmospheric Pollution (with Emphasis on Trace Elements) - BioMAP, was organized as a follow-up to the 1997 BioMAP workshop held in Lisbon, Portugal. The proceedings of the first workshop were published in IAEA-TECDOC-1152. The second workshop was held in Praia da Vitoria, Azores Islands, Portugal, from 28 August to 3 September 2000. It was organized in co-operation with the

  5. Biomonitoring of atmospheric pollution (with emphasis on trace elements) - BioMap II. Proceedings of an international workshop

    Energy Technology Data Exchange (ETDEWEB)

    NONE

    2003-01-01

    Certain types of organisms integrate pollution over time, reducing the need for continuous chemical monitoring, thus avoiding the difficulty of interpreting 'snapshot' measurements and offering the potential of retrospective monitoring. Such organisms enrich the substance to be determined so that the analytical accessibility is improved and the measurement uncertainty reduced. By observing and measuring the changes in an appropriately selected organism, a conclusion as to the kind of pollution, its source, and its intensity can be drawn. The IAEA is making concerted efforts to promote the practical use of nuclear and related analytical techniques in studies of non-radioactive environmental pollutants that may impact on human health, and one of the main emphasis is on studying air contaminants. The IAEA has been systematically supporting biomonitoring atmospheric pollution for 10 years in the framework of its project on Environmental Pollution Monitoring and Research Using Nuclear and Related Analytical Techniques. The objective of this project is to identify the source and evaluate the fate of key non-radioactive environmental contaminants and provide the basis for improved health for human populations. The project has been implemented through a Coordinated Research Project on Validation and Application of Plants as Biomonitors of Trace Element Atmospheric Pollution Analysed by Nuclear and Related Techniques, several technical co-operation projects, and some dedicated analytical quality control activities. Within the scope of these efforts, the Second International Workshop on Biomonitoring of Atmospheric Pollution (with Emphasis on Trace Elements) - BioMAP, was organized as a follow-up to the 1997 BioMAP workshop held in Lisbon, Portugal. The proceedings of the first workshop were published in IAEA-TECDOC-1152. The second workshop was held in Praia da Vitoria, Azores Islands, Portugal, from 28 August to 3 September 2000. It was organized in co-operation with the

  6. Seasonal comparison of moss bag technique against vertical snow samples for monitoring atmospheric pollution.

    Science.gov (United States)

    Salo, Hanna; Berisha, Anna-Kaisa; Mäkinen, Joni

    2016-03-01

    This is the first study seasonally applying Sphagnum papillosum moss bags and vertical snow samples for monitoring atmospheric pollution. Moss bags, exposed in January, were collected together with snow samples by early March 2012 near the Harjavalta Industrial Park in southwest Finland. Magnetic, chemical, scanning electron microscopy-energy dispersive X-ray spectroscopy (SEM-EDX), K-means clustering, and Tomlinson pollution load index (PLI) data showed parallel spatial trends of pollution dispersal for both materials. Results strengthen previous findings that concentrate and slag handling activities were important (dust) emission sources while the impact from Cu-Ni smelter's pipe remained secondary at closer distances. Statistically significant correlations existed between the variables of snow and moss bags. As a summary, both methods work well for sampling and are efficient pollutant accumulators. Moss bags can be used also in winter conditions and they provide more homogeneous and better controlled sampling method than snow samples. Copyright © 2015. Published by Elsevier B.V.

  7. Online vehicle and atmospheric pollution monitoring using GIS and wireless sensor networks

    International Nuclear Information System (INIS)

    Cordova-Lopez, L E; Mason, A; Cullen, J D; Shaw, A; Al-Shamma'a, A I

    2007-01-01

    A Geographical Information System (GIS) is a computer system designed to integrate, store, edit, analyse, share and display geographically referenced data. A wireless sensor network (WSN) is a wireless network of spatially distributed autonomous devices using sensors to monitor physical or environmental conditions. This paper presents the integration of these two technologies to create a system able to detect measure and transmit information regarding the presence and quantities of internal combustion derived pollution and the geographical location in real time with the aim of creating pollution maps in urban environments

  8. An experience in Montenegro with atmospheric pollution by means of lichens

    International Nuclear Information System (INIS)

    Jovanovic, S.

    2000-01-01

    The very first study of the atmospheric pollution by means of bioindicators in the region of Montenegro was performed in 1992-93. The study, supported by the Commission of the European Union, was focused to the impact of an aluminium smelter plant to the air pollution in its surroundings. The plant (KAP) is situated 10 km to the south of Podgorica (capital of Montenegro) and produces some 100,000 tons of cast aluminium per year, using French (Pechine) technology. The technological process contributes in several manners to the atmospheric pollution. We investigated an area up to 50 km distances from the plant. Epiphytic lichens (Hypogymnia caperata) were collected from the tree bark 2 m above the ground. In the near vicinity of the plant no epiphytic lichens could have been found (died out due to high pollution levels). Instead, the more resistant lithophytic varieties (Lecanora expallens) were collected therein. Samples of wild grasses and pine needles were taken at the same spots, so as to compare the three indicators. We further found 5-10 times higher pollutant accumulation factors in lichens than in grasses or pine needles, emphasising thus the monitoring sensitivity of the lichens. Soil samples were also taken at the spots and analysed, but no impact factors for the soil were calculated. Samples were analysed by means of the k 0 -method of neutron activation analysis at 'Pierre Sue' Laboratory, Nuclear Research Centre, Saclay/Paris, France. Three types of analyses were made: (i) with short (matter of a few minutes) irradiations at the reactor ORPHEE , followed by analysing the short lived nuclides; (ii) with long (matter of hours) irradiations at the reactor OSIRIS, followed by analysing the long lived nuclides and occasionally - when necessary - (iii) epithermal analyses, in order to suppress the induced activities of certain matrix elements (e.g.Na) and obtain better sensitivity for the other elements. The following elements were determined down to

  9. Problematic of atmospheric pollution in Lebanon: the better stake is apprehended, the best acts are taken

    International Nuclear Information System (INIS)

    Chehab, Said

    1999-01-01

    Lebanon has imported in 1996 5000 Kt of carburants causing about 80 Kt of SO x ; 40 Kt of NO x ; 3 Kt of dusts and 3.5 million tons of CO 2 . The atmospheric pollution in Lebanon is due to three main sources: - Thermal central of electric production - Industries (cement) - Transportation sector The document describes in tables: the inventory of pollutants and pollutant emissions in 1993 and 2010; industrial and heating gas oil; liquified petroleum gas commercial propane; fuel oil for EDL; consumption of energy in 1996; sectorial distribution of pollutants PPM; emissions of CO 2 per tons per habitant in 1993; consumption in 1993 broken down by use and application. Finally, three projects concerning public transportation were presented

  10. An index for estimating the potential metal pollution contribution to atmospheric particulate matter from road dust in Beijing.

    Science.gov (United States)

    Zhao, Hongtao; Shao, Yaping; Yin, Chengqing; Jiang, Yan; Li, Xuyong

    2016-04-15

    The resuspension of road dust from street surfaces could be a big contributor to atmospheric particulate pollution in the rapid urbanization context in the world. However, to date what its potential contribution to the spatial pattern is little known. Here we developed an innovative index model called the road dust index (RIatmospheric suspended particles. The factors were ranked and weighted based on road dust characteristics (the amounts, grain sizes, and mobilities of the road dust, and the concentrations and toxicities of metals in the road dust). We then applied the RIatmospheric suspended particles. The results demonstrated that the road dust in urban areas has higher potential risk of metal to atmospheric particles than that in rural areas. The RIatmospheric suspended particles and for controlling atmospheric particulate pollution caused by road dust emissions. Copyright © 2016 Elsevier B.V. All rights reserved.

  11. Flux rates of atmospheric lead pollution within soils of a small catchment in northern Sweden and their implications for future stream water quality.

    Science.gov (United States)

    Klaminder, Jonatan; Bindler, Richard; Laudon, Hjalmar; Bishop, Kevin; Emteryd, Ove; Renberg, Ingemar

    2006-08-01

    It is not well-known how the accumulated pool of atmospheric lead pollution in the boreal forest soil will affect the groundwater and surface water chemistry in the future as this lead migrates through the soil profile. This study uses stable lead isotopes (206Pb/207Pb and 208Pb/ 207Pb ratios) to trace the transport of atmospheric lead pollution within the soil of a small catchment and predict future lead level changes in a stream draining the catchment. Low 206Pb/207Pb and 208Pb/207Pb ratios for the lead in the soil water (1.16 +/- 0.02; 2.43 +/- 0.03) and streamwater (1.18 +/- 0.03; 2.42 +/- 0.03) in comparison to that of the mineral soil (>1.4; >2.5) suggest that atmospheric pollution contributes by about 90% (65-100%) to the lead pool found in these matrixes. Calculated transport rates of atmospheric lead along a soil transect indicate that the mean residence time of lead in organic and mineral soil layers is at a centennial to millennial time scale. A maximum release of the present pool of lead pollution in the soil to the stream is predicted to occur within 200-800 years. Even though the uncertainty of the prediction is large, it emphasizes the magnitude of the time lag between the accumulation of atmospheric lead pollution in soils and the subsequent response in streamwater quality.

  12. A case study in atmospheric lead pollution of Northern-German coastal regions

    Energy Technology Data Exchange (ETDEWEB)

    Kapitza, H.; Eppel, D.P. [GKSS-Forschungszentrum Geesthacht GmbH (Germany). Inst. fuer Gewaesserphysik

    1998-12-31

    Transport and deposition of atmospheric lead over the coastal zone of Northern Germany are investigated. It is shown that marked differences in the impact of the ecologically valuable wadden sea areas can occur between summer and winter time. Due to the formation of sea breeze systems in summer the coastal zone is likely to be less stressed than in winter when the pollutant is confined to a shallow layer above ground. (orig.) 10 refs.

  13. Build-up and wash-off dynamics of atmospherically derived Cu, Pb, Zn and TSS in stormwater runoff as a function of meteorological characteristics.

    Science.gov (United States)

    Murphy, Louise U; Cochrane, Thomas A; O'Sullivan, Aisling

    2015-03-01

    Atmospheric pollutants deposited on impermeable surfaces can be an important source of pollutants to stormwater runoff; however, modelling atmospheric pollutant loads in runoff has rarely been done, because of the challenges and uncertainties in monitoring their contribution. To overcome this, impermeable concrete boards (≈ 1m(2)) were deployed for 11 months in different locations within an urban area (industrial, residential and airside) throughout Christchurch, New Zealand, to capture spatially distributed atmospheric deposition loads in runoff over varying meteorological conditions. Runoff was analysed for total and dissolved Cu, Zn, Pb, and total suspended solids (TSS). Mixed-effect regression models were developed to simulate atmospheric pollutant loads in stormwater runoff. In addition, the models were used to explain the influence of different meteorological characteristics (e.g. antecedent dry days and rain depth) on pollutant build-up and wash-off dynamics. The models predicted approximately 53% to 69% of the variation in pollutant loads and were successful in predicting pollutant-load trends over time which can be useful for general stormwater planning processes. Results from the models illustrated the importance of antecedent dry days on pollutant build-up. Furthermore, results indicated that peak rainfall intensity and rain duration had a significant relationship with TSS and total Pb, whereas, rain depth had a significant relationship with total Cu and total Zn. This suggested that the pollutant speciation phase plays an important role in surface wash-off. Rain intensity and duration had a greater influence when the pollutants were predominantly in their particulate phase. Conversely, rain depth exerted a greater influence when a high fraction of the pollutants were predominantly in their dissolved phase. For all pollutants, the models were represented by a log-arctan relationship for pollutant build-up and a log-log relationship for pollutant wash

  14. An advanced open path atmospheric pollution monitor for large areas

    Energy Technology Data Exchange (ETDEWEB)

    Taylor, L.; Suhre, D.; Mani, S. [and others

    1996-12-31

    Over 100 million gallons of radioactive and toxic waste materials generated in weapon materials production are stored in 322 tanks buried within large areas at DOE sites. Toxic vapors occur in the tank headspace due to the solvents used and chemical reactions within the tanks. To prevent flammable or explosive concentration of volatile vapors, the headspace are vented, either manually or automatically, to the atmosphere when the headspace pressure exceeds preset values. Furthermore, 67 of the 177 tanks at the DOE Hanford Site are suspected or are known to be leaking into the ground. These underground storage tanks are grouped into tank farms which contain closely spaced tanks in areas as large as 1 km{sup 2}. The objective of this program is to protect DOE personnel and the public by monitoring the air above these tank farms for toxic air pollutants without the monitor entering the tanks farms, which can be radioactive. A secondary objective is to protect personnel by monitoring the air above buried 50 gallon drums containing moderately low radioactive materials but which could also emit toxic air pollutants.

  15. Metal concentrations in homing pigeon lung tissue as a biomonitor of atmospheric pollution.

    Science.gov (United States)

    Cui, Jia; Halbrook, Richard S; Zang, Shuying; Han, Shuang; Li, Xinyu

    2018-03-01

    Atmospheric pollution in urban areas is a major worldwide concern with potential adverse impacts on wildlife and humans. Biomonitoring can provide direct evidence of the bioavailability and bioaccumulation of toxic metals in the environment that is not available with mechanical air monitoring. The current study continues our evaluation of the usefulness of homing pigeon lung tissue as a biomonitor of atmospheric pollution. Homing pigeons (1-2, 5-6, and 9-10+ year old (yo)) collected from Guangzhou during 2015 were necropsied and concentrations of cadmium (Cd), lead (Pb), and mercury (Hg) were measured in lung tissue. Lung Cd and Pb concentrations were significantly greater in 9-10+-year-old pigeons compared with those in other age groups, indicating their bioavailability and bioaccumulation. Lung Pb and Cd concentrations measured in 5-yo pigeons collected from Guangzhou during 2015 were significantly lower than concentrations reported in 5-yo homing pigeons collected from Guangzhou during 2011 and correlated with concentrations measured using mechanical air monitoring. In addition to temporal differences, spatial differences in concentrations of Cd, Pb, and Hg reported in ambient air samples and in pigeon lung tissues collected from Beijing and Guangzhou are discussed.

  16. The influence of atmospheric circulation on the air pollution concentration and temperature inversion in Sosnowiec. Case study

    Directory of Open Access Journals (Sweden)

    Widawski Artur

    2015-06-01

    Full Text Available Sosnowiec is located in the Katowice Region, which is the most urbanized and industrialized region in Poland. Urban areas of such character favor enhancement of pollution concentration in the atmosphere and the consequent emergence of smog. Local meteorological and circulation conditions significantly influence not only on the air pollution level but also change air temperature considerably in their centers and immediate vicinities. The synoptic situation also plays the major role in dispersal and concentration of air pollutants and changes in temperature profile. One of the most important are the near-ground (100 m inversions of temperature revealed their highest values on clear winter days and sometimes stay still for the whole day and night. Air temperature inversions in Sosnowiec occur mainly during anticyclone stagnation (Ca-anticyclone centre and Ka-anticyclonic ridge and in anticyclones with air advection from the south and southwest (Sa and SWa which cause significantly increase of air pollution values. The detailed evaluation of the influence of circulation types on the appearance of a particular concentration of pollutants carried out in this work has confirmed the predominant influence of individual circulation types on the development of air pollution levels at the Katowice region. This paper presents research case study results of the thermal structure of the near-ground atmospheric layer (100 m and air pollution parameters (PM10, SO2, NO, NO2 changes in selected days of 2005 year according to regional synoptic circulation types. The changes in urban environment must be taken into account in analyses of multiyear trends of air temperature and air conditions on the regional and global scales.

  17. Mixing state of particles with secondary species by single particle aerosol mass spectrometer in an atmospheric pollution event

    Science.gov (United States)

    Xu, Lingling; Chen, Jinsheng

    2016-04-01

    Single particle aerosol mass spectrometer (SPAMS) was used to characterize size distribution, chemical composition, and mixing state of particles in an atmospheric pollution event during 20 Oct. - 5 Nov., 2015 in Xiamen, Southeast China. A total of 533,012 particle mass spectra were obtained and clustered into six groups, comprising of industry metal (4.5%), dust particles (2.6%), carbonaceous species (70.7%), K-Rich particles (20.7%), seasalt (0.6%) and other particles (0.9%). Carbonaceous species were further divided into EC (70.6%), OC (28.5%), and mixed ECOC (0.9%). There were 61.7%, 58.3%, 4.0%, and 14.6% of particles internally mixed with sulfate, nitrate, ammonium and C2H3O, respectively, indicating that these particles had undergone significant aging processing. Sulfate was preferentially mixed with carbonaceous particles, while nitrate tended to mix with metal-containing and dust particles. Compared to clear days, the fractions of EC-, metal- and dust particles remarkably increased, while the fraction of OC-containing particles decreased in pollution days. The mixing state of particles, excepted for OC-containing particles with secondary species was much stronger in pollution days than that in clear days, which revealed the significant influence of secondary particles in atmospheric pollution. The different activity of OC-containing particles might be related to their much smaller aerodynamic diameter. These results could improve our understanding of aerosol characteristics and could be helpful to further investigate the atmospheric process of particles.

  18. Precision Orbit Derived Atmospheric Density: Development and Performance

    Science.gov (United States)

    McLaughlin, C.; Hiatt, A.; Lechtenberg, T.; Fattig, E.; Mehta, P.

    2012-09-01

    Precision orbit ephemerides (POE) are used to estimate atmospheric density along the orbits of CHAMP (Challenging Minisatellite Payload) and GRACE (Gravity Recovery and Climate Experiment). The densities are calibrated against accelerometer derived densities and considering ballistic coefficient estimation results. The 14-hour density solutions are stitched together using a linear weighted blending technique to obtain continuous solutions over the entire mission life of CHAMP and through 2011 for GRACE. POE derived densities outperform the High Accuracy Satellite Drag Model (HASDM), Jacchia 71 model, and NRLMSISE-2000 model densities when comparing cross correlation and RMS with accelerometer derived densities. Drag is the largest error source for estimating and predicting orbits for low Earth orbit satellites. This is one of the major areas that should be addressed to improve overall space surveillance capabilities; in particular, catalog maintenance. Generally, density is the largest error source in satellite drag calculations and current empirical density models such as Jacchia 71 and NRLMSISE-2000 have significant errors. Dynamic calibration of the atmosphere (DCA) has provided measurable improvements to the empirical density models and accelerometer derived densities of extremely high precision are available for a few satellites. However, DCA generally relies on observations of limited accuracy and accelerometer derived densities are extremely limited in terms of measurement coverage at any given time. The goal of this research is to provide an additional data source using satellites that have precision orbits available using Global Positioning System measurements and/or satellite laser ranging. These measurements strike a balance between the global coverage provided by DCA and the precise measurements of accelerometers. The temporal resolution of the POE derived density estimates is around 20-30 minutes, which is significantly worse than that of accelerometer

  19. Influence of climatic factors and pollution on the atmospheric corrosion of steels. Laboratory measurements

    International Nuclear Information System (INIS)

    Muylder, Jean van; Pourbaix, Marcel

    1977-01-01

    The influence of climatic and polluting factors on the atmospheric corrosion of four steels has been examined in the laboratory by an original accelerated electrochemical testing method. This research has led notably to the following conclusions: the corrosion behavior of the steels very much depends on the chloride- and SO 2 -contents of the rain water, as well as on the temperature of the metal during the drying periods. The best patinas have been obtained by submitting the steel successively to the corroding action of a solution of bisulphite and to the alternate actions of non-polluted rains and of drying, preferably at about 60 0 C. As a result of this, the formation of a protective patina may be accelerated by different methods. The relative merits of different steels under different conditions of atmospheric exposure may be predetermined by laboratory tests lasting several weeks. It is useful, when exposing steels in natural exposure sites, to measure as often as feasible the electrode potentials and the temperature of the steel specimens

  20. Determination of equivalent mixing height and atmospheric stability assessment

    International Nuclear Information System (INIS)

    Simon, J.; Bulko, M.; Holy, K.

    2007-01-01

    Atmospheric stability is an indicator that reflects the intensity of boundary layer mixing processes. This feature of the atmosphere is especially important since it defines dispersive atmospheric conditions and provides information on how effectively the anthropogenic pollution will be transferred to the higher levels of the atmosphere. The assessment of atmospheric dispersiveness plays a crucial role in the protection of air quality and public health in big cities. The presented paper deals with determination of atmospheric stability via so called Equivalent Mixing Height (EMH) quantity using a radioactive noble gas 222 Rn. A method of deriving a link between 222 Rn activity concentration, eddy diffusion coefficient and EMH using fluid mechanics is also outlined in this work. (authors)

  1. Pb isotopic composition of the atmosphere of the Sao Paulo city, Brazil, and isotopic characterization of some pollutant sources

    International Nuclear Information System (INIS)

    Aily, C.; Babinski, M.; Ruiz, I.R.; Sato, K

    2001-01-01

    Lead isotopes are known to be good tools for surveying lead origin in atmospheric samples (Chow et al., 1975). Lead has four naturally occurring stable isotopes: 206 Pb, 207 Pb, 208 Pb and 204 Pb. The first three isotopes are end products of radioactive decay chains from 238 U, 235 U and 232 Th, respectively, and the last one is non-radiogenic. Therefore, their abundance and the ratios among the four isotopes gradually change with time. Lead in the atmosphere comes from various sources, such as leaded gasoline, industrial emissions and coal combustion. Thus, lead isotope ratios different from those of the mother rock in the region are often observed in the atmosphere (Tatsumoto and Patterson, 1963). Lead is emitted to the atmosphere in fine particles, which can be transported within air masses for very long distances, e. g. from mid latitude regions to the Artic and Antarctica (Sturges and Barrie, 1989). Lead isotopes have been used to trace the pollutant sources in many cities of the world. However, a systematic study using this methodology has not been done in any Brazilian city. The main purpose of the present work is to characterize the Pb isotope composition in the atmosphere in Sao Paulo city, and suggest the possible pollutant sources. For our study lead isotopes were measured in different samples: aerosols and rainwater which would yield the Pb isotope composition of the atmosphere. Samples of gasoline and ethanol, gutter sweepings, soot from vehicle exhaust pipes, and filters containing particulate material from industrial emissions were also analyzed, since they were considered potential pollutant sources of the atmosphere. In order to obtain the local geogenic Pb isotopic composition we also analyzed rock and K-feldspar samples. Lead concentrations were only determined on aerosols and rainwater samples (au)

  2. Widespread pollution of the South American atmosphere predates the industrial revolution by 240 years

    Science.gov (United States)

    Uglietti, Chiara; Gabrielli, Paolo; Cooke, Colin; Vallelonga, Paul; Thompson, Lonnie

    2015-04-01

    In the Southern Hemisphere, evidence for preindustrial atmospheric pollution is restricted to a few geological archives of low temporal resolution that record trace element deposition originating from past mining and metallurgical operations in South America. Therefore the timing and the spatial impact of these activities on the past atmosphere remain poorly constrained. Here we present an annually resolved ice-core record (793-1989 AD) from the high altitude drilling site of Quelccaya (Peru) that archives preindustrial and industrial variations in trace elements. During the pre-colonial period (i.e., pre-1532 AD), the deposition of trace elements was mainly dominated by the fallout of aeolian dust and of ash from occasional volcanic eruptions indicating that metallurgic production during the Inca Empire (1438-1532 AD) had a negligible impact on the South American atmosphere. In contrast, a widespread anthropogenic signal is evident after 1540 AD, which corresponds with the beginning of colonial mining and metallurgy in Peru and Bolivia, 240 years prior to the Industrial Revolution. This shift was due to a major technological transition for silver extraction in South America (1572 AD), from lead-based smelting to mercury amalgamation, which precipitated a massive increase in mining activities. However, deposition of toxic trace metals during the Colonial era was still several factors lower than 20th century pollution that was unprecedented over the entirety of human history.

  3. Widespread pollution of the South American atmosphere predates the industrial revolution by 240 y.

    Science.gov (United States)

    Uglietti, Chiara; Gabrielli, Paolo; Cooke, Colin A; Vallelonga, Paul; Thompson, Lonnie G

    2015-02-24

    In the Southern Hemisphere, evidence for preindustrial atmospheric pollution is restricted to a few geological archives of low temporal resolution that record trace element deposition originating from past mining and metallurgical operations in South America. Therefore, the timing and the spatial impact of these activities on the past atmosphere remain poorly constrained. Here we present an annually resolved ice core record (A.D. 793-1989) from the high-altitude drilling site of Quelccaya (Peru) that archives preindustrial and industrial variations in trace elements. During the precolonial period (i.e., pre-A.D. 1532), the deposition of trace elements was mainly dominated by the fallout of aeolian dust and of ash from occasional volcanic eruptions, indicating that metallurgic production during the Inca Empire (A.D. 1438-1532) had a negligible impact on the South American atmosphere. In contrast, a widespread anthropogenic signal is evident after around A.D. 1540, which corresponds with the beginning of colonial mining and metallurgy in Peru and Bolivia, ∼240 y before the Industrial Revolution. This shift was due to a major technological transition for silver extraction in South America (A.D. 1572), from lead-based smelting to mercury amalgamation, which precipitated a massive increase in mining activities. However, deposition of toxic trace metals during the Colonial era was still several factors lower than 20th century pollution that was unprecedented over the entirety of human history.

  4. Use of hydraulic and aerial mock up to study atmospheric pollution

    International Nuclear Information System (INIS)

    Facy, L.; Perrin De Brichambaut, C.; Doury, A.; Le Quinio, R.

    1962-01-01

    Fundamental studies on turbulent atmospheric diffusion of finely divided particles, cannot remain on a purely theoretical basis. Further experimental studies must be considered. - In full scale, from accidental and induced releases. - On a reduced scale, in aerodynamic wind tunnels or hydraulic water tunnels. A first set of studies on reduced scale models has been worked out according to a contract between French 'Meteorologie Nationale' and French 'Commissariat a l'Energie Atomique' and with the Collaboration of Saint-Cyr 'Institut Aerotechnique'. Essentially two kinds of results have been obtained: - The mathematical model of SUTTON for the turbulent diffusion in the atmosphere, deduced from the SUTTON theory, generally used by us, has been correctly verified, qualitatively and quantitatively whenever experiments were consistent with the theory conditions. - The quantitative assays of photographic and cinematographic visualization have given precise details on the phenomena inaccessible to calculations, due to the influence of obstacles and release conditions. - Generally, it can be asserted, that the atmospheric pollution studies are worked out by mock up experimentations and that, in some cases these experiments never can be replaced by mathematically pure models. (authors) [fr

  5. [Pollution Evaluation and Risk Assessment of Heavy Metals from Atmospheric Deposition in the Parks of Nanjing].

    Science.gov (United States)

    Wang, Cheng; Qian, Xin; Li, Hui-ming; Sun, Yi-xuan; Wang, Jin-hua

    2016-05-15

    Contents of heavy metals involving As, Cd, Cr, Cu, Ni, Pb and Zn from atmospheric deposition in 10 parks of Nanjing were analyzed. The pollution level, ecological risk and health risk were evaluated using Geoaccumulation Index, Potential Ecological Risk Index and the US EPA Health Risk Assessment Model, respectively. The results showed that the pollution levels of heavy metals in Swallow Rock Park, Swallow Rock Park and Mochou Lake Park were higher than the others. Compared to other cities such as Changchun, Wuhan and Beijing, the contents of heavy metals in atmospheric deposition of parks in Nanjing were higher. The evaluation results of Geoaccumulation Index showed that Pb was at moderate pollution level, Zn and Cu were between moderate and serious levels, while Cd was between serious and extreme levels. The ecological risk level of Cd was high. The assessment results of Health Risk Assessment Model indicated that there was no non-carcinogenic risk for all the seven heavy metals. For carcinogenic risk, the risks of Cd, Cr and Ni were all negligible (Risk < 1 x 10⁻⁶), whereas As had carcinogenic risk possibility but was considered to be acceptable (10⁻⁶ < Risk < 10⁻⁴).

  6. Trentepohlia algae biofilms as bioindicator of atmospheric metal pollution.

    Science.gov (United States)

    García-Florentino, Cristina; Maguregui, Maite; Morillas, Héctor; Marcaida, Iker; Salcedo, Isabel; Madariaga, Juan Manuel

    2018-06-01

    In this work, a reddish biocolonization composed mainly by Trentepohlia algae affecting a synthetic building material from a modern building from the 90s located in the Bizkaia Science and Technology Park (Zamudio, North of Spain) was characterized and its ability to accumulate metals coming from the surrounding atmosphere was evaluated. To asses if these biofilms can act as bioindicators of the surrounding metal pollution, a fast non-invasive in situ methodology based on the use of hand-held energy dispersive X-ray fluorescence (HH-ED-XRF) was used. In order to corroborate the in situ obtained conclusions, some fragments from the affected material were taken to analyze the metal distribution by means of micro-energy dispersive X-ray fluorescence spectroscopy (μ-ED-XRF) and to confirm the presence of metal particles deposited on it using Scanning Electron Microscopy coupled to an Energy Dispersive Spectrometer (SEM-EDS). In order to confirm if Trentepohlia algae biofilms growing on the surface of building materials could be a fast way to in situ provide information about the surrounding metal pollution, a second Trentepohlia algae biofilm growing on a different kind of material (sandstone) was analyzed from an older historical building, La Galea Fortress (Getxo, North of Spain). Copyright © 2018. Published by Elsevier B.V.

  7. Outdoor air Pollution

    CSIR Research Space (South Africa)

    Forbes, PBC

    2016-07-01

    Full Text Available This chapter focuses on the air pollutants which are generally found in the troposphere and does not provide detail on specific areas where atmospheric pollutants and atmospheric chemistry may differ from that generally found, such as in the arctic...

  8. Effects of ascorbate feeding on chlorophyll fluorescence and xanthophyll cycle components in the lichen Parmelia quercina (Willd.) Vainio exposed to atmospheric pollutants

    Energy Technology Data Exchange (ETDEWEB)

    Calatayud, A.; Deltoro, V.I.; Barreno, E. [Univ. de Valencia, Inst. `Cavanilles` de Biodiversitat y Biologia Evolutiva, Burjassot (Spain); Abadia, A. [Estacion Experimental Aula Dei, CSIC, Dept. of Plant Nutrition, Zaragoza (Spain)

    1999-08-01

    The effects of environmental stresses on photosynthetic responses, ascorbate levels and pigment composition were investigated in samples of Parmelia quercina (Willd.) Vainio from control and polluted regions of the northern Castellon area (Valencia, Spain). In response to sustained pollutant stress in the field, lichen thalli has closed PSII traps and exhibited lower rates of electron transport and non-radiative energy dissipation. The xanthophyll concentration was not affected by exposure to atmospheric pollutants. The ascorbate concentration was lower in samples exposed to ambient air pollutants compared to control thalli. Ascorbate feeding of thalli from polluted sites stimulated electron flow, photochemical quenching and non-raditive energy dissipation. Additionally, ascorbate feeding enhances the de-epoxidation state of the xanthophyll pool in polluted thalli. The partial recovery for non-radiative energy dissipation was presumabley due to the interaction between the increased thylakoid pH gradient and de-epoxidized xanthophylls. Furhtermore, ascorbate feeding descreased photon excess in thalli from polluted sites owing to the stimulation of linear electron flow and non-radiative energy dissipation. The present study suggests that atmospheric pollutants besides their intrinsic toxicity, put on an additional burden by hampering the operation of photoprotective mechanisms. (au)

  9. A chemometric approach to the evaluation of atmospheric and fluvial pollutant inputs in aquatic systems: The Guadalquivir River estuary as a case study

    International Nuclear Information System (INIS)

    Lopez-Lopez, Jose A.; Garcia-Vargas, Manuel; Moreno, Carlos

    2011-01-01

    To establish the quality of waters it is necessary to identify both point and non-point pollution sources. In this work, we propose the combination of clean analytical methodologies and chemometric tools to study discrete and diffuse pollution caused in a river by tributaries and precipitations, respectively. During a two-year period, water samples were taken in the Guadalquivir river (selected as a case study) and its main tributaries before and after precipitations. Samples were characterized by analysing nutrients, pH, dissolved oxygen, total and volatile suspended solids, carbon species, and heavy metals. Results were used to estimate fluvial and atmospheric inputs and as tracers for anthropic activities. Multivariate analysis was used to estimate the background pollution, and to identify pollution inputs. Principal Component Analysis and Cluster Analysis were used as data exploratory tools, while box-whiskers plots and Linear Discriminant Analysis were used to analyse and distinguish the different types of water samples. - Highlights: → Atmospheric and fluvial inputs of pollutants in Guadalquivir River were identified. → Point (tributary rivers) and non-point sources (rains) were studied. → Nature and extension of anthropogenic pollution in the river were established. - By combining trace environmental analysis and selected chemometric tools atmospheric and fluvial inputs of pollutants in rivers may be identified. The extension of the pollution originated by each anthropic activity developed along the River may be established, as well as the identification of the pollution introduced into the river by the tributary rivers (point sources) and by rains (non-point sources).

  10. Effect of cadmium pollution of atmospheric origin on field-grown maize in two consecutive years with diverse weather conditions.

    Science.gov (United States)

    Anda, Angéla; Illés, Bernadett; Soós, G

    2013-12-01

    The aim of the study was to analyse the effect of atmospheric cadmium (Cd) pollution of atmospheric origin in maize compared to a control without Cd pollution. The plant parameters investigated were the timing of phenological phases, leaf area index (LAI) and yield, while radiation and water regime parameters were represented by albedo (reflection grade) and evapotranspiration, respectively. In treatments with and without irrigation, Cd caused a significant reduction in LAI, accompanied by lower evapotranspiration. The mean annual albedo in the Cd-polluted treatment only rose to a moderate extent in 2011 (in 2010 there was hardly any change), but changes within the year were more pronounced in certain phases of development. Cd led to greater reflection of radiation by plants during the vegetative phase, so the radiation absorption of the canopy was reduced leading to a lower level of evapotranspiration. In the dry, hot year of 2011 maize plants in the non-irrigated treatments showed a substantial reduction in grain dry matter, but maize yield losses could be reduced by irrigation in areas exposed to Cd pollution.

  11. Improving the use of lichens as biomonitors of atmospheric metal pollution

    International Nuclear Information System (INIS)

    Branquinho, C.; Catarino, F.; Brown, D.H.

    2000-01-01

    Improving the use of lichens as biomonitors of atmospheric metal pollution is the main objective of this work. For that a better insight into the availability and location of heavy metals in lichens subjected to polluted conditions both under laboratory and field conditions was attained. The data in this work supported the hypothesis that the absence of the lichen Ramalina fastigiata near a copper mine site, located in the south of Portugal, was related with toxic levels of Cu-dust near the centre of the mine. Lichen biodiversity, measured by the parameter number of lichen species, reflected the impact of the copper-mine dust emissions. The extent of the impact was more widespread towards cast, which appears to be correlated with the frequency of the winds. The chemical analysis of in-situ samples of R. fastigiata collected at different distances and in different directions from the mine showed that Cu, K and Mg were emitted from the centre of the mine site, confirming that major sources of atmospheric dust were located there. Total inhibition of PSII (photosystem II) photochemical reactions occurred in R. fastigiata both under field and controlled conditions, when intracellular Cu concentrations exceeded a threshold of ca. 2.0 μmol g -1 . No samples of this species were found under field conditions beyond the Cu threshold, suggesting that the absence of the lichen R. fastigiata might be used as an indicator of intracellular Cu concentrations above 2.0 μmol g -1 in the surroundings of the copper-mine. The fluorescence parameter F v /F m proved to be a good estimator of the survival capacity of R. fastigiata under field conditions and thus a useful parameter in determining the sensitivity of the lichens (photobiont) to Cu pollution. The intracellular location of Cu, K and Mg allowed to explain the physiological changes and the survival of the species in the surroundings of the copper-mine. (author)

  12. Some aspects of the effect of atmospheric pollution on the lichen flora to the west of Consett Co. , Durham

    Energy Technology Data Exchange (ETDEWEB)

    Griffith, J L

    1966-01-01

    The effect of atmospheric pollution on the growth of lichens has long been discussed. This work was aimed at obtaining data on the effect of such pollution, from the Iron and Steel works at Consett Co. Durham, on the lichen flora of the district. The degree of pollution found to the west of Consett was evaluated by analysis of lichen thallus for sulfur and from bark washings for amounts of deposited matter. These results were compared with standard pollution data at Consett, obtained from the DSIR, and a pollution gradient passing west from Consett was plotted. The distribution of corticolous, saxicolous and terricolous lichens in this area was mapped. The results from these distributions were applied to the pollution data and the control of lichens by pollution shown. The modification of the pollution effect by humidity factors is also discussed.

  13. Atmospheric ions and pollution

    International Nuclear Information System (INIS)

    Renoux, A.

    1977-01-01

    The various types of atmospheric ions are defined, the main sources of natural atmospheric radioactivity inducing the formation of radioactive ions in the air are then recalled. The basic equations governing the formation of these ions are indicated and the most current experimental methods used for detecting them are described (Zeleny tubes, Erikson tubes). The special properties of these ions are examined, they are particularly emphasized for the smaller ones. The existence of a discret spectrum of mobilities is shown and the presence of big negative radioactive ions is investigated. Indicative information are given on the granulometric distribution of the atmospheric radioactivity in the air, from small positive Ra A ion fixation on aerosols [fr

  14. Evaluating the suitability of different environmental samples for tracing atmospheric pollution in industrial areas.

    Science.gov (United States)

    Francová, Anna; Chrastný, Vladislav; Šillerová, Hana; Vítková, Martina; Kocourková, Jana; Komárek, Michael

    2017-01-01

    Samples of lichens, snow and particulate matter (PM 10 , 24 h) are used for the source identification of air pollution in the heavily industrialized region of Ostrava, Upper Silesia, Czech Republic. An integrated approach that uses different environmental samples for metal concentration and Pb isotope analyses was applied. The broad range of isotope ratios in the samples indicates a combination of different pollution sources, the strongest among them being the metallurgical industry, bituminous coal combustion and traffic. Snow samples are proven as the most relevant indicator for tracing metal(loid)s and recent local contamination in the atmosphere. Lichens can be successfully used as tracers of the long-term activity of local and remote sources of contamination. The combination of PM 10 with snow can provide very useful information for evaluation of current pollution sources. Copyright © 2016 Elsevier Ltd. All rights reserved.

  15. Deposition and retention of air pollutants on vegetation and other atmospheric interfaces

    International Nuclear Information System (INIS)

    Jonas, R.

    1984-09-01

    The question of the deposition of aerosols and gases are applied to biological and ecological problems concerning the filtering aspect of atmospheric interfaces, especially vegetation, with respect to air pollution, and also the resulting pollutant effect. In order to determine the deposition of aerosols, numerous field experiments were carried out. The deposition of gases was treated on the basis of current literature data. The experiments indicate that the deposition of aerosols on grass largely depends on aerosol diameter, dry weight per unit area and the wind velocity or turbulence of the air layer near the ground. Of the interfaces studied, namely soil without vegetation, water, filter paper, smooth and structured metals, grass, clover and trees, the latter had the greatest dust collecting capability. It is recommended that in the afforestation of areas in the close proximity of industrial regions the common beech, silver birch and Japanese larch should be taken into particular consideration due to their great deposition effectiveness with respect to dusts and their comparatively high resistance to pollutant gases. Silver birch and moreover red horse chestnut should be considered for filtering the air in urban regions because of the high aerosol deposition. (orig./HP) [de

  16. The linear accumulation of atmospheric mercury by vegetable and grass leaves: Potential biomonitors for atmospheric mercury pollution.

    Science.gov (United States)

    Niu, Zhenchuan; Zhang, Xiaoshan; Wang, Sen; Ci, Zhijia; Kong, Xiangrui; Wang, Zhangwei

    2013-09-01

    One question in the use of plants as biomonitors for atmospheric mercury (Hg) is to confirm the linear relationships of Hg concentrations between air and leaves. To explore the origin of Hg in the vegetable and grass leaves, open top chambers (OTCs) experiment was conducted to study the relationships of Hg concentrations between air and leaves of lettuce (Lactuca sativa L.), radish (Raphanus sativus L.), alfalfa (Medicago sativa L.) and ryegrass (Lolium perenne L.). The influence of Hg in soil on Hg accumulation in leaves was studied simultaneously by soil Hg-enriched experiment. Hg concentrations in grass and vegetable leaves and roots were measured in both experiments. Results from OTCs experiment showed that Hg concentrations in leaves of the four species were significantly positively correlated with those in air during the growth time (p  0.05). Thus, Hg in grass leaves is mainly originated from the atmosphere, and grass leaves are more suitable as potential biomonitors for atmospheric Hg pollution. The effect detection limits (EDLs) for the leaves of alfalfa and ryegrass were 15.1 and 22.2 ng g(-1), respectively, and the biological detection limit (BDL) for alfalfa and ryegrass was 3.4 ng m(-3).

  17. Modelling atmospheric transport of persistent organic pollutants in the Northern Hemisphere with a 3-D dynamical model: DEHM-POP

    OpenAIRE

    Hansen , K. M.; Christensen , J. H.; Brandt , J.; Frohn , L. M.; Geels , C.

    2004-01-01

    International audience; The Danish Eulerian Hemispheric Model (DEHM) is a 3-D dynamical atmospheric transport model originally developed to describe the atmospheric transport of sulphur into the Arctic. A new version of the model, DEHM-POP, developed to study the atmospheric transport and environmental fate of persistent organic pollutants (POPs) is presented. During environmental cycling, POPs can be deposited and re-emitted several times before reaching a final destination. A description of...

  18. Variational approach to direct and inverse problems of atmospheric pollution studies

    Science.gov (United States)

    Penenko, Vladimir; Tsvetova, Elena; Penenko, Alexey

    2016-04-01

    We present the development of a variational approach for solving interrelated problems of atmospheric hydrodynamics and chemistry concerning air pollution transport and transformations. The proposed approach allows us to carry out complex studies of different-scale physical and chemical processes using the methods of direct and inverse modeling [1-3]. We formulate the problems of risk/vulnerability and uncertainty assessment, sensitivity studies, variational data assimilation procedures [4], etc. A computational technology of constructing consistent mathematical models and methods of their numerical implementation is based on the variational principle in the weak constraint formulation specifically designed to account for uncertainties in models and observations. Algorithms for direct and inverse modeling are designed with the use of global and local adjoint problems. Implementing the idea of adjoint integrating factors provides unconditionally monotone and stable discrete-analytic approximations for convection-diffusion-reaction problems [5,6]. The general framework is applied to the direct and inverse problems for the models of transport and transformation of pollutants in Siberian and Arctic regions. The work has been partially supported by the RFBR grant 14-01-00125 and RAS Presidium Program I.33P. References: 1. V. Penenko, A.Baklanov, E. Tsvetova and A. Mahura . Direct and inverse problems in a variational concept of environmental modeling //Pure and Applied Geoph.(2012) v.169: 447-465. 2. V. V. Penenko, E. A. Tsvetova, and A. V. Penenko Development of variational approach for direct and inverse problems of atmospheric hydrodynamics and chemistry, Izvestiya, Atmospheric and Oceanic Physics, 2015, Vol. 51, No. 3, p. 311-319, DOI: 10.1134/S0001433815030093. 3. V.V. Penenko, E.A. Tsvetova, A.V. Penenko. Methods based on the joint use of models and observational data in the framework of variational approach to forecasting weather and atmospheric composition

  19. Indices of atmospheric purity and fluoride pollution pattern in Arvida, Quebec

    Energy Technology Data Exchange (ETDEWEB)

    LeBlanc, F; Rao, D N; Comeau, G

    1972-01-01

    Indices of atmospheric purity (IAP) of 42 sites located in all directions from the aluminum factory at Arvida and spread out in about 250-km/sup 2/ area, were determined on the basis of phytosociology of epiphytes of Populus balsamifera. These index values ranging from 0 to 103 were arranged into six groups and the investigated area was accordingly delineated into six IAP zones to represent areas with different levels of fluoride pollution. A relative picture of the approximate limits of fluoride contamination in different zones is obtained by the fluoride accumulation in Parmelia sulcata thalli transplanted at various sites in the area.

  20. The estimation of areas of ground that may be contaminated after an accidental release of pollutant to the atmosphere

    International Nuclear Information System (INIS)

    Corbett, J.O.

    1979-01-01

    A method is developed for calculating the area of ground contaminated above a prescribed level after an accidental release of radioactivity or any other pollutant to the atmosphere. Numerical calculations are made for a wide range of releases, atmospheric conditions and rates of wet and dry deposition. It is shown that high atmospheric stability and rain both tend to maximize the area of significant contamination for most of the plausible range of releases. However, for very large hypothetical releases, dry conditions with an unstable atmosphere spread significant contamination furthest afield. (author)

  1. [Development and current status of atmospheric pollution].

    Science.gov (United States)

    Elichegaray, C; Bouallala, S; Maitre, A; Ba, M

    2009-02-01

    Air quality is a public health issue and this article includes a reminder of the related causes and issues and a description of the monitoring of ambient air quality in France. It also provides a review of major developments in recent years of the pollutants measured. Emissions of major air pollutants have declined significantly since the 1970s, and this is reflected in an overall improvement in the quality of ambient air. Nevertheless, various forms of air pollution remain a concern (in the case of photochemical pollution) and health data show that air pollution is still a cause of morbidity and mortality. The fight against air pollution must remain a priority and requires multi-pollutant and multi-effect approaches. The National Health and Environment Program adopted during the Grenelle environment stakeholder consultation processes includes targets for reducing human exposure to air pollution, especially particulate matter, as well as measures to improve indoor air quality. In a context dominated by the struggle against the emission of greenhouse gases, problems of air quality should not be underestimated and policies relating to climate protection must be taken into account.

  2. Atmospheric stability and atmospheric circulation in Athens, Greece

    International Nuclear Information System (INIS)

    Synodinou, B.M.; Petrakis, M.; Kassomenos, P.; Lykoudis, S.

    1996-01-01

    In the evaluation and study of atmospheric pollution reference is always made to the stability criteria. These criteria, usually represented as functions of different meteorological data such as wind speed and direction, temperature, solar radiation, etc., play a very important role in the investigation of different parameters that affect the build up of pollution episodes mainly in urban areas. In this paper an attempt is made to evaluate the atmospheric stability criteria based on measurements obtained from two locations in and nearby Athens. The atmospheric stability is then examined along with the other meteorological parameters

  3. Evaluation of the pollution and human health risks posed by heavy metals in the atmospheric dust in Ebinur Basin in Northwest China.

    Science.gov (United States)

    Abuduwailil, Jilili; Zhaoyong, Zhang; Fengqing, Jiang

    2015-09-01

    Recently, a large amount of research assessing pollution levels and the related health risks posed by atmosphere dust has been undertaken worldwide. However, little work has been done in the oases of the arid regions of Northwest China. In this paper, we studied the pollution and health risks over a year of seven heavy metals in the atmospheric dust of Ebinur Basin, a typical oasis in Northwest China. The results showed the following: (1) The annual amount of atmospheric deposition in Ebinur Basin was 298.23 g m(-2) and the average monthly atmospheric deposition was 25.06 g m(-2). The average and maximum values of the seven heavy metals measured were all below the National Soil Environmental Quality Standards (2nd). (2) Heavy metals of Cu, Cr, and As in the atmospheric deposition mainly originated from the natural geological background, while Zn came from human activity. This study also showed that among the seven measured heavy metals, the ratios of the no-pollution status of Pb, Cd, and Hg were higher than those of others with moderate degrees of pollution also accounting for a certain ratio. (3) The carcinogenic risks from As, Cd, and Cr were all lower than the corresponding standard limit values, and these metals are considered not harmful to the health of the basin. However, there is a relatively high risk of exposure for children from hand-to-mouth intake, which is worthy of attention. This research showed that both human activity and natural factors, such as wind and altitude, influenced the heavy metal contents in the atmospheric dust of the study area. Furthermore, recent human activity in the study area had the most negative influence on the accumulation of the heavy metals and the corresponding health risks, especially for Hg, Pb, and Cd, which is worthy of attention.

  4. Pollutant Plume Dispersion in the Atmospheric Boundary Layer over Idealized Urban Roughness

    Science.gov (United States)

    Wong, Colman C. C.; Liu, Chun-Ho

    2013-05-01

    The Gaussian model of plume dispersion is commonly used for pollutant concentration estimates. However, its major parameters, dispersion coefficients, barely account for terrain configuration and surface roughness. Large-scale roughness elements (e.g. buildings in urban areas) can substantially modify the ground features together with the pollutant transport in the atmospheric boundary layer over urban roughness (also known as the urban boundary layer, UBL). This study is thus conceived to investigate how urban roughness affects the flow structure and vertical dispersion coefficient in the UBL. Large-eddy simulation (LES) is carried out to examine the plume dispersion from a ground-level pollutant (area) source over idealized street canyons for cross flows in neutral stratification. A range of building-height-to-street-width (aspect) ratios, covering the regimes of skimming flow, wake interference, and isolated roughness, is employed to control the surface roughness. Apart from the widely used aerodynamic resistance or roughness function, the friction factor is another suitable parameter that measures the drag imposed by urban roughness quantitatively. Previous results from laboratory experiments and mathematical modelling also support the aforementioned approach for both two- and three-dimensional roughness elements. Comparing the UBL plume behaviour, the LES results show that the pollutant dispersion strongly depends on the friction factor. Empirical studies reveal that the vertical dispersion coefficient increases with increasing friction factor in the skimming flow regime (lower resistance) but is more uniform in the regimes of wake interference and isolated roughness (higher resistance). Hence, it is proposed that the friction factor and flow regimes could be adopted concurrently for pollutant concentration estimate in the UBL over urban street canyons of different roughness.

  5. Characterization of the atmospheric pollution level in Sfax (Tunisia): influence of sources and meteorological factors; Caracterisation du niveau de pollution atmospherique dans la ville de Sfax (Tunisie): influence des sources et des facteurs meteorologiques

    Energy Technology Data Exchange (ETDEWEB)

    Azri, Ch.; Maalej, A.; Medhioub, K. [Ecole Nationale d' ingenieurs de Sfax, Unite de Recherche Etude et Gestion des Environnements Cotiers et Urbains (Tunisia); Tlili, A. [Faculte des Sciences de Sfax, Dept. de Geologie (Tunisia)

    2002-01-01

    This study held in Sfax City (Tunisia), showed that the atmospheric pollution level is strongly influenced by industrial sources, obstacles and meteorological factors. The factory of phosphate treatment 'SIAPE' displayed the main polluting source in the City. It is the principal issuing of SO{sub x} and toxic metals. The phosphogypsum deposit displayed an obstacle to the atmospheric diffusion of pollutants. Their stagnation is accentuated under smoky conditions. Several episodes of SO{sub 2} and dust are attributed to the effect of marked thermal inversions and the sirocco wind. The limited influence of traffic was proved by the registration of NO{sub x}, which showed low concentrations. It is conditioned by the change of fashion life of people and their customs of work (Ramadan month, agricultural activities). As a result, the adequate treatment of atmospheric industrial emanations (notably those of SIAPE) and the evacuation of artificial obstacles have to be considered. (authors)

  6. Measurement of radioactive aerosols as an original indicator of atmospheric pollution in urban areas

    International Nuclear Information System (INIS)

    Le Petit, G.; Millies-Lacroix, J. C.

    1998-01-01

    The Service Radioanalyses, Chimie et Environnment (Departement Analyses Surveillance de l'Environnement) of the French Atomic Energy Commission, located in suburban Paris, has for many years been conducting atmospheric radioactivity measurements. Since 1994, the laboratory has been using high volume air samplers equipped with filters for the weekly collection of atmospheric aerosols at a mean rate of about 600 m 3 .h -1 . The polypropylene filters, with a collection efficiency in excess of 93%, are compacted after sampling. The atmospheric radioactivity is measured by HP Ge gamma spectrometry after decay of short-lived natural relationship products. A study conducted in 1996 shows good correlation between the evolution with time of some of the indicators routinely used by AIRPARIF, the organization in charge of monitoring the air quality in the Ile-de-France region, to measure atmospheric pollution in the Paris area (SO 2 , NO) and that related to radioactivity of terrestrial ( 210 Pb, 40 K) and anthropogenic ( 137 Cs) origin, as well as the amount of aerosols collected. Further, the distribution in time of the atmospheric radioactivity of cosmogenic origin ( 7 Be) shows a yearly evolution somewhat similar to that observed with ozone

  7. Laser-excited fluorescence for measuring atmospheric pollution

    Science.gov (United States)

    Menzies, R. T.

    1975-01-01

    System measures amount of given pollutant at specific location. Infrared laser aimed at location has wavelength that will cause molecules of pollutant to fluoresce. Detector separates fluorescence from other radiation and measures its intensity to indicate concentration of pollutant.

  8. An effective chaos-geometric computational approach to analysis and prediction of evolutionary dynamics of the environmental systems: Atmospheric pollution dynamics

    Science.gov (United States)

    Buyadzhi, V. V.; Glushkov, A. V.; Khetselius, O. Yu; Bunyakova, Yu Ya; Florko, T. A.; Agayar, E. V.; Solyanikova, E. P.

    2017-10-01

    The present paper concerns the results of computational studying dynamics of the atmospheric pollutants (dioxide of nitrogen, sulphur etc) concentrations in an atmosphere of the industrial cities (Odessa) by using the dynamical systems and chaos theory methods. A chaotic behaviour in the nitrogen dioxide and sulphurous anhydride concentration time series at several sites of the Odessa city is numerically investigated. As usually, to reconstruct the corresponding attractor, the time delay and embedding dimension are needed. The former is determined by the methods of autocorrelation function and average mutual information, and the latter is calculated by means of a correlation dimension method and algorithm of false nearest neighbours. Further, the Lyapunov’s exponents spectrum, Kaplan-Yorke dimension and Kolmogorov entropy are computed. It has been found an existence of a low-D chaos in the time series of the atmospheric pollutants concentrations.

  9. The effect of nitrogen additions on bracken fern and its insect herbivores at sites with high and low atmospheric pollution

    Science.gov (United States)

    M.E. Jones; M.E. Fenn; T.D. Paine

    2011-01-01

    The impact of atmospheric pollution, including nitrogen deposition, on bracken fern herbivores has never been studied. Bracken fern is globally distributed and has a high potential to accumulate nitrogen in plant tissue. We examined the response of bracken fern and its herbivores to N fertilization at a high and low pollution site in forests downwind of Los Angeles,...

  10. A simple method employed for the treatment of filters used in atmospheric pollution studies

    International Nuclear Information System (INIS)

    Prendez B, M.M.; Ortiz C, J.L.; Garrido, J.I.; Huerta P, R.; Alvarez B, C.; Zolezzi C, S.R.

    1983-01-01

    A simple and rapid method for the multielement routine analysis of atmospheric particulate matter is described. The samples collected on four different types of filters were treated with HNO 3 and HCl at 110-120 deg C in pyrex glassware. Time required for the different stages of the treatment was determined by using 60 Co, 65 Zn and 137 Cs as radioactive tracers. Atomic absorption spectrophotometry was used to determine the concentration of the elements. The efficiency for 11 elements (Mg, Cr, Mn, Fe, Co, Ni, Cu, Zn, Cd, Hg and Pb) was determined. The method was succesfully employed for the treatment of filters used in atmospheric pollution studies in both urban and rural areas. (author)

  11. Calculation and analysis of environmental costs of the atmospheric pollution from brazilian oil refinery; Calculo e analise dos custos ambientais da poluicao atmosferica emitida por uma refinaria de petroleo brasileira

    Energy Technology Data Exchange (ETDEWEB)

    Mariano, Jacqueline [Universidade Federal do Rio de Janeiro (UFRJ), RJ (Brazil). Coordenacao dos Programas de Pos-graduacao de Engenharia (COPPE). Programa de Planejamento Energetico

    2004-07-01

    The present study presents a calculation of the environmental costs associated with the atmospheric pollution from a brazilian oil refinery and its analysis (the name of this oil refinery is confidential, for this reason it will not be mentioned). The calculation of the costs was based on a study of north-american researchers, about the environmental costs of five main atmospheric pollutants: particulate matter, sulphur oxides, nitrogen oxides, volatile organic compounds (VOC's) and carbon monoxide. The original American study offers an statistical analysis of several other American studies about environmental costs of atmospheric pollution, that present maximum, medium and minimum costs. Based on these values, the total environmental costs of the atmospheric pollution from the brazilian oil refinery were calculated, considering a fifty year operational time for the facility. The internalization of the atmospheric pollution environmental costs by the refiners is aligned with the world tendency of enforcement of the environmental limitations faced by the oil refining sector, and therefore, the adoption of a pro-active attitude is recommended by the present study. (author)

  12. NODC Standard Format Marine Toxic Substances and Pollutants (F144) Data (1971-1989) (NODC Accession 0014199)

    Data.gov (United States)

    National Oceanic and Atmospheric Administration, Department of Commerce — This data type contains data on ambient concentrations of toxic substances and other pollutants in the marine environment. The data derive from laboratory analyses...

  13. DEVELOPMENT OF MATHEMATICAL MEANS FOR ESTIMATION OF ECOLOGICAL AND ECONOMICAL LOSSES FROM POLLUTION OF ATMOSPHERIC AIR IN ZONES OF TECHNOGENIC OBJECTS IMPACT

    Directory of Open Access Journals (Sweden)

    O. POPOV

    2015-10-01

    Full Text Available The article describes the solution of one of the most important problems of rational use of natural resources. Modern mathematical tools for damage estimation, which are caused by atmospheric pollution to natural objects, and also methods for calculation of the cost for their renewal were developed. The solution of problem was divided into 3 stages. At the first stage it was defined basic anthropogenic sources of pollution, was illustrated conceptual behavior of pollutants in the atmosphere emitted by technological stationary point source. Choice of mathematical model that allows to determine the distribution of pollutants concentration in the air in zones of pollution by point stationary sources in the short-term discharges was proved. At the second stage it was developed mathematical tools to determine the level of objects damage, which were in the zone of pollution, depending on the intensity and duration of exposure of technogenic sources. At the third stage it was developed mathematical models to determine the recoverable amount of natural objects depending on their level of damage. Model example of developed means usage was described. Advantages of developed means over existed analogs were noticed.

  14. Using an epiphytic moss to identify previously unknown sources of atmospheric cadmium pollution.

    Science.gov (United States)

    Donovan, Geoffrey H; Jovan, Sarah E; Gatziolis, Demetrios; Burstyn, Igor; Michael, Yvonne L; Amacher, Michael C; Monleon, Vicente J

    2016-07-15

    Urban networks of air-quality monitors are often too widely spaced to identify sources of air pollutants, especially if they do not disperse far from emission sources. The objectives of this study were to test the use of moss bio-indicators to develop a fine-scale map of atmospherically-derived cadmium and to identify the sources of cadmium in a complex urban setting. We collected 346 samples of the moss Orthotrichum lyellii from deciduous trees in December, 2013 using a modified randomized grid-based sampling strategy across Portland, Oregon. We estimated a spatial linear model of moss cadmium levels and predicted cadmium on a 50m grid across the city. Cadmium levels in moss were positively correlated with proximity to two stained-glass manufacturers, proximity to the Oregon-Washington border, and percent industrial land in a 500m buffer, and negatively correlated with percent residential land in a 500m buffer. The maps showed very high concentrations of cadmium around the two stained-glass manufacturers, neither of which were known to environmental regulators as cadmium emitters. In addition, in response to our findings, the Oregon Department of Environmental Quality placed an instrumental monitor 120m from the larger stained-glass manufacturer in October, 2015. The monthly average atmospheric cadmium concentration was 29.4ng/m(3), which is 49 times higher than Oregon's benchmark of 0.6ng/m(3), and high enough to pose a health risk from even short-term exposure. Both stained-glass manufacturers voluntarily stopped using cadmium after the monitoring results were made public, and the monthly average cadmium levels precipitously dropped to 1.1ng/m(3) for stained-glass manufacturer #1 and 0.67ng/m(3) for stained-glass manufacturer #2. Published by Elsevier B.V.

  15. Macro impact of the law on prevention and control of atmospheric pollution on power industry development

    Energy Technology Data Exchange (ETDEWEB)

    Wang, Z. [State Power Corporation (China). Dept. of Science, Technology and Environment

    2001-07-01

    The newly revised and enlarged main contents of China's Law of Prevention and Control of Atmospheric Pollution, which came into force on 1 September 2000, are described. The macro impacts of the law on the power industry development are analyzed mainly in respect to power demand and readjustment of power structure and layout, clean production and pollution control level, scientific management of environmental protection, in accordance with law as well as changes of construction and operation costs. Several questions worthy to be noted in course of implementation of the new law are enumerated. 1 tab.

  16. Formulating a problem for functions of the effect in models of atmospheric pollution with parametric consideration of diffusion in the near earth layer

    Energy Technology Data Exchange (ETDEWEB)

    Ganev, K; Yordanov, D

    1983-01-01

    The formulation of a diffusion problem for numerical models, in which the near earth layer of the atmosphere (PSA) is considered parametrically relative to the zones of pollution (the protected zones) which are also located in the near earth layer of atmosphere, is examined. In modeling atmospheric pollution, the semiempirical equation of turublent diffusion is the starting point. The results are cited of numerical calculations of the functions of the effect for the city of Sofia (the case of an even relief and the disposition of the protected zone totally within the region for which the problem is being solved). The isolines of the integral function of the effect relative to the near earth layer of the atmosphere above the city of Sofia are cited for different meteorological conditions.

  17. Air Pollution.

    Science.gov (United States)

    Barker, K.; And Others

    Pollution of the general environment, which exposes an entire population group for an indeterminate period of time, certainly constitutes a problem in public health. Serious aid pollution episodes have resulted in increased mortality and a possible relationship between chronic exposure to a polluted atmosphere and certain diseases has been…

  18. Interaction of atmospheric pollutants

    Energy Technology Data Exchange (ETDEWEB)

    Bustueva, K A; Sanotsky, I V

    1975-01-01

    In evaluating the health effects of chemical and physical factors, it is of great importance to know the possible interactions between different pollutants. The biological effects of interactions, when present, may be synergistic, antagonistic or additive. Each type of interaction calls for a different evaluation and different practical measures. As yet the understanding of such effects is not clear, probably because of differing definitions of terminology. For example, the combined effect of sulfur dioxide and particulates is interpreted as a synergistic effect; in the author's opinion, this is an aggravating effect. The type of interaction depends on the levels of concentration observed, for example, the synergism shown at high levels of concentration is not always demonstrated for low levels of concentration. In fact there is little evidence of synergistic effects from ambient air pollutant; the more common type of interaction is additive in effect. 12 references.

  19. Historical reconstruction of mercury pollution across the Tibetan Plateau using lake sediments.

    Science.gov (United States)

    Yang, Handong; Battarbee, Richard W; Turner, Simon D; Rose, Neil L; Derwent, Richard G; Wu, Guangjian; Yang, Ruiqiang

    2010-04-15

    The Tibetan Plateau is described as the "Roof of the World" averaging over 4000 m above sea level; it is remote, isolated, and presumed to be a pristine region. In order to study the history of atmospheric mercury (Hg) pollution and its spatial variation across the Plateau, lakes were chosen from three areas forming a north to south transect. Sediment cores were taken from three sites in each area and dated using the radionuclides 210Pb and 137Cs. Analysis of the cores yielded the first comprehensive Hg reconstructions for the Plateau, showing clear Hg pollution at all sites. The first indication of Hg pollution is much earlier than the onset of the industrial revolution in Europe, but the most significant pollution increase is from the 1970s, followed by a further marked increase from the 1990s. The mean post-2000 atmospheric pollution Hg accumulation rates for the sampling sites were estimated at between 5.1 and 7.9 microg m(-2) yr(-1). The increase in Hg pollution over the last few decades is synchronous with the recent economic development in Asia (especially China and India), and pollution Hg levels continue to increase. Furthermore, contemporary sediment Hg accumulation rate data are in broad agreement with Hg deposition values derived from global models that attribute pollution to sources mainly within southeast Asia. As most of the sites are exceptionally remote and situated above the atmospheric boundary layer, these results underline the need to understand the local Hg cycle in both regional and global context.

  20. Studies of the long-range transport of atmospheric pollutant using nuclear-related analytical techniques. Appendix 7

    International Nuclear Information System (INIS)

    Yang Shaojin

    1995-01-01

    Atmospheric aerosol and rainwater samples collected in the different Western Pacific areas were analyzed by instrumental neutron activation and proton induced x-ray emission to (1) determine the atmospheric concentrations of trace elements over the Western Pacific and (2) to estimate the atmospheric deposition of trace elements and dust-soil material to this region. High abundance of pollutant and crustal elements relative to oceanic sources was observed. Some characteristics of marine atmosphere relating to long-range transport of crustal and anthropogenic elements from continent to the remote ocean are discussed. The total dust-soil particle mass is estimated to be 0.066-1.2 μg/m 3 over the Western Pacific Ocean areas. Atmospheric inputs of dust-soil particles control the marine particle concentrations of crustal elements. A total of 99 atmospheric samples with the 'Gent' filter unit were collected during October 1993 and September 1994 at a western suburb of Beijing, China (40 deg. N,116 deg. E), and completed the analysis of these filters by both INAA and PIXE. (author)

  1. Atmospheric pollution with copper around the copper mine and flotation, 'Buchim', Republic of Macedonia, using biomonitoring moss and lichen technique

    International Nuclear Information System (INIS)

    Balabanova, Biljana; Bacheva, Katerina; Shajn, Robert; Stafilov, Trajche

    2009-01-01

    This paper has studied the atmospheric pollution with copper due to copper mining and flotation 'Buchim' near Radovish, Republic of Macedonia. The copper ore and ore tailings continually are exposed to open air, which occur winds carry out the fine particles in to atmosphere. Moss (Hyloconium splendens and Pleurozium schrebery) and lichen (Hypogymnia physodes and Parmelia sulcata) samples were used for biomonitoring the possible atmospheric pollution with copper in the mine vicinity. Moss and lichen samples were digested by using of microwave digestion system and copper was analyzed by atomic emission spectrometry with inductively coupled plasma (ICPAES). The obtained values for the content of copper in moss and lichen samples were statistically processed using the nonparametric and parametric analysis. Maps of areal deposition of copper show an increase content of copper in the vicinity of mine, but long distance distribution of this element is not established yet.

  2. CFD modelling for atmospheric pollutants/aerosols studies within the complex terrains of urban areas and industrial sites

    Czech Academy of Sciences Publication Activity Database

    Střižík, Michal; Zelinger, Zdeněk; Nevrlý, V.; Kubát, Pavel; Berger, P.; Černý, A.; Engst, P.; Bitala, P.; Janečková, Radmila; Grigorová, Eva; Bestová, I.; Čadil, J.; Danihelka, P.; Kadeřábek, P.; Kozubková, M.; Drábková, S.; Hartman, D.; Bojko, M.; Zavila, O.

    2014-01-01

    Roč. 54, č. 1 (2014), s. 73-90 ISSN 0957-4352 R&D Projects: GA MŠk LD12020 Institutional support: RVO:61388955 Keywords : Air pollution * Atmospheric movements * Computational fluid dynamics Subject RIV: CF - Physical ; Theoretical Chemistry Impact factor: 0.433, year: 2014

  3. Development of mathematical techniques for the assimilation of remote sensing data into atmospheric models

    International Nuclear Information System (INIS)

    Seinfeld, J.H.

    1982-01-01

    The problem of the assimilation of remote sensing data into mathematical models of atmospheric pollutant species was investigated. The data assimilation problem is posed in terms of the matching of spatially integrated species burden measurements to the predicted three-dimensional concentration fields from atmospheric diffusion models. General conditions were derived for the reconstructability of atmospheric concentration distributions from data typical of remote sensing applications, and a computational algorithm (filter) for the processing of remote sensing data was developed

  4. Development of mathematical techniques for the assimilation of remote sensing data into atmospheric models

    International Nuclear Information System (INIS)

    Seinfeld, J.H.

    1982-01-01

    The problem of the assimilation of remote sensing data into mathematical models of atmospheric pollutant species was investigated. The problem is posed in terms of the matching of spatially integrated species burden measurements to the predicted three dimensional concentration fields from atmospheric diffusion models. General conditions are derived for the reconstructability of atmospheric concentration distributions from data typical of remote sensing applications, and a computational algorithm (filter) for the processing of remote sensing data is developed

  5. The spatial-temporal distribution of the atmospheric polluting agents during the period 2000-2005 in the Urban Area of Guadalajara, Jalisco, Mexico.

    Science.gov (United States)

    Sánchez, Hermes U Ramírez; García, María D Andrade; Bejaran, Rubén; Guadalupe, Mario E García; Vázquez, Antonio Wallo; Toledano, Ana C Pompa; Villasenor, Odila de la Torre

    2009-06-15

    In the large cities, the disordered urban development, the industrial activities, and the transport, have caused elevated concentrations of polluting agents and possible risks to the health of the population. The metropolises located in valleys with little ventilation (such as the Urban Area of Guadalajara: UAG) present low dispersion of polluting agents can cause high risk of respiratory and cardiovascular diseases. The objective of this work was to describe the spatial-temporal distribution of the atmospheric polluting agents: carbon monoxide (CO), nitrogen dioxide (NO(2)), sulfur dioxide (SO(2)), particles smaller than 10 microns (microm) (PM(10)) and ozone (O(3)) in the UAG during the period 2000-2005. A spatial-temporal distribution analysis was made by means of graphic interpolation (Kriging method) of the statistical parameters of CO, NO(2), SO(2), PM(10) and O(3) with the collected data from eight stations of atmospheric monitoring in the UAG. The results show that the distributions of the atmospheric polluting agents are variable during the analyzed years. The polluting agent with highest concentration is PM(10) (265.42 microg/m(3)), followed by O(3) (0.11 ppm), NO(2) (0.11 ppm), CO (9.17 ppm) and SO(2) (0.05 ppm). The most affected zone is the southeast of the UAG. The results showed that an important percentage of days exceed the Mexican norms of air quality (93-199 days/year).

  6. Regulations Concerning Agriculture and Air Pollution

    Directory of Open Access Journals (Sweden)

    Chiara Bertora

    2010-03-01

    Full Text Available The main issues related to the atmospheric pollution are the stratospheric ozone depletion, the transboundary air pollution, the troposphere air quality and the climate change. The three last decades have seen the birth of several measures for the atmosphere safeguard. Agricultural activities play a key role in determining, preventing and mitigating atmospheric pollution. The emission to atmosphere of different ozone-depleting substances is regulated by the Montreal Protocol. The role of agriculture activity in ozone depletion is linked to the utilization of methyl bromide as soil sterilant and to the emission of nitrogen oxides and nitrous oxide, from agricultural soils. The Convention on long-range transboundary air pollution regulates the emission of several pollutants, i.e. sulphur dioxide, nitrogen oxides, ammonia, non methane volatile organic compounds, carbon monoxide, heavy metals, persistent organic pollutants, and tropospheric ozone. The agriculture sector is responsible for a large part of the emissions of ammonia and nitrogen oxides, mainly through manure management and nitrogen fertilization, and of most persistent organic pollutants, largely used in the past as insecticides and fungicides. The increase of the greenhouse gases (GHGs concentration in the atmosphere is under the control of the Kyoto Protocol. Agriculture accounts for 59-63% of global non-CO2 GHGs emissions but at the same time it contributes to the atmospheric CO2 concentration stabilisation through the substitution of fossil fuels by biofuels and the sequestration of C in soil and vegetal biomass. In this paper we provide an outline of the numerous scientific and legislative initiatives aimed at protecting the atmosphere, and we analyse in detail the agriculture sector in order to highlight both its contribution to atmospheric pollution and the actions aimed at preventing and mitigating it.

  7. Measurements and modelling of atmospheric pollution over the Paris area: an overview of the ESQUIF Project

    Directory of Open Access Journals (Sweden)

    L. Menut

    2000-11-01

    Full Text Available The "Étude et Simulation de la QUalité de l'air en Ile de France" (ESQUIF project is the first integrated project dedicated to the study of the processes leading to air pollution events over the Paris area. The project was carried out over two years (summer 1998 to winter 2000 to document all types of meteorological conditions favourable to air quality degradation, and in particular to photo oxydant formation. The goals of ESQUIF are (1 to improve our understanding of the relevant chemical and dynamical processes and, in turn, improve their parametrizations in numerical models, and (2 to improve and validate existing models dedicated to pollution analysis, scenarios and/or forecasting, by establishing a comprehensive and thorough database. We present the rationale of the ESQUIF project and we describe the experimental set-up. We also report on the first experiments which took place during the summer of 1998 involving surface networks, and remote sensing instruments as well as several aircraft. Focusing on three days of August 1998, the relative contributions of long-range transported and locally-produced ozone to the elevated ozone concentrations observed during this period are discussed and chemistry-transport model preliminary results on this period are compared to measurements.Key words: Atmospheric composition and structure (pollution – urban and regional; troposphere – composition and chemistry – Meteorology and atmospheric dynamics (mesoscale meteorology

  8. Reconstruction of atmospheric trace metals pollution in Southwest China using sediments from a large and deep alpine lake: Historical trends, sources and sediment focusing.

    Science.gov (United States)

    Lin, Qi; Liu, Enfeng; Zhang, Enlou; Nath, Bibhash; Shen, Ji; Yuan, Hezhong; Wang, Rong

    2018-02-01

    Atmospheric pollution, one of the leading environmental problems in South and East Asia, and its impact on the terrestrial environmental quality remain poorly understood particularly in alpine areas where both historical and present-day mining and smelting operations might leave an imprint. Here, we reconstructed atmospheric trace metals pollution during the past century using core sediments from a large and deep alpine lake in Southwest China. The implication of in lake and/or in watershed sediment focusing in pollution quantification is discussed by analyzing 15 sediment cores. Factor analysis and enrichment factor indicated Cd, Pb and Sb as the typical pollutants. Distinct peaks of Pb and Sb pollution were observed around the 1920s, but little Pb pollution was detected in recent decades, different from other studies in similar regions. Cadmium pollution was observed until the mid-1980s synchronized with Sb. The distinctive variations in atmospheric trace metal pollution process in Southwest China highlight the regional and sub-regional sources of metal pollutants, which should be primarily attributed to non-ferrous metal smelting emissions. Both natural and anthropogenic metals showed wide concentration ranges though exhibited similar temporal trends in the 15 cores. Spatial variations of anthropogenic metals were influenced by the in-watershed pollutants remobilization, whereas, natural metals were regulated by the detrital materials in the sub-basin. In-lake sediment focusing had little influence on the spatial distributions of all metals, different from the traditional sediment focusing pattern observed in small lakes. Anthropogenic Cd accumulation in sediments ranged from 1.5 to 10.1mgm -2 in a specific core with an average of 6.5mgm -2 for the entire lake, highlighting that a reliable whole-lake pollutant budget requires an analysis of multiple cores. Our study suggests that the management of aquatic ecosystem health should take the remobilization of in

  9. [Prolonged exposure to atmospheric air pollution and mortality from respiratory causes].

    Science.gov (United States)

    Eilstein, D

    2009-12-01

    Different designs can be used to analyze the relationships between respiratory mortality and long term exposure to atmospheric pollution: epidemiological studies (cohort, prevalence study) demonstrate the reality of the relationship and toxicological studies explain it. Cohort studies have the advantage of being able to take into account many confounding factors and thus avoid biases (which is not the case with prevalence studies), but require significant human and financial resources. They were first adopted in the US, but are now more often applied in Europe. The results are relatively consistent, as they all show a statistically significant association between an increase in particulate pollution and cardiopulmonary mortality. Mortality from lung cancer is also associated with long term exposition to particles and sometimes to ozone or nitrogen oxides. Cerebrovascular diseases and sudden death of young children have also been associated with particulate pollution. The relationships are more powerful for long term than short term exposure but are also linear and without threshold. In order to explain these effects (today the causality of the relationship is certain) there are many possible factors, particularly regarding particulate exposures: an increase in cardiovascular risk biomarkers (fibrinogen, white blood cells, and platelets), atherosclerosis, chronic inflammation of lung tissues increased by acute exposure, etc. More and more studies address the interaction between gene and environment and even epigenetic phenomena which could be responsible of these effects. Public Health impact could be quantified. The European E&H surveillance program Apheis, for example, estimated that if PM2.5 levels remained below 15 microg/m(3), a 30 year old person could see his life expectancy increased by 1 month to 2 years, depending on the studied city. Finally, mortality is not the only relevant indicator for health effects of air pollution. ISAAC studies address asthma

  10. Measurement of radioactive aerosols as an original indicator of atmospheric pollution in urban areas

    International Nuclear Information System (INIS)

    Le Petit, G.; Millies-Lacroix, J.-C.; Simon, F.

    1998-01-01

    The Service Radioanalyses, Chimie et Environnement (Departement Analyses Surveillance de l'Environnement) of the French Atomic Energy Commission, located in suburban Paris, has for many years been conducting atmospheric radioactivity measurements. Since 1994, the laboratory has been using high volume air samplers equipped with filters for the weekly collection of atmospheric aerosols at a mean rate of about 600 m 3 .h -1 . The polypropylene filters, with a collection efficiency in excess of 93%, are compacted after sampling. The atmospheric radioactivity is measured by HP Ge gamma spectrometry after decay of short-lived natural relationship products. A study conducted in 1996 shows good correlation between the evolution with time of some of the indicators routinely used by AIRPARIF, the organization in charge of monitoring of the air quality in the Ile-de-France region, to measure atmospheric pollution in the Paris area (SO 2 , NO) and that related to radioactivity of terrestrial ( 210 Pb, 40 K) and anthropogenic ( 137 Cs) origin, as well as the amount of aerosols collected. Further, the distribution in time of the atmospheric radioactivity of cosmogenic origin ( 7 Be) shows a yearly evolution somewhat similar to that observed with ozone. (author). 16 refs., 21 figs., 1 tab

  11. Methodological approach in determination of small spatial units in a highly complex terrain in atmospheric pollution research: the case of Zasavje region in Slovenia.

    Science.gov (United States)

    Kukec, Andreja; Boznar, Marija Z; Mlakar, Primoz; Grasic, Bostjan; Herakovic, Andrej; Zadnik, Vesna; Zaletel-Kragelj, Lijana; Farkas, Jerneja; Erzen, Ivan

    2014-05-01

    The study of atmospheric air pollution research in complex terrains is challenged by the lack of appropriate methodology supporting the analysis of the spatial relationship between phenomena affected by a multitude of factors. The key is optimal design of a meaningful approach based on small spatial units of observation. The Zasavje region, Slovenia, was chosen as study area with the main objective to investigate in practice the role of such units in a test environment. The process consisted of three steps: modelling of pollution in the atmosphere with dispersion models, transfer of the results to geographical information system software, and then moving on to final determination of the function of small spatial units. A methodology capable of designing useful units for atmospheric air pollution research in highly complex terrains was created, and the results were deemed useful in offering starting points for further research in the field of geospatial health.

  12. Characteristics of atmospheric visibility and its relationship with air pollution in Korea.

    Science.gov (United States)

    Lee, Jeong-Young; Jo, Wan-Kuen; Chun, Ho-Hwan

    2014-09-01

    Although analysis of long-term data is necessary to obtain reliable information on characteristics of atmospheric visibility and its relationship with air pollution, it has rarely been performed. Therefore, a long-term evaluation of atmospheric visibility in characteristically different Korean cities, as well as a remote island, during 2001 to 2009, was performed in this study. In general, visibility decreased in the studied areas during the 9-yr study period. In addition, all areas displayed a distinct seasonal trend, with high visibility in the cold season relative to the warm season. Weekday visibility, however, did not significantly differ from weekend visibility. Similarly, the number of days per year for both low (19 km) fluctuated during the study period. Busan (a coastal city) exhibited the highest visibility, with an overall average of 17.6 km, followed by Daegu (a basin city), Ulsan (with concentrated petrochemical industries), Ullungdo (a remote island), and Seoul (the capital of Korea). Visibility was found to be significantly correlated with target air pollutants, except for ozone, for all metropolitan cities, whereas it was significantly correlated only with particulate matter with an aerodynamic diameter <10 μm (PM10) and ozone on the remote island (Ullungdo). Among the metropolitan cities, Seoul exhibited the lowest visibility for both the PM10 standard exceedance and non-exceedance days, followed by Ulsan, Daegu, and Busan. The results of this study can be used to establish effective strategies for improving urban visibility and air quality. Copyright © by the American Society of Agronomy, Crop Science Society of America, and Soil Science Society of America, Inc.

  13. The chemical composition of red giants in 47 Tucanae. II. Magnesium isotopes and pollution scenarios

    Science.gov (United States)

    Thygesen, A. O.; Sbordone, L.; Ludwig, H.-G.; Ventura, P.; Yong, D.; Collet, R.; Christlieb, N.; Melendez, J.; Zaggia, S.

    2016-04-01

    Context. The phenomenon of multiple populations in globular clusters is still far from understood, with several proposed mechanisms to explain the observed behaviour. The study of elemental and isotopic abundance patterns are crucial for investigating the differences among candidate pollution mechanisms. Aims: We derive magnesium isotopic ratios for 13 stars in the globular cluster 47 Tucanae (NGC 104) to provide new, detailed information about the nucleosynthesis that has occurred within the cluster. For the first time, the impact of 3D model stellar atmospheres on the derived Mg isotopic ratios is investigated. Methods: Using both tailored 1D atmospheric models and 3D hydrodynamical models, we derive magnesium isotopic ratios from four features of MgH near 5135 Å in 13 giants near the tip of the red giant branch, using high signal-to-noise, high-resolution spectra. Results: We derive the magnesium isotopic ratios for all stars and find no significant offset of the isotopic distribution between the pristine and the polluted populations. Furthermore, we do not detect any statistically significant differences in the spread in the Mg isotopes in either population. No trends were found between the Mg isotopes and [Al/Fe]. The inclusion of 3D atmospheres has a significant impact on the derived 25Mg/24Mg ratio, increasing it by a factor of up to 2.5, compared to 1D. The 26Mg/24Mg ratio, on the other hand, essentially remains unchanged. Conclusions: We confirm the results seen from other globular clusters, where no strong variation in the isotopic ratios is observed between stellar populations, for observed ranges in [Al/Fe]. We see no evidence for any significant activation of the Mg-Al burning chain. The use of 3D atmospheres causes an increase of a factor of up to 2.5 in the fraction of 25Mg, resolving part of the discrepancy between the observed isotopic fraction and the predictions from pollution models. Based on observations made with the ESO Very Large Telescope

  14. Using sensitivity derivatives for design and parameter estimation in an atmospheric plasma discharge simulation

    International Nuclear Information System (INIS)

    Lange, Kyle J.; Anderson, W. Kyle

    2010-01-01

    The problem of applying sensitivity analysis to a one-dimensional atmospheric radio frequency plasma discharge simulation is considered. A fluid simulation is used to model an atmospheric pressure radio frequency helium discharge with a small nitrogen impurity. Sensitivity derivatives are computed for the peak electron density with respect to physical inputs to the simulation. These derivatives are verified using several different methods to compute sensitivity derivatives. It is then demonstrated how sensitivity derivatives can be used within a design cycle to change these physical inputs so as to increase the peak electron density. It is also shown how sensitivity analysis can be used in conjunction with experimental data to obtain better estimates for rate and transport parameters. Finally, it is described how sensitivity analysis could be used to compute an upper bound on the uncertainty for results from a simulation.

  15. Use of the indicator activation method in studies of the propagation of pollutants in the atmosphere

    International Nuclear Information System (INIS)

    Alps, W.; Kuehn, W.

    1979-01-01

    The pollution of the atmosphere near ground level with various noxal substances, originating in industrial irradiation centres and in connection with the generation of nuclear power, has recently prompted detailed investigations of the propagation of aerosols, taking into account the roughness of the terrain and the vegetation. For this purpose pyrotechnic aerosols have been developed, labelled with an easily activated element, which can be released at any point in the atmosphere in the form of pulsed, linear or paint sources for propagation investigations. The paper reports on experiments over terrain with various types of natural vegetation. (orig.) [de

  16. Lowest-order average effect of turbulence on atmospheric profiles derived from radio occultation

    International Nuclear Information System (INIS)

    Eshleman, V.R.; Haugstad, B.S.

    1977-01-01

    Turbulence in planetary atmospheres and ionospheres causes changes in angles of refraction of radio waves used in occultation experiments. Atmospheric temperature and pressure profiles, and ionospheric electron concentration profiles, derived from radio occultation measurements of Doppler frequency contain errors due to such angular offsets. The lowest-order average errors are derived from a geometrical-optics treatment of the radio-wave phase advance caused by the addition of uniform turbulence to an initially homogeneous medium. It is concluded that the average profile errors are small and that precise Doppler frequency measurements at two or more wavelengths could be used to help determine characteristics of the turbulence, as well as accuracy limits and possible correction terms for the profiles. However, a more detailed study of both frequency and intensity characteristics in radio and optical occultation measurements of turbulent planetary atmospheres and ionospheres is required to realize the full potential of such measurements

  17. Air pollution

    International Nuclear Information System (INIS)

    Nelson, P.

    2000-01-01

    Australian cites experience a number of current and emerging air pollution problems. Concentrations of traditional primary pollutants such as CO, lead and dust have fallen in recent years as a consequence of air pollutant control measures, and the widespread introduction of lead-free petrol. However, recommended guidelines for ozone, the principal component of photochemical smog, are regularly exceeded in major capital cities in the summer months. In addition, it is predicted that extensive urban expansion will lead to much greater dependence on the motor vehicle as the primary means of transportation. Effects of air pollution are felt at a variety of scales. Traditionally, concerns about gaseous and particulate emissions from industrial and vehicular sources were focused on local impacts due to exposure to toxic species such as CO and lead. As noted above, concentrations of these pollutants have been reduced by a variety of control measures. Pollutants which have effects at a regional scale, such as photochemically-produced ozone, and acidic gases and particles have proved more difficult to reduce. In general, these pollutants arc not the result of direct emissions to atmosphere, but result from complex secondary processes driven by photochemical reactions of species such as NO 2 and aldehydes. In addition, global effects of gaseous and particulate emissions to the atmosphere have received significant recent attention, concentrations of atmospheric CO 2 with predicted impacts on global climate, and ozone depletion due to anthropogenic emissions of chlorine-containing chemicals are the two major examples. Combustion processes from petrol- and diesel-fuelled vehicles, make major contributions to air pollution, and the magnitude of this contribution is discussed in this article

  18. Atmospheric pollution and the prevalence of asthma: study among schoolchildren of 2 areas in Rio de Janeiro, Brazil.

    Science.gov (United States)

    Rios, José Luiz Magalhães; Boechat, José Laerte; Sant'Anna, Clemax Couto; França, Alfeu Tavares

    2004-06-01

    Air pollutants have been associated with the exacerbation of respiratory diseases. They may intensify the inflammatory allergic response and airways reactivity to inhaled allergens. However, it is still not clear if air pollution contributes to the increased prevalence of asthma. To investigate if different levels of air pollution exposure can be related to differences in the prevalence of asthma. The International Study of Asthma and Allergies in Childhood (ISAAC) protocol was used to determine and compare the prevalence of asthma among schoolchildren in 2 cities of the metropolitan region of Rio de Janeiro, Brazil, Duque de Caxias (DC) and Seropédica (SR), which have different levels of atmospheric pollution. The research involved 4,064 students aged 13 to 14 years from 49 schools in DC and 1,129 from 17 schools in SR. Air pollution was evaluated by the concentration of inhalable particulate matter (PM10). ISAAC's written questionnaire was answered by 4,040 students aged 13 to 14 years in DC and 1,080 in SR. Between 1998 and 2000, the PM10 annual arithmetic mean was 124 microg/m3 in DC and 35 microg/m3 in SR (acceptable level is up to 50 microg/m3). The prevalence of wheezing ever was 35.1% in DC and 29.9% in SR (P = .001), and the prevalence of wheezing in the last 12 months was 19.0% in DC and 15.0% in SR (P = .002). In DC, 14.5% of the adolescents presented 1 to 3 crises of wheezing in the last year, whereas in SR only 11.0% presented 1 to 3 crises (P = .003). In this study, the prevalence of asthma in adolescents was directly related to atmospheric pollution.

  19. Atmospheric pollution biomonitoring of the Sao Paulo metropolitan region using epiphytic lichens

    International Nuclear Information System (INIS)

    Fuga, Alessandra

    2006-01-01

    Due to the increasing problems of atmospheric pollution in the Sao Paulo metropolitan region that affect the environment and human health the application of biomonitoring methodologies using cosmopolite organisms has now become relevant. Biomonitoring is a method to evaluate the response of live organisms to pollution. This method offers advantages such as reduced costs, efficient monitoring of large geographic areas and accumulated pollutants over a large period in which low concentrations of chemicals elements in the environment can be evaluated. In the present study, neutron activation analysis method was applied to determine elements accumulated in Canoparmelia texana lichenized fungi. Samples were collected in two distinct areas: Carlos Botelho (PECB) and Intervales (PEI) State Parks that are considered as non-polluted areas and that belong to the Atlantic Forest - SP ecosystem; and Sao Paulo city metropolitan region in sites near automatic monitoring stations of the Environmental Protection Agency of the State of Sao Paulo (CETESB). The lichens collected from the bark of the trees were properly treated, and irradiated with neutrons from IEA-R1 nuclear reactor along with synthetic standards of elements. The precision and the accuracy of the results were evaluated by the analyses of IAEA-336 LICHEN and Mixed Polish Herbs (INCT -MPH-2) certified reference materials. The results obtained for these materials were in accordance with the certified values and presented good precision with variation coefficients ranging from 0.9 to 14.6%. Results obtained for lichens showed that elements As, Co, Cr, Cs, La, Mo, Sb, Sc, Se and U are present at ng g -1 levels, Ba, Br, Cl, Fe, K, Mn, Na, Rb and Zn at μg g -1 and Ca at mg g -1 . By applying cluster and discriminant analyses to the results for the lichen samples from areas with different levels of pollution, the sampling sites were grouped according to their chemical similarities and their elemental composition. It was

  20. L'IIASA and the integrated simulation of the trans-border atmospheric pollution assessment and evaluation; L'IIASA et la modelisation integree de la pollution atmospherique transfrontiere. Bilan et evaluation

    Energy Technology Data Exchange (ETDEWEB)

    Soleille, S.; Brignon, J.M.; Farret, R.; Landrieu, G.; Le Gall, A.C.; Rouil, L

    2003-09-15

    The RAINS model is an integrated evaluation model for many pollutants and many effects, developed by he IIASA. This model studies the emissions of 4 atmospheric pollutants (nitrogen oxides, sulfur oxides, ammonium and volatile organic compounds) and the necessary costs to reduce them and the dispersion of these pollutants and their effects (tropospheric ozone formation, acidification and eutrophication). The model can be used in activities scenario mode (energy, agriculture, transports...) to calculate the emissions and their effects or in optimization mode to calculate strategies of emissions control from environmental constraints. (A.L.B.)

  1. Air pollution problem in the Mexico City metropolitan zone: Photochemical pollution

    Energy Technology Data Exchange (ETDEWEB)

    Alvarez, H.B.; Alvarez, P.S.; Echeverria, R.S.; Jardon, R.T. [Centro de Ciencias de la Atmosfera (Mexico). Seccion de Contaminacion Ambiental

    1997-12-31

    Mexico City Metropolitan Zone (MCMZ) represents an example of a megacity where the air pollution problem has reached an important evolution in a very short time, causing a risk in the health of a population of more than 20 million inhabitants. The atmospheric pollution problem in the MCMZ, began several decades ago, but it increased drastically in the middle of the 80`s. It is important to recognize that in the 60`s, 70`s and the first half of the 80`s the main pollutants were sulfur dioxide and total suspended particles. However since the second half of the 80`s until now, ozone is the most important air pollutant besides of the suspended particles (PM{sub 10}) and other toxic pollutants (1--8). The purpose of this paper is to discuss the evolution of the ozone atmospheric pollution problem in the MCMZ, as well as to analyze the results of several implemented air pollution control strategies.

  2. Historical reconstruction of atmospheric lead pollution in central Yunnan province, southwest China: an analysis based on lacustrine sedimentary records.

    Science.gov (United States)

    Liu, Enfeng; Zhang, Enlou; Li, Kai; Nath, Bibhash; Li, Yanling; Shen, Ji

    2013-12-01

    Atmospheric lead (Pb) pollution during the last century in central Yunnan province, one of the largest non-ferrous metal production centers in China, was reconstructed using sediment cores collected from Fuxian and Qingshui Lakes. Lead concentrations and isotopic ratios ((207)Pb/(206)Pb and (208)Pb/(206)Pb) were measured in sediment cores from both lakes. The operationally defined chemical fractions of Pb in sediment core from Fuxian Lake were determined by the optimized BCR procedure. The chronology of the cores was reconstructed using (210)Pb and (137)Cs dating methods. Similar three-phase variations in isotopic ratios and enrichment factors of Pb were observed in the sediment cores from both lakes. Before the 1950s, the sediment data showed low (207)Pb/(206)Pb and (208)Pb/(206)Pb ratios and enrichment factors (EFs=~1), indicating that the sedimentary Pb was predominantly of lithogenic origin. However, these indices were increased gradually between the 1950s and the mid-1980s, implying an atmospheric Pb deposition. The EFs and isotopic ratios of Pb reached their peak during recent years, indicating aggravating atmospheric Pb pollution. The average anthropogenic Pb fluxes since the mid-1980s were estimated to be 0.032 and 0.053 g m(-2) year(-1) recorded in Fuxian and Qingshui cores, respectively. The anthropogenic Pb was primarily concentrated in the reducible fraction. Combining the results of Pb isotopic compositions and chemical speciations in the sediment cores and in potential sources, we deduced that recent aggravating atmospheric Pb pollution in central Yunnan province should primarily be attributed to regional emissions from non-ferrous metal production industries.

  3. The IPAC-NC field campaign: a pollution and oxidization pool in the lower atmosphere over Huabei, China

    Directory of Open Access Journals (Sweden)

    J. Z. Ma

    2012-05-01

    Full Text Available In the past decades, regional air pollution characterized by photochemical smog and grey haze-fog has become a severe environmental problem in China. To investigate this, a field measurement campaign was performed in the Huabei region, located between 32–42° N latitude in eastern China, during the period 2 April–16 May 2006 as part of the project "Influence of Pollution on Aerosols and Cloud Microphysics in North China" (IPAC-NC. It appeared that strong pollution emissions from urban and industrial centers tend to accumulate in the lower atmosphere over the central area of Huabei. We observed widespread, very high SO2 mixing ratios, about 20–40 ppbv at 0.5–1.5 km altitude and 10–30 ppbv at 1.5–3.0 km altitude. Average CO mixing ratios were 0.65–0.7 ppmv at 0.5–1.5 km altitude, and very high CO around 1 ppmv was observed during some flights, and even higher levels at the surface. We find the high pollution concentrations to be associated with enhanced levels of OH and HO2 radicals, calculated with a chemical box model constrained by the measurements. In the upper part of the boundary layer and in the lower free troposphere, high CO and SO2 compete with relatively less NO2 in reacting with OH, being efficiently recycled through HO2, preventing a net loss of HOx radicals. In addition to reactive hydrocarbons and CO, the oxidation of SO2 causes significant ozone production over Huabei (up to ~13% or 2.0 ppbv h−1 at 0.8 km altitude. Our results indicate that the lower atmosphere over Huabei is not only strongly polluted but also acts as an oxidation pool, with pollutants undergoing very active photochemistry over this part of China.

  4. [Characteristics of mercury pollution in soil and atmosphere in Songhua River upstream Jia-pi-gou gold mining area].

    Science.gov (United States)

    Zhang, Gang; Wang, Ning; Wang, Yuan; Liu, Te; Ai, Jian-Chao

    2012-09-01

    In the studied area of Jia-pi-gou at the upstream area of Songhua River, algamation process has been applied as a dominant method to extract gold for more than one hundred and eighty years, resulting in severe mercury environmental pollution. The total mercury contents in the atmosphere and soil have been determined by mercury analyzer (Zeeman RA915+) and cold atomic absorption spectrophotometry (GB/T 17136-1997), respectively. To study the pollution characteristics of mercury in the soil and atmosphere, the mercury flux at the interface between the soil and the atmosphere of 4 sampling sites Lao-jin-chang, Er-dao-gou, Er-dao-cha and community of Jia-pi-gou have been determined with the method of dynamic flux chamber. Furthermore, linear regression analyses on the total mercury contents between soil and atmosphere have been carried out and the correlation coefficient of mercury exchange flux between soil and atmosphere and meteorological factors has been studied. The results are as follows: (1) The mean value of mercury content in the atmosphere is (71.08 +/- 38.22) ng x m(-3). (2) The mean value of mercury content in the soil is (0.913 1 +/- 0.040 8) mg x kg(-1); it shows remarkably positive correlation between the mercury contents in soil and in the atmosphere. (3) The mercury exchange flux between soil and atmosphere in different locations are Lao-jin-chang [(129.13 +/- 496.07) ng (m2 x h)(-1)], Er-dao-gou [(98.64 +/- 43.96) ng x (m2 x h)(-1)], Er-dao-cha [(23.17 +/- 171.23) ng x (m2 x h)(-1)], and community of Jia-pi-gou [(7.12 +/- 46.33) ng x (m2 x h)(-1)]. (4) Solar radiation is the major influential factor in the mercury exchange flux between the soil and atmosphere in Lao-jin-chang, Er-dao-cha and community of Jia-pi-gou. Solar radiation, air temperature and soil temperature jointly influence the process of the mercury exchange flux between the soil and atmosphere in Er-dao-gou. Under the disturbance of terrain, three noticeably distinctive trend features

  5. PREDICTION OF ATMOSPHERIC AIR POLLUTION BY EMISSIONS OF MOTOR TRANSPORT TAKING INTO ACCOUNT THE CHEMICAL TRANSFORMATION OF HARMFUL SUBSTANCES

    Directory of Open Access Journals (Sweden)

    M. M. Biliaiev

    2017-06-01

    Full Text Available Purpose. Development of 3D numerical models, which allow us to calculate air pollution process from road transport emissions based on chemical transformation of pollutants. Creating numerical models, which would give the opportunity to predict the level of air pollution in urban areas. Methodology. To address the evaluation of the air pollution problem of emissions of vehicles the equations of aerodynamics and mass transfer were used. In order to solve differential equations of aerodynamics and mass transfer the finite difference methods are used. For the numerical integration of the equation for the velocity potential the method of conditional approximation was applied. The equation for the velocity potential written in difference form, is being split into two equations, and at each step of splitting the unknown value of the potential speed is determined by the explicit scheme of running account and the difference scheme itself is implicit. For the numerical integration of the equation of dispersion of emissions in the atmosphere is used implicit alternating-triangular difference splitting scheme. Emissions from the road are simulated by a series of point sources of a given intensity. The developed numerical models are the basis of established software package.Findings. There were developed 3D numerical models, which belong to the class «diagnostic models». These models take into account the main physical factors affecting the process of dispersion of pollutants in the atmosphere when emissions from road transport taking into account the chemical transformation of pollutants. On the basis of the constructed numerical models a computational experiment to assess the level of air pollution in the street was carried out. Originality. Numerical models that allow you to calculate the 3D aerodynamic of wind flow in urban areas and the process of mass transfer of emissions from the road were developed. The models make it possible to account the

  6. Identification of Heavy Metal Pollution Derived From Traffic in Roadside Soil Using Magnetic Susceptibility.

    Science.gov (United States)

    Yang, Pingguo; Ge, Jing; Yang, Miao

    2017-06-01

    The study integrates surface and vertical distribution of magnetic susceptibility and heavy metal contents (Pb, Cu, Zn and Fe) to characterize the signature of vehicle pollutants in roadside soils at Linfen city, China. Sites with reforestation and without vegetation cover were investigated. The results showed that magnetic susceptibility and heavy metal contents were higher at the roadside without trees than in the reforest belt. The variations of magnetic susceptibility and heavy metal contents decreased both with distance and with depth. The maximum value was observed at 5-10 m away from the roadside edge. The vertical distribution in soil revealed accumulation of pollutants in 0-5 cm topsoils. The average contents were higher than the background values and in the order Fe (107.21 g kg -1 ), Zn (99.72 mg kg -1 ), Pb (90.99 mg kg -1 ), Cu (36.14 mg kg -1 ). Coarse multi domain grains were identified as the dominating magnetic particles. Multivariate statistical and SEM/EDX analyses suggested that the heavy metals derived from traffic sources. Trees act as efficient receptors and green barrier, which can reduce vehicle derived pollution.

  7. Distribution of air pollutants in the Inn Valley atmosphere during high concentration events in winter 2006

    International Nuclear Information System (INIS)

    Schnitzhofer, R.; Norman, M; Dunkl, J.; Wistaler, A.; Hansel, A.; Neininger, B.; Gohm, A.

    2006-01-01

    Full text: The goal of the INNOX field campaign, which took place during January and February 2006 near the town of Schwaz, was to obtain a three-dimensional picture of the spatial distribution of air pollutants in the Inn Valley during wintertime. For this purpose continuous ground based measurements and, on six chosen days, vertical profiles within the lowest 200 m above ground level (AGL) of the valley atmosphere of certain VOCs (benzene, toluene, etc.) and CO were performed using a proton-transfer-reaction mass spectrometry instrument (PTR-MS). For the soundings a 200-m long teflon line was fixed on a tethered balloon through which the air was sucked to the PTR-MS instrument and to a CO analyser. Next to the inlet on the tethered balloon meteorological data, such as air temperature, pressure, wind, were measured as well. Above the lowest 200 m AGL a research aircraft from MetAir AG (Switzerland), equipped with various instruments for in-situ measurements of air pollutants and meteorological data, was operated. A typical flight pattern consisted of five vertical cross sections between about 150 to 2500 m AGL and lasted about three hours. Altogether 25 hours of aircraft measurements were carried out on six different days. The combination of low-level balloon measurements and upper-level aircraft observations yields vertical profiles of various parameters which cover the whole valley atmosphere. Preliminary results which show strong vertical but also horizontal gradients of air pollutant concentrations will be presented. (author)

  8. Measurements and modelling of atmospheric pollution over the Paris area: an overview of the ESQUIF Project

    Directory of Open Access Journals (Sweden)

    L. Menut

    Full Text Available The "Étude et Simulation de la QUalité de l'air en Ile de France" (ESQUIF project is the first integrated project dedicated to the study of the processes leading to air pollution events over the Paris area. The project was carried out over two years (summer 1998 to winter 2000 to document all types of meteorological conditions favourable to air quality degradation, and in particular to photo oxydant formation. The goals of ESQUIF are (1 to improve our understanding of the relevant chemical and dynamical processes and, in turn, improve their parametrizations in numerical models, and (2 to improve and validate existing models dedicated to pollution analysis, scenarios and/or forecasting, by establishing a comprehensive and thorough database. We present the rationale of the ESQUIF project and we describe the experimental set-up. We also report on the first experiments which took place during the summer of 1998 involving surface networks, and remote sensing instruments as well as several aircraft. Focusing on three days of August 1998, the relative contributions of long-range transported and locally-produced ozone to the elevated ozone concentrations observed during this period are discussed and chemistry-transport model preliminary results on this period are compared to measurements.

    Key words: Atmospheric composition and structure (pollution – urban and regional; troposphere – composition and chemistry – Meteorology and atmospheric dynamics (mesoscale meteorology

  9. An analytical model for radioactive pollutant release simulation in the atmospheric boundary layer

    International Nuclear Information System (INIS)

    Weymar, Guilherme J.; Vilhena, Marco T.; Bodmann, Bardo E.J.; Buske, Daniela; Quadros, Regis

    2013-01-01

    Simulations of emission of radioactive substances in the atmosphere from the Brazilian nuclear power plant Angra 1 are a necessary tool for control and elaboration of emergency plans as a preventive action for possible accidents. In the present work we present an analytical solution for radioactive pollutant dispersion in the atmosphere, solving the time-dependent three-dimensional advection-diffusion equation. The experiment here used as a reference in the simulations consisted of the controlled releases of radioactive tritiated water vapor from the meteorological tower close to the power plant at Itaorna Beach. The wind profile was determined using experimental meteorological data and the micrometeorological parameters were calculated from empirical equations obtained in the literature. We report on a novel analytical formulation for the concentration of products of a radioactive chain released in the atmospheric boundary layer and solve the set of coupled equations for each chain radionuclide by the GILTT solution, assuming the decay of all progenitors radionuclide for each equation as source term. Further we report on numerical simulations, as an explicit but fictitious example and consider three radionuclides in the radioactive chain of Uranium 235. (author)

  10. An analytical model for radioactive pollutant release simulation in the atmospheric boundary layer

    Energy Technology Data Exchange (ETDEWEB)

    Weymar, Guilherme J.; Vilhena, Marco T.; Bodmann, Bardo E.J., E-mail: guicefetrs@gmail.com, E-mail: mtmbvilhena@gmail.com, E-mail: bejbodmann@gmail.com [Universidade Federal do Rio Grande do Sul (UFRGS), Porto Alegre, RS (Brazil). Programa de Pos-Graduacao em Engenharia Mecanica; Buske, Daniela; Quadros, Regis, E-mail: danielabuske@gmail.com, E-mail: quadros99@gmail.com [Universidade Federal de Pelotas (UFPel), Capao do Leao, RS (Brazil). Programa de Pos-Graduacao em Modelagem Matematica

    2013-07-01

    Simulations of emission of radioactive substances in the atmosphere from the Brazilian nuclear power plant Angra 1 are a necessary tool for control and elaboration of emergency plans as a preventive action for possible accidents. In the present work we present an analytical solution for radioactive pollutant dispersion in the atmosphere, solving the time-dependent three-dimensional advection-diffusion equation. The experiment here used as a reference in the simulations consisted of the controlled releases of radioactive tritiated water vapor from the meteorological tower close to the power plant at Itaorna Beach. The wind profile was determined using experimental meteorological data and the micrometeorological parameters were calculated from empirical equations obtained in the literature. We report on a novel analytical formulation for the concentration of products of a radioactive chain released in the atmospheric boundary layer and solve the set of coupled equations for each chain radionuclide by the GILTT solution, assuming the decay of all progenitors radionuclide for each equation as source term. Further we report on numerical simulations, as an explicit but fictitious example and consider three radionuclides in the radioactive chain of Uranium 235. (author)

  11. Role of sectoral and multi-pollutant emission control strategies in improving atmospheric visibility in the Yangtze River Delta, China

    International Nuclear Information System (INIS)

    Huang, Kan; Fu, Joshua S.; Gao, Yang; Dong, Xinyi; Zhuang, Guoshun; Lin, Yanfen

    2014-01-01

    The Community Multi-scale Air Quality modeling system is used to investigate the response of atmospheric visibility to the emission reduction from different sectors (i.e. industries, traffic and power plants) in the Yangtze River Delta, China. Visibility improvement from exclusive reduction of NO x or VOC emission was most inefficient. Sulfate and organic aerosol would rebound if NO x emission was exclusively reduced from any emission sector. The most efficient way to improve the atmospheric visibility was proven to be the multi-pollutant control strategies. Simultaneous emission reductions (20–50%) on NO x , VOC and PM from the industrial and mobile sectors could result in 0.3–1.0 km visibility improvement. And the emission controls on both NO x (85%) and SO 2 (90%) from power plants gained the largest visibility improvement of up to 4.0 km among all the scenarios. The seasonal visibility improvement subject to emission controls was higher in summer while lower in the other seasons. -- Highlights: • Atmospheric visibility in the Yangtze River Delta is modeled and evaluated. • Responses of visibility changes to various emission reduction scenarios are compared. • Sulfate aerosol will increase if only NO x emission is reduced. • The multi-pollutant control strategy is most efficient for improving visibility. -- Responses of visibility changes to various emission reduction scenarios are compared. The multi-pollutant control strategy is most efficient for improving visibility in YRD, China

  12. Atmospheric pollution, eco-products, wastes management: some opinions and attitudes at the beginning of 2002; Pollution atmospherique, eco-produits, gestion des dechets: quelques opinions et attitudes au debut 2002

    Energy Technology Data Exchange (ETDEWEB)

    NONE

    2002-07-01

    This document presents the results (statistical data) to the questions asked by the ADEME in the inquiry of the CREDOC concerning the ''French way of life and aspirations'' and realized in the beginning of the year 2002. The questions dealt with the following five topics: the french attitude facing the atmospheric pollution; the renouncing of the vehicle during the days of high urban pollution; the French and the remote-working; the consumption and the environment control. (A.L.B.)

  13. Atmosphere physics and chemistry

    International Nuclear Information System (INIS)

    Delmas, R.; Megie, G.; Peuch, V.H.

    2005-10-01

    Since the 1970's, the awareness about the atmospheric pollution threat has led to a spectacular development of the researches on the complex interactions between the chemical composition of the atmosphere and the climate. This book makes a synthesis of the state-of-the-art in this very active domain of research. Content: introduction, atmosphere dynamics and transport, matter-radiation interaction and radiant transfer, physico-chemical processes, atmospheric aerosol and heterogenous chemistry, anthropic and natural emissions and deposition, stratospheric chemical system, tropospheric chemical system, polluted boundary layer, paleo-environments and ice archives, role of atmospheric chemistry in global changes, measurement principles and instruments, numerical modeling, experimental strategy, regulation and management of the atmospheric environment, index. (J.S.)

  14. Critical levels and loads of atmospheric pollutants for terrestrial and aquatic ecosystems. The emergence of a scientific concept. Application potentials and their limits

    International Nuclear Information System (INIS)

    Landmann, G.

    1993-01-01

    The 'critical loads and levels' are defined as the highest atmospheric deposition rate or concentration of a gaseous pollutant, respectively, that will not cause harmful effects on sensitive elements of an ecosystem. The recent emergence of the concept of critical loads and levels is described, from the first explicit mention in 1986 to the production of the first European maps in 1991. The difficulties linked to the definition of the concept and to its english-derived terminology are discussed. The main approaches used for assessing critical loads and levels are briefly described. Important research is developed under the auspices of the Convention of Geneva (Long Range Transboundary Air Pollution Transport, UN-ECE), arising from intensive studies which have been carried out on the effects of air pollution on terrestrial and aquatic ecosystems for the past ten or fifteen years. Current knowledge is summarized, as well as the remaining gaps (and questions) which hinder the calculation of the critical thresholds. Finally, beyond the fundamental relevance of this scientifically sound and easily understood concept, its limits are pointed out. In brief, the 'critical loads and levels' concept is attractive and motivating to many scientists: it implies to apply an integrated and finalized approach, favors the prospecting of poorly known ecosystems and regions, and represents an interesting interface with decision makers

  15. Biomonitoring of the atmospheric pollution using lichens in the metropolitan area of Sao Paulo city, Brazil

    International Nuclear Information System (INIS)

    Saiki, M.; Fuga, A.; Alves, E.R.; Vasconcellos, M.B.A.; Marcelli, M.P.

    2007-01-01

    The atmospheric pollution of Sao Paulo city is a serious problem due to the expansion of industrial area, increasing number of vehicles and population density. This work presents results obtained in the analysis of lichens collected in different sites of Sao Paulo city and in non-polluted areas of Atlantic Forest. Concentrations of twenty elements were determined in Canoparmelia texanaspecies and comparisons were made between the results obtained in lichens from different sites. High concentrations of the elements As, Ba, Cd, Co, Cr, Fe, La, Mn, Sb and Zn were found for samples collected in sites located near industries and petrochemical plant. Br and Sb concentrations were also high in lichens from sites affected by vehicular emissions. (author)

  16. The chemistry of the global atmosphere; International Symposium of the Commission for Atmospheric Chemistry and Global Pollution of IAMAP, 7th, Chamrousse, France, Sept. 5-11, 1990, Selected Papers

    Science.gov (United States)

    Buat-Menard, P. (Editor); Delmas, R. J. (Editor)

    1992-01-01

    Topics presented include the adsorption and reaction of trichlorofluoromethane on various particles, equilibria of the marine multiphase ammonia system, a novel ozone sensor for direct eddy flux measurements, and characterization of the carbonate content of atmospheric aerosols. Also presented are variations in heavy metals concentrations in Antarctic snows, sources of continental dust over Antarctica during the last glacial cycle, an inventory of anthropogenic emissions and air pollution in the USSR, and atmospheric nuclei in the remote free-troposphere.

  17. Study on atmosphere pollution by PIXE analysis combining with statistical method

    International Nuclear Information System (INIS)

    Zhu Guanghua

    1994-06-01

    Atmospheric aerosol samples were collected using an 8-stage cascade impactor or an automatic time sequence step sampler at Jomo Langma, Zhangye at the edge of Gobi Desert and Beijing. Element concentration were analyzed by PIXE (proton induced X-ray emission) technique. The data were analyzed by APCA (absolute principal component analysis) to determine the principal components. The sources and contribution to the aerosol in the above three regions were discussed. The result shows that the PIXE has high sensitivity, multi-element capability, high speed and non-destruction advantages. APCA analytical method can effectively determine the aerosol components in urban area, and it also can distinguish between local components and remote components in the area far from the pollution resources

  18. A combined MOIP-MCDA approach to building and screening atmospheric pollution control strategies in urban regions.

    Science.gov (United States)

    Mavrotas, George; Ziomas, Ioannis C; Diakouaki, Danae

    2006-07-01

    This article presents a methodological approach for the formulation of control strategies capable of reducing atmospheric pollution at the standards set by European legislation. The approach was implemented in the greater area of Thessaloniki and was part of a project aiming at the compliance with air quality standards in five major cities in Greece. The methodological approach comprises two stages: in the first stage, the availability of several measures contributing to a certain extent to reducing atmospheric pollution indicates a combinatorial problem and favors the use of Integer Programming. More specifically, Multiple Objective Integer Programming is used in order to generate alternative efficient combinations of the available policy measures on the basis of two conflicting objectives: public expenditure minimization and social acceptance maximization. In the second stage, these combinations of control measures (i.e., the control strategies) are then comparatively evaluated with respect to a wider set of criteria, using tools from Multiple Criteria Decision Analysis, namely, the well-known PROMETHEE method. The whole procedure is based on the active involvement of local and central authorities in order to incorporate their concerns and preferences, as well as to secure the adoption and implementation of the resulting solution.

  19. A Combined MOIP-MCDA Approach to Building and Screening Atmospheric Pollution Control Strategies in Urban Regions

    Science.gov (United States)

    Mavrotas, George; Ziomas, Ioannis C.; Diakouaki, Danae

    2006-07-01

    This article presents a methodological approach for the formulation of control strategies capable of reducing atmospheric pollution at the standards set by European legislation. The approach was implemented in the greater area of Thessaloniki and was part of a project aiming at the compliance with air quality standards in five major cities in Greece. The methodological approach comprises two stages: in the first stage, the availability of several measures contributing to a certain extent to reducing atmospheric pollution indicates a combinatorial problem and favors the use of Integer Programming. More specifically, Multiple Objective Integer Programming is used in order to generate alternative efficient combinations of the available policy measures on the basis of two conflicting objectives: public expenditure minimization and social acceptance maximization. In the second stage, these combinations of control measures (i.e., the control strategies) are then comparatively evaluated with respect to a wider set of criteria, using tools from Multiple Criteria Decision Analysis, namely, the well-known PROMETHEE method. The whole procedure is based on the active involvement of local and central authorities in order to incorporate their concerns and preferences, as well as to secure the adoption and implementation of the resulting solution.

  20. Western forests and air pollution

    International Nuclear Information System (INIS)

    Olson, R.K.; Binkley, D.; Boehm, M.

    1992-01-01

    The book addresses the relationships between air pollution in the western United States and trends in the growth and condition of Western coniferous forests. The major atmospheric pollutants to which forest in the region are exposed are sulfur and nitrogen compounds and ozone. The potential effects of atmospheric pollution on these forests include foliar injury, alteration of growth rates and patterns, soil acidification, shifts in species composition, and modification of the effects of natural stresses

  1. [Atmospheric pollution characteristic during fireworks burning time in spring festival in Quanzhou suburb].

    Science.gov (United States)

    Zhao, Jin-ping; Xu, Ya; Zhang, Fu-wang; Chen, Jin-sheng

    2011-05-01

    Atmospheric pollution characteristics during fireworks burning time in 2009 Spring Festival in Quangzhou suburb were studied. Particulate aerosol has been monitored and collected using real-time monitor and middle-volume sampler during fireworks burning time. The objectives of this study were to identify the contents and distributing characteristics of particles, polycyclic aromatic hydrocarbon (PAHs) and water-soluble ions and to discuss sources of these pollutants. The results showed that PM2.5 and PM10 were increased significantly during fireworks burning time. The highest concentration of particles presented time of 00:57-01:27 on New Year's Eve, which the average concentration of PM2.5 and PM10 were reached 1102.43 microm(-3) and 1610.22 microg x m(-3) in 30 min. The concentration of particle- and gas-PAHs were 54.18 ng x m(-1) and 47.10 ng x m(-3), respectively, during fireworks burning time in New Year's Eve, which were higher than that in the normal day. It can be judged by the diagnostic ratios that the primary source of PAHs in Quanzhou suburb were the combustion of coal, biomass and the exhaust emission from diesel vehicles in this region. Results of water-soluble ions indicated that fireworks burning were the main reason to lead to higher concentration of these ions during Spring Festival. Moreover, pollution gases of NOx and SO2 that were origined from fireworks burning, coal combustion and exhaust emission from motor vehicle were supplied precursors to form secondary pollutants, such as NO3- and SO4(2-).

  2. Forecasting human exposure to atmospheric pollutants in Portugal - A modelling approach

    Science.gov (United States)

    Borrego, C.; Sá, E.; Monteiro, A.; Ferreira, J.; Miranda, A. I.

    2009-12-01

    Air pollution has become one main environmental concern because of its known impact on human health. Aiming to inform the population about the air they are breathing, several air quality modelling systems have been developed and tested allowing the assessment and forecast of air pollution ambient levels in many countries. However, every day, an individual is exposed to different concentrations of atmospheric pollutants as he/she moves from and to different outdoor and indoor places (the so-called microenvironments). Therefore, a more efficient way to prevent the population from the health risks caused by air pollution should be based on exposure rather than air concentrations estimations. The objective of the present study is to develop a methodology to forecast the human exposure of the Portuguese population based on the air quality forecasting system available and validated for Portugal since 2005. Besides that, a long-term evaluation of human exposure estimates aims to be obtained using one-year of this forecasting system application. Additionally, a hypothetical 50% emission reduction scenario has been designed and studied as a contribution to study emission reduction strategies impact on human exposure. To estimate the population exposure the forecasting results of the air quality modelling system MM5-CHIMERE have been combined with the population spatial distribution over Portugal and their time-activity patterns, i.e. the fraction of the day time spent in specific indoor and outdoor places. The population characterization concerning age, work, type of occupation and related time spent was obtained from national census and available enquiries performed by the National Institute of Statistics. A daily exposure estimation module has been developed gathering all these data and considering empirical indoor/outdoor relations from literature to calculate the indoor concentrations in each one of the microenvironments considered, namely home, office/school, and other

  3. Aleppo pine bark as a biomonitor of atmospheric pollution in the arid environment of Jordan

    Energy Technology Data Exchange (ETDEWEB)

    Al-Alawi, Mu' taz M.; Jiries, Anwar [Prince Faisal Center for Dead Sea, Environmental and Energy Research, Mu' tah University, Al-Karak (Jordan); Carreras, Hebe [University of Cordoba, FCEFyN, Cordoba (Argentina); Alawi, Mahmoud [Chemistry Department, University of Jordan, Amman (Jordan); Charlesworth, Susanne M. [Geography, Environment and Disaster Management, Coventry University, Coventry (United Kingdom); Batarseh, Mufeed I.

    2007-11-15

    Monitoring of atmospheric pollution using Aleppo bark as a bioindicator was carried out in the industrial area surrounding the Al-Hussein thermal power station and the oil refinery at Al-Hashimyeh town, Jordan. The concentrations of heavy metals (copper, lead, cadmium, manganese, cobalt, nickel, zinc, iron, and chromium) were analyzed in bark samples collected from the study area during July 2004. The results showed that high levels of heavy metals were found in tree bark samples retrieved from all studied sites compared with the remote reference site. This is, essentially, due to the fact that the oil refinery and the thermal power plant still use low-quality fuel oil from the by-products of oil refining. Automobile emissions are another source of pollution since the study area is located along a major heavy-traffic highway. It was found that the area around the study sites (Al-Hashimyeh town, Zarqa) is polluted with high levels of heavy metals. Pine bark was found to be a suitable bioindicator of aerial fallout of heavy metals in arid regions. (Abstract Copyright [2007], Wiley Periodicals, Inc.)

  4. The atmospheric pollution in a few words; La pollution atmospherique en bref

    Energy Technology Data Exchange (ETDEWEB)

    NONE

    2002-07-01

    This paper takes stock briefly on the different pollution sources (carbon dioxide, nitrogen oxides, sulfur dioxide, VOC, methane...), the mechanisms (acidification, photochemical pollution, eutrophication, greenhouse effect, ozone...) and the effects on the health. (A.L.B.)

  5. STUDY OF ACAROID MITES POLLUTION IN STORED FRUIT-DERIVED CHINESE MEDICINAL MATERIALS.

    Science.gov (United States)

    Xu, Li-fa; Li, He-xia; Xu, Peng-fei; Xu, Hai-feng; Li, Chao-pin

    2015-08-01

    to investigate the species and breeding density of acaroid mites in stored fruit-derived Chinese medicinal materials in Anhui province. samples of stored fruit-derived Chinese medicinal materials were collected from 30 herb stores and storehouses in 17 Anhui cities, where the breeding acaroids mites were detected. 20 species of acaroids mites were found in 33 samples, belonging to 15 genus, 5 families of the acaridae respectively, among which T. putrescentiae, A. farinae, C. lactis, and C. berlesei are predominant species. stored fruit-derived Chinese medicinal materials in Anhui areas suffer from serious acaroid mites pollution. Therefore, proactive measures should be taken to control acaroid mites from breeding in an effort to reduce the harm on medicinal materials. Copyright AULA MEDICA EDICIONES 2014. Published by AULA MEDICA. All rights reserved.

  6. Mathematical models for atmospheric pollutants. Final report

    International Nuclear Information System (INIS)

    Drake, R.L.; Barrager, S.M.

    1979-08-01

    The present and likely future roles of mathematical modeling in air quality decisions are described. The discussion emphasizes models and air pathway processes rather than the chemical and physical behavior of specific anthropogenic emissions. Summarized are the characteristics of various types of models used in the decision-making processes. Specific model subclasses are recommended for use in making air quality decisions that have site-specific, regional, national, or global impacts. The types of exposure and damage models that are currently used to predict the effects of air pollutants on humans, other animals, plants, ecosystems, property, and materials are described. The aesthetic effects of odor and visibility and the impact of pollutants on weather and climate are also addressed. Technical details of air pollution meteorology, chemical and physical properties of air pollutants, solution techniques, and air quality models are discussed in four appendices bound in separate volumes

  7. Ocean-atmosphere pollutant circulation processes: The Heligoland Bight ecosystem (PRISMA). 2. interim report (1991)

    International Nuclear Information System (INIS)

    1992-04-01

    The PRISMA BMFT project is an important stage on the way to a comprehensive knowledge of the impacts of pollutants on the North Sea/Heligoland Bight ecosystem. The overall project is dedicated to the development, verification and application of a complex shelf-sea model which provides qualitative and quantitative data about the causal interactions between the basic atmospheric conditions, the hydrodynamics and thermodynamics of the water, the chemical reactons in the air, in the water and the sediments, and the activity of organisms. The model comprises a compact set of formulae, process formulations, initial and marginal conditions and empirical parameters which serves to describe the origin, transport, reactions and final deposition of pollutants in the North Sea, helps to analyze and elucidate the present condition of the ecosystem and its spatial and temporal variability, and provides forecasts in accordance with the changing natural and anthropogenic environmental conditions. (orig.) [de

  8. Atmospheric mercury deposition and its contribution of the regional atmospheric transport to mercury pollution at a national forest nature reserve, southwest China.

    Science.gov (United States)

    Ma, Ming; Wang, Dingyong; Du, Hongxia; Sun, Tao; Zhao, Zheng; Wei, Shiqing

    2015-12-01

    Atmospheric mercury deposition by wet and dry processes contributes to the transformation of mercury from atmosphere to terrestrial and aquatic systems. Factors influencing the amount of mercury deposited to subtropical forests were identified in this study. Throughfall and open field precipitation samples were collected in 2012 and 2013 using precipitation collectors from forest sites located across Mt. Jinyun in southwest China. Samples were collected approximately every 2 weeks and analyzed for total (THg) and methyl mercury (MeHg). Forest canopy was the primary factor on THg and MeHg deposition. Simultaneously, continuous measurements of atmospheric gaseous elemental mercury (GEM) were carried out from March 2012 to February 2013 at the summit of Mt. Jinyun. Atmospheric GEM concentrations averaged 3.8 ± 1.5 ng m(-3), which was elevated compared with global background values. Sources identification indicated that both regional industrial emissions and long-range transport of Hg from central, northeast, and southwest China were corresponded to the elevated GEM levels. Precipitation deposition fluxes of THg and MeHg in Mt. Jinyun were slightly higher than those reported in Europe and North America, whereas total fluxes of MeHg and THg under forest canopy on Mt. Jiuyun were 3 and 2.9 times of the fluxes of THg in wet deposition in the open. Highly elevated litterfall deposition fluxes suggest that even in remote forest areas of China, deposition of atmospheric Hg(0) via uptake by vegetation leaf may be a major pathway for the deposition of atmospheric Hg. The result illustrates that areas with greater atmospheric pollution can be expected to have greater fluxes of Hg to soils via throughfall and litterfall.

  9. Towards a monitoring strategy to assess the anthropogenic signature of traffic derived pollution

    Science.gov (United States)

    Ojha, G.; Appel, E.; Magiera, T.; Wawer, M.

    2013-12-01

    Soil contamination along roadsides is one important factor of anthropogenic linear pollution source. In our present study we focus on typical traffic pollutants like heavy metals (HM), platinum group elements (PGEs), polycyclic aromatic hydrocarbons (PAHs) and investigate the use of magnetic parameters, in particular to discriminate the distribution of contaminants by surface runoff, splash-water and airborne transport. For monitoring we removed 10-15 cm of top soil at 1 m distance from the roadside edge and replaced it by 30 plastic boxes, and installed pillars at 1 m and 2 m distances to the roadside with samplers in different heights (ground, 0.5 m, 2 m) as well as 4 m long u-channels (surface and 2.5 cm above ground) perpendicular to the road. Clean quartz sand was used as collector material. Mass-specific magnetic susceptibility (χ) and the concentration of pollutants (HM, PAH) all show a significant increase with time in the box samples, however, there are obviously also seasonal and site-dependent effects which lead to more stable values over several months or even some decrease in the upper few cm due to vertical migration. Similar significant differences of χ, PAH and HM concentrations and an importance of splash-water were noticed in pillars and u-channels within one year of monitoring. Magnetic results revealed that magnetite-like phases are responsible for the enhancement of magnetic concentration. A good correlation between χ and semi-volatile and particle-bound PAH phases as well as HM suggests that χ can be used as a proxy for traffic derived PAH and HM pollution. SEM observations and EDX analyses identified a dominance of angular and aggregates-shaped particles with composition of Fe-Cr-Ni derived from traffic-specific activities (abrasion of tyres, exhausts and brake linings). The results from our monitoring studies will be utilized to develop new innovative roadside pollution monitoring concepts.

  10. Source reconciliation of atmospheric gas-phase and particle-phase pollutants during a severe photochemical smog episode.

    Science.gov (United States)

    Schauer, James J; Fraser, Matthew P; Cass, Glen R; Simoneit, Bernd R T

    2002-09-01

    A comprehensive organic compound-based receptor model is developed that can simultaneously apportion the source contributions to atmospheric gas-phase organic compounds, semivolatile organic compounds, fine particle organic compounds, and fine particle mass. The model is applied to ambient data collected at four sites in the south coast region of California during a severe summertime photochemical smog episode, where the model determines the direct primary contributions to atmospheric pollutants from 11 distinct air pollution source types. The 11 sources included in the model are gasoline-powered motor vehicle exhaust, diesel engine exhaust, whole gasoline vapors, gasoline headspace vapors, organic solvent vapors, whole diesel fuel, paved road dust, tire wear debris, meat cooking exhaust, natural gas leakage, and vegetative detritus. Gasoline engine exhaust plus whole gasoline vapors are the predominant sources of volatile organic gases, while gasoline and diesel engine exhaust plus diesel fuel vapors dominate the emissions of semivolatile organic compounds from these sources during the episode studied at all four air monitoring sites. The atmospheric fine particle organic compound mass was composed of noticeable contributions from gasoline-powered motor vehicle exhaust, diesel engine exhaust, meat cooking, and paved road dust with smaller but quantifiable contributions from vegetative detritus and tire wear debris. In addition, secondary organic aerosol, which is formed from the low-vapor pressure products of gas-phase chemical reactions, is found to be a major source of fine particle organic compound mass under the severe photochemical smog conditions studied here. The concentrations of secondary organic aerosol calculated in the present study are compared with previous fine particle source apportionment results for less intense photochemical smog conditions. It is shown that estimated secondary organic aerosol concentrations correlate fairly well with the

  11. Atmospheric pollution and plants, especially trees in cities

    International Nuclear Information System (INIS)

    Pauly, T.; Lohou, C.

    1992-01-01

    Trees in down live in ecologically difficult conditions and suffer a great number of aggressions. Air pollution only increases their state of weakness. Studies in this field are only at their infancy. The part of responsibility of air pollution on the decay of trees is very difficult to determine. However the effect of some pollutants can be observed at present (sulfur dioxide, ozone, hydrocarburants, dust, PAN, lead...). New special equipment will determine, quantify and perhaps resolve some problems of pollution and vegetation in our cities in the future. 11 refs

  12. Atmospheric element pollutant evaluation at the Sao Paulo University campus, Sao Paulo using Canoparmelia texana Lichen species

    Energy Technology Data Exchange (ETDEWEB)

    Rocha, Rosiana R.; Saiki, Mitiko, E-mail: rosianarocha@yahoo.com.br [Instituto de Pesquisas Energeticas e Nucleares (IPEN/CNEN-SP), Sao Paulo, SP (Brazil)

    2015-07-01

    The use of lichens as biomonitors of atmospheric pollutants has been considered as a very suitable tool when compared to conventional methods of direct measurements. Lichens in particular are widely used as biomonitors due to its easy sampling, low cost and resistance to environmental stresses. In this study, neutron activation analysis (NAA) was applied for element determinations in Canoparmelia texana lichenized fungi species. The samples were collected from tree barks in different sites at the Sao Paulo University Campus and in sites of areas considered non-polluted. Comparisons were made between the element concentration obtained in lichen from the study area and those from non-polluted sites. Results indicated that lichens from study area presented higher concentrations of As, Br, Ca, Cd, Co, Cr, Cs, Fe, K, La, Rb, Sb, Se and U than clean areas. The principal components analysis (PCA) was applied to the results obtained and five principal components were found as being responsible for almost 77 % of the variance. These findings suggest that element pollutants found may be associated with vehicular emissions, construction of buildings and metallurgical activities. (author)

  13. Atmospheric element pollutant evaluation at the Sao Paulo University campus, Sao Paulo using Canoparmelia texana Lichen species

    International Nuclear Information System (INIS)

    Rocha, Rosiana R.; Saiki, Mitiko

    2015-01-01

    The use of lichens as biomonitors of atmospheric pollutants has been considered as a very suitable tool when compared to conventional methods of direct measurements. Lichens in particular are widely used as biomonitors due to its easy sampling, low cost and resistance to environmental stresses. In this study, neutron activation analysis (NAA) was applied for element determinations in Canoparmelia texana lichenized fungi species. The samples were collected from tree barks in different sites at the Sao Paulo University Campus and in sites of areas considered non-polluted. Comparisons were made between the element concentration obtained in lichen from the study area and those from non-polluted sites. Results indicated that lichens from study area presented higher concentrations of As, Br, Ca, Cd, Co, Cr, Cs, Fe, K, La, Rb, Sb, Se and U than clean areas. The principal components analysis (PCA) was applied to the results obtained and five principal components were found as being responsible for almost 77 % of the variance. These findings suggest that element pollutants found may be associated with vehicular emissions, construction of buildings and metallurgical activities. (author)

  14. Modelling of pollution dispersion in atmosphere

    International Nuclear Information System (INIS)

    Borysiewicz, M.; Stankiewicz, R.

    1994-01-01

    The paper contains the review of the mathematical foundation of atmospheric dispersion models. The atmospheric phenomena relevant to atmospheric dispersion model are discussed. In particular the parametrization of processes with time and space scales smaller than numerical grid size, limited by available computer power, is presented. The special attention was devoted to similarity theory and parametrization of boundary layer. The numerical methods are analysed and the drawbacks of the method are presented. (author). 99 refs, 15 figs, 3 tabs

  15. Lead chromate detected as a source of atmospheric Pb and Cr (VI) pollution

    Science.gov (United States)

    Lee, Pyeong-Koo; Yu, Soonyoung; Chang, Hye Jung; Cho, Hye Young; Kang, Min-Ju; Chae, Byung-Gon

    2016-10-01

    Spherical black carbon aggregates were frequently observed in dust dry deposition in Daejeon, Korea. They were tens of micrometers in diameter and presented a mixture of black carbon and several mineral phases. Transmission electron microscopy (TEM) observations with energy-dispersive X-ray spectroscopy (EDS) and selected area diffraction pattern (SADP) analyses confirmed that the aggregates were compact and included significant amounts of lead chromate (PbCrO4). The compositions and morphologies of the nanosized lead chromate particles suggest that they probably originated from traffic paint used in roads and were combined as discrete minerals with black carbon. Based on Pb isotope analysis and air-mass backward trajectories, the dust in Daejeon received a considerable input of anthropogenic pollutants from heavily industrialized Chinese cities, which implies that long-range transported aerosols containing PbCrO4 were a possible source of the lead and hexavalent chromium levels in East Asia. Lead chromate should be considered to be a source of global atmospheric Pb and Cr(VI) pollution, especially given its toxicity.

  16. Lead chromate detected as a source of atmospheric Pb and Cr (VI) pollution.

    Science.gov (United States)

    Lee, Pyeong-Koo; Yu, Soonyoung; Chang, Hye Jung; Cho, Hye Young; Kang, Min-Ju; Chae, Byung-Gon

    2016-10-25

    Spherical black carbon aggregates were frequently observed in dust dry deposition in Daejeon, Korea. They were tens of micrometers in diameter and presented a mixture of black carbon and several mineral phases. Transmission electron microscopy (TEM) observations with energy-dispersive X-ray spectroscopy (EDS) and selected area diffraction pattern (SADP) analyses confirmed that the aggregates were compact and included significant amounts of lead chromate (PbCrO 4 ). The compositions and morphologies of the nanosized lead chromate particles suggest that they probably originated from traffic paint used in roads and were combined as discrete minerals with black carbon. Based on Pb isotope analysis and air-mass backward trajectories, the dust in Daejeon received a considerable input of anthropogenic pollutants from heavily industrialized Chinese cities, which implies that long-range transported aerosols containing PbCrO 4 were a possible source of the lead and hexavalent chromium levels in East Asia. Lead chromate should be considered to be a source of global atmospheric Pb and Cr(VI) pollution, especially given its toxicity.

  17. Atmospheric Pollution from Shipping and Oil platforms of West Africa (APSOWA) observed during the airborne DACCIWA campaign

    Science.gov (United States)

    Krysztofiak-Tong, Gisèle; Brocchi, Vanessa; Catoire, Valéry; Stratmann, Greta; Sauer, Daniel; Deroubaix, Adrien; Deetz, Konrad; Schlager, Hans

    2017-04-01

    In the framework of the European DACCIWA (Dynamics-Aerosol-Chemistry-Cloud Interactions in West Africa) project, the airborne study APSOWA (Atmospheric Pollution from Shipping and Oil platforms of West Africa) has been conducted in July 2016 to study emissions from oil rigs and maritime traffic in the Gulf of Guinea. The measurements were performed during four flights of about 3-4 hours including meandering transects through emission plumes in the planetary boundary layer (around 300 m asl) off the coast of West Africa from Ivory Coast to Togo. Several instruments have been used on-board the DLR Falcon-20, providing measurements of the pollutants O3, CO, NO2, SO2, aerosol content and meteorological parameters. This set of trace gases can be used to fingerprint different sources of local air pollution. The first part of our study is focused on the FPSO Kwame Nkrumah facility operating in the Jubilee oil field off the coast of Ghana. Aircraft observations have been combined with a nested-grid regional scale Lagrangian particle dispersion model (FLEXPART) to estimate surface emission fluxes from this platform. A simplified inverse method is used and repeated until the modelling output and aircraft observations converged. The estimated fluxes of CO, SO2, NO2 are compared to global (EDGAR, MACCity) and regional (Deetz and Vogel, 2017, in press) inventories. A second part of the study provides the first results of the APSOWA flights for the study of the impact of shipping emissions on the regional air quality. Using data from Marine Traffic, ship positions during the campaign are identified. Then, FLEXPART is used to quantify the contributions of the ship emissions to the aircraft observations. Finally, direct measurements in the MBL around 4°N latitude along the Ghana coast show no strong evidence of the presence of an atmospheric pollution maritime corridor simulated by MACCity.

  18. Krypton-85 pollution and atmospheric electricity

    International Nuclear Information System (INIS)

    Harrison, R.G.; ApSimon, H.M.

    1994-01-01

    Krypton-86 is a chemically inert radioactive gas present in the atmosphere, concentrations of which have been greatly increased by nuclear reprocessing and weapons testing since 1945. The long half-life (10.7 yr), allows the gas to mix thoroughly in the atmosphere. Ionization caused by krypton-85 increases the electrical conductivity of atmospheric air. Further increases in krypton-85 emissions seem inevitable. The increase in air conductivity due to release of krypton-85 will vary with height, and be larger over the oceans than over the land. Increases in conductivity will produce uncertain effects on atmospheric phenomena, so changes are compared in magnitude with other factors perturbing the conductivity, such as combustion aerosol burdens, volcanic eruptions and nuclear weapons testing. Conductivity changes are expected to have the greatest significance for meteorological phenomena close to the source. (Author)

  19. A procedure for estimating site specific derived limits for the discharge of radioactive material to the atmosphere

    CERN Document Server

    Hallam, J; Jones, J A

    1983-01-01

    Generalised Derived Limits (GDLs) for the discharge of radioactive material to the atmosphere are evaluated using parameter values to ensure that the exposure of the critical group is unlikely to be underestimated significantly. Where the discharge is greater than about 5% of the GDL, a more rigorous estimate of the derived limit may be warranted. This report describes a procedure for estimating site specific derived limits for discharges of radioactivity to the atmosphere taking into account the conditions of the release and the location and habits of the exposed population. A worksheet is provided to assist in carrying out the required calculations.

  20. First simultaneous space measurements of atmospheric pollutants in the boundary layer from IASI: A case study in the North China Plain

    International Nuclear Information System (INIS)

    Boynard, Anne; Safieddine, Sarah; Oudot, Charlotte; Hadji-Lazaro, Juliette; Clerbaux, Cathy; Clarisse, Lieven; Bauduin, Sophie; Hurtmans, Daniel; Coheur, Pierre-Francois; Pommier, Matthieu; Van Damme, Martin

    2014-01-01

    In this paper we investigate a severe pollution episode that occurred in Beijing, Tianjin, and the Hebei province in January 2013. The episode was caused by the combination of anthropogenic emissions and a high-pressure system that trapped pollutants in the boundary layer. Using IASI (Infrared Atmospheric Sounding Interferometer) satellite measurements, high concentrations of key trace gases such as carbon monoxide (CO), sulfur dioxide (SO 2 ), and ammonia (NH 3 ) along with ammonium sulfate aerosol ((NH 4 ) 2 SO 4 ) are found. We show that IASI is able to detect boundary layer pollution in case of large negative thermal contrast combined with high levels of pollution. Our findings demonstrate that anthropogenic key pollutants, such as CO and SO 2 , can be monitored by IASI in the North China Plain during wintertime in support of air quality evaluation and management. (authors)

  1. Dispersion of effluents in the atmosphere; Dispersion des effluents dans l`atmosphere

    Energy Technology Data Exchange (ETDEWEB)

    NONE

    1999-12-31

    This conference day was organized by the `convection` section of the French association of thermal engineers with the support of the environment and energy mastery agency (ADEME). This book of proceedings contains 10 papers entitled: `physical modeling of atmospheric dispersion in wind tunnels. Some industrial examples`; `modeling of the noxious effects of a fire on the environment of an industrial site: importance of thermal engineering related hypotheses`; `atmospheric diffusion of a noxious cloud: fast evaluation method of safety areas around refrigerating installations that use ammonia`; `modeling of atmospheric flows in urban areas in order to study the dispersion of pollutants`; `use of a dispersion parameter to characterize the evolution of a diffusion process downstream of a linear source of passive contaminant placed inside a turbulent boundary layer`; `elements of reflexion around the development of an analytical methodology applied to the elaboration of measurement strategies of air quality in ambient and outdoor atmospheres around industrial sites`; `state-of-the-art about treatment techniques for VOC-rich gaseous effluents`; `characteristics of the time variation of the atmospheric pollution in the Paris region and visualization of its space distribution`; `mass-spectrometry for the measurement of atmospheric pollutants`; `volume variations in natural convection turbulence`. (J.S.)

  2. Dispersion of effluents in the atmosphere; Dispersion des effluents dans l`atmosphere

    Energy Technology Data Exchange (ETDEWEB)

    NONE

    1998-12-31

    This conference day was organized by the `convection` section of the French association of thermal engineers with the support of the environment and energy mastery agency (ADEME). This book of proceedings contains 10 papers entitled: `physical modeling of atmospheric dispersion in wind tunnels. Some industrial examples`; `modeling of the noxious effects of a fire on the environment of an industrial site: importance of thermal engineering related hypotheses`; `atmospheric diffusion of a noxious cloud: fast evaluation method of safety areas around refrigerating installations that use ammonia`; `modeling of atmospheric flows in urban areas in order to study the dispersion of pollutants`; `use of a dispersion parameter to characterize the evolution of a diffusion process downstream of a linear source of passive contaminant placed inside a turbulent boundary layer`; `elements of reflexion around the development of an analytical methodology applied to the elaboration of measurement strategies of air quality in ambient and outdoor atmospheres around industrial sites`; `state-of-the-art about treatment techniques for VOC-rich gaseous effluents`; `characteristics of the time variation of the atmospheric pollution in the Paris region and visualization of its space distribution`; `mass-spectrometry for the measurement of atmospheric pollutants`; `volume variations in natural convection turbulence`. (J.S.)

  3. Comparison between atmospheric pollutants from urban and rural areas employing the transplanted Usnea amblyoclada lichen species

    International Nuclear Information System (INIS)

    Mendes, Fabiana S.; Saiki, Mitiko; Genezini, Frederico A.; Alves, Edson R.; Santos, Jose O.; Martins, Marco A.G.; Saldiva, Paulo H.N.

    2011-01-01

    Over the last decades, lichens have been used as biomonitors in studies related to atmospheric pollution of several elements. The capability of absorbing and accumulating aerial pollutants, their longevity and resistance to environmental stresses have made lichens suitable for studies on air quality evaluation. In this study, a preliminary investigation employing Usnea amblyoclata lichen species and instrumental neutron activation analysis was performed to compare the levels of elements in the air of an urban and rural area. Samples of Usnea amblyoclada (Mull. Arg) collected in a clean area were exposed in a polluted area by vehicular emissions in Sao Paulo city and in a rural area of Caucaia do Alto Municipality, Cotia, SP. After 6 months of exposure the lichens were collected, cleaned, freeze-dried and ground for analyses. Samples and elemental standards were irradiated at the IEA-R1 nuclear research reactor and their induced activities were measured using a gamma ray spectrometer. Results indicated that lichens exposed in the polluted urban area presented higher levels of Ba, Br, Ca, Co, Cr, La, Sb, Sc, Se, Th, V and Zn than those from the rural area. Besides that ,concentrations of As, Ba, Br, Ca, Co, Cr, Fe, Hf, La, Mg, Th, Sc and V in lichens exposed in the rural and polluted urban area were higher than those that were not exposed. Quality control of analytical results was achieved by the analyses of certified reference material. Lichen species used in this study proved to be very useful for active monitoring of a polluted urban environment. (author)

  4. Comparison between atmospheric pollutants from urban and rural areas employing the transplanted Usnea amblyoclada lichen species

    Energy Technology Data Exchange (ETDEWEB)

    Mendes, Fabiana S.; Saiki, Mitiko; Genezini, Frederico A.; Alves, Edson R.; Santos, Jose O., E-mail: mitiko@ipen.br, E-mail: fredzini@ipen.br, E-mail: eralves@ipen.br [Instituto de Pesquisas Energeticas e Nucleares (IPEN/CNEN-SP), Sao Paulo, SP (Brazil); Martins, Marco A.G.; Saldiva, Paulo H.N., E-mail: marcogarciam@usp.br, E-mail: pepino@usp.br [Faculdade de Medicina da Universidade de Sao Paulo (FMUSP), Sao Paulo, SP (Brazil)

    2011-07-01

    Over the last decades, lichens have been used as biomonitors in studies related to atmospheric pollution of several elements. The capability of absorbing and accumulating aerial pollutants, their longevity and resistance to environmental stresses have made lichens suitable for studies on air quality evaluation. In this study, a preliminary investigation employing Usnea amblyoclata lichen species and instrumental neutron activation analysis was performed to compare the levels of elements in the air of an urban and rural area. Samples of Usnea amblyoclada (Mull. Arg) collected in a clean area were exposed in a polluted area by vehicular emissions in Sao Paulo city and in a rural area of Caucaia do Alto Municipality, Cotia, SP. After 6 months of exposure the lichens were collected, cleaned, freeze-dried and ground for analyses. Samples and elemental standards were irradiated at the IEA-R1 nuclear research reactor and their induced activities were measured using a gamma ray spectrometer. Results indicated that lichens exposed in the polluted urban area presented higher levels of Ba, Br, Ca, Co, Cr, La, Sb, Sc, Se, Th, V and Zn than those from the rural area. Besides that ,concentrations of As, Ba, Br, Ca, Co, Cr, Fe, Hf, La, Mg, Th, Sc and V in lichens exposed in the rural and polluted urban area were higher than those that were not exposed. Quality control of analytical results was achieved by the analyses of certified reference material. Lichen species used in this study proved to be very useful for active monitoring of a polluted urban environment. (author)

  5. Marine Pollution Prevention Act

    Data.gov (United States)

    National Oceanic and Atmospheric Administration, Department of Commerce — The Marine Pollution Prevention Act of 2008 implements the International Convention for the Prevention of Pollution from Ships, including related Protocols (MARPOL)...

  6. Atmospheric 14C variations derived from tree rings during the early Younger Dryas

    Science.gov (United States)

    Hua, Quan; Barbetti, Mike; Fink, David; Kaiser, Klaus Felix; Friedrich, Michael; Kromer, Bernd; Levchenko, Vladimir A.; Zoppi, Ugo; Smith, Andrew M.; Bertuch, Fiona

    2009-12-01

    Atmospheric radiocarbon variations over the Younger Dryas interval, from ˜13,000 to 11,600 cal yr BP, are of immense scientific interest because they reveal crucial information about the linkages between climate, ocean circulation and the carbon cycle. However, no direct and reliable atmospheric 14C records based on tree rings for the entire Younger Dryas have been available. In this paper, we present (1) high-precision 14C measurements on the extension of absolute tree-ring chronology from 12,400 to 12,560 cal yr BP and (2) high-precision, high-resolution atmospheric 14C record derived from a 617-yr-long tree-ring chronology of Huon pine from Tasmania, Australia, spanning the early Younger Dryas. The new tree-ring 14C records bridge the current gap in European tree-ring radiocarbon chronologies during the early Younger Dryas, linking the floating Lateglacial Pine record to the absolute tree-ring timescale. A continuous and reliable atmospheric 14C record for the past 14,000 cal yr BP including the Younger Dryas is now available. The new records indicate that the abrupt rise in atmospheric Δ 14C associated with the Younger Dryas onset occurs at ˜12,760 cal yr BP, ˜240 yrs later than that recorded in Cariaco varves, with a smaller magnitude of ˜40‰ followed by several centennial Δ 14C variations of 20-25‰. Comparing the tree-ring Δ 14C to marine-derived Δ 14C and modelled Δ 14C based on ice-core 10Be fluxes, we conclude that changes in ocean circulation were mainly responsible for the Younger Dryas onset, while a combination of changes in ocean circulation and 14C production rate were responsible for atmospheric Δ 14C variations for the remainder of the Younger Dryas.

  7. [Pollution evaluation and health risk assessment of heavy metals from atmospheric deposition in Lanzhou].

    Science.gov (United States)

    Li, Ping; Xue, Su-Yin; Wang, Sheng-Li; Nan, Zhong-Ren

    2014-03-01

    In order to evaluate the contamination and health risk of heavy metals from atmospheric deposition in Lanzhou, samples of atmospheric deposition were collected from 11 sampling sites respectively and their concentrations of heavy metals were determined. The results showed that the average contents of Cu, Pb, Cd, Cr, Ni, Zn and Mn were 82.22, 130.31, 4.34, 88.73, 40.64, 369.23 and 501.49 mg x kg(-1), respectively. There was great difference among different functional areas for all elements except Mn. According to the results, the enrichment factor score of Mn was close to 1, while the enrichment of Zn, Ni, Cu and Cr was more serious, and Pb and Cd were extremely enriched. The assessment results of geoaccumulation index of potential ecological risk indicated that the pollution of Cd in the atmospheric deposition of Lanzhou should be classified as extreme degree, and that of Cu, Ni, Zn, Pb as between slight and extreme degrees, and Cr as practically uncontaminated. Contaminations of atmospheric dust by heavy metals in October to the next March were more serious than those from April to August. Health risk assessment indicated that the heavy metals in atmospheric deposition were mainly ingested by human bodies through hand-mouth ingestion. The non-cancer risk was higher for children than for adults. The order of non-cancer hazard indexes of heavy metals was Pb > Cr > Cd > Cu > Ni > Zn. The non-cancer hazard indexes and carcinogen risks of heavy metals were both lower than their threshold values, suggesting that they will not harm the health.

  8. Chromatographic air analyser microsystem for the selective and sensitive detection of atmospheric pollutants

    International Nuclear Information System (INIS)

    Sanchez, Jean-Baptiste; Lahlou, Houda; Mohsen, Yehya; Berger, Franck; Vilanova, Xavier; Correig, Xavier

    2011-01-01

    The development of industry and automotive trafic produces Volatile Organic Compounds (VOCs) whose toxicity can affect seriously human health and environment. The level of those contaminants in air must be as low as possible. In this context, there is a need for in situ systems that could monitor selectively the concentration of these compounds. The aim of this study is to demonstrate the efficiency of a system build with a pre-concentrator, a chromatographic micro-column and a tin oxide-based gas sensor for the selective and sensitive detection of atmospheric pollutants. In particular, this study is focused on the selective detection of benzene and 1,3 butadiene.

  9. Body burden of pesticides and wastewater-derived pollutants on freshwater invertebrates: Method development and application in the Danube River

    International Nuclear Information System (INIS)

    Inostroza, Pedro A.; Wicht, Anna-Jorina; Huber, Thomas; Nagy, Claudia; Brack, Werner; Krauss, Martin

    2016-01-01

    While environmental risk assessment is typically based on toxicant concentrations in water and/or sediment, awareness is increasing that internal concentrations or body burdens are the key to understand adverse effects in organisms. In order to link environmental micropollutants as causes of observed effects, there is an increasing demand for methods to analyse these chemicals in organisms. Here, a multi-target screening method based on pulverised liquid extraction (PuLE) and a modified QuEChERS approach with an additional hexane phase was developed. It is capable to extract and quantify organic micropollutants of diverse chemical classes in freshwater invertebrates. The method was tested on gammarids from the Danube River (within the Joint Danube Survey 3) and target compounds were analysed by liquid chromatography-tandem mass spectrometry (LC-MS/MS). Furthermore, a non-target screening using high resolution-tandem mass spectrometry (LC-HRMS/MS) was conducted. A total of 17 pollutants were detected and/or quantified in gammarids at low concentrations. Pesticide concentrations ranged from 0.1 to 6.52 ng g −1 (wet weight), those of wastewater-derived pollutants from 0.1 to 2.83 ng g −1 (wet weight). The presence of wastewater-derived pollutants was prominent at all spots sampled. Using non-target screening, we could successfully identify several chlorinated compounds. These results demonstrate for the first time the presence of pesticides and wastewater-derived pollutants in invertebrates of the Danube River. - Highlights: • A method based on pulverised liquid extraction/QuEChERS for organic micropollutants in invertebrates was developed. • The method is applicable in assessing target environmental pollutants in invertebrates by LC-MS/MS. • The method allows for a nontarget screening of extracts by LC-HRMS. • First body burden analysis of pesticides and wastewater-derived pollutants in invertebrates in the Danube River is reported. - Capsule: A multi

  10. Impact of two chemistry mechanisms fully coupled with mesoscale model on the atmospheric pollutants distribution

    Science.gov (United States)

    Arteta, J.; Cautenet, S.; Taghavi, M.; Audiffren, N.

    Air quality models (AQM) consist of many modules (meteorology, emission, chemistry, deposition), and in some conditions such as: vicinity of clouds or aerosols plumes, complex local circulations (mountains, sea breezes), fully coupled models (online method) are necessary. In order to study the impact of lumped chemical mechanisms in AQM simulations, we examine the ability of both different chemical mechanisms: (i) simplified: Condensed Version of the MOdèle de Chimie Atmosphérique 2.2 (CV-MOCA2.2), and (ii) reference: Regional Atmospheric Chemistry Model (RACM), which are coupled online with the Regional Atmospheric Modeling Systems (RAMS) model, on the distribution of pollutants. During the ESCOMPTE experiment (Expérience sur Site pour COntraindre les Modèles de Pollution et de Transport d'Emissions) conducted over Southern France (including urban and industrial zones), Intensive observation periods (IOP) characterized by various meteorological and mixed chemical conditions are simulated. For both configurations of modeling, numerical results are compared with surface measurements (75 stations) for primary (NO x) and secondary (O 3) species. We point out the impact of the two different chemical mechanisms on the production of species involved in the oxidizing capacity such as ozone and radicals within urban and industrial areas. We highlight that both chemical mechanisms produce very similar results for the main pollutants (NO x and O 3) in three-dimensional (3D) distribution, despite large discrepancies in 0D modeling. For ozone concentration, we found sometimes small differences (5-10 ppb) between the mechanisms under study according to the cases (polluted or not). The relative difference between the two mechanisms over the whole domain is only -7% for ozone from CV-MOCA 2.2 versus RACM. When the order of magnitude is needed rather than an accurate estimate, a reduced mechanism is satisfactory. It has the advantage of running faster (four times less than CPU

  11. Some discussions on micrometeorology and atmospheric diffusion of classic and radioactive industrial pollutions. 1

    International Nuclear Information System (INIS)

    Veverka, O.; Vlachovsky, K.; Valenta, V.

    1976-01-01

    The fundamental static equations are given describing the atmosphere. Relations are derived for the description of dynamic phenomena, such as changes in temperature, pressure and density of the air in the lower part of the atmosphere. The effect of wind is considered and the expressions are presented for the vertical profile of wind velocity. The properties of flow are discussed in the fully developed boundary layer, such as stress, viscous stress and dynamic viscosity. The concept of surface roughness and its significance for micrometeorology is dealt with. (L.O.)

  12. Some discussions on micrometeorology and atmospheric diffusion of classic and radioactive industrial pollutions. 5

    International Nuclear Information System (INIS)

    Veverka, O.; Valenta, V.; Vlachovsky, K.

    1976-01-01

    The formulae are given expressing the atmospheric dispersion of industrial emissions released from the stacks of industrial plants and power plants. Gaussian distribution of the emissions is assumed. The behaviour of the plume is discussed and the concepts of lofting and fumigation are explained. Generalized relations are derived for the calculation of the atmospheric dispersion of gaseous wastes applicable to both high and short stack disposal and to the leakage from buildings, assuming that the source of emissions is of a point type and emissions are released continuously. (L.O.)

  13. Causes of daily cycle variability of atmospheric pollutants in a western Mediterranean urban site (DAURE campaign)

    Science.gov (United States)

    Reche, Cristina; Moreno, Teresa; Viana, Mar; Querol, Xavier; Alastuey, Andrés.; Jimenez, Jose L.; Pandolfi, Marco; Amato, Fulvio; Pérez, Noemí; Moreno, Natalia

    2010-05-01

    The 2009 DAURE Aerosol Campaign (23-February-2009 to 27-March-2009 and 1-July to 31-July) (see Presentation: Pandolfi et al., section AS3.2) had the objective of characterising the main sources and chemical processes controlling atmospheric pollution due to particulate matter in the Mediterranean site of Barcelona (Spain). An urban and a rural background site were selected in order to describe both kinds of pollution setting. Several parameters were taken into consideration, including the variability of mass concentration in the coarse and fine fractions, particle number, amount of black carbon and the concentration of gaseous pollutants (SO2, H2S, NO, NO2, CO, O3) present. Comparisons between the chemical composition of ambient atmospheric particles during day versus night were made using twelve-hour PM samples. The data shown here are focused on results obtained for the urban site where two main atmospheric settings were distinguishable in winter, namely Atlantic advection versus local air mass recirculation. During the warmer months Saharan dust intrusions added a third important influence on PM background. The data demonstrate that superimposed upon these background influences on city air quality are important local contributions from road traffic, construction-demolition works and shipping. There is also a major local contribution of secondary aerosols, with elevated number of particles occurring at midday (and especially in summer) when nucleation processes are favoured by photochemistry. Concentrations of SO2 peak at different times to the other gaseous pollutants due to regular daytime onshore south-easterly breezes bringing harbour emissions into the city. Road traffic in Barcelona also has a great impact on air quality, as demonstrated by daily and weekly cycles of gaseous pollutants, black carbon and the finer fraction of PM, with peaks being coincident with traffic rush-hours (8-10h and 20-22h), levels of pollution increasing from Monday to Friday, and

  14. Atmospheric deposition of selected chemicals and their effect on nonpoint-source pollution in the Twin Cities Metropolitan Area, Minnesota

    Science.gov (United States)

    Brown, R.G.

    1984-01-01

    Atmospheric deposition and subsequent runoff concentrations of total Kjeldahl nitrogen, dissolved nitrite-plus-nitrate nitrogen, total phosphorus, total sulfate (only for atmospheric deposition), total chloride, and total lead were studied from April 1 to October 31, 1980, in one rural and three urban watersheds in the Twin Cities Metropolitan Area, Minnesota. Seasonal patterns of wetfall and dryfall generally were similar for all constituents except chloride in both rural and urban watersheds. Similarity between constituents and between rural and urban watersheds suggested that regional air masses transported from the Gulf of Mexico by frontal storm movements influence seasonal patterns of atmospheric deposition in the metropolitan area. Local influences such as industrial, agricultural, and vehicular air pollutants were found to influence the magnitude or rate of atmospheric deposition rather than the seasonal pattern. Chloride was primarily influenced by northwest frontal storms laden with coastal chloride. Local influences such as dust from road deicing salt dust are thought to have caused an increase in atmospheric chloride during June.

  15. Impact of a future H2 transportation on atmospheric pollution in Europe

    Science.gov (United States)

    Popa, M. E.; Segers, A. J.; Denier van der Gon, H. A. C.; Krol, M. C.; Visschedijk, A. J. H.; Schaap, M.; Röckmann, T.

    2015-07-01

    Hydrogen (H2) is being explored as a fuel for passenger vehicles; it can be used in fuel cells to power electric motors or burned in internal combustion engines. In order to evaluate the potential influence of a future H2-based road transportation on the regional air quality in Europe, we implemented H2 in the atmospheric transport and chemistry model LOTOS-EUROS. We simulated the present and future (2020) air quality, using emission scenarios with different proportions of H2 vehicles and different H2 leakage rates. The reference future scenario does not include H2 vehicles, and assumes that all present and planned European regulations for emissions are fully implemented. We find that, in general, the air quality in 2020 is significantly improved compared to the current situation in all scenarios, with and without H2 cars. In the future scenario without H2 cars, the pollution is reduced due to the strict European regulations: annually averaged CO, NOx and PM2.5 over the model domain decrease by 15%, 30% and 20% respectively. The additional improvement brought by replacing 50% or 100% of traditionally-fueled vehicles by H2 vehicles is smaller in absolute terms. If 50% of vehicles are using H2, the CO, NOx and PM2.5 decrease by 1%, 10% and 1% respectively, compared to the future scenario without H2 cars. When all vehicles run on H2, then additional decreases in CO, NOx and PM2.5 are 5%, 40%, and 5% relative to the no-H2 cars future scenario. Our study shows that H2 vehicles may be an effective pathway to fulfill the strict future EU air quality regulations. O3 has a more complicated behavior - its annual average decreases in background areas, but increases in the high-NOx area in western Europe, with the decrease in NOx. A more detailed analysis shows that the population exposure to high O3 levels decreases nevertheless. In all future scenarios, traffic emissions account for only a small proportion of the total anthropogenic emissions, thus it becomes more important

  16. Research on airborne comprehensive survey system of atmosphere quality

    International Nuclear Information System (INIS)

    Yu Zhentao; Yu Yanbin

    1998-01-01

    The global atmosphere pollution is becoming more and more serious, affecting the human existence and development. Besides, the high spectrum resolution remote sensing technique, which has been applied to observe topographic features, identify military objectives and distinguish lithology and vegetation, has the relation to atmosphere quality and is influenced by atmosphere pollution (including radon pollution) and dust content in the atmosphere, it is imperative to monitor atmosphere quality. Based upon the selection of some main parameters evaluating atmospheric quality and necessary equipment, the author introduces the design of multiple airborne comprehensive survey system of atmosphere quality and how to deal with problems that crop up during the hardware designing and software programming

  17. [Pollution Level and Source Apportionment of Atmospheric Particles PM₂.₅ in Southwest Suburb of Chengdu in Spring].

    Science.gov (United States)

    Lin, Yu; Ye, Zhi-xiang; Yang, Huai-jin; Zhang, Ju; Yin, Wei-wen; Li, Xiao-fen

    2016-05-15

    In order to understand the characteristics of PM₂.₅ pollution in the atmosphere of Chengdu southwest suburb, PM₂.₅ particles in Chengdu southwest suburb were collected and analyzed from March 18 to March 31st, 2015. The results showed that the daily average concentration of PM₂.₅ in the southwest suburb of Chengdu reached 121.21 µg · m⁻³, and the average daily concentration of 24 samples in 31 PM₂.₅ samples was over 75 µg · m⁻³, the daily excessive rate was 77%, indicating the PM₂.₅ pollution in the study area was serious in March. When studying the relationship between atmospheric and meteorological factors, it was found that there was a significant index correlation between PM₂.₅ concentration and atmospheric visibility, and it had a positive correlation with temperature and humidity, but the correlation was not obvious. NH₄⁺ (16.24%), SO₄²- (12.58%) and NO₃⁻ (9.91%) were dominant in PM₂.₅ The ratio of NO₃⁻/SO₄²⁻ was 0.77, which indicated that the pollution of stationary sources in the southwest suburb was more severe than that of mobile sources. Organic carbon (OC)/elemental carbon (EC) ratios were higher than 2, which indicated the existence of second organic carbon (SOC). Using OC/EC ratio method to estimate the concentration of SOC, it was found that the average concentration of SOC in the southwest suburb of Chengdu in March was 3.49 µ · m⁻³, and the contribution rate of OC was 20.6%, which showed that the main source of OC in the southwest suburb of Chengdu was primary discharge. The correlation analysis of OC and EC showed that the correlation coefficient reached 0.95, indicating that the OC and EC sources were similar and relatively stable, and there was a great impact of local source emissions on Chengdu southwest suburb in spring, and primary discharge played a dominant role, while the contribution of SOC to OC was relatively small, which was consistent with the SOC characteristics obtained

  18. Early atmospheric metal pollution provides evidence for Chalcolithic/Bronze Age mining and metallurgy in Southwestern Europe.

    Science.gov (United States)

    Martínez Cortizas, Antonio; López-Merino, Lourdes; Bindler, Richard; Mighall, Tim; Kylander, Malin E

    2016-03-01

    Although archaeological research suggests that mining/metallurgy already started in the Chalcolithic (3rd millennium BC), the earliest atmospheric metal pollution in SW Europe has thus far been dated to ~3500-3200 cal.yr. BP in paleo-environmental archives. A low intensity, non-extensive mining/metallurgy and the lack of appropriately located archives may be responsible for this mismatch. We have analysed the older section (>2100 cal.yr. BP) of a peat record from La Molina (Asturias, Spain), a mire located in the proximity (35-100 km) of mines which were exploited in the Chalcolithic/Bronze Age, with the aim of assessing evidence of this early mining/metallurgy. Analyses included the determination of C as a proxy for organic matter content, lithogenic elements (Si, Al, Ti) as markers of mineral matter, and trace metals (Cr, Cu, Zn, Pb) and stable Pb isotopes as tracers of atmospheric metal pollution. From ~8000 to ~4980 cal.yr. BP the Pb composition is similar to that of the underlying sediments (Pb 15 ± 4 μg g(-1); (206)Pb/(207)Pb 1.204 ± 0.002). A sustained period of low (206)Pb/(207)Pb ratios occurred from ~4980 to ~2470 cal.yr. BP, which can be divided into four phases: Chalcolithic (~4980-3700 cal.yr. BP), (206)Pb/(207)Pb ratios decline to 1.175 and Pb/Al ratios increase; Early Bronze Age (~3700-3500 cal.yr. BP), (206)Pb/(207)Pb increase to 1.192 and metal/Al ratios remain stable; Late Bronze Age (~3500-2800 cal.yr. BP), (206)Pb/(207)Pb decline to their lowest values (1.167) while Pb/Al and Zn/Al increase; and Early Iron Age (~2800-2470 cal.yr. BP), (206)Pb/(207)Pb increase to 1.186, most metal/Al ratios decrease but Zn/Al shows a peak. At the beginning of the Late Iron Age, (206)Pb/(207)Pb ratios and metal enrichments show a rapid return to pre-anthropogenic values. These results provide evidence of regional/local atmospheric metal pollution triggered by the earliest phases of mining/metallurgy in the area, and reconcile paleo-environmental and

  19. Effects of heating atmosphere on formation of crystalline citrate-derived LaAlO3 nanoparticles

    International Nuclear Information System (INIS)

    Yu, Hsuan-Fu; Guo, Yu-Man

    2011-01-01

    Research highlights: → LaAlO 3 can be crystallized at 550 deg. C in an oxygen-enriched atmosphere. → Calcining the citrate precursor in oxygen atmosphere lowers the reaction temperatures to form crystalline LaAlO 3 . → In oxygen atmosphere, pure citrate-derived LaAlO 3 nanoparticles can be produced at 700 deg. C. - Abstract: Crystalline LaAlO 3 nanoparticles were synthesized at relative low temperatures, using a citrate-precursor technique. La(NO 3 ) 3 , Al(NO 3 ) 3 , and C 3 H 4 (OH)(COOH) 3 , in a molar ratio of 1:1:1, were dissolved in deionized water. NH 4 OH was used to adjust the aqueous solution to pH 7. After drying, the citrate precursors were charred at 350 deg. C, followed by calcination at different temperatures, in air or oxygen atmosphere. The thermochemical properties of the resultant particles were analyzed using thermogravimetric and differential thermal analysis, X-ray diffractometry, infrared spectroscopy, scanning electron microscopy, and transmission electron microscopy. Effects of calcination temperature and heating atmosphere on the formation of crystalline LaAlO 3 nanoparticles were investigated. In O 2 atmosphere, clacining the citrate-derived charred solid precursor at 700 deg. C for 3 h can decompose all intermediates to produce pure LaAlO 3 nanoparticles (particle sizes ≤ 100 nm) with an average crystallite size of about 24 nm and possessing high sinterability.

  20. Atmospheric Pollution and Urban Development in China

    OpenAIRE

    Guinot, Benjamin

    2011-01-01

    Chinese cities face the challenge of battling air pollution during a time of rapid urbanisation and rising energy demand. Poor air quality is heightening anxiety over the environment. Given pollution’s economic cost, a real policy of monitoring and control has emerged at the national level. Chinese researchers and industry have come up with technological responses to the enormous challenges. While some showcase cities have boosted their pollution-control measures, the situation in smaller one...

  1. Opinions of the French on the atmospheric pollution, the wastes management and the eco-products; Opinions des francais sur la pollution atmospherique, la gestion des dechets et les eco-produits

    Energy Technology Data Exchange (ETDEWEB)

    NONE

    1999-06-01

    Five main opinions can be presented from the answers analysis to the inquiry realized in 1999 by the ADEME on the French way of life and aspirations. The French think that the atmospheric pollution is dangerous for the health and that they are badly informed about the air quality of their town. 87% of the motorists are ready to leave their vehicles the days of high urban pollution level. In less of two years the green products credibility is worsening. Nevertheless the consumer believes sensitive to the ecological arguments. Finally the French are very favorable to the domestic wastes control. (A.L.B.)

  2. Mapping atmospheric aerosols with a citizen science network of smartphone spectropolarimeters

    Science.gov (United States)

    Snik, Frans; Rietjens, Jeroen H. H.; Apituley, Arnoud; Volten, Hester; Mijling, Bas; Di Noia, Antonio; Heikamp, Stephanie; Heinsbroek, Ritse C.; Hasekamp, Otto P.; Smit, J. Martijn; Vonk, Jan; Stam, Daphne M.; Harten, Gerard; Boer, Jozua; Keller, Christoph U.

    2014-10-01

    To assess the impact of atmospheric aerosols on health, climate, and air traffic, aerosol properties must be measured with fine spatial and temporal sampling. This can be achieved by actively involving citizens and the technology they own to form an atmospheric measurement network. We establish this new measurement strategy by developing and deploying iSPEX, a low-cost, mass-producible optical add-on for smartphones with a corresponding app. The aerosol optical thickness (AOT) maps derived from iSPEX spectropolarimetric measurements of the daytime cloud-free sky by thousands of citizen scientists throughout the Netherlands are in good agreement with the spatial AOT structure derived from satellite imagery and temporal AOT variations derived from ground-based precision photometry. These maps show structures at scales of kilometers that are typical for urban air pollution, indicating the potential of iSPEX to provide information about aerosol properties at locations and at times that are not covered by current monitoring efforts.

  3. Global atmospheric changes.

    Science.gov (United States)

    Piver, W T

    1991-12-01

    Increasing concentrations of CO2 and other greenhouse gases in the atmosphere can be directly related to global warming. In terms of human health, because a major cause of increasing atmospheric concentrations of CO2 is the increased combustion of fossil fuels, global warming also may result in increases in air pollutants, acid deposition, and exposure to ultraviolet (UV) radiation. To understand better the impacts of global warming phenomena on human health, this review emphasizes the processes that are responsible for the greenhouse effect, air pollution, acid deposition, and increased exposure to UV radiation.

  4. First simultaneous space measurements of atmospheric pollutants in the boundary layer from IASI: a case study in the North China Plain

    Science.gov (United States)

    Boynard, Anne; Clerbaux, Cathy; Clarisse, Lieven; Safieddine, Sarah; Pommier, Matthieu; Van Damme, Martin; Bauduin, Sophie; Oudot, Charlotte; Hadji-Lazaro, Juliette; Hurtmans, Daniel; Coheur, Pierre-François

    2014-05-01

    An extremely severe and persistent smog episode occurred in January 2013 over China. The levels of air pollution have been dangerously high, reaching 40 times recommended safety levels and have affected health of millions of people. China faced one of the worst periods of air quality in recent history and drew worldwide attention. This pollution episode was caused by the combination of anthropogenic emissions and stable meteorological conditions (absence of wind and temperature inversion) that trapped pollutants in the boundary layer. To characterize this episode, we used the IASI (Infrared Atmospheric Sounding Interferometer) instrument onboard the MetOp-A platform. IASI observations show high concentrations of key trace gases such as carbon monoxide (CO), sulfur dioxide (SO2) and ammonia (NH3) along with ammonium sulfate aerosol. We show that IASI is able to detect boundary layer pollution in case of large negative thermal contrast combined with high levels of pollution. Our findings demonstrate the ability of thermal infrared instrument such as IASI to monitor boundary layer pollutants, which can support air quality evaluation and management.

  5. Some indices of bodily reaction of traffic controllers to atmospheric pollution by automobile exhaust gases

    Energy Technology Data Exchange (ETDEWEB)

    Partsef, D.P.; Bessonova, N.A.

    1976-12-01

    The authors studied pollution of the atmospheric air at 20 posts on Moscow streets with various intensity of auto traffic. They sampled for carbon monoxide, hydrocarbons, nitrogen dioxide, dust, acrolein, oxidants, and ozone and found that the concentration of these substances was a direct function of the intensity of auto flow and a reverse function of the width of the highway. Traffic controllers exhibited increased carboxyhemoglobin blood levels, decrease in bactericidal properties and increase in number of colonies of skin microorganisms. The controller complained in weariness, cardiovascular and gastrointestinal disturbances.

  6. [The response of the upper respiratory tract to the impact of atmospheric pollution].

    Science.gov (United States)

    Mukhamadiev, R A; Ismagilov, Sh M

    2015-01-01

    The present literature review characterizes the environmental conditions in the Russian Federation in general and the Republic of Tatarstan in particular with special reference to the influence of atmospheric pollution on the development and the clinical picture of the diseases of the respiratory organs including pathology of the upper respiratory tract in the populations of the industrial centres and other environmentally unfriendly areas. The views of the domestic and foreign authors concerning the role of the environmental factors in the clinical picture of the upper respiratory tract disorders are described in detail. The authors emphasize the necessity of the further investigationsinto this problem and the development of the methods for the prevention of diseases of the upper respiratory react.

  7. Atmospheric pollution in the Tula Industrial Corridor studied using a bio monitor and nuclear analytical techniques

    Energy Technology Data Exchange (ETDEWEB)

    Martinez C, M. A.; Solis, C.; Andrade, E. [UNAM, Instituto de Fisica, Apdo. Postal 20-364, 01000 Mexico D. F. (Mexico); Beltran H, R. I. [Universidad Autonoma del Estado de Hidalgo, Centro de Investigaciones Quimicas, Carretera Pachuca-Tulancingo Km. 4.5, 42184 Pachuca, Hidalgo (Mexico); Issac O, K. [Universidad Autonoma del Estado de Mexico, Facultad de Medicina, Paseo Tollocan s/n, esq. Jesus Carranza, 50120 Toluca, Estado de Mexico (Mexico); Lucho C, C. A. [Universidad Politecnica de Pachuca, Carretera Pachuca-Cd. Sahagun Km. 20, Hidalgo (Mexico); Lopez R, M. C.; Longoria, L. C. [ININ, Carretera Mexico-Toluca s/n, 52750 Ocoyoacac, Estado de Mexico (Mexico)

    2011-02-15

    This study deals with the application of nuclear analytical techniques to analyze trace elements in the biological monitor Tillandsia usneoides. Biological monitors provides an alternative advantageous way of particulate matter sampling in air pollution studies, since there is no need of special sampling devices, accumulation time can be as long as desired. T. usneoides, which occurs naturally throughout Mexico, was used to monitor air quality of Tula-Vito-Apasco (TVA) industrial corridor at central Mexico. This area is considered one of the critical zones of the country because of atmospheric contaminants high concentration. Particulate matter is regulated by Mexican norms, but its chemical composition is not. Plants were transplanted from a clean environment to four sites at the TVA corridor, and exposed for 12 weeks from February to April 2008. Trace element accumulation of plants was determined by particle induced X-ray emission and neutron activation analysis. Results reveal differences in trace elements distribution among sites in the TVA corridor. Furthermore, anthropogenic elements (S, V) and crustal elements (Ca) in T. usneoides exhibit high levels. Highly toxic elements such as Hg, As and Cr although present at trace levels, showed un enrichment relative to the initial values, when transplanted to the TVA corridor. Results show that monitoring with T. usneoides allows a first approximation of air sources to provide insights of the atmospheric pollution in the TVA corridor. (Author)

  8. Atmospheric pollution in the Tula Industrial Corridor studied using a bio monitor and nuclear analytical techniques

    International Nuclear Information System (INIS)

    Martinez C, M. A.; Solis, C.; Andrade, E.; Beltran H, R. I.; Issac O, K.; Lucho C, C. A.; Lopez R, M. C.; Longoria, L. C.

    2011-01-01

    This study deals with the application of nuclear analytical techniques to analyze trace elements in the biological monitor Tillandsia usneoides. Biological monitors provides an alternative advantageous way of particulate matter sampling in air pollution studies, since there is no need of special sampling devices, accumulation time can be as long as desired. T. usneoides, which occurs naturally throughout Mexico, was used to monitor air quality of Tula-Vito-Apasco (TVA) industrial corridor at central Mexico. This area is considered one of the critical zones of the country because of atmospheric contaminants high concentration. Particulate matter is regulated by Mexican norms, but its chemical composition is not. Plants were transplanted from a clean environment to four sites at the TVA corridor, and exposed for 12 weeks from February to April 2008. Trace element accumulation of plants was determined by particle induced X-ray emission and neutron activation analysis. Results reveal differences in trace elements distribution among sites in the TVA corridor. Furthermore, anthropogenic elements (S, V) and crustal elements (Ca) in T. usneoides exhibit high levels. Highly toxic elements such as Hg, As and Cr although present at trace levels, showed un enrichment relative to the initial values, when transplanted to the TVA corridor. Results show that monitoring with T. usneoides allows a first approximation of air sources to provide insights of the atmospheric pollution in the TVA corridor. (Author)

  9. Attempt at mapping acidic atmospheric pollution in the north of France in relation to the toxic sensitivity of epiphytic lichens

    Energy Technology Data Exchange (ETDEWEB)

    Gehu, J M; Bon, M; Delzenne, C; Rose, F

    1973-01-29

    The authors present, for the first time in France, a map of acidic atmospheric pollution (for the departments of Nord, Pas-de-calais and Somme) based on the study of the epiphytic lichen flora and its distribution in ten zones of toxic sensitivity, using the Hawksworth and Rose scale.

  10. Study of occupational health impact of atmospheric pollution on exposed workers at an iron and steel complex by using neutron activation analysis of scalp hair

    International Nuclear Information System (INIS)

    Chai, Z.F.; Qian, Q.F.; Feng, X.Q.; Zhang, P.Q.; Liu, N.Q.; Feng, W.Y.

    2004-01-01

    The occupational health impact of atmospheric pollution on exposed workers at one iron and steel complex was studied by instrumental neutron activation analysis of workers' hair samples and medical examination. The experimental results indicate that there is a positive correlation between the high inhalation amounts of iron and other trace elements by the exposed workers and the symptom of their high blood pressure and hypoglycemia, which implies that the atmospheric environment polluted by iron and steel industry has an adverse health impact on the exposed workers. The measures to relieve and abate the occupational diseases caused by air-borne particulate matter should be taken. (author)

  11. Effects of atmospheric deposition of energy-related pollutants on water quality: a review and assessment

    International Nuclear Information System (INIS)

    Davis, M.J.

    1981-05-01

    The effects on surface-water quality of atmospheric pollutants that are generated during energy production are reviewed and evaluated. Atmospheric inputs from such sources to the aquatic environment may include trace elements, organic compounds, radionuclides, and acids. Combustion is the largest energy-related source of trace-element emissions to the atmosphere. This report reviews the nature of these emissions from coal-fired power plants and discusses their terrestrial and aquatic effects following deposition. Several simple models for lakes and streams are developed and are applied to assess the potential for adverse effects on surface-water quality of trace-element emissions from coal combustion. The probability of acute impacts on the aquatic environment appears to be low; however, more subtle, chronic effects are possible. The character of acid precipitation is reviewed, with emphasis on aquatic effects, and the nature of existing or potential effects on water quality, aquatic biota, and water supply is considered. The response of the aquatic environment to acid precipitation depends on the type of soils and bedrock in a watershed and the chemical characteristics of the water bodies in question. Methods for identifying regions sensitive to acid inputs are reviewed. The observed impact of acid precipitation ranges from no effects to elimination of fish populations. Coal-fired power plants and various stages of the nuclear fuel cycle release radionuclides to the atmosphere. Radioactive releases to the atmosphere from these sources and the possible aquatic effects of such releases are examined. For the nuclear fuel cycle, the major releases are from reactors and reprocessing. Although aquatic effects of atmospheric releases have not been fully quantified, there seems little reason for concern for man or aquatic biota

  12. Assessing the impact of anthropogenic pollution on isoprene-derived secondary organic aerosol formation in PM2.5 collected from the Birmingham, Alabama, ground site during the 2013 Southern Oxidant and Aerosol Study

    Directory of Open Access Journals (Sweden)

    W. Rattanavaraha

    2016-04-01

    Full Text Available In the southeastern US, substantial emissions of isoprene from deciduous trees undergo atmospheric oxidation to form secondary organic aerosol (SOA that contributes to fine particulate matter (PM2.5. Laboratory studies have revealed that anthropogenic pollutants, such as sulfur dioxide (SO2, oxides of nitrogen (NOx, and aerosol acidity, can enhance SOA formation from the hydroxyl radical (OH-initiated oxidation of isoprene; however, the mechanisms by which specific pollutants enhance isoprene SOA in ambient PM2.5 remain unclear. As one aspect of an investigation to examine how anthropogenic pollutants influence isoprene-derived SOA formation, high-volume PM2.5 filter samples were collected at the Birmingham, Alabama (BHM, ground site during the 2013 Southern Oxidant and Aerosol Study (SOAS. Sample extracts were analyzed by gas chromatography–electron ionization-mass spectrometry (GC/EI-MS with prior trimethylsilylation and ultra performance liquid chromatography coupled to electrospray ionization high-resolution quadrupole time-of-flight mass spectrometry (UPLC/ESI-HR-QTOFMS to identify known isoprene SOA tracers. Tracers quantified using both surrogate and authentic standards were compared with collocated gas- and particle-phase data as well as meteorological data provided by the Southeastern Aerosol Research and Characterization (SEARCH network to assess the impact of anthropogenic pollution on isoprene-derived SOA formation. Results of this study reveal that isoprene-derived SOA tracers contribute a substantial mass fraction of organic matter (OM ( ∼  7 to  ∼  20 %. Isoprene-derived SOA tracers correlated with sulfate (SO42− (r2 = 0.34, n = 117 but not with NOx. Moderate correlations between methacrylic acid epoxide and hydroxymethyl-methyl-α-lactone (together abbreviated MAE/HMML-derived SOA tracers with nitrate radical production (P[NO3] (r2 = 0.57, n = 40 were observed during nighttime, suggesting a

  13. Influence of Air Pollution on Chemical Quality of Wet Atmospheric Deposition: a Case Study in Urmia, Iran

    Directory of Open Access Journals (Sweden)

    Yaghoub Hajizadeh

    2017-10-01

    Full Text Available Increased combustion of fossil fuel owing to the energy requirement is a main cause of air pollution throughout the world. Atmospheric precipitation is considered as a major water resource for indoor, municipal, industrial and agricultural uses. This study was aimed to evaluate the effect of air pollution on chemical quality of rain and snow in Urmia, a city in northwest of Iran. Sampling was performed during the wet seasons from October to March at six sampling stations in different locations of the city. Acidity, alkalinity, NO3- , SO42-, Cl- and pH contents of the collected samples were analyzed. All samples showed a pH value of more than 6.8, and lower acidity than alkalinity, therefore, the precipitations were not acidic. Maximum concentrations of SO42- and NO3- in the samples were 5 and 8.8mg/L, respectively. Chloride was varied from 1 to 11.5 mg/L with the highest measures observing in autumn. According to the results, concentrations of the analyzed parameters in wet precipitations in Urmia were within the natural ranges except chloride ions, which was higher than its common level in the atmosphere. This phenomenon may be the result of desert dusts which transfers by wind from the west border to Iran. ‎

  14. Air Pollution and Environmental Justice Awareness

    Science.gov (United States)

    Bouvier-Brown, N. C.

    2014-12-01

    Air pollution is not equally dispersed in all neighborhoods and this raises many social concerns, such as environmental justice. "Real world" data, whether extracted from online databases or collected in the field, can be used to demonstrate air quality patterns. When students explore these trends, they not only learn about atmospheric chemistry, but they also become socially aware of any inequities. This presentation outlines specific ways to link air pollution and environmental justice suitable for an undergraduate upper division Air Pollution or Atmospheric Chemistry course.

  15. The effects of air pollution and climatic factors on atmospheric corrosion of marble under field exposure

    International Nuclear Information System (INIS)

    Lan, Tran Thi Ngoc; Nishimura, Rokuro; Tsujino, Yoshio; Satoh, Yukihiro; Thi Phuong Thoa, Nguyen; Yokoi, Masayuki; Maeda, Yasuaki

    2005-01-01

    The atmospheric corrosion of marble was evaluated in terms of SO 2 concentration as air pollution and climatic factors such as rainfall, relative humidity, temperature and so on under the field exposure. Marble of calcite type (CaCO 3 ) was exposed to outdoor atmospheric environment with and without a rain shelter at four test sites in the southern part of Vietnam for 3-month, 1- and 2-year periods from July 2001 to September 2003. The thickness loss of marble was investigated gravimetrically. X-ray diffraction and X-ray fluorescent methods were applied to study corrosion products on marble. The corrosion product of marble was only gypsum (CaSO 4 . 2H 2 O) and was washed out by rain under the unsheltered exposure condition. It was found that the most substantial factors influencing the corrosion of marble were rainfall, SO 2 concentration in the air and relative humidity. Based on the results obtained, we estimated the dose-response functions for the atmospheric corrosion of marble in the southern part of Vietnam

  16. Air pollution tracer studies in the lower atmosphere (citations from the NTIS data base). Report for 1964-Jan 80

    International Nuclear Information System (INIS)

    Cavagnaro, D.M.

    1980-02-01

    The cited reports cover research on the use of tracers to study lower atmospheric air pollution movements. The tracer used include sulfur hexafluoride, krypton 85, carbon 14, and other radioactive isotopes. The studies cite the results and techniques used, tracer movement from nuclear power plants, industrial stacks, urban areas, and the detectors used in their measurement

  17. Atmospheric transport of persistent organic pollutants - development of a 3-d dynamical transport model covering the northern hemisphere

    Science.gov (United States)

    Hansen, K. M.; Christensen, J. H.; Geels, C.; Frohn, L. M.; Brandt, J.

    2003-04-01

    The Danish Eulerian Hemispheric Model (DEHM) is a 3-D dynamical atmospheric transport model originally developed to describe the atmospheric transport of sulphur, lead, and mercury to the Arctic. The model has been validated carefully for these compounds. A new version of DEHM is currently being developed to describe the atmospheric transport of persistent organic pollutants (POPs) which are toxic, lipophilic and bio-accumulating compounds showing great persistence in the environment. The model has a horizontal resolution of 150 km x 150 km and 18 vertical layers, and it is driven by meteorological data from the numerical weather prediction model MM5V2. During environmental cycling POPs can be deposited and re-emitted several times before reaching a final destination. A description of the exchange processes between the land/ocean surfaces and the atmosphere is included in the model to account for this multi-hop transport. The present model version describes the atmospheric transport of the pesticide alpha-hexachlorocyclohexane (alpha-HCH). Other POPs may be included when proper data on emissions and physical-chemical parameters becomes available. The model-processes and the first model results are presented. The atmospheric transport of alpha-HCH for the 1990s is well described by the model.

  18. [The application of the multidimensional statistical methods in the evaluation of the influence of atmospheric pollution on the population's health].

    Science.gov (United States)

    Surzhikov, V D; Surzhikov, D V

    2014-01-01

    The search and measurement of causal relationships between exposure to air pollution and health state of the population is based on the system analysis and risk assessment to improve the quality of research. With this purpose there is applied the modern statistical analysis with the use of criteria of independence, principal component analysis and discriminate function analysis. As a result of analysis out of all atmospheric pollutants there were separated four main components: for diseases of the circulatory system main principal component is implied with concentrations of suspended solids, nitrogen dioxide, carbon monoxide, hydrogen fluoride, for the respiratory diseases the main c principal component is closely associated with suspended solids, sulfur dioxide and nitrogen dioxide, charcoal black. The discriminant function was shown to be used as a measure of the level of air pollution.

  19. A numerical study for the assessment of pollutant dispersion from Kostolac B power plant to Viminacium for different atmospheric conditions

    Directory of Open Access Journals (Sweden)

    Kozić Mirko S.

    2015-01-01

    Full Text Available The level of pollution concentration to the archaeological site Viminacium caused by the stack of Kostolac B power plant is analyzed using CFD software. The wind is directed from the stack toward Viminacium-Archaeological Site, Therma and Viminacium - Museum. Three different meteorological conditions resulting in fanning, fumigating and looping plume are modelled. The temperature gradient as the most important factor defining the conditions of the atmosphere is included through the appropriate boundary conditions. It is shown that concentrations of the pollutants on the objects of Viminacium are very low. It can be attributed to the stack height and high temperature of the smoke at its exit. It also indicates that other sources of pollution such as open ash dumps and acid rain should be checked.

  20. RNA-based molecular survey of biodiversity of limestone tombstone microbiota in response to atmospheric sulphur pollution.

    Science.gov (United States)

    Villa, F; Vasanthakumar, A; Mitchell, R; Cappitelli, F

    2015-01-01

    Outdoor stoneworks sustain biofilm formation and are constantly at risk of deterioration by micro-organisms. In this study, the biofilm microflora of historic limestone tombstones located in a highly polluted urban environment (Cambridge, MA) and in a less polluted location (Lexington, MA) were compared using comprehensive RNA-based molecular analyses of 16S rRNA gene sequences as well as sequences of genes for different pathways of sulphur metabolism (soxB, apsA, dsrA). The metabolically active micro-organisms detected by denaturing gradient gel electrophoresis analysis of 16S rRNA fragments were predominantly represented by cyanobacteria (belonging to the family Nostocaceae and to the genus Chroococcidiopsis) in both polluted and unpolluted environments. The investigation of soxB, apsA, dsrA transcripts reflected the abundance and the diversity of sulphur-oxidizing and sulphate-reducing bacteria in the Cambridge samples in comparison with the Lexington samples. The investigation revealed that in addition to phototrophic sulphur bacteria belonging to the genera Thiocapsa, Halochromatium, Allochromatium, Thiococcus and Thermochromatium, other sulphate-oxidizing prokaryotes (e.g. the genus Thiobacillus) as well as sequences of Deltaproteobacteria from the genus Desulfovibrio occurred at the polluted urban site. The interactions between the main functional groups retrieved from the limestone tombstones were discussed. The biofilm microflora inhabiting historic limestones are a multi-component open ecosystem sensitively reacting to all environmental factors including air pollutants. Little is known about specific target groups that are active in the biofilm and their physiological functions. For the first time, transcripts involved in important energy-yielding processes were investigated to reveal the metabolic capabilities of the microflora in response to atmospheric sulphur pollution. This work provides novel and important information about the ecology of limestone

  1. Link between sewage-derived nitrogen pollution and coral disease severity in Guam

    International Nuclear Information System (INIS)

    Redding, Jamey E.; Myers-Miller, Roxanna L.; Baker, David M.; Fogel, Marilyn; Raymundo, Laurie J.; Kim, Kiho

    2013-01-01

    Highlights: • We evaluated sources of nitrogen pollution in coastal waters of Guam. • Stable isotope analyses showed the dominance of sewage-derived nitrogen. • Nitrogen inputs correlated with coral disease severity. • Planned population increase on Guam will exacerbate impact of coral diseases. -- Abstract: The goals of this study were to evaluate the contribution of sewage-derived N to reef flat communities in Guam and to assess the impact of N inputs on coral disease. We used stable isotope analysis of macroalgae and a soft coral, sampled bimonthly, as a proxy for N dynamics, and surveyed Porites spp., a dominant coral taxon on Guam’s reefs, for white syndrome disease severity. Results showed a strong influence of sewage-derived N in nearshore waters, with δ 15 N values varying as a function of species sampled, site, and sampling date. Increases in sewage-derived N correlated significantly with increases in the severity of disease among Porites spp., with δ 15 N values accounting for more than 48% of the variation in changes in disease severity. The anticipated military realignment and related population increase in Guam are expected to lead to increased white syndrome infections and other coral diseases

  2. Atmospheric Pollution and Greenhouse Emissions over 14 Largest Megacities of the World

    Science.gov (United States)

    Chen, X.; Singh, R. P.

    2017-12-01

    Megacities have more than 10 million people, some of them are located in developing/developed countries. We have considered the top 14 megacities of the world. Due to growing industries, urbanization, vehicular density, and energy demand, greenhouse gas emissions have increased, which has degraded air quality. In some countries, clean air act has improved the air quality. We have considered multiple satellites and have retrieved atmospheric pollution parameters (aerosol optical depth-AOD and angstrom exponent) and greenhouse gases to study their variability from the period 2002-2016. High AOD represents high pollution level, which are prominent during winter and spring for Manila, Tokyo, Beijing, Moscow, Mexico City, Mumbai, Seoul, Dhaka, Cairo, and Bangkok. During summer and fall, Delhi, Karachi, and Sao Paulo have high values. During spring season, some of the megacities show significant higher pollution levels (high AOD) associated with the dust storms; however, Moscow and Karachi show contrasting behaviors. The angstrom exponent parameter has high values in the spring and summer for Manila, Shanghai, Beijing, Moscow, Sao Paulo, Mexico City, Seoul, and Cairo. Moscow shows a significant low value in April 2012. Delhi, Karachi, Mumbai, Dhaka, and Bangkok have high values in fall and winter. Dhaka shows significant low values in August 2003, June 2005, June 2008, July 2011, and June 2016. The total ozone column concentrations have high values during summer and spring, and low values during fall and winter. The methane concentrations are higher during fall and winter, and lower during spring and summer. An increasing trend of methane level is observed over all the megacities from 2002 until now. The increasing greenhouse gases in megacities have direct impact on human health and weather conditions. Some of the megacities suffer from dense haze, fog and smog, which impact the day-to-day lives of residents due to increasing concentrations of greenhouse gases.

  3. Contribution of atmospheric nitrogen deposition to diffuse pollution in a typical hilly red soil catchment in southern China.

    Science.gov (United States)

    Shen, Jianlin; Liu, Jieyun; Li, Yong; Li, Yuyuan; Wang, Yi; Liu, Xuejun; Wu, Jinshui

    2014-09-01

    Atmospheric nitrogen (N) deposition is currently high and meanwhile diffuse N pollution is also serious in China. The correlation between N deposition and riverine N export and the contribution of N deposition to riverine N export were investigated in a typical hilly red soil catchment in southern China over a two-year period. N deposition was as high as 26.1 to 55.8kgN/(ha·yr) across different land uses in the studied catchment, while the riverine N exports ranged from 7.2 to 9.6kgN/(ha·yr) in the forest sub-catchment and 27.4 to 30.3kgN/(ha·yr) in the agricultural sub-catchment. The correlations between both wet N deposition and riverine N export and precipitation were highly positive, and so were the correlations between NH4(+)-N or NO3(-)-N wet deposition and riverine NH4(+)-N or NO3(-)-N exports except for NH4(+)-N in the agricultural sub-catchment, indicating that N deposition contributed to riverine N export. The monthly export coefficients of atmospheric deposited N from land to river in the forest sub-catchment (with a mean of 14%) presented a significant positive correlation with precipitation, while the monthly contributions of atmospheric deposition to riverine N export (with a mean of 18.7% in the agricultural sub-catchment and a mean of 21.0% in the whole catchment) were significantly and negatively correlated with precipitation. The relatively high contribution of N deposition to diffuse N pollution in the catchment suggests that efforts should be done to control anthropogenic reactive N emissions to the atmosphere in hilly red soil regions in southern China. Copyright © 2014. Published by Elsevier B.V.

  4. Atmospheric dry deposition of inorganic and organic nitrogen to the Bay of Bengal: Impact of continental outflow

    Digital Repository Service at National Institute of Oceanography (India)

    Srinivas, B.; Sarin, M.M.; Sarma, V.V.S.S.

    neutralizing species in the atmosphere such as mineral aerosols and sea salts (Pakkanen, 1996). Particulate NH 4 + is derived from gaseous NH 3 , which is supplied to the atmosphere as a result of agricultural activities. Until recently, the principal... of Bengal. In IGP, biomass burning emissions (post-harvest burning of agricultural-waste) is a dominant source of pollutants. In addition, large-scale application of fertilizers (ammonia and urea based) in the agricultural dominated region represent a...

  5. Fluoride pollution of atmospheric precipitation and its relationship with air circulation and weather patterns (Wielkopolski National Park, Poland).

    Science.gov (United States)

    Walna, Barbara; Kurzyca, Iwona; Bednorz, Ewa; Kolendowicz, Leszek

    2013-07-01

    A 2-year study (2010-2011) of fluorides in atmospheric precipitation in the open area and in throughfall in Wielkopolski National Park (west-central Poland) showed their high concentrations, reaching a maximum value of 2 mg/l under the tree crowns. These high values indicate substantial deposition of up to 52 mg/m(2)/year. In 2011, over 51% of open area precipitation was characterized by fluoride concentration higher than 0.10 mg/l, and in throughfall such concentrations were found in more than 86% of events. In 2010, a strong connection was evident between fluoride and acid-forming ions, and in 2011, a correlation between phosphate and nitrite ions was seen. Analysis of available data on F(-) concentrations in the air did not show an unequivocal effect on F(-) concentrations in precipitation. To find reasons for and source areas of high fluoride pollution, the cases of extreme fluoride concentration in rainwater were related to atmospheric circulation and weather patterns. Weather conditions on days of extreme pollution were determined by movement of weather fronts over western Poland, or by small cyclonic centers with meteorological fronts. Macroscale air advection over the sampling site originated in the western quadrant (NW, W, and SW), particularly in the middle layers of the troposphere (2,500-5,000 m a.s.l.). Such directions indicate western Poland and Germany as possible sources of the pollution. At the same time in the lower troposphere, air inflow was frequently from the north, showing short distance transport from local emitters, and from the agglomeration of Poznań.

  6. Anthropogenous modifications of the atmosphere. The atmospheric ozone threat

    International Nuclear Information System (INIS)

    Aimedieu, P.

    1991-01-01

    Ozone role and atmospheric chemistry are first reviewed: chemical reactions and vertical distribution of ozone in the atmosphere. The origins of chlorofluorocarbon air pollution and the role of the various types of CFC on ozone depletion, greenhouse effect, cancer, etc. are then discussed. The political and environmental discussions concerning these phenomena are also reviewed

  7. Investigating the origin of Pb pollution in a terrestrial soil-plant-snail food chain by means of Pb isotope ratios

    Energy Technology Data Exchange (ETDEWEB)

    Notten, M.J.M. [Institute of Ecological Science, Department of System Ecology, Vrije Universiteit Amsterdam, De Boelelaan 1085, 1081 HV, Amsterdam (Netherlands)], E-mail: m.notten@nunhems.com; Walraven, N. [Faculty of Geosciences, Department of Earth Sciences/Geochemistry, University of Utrecht, Budapestlaan 4, 3508 TA Utrecht (Netherlands); Beets, C.J. [Institute of Earth Sciences, Department of Quaternary Geology and Geomorphology, Vrije Universiteit Amsterdam, De Boelelaan 1085, 1081 HV Amsterdam (Netherlands); Vroon, P. [Institute of Earth Sciences, Department of Petrology, Vrije Universiteit Amsterdam, De Boelelaan 1085, 1081 HV Amsterdam (Netherlands); Rozema, J.; Aerts, R. [Institute of Ecological Science, Department of System Ecology, Vrije Universiteit Amsterdam, De Boelelaan 1085, 1081 HV, Amsterdam (Netherlands)

    2008-06-15

    Lead isotope ratios were used to trace the origin of Pb in a soil-plant (Urtica dioica)-snail (Cepaea nemoralis) food chain in two polluted locations in the floodplains of the rivers Meuse and Rhine (Biesbosch National Park) and one reference location in the Netherlands. Lead isotope ratios and concentrations were determined in soil, litter, plant leaves, snails, rainwater and airborne particulate matter. Anthropogenic Pb in the soils of all locations was found to be derived from deposition of Pb polluted river sediments. Discharging rivers influenced the reference location before being reclaimed from the sea. The river sediment contains anthropogenic Pb from various sources related to industrial activities in the hinterland of the rivers Meuse and Rhine. Lead in the atmosphere contributed substantially to Pb pollution and Pb transfer in plant leaves and snails in all locations. Lead pollution in plant leaves and snails can be explained from a mixture of river sediment-Pb and atmospheric Pb from various transfer routes that involve low concentrations.

  8. Investigating the origin of Pb pollution in a terrestrial soil-plant-snail food chain by means of Pb isotope ratios

    International Nuclear Information System (INIS)

    Notten, M.J.M.; Walraven, N.; Beets, C.J.; Vroon, P.; Rozema, J.; Aerts, R.

    2008-01-01

    Lead isotope ratios were used to trace the origin of Pb in a soil-plant (Urtica dioica)-snail (Cepaea nemoralis) food chain in two polluted locations in the floodplains of the rivers Meuse and Rhine (Biesbosch National Park) and one reference location in the Netherlands. Lead isotope ratios and concentrations were determined in soil, litter, plant leaves, snails, rainwater and airborne particulate matter. Anthropogenic Pb in the soils of all locations was found to be derived from deposition of Pb polluted river sediments. Discharging rivers influenced the reference location before being reclaimed from the sea. The river sediment contains anthropogenic Pb from various sources related to industrial activities in the hinterland of the rivers Meuse and Rhine. Lead in the atmosphere contributed substantially to Pb pollution and Pb transfer in plant leaves and snails in all locations. Lead pollution in plant leaves and snails can be explained from a mixture of river sediment-Pb and atmospheric Pb from various transfer routes that involve low concentrations

  9. LIDAR for atmosphere research over Africa

    CSIR Research Space (South Africa)

    Sivakumar, V

    2008-11-01

    Full Text Available d’aéronomie, CNRS, Paris, France 1Email: SVenkataraman@csir.co.za – www.csir.co.za K-6665 [www.kashangroup.com] Lidar for atmospheric studies: The CSIR’s laser research into monitoring various pollutants in the lower atmosphere via... to lidar applications for atmosphere studies including pollutant monitoring. The following salient features emanated from the survey: • Around 80% of the lidars are in the northern hemisphere • Of the 20% in the southern hemisphere region...

  10. Lidar: air pollution applications

    International Nuclear Information System (INIS)

    Collis, R.T.H.

    1977-01-01

    This introduction to the use of lidar in air pollution applications is mainly concerned with its capability to detect and monitor atmospheric particulates by elastic backscattering. Even when quite imperceptible to the eye, such particulates may be detected at ranges of several kilometers even by lidars of modest performance. This capability is valuable in connection with air pollution in the following ways: by mapping and tracking inhomogeneities in particulate concentration, atmospheric structure and motion may be monitored; measurements of the optical properties of the atmosphere provide an indication of turbidity or of particulate number or mass concentrations; and the capability of obtaining at a single point return signals from remote atmospheric volumes makes it possible to make range-resolved measurements of gaseous concentration along the path by using the resonant absorption of energy of appropriate wavelengths

  11. Dust pollution of the atmosphere in the vicinity of coal-fired power plant (Omsk City, Russia)

    Science.gov (United States)

    Talovskaya, Anna V.; Raputa, Vladimir F.; Litay, Victoriya V.; Yazikov, Egor G.; Yaroslavtseva, Tatyana V.; Mikhailova, Kseniya Y.; Parygina, Irina A.; Lonchakova, Anna D.; Tretykova, Mariya I.

    2015-11-01

    The article shows the results of dust pollution level of air in the vicinity of coal-fired power plant of Omsk city on the base of study snow cover pollution. The samples were collected west-, east- and northeastwards at a distance of 0,75-6 km from the chimney for range-finding of dust emission transfer. The research findings have shown the dust load changes from 53 till 343 mg•(m2·day)-1 in the vicinity of power plant. The ultimate dust load was detected at a distance of 3-3,5 km. On the basis of asymptotics of equation solution for impurity transfer, we have made numerical analysis of dust load rate. With the usage of ground-based facilities and satellites we have determined the wind shifts in the atmospheric boundary layer have a significant impact on the field forming of long-term dustfall.

  12. Body burden of pesticides and wastewater-derived pollutants on freshwater invertebrates: Method development and application in the Danube River.

    Science.gov (United States)

    Inostroza, Pedro A; Wicht, Anna-Jorina; Huber, Thomas; Nagy, Claudia; Brack, Werner; Krauss, Martin

    2016-07-01

    While environmental risk assessment is typically based on toxicant concentrations in water and/or sediment, awareness is increasing that internal concentrations or body burdens are the key to understand adverse effects in organisms. In order to link environmental micropollutants as causes of observed effects, there is an increasing demand for methods to analyse these chemicals in organisms. Here, a multi-target screening method based on pulverised liquid extraction (PuLE) and a modified QuEChERS approach with an additional hexane phase was developed. It is capable to extract and quantify organic micropollutants of diverse chemical classes in freshwater invertebrates. The method was tested on gammarids from the Danube River (within the Joint Danube Survey 3) and target compounds were analysed by liquid chromatography-tandem mass spectrometry (LC-MS/MS). Furthermore, a non-target screening using high resolution-tandem mass spectrometry (LC-HRMS/MS) was conducted. A total of 17 pollutants were detected and/or quantified in gammarids at low concentrations. Pesticide concentrations ranged from 0.1 to 6.52 ng g(-1) (wet weight), those of wastewater-derived pollutants from 0.1 to 2.83 ng g(-1) (wet weight). The presence of wastewater-derived pollutants was prominent at all spots sampled. Using non-target screening, we could successfully identify several chlorinated compounds. These results demonstrate for the first time the presence of pesticides and wastewater-derived pollutants in invertebrates of the Danube River. Copyright © 2016 Elsevier Ltd. All rights reserved.

  13. Heavy Metal Pollution in Settled Dust Associated with Different Urban Functional Areas in a Heavily Air-Polluted City in North China

    Science.gov (United States)

    Wan, Dejun; Han, Zhangxiong; Yang, Jinsong; Yang, Guanglin; Liu, Xingqi

    2016-01-01

    Understanding variations of heavy metals in atmospheric particles between different functional areas is significant for pollution control and urban planning in cities. To reveal pollution and spatial distribution of heavy metals in atmospheric particles from different urban functional areas in Shijiazhuang in North China, 43 settled dust samples were collected over the main urban area and heavy metal concentrations were determined in their pollution indexes (IPIs) of the ten heavy metals are 2.7–13.6 (5.7 ± 2.2), suggesting high or very high pollution levels of most dust. Relatively lower IPIs occur mainly in the administration-education area, the commercial area, and other unclassified sites; while peaks occur mainly in the North Railway Station, the northeastern industrial area, and some sites near heavily trafficked areas, implying the significant influence of intensive industrial (including coal combustion) and traffic activities on atmospheric heavy metal accumulation. These results suggest a clear need of mitigating atmospheric heavy metal pollution via controlling emissions of toxic metals (especially Cd and Pb) from industrial and traffic sources in the city. PMID:27834903

  14. Heavy Metal Pollution in Settled Dust Associated with Different Urban Functional Areas in a Heavily Air-Polluted City in North China.

    Science.gov (United States)

    Wan, Dejun; Han, Zhangxiong; Yang, Jinsong; Yang, Guanglin; Liu, Xingqi

    2016-11-10

    Understanding variations of heavy metals in atmospheric particles between different functional areas is significant for pollution control and urban planning in cities. To reveal pollution and spatial distribution of heavy metals in atmospheric particles from different urban functional areas in Shijiazhuang in North China, 43 settled dust samples were collected over the main urban area and heavy metal concentrations were determined in their pollution indexes (IPIs) of the ten heavy metals are 2.7-13.6 (5.7 ± 2.2), suggesting high or very high pollution levels of most dust. Relatively lower IPIs occur mainly in the administration-education area, the commercial area, and other unclassified sites; while peaks occur mainly in the North Railway Station, the northeastern industrial area, and some sites near heavily trafficked areas, implying the significant influence of intensive industrial (including coal combustion) and traffic activities on atmospheric heavy metal accumulation. These results suggest a clear need of mitigating atmospheric heavy metal pollution via controlling emissions of toxic metals (especially Cd and Pb) from industrial and traffic sources in the city.

  15. Background Atmospheric Levels of Aldehydes, BTEX and PM10 Pollutants in a Medium-Sized City of Southern Italy

    International Nuclear Information System (INIS)

    Iovino, P.; Salvestrini, S.; Capasso, S.

    2007-01-01

    Background atmospheric levels of aldehydes, BTEX and PM10 pollutants were measured in the suburb of Caserta (Italy), 75 thousands inhabitants, 41 0 04' N, on rainless weekdays and weekends during 2005. On weekdays the average daily concentrations (μg m -3 ) were 41.6 PM10, 8.6 benzene, 25.2 toluene, 6.3 ethylbenzene, 14.0 (m+p)-xylene, 11.7 o-xylene, 6.5 formaldehyde, 3.3 acetaldehyde. All the pollutant concentrations were strictly correlated (mean correlation coefficients = 0.90). At weekends the concentrations were lower by about 1.6 times. Both on weekdays and at weekends the PM10 and benzene levels exceeded the limits set by the EU Directive 30/1999 and 69/2000, respectively

  16. [Study on emission standard system of air pollutants].

    Science.gov (United States)

    Jiang, Mei; Zhang, Guo-Ning; Zhang, Ming-Hui; Zou, Lan; Wei, Yu-Xia; Ren, Chun

    2012-12-01

    Scientific and reasonable emission standard system of air pollutants helps to systematically control air pollution, enhance the protection of the atmospheric environment effect and improve the overall atmospheric environment quality. Based on the study of development, situation and characteristics of national air pollutants emission standard system, the deficiencies of system were pointed out, which were not supportive, harmonious and perfect, and the improvement measures of emission standard system were suggested.

  17. Concentration of elements in atmospheric aerosol in Bratislava

    International Nuclear Information System (INIS)

    Meresova, J.; Florek, M.; Holy, K.; Sykora, I.; Frontasyeva, M.V.; Pavlov, S.S.

    2006-01-01

    The concentrations of 41 chemical elements (heavy metals, rare earths, and actinides) were determined in atmospheric aerosol using nuclear and related analytical techniques. The sampling location in Bratislava (Slovak Republic). The main goal of this study is the quantification of the atmospheric pollution and its trend. The elemental content in filters was measured using instrumental neutron activation analysis at IBR-2 reactor in JINR Dubna and by atomic absorption spectrometry in Bratislava. The obtained results confirm the decreasing trend of pollution by most of the heavy metals in Bratislava atmosphere, and they are compared with the contents of pollutants in atmosphere of other cities. We determined also the composition of clear filter materials. (Authors)

  18. Overview of Megacity Air Pollutant Emissions and Impacts

    Science.gov (United States)

    Kolb, C. E.

    2013-05-01

    The urban metabolism that characterizes major cities consumes very large qualities of humanly produced and/or processed food, fuel, water, electricity, construction materials and manufactured goods, as well as, naturally provided sunlight, precipitation and atmospheric oxygen. The resulting urban respiration exhalations add large quantities of trace gas and particulate matter pollutants to urban atmospheres. Key classes of urban primary air pollutants and their sources will be reviewed and important secondary pollutants identified. The impacts of these pollutants on urban and downwind regional inhabitants, ecosystems, and climate will be discussed. Challenges in quantifying the temporally and spatially resolved urban air pollutant emissions and secondary pollutant production rates will be identified and possible measurement strategies evaluated.

  19. Analysis of smoke trailers at individual classes of atmosphere stability

    International Nuclear Information System (INIS)

    Carach, V.; Macala, J.

    2007-01-01

    At the present most endangered element of the environment is currently atmosphere and its pollution that rapidly accrue. Pollutants are emitted from air pollution sources. The output of pollutant from air pollution source is creating so-called smoke screen. Smoke screens can be observed from point sources of air pollution - smokestacks, up-cast. The purpose of this article was to build theoretical models of smoke screens rise from point source at different meteorological conditions characterized with fifth classes of atmosphere stability. (authors)

  20. The washout effects of rainfall on atmospheric particulate pollution in two Chinese cities.

    Science.gov (United States)

    Guo, Ling-Chuan; Zhang, Yonghui; Lin, Hualiang; Zeng, Weilin; Liu, Tao; Xiao, Jianpeng; Rutherford, Shannon; You, Jing; Ma, Wenjun

    2016-08-01

    Though rainfall is recognized as one of the main mechanisms to reduce atmospheric particulate pollution, few studies have quantified this effect, particularly the corresponding lag effect and threshold. This study aimed to investigate the association between rainfall and air quality using a distributed lag non-linear model. Daily data on ambient PM2.5 and PM2.5-10 (particulate matter with an aerodynamic diameter less than 2.5 μm and from 2.5 to 10 μm) and meteorological factors were collected in Guangzhou and Xi'an from 2013 to 2014. A better washout effect was found for PM2.5-10 than for PM2.5, and the rainfall thresholds for both particle fractions were 7 mm in Guangzhou and 1 mm in Xi'an. The decrease in PM2.5 levels following rain lasted for 3 and 6 days in Guangzhou and Xi'an, respectively. Rainfall had a better washout effect in Xi'an compared with that in Guangzhou. Findings from this study contribute to a better understanding of the washout effects of rainfall on particulate pollution, which may help to understand the category and sustainability of dust-haze and enforce anthropogenic control measures in time. Copyright © 2016 Elsevier Ltd. All rights reserved.

  1. Early atmospheric metal pollution provides evidence for Chalcolithic/Bronze Age mining and metallurgy in Southwestern Europe

    Energy Technology Data Exchange (ETDEWEB)

    Martínez Cortizas, Antonio, E-mail: antonio.martinez.cortizas@usc.es [Departamento de Edafoloxía e Química Agrícola, Facultade de Bioloxía, Universidade de Santiago de Compostela, Campus Sur s/n, Santiago de Compostela (Spain); López-Merino, Lourdes, E-mail: lourdes.lopez-merino@brunel.ac.uk [Institute of Environment, Health and Societies, Brunel University London, UB8 3PH Uxbridge (United Kingdom); Bindler, Richard, E-mail: richard.bindler@umu.se [Department of Ecology and Environmental Science, Umeå University, Umeå (Sweden); Mighall, Tim, E-mail: t.mighall@abdn.ac.uk [Department of Geography & Environment, School of Geosciences, University of Aberdeen, Elphinstone Road, Aberdeen AB24 3UF (United Kingdom); Kylander, Malin E., E-mail: malin.kylander@geo.su.se [Department of Geological Sciences and the Bolin Centre for Climate Research, Stockholm University, SE-10691, Stockholm (Sweden)

    2016-03-01

    Although archaeological research suggests that mining/metallurgy already started in the Chalcolithic (3rd millennium BC), the earliest atmospheric metal pollution in SW Europe has thus far been dated to ~ 3500–3200 cal. yr. BP in paleo-environmental archives. A low intensity, non-extensive mining/metallurgy and the lack of appropriately located archives may be responsible for this mismatch. We have analysed the older section (> 2100 cal. yr. BP) of a peat record from La Molina (Asturias, Spain), a mire located in the proximity (35–100 km) of mines which were exploited in the Chalcolithic/Bronze Age, with the aim of assessing evidence of this early mining/metallurgy. Analyses included the determination of C as a proxy for organic matter content, lithogenic elements (Si, Al, Ti) as markers of mineral matter, and trace metals (Cr, Cu, Zn, Pb) and stable Pb isotopes as tracers of atmospheric metal pollution. From ~ 8000 to ~ 4980 cal. yr. BP the Pb composition is similar to that of the underlying sediments (Pb 15 ± 4 μg g{sup −1}; {sup 206}Pb/{sup 207}Pb 1.204 ± 0.002). A sustained period of low {sup 206}Pb/{sup 207}Pb ratios occurred from ~ 4980 to ~ 2470 cal. yr. BP, which can be divided into four phases: Chalcolithic (~ 4980–3700 cal. yr. BP), {sup 206}Pb/{sup 207}Pb ratios decline to 1.175 and Pb/Al ratios increase; Early Bronze Age (~ 3700–3500 cal. yr. BP), {sup 206}Pb/{sup 207}Pb increase to 1.192 and metal/Al ratios remain stable; Late Bronze Age (~ 3500–2800 cal. yr. BP), {sup 206}Pb/{sup 207}Pb decline to their lowest values (1.167) while Pb/Al and Zn/Al increase; and Early Iron Age (~ 2800–2470 cal. yr. BP), {sup 206}Pb/{sup 207}Pb increase to 1.186, most metal/Al ratios decrease but Zn/Al shows a peak. At the beginning of the Late Iron Age, {sup 206}Pb/{sup 207}Pb ratios and metal enrichments show a rapid return to pre-anthropogenic values. These results provide evidence of regional/local atmospheric metal pollution triggered by the

  2. Solar energy and the abatement of atmospheric emissions

    International Nuclear Information System (INIS)

    Mirasgedis, S.; Diakoulaki, D.; Assimacopoulos, D.

    1996-01-01

    In spite of the fact that solar energy is a ''clean'' energy form, gaseous pollutants are emitted during the manufacturing of the systems necessary for its utilisation. An attempt is made in this paper to estimate the level of atmospheric pollutants emitted during the successive stages which make up the manufacture process for solar water heating (SWH) systems, and to evaluate these results in comparison with the respective pollutant emission levels attributed to the generation of electricity in Greece's conventional power plants. As energy consumption is recognised as the main source of atmospheric pollution, a Life Cycle Analysis (LCA) method was applied, focusing on the most energy-consuming stages of the SWH system production process. The conclusions of the analysis indicate that the emissions of gaseous pollutants associated with the utilisation of solar energy are considerably lower than those caused by the production of electricity in conventional systems, thereby substantiating that solar energy utilisation can make a notable contribution to the abatement of atmospheric pollution. (author)

  3. The effects of short- and long-term air pollutants on plant phenology and leaf characteristics

    International Nuclear Information System (INIS)

    Jochner, Susanne; Markevych, Iana; Beck, Isabelle; Traidl-Hoffmann, Claudia

    2015-01-01

    Pollution adversely affects vegetation; however, its impact on phenology and leaf morphology is not satisfactorily understood yet. We analyzed associations between pollutants and phenological data of birch, hazel and horse chestnut in Munich (2010) along with the suitability of leaf morphological parameters of birch for monitoring air pollution using two datasets: cumulated atmospheric concentrations of nitrogen dioxide and ozone derived from passive sampling (short-term exposure) and pollutant information derived from Land Use Regression models (long-term exposure). Partial correlations and stepwise regressions revealed that increased ozone (birch, horse chestnut), NO_2, NO_x and PM levels (hazel) were significantly related to delays in phenology. Correlations were especially high when rural sites were excluded suggesting a better estimation of long-term within-city pollution. In situ measurements of foliar characteristics of birch were not suitable for bio-monitoring pollution. Inconsistencies between long- and short-term exposure effects suggest some caution when interpreting short-term data collected within field studies. - Highlights: • We present results of a field survey examining pollution effects on vegetation. • Particularly ozone was significantly associated with delays in spring phenology. • Leaf morphology of birch was found to be inadequate for bio-monitoring pollution. • Inconsistencies between long-/short-term exposure effects suggest caution. - Pollutants were significantly associated with delays in spring phenology. However, inconsistencies between long- and short-term exposure effects suggest some caution when interpreting results.

  4. Air Pollution Surveillance Systems

    Science.gov (United States)

    Morgan, George B.; And Others

    1970-01-01

    Describes atmospheric data monitoring as part of total airpollution control effort. Summarizes types of gaseous, liquid and solid pollutants and their sources; contrast between urban and rural environmental air quality; instrumentation to identify pollutants; and anticipated new non-wet chemical physical and physiochemical techniques tor cetection…

  5. Contribution to the study of the behaviour of polluted atmospheres under low β radiation rates

    International Nuclear Information System (INIS)

    Colin, J.P.

    1981-01-01

    In some cases where nuclear power plants are built in industrial areas, radiochemical impacts might occur at the same time as radiobiological impacts. These radiochemical impacts would be due to interactions between gaseous radioactive emissions and pollutants of the ambient atmosphere in these areas. Fundamental data needed for evaluating this have been brought together in this paper. The published data on air radiochemistry are discussed in detail, particularly for low radiation rates and low pollutant levels. But generally, published data appear to be plainly insufficient because of the high level of radiation rates and concentrations, particularly for NOsub(x). So the experimental study concerns nitrogen oxides mainly. Mixtures with concentration of about 1 ppmV of NO 2 , NO or SO 2 are irradiated, in a glass chamber, by β radiations from krypton 85. Mixtures are analyzed after various time lapses. The irradiation of NO and NO 2 polluted air leads to a progressive disappearance of NO and NO 2 and to the formation of a great amount of O 3 and N 2 O 5 (so the total amount of nitrogen oxides is increasing). Results can be explained with a radicalar model. With water vapor, the disappearance speed of NO and NO 2 is increased, the formation speed of O 3 is reduced. Some results of SO 2 irradiation are given [fr

  6. Coupled Human-Atmosphere-System Thinking

    Science.gov (United States)

    Schmale, Julia; Chabay, Ilan

    2014-05-01

    With the discovery of fire, humankind started changing the composition of the atmosphere. Beginning with the industrial revolution, this has led to significant environmental problems, mainly air pollution and climate change. While climate change has been recognized as one key challenge of the Anthropocene, air pollution contributes to the top causes of global premature mortality. Air pollution also plays a key role in contamination of ecosystems and bio-magnification of toxins along food chains. Even though emissions leading to air pollution and climate change often originate from the same sources, they are generally perceived and regulated separately. Climate change impacts are global and hence are tackled at an international level. Conversely, air pollution has local to regional impacts and is thus a matter of national or regional legislation. This legislative and policy divide is generally useful, since full integration could lead, for example, to detrimental delays in action against air pollution through protracted international climate negotiations. However, the separation obscures the fact that almost any kind of human activity leads to the simultaneous emission of air pollutants, toxins and long-lived greenhouse gases. The atmosphere functions as a "dump" for human generated gaseous waste, which is then dispersed and transformed, partly chemically and partly micro-physically, perturbing natural processes in the atmosphere and leading to manifold impacts. In addition, air pollutants affect the Earth's radiative balance directly and indirectly, hence affecting climate change, while a changing climate in turn affects air pollution. Current policies often neglect these linkages and favor mitigation in one arena, which sometimes has detrimental effects on the other. One example is domestic wood burning, which though nearly carbon neutral, deteriorates air quality. Moreover, the design of appliances, machinery, or infrastructure generally does not attempt to

  7. Environmental pollution in mines and its adjoining area

    International Nuclear Information System (INIS)

    Ganguly, S.; Mozumdar, T.K.; Mahajan, V.

    1998-01-01

    Atmospheric pollution depends on the type of fuel burnt, the type of industry in the locality, the weather condition and other factors. In coal fields, the chief sources of pollutants are coal and gasoline. There has been no systematic and regular survey to find out the extent of atmospheric pollution in the country. However, some works have been done by different organisations on the basis of spot detection and short-term surveys

  8. Air Pollutants Minimalization of Pollutant Absorber with Condensation System

    International Nuclear Information System (INIS)

    Ruhiat, Yayat; Wibowo, Firmanul Catur; Oktarisa, Yuvita

    2017-01-01

    Industrial development has implications for pollution, one of it is air pollution. The amount of air pollutants emitted from industrial depend on several factors which are capacity of its fuel, high chimneys and atmospheric stability. To minimize pollutants emitted from industries is created a tool called Pollutant Absorber (PA) with a condensing system. Research and Development with the approach of Design for Production was used as methodology in making PA. To test the function of PA, the simulation had been done by using the data on industrial emissions Cilegon industrial area. The simulation results in 15 years period showed that the PA was able to minimize the pollutant emissions of SO2 by 38% NOx by 37% and dust by 64%. Differences in the absorption of pollutants shows the weakness of particle separation process in the separator. This condition happen because the condensation process is less optimal during the absorption and separation in the separator. (paper)

  9. Modelling of the diffusion of pollutants in the atmosphere under varying conditions in large cultivated regions

    International Nuclear Information System (INIS)

    Wueneke, C.D.; Schultz, H.

    1975-01-01

    The most important routines of a numerical code based on the particle-in-cell-method for calculating the transport and the turbulent dispersion of inert and radio-active pollutants in the atmosphere have been programmed and have been tested successfully on the CDC computer CYBER 73/76 of the Regional Computer Centre for Niedersachsen in Hanover. Compared to the Gaussian plume model such a numerical code based on the particle-in-cell-method offers several advantages for the computation of the diffusion under varying conditions in large cultivated regions. (orig.) [de

  10. Environment, pollution and growing health hazards

    International Nuclear Information System (INIS)

    Mehmud, S.

    1987-01-01

    The atmosphere surround the planet like a mantle and compositions of atmosphere also changes. The role of high concentration in the stratosphere is vital in as much as it act as a very effective filter for absorbing ultraviolet rays. Different type of wastes that is industrial waste, domestic waste, etc. are being mixed in the environment. The procedure for monitoring pollution in the atmosphere involves the use of a laser radar (LIDAR). Laser beam is sent out in the atmosphere and point of the laser beam back-scattered by the pollutants. Aerosols to the laser radar which receives and processes it with the help of a high speed digital computer. (A.B.)

  11. Atmospheric sciences annual progress report, 1974

    International Nuclear Information System (INIS)

    Tucker, W.D.

    1975-11-01

    Activities in atmospheric sciences in the Department of Applied Science at Brookhaven National Laboratory carried out during 1974 are described. Included are contributions from the Meteorology, Atmospheric Diagnostics, Atmospheric Chemistry Research, and Atmospheric Instrumentation Groups. Programs in Meteorology reported on include diffusion from an off-shore source, plume dynamics studies, modeling of coastal effects on wind and temperature fields and pollutant distributions, effects of indoor shelter on inhalation of airborne radionuclides, chemical-dynamical interactions, techniques for determining acid-rain impact upon the ecology of the eastern U.S., and climatology. Work under Atmospheric Chemistry Research was concentrated on atmospheric aerosol studies, including formation by free radical and neutral association reactions, identification of reactive systems leading to aerosol formation, growth of sodium aerosols under atmospheric conditions and clustering reactions. Atmospheric Diagnostics presents work on field sampling and analytical technology for atmospheric pollutants, airborne sampling systems, atmospheric sulfate particulates methodology, and on a pyroturbidometric method for particulate sulfate discrimination and determination. Methodology for the use of sulfur hexafluoride in field tracer studies is discussed under Atmospheric Instrumentation. A list of publications is included

  12. Hydrocarbons and air pollution

    International Nuclear Information System (INIS)

    Herz, O.

    1992-01-01

    This paper shows the influence of hydrocarbons vapors, emitted by transports or by volatile solvents using, on air pollution. Hydrocarbons are the principal precursors of photochemical pollution. After a brief introduction on atmospheric chemistry and photochemical reactions, the author describes the french prevention program against hydrocarbons emissions. In the last chapter, informations on international or european community programs for photochemical pollution study are given. 5 figs., 10 tabs

  13. Estimating the influence of different urban canopy cover types on atmospheric particulate matter (PM10) pollution abatement in London UK.

    Science.gov (United States)

    Tallis, Matthew; Freer-Smith, Peter; Sinnett, Danielle; Aylott, Matthew; Taylor, Gail

    2010-05-01

    In the urban environment atmospheric pollution by PM10 (particulate matter with a diameter less than 10 x 10-6 m) is a problem that can have adverse effects on human health, particularly increasing rates of respiratory disease. The main contributors to atmospheric PM10 in the urban environment are road traffic, industry and power production. The urban tree canopy is a receptor for removing PM10s from the atmosphere due to the large surface areas generated by leaves and air turbulence created by the structure of the urban forest. In this context urban greening has long been known as a mechanism to contribute towards PM10 removal from the air, furthermore, tree canopy cover has a role in contributing towards a more sustainable urban environment. The work reported here has been carried out within the BRIDGE project (SustainaBle uRban plannIng Decision support accountinG for urban mEtabolism). The aim of this project is to assess the fluxes of energy, water, carbon dioxide and particulates within the urban environment and develope a DSS (Decision Support System) to aid urban planners in sustainable development. A combination of published urban canopy cover data from ground, airborne and satellite based surveys was used. For each of the 33 London boroughs the urban canopy was classified to three groups, urban woodland, street trees and garden trees and each group quantified in terms of ground cover. The total [PM10] for each borough was taken from the LAEI (London Atmospheric Emissions Inventory 2006) and the contribution to reducing [PM10] was assessed for each canopy type. Deposition to the urban canopy was assessed using the UFORE (Urban Forest Effects Model) approach. Deposition to the canopy, boundary layer height and percentage reduction of the [PM10] in the atmosphere was assessed using both hourly meterological data and [PM10] and seasonal data derived from annual models. Results from hourly and annual data were compared with measured values. The model was then

  14. Mass flows of nitrogen-containing pollutants between atmosphere and forest ecosystem. Massenfluesse stickstoffhaltiger Schadstoffe zwischen Atmosphere und Waldoekosystem

    Energy Technology Data Exchange (ETDEWEB)

    Jaeschke, W.; Grieser, J.; Herrmann, U.; Kessel, M.; Kosiol, W.; Nietzsche, I.; Sattler, T. (Frankfurt Univ. (Germany). Zentrum fuer Umweltforschung)

    1992-01-01

    In the discussion about the possible causes of novel forest decline, nitrogen-containing components in the atmosphere have received increased interest in recent years. At the Centre for Environmental Research of the University of Frankfurt, a new approach to this problem was tried within the framework of the coordinated research project Frankfurter Stadtwald. A whole number of concentrations and flows of different pollutants were used to make up a balance for the area of investigation. Where possible, all relevant concentrations and flows were to be measured or at least realistically estimated. Therefore several measuring set-ups were realized. From the compiled data, a budget of nitrogen-containing components for the area of investigation was made up. This novel approach gives an idea of the concentrations and flows of a multitude of nitrogen compounds in an ecosystem like the Frankfurter Stadtwald. These constitute a necessary basis for impact investigations by botanists to explain novel forest decline. (orig./KW) With 90 figs., 23 tabs.

  15. Modelling atmospheric transport of persistent organic pollutants in the Northern Hemisphere with a 3-D dynamical model: DEHM-POP

    Science.gov (United States)

    Hansen, K. M.; Christensen, J. H.; Brandt, J.; Frohn, L. M.; Geels, C.

    2004-03-01

    The Danish Eulerian Hemispheric Model (DEHM) is a 3-D dynamical atmospheric transport model originally developed to describe the atmospheric transport of sulphur into the Arctic. A new version of the model, DEHM-POP, developed to study the atmospheric transport and environmental fate of persistent organic pollutants (POPs) is presented. During environmental cycling, POPs can be deposited and re-emitted several times before reaching a final destination. A description of the exchange processes between the land/ocean surfaces and the atmosphere is included in the model to account for this multi-hop transport. The α-isomer of the pesticide hexachlorocyclohexane (α-HCH) is used as tracer in the model development. The structure of the model and processes included are described in detail. The results from a model simulation showing the atmospheric transport for the years 1991 to 1998 are presented and evaluated against measurements. The annual averaged atmospheric concentration of α-HCH for the 1990s is well described by the model; however, the shorter-term average concentration for most of the stations is not well captured. This indicates that the present simple surface description needs to be refined to get a better description of the air-surface exchange proceses of POPs.

  16. A field study of pollutant deposition in radiation fog

    Energy Technology Data Exchange (ETDEWEB)

    Waldman, J.M.; Jacob, D.J.; Munger, J.W.; Hoffman, M.R.

    1986-04-01

    Deposition during fog episodes can make a significant contribution to the overall flux of pollutants in certain ecosystems. Furthermore, when atmospheric stagnation prevents normal ventilation in a region, fog deposition may become the main route of pollutant removal. Fogs can consequently exert dominant control over pollutant levels in certain atmospheres. The southern San Joaquin Valley (SJV) of California is a region prone to wintertime episodes of atmospheric stagnation. These lead to elevated pollutant concentrations and/or dense, widespread fogs. Major oil-recovery operations plus widespread agricultural and livestock feeding activities are important sources of SO/sub 2/, NO/sub X/ and NH/sub 3/ in the valley. A multifaceted program of field monitoring was conducted in the SJV during the winter 1984-1985, focusing on aspects of pollutant scavenging and removal in the fog-laden atmosphere. Concentrations of major species were measured in gas, dry aerosol and fogwater phases. In addition, depositional fluxes were monitored by surrogate-surface methods. These measurements were employed to directly assess the magnitude of removal enhancement by fog.

  17. Mosses Are Better than Leaves of Vascular Plants in Monitoring Atmospheric Heavy Metal Pollution in Urban Areas.

    Science.gov (United States)

    Jiang, Yanbin; Fan, Miao; Hu, Ronggui; Zhao, Jinsong; Wu, Yupeng

    2018-05-29

    Mosses and leaves of vascular plants have been used as bioindicators of environmental contamination by heavy metals originating from various sources. This study aims to compare the metal accumulation capabilities of mosses and vascular species in urban areas and quantify the suitability of different taxa for monitoring airborne heavy metals. One pleurocarpous feather moss species, Haplocladium angustifolium , and two evergreen tree species, Cinnamomum bodinieri Osmanthus fragrans , and substrate soil were sampled in the urban area of different land use types in Wuhan City in China. The concentrations of Ag, As, Cd, Co, Cr, Cu, Mn, Mo, Ni, V, Pb, and Zn in these samples were analyzed by inductively coupled plasma mass spectrometry. The differences of heavy metals concentration in the three species showed that the moss species was considerably more capable of accumulating heavy metals than tree leaves (3 times to 51 times). The accumulated concentration of heavy metals in the moss species depended on the metal species and land use type. The enrichment factors of metals for plants and the correlations of metals in plants with corresponding metals in soil reflected that the accumulated metals in plants stemmed mostly from atmospheric deposition, rather than the substrate soil. Anthropogenic factors, such as traffic emissions from automobile transportation and manufacturing industries, were primarily responsible for the variations in metal pollutants in the atmosphere and subsequently influenced the metal accumulation in the mosses. This study elucidated that the moss species H. angustifolium is relatively more suitable than tree leaves of C. bodinieri and O. fragrans in monitoring heavy metal pollution in urban areas, and currently Wuhan is at a lower contamination level of atmospheric heavy metals than some other cities in China.

  18. Isotopic Recorders of Pollution in Heterogeneous Urban Areas

    Science.gov (United States)

    Pataki, D. E.; Cobley, L.; Smith, R. M.; Ehleringer, J. R.; Chritz, K.

    2017-12-01

    A significant difficulty in quantifying urban pollution lies in the extreme spatial and temporal heterogeneity of cities. Dense sources of both point and non-point source pollution as well as the dynamic role of human activities, which vary over very short time scales and small spatial scales, complicate efforts to establish long-term urban monitoring networks that are relevant at neighborhood, municipal, and regional scales. Fortunately, the natural abundance of isotopes of carbon, nitrogen, and other elements provides a wealth of information about the sources and fate of urban atmospheric pollution. In particular, soils and plant material integrate pollution sources and cycling over space and time, and have the potential to provide long-term records of pollution dynamics that extend back before atmospheric monitoring data are available. Similarly, sampling organic material at high spatial resolution can provide "isoscapes" that shed light on the spatial heterogeneity of pollutants in different urban parcels and neighborhoods, along roads of varying traffic density, and across neighborhoods of varying affluence and sociodemographic composition. We have compiled numerous datasets of the isotopic composition of urban organic matter that illustrate the potential for isotopic monitoring of urban areas as a means of understanding hot spots and hot moments in urban atmospheric biogeochemistry. Findings to date already reveal the critical role of affluence, economic activity, demographic change, and land management practices in influencing urban pollution sources and sinks, and suggest an important role of stable isotope and radioisotope measurements in urban atmospheric and biogeochemical monitoring.

  19. Reduction of air pollutants - a tool for control of atmospheric corrosion

    Directory of Open Access Journals (Sweden)

    Kucera, V.

    2003-12-01

    Full Text Available In most urban areas in Europe and Northern America serious corrosion impacts on buildings and cultural monuments have been caused by emissions of pollutants. The rapidly increasing pollution levels in many of the developing countries also exert a serious threat to materials. Beside the very important role of SO2 also the direct or synergistic effect of NOx and O3, the particulates and rain acidity may contribute in an important way to materials degradation. Results from extensive international field exposure programs i.e. within the UN/ECE have enabled development of dose-response relations which describe the effect of dry and wet deposition of pollutants on corrosion of different material groups. In most of the industrialized countries decreasing trends of sulphur and nitrogen pollutants and of acidity of precipitation have resulted in decreased corrosion rates. The concept of acceptable levels of pollutants is a useful tool in planning of abatement strategies and for defining of conditions for a suitable development in the field of corrosion of constructions in the atmosphere.

    La contaminación de la atmósfera ha sido la principal razón del grave deterioro de las edificaciones y de los monumentos en numerosas ciudades de Europa y Norteamérica. De otro lado, el acelerado incremento de los niveles de contaminación en los países menos desarrollados está poniendo en peligro la estabilidad de los materiales utilizados. Además del importante papel que en este sentido juega el SO2, la acción directa o el efecto sinérgico de los NOx y el O3, al igual que el material particulado y las lluvias acidas contribuyen a agravar el problema. Resultados de vastos programas internacionales de investigación como, por ejemplo, el UN/ECE, han permitido desarrollar relaciones dosis-respuesta que describen el efecto de la deposición de los contaminantes sobre la corrosión de

  20. Numerical Simulation to Air Pollution Emission Control near an Industrial Zone

    OpenAIRE

    Oyjinda, Pravitra; Pochai, Nopparat

    2017-01-01

    A rapid industrial development causes several environment pollution problems. One of the main problems is air pollution, which affects human health and the environment. The consideration of an air pollutant has to focus on a polluted source. An industrial factory is an important reason that releases the air pollutant into the atmosphere. Thus a mathematical model, an atmospheric diffusion model, is used to estimate air quality that can be used to describe the sulfur dioxide dispersion. In thi...

  1. Synthesis of octahedral like Cu-BTC derivatives derived from MOF calcined under different atmosphere for application in CO oxidation

    Science.gov (United States)

    Yang, Yiqiong; Dong, Han; Wang, Yin; He, Chi; Wang, Yuxin; Zhang, Xiaodong

    2018-02-01

    A series of octahedral structure Cu-BTC derivatives were successfully achieved through direct calcination of copper based metal organic framework Cu-BTC under different atmosphere (CO reaction gas, oxidizing gas O2, reducing gas H2, inert gas Ar). The Cu-BTC derivatives were characterized by X-ray diffraction (XRD), scanning electron microscope (SEM), transmission electron microscopy (TEM), high-resolution transmission electron microscopy (HRTEM), laser Raman spectroscopy (LRS), N2 adsorption-desorption isotherm, element analysis, H2-temperature program reduction (H2-TPR) and X-ray photoelectron spectroscopic (XPS). It is found that Cu-BTC derivative derived from MOF calcined under reaction gas/O2 (Cu-BTC-CO/Cu-BTC-O) only retain Cu2O and CuO species. In addition, a weak Cu-BTC structure and Cu particles were observed on Cu-BTC derivative derived from MOF calcined under H2 (Cu-BTC-H). Obviously differently, Cu-BTC derivative derived from MOF calcined under Ar (Cu-BTC-Ar) still retains good MOF structure. The catalytic performance for CO oxidation over Cu-BTC derivatives was studied. It was found that Cu-BTC-CO showed a smaller specific surface area (8.0 m2/g), but presented an excellent catalytic performance, long-term stability and cycling stability with a complete CO conversion temperature (T100) of 140 °C, which was ascribed to the higher Cu2O/CuO ratio, good low temperature reduction behavior and a high quantity of surface active oxygen species.

  2. E-Alerts: Environmental pollution and control (air pollution and control). E-mail newsletter

    Energy Technology Data Exchange (ETDEWEB)

    NONE

    1999-04-01

    Topics of discussion include the following: Air pollution from flue gases, exhaust gases, odors, dust, smog, microorganisms, etc.; Control techniques and equipment; Sampling and analytical techniques, and equipment; Waste gas recovery; Biological and ecological effects; Air pollution chemistry; Acid precipitation; Atmospheric motion; Laws, legislation, and regulations; Public administration; Economics; Land use.

  3. Impact of preindustrial to present-day changes in short-lived pollutant emissions on atmospheric composition and climate forcing

    Science.gov (United States)

    Naik, Vaishali; Horowitz, Larry W.; Fiore, Arlene M.; Ginoux, Paul; Mao, Jingqiu; Aghedo, Adetutu M.; Levy, Hiram

    2013-07-01

    We describe and evaluate atmospheric chemistry in the newly developed Geophysical Fluid Dynamics Laboratory chemistry-climate model (GFDL AM3) and apply it to investigate the net impact of preindustrial (PI) to present (PD) changes in short-lived pollutant emissions (ozone precursors, sulfur dioxide, and carbonaceous aerosols) and methane concentration on atmospheric composition and climate forcing. The inclusion of online troposphere-stratosphere interactions, gas-aerosol chemistry, and aerosol-cloud interactions (including direct and indirect aerosol radiative effects) in AM3 enables a more complete representation of interactions among short-lived species, and thus their net climate impact, than was considered in previous climate assessments. The base AM3 simulation, driven with observed sea surface temperature (SST) and sea ice cover (SIC) over the period 1981-2007, generally reproduces the observed mean magnitude, spatial distribution, and seasonal cycle of tropospheric ozone and carbon monoxide. The global mean aerosol optical depth in our base simulation is within 5% of satellite measurements over the 1982-2006 time period. We conduct a pair of simulations in which only the short-lived pollutant emissions and methane concentrations are changed from PI (1860) to PD (2000) levels (i.e., SST, SIC, greenhouse gases, and ozone-depleting substances are held at PD levels). From the PI to PD, we find that changes in short-lived pollutant emissions and methane have caused the tropospheric ozone burden to increase by 39% and the global burdens of sulfate, black carbon, and organic carbon to increase by factors of 3, 2.4, and 1.4, respectively. Tropospheric hydroxyl concentration decreases by 7%, showing that increases in OH sinks (methane, carbon monoxide, nonmethane volatile organic compounds, and sulfur dioxide) dominate over sources (ozone and nitrogen oxides) in the model. Combined changes in tropospheric ozone and aerosols cause a net negative top-of-the-atmosphere

  4. Pollution and Climate Change

    Science.gov (United States)

    Larr, Allison S.; Neidell, Matthew

    2016-01-01

    Childhood is a particularly sensitive time when it comes to pollution exposure. Allison Larr and Matthew Neidell focus on two atmospheric pollutants--ozone and particulate matter--that can harm children's health in many ways. Ozone irritates the lungs, causing various respiratory symptoms; it can also damage the lung lining or aggravate lung…

  5. Atmospheric pollutant and other data from the TRIDENT and tower as part of the International Decade of Ocean Exploration (IDOE) from 1972-02-01 to 1972-09-01 (NCEI Accession 7300574)

    Data.gov (United States)

    National Oceanic and Atmospheric Administration, Department of Commerce — Atmospheric pollutant and other data were collected from the TRIDENT and tower from 01 February 1972 to 01 September 1972. Data include trace metals in the...

  6. Assessment of atmospheric metallic pollution in the metropolitan region of Sao Paulo, Brazil, employing Tillandsia usneoides L. as biomonitor

    International Nuclear Information System (INIS)

    Nogueira, Claudio Ailton

    2006-01-01

    Tillandsia usneoides L. is an epiphytic bromeliad that lives on trees or other kinds of inert substrates, absorbing water and nutrients directly from the environment without roots. Due to its morphological and physiological characteristics, this species accumulates the pollutants present in the atmosphere. In the present work, Tillandsia usneoides was used as a bio monitor of metal atmospheric pollution in Sao Paulo, Brazil, which is the biggest city in South America with a population of 18 million inhabitants and a strong industrial activity. The urban area is polluted by industrial emissions but, according to the Environmental Protection Agency of the State of Sao Paulo (CETESB), the governmental agency of air quality control, regularly occurring emissions from about 7.8 million motor vehicles provide the principal source of air pollution. The Tillandsia samples were collected from an unpolluted area and were exposed bimonthly in 10 sites of the city with different pollution levels and in a control site. After exposure, trace metals were analyzed in the plant by instrumental neutron activation analysis and ICP-MS (Pb, Cd, Co, Cu, Ni, Sb e V). The results of the investigation showed a notable concentration of Co and Ni in the plants exposed in an industrial area where there is a metal processing plant, which produces about 600 tons/year of Co and 16,000 tons/year of Ni. Copper and chromium were equally distributed in industrial regions and in sites near heavy traffic avenues, suggesting that these elements can be associated to both vehicular and industrial sources. A high accumulation of Cd in the plant exposed in industrial areas indicates industrial activities as the main source of this element. For Pb, no evident sources could be identified so far as it was spread evenly along the monitoring sites. Traffic-related elements such as Zn, Ba and Sb presented high concentrations in plants exposed in sites near to heavy traffic avenues (cars, buses and trucks) and

  7. Atmospheric emissions from power plant cooling towers

    International Nuclear Information System (INIS)

    Micheletti, W.

    2006-01-01

    Power plant recirculated cooling systems (cooling towers) are not typically thought of as potential sources of air pollution. However, atmospheric emissions can be important considerations that may influence cooling tower design and operation. This paper discusses relevant U.S. environmental regulations for potential atmospheric pollutants from power plant cooling towers, and various methods for estimating and controlling these emissions. (orig.)

  8. Evaluating the uncertainties of thermal catalytic conversion in measuring atmospheric nitrogen dioxide at four differently polluted sites in China

    Science.gov (United States)

    Xu, Zheng; Wang, Tao; Xue, L. K.; Louie, Peter K. K.; Luk, Connie W. Y.; Gao, J.; Wang, S. L.; Chai, F. H.; Wang, W. X.

    2013-09-01

    A widely used method for measuring nitrogen dioxide (NO2) in the atmosphere is the conversion of NO2 to nitric oxide (NO) on the hot surface of a molybdenum oxide (MoO) catalyst followed by the chemiluminescence detection of NO. Although it has long been recognized that this type of conversion may suffer from the positive interference of other oxidized nitrogen compounds, evaluations of such interference in the atmosphere are scarce, thus rendering it difficult to make use of a large portion of the NO2 or NOx data obtained via this method (often denoted as NO2* or NOx*). In the present study, we compared the MoO converter with a selective, more accurate photolytic approach at four differently polluted sites in China. The converter worked well at the urban site, which was greatly affected by fresh emissions, but, on average, overestimated NO2 by 30%-50% at the two suburban sites and by more than 130% at the mountain-top site during afternoon hours, with a much larger positive bias seen during the top 10% of ozone events. The degree of overestimation depended on both air-parcel age and the composition of the oxidation products/intermediates of NOx (NOz). We attempted to derive an empirical formula to correct for this overestimation using concurrently measured O3, NO, and NO2* at the two suburban sites. Although the formula worked well at each individual site, the different NOz partitions at the sites made it difficult to obtain a universal formula. In view of the difficulty of assessing the uncertainties of the conventional conversion method, thus limiting the usability of data obtained via this method in atmospheric research, we suggest that, in areas away from fresh NOx emission sources, either a more selective NO2 measurement method or a NOy (NOx and its reaction products and intermediates) instrument should be adopted.

  9. [Regional atmospheric environment risk source identification and assessment].

    Science.gov (United States)

    Zhang, Xiao-Chun; Chen, Wei-Ping; Ma, Chun; Zhan, Shui-Fen; Jiao, Wen-Tao

    2012-12-01

    Identification and assessment for atmospheric environment risk source plays an important role in regional atmospheric risk assessment and regional atmospheric pollution prevention and control. The likelihood exposure and consequence assessment method (LEC method) and the Delphi method were employed to build a fast and effective method for identification and assessment of regional atmospheric environment risk sources. This method was applied to the case study of a large coal transportation port in North China. The assessment results showed that the risk characteristics and the harm degree of regional atmospheric environment risk source were in line with the actual situation. Fast and effective identification and assessment of risk source has laid an important foundation for the regional atmospheric environmental risk assessment and regional atmospheric pollution prevention and control.

  10. Modeling of atmospheric pollution at the regional scale: application to the Esquif campaign; Modelisation a l'echelle regionale de la pollution atmospherique: application a la campagne Esquif

    Energy Technology Data Exchange (ETDEWEB)

    Sarrat, C

    2003-06-01

    The Esquif experimental campaign (study and simulation of air quality in Ile-de-France (Paris region, France)) took place between 1998 and 2000 with the aim of better understanding the dynamical and chemical processes leading to atmospheric pollution peaks in Paris. The construction of a rich and diversified database (12 periods of intensive monitoring (PIM)) has been implemented with the aim of improving the existing chemical-transport models in general and air quality forecasting models in particular. In the framework of this study, the data collected during PIM 2 and 6 were used for the validation and analysis of situations of intensive pollution, simulated with the meso-scale numerical meteorological and chemical model Meso-NHC. The validation of both the dynamic fields (temperature and potential temperature, wind, height of the boundary layer) and the chemical fields (mainly O{sub 3}, NO{sub x}, NO{sub y}, PAN, isoprene) of the model allows to discuss some of the parameters of the model such as the initialization, the boundary forcing and the resolution. Then, a study of the dynamical processes allows to analyze the formation and reinforcement of the pollution conditions. Stress is put on the interaction of the regional scale processes with the photochemical pollution events. In this framework, the dynamical-chemical interaction processes are analyzed in detail, in particular when pollution levels are reinforced by the intrusion of residual ozone inside the convective boundary layer, dragged by the turbulence. Also, the impact of the urban hot island and of the urban wind on the redistribution of primary and secondary pollutants are considered. An analysis of the impact of hydrocarbons of biogenic origin on the ozone concentrations with respect to the temperature and to the presence of primary compounds has been performed for the PIM 2 and 6 of the Esquif campaign. (J.S.)

  11. Use of hydraulic and aerial mock up to study atmospheric pollution; L'utilisation des maquettes aeriennes et hydrauliques pour l'etude de la pollution atmospherique

    Energy Technology Data Exchange (ETDEWEB)

    Facy, L; Perrin De Brichambaut, C; Doury, A; Le Quinio, R

    1962-07-01

    Fundamental studies on turbulent atmospheric diffusion of finely divided particles, cannot remain on a purely theoretical basis. Further experimental studies must be considered. - In full scale, from accidental and induced releases. - On a reduced scale, in aerodynamic wind tunnels or hydraulic water tunnels. A first set of studies on reduced scale models has been worked out according to a contract between French 'Meteorologie Nationale' and French 'Commissariat a l'Energie Atomique' and with the Collaboration of Saint-Cyr 'Institut Aerotechnique'. Essentially two kinds of results have been obtained: - The mathematical model of SUTTON for the turbulent diffusion in the atmosphere, deduced from the SUTTON theory, generally used by us, has been correctly verified, qualitatively and quantitatively whenever experiments were consistent with the theory conditions. - The quantitative assays of photographic and cinematographic visualization have given precise details on the phenomena inaccessible to calculations, due to the influence of obstacles and release conditions. - Generally, it can be asserted, that the atmospheric pollution studies are worked out by mock up experimentations and that, in some cases these experiments never can be replaced by mathematically pure models. (authors) [French] Les etudes fondamentales portant sur la diffusion turbulente dans l'atmosphere de quantites de matieres finement divisees, ne peuvent se maintenir sur un plan exclusivement theorique. C'est pourquoi des etudes experimentales complementaires doivent etre obligatoirement envisagees: - en vraie grandeur, a partir d'emissions accidentelles ou provoquees; - sur modeles reduits, en soufflerie aerodynamique ou en veine hydraulique. En ce qui concerne les modeles reduits, une premiere serie d'etudes a pu etre menee a bien, dans le cadre d'un contrat passe entre la Meteorologie Nationale et le Commissariat a l'Energie Atomique, et avec la collaboration de l'Institut Aerotechnique de Saint

  12. Annual and long-term prediction of the atmospheric corrosion of metals

    International Nuclear Information System (INIS)

    Morcillo, M.

    1998-01-01

    The atmospheric corrosion of metals is known to be a discontinuous electrochemical process which takes place only when the metallic surface is wet or moistened by different meteorological phenomena (rain, humidity condensation, fog, etc.) The magnitude of atmospheric corrosion would be relatively low if it were not for the presence of certain pollutants in the atmosphere, mainly sulphur dioxide (anthropogenic pollutant) and marine chlorides (natural pollutant). The literature contains different models for predicting the atmospheric metals over short periods (generally one year) and long periods (15, 20 or more years) of atmospheric exposure. In addition to the different meteorological factors (volume of precipitation, days of rain, relative humidity (RH), T, etc.), atmospheric SO 2 deposition rate and atmospheric salinity (Cl - ) appear as independent variables in all of these models. (Author)

  13. Lead isotopes as an environmental indicator of pollution sources

    International Nuclear Information System (INIS)

    Aaberg, G.; Pacyna, J.; Stray, H.

    1997-02-01

    An interesting question when determining and quantifying pollution is the characterisation of the sources. Also, is the pollution locally derived or is it longtransported? Analyses of Pb isotope ratios and Pb concentrations on airfilter from Oslo, Norway, together with analyses of coal of different origin and wood, show that the decrease in total Pb in the first half of the 1990's is not due only to the reduction of leaded petrol but that there are other important sources for the pollution which have been cut down. The reduction in emissions from coal burning in Europe can be seen on airfilter from Oslo and also the following reduction in leaded petrol. An isotopic study of lead on airfilter from the countryside outside Oslo implies that the finer particles have been atmospherically long transported while the coarser particles are of a more local origin, e.g. from domestic burning of wood. The above results show that the use of a natural isotopic system like Pb is a powerful tool for e.g. the determination of pollution, routes of its transportation, for the monitoring of processes of the present, and for provenance determinations. 7 refs., 8 figs., 2 tabs

  14. Atmospheric composition and micro-climate in the Alhambra monument, Granada (Spain), in the context of preventive conservation

    Science.gov (United States)

    Horemans, B.; Schalm, O.; De Wael, K.; Cardell, C.; Van Grieken, R.

    2012-07-01

    The world famous Alhambra monument in Granada, Southern Spain, listed as UNESCO world cultural heritage since 1984, represents probably the most beautiful example of Islamic art and architecture from the Middle Ages in Europe. It is visited by ca. 2 million people annually. Granada is situated in a natural basin, surrounded by mountains with altitudes up to 3500 m. Due to this topography and the prevailing low wind speeds, pollution-derived and especially traffic-derived particulate matter often accumulates in the urban air. In order to evaluate the potential conservation risks from the surrounding air, the atmospheric composition in the Alhambra monument was evaluated. Indoor temperature and relative humidity fluctuations were evaluated for their potential degenerative effects. Furthermore, the atmospheric composition in the Alhambra was analyzed in terms of inorganic gases (NO2, SO2, O3, and NH3) and black carbon. It was found that the open architecture protected the indoor environments from developing a potentially harmful microclimate, such as the build-up of humidity resulting from the huge number of daily tourists. On the downside, the strong ventilation made the indoor air hardly different from outdoor air, as characterized by strong diurnal temperature and relative humidity gradients and high traffic-derived pollutant levels.

  15. Atmospheric composition and micro-climate in the Alhambra monument, Granada (Spain), in the context of preventive conservation

    International Nuclear Information System (INIS)

    Horemans, B; Schalm, O; De Wael, K; Van Grieken, R; Cardell, C

    2012-01-01

    The world famous Alhambra monument in Granada, Southern Spain, listed as UNESCO world cultural heritage since 1984, represents probably the most beautiful example of Islamic art and architecture from the Middle Ages in Europe. It is visited by ca. 2 million people annually. Granada is situated in a natural basin, surrounded by mountains with altitudes up to 3500 m. Due to this topography and the prevailing low wind speeds, pollution-derived and especially traffic-derived particulate matter often accumulates in the urban air. In order to evaluate the potential conservation risks from the surrounding air, the atmospheric composition in the Alhambra monument was evaluated. Indoor temperature and relative humidity fluctuations were evaluated for their potential degenerative effects. Furthermore, the atmospheric composition in the Alhambra was analyzed in terms of inorganic gases (NO 2 , SO 2 , O 3 , and NH 3 ) and black carbon. It was found that the open architecture protected the indoor environments from developing a potentially harmful microclimate, such as the build-up of humidity resulting from the huge number of daily tourists. On the downside, the strong ventilation made the indoor air hardly different from outdoor air, as characterized by strong diurnal temperature and relative humidity gradients and high traffic-derived pollutant levels.

  16. Air pollution and respiratory illness

    Energy Technology Data Exchange (ETDEWEB)

    Indra, G. [DIET, Uttamasolapuram, Salem (India)

    2005-07-01

    This presentation provides an overview of air pollution and impacts on public health. It provides a definition of pollution according to the Oxford English dictionary and categorizes the different types of pollution according to air, water, land and noise. It discusses air pollution and its pollutants (gaseous and particulate pollutants) as well as the diameter of the pollutant (dust, smoke, and gas). The paper also illustrates the formation of acid rain and discusses the amount of pollutants in the atmosphere per year. It presents occupational diseases, discusses radio active pollutants, respiratory illnesses as well as pollution prevention and control. The paper concluded that more research is needed to obtain information on ways to reduce the quantity of pollutants being discharged from special processes. 3 refs., 2 figs., 2 tabs.

  17. Impact Assessment of Atmospheric Pollutants Emissions from ...

    African Journals Online (AJOL)

    Michael

    2016-12-02

    Dec 2, 2016 ... Pollutants Emissions from Mining Operations at Ghana Managanese Company Ltd.”, Ghana Mining Journal, ..... Mexico Institute of Mining and Technology, ... Management, Arsenic Sequestration, and Water Quality Issues.

  18. Meteorological Drivers of Extreme Air Pollution Events

    Science.gov (United States)

    Horton, D. E.; Schnell, J.; Callahan, C. W.; Suo, Y.

    2017-12-01

    The accumulation of pollutants in the near-surface atmosphere has been shown to have deleterious consequences for public health, agricultural productivity, and economic vitality. Natural and anthropogenic emissions of ozone and particulate matter can accumulate to hazardous concentrations when atmospheric conditions are favorable, and can reach extreme levels when such conditions persist. Favorable atmospheric conditions for pollutant accumulation include optimal temperatures for photochemical reaction rates, circulation patterns conducive to pollutant advection, and a lack of ventilation, dispersion, and scavenging in the local environment. Given our changing climate system and the dual ingredients of poor air quality - pollutants and the atmospheric conditions favorable to their accumulation - it is important to characterize recent changes in favorable meteorological conditions, and quantify their potential contribution to recent extreme air pollution events. To facilitate our characterization, this study employs the recently updated Schnell et al (2015) 1°×1° gridded observed surface ozone and particulate matter datasets for the period of 1998 to 2015, in conjunction with reanalysis and climate model simulation data. We identify extreme air pollution episodes in the observational record and assess the meteorological factors of primary support at local and synoptic scales. We then assess (i) the contribution of observed meteorological trends (if extant) to the magnitude of the event, (ii) the return interval of the meteorological event in the observational record, simulated historical climate, and simulated pre-industrial climate, as well as (iii) the probability of the observed meteorological trend in historical and pre-industrial climates.

  19. Air pollution in the Slovak Republic, 2004

    International Nuclear Information System (INIS)

    Mitosinkova, M.; Kozakovic, L.; Zavodsky, D.; Sajtakova, E.; Szemesova, J.; Pukancikova, K.

    2006-01-01

    A report on air quality and contribution of individual sources on its pollution in the Slovak Republic in 2004 is presented. This report consists of two parts: (1) Pollutants part and (2) Emission part. Pollutants part is divided into the following chapters: Regional air pollution and quality of precipitation; Local air pollution; Atmospheric ozone. Emission part is divided into the following chapters: Inventory control of emissions and sources of pollution, Emission of greenhouse gases

  20. Air pollution in the Slovak Republic, 2003

    International Nuclear Information System (INIS)

    Mitosinkova, M.; Kozakovic, L.; Zavodsky, D.; Sajtakova, E.; Szemesova, J.; Pukancikova, K.

    2005-01-01

    A report on air quality and contribution of individual sources on its pollution in the Slovak Republic in 2003 is presented. This report consists of two parts: (1) Pollutants part and (2) Emission part. Pollutants part is divided into the following chapters: Regional air pollution and quality of of precipitation; Local air pollution; Atmospheric ozone. Emission part is divided into the following chapters: Inventory control of emissions and sources of pollution, Emission of greenhouse gases

  1. Detecting atmospheric pollution in surface soils using magnetic measurements: A reappraisal using an England and Wales database

    International Nuclear Information System (INIS)

    Blundell, A.; Hannam, J.A.; Dearing, J.A.; Boyle, J.F.

    2009-01-01

    Industrial activity such as burning of fossil fuels produces magnetically enhanced particulates. These particulates consist of coarse-grained multidomain and stable single domain magnetic minerals. Two threshold values of low field magnetic susceptibility (χ LF ) and frequency dependent susceptibility percentage (χ FD %) discriminate ferrimagnetic minerals of these sizes and can act as a tracer of magnetic pollution. Application of the thresholds to a magnetic topsoil data set (n = 5656 across England and Wales) revealed 637 samples potentially dominated by pollution particulates. The magnetic parameters of these samples display a negative correlation with distance to urban areas and positive correlations with metals associated with anthropogenic activity (Cu, Pb, and Zn). Results of experimentation with threshold values and modelling of magnetic anomalies suggest that regional factors such as geology and potential for pedogenic secondary magnetic enhancement should be considered when setting threshold values. - An application of magnetic susceptibility and frequency dependent susceptibility thresholds across England and Wales to determine topsoil dominated by pollution derived particles.

  2. Occurrence of quaternary ammonium compounds (QACs) and their application as a tracer for sewage derived pollution in urban estuarine sediments

    International Nuclear Information System (INIS)

    Li, Xiaolin; Luo, Xiaojun; Mai, Bixian; Liu, Jingqin; Chen, Li; Lin, Shanshan

    2014-01-01

    Particle reactive organic contaminants in estuarine sediments can lead to various environmental problems affecting ecosystem and public health. In this study, the occurrence and homologous distribution pattern of quaternary ammonium compounds (QACs) in the surficial sediments collected from the Pearl River Estuary (PRE), China were examined along with polychlorinated biphenyls (PCBs) and polybrominated diphenylethers (PBDEs). The composition pattern of the QACs was found to be uniform in most of the sediments analyzed throughout the PRE, and the average composition pattern was identical to that determined in the sewage sludge from Guangzhou, the biggest city in the PRE. Dialkyldimethylammonium compounds, the most abundant type of QACs, positively correlated to the total concentrations of PCBs and PBDEs in most of the sediments with similar composition patterns. Therefore, the QACs are proposed as potential tracers to evaluate the transport of sewage-derived pollution in estuarine environments. -- Highlights: • Analysis method is developed for quaternary ammonium compounds (QACs) in sediment. • Occurrence of QACs is observed in the Pearl River Estuary, China for the first time. • QACs are proposed to be a tracer for sewage derived pollution in estuarine sediment. -- QACs were found to be present in the estuarine sediments in China for the first time and proposed as potential tracers for sewage-derived pollution in urban estuary

  3. Modeling of hazardous air pollutant removal in the pulsed corona discharge

    International Nuclear Information System (INIS)

    Derakhshesh, Marzie; Abedi, Jalal; Omidyeganeh, Mohammad

    2009-01-01

    This study investigated the effects of two parts of the performance equation of the pulsed corona reactor, which is one of the non-thermal plasma processing tools of atmospheric pressure for eliminating pollutant streams. First, the effect of axial dispersion in the diffusion term and then the effect of different orders of the reaction in the decomposition rate term were considered. The mathematical model was primarily developed to predict the effluent concentration of the pulsed corona reactor using mass balance, and considering axial dispersion, linear velocity and decomposition rate of pollutant. The steady state form of this equation was subsequently solved assuming different reaction orders. For the derivation of the performance equation of the reactor, it was assumed that the decomposition rate of the pollutant was directly proportional to discharge power and the concentration of the pollutant. The results were validated and compared with another predicted model using their experimental data. The model developed in this study was also validated with two other experimental data in the literature for N 2 O

  4. Atmospheric concentrations of persistent organic pollutants over the Pacific Ocean near southern Taiwan and the northern Philippines.

    Science.gov (United States)

    Chao, How-Ran; Lin, Ding-Yan; Chen, Kuang-Yu; Gou, Yan-Yu; Chiou, Tsyr-Huei; Lee, Wen-Jhy; Chen, Shui-Jen; Wang, Lin-Chi

    2014-09-01

    This study investigates the atmospheric occurrence of persistent organic pollutants (POPs) over the Pacific Ocean near southern Taiwan and the northern Philippines. We determined sixty-six compounds, including polychlorinated dibenzo-p-dioxins and dibenzofurans (PCDD/Fs), dioxin-like polychlorinated biphenyls (DLPCBs), polybrominated diphenyl ethers (PBDEs), as well as polychlorinated diphenyl ethers (PCDEs), polybrominated dibenzo-p-dioxins and dibenzofurans (PBDD/Fs), and polybrominated biphenyls (PBBs), in air samples simultaneously collected from the offshore oceanic atmosphere (n=6) and over a rural area (n=2). We calculated the atmospheric World Health Organization 2005 toxic equivalency levels (WHO2005-TEQ), for the total dioxin-like POPs, including PCDD/Fs, DLPCBs, and PBDD/Fs, being 0.00612 pg WHO2005-TEQ/m(3) and 0.0138 pg WHO2005-TEQ/m(3) over the ocean and land, respectively. We found unexpected lower averaged atmospheric PBDE concentrations in the rural area (15.9 pg/m(3)) than over the ocean (31.1 pg/m(3)) due to higher levels of the BDE209 congener, although the difference was not statistically significant. We have compared and reported our field results with previously published datasets over the global oceans, which suggest PCBs and PBDEs are the dominant chemical contaminants in the global oceanic atmosphere among these halogenated POPs (e.g. PCBs and Σdi-hepta PBDEs could be found in the range of 0.09-48.7 and 8.07-94.0 pg/m(3), respectively, including our dataset). However, there are still very few investigations on the global atmospheric levels of PBDD/Fs, PCDEs and PBBs and our data sums to these earlier studies. Finally, we point out that the halogenated POPs originated from Taiwan or the continental East Asia which could easily reach remote ocean sites via atmospheric transport. Copyright © 2014 Elsevier B.V. All rights reserved.

  5. Assessment of social losses of pollution's health caused by man-made pollution of atmospheric air with emissions of particulate matters (PM10

    Directory of Open Access Journals (Sweden)

    Turos Ye.I.

    2017-04-01

    Full Text Available According to available estimates, about 3% of lethal outcomes from cardiac-pulmonary pathology and 5% from lung cancer are related to the impact of patriculate matters (PM. In the course of the study there were assessed social losses of population’s health (additional death cases caused by risk conditions of atmospheric air pollution with PM of various air-dynamic diameter (PM10, proper to emissions of various industrial enterprises. It was established that 90% of population of cities under study live under high exposures (≥50 µg/m3 health and risks for population (IRM=10-3÷10-4, caused by PM10 emissions. Results showed that metallurgical industry is responsible for 7,2 to 2193 additional mortality cases. The impact of machine building enterprises – from 0.06 to 21 cases; coke and chemical – from 1.5 to 36 cases; mining – from 1.1 to 14,6 cases. The findings revealed 0.6 % increase in lifetime mortality for each 10 µg/m3 in 24-hour average PM10 concentration. Based on research outcomes, a set of instruments was developed for implementation of air pollution risk management programs aimed at mitigation of health risks from (PM10 in highly exposed groups.

  6. Pollutant transformations over Lake Michigan

    International Nuclear Information System (INIS)

    Alkezweeny, A.J.; Arbuthnot, D.R.; Busness, K.M.; Easter, R.C.; Hales, J.M.; Lee, R.N.; Young, J.M.

    1979-01-01

    An aircraft, a chartered boat, and a constant altitude balloon were used to study pollutant transformations over Lake Michigan in a Lagrangian frame of reference. The experiments were conducted during the summer under strong atmospheric stability where diffusion and dry deposition of pollutants can be neglected

  7. Assessment of the Atmospheric Suspended Particles Pollution in the Madrid Air Quality Networks

    International Nuclear Information System (INIS)

    Salvador, P.; Artinano, B.

    2000-01-01

    Suspended particles are a very complex type of atmospheric pollution because of their chemical composition and size. In fact, there are a quite high number of particles sources which are linked to different physicochemical processes that determine their size. At present particles smaller than 10 μm are considered the most dangerous, as has been recently pointed out by numerous epidemiologic studies. In this way, more restrictive concentration limit values have been approved in the EU countries, so an assessment of present airborne concentration values and the sources apportionment in their most representative areas is needed. In the Madrid Community a first approaching of these and other aims, has been carried out from an analysis of the Madrid Air Quality networks data. This will contribute to the establishment of concentration levels abatement strategies. (Author) 111 refs

  8. A campaign to study atmospheric pollution at the regional scale: the Escompte programme; Une experience d'etude de la pollution atmospherique a l'echelle regionale. Le programme Escompte

    Energy Technology Data Exchange (ETDEWEB)

    Durand, P. [Meteo-France - Centre National de Recherches Meteorologiques, Centre National de la Recherche Scientifique (CNRS URA 1357), 31 - Toulouse (France); Cros, B. [Observatoire Midi-Pyrenees, Lab. d' Aerologie, Centre National de la Recherche Scientifique (CNRS UMR 5560), 31 - Toulouse (France)

    2004-02-01

    The Escompte programme was set up to improve and validate regional scale chemistry-transport numerical models. During summer 2001, an ambitious field campaign collected data on the meteorological and chemical parameters of the atmosphere during some photo-oxidant pollution events. Performed in the region of Marseille city and Berre lake, this campaign deployed a huge quantity of instruments, and constitutes one of the major operations in this field. (authors)

  9. [Impact of atmospheric total suspended particulate pollution on photosynthetic parameters of street mango trees in Xiamen City].

    Science.gov (United States)

    Yu, Yu-xian; Chen, Jin-sheng; Ren, Yin; Li, Fang-yi; Cui, Sheng-hui

    2010-05-01

    With the development of urbanization, total suspended particulate (TSP) pollution is getting serious, and the normal physiological processes of urban vegetation are profoundly affected while adsorbing and purifying the particulates. In this study, four areas were selected, i.e., Tingxi reservoir (clean control area), Xiamen University (cultural and educational area), Xianyue (business area), and Haicang (industrial area), with their atmospheric TSP concentrations and the photosynthetic parameters of street Mango (Mangifera indica) trees monitored in April and May, 2009. The daily average concentration of TSP in Tingxi, Xiamen University, Xianyue, and Haicang was 0.061, 0.113, 0.120 and 0.205 mg x m(-3), respectively, and the impact of TSP stress on M. indica was in the sequence of Haicang > Xianyue > Xiamen University > Tingxi. TSP pollution negatively affected the net photosynthetic rate, stomatal conductance, and transpiration rate of M. indica, and induced intercellular CO2 concentration changed significantly. High TSP concentration could cause the decline of net photosynthetic rate via stomatal limitation.

  10. Monitoring and inventorying of the pollutant emissions from thermal power plants

    International Nuclear Information System (INIS)

    Vladescu, Gherghina; Iordache, Daniela; Iordache, Victorita; Ciomaga, Carmencita; Matei, Magdalena; Ilie, Ion; Motiu, Cornel

    2001-01-01

    Pollution due to emissions discharged in atmosphere as a result of human (anthropogenic) activities and the related environmental effects, such as acid depositions, land quality degradation, global warming/climate changes, building degradation, ozone layer depletion required the monitoring and inventorying of the polluting emissions at the local, regional and global levels. The paper briefly presents the international requirements concerning the development of a polluting emission inventory, the European methodologies for air polluting emission inventorying, programs and methodologies used in the Romanian electricity production sector for inventorying the polluting emissions and calculation of the dispersion of the pollutants discharged in the atmosphere. (author)

  11. Errors in spectroscopic measurements of SO2 due to nonexponential absorption of laser radiation, with application to the remote monitoring of atmospheric pollutants

    International Nuclear Information System (INIS)

    Brassington, D.J.; Moncrieff, T.M.; Felton, R.C.; Jolliffe, B.W.; Marx, B.R.; Rowley, W.R.C.; Woods, P.T.

    1984-01-01

    Methods of measuring the concentration of atmospheric pollutants by laser absorption spectroscopy, such as differential absorption lidar (DIAL) and integrated long-path techniques, all rely on the validity of Beer's exponential absorption law. It is shown here that departures from this law occur if the probing laser has a bandwidth larger than the wavelength scale of structure in the absorption spectrum of the pollutant. A comprehensive experimental and theoretical treatment of the errors resulting from these departures is presented for the particular case of SO 2 monitoring at approx.300 nm. It is shown that the largest error occurs where the initial calibration measurement of absorption cross section is made at low pressure, in which case errors in excess of 5% in the cross section could occur for laser bandwidths >0.01 nm. Atmospheric measurements by DIAL or long-path methods are in most cases affected less, because pressure broadening smears the spectral structure, but when measuring high concentrations errors can exceed 5%

  12. Resonance Raman imaging as a tool to assess the atmospheric pollution level: carotenoids in Lecanoraceae lichens as bioindicators.

    Science.gov (United States)

    Ibarrondo, I; Prieto-Taboada, N; Martínez-Arkarazo, I; Madariaga, J M

    2016-04-01

    Raman spectroscopy differentiation of carotenoids has traditionally been based on the ν 1 position (C = C stretching vibrations in the polyene chain) in the 1500-1600 cm(-1) range, using a 785 nm excitation laser. However, when the number of conjugated double bonds is similar, as in the cases of zeaxanthin and β-carotene, this distinction is still ambiguous due to the closeness of the Raman bands. This work shows the Raman results, obtained in resonance conditions using a 514 mm laser, on Lecanora campestris and Lecanora atra species, which can be used to differentiate and consequently characterize carotenoids. The presence of the carotenoid found in Lecanoraceae lichens has been demonstrated to depend on the atmospheric pollution level of the environment they inhabit. Astaxanthin, a superb antioxidant, appears as the principal xanthophyll in highly polluted sites, usually together with the UV screening pigment scytonemin; zeaxanthin is the major carotenoid in medium polluted environments, while β-carotene is the major carotenoid in cleaner environments. Based on these observations, an indirect classification of the stress suffered in a given environment can be assessed by simply analysing the carotenoid content in the Lecanoraceae lichens by using resonance Raman imaging.

  13. Dating Antarctic soils using atmosphere-derived 10Be and nitrate

    International Nuclear Information System (INIS)

    Graham, I.J.; Ditchburn, R.G.; Claridge, G.G.C.; Whitehead, N.E.; Zondervan, A.; Sheppard, D.S.

    2002-01-01

    Because they are slow forming, Antarctic soils have the potential to yield considerable climatic information from the past c.20 m.y. However, these soils have proved difficult to date absolutely by conventional means. Here we present a novel approach to the problem, based on atmosphere-derived 10 Be and nitrate contents. In situations where medium to long term deposition rates can be reasonably estimated from ice core data, the total nitrate inventory in an Antarctic soil can place constraints on its formation age. 10 Be radioactive decay may then be used, assuming steady state equilibrium, to further refine the age profile. We have applied such models to a complex soil from the Taylor Valley region in South Victoria Land, deriving an overall nitrate inventory age of c. 18 Ma, and 10 Be decay ages for the upper and middle layers of c.15 and c.17 Ma, respectively. These results are consistent with the >10 Ma age of the soil deduced from stratigraphic and geomorphological information. (author). 28 refs., 4 figs., 2 tabs

  14. First retrieval of hourly atmospheric radionuclides just after the Fukushima accident by analyzing filter-tapes of operational air pollution monitoring stations.

    Science.gov (United States)

    Tsuruta, Haruo; Oura, Yasuji; Ebihara, Mitsuru; Ohara, Toshimasa; Nakajima, Teruyuki

    2014-10-22

    No observed data have been found in the Fukushima Prefecture (FP) for the time-series of atmospheric radionuclides concentrations just after the Fukushima Daiichi Nuclear Power Plant (FD1NPP) accident. Accordingly, current estimates of internal radiation doses from inhalation, and atmospheric radionuclide concentrations by atmospheric transport models are highly uncertain. Here, we present a new method for retrieving the hourly atmospheric (137)Cs concentrations by measuring the radioactivity of suspended particulate matter (SPM) collected on filter tapes in SPM monitors which were operated even after the accident. This new dataset focused on the period of March 12-23, 2011 just after the accident, when massive radioactive materials were released from the FD1NPP to the atmosphere. Overall, 40 sites of the more than 400 sites in the air quality monitoring stations in eastern Japan were studied. For the first time, we show the spatio-temporal variation of atmospheric (137)Cs concentrations in the FP and the Tokyo Metropolitan Area (TMA) located more than 170 km southwest of the FD1NPP. The comprehensive dataset revealed how the polluted air masses were transported to the FP and TMA, and can be used to re-evaluate internal exposure, time-series radionuclides release rates, and atmospheric transport models.

  15. First retrieval of hourly atmospheric radionuclides just after the Fukushima accident by analyzing filter-tapes of operational air pollution monitoring stations

    Science.gov (United States)

    Tsuruta, Haruo; Oura, Yasuji; Ebihara, Mitsuru; Ohara, Toshimasa; Nakajima, Teruyuki

    2014-01-01

    No observed data have been found in the Fukushima Prefecture (FP) for the time-series of atmospheric radionuclides concentrations just after the Fukushima Daiichi Nuclear Power Plant (FD1NPP) accident. Accordingly, current estimates of internal radiation doses from inhalation, and atmospheric radionuclide concentrations by atmospheric transport models are highly uncertain. Here, we present a new method for retrieving the hourly atmospheric 137Cs concentrations by measuring the radioactivity of suspended particulate matter (SPM) collected on filter tapes in SPM monitors which were operated even after the accident. This new dataset focused on the period of March 12–23, 2011 just after the accident, when massive radioactive materials were released from the FD1NPP to the atmosphere. Overall, 40 sites of the more than 400 sites in the air quality monitoring stations in eastern Japan were studied. For the first time, we show the spatio-temporal variation of atmospheric 137Cs concentrations in the FP and the Tokyo Metropolitan Area (TMA) located more than 170 km southwest of the FD1NPP. The comprehensive dataset revealed how the polluted air masses were transported to the FP and TMA, and can be used to re-evaluate internal exposure, time-series radionuclides release rates, and atmospheric transport models. PMID:25335435

  16. Hazardous gas treatment by atmospheric discharges

    International Nuclear Information System (INIS)

    Mizeraczyk, J.

    2005-01-01

    The emissions of NO x ; SO x , CO 2 and volatile organic compounds (VOCs) including fluorocarbons to the atmosphere influence heavily our environment, NO x and SO x emitted to the atmosphere are the major cause of acid rains, while CO 2 and VOCs emissions cause the greenhouse effect which leads to abnormal global heating of the atmosphere and creating in a temperature inversion layer that traps gaseous pollutants. Therefore, there is an increasing interest in controlling these emissions. A new technique, which uses the plasma processes induced by energetic electrons, emerges as one of the most effective methods of reducing concentrations of the emitted gaseous pollutants. Various plasma techniques have been tested for gaseous pollution control. The electron bean irradiation was found to be physically and economically efficient for NO x and SO x reduction in the exhaust gases from electrical and heat power plants. The capability of the non-thermal plasmas, produced in atmospheric pressure electrical discharges, for decomposition of the gaseous pollutants has been widely tested. These atmospheric pressure electrical discharges are dielectric barrier discharges, pulsed and de corona discharges (in the reactors with the point-to-plate, wire-cylinder and wire-plate geometries, in the reactors with flow stabilized corona torch and corona radical shower), gliding discharges, inductively coupled high-frequency discharges, ac surface discharges, ac discharges in the packed bed reactors, and microwave torch discharges. In this paper, after reviewing the methods and devices used for producing the non-thermal plasmas for gaseous pollutant control, some results of the laboratory experiments on the plasmas abatement of NO x ; SO x and various VOCs will be presented, followed by a discussion on the energy efficiency and by-products. Also some results obtained in the pilot-plants will be given. finally other possible applications of the presented plasma devices for controlling

  17. Urban atmospheric contamination

    International Nuclear Information System (INIS)

    Baldasano Jose, M.

    1997-01-01

    The problems of contamination are not only limited to this century, pale pathology evidences of the effects of the contamination of the air exist in interiors in the health of the old ones; the article mention the elements that configure the problem of the atmospheric contamination, atmospheric pollutants and emission sources, orography condition and effects induced by the urbanization process

  18. To a scientific substantiation of a practical method of inspection of radiating conditions on territories, polluted with atmospheric fallout

    International Nuclear Information System (INIS)

    Burmistrov, V.R; Makarenko, N.G.; Karimova, L.M.

    2001-01-01

    Full text: In the report a question on necessity of practical development of a method of inspection of radiating fields, adapted to a nature of pollution is put. 50-year study of radionuclides pollution, dropping out from atmosphere after nuclear tests or failures, have shown non-perspective of traditional techniques of inspection of a radiating conditions on large territories. The detailed measurements covering surface without gaps are very expensive, and use of a unloaded grid requires interpolation irregular mosaic structure. Detection Fractal structure at the analysis Chernobyl losses and pollution of fragments of Semipalatinsk test nuclear site specify necessity of the account of self-similar properties of pollution in philosophy of measurement. For realization of potential opportunities Fractal field the special circuit of measurements, distinguished from, is required standard. Fractal approach requires shooting with system of crossed vicinities on chosen detailed platforms, making a rather small part of surveyed territory. These data will allow to reveal scale laws, which are universal in a significant range of scales. Using scaling of small platforms, it is possible to receive correct estimation of structure of pollution of large territories. The stated above reasons are based on our experiments on fractal approach to the analysis of continuous shooting (aero-scale shooting of scale 1:5000) in a zone of Semipalatinsk test site on three platforms by the sizes on 1000x400 m 2 . Our results specify necessity revision almost of all conclusions, received earlier on the basis of traditional techniques

  19. Atmospheric mercury pollution around a chlor-alkali plant in Flix (NE Spain): an integrated analysis.

    Science.gov (United States)

    Esbrí, José M; López-Berdonces, Miguel Angel; Fernández-Calderón, Sergio; Higueras, Pablo; Díez, Sergi

    2015-04-01

    An integrated analysis approach has been applied to a mercury (Hg) case study on a chlor-alkali plant located in the Ebro River basin, close to the town of Flix (NE Spain). The study focused on atmospheric Hg and its incorporation in soils and lichens close to a mercury cell chlor-alkali plant (CAP), which has been operating since the end of the 19th century. Atmospheric Hg present in the area was characterized by means of seven total gaseous mercury (TGM) surveys carried out from 2007 to 2012. Surveys were carried out by car, walking, and at fixed locations, and covered an area of some 12 km(2) (including the CAP area, the village in which workers live, Flix town, and the Sebes Wildlife Reserve). Finally, an atmospheric Hg dispersion model was developed with ISC-AERMOD software validated by a lichen survey of the area. The results for the atmospheric compartment seem to indicate that the Flix area currently has the highest levels of Hg pollution in Spain on the basis of the extremely high average concentrations in the vicinity of the CAP (229 ng m(-3)). Moreover, the Hg(0) plume affects Flix town center to some extent, with values well above the international thresholds for residential areas. Wet and dry Hg deposition reached its highest values on the banks of the Ebro River, and this contributes to increased soil contamination (range 44-12,900 ng g(-1), average 775 ng g(-1)). A good fit was obtained between anomalous areas indicated by lichens and the dispersion model for 1 year.

  20. The acid-catalyzed hydrolysis of an α-pinene-derived organic nitrate: kinetics, products, reaction mechanisms, and atmospheric impact

    Science.gov (United States)

    Rindelaub, Joel D.; Borca, Carlos H.; Hostetler, Matthew A.; Slade, Jonathan H.; Lipton, Mark A.; Slipchenko, Lyudmila V.; Shepson, Paul B.

    2016-12-01

    The production of atmospheric organic nitrates (RONO2) has a large impact on air quality and climate due to their contribution to secondary organic aerosol and influence on tropospheric ozone concentrations. Since organic nitrates control the fate of gas phase NOx (NO + NO2), a byproduct of anthropogenic combustion processes, their atmospheric production and reactivity is of great interest. While the atmospheric reactivity of many relevant organic nitrates is still uncertain, one significant reactive pathway, condensed phase hydrolysis, has recently been identified as a potential sink for organic nitrate species. The partitioning of gas phase organic nitrates to aerosol particles and subsequent hydrolysis likely removes the oxidized nitrogen from further atmospheric processing, due to large organic nitrate uptake to aerosols and proposed hydrolysis lifetimes, which may impact long-range transport of NOx, a tropospheric ozone precursor. Despite the atmospheric importance, the hydrolysis rates and reaction mechanisms for atmospherically derived organic nitrates are almost completely unknown, including those derived from α-pinene, a biogenic volatile organic compound (BVOC) that is one of the most significant precursors to biogenic secondary organic aerosol (BSOA). To better understand the chemistry that governs the fate of particle phase organic nitrates, the hydrolysis mechanism and rate constants were elucidated for several organic nitrates, including an α-pinene-derived organic nitrate (APN). A positive trend in hydrolysis rate constants was observed with increasing solution acidity for all organic nitrates studied, with the tertiary APN lifetime ranging from 8.3 min at acidic pH (0.25) to 8.8 h at neutral pH (6.9). Since ambient fine aerosol pH values are observed to be acidic, the reported lifetimes, which are much shorter than that of atmospheric fine aerosol, provide important insight into the fate of particle phase organic nitrates. Along with rate constant

  1. Validation of Atmospheric Water Vapor Derived from Ship-Borne GPS Measurements in the Chinese Bohai Sea

    Directory of Open Access Journals (Sweden)

    Shi-Jie Fan

    2016-04-01

    Full Text Available Atmospheric water vapor (AWV was investigated for the first time in the Chinese Bohai Sea using a Global Positioning System (GPS receiver aboard a lightweight (300-ton ship. An experiment was conducted to retrieve the AWV using the state-of-the-art GPS precise point positioning (PPP technique. The effects of atmospheric weighted mean temperature model and zenith wet delay constraint on GPS AWV estimates were discussed in the PPP estimation system. The GPS-derived precipitable water vapor (PWV and slant-path water vapor (SWV were assessed by comparing with those derived from the Fifth Generation NCAR/Penn State Mesoscale Model (MM5. The results showed the PWV and SWV differences between those derived from both GPS and MM5 are 1.5 mm root mean square (RMS with a bias of 0.2 and 3.9 mm RMS with a bias of -0.7 mm respectively. These good agreements indicate that the GPS-derived AWV in dynamic environments has a comparable accuracy with that of the MM5 model. This suggests that high accuracy and high spatio-temporal resolution humidity fields can be obtained using GPS in the Chinese Bohai Sea, which offers significant potential for meteorological applications and climate studies in this region.

  2. Modeling of atmospheric pollution at the regional scale: application to the Esquif campaign; Modelisation a l'echelle regionale de la pollution atmospherique: application a la campagne Esquif

    Energy Technology Data Exchange (ETDEWEB)

    Sarrat, C.

    2003-06-01

    The Esquif experimental campaign (study and simulation of air quality in Ile-de-France (Paris region, France)) took place between 1998 and 2000 with the aim of better understanding the dynamical and chemical processes leading to atmospheric pollution peaks in Paris. The construction of a rich and diversified database (12 periods of intensive monitoring (PIM)) has been implemented with the aim of improving the existing chemical-transport models in general and air quality forecasting models in particular. In the framework of this study, the data collected during PIM 2 and 6 were used for the validation and analysis of situations of intensive pollution, simulated with the meso-scale numerical meteorological and chemical model Meso-NHC. The validation of both the dynamic fields (temperature and potential temperature, wind, height of the boundary layer) and the chemical fields (mainly O{sub 3}, NO{sub x}, NO{sub y}, PAN, isoprene) of the model allows to discuss some of the parameters of the model such as the initialization, the boundary forcing and the resolution. Then, a study of the dynamical processes allows to analyze the formation and reinforcement of the pollution conditions. Stress is put on the interaction of the regional scale processes with the photochemical pollution events. In this framework, the dynamical-chemical interaction processes are analyzed in detail, in particular when pollution levels are reinforced by the intrusion of residual ozone inside the convective boundary layer, dragged by the turbulence. Also, the impact of the urban hot island and of the urban wind on the redistribution of primary and secondary pollutants are considered. An analysis of the impact of hydrocarbons of biogenic origin on the ozone concentrations with respect to the temperature and to the presence of primary compounds has been performed for the PIM 2 and 6 of the Esquif campaign. (J.S.)

  3. China's international trade and air pollution in the United States.

    Science.gov (United States)

    Lin, Jintai; Pan, Da; Davis, Steven J; Zhang, Qiang; He, Kebin; Wang, Can; Streets, David G; Wuebbles, Donald J; Guan, Dabo

    2014-02-04

    China is the world's largest emitter of anthropogenic air pollutants, and measurable amounts of Chinese pollution are transported via the atmosphere to other countries, including the United States. However, a large fraction of Chinese emissions is due to manufacture of goods for foreign consumption. Here, we analyze the impacts of trade-related Chinese air pollutant emissions on the global atmospheric environment, linking an economic-emission analysis and atmospheric chemical transport modeling. We find that in 2006, 36% of anthropogenic sulfur dioxide, 27% of nitrogen oxides, 22% of carbon monoxide, and 17% of black carbon emitted in China were associated with production of goods for export. For each of these pollutants, about 21% of export-related Chinese emissions were attributed to China-to-US export. Atmospheric modeling shows that transport of the export-related Chinese pollution contributed 3-10% of annual mean surface sulfate concentrations and 0.5-1.5% of ozone over the western United States in 2006. This Chinese pollution also resulted in one extra day or more of noncompliance with the US ozone standard in 2006 over the Los Angeles area and many regions in the eastern United States. On a daily basis, the export-related Chinese pollution contributed, at a maximum, 12-24% of sulfate concentrations over the western United States. As the United States outsourced manufacturing to China, sulfate pollution in 2006 increased in the western United States but decreased in the eastern United States, reflecting the competing effect between enhanced transport of Chinese pollution and reduced US emissions. Our findings are relevant to international efforts to reduce transboundary air pollution.