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Sample records for antiferromagnetic spin fluctuations

  1. Hole pairing induced by antiferromagnetic spin fluctuations

    International Nuclear Information System (INIS)

    Su, Z.B.; Yu Lu; Dong, J.M.; Tosatti, E.

    1987-08-01

    The effective interaction induced by antiferromagnetic spin fluctuations is considered in the random phase approximation in the context of the recently discovered high T c oxide superconductors. This effective attraction favours a triplet pairing of holes. The implications of such pairing mechanism are discussed in connection with the current experimental observations. (author). 30 refs, 2 figs

  2. Spin wave spectrum and zero spin fluctuation of antiferromagnetic solid 3He

    International Nuclear Information System (INIS)

    Roger, M.; Delrieu, J.M.

    1981-08-01

    The spin wave spectrum and eigenvectors of the uudd antiferromagnetic phase of solid 3 He are calculated; an optical mode is predicted around 150 - 180 Mc and a zero point spin deviation of 0.74 is obtained in agreement with the antiferromagnetic resonance frequency measured by Osheroff

  3. Antiferromagnetic spin fluctuations in the heavy-fermion superconductor Ce2PdIn8

    Science.gov (United States)

    Tran, V. H.; Hillier, A. D.; Adroja, D. T.; Kaczorowski, D.

    2012-09-01

    Inelastic neutron scattering and muon spin relaxation/rotation (μSR) measurements were performed on the heavy-fermion superconductor Ce2PdIn8. The observed scaling of the imaginary part of the dynamical susceptibility χ''Tα∝f(ℏω/kBT) with α=3/2 revealed a non-Fermi liquid character of the normal state, being due to critical antiferromagnetic fluctuations near a T=0 quantum phase transition. The longitudinal-field μSR measurements indicated that superconductivity and antiferromagnetic spin fluctuations coexist in Ce2PdIn8 on a microscopic scale. The observed power-law temperature dependence of the magnetic penetration depth λ∝T3/2, deduced from the transverse-field μSR data, strongly confirms an unconventional superconductivity in this compound.

  4. Quantum fluctuations in the competition among spin glass, antiferromagnetism and local pairing superconductivity

    International Nuclear Information System (INIS)

    Magalhaes, S.G.; Zimmer, F.M.; Kipper, C.J.; Calegari, E.J.

    2007-01-01

    The competition among spin glass (SG), antiferromagnetism (AF) and local pairing superconductivity (PAIR) is studied in a two-sublattice fermionic Ising SG model with a local BCS pairing interaction in the presence of a transverse magnetic field Γ. The spins in different sublattices interact with Gaussian random couplings with an antiferromagnetic mean. The problem is formulated in a Grassmann path integral formalism. The static ansatz and the replica symmetry are used to obtain the half-filling thermodynamic potential. The results are shown in phase diagrams that exhibit a complex transition line separating the PAIR phase from the others. This line is second order at high temperature which ends in a tricritical point. The presence of Γ affects deeply the transition lines

  5. {mu}SR study of organic systems: ferromagnetism, antiferromagnetism, the spin-crossover effect, and fluctuations in magnetic nanodiscs

    Energy Technology Data Exchange (ETDEWEB)

    Blundell, S.J.; Pratt, F.L.; Lancaster, T.; Marshall, I.M.; Steer, C.A.; Hayes, W.; Sugano, T.; Letard, J.-F.; Caneschi, A.; Gatteschi, D.; Heath, S.L

    2003-02-01

    We present the results of recent {mu}SR experiments on a variety of novel organic and molecular magnetic systems. Muons are sensitive to local static fields and magnetic fluctuations, but can probe much more than just the onset of long-range magnetic order. We review our work on nitronyl nitroxide organic ferromagnets and antiferromagnets. We describe a muon study of the spin-crossover phenomenon which has been studied in Fe(PM-PEA){sub 2}(NCS){sub 2}, and which shows Gaussian and root-exponential muon relaxation in the high-spin and low-spin phases, respectively. Experiments on a disc-shaped molecular complex containing Fe{sub 19} (with spin ((31)/(2))) reveal the effects of quantum tunneling of magnetization and allow an estimate of the quantum tunneling rate.

  6. μSR study of organic systems: ferromagnetism, antiferromagnetism, the spin-crossover effect, and fluctuations in magnetic nanodiscs

    International Nuclear Information System (INIS)

    Blundell, S.J.; Pratt, F.L.; Lancaster, T.; Marshall, I.M.; Steer, C.A.; Hayes, W.; Sugano, T.; Letard, J.-F.; Caneschi, A.; Gatteschi, D.; Heath, S.L.

    2003-01-01

    We present the results of recent μSR experiments on a variety of novel organic and molecular magnetic systems. Muons are sensitive to local static fields and magnetic fluctuations, but can probe much more than just the onset of long-range magnetic order. We review our work on nitronyl nitroxide organic ferromagnets and antiferromagnets. We describe a muon study of the spin-crossover phenomenon which has been studied in Fe(PM-PEA) 2 (NCS) 2 , and which shows Gaussian and root-exponential muon relaxation in the high-spin and low-spin phases, respectively. Experiments on a disc-shaped molecular complex containing Fe 19 (with spin ((31)/(2))) reveal the effects of quantum tunneling of magnetization and allow an estimate of the quantum tunneling rate

  7. Antiferromagnetic spin-orbitronics

    KAUST Repository

    Manchon, Aurelien; Saidaoui, Hamed Ben Mohamed; Ghosh, Sumit

    2015-01-01

    Antiferromagnets have long remained an intriguing and exotic state of matter, whose application has been restricted to enabling interfacial exchange bias in metallic and tunneling spin-valves [1]. Their role in the expanding field of applied spintronics has been mostly passive and the in-depth investigation of their basic properties mostly considered from a fundamental perspective.

  8. Antiferromagnetic spin-orbitronics

    KAUST Repository

    Manchon, Aurelien

    2015-05-01

    Antiferromagnets have long remained an intriguing and exotic state of matter, whose application has been restricted to enabling interfacial exchange bias in metallic and tunneling spin-valves [1]. Their role in the expanding field of applied spintronics has been mostly passive and the in-depth investigation of their basic properties mostly considered from a fundamental perspective.

  9. Charged domain-wall dynamics in doped antiferromagnets and spin fluctuations in cuprate superconductors

    International Nuclear Information System (INIS)

    Zaanen, J.; Horbach, M.L.; van Saarloos, W.

    1996-01-01

    Evidence is accumulating that the electron liquid in the cuprate superconductors is characterized by many-hole correlations of the charged magnetic domain-wall type. Here we focus on the strong-coupling limit where all holes are bound to domain walls. We assert that at high temperatures a classical domain-wall fluid is realized and show that the dynamics of such a fluid is characterized by spatial and temporal crossover scales set by temperature itself. The fundamental parameters of this fluid are such that the domain-wall motions dominate the low-frequency spin fluctuations and we derive predictions for the behavior of the dynamical magnetic susceptibility. We argue that a crossover occurs from a high-temperature classical to a low-temperature quantum regime, in direct analogy with helium. We discuss some general characteristics of the domain-wall quantum liquid, realized at low temperatures. copyright 1996 The American Physical Society

  10. Spin Dynamics and Critical Fluctuations in a Two-Dimensional Random Antiferromagnet

    DEFF Research Database (Denmark)

    Als-Nielsen, Jens Aage; Birgeneau, R. J.; Guggenheim, H. J.

    1975-01-01

    A comprehensive elastic- and inelastic-neutron-scattering study of the binary mixed antiferromagnet Rb2Mn0.5Ni0.5F4 has been carried out. The pure materials, Rb2MnF4 and Rb2NiF4 are [2d] near-Heisenberg antiferromagnets of the K2NiF4 type. Elastic-scattering experiments demonstrate that the Mn...

  11. Superconductivity and spin fluctuations

    International Nuclear Information System (INIS)

    Scalapino, D.J.

    1999-01-01

    The organizers of the Memorial Session for Herman Rietschel asked that the author review some of the history of the interplay of superconductivity and spin fluctuations. Initially, Berk and Schrieffer showed how paramagnon spin fluctuations could suppress superconductivity in nearly-ferromagnetic materials. Following this, Rietschel and various co-workers wrote a number of papers in which they investigated the role of spin fluctuations in reducing the Tc of various electron-phonon superconductors. Paramagnon spin fluctuations are also believed to provide the p-wave pairing mechanism responsible for the superfluid phases of 3 He. More recently, antiferromagnetic spin fluctuations have been proposed as the mechanism for d-wave pairing in the heavy-fermion superconductors and in some organic materials as well as possibly the high-Tc cuprates. Here the author will review some of this early history and discuss some of the things he has learned more recently from numerical simulations

  12. Spin reorientation via antiferromagnetic coupling

    Energy Technology Data Exchange (ETDEWEB)

    Ranjbar, M., E-mail: mojtaba.ranjbar@physics.gu.se [Data Storage Institute, A-STAR (Agency for Science, Technology and Research), 5, Engineering Drive 1, Singapore 117608 (Singapore); Department of Physics, University of Gothenburg, 412 96 Gothenburg (Sweden); Sbiaa, R. [Data Storage Institute, A-STAR (Agency for Science, Technology and Research), 5, Engineering Drive 1, Singapore 117608 (Singapore); Department of Physics, Sultan Qaboos University, P.O. Box 36, PC 123, Muscat (Oman); Dumas, R. K. [Department of Physics, University of Gothenburg, 412 96 Gothenburg (Sweden); Åkerman, J. [Department of Physics, University of Gothenburg, 412 96 Gothenburg (Sweden); Materials Physics, School of ICT, Royal Institute of Technology (KTH), 164 40 Kista (Sweden); Piramanayagam, S. N. [Data Storage Institute, A-STAR (Agency for Science, Technology and Research), 5, Engineering Drive 1, Singapore 117608 (Singapore)

    2014-05-07

    Spin reorientation in antiferromagnetically coupled (AFC) Co/Pd multilayers, wherein the thickness of the constituent Co layers was varied, was studied. AFC-Co/Pd multilayers were observed to have perpendicular magnetic anisotropy even for a Co sublayer thickness of 1 nm, much larger than what is usually observed in systems without antiferromagnetic coupling. When similar multilayer structures were prepared without antiferromagnetic coupling, this effect was not observed. The results indicate that the additional anisotropy energy contribution arising from the antiferromagnetic coupling, which is estimated to be around 6 × 10{sup 6} ergs/cm{sup 3}, induces the spin-reorientation.

  13. Spin fluctuations and the

    Directory of Open Access Journals (Sweden)

    V.M. Loktev

    2008-09-01

    Full Text Available We analyze the spectral properties of a phenomenological model for a weakly doped two-dimensional antiferromagnet, in which the carriers move within one of the two sublattices where they were introduced. Such a constraint results in the free carrier spectra with the maxima at k=(± π/2 , ± π/2 observed in some cuprates. We consider the spectral properties of the model by taking into account fluctuations of the spins in the antiferromagnetic background. We show that such fluctuations lead to a non-pole-like structure of the single-hole Green's function and these fluctuations can be responsible for some anomalous "strange metal" properties of underdoped cuprates in the nonsuperconducting regime.

  14. Neutron scattering studies of two-dimensional antiferromagnetic spin fluctuations in insulating and superconducting S = ½ systems

    DEFF Research Database (Denmark)

    Christensen, Niels Bech

    . Along the antiferromagnetic zone boundary a pronounced intensity variation is found for the dominant single-magnon excitations. This variation tracks an already known zone boundary dispersion. Usingpolarization analysis to separate the components of the excitation spectrum, a continuum of longitudinally...... polarized multimagnon excitations is discovered at energies above the single-magnon branch. At low energies, the findings are well described bylinear spin wave theory. At high energies, linear spin wave theory fails and instead the data are very well accounted for by state-of-the-art Quantum Monte Carlo...

  15. Neutron scattering studies of two-dimensional antiferromagnetic spin fluctuations in insulating and superconducting S = 1/2 systems

    Energy Technology Data Exchange (ETDEWEB)

    Bech Christensen, N

    2005-01-01

    Time-of-flight and polarized triple axis neutron scattering is used to probe the spin excitations of Cu(DCOO){sub 2}x4D{sub 2}O and La{sub 2-x}Sr{sub x}CuO{sub 4}. The first part of the thesis contains an investigation of the excitation spectrum of the square lattice S = 1/2 Heisenberg antiferromagnet Cu(DCOO){sub 2}4D{sub 2}O. Along the antiferromagnetic zone boundary a pronounced intensity variation is found for the dominant single-magnon excitations. This variation tracks an already known zone boundary dispersion. Using polarization analysis to separate the components of the excitation spectrum, a continuum of longitudinally polarized multimagnon excitations is discovered at energies above the single-magnon branch. At low energies, the findings are well described by linear spin wave theory. At high energies, linear spin wave theory fails and instead the data are very well accounted for by state-of-the-art Quantum Monte Carlo computations. In the second part of the thesis, the spin excitation spectra of the high temperature superconductors La{sub 1.90}Sr{sub 0.10}CuO{sub 4} and La{sub 1.84}Sr{sub 0.16}Cu characterized. The main discovery is that the excitations are dispersive at both doping levels. The dispersion strongly resembles that seen in other high-T{sub c} superconductors. The presence of dispersive excitations does not require superconductivity to exist. For La{sub 1.84}Sr{sub 0.16}CuO{sub 4}, but not for La{sub 1.90}Sr{sub 0.10}CuO{sub 4}, the onset superconductivity gives rise to a spectral weight shift which displays qualitative and quantitative similarities to the resonance mode observed in other high-T{sub c} superconductors. (au)

  16. Neutron scattering studies of two-dimensional antiferromagnetic spin fluctuations in insulating and superconducting S = 1/2 systems

    International Nuclear Information System (INIS)

    Bech Christensen, N.

    2005-01-01

    Time-of-flight and polarized triple axis neutron scattering is used to probe the spin excitations of Cu(DCOO) 2 x4D 2 O and La 2-x Sr x CuO 4 . The first part of the thesis contains an investigation of the excitation spectrum of the square lattice S = 1/2 Heisenberg antiferromagnet Cu(DCOO) 2 4D 2 O. Along the antiferromagnetic zone boundary a pronounced intensity variation is found for the dominant single-magnon excitations. This variation tracks an already known zone boundary dispersion. Using polarization analysis to separate the components of the excitation spectrum, a continuum of longitudinally polarized multimagnon excitations is discovered at energies above the single-magnon branch. At low energies, the findings are well described by linear spin wave theory. At high energies, linear spin wave theory fails and instead the data are very well accounted for by state-of-the-art Quantum Monte Carlo computations. In the second part of the thesis, the spin excitation spectra of the high temperature superconductors La 1.90 Sr 0.10 CuO 4 and La 1.84 Sr 0.16 Cu characterized. The main discovery is that the excitations are dispersive at both doping levels. The dispersion strongly resembles that seen in other high-T c superconductors. The presence of dispersive excitations does not require superconductivity to exist. For La 1.84 Sr 0.16 CuO 4 , but not for La 1.90 Sr 0.10 CuO 4 , the onset superconductivity gives rise to a spectral weight shift which displays qualitative and quantitative similarities to the resonance mode observed in other high-T c superconductors. (au)

  17. Spin Structure Analyses of Antiferromagnets

    International Nuclear Information System (INIS)

    Chung, Jae Ho; Song, Young Sang; Lee, Hak Bong

    2010-05-01

    We have synthesized series of powder sample of incommensurate antiferromagnetic multiferroics, (Mn, Co)WO 4 and Al doped Ba 0.5 Sr 1.5 Zn 2 Fe 12 O 22 , incommensurate antiferromagnetic multiferroics. Their spin structure was studied by using the HRPD. In addition, we have synthesized series of crystalline samples of incommensurate multiferroics, (Mn, Co)WO 4 and olivines. Their spin structure was investigated using neutron diffraction under high magnetic field. As a result, we were able to draw the phase diagram of (Mn, Co)WO 4 as a function of composition and temperature. We learned the how the spin structure changes with increased ionic substitution. Finally we have drawn the phase diagram of the multicritical olivine Mn2SiS4/Mn2GeS4 as a function of filed and temperature through the spin structure studies

  18. Spin diffusion and torques in disordered antiferromagnets

    KAUST Repository

    Manchon, Aurelien

    2017-02-01

    We have developed a drift-diffusion equation of spin transport in collinear bipartite metallic antiferromagnets. Starting from a model tight-binding Hamiltonian, we obtain the quantum kinetic equation within Keldysh formalism and expand it to the lowest order in spatial gradient using Wigner expansion method. In the diffusive limit, these equations track the spatio-temporal evolution of the spin accumulations and spin currents on each sublattice of the antiferromagnet. We use these equations to address the nature of the spin transfer torque in (i) a spin-valve composed of a ferromagnet and an antiferromagnet, (ii) a metallic bilayer consisting of an antiferromagnet adjacent to a heavy metal possessing spin Hall effect, and in (iii) a single antiferromagnet possessing spin Hall effect. We show that the latter can experience a self-torque thanks to the non-vanishing spin Hall effect in the antiferromagnet.

  19. Spin diffusion and torques in disordered antiferromagnets

    KAUST Repository

    Manchon, Aurelien

    2017-01-01

    We have developed a drift-diffusion equation of spin transport in collinear bipartite metallic antiferromagnets. Starting from a model tight-binding Hamiltonian, we obtain the quantum kinetic equation within Keldysh formalism and expand it to the lowest order in spatial gradient using Wigner expansion method. In the diffusive limit, these equations track the spatio-temporal evolution of the spin accumulations and spin currents on each sublattice of the antiferromagnet. We use these equations to address the nature of the spin transfer torque in (i) a spin-valve composed of a ferromagnet and an antiferromagnet, (ii) a metallic bilayer consisting of an antiferromagnet adjacent to a heavy metal possessing spin Hall effect, and in (iii) a single antiferromagnet possessing spin Hall effect. We show that the latter can experience a self-torque thanks to the non-vanishing spin Hall effect in the antiferromagnet.

  20. Long-range interactions in antiferromagnetic quantum spin chains

    Science.gov (United States)

    Bravo, B.; Cabra, D. C.; Gómez Albarracín, F. A.; Rossini, G. L.

    2017-08-01

    We study the role of long-range dipolar interactions on antiferromagnetic spin chains, from the classical S →∞ limit to the deep quantum case S =1 /2 , including a transverse magnetic field. To this end, we combine different techniques such as classical energy minima, classical Monte Carlo, linear spin waves, bosonization, and density matrix renormalization group (DMRG). We find a phase transition from the already reported dipolar ferromagnetic region to an antiferromagnetic region for high enough antiferromagnetic exchange. Thermal and quantum fluctuations destabilize the classical order before reaching magnetic saturation in both phases, and also close to zero field in the antiferromagnetic phase. In the extreme quantum limit S =1 /2 , extensive DMRG computations show that the main phases remain present with transition lines to saturation significatively shifted to lower fields, in agreement with the bosonization analysis. The overall picture maintains a close analogy with the phase diagram of the anisotropic XXZ spin chain in a transverse field.

  1. Magnon Spin Nernst Effect in Antiferromagnets

    Science.gov (United States)

    Zyuzin, Vladimir A.; Kovalev, Alexey A.

    2016-11-01

    We predict that a temperature gradient can induce a magnon-mediated spin Hall response in an antiferromagnet with nontrivial magnon Berry curvature. We develop a linear response theory which gives a general condition for a Hall current to be well defined, even when the thermal Hall response is forbidden by symmetry. We apply our theory to a honeycomb lattice antiferromagnet and discuss a role of magnon edge states in a finite geometry.

  2. Magnon Spin Nernst Effect in Antiferromagnets.

    Science.gov (United States)

    Zyuzin, Vladimir A; Kovalev, Alexey A

    2016-11-18

    We predict that a temperature gradient can induce a magnon-mediated spin Hall response in an antiferromagnet with nontrivial magnon Berry curvature. We develop a linear response theory which gives a general condition for a Hall current to be well defined, even when the thermal Hall response is forbidden by symmetry. We apply our theory to a honeycomb lattice antiferromagnet and discuss a role of magnon edge states in a finite geometry.

  3. Heat-driven spin torques in antiferromagnets

    Science.gov (United States)

    Białek, Marcin; Bréchet, Sylvain; Ansermet, Jean-Philippe

    2018-04-01

    Heat-driven magnetization damping, which is a linear function of a temperature gradient, is predicted in antiferromagnets by considering the sublattice dynamics subjected to a heat-driven spin torque. This points to the possibility of achieving spin torque oscillator behavior. The model is based on the magnetic Seebeck effect acting on sublattices which are exchange coupled. The heat-driven spin torque is estimated and the feasibility of detecting this effect is discussed.

  4. Spin transport and spin torque in antiferromagnetic devices

    Science.gov (United States)

    Železný, J.; Wadley, P.; Olejník, K.; Hoffmann, A.; Ohno, H.

    2018-03-01

    Ferromagnets are key materials for sensing and memory applications. In contrast, antiferromagnets, which represent the more common form of magnetically ordered materials, have found less practical application beyond their use for establishing reference magnetic orientations via exchange bias. This might change in the future due to the recent progress in materials research and discoveries of antiferromagnetic spintronic phenomena suitable for device applications. Experimental demonstration of the electrical switching and detection of the Néel order open a route towards memory devices based on antiferromagnets. Apart from the radiation and magnetic-field hardness, memory cells fabricated from antiferromagnets can be inherently multilevel, which could be used for neuromorphic computing. Switching speeds attainable in antiferromagnets far exceed those of ferromagnetic and semiconductor memory technologies. Here, we review the recent progress in electronic spin-transport and spin-torque phenomena in antiferromagnets that are dominantly of the relativistic quantum-mechanical origin. We discuss their utility in pure antiferromagnetic or hybrid ferromagnetic/antiferromagnetic memory devices.

  5. Spin structures in antiferromagnetic nanoparticles

    DEFF Research Database (Denmark)

    Brok, Erik

    dependence of the magnetisation in certain nanoparticle systems, as welll bulk systems with spin canting due to defects. In accordance with this model magnetisation measurements on goethtie (a-FeOOH) nanoparticles are presented, showing a low temperature increase in the magnetisation. The spin orientation...... experimental data from unpolarised neutron diffraction. The spin orientation is found to be close to the particle plane, which is the (111) plane of the FCC structure of NiO for particles with thickness ranging from 2.2 nm to bulk (= 200 nm) particles. In the smallest particles, with a thickness of 2.0 nm, we...

  6. Spin Transport in Ferromagnetic and Antiferromagnetic Textures

    KAUST Repository

    Akosa, Collins A.

    2016-12-07

    In this dissertation, we provide an accurate description of spin transport in magnetic textures and in particular, we investigate in detail, the nature of spin torque and magnetic damping in such systems. Indeed, as will be further discussed in this thesis, the current-driven velocity of magnetic textures is related to the ratio between the so-called non-adiabatic torque and magnetic damping. Uncovering the physics underlying these phenomena can lead to the optimal design of magnetic systems with improved efficiency. We identified three interesting classes of systems which have attracted enormous research interest (i) Magnetic textures in systems with broken inversion symmetry: We investigate the nature of magnetic damping in non-centrosymmetric ferromagnets. Based on phenomenological and microscopic derivations, we show that the magnetic damping becomes chiral, i.e. depends on the chirality of the magnetic texture. (ii) Ferromagnetic domain walls, skyrmions and vortices: We address the physics of spin transport in sharp disordered magnetic domain walls and vortex cores. We demonstrate that upon spin-independent scattering, the non-adiabatic torque can be significantly enhanced. Such an enhancement is large for vortex cores compared to transverse domain walls. We also show that the topological spin currents owing in these structures dramatically enhances the non-adiabaticity, an effect unique to non-trivial topological textures (iii) Antiferromagnetic skyrmions: We extend this study to antiferromagnetic skyrmions and show that such an enhanced topological torque also exist in these systems. Even more interestingly, while such a non-adiabatic torque inuences the undesirable transverse velocity of ferromagnetic skyrmions, in antiferromagnetic skyrmions, the topological non-adiabatic torque directly determines the longitudinal velocity. As a consequence, scaling down the antiferromagnetic skyrmion results in a much more efficient spin torque.

  7. Robust spin transfer torque in antiferromagnetic tunnel junctions

    KAUST Repository

    Saidaoui, Hamed Ben Mohamed; Waintal, Xavier; Manchon, Aurelien

    2017-01-01

    We theoretically study the current-induced spin torque in antiferromagnetic tunnel junctions, composed of two semi-infinite antiferromagnetic layers separated by a tunnel barrier, in both clean and disordered regimes. We find that the torque

  8. High-field spin dynamics of antiferromagnetic quantum spin chains

    DEFF Research Database (Denmark)

    Enderle, M.; Regnault, L.P.; Broholm, C.

    2000-01-01

    present recent work on the high-field spin dynamics of the S = I antiferromagnetic Heisenberg chains NENP (Haldane ground state) and CsNiCl3 (quasi-1D HAF close to the quantum critical point), the uniform S = 1/2 chain CTS, and the spin-Peierls system CuGeO3. (C) 2000 Elsevier Science B,V. All rights...

  9. Robust spin transfer torque in antiferromagnetic tunnel junctions

    KAUST Repository

    Saidaoui, Hamed Ben Mohamed

    2017-04-18

    We theoretically study the current-induced spin torque in antiferromagnetic tunnel junctions, composed of two semi-infinite antiferromagnetic layers separated by a tunnel barrier, in both clean and disordered regimes. We find that the torque enabling electrical manipulation of the Néel antiferromagnetic order parameter is out of plane, ∼n×p, while the torque competing with the antiferromagnetic exchange is in plane, ∼n×(p×n). Here, p and n are the Néel order parameter direction of the reference and free layers, respectively. Their bias dependence shows behavior similar to that in ferromagnetic tunnel junctions, the in-plane torque being mostly linear in bias, while the out-of-plane torque is quadratic. Most importantly, we find that the spin transfer torque in antiferromagnetic tunnel junctions is much more robust against disorder than that in antiferromagnetic metallic spin valves due to the tunneling nature of spin transport.

  10. Spin-isotropic continuum of spin excitations in antiferromagnetically ordered Fe1.07Te

    Science.gov (United States)

    Song, Yu; Lu, Xingye; Regnault, L.-P.; Su, Yixi; Lai, Hsin-Hua; Hu, Wen-Jun; Si, Qimiao; Dai, Pengcheng

    2018-02-01

    Unconventional superconductivity typically emerges in the presence of quasidegenerate ground states, and the associated intense fluctuations are likely responsible for generating the superconducting state. Here we use polarized neutron scattering to study the spin space anisotropy of spin excitations in Fe1.07Te exhibiting bicollinear antiferromagnetic (AF) order, the parent compound of FeTe1 -xSex superconductors. We confirm that the low-energy spin excitations are transverse spin waves, consistent with a local-moment origin of the bicollinear AF order. While the ordered moments lie in the a b plane in Fe1.07Te , it takes less energy for them to fluctuate out of plane, similar to BaFe2As2 and NaFeAs. At energies above E ≳20 meV, we find magnetic scattering to be dominated by an isotropic continuum that persists up to at least 50 meV. Although the isotropic spin excitations cannot be ascribed to spin waves from a long-range-ordered local-moment antiferromagnet, the continuum can result from the bicollinear magnetic order ground state of Fe1.07Te being quasidegenerate with plaquette magnetic order.

  11. Dynamics of an inhomogeneous anisotropic antiferromagnetic spin chain

    International Nuclear Information System (INIS)

    Daniel, M.; Amuda, R.

    1994-11-01

    We investigate the nonlinear spin excitations in the two sublattice model of a one dimensional classical continuum Heisenberg inhomogeneous antiferromagnetic spin chain. The dynamics of the inhomogeneous chain reduces to that of its homogeneous counterpart when the inhomogeneity assumes a particular form. Apart from the usual twists and pulses, we obtain some planar configurations representing the nonlinear dynamics of spins. (author). 12 refs

  12. Spin waves in antiferromagnetic FeF2

    DEFF Research Database (Denmark)

    Hutchings, M T; Rainford, B.D.; Guggenheim, H J

    1970-01-01

    Spin-wave dispersion in antiferromagnetic FeF2 has been investigated by inelastic neutron scattering using a chopper time-of-flight spectrometer. The single mode observed has a relatively flat dispersion curve rising from 53 cm-1 at the zone centre to 79 cm-1 at the zone boundary. A spin Hamilton......Spin-wave dispersion in antiferromagnetic FeF2 has been investigated by inelastic neutron scattering using a chopper time-of-flight spectrometer. The single mode observed has a relatively flat dispersion curve rising from 53 cm-1 at the zone centre to 79 cm-1 at the zone boundary. A spin...

  13. Spin Hall magnetoresistance in antiferromagnet/normal metal bilayers

    KAUST Repository

    Manchon, Aurelien

    2017-01-01

    We investigate the emergence of spin Hall magnetoresistance in a magnetic bilayer composed of a normal metal adjacent to an antiferromagnet. Based on a recently derived drift diffusion equation, we show that the resistance of the bilayer depends on the relative angle between the direction transverse to the current flow and the Néel order parameter. While this effect presents striking similarities with the spin Hall magnetoresistance recently reported in ferromagnetic bilayers, its physical origin is attributed to the anisotropic spin relaxation of itinerant spins in the antiferromagnet.

  14. Spin Currents and Spin Orbit Torques in Ferromagnets and Antiferromagnets

    Science.gov (United States)

    Hung, Yu-Ming

    This thesis focuses on the interactions of spin currents and materials with magnetic order, e.g., ferromagnetic and antiferromagnetic thin films. The spin current is generated in two ways. First by spin-polarized conduction-electrons associated with the spin Hall effect in heavy metals (HMs) and, second, by exciting spin-waves in ferrimagnetic insulators using a microwave frequency magnetic field. A conduction-electron spin current can be generated by spin-orbit coupling in a heavy non-magnetic metal and transfer its spin angular momentum to a ferromagnet, providing a means of reversing the magnetization of perpendicularly magnetized ultrathin films with currents that flow in the plane of the layers. The torques on the magnetization are known as spin-orbit torques (SOT). In the first part of my thesis project I investigated and contrasted the quasistatic (slowly swept current) and pulsed current-induced switching characteristics of micrometer scale Hall crosses consisting of very thin (magnetized CoFeB layers on beta-Ta. While complete magnetization reversal occurs at a threshold current density in the quasistatic case, pulses with short duration (≤10 ns) and larger amplitude (≃10 times the quasistatic threshold current) lead to only partial magnetization reversal and domain formation. The partial reversal is associated with the limited time for reversed domain expansion during the pulse. The second part of my thesis project studies and considers applications of SOT-driven domain wall (DW) motion in a perpendicularly magnetized ultrathin ferromagnet sandwiched between a heavy metal and an oxide. My experiment results demonstrate that the DW motion can be explained by a combination of the spin Hall effect, which generates a SOT, and Dzyaloshinskii-Moriya interaction, which stabilizes chiral Neel-type DW. Based on SOT-driven DW motion and magnetic coupling between electrically isolated ferromagnetic elements, I proposed a new type of spin logic devices. I then

  15. Spin transfer torque in antiferromagnetic spin valves: From clean to disordered regimes

    KAUST Repository

    Saidaoui, Hamed Ben Mohamed

    2014-05-28

    Current-driven spin torques in metallic spin valves composed of antiferromagnets are theoretically studied using the nonequilibrium Green\\'s function method implemented on a tight-binding model. We focus our attention on G-type and L-type antiferromagnets in both clean and disordered regimes. In such structures, spin torques can either rotate the magnetic order parameter coherently (coherent torque) or compete with the internal antiferromagnetic exchange (exchange torque). We show that, depending on the symmetry of the spin valve, the coherent and exchange torques can either be in the plane, ∝n×(q×n) or out of the plane ∝n×q, where q and n are the directions of the order parameter of the polarizer and the free antiferromagnetic layers, respectively. Although disorder conserves the symmetry of the torques, it strongly reduces the torque magnitude, pointing out the need for momentum conservation to ensure strong spin torque in antiferromagnetic spin valves.

  16. Spin transfer torque in antiferromagnetic spin valves: From clean to disordered regimes

    KAUST Repository

    Saidaoui, Hamed Ben Mohamed; Manchon, Aurelien; Waintal, Xavier

    2014-01-01

    Current-driven spin torques in metallic spin valves composed of antiferromagnets are theoretically studied using the nonequilibrium Green's function method implemented on a tight-binding model. We focus our attention on G-type and L-type antiferromagnets in both clean and disordered regimes. In such structures, spin torques can either rotate the magnetic order parameter coherently (coherent torque) or compete with the internal antiferromagnetic exchange (exchange torque). We show that, depending on the symmetry of the spin valve, the coherent and exchange torques can either be in the plane, ∝n×(q×n) or out of the plane ∝n×q, where q and n are the directions of the order parameter of the polarizer and the free antiferromagnetic layers, respectively. Although disorder conserves the symmetry of the torques, it strongly reduces the torque magnitude, pointing out the need for momentum conservation to ensure strong spin torque in antiferromagnetic spin valves.

  17. Magnetism of one-dimensional strongly repulsive spin-1 bosons with antiferromagnetic spin-exchange interaction

    International Nuclear Information System (INIS)

    Lee, J. Y.; Guan, X. W.; Batchelor, M. T.; Lee, C.

    2009-01-01

    We investigate magnetism and quantum phase transitions in a one-dimensional system of integrable spin-1 bosons with strongly repulsive density-density interaction and antiferromagnetic spin-exchange interaction via the thermodynamic Bethe ansatz method. At zero temperature, the system exhibits three quantum phases: (i) a singlet phase of boson pairs when the external magnetic field H is less than the lower critical field H c1 ; (ii) a ferromagnetic phase of atoms in the hyperfine state |F=1, m F =1> when the external magnetic field exceeds the upper critical field H c2 ; and (iii) a mixed phase of singlet pairs and unpaired atoms in the intermediate region H c1 c2 . At finite temperatures, the spin fluctuations affect the thermodynamics of the model through coupling the spin bound states to the dressed energy for the unpaired m F =1 bosons. However, such spin dynamics is suppressed by a sufficiently strong external field at low temperatures. Thus the singlet pairs and unpaired bosons may form a two-component Luttinger liquid in the strong coupling regime.

  18. Spin Wave Theory in Two-Dimensional Coupled Antiferromagnets

    Science.gov (United States)

    Shimahara, Hiroshi

    2018-04-01

    We apply spin wave theory to two-dimensional coupled antiferromagnets. In particular, we primarily examine a system that consists of small spins coupled by a strong exchange interaction J1, large spins coupled by a weak exchange interaction J2, and an anisotropic exchange interaction J12 between the small and large spins. This system is an effective model of the organic antiferromagnet λ-(BETS)2FeCl4 in its insulating phase, in which intriguing magnetic phenomena have been observed, where the small and large spins correspond to π electrons and 3d spins, respectively. BETS stands for bis(ethylenedithio)tetraselenafulvalene. We obtain the antiferromagnetic transition temperature TN and the sublattice magnetizations m(T) and M(T) of the small and large spins, respectively, as functions of the temperature T. When T increases, m(T) is constant with a slight decrease below TN, even where M(T) decreases significantly. When J1 ≫ J12 and J2 = 0, an analytical expression for TN is derived. The estimated value of TN and the behaviors of m(T) and M(T) agree with the observations of λ-(BETS)2FeCl4.

  19. Role of the antiferromagnetic bulk spins in exchange bias

    Energy Technology Data Exchange (ETDEWEB)

    Schuller, Ivan K. [Center for Advanced Nanoscience and Physics Department, University of California San Diego, La Jolla, CA 92093 (United States); Morales, Rafael, E-mail: rafael.morales@ehu.es [Department of Chemical-Physics & BCMaterials, University of the Basque Country UPV/EHU (Spain); IKERBASQUE, Basque Foundation for Science, 48011 Bilbao (Spain); Batlle, Xavier [Departament Física Fonamental and Institut de Nanociència i Nanotecnologia, Universitat de Barcelona, c/ Martí i Franqués s/n, 08028 Barcelona, Catalonia (Spain); Nowak, Ulrich [Department of Physics, University of Konstanz, 78464 Konstanz (Germany); Güntherodt, Gernot [Physics Institute (IIA), RWTH Aachen University, Campus RWTH-Melaten, 52074 Aachen (Germany)

    2016-10-15

    This “Critical Focused Issue” presents a brief review of experiments and models which describe the origin of exchange bias in epitaxial or textured ferromagnetic/antiferromagnetic bilayers. Evidence is presented which clearly indicates that inner, uncompensated, pinned moments in the bulk of the antiferromagnet (AFM) play a very important role in setting the magnitude of the exchange bias. A critical evaluation of the extensive literature in the field indicates that it is useful to think of this bulk, pinned uncompensated moments as a new type of a ferromagnet which has a low total moment, an ordering temperature given by the AFM Néel temperature, with parallel aligned moments randomly distributed on the regular AFM lattice. - Highlights: • We address the role of bulk antiferromagnetic spins in the exchange bias phenomenon. • Significant experiments on how bulk AFM spins determine exchange bias are highlighted. • We explain the model that accounts for experimental results.

  20. Role of the antiferromagnetic bulk spins in exchange bias

    International Nuclear Information System (INIS)

    Schuller, Ivan K.; Morales, Rafael; Batlle, Xavier; Nowak, Ulrich; Güntherodt, Gernot

    2016-01-01

    This “Critical Focused Issue” presents a brief review of experiments and models which describe the origin of exchange bias in epitaxial or textured ferromagnetic/antiferromagnetic bilayers. Evidence is presented which clearly indicates that inner, uncompensated, pinned moments in the bulk of the antiferromagnet (AFM) play a very important role in setting the magnitude of the exchange bias. A critical evaluation of the extensive literature in the field indicates that it is useful to think of this bulk, pinned uncompensated moments as a new type of a ferromagnet which has a low total moment, an ordering temperature given by the AFM Néel temperature, with parallel aligned moments randomly distributed on the regular AFM lattice. - Highlights: • We address the role of bulk antiferromagnetic spins in the exchange bias phenomenon. • Significant experiments on how bulk AFM spins determine exchange bias are highlighted. • We explain the model that accounts for experimental results.

  1. Pure spin current manipulation in antiferromagnetically exchange coupled heterostructures

    Science.gov (United States)

    Avilés-Félix, L.; Butera, A.; González-Chávez, D. E.; Sommer, R. L.; Gómez, J. E.

    2018-03-01

    We present a model to describe the spin currents generated by ferromagnet/spacer/ferromagnet exchange coupled trilayer systems and heavy metal layers with strong spin-orbit coupling. By exploiting the magnitude of the exchange coupling (oscillatory RKKY-like coupling) and the spin-flop transition in the magnetization process, it has been possible to produce spin currents polarized in arbitrary directions. The spin-flop transition of the trilayer system originates pure spin currents whose polarization vector depends on the exchange field and the magnetization equilibrium angles. We also discuss a protocol to control the polarization sign of the pure spin current injected into the metallic layer by changing the initial conditions of magnetization of the ferromagnetic layers previously to the spin pumping and inverse spin Hall effect experiments. The small differences in the ferromagnetic layers lead to a change in the magnetization vector rotation that permits the control of the sign of the induced voltage components due to the inverse spin Hall effect. Our results can lead to important advances in hybrid spintronic devices with new functionalities, particularly, the ability to control microscopic parameters such as the polarization direction and the sign of the pure spin current through the variation of macroscopic parameters, such as the external magnetic field or the thickness of the spacer in antiferromagnetic exchange coupled systems.

  2. Long range anti-ferromagnetic spin model for prebiotic evolution

    International Nuclear Information System (INIS)

    Nokura, Kazuo

    2003-01-01

    I propose and discuss a fitness function for one-dimensional binary monomer sequences of macromolecules for prebiotic evolution. The fitness function is defined by the free energy of polymers in the high temperature random coil phase. With repulsive interactions among the same kind of monomers, the free energy in the high temperature limit becomes the energy function of the one-dimensional long range anti-ferromagnetic spin model, which is shown to have a dynamical phase transition and glassy states

  3. Longitudinal Spin Excitations and Magnetic Anisotropy in Antiferromagnetically Ordered BaFe_{2}As_{2}

    Directory of Open Access Journals (Sweden)

    Chong Wang

    2013-12-01

    Full Text Available We report on a spin-polarized inelastic neutron-scattering study of spin waves in the antiferromagnetically ordered state of BaFe_{2}As_{2}. Three distinct excitation components are identified, with spins fluctuating along the c axis, perpendicular to the ordering direction in the ab plane and parallel to the ordering direction. While the first two “transverse” components can be described by a linear spin-wave theory with magnetic anisotropy and interlayer coupling, the third “longitudinal” component is generically incompatible with the local-moment picture. It points toward a contribution of itinerant electrons to the magnetism that is already in the parent compound of this family of Fe-based superconductors.

  4. Magnon Spin-Momentum Locking: Various Spin Vortices and Dirac magnons in Noncollinear Antiferromagnets

    Science.gov (United States)

    Okuma, Nobuyuki

    2017-09-01

    We generalize the concept of the spin-momentum locking to magnonic systems and derive the formula to calculate the spin expectation value for one-magnon states of general two-body spin Hamiltonians. We give no-go conditions for magnon spin to be independent of momentum. As examples of the magnon spin-momentum locking, we analyze a one-dimensional antiferromagnet with the Néel order and two-dimensional kagome lattice antiferromagnets with the 120° structure. We find that the magnon spin depends on its momentum even when the Hamiltonian has the z -axis spin rotational symmetry, which can be explained in the context of a singular band point or a U (1 ) symmetry breaking. A spin vortex in momentum space generated in a kagome lattice antiferromagnet has the winding number Q =-2 , while the typical one observed in topological insulator surface states is characterized by Q =+1 . A magnonic analogue of the surface states, the Dirac magnon with Q =+1 , is found in another kagome lattice antiferromagnet. We also derive the sum rule for Q by using the Poincaré-Hopf index theorem.

  5. Magnon Spin-Momentum Locking: Various Spin Vortices and Dirac magnons in Noncollinear Antiferromagnets.

    Science.gov (United States)

    Okuma, Nobuyuki

    2017-09-08

    We generalize the concept of the spin-momentum locking to magnonic systems and derive the formula to calculate the spin expectation value for one-magnon states of general two-body spin Hamiltonians. We give no-go conditions for magnon spin to be independent of momentum. As examples of the magnon spin-momentum locking, we analyze a one-dimensional antiferromagnet with the Néel order and two-dimensional kagome lattice antiferromagnets with the 120° structure. We find that the magnon spin depends on its momentum even when the Hamiltonian has the z-axis spin rotational symmetry, which can be explained in the context of a singular band point or a U(1) symmetry breaking. A spin vortex in momentum space generated in a kagome lattice antiferromagnet has the winding number Q=-2, while the typical one observed in topological insulator surface states is characterized by Q=+1. A magnonic analogue of the surface states, the Dirac magnon with Q=+1, is found in another kagome lattice antiferromagnet. We also derive the sum rule for Q by using the Poincaré-Hopf index theorem.

  6. Magnetic Transport in Spin Antiferromagnets for Spintronics Applications

    Directory of Open Access Journals (Sweden)

    Mohamed Azzouz

    2017-10-01

    Full Text Available Had magnetic monopoles been ubiquitous as electrons are, we would probably have had a different form of matter, and power plants based on currents of these magnetic charges would have been a familiar scene of modern technology. Magnetic dipoles do exist, however, and in principle one could wonder if we can use them to generate magnetic currents. In the present work, we address the issue of generating magnetic currents and magnetic thermal currents in electrically-insulating low-dimensional Heisenberg antiferromagnets by invoking the (broken electricity-magnetism duality symmetry. The ground state of these materials is a spin-liquid state that can be described well via the Jordan–Wigner fermions, which permit an easy definition of the magnetic particle and thermal currents. The magnetic and magnetic thermal conductivities are calculated in the present work using the bond–mean field theory. The spin-liquid states in these antiferromagnets are either gapless or gapped liquids of spinless fermions whose flow defines a current just as the one defined for electrons in a Fermi liquid. The driving force for the magnetic current is a magnetic field with a gradient along the magnetic conductor. We predict the generation of a magneto-motive force and realization of magnetic circuits using low-dimensional Heisenberg antiferromagnets. The present work is also about claiming that what the experiments in spintronics attempt to do is trying to treat the magnetic degrees of freedoms on the same footing as the electronic ones.

  7. Spin freezing in the geometrically frustrated pyrochlore antiferromagnet Tb2Mo2O7

    DEFF Research Database (Denmark)

    Gaulin, B.D.; Reimers, J.N.; Mason, T.E.

    1992-01-01

    The magnetic metal ions in the cubic pyrochlore Tb2Mo2O7 form an infinite three-dimensional network of corner-sharing tetrahedra with a very high potential for frustration in the presence of antiferromagnetism. We have performed neutron scattering measurements which show short-range spatial...... correlations that develop continuously with decreasing temperature, while the characteristic time scale for the fluctuating moments decreases dramatically below T(f) is similar to 25 K. Therefore, this pure material, which possesses frustration that is purely geometrical in origin, displays a spin-glass state...

  8. Properties of Haldane Excitations and Multiparticle States in the Antiferromagnetic Spin-1 Chain Compound CsNiCl3

    International Nuclear Information System (INIS)

    Kenzelmann, M.; Cowley, R.A.; Buyers, W.J.L.; Tun, Z.; Coldea, Radu; Enderle, M.

    2002-01-01

    We report inelastic time-of-flight and triple-axis neutron scattering measurements of the excitation spectrum of the coupled antiferromagnetic spin-1 Heisenberg chain system CsNiCl 3 . Measurements over a wide range of wave-vector transfers along the chain confirm that above T N CsNiCl 3 is in a quantum-disordered phase with an energy gap in the excitation spectrum. The spin correlations fall off exponentially with increasing distance with a correlation length ζ = 4.0(2) sites at T = 6.2K. This is shorter than the correlation length for an antiferromagnetic spin-1 Heisenberg chain at this temperature, suggesting that the correlations perpendicular to the chain direction and associated with the interchain coupling lower the single-chain correlation length. A multiparticle continuum is observed in the quantum-disordered phase in the region in reciprocal space where antiferromagnetic fluctuations are strongest, extending in energy up to twice the maximum of the dispersion of the well-defined triplet excitations. We show that the continuum satisfies the Hohenberg-Brinkman sum rule. The dependence of the multiparticle continuum on the chain wave vector resembles that of the two-spinon continuum in antiferromagnetic spin-1/2 Heisenberg chains. This suggests the presence of spin-1/2 degrees of freedom in CsNiCl 3 for T ∼< 12 K, possibly caused by multiply frustrated interchain interactions.

  9. Spin pumping and inverse spin Hall effects in heavy metal/antiferromagnet/Permalloy trilayers

    Science.gov (United States)

    Saglam, Hilal; Zhang, Wei; Jungfleisch, M. Benjamin; Jiang, Wanjun; Pearson, John E.; Hoffmann, Axel

    Recent work shows efficient spin transfer via spin waves in insulating antiferromagnets (AFMs), suggesting that AFMs can play a more active role in the manipulation of ferromagnets. We use spin pumping and inverse spin Hall effect experiments on heavy metal (Pt and W)/AFMs/Py (Ni80Fe20) trilayer structures, to examine the possible spin transfer phenomenon in metallic AFMs, i . e . , FeMn and PdMn. Previous work has studied electronic effects of the spin transport in these materials, yielding short spin diffusion length on the order of 1 nm. However, the work did not examine whether besides diffusive spin transport by the conduction electrons, there are additional spin transport contributions from spin wave excitations. We clearly observe spin transport from the Py spin reservoir to the heavy metal layer through the sandwiched AFMs with thicknesses well above the previously measured spin diffusion lengths, indicating that spin transport by spin waves may lead to non-negligible contributions This work was supported by US DOE, OS, Materials Sciences and Engineering Division. Lithographic patterning was carried out at the CNM, which is supported by DOE, OS under Contract No. DE-AC02-06CH11357.

  10. Spin Hartree-Fock approach to studying quantum Heisenberg antiferromagnets in low dimensions

    Science.gov (United States)

    Werth, A.; Kopietz, P.; Tsyplyatyev, O.

    2018-05-01

    We construct a new mean-field theory for a quantum (spin-1/2) Heisenberg antiferromagnet in one (1D) and two (2D) dimensions using a Hartree-Fock decoupling of the four-point correlation functions. We show that the solution to the self-consistency equations based on two-point correlation functions does not produce any unphysical finite-temperature phase transition, in accord with the Mermin-Wagner theorem, unlike the common approach based on the mean-field equation for the order parameter. The next-neighbor spin-spin correlation functions, calculated within this approach, reproduce closely the strong renormalization by quantum fluctuations obtained via a Bethe ansatz in 1D and a small renormalization of the classical antiferromagnetic state in 2D. The heat capacity approximates with reasonable accuracy the full Bethe ansatz result at all temperatures in 1D. In 2D, we obtain a reduction of the peak height in the heat capacity at a finite temperature that is accessible by high-order 1 /T expansions.

  11. Studies of diluted antiferromagnets MnxMg1-xTiO3 with x=0.55 and 0.70 by muon spin relaxation method

    International Nuclear Information System (INIS)

    Fukaya, A.; Ito, A.; Torikai, E.; Nishiyama, K.; Nagamine, K.

    1997-01-01

    Longitudinal fields μSR measurements have been performed in order to probe the spin dynamics in the diluted antiferromagnets Mn x Mg 1-x TiO 3 with x=0.70 and 0.55. In the x=0.70 sample which forms the antiferromagnetic long-range order, the static and fluctuating fields coexist at the muon stopping site below T N . On the other hand, in the x=0.55 sample which shows the spin-glass behavior, the local fields fluctuate rather fast even below T SG . We infer that this drastic change occurs when Mn x Mg 1-x TiO 3 transforms from an antiferromagnetic system to a spin-glass system by dilution

  12. Electrical switching of antiferromagnets via strongly spin-orbit coupled materials

    Science.gov (United States)

    Li, Xi-Lai; Duan, Xiaopeng; Semenov, Yuriy G.; Kim, Ki Wook

    2017-01-01

    Electrically controlled ultra-fast switching of an antiferromagnet (AFM) is shown to be realizable by interfacing it with a material of strong spin-orbit coupling. The proximity interaction between the sublattice magnetic moments of a layered AFM and the spin-polarized free electrons at the interface offers an efficient way to manipulate antiferromagnetic states. A quantitative analysis, using the combination with a topological insulator as an example, demonstrates highly reliable 90° and 180° rotations of AFM magnetic states under two different mechanisms of effective torque generation at the interface. The estimated switching speed and energy requirement are in the ps and aJ ranges, respectively, which are about two-three orders of magnitude better than the ferromagnetic counterparts. The observed differences in the magnetization dynamics may explain the disparate characteristic responses. Unlike the usual precessional/chiral motions in the ferromagnets, those of the AFMs can essentially be described as a damped oscillator with a more direct path. The impact of random thermal fluctuations is also examined.

  13. Low-temperature spin transport in a S = 1 one-dimensional antiferromagnet

    International Nuclear Information System (INIS)

    Pires, A S T; Lima, L S

    2009-01-01

    We study spin transport in the insulating antiferromagnet with S = 1 in one dimension. The spin conductivity is calculated, at zero temperature, using a modified spin wave theory and the Kubo formalism, within the ladder approximation. Two-magnon processes provide the dominant contribution to the spin conductivity. At finite temperature, free magnons are activated, and turn the system into a perfect spin conductor, i.e., the spin conductivity has a Drude form with infinite scattering time.

  14. Spin fluctuation theory of itinerant electron magnetism

    CERN Document Server

    Takahashi, Yoshinori

    2013-01-01

    This volume shows how collective magnetic excitations determine most of  the magnetic properties of itinerant electron magnets. Previous theories were mainly restricted to the Curie-Weiss law temperature dependence of magnetic susceptibilities. Based on the spin amplitude conservation idea including the zero-point fluctuation amplitude, this book shows that the entire temperature and magnetic field dependence of magnetization curves, even in the ground state, is determined by the effect of spin fluctuations. It also shows that the theoretical consequences are largely in agreement with many experimental observations. The readers will therefore gain a new comprehensive perspective of their unified understanding of itinerant electron magnetism.

  15. Neutron scattering study on the spin dynamics of the two dimensional square lattice antiferromagnet, La2NiO4

    International Nuclear Information System (INIS)

    Nakajima, Kenji; Yamada, Kazuyoshi; Hosoya, Syoichi; Endoh, Yasuo; Omata, Tomoya; Arai, Masatoshi; Taylor, A.

    1993-01-01

    The spin dynamics of an S = 1, two dimensional (2D) square lattice antiferromagnet, La 2 NiO 4 was studied by neutron scattering experiments in wide energy (E N ), the spin wave excitations of La 2 NiO 4 are well described by a classical spin wave theory. The nearest-neighbor-exchange coupling constant, the in-plane and the out-of-plane anisotropy constants at 10 K were determined to be 28.7±0.7 meV, 0.10±0.02 meV and 1.26±0.12 meV, respectively. Above T N , the 2D spin fluctuation was observed over 600 K. The critical slowing down behavior of the fluctuation was observed in the enhancement of the low energy component toward T N . On the other hand, the high energy component is hardly affected by the three dimensional magnetic transition and still exists even at T N as observed in La 2 CuO 4 . The spin correlation length and the static structure factor at the 2D zone center were measured and compared with theoretical calculations for 2D Heisenberg antiferromagnets. (author)

  16. Dynamics of a driven spin coupled to an antiferromagnetic spin bath

    International Nuclear Information System (INIS)

    Yuan Xiaozhong; Goan, Hsi-Sheng; Zhu, Ka-Di

    2011-01-01

    We study the behavior of the Rabi oscillations of a driven central spin (qubit) coupled to an antiferromagnetic spin bath (environment). It is found that the decoherence behavior of the central spin depends on the detuning, driving strength, qubit-bath coupling and an important factor Ω, associated with the number of coupled atoms, the detailed lattice structure and the temperature of the environment. If detuning exists, Rabi oscillations may show the behavior of collapses and revivals; however, if detuning is absent, such a behavior will not appear. We investigate the weighted frequency distribution of the time evolution of the central spin inversion and give a reasonable explanation of this phenomenon of collapses and revivals. We also discuss the decoherence and pointer states of the qubit from the perspective of von Neumann entropy. We found that the eigenstates of the qubit self-Hamiltonian emerge as pointer states in the weak system-environment coupling limit.

  17. Superconductivity mediated by quantum critical antiferromagnetic fluctuations: The rise and fall of hot spots

    Science.gov (United States)

    Wang, Xiaoyu; Schattner, Yoni; Berg, Erez; Fernandes, Rafael M.

    2017-05-01

    In several unconventional superconductors, the highest superconducting transition temperature Tc is found in a region of the phase diagram where the antiferromagnetic transition temperature extrapolates to zero, signaling a putative quantum critical point. The elucidation of the interplay between these two phenomena—high-Tc superconductivity and magnetic quantum criticality—remains an important piece of the complex puzzle of unconventional superconductivity. In this paper, we combine sign-problem-free quantum Monte Carlo simulations and field-theoretical analytical calculations to unveil the microscopic mechanism responsible for the superconducting instability of a general low-energy model, called the spin-fermion model. In this approach, low-energy electronic states interact with each other via the exchange of quantum critical magnetic fluctuations. We find that even in the regime of moderately strong interactions, both the superconducting transition temperature and the pairing susceptibility are governed not by the properties of the entire Fermi surface, but instead by the properties of small portions of the Fermi surface called hot spots. Moreover, Tc increases with increasing interaction strength, until it starts to saturate at the crossover from hot-spots-dominated to Fermi-surface-dominated pairing. Our work provides not only invaluable insights into the system parameters that most strongly affect Tc, but also important benchmarks to assess the origin of superconductivity in both microscopic models and actual materials.

  18. Correlation functions of electronic and nuclear spins in a Heisenberg antiferromagnet semi-infinite medium

    International Nuclear Information System (INIS)

    Sarmento, E.F.

    1981-01-01

    Results are found for the dynamical correlation functions (or its corresponding Green's functions) among any combination including operator pairs of electronic and nuclear spins in an antiferromagnet semi-infinite medium, at low temperatures T [pt

  19. Collective spin fluctuations in diluted magnetic semiconductors

    Czech Academy of Sciences Publication Activity Database

    König, J.; Schliemann, J.; Jungwirth, Tomáš; MacDonald, A. H.

    2002-01-01

    Roč. 12, - (2002), s. 379-382 ISSN 1386-9477 Institutional research plan: CEZ:AV0Z1010914 Keywords : spin fluctuation * magnetic semiconductors Subject RIV: BM - Solid Matter Physics ; Magnetism Impact factor: 1.107, year: 2002

  20. External magnetic field induced anomalies of spin nuclear dynamics in thin antiferromagnetic films

    International Nuclear Information System (INIS)

    Tarasenko, S.V.

    1995-01-01

    It is shown that if the thickness of homogeneously magnetized plate of high-axial antiferromagnetic within H external magnetic field becomes lower the critical one, then the effect of dynamic magnetoelastic interaction on Soul-Nakamura exchange of nuclear spins results in formation of qualitatively new types of spreading nuclear spin waves no else compared neither within the model of unrestricted magnetic nor at H = 0 in case of thin plate of high-axial antiferromagnetic. 10 refs

  1. Antiferromagnetic spin phase transition in nuclear matter with effective Gogny interaction

    International Nuclear Information System (INIS)

    Isayev, A.A.; Yang, J.

    2004-01-01

    The possibility of ferromagnetic and antiferromagnetic phase transitions in symmetric nuclear matter is analyzed within the framework of a Fermi liquid theory with the effective Gogny interaction. It is shown that at some critical density nuclear matter with the D1S effective force undergoes a phase transition to the antiferromagnetic spin state (opposite directions of neutron and proton spins). The self-consistent equations of spin polarized nuclear matter with the D1S force have no solutions corresponding to ferromagnetic spin ordering (the same direction of neutron and proton spins) and, hence, the ferromagnetic transition does not appear. The dependence of the antiferromagnetic spin polarization parameter as a function of density is found at zero temperature

  2. Spin-orbit torque in two-dimensional antiferromagnetic topological insulators

    KAUST Repository

    Ghosh, Sumit; Manchon, Aurelien

    2017-01-01

    We investigate spin transport in two-dimensional ferromagnetic (FTI) and antiferromagnetic (AFTI) topological insulators. In the presence of an in-plane magnetization AFTI supports zero energy modes, which enables topologically protected edge conduction at low energy. We address the nature of current-driven spin torque in these structures and study the impact of spin-independent disorder. Interestingly, upon strong disorder the spin torque develops an antidamping component (i.e., even upon magnetization reversal) along the edges, which could enable current-driven manipulation of the antiferromagnetic order parameter. This antidamping torque decreases when increasing the system size and when the system enters the trivial insulator regime.

  3. Spin-orbit torque in two-dimensional antiferromagnetic topological insulators

    KAUST Repository

    Ghosh, Sumit

    2017-01-24

    We investigate spin transport in two-dimensional ferromagnetic (FTI) and antiferromagnetic (AFTI) topological insulators. In the presence of an in-plane magnetization AFTI supports zero energy modes, which enables topologically protected edge conduction at low energy. We address the nature of current-driven spin torque in these structures and study the impact of spin-independent disorder. Interestingly, upon strong disorder the spin torque develops an antidamping component (i.e., even upon magnetization reversal) along the edges, which could enable current-driven manipulation of the antiferromagnetic order parameter. This antidamping torque decreases when increasing the system size and when the system enters the trivial insulator regime.

  4. Signatures of a gearwheel quantum spin liquid in a spin-1/2 pyrochlore molybdate Heisenberg antiferromagnet

    Science.gov (United States)

    Iqbal, Yasir; Müller, Tobias; Riedl, Kira; Reuther, Johannes; Rachel, Stephan; Valentí, Roser; Gingras, Michel J. P.; Thomale, Ronny; Jeschke, Harald O.

    2017-12-01

    We theoretically investigate the low-temperature phase of the recently synthesized Lu2Mo2O5N2 material, an extraordinarily rare realization of a S =1 /2 three-dimensional pyrochlore Heisenberg antiferromagnet in which Mo5 + are the S =1 /2 magnetic species. Despite a Curie-Weiss temperature (ΘCW) of -121 (1 ) K, experiments have found no signature of magnetic ordering or spin freezing down to T*≈0.5 K. Using density functional theory, we find that the compound is well described by a Heisenberg model with exchange parameters up to third nearest neighbors. The analysis of this model via the pseudofermion functional renormalization group method reveals paramagnetic behavior down to a temperature of at least T =| ΘCW|/100 , in agreement with the experimental findings hinting at a possible three-dimensional quantum spin liquid. The spin susceptibility profile in reciprocal space shows momentum-dependent features forming a "gearwheel" pattern, characterizing what may be viewed as a molten version of a chiral noncoplanar incommensurate spiral order under the action of quantum fluctuations. Our calculated reciprocal space susceptibility maps provide benchmarks for future neutron scattering experiments on single crystals of Lu2Mo2O5N2 .

  5. Finding new superconductors: the spin-fluctuation gateway to high Tc and possible room temperature superconductivity.

    Science.gov (United States)

    Pines, David

    2013-10-24

    We propose an experiment-based strategy for finding new high transition temperature superconductors that is based on the well-established spin fluctuation magnetic gateway to superconductivity in which the attractive quasiparticle interaction needed for superconductivity comes from their coupling to dynamical spin fluctuations originating in the proximity of the material to an antiferromagnetic state. We show how lessons learned by combining the results of almost three decades of intensive experimental and theoretical study of the cuprates with those found in the decade-long study of a strikingly similar family of unconventional heavy electron superconductors, the 115 materials, can prove helpful in carrying out that search. We conclude that, since Tc in these materials scales approximately with the strength of the interaction, J, between the nearest neighbor local moments in their parent antiferromagnetic state, there may not be a magnetic ceiling that would prevent one from discovering a room temperature superconductor.

  6. Mechanisms for spin supersolidity in S=(1/2) spin-dimer antiferromagnets

    International Nuclear Information System (INIS)

    Picon, J.-D.; Albuquerque, A. F.; Schmidt, K. P.; Laflorencie, N.; Troyer, M.; Mila, F.

    2008-01-01

    Using perturbative expansions and the contractor renormalization (CORE) algorithm, we obtain effective hard-core bosonic Hamiltonians describing the low-energy physics of S=1/2 spin-dimer antiferromagnets known to display supersolid phases under an applied magnetic field. The resulting effective models are investigated by means of mean-field analysis and quantum Monte Carlo simulations. A ''leapfrog mechanism,'' through means of which extra singlets delocalize in a checkerboard-solid environment via correlated hoppings, is unveiled that accounts for the supersolid behavior

  7. Odd number of coupled antiferromagnetic anisotropic Heisenberg chains: Spin wave theory

    International Nuclear Information System (INIS)

    Benyoussef, A.

    1996-10-01

    The effect of the chain and perpendicular anisotropies on the energy gap for odd number of coupled quantum spin-1/2 antiferromagnetic anisotropic Heisenberg chains is investigated using a spin wave theory. The energy gap opens above a critical anisotropic value. The known results of the isotropic case have been obtained. (author). 11 refs, 4 figs

  8. Nuclear spin-magnon relaxation in two-dimensional Heisenberg antiferromagnets

    International Nuclear Information System (INIS)

    Wal, A.J. van der.

    1979-01-01

    Experiments are discussed of the dependence on temperature and magnetic field of the longitudinal relaxation time of single crystals of antiferromagnetically ordered insulators, i.e. in the temperature range below the Neel temperature and in fields up to the spin-flop transition. The experiments are done on 19 F nuclei in the Heisenberg antiferromagnets K 2 MnF 4 and K 2 NiF 4 , the magnetic structure of which is two-dimensional quadratic. (C.F.)

  9. Two-magnon Raman scattering in a spin density wave antiferromagnet

    OpenAIRE

    Schoenfeld, Friedhelm; Kampf, Arno P.; Mueller-Hartmann, Erwin

    1996-01-01

    We present the results for a model calculation of resonant two-magnon Raman scattering in a spin density wave (SDW) antiferromagnet. The resonant enhancement of the two-magnon intensity is obtained from a microscopic analysis of the photon-magnon coupling vertex. By combining magnon-magnon interactions with `triple resonance` phenomena in the vertex function the resulting intensity line shape is found to closely resemble the measured two-magnon Raman signal in antiferromagnetic cuprates. Both...

  10. Three-dimensional spin mapping of antiferromagnetic nanopyramids having spatially alternating surface anisotropy at room temperature.

    Science.gov (United States)

    Wang, Kangkang; Smith, Arthur R

    2012-11-14

    Antiferromagnets play a key role in modern spintronic devices owing to their ability to modify the switching behavior of adjacent ferromagnets via the exchange bias effect. Consequently, detailed measurements of the spin structure at antiferromagnetic interfaces and surfaces are highly desirable, not only for advancing technologies but also for enabling new insights into the underlying physics. Here using spin-polarized scanning tunneling microscopy at room-temperature, we reveal in three-dimensions an orthogonal spin structure on antiferromagnetic compound nanopyramids. Contrary to expected uniaxial anisotropy based on bulk properties, the atomic terraces are found to have alternating in-plane and out-of-plane magnetic anisotropies. The observed layer-wise alternation in anisotropy could have strong influences on future nanoscale spintronic applications.

  11. Real-space imaging of non-collinear antiferromagnetic order with a single-spin magnetometer

    Science.gov (United States)

    Gross, I.; Akhtar, W.; Garcia, V.; Martínez, L. J.; Chouaieb, S.; Garcia, K.; Carrétéro, C.; Barthélémy, A.; Appel, P.; Maletinsky, P.; Kim, J.-V.; Chauleau, J. Y.; Jaouen, N.; Viret, M.; Bibes, M.; Fusil, S.; Jacques, V.

    2017-09-01

    Although ferromagnets have many applications, their large magnetization and the resulting energy cost for switching magnetic moments bring into question their suitability for reliable low-power spintronic devices. Non-collinear antiferromagnetic systems do not suffer from this problem, and often have extra functionalities: non-collinear spin order may break space-inversion symmetry and thus allow electric-field control of magnetism, or may produce emergent spin-orbit effects that enable efficient spin-charge interconversion. To harness these traits for next-generation spintronics, the nanoscale control and imaging capabilities that are now routine for ferromagnets must be developed for antiferromagnetic systems. Here, using a non-invasive, scanning single-spin magnetometer based on a nitrogen-vacancy defect in diamond, we demonstrate real-space visualization of non-collinear antiferromagnetic order in a magnetic thin film at room temperature. We image the spin cycloid of a multiferroic bismuth ferrite (BiFeO3) thin film and extract a period of about 70 nanometres, consistent with values determined by macroscopic diffraction. In addition, we take advantage of the magnetoelectric coupling present in BiFeO3 to manipulate the cycloid propagation direction by an electric field. Besides highlighting the potential of nitrogen-vacancy magnetometry for imaging complex antiferromagnetic orders at the nanoscale, these results demonstrate how BiFeO3 can be used in the design of reconfigurable nanoscale spin textures.

  12. Correlation functions of electronic and nuclear spins in a Heisenberg antiferromagnet semi-infinite media

    International Nuclear Information System (INIS)

    Sarmento, E.F.

    1980-01-01

    Results are found for the correlation dynamic functions (or the correspondent green functions) between any combination including pairs of electronic anel nuclear spin operators in an antiferromagnet semi-infinite media., at low temperature T N . These correlation functions, are used to investigate, at the same time, the properties of surface spin waves in volume and surface. The dispersion relatons of nuclear and electronic spin waves coupled modes, in surface are found, resolving a system of linearized equatons of spin operators a system of linearized equations of spin operators. (author) [pt

  13. Spin-waves in antiferromagnetic single crystal LiFePO$_4$

    OpenAIRE

    Li, Jiying; Garlea, Vasile O.; Zarestky, Jerel L.; Vaknin, David

    2005-01-01

    Spin-wave dispersions in the antiferromagnetic state of single crystal LiFePO$_4$ were determined by inelastic neutron scattering measurements. The dispersion curves measured from the (010) reflection along both {\\it a}$^\\ast$ and {\\it b}$^\\ast$ reciprocal-space directions reflect the anisotropic coupling of the layered Fe$^{2+}$ (S = 2) spin-system. The spin-wave dispersion curves were theoretically modeled using linear spin-wave theory by including in the spin-Hamiltonian in-plane nearest- ...

  14. Magnonic quantum spin Hall state in the zigzag and stripe phases of the antiferromagnetic honeycomb lattice

    Science.gov (United States)

    Lee, Ki Hoon; Chung, Suk Bum; Park, Kisoo; Park, Je-Geun

    2018-05-01

    We investigated the topological property of magnon bands in the collinear magnetic orders of zigzag and stripe phases for the antiferromagnetic honeycomb lattice and identified Berry curvature and symmetry constraints on the magnon band structure. Different symmetries of both zigzag and stripe phases lead to different topological properties, in particular, the magnon bands of the stripe phase being disentangled with a finite Dzyaloshinskii-Moriya (DM) term with nonzero spin Chern number. This is corroborated by calculating the spin Nernst effect. Our study establishes the existence of a nontrivial magnon band topology for all observed collinear antiferromagnetic honeycomb lattices in the presence of the DM term.

  15. Spin-Hall effect and emergent antiferromagnetic phase transition in n-Si

    Science.gov (United States)

    Lou, Paul C.; Kumar, Sandeep

    2018-04-01

    Spin current experiences minimal dephasing and scattering in Si due to small spin-orbit coupling and spin-lattice interactions is the primary source of spin relaxation. We hypothesize that if the specimen dimension is of the same order as the spin diffusion length then spin polarization will lead to non-equilibrium spin accumulation and emergent phase transition. In n-Si, spin diffusion length has been reported up to 6 μm. The spin accumulation in Si will modify the thermal transport behavior of Si, which can be detected with thermal characterization. In this study, we report observation of spin-Hall effect and emergent antiferromagnetic phase transition behavior using magneto-electro-thermal transport characterization. The freestanding Pd (1 nm)/Ni80Fe20 (75 nm)/MgO (1 nm)/n-Si (2 μm) thin film specimen exhibits a magnetic field dependent thermal transport and spin-Hall magnetoresistance behavior attributed to Rashba effect. An emergent phase transition is discovered using self-heating 3ω method, which shows a diverging behavior at 270 K as a function of temperature similar to a second order phase transition. We propose that spin-Hall effect leads to the spin accumulation and resulting emergent antiferromagnetic phase transition. We propose that the length scale for Rashba effect can be equal to the spin diffusion length and two-dimensional electron gas is not essential for it. The emergent antiferromagnetic phase transition is attributed to the site inversion asymmetry in diamond cubic Si lattice.

  16. Nuclear spin relaxation in a spin-1/2 antiferromagnetic Heisenberg chain at high fields

    International Nuclear Information System (INIS)

    Lyo, S.K.

    1981-01-01

    The proton spin relaxation rate is calculated in the one-dimensional spin-1/2 Heisenberg antiferromagnet α-bis (N-methylsalicylaldiminato)-copper (II), α-CuNSal by using a fermion representation for magnons above the critical field where the magnon spectrum develops a gap. The one-magnon process which is dominant below the critical field is shown to be absent in the presence of a gap in contrast to a previous theory. Instead, we find that the three-magnon rate is large enough to explain the data at low fields. The two-magnon off-resonance damping which enters the expression for the three-magnon rate is calculated by solving the two-magnon scattering exactly, leading to a much smaller value of the rate than that predicted by the Born approximation. Also, in an unsuccessful attempt to resolve the discrepancy between the recently calculated two-magnon rate (dominant at high fields) and the data of α-CuNSal reported by Azevedo et al., we carry out the vertex correction for the spin-density correlation function by summing the RPA series as well as the exchange ladders for the polarization part. We find that, although the exchange enhancement is significantly large, it is nearly canceled out by the RPA correction, and the net effect of the vertex correction is small. This result agrees with the recent data of the similar spin-1/2 antiferromagnetic Heisenberg chain system CuSO 4 x5H 2 O reported by Groen et al. On the other hand, it disagrees with a recent calculation of the two-magnon rate based on a boson representation of spins. To resolve this discrepancy we examine the effect of the boson self-energy correction on the two-magnon rate. The boson spectral shift is found to be quite large in the region where the cited two-boson rate deviates from the two-fermion rate. As a result the two-boson rate is significantly reduced, leading to reasonable agreement with the two-fermion rate

  17. Vectorial mapping of noncollinear antiferromagnetic structure of semiconducting FeSe surface with spin-polarized scanning tunneling microscopy

    Energy Technology Data Exchange (ETDEWEB)

    Zhang, K. F.; Yang, Fang; Song, Y. R. [Key Laboratory of Artificial Structures and Quantum Control (Ministry of Education), Department of Physics and Astronomy, Shanghai Jiao Tong University, Shanghai 200240 (China); Zhang, Xiaole [Institute of Natural Sciences, Shanghai Jiao Tong University, Shanghai 200240 (China); The State Key Laboratory of Advanced Optical Communication Systems and Networks, Department of Physics and Astronomy, Shanghai Jiao Tong University, Shanghai 200240 (China); Chen, Xianfeng [The State Key Laboratory of Advanced Optical Communication Systems and Networks, Department of Physics and Astronomy, Shanghai Jiao Tong University, Shanghai 200240 (China); Liu, Canhua; Qian, Dong; Gao, C. L., E-mail: clgao@sjtu.edu.cn; Jia, Jin-Feng [Key Laboratory of Artificial Structures and Quantum Control (Ministry of Education), Department of Physics and Astronomy, Shanghai Jiao Tong University, Shanghai 200240 (China); Collaborative Innovation Center of Advanced Microstructures, Nanjing (China); Luo, Weidong, E-mail: wdluo@sjtu.edu.cn [Key Laboratory of Artificial Structures and Quantum Control (Ministry of Education), Department of Physics and Astronomy, Shanghai Jiao Tong University, Shanghai 200240 (China); Institute of Natural Sciences, Shanghai Jiao Tong University, Shanghai 200240 (China); Collaborative Innovation Center of Advanced Microstructures, Nanjing (China)

    2016-02-08

    Antiferromagnetic semiconductors gain increasing interest due to their possible application in spintronics. Using spin polarized scanning tunneling microscopy operating in a vector field, we mapped the noncollinear antiferromagnetic spin structure of a semiconducting hexagonal FeSe surface on the atomic scale. The surface possesses an in-plane compensated Néel structure which is further confirmed by first-principles calculations.

  18. Vectorial mapping of noncollinear antiferromagnetic structure of semiconducting FeSe surface with spin-polarized scanning tunneling microscopy

    International Nuclear Information System (INIS)

    Zhang, K. F.; Yang, Fang; Song, Y. R.; Zhang, Xiaole; Chen, Xianfeng; Liu, Canhua; Qian, Dong; Gao, C. L.; Jia, Jin-Feng; Luo, Weidong

    2016-01-01

    Antiferromagnetic semiconductors gain increasing interest due to their possible application in spintronics. Using spin polarized scanning tunneling microscopy operating in a vector field, we mapped the noncollinear antiferromagnetic spin structure of a semiconducting hexagonal FeSe surface on the atomic scale. The surface possesses an in-plane compensated Néel structure which is further confirmed by first-principles calculations

  19. Spin-motive Force Induced by Domain Wall Dynamics in the Antiferromagnetic Spin Valve

    Science.gov (United States)

    Sugano, Ryoko; Ichimura, Masahiko; Takahashi, Saburo; Maekawa, Sadamichi; Crest Collaboration

    2014-03-01

    In spite of no net magnetization in antiferromagnetic (AF) textures, the local magnetic properties (Neel magnetization) can be manipulated in a similar fashion to ferromagnetic (F) ones. It is expected that, even in AF metals, spin transfer torques (STTs) lead to the domain wall (DW) motion and that the DW motion induces spin-motive force (SMF). In order to study the Neel magnetization dynamics and the resultant SMF, we treat the nano-structured F1/AF/F2 junction. The F1 and F2 leads behave as a spin current injector and a detector, respectively. Each F lead is fixed in the different magnetization direction. Torsions (DW in AF) are introduced reflecting the fixed magnetization of two F leads. We simulated the STT-induced Neel magnetization dynamics with the injecting current from F1 to F2 and evaluate induced SMF. Based on the adiabatic electron dynamics in the AF texture, Langevin simulations are performed at finite temperature. This research was supported by JST, CREST, Japan.

  20. Spin-orbit torques in locally and globally noncentrosymmetric crystals: Antiferromagnets and ferromagnets

    KAUST Repository

    Železný, J.

    2017-01-10

    One of the main obstacles that prevents practical applications of antiferromagnets is the difficulty of manipulating the magnetic order parameter. Recently, following the theoretical prediction [J. Železný, Phys. Rev. Lett. 113, 157201 (2014)]PRLTAO0031-900710.1103/PhysRevLett.113.157201, the electrical switching of magnetic moments in an antiferromagnet was demonstrated [P. Wadley, Science 351, 587 (2016)]SCIEAS0036-807510.1126/science.aab1031. The switching is due to the so-called spin-orbit torque, which has been extensively studied in ferromagnets. In this phenomena a nonequilibrium spin-polarization exchange coupled to the ordered local moments is induced by current, hence exerting a torque on the order parameter. Here we give a general systematic analysis of the symmetry of the spin-orbit torque in locally and globally noncentrosymmetric crystals. We study when the symmetry allows for a nonzero torque, when is the torque effective, and its dependence on the applied current direction and orientation of magnetic moments. For comparison, we consider both antiferromagnetic and ferromagnetic orders. In two representative model crystals we perform microscopic calculations of the spin-orbit torque to illustrate its symmetry properties and to highlight conditions under which the spin-orbit torque can be efficient for manipulating antiferromagnetic moments.

  1. Spin-orbit torques in locally and globally noncentrosymmetric crystals: Antiferromagnets and ferromagnets

    KAUST Repository

    Železný , J.; Gao, H.; Manchon, Aurelien; Freimuth, Frank; Mokrousov, Yuriy; Zemen, J.; Mašek, J.; Sinova, Jairo; Jungwirth, T.

    2017-01-01

    One of the main obstacles that prevents practical applications of antiferromagnets is the difficulty of manipulating the magnetic order parameter. Recently, following the theoretical prediction [J. Železný, Phys. Rev. Lett. 113, 157201 (2014)]PRLTAO0031-900710.1103/PhysRevLett.113.157201, the electrical switching of magnetic moments in an antiferromagnet was demonstrated [P. Wadley, Science 351, 587 (2016)]SCIEAS0036-807510.1126/science.aab1031. The switching is due to the so-called spin-orbit torque, which has been extensively studied in ferromagnets. In this phenomena a nonequilibrium spin-polarization exchange coupled to the ordered local moments is induced by current, hence exerting a torque on the order parameter. Here we give a general systematic analysis of the symmetry of the spin-orbit torque in locally and globally noncentrosymmetric crystals. We study when the symmetry allows for a nonzero torque, when is the torque effective, and its dependence on the applied current direction and orientation of magnetic moments. For comparison, we consider both antiferromagnetic and ferromagnetic orders. In two representative model crystals we perform microscopic calculations of the spin-orbit torque to illustrate its symmetry properties and to highlight conditions under which the spin-orbit torque can be efficient for manipulating antiferromagnetic moments.

  2. Itinerant spin dynamics in iron-based superconductors and cerium-based heavy-fermion antiferromagnets

    Energy Technology Data Exchange (ETDEWEB)

    Friemel, Gerd

    2014-05-26

    This thesis contains a comprehensive study of the spin excitations by inelastic neutron scattering (INS) in two different correlated electron systems: the alkali-metal iron selenide superconductors (FeSe122) A{sub x}Fe{sub 2-y}Se{sub 2} (A=K, Rb, Cs) and the heavy-fermion antiferromagnet CeB6. Both systems exhibit intense modes in their spin-fluctuation spectrum below their respective transition temperatures that can be derived from the spin dynamics of the itinerant quasiparticles. However, the implications of these observations, presented here, are different for each particular compound. The A{sub x}Fe{sub 2-y}Se{sub 2} superconductors, with a uniform T{sub c} of 32 K, belong to a qualitative new family of superconductors. They possess a distinctly different Fermi surface compared to the iron-arsenide-based analogues XFe{sub 2}As{sub 2} (X=Ca, Sr, Ba). Instead of the central hole pockets at Γ and the electron pockets at X((1)/(2) 0), which are nested by the Q{sub AFM} = ((1)/(2) 0) vector, there exist only large electron pockets at the X point. Therefore, the magnetic instability along Q{sub AFM} that presumably provides the pairing glue for the superconductivity in the shape of spin fluctuations is absent in the FeSe122. The search for spin fluctuations by INS was motivated by a theoretical analysis that predicted their presence at an incommensurate wave vector near Q = (0.5 δ), δ = 0.3125 which results from a quasinesting by Q between the flat parts of the electron pockets. Two samples, namely Rb{sub 0.8}Fe{sub 1.6}Se{sub 2} and K{sub 0.77}Fe{sub 1.85}Se{sub 2}, were prepared and both showed a sizable anisotropic magnetic response at Q{sub sf} = ((1)/(2) (1)/(4)) in the normal state. Furthermore, upon entering the superconducting (SC) state a strong excitation appears at ℎω{sub res} = 14 meV in the spectrum at Q{sub sf}, which is referred to as magnetic resonant mode. This mode is interpreted as a bound spin-1 exciton below the SC charge gap. Its presence

  3. Itinerant spin dynamics in iron-based superconductors and cerium-based heavy-fermion antiferromagnets

    International Nuclear Information System (INIS)

    Friemel, Gerd

    2014-01-01

    This thesis contains a comprehensive study of the spin excitations by inelastic neutron scattering (INS) in two different correlated electron systems: the alkali-metal iron selenide superconductors (FeSe122) A x Fe 2-y Se 2 (A=K, Rb, Cs) and the heavy-fermion antiferromagnet CeB6. Both systems exhibit intense modes in their spin-fluctuation spectrum below their respective transition temperatures that can be derived from the spin dynamics of the itinerant quasiparticles. However, the implications of these observations, presented here, are different for each particular compound. The A x Fe 2-y Se 2 superconductors, with a uniform T c of 32 K, belong to a qualitative new family of superconductors. They possess a distinctly different Fermi surface compared to the iron-arsenide-based analogues XFe 2 As 2 (X=Ca, Sr, Ba). Instead of the central hole pockets at Γ and the electron pockets at X((1)/(2) 0), which are nested by the Q AFM = ((1)/(2) 0) vector, there exist only large electron pockets at the X point. Therefore, the magnetic instability along Q AFM that presumably provides the pairing glue for the superconductivity in the shape of spin fluctuations is absent in the FeSe122. The search for spin fluctuations by INS was motivated by a theoretical analysis that predicted their presence at an incommensurate wave vector near Q = (0.5 δ), δ = 0.3125 which results from a quasinesting by Q between the flat parts of the electron pockets. Two samples, namely Rb 0.8 Fe 1.6 Se 2 and K 0.77 Fe 1.85 Se 2 , were prepared and both showed a sizable anisotropic magnetic response at Q sf = ((1)/(2) (1)/(4)) in the normal state. Furthermore, upon entering the superconducting (SC) state a strong excitation appears at ℎω res = 14 meV in the spectrum at Q sf , which is referred to as magnetic resonant mode. This mode is interpreted as a bound spin-1 exciton below the SC charge gap. Its presence implies an unconventional order parameter, which changes the sign between the electron

  4. Nonlocally sensing the magnetic states of nanoscale antiferromagnets with an atomic spin sensor.

    Science.gov (United States)

    Yan, Shichao; Malavolti, Luigi; Burgess, Jacob A J; Droghetti, Andrea; Rubio, Angel; Loth, Sebastian

    2017-05-01

    The ability to sense the magnetic state of individual magnetic nano-objects is a key capability for powerful applications ranging from readout of ultradense magnetic memory to the measurement of spins in complex structures with nanometer precision. Magnetic nano-objects require extremely sensitive sensors and detection methods. We create an atomic spin sensor consisting of three Fe atoms and show that it can detect nanoscale antiferromagnets through minute, surface-mediated magnetic interaction. Coupling, even to an object with no net spin and having vanishing dipolar stray field, modifies the transition matrix element between two spin states of the Fe atom-based spin sensor that changes the sensor's spin relaxation time. The sensor can detect nanoscale antiferromagnets at up to a 3-nm distance and achieves an energy resolution of 10 μeV, surpassing the thermal limit of conventional scanning probe spectroscopy. This scheme permits simultaneous sensing of multiple antiferromagnets with a single-spin sensor integrated onto the surface.

  5. Nonlocally sensing the magnetic states of nanoscale antiferromagnets with an atomic spin sensor

    Science.gov (United States)

    Yan, Shichao; Malavolti, Luigi; Burgess, Jacob A. J.; Droghetti, Andrea; Rubio, Angel; Loth, Sebastian

    2017-01-01

    The ability to sense the magnetic state of individual magnetic nano-objects is a key capability for powerful applications ranging from readout of ultradense magnetic memory to the measurement of spins in complex structures with nanometer precision. Magnetic nano-objects require extremely sensitive sensors and detection methods. We create an atomic spin sensor consisting of three Fe atoms and show that it can detect nanoscale antiferromagnets through minute, surface-mediated magnetic interaction. Coupling, even to an object with no net spin and having vanishing dipolar stray field, modifies the transition matrix element between two spin states of the Fe atom–based spin sensor that changes the sensor’s spin relaxation time. The sensor can detect nanoscale antiferromagnets at up to a 3-nm distance and achieves an energy resolution of 10 μeV, surpassing the thermal limit of conventional scanning probe spectroscopy. This scheme permits simultaneous sensing of multiple antiferromagnets with a single-spin sensor integrated onto the surface. PMID:28560346

  6. Extended quantum critical phase in a magnetized spin-1/2 antiferromagnetic chain

    DEFF Research Database (Denmark)

    Stone, M.B.; Reich, D.H.; Broholm, C.

    2003-01-01

    Measurements are reported of the magnetic field dependence of excitations in the quantum critical state of the spin S=1/2 linear chain Heisenberg antiferromagnet copper pyrazine dinitrate (CuPzN). The complete spectrum was measured at k(B)T/Jless than or equal to0.025 for H=0 and H=8.7 T, where...

  7. Spin-transfer torques in antiferromagnetic textures: efficiency and quantification method

    Czech Academy of Sciences Publication Activity Database

    Yamane, Y.; Ieda, J.; Sinova, Jairo

    2016-01-01

    Roč. 94, č. 5 (2016), 1-8, č. článku 054409. ISSN 2469-9950 R&D Projects: GA ČR GB14-37427G Institutional support: RVO:68378271 Keywords : spin-transfer torques * antiferromagnets Subject RIV: BL - Plasma and Gas Discharge Physics Impact factor: 3.836, year: 2016

  8. Adiabatic demagnetization of the antiferromagnetic spin-1/2 Heisenberg hexagonal cluster

    International Nuclear Information System (INIS)

    Deb, Moumita; Ghosh, Asim Kumar

    2016-01-01

    Exact analytic expressions of eigenvalues of the antiferromagnetic spin-1/2 Heisenberg hexagon in the presence of uniform magnetic field have been obtained. Magnetization process, nature of isentrops and properties of magneto caloric effect in terms of adiabatic demagnetization have been investigated. Theoretical results have been used to study the magneto caloric effect of the spin-1/2 Heisenberg hexagonal compound Cu_3WO_6.

  9. Antiferromagnetic Ising model decorated with D-vector spins: Transversal and longitudinal local fields effects

    International Nuclear Information System (INIS)

    Vasconcelos Dos Santos, R.J.; Coutinho, S.

    1995-01-01

    The effect of a local field acting on decorating classical D-vector bond spins of an antiferromagnetic Ising model on the square lattice is studied for both the annealed isotropic and the axial decorated cases. In both models the effect on the phase diagrams of the transversal and the longitudinal components of the local field acting on the decorating spins are fully analyzed and discussed

  10. Skyrmion dynamics in single-hole Neel ordered doped two-dimensional antiferromagnets with arbitrary spin

    International Nuclear Information System (INIS)

    Moura, A.R.; Pereira, A.R.; Moura-Melo, W.A.; Pires, A.S.T.

    2008-01-01

    We develop an effective theory to study the skyrmion dynamics in the presence of a hole (removed spins from the lattice) in Neel ordered two-dimensional antiferromagnets with arbitrary spin value S. The general equation of motion for the 'mass center' of this structure is obtained. The frequency of small amplitude oscillations of pinned skyrmions around the defect center is calculated. It is proportional to the hole size and inversely proportional to the square of the skyrmion size

  11. Strong Coupling of Microwave Photons to Antiferromagnetic Fluctuations in an Organic Magnet

    Science.gov (United States)

    Mergenthaler, Matthias; Liu, Junjie; Le Roy, Jennifer J.; Ares, Natalia; Thompson, Amber L.; Bogani, Lapo; Luis, Fernando; Blundell, Stephen J.; Lancaster, Tom; Ardavan, Arzhang; Briggs, G. Andrew D.; Leek, Peter J.; Laird, Edward A.

    2017-10-01

    Coupling between a crystal of di(phenyl)-(2,4,6-trinitrophenyl)iminoazanium radicals and a superconducting microwave resonator is investigated in a circuit quantum electrodynamics (circuit QED) architecture. The crystal exhibits paramagnetic behavior above 4 K, with antiferromagnetic correlations appearing below this temperature, and we demonstrate strong coupling at base temperature. The magnetic resonance acquires a field angle dependence as the crystal is cooled down, indicating anisotropy of the exchange interactions. These results show that multispin modes in organic crystals are suitable for circuit QED, offering a platform for their coherent manipulation. They also utilize the circuit QED architecture as a way to probe spin correlations at low temperature.

  12. Antiferromagnetic Spin Coupling between Rare Earth Adatoms and Iron Islands Probed by Spin-Polarized Tunneling.

    Science.gov (United States)

    Coffey, David; Diez-Ferrer, José Luis; Serrate, David; Ciria, Miguel; de la Fuente, César; Arnaudas, José Ignacio

    2015-09-03

    High-density magnetic storage or quantum computing could be achieved using small magnets with large magnetic anisotropy, a requirement that rare-earth iron alloys fulfill in bulk. This compelling property demands a thorough investigation of the magnetism in low dimensional rare-earth iron structures. Here, we report on the magnetic coupling between 4f single atoms and a 3d magnetic nanoisland. Thulium and lutetium adatoms deposited on iron monolayer islands pseudomorphically grown on W(110) have been investigated at low temperature with scanning tunneling microscopy and spectroscopy. The spin-polarized current indicates that both kind of adatoms have in-plane magnetic moments, which couple antiferromagnetically with their underlying iron islands. Our first-principles calculations explain the observed behavior, predicting an antiparallel coupling of the induced 5d electrons magnetic moment of the lanthanides with the 3d magnetic moment of iron, as well as their in-plane orientation, and pointing to a non-contribution of 4f electrons to the spin-polarized tunneling processes in rare earths.

  13. Evolution of Spin fluctuations in CaFe2As2 with Co-doping.

    Science.gov (United States)

    Sapkota, A.; Das, P.; Böhmer, A. E.; Abernathy, D. L.; Canfield, P. C.; Kreyssig, A.; McQueeney, R. J.; Goldman, A. I.

    Spin fluctuations are an essential ingredient for superconductivity in Fe-based supercondcutors. In Co-doped BaFe2As2, the system goes from the antiferromagnetic (AFM) state to the superconducting (SC) state with Co doping, and the spin fluctuations also evolve from well-defined spin waves with spin gap in the AFM regime to gapless overdamped or diffused fluctuations in the SC regime. CaFe2As2 has a stronger magneto-elastic coupling than BaFe2As2 and no co-existence of SC and AFM region as observed in BaFe2As2 with Co doping. Here, we will discuss the evolution of spin fluctuations in CaFe2As2 with Co doping. Work at the Ames Laboratory was supported by US DOE, Basic Energy Sciences, Division of Material Sciences and Engineering, under contract No. DE-AC02-07CH11358. This research used resources of SNS, a DOE office of science user facility operated by ORNL.

  14. Effect of antiferromagnetic interfacial coupling on spin-wave resonance frequency of multi-layer film

    Energy Technology Data Exchange (ETDEWEB)

    Qiu, Rong-ke, E-mail: rkqiu@163.com; Cai, Wei

    2017-08-15

    Highlights: • A quantum approach is developed to study the SWR of a bicomponent multi-layer films. • The comparison of the SWR in films with FM and AFM interfacial coupling has been made. • The present results show the method to enhance and adjust the SWR frequency of films. - Abstract: We investigate the spin-wave resonance (SWR) frequency in a bicomponent bilayer and triple-layer films with antiferromagnetic or ferromagnetic interfacial couplings, as function of interfacial coupling, surface anisotropy, interface anisotropy, thickness and external magnetic field, using the linear spin-wave approximation and Green’s function technique. The microwave properties for multi-layer magnetic film with antiferromagnetic interfacial coupling is different from those for multi-layer magnetic film with ferromagnetic interfacial coupling. For the bilayer film with antiferromagnetic interfacial couplings, as the lower (upper) surface anisotropy increases, only the SWR frequencies of the odd (even) number modes increase. The lower (upper) surface anisotropy does not affect the SWR frequencies of the even (odd) number modes{sub .} For the multi-layer film with antiferromagnetic interfacial coupling, the SWR frequency of modes m = 1, 3 and 4 decreases while that of mode m = 2 increases with increasing thickness of the film within a proper parameter region. The present results could be useful in enhancing our fundamental understanding and show the method to enhance and adjust the SWR frequency of bicomponent multi-layer magnetic films with antiferromagnetic or ferromagnetic interfacial coupling.

  15. Superconducting quasiparticle lifetimes due to spin-fluctuation scattering

    International Nuclear Information System (INIS)

    Quinlan, S.M.; Scalapino, D.J.; Bulut, N.

    1994-01-01

    Superconducting quasiparticle lifetimes associated with spin-fluctuation scattering are calculated. A Berk-Schrieffer interaction with an irreducible susceptibility given by a BCS form is used to model the quasiparticle damping due to spin fluctuations. Results are presented for both s-wave and d-wave gaps. Also, quasiparticle lifetimes due to impurity scattering are calculated for a d-wave superconductor

  16. Fe-induced enhancement of antiferromagnetic spin correlations in Mn2-xFexBO4

    Science.gov (United States)

    Kazak, N. V.; Platunov, M. S.; Knyazev, Yu. V.; Moshkina, E. M.; Gavrilkin, S. Yu.; Bayukov, O. A.; Gorev, M. V.; Pogoreltsev, E. I.; Zeer, G. M.; Zharkov, S. M.; Ovchinnikov, S. G.

    2018-04-01

    Fe substitution effect on the magnetic behavior of Mn2-xFexBO4 (x = 0.3, 0.5, 0.7) warwickites has been investigated combining Mössbauer spectroscopy, dc magnetization, ac magnetic susceptibility, and heat capacity measurements. The Fe3+ ions distribution over two crystallographic nonequivalent sites is studied. The Fe introduction breaks a long-range antiferromagnetic order and leads to onset of spin-glass ground state. The antiferromagnetic short-range-order spin correlations persist up to temperatures well above TSG reflecting in increasing deviations from the Curie-Weiss law, the reduced effective magnetic moment and "missing" entropy. The results are interpreted in the terms of the progressive increase of the frustration effect and the formation of spin-correlated regions.

  17. Spin-Driven Emergent Antiferromagnetism and Metal-Insulator Transition in Nanoscale p-Si

    Science.gov (United States)

    Lou, Paul C.; Kumar, Sandeep

    2018-04-01

    The entanglement of the charge, spin and orbital degrees of freedom can give rise to emergent behavior especially in thin films, surfaces and interfaces. Often, materials that exhibit those properties require large spin orbit coupling. We hypothesize that the emergent behavior can also occur due to spin, electron and phonon interactions in widely studied simple materials such as Si. That is, large intrinsic spin-orbit coupling is not an essential requirement for emergent behavior. The central hypothesis is that when one of the specimen dimensions is of the same order (or smaller) as the spin diffusion length, then non-equilibrium spin accumulation due to spin injection or spin-Hall effect (SHE) will lead to emergent phase transformations in the non-ferromagnetic semiconductors. In this experimental work, we report spin mediated emergent antiferromagnetism and metal insulator transition in a Pd (1 nm)/Ni81Fe19 (25 nm)/MgO (1 nm)/p-Si (~400 nm) thin film specimen. The spin-Hall effect in p-Si, observed through Rashba spin-orbit coupling mediated spin-Hall magnetoresistance behavior, is proposed to cause the spin accumulation and resulting emergent behavior. The phase transition is discovered from the diverging behavior in longitudinal third harmonic voltage, which is related to the thermal conductivity and heat capacity.

  18. Spin-lattice effects in selected antiferromagnetic materials

    Czech Academy of Sciences Publication Activity Database

    Zherlitsyn, S.; Yasin, S.; Wosnitza, J.; Zvyagin, A.A.; Andreev, Alexander V.; Tsurkan, V.

    2014-01-01

    Roč. 40, č. 2 (2014), s. 123-133 ISSN 1063-777X R&D Projects: GA ČR GAP204/12/0150 Grant - others:AVČR(CZ) M100101203 Keywords : low-dimensional spin systems * frustrated chromium spinels * spin-strain interaction * uranium -based compounds Subject RIV: BM - Solid Matter Physics ; Magnetism Impact factor: 0.786, year: 2014

  19. Magnetic order, magnetic correlations, and spin dynamics in the pyrochlore antiferromagnet Er2Ti2O7

    Science.gov (United States)

    Dalmas de Réotier, P.; Yaouanc, A.; Chapuis, Y.; Curnoe, S. H.; Grenier, B.; Ressouche, E.; Marin, C.; Lago, J.; Baines, C.; Giblin, S. R.

    2012-09-01

    Er2Ti2O7 is believed to be a realization of an XY antiferromagnet on a frustrated lattice of corner-sharing regular tetrahedra. It is presented as an example of the order-by-disorder mechanism in which fluctuations lift the degeneracy of the ground state, leading to an ordered state. Here we report detailed measurements of the low-temperature magnetic properties of Er2Ti2O7, which displays a second-order phase transition at TN≃1.2 K with coexisting short- and long-range orders. Magnetic susceptibility studies show that there is no spin-glass-like irreversible effect. Heat capacity measurements reveal that the paramagnetic critical exponent is typical of a 3-dimensional XY magnet while the low-temperature specific heat sets an upper limit on the possible spin-gap value and provides an estimate for the spin-wave velocity. Muon spin relaxation measurements show the presence of spin dynamics in the nanosecond time scale down to 21 mK. This time range is intermediate between the shorter time characterizing the spin dynamics in Tb2Sn2O7, which also displays long- and short-range magnetic order, and the time scale typical of conventional magnets. Hence the ground state is characterized by exotic spin dynamics. We determine the parameters of a symmetry-dictated Hamiltonian restricted to the spins in a tetrahedron, by fitting the paramagnetic diffuse neutron scattering intensity for two reciprocal lattice planes. These data are recorded in a temperature region where the assumption that the correlations are limited to nearest neighbors is fair.

  20. Dynamic selective switching in antiferromagnetically-coupled bilayers close to the spin reorientation transition

    International Nuclear Information System (INIS)

    Fernández-Pacheco, A.; Mansell, R.; Petit, D.; Lee, J. H.; Cowburn, R. P.; Ummelen, F. C.; Swagten, H. J. M.

    2014-01-01

    We have designed a bilayer synthetic antiferromagnet where the order of layer reversal can be selected by varying the sweep rate of the applied magnetic field. The system is formed by two ultra-thin ferromagnetic layers with different proximities to the spin reorientation transition, coupled antiferromagnetically using Ruderman-Kittel-Kasuya-Yosida interactions. The different dynamic magnetic reversal behavior of both layers produces a crossover in their switching fields for field rates in the kOe/s range. This effect is due to the different effective anisotropy of both layers, added to an appropriate asymmetric antiferromagnetic coupling between them. Field-rate controlled selective switching of perpendicular magnetic anisotropy layers as shown here can be exploited in sensing and memory applications.

  1. Collinear order in the frustrated spin-(1)/(2) antiferromagnet Li{sub 2}CuW{sub 2}O{sub 8}

    Energy Technology Data Exchange (ETDEWEB)

    Tsirlin, Alexander A. [NICPB, Tallinn (Estonia); Nath, Ramesh; Ranjith, Kumar [Indian Institute of Science Education and Research, Trivandrum (India); Kasinathan, Deepa [MPI CPfS, Dresden (Germany); Skoulatos, Markos [Laboratory of Neutron Scattering, PSI, Villigen (Switzerland)

    2015-07-01

    Li{sub 2}CuW{sub 2}O{sub 8} is a three-dimensional spin-(1)/(2) antiferromagnet that features collinear spin order despite abundant magnetic frustration that would normally trigger a non-collinear incommensurate order, at least on the classical level. Using density-functional calculations, we establish the spin lattice comprising two non-coplanar triangular networks that introduce frustration along all three crystallographic directions. Magnetic susceptibility and heat capacity reveal a 1D-like magnetic response, which is, however, inconsistent with the naive spin-chain model. Moreover, the high saturation field of 29 T compared to the susceptibility maximum at as low as 8.5 K give strong evidence for the importance of interchain couplings and the magnetic frustration. Below T{sub N} ≅ 3.9 K, Li{sub 2}CuW{sub 2}O{sub 8} develops collinear magnetic order with parallel spins along a and c and antiparallel spins along b. The ordered moment is about 0.7 μ{sub B} according to neutron powder diffraction. This qualifies Li{sub 2}CuW{sub 2}O{sub 8} as a unique three-dimensional spin-(1)/(2) antiferromagnet, where collinear magnetic order is stabilized by quantum fluctuations.

  2. Magnetic Raman Scattering in Two-Dimensional Spin-1/2 Heisenberg Antiferromagnets: Explanation of the Spectral Shape Anomaly

    Science.gov (United States)

    Nori, F.; Merlin, R.; Haas, S.; Sandvick, A.; Dagotto, E.

    1996-03-01

    We calculate(F. Nori, R.Merlin, S. Haas, A.W. Sandvik, and E. Dagotto, Physical Review Letters) 75, 553 (1995). the Raman spectrum of the two-dimensional (2D) spin-1/2 Heisenberg antiferromagnet by exact diagonalization and quantum Monte Carlo techniques on clusters of up to 144 sites. On a 16-site cluster, we consider the phonon-magnon interaction which leads to random fluctuations of the exchange integral. Results are in good agreement with experiments on various high-Tc precursors, such as La_2CuO4 and YBa_2Cu_3O_6.2. In particular, our calculations reproduce the broad lineshape of the two-magnon peak, the asymmetry about its maximum, the existence of spectral weight at high energies, and the observation of nominally forbidden A_1g scattering.

  3. Dynamical Negative Differential Resistance in Antiferromagnetically Coupled Few-Atom Spin Chains

    Science.gov (United States)

    Rolf-Pissarczyk, Steffen; Yan, Shichao; Malavolti, Luigi; Burgess, Jacob A. J.; McMurtrie, Gregory; Loth, Sebastian

    2017-11-01

    We present the appearance of negative differential resistance (NDR) in spin-dependent electron transport through a few-atom spin chain. A chain of three antiferromagnetically coupled Fe atoms (Fe trimer) was positioned on a Cu2 N /Cu (100 ) surface and contacted with the spin-polarized tip of a scanning tunneling microscope, thus coupling the Fe trimer to one nonmagnetic and one magnetic lead. Pronounced NDR appears at the low bias of 7 mV, where inelastic electron tunneling dynamically locks the atomic spin in a long-lived excited state. This causes a rapid increase of the magnetoresistance between the spin-polarized tip and Fe trimer and quenches elastic tunneling. By varying the coupling strength between the tip and Fe trimer, we find that in this transport regime the dynamic locking of the Fe trimer competes with magnetic exchange interaction, which statically forces the Fe trimer into its high-magnetoresistance state and removes the NDR.

  4. Spin-waves in Antiferromagnetic Single-crystal LiFePO4

    International Nuclear Information System (INIS)

    Li, Jiying; Garlea, Vasile O.; Zarestky, Jarel; Vaknin, D.

    2006-01-01

    Spin-wave dispersions in the antiferromagnetic state of single-crystal LiFePO 4 were determined by inelastic neutron scattering measurements. The dispersion curves measured from the (0,1,0) reflection along both a* and b* reciprocal-space directions reflect the anisotropic coupling of the layered Fe 2+ (S=2) spin system. The spin-wave dispersion curves were theoretically modeled using linear spin-wave theory by including in the spin Hamiltonian in-plane nearest- and next-nearest-neighbor interactions (J 1 and J 2 ), inter-plane nearest-neighbor interactions (J(perpendicular)) and a single-ion anisotropy (D). A weak (0,1,0) magnetic peak was observed in elastic neutron scattering studies of the same crystal indicating that the ground state of the staggered iron moments is not along the (0,1,0) direction, as previously reported from polycrystalline samples studies, but slightly rotated away from this axis.

  5. Self-consistent hole motion and spin excitations in a quantum antiferromagnet

    International Nuclear Information System (INIS)

    Su, Z.B.; Yu, L.; Li, Y.M.; Lai, W.Y.

    1989-12-01

    A new quantum Bogoliubov-de Gennes (BdeG) formalism is developed to study the self-consistent motion of holes and spin excitations in a quantum antiferromagnet within the generalized t-J model. On the one hand, the effects of local distortion of spin configurations and the renormalization of the hole motion due to virtual excitations of the distorted spin background are treated on an equal footing to obtain the hole wave function and its spectrum, as well as the effective mass for a propagating hole. On the other hand, the change of the spin excitation spectrum and the spin correlations due to the presence of dynamical holes are studied within the same adiabatic approximation. The stability of the hole states with respect to such changes justifies the self-consistency of the proposed formalism. (author). 25 refs, 6 figs, 1 tab

  6. Orphan Spins in the S=5/2 Antiferromagnet CaFe_{2}O_{4}.

    Science.gov (United States)

    Stock, C; Rodriguez, E E; Lee, N; Demmel, F; Fouquet, P; Laver, M; Niedermayer, Ch; Su, Y; Nemkovski, K; Green, M A; Rodriguez-Rivera, J A; Kim, J W; Zhang, L; Cheong, S-W

    2017-12-22

    CaFe_{2}O_{4} is an anisotropic S=5/2 antiferromagnet with two competing A (↑↑↓↓) and B (↑↓↑↓) magnetic order parameters separated by static antiphase boundaries at low temperatures. Neutron diffraction and bulk susceptibility measurements, show that the spins near these boundaries are weakly correlated and a carry an uncompensated ferromagnetic moment that can be tuned with a magnetic field. Spectroscopic measurements find these spins are bound with excitation energies less than the bulk magnetic spin waves and resemble the spectra from isolated spin clusters. Localized bound orphaned spins separate the two competing magnetic order parameters in CaFe_{2}O_{4}.

  7. Orphan Spins in the S =5/2 Antiferromagnet CaFe2O4

    Science.gov (United States)

    Stock, C.; Rodriguez, E. E.; Lee, N.; Demmel, F.; Fouquet, P.; Laver, M.; Niedermayer, Ch.; Su, Y.; Nemkovski, K.; Green, M. A.; Rodriguez-Rivera, J. A.; Kim, J. W.; Zhang, L.; Cheong, S.-W.

    2017-12-01

    CaFe2O4 is an anisotropic S =5/2 antiferromagnet with two competing A (↑↑↓↓) and B (↑↓↑↓) magnetic order parameters separated by static antiphase boundaries at low temperatures. Neutron diffraction and bulk susceptibility measurements, show that the spins near these boundaries are weakly correlated and a carry an uncompensated ferromagnetic moment that can be tuned with a magnetic field. Spectroscopic measurements find these spins are bound with excitation energies less than the bulk magnetic spin waves and resemble the spectra from isolated spin clusters. Localized bound orphaned spins separate the two competing magnetic order parameters in CaFe2 O4 .

  8. Spin-orbit coupling induced anisotropy effects in bimetallic antiferromagnets: A route towards antiferromagnetic spintronics

    Czech Academy of Sciences Publication Activity Database

    Shick, Alexander; Khmelevskyi, S.; Mryasov, O. N.; Wunderlich, J.; Jungwirth, Tomáš

    2010-01-01

    Roč. 81, č. 21 (2010), 212409/1-212409/4 ISSN 1098-0121 R&D Projects: GA AV ČR IAA100100912; GA ČR GA202/07/0456; GA AV ČR KAN400100652; GA ČR GEFON/06/E002 EU Projects: European Commission(XE) 215368 - SemiSpinNet; European Commission(XE) 214499 - NAMASTE Grant - others:AV ČR(CZ) AP0801 Program:Akademická prémie - Praemium Academiae Institutional research plan: CEZ:AV0Z10100520; CEZ:AV0Z10100521 Keywords : magnetic anisotropy * tunneling anisotropic magneto-resistance * exchange bias Subject RIV: BM - Solid Matter Physics ; Magnetism Impact factor: 3.772, year: 2010 http://link.aps.org/doi/10.1103/PhysRevB.81.212409

  9. su(1,2) Algebraic Structure of XYZ Antiferromagnetic Model in Linear Spin-Wave Frame

    International Nuclear Information System (INIS)

    Jin Shuo; Xie Binghao; Yu Zhaoxian; Hou Jingmin

    2008-01-01

    The XYZ antiferromagnetic model in linear spin-wave frame is shown explicitly to have an su(1,2) algebraic structure: the Hamiltonian can be written as a linear function of the su(1,2) algebra generators. Based on it, the energy eigenvalues are obtained by making use of the similar transformations, and the algebraic diagonalization method is investigated. Some numerical solutions are given, and the results indicate that only one group solution could be accepted in physics

  10. Nearly Deconfined Spinon Excitations in the Square-Lattice Spin-1/2 Heisenberg Antiferromagnet

    Directory of Open Access Journals (Sweden)

    Hui Shao

    2017-12-01

    Full Text Available We study the spin-excitation spectrum (dynamic structure factor of the spin-1/2 square-lattice Heisenberg antiferromagnet and an extended model (the J-Q model including four-spin interactions Q in addition to the Heisenberg exchange J. Using an improved method for stochastic analytic continuation of imaginary-time correlation functions computed with quantum Monte Carlo simulations, we can treat the sharp (δ-function contribution to the structure factor expected from spin-wave (magnon excitations, in addition to resolving a continuum above the magnon energy. Spectra for the Heisenberg model are in excellent agreement with recent neutron-scattering experiments on Cu(DCOO_{2}·4D_{2}O, where a broad spectral-weight continuum at wave vector q=(π,0 was interpreted as deconfined spinons, i.e., fractional excitations carrying half of the spin of a magnon. Our results at (π,0 show a similar reduction of the magnon weight and a large continuum, while the continuum is much smaller at q=(π/2,π/2 (as also seen experimentally. We further investigate the reasons for the small magnon weight at (π,0 and the nature of the corresponding excitation by studying the evolution of the spectral functions in the J-Q model. Upon turning on the Q interaction, we observe a rapid reduction of the magnon weight to zero, well before the system undergoes a deconfined quantum phase transition into a nonmagnetic spontaneously dimerized state. Based on these results, we reinterpret the picture of deconfined spinons at (π,0 in the experiments as nearly deconfined spinons—a precursor to deconfined quantum criticality. To further elucidate the picture of a fragile (π,0-magnon pole in the Heisenberg model and its depletion in the J-Q model, we introduce an effective model of the excitations in which a magnon can split into two spinons that do not separate but fluctuate in and out of the magnon space (in analogy to the resonance between a photon and a particle-hole pair in

  11. Spin frustration effects in an odd-member antiferromagnetic ring and the magnetic Mobius strip

    International Nuclear Information System (INIS)

    Cador, Olivier; Gatteschi, Dante; Sessoli, Roberta; Barra, Anne-Laure; Timco, Grigore A.; Winpenny, Richard E.P.

    2005-01-01

    The magnetic properties of the first odd-member antiferromagnetic ring comprising eight chromium(III) ions, S=32 spins, and one nickel(II) ion, S=1 spin, are investigated. The ring possesses an even number of unpaired electrons and a S=0 ground state but, due to competing AF interactions, the first excited spin states are close in energy. The spin frustrated ring is visualized by a Mobius strip. The 'knot' of the strip represents the region of the ring where the AF interactions are more frustrated. In the particular case of this bimetallic ring electron paramagnetic resonance (EPR) has unambiguously shown that the frustration is delocalized on the chromium chain, while the antiparallel alignment is more rigid at the nickel site

  12. Spin frustration effects in an odd-member antiferromagnetic ring and the magnetic Mobius strip

    Energy Technology Data Exchange (ETDEWEB)

    Cador, Olivier [Laboratory of Molecular Magnetism, Department of Chemistry and UdR INSTM, Universita degli Studi di Firenze, Via Lastruccia n. 3, 50019 Sesto Fiorentino (Italy); Gatteschi, Dante [Laboratory of Molecular Magnetism, Department of Chemistry and UdR INSTM, Universita degli Studi di Firenze, Via Lastruccia n. 3, 50019 Sesto Fiorentino (Italy); Sessoli, Roberta [Laboratory of Molecular Magnetism, Department of Chemistry and UdR INSTM, Universita degli Studi di Firenze, Via Lastruccia n. 3, 50019 Sesto Fiorentino (Italy)]. E-mail: roberta.sessoli@unifi.it; Barra, Anne-Laure [Laboratoire des Champs Magnetiques Intenses-CNRS, F-38042 Grenoble Cede 9 (France); Timco, Grigore A. [Department of Chemistry, University of Manchester, Oxford Road, Manchester M13 9PL (United Kingdom); Winpenny, Richard E.P. [Department of Chemistry, University of Manchester, Oxford Road, Manchester M13 9PL (United Kingdom)

    2005-04-15

    The magnetic properties of the first odd-member antiferromagnetic ring comprising eight chromium(III) ions, S=32 spins, and one nickel(II) ion, S=1 spin, are investigated. The ring possesses an even number of unpaired electrons and a S=0 ground state but, due to competing AF interactions, the first excited spin states are close in energy. The spin frustrated ring is visualized by a Mobius strip. The 'knot' of the strip represents the region of the ring where the AF interactions are more frustrated. In the particular case of this bimetallic ring electron paramagnetic resonance (EPR) has unambiguously shown that the frustration is delocalized on the chromium chain, while the antiparallel alignment is more rigid at the nickel site.

  13. Spin fluctuation and small polaron conduction dominated electrical ...

    Indian Academy of Sciences (India)

    Administrator

    temperature regime (20 K < T < 53 K), shows a minima near 53 K and increases with T ... Manganite nanoparticles; resistivity; spin fluctuation; electron–phonon interaction; electron– ... the low-doped regime because of the series of structural,.

  14. Antiferromagnetic spintronics

    Science.gov (United States)

    Baltz, V.; Manchon, A.; Tsoi, M.; Moriyama, T.; Ono, T.; Tserkovnyak, Y.

    2018-01-01

    Antiferromagnetic materials could represent the future of spintronic applications thanks to the numerous interesting features they combine: they are robust against perturbation due to magnetic fields, produce no stray fields, display ultrafast dynamics, and are capable of generating large magnetotransport effects. Intense research efforts over the past decade have been invested in unraveling spin transport properties in antiferromagnetic materials. Whether spin transport can be used to drive the antiferromagnetic order and how subsequent variations can be detected are some of the thrilling challenges currently being addressed. Antiferromagnetic spintronics started out with studies on spin transfer and has undergone a definite revival in the last few years with the publication of pioneering articles on the use of spin-orbit interactions in antiferromagnets. This paradigm shift offers possibilities for radically new concepts for spin manipulation in electronics. Central to these endeavors are the need for predictive models, relevant disruptive materials, and new experimental designs. This paper reviews the most prominent spintronic effects described based on theoretical and experimental analysis of antiferromagnetic materials. It also details some of the remaining bottlenecks and suggests possible avenues for future research. This review covers both spin-transfer-related effects, such as spin-transfer torque, spin penetration length, domain-wall motion, and "magnetization" dynamics, and spin-orbit related phenomena, such as (tunnel) anisotropic magnetoresistance, spin Hall, and inverse spin galvanic effects. Effects related to spin caloritronics, such as the spin Seebeck effect, are linked to the transport of magnons in antiferromagnets. The propagation of spin waves and spin superfluids in antiferromagnets is also covered.

  15. Current-induced spin-orbit torques in ferromagnetic and antiferromagnetic systems

    KAUST Repository

    Manchon, Aurelien

    2018-01-29

    Spin-orbit coupling in inversion-asymmetric magnetic crystals and structures has emerged as a powerful tool to generate complex magnetic textures, interconvert charge and spin under applied current, and control magnetization dynamics. Current-induced spin-orbit torques mediate the transfer of angular momentum from the lattice to the spin system, leading to sustained magnetic oscillations or switching of ferromagnetic as well as antiferromagnetic structures. The manipulation of magnetic order, domain walls and skyrmions by spin-orbit torques provides evidence of the microscopic interactions between charge and spin in a variety of materials and opens novel strategies to design spintronic devices with potentially high impact in data storage, nonvolatile logic, and magnonic applications. This paper reviews recent progress in the field of spin-orbitronics, focusing on theoretical models, material properties, and experimental results obtained on bulk noncentrosymmetric conductors and multilayer heterostructures, including metals, semiconductors, and topological insulator systems. Relevant aspects for improving the understanding and optimizing the efficiency of nonequilibrium spin-orbit phenomena in future nanoscale devices are also discussed.

  16. Current-induced spin-orbit torques in ferromagnetic and antiferromagnetic systems

    KAUST Repository

    Manchon, Aurelien; Miron, I. M.; Jungwirth, T.; Sinova, J.; Zelezný , J.; Thiaville, A.; Garello, K.; Gambardella, P.

    2018-01-01

    Spin-orbit coupling in inversion-asymmetric magnetic crystals and structures has emerged as a powerful tool to generate complex magnetic textures, interconvert charge and spin under applied current, and control magnetization dynamics. Current-induced spin-orbit torques mediate the transfer of angular momentum from the lattice to the spin system, leading to sustained magnetic oscillations or switching of ferromagnetic as well as antiferromagnetic structures. The manipulation of magnetic order, domain walls and skyrmions by spin-orbit torques provides evidence of the microscopic interactions between charge and spin in a variety of materials and opens novel strategies to design spintronic devices with potentially high impact in data storage, nonvolatile logic, and magnonic applications. This paper reviews recent progress in the field of spin-orbitronics, focusing on theoretical models, material properties, and experimental results obtained on bulk noncentrosymmetric conductors and multilayer heterostructures, including metals, semiconductors, and topological insulator systems. Relevant aspects for improving the understanding and optimizing the efficiency of nonequilibrium spin-orbit phenomena in future nanoscale devices are also discussed.

  17. Magnetic ordering in tetragonal FeS: Evidence for strong itinerant spin fluctuations

    Energy Technology Data Exchange (ETDEWEB)

    Kwon, K.D.; Refson, K.; Bone, S.; Qiao, R.; Yang, W.; Liu, Z.; Sposito, G.

    2010-11-01

    Mackinawite is a naturally occurring layer-type FeS mineral important in biogeochemical cycles and, more recently, in the development of microbial fuel cells. Conflicting results have been published as to the magnetic properties of this mineral, with Moessbauer spectroscopy indicating no magnetic ordering down to 4.2 K but density functional theory (DFT) predicting an antiferromagnetic ground state, similar to the Fe-based high-temperature superconductors with which it is isostructural and for which it is known that magnetism is suppressed by strong itinerant spin fluctuations. We investigated this latter possibility for mackinawite using photoemission spectroscopy, near-edge x-ray absorption fine structure spectroscopy, and DFT computations. Our Fe 3{sub s} core-level photoemission spectrum of mackinawite showed a clear exchange-energy splitting (2.9 eV) consistent with a 1 {micro}{sub B} magnetic moment on the Fe ions, while the Fe L-edge x-ray absorption spectrum indicated rather delocalized Fe 3{sub d} electrons in mackinawite similar to those in Fe metal. Our DFT computations demonstrated that the ground state of mackinawite is single-stripe antiferromagnetic, with an Fe magnetic moment (2.7 {micro}{sub B}) that is significantly larger than the experimental estimate and has a strong dependence on the S height and lattice parameters. All of these trends signal the existence of strong itinerant spin fluctuations. If spin fluctuations prove to be mediators of electron pairing, we conjecture that mackinawite may be one of the simplest Fe-based superconductors.

  18. Magnetic Anisotropy by Rashba Spin-Orbit Coupling in Antiferromagnetic Thin Films

    Science.gov (United States)

    Ieda, Jun'ichi; Barnes, Stewart E.; Maekawa, Sadamichi

    2018-05-01

    Magnetic anisotropy in an antiferromagnet (AFM) with inversion symmetry breaking (ISB) is investigated. The magnetic anisotropy energy (MAE) resulting from the Rashba spin-orbit and s-d type exchange interactions is determined for two different models of AFMs. The global ISB model, representing the effect of a surface, an interface, or a gating electric field, results in an easy-plane magnetic anisotropy. In contrast, for a local ISB model, i.e., for a noncentrosymmetric AFM, perpendicular magnetic anisotropy (PMA) arises. Both results differ from the ferromagnetic case, in which the result for PMA depends on the band structure and dimensionality. These MAE contributions play a key role in determining the direction of the Néel order parameter in antiferromagnetic nanostructures, and reflect the possibility of electrical-field control of the Néel vector.

  19. Spin wave dynamics in Heisenberg ferromagnetic/antiferromagnetic single-walled nanotubes

    Energy Technology Data Exchange (ETDEWEB)

    Mi, Bin-Zhou, E-mail: mbzfjerry2008@126.com [Department of Basic Curriculum, North China Institute of Science and Technology, Beijing 101601 (China); Department of Physics, School of Mathematics and Physics, University of Science and Technology Beijing, Beijing 100083 (China)

    2016-09-15

    The spin wave dynamics, including the magnetization, spin wave dispersion relation, and energy level splitting, of Heisenberg ferromagnetic/antiferromagnetic single-walled nanotubes are systematically calculated by use of the double-time Green’s function method within the random phase approximation. The role of temperature, diameter of the tube, and wave vector on spin wave energy spectrum and energy level splitting are carefully analyzed. There are two categories of spin wave modes, which are quantized and degenerate, and the total number of independent magnon branches is dependent on diameter of the tube, caused by the physical symmetry of nanotubes. Moreover, the number of flat spin wave modes increases with diameter of the tube rising. The spin wave energy and the energy level splitting decrease with temperature rising, and become zero as temperature reaches the critical point. At any temperature, the energy level splitting varies with wave vector, and for a larger wave vector it is smaller. When pb=π, the boundary of first Brillouin zone, spin wave energies are degenerate, and the energy level splittings are zero.

  20. Geometric phase of a central spin coupled to an antiferromagnetic environment

    International Nuclear Information System (INIS)

    Yuan Xiaozhong; Zhu Kadi; Goan, H.-S.

    2010-01-01

    Using the spin-wave approximation, we study the geometric phase (GP) of a central spin (signal qubit) coupled to an antiferromagnetic (AF) environment under the application of an external global magnetic field. The external magnetic field affects the GP of the qubit directly and also indirectly through its effect on the AF environment. We find that when the applied magnetic field is increased to the critical magnetic field point, the AF environment undergoes a spin-flop transition, a first-order phase transition, and at the same time the GP of the qubit changes abruptly to zero. This sensitive change of the GP of a signal qubit to the parameter change of a many-body environment near its critical point may serve as another efficient tool or witness to study the many-body phase transition. The influences of the AF environment temperature and crystal anisotropy field on the GP are also investigated.

  1. Spin-Resolved Photoemission on Anti-Ferromagnets: Direct Observation of Zhang-Rice Singlets in CuO

    NARCIS (Netherlands)

    Tjeng, L.H.; Sinkovic, B.; Brookes, N.B.; Goedkoop, J.B.; Hesper, R.; Pellegrin, E.; Groot, F.M.F. de; Altieri, S.; Hulbert, S.L.; Shekel, E.; Sawatzky, G.A.

    1997-01-01

    We demonstrate that it is possible to obtain spin-resolved valence band spectra with a very high degree of spin polarization from antiferromagnetic transition metal materials if the excitation light is circularly polarized and has an energy close to the cation 2p3/2 (L3) white line. We are able to

  2. Interplay between the Dzyaloshinskii-Moriya term and external fields on spin transport in the spin-1/2 one-dimensional antiferromagnet

    Science.gov (United States)

    Lima, L. S.

    2018-05-01

    We study the effect of the uniform Dzyaloshinskii-Moriya interaction (symmetric exchange anisotropy) and arbitrary oriented external magnetic fields on spin conductivity in the spin-1/2 one-dimensional Heisenberg antiferromagnet. The spin conductivity is calculated employing abelian bosonization and the Kubo formalism of transport. We investigate the influence of three competing phases at zero-temperature, (Néel phase, dimerized phase and gapless Luttinger liquid phase) on the AC spin conductivity.

  3. Generalized theory of spin fluctuations in itinerant electron magnets: Crucial role of spin anharmonicity

    International Nuclear Information System (INIS)

    Solontsov, A.

    2015-01-01

    The paper critically overviews the recent developments of the theory of spatially dispersive spin fluctuations (SF) in itinerant electron magnetism with particular emphasis on spin-fluctuation coupling or spin anharmonicity. It is argued that the conventional self-consistent renormalized (SCR) theory of spin fluctuations is usually used aside of the range of its applicability actually defined by the constraint of weak spin anharmonicity based on the random phase approximation (RPA) arguments. An essential step in understanding SF in itinerant magnets beyond RPA-like arguments was made recently within the soft-mode theory of SF accounting for strong spin anharmonicity caused by zero-point SF. In the present paper we generalize it to apply for a wider range of temperatures and regimes of SF and show it to lead to qualitatively new results caused by zero-point effects. - Highlights: • We review the spin-fluctuation theory of itinerant electron magnets with account of zero-point effects. • We generalize the existing theory to account for different regimes of spin fluctuations. • We show that zero-point spin fluctuations play a crucial role in both low- and high-temperature properties of metallic magnets. • We argue that a new scheme of calculation of ground state properties of magnets is needed including zero-point effects

  4. Spin fluctuations in EuS

    International Nuclear Information System (INIS)

    Hartmann, A.

    1996-02-01

    Demagnetization effects break the isotropy of spin waves. During spring 1995, Peter Boeni et al. performed polarized neutron measurements on EuS using the triple axis spectrometer IN14 at the ILL in Grenoble, in order to investigate the influence of dipolar interactions on the spin waves. In the following work the analysis of the experimental data is described. (author) 25 figs., 2 tabs., 9 refs

  5. Phase Diagram in a Random Mixture of Two Antiferromagnets with Competing Spin Anisotropies. I

    Science.gov (United States)

    Someya, Yoshiko

    1981-12-01

    The phase diagram of a random mixture of two antiferromagnets with competing spin anisotropies (A1-xBx) has been analyzed by extending the theory of Matsubara and Inawashiro, and Oguchi and Ishikawa. In the model assumed, the anisotropy energies are expressed by the anisotropic exchange interactions. According to this formulation, it has been shown that the concentration dependence of TN becomes a function of \\includegraphics{dummy.eps}, where P, Q=A, B; SP is a magnitude of P-spin, and JPQη is a η component of exchange integral between P- and Q-spin). Further, the phase boundary between an AF phase and an OAF (oblique antiferromagnetic) phase at T{=}0 K has been shown to be determined by α({\\equiv}SB/SA), if \\includegraphics{dummy.eps} are given. The obtained phase diagrams for Fe1-xCoxCl2, K2Mn1-xFexF4 and Fe1-xCoxCl2\\cdot2H2O are compared with the experimental ones.

  6. RVB signatures in the spin dynamics of the square-lattice Heisenberg antiferromagnet

    Science.gov (United States)

    Ghioldi, E. A.; Gonzalez, M. G.; Manuel, L. O.; Trumper, A. E.

    2016-03-01

    We investigate the spin dynamics of the square-lattice spin-\\frac{1}{2} Heisenberg antiferromagnet by means of an improved mean-field Schwinger boson calculation. By identifying both, the long-range Néel and the RVB-like components of the ground state, we propose an educated guess for the mean-field magnetic excitation consisting on a linear combination of local and bond spin flips to compute the dynamical structure factor. Our main result is that when this magnetic excitation is optimized in such a way that the corresponding sum rule is fulfilled, we recover the low- and high-energy spectral weight features of the experimental spectrum. In particular, the anomalous spectral weight depletion at (π,0) found in recent inelastic neutron scattering experiments can be attributed to the interference of the triplet bond excitations of the RVB component of the ground state. We conclude that the Schwinger boson theory seems to be a good candidate to adequately interpret the dynamic properties of the square-lattice Heisenberg antiferromagnet.

  7. Anisotropy, magnetic field and stress influences on the phase transitions on spin-flop-type antiferromagnets

    International Nuclear Information System (INIS)

    Machado, S.F.; Espirito Santo Univ., Vitoria; Tsallis, C.

    1983-01-01

    Within a mean field approximation, the influences of anisotropy (in the spin space) and external uniaxial stress on the Heisenberg antiferromagnet in the presence of magnetic field are discussed. The phase diagram evolution (as function of anisotropy and stress) which is obtained, enables a satisfactory overall interpretation of recent experiments on Mn(Br sub(1-x) Cl sub(x)) 2 .4H 2 O, K 2 [FeCl 5 (H 2 O)], CoCl 2 .6H 2 O and (C 2 H 5 NH 3 ) 2 CuCl 4 . (Author) [pt

  8. Multicritical phase diagrams of the antiferromagnetic spin-3/2 Blume-Capel model

    Energy Technology Data Exchange (ETDEWEB)

    Keskin, Mustafa [Department of Physics, Erciyes University, 38039 Kayseri (Turkey)]. E-mail: keskin@erciyes.edu.tr; Ali Pinar, M. [Institute of Science, Erciyes University, 38039 Kayseri (Turkey); Erdinc, Ahmet [Department of Physics, Erciyes University, 38039 Kayseri (Turkey); Canko, Osman [Department of Physics, Erciyes University, 38039 Kayseri (Turkey)

    2006-04-24

    The antiferromagnetic spin-3/2 Blume-Capel model in an external magnetic field is investigated, and the phase diagrams are obtained in detail by using the cluster variation method. The model exhibits distinct critical regions, including the first-order, second-order and special points: two double critical points, a critical end point, a tricritical point and a zero-temperature critical point. The new phase diagram topology is also found that was not obtained previously. Comparison of the results with those of other studies on this, and closely related systems, is made.

  9. Multicritical phase diagrams of the antiferromagnetic spin-3/2 Blume-Capel model

    International Nuclear Information System (INIS)

    Keskin, Mustafa; Ali Pinar, M.; Erdinc, Ahmet; Canko, Osman

    2006-01-01

    The antiferromagnetic spin-3/2 Blume-Capel model in an external magnetic field is investigated, and the phase diagrams are obtained in detail by using the cluster variation method. The model exhibits distinct critical regions, including the first-order, second-order and special points: two double critical points, a critical end point, a tricritical point and a zero-temperature critical point. The new phase diagram topology is also found that was not obtained previously. Comparison of the results with those of other studies on this, and closely related systems, is made

  10. Magnon diffusion theory for the spin Seebeck effect in ferromagnetic and antiferromagnetic insulators

    Science.gov (United States)

    Rezende, Sergio M.; Azevedo, Antonio; Rodríguez-Suárez, Roberto L.

    2018-05-01

    In magnetic insulators, spin currents are carried by the elementary excitations of the magnetization: spin waves or magnons. In simple ferromagnetic insulators there is only one magnon mode, while in two-sublattice antiferromagnetic insulators (AFIs) there are two modes, which carry spin currents in opposite directions. Here we present a theory for the diffusive magnonic spin current generated in a magnetic insulator layer by a thermal gradient in the spin Seebeck effect. We show that the formulations describing magnonic perturbation using a position-dependent chemical potential and those using a magnon accumulation are completely equivalent. Then we develop a drift–diffusion formulation for magnonic spin transport treating the magnon accumulation governed by the Boltzmann transport and diffusion equations and considering the full boundary conditions at the surfaces and interfaces of an AFI/normal metal bilayer. The theory is applied to the ferrimagnetic yttrium iron garnet and to the AFIs MnF2 and NiO, providing good quantitative agreement with experimental data.

  11. Persistence of the gapless spin liquid in the breathing kagome Heisenberg antiferromagnet

    Science.gov (United States)

    Iqbal, Yasir; Poilblanc, Didier; Thomale, Ronny; Becca, Federico

    2018-03-01

    The nature of the ground state of the spin S =1 /2 Heisenberg antiferromagnet on the kagome lattice with breathing anisotropy (i.e., with different superexchange couplings J▵ and J▿ within elementary up- and down-pointing triangles) is investigated within the framework of Gutzwiller projected fermionic wave functions and Monte Carlo methods. We analyze the stability of the U(1 ) Dirac spin liquid with respect to the presence of fermionic pairing that leads to a gapped Z2 spin liquid. For several values of the ratio J▿/J▵ , the size scaling of the energy gain due to the pairing fields and the variational parameters are reported. Our results show that the energy gain of the gapped spin liquid with respect to the gapless state either vanishes for large enough system size or scales to zero in the thermodynamic limit. Similarly, the optimized pairing amplitudes (responsible for opening the spin gap) are shown to vanish in the thermodynamic limit. Our outcome is corroborated by the application of one and two Lanczos steps to the gapless and gapped wave functions, for which no energy gain of the gapped state is detected when improving the quality of the variational states. Finally, we discuss the competition with the "simplex" Z2 resonating-valence-bond spin liquid, valence-bond crystal, and nematic states in the strongly anisotropic regime, i.e., J▿≪J▵ .

  12. Magnetic structure and spin dynamics of the quasi-one-dimensional spin-chain antiferromagnet BaCo2V2O8

    DEFF Research Database (Denmark)

    Kawasaki, Yu; Gavilano, Jorge L.; Keller, Lukas

    2011-01-01

    ,0,1), independent of external magnetic fields for fields below a critical value H-c(T). The ordered moments of 2.18 mu(B) per Co ion are aligned along the crystallographic c axis. Within the screw chains, along the c axis, the moments are arranged antiferromagnetically. In the basal planes the spins are arranged......We report a neutron diffraction and muon spin relaxation mu SR study of static and dynamical magnetic properties of BaCo2V2O8, a quasi-one-dimensional spin-chain system. A proposed model for the antiferromagnetic structure includes: a propagation vector (k) over right arrow (AF) = (0...

  13. Antiferromagnetic spintronics

    KAUST Repository

    Baltz, V.; Manchon, Aurelien; Tsoi, M.; Moriyama, T.; Ono, T.; Tserkovnyak, Y.

    2018-01-01

    Antiferromagnetic materials could represent the future of spintronic applications thanks to the numerous interesting features they combine: they are robust against perturbation due to magnetic fields, produce no stray fields, display ultrafast dynamics, and are capable of generating large magnetotransport effects. Intense research efforts over the past decade have been invested in unraveling spin transport properties in antiferromagnetic materials. Whether spin transport can be used to drive the antiferromagnetic order and how subsequent variations can be detected are some of the thrilling challenges currently being addressed. Antiferromagnetic spintronics started out with studies on spin transfer and has undergone a definite revival in the last few years with the publication of pioneering articles on the use of spin-orbit interactions in antiferromagnets. This paradigm shift offers possibilities for radically new concepts for spin manipulation in electronics. Central to these endeavors are the need for predictive models, relevant disruptive materials, and new experimental designs. This paper reviews the most prominent spintronic effects described based on theoretical and experimental analysis of antiferromagnetic materials. It also details some of the remaining bottlenecks and suggests possible avenues for future research. This review covers both spin-transfer-related effects, such as spin-transfer torque, spin penetration length, domain-wall motion, and

  14. Antiferromagnetic spintronics

    KAUST Repository

    Baltz, V.

    2018-02-15

    Antiferromagnetic materials could represent the future of spintronic applications thanks to the numerous interesting features they combine: they are robust against perturbation due to magnetic fields, produce no stray fields, display ultrafast dynamics, and are capable of generating large magnetotransport effects. Intense research efforts over the past decade have been invested in unraveling spin transport properties in antiferromagnetic materials. Whether spin transport can be used to drive the antiferromagnetic order and how subsequent variations can be detected are some of the thrilling challenges currently being addressed. Antiferromagnetic spintronics started out with studies on spin transfer and has undergone a definite revival in the last few years with the publication of pioneering articles on the use of spin-orbit interactions in antiferromagnets. This paradigm shift offers possibilities for radically new concepts for spin manipulation in electronics. Central to these endeavors are the need for predictive models, relevant disruptive materials, and new experimental designs. This paper reviews the most prominent spintronic effects described based on theoretical and experimental analysis of antiferromagnetic materials. It also details some of the remaining bottlenecks and suggests possible avenues for future research. This review covers both spin-transfer-related effects, such as spin-transfer torque, spin penetration length, domain-wall motion, and

  15. Padé approximations for the magnetic susceptibilities of Heisenberg antiferromagnetic spin chains for various spin values

    International Nuclear Information System (INIS)

    Law, J M; Benner, H; Kremer, R K

    2013-01-01

    The temperature dependence of the spin susceptibilities of S = 1, 3/2 , 2, 5/2 and 7/2 Heisenberg antiferromagnetic 1D spins chains with nearest-neighbor coupling was simulated via quantum Monte Carlo calculations, within the reduced temperature range of 0.005 ≤ T* ≤ 100, and fitted to a Padé approximation with deviations between the simulated and fitted data of the same order of magnitude as or smaller than the quantum Monte Carlo simulation error. To demonstrate the practicality of our theoretical findings, we compare these results with the susceptibility of the well known 1D chain compound TMMC ([(CH 3 ) 4 N[MnCl 3

  16. Improved spin wave theory: An application to the spin-1/2 antiferromagnetic Heisenberg model on a square lattice

    International Nuclear Information System (INIS)

    Tao, Ruibao.

    1991-09-01

    A method is developed to make a Bose transformation which is restricted in proper space. A self-consistent independent spin wave representation (SCISWR) is found for two dimensional isotropic antiferromagnet of Heisenberg square lattices. In the SCISWR, we have successfully done the renormalization from both the dynamic and kinematic interaction and calculated the corrections from the correlations of the nearest neighbour and next nearest neighbour sites. An anisotropic excitation energy of spin wave in improper space is found self-consistently and has a gap. The difficulty of divergence appearing from higher order perturbation terms in the conventional spin wave theory has been overcome and the convergence in our approach seems quite good. We find the energy of ground state E approx. -0.659 in low order approximation and the magnetization of sublattice M z = 0.430 x (N/2) for system with spin 1/2. It is also proved that a physical spin excitation restricted in proper space is still isotropic and has no gap. (author). 17 refs

  17. Effect of Noise on the Decoherence of a Central Electron Spin Coupled to an Antiferromagnetic Spin Bath

    Directory of Open Access Journals (Sweden)

    G. C. Fouokeng

    2014-01-01

    Full Text Available We analyze the influence of a two-state autocorrelated noise on the decoherence and on the tunneling Landau-Zener (LZ transitions during a two-level crossing of a central electron spin (CES coupled to a one dimensional anisotropic-antiferomagnetic spin, driven by a time-dependent global external magnetic field. The energy splitting of the coupled spin system is found through an approach that computes the noise-averaged frequency. At low magnetic field intensity, the decoherence (or entangled state of a coupled spin system is dominated by the noise intensity. The effects of the magnetic field pulse and the spin gap antiferromagnetic material used suggest to us that they may be used as tools for the direct observation of the tunneling splitting through the LZ transitions in the sudden limit. We found that the dynamical frequencies display basin-like behavior decay with time, with the birth of entanglement, while the LZ transition probability shows Gaussian shape.

  18. Thermal conductivity of a quantum spin-1/2 antiferromagnetic chain with magnetic impurities

    International Nuclear Information System (INIS)

    Zviagin, A.A.

    2008-01-01

    We present an exact theory that describes how magnetic impurities change the behavior of the thermal conductivity for the integrable Heisenberg antiferromagnetic quantum spin-1/2 chain. Single magnetic impurities and a large concentration of impurities with similar values of the couplings to the host chain (a weak disorder) do not change the linear-in-temperature low-T behavior of the thermal conductivity: Only the slope of that behavior becomes smaller, compared to the homogeneous case. The strong disorder in the distribution of the impurity-host couplings produces more rapid temperature growth of the thermal conductivity, compared to the linear-in-T dependence of the homogeneous chain and the chain with weak disorder. Recent experiments on the thermal conductivity in inhomogeneous quasi-one-dimensional quantum spin systems manifest qualitative agreement with our results

  19. Magnetoresistance in RCo2 spin-fluctuation systems

    International Nuclear Information System (INIS)

    Gratz, E.; Nowotny, H.; Enser, J.; Bauer, E.; Hense, K.

    2004-01-01

    The effect of the spin fluctuations on the field and temperature dependence of the magnetoresistance in ScCo 2 and LuCo 2 was studied. The experimental data where explained assuming two competing mechanisms determining the magnetoresistance of these substances. One is the 'normal magnetoresistance' caused by the influence of the Lorentz force on conduction electron trajectories. The other is due to the suppression of the spin fluctuations caused by an external magnetic field. This interplay give rise to a pronounced drop of the magnetoresistance towards the lower temperature range

  20. Direct evidence of spin frustration in the fcc antiferromagnet NiS sub 2

    CERN Document Server

    Matsuura, M; Endoh, Y; Hirota, K; Yamada, K

    2002-01-01

    NiS sub 2 is a well-known Mott insulator with anomalous antiferromagnetic long-range order of coexistent type I (Q sub M =(1,0,0), T sub N sub 1 =40 K) and type II (Q sub M =(1/2,1/2,1/2), T sub N sub 2 =30 K). Extensive neutron-scattering measurements reveal that magnetism in NiS sub 2 is governed by geometrical spin frustration, resulting in magnetic diffuse scattering extending along the fcc zone boundary. Although the diffuse scattering exists at temperatures as high as 250 K (6T sub N sub 1), it disappears rapidly below T sub N sub 2 , associated with minor crystal distortion. We observed a clear energy gap in addition to the low-energy spin-wave excitation at significantly below 30 K, and obtain evidence that degeneracy due to the coexistence of the two types of antiferromagnetism is relieved in the ground state via the reduction in symmetry due to distortion. (orig.)

  1. Influence of spin and charge fluctuations on spectra of the two-dimensional Hubbard model

    Science.gov (United States)

    Sherman, A.

    2018-05-01

    The influence of spin and charge fluctuations on spectra of the two-dimensional fermionic Hubbard model is considered using the strong coupling diagram technique. Infinite sequences of diagrams containing ladder inserts, which describe the interaction of electrons with these fluctuations, are summed, and obtained equations are self-consistently solved for the ranges of Hubbard repulsions , temperatures and electron concentrations with t the intersite hopping constant. For all considered U the system exhibits a transition to the long-range antiferromagnetic order at . At the same time no indication of charge ordering is observed. Obtained solutions agree satisfactorily with results of other approaches and obey moments sum rules. In the considered region of the U-T plane, the curve separating metallic solutions passes from at the highest temperatures to U  =  2t at for half-filling. If only short-range fluctuations are allowed for the remaining part of this region is occupied by insulating solutions. Taking into account long-range fluctuations leads to strengthening of maxima tails, which transform a part of insulating solutions into bad-metal states. For low T, obtained results allow us to trace the gradual transition from the regime of strong correlations with the pronounced four-band structure and well-defined Mott gap for to the Slater regime of weak correlations with the spectral intensity having a dip along the boundary of the magnetic Brillouin zone due to an antiferromagnetic ordering for . For and doping leads to the occurrence of a pseudogap near the Fermi level, which is a consequence of the splitting out of a narrow band from a Hubbard subband. Obtained spectra feature waterfalls and Fermi arcs, which are similar to those observed in hole-doped cuprates.

  2. Large anomalous Nernst and spin Nernst effects in the noncollinear antiferromagnets Mn3X (X =Sn ,Ge ,Ga )

    Science.gov (United States)

    Guo, Guang-Yu; Wang, Tzu-Cheng

    2017-12-01

    Noncollinear antiferromagnets have recently been attracting considerable interest partly due to recent surprising discoveries of the anomalous Hall effect (AHE) in them and partly because they have promising applications in antiferromagnetic spintronics. Here we study the anomalous Nernst effect (ANE), a phenomenon having the same origin as the AHE, and also the spin Nernst effect (SNE) as well as AHE and the spin Hall effect (SHE) in noncollinear antiferromagnetic Mn3X (X =Sn , Ge, Ga) within the Berry phase formalism based on ab initio relativistic band structure calculations. For comparison, we also calculate the anomalous Nernst conductivity (ANC) and anomalous Hall conductivity (AHC) of ferromagnetic iron as well as the spin Nernst conductivity (SNC) of platinum metal. Remarkably, the calculated ANC at room temperature (300 K) for all three alloys is huge, being 10-40 times larger than that of iron. Moreover, the calculated SNC for Mn3Sn and Mn3Ga is also larger, being about five times larger than that of platinum. This suggests that these antiferromagnets would be useful materials for thermoelectronic devices and spin caloritronic devices. The calculated ANC of Mn3Sn and iron are in reasonably good agreement with the very recent experiments. The calculated SNC of platinum also agrees with the very recent experiments in both sign and magnitude. The calculated thermoelectric and thermomagnetic properties are analyzed in terms of the band structures as well as the energy-dependent AHC, ANC, SNC, and spin Hall conductivity via the Mott relations.

  3. Spin-1/2 Heisenberg antiferromagnet on the pyrochlore lattice: An exact diagonalization study

    Science.gov (United States)

    Chandra, V. Ravi; Sahoo, Jyotisman

    2018-04-01

    We present exact diagonalization calculations for the spin-1/2 nearest-neighbor antiferromagnet on the pyrochlore lattice. We study a section of the lattice in the [111] direction and analyze the Hamiltonian of the breathing pyrochlore system with two coupling constants J1 and J2 for tetrahedra of different orientations and investigate the evolution of the system from the limit of disconnected tetrahedra (J2=0 ) to a correlated state at J1=J2 . We evaluate the low-energy spectrum, two and four spin correlations, and spin chirality correlations for a system size of up to 36 sites. The model shows a fast decay of spin correlations and we confirm the presence of several singlet excitations below the lowest magnetic excitation. We find chirality correlations near J1=J2 to be small at the length scales available at this system size. Evaluation of dimer-dimer correlations and analysis of the nature of the entanglement of the tetrahedral unit shows that the triplet sector of the tetrahedron contributes significantly to the ground-state entanglement at J1=J2 .

  4. Search for the Heisenberg spin glass on rewired cubic lattices with antiferromagnetic interaction

    International Nuclear Information System (INIS)

    Surungan, Tasrief

    2016-01-01

    Spin glass (SG) is a typical magnetic system which is mainly characterized by a frozen random spin orientation at low temperatures. Frustration and randomness are considered to be the key ingredients for the existence of SGs. Previously, Bartolozzi et al . [Phys. Rev. B73, 224419 (2006)] found that the antiferromagnetic (AF) Ising spins on scale free network (SFN) exhibited SG behavior. This is purely AF system, a new type of SG different from the canonical one which requires the presence of both FM and AF couplings. In this new system, frustration is purely due to a topological factor and its randomness is brought by irregular connectivity. Recently, it was reported that the AF Heisenberg model on SFN exhibited SG behavior [Surungan et al ., JPCS, 640, 012005 (2015)/doi:10.1088/1742-6596/640/1/012005]. In order to accommodate the notion of spatial dimension, we further investigated this type of system by studying an AF Heisenberg model on rewired cubic lattices, constructed by adding one extra bond randomly connecting each spin to one of its next-nearest neighbors. We used Replica Exchange algorithm of Monte Carlo Method and calculated the SG order parameter to search for the existence of SG phase. (paper)

  5. Antiferromagnetic Ordering in Quasi-Triangular Localized Spin System, β'-Et2Me2P[Pd(dmit)2]2, Studied by 13C NMR

    Science.gov (United States)

    Otsuka, Kei; Iikubo, Hideaki; Kogure, Takayuki; Takano, Yoshiki; Hiraki, Ko-ichi; Takahashi, Toshihiro; Cui, Hengbo; Kato, Reizo

    2014-05-01

    We performed 13C NMR measurements of a selectively 13C isotope-labeled single-crystal sample of a frustrated spin system, β'-Et2Me2P[Pd(dmit)2]2. A long-range antiferromagnetic (AF) ordering below 17 K was confirmed by the observation of NMR spectrum broadening and well split resonance lines at lower temperatures. NMR spectra in the AF state can be well explained by a two sublattice model. From the analysis of the angular dependence of the NMR spectrum, we clarified the magnetic structure in the AF state, where the easy and hard axes are the crystallographic c*- and b-axes, respectively, and the effective localized moments are quite small, ˜0.28 μB/dimer. This suggests a strong quantum fluctuation effect due to magnetic frustrations in a quasi-triangular spin-1/2 system.

  6. Temperature dependence of fluctuation time scales in spin glasses

    DEFF Research Database (Denmark)

    Kenning, Gregory G.; Bowen, J.; Sibani, Paolo

    2010-01-01

    Using a series of fast cooling protocols we have probed aging effects in the spin glass state as a function of temperature. Analyzing the logarithmic decay found at very long time scales within a simple phenomenological barrier model, leads to the extraction of the fluctuation time scale of the s...

  7. Theory of spin-fluctuation induced superconductivity in iron-based superconductors

    International Nuclear Information System (INIS)

    Zhang, Junhua

    2011-01-01

    In this dissertation we focus on the investigation of the pairing mechanism in the recently discovered high-temperature superconductor, iron pnictides. Due to the proximity to magnetic instability of the system, we considered short-range spin fluctuations as the major mediating source to induce superconductivity. Our calculation supports the magnetic fluctuations as a strong candidate that drives Cooper-pair formation in this material. We find the corresponding order parameter to be of the so-called ss-wave type and show its evolution with temperature as well as the capability of supporting high transition temperature up to several tens of Kelvin. On the other hand, our itinerant model calculation shows pronounced spin correlation at the observed antiferromagnetic ordering wave vector, indicating the underlying electronic structure in favor of antiferromagnetic state. Therefore, the electronic degrees of freedom could participate both in the magnetic and in the superconducting properties. Our work shows that the interplay between magnetism and superconductivity plays an important role to the understanding of the rich physics in this material. The magnetic-excitation spectrum carries important information on the nature of magnetism and the characteristics of superconductivity. We analyze the spin excitation spectrum in the normal and superconducting states of iron pnictides in the magnetic scenario. As a consequence of the sign-reversed gap structure obtained in the above, a spin resonance mode appears below the superconducting transition temperature. The calculated resonance energy, scaled with the gap magnitude and the magnetic correlation length, agrees well with the inelastic neutron scattering (INS) measurements. More interestingly, we find a common feature of those short-range spin fluctuations that are capable of inducing a fully gapped ss state is the momentum anisotropy with elongated span along the direction transverse to the antiferromagnetic momentum

  8. Role of the antiferromagnetic pinning layer on spin wave properties in IrMn/NiFe based spin-valves

    Energy Technology Data Exchange (ETDEWEB)

    Gubbiotti, G., E-mail: gubbiotti@fisica.unipg.it; Tacchi, S. [Istituto Officina dei Materiali del CNR (IOM-CNR), Unità di Perugia, I-06123 Perugia (Italy); Del Bianco, L. [Department of Physics and Astronomy, University of Bologna, I-40127 Bologna (Italy); Department of Physics and Earth Sciences and CNISM, University of Ferrara, I-44122 Ferrara (Italy); Bonfiglioli, E.; Giovannini, L.; Spizzo, F.; Zivieri, R. [Department of Physics and Earth Sciences and CNISM, University of Ferrara, I-44122 Ferrara (Italy); Tamisari, M. [Department of Physics and Earth Sciences and CNISM, University of Ferrara, I-44122 Ferrara (Italy); Dipartimento di Fisica e Geologia, Università di Perugia, I-06123 Perugia (Italy)

    2015-05-07

    Brillouin light scattering (BLS) was exploited to study the spin wave properties of spin-valve (SV) type samples basically consisting of two 5 nm-thick NiFe layers (separated by a Cu spacer of 5 nm), differently biased through the interface exchange coupling with an antiferromagnetic IrMn layer. Three samples were investigated: a reference SV sample, without IrMn (reference); one sample with an IrMn underlayer (10 nm thick) coupled to the bottom NiFe film; one sample with IrMn underlayer and overlayer of different thickness (10 nm and 6 nm), coupled to the bottom and top NiFe film, respectively. The exchange coupling with the IrMn, causing the insurgence of the exchange bias effect, allowed the relative orientation of the NiFe magnetization vectors to be controlled by an external magnetic field, as assessed through hysteresis loop measurements by magneto-optic magnetometry. Thus, BLS spectra were acquired by sweeping the magnetic field so as to encompass both the parallel and antiparallel alignment of the NiFe layers. The BLS results, well reproduced by the presented theoretical model, clearly revealed the combined effects on the spin dynamic properties of the dipolar interaction between the two NiFe films and of the interface IrMn/NiFe exchange coupling.

  9. Iridates and RuCl3 - from Heisenberg antiferromagnets to potential Kitaev spin-liquids

    Science.gov (United States)

    van den Brink, Jeroen

    The observed richness of topological states on the single-electron level prompts the question what kind of topological phases can develop in more strongly correlated, many-body electron systems. Correlation effects, in particular intra- and inter-orbital electron-electron interactions, are very substantial in 3 d transition-metal compounds such as the copper oxides, but the spin-orbit coupling (SOC) is weak. In 5 d transition-metal compounds such as iridates, the interesting situation arises that the SOC and Coulomb interactions meet on the same energy scale. The electronic structure of iridates thus depends on a strong competition between the electronic hopping amplitudes, local energy-level splittings, electron-electron interaction strengths, and the SOC of the Ir 5d electrons. The interplay of these ingredients offers the potential to stabilise relatively well-understood states such as a 2D Heisenberg-like antiferromagnet in Sr2IrO4, but in principle also far more exotic ones, such a topological Kitaev quantum spin liquid, in (hyper)honeycomb iridates. I will discuss the microscopic electronic structures of these iridates, their proximity to idealized Heisenberg and Kitaev models and our contributions to establishing the physical factors that appear to have preempted the realization of quantum spin liquid phases so far and include a discussion on the 4d transition metal chloride RuCl3. Supported by SFB 1143 of the Deutsche Forschungsgemeinschaft.

  10. Search for the Heisenberg spin glass on rewired square lattices with antiferromagnetic interaction

    Energy Technology Data Exchange (ETDEWEB)

    Surungan, Tasrief, E-mail: tasrief@unhas.ac.id; Bansawang, B.J.; Tahir, Dahlang [Department of Physics, Hasanuddin University, Makassar, South Sulawesi 90245 (Indonesia)

    2016-03-11

    Spin glass (SG) is a typical magnetic system with frozen random spin orientation at low temperatures. The system exhibits rich physical properties, such as infinite number of ground states, memory effect, and aging phenomena. There are two main ingredients considered to be pivotal for the existence of SG behavior, namely, frustration and randomness. For the canonical SG system, frustration is led by the presence of competing interaction between ferromagnetic (FM) and antiferromagnetic (AF) couplings. Previously, Bartolozzi et al. [Phys. Rev. B73, 224419 (2006)], reported the SG properties of the AF Ising spins on scale free network (SFN). It is a new type of SG, different from the canonical one which requires the presence of both FM and AF couplings. In this new system, frustration is purely caused by the topological factor and its randomness is related to the irregular connectvity. Recently, Surungan et. al. [Journal of Physics: Conference Series, 640, 012001 (2015)] reported SG bahavior of AF Heisenberg model on SFN. We further investigate this type of system by studying an AF Heisenberg model on rewired square lattices. We used Replica Exchange algorithm of Monte Carlo Method and calculated the SG order parameter to search for the existence of SG phase.

  11. Search for the Heisenberg spin glass on rewired square lattices with antiferromagnetic interaction

    International Nuclear Information System (INIS)

    Surungan, Tasrief; Bansawang, B.J.; Tahir, Dahlang

    2016-01-01

    Spin glass (SG) is a typical magnetic system with frozen random spin orientation at low temperatures. The system exhibits rich physical properties, such as infinite number of ground states, memory effect, and aging phenomena. There are two main ingredients considered to be pivotal for the existence of SG behavior, namely, frustration and randomness. For the canonical SG system, frustration is led by the presence of competing interaction between ferromagnetic (FM) and antiferromagnetic (AF) couplings. Previously, Bartolozzi et al. [Phys. Rev. B73, 224419 (2006)], reported the SG properties of the AF Ising spins on scale free network (SFN). It is a new type of SG, different from the canonical one which requires the presence of both FM and AF couplings. In this new system, frustration is purely caused by the topological factor and its randomness is related to the irregular connectvity. Recently, Surungan et. al. [Journal of Physics: Conference Series, 640, 012001 (2015)] reported SG bahavior of AF Heisenberg model on SFN. We further investigate this type of system by studying an AF Heisenberg model on rewired square lattices. We used Replica Exchange algorithm of Monte Carlo Method and calculated the SG order parameter to search for the existence of SG phase.

  12. Gapless Spin-Liquid Ground State in the S =1 /2 Kagome Antiferromagnet

    Science.gov (United States)

    Liao, H. J.; Xie, Z. Y.; Chen, J.; Liu, Z. Y.; Xie, H. D.; Huang, R. Z.; Normand, B.; Xiang, T.

    2017-03-01

    The defining problem in frustrated quantum magnetism, the ground state of the nearest-neighbor S =1 /2 antiferromagnetic Heisenberg model on the kagome lattice, has defied all theoretical and numerical methods employed to date. We apply the formalism of tensor-network states, specifically the method of projected entangled simplex states, which combines infinite system size with a correct accounting for multipartite entanglement. By studying the ground-state energy, the finite magnetic order appearing at finite tensor bond dimensions, and the effects of a next-nearest-neighbor coupling, we demonstrate that the ground state is a gapless spin liquid. We discuss the comparison with other numerical studies and the physical interpretation of this result.

  13. Theory of Topological Spin Hall Effect in Antiferromagnetic Skyrmion: Impact on Current-induced Motion

    KAUST Repository

    Akosa, Collins Ashu

    2017-09-09

    We demonstrate that the nontrivial magnetic texture of antiferromagnetic skyrmions (AFM-Sks) promotes a non-vanishing topological spin Hall effect (TSHE) on the flowing electrons. This results in a substantial enhancement of the non-adiabatic torque and hence improves the skyrmion mobility. This non-adiabatic torque increases when decreasing the skyrmion size, and therefore scaling down results in a much higher torque efficiency. In clean AFM-Sks, we find a significant boost of the TSHE close to van Hove singularity. Interestingly, this effect is enhanced away from the band gap in the presence of non-magnetic interstitial defects. Furthermore, unlike their ferromagnetic counterpart, TSHE in AFM-Sks increases with increase in disorder strength thus opening promising avenues for materials engineering of this effect.

  14. A spin-valve-like magnetoresistance of an antiferromagnet-based tunnel junction

    Czech Academy of Sciences Publication Activity Database

    Park, B.G.; Wunderlich, Joerg; Martí, X.; Holý, V.; Kurosaki, Y.; Yamada, M.; Yamamoto, H.; Nishide, A.; Hayakawa, J.; Takahashi, H.; Shick, Alexander; Jungwirth, Tomáš

    2011-01-01

    Roč. 10, č. 5 (2011), s. 347-351 ISSN 1476-1122 R&D Projects: GA AV ČR KAN400100652; GA MŠk LC510; GA MŠk(CZ) 7E08087 EU Projects: European Commission(XE) 268066 - 0MSPIN; European Commission(XE) 214499 - NAMASTE; European Commission(XE) 215368 - SemiSpinNet Grant - others:AV ČR(CZ) AP0801 Program:Akademická prémie - Praemium Academiae Institutional research plan: CEZ:AV0Z10100521; CEZ:AV0Z10100520 Keywords : spintronics * antiferromagnets Subject RIV: BM - Solid Matter Physics ; Magnetism Impact factor: 32.841, year: 2011

  15. A separation of antiferromagnetic spin motion modes in the training effect of exchange biased Co/CoO film with in-plane anisotropy

    Energy Technology Data Exchange (ETDEWEB)

    Wu, R. [State Key Laboratory for Mesoscopic Physics, School of Physics, Peking University, Beijing 100871 (China); Department of Materials Science and Metallurgy, University of Cambridge, Cambridge CB3 0FS (United Kingdom); Yun, C.; Ding, S. L.; Wen, X.; Liu, S. Q.; Wang, C. S.; Han, J. Z.; Du, H. L. [State Key Laboratory for Mesoscopic Physics, School of Physics, Peking University, Beijing 100871 (China); Yang, J. B., E-mail: jbyang@pku.edu.cn [State Key Laboratory for Mesoscopic Physics, School of Physics, Peking University, Beijing 100871 (China); Collaborative Innovation Center of Quantum Matter, Beijing 100871 (China)

    2016-08-07

    The motion of antiferromagnetic interfacial spins is investigated through the temperature evolution of training effect in a Co/CoO film with in-plane biaxial anisotropy. Significant differences in the training effect and its temperature dependence are observed in the magnetic easy axis and hard axis (HA) and ascribed to the different motion modes of antiferromagnetic interfacial spins, the collective spin cluster rotation (CSR) and the single spin reversal (SSR), caused by different magnetization reversal modes of ferromagnetic layer. These motion modes of antiferromagnetic spins are successfully separated using a combination of an exponential function and a classic n{sup −1/2} function. A larger CSR to SSR ratio and a shorter lifetime of CSR found in the HA indicates that the domain rotation in the ferromagnetic layer tends to activate and accelerate a CSR mode in the antiferromagnetic spins.

  16. A separation of antiferromagnetic spin motion modes in the training effect of exchange biased Co/CoO film with in-plane anisotropy

    International Nuclear Information System (INIS)

    Wu, R.; Yun, C.; Ding, S. L.; Wen, X.; Liu, S. Q.; Wang, C. S.; Han, J. Z.; Du, H. L.; Yang, J. B.

    2016-01-01

    The motion of antiferromagnetic interfacial spins is investigated through the temperature evolution of training effect in a Co/CoO film with in-plane biaxial anisotropy. Significant differences in the training effect and its temperature dependence are observed in the magnetic easy axis and hard axis (HA) and ascribed to the different motion modes of antiferromagnetic interfacial spins, the collective spin cluster rotation (CSR) and the single spin reversal (SSR), caused by different magnetization reversal modes of ferromagnetic layer. These motion modes of antiferromagnetic spins are successfully separated using a combination of an exponential function and a classic n"−"1"/"2 function. A larger CSR to SSR ratio and a shorter lifetime of CSR found in the HA indicates that the domain rotation in the ferromagnetic layer tends to activate and accelerate a CSR mode in the antiferromagnetic spins.

  17. An S=1/2 impurity spin in the antiferromagnetic S=1 bond-alternating chain

    Energy Technology Data Exchange (ETDEWEB)

    Ogawa, Nobuyuki [Gifu National College of Technology, Dept. of Fundamental Science, Gifu (Japan); Hikihara, Toshiya [National Inst. for Materials Science, Computational Material Research Group, Tsukuba, Ibaraki (Japan); Kaburagi, Makoto [Kobe Univ., Faculty of Cross-Cultural Studies, Kobe, Hyogo (Japan); Tonegawa, Takashi [Fukui Univ. of Technology, Dept. of Mechanical Engineering, Fukui (Japan)

    2002-06-01

    We explore low-lying excited states as well as the ground state of the antiferromagnetic S=1 bond-alternating chain with an S=1/2 impurity spin. For the case where the ground-state phase of the host system is the Haldane phase, we review a numerical analysis of the electron-spin-resonance experimental results on the NENP: Cu{sup 2+} system. For the case where the ground-state phase of the host system is the dimer phase, on the other hand, we calculate, using the exact-diagonalization method, the dependences of the energy differences between the ground and low-lying excited states upon both the impurity-host exchange constant and the single-ion-type anisotropy constant, and also calculate, using the density-matrix renormalization-group method, the external-magnetic-field dependence of the impurity-spin magnetization in the ground state. In these calculations, we keep the NTENP: Cu{sup 2+} system in mind to choose the value of the bond-alternation parameter. We find that a few low-lying excited states which are expected from the valence-bond-solid picture appear as the impurity states in the energy gap between the singlet ground and triplet first-excited states (the dimer gap). Furthermore, for certain values of the above constants, we find that the impurity-spin magnetization shows a clear jump at a magnetic field which is in the dimer-gap region or in the magnetization-plateau region of the host system, and also that the impurity-spin magnetization has a magnetic-field region where it decreases as a function of the magnetic field. (author)

  18. Spin wave energy dispersion in KCuF/sub 3/: a nearly one-dimensional spin-1/2 antiferromagnet. [4. 7/sup 0/K

    Energy Technology Data Exchange (ETDEWEB)

    Hutchings, M T; Ikeda, H; Milne, J M

    1979-09-28

    Using inelastic neutron scattering techniques, the spin wave energy dispersion in the (010) plane of the distorted perovskite KCuF/sub 3/, which exhibits many magnetic properties of the spin-1/2 one-dimensional antiferromagnet, has been investigated at 4.7 K (T/sub N/ = 39 K). The measurements confirm the very strong exchange interaction between the spins in the (001) direction, and show that in this direction the expression for the excitation energies of the spin-1/2 antiferromagnetic chain given by J des Cloizeaux and J J Pearson is obeyed. The exchange interaction between these chains is found to be only 1.6% of that within the chains.

  19. Effect of nanostructure layout on spin pumping phenomena in antiferromagnet/nonmagnetic metal/ferromagnet multilayered stacks

    Directory of Open Access Journals (Sweden)

    A. F. Kravets

    2017-05-01

    Full Text Available In this work we focus on magnetic relaxation in Mn80Ir20(12 nm/Cu(6 nm/Py(dF antiferromagnet/Cu/ferromagnet (AFM/Cu/FM multilayers with different thickness of the ferromagnetic permalloy layer. An effective FM-AFM interaction mediated via the conduction electrons in the nonmagnetic Cu spacer – the spin-pumping effect – is detected as an increase in the linewidth of the ferromagnetic resonance (FMR spectra and a shift of the resonant magnetic field. We further find experimentally that the spin-pumping-induced contribution to the linewidth is inversely proportional to the thickness of the Py layer. We show that this thickness dependence likely originates from the dissipative dynamics of the free and localized spins in the AFM layer. The results obtained could be used for tailoring the dissipative properties of spintronic devices incorporating antiferromagnetic layers.

  20. Calorimetric evidence for localized spin fluctuations in UA12

    International Nuclear Information System (INIS)

    Trainor, R.J.; Brodsky, M.B.; Isaacs, L.L.

    1974-01-01

    Results of heat capacity measurements on UAl 2 between 1.8 and 400 0 K are presented. The data are compared with recent resistivity and susceptibility measurements which indicate the existence of localized spin fluctuations in a narrow 5f band. Below about 50 0 K the electronic contribution to the heat capacity becomes large, equivalent to γ approximately 70 mJ/mole-K 2 . Below 6 0 K there is an upturn in C/T which is proportional to T 2 log (T/T/sub SF/), where T/sub SF/ = 10.6 0 K is identified as the spin fluctuation temperature. Extrapolation of this term to zero temperature yields m*/m approximately 2 for the spin-fluctuation mass enhancement. At 300 0 K, UAl 2 exhibits more typical metallic behavior, with γ approximately 15 mJ/mole-K 2 . Data are also presented for nonmagnetic URh 3 ; at low temperatures C = γT + βT 3 , with γ = 14.5 mJ/mole-K 2 and β corresponding to theta/sub D/ = 336 0 K. (U.S.)

  1. Surface-spin magnetism of antiferromagnetic NiO in nanoparticle and bulk morphology

    International Nuclear Information System (INIS)

    Jagodic, M; Jaglicic, Z; Jelen, A; Dolinsek, J; Lee, Jin Bae; Kim, Hae Jin; Kim, Young-Min

    2009-01-01

    The surface-spin magnetism of the antiferromagnetic (AFM) material NiO in nanoparticle and bulk morphology was investigated by magnetic measurements (temperature-dependent zero-field-cooled (zfc) and field-cooled (fc) dc susceptibility, ac susceptibility and zfc and fc hysteresis loops). We addressed the question of whether the multisublattice ordering of the uncompensated surface spins and the exchange bias (EB) effect are only present in the nanoparticles, originating from their high surface-to-volume ratio or if these surface phenomena are generally present in the AFM materials regardless of their bulky or nanoparticle morphology, but the effect is just too small to be detected experimentally in the bulk due to a very small surface magnetization. Performing experiments on the NiO nanoparticles of different sizes and bulk NiO grains, we show that coercivity enhancement and hysteresis loop shift in the fc experiments, considered to be the key experimental manifestations of multisublattice ordering and the EB effect, are true nanoscale phenomena only present in the nanoparticles and absent in the bulk.

  2. Coexistence of ferromagnetism and spin glass behavior in antiferromagnetic Y2BaCuO5

    International Nuclear Information System (INIS)

    Zhu, Zhonghua; Gao, Daqiang; Zhang, Jing; Shi, Zhenhua; Gao, Hua; Yang, Zhaolong; Zhang, Zhipeng; Xue, Desheng

    2013-01-01

    Highlights: • Room temperature ferromagnetism is observed in ultrafine Y 2 BaCuO 5 particles. • The observed ferromagnetism originates from the oxygen defects. • A very interesting spin glass transition located at about 110 K is found. -- Abstract: We report the synthesis of a series of Y 2 BaCuO 5 samples by varying the annealing temperature with a citrate pyrolysis technique. X-ray diffraction patterns, scanning electron microscopy and transmission electron microscopy observation show the formation of a columnar Y 2 BaCuO 5 phase and these samples are composed of many irregular particles with different particle size. Magnetic measurements show that these samples exhibit room temperature ferromagnetism and the saturation magnetization decreases with increasing sintering temperature. Post-heating treatment under argon atmosphere can enhance the ferromagnetism greatly, suggesting that the magnetism is attributed to the surface oxygen defects. By measuring magnetization versus temperature curves after zero field cooling with various applied magnetic fields, two magnetic phase transitions located at about 11 and 110 K are revealed. The position of the peak at about 11 K is independent of the magnetic field; the other peak, however, becomes rounder and shifts to lower temperatures with increasing the magnetic field, showing a strong field dependence. In addition, the virgin magnetization curves with the measured temperature below 110 K display an S-type. These features are suggestive of an antiferromagnetic phase transition at about 11 K and a spin glass transition at about 110 K

  3. Terahertz-Frequency Spin Hall Auto-oscillator Based on a Canted Antiferromagnet

    Science.gov (United States)

    Sulymenko, O. R.; Prokopenko, O. V.; Tiberkevich, V. S.; Slavin, A. N.; Ivanov, B. A.; Khymyn, R. S.

    2017-12-01

    We propose a design of a terahertz-frequency signal generator based on a layered structure consisting of a current-driven platinum (Pt) layer and a layer of an antiferromagnet (AFM) with easy-plane anisotropy, where the magnetization vectors of the AFM sublattices are canted inside the easy plane by the Dzyaloshinskii-Moriya interaction (DMI). The dc electric current flowing in the Pt layer creates due to the spin Hall effect, a perpendicular spin current that, being injected in the AFM layer, tilts the DMI-canted AFM sublattices out of the easy plane, thus exposing them to the action of a strong internal exchange magnetic field of the AFM. The sublattice magnetizations, along with the small net magnetization vector mDMI of the canted AFM, start to rotate about the hard anisotropy axis of the AFM with the terahertz frequency proportional to the injected spin current and the AFM exchange field. The rotation of the small net magnetization mDMI results in the terahertz-frequency dipolar radiation that can be directly received by an adjacent (e.g., dielectric) resonator. We demonstrate theoretically that the radiation frequencies in the range f =0.05 - 2 THz are possible at the experimentally reachable magnitudes of the driving current density, and we evaluate the power of the signal radiated into different types of resonators. This power increases with the increase of frequency f , and it can exceed 1 μ W at f ˜0.5 THz for a typical dielectric resonator of the electric permittivity ɛ ˜10 and a quality factor Q ˜750 .

  4. Spiral phases of doped antiferromagnets

    International Nuclear Information System (INIS)

    Shraiman, B.I.; Siggia, E.D.

    1990-01-01

    The dipole density field describing the holls in a doped antiferromagnet is considered for law hole density in the semiclassical limit. This yields a phase in which the order parameter is planar and spirals round a fixed direction. The single spiral state breaks the continuous spin rotational symmetry and exhibits long-range order at zero temperature. In it there is a global spin direction as rotation axis. The double spiral state, in which there are two perpendicular directions, is isotropic in both spin and real space. Several results of microscopic calculations, carried out to understand the electronic states, quantum fluctuations, lattice effects and normal mode dynamics, are recapitulated. 8 refs

  5. Dynamics of dimer and z spin component fluctuations in spin-1/2 XY chain

    Directory of Open Access Journals (Sweden)

    P.Hlushak

    2005-01-01

    Full Text Available One-dimensional quantum spin-1/2 XY models admit the rigorous analysis not only of their static properties (i.e. the thermodynamic quantities and the equal-time spin correlation functions but also of their dynamic properties (i.e. the different-time spin correlation functions, the dynamic susceptibilities, the dynamic structure factors. This becomes possible after exploiting the Jordan-Wigner transformation which reduces the spin model to a model of spinless noninteracting fermions. A number of dynamic quantities (e.g. related to transverse spin operator or dimer operator fluctuations are entirely determined by two-fermion excitations and can be examined in much detail.

  6. Single-pulse terahertz coherent control of spin resonance in the canted antiferromagnet YFeO3, mediated by dielectric anisotropy

    DEFF Research Database (Denmark)

    Jin, Zuanming; Mics, Zoltán; Ma, Guohong

    2013-01-01

    We report on the coherent control of terahertz (THz) spin waves in a canted antiferromagnet yttrium orthoferrite, YFeO3, associated with a quasiferromagnetic (quasi-FM) spin resonance at a frequency of 0.3 THz, using a single-incident THz pulse. The spin resonance is excited impulsively by the ma...... polarization of the THz oscillation at the spin resonance frequency, suggests a key role of magnon–phonon coupling in spin-wave energy dissipation....

  7. Coherence properties of holes subject to a fluctuating spin chirality

    International Nuclear Information System (INIS)

    Wheatley, J.M.; Hong, T.M.

    1991-01-01

    The coherence properties of holes coupled to short-ranged chiral spin fluctuations with a characteristic chiral spin fluctuation time τ ch =ω ch -1 are investigated in two dimensions. At temperatures kT much-lt 4π 2 left-angle φ 2 right-angle -1 ℎω ch hole quasiparticles exist and propagate with a renormalized mass m * /m=1+left-angle φ 2 right-angle ℎ/16πma 0 2 ω ch . $langle phi sup 2 rangle--- is the amplitude of the local fictitious flux fluctuation and a 0 is a lattice cutoff. At temperatures kT much-gt 4π 2 left-angle φ 2 right-angle -1 ℎω ch an effective-mass approximation is invalid and we find that the hole diffuses according to a logarithmic diffusion law in the quasistatic chiral field. The unusual diffusion law is a consequence of the long-ranged nature of the gauge field. The result shows that the holes do not form a coherent quantum fluid in the quasistatic regime

  8. Grüneisen Parameter and Thermal Expansion by the Self-Consistent Renormalization Theory of Spin Fluctuations

    Science.gov (United States)

    Watanabe, Shinji; Miyake, Kazumasa

    2018-03-01

    The thermal expansion coefficient α and the Grüneisen parameter Γ near the magnetic quantum critical point (QCP) are derived on the basis of the self-consistent renormalization (SCR) theory of spin fluctuations. From the SCR entropy, the specific heat CV, α, and Γ are shown to be expressed in a simple form as CV = Ca - Cb, α = αa + αb, and Γ = Γa + Γb, respectively, where Ci, αi, and Γi (i = a, b) are related with each other. As the temperature T decreases, Ca, αb, and Γb become dominant in CV, α, and Γ, respectively. The inverse susceptibility of spin fluctuation coupled to the volume V in Γb is found to give rise to the divergence of Γ at the QCP for each class of ferromagnetism and antiferromagnetism (AFM) in spatial dimensions d = 3 and 2. This V-dependent inverse susceptibility in αb and Γb contributes to the T dependences of α and Γ, and even affects their criticality in the case of the AFM QCP in d = 2. Γa is expressed as Γ a(T = 0) = - V/T0( {partial T0}/{partial V} )T = 0 with T0 being the characteristic temperature of spin fluctuation, which has an enhanced value in heavy electron systems.

  9. Antiferromagnetic coupling in a six-coordinate high spin cobalt(II)-semiquinonato complex.

    Science.gov (United States)

    Caneschi, Andrea; Dei, Andrea; Gatteschi, Dante; Tangoulis, Vassilis

    2002-07-01

    The 3,5-di-tert-butyl-catecholato and 9,10-phenanthrenecatecholato adducts of the cobalt-tetraazamacrocycle complex Co(Me(4)cyclam)(2+) (Me(4)cyclam = 1,4,8,11-tetramethyl-1,4,8,11-tetraazacyclotetradecane) were synthesized and oxidized. The oxidation reaction products were isolated in the solid state as hexafluorophosphate derivatives. Both these complexes can be formulated as 1:1 cobalt(II)-semiquinonato complexes, that is, Co(Me(4)cyclam)(DBSQ)PF(6) (1) and Co(Me(4)cyclam)(PhSQ)PF(6) (2), in the temperature range 4-300 K, in striking contrast with the charge distribution found in similar adducts formed by related tetraazamacrocycles. The synthesis strategy and the structural, spectroscopic, and magnetic properties are reported and discussed. The crystallographic data for 2 are as follows: monoclinic, space group P2(1)/a, nomicron. 14, a = 14.087(4) A, b = 15.873(4) A, c = 14.263 (7) A, alpha = 89.91(3) degrees, beta = 107.34(2) degrees, gamma = 90.08(2) degrees, Z = 4. Both these complexes are characterized by triplet electronic ground states arising from the antiferromagnetic coupling between the high-spin d(7) metal ion and the radical ligand.

  10. Quantum-Classical Phase Transition of the Escape Rate of Two-Sublattice Antiferromagnetic Large Spins

    Science.gov (United States)

    Owerre, Solomon Akaraka; Paranjape, M. B.

    2014-11-01

    The Hamiltonian of a two-sublattice antiferromagnetic spins, with single (hard-axis) and double ion anisotropies described by H = J {\\hat S}1...\\hatS 2-2Jz \\hat {S}1z\\hat {S}2z+K(\\hat {S}1z2 +\\hat {S}2z2) is investigated using the method of effective potential. The problem is mapped to a single particle quantum-mechanical Hamiltonian in terms of the relative coordinate and reduced mass. We study the quantum-classical phase transition of the escape rate of this model. We show that the first-order phase transition for this model sets in at the critical value Jc = (Kc+Jz, c)/2 while for the anisotropic Heisenberg coupling H = J(S1xS2x +S1yS2y) + JzS1zS2z + K(S1z2+ S2z2) we obtain Jc = (2Kc-Jz, c)/3. The phase diagrams of the transition are also studied.

  11. Investigation of the stationary state of parametric spin waves in antiferromagnetics by the modulation technique

    International Nuclear Information System (INIS)

    Andrienko, A.V.; Safonov, V.L.; Yakubovskij, A.Yu.

    1987-01-01

    The response of parametric electron and nuclear spin waves to weak modulation of a stationary magnetic field is investigated in the antiferromagnetics MnCO 3 and CsMnF 3 . The modulation response is calculated by taking into accout the phase mechanism of restriction of the parametric wave amplitude and positive nonlinear attenuation of the waves. Some characteristics of the stationary state of parametric electron and nuclear magnons are determined within the framework of the model by analysis of the experimental results: the nonlinear magnon interaction coefficient S k and the parameter κ which characterizes the relative contribution from positive nonlinear attenuation and the phase mechanism to the restriction of the number of parametric magnons. An anomaly in the behavior of the modulation response of the parametric nuclear magnons is observed in CsMnF 3 ; this is manifest in asubstantial decrease of the modulation response in a narrow supercriticality and modulation frequency range. A giant hexagonal anisotropy of the modulation response and nonlinear dynamic susceptibility of the nuclear magnons is observed in the same crystal. This may indicate a nonisotropic distribution of the magnons in k-space

  12. Spin glass behavior of the antiferromagnetic Heisenberg model on scale free network

    International Nuclear Information System (INIS)

    Surungan, Tasrief; Zen, Freddy P; Williams, Anthony G

    2015-01-01

    Randomness and frustration are considered to be the key ingredients for the existence of spin glass (SG) phase. In a canonical system, these ingredients are realized by the random mixture of ferromagnetic (FM) and antiferromagnetic (AF) couplings. The study by Bartolozzi et al. [Phys. Rev. B73, 224419 (2006)] who observed the presence of SG phase on the AF Ising model on scale free network (SFN) is stimulating. It is a new type of SG system where randomness and frustration are not caused by the presence of FM and AF couplings. To further elaborate this type of system, here we study Heisenberg model on AF SFN and search for the SG phase. The canonical SG Heisenberg model is not observed in d-dimensional regular lattices for (d ≤ 3). We can make an analogy for the connectivity density (m) of SFN with the dimensionality of the regular lattice. It should be plausible to find the critical value of m for the existence of SG behaviour, analogous to the lower critical dimension (d l ) for the canonical SG systems. Here we study system with m = 2, 3, 4 and 5. We used Replica Exchange algorithm of Monte Carlo Method and calculated the SG order parameter. We observed SG phase for each value of m and estimated its corersponding critical temperature. (paper)

  13. Superconducting fluctuations in systems with Rashba-spin-orbit coupling

    Energy Technology Data Exchange (ETDEWEB)

    Beyl, Stefan [Institut fuer Theoretische Physik und Astrophysik, Universitaet Wuerzburg (Germany); Orth, Peter P.; Scheurer, Mathias; Schmalian, Joerg [Institut fuer Theorie der Kondensierten Materie, Karlsruher Institut fuer Technologie (Germany)

    2015-07-01

    We investigate the BEC-BCS crossover in a two-dimensional system with Rashba-spin-orbit coupling. To include the effects of phase and amplitude fluctuations of the superconducting order parameter we perform a loop expansion of the effective field theory. We analyze in particular the probability of a low density superconducting quantum phase transition. The theory is relevant to LaAlO{sub 3}/SrTiO{sub 3} interfaces and two-dimensional cold atom systems with synthetic gauge fields.

  14. Dynamic magnetic behavior of the mixed spin (2, 5/2) Ising system with antiferromagnetic/antiferromagnetic interactions on a bilayer square lattice

    International Nuclear Information System (INIS)

    Ertaş Mehmet; Keskin Mustafa

    2013-01-01

    Using the mean-field theory and Glauber-type stochastic dynamics, we study the dynamic magnetic properties of the mixed spin (2, 5/2) Ising system for the antiferromagnetic/antiferromagnetic (AFM/AFM) interactions on the bilayer square lattice under a time varying (sinusoidal) magnetic field. The time dependence of average magnetizations and the thermal variation of the dynamic magnetizations are examined to calculate the dynamic phase diagrams. The dynamic phase diagrams are presented in the reduced temperature and magnetic field amplitude plane and the effects of interlayer coupling interaction on the critical behavior of the system are investigated. We also investigate the influence of the frequency and find that the system displays richer dynamic critical behavior for higher values of frequency than that of the lower values of it. We perform a comparison with the ferromagnetic/ferromagnetic (FM/FM) and AFM/FM interactions in order to see the effects of AFM/AFM interaction and observe that the system displays richer and more interesting dynamic critical behaviors for the AFM/AFM interaction than those for the FM/FM and AFM/FM interactions. (general)

  15. Mermin-Wagner physics, (H ,T ) phase diagram, and candidate quantum spin-liquid phase in the spin-1/2 triangular-lattice antiferromagnet Ba8CoNb6O24

    Science.gov (United States)

    Cui, Y.; Dai, J.; Zhou, P.; Wang, P. S.; Li, T. R.; Song, W. H.; Wang, J. C.; Ma, L.; Zhang, Z.; Li, S. Y.; Luke, G. M.; Normand, B.; Xiang, T.; Yu, W.

    2018-04-01

    Ba8CoNb6O24 presents a system whose Co2 + ions have an effective spin 1/2 and construct a regular triangular-lattice antiferromagnet (TLAFM) with a very large interlayer spacing, ensuring purely two-dimensional character. We exploit this ideal realization to perform a detailed experimental analysis of the S =1 /2 TLAFM, which is one of the keystone models in frustrated quantum magnetism. We find strong low-energy spin fluctuations and no magnetic ordering, but a diverging correlation length down to 0.1 K, indicating a Mermin-Wagner trend toward zero-temperature order. Below 0.1 K, however, our low-field measurements show an unexpected magnetically disordered state, which is a candidate quantum spin liquid. We establish the (H ,T ) phase diagram, mapping in detail the quantum fluctuation corrections to the available theoretical analysis. These include a strong upshift in field of the maximum ordering temperature, qualitative changes to both low- and high-field phase boundaries, and an ordered regime apparently dominated by the collinear "up-up-down" state. Ba8CoNb6O24 , therefore, offers fresh input for the development of theoretical approaches to the field-induced quantum phase transitions of the S =1 /2 Heisenberg TLAFM.

  16. Low to High Spin-State Transition Induced by Charge Ordering in Antiferromagnetic YBaCo2O5

    International Nuclear Information System (INIS)

    Vogt, T.; Woodward, P. M.; Karen, P.; Hunter, B. A.; Henning, P.; Moodenbaugh, A. R.

    2000-01-01

    The oxygen-deficient double perovskite YBaCo 2 O 5 , containing corner-linked CoO 5 square pyramids as principal building units, undergoes a paramagnetic to antiferromagnetic spin ordering at 330 K. This is accompanied by a tetragonal to orthorhombic distortion. Below 220 K orbital ordering and long-range Co 2+ /Co 3+ charge ordering occur as well as a change in the Co 2+ spin state from low to high spin. This transition is shown to be very sensitive to the oxygen content of the sample. To our knowledge this is the first observation of a spin-state transition induced by long-range orbital and charge ordering. (c) 2000 The American Physical Society

  17. Magnetization plateaus in the spin-1/2 antiferromagnetic Heisenberg model on a kagome-strip chain

    Science.gov (United States)

    Morita, Katsuhiro; Sugimoto, Takanori; Sota, Shigetoshi; Tohyama, Takami

    2018-01-01

    The spin-1/2 Heisenberg model on a kagome lattice is a typical frustrated quantum spin system. The basic structure of a kagome lattice is also present in the kagome-strip lattice in one dimension, where a similar type of frustration is expected. We thus study the magnetization plateaus of the spin-1/2 Heisenberg model on a kagome-strip chain with three-independent antiferromagnetic exchange interactions using the density-matrix renormalization-group method. In a certain range of exchange parameters, we find twelve kinds of magnetization plateaus, nine of which have magnetic structures breaking translational and/or reflection symmetry spontaneously. The structures are classified by an array of five-site unit cells with specific bond-spin correlations. In a case with a nontrivial plateau, namely a 3/10 plateau, we find long-period magnetic structure with a period of four unit cells.

  18. Evolution of spin excitations in a gapped antiferromagnet from the quantum to the high-temperature limit

    DEFF Research Database (Denmark)

    Kenzelmann, M.; Cowley, R.A.; Buyers, W.J.L.

    2002-01-01

    We have mapped from the quantum to the classical limit the spin excitation spectrum of the antiferromagnetic spin-1 Heisenberg chain system CsNiCl3 in its paramagnetic phase from T=5 to 200 K. Neutron scattering shows that the excitations are resonant and dispersive up to at least T=70 Ksimilar...... is in agreement with quantum Monte Carlo calculations for the spin-1 chain. xi is also consistent with the single mode approximation, suggesting that the excitations are short-lived single particle excitations. Below T=12 K where three-dimensional spin correlations are important, xi is shorter than predicted...... and the experiment is not consistent with the random phase approximation for coupled quantum chains. At T=200 K, the structure factor and second energy moment of the excitation spectrum are in excellent agreement with the high-temperature series expansion....

  19. Antiferromagnetic skyrmions

    Science.gov (United States)

    Tretiakov, Oleg; Barker, Joseph

    Skyrmions are topologically protected entities in magnetic materials which have the potential to be used in spintronics for information storage and processing. However, skyrmions in ferromagnets have some intrinsic difficulties which must be overcome to use them for spintronic applications, such as the inability to move straight along current. We show that skyrmions can also be stabilized and manipulated in antiferromagnetic materials. An antiferromagnetic skyrmion is a compound topological object with a similar but of opposite sign spin texture on each sublattice, which e.g. results in a complete cancelation of the Magnus force. We find that the composite nature of antiferromagnetic skyrmions gives rise to different dynamical behavior, both due to an applied current and temperature effects. O.A.T. and J.B. acknowledge support by the Grants-in-Aid for Scientific Research (Nos. 25800184, 25247056, 25220910 and 15H01009) from the Ministry of Education, Culture, Sports, Science and Technology (MEXT) of Japan and SpinNet.

  20. Muon spin relaxation measurements of the fluctuation modes in spin-glass AgNm

    Energy Technology Data Exchange (ETDEWEB)

    Heffner, R.H.; Leon, M.; Schillaci, M.E.; MacLaughlin, D.E.; Dodds, S.A.

    1983-01-01

    Recently reported zero-field ..mu..SR measurements below the spin-glass transition temperature in AgMn (1.6 at%) show a temperature dependent inhomogeneous width. The authors discuss these data in terms of a model in which the local field undergoes limited-amplitude fluctuations. The authors find that both very slow (approx. = 0.3 ..mu..s/sup -1/) and rapid (approx. = 3000 ..mu..s/sup -1/) fluctuations are required. 10 references, 1 figure, 1 table.

  1. Microscopic theory of the nearest-neighbor valence bond sector of the spin-1/2 kagome antiferromagnet

    Science.gov (United States)

    Ralko, Arnaud; Mila, Frédéric; Rousochatzakis, Ioannis

    2018-03-01

    The spin-1/2 Heisenberg model on the kagome lattice, which is closely realized in layered Mott insulators such as ZnCu3(OH) 6Cl2 , is one of the oldest and most enigmatic spin-1/2 lattice models. While the numerical evidence has accumulated in favor of a quantum spin liquid, the debate is still open as to whether it is a Z2 spin liquid with very short-range correlations (some kind of resonating valence bond spin liquid), or an algebraic spin liquid with power-law correlations. To address this issue, we have pushed the program started by Rokhsar and Kivelson in their derivation of the effective quantum dimer model description of Heisenberg models to unprecedented accuracy for the spin-1/2 kagome, by including all the most important virtual singlet contributions on top of the orthogonalization of the nearest-neighbor valence bond singlet basis. Quite remarkably, the resulting picture is a competition between a Z2 spin liquid and a diamond valence bond crystal with a 12-site unit cell, as in the density-matrix renormalization group simulations of Yan et al. Furthermore, we found that, on cylinders of finite diameter d , there is a transition between the Z2 spin liquid at small d and the diamond valence bond crystal at large d , the prediction of the present microscopic description for the two-dimensional lattice. These results show that, if the ground state of the spin-1/2 kagome antiferromagnet can be described by nearest-neighbor singlet dimers, it is a diamond valence bond crystal, and, a contrario, that, if the system is a quantum spin liquid, it has to involve long-range singlets, consistent with the algebraic spin liquid scenario.

  2. Perspectives of antiferromagnetic spintronics

    Science.gov (United States)

    Jungfleisch, Matthias B.; Zhang, Wei; Hoffmann, Axel

    2018-04-01

    Antiferromagnets are promising for future spintronic applications owing to their advantageous properties: They are magnetically ordered, but neighboring magnetic moments point in opposite directions, which results in zero net magnetization. This means antiferromagnets produce no stray fields and are insensitive to external magnetic field perturbations. Furthermore, they show intrinsic high frequency dynamics, exhibit considerable spin-orbit and magneto-transport effects. Over the past decade, it has been realized that antiferromagnets have more to offer than just being utilized as passive components in exchange bias applications. This development resulted in a paradigm shift, which opens the pathway to novel concepts using antiferromagnets for spin-based technologies and applications. This article gives a broad perspective on antiferromagnetic spintronics. In particular, the manipulation and detection of antiferromagnetic states by spintronics effects, as well as spin transport and dynamics in antiferromagnetic materials will be discussed. We will also outline current challenges and future research directions in this emerging field.

  3. Spin-flip transition and Faraday effect in antiferromagnet KMnF3 in megagauss magnetic field

    International Nuclear Information System (INIS)

    Mukhin, A.A.; Plis, V.I.; Popov, A.I.; Zvezdin, A.K.; Platonov, V.; Tatsenko, O.M.

    1998-01-01

    Faraday effect in the antiferromagnet KMnF 3 has been investigated in pulse explosive fields up to 500 T at T=78 K. The laser wavelength 0.63 μm was used in the experiment. The magnetic field dependence of Faraday rotation in this antiferromagnet shows a unique feature of a lack of saturation effect in the fields up to 500 T whereas critical field of spin-flip transition is about 120 T. The theoretical analysis of microscopic nature of Faraday rotation, including the diamagnetic, magneto-dipole and paramagnetic mechanisms has been performed. The strong competition of these mechanisms is important to explain the extremely small value of the effect and its unusual magnetic field dependence

  4. Zero-Field Spin Structure and Spin Reorientations in Layered Organic Antiferromagnet, κ-(BEDT-TTF)2Cu[N(CN)2]Cl, with Dzyaloshinskii-Moriya Interaction

    Science.gov (United States)

    Ishikawa, Rui; Tsunakawa, Hitoshi; Oinuma, Kohsuke; Michimura, Shinji; Taniguchi, Hiromi; Satoh, Kazuhiko; Ishii, Yasuyuki; Okamoto, Hiroyuki

    2018-06-01

    Detailed magnetization measurements enabled us to claim that the layered organic insulator κ-(BEDT-TTF)2Cu[N(CN)2]Cl [BEDT-TTF: bis(ethylenedithio)tetrathiafulvalene] with the Dzyaloshinskii-Moriya interaction has an antiferromagnetic spin structure with the easy axis being the crystallographic c-axis and the net canting moment parallel to the a-axis at zero magnetic field. This zero-field spin structure is significantly different from that proposed in the past studies. The assignment was achieved by arguments including a correction of the direction of the weak ferromagnetism, reinterpretations of magnetization behaviors, and reasoning based on known high-field spin structures. We suggest that only the contributions of the strong intralayer antiferromagnetic interaction, the moderately weak Dzyaloshinskii-Moriya interaction, and the very weak interlayer ferromagnetic interaction can realize this spin structure. On the basis of this model, characteristic magnetic-field dependences of the magnetization can be interpreted as consequences of intriguing spin reorientations. The first reorientation is an unusual spin-flop transition under a magnetic field parallel to the b-axis. Although the existence of this transition is already known, the interpretation of what happens at this transition has been significantly revised. We suggest that this transition can be regarded as a spin-flop phenomenon of the local canting moment. We also claim that half of the spins rotate by 180° at this transition, in contrast to the conventional spin flop transition. The second reorientation is the gradual rotation of the spins during the variation of the magnetic field parallel to the c-axis. In this process, all the spins rotate around the Dzyaloshinskii-Moriya vectors by 90°. The results of our simulation based on the classical spin model well reproduce these spin reorientation behaviors, which strongly support our claimed zero-field spin structure. The present study highlights the

  5. Effective S =2 antiferromagnetic spin chain in the salt (o -MePy-V)FeCl4

    Science.gov (United States)

    Iwasaki, Y.; Kida, T.; Hagiwara, M.; Kawakami, T.; Hosokoshi, Y.; Tamekuni, Y.; Yamaguchi, H.

    2018-02-01

    We present a model compound for the S =2 antiferromagnetic (AF) spin chain composed of the salt (o -MePy-V ) FeCl4 . Ab initio molecular-orbital calculations indicate the formation of a partially stacked two-dimensional (2D) spin model comprising five types of exchange interactions between S =1 /2 and S =5 /2 spins, which locate on verdazyl radical and Fe ion, respectively. The magnetic properties of the synthesized crystals indicate that the dominant interaction between the S =1 /2 and S =5 /2 spins stabilizes an S =2 spin in the low-temperature region, and an effective S =2 AF chain is formed for T ≪10 K and H chain. At higher fields above quantitatively 4 T, the magnetization curve assumes two-thirds of the full saturation value for fields between 4 and 20 T, and approaches saturation at ˜40 T. The spin model in the high-field region can be considered as a quasi-2D S =1 /2 honeycomb lattice under an effective internal field caused by the fully polarized S =5 /2 spin.

  6. Spin-triplet excitons and anisotropy effects in the S=12 gapped antiferromagnet BaCuSi2O6

    International Nuclear Information System (INIS)

    Zvyagin, S.A.; Wosnitza, J.; Krzystek, J.; Stern, R.; Jaime, M.; Sasago, Y.; Uchinokura, K.

    2007-01-01

    BaCuSi 2 O 6 can be regarded as an almost ideal realization of an S=12 system of weakly interacting spin dimers with spin-singlet ground state and gapped excitation spectrum. We argue that the fine structure observed in low-temperature EPR spectra of BaCuSi 2 O 6 is a fingerprint of triplet excitations (excitons). Analyzing the angular dependence of the exciton modes allows us to precisely calculate the zero-field splitting within the triplet states and, correspondingly, the anisotropy parameter, D=0.07cm -1 . The proposed procedure can be applied for studying anisotropy effects in a large number of S=12 gapped quantum antiferromagnets with dimerized or alternating spin structure

  7. Unusual magnetic excitations in the weakly ordered spin- 12 chain antiferromagnet Sr2CuO3: Possible evidence for Goldstone magnon coupled with the amplitude mode

    International Nuclear Information System (INIS)

    Sergeicheva, E. G.; Sosin, S. S.; Prozorova, L. A.; Gu, G. D.; Zaliznyak, I. A.

    2017-01-01

    We report on an electron spin resonance (ESR) study of a nearly one-dimensional (1D) spin-1/2 chain antiferromagnet, Sr 2 CuO 3 , with extremely weak magnetic ordering. The ESR spectra at T > T N , in the disordered Luttinger-spin-liquid phase, reveal nearly ideal Heisenberg-chain behavior with only a very small, field-independent linewidth, ~1/T. In the ordered state, below T N , we identify field-dependent antiferromagnetic resonance modes, which are well described by pseudo-Goldstone magnons in the model of a collinear biaxial antiferromagnet. Additionally, we observe a major resonant mode with unusual and strongly anisotropic properties, which is not anticipated by the conventional theory of Goldstone spin waves. Lastly, we propose that this unexpected magnetic excitation can be attributed to a field-independent magnon mode renormalized due to its interaction with the high-energy amplitude (Higgs) mode in the regime of weak spontaneous symmetry breaking.

  8. Spin-fluctuation mechanism of high-Tc superconductivity and order-parameter symmetry

    International Nuclear Information System (INIS)

    Izyumov, Yurii A

    1999-01-01

    The notion that electrons in high-T c cuprates pair via antiferromagnetic spin fluctuations is discussed and the symmetry of the superconducting order parameter is analyzed. Three approaches to the problem, one phenomenological (with an experimental dynamic magnetic susceptibility) and two microscopic (involving, respectively, the Hubbard model and the tJ-model) are considered and it is shown that in each case strong-coupling theory leads to a d-wave order parameter with zeros at the Fermi surface. The review then proceeds to consider experimental techniques in which the d-symmetry of the order parameter may manifest itself. These include low-temperature thermodynamic measurements, measurements of the penetration depth and the upper critical field, Josephson junction experiments to obtain the phase of the superconducting order parameter, and various spectroscopic methods. The experimental data suggest that the order parameter in cuprates is d x 2 -y 2 -wave. Ginzburg-Landau theory for a superconductor with a d-wave order parameter is outlined and both an isolated vortex and a vortex lattice are investigated. Finally, some theoretical aspects of the effects of nonmagnetic impurities on a d-wave superconductor are considered. (reviews of topical problems)

  9. Quantum Criticality of an Ising-like Spin-1 /2 Antiferromagnetic Chain in a Transverse Magnetic Field

    Science.gov (United States)

    Wang, Zhe; Lorenz, T.; Gorbunov, D. I.; Cong, P. T.; Kohama, Y.; Niesen, S.; Breunig, O.; Engelmayer, J.; Herman, A.; Wu, Jianda; Kindo, K.; Wosnitza, J.; Zherlitsyn, S.; Loidl, A.

    2018-05-01

    We report on magnetization, sound-velocity, and magnetocaloric-effect measurements of the Ising-like spin-1 /2 antiferromagnetic chain system BaCo2V2O8 as a function of temperature down to 1.3 K and an applied transverse magnetic field up to 60 T. While across the Néel temperature of TN˜5 K anomalies in magnetization and sound velocity confirm the antiferromagnetic ordering transition, at the lowest temperature the field-dependent measurements reveal a sharp softening of sound velocity v (B ) and a clear minimum of temperature T (B ) at B⊥c,3 D=21.4 T , indicating the suppression of the antiferromagnetic order. At higher fields, the T (B ) curve shows a broad minimum at B⊥c=40 T , accompanied by a broad minimum in the sound velocity and a saturationlike magnetization. These features signal a quantum phase transition, which is further characterized by the divergent behavior of the Grüneisen parameter ΓB∝(B -B⊥c)-1. By contrast, around the critical field, the Grüneisen parameter converges as temperature decreases, pointing to a quantum critical point of the one-dimensional transverse-field Ising model.

  10. Photoinduced Coherent Spin Fluctuation in Primary Dynamics of Insulator to Metal Transition in Perovskite Cobalt Oxide

    Directory of Open Access Journals (Sweden)

    Arima T.

    2013-03-01

    Full Text Available Coherent spin fluctuation was detected in the photoinduced Mott insulator-metal transition in perovskite cobalt oxide by using 3 optical-cycle infrared pulse. Such coherent spin fluctuation is driven by the perovskite distortion changing orbital gap.

  11. Effect of spin fluctuations in magnetocaloric and magnetoresistance properties of Dy10Co20Si70 alloy

    Science.gov (United States)

    Rashid, T. P.; Arun, K.; Curlik, Ivan; Ilkovic, Sergej; Reiffers, Marian; Dzubinska, Andrea; Nagalakshmi, R.

    2017-09-01

    Systematic investigations on the structure, magnetic, thermodynamic, magnetocaloric and magnetoresistance (MR) properties of the arc melted Dy10Co20Si70 alloy are presented. The Dy10Co20Si70 alloy crystallizes in tetragonal BaNiSn3-type DyCoSi3 (space group = I4mm; No. 107) as a major phase and CaF2-type CoSi2 (space group = Fm-3m; No. 225) and C-type Si (space group = Fd-3m; No. 227) as minor phases. The title compound exhibits multiple magnetic transitions having antiferromagnetic ordering at temperatures, viz., T1 = 10.8 K, T2 = 8.8 K and T3 = 3.3 K. The magnetic and thermodynamic studies confirm these magnetic anomalies in the compound. The large value of maximum magnetic entropy change, -ΔSMM a x = 16.4 and 26.6 J/kg K for the field change ΔH of 50 and 90 kOe, respectively, observed in the compound is associated with field induced magnetic transitions. Asymmetric broadening of the magnetic entropy change peaks above the ordering temperatures resulting in significant refrigerant capacities of 361 and 868 J/kg for ΔH = 50 and 90 kOe, respectively, in the compound is due to the spin fluctuation effect. The sign reversal in MR measurements is attributed to the field induced antiferromagnetic to ferromagnetic transition. A large positive MR (42% in 90 kOe) is observed at 2 K. The H2 dependence of both the magnetocaloric effect (MCE) and MR in the paramagnetic regime indicates the role of the applied magnetic field in suppressing the spin fluctuations. The large MCE and MR together with no thermal or magnetic hysteresis establish this new compound as an attractive multifunctional magnetic material.

  12. Vertex functions at finite momentum: Application to antiferromagnetic quantum criticality

    Science.gov (United States)

    Wölfle, Peter; Abrahams, Elihu

    2016-02-01

    We analyze the three-point vertex function that describes the coupling of fermionic particle-hole pairs in a metal to spin or charge fluctuations at nonzero momentum. We consider Ward identities, which connect two-particle vertex functions to the self-energy, in the framework of a Hubbard model. These are derived using conservation laws following from local symmetries. The generators considered are the spin density and particle density. It is shown that at certain antiferromagnetic critical points, where the quasiparticle effective mass is diverging, the vertex function describing the coupling of particle-hole pairs to the spin density Fourier component at the antiferromagnetic wave vector is also divergent. Then we give an explicit calculation of the irreducible vertex function for the case of three-dimensional antiferromagnetic fluctuations, and show that it is proportional to the diverging quasiparticle effective mass.

  13. Novel spin excitation in the high field phase of an S=1 antiferromagnetic chain

    International Nuclear Information System (INIS)

    Hagiwara, M.; Kashiwagi, T.; Kimura, S.; Honda, Z.; Kindo, K.

    2007-01-01

    We report the results of high-field multi-frequency ESR experiment on the S=1 Heisenberg antiferromagnetic chain Ni(C 5 H 14 N 2 ) 2 N 3 (PF 6 ) for the fields up to about 55T and the frequencies up to about 2THz. We have found that excitation branches above the critical field (H c ) where the energy gap closes change into one branch around 15T which becomes close to the paramagnetic line at high fields. The branch above 15T fits well the conventional antiferromagnetic resonance mode with easy planar anisotropy. We compare the results with those in a weakly coupled antiferromagnetic dimer compound KCuCl 3 and discuss the origin of the branches observed above H c

  14. Perspectives of antiferromagnetic spintronics

    Energy Technology Data Exchange (ETDEWEB)

    Jungfleisch, Matthias B.; Zhang, Wei; Hoffmann, Axel

    2018-04-01

    Antiferromagnets are promising for future spintronics applications owing to their interesting properties: They are magnetically ordered, but neighboring magnetic moments point in opposite directions which results in zero net magneti- zation. This means antiferromagnets produce no stray fields and are insensitive to external magnetic field perturbations. Furthermore, they show intrinsic high frequency dynamics, exhibit considerable spin-orbit and magneto-transport effects. Over the past decade, it has been realized that antiferromagnets have more to offer than just being utilized as passive components in exchange bias applications. This development resulted in a paradigm shift, which opens the pathway to novel concepts using antiferromagnets for spin-based technologies and applications. This article gives a broad per- spective on antiferromagnetic spintronics. In particular, the manipulation and detection of anitferromagnetic states by spintronics effects, as well as spin transport and dynamics in antiferromagnetic materials will be discussed. We will also outline current challenges and future research directions in this emerging field.

  15. Model of ultrafast demagnetization driven by spin-orbit coupling in a photoexcited antiferromagnetic insulator Cr2O3

    Science.gov (United States)

    Guo, Feng; Zhang, Na; Jin, Wei; Chang, Jun

    2017-06-01

    We theoretically study the dynamic time evolution following laser pulse pumping in an antiferromagnetic insulator Cr2O3. From the photoexcited high-spin quartet states to the long-lived low-spin doublet states, the ultrafast demagnetization processes are investigated by solving the dissipative Schrödinger equation. We find that the demagnetization times are of the order of hundreds of femtoseconds, in good agreement with recent experiments. The switching times could be strongly reduced by properly tuning the energy gaps between the multiplet energy levels of Cr3+. Furthermore, the relaxation times also depend on the hybridization of atomic orbitals in the first photoexcited state. Our results suggest that the selective manipulation of the electronic structure by engineering stress-strain or chemical substitution allows effective control of the magnetic state switching in photoexcited insulating transition-metal oxides.

  16. Low temperature magnetic properties and spin dynamics in single crystals of Cr{sub 8}Zn antiferromagnetic molecular rings

    Energy Technology Data Exchange (ETDEWEB)

    Adelnia, Fatemeh [Dipartimento di Fisica, Università degli Studi di Milano and INSTM, I-20133 Milano (Italy); Dipartimento di Fisica, Università degli Studi di Pavia and INSTM, I-27100 Pavia (Italy); Chiesa, Alessandro; Bordignon, Sara; Carretta, Stefano [Dipartimento di Fisica e Scienze della Terra, Università degli Studi di Parma, I-43124 Parma (Italy); Ghirri, Alberto; Candini, Andrea [CNR Institute Nanosciences S3, I- 41125 Modena (Italy); Cervetti, Christian [Dipartimento di Scienze Fisiche, Informatiche, Matematiche, Università di Modena e Reggio Emilia, I-41125 Modena (Italy); Evangelisti, Marco [CNR Institute Nanosciences S3, I- 41125 Modena (Italy); Dipartimento di Scienze Fisiche, Informatiche, Matematiche, Università di Modena e Reggio Emilia, I-41125 Modena (Italy); Instituto de Ciencia de Materiales de Aragón and Departamento de Física de la Materia Condensada, CSIC-Universidad de Zaragoza, 50009 Zaragoza (Spain); Affronte, Marco [CNR Institute Nanosciences S3, I- 41125 Modena (Italy); Dipartimento di Scienze Fisiche, Informatiche, Matematiche, Università di Modena e Reggio Emilia, I-41125 Modena (Italy); Sheikin, Ilya [Grenoble High Magnetic Field Laboratory, CNRS-LNCMI, 25, B.P. 166, 38042 Grenoble Cedex 9 (France); Winpenny, Richard; Timco, Grigore [The Lewis Magnetism Laboratory, The University of Manchester, M13 9PL Manchester (United Kingdom); Borsa, Ferdinando [Dipartimento di Fisica, Università degli Studi di Pavia and INSTM, I-27100 Pavia (Italy); and others

    2015-12-28

    A detailed experimental investigation of the effects giving rise to the magnetic energy level structure in the vicinity of the level crossing (LC) at low temperature is reported for the open antiferromagnetic molecular ring Cr{sub 8}Zn. The study is conducted by means of thermodynamic techniques (torque magnetometry, magnetization and specific heat measurements) and microscopic techniques (nuclear magnetic resonance line width, nuclear spin lattice, and spin-spin relaxation measurements). The experimental results are shown to be in excellent agreement with theoretical calculations based on a minimal spin model Hamiltonian, which includes a Dzyaloshinskii-Moriya interaction. The first ground state level crossing at μ{sub 0}H{sub c1} = 2.15 T is found to be an almost true LC while the second LC at μ{sub 0}H{sub c2} = 6.95 T has an anti-crossing gap of Δ{sub 12} = 0.19 K. In addition, both NMR and specific heat measurements show the presence of a level anti-crossing between excited states at μ{sub 0}H = 4.5 T as predicted by the theory. In all cases, the fit of the experimental data is improved by introducing a distribution of the isotropic exchange couplings (J), i.e., using a J strain model. The peaks at the first and second LCs in the nuclear spin-lattice relaxation rate are dominated by inelastic scattering and a value of Γ ∼ 10{sup 10} rad/s is inferred for the life time broadening of the excited state of the open ring, due to spin phonon interaction. A loss of NMR signal (wipe-out effect) is observed for the first time at LC and is explained by the enhancement of the spin-spin relaxation rate due to the inelastic scattering.

  17. Single reference Coupled Cluster treatment of nearly degenerate problems: Cohesive energy of antiferromagnetic lattices of spin 1 centers

    International Nuclear Information System (INIS)

    Malrieu, Jean-Paul

    2012-01-01

    Lattices of antiferromagnetically coupled spins, ruled by Heisenberg Hamiltonians, are intrinsically highly degenerate systems. The present work tries to estimate the ground state energy of regular bipartite spin lattices of S = 1 sites from a single reference Coupled Cluster expansion starting from a Néel function, taken as reference. The simultaneous changes of spin momentum on adjacent sites play the role of the double excitations in molecular electronic problems. Propagation of the spin changes plays the same role as the triple excitations. The treatment takes care of the deviation of multiple excitation energies from additivity. Specific difficulties appear for 1D chains, which are not due to a near degeneracy between the reference and the vectors which directly interact with it but to the complexity of the processes which lead to the low energy configurations where a consistent reversed-Néel domain is created inside the Néel starting spin wave. Despite these difficulties a reasonable value of the cohesive energy is obtained.

  18. Single reference Coupled Cluster treatment of nearly degenerate problems: Cohesive energy of antiferromagnetic lattices of spin 1 centers

    Science.gov (United States)

    Malrieu, Jean-Paul

    2012-06-01

    Lattices of antiferromagnetically coupled spins, ruled by Heisenberg Hamiltonians, are intrinsically highly degenerate systems. The present work tries to estimate the ground state energy of regular bipartite spin lattices of S = 1 sites from a single reference Coupled Cluster expansion starting from a Néel function, taken as reference. The simultaneous changes of spin momentum on adjacent sites play the role of the double excitations in molecular electronic problems. Propagation of the spin changes plays the same role as the triple excitations. The treatment takes care of the deviation of multiple excitation energies from additivity. Specific difficulties appear for 1D chains, which are not due to a near degeneracy between the reference and the vectors which directly interact with it but to the complexity of the processes which lead to the low energy configurations where a consistent reversed-Néel domain is created inside the Néel starting spin wave. Despite these difficulties a reasonable value of the cohesive energy is obtained.

  19. Ground-state phases of the spin-1 J1-J2 Heisenberg antiferromagnet on the honeycomb lattice

    Science.gov (United States)

    Li, P. H. Y.; Bishop, R. F.

    2016-06-01

    We study the zero-temperature quantum phase diagram of a spin-1 Heisenberg antiferromagnet on the honeycomb lattice with both nearest-neighbor exchange coupling J1>0 and frustrating next-nearest-neighbor coupling J2≡κ J1>0 , using the coupled cluster method implemented to high orders of approximation, and based on model states with different forms of classical magnetic order. For each we calculate directly in the bulk thermodynamic limit both ground-state low-energy parameters (including the energy per spin, magnetic order parameter, spin stiffness coefficient, and zero-field uniform transverse magnetic susceptibility) and their generalized susceptibilities to various forms of valence-bond crystalline (VBC) order, as well as the energy gap to the lowest-lying spin-triplet excitation. In the range 0 κc 2=0.340 (5 ) . Two different paramagnetic phases are found to exist in the intermediate region. Over the range κc1<κ<κci=0.305 (5 ) we find a gapless phase with no discernible magnetic order, which is a strong candidate for being a quantum spin liquid, while over the range κci<κ <κc 2 we find a gapped phase, which is most likely a lattice nematic with staggered dimer VBC order that breaks the lattice rotational symmetry.

  20. Spin canting in a Dy-based single-chain magnet with dominant next-nearest-neighbor antiferromagnetic interactions

    Science.gov (United States)

    Bernot, K.; Luzon, J.; Caneschi, A.; Gatteschi, D.; Sessoli, R.; Bogani, L.; Vindigni, A.; Rettori, A.; Pini, M. G.

    2009-04-01

    We investigate theoretically and experimentally the static magnetic properties of single crystals of the molecular-based single-chain magnet of formula [Dy(hfac)3NIT(C6H4OPh)]∞ comprising alternating Dy3+ and organic radicals. The magnetic molar susceptibility χM displays a strong angular variation for sample rotations around two directions perpendicular to the chain axis. A peculiar inversion between maxima and minima in the angular dependence of χM occurs on increasing temperature. Using information regarding the monomeric building block as well as an ab initio estimation of the magnetic anisotropy of the Dy3+ ion, this “anisotropy-inversion” phenomenon can be assigned to weak one-dimensional ferromagnetism along the chain axis. This indicates that antiferromagnetic next-nearest-neighbor interactions between Dy3+ ions dominate, despite the large Dy-Dy separation, over the nearest-neighbor interactions between the radicals and the Dy3+ ions. Measurements of the field dependence of the magnetization, both along and perpendicularly to the chain, and of the angular dependence of χM in a strong magnetic field confirm such an interpretation. Transfer-matrix simulations of the experimental measurements are performed using a classical one-dimensional spin model with antiferromagnetic Heisenberg exchange interaction and noncollinear uniaxial single-ion anisotropies favoring a canted antiferromagnetic spin arrangement, with a net magnetic moment along the chain axis. The fine agreement obtained with experimental data provides estimates of the Hamiltonian parameters, essential for further study of the dynamics of rare-earth-based molecular chains.

  1. Investigation of the spin-1 honeycomb antiferromagnet BaNi2V2O8 with easy-plane anisotropy

    Science.gov (United States)

    Klyushina, E. S.; Lake, B.; Islam, A. T. M. N.; Park, J. T.; Schneidewind, A.; Guidi, T.; Goremychkin, E. A.; Klemke, B.; Mânsson, M.

    2017-12-01

    The magnetic properties of the two-dimensional, S =1 honeycomb antiferromagnet BaNi2V2O8 have been comprehensively studied using dc susceptibility measurements and inelastic neutron scattering techniques. The magnetic excitation spectrum is found to be dispersionless within experimental resolution between the honeycomb layers, while it disperses strongly within the honeycomb plane where it consists of two gapped spin-wave modes. The magnetic excitations are compared to linear spin-wave theory allowing the Hamiltonian to be determined. The first- and second-neighbor magnetic exchange interactions are antiferromagnetic and lie within the ranges 10.90 meV ≤Jn≤13.35 meV and 0.85 meV ≤Jn n≤1.65 meV, respectively. The interplane coupling Jout is four orders of magnitude weaker than the intraplane interactions, confirming the highly two-dimensional magnetic behavior of this compound. The sizes of the energy gaps are used to extract the magnetic anisotropies and reveal substantial easy-plane anisotropy and a very weak in-plane easy-axis anisotropy. Together these results reveal that BaNi2V2O8 is a candidate compound for the investigation of vortex excitations and Berezinsky-Kosterliz-Thouless phenomenon.

  2. Influence of longitudinal spin fluctuations on the phase transition features in chiral magnets

    Science.gov (United States)

    Belemuk, A. M.; Stishov, S. M.

    2018-04-01

    Using the classical Monte Carlo calculations, we investigate the effects of longitudinal spin fluctuations on the helimagnetic transition in a Heisenberg magnet with the Dzyaloshinskii-Moriya interaction. We use variable spin amplitudes in the framework of the spin-lattice Hamiltonian. It is this kind of fluctuations that naturally occur in an itinerant system. We show that the basic features of the helical phase transition are not changed much by the longitudinal spin fluctuations though the transition temperature Tc and the fluctuation hump seen in specific heat at T >Tc is significantly affected. We report thermodynamic and structural effects of these fluctuations. By increasing the system size in the Monte Carlo modeling, we are able to reproduce the ring shape scattering intensity above the helimagnetic transition temperature Tc, which transforms into the spiral spots seen below Tc in the neutron scattering experiments.

  3. Fractional Spin Fluctuations as a Precursor of Quantum Spin Liquids: Majorana Dynamical Mean-Field Study for the Kitaev Model.

    Science.gov (United States)

    Yoshitake, Junki; Nasu, Joji; Motome, Yukitoshi

    2016-10-07

    Experimental identification of quantum spin liquids remains a challenge, as the pristine nature is to be seen in asymptotically low temperatures. We here theoretically show that the precursor of quantum spin liquids appears in the spin dynamics in the paramagnetic state over a wide temperature range. Using the cluster dynamical mean-field theory and the continuous-time quantum Monte Carlo method, which are newly developed in the Majorana fermion representation, we calculate the dynamical spin structure factor, relaxation rate in nuclear magnetic resonance, and magnetic susceptibility for the honeycomb Kitaev model whose ground state is a canonical example of the quantum spin liquid. We find that dynamical spin correlations show peculiar temperature and frequency dependence even below the temperature where static correlations saturate. The results provide the experimentally accessible symptoms of the fluctuating fractionalized spins evincing the quantum spin liquids.

  4. Hanle effect in (In,Ga)As quantum dots: Role of nuclear spin fluctuations

    OpenAIRE

    Kuznetsova, M. S.; Flisinski, K.; Gerlovin, I. Ya.; Ignatiev, I. V.; Kavokin, K. V.; Verbin, S. Yu.; Yakovlev, D. R.; Reuter, D.; Wieck, A. D.; Bayer, M.

    2013-01-01

    The role of nuclear spin fluctuations in the dynamic polarization of nuclear spins by electrons is investigated in (In,Ga)As quantum dots. The photoluminescence polarization under circularly polarized optical pumping in transverse magnetic fields (Hanle effect) is studied. A weak additional magnetic field parallel to the optical axis is used to control the efficiency of nuclear spin cooling and the sign of nuclear spin temperature. The shape of the Hanle curve is drastically modified with cha...

  5. Density of states and phase diagram of the antiferromagnetic spin chain with Dzyaloshinsky-Moriya interaction and spin-phonon coupling

    International Nuclear Information System (INIS)

    Wang Qin; Chen Hong; Zheng Hang

    2007-01-01

    The effects of DM interaction on the density-of-states, the dimerization and the phase diagram in the antiferromagnetic Heisenberg chain coupled with quantum phonons have been studied by a nonadiabatic analytical approach. The results show that the effect of the DM interaction is to increase the staggered antisymmetric spin exchange interaction order but to decrease the spin dimerization and their competitions result in the lattice dimerization ordering parameter to increase for large staggered DM interaction parameter β and decrease for small β. A crossover of β exists in which the dimerization ordering parameter changes non-monotonously. As the DM interaction parameter D increases, depending on the appropriate values of spin-phonon coupling, phonon frequency and β, the system undergoes phase transition from spin gapless state to gapped state or reversely and can even reenter between the two states. The relation between the phonon-staggered ordering parameter, the spin-dimer order parameter and the staggered DM interaction order parameter gives clearly their contributing weights to the lattice dimerization

  6. Gapped paramagnetic state in a frustrated spin-1/2 Heisenberg antiferromagnet on the cross-striped square lattice

    Science.gov (United States)

    Li, P. H. Y.; Bishop, R. F.

    2018-03-01

    We implement the coupled cluster method to very high orders of approximation to study the spin-1/2 J1 -J2 Heisenberg model on a cross-striped square lattice. Every nearest-neighbour pair of sites on the square lattice has an isotropic antiferromagnetic exchange bond of strength J1 > 0 , while the basic square plaquettes in alternate columns have either both or neither next-nearest-neighbour (diagonal) pairs of sites connected by an equivalent frustrating bond of strength J2 ≡ αJ1 > 0 . By studying the magnetic order parameter (i.e., the average local on-site magnetization) in the range 0 ≤ α ≤ 1 of the frustration parameter we find that the quasiclassical antiferromagnetic Néel and (so-called) double Néel states form the stable ground-state phases in the respective regions α α1bc = 0.615(5) . The double Néel state has Néel (⋯ ↑↓↑↓ ⋯) ordering along the (column) direction parallel to the stripes of squares with both or no J2 bonds, and spins alternating in a pairwise (⋯ ↑↑↓↓↑↑↓↓ ⋯) fashion along the perpendicular (row) direction, so that the parallel pairs occur on squares with both J2 bonds present. Further explicit calculations of both the triplet spin gap and the zero-field uniform transverse magnetic susceptibility provide compelling evidence that the ground-state phase over all or most of the intermediate regime α1ac < α < α1bc is a gapped state with no discernible long-range magnetic order.

  7. Superconductivity, Antiferromagnetism, and Kinetic Correlation in Strongly Correlated Electron Systems

    Directory of Open Access Journals (Sweden)

    Takashi Yanagisawa

    2015-01-01

    Full Text Available We investigate the ground state of two-dimensional Hubbard model on the basis of the variational Monte Carlo method. We use wave functions that include kinetic correlation and doublon-holon correlation beyond the Gutzwiller ansatz. It is still not clear whether the Hubbard model accounts for high-temperature superconductivity. The antiferromagnetic correlation plays a key role in the study of pairing mechanism because the superconductive phase exists usually close to the antiferromagnetic phase. We investigate the stability of the antiferromagnetic state when holes are doped as a function of the Coulomb repulsion U. We show that the antiferromagnetic correlation is suppressed as U is increased exceeding the bandwidth. High-temperature superconductivity is possible in this region with enhanced antiferromagnetic spin fluctuation and pairing interaction.

  8. Theory of antiferromagnetic pairing in cuprate superconductors

    International Nuclear Information System (INIS)

    Plakida, N.M.

    2006-01-01

    A review of the antiferromagnetic exchange and spin-fluctuation pairing theory in the cuprate superconductors is given. We briefly discuss a phenomenological approach and a theory in the limit of weak Coulomb correlations. A microscopic theory in the strong correlation limit is presented in more detail. In particular, results of our recently developed theory for the effective p-d Hubbard model and the reduced t-J model are given. We have proved that retardation effects for the antiferromagnetic exchange interaction are unimportant that results in pairing of all charge carriers in the conduction band and high Tc proportional to the Fermi energy. The spin-fluctuation interaction caused by kinematic interaction gives an additional contribution to the d-wave pairing. Dependence of Tc on the hole concentration and the lattice constant (or pressure) and an oxygen isotope shift are discussed

  9. Control of antiferromagnetic spin axis orientation in bilayer Fe/CuMnAs films

    Czech Academy of Sciences Publication Activity Database

    Wadley, P.; Edmonds, K. W.; Shahedkhah, M.R.; Campion, R. P.; Gallagher, B. L.; Železný, Jakub; Kuneš, Jan; Novák, Vít; Jungwirth, Tomáš; Saidl, Vít; Němec, P.; Maccherozzi, F.; Dhesi, S.S.

    2017-01-01

    Roč. 7, Sep (2017), 1-6, č. článku 11147. ISSN 2045-2322 R&D Projects: GA MŠk LM2015087; GA ČR GB14-37427G Institutional support: RVO:68378271 Keywords : antiferromagnetic spintronics * exchange coupling Subject RIV: BM - Solid Matter Physics ; Magnetism OBOR OECD: Condensed matter physics (including formerly solid state physics, supercond.) Impact factor: 4.259, year: 2016

  10. High antiferromagnetic domain wall velocity induced by Néel spin-orbit torques

    Czech Academy of Sciences Publication Activity Database

    Gomonay, O.; Jungwirth, Tomáš; Sinova, Jairo

    2016-01-01

    Roč. 117, č. 1 (2016), 1-5, č. článku 017202. ISSN 0031-9007 R&D Projects: GA MŠk(CZ) LM2011026; GA ČR GB14-37427G EU Projects: European Commission(XE) 268066 - 0MSPIN Institutional support: RVO:68378271 Keywords : spintronics * domain walls * antiferromagnets Subject RIV: BM - Solid Matter Physics ; Magnetism Impact factor: 8.462, year: 2016

  11. Role of quantum fluctuations on spin liquids and ordered phases in the Heisenberg model on the honeycomb lattice

    Science.gov (United States)

    Merino, Jaime; Ralko, Arnaud

    2018-05-01

    Motivated by the rich physics of honeycomb magnetic materials, we obtain the phase diagram and analyze magnetic properties of the spin-1 /2 and spin-1 J1-J2-J3 Heisenberg model on the honeycomb lattice. Based on the SU(2) and SU(3) symmetry representations of the Schwinger boson approach, which treats disordered spin liquids and magnetically ordered phases on an equal footing, we obtain the complete phase diagrams in the (J2,J3) plane. This is achieved using a fully unrestricted approach which does not assume any pre-defined Ansätze. For S =1 /2 , we find a quantum spin liquid (QSL) stabilized between the Néel, spiral, and collinear antiferromagnetic phases in agreement with previous theoretical work. However, by increasing S from 1 /2 to 1, the QSL is quickly destroyed due to the weakening of quantum fluctuations indicating that the model already behaves as a quasiclassical system. The dynamical structure factors and temperature dependence of the magnetic susceptibility are obtained in order to characterize all phases in the phase diagrams. Moreover, motivated by the relevance of the single-ion anisotropy, D , to various S =1 honeycomb compounds, we have analyzed the destruction of magnetic order based on an SU(3) representation of the Schwinger bosons. Our analysis provides a unified understanding of the magnetic properties of honeycomb materials realizing the J1-J2-J3 Heisenberg model from the strong quantum spin regime at S =1 /2 to the S =1 case. Neutron scattering and magnetic susceptibility experiments can be used to test the destruction of the QSL phase when replacing S =1 /2 by S =1 localized moments in certain honeycomb compounds.

  12. High-field spin dynamics of the one-dimensional spin-1/2 Heisenberg antiferromagnetα-bis (N-methylsalicylaldiminato copper) (II) (α-CuNSal)

    International Nuclear Information System (INIS)

    Azevedo, L.J.; Narath, A.; Richards, P.M.; Soos, Z.G.

    1980-01-01

    Proton spin-lattice relaxation rates in the one-dimensional (1D) spin-1/2 Heisenberg antiferromagnet α-bis (N-methylsalicylaldiminato) copper (II), α-CuNSal, have been measured in applied fields up to 125 kOe in the temperature range 1-- 4 K. The strong coupling of protons close to the antiferromagnetic (AF) chain serves as a convenient probe to study the dynamics of the AF chain through the field-induced antiferromagnetic to ferromagnetic (F) phase transition. The magnetization of the AF chain, as measured by the proton field shift, is in close agreement with calculations by Bonner and Fisher and yields an exchange interaction J/k/sub B/=3.04 +- 0.04 K. The proton relaxation rate has isotropic (hyperfine coupled) and anisotropic (dipolar) components. We identify the isotropic relaxation rate with a creation or destruction of one-spin excitations (magnons) and the anisotropic rate with two-magnon processes. The measured one-magnon relaxation rate shows an enhancement near the critical field for the AF → F transition and a strong decrease of more than four decades as the critical field is exceeded. A no-adjustable-parameter calculation based on the fermion model quantitatively agrees with the measured one-magnon relaxation rate, both above and below the critical field H/sub c/. The enhanced relaxation at H/sub c/ is correctly predicted as a consequence of the divergence of the 1D density of magnon states, where a gap in the spin-wave spectrum exists. Above H/sub c/ a finite magnon lifetime must be included in order to produce a nonzero one-magnon relaxation rate. This is also calculated with no adjustable parameters. The two-magnon relaxation rate also shows a decrease as the critical field is exceeded and the calculated relaxation rate agrees well with experiment at low temperatures, provided, however, that one uses a boson rather than fermion picture

  13. Characterisation of spin-waves in copper(II) deuteroformate tetradeuterate: A square ¤S¤=1/2 Heisenberg antiferromagnet

    DEFF Research Database (Denmark)

    Clarke, S.J.; Harrison, A.; Mason, T.E.

    1999-01-01

    Copper(II) formate tetrahydrate (CFTH) is a model square S = 1/2 Heisenberg antiferromagnet with T-N = 16.54 +/- 0.05 K. The dispersion of spin-waves in the magnetic layers of a fully deuterated sample of this material has been mapped at 4.3 K by inelastic neutron scattering from the zone centre ...

  14. Exchange and spin-fluctuation superconducting pairing in the strong correlation limit of the Hubbard model

    International Nuclear Information System (INIS)

    Plakida, N. M.; Anton, L.; Adam, S. . Department of Theoretical Physics, Horia Hulubei National Institute for Physics and Nuclear Engineering, PO Box MG-6, RO-76900 Bucharest - Magurele; RO); Adam, Gh. . Department of Theoretical Physics, Horia Hulubei National Institute for Physics and Nuclear Engineering, PO Box MG-6, RO-76900 Bucharest - Magurele; RO)

    2001-01-01

    contrast, the exchange interaction is maximal along the above mentioned lines inside BZ and it couples the electrons (holes) in a much broader energy shell, of the order of the bandwidth W= 8 t eff due to the interband hopping where the retardation effects are unimportant. Samplings of the wave-vector behavior of the order parameters Φ 22 (k) over the first quadrant of the BZ at several temperatures show the occurrence of a peculiar d x 2 -y 2 -wave gap pattern which strongly depends on the type of the involved interactions. In conclusion, the present investigation points to the existence of a singlet d x 2 -y 2 -wave superconducting pairing for holes or electrons in the two-band Hubbard model mediated by the exchange interaction and antiferromagnetic spin-fluctuation scattering induced by the kinematic interaction, characteristic to the Hubbard model. These mechanisms of superconducting pairing are absent in the fermionic models. Our results agree with the recent investigations of the Hubbard model within the dynamical cluster approximation, where the self-energy has been calculated in the non-crossing approximation for the 4-cluster model. (authors)

  15. Fullerene/layered antiferromagnetic reconstructed spinterface: Subsurface layer dominates molecular orbitals' spin-split and large induced magnetic moment

    Science.gov (United States)

    Shao, Yangfan; Pang, Rui; Pan, Hui; Shi, Xingqiang

    2018-03-01

    The interfaces between organic molecules and magnetic metals have gained increasing interest for both fundamental reasons and applications. Among them, the C60/layered antiferromagnetic (AFM) interfaces have been studied only for C60 bonded to the outermost ferromagnetic layer [S. L. Kawahara et al., Nano Lett. 12, 4558 (2012) and D. Li et al., Phys. Rev. B 93, 085425 (2016)]. Here, via density functional theory calculations combined with evidence from the literature, we demonstrate that C60 adsorption can reconstruct the layered-AFM Cr(001) surface at elevated annealing temperatures so that C60 bonds to both the outermost and the subsurface Cr layers in opposite spin directions. Surface reconstruction drastically changes the adsorbed molecule spintronic properties: (1) the spin-split p-d hybridization involves multi-orbitals of C60 and top two layers of Cr with opposite spin-polarization, (2) the subsurface Cr atom dominates the C60 electronic properties, and (3) the reconstruction induces a large magnetic moment of 0.58 μB in C60 as a synergistic effect of the top two Cr layers. The induced magnetic moment in C60 can be explained by the magnetic direct-exchange mechanism, which can be generalized to other C60/magnetic metal systems. Understanding these complex hybridization behaviors is a crucial step for molecular spintronic applications.

  16. Writing and reading antiferromagnetic Mn2Au by Néel spin-orbit torques and large anisotropic magnetoresistance.

    Science.gov (United States)

    Bodnar, S Yu; Šmejkal, L; Turek, I; Jungwirth, T; Gomonay, O; Sinova, J; Sapozhnik, A A; Elmers, H-J; Kläui, M; Jourdan, M

    2018-01-24

    Using antiferromagnets as active elements in spintronics requires the ability to manipulate and read-out the Néel vector orientation. Here we demonstrate for Mn 2 Au, a good conductor with a high ordering temperature suitable for applications, reproducible switching using current pulse generated bulk spin-orbit torques and read-out by magnetoresistance measurements. Reversible and consistent changes of the longitudinal resistance and planar Hall voltage of star-patterned epitaxial Mn 2 Au(001) thin films were generated by pulse current densities of ≃10 7  A/cm 2 . The symmetry of the torques agrees with theoretical predictions and a large read-out magnetoresistance effect of more than ≃6% is reproduced by ab initio transport calculations.

  17. Spin-density correlations in the dynamic spin-fluctuation theory: Comparison with polarized neutron scattering experiments

    Energy Technology Data Exchange (ETDEWEB)

    Melnikov, N.B., E-mail: melnikov@cs.msu.su [Lomonosov Moscow State University, Moscow 119991 (Russian Federation); Reser, B.I., E-mail: reser@imp.uran.ru [Miheev Institute of Metal Physics, Ural Branch of Russian Academy of Sciences, Ekaterinburg 620990 (Russian Federation); Paradezhenko, G.V., E-mail: gparadezhenko@cs.msu.su [Lomonosov Moscow State University, Moscow 119991 (Russian Federation)

    2016-08-01

    To study the spin-density correlations in the ferromagnetic metals above the Curie temperature, we relate the spin correlator and neutron scattering cross-section. In the dynamic spin-fluctuation theory, we obtain explicit expressions for the effective and local magnetic moments and spatial spin-density correlator. Our theoretical results are demonstrated by the example of bcc Fe. The effective and local moments are found in good agreement with results of polarized neutron scattering experiment over a wide temperature range. The calculated short-range order is small (up to 4 Å) and slowly decreases with temperature.

  18. Exact ground and excited states of an antiferromagnetic quantum spin model

    International Nuclear Information System (INIS)

    Bose, I.

    1989-08-01

    A quasi-one-dimensional spin model which consists of a chain of octahedra of spins has been suggested for which a certain parameter regime of the Hamiltonian, the ground state, can be written down exactly. The ground state is highly degenerate and can be other than a singlet. Also, several excited states can be constructed exactly. The ground state is a local RVB state for which resonance is confined to rings of spins. Some exact numerical results for an octahedron of spins have also been reported. (author). 16 refs, 2 figs, 1 tab

  19. Disorder effects in the S=1 antiferromagnetic spin ladder CaV{sub 2}O{sub 4}

    Energy Technology Data Exchange (ETDEWEB)

    Guitarra, S.R. [Colegio de Ciencias e Ingeniería, Universidad San Francisco de Quito, Quito (Ecuador); Caneiro, A. [Instituto Balseiro - Centro Atómico Bariloche, 8400 Bariloche (Argentina); Niebieskikwiat, D., E-mail: dniebieskikwiat@usfq.edu.ec [Colegio de Ciencias e Ingeniería, Universidad San Francisco de Quito, Quito (Ecuador)

    2015-10-15

    We study the physical properties of the antiferromagnetic spin ladder CaV{sub 2}O{sub 4} (CVO) and the Y-doped related compound Ca{sub 0.9}Y{sub 0.1}V{sub 2}O{sub 4}. In the latter, X-ray diffraction demonstrates the segregation of a small amount of a vanadium–perovskite impurity phase, leading to the formation of V vacancies within the main CVO-type structure. The 1D character of this calcium–vanadite enhances the influence of the vacancies on the electric and magnetic properties of Ca{sub 0.9}Y{sub 0.1}V{sub 2}O{sub 4}. Electrical transport is characterized by a variable-range hopping mechanism determined by the charging energy of nm-sized segments of V chains delimited by V vacancies, i.e. a Coulomb gap is formed at the Fermi level. These vacancies also locally affect the magnetic correlations, breaking the long-range AFM order observed in CaV{sub 2}O{sub 4} and producing exchange bias when the Y-doped sample is cooled with an applied magnetic field. - Highlights: • We study disorder effects in the quasi-1D antiferromagnetic spin ladder CaV{sub 2}O{sub 4}. • V vacancies in CaV{sub 2}O{sub 4} lead to variable-range hopping electrical transport. • The charging energy of nm-sized V chains determine the transport mechanism exponents. • V vacancies break the long-range AFM order of CaV{sub 2}O{sub 4}. • Local magnetic correlations in the vicinity of the defects produce exchange bias.

  20. Single-site approximation for the s-f model of antiferromagnetic semiconductors

    International Nuclear Information System (INIS)

    Takahashi, Masao; Nolting, Wolfgang

    2001-01-01

    For the s-f model of an antiferromagnetic semiconductor, the effect of the antiferromagnetic ordering of the localized spins on the conduction-electron state is investigated over a wide range of exchange strengths by combining the effective-medium approach with the Green's function in the 2x2 sublattice Bloch function representation. The band splitting due to the reduced magnetic Brillouin zone occurs below the Neel temperature. There is a marked effect of the thermal fluctuation of the antiferromagnetically ordered localized spins on the conduction electron at the energies near the top (bottom) of the lower- (higher-) energy subband

  1. Suppression of spin fluctuations in TiBe2 by high magnetic fields

    International Nuclear Information System (INIS)

    Stewart, G.R.; Smith, J.L.; Brandt, B.L.

    1982-01-01

    Measurement of the low-temperature specific heat of a well-characterized 15.6-mg sample of TiBe 2 was performed in magnetic fields of 0, 6.5, 11.4, 14.2, and 17.0 T. The results indicate a striking depression of the spin-fluctuation-caused upturn with increasing field in the lower-temperature specific heat and very little change at higher temperatures where the spin fluctuations are less predominant. A field for full suppression of the spin fluctuations is extrapolated to be above about 25 T. The field at which the onset of spin-fluctuation depression occurs is 5.2 +- 0.3 T, suggesting that the previously observed anomalies in the susceptibility and differential susceptibility of TiBe 2 at 5.5 T are connected to the onset of the depression of spin fluctuations. Furthermore, this onset of spin-fluctuation depression at 5.2 +- 0.3 T coupled with the extrapolation to full suppression above 25 T serves to unify the interpretations of previous data on TiBe 2 by Wohlfarth, by Acker et al., and by van Deursen et al. which were previously thought to be in contradiction

  2. Electronic structure and quantum spin fluctuations at the magnetic phase transition in MnSi

    Science.gov (United States)

    Povzner, A. A.; Volkov, A. G.; Nogovitsyna, T. A.

    2018-05-01

    The effect of spin fluctuations on the heat capacity and homogeneous magnetic susceptibility of the chiral magnetic MnSi in the vicinity of magnetic transition has been investigated by using the free energy functional of the coupled electron and spin subsystems and taking into account the Dzyaloshinsky-Moriya interaction. For helical ferromagnetic ordering, we found that zero-point fluctuations of the spin density are large and comparable with fluctuations of the non-uniform magnetization. The amplitude of zero-point spin fluctuations shows a sharp decrease in the region of the magnetic phase transition. It is shown that sharp decrease of the amplitude of the quantum spin fluctuations results in the lambda-like maxima of the heat capacity and the homogeneous magnetic susceptibility. Above the temperature of the lambda anomaly, the spin correlation radius becomes less than the period of the helical structure and chiral fluctuations of the local magnetization appear. It is shown that formation of a "shoulder" on the temperature dependence of the heat capacity is due to disappearance of the local magnetization. Our finding allows to explain the experimentally observed features of the magnetic phase transition of MnSi as a result of the crossover of quantum and thermodynamic phase transitions.

  3. Spin gap and antiferromagnetic correlations in the kondo insulator CeNiSn

    DEFF Research Database (Denmark)

    Mason, T.E.; Aeppli, G.; Ramirez, A.P.

    1992-01-01

    Neutron scattering measurements show that the crossover (at T less than or similar to 10 K) from metallic heavy-fermion to semiconducting behavior coincides with the formation of a gap in the magnetic excitation spectrum of CeNiSn. In contrast to the simple band picture of an insulator, the gap...... is well defined only at particular values of the momentum transfer Q. While substantial antiferromagnetic correlations in the a-c plane characterize the low-T state, the corresponding zero-frequency response function is Q independent....

  4. Spin-orbit torques in locally and globally noncentrosymmetric crystals: antiferromagnets and ferromagnets

    Czech Academy of Sciences Publication Activity Database

    Železný, Jakub; Gao, H.; Manchon, A.; Freimuth, F.; Mokrousov, Y.; Zemen, J.; Mašek, Jan; Sinova, Jairo; Jungwirth, Tomáš

    2017-01-01

    Roč. 95, č. 1 (2017), 1-18, č. článku 014403. ISSN 2469-9950 R&D Projects: GA MŠk LM2015087; GA ČR GB14-37427G; GA MŠk(CZ) LM2011026 EU Projects: European Commission(XE) 268066 - 0MSPIN Institutional support: RVO:68378271 Keywords : spintronics * antiferromagnets Subject RIV: BM - Solid Matter Physics ; Magnetism OBOR OECD: Condensed matter physics (including formerly solid state physics, supercond.) Impact factor: 3.836, year: 2016

  5. Electric control of Dirac quasiparticles by spin-orbit torque in an antiferromagnet

    Czech Academy of Sciences Publication Activity Database

    Šmejkal, Libor; Železný, Jakub; Sinova, Jairo; Jungwirth, Tomáš

    2017-01-01

    Roč. 118, č. 10 (2017), 1-5, č. článku 106402. ISSN 0031-9007 R&D Projects: GA MŠk LM2015087; GA ČR GB14-37427G EU Projects: European Commission(XE) 610115 - SC2 Institutional support: RVO:68378271 Keywords : spintronics * topological Dirac fermions * antiferromagnets Subject RIV: BM - Solid Matter Physics ; Magnetism OBOR OECD: Condensed matter physics (including formerly solid state physics, supercond.) Impact factor: 8.462, year: 2016

  6. Proposal for quantum gates in permanently coupled antiferromagnetic spin rings without need of local fields.

    Science.gov (United States)

    Troiani, Filippo; Affronte, Marco; Carretta, Stefano; Santini, Paolo; Amoretti, Giuseppe

    2005-05-20

    We propose a scheme for the implementation of quantum gates which is based on the qubit encoding in antiferromagnetic molecular rings. We show that a proper engineering of the intercluster link would result in an effective coupling that vanishes as far as the system is kept in the computational space, while it is turned on by a selective excitation of specific auxiliary states. These are also shown to allow the performing of single-qubit and two-qubit gates without an individual addressing of the rings by means of local magnetic fields.

  7. Spin fluctuations in iron based superconductors probed by NMR relaxation rate

    Energy Technology Data Exchange (ETDEWEB)

    Graefe, Uwe; Kuehne, Tim; Wurmehl, Sabine; Buechner, Bernd; Grafe, Hans-Joachim [IFW Dresden, Institute for Solid State Research, PF 270116, 01171 Dresden (Germany); Hammerath, Franziska [IFW Dresden, Institute for Solid State Research, PF 270116, 01171 Dresden (Germany); Department of Physics ' ' A. Volta' ' , University of Pavia-CNISM, I-27100 Pavia (Italy); Lang, Guillaume [3LPEM-UPR5, CNRS, ESPCI Paris Tech, 10 Rue Vauquelin, 75005 Paris (France)

    2013-07-01

    We present {sup 75}As nuclear magnetic resonance (NMR) results in F doped LaOFeAs iron pnictides. In the underdoped superconducting samples, pronounced spin fluctuations lead to a peak in the NMR spin lattice relaxation rate, (T{sub 1}T){sup -1}. The peak shows a typical field dependence that indicates a critical slowing of spin fluctuations: it is reduced in height and shifted to higher temperatures. In contrast, a similar peak in the underdoped magnetic samples at the ordering temperature of the spin density wave does not show such a field dependence. Furthermore, the peak is absent in optimally and overdoped samples, suggesting the absence of strong spin fluctuations. Our results indicate a glassy magnetic ordering in the underdoped samples that is in contrast to the often reported Curie Weiss like increase of spin fluctuations towards T{sub c}. Additional measurements of the linewidth and the spin spin relaxation rate are in agreement with such a glassy magnetic ordering that is most likely competing with superconductivity. Our results will be compared to Co doped BaFe{sub 2}As{sub 2}, where a similar peak in (T{sub 1}T){sup -1} has been observed.

  8. Influence of quantum phase transition on spin transport in the quantum antiferromagnet in the honeycomb lattice

    Science.gov (United States)

    Lima, L. S.

    2017-06-01

    We use the SU(3) Schwinger boson theory to study the spin transport properties of the two-dimensional anisotropic frustrated Heisenberg model in a honeycomb lattice at T = 0 with single ion anisotropy and third neighbor interactions. We have investigated the behavior of the spin conductivity for this model that presents exchange interactions J1 , J2 and J3 . We study the spin transport in the Bose-Einstein condensation regime where the bosons tz are condensed. Our results show an influence of the quantum phase transition point on the spin conductivity behavior. We also have made a diagrammatic expansion for the Green-function and did not obtain any significant change of the results.

  9. Phase diagrams of antiferromagnetic spin-1 bosons on a square optical lattice with the quadratic Zeeman effect

    Science.gov (United States)

    de Forges de Parny, L.; Rousseau, V. G.

    2018-02-01

    We study the quadratic Zeeman effect (QZE) in a system of antiferromagnetic spin-1 bosons on a square lattice and derive the ground-state phase diagrams by means of quantum Monte Carlo simulations and mean-field treatment. The QZE imbalances the populations of the magnetic sublevels σ =±1 and σ =0 , and therefore affects the magnetic and mobility properties of the phases. Both methods show that the tip of the even Mott lobes, stabilized by singlet state, is destroyed when turning on the QZE, thus leaving the space to the superfluid phase. Contrariwise, the tips of odd Mott lobes remain unaffected. Therefore, the Mott-superfluid transition with even filling strongly depends on the strength of the QZE, and we show that the QZE can act as a control parameter for this transition at fixed hopping. Using quantum Monte Carlo simulations, we elucidate the nature of the phase transitions and examine in detail the nematic order: the first-order Mott-superfluid transition with even filling observed in the absence of QZE becomes second order for weak QZE, in contradistinction to our mean-field results which predict a first-order transition in a larger range of QZE. Furthermore, a spin nematic order with director along the z axis is found in the odd Mott lobes and in the superfluid phase for energetically favored σ =±1 states. In the superfluid phase with even filling, the x y components of the nematic director remain finite only for moderate QZE.

  10. Effect of spin fluctuations on the electronic structure in iron-based superconductors

    Science.gov (United States)

    Heimes, Andreas; Grein, Roland; Eschrig, Matthias

    2012-08-01

    Magnetic inelastic neutron scattering studies of iron-based superconductors reveal a strongly temperature-dependent spin-fluctuation spectrum in the normal conducting state, which develops a prominent low-energy resonance feature when entering the superconducting state. Angle-resolved photoemission spectroscopy (ARPES) and scanning tunneling spectroscopy (STS) allow us to study the fingerprints of fluctuation modes via their interactions with electronic quasiparticles. We calculate such fingerprints in 122 iron pnictides using an experimentally motivated spin-fluctuation spectrum and make a number of predictions that can be tested in ARPES and STS experiments. This includes discussions of the quasiparticle scattering rate and the superconducting order parameter. In quantitative agreement with experiment we reproduce the quasiparticle dispersions obtained from momentum distribution curves as well as energy distribution curves. We discuss the relevance of the coupling between spin fluctuations and electronic excitations for the superconducting mechanism.

  11. Dependence of Tc on the q -ω structure of the spin-fluctuation spectrum

    Science.gov (United States)

    Dahm, Thomas; Scalapino, D. J.

    2018-05-01

    A phenomenological spin-fluctuation analysis [Dahm et al., Nat. Phys. 5, 217 (2009), 10.1038/nphys1180], based upon inelastic neutron scattering (INS) and angular resolved photoemission spectroscopy (ARPES) data for YBCO6.6(Tc=61 K) , is used to calculate the functional derivative of the d -wave eigenvalue λd of the linearized gap equation with respect to the imaginary part of the spin susceptibility χ''(q ,ω ) at 70 K. For temperatures near Tc, the variation of Tc with respect to χ''(q ,ω ) is proportional to this functional derivative. We find that above an energy ˜4 Tc the functional derivative becomes positive so that adding spin-fluctuation spectral weight at higher frequencies leads to an increase in Tc. The strongest pairing occurs for large momentum transfers, and small momentum spin-fluctuations suppress the pairing.

  12. Spintronics of antiferromagnetic systems

    International Nuclear Information System (INIS)

    Gomonaj, E.V.; Loktev, V.M.

    2014-01-01

    Spintronics of antiferromagnetics is a new field that has developed in a fascinating research topic in physics of magnetism. Antiferromagnetics, like ferromagnetic materials experience the influence of spin-polarized current, even though they show no macroscopic magnetization. The mechanism of this phenomenon is related to spin-dependent interaction between free and localized electrons-sd-exchange. Due to the peculiarities of antiferromagnetic materials (complicated magnetic structure, essential role of the exchange interactions, lack of macroscopic magnetization) spintronics of antiferromagnets appeals to new theoretical and experimental approaches. The purpose of this review is to systemize and summarize the recent progress in this field. We start with a short introduction into the structure and dynamics of antiferromagnets and proceed with discussion of different microscopic and phenomenological theories for description of current-induced phenomena in ferro-/antiferromagnetic heterostructures. We also consider the problems of the reverse influence of antiferromagnetic ordering on current, and effectiveness of the fully antiferromagnetic spin valve. In addition, we shortly review and interpret the available experimental results.

  13. Response functions of cold neutron matter: density, spin and current fluctuations

    Energy Technology Data Exchange (ETDEWEB)

    Keller, Jochen; Sedrakian, Armen [Institut fuer Theoretische Physik, Goethe-Universitaet, Frankfurt am Main (Germany)

    2014-07-01

    We study the response of a single-component pair-correlated baryonic Fermi-liquid to density, spin, and their current perturbations. A complete set of response functions is calculated in the low-temperature regime. We derive the spectral functions of collective excitations associated with the density, density-current, spin, and spin-current perturbations. The dispersion relations of density and spin fluctuations are determined and it is shown that the density fluctuations lead to exciton-like undamped bound states, whereas the spin excitations correspond to diffusive modes above the pair-breaking threshold. The contribution of the collective pair-breaking modes to the specific heat of neutron matter at subnuclear densities is computed and is shown to be comparable to that of the degenerate electron gas at not too low temperatures.

  14. Simulations of ground state fluctuations in mean-field Ising spin glasses

    International Nuclear Information System (INIS)

    Boettcher, Stefan

    2010-01-01

    The scaling of fluctuations in the distribution of ground state energies or costs with the system size N for Ising spin glasses is considered using an extensive set of simulations with the extremal optimization heuristic across a range of different models on sparse and dense graphs. These models exhibit very diverse behaviors, and an asymptotic extrapolation is often complicated by higher-order corrections in size. The clearest picture, in fact, emerges from the study of graph bipartitioning, a combinatorial optimization problem closely related to spin glasses. Asides from two-spin interactions with discrete bonds, we also consider problems with Gaussian bonds and three-spin interactions, which behave quite differently

  15. Magnetic dichroism and spin structure of antiferromagnetic NiO(001) films

    NARCIS (Netherlands)

    Altieri, S; Finazzi, M; Hsieh, HH; Lin, HJ; Chen, CT; Hibma, T; Valeri, S; Sawatzky, GA

    2003-01-01

    We find that Ni L-2 edge x-ray magnetic linear dichroism is fully reversed for NiO(001) films on materials with reversed lattice mismatch. We relate this phenomenon to a preferential stabilization of magnetic S domains with main spin component either in or out of the plane, via dipolar interactions.

  16. Quantum Number Fractionalization in Antiferromagnets

    OpenAIRE

    Laughlin, R. B.; Giuliano, D.; Caracciolo, R.; White, O.

    1998-01-01

    This is a pedagogical introduction to the mathematics of 1-dimensional spin-1/2 antiferromagnets. Topics covered include the Haldane-Shastry Hamiltonian, vector ``supercharges'', conserved spin currents, spinons, the supersymmetric Kuramoto-Yokoyama Hamiltonian, and holons.

  17. Critical behavior of 2 and 3 dimensional ferro- and antiferromagnetic spin ice systems in the framework of the Effective Field Renormalization Group technique

    OpenAIRE

    Garcia-Adeva, A. J.; Huber, D. L.

    2001-01-01

    In this work we generalize and subsequently apply the Effective Field Renormalization Group technique to the problem of ferro- and antiferromagnetically coupled Ising spins with local anisotropy axes in geometrically frustrated geometries (kagome and pyrochlore lattices). In this framework, we calculate the various ground states of these systems and the corresponding critical points. Excellent agreement is found with exact and Monte Carlo results. The effects of frustration are discussed. As ...

  18. Spin model for nontrivial types of magnetic order in inverse-perovskite antiferromagnets

    Science.gov (United States)

    Mochizuki, Masahito; Kobayashi, Masaya; Okabe, Reoya; Yamamoto, Daisuke

    2018-02-01

    Nontrivial magnetic orders in the inverse-perovskite manganese nitrides are theoretically studied by constructing a classical spin model describing the magnetic anisotropy and frustrated exchange interactions inherent in specific crystal and electronic structures of these materials. With a replica-exchange Monte Carlo technique, a theoretical analysis of this model reproduces the experimentally observed triangular Γ5 g and Γ4 g spin-ordered patterns and the systematic evolution of magnetic orders. Our Rapid Communication solves a 40-year-old problem of nontrivial magnetism for the inverse-perovskite manganese nitrides and provides a firm basis for clarifying the magnetism-driven negative thermal expansion phenomenon discovered in this class of materials.

  19. Photoinduced second harmonic generation of LaFe4Sb12near spin fluctuated critical points

    International Nuclear Information System (INIS)

    Nouneh, K.; Viennois, R.; Kityk, I.V.; Terki, F.; Charar, S.; Benet, S.; Paschen, S.

    2004-01-01

    The temperature dependence of the resistivity, the Seebeck coefficient and photoinduced second harmonic generation (PISHG) are studied near the quantum critical point in the skutterudite compound LaFe 4 Sb 12 , possessing increased spin fluctuations. We observed a large maximum of the PISHG at a temperature of about 15 K. The PISHG signal increases substantially below 35 K. We found a correlation between the temperature dependences of PISHG, resistivity and Seebeck coefficient. We proposed a phenomenological explanation for the occurrence of the PISHG signal in LaFe 4 Sb 12 implying strong spin fluctuations exist in this system, which may present some interest for the study of other spin fluctuation systems. Physical insight into the phenomenon observed is grounded in the participation of anharmonic electron-phonon and electron-paramagnon interactions stimulated by inducing light in the interactions with the photoexcited dipole moments. (copyright 2004 WILEY-VCH Verlag GmbH and Co. KGaA, Weinheim) (orig.)

  20. Protocol for generating multiphoton entangled states from quantum dots in the presence of nuclear spin fluctuations

    DEFF Research Database (Denmark)

    Denning, Emil Vosmar; Iles-Smith, Jake; McCutcheon, Dara P. S.

    2017-01-01

    Multiphoton entangled states are a crucial resource for many applications inquantum information science. Semiconductor quantum dots offer a promising route to generate such states by mediating photon-photon correlations via a confinedelectron spin, but dephasing caused by the host nuclear spin...... environment typically limits coherence (and hence entanglement) between photons to the spin T2* time of a few nanoseconds. We propose a protocol for the deterministic generation of multiphoton entangled states that is inherently robust against the dominating slow nuclear spin environment fluctuations, meaning...... that coherence and entanglement is instead limited only by the much longer spin T2 time of microseconds. Unlike previous protocols, the present schemeallows for the generation of very low error probability polarisation encoded three-photon GHZ states and larger entangled states, without the need for spin echo...

  1. Spin-valves with modified synthetic antiferromagnets exhibiting an enhanced bias point control capability at submicrometer dimensions

    International Nuclear Information System (INIS)

    Park, J.-S.; Lee, S.-R.; Kim, Y.K.

    2004-01-01

    Bias point control is of practical importance for operating read sensors for magnetic recording and magnetic random access memory devices. To attain bias point control capability, in particular, at submicrometer cell size, a modified synthetic antiferromagnet-based spin-valve (MSSV) structure was devised. A series of calculations were carried out to investigate the effect of size variation on their MR transfer behaviors. The cell dimension was varied from 10 to 0.05 μm. The typical MSSV comprises IrMn (9.0)/CoFe (P1, 1.5)/Ru (0.7)/CoFe (P2, 3.0)/Ru (0.7)/CoFe (P3, 1.5)/Cu (2.8)/CoFe (1.6)/NiFe (3.2) (in nm). As the cell size decreased, the bias point in the MSSV maintained nearly zero regardless of the cell size. The bias point was further tuned by varying the P3 layer thickness. Moreover, the effective exchange field (H ex.eff ) of the MSSV was much larger than that of the conventional SSV. The field sensitivity of the MSSV was very high indicating that the free layer can rotate more sharply

  2. Spin-valves with modified synthetic antiferromagnets exhibiting an enhanced bias point control capability at submicrometer dimensions

    Science.gov (United States)

    Park, Jeong-Suk; Lee, Seong-Rae; Kim, Young Keun

    2004-08-01

    Bias point control is of practical importance for operating read sensors for magnetic recording and magnetic random access memory devices. To attain bias point control capability, in particular, at submicrometer cell size, a modified synthetic antiferromagnet-based spin-valve (MSSV) structure was devised. A series of calculations were carried out to investigate the effect of size variation on their MR transfer behaviors. The cell dimension was varied from 10 to 0.05 μm. The typical MSSV comprises IrMn (9.0)/CoFe (P1, 1.5)/Ru (0.7)/CoFe (P2, 3.0)/Ru (0.7)/CoFe (P3, 1.5)/Cu (2.8)/CoFe (1.6)/NiFe (3.2) (in nm). As the cell size decreased, the bias point in the MSSV maintained nearly zero regardless of the cell size. The bias point was further tuned by varying the P3 layer thickness. Moreover, the effective exchange field ( Hex.eff) of the MSSV was much larger than that of the conventional SSV. The field sensitivity of the MSSV was very high indicating that the free layer can rotate more sharply.

  3. Spin fluctuations and low temperature features of thermal coefficient of linear expansion of iron monosilicide

    International Nuclear Information System (INIS)

    Volkov, A.G.; Kortov, S.V.; Povzner, A.A.

    1996-01-01

    The low temperature measurements of thermal coefficient of linear expansion of strong paramagnet FeSi are carried out. The results obtained are discussed with in the framework of spin-fluctuation theory. It is shown that electronic part of the thermal coefficient of linear expansion is negative in the range of temperatures lower that of the semiconductor-metal phase transition. In metal phase it becomes positive. This specific features of the thermal coefficient is explained by the spin-fluctuation renormalization of d-electronic states density

  4. Similarity between the superconductivity in the graphene with the spin transport in the two-dimensional antiferromagnet in the honeycomb lattice

    Science.gov (United States)

    Lima, L. S.

    2017-02-01

    We have used the Dirac's massless quasi-particles together with the Kubo's formula to study the spin transport by electrons in the graphene monolayer. We have calculated the electric conductivity and verified the behavior of the AC and DC currents of this system, that is a relativistic electron plasma. Our results show that the AC conductivity tends to infinity in the limit ω → 0 , similar to the behavior obtained for the spin transport in the two-dimensional frustrated antiferromagnet in the honeycomb lattice. We have made a diagrammatic expansion for the Green's function and we have not gotten significative change in the results.

  5. Magnetic fluctuations in heavy-fermion metals

    DEFF Research Database (Denmark)

    Mason, T.E.; Petersen, T.; Aeppli, G.

    1995-01-01

    Elastic and inelastic neutron scattering have been used to study the antiferromagnetic ordering and magnetic excitations of the U heavy-fermion superconductors UPd2Al3 and URu2Si2 above and below T-N. While both materials exhibit the coexistence of superconductivity and antiferromagnetic order......, the nature of the antiferromagnetic order and magnetic fluctuations is qualitatively quite different. UPd2Al3 resembles a rare earth magnetic system with coupling of the 4f electrons to the conduction electrons manifested in a broadening of otherwise conventional spin wave excitations. This is in marked...

  6. The slave-fermion approach of spin fluctuations in ferromagnet metals

    Science.gov (United States)

    Hu, C. D.

    2015-11-01

    In this work we propose a method to treat the spin fluctuations in itinerant ferromagnets. It is able to do calculation with a convergent series. The slave fermion method is applied to separate the charge (denoted by fermions) and spin (denoted by bosons) degrees of freedom. The spin operators are then replaced by the Schwinger boson fields. This way, the interaction term in the model can be reduced to a very simple form and can be teated without difficulty. Finally the equations of motion are derived in order to obtain the forms of Green's functions of fermions and bosons. The result is applied to the calculation of resistivity as a function temperature.

  7. Observation of layered antiferromagnetism in self-assembled parallel NiSi nanowire arrays on Si(110) by spin-polarized scanning tunneling spectromicroscopy

    Science.gov (United States)

    Hong, Ie-Hong; Hsu, Hsin-Zan

    2018-03-01

    The layered antiferromagnetism of parallel nanowire (NW) arrays self-assembled on Si(110) have been observed at room temperature by direct imaging of both the topographies and magnetic domains using spin-polarized scanning tunneling microscopy/spectroscopy (SP-STM/STS). The topographic STM images reveal that the self-assembled unidirectional and parallel NiSi NWs grow into the Si(110) substrate along the [\\bar{1}10] direction (i.e. the endotaxial growth) and exhibit multiple-layer growth. The spatially-resolved SP-STS maps show that these parallel NiSi NWs of different heights produce two opposite magnetic domains, depending on the heights of either even or odd layers in the layer stack of the NiSi NWs. This layer-wise antiferromagnetic structure can be attributed to an antiferromagnetic interlayer exchange coupling between the adjacent layers in the multiple-layer NiSi NW with a B2 (CsCl-type) crystal structure. Such an endotaxial heterostructure of parallel magnetic NiSi NW arrays with a layered antiferromagnetic ordering in Si(110) provides a new and important perspective for the development of novel Si-based spintronic nanodevices.

  8. Spin fluctuations and superconductivity in Mo.sub.3./sub.Sb.sub.7./sub..

    Czech Academy of Sciences Publication Activity Database

    Candolfi, C.; Lenoir, B.; Dauscher, A.; Bellouard, C.; Hejtmánek, Jiří; Šantavá, Eva; Tobola, J.

    2007-01-01

    Roč. 99, č. 3 (2007), 037006/1-037006/4 ISSN 0031-9007 Institutional research plan: CEZ:AV0Z10100521 Keywords : spin fluctuations * paramagnons * superconductivity Subject RIV: BM - Solid Matter Physics ; Magnetism Impact factor: 6.944, year: 2007

  9. Doping dependence of spin fluctuations and electron correlations in iron pnictides

    Czech Academy of Sciences Publication Activity Database

    Ikeda, H.; Arita, R.; Kuneš, Jan

    2010-01-01

    Roč. 82, č. 2 (2010), 024508/1-024508/6 ISSN 1098-0121 Institutional research plan: CEZ:AV0Z10100521 Keywords : iron pnicitdes * dynamic spin susceptibility * fluctuation-exchange approximation Subject RIV: BM - Solid Matter Physics ; Magnetism Impact factor: 3.772, year: 2010 http://prb.aps.org/abstract/PRB/v82/i2/e024508

  10. Itinerant ferromagnetism in actinide 5 f -electron systems: Phenomenological analysis with spin fluctuation theory

    Science.gov (United States)

    Tateiwa, Naoyuki; Pospíšil, Jiří; Haga, Yoshinori; Sakai, Hironori; Matsuda, Tatsuma D.; Yamamoto, Etsuji

    2017-07-01

    We have carried out an analysis of magnetic data in 69 uranium, 7 neptunium, and 4 plutonium ferromagnets with the spin fluctuation theory developed by Takahashi [Y. Takahashi, J. Phys. Soc. Jpn. 55, 3553 (1986), 10.1143/JPSJ.55.3553]. The basic and spin fluctuation parameters of the actinide ferromagnets are determined and the applicability of the spin fluctuation theory to actinide 5 f system has been discussed. Itinerant ferromagnets of the 3 d transition metals and their intermetallics follow a generalized Rhodes-Wohlfarth relation between peff/ps and TC/T0 , viz., peff/ps∝(TC/T0) -3 /2 . Here, ps, peff, TC, and T0 are the spontaneous and effective magnetic moments, the Curie temperature, and the width of spin fluctuation spectrum in energy space, respectively. The same relation is satisfied for TC/T0uranium and neptunium ferromagnets below (TC/T0)kink=0.32 ±0.02 , where a kink structure appears in relation between the two quantities. ps increases more weakly above (TC/T0)kink. A possible interpretation with the TC/T0 dependence of ps is given.

  11. Enhanced quantum spin fluctuations in a binary Bose-Einstein condensate

    Science.gov (United States)

    Bisset, R. N.; Kevrekidis, P. G.; Ticknor, C.

    2018-02-01

    For quantum fluids, the role of quantum fluctuations may be significant in several regimes such as when the dimensionality is low, the density is high, the interactions are strong, or for low particle numbers. In this paper, we propose a fundamentally different regime for enhanced quantum fluctuations without being restricted by any of the above conditions. Instead, our scheme relies on the engineering of an effective attractive interaction in a dilute, two-component Bose-Einstein condensate (BEC) consisting of thousands of atoms. In such a regime, the quantum spin fluctuations are significantly enhanced (atom bunching with respect to the noninteracting limit) since they act to reduce the interaction energy, a remarkable property given that spin fluctuations are normally suppressed (antibunching) at zero temperature. In contrast to the case of true attractive interactions, our approach is not vulnerable to BEC collapse. We numerically demonstrate that these quantum fluctuations are experimentally accessible by either spin or single-component Bragg spectroscopy, offering a useful platform on which to test beyond-mean-field theories. We also develop a variational model and use it to analytically predict the shift of the immiscibility critical point, finding good agreement with our numerics.

  12. Superconductivity in doped antiferromagnets

    International Nuclear Information System (INIS)

    Lagos, M.

    1990-09-01

    The antiferromagnetic S = 1/2 Heisenberg model is extended to account for the presence of holes. The holes move along a sublattice whose sites are located in between the spin sites. The spin-hole coupling arises from the modification of the exchange interaction between two neighbouring spins when the site between them is occupied by a hole. this physical picture leads to a generalized version of the so called t-J model Hamiltonian. The use of a recently developed method that introduces spin-O excitations for dealing with the Heisenberg antiferromagnetic model allows us to map the model Hamiltonian onto a Froelich one, with the spin-O magnetic excitations substituting phonons. The case of electrons moving along the spin sites is discussed as well. (author). 16 refs, 2 figs

  13. Magnetic fluctuations in UNi4B

    DEFF Research Database (Denmark)

    Mentink, S.A.M.; Mason, T.E.; Buyers, W.J.L.

    1997-01-01

    We investigate the magnetic fluctuation spectrum of the geometrically frustrated antiferromagnetic compound UNi4B, which partially orders below T-N = 20 K. An overdamped spin excitation is observed at the AF wave vector around 2.4 meV. Low-frequency, weakly Q-dependent inelastic scattering...

  14. Quantifying fluctuations of resting state networks using arterial spin labeling perfusion MRI.

    Science.gov (United States)

    Dai, Weiying; Varma, Gopal; Scheidegger, Rachel; Alsop, David C

    2016-03-01

    Blood oxygen level dependent (BOLD) functional magnetic resonance imaging (fMRI) has been widely used to investigate spontaneous low-frequency signal fluctuations across brain resting state networks. However, BOLD only provides relative measures of signal fluctuations. Arterial Spin Labeling (ASL) MRI holds great potential for quantitative measurements of resting state network fluctuations. This study systematically quantified signal fluctuations of the large-scale resting state networks using ASL data from 20 healthy volunteers by separating them from global signal fluctuations and fluctuations caused by residual noise. Global ASL signal fluctuation was 7.59% ± 1.47% relative to the ASL baseline perfusion. Fluctuations of seven detected resting state networks vary from 2.96% ± 0.93% to 6.71% ± 2.35%. Fluctuations of networks and residual noise were 6.05% ± 1.18% and 6.78% ± 1.16% using 4-mm resolution ASL data applied with Gaussian smoothing kernel of 6mm. However, network fluctuations were reduced by 7.77% ± 1.56% while residual noise fluctuation was markedly reduced by 39.75% ± 2.90% when smoothing kernel of 12 mm was applied to the ASL data. Therefore, global and network fluctuations are the dominant structured noise sources in ASL data. Quantitative measurements of resting state networks may enable improved noise reduction and provide insights into the function of healthy and diseased brain. © The Author(s) 2015.

  15. Dynamic Spin-Lattice Coupling and Nematic Fluctuations in NaFeAs

    Directory of Open Access Journals (Sweden)

    Yu Li

    2018-06-01

    Full Text Available We use inelastic neutron scattering to study acoustic phonons and spin excitations in single crystals of NaFeAs, a parent compound of iron-pnictide superconductors. NaFeAs exhibits a tetragonal-to-orthorhombic structural transition at T_{s}≈58  K and a collinear antiferromagnetic order at T_{N}≈45  K. While longitudinal and out-of-plane transverse acoustic phonons behave as expected, the in-plane transverse acoustic phonons reveal considerable softening on cooling to T_{s} and then harden on approaching T_{N} before saturating below T_{N}. In addition, we find that spin-spin correlation lengths of low-energy magnetic excitations within the FeAs layer and along the c axis increase dramatically below T_{s} and show a weak anomaly across T_{N}. These results suggest that the electronic nematic phase present in the paramagnetic tetragonal phase is closely associated with dynamic spin-lattice coupling, possibly arising from the one-phonon–two-magnon mechanism.

  16. Topological-Sector Fluctuations and Curie-Law Crossover in Spin Ice

    Directory of Open Access Journals (Sweden)

    L. D. C. Jaubert

    2013-02-01

    Full Text Available At low temperatures, a spin ice enters a Coulomb phase—a state with algebraic correlations and topologically constrained spin configurations. We show how analytical and numerical approaches for model spin-ice systems reveal a crossover between two Curie laws. One of these laws characterizes the high-temperature paramagnetic regime, while the other, which we call the “spin-liquid Curie law,” characterizes the low-temperature Coulomb-phase regime, which provides implicit evidence that the topological sector fluctuates. We compare our theory with experiment for Ho_{2}Ti_{2}O_{7}, where this process leads to a nonstandard temperature evolution of the bulk susceptibility and the wave-vector-dependent magnetic susceptibility, as measured by neutron scattering. Theory and experiment agree for bulk quantities and at large scattering wave vectors, but differences at small wave vectors indicate that the classical spin-ice states are not equally populated at low temperatures. More generally, the crossover appears to be a generic property of the emergent gauge field for a classical spin liquid, and it sheds light on the experimental difficulty of measuring a precise Curie-Weiss temperature in frustrated materials. The susceptibility at finite wave vectors is shown to be a local probe of fluctuations among topological sectors on varying length scales.

  17. Glass-like recovery of antiferromagnetic spin ordering in a photo-excited manganite Pr0.7Ca0.3MnO3

    Energy Technology Data Exchange (ETDEWEB)

    Zhou, S. Y.; Langner, M. C.; Zhu, Y.; Chuang, Y. -D.; Rini, M.; Glover, T. E.; Hertlein, M. P.; Gonzalez, A.G. Cruz; Tahir, N.; Tomioka, Y.; Tokura, Y.; Hussain, Z.; Schoenlein, R. W.

    2014-01-16

    Electronic orderings of charges, orbitals and spins are observed in many strongly correlated electron materials, and revealing their dynamics is a critical step toward understanding the underlying physics of important emergent phenomena. Here we use time-resolved resonant soft x-ray scattering spectroscopy to probe the dynamics of antiferromagnetic spin ordering in the manganite Pr0:7Ca0:3MnO3 following ultrafast photo-exitation. Our studies reveal a glass-like recovery of the spin ordering and a crossover in the dimensionality of the restoring interaction from quasi-1D at low pump fluence to 3D at high pump fluence. This behavior arises from the metastable state created by photo-excitation, a state characterized by spin disordered metallic droplets within the larger charge- and spin-ordered insulating domains. Comparison with time-resolved resistivity measurements suggests that the collapse of spin ordering is correlated with the insulator-to-metal transition, but the recovery of the insulating phase does not depend on the re-establishment of the spin ordering.

  18. Effect of thermal fluctuations in spin-torque driven magnetization dynamics

    International Nuclear Information System (INIS)

    Bonin, R.; Bertotti, G.; Serpico, C.; Mayergoyz, I.D.; D'Aquino, M.

    2007-01-01

    Nanomagnets with uniaxial symmetry driven by an external field and spin-polarized currents are considered. Anisotropy, applied field, and spin polarization are all aligned along the symmetry axis. Thermal fluctuations are described by adding a Gaussian white noise stochastic term to the Landau-Lifshitz-Gilbert equation for the deterministic dynamics. The corresponding Fokker-Planck equation is derived. It is shown that deterministic dynamics, thermal relaxation, and transition rate between stable states are governed by an effective potential including the effect of current injection

  19. Effect of thermal fluctuations in spin-torque driven magnetization dynamics

    Energy Technology Data Exchange (ETDEWEB)

    Bonin, R. [INRiM, I-10135 Turin (Italy)]. E-mail: bonin@inrim.it; Bertotti, G. [INRiM, I-10135 Turin (Italy); Serpico, C. [Dipartimento di Ingegneria Elettrica, Universita di Napoli ' Federico II' I-80125 Naples (Italy); Mayergoyz, I.D. [Department of Electrical and Computer Engineering, University of Maryland, College Park, MD 20742 (United States); D' Aquino, M. [Dipartimento per le Tecnologie, Universita di Napoli ' Parthenope' , I-80133 Naples (Italy)

    2007-09-15

    Nanomagnets with uniaxial symmetry driven by an external field and spin-polarized currents are considered. Anisotropy, applied field, and spin polarization are all aligned along the symmetry axis. Thermal fluctuations are described by adding a Gaussian white noise stochastic term to the Landau-Lifshitz-Gilbert equation for the deterministic dynamics. The corresponding Fokker-Planck equation is derived. It is shown that deterministic dynamics, thermal relaxation, and transition rate between stable states are governed by an effective potential including the effect of current injection.

  20. Reduction of weak interaction rates in neutron stars by nucleon spin fluctuations: Degenerate case

    International Nuclear Information System (INIS)

    Raffelt, G.; Strobel, T.

    1997-01-01

    Nucleon spin fluctuations in a dense medium reduce the open-quotes naiveclose quotes values of weak interaction rates (neutrino opacities, neutrino emissivities). We extend previous studies of this effect to the degenerate case which is appropriate for neutron stars a few ten seconds after formation. If neutron-neutron interactions by a one-pion exchange potential are the dominant cause of neutron spin fluctuations, a perturbative calculation of weak interaction rates is justified for T approx-lt 3m/(4πα π 2 )∼1MeV, where m is the neutron mass and α π ∼15 the pion fine-structure constant. At higher temperatures, the application of Landau close-quote s theory of Fermi liquids is no longer justified; i.e., the neutrons cannot be viewed as simple quasiparticles in any obvious sense. copyright 1997 The American Physical Society

  1. Effect of pressure on spin fluctuations and superconductivity in heavy-fermion UPt3

    International Nuclear Information System (INIS)

    Willis, J.O.; Thompson, J.D.; Fisk, Z.; de Visser, A.; Franse, J.J.M.; Menovsky, A.

    1985-01-01

    We have determined the effect of hydrostatic pressure on the susceptibility, on the T 2 temperature dependence of the spin-fluctuation resistivity, and on superconductivity in UPt 3 . The spin-fluctuation temperature T/sub s/, derived from the slope of resistivity versus T 2 , is used within a Fermi-liquid picture to calculate the susceptibility chi at T = 0 K. The depression of this calculated chi with pressure agrees with the directly measured value partial lnchi/partialP = -24 Mbar -1 . Both the superconducting transition temperature T/sub c/ and the initial slope of the upper critical field also decrease under pressure. We find that partial lnT/sub c//partialP = -25 Mbar -1 and speculate upon correlations between chi and T/sub c/

  2. Anomalous behavior of spin fluctuations in polycrystalline NdBa_2Cu_3O_7-δ

    Science.gov (United States)

    Abdelrazek, M. M.; Reyes, A. P.; Kuhns, P. L.; Moulton, W. G.; Halperin, W. P.; Kishio, K.

    2001-03-01

    Critical slowing down of Nd spin fluctuations have been observed in 92K superconductor NdBa_2Cu_3O_7-δ at temperatures well below Tc and orders of magnitude higher than TN ( ~0.5K). Nuclear spin-lattice relaxation rate 1/T1 at the planar O(2,3) and bridging O(4) oxygen sites have been measured as a function of temperature in fields up to 37T. Data is characterized by an extremely fast relaxation, roughly two orders of magnitude larger than those of YBCO, suggestive of Nd origin. The temperature dependence shows neither Tc nor the pseudo-gap but rather a well-defined field-dependent peak for both sites. Preliminary analysis suggests 1/T1 follows the typical behavior of freezing of spin fluctuations, when the inverse correlation time of the Nd spins τc becomes comparable to NMR frequency, ω τc ~ 1. The field dependence originates from the tail of the power spectrum beyond the 1/τc cutoff. The implications of these results to superconductivity in these systems will be discussed.

  3. Ising-like spin anisotropy and competing antiferromagnetic-ferromagnetic orders in GdBaCo2O5.5 single crystals.

    Science.gov (United States)

    Taskin, A A; Lavrov, A N; Ando, Yoichi

    2003-06-06

    In RBaCo2O5+x compounds (R is rare earth), a ferromagnetic-antiferromagnetic competition is accompanied by a giant magnetoresistance. We study the magnetization of detwinned GdBaCo2O5.5 single crystals and find a remarkable uniaxial anisotropy of Co3+ spins which is tightly linked with the chain oxygen ordering in GdO0.5 planes. Reflecting the underlying oxygen order, CoO2 planes also develop a spin-state order consisting of Co3+ ions in alternating rows of S=1 and S=0 states. The magnetic structure appears to be composed of weakly coupled ferromagnetic ladders with Ising-like moments, which gives a simple picture for magnetotransport phenomena.

  4. Critical behavior of two- and three-dimensional ferromagnetic and antiferromagnetic spin-ice systems using the effective-field renormalization group technique

    Science.gov (United States)

    Garcia-Adeva, Angel J.; Huber, David L.

    2001-07-01

    In this work we generalize and subsequently apply the effective-field renormalization-group (EFRG) technique to the problem of ferro- and antiferromagnetically coupled Ising spins with local anisotropy axes in geometrically frustrated geometries (kagomé and pyrochlore lattices). In this framework, we calculate the various ground states of these systems and the corresponding critical points. Excellent agreement is found with exact and Monte Carlo results. The effects of frustration are discussed. As pointed out by other authors, it turns out that the spin-ice model can be exactly mapped to the standard Ising model, but with effective interactions of the opposite sign to those in the original Hamiltonian. Therefore, the ferromagnetic spin ice is frustrated and does not order. Antiferromagnetic spin ice (in both two and three dimensions) is found to undergo a transition to a long-range-ordered state. The thermal and magnetic critical exponents for this transition are calculated. It is found that the thermal exponent is that of the Ising universality class, whereas the magnetic critical exponent is different, as expected from the fact that the Zeeman term has a different symmetry in these systems. In addition, the recently introduced generalized constant coupling method is also applied to the calculation of the critical points and ground-state configurations. Again, a very good agreement is found with exact, Monte Carlo, and renormalization-group calculations for the critical points. Incidentally, we show that the generalized constant coupling approach can be regarded as the lowest-order limit of the EFRG technique, in which correlations outside a frustrated unit are neglected, and scaling is substituted by strict equality of the thermodynamic quantities.

  5. Influence of Al-atoms on the spin fluctuation scattering in R(Co,Al)2 compounds

    International Nuclear Information System (INIS)

    Duc, N.H.; Hung, D.T.; Kim-Ngan, N.H.; Sechovsky, V.

    1992-01-01

    The resistivity and magnetisation have been measured for the R(Co 1-x Al x ) 2 compounds with R=Nd, Gd, Tb, Dy, Ho, Er and Lu. For x=0.2 the resistivity enhancement is observed below T c , however, for the compounds with R=Lu-Tb only. The results are discussed in terms of the spin fluctuation scattering and indicate that the enhancement of the spin fluctuation scattering is strongly related to the lattice parameter. (orig.)

  6. Focused issue on antiferromagnetic spintronics: An overview (Part of a collection of reviews on antiferromagnetic spintronics)

    KAUST Repository

    Jungwirth, T.

    2017-05-30

    This focused issue attempts to provide a comprehensive introduction into the field of antiferromagnetic spintronics. Apart from the brief overview below, it features five review articles. The intention is to cover in a coherent and complementary way key physical aspects of the antiferromagnetic spintronics research. These range from microelectronic memory devices and optical manipulation and detection of antiferromagnetic spins, to the fundamentals of antiferromagnetic dynamics in uniform or spin-textured systems, and to the interplay of antiferromagnetic spintronics with topological phenomena. The antiferromagnetic ordering can take a number of forms including fully compensated collinear, non-collinear, and non-coplanar magnetic lattices, compensated and uncompensated ferrimagnets, or metamagnetic materials hosting an antiferromagnetic to ferromagnetic phase transition. Apart from the variety of distinct magnetic crystal structures, the focused issue also encompasses spintronic phenomena and devices studied in antiferromagnet/ferromagnet heterostructures and in synthetic antiferromagnets.

  7. Focused issue on antiferromagnetic spintronics: An overview (Part of a collection of reviews on antiferromagnetic spintronics)

    KAUST Repository

    Jungwirth, T.; Sinova, J.; Manchon, Aurelien; Marti, X.; Wunderlich, J.; Felser, C.

    2017-01-01

    This focused issue attempts to provide a comprehensive introduction into the field of antiferromagnetic spintronics. Apart from the brief overview below, it features five review articles. The intention is to cover in a coherent and complementary way key physical aspects of the antiferromagnetic spintronics research. These range from microelectronic memory devices and optical manipulation and detection of antiferromagnetic spins, to the fundamentals of antiferromagnetic dynamics in uniform or spin-textured systems, and to the interplay of antiferromagnetic spintronics with topological phenomena. The antiferromagnetic ordering can take a number of forms including fully compensated collinear, non-collinear, and non-coplanar magnetic lattices, compensated and uncompensated ferrimagnets, or metamagnetic materials hosting an antiferromagnetic to ferromagnetic phase transition. Apart from the variety of distinct magnetic crystal structures, the focused issue also encompasses spintronic phenomena and devices studied in antiferromagnet/ferromagnet heterostructures and in synthetic antiferromagnets.

  8. Possible mechanism to enhance spin-fluctuation-mediated superconductivity in two-dimensional organic conductor

    Energy Technology Data Exchange (ETDEWEB)

    Nonoyama, Yoshito; Maekawa, Yukiko; Kobayashi, Akito; Suzumura, Yoshikazu [Department of Physics, Nagoya University, Nagoya 464-8602 (Japan); Yamada, Jun-ichi [Department of Material Science, Graduate School of Material Science, University of Hyogo, Hyogo 678-1297 (Japan)], E-mail: nonoyama@slab.phys.nagoya-u.ac.jp

    2008-10-15

    Mechanisms of superconductivity in quasi-two-dimensional organic conductors have been investigated using an extended Hubbard model by using the transfer energies between BDA-TTP molecules for {beta}-(BDA-TTP){sub 2}I{sub 3} based on the X-ray experiment data and the extended Hueckel calculation. We obtain several mean-field solutions with charge orderings which may represent short-range orderings or low-energy fluctuations in the low-dimensional electronic system. In the pressure-temperature phase diagram, a charge ordered metal state almost degenerates with a normal metal state between an insulating phase with charge ordering and the normal metal phase. Using the random phase approximation (RPA) and the linearized gap equation, the transition temperature of the superconducting state is estimated for the charge-ordered metal state and the normal metal state. It is found that transition temperature of the superconductivity induced by spin fluctuations in the charge-ordered metal state is much higher than that of the normal metal state and that the superconductivity in the charge-ordered metal state is the gapless d-wave. This suggests that the short range charge ordering may also contribute to an enhancement of spin-fluctuation-mediated superconductivity. The difference in the superconducting states between {beta}-(BDA-TTP){sub 2}I{sub 3} and {beta}-(BDA-TTP){sub 2}SbF{sub 6} are briefly discussed.

  9. Possible mechanism to enhance spin-fluctuation-mediated superconductivity in two-dimensional organic conductor

    International Nuclear Information System (INIS)

    Nonoyama, Yoshito; Maekawa, Yukiko; Kobayashi, Akito; Suzumura, Yoshikazu; Yamada, Jun-ichi

    2008-01-01

    Mechanisms of superconductivity in quasi-two-dimensional organic conductors have been investigated using an extended Hubbard model by using the transfer energies between BDA-TTP molecules for β-(BDA-TTP) 2 I 3 based on the X-ray experiment data and the extended Hueckel calculation. We obtain several mean-field solutions with charge orderings which may represent short-range orderings or low-energy fluctuations in the low-dimensional electronic system. In the pressure-temperature phase diagram, a charge ordered metal state almost degenerates with a normal metal state between an insulating phase with charge ordering and the normal metal phase. Using the random phase approximation (RPA) and the linearized gap equation, the transition temperature of the superconducting state is estimated for the charge-ordered metal state and the normal metal state. It is found that transition temperature of the superconductivity induced by spin fluctuations in the charge-ordered metal state is much higher than that of the normal metal state and that the superconductivity in the charge-ordered metal state is the gapless d-wave. This suggests that the short range charge ordering may also contribute to an enhancement of spin-fluctuation-mediated superconductivity. The difference in the superconducting states between β-(BDA-TTP) 2 I 3 and β-(BDA-TTP) 2 SbF 6 are briefly discussed.

  10. Co-existence of long-range order and spin fluctuation in a new geometric frustration series M2(OH)3Cl

    International Nuclear Information System (INIS)

    Zheng, X.G.; Hagihala, Masato; Toriyi, Takato

    2007-01-01

    Recently, we observed the co-existence of a long-range magnetic order and spin fluctuation in a clean compound of clinoatacamite, Cu 2 (OH) 3 Cl (PRL95 (2005) 057201). The present work reports magnetic studies on other compounds of this transition metal series M 2 (OH) 3 Cl, where M represents three-dimensional (3D)-electron magnetic ions of Co 2+ , Fe 2+ , etc., respectively. The present study shows that this co-existence is a common feature of the M 2 Cl(OH) 3 series, no matter whether it is anti-ferromagnetic, as in the case of Fe 2 (OH) 3 Cl (T N =15 K), or ferromagnetic, as in the case of Co 2 (OH) 3 Cl (T C =10.5 K). These compounds show a 3D network of corner-sharing tetrahedrons for the magnetic ions. The tetrahedron is slightly tilted with roughly 10% longer distance between the M-M bonded by Cl than those bonded by O and this distortion is suspected to be responsible for the partial order. This research suggests that the transition metal hydroxyhalide M 2 Cl(OH) 3 series are new geometric frustration system on tetrahedral lattice for d-electron spins

  11. Doping evolution of spin fluctuations and their peculiar suppression at low temperatures in Ca(Fe 1 -xCox)2As2

    Science.gov (United States)

    Sapkota, A.; Das, P.; Böhmer, A. E.; Ueland, B. G.; Abernathy, D. L.; Bud'ko, S. L.; Canfield, P. C.; Kreyssig, A.; Goldman, A. I.; McQueeney, R. J.

    2018-05-01

    Results of inelastic neutron scattering measurements are reported for two annealed compositions of Ca(Fe 1 -xCox)2As2,x =0.026 and 0.030, which possess stripe-type antiferromagnetically ordered and superconducting ground states, respectively. In the AFM ground state, well-defined and gapped spin waves are observed for x =0.026 , similar to the parent CaFe2As2 compound. We conclude that the well-defined spin waves are likely to be present for all x corresponding to the AFM state. This behavior is in contrast to the smooth evolution to overdamped spin dynamics observed in Ba(Fe 1 -xCox)2As2 , wherein the crossover corresponds to microscopically coexisting AFM order and SC at low temperature. The smooth evolution is likely absent in Ca(Fe 1 -xCox)2As2 due to the mutual exclusion of AFM ordered and SC states. Overdamped spin dynamics characterize paramagnetism of the x =0.030 sample and high-temperature x =0.026 sample. A sizable loss of magnetic intensity is observed over a wide energy range upon cooling the x =0.030 sample, at temperatures just above and within the superconducting phase. This phenomenon is unique amongst the iron-based superconductors and is consistent with a temperature-dependent reduction in the fluctuating moment. One possible scenario ascribes this loss of moment to a sensitivity to the c -axis lattice parameter in proximity to the nonmagnetic collapsed tetragonal phase and another scenario ascribes the loss to a formation of a pseudogap.

  12. Superconductivity and spin fluctuations in M-Zr metallic glasses (M = Cu, Ni, Co, and Fe)

    International Nuclear Information System (INIS)

    Altounian, Z.; Strom-Olsen, J.O.

    1983-01-01

    The superconducting transition temperature, upper critical field, and magnetic susceptibility have been measured in four binary metallic glass systems: Cu-Zr, Ni-Zr, Co-Zr, and Fe-Zr. For each alloy system, a full and continuous range of Zr-rich compositions accessible by melt spinning has been examined. For Cu-Zr, the range is 0.75>x>0.30; for Ni-Zr, 0.80>x>0.30; for Co-Zr, 0.80>x>0.48, and for Fe-Zr, 0.80>x>0.55 (x being the concentration of Zr in at. %). The results show clearly the influence of spin fluctuations in reducing the superconducting transition temperature. The data have been successfully analyzed using a modified form of the McMillan equation together with expressions for the Stoner enhanced magnetic susceptibility and the Ginsburg-Landau-Abrikosov-Gor'kov expression for the upper critical field

  13. NMR line broadening in solids by slowing down of spin fluctuations

    International Nuclear Information System (INIS)

    Mehring, M.; Sinning, G.; Pines, A.; California Univ., Berkeley

    1976-01-01

    The 109 Ag nuclear magnetic resonance line in a sample of polycrystalline AgF is observed to broaden substantially when the 19 F spins are irradiated near the magic angle in their rotating frame. This is due to the reduction of 19 F- 19 F dipolar coupling, which normally causes fluctuations in the 19 F- 109 Ag interactions (Abragam and Winter), inducing an exchange narrowing analogous to classical motional narrowing. The 109 Ag linewidths obtained over the entire motional range at different 19 F frequencies are compared with those calculated exactly from the ratio of second to fourth moment. (orig.) [de

  14. Properties of spin-1/2 triangular-lattice antiferromagnets CuY2Ge2O8 and CuLa2Ge2O8

    Science.gov (United States)

    Cho, Hwanbeom; Kratochvílová, Marie; Sim, Hasung; Choi, Ki-Young; Kim, Choong Hyun; Paulsen, Carley; Avdeev, Maxim; Peets, Darren C.; Jo, Younghun; Lee, Sanghyun; Noda, Yukio; Lawler, Michael J.; Park, Je-Geun

    2017-04-01

    We found new two-dimensional (2D) quantum (S =1 /2 ) antiferromagnetic systems: Cu R E2G e2O8 (R E =Y and La). According to our analysis of high-resolution x-ray and neutron diffraction experiments, the Cu network of Cu R E2G e2O8 (R E =Y and La) exhibits a 2D triangular lattice linked via weak bonds along the perpendicular b axis. Our bulk characterizations from 0.08 to 400 K show that they undergo a long-range order at 0.51(1) and 1.09(4) K for the Y and La systems, respectively. Interestingly, they also exhibit field induced phase transitions. For theoretical understanding, we carried out the density functional theory (DFT) band calculations to find that they are typical charge-transfer-type insulators with a gap of Eg≅2 eV . Taken together, our observations make Cu R E2G e2O8 (R E =Y and La) additional examples of low-dimensional quantum spin triangular antiferromagnets with the low-temperature magnetic ordering.

  15. Magnetic structures of (Co2-xNix)(OH)PO4 (x = 0.1,0.3) spin glass-like state in antiferromagnetically ordered phases

    International Nuclear Information System (INIS)

    Pedro, I de; Rojo, J M; Pizarro, J L; Fernandez, J RodrIguez; Marcos, J Sanchez; Fernandez-DIaz, M T; Arriortua, M I; Rojo, T

    2006-01-01

    Compounds of the general formula Co 2-x Ni x (OH)PO 4 (x = 0.1, 0.3) have been synthesized under mild hydrothermal conditions. Neutron powder diffraction, susceptibility and heat capacity measurements were carried out on polycrystalline samples. The cobalt-nickel compounds are ordered as three-dimensional antiferromagnets with ordering temperatures of 70 and 64 K for x = 0.1 and x = 0.3, respectively. The magnetic study shows a spin glass-like state below 11 and 5 K for Co 1.9 Ni 0.1 (OH)PO 4 and Co 1.7 Ni 0.3 (OH)PO 4 , respectively. Specific heat data present peaks at 68 and 61 K for Co 1.9 Ni 0.1 and Co 1.7 Ni 0.3 , respectively. These peaks show broad shoulders between approximately 15 and 40 K. The lack of any distinguishable anomaly below 10 K supports the spin glass nature of the low temperature transitions. Refinement of room temperature neutron diffraction data indicates that the Ni(II) ions are in octahedral co-ordination with the practical absence of these ions in the trigonal bipyramidal sites. The magnetic structures of Co 2-x Ni x (OH)PO 4 consist of ferromagnetic arrangements between the octahedral chains and trigonal bipyramidal dimers within the xz plane with the magnetic moments along the z axis. The ferromagnetic layers are disposed antiparallel to one another along the y direction establishing the three-dimensional antiferromagnetic order (T N ∼70 K for Co 1.9 Ni 0.1 and ∼64 K for Co 1.7 Ni 0.3 ). The different exchange pathways, the anisotropy of the Co(II) ions and the frustration of the magnetic moments in the trigonal bipyramidal geometry could be responsible for the freezing process

  16. Structure and thermodynamic properties of (C5H12N)CuBr3: a new weakly coupled antiferromagnetic spin-1/2 chain complex lying in the 1D-3D dimensional cross-over regime.

    Science.gov (United States)

    Pan, Bingying; Wang, Yang; Zhang, Lijuan; Li, Shiyan

    2014-04-07

    Single crystals of a metal organic complex (C5H12N)CuBr3 (C5H12N = piperidinium, pipH for short) have been synthesized, and the structure was determined by single-crystal X-ray diffraction. (pipH)CuBr3 crystallizes in the monoclinic group C2/c. Edging-sharing CuBr5 units link to form zigzag chains along the c axis, and the neighboring Cu(II) ions with spin-1/2 are bridged by bibromide ions. Magnetic susceptibility data down to 1.8 K can be well fitted by the Bonner-Fisher formula for the antiferromagnetic spin-1/2 chain, giving the intrachain magnetic coupling constant J ≈ -17 K. At zero field, (pipH)CuBr3 shows three-dimensional (3D) order below TN = 1.68 K. Calculated by the mean-field theory, the interchain coupling constant J' = -0.91 K is obtained and the ordered magnetic moment m0 is about 0.23 μB. This value of m0 makes (pipH)CuBr3 a rare compound suitable to study the 1D-3D dimensional cross-over problem in magnetism, since both 3D order and one-dimensional (1D) quantum fluctuations are prominent. In addition, specific heat measurements reveal two successive magnetic transitions with lowering temperature when external field μ0H ≥ 3 T is applied along the a' axis. The μ0H-T phase diagram of (pipH)CuBr3 is roughly constructed.

  17. Role of fluctuations in the phase transitions of coupled plaquette spin models of glasses

    Directory of Open Access Journals (Sweden)

    Giulio Biroli, Charlotte Rulquin, Gilles Tarjus, Marco Tarzia

    2016-10-01

    Full Text Available We study the role of fluctuations on the thermodynamic glassy properties of plaquette spin models, more specifically on the transition involving an overlap order parameter in the presence of an attractive coupling between different replicas of the system. We consider both short-range fluctuations associated with the local environment on Bethe lattices and long-range fluctuations that distinguish Euclidean from Bethe lattices with the same local environment. We find that the phase diagram in the temperature-coupling plane is very sensitive to the former but, at least for the $3$-dimensional (square pyramid model, appears qualitatively or semi-quantitatively unchanged by the latter. This surprising result suggests that the mean-field theory of glasses provides a reasonable account of the glassy thermodynamics of models otherwise described in terms of the kinetically constrained motion of localized defects and taken as a paradigm for the theory of dynamic facilitation. We discuss the possible implications for the dynamical behavior.

  18. Performance comparison of dynamical decoupling sequences for a qubit in a rapidly fluctuating spin bath

    International Nuclear Information System (INIS)

    Alvarez, Gonzalo A.; Suter, Dieter; Ajoy, Ashok; Peng Xinhua

    2010-01-01

    Avoiding the loss of coherence of quantum mechanical states is an important prerequisite for quantum information processing. Dynamical decoupling (DD) is one of the most effective experimental methods for maintaining coherence, especially when one can access only the qubit system and not its environment (bath). It involves the application of pulses to the system whose net effect is a reversal of the system-environment interaction. In any real system, however, the environment is not static, and therefore the reversal of the system-environment interaction becomes imperfect if the spacing between refocusing pulses becomes comparable to or longer than the correlation time of the environment. The efficiency of the refocusing improves therefore if the spacing between the pulses is reduced. Here, we quantify the efficiency of different DD sequences in preserving different quantum states. We use 13 C nuclear spins as qubits and an environment of 1 H nuclear spins as the environment, which couples to the qubit via magnetic dipole-dipole couplings. Strong dipole-dipole couplings between the proton spins result in a rapidly fluctuating environment with a correlation time of the order of 100 μs. Our experimental results show that short delays between the pulses yield better performance if they are compared with the bath correlation time. However, as the pulse spacing becomes shorter than the bath correlation time, an optimum is reached. For even shorter delays, the pulse imperfections dominate over the decoherence losses and cause the quantum state to decay.

  19. Zn and Ni substitutional effects on spin fluctuations in YBa sub 2 Cu sub 3 O sub 7 by sup 6 sup 3 sup , sup 6 sup 5 Cu NQR

    CERN Document Server

    Han, K S; Mean, B J; Lee, K H; Seo, S W; Lee, M H; Lee, W C

    2000-01-01

    We have prepared Zn- and Ni-substituted YBa sub 2 Cu sub 3 O sub 7 (YBa sub 2 Cu sub 3 sub - sub x M sub x O sub 7 , M=Zn or Ni, x=0.00 approx 0.09) and performed sup 6 sup 3 sup , sup 6 sup 5 Cu nuclear quadrupole resonance (NQR) measurements for the plane site at 300 and 100 K. Substitutional effects on the relaxation rates are markedly different. Both the spin-lattice and the spin-spin relaxation rates decrease for Zn-doped YBCO. However, those increase for Ni-doped YBCO. This contrast in local electronic dynamics provides clear microscopic evidence that Zn forms no local moment while Ni develops a local moment. Consequently, the antiferromagnetic spin fluctuation is suppressed by Zn doping whereas it is preserved by Ni doping. This is also confirmed by the ratio of the sup 6 sup 3 sup , sup 6 sup 5 Cu spin-lattice relaxation rates for the plane coppers.

  20. Critical behavior of AC antiferromagnetic and ferromagnetic susceptibilities of a spin-1/2 metamagnetic Ising system

    International Nuclear Information System (INIS)

    Gulpinar, Gul; Vatansever, Erol

    2012-01-01

    In this study, the temperature variations of the equilibrium and the non-equilibrium antiferromagnetic and ferromagnetic susceptibilities of a metamagnetic system are examined near the critical point. The kinetic equations describing the time dependencies of the total and staggered magnetizations are derived by utilizing linear response theory. In order to obtain dynamic magnetic relaxation behavior of the system, the stationary solutions of the kinetic equations in existence of sinusoidal staggered and physical external magnetic fields are performed. In addition, the static and dynamical mean field critical exponents are calculated in order to formulate the critical behavior of antiferromagnetic and ferromagnetic magnetic response of a metamagnetic system. Finally, a comparison of the findings of this study with previous theoretical and experimental studies is represented and it is shown that a good agreement is found with our results. - Highlights: ► Staggered dynamic susceptibility diverges as T→T N in the low frequency region. ► Dynamic total susceptibility exhibits a finite jump discontinuity as T→T N while wτ 2 ⪡1. ► The slope of the staggered magnetic dispersion curve chances in sign as T→T N .

  1. Effects of coexisting spin disorder and antiferromagnetism on the magnetic behavior of nanostructured (Fe{sub 79}Mn{sub 21}){sub 1−x}Cu{sub x} alloys

    Energy Technology Data Exchange (ETDEWEB)

    Mizrahi, M., E-mail: mizrahi@fisica.unlp.edu.ar, E-mail: cabrera@fisica.unlp.edu.ar [INIFTA-CCT- La Plata-CONICET and Departamento de Física, Facultad de Ciencias Exactas, C. C. 67, Universidad Nacional de La Plata, 1900 La Plata (Argentina); Cabrera, A. F., E-mail: mizrahi@fisica.unlp.edu.ar, E-mail: cabrera@fisica.unlp.edu.ar; Desimoni, J. [IFLP-CCT-La Plata-CONICET and Departamento de Física, Facultad de Ciencias Exactas C.C. 67, Universidad Nacional de La Plata, 1900 La Plata (Argentina); Stewart, S. J. [IFLP-CCT-La Plata-CONICET and Departamento de Física, Facultad de Ciencias Exactas C.C. 67, Universidad Nacional de La Plata, 1900 La Plata (Argentina); Instituto Ciencias de la Salud, Universidad Nacional Arturo Jauretche, Av. Calchaquí No. 6200, Florencio Varela (Argentina)

    2014-06-07

    We report a magnetic study on nanostructured (Fe{sub 79}Mn{sub 21}){sub 1−x}Cu{sub x} (0.00 ≤ x ≤ 0.30) alloys using static magnetic measurements. The alloys are mainly composed by an antiferromagnetic fcc phase and a disordered region that displays a spin-glass-like behavior. The interplay between the antiferromagnetic and magnetically disordered phases establishes an exchange anisotropy that gives rise to a loop shift at temperatures below the freezing temperature of moments belonging to the disordered region. The loop shift is more noticeable as the Cu content increases, which also enhances the spin-glass-like features. Further, in the x = 0.30 alloy the alignment imposed by applied magnetic fields higher than 4 kOe prevail over the configuration determined by the frustration mechanism that characterizes the spin glass-like phase.

  2. Low-energy spin fluctuations in the non-Fermi-liquid compound YbRh2Si2

    Directory of Open Access Journals (Sweden)

    O. Stockert et al

    2007-01-01

    Full Text Available We report on inelastic neutron scattering experiments on YbRh2Si2 powder to study the low-energy spin dynamics at temperatures between T=0.8 and 22 K. The low-energy magnetic response is quasielastic. However, it exhibits an unusual form not modelled by a simple relaxation rate yielding a Lorentzian lineshape, but can satisfactorily be described by a phenomenological model involving a distribution of relaxation rates. The lower bound of the relaxation rates varies roughly linear with temperature indicating a pronounced slowing down of the critical modes above the antiferromagnetic ordering temperature TNapprox70 mK.

  3. Numerical study of the enlarged O(5) symmetry of the 3D antiferromagnetic RP2 spin model

    International Nuclear Information System (INIS)

    Fernandez, L.A.; Martin-Mayor, V.; Sciretti, D.; Tarancon, A.; Velasco, J.L.

    2005-01-01

    We investigate by means of Monte Carlo simulation and finite-size scaling analysis the critical properties of the three-dimensional O(5) non-linear σ model and of the antiferromagnetic RP 2 model, both of them regularized on a lattice. High accuracy estimates are obtained for the critical exponents, universal dimensionless quantities and critical couplings. It is concluded that both models belong to the same universality class, provided that rather non-standard identifications are made for the momentum-space propagator of the RP 2 model. We have also investigated the phase diagram of the RP 2 model extended by a second-neighbor interaction. A rich phase diagram is found, where most of the phase transitions are of the first order

  4. Pressure dependence of critical temperature of bulk FeSe from spin fluctuation theory

    Science.gov (United States)

    Hirschfeld, Peter; Kreisel, Andreas; Wang, Yan; Tomic, Milan; Jeschke, Harald; Jacko, Anthony; Valenti, Roser; Maier, Thomas; Scalapino, Douglas

    2013-03-01

    The critical temperature of the 8K superconductor FeSe is extremely sensitive to pressure, rising to a maximum of 40K at about 10GPa. We test the ability of the current generation of fluctuation exchange pairing theories to account for this effect, by downfolding the density functional theory electronic structure for each pressure to a tight binding model. The Fermi surface found in such a procedure is then used with fixed Hubbard parameters to determine the pairing strength using the random phase approximation for the spin singlet pairing vertex. We find that the evolution of the Fermi surface captured by such an approach is alone not sufficient to explain the observed pressure dependence, and discuss alternative approaches. PJH, YW, AK were supported by DOE DE-FG02-05ER46236, the financial support of MT, HJ, and RV from the DFG Schwerpunktprogramm 1458 is kindly acknowledged.

  5. Phenomenological approach to spin fluctuations in itinerant magnets and superconductors from ab initio calculations

    Energy Technology Data Exchange (ETDEWEB)

    Ortenzi, Luciano

    2013-10-17

    In this thesis I study the interplay between magnetism and superconductivity in itinerant magnets and superconductors. I do this by applying a semiphenomenological method to four representative compounds. In particular I use the discrepancies (whenever present) between density functional theory (DFT) calculations and the experiments in order to construct phenomenological models which explain the magnetic, superconducting and optical properties of four representative systems. I focus my attention on the superconducting and normal state properties of the recently discovered APt3P superconductors, on superconducting hole-doped CuBiSO, on the optical properties of LaFePO and finally on the ferromagnetic-paramagnetic transition of Ni3Al under pressure. At the end I present a new method which aims to describe the effect of spin fluctuations in itinerant magnets and superconductors that can be used to monitor the evolution of the electronic structure from non magnetic to magnetic in systems close to a quantum critical point.

  6. Critical slowing down of spin fluctuations in BiFeO3

    International Nuclear Information System (INIS)

    Scott, J F; Singh, M K; Katiyar, R S

    2008-01-01

    In earlier work we reported the discovery of phase transitions in BiFeO 3 evidenced by divergences in the magnon light-scattering cross-sections at 140 and 201 K (Singh et al 2008 J. Phys.: Condens. Matter 20 252203) and fitted these intensity data to critical exponents α = 0.06 and α' = 0.10 (Scott et al 2008 J. Phys.: Condens. Matter 20 322203), under the assumption that the transitions are strongly magnetoelastic (Redfern et al 2008 at press) and couple to strain divergences through the Pippard relationship (Pippard 1956 Phil. Mag. 1 473). In the present paper we extend those criticality studies to examine the magnon linewidths, which exhibit critical slowing down (and hence linewidth narrowing) of spin fluctuations. The linewidth data near the two transitions are qualitatively different and we cannot reliably extract a critical exponent ν, although the mean field value ν = 1/2 gives a good fit near the lower transition.

  7. Nonlinear spin fluctuations in the Fermi liquid of itinerant electron ferromagnets

    International Nuclear Information System (INIS)

    Solontsov, A.; Lacroix, C.

    2003-01-01

    A microscopic derivation of nonlinear equations of magnetic dynamics for itinerant ferromagnets is presented within the electron Fermi liquid model accounting for both long-range Coulomb and short-range interactions of quasiparticles, which founds the basis for the phenomenological description of nonlinear spin fluctuations (SF) using the Ginsburg-Landau formalism. Crystal lattice is shown to play a significant role screening the long-range Coulomb interaction and affecting magnetic dynamics. The spectrum of longitudinal SF with account of nonlinear mode-mode coupling is shown to result from an interplay of quasielastic SF and inelastic excitations near the magnon frequencies, both having mainly the nonlinear nature and arising due to their emission (absorption) by magnons

  8. Diamond lattice Heisenberg antiferromagnet

    Science.gov (United States)

    Oitmaa, J.

    2018-04-01

    We investigate ground-state and high-temperature properties of the nearest-neighbour Heisenberg antiferromagnet on the three-dimensional diamond lattice, using series expansion methods. The ground-state energy and magnetization, as well as the magnon spectrum, are calculated and found to be in good agreement with first-order spin-wave theory, with a quantum renormalization factor of about 1.13. High-temperature series are derived for the free energy, and physical and staggered susceptibilities for spin S  =  1/2, 1 and 3/2, and analysed to obtain the corresponding Curie and Néel temperatures.

  9. Static and dynamic spin fluctuations in the spin glass doping regime in La2-xSrxCuO4+y

    International Nuclear Information System (INIS)

    Birgeneau, R.J.; Belk, N.; Kastner, M.A.; Keimer, B.; Shirane, G.

    1991-01-01

    We review the results of neutron scattering studies of the static and dynamic spin fluctuations crystals of La 2-x Sr x CuO 4+δ in the doping regime intermediate between the Neel and superconducting regions. In this regime the in-plane resistance is linear in temperature down to ∼80 K with a crossover due to logarithmic conductance effects at lower temperatures. The static spin correlations are well-described by a simple model in which the inverse correlation length κ(x,T) =κ(x,0) + κ(0,T). The most dramatic new result is the discovery by Keimer et al. that the dynamic spin fluctuations exhibit a temperature dependence which is a simple function of ω/T for temperatures 10 K≤T≤500 K for a wide range of energies. This scaling leads to a natural explanation of a variety of normal state properties of the copper oxides. 21 refs., 4 figs

  10. Spin liquid in a single crystal of the frustrated diamond lattice antiferromagnet CoAl2O4

    DEFF Research Database (Denmark)

    Zaharko, O.; Christensen, Niels Bech; Cervellino, A.

    2011-01-01

    at the q = 0 positions are broad and their line shapes have strong Lorentzian contributions. Additionally, the peaks are connected by weak diffuse streaks oriented along the directions. The observed short-range magnetic correlations are explained within the spiral spin-liquid model. The specific...... shape of the energy landscape of the system, with an extremely flat energy minimum around q = 0 and many low-lying excited spiral states with q = , results in thermal population of this manifold at finite temperatures. The agreement between the experimental results and the spiral spin-liquid model...... is only qualitative, indicating that microstructure effects might be important to achieve quantitative agreement. Application of a magnetic field significantly perturbs the spiral spin-liquid correlations. The magnetic peaks remain broad but acquire more Gaussian line shapes and increase in intensity...

  11. High-order study of the quantum critical behavior of a frustrated spin-1/2 antiferromagnet on a stacked honeycomb bilayer

    Science.gov (United States)

    Bishop, R. F.; Li, P. H. Y.

    2017-12-01

    We study a frustrated spin-1/2 J1-J2-J3-J1⊥ Heisenberg antiferromagnet on an A A -stacked bilayer honeycomb lattice. In each layer we consider nearest-neighbor (NN), next-nearest-neighbor, and next-next-nearest-neighbor antiferromagnetic (AFM) exchange couplings J1,J2 , and J3, respectively. The two layers are coupled with an AFM NN exchange coupling J1⊥≡δ J1 . The model is studied for arbitrary values of δ along the line J3=J2≡α J1 that includes the most highly frustrated point at α =1/2 , where the classical ground state is macroscopically degenerate. The coupled cluster method is used at high orders of approximation to calculate the magnetic order parameter and the triplet spin gap. We are thereby able to give an accurate description of the quantum phase diagram of the model in the α δ plane in the window 0 ≤α ≤1 ,0 ≤δ ≤1 . This includes two AFM phases with Néel and striped order, and an intermediate gapped paramagnetic phase that exhibits various forms of valence-bond crystalline order. We obtain accurate estimations of the two phase boundaries, δ =δci(α) , or equivalently, α =αc i(δ ) , with i =1 (Néel) and 2 (striped). The two boundaries exhibit an "avoided crossing" behavior with both curves being re-entrant. Thus, in this α δ window, Néel order exists only for values of δ in the range δc1 (α ) , with δc1 0 for αc 1(0 ) ≈0.49 (1 ) , and striped order similarly exists only for values of δ in the range δc2 (α ) , with δc2 αc2(0) ≈0.600 (5 ) and δc2 0 for αc 2(0 ) >α >α2<≈0.56 (1 ) .

  12. Soft modes in the easy plane pyrochlore antiferromagnet

    International Nuclear Information System (INIS)

    Champion, J D M; Holdsworth, P C W

    2004-01-01

    Thermal fluctuations lift the high ground state degeneracy of the classical nearest neighbour pyrochlore antiferromagnet, with easy plane anisotropy, giving a first-order phase transition to a long range ordered state. We show, from spin wave analysis and numerical simulation, that even below this transition a continuous manifold of states, of dimension N 2/3 , exist (N is the number of degrees of freedom). As the temperature goes to zero a further 'order by disorder' selection is made from this manifold. The pyrochlore antiferromagnet Er 2 Ti 2 O 7 is believed to have an easy plane anisotropy and is reported to have the same magnetic structure. This is perhaps surprising, given that the dipole interaction lifts the degeneracy of the classical model in favour of a different structure. We interpret our results in the light of these facts

  13. Weak doping dependence of the antiferromagnetic coupling between nearest-neighbor Mn2 + spins in (Ba1 -xKx) (Zn1-yMny) 2As2

    Science.gov (United States)

    Surmach, M. A.; Chen, B. J.; Deng, Z.; Jin, C. Q.; Glasbrenner, J. K.; Mazin, I. I.; Ivanov, A.; Inosov, D. S.

    2018-03-01

    Dilute magnetic semiconductors (DMS) are nonmagnetic semiconductors doped with magnetic transition metals. The recently discovered DMS material (Ba1 -xKx) (Zn1-yMny) 2As2 offers a unique and versatile control of the Curie temperature TC by decoupling the spin (Mn2 +, S =5 /2 ) and charge (K+) doping in different crystallographic layers. In an attempt to describe from first-principles calculations the role of hole doping in stabilizing ferromagnetic order, it was recently suggested that the antiferromagnetic exchange coupling J between the nearest-neighbor Mn ions would experience a nearly twofold suppression upon doping 20% of holes by potassium substitution. At the same time, further-neighbor interactions become increasingly ferromagnetic upon doping, leading to a rapid increase of TC. Using inelastic neutron scattering, we have observed a localized magnetic excitation at about 13 meV associated with the destruction of the nearest-neighbor Mn-Mn singlet ground state. Hole doping results in a notable broadening of this peak, evidencing significant particle-hole damping, but with only a minor change in the peak position. We argue that this unexpected result can be explained by a combined effect of superexchange and double-exchange interactions.

  14. Pairing versus phase coherence of doped holes in distinct quantum spin backgrounds

    Science.gov (United States)

    Zhu, Zheng; Sheng, D. N.; Weng, Zheng-Yu

    2018-03-01

    We examine the pairing structure of holes injected into two distinct spin backgrounds: a short-range antiferromagnetic phase versus a symmetry protected topological phase. Based on density matrix renormalization group (DMRG) simulation, we find that although there is a strong binding between two holes in both phases, phase fluctuations can significantly influence the pair-pair correlation depending on the spin-spin correlation in the background. Here the phase fluctuation is identified as an intrinsic string operator nonlocally controlled by the spins. We show that while the pairing amplitude is generally large, the coherent Cooper pairing can be substantially weakened by the phase fluctuation in the symmetry-protected topological phase, in contrast to the short-range antiferromagnetic phase. It provides an example of a non-BCS mechanism for pairing, in which the paring phase coherence is determined by the underlying spin state self-consistently, bearing an interesting resemblance to the pseudogap physics in the cuprate.

  15. Antiferromagnetic spintronics

    Czech Academy of Sciences Publication Activity Database

    Jungwirth, Tomáš; Martí, Xavier; Wadley, P.; Wunderlich, Joerg

    2016-01-01

    Roč. 11, č. 3 (2016), 231-241 ISSN 1748-3387 R&D Projects: GA MŠk(CZ) LM2011026; GA ČR GB14-37427G EU Projects: European Commission(XE) 268066 - 0MSPIN Institutional support: RVO:68378271 Keywords : antiferromagnets * spintronics Subject RIV: BM - Solid Matter Physics ; Magnetism Impact factor: 38.986, year: 2016

  16. Neutron spin-echo studies on dynamic and static fluctuations in two types of poly(vinyl alcohol) gels

    International Nuclear Information System (INIS)

    Kanaya, T.; Takahashi, N.; Nishida, K.; Seto, H.; Nagao, M.; Takeda, T.

    2005-01-01

    We report neutron spin-echo measurements on two types of poly(vinyl alcohol) (PVA) gels. The first is PVA gel in a mixture of dimethyl sulfoxide (DMSO) and water with volume ratio 60/40, and the second is PVA gel in an aqueous borax solution. The observed normalized intermediate scattering functions I(Q,t)/I(Q,0) are very different between them. The former I(Q,t)/I(Q,0) shows a nondecaying component in addition to a fast decay, but the latter does not have the nondecaying one. This clearly indicates that the fluctuations in the former PVA gel consist of static and dynamic fluctuations whereas the latter PVA gel does include only the dynamic fluctuations. The dynamic fluctuations of the former and latter gels have been analyzed in terms of a restricted motion in the network and Zimm motion, respectively, and the origins of these motions will be discussed

  17. Quantum criticality among entangled spin chains

    Science.gov (United States)

    Blanc, N.; Trinh, J.; Dong, L.; Bai, X.; Aczel, A. A.; Mourigal, M.; Balents, L.; Siegrist, T.; Ramirez, A. P.

    2018-03-01

    An important challenge in magnetism is the unambiguous identification of a quantum spin liquid1,2, of potential importance for quantum computing. In such a material, the magnetic spins should be fluctuating in the quantum regime, instead of frozen in a classical long-range-ordered state. While this requirement dictates systems3,4 wherein classical order is suppressed by a frustrating lattice5, an ideal system would allow tuning of quantum fluctuations by an external parameter. Conventional three-dimensional antiferromagnets can be tuned through a quantum critical point—a region of highly fluctuating spins—by an applied magnetic field. Such systems suffer from a weak specific-heat peak at the quantum critical point, with little entropy available for quantum fluctuations6. Here we study a different type of antiferromagnet, comprised of weakly coupled antiferromagnetic spin-1/2 chains as realized in the molecular salt K2PbCu(NO2)6. Across the temperature-magnetic field boundary between three-dimensional order and the paramagnetic phase, the specific heat exhibits a large peak whose magnitude approaches a value suggestive of the spinon Sommerfeld coefficient of isolated quantum spin chains. These results demonstrate an alternative approach for producing quantum matter via a magnetic-field-induced shift of entropy from one-dimensional short-range order to a three-dimensional quantum critical point.

  18. Antiferromagnetic resonance excited by oscillating electric currents

    Science.gov (United States)

    Sluka, Volker

    2017-12-01

    In antiferromagnetic materials the order parameter exhibits resonant modes at frequencies that can be in the terahertz range, making them interesting components for spintronic devices. Here, it is shown that antiferromagnetic resonance can be excited using the inverse spin-Hall effect in a system consisting of an antiferromagnetic insulator coupled to a normal-metal waveguide. The time-dependent interplay between spin torque, ac spin accumulation, and magnetic degrees of freedom is studied. It is found that the dynamics of the antiferromagnet affects the frequency-dependent conductivity of the normal metal. Further, a comparison is made between spin-current-induced and Oersted-field-induced excitation under the condition of constant power injection.

  19. Linearized Jastrow-style fluctuations on spin-projected Hartree-Fock

    International Nuclear Information System (INIS)

    Henderson, Thomas M.; Scuseria, Gustavo E.

    2013-01-01

    The accurate and efficient description of strong electronic correlations remains an important objective in electronic structure theory. Projected Hartree-Fock theory, where symmetries of the Hamiltonian are deliberately broken and projectively restored, all with a mean-field computational scaling, shows considerable promise in this regard. However, the method is neither size extensive nor size consistent; in other words, the correlation energy per particle beyond broken-symmetry mean field vanishes in the thermodynamic limit, and the dissociation limit of a molecule is not the sum of the fragment energies. These two problems are closely related. Recently, Neuscamman [Phys. Rev. Lett. 109, 203001 (2012)] has proposed a method to cure the lack of size consistency in the context of the antisymmetrized geminal power wave function (equivalent to number-projected Hartree-Fock-Bogoliubov) by using a Jastrow-type correlator in Hilbert space. Here, we apply the basic idea in the context of projected Hartree-Fock theory, linearizing the correlator for computational simplicity but extending it to include spin fluctuations. Results are presented for the Hubbard Hamiltonian and for some simple molecular systems

  20. Metallic magnets without inversion symmetry and antiferromagnetic quantum critical points

    Energy Technology Data Exchange (ETDEWEB)

    Fischer, I.A.

    2006-07-01

    studied how the interplay of precession and damping affects various thermodynamic and transport quantities. We found that the susceptibility {chi}={delta}M/{delta}B is the thermodynamic quantity which shows the most significant change upon approaching the quantum critical point and which gives experimental access to the (dangerously irrelevant) spin-spin interactions. Finally, we studied the quantum critical behaviour of two-dimensional antiferromagnetic metals. Going beyond an order parameter theory, we included the electronic quasiparticles as well as the fluctuating magnetization in a functional Renormalization Group calculation. Preliminary results indicate a divergence in the fRG-equations already at a finite distance from the quantum critical point. this is incompatible with the Hertz-Millis picture. (orig.)

  1. Role of disorder in the multi-critical region of d-wave superconductivity and antiferromagnetism

    International Nuclear Information System (INIS)

    Yanase, Youichi; Ogata, Masao

    2007-01-01

    We investigate the disorder-induced microscopic inhomogeneity in the multi-critical region of d-wave superconductivity and antiferromagnetism on the basis of the microscopic t-t ' -U-V model. We find that a small amount of point disorder induces the nano-scale inhomogeneity of spin and superconducting fluctuations when the coherence length of superconductivity is remarkably short as in the under-doped cuprates. Then, the two fluctuations spatially segregate to avoid their competition. We show the remarkable electron-hole asymmetry in high-T c cuprates where the quite different spatial structure is expected in the electron-doped materials

  2. Superconductivity, spin fluctuations and lattice instability of V2ZrHsub(x)

    International Nuclear Information System (INIS)

    Keiber, H.

    1984-07-01

    A calorimeter was reassembled in order to determine the specific heat of small specimens of only approx. 100 mg mass. The equipment has been so designed that measurements between 1.5 K and 30 K by the adiabatic method can be performed also in high external magnetic fields of 13 tesla. On the basis of calibration measurements on germanium at 0 and 13 tesla the upper limit of the measuring error can be given as proportional 2% with the possibility of resolving specific heats of 10 -7 joule/kelvin. The equipment was used to measure the specific heat of the V 2 ZrHsub(x) system. In combination with susceptibility and neutron scatter measurements individual Sommerfeld constants, γ, can be unequivocally attributed to the cubic and rhombohedral phases of V 2 Zr. The value of lambda of 2.6 obtained by comparison with calculations of the band structure is in contradiction to the measured transition temperature of only 8.7 K provided that exclusive electron-phonon interaction is assumed. This result and the minor change of the transition temperature following drastic change of γ after the cubic -> rhombohedral phase transition was assigned to the influence of spin fluctuations. A homogeneous hydrogen load of V 2 Zr is possible only above T proportional 260 k. Below this temperature the boundary of a two-phase domain is surpassed. With the help of measurements of the lattice constants as a function of the temperature is was possible to prepare a rough phase diagram. (orig.) [de

  3. Angle and frequency dependence of self-energy from spin fluctuation mediated d-wave pairing for high temperature superconductors.

    Science.gov (United States)

    Hong, Seung Hwan; Choi, Han-Yong

    2013-09-11

    We investigated the characteristics of spin fluctuation mediated superconductivity employing the Eliashberg formalism. The effective interaction between electrons was modeled in terms of the spin susceptibility measured by inelastic neutron scattering experiments on single crystal La(2-x)Sr(x)CuO4 superconductors. The diagonal self-energy and off-diagonal self-energy were calculated by solving the coupled Eliashberg equation self-consistently for the chosen spin susceptibility and tight-binding dispersion of electrons. The full momentum and frequency dependence of the self-energy is presented for optimally doped, overdoped, and underdoped LSCO cuprates in a superconductive state. These results may be compared with the experimentally deduced self-energy from ARPES experiments.

  4. Spin fluctuation mechanism to normal state resistivity of iron-based superconductors La(O1-xFx)FeAs

    International Nuclear Information System (INIS)

    Choudhary, K.K.; Singh, S.; Prasad, D.; Kaurav, N.; Varshney, Dinesh

    2010-01-01

    Temperature-dependant resistivity of iron-based superconductors La(O 1-x F x )FeAs (for x = 0.12) is theoretically analysed by considering the strong spin fluctuations effect. In addition to the spin fluctuation-induced contribution the electron-phonon ρ e-ph (T) = AT, and electron-electron ρ e-e (T) = BT 2 contributions are also incorporated for complete understanding of experimental data. (author)

  5. Suppression of Electron Spin Relaxation in Mn-Doped GaAs

    Science.gov (United States)

    Astakhov, G. V.; Dzhioev, R. I.; Kavokin, K. V.; Korenev, V. L.; Lazarev, M. V.; Tkachuk, M. N.; Kusrayev, Yu. G.; Kiessling, T.; Ossau, W.; Molenkamp, L. W.

    2008-08-01

    We report a surprisingly long spin relaxation time of electrons in Mn-doped p-GaAs. The spin relaxation time scales with the optical pumping and increases from 12 ns in the dark to 160 ns upon saturation. This behavior is associated with the difference in spin relaxation rates of electrons precessing in the fluctuating fields of ionized or neutral Mn acceptors, respectively. For the latter, the antiferromagnetic exchange interaction between a Mn ion and a bound hole results in a partial compensation of these fluctuating fields, leading to the enhanced spin memory.

  6. Breakdown of antiferromagnet order in polycrystalline NiFe/NiO bilayers probed with acoustic emission

    Science.gov (United States)

    Lebyodkin, M. A.; Lebedkina, T. A.; Shashkov, I. V.; Gornakov, V. S.

    2017-07-01

    Magnetization reversal of polycrystalline NiFe/NiO bilayers was investigated using magneto-optical indicator film imaging and acoustic emission techniques. Sporadic acoustic signals were detected in a constant magnetic field after the magnetization reversal. It is suggested that they are related to elastic waves excited by sharp shocks in the NiO layer with strong magnetostriction. Their probability depends on the history and number of repetitions of the field cycling, thus testifying the thermal-activation nature of the long-time relaxation of an antiferromagnetic order. These results provide evidence of spontaneous thermally activated switching of the antiferromagnetic order in NiO grains during magnetization reversal in ferromagnet/antiferromagnet (FM/AFM) heterostructures. The respective deformation modes are discussed in terms of the thermal fluctuation aftereffect in the Fulcomer and Charap model which predicts that irreversible breakdown of the original spin orientation can take place in some antiferromagnetic grains with disordered anisotropy axes during magnetization reversal of exchange-coupled FM/AFM structures. The spin reorientation in the saturated state may induce abrupt distortion of isolated metastable grains because of the NiO magnetostriction, leading to excitation of shock waves and formation of plate (or Lamb) waves.

  7. NMR evidence for spin fluctuations in underdoped LaO{sub 1-x}F{sub x}FeAs

    Energy Technology Data Exchange (ETDEWEB)

    Hammerath, Franziska; Grafe, Hans-Joachim; Lang, Guillaume; Behr, Guenter; Werner, Jochen; Buechner, Bernd [Leibniz-Institut fuer Festkoerper- und Werkstoffforschung, Dresden (Germany); Paar, Dalibor [Department of Physics, Faculty of Science, University of Zagreb (Croatia)

    2012-07-01

    We present {sup 75}As Nuclear Magnetic Resonance (NMR) measurements on the iron-based superconductor LaO{sub 1-x}F{sub x}FeAs with 0 {<=} x {<=} 0.1, covering a broad range of the phase diagram from magnetically-ordered to optimally-doped superconducting samples. For underdoped samples (x=0.05,x=0.075) the {sup 75}As NMR spin-lattice relaxation rate (T{sub 1}T){sup -1} shows a Curie-Weiss-like increase at intermediate temperatures, indicating the slowing down of spin fluctuations. However, a simple Curie-Weiss fit fails to describe (T{sub 1}T){sup -1}(T) above 250 K and the occurrence of a peak in (T{sub 1}T){sup -1} slightly above T{sub c}. Instead, the data can be well described by considering a BPP-model for fluctuating magnetic fields in combination with a doping-independent linear temperature dependence at high temperature. At optimal doping (x=0.1) spin fluctuations are suppressed and only the linear contribution to (T{sub 1}T){sup -1} is left. This stands in contrast to other pnictides, such as Ba(Fe{sub 1-x}Co{sub x}As){sub 2} and Ba(FeAs{sub 1-x}P{sub x}){sub 2}. Our analysis is consistent with charge carrier localization in underdoped LaO{sub 1-x}F{sub x}FeAs as seen by means of resistivity measurements.

  8. Spin wave collapse and incommensurate fluctuations in URu2Si2

    DEFF Research Database (Denmark)

    Buyers, W.J.L.; Tun, Z.; Petersen, T.

    1994-01-01

    To test if the T(N) = 17.7 K transition in URu2Si2 is driven by a divergence of a magnetic order parameter we performed high-resolution neutron scattering. At the ordering wave vector the spin-wave energy collapsed. and the susceptibility diverged as T(N) was approached. This confirms that the or...... that the order parameter is the magnetic dipole, as shown by recent symmetry arguments and polarized neutron experiments [1]. We also observe incommensurate fluctuations, suggesting that competing temperature-dependent interactions may influence this weak-moment transition.......To test if the T(N) = 17.7 K transition in URu2Si2 is driven by a divergence of a magnetic order parameter we performed high-resolution neutron scattering. At the ordering wave vector the spin-wave energy collapsed. and the susceptibility diverged as T(N) was approached. This confirms...

  9. Neutron Inelastic Scattering Study of Transverse Spin Fluctuations in CsNiF3: a Soliton-only Central Peak

    DEFF Research Database (Denmark)

    Steiner, M.; Kakurai, K.; Knop, W.

    1982-01-01

    We have observed a quasi-elastic contribution to the spectrum of the transverse spin fluctuations Sperp;(Q, ω), perpendicular to an applied magnetic field in the easy plane of the one-dimensional ferromagnet CsNiF3. According to the present theoretical understanding this contribution is due solel...... to soliton quasi-particles and it should not contain two-magnon scattering. The observed dependence on momentum transfer is as expected for soliton scattering with zero intensity at qc = 0 rising through a maximum with increasing qc....

  10. Magnetic fluctuations and correlations in MnSi : Evidence for a chiral skyrmion spin liquid phase

    NARCIS (Netherlands)

    Pappas, C.; Lelièvre-Berna, E.; Bentley, P.; Falus, P.; Fouquet, P.; Farago, B.

    2011-01-01

    We present a comprehensive analysis of high-resolution neutron scattering data involving neutron spin echo spectroscopy and spherical polarimetry, which confirm the first-order nature of the helical transition in MnSi. The experiments reveal the existence of a totally chiral dynamic phase in a very

  11. A study of the quantum classical crossover in the spin dynamics of the 2D S = 5/2 antiferromagnet Rb2MnF4: neutron scattering, computer simulations and analytic theories

    International Nuclear Information System (INIS)

    Huberman, T; Tennant, D A; Cowley, R A; Coldea, R; Frost, C D

    2008-01-01

    We report comprehensive inelastic neutron scattering measurements of the magnetic excitations in the 2D spin-5/2 Heisenberg antiferromagnet Rb 2 MnF 4 as a function of temperature from deep in the Néel ordered phase up to paramagnetic, 0.13 B T/4JS −1 for temperatures up to near the Curie–Weiss temperature, Θ CW . For wavevectors smaller than ξ −1 , relaxational dynamics occurs. The observed renormalization of spin wave energies, and evolution of excitation lineshapes, with increasing temperature are quantitatively compared with finite-temperature spin wave theory and computer simulations for classical spins. Random phase approximation calculations provide a good description of the low temperature renormalization of spin waves. In contrast, lifetime broadening calculated using the first Born approximation shows, at best, modest agreement around the zone boundary at low temperatures. Classical dynamics simulations using an appropriate quantum classical correspondence were found to provide a good description of the intermediate and high temperature regimes over all wavevector and energy scales, and the crossover from quantum to classical dynamics observed around Θ CW /S, where the spin S = 5/2. A characterization of the data over the whole wavevector/energy/temperature parameter space is given. In this, T 2 behaviour is found to dominate the wavevector and temperature dependence of the linewidths over a large parameter range, and no evidence of hydrodynamic behaviour or dynamical scaling behaviour found within the accuracy of the datasets. An efficient and easily implemented classical dynamics methodology is presented that provides a practical method for modelling other semiclassical quantum magnets

  12. Two-magnon Raman scattering in a Mott-Hubbard antiferromagnet

    International Nuclear Information System (INIS)

    Basu, S.; Singh, A.

    1996-01-01

    A perturbation-theoretic diagrammatic scheme is developed for systematically studying the two-magnon Raman scattering in a Mott-Hubbard antiferromagnet. The fermionic structure of the magnon interaction vertex is obtained at order-1/N level in an inverse-degeneracy expansion, and the relevant two-magnon propagator is obtained by incorporating magnon interactions at a ladder-sum level. Evaluation of the magnon interaction vertex in the large-U limit yields a nearest-neighbor instantaneous interaction with interaction energy -J. Application of this approach to the intermediate-U regime, which is of relevance for cuprate antiferromagnets, is also discussed. Incorporating the zero-temperature magnon damping, which is estimated in terms of quantum spin fluctuations, the two-magnon Raman scattering intensity is evaluated and compared with experiments on La 2 CuO 4 . copyright 1996 The American Physical Society

  13. Dipolar Antiferromagnetism and Quantum Criticality in LiErF4

    International Nuclear Information System (INIS)

    Kraemer, Conradin; Nikseresht, Neda; Piatek, Julian; Tsyrulin, Nikolay; Piazza, Bastien; Kiefer, Klaus; Klemke, Bastian; Rosenbaum, Thomas; Aeppli, Gabriel; Gannarelli, Che; Prokes, Karel; Straessle, Thierry; Keller, Lukas; Zaharko, Oksana; Kraemer, Karl; Ronnow, Henrik

    2012-01-01

    Magnetism has been predicted to occur in systems in which dipolar interactions dominate exchange. We present neutron scattering, specific heat, and magnetic susceptibility data for LiErF 4 , establishing it as a model dipolar-coupled antiferromagnet with planar spin-anisotropy and a quantum phase transition in applied field H c# parallel# = 4.0 ± 0.1 kilo-oersteds. We discovered non-mean-field critical scaling for the classical phase transition at the antiferromagnetic transition temperature that is consistent with the two-dimensional XY/h 4 universality class; in accord with this, the quantum phase transition at H c exhibits three-dimensional classical behavior. The effective dimensional reduction may be a consequence of the intrinsic frustrated nature of the dipolar interaction, which strengthens the role of fluctuations.

  14. The low-temperature phase of the Heisenberg antiferromagnet in a fermionic representation

    International Nuclear Information System (INIS)

    Azakov, S.; Dilaver, M.; Oztas, A.M.

    1999-09-01

    Thermal properties of the ordered phase of the spin 1/2 isotropic Heisenberg Antiferromagnet on a d-dimensional hypercubical lattice are studied within the fermionic representation when the constraint of a single occupancy condition is taken into account by the method suggested by Popov and Fedotov. Using a saddle point approximation in the path integral approach we discuss not only the leading order but also the fluctuations around the saddle point at one-loop level. The influence of taking into account the single occupancy condition is discussed at all steps. (author)

  15. Exchange bias in diluted-antiferromagnet/antiferromagnet bilayers

    International Nuclear Information System (INIS)

    Mao, Zhongquan; Zhan, Xiaozhi; Chen, Xi

    2015-01-01

    The hysteresis-loop properties of a diluted-antiferromagnetic (DAF) layer exchange coupling to an antiferromagnetic (AF) layer are investigated by means of numerical simulations. Remarkable loop shift and coercivity enhancement are observed in such DAF/AF bilayers, while they are absent in the uncoupled DAF single layer. The influences of pinned domains, dilution, cooling field and DAF layer thickness on the loop shift are investigated systematically. The result unambiguously confirms an exchange bias (EB) effect in the DAF/AF bilayers. It also reveals that the EB effect originates from the pinned AF domains within the DAF layer. In contrast to conventional EB systems, frozen uncompensated spins are not found at the interface of the AF pinning layer. (paper)

  16. Electric control of antiferromagnets

    OpenAIRE

    Fina, I.; Marti, X.

    2016-01-01

    In the past five years, most of the paradigmatic concepts employed in spintronics have been replicated substituting ferromagnets by antiferromagnets in critical parts of the devices. The numerous research efforts directed to manipulate and probe the magnetic moments in antiferromagnets have been gradually established a new and independent field known as antiferromagnetic spintronics. In this paper, we focus on the electrical control and detection of antiferromagnetic moments at a constant tem...

  17. Theory of the upper critical field in antiferromagnetic superconductors

    International Nuclear Information System (INIS)

    Ro, C.; Levin, K.

    1984-01-01

    We compute the temperature T dependence of the upper critical field H/sub c/2(T) in antiferromagnetic (AF) superconductors. Using a strong-coupling formalism we explicitly treat the effects of the molecular field H/sub Q/, inelastic and elastic spin-fluctuation scattering and magnetic as well as nonmagnetic impurities. A sum rule is used to relate the T dependence of H/sub Q/ to that of the spin-fluctuation scattering. The decreased pair breaking observed below the Neel temperature in SmRh 4 B 4 and the increased pair breaking seen in the AF Chevrel compounds will both occur in our theory for a reasonable choice of parameters. For larger values of the dimensionless spin-exchange coupling constant N(0)J/sup c/f, spin-fluctuation-scattering effects dominate over those of H/sub Q/ and decreased pair breaking is observed below T/sub N/. For smaller values of the coupling constant, the converse is true. Impurity scattering is treated in a self-consistent fashion. As a consequence, the molecular field H/sub Q/ is altered by nonmagnetic impurities. This leads to important pair-breaking effects in H/sub c/2. A physical manifestation of this pair breaking is a qualitative change in the shape of the H/sub c/2 versus T curve, as nonmagnetic impurities are added. We give detailed predictions for the expected effects of these impurities on H/sub c/2 which can be tested experimentally

  18. Scattering of neutrons and critical phenomena in antiferromagnetic fermi liquid

    International Nuclear Information System (INIS)

    Akhiezer, I.A.; Barannik, E.A.

    1980-01-01

    The scattering of slow neutrons in an antiferromagnetic with collectivized magnetic electrons is considered and it is shown to significantly differ from the neutron scattering in an antiferromagnetic with localized magnetic electrons. The behaviour of scattering cross sections and fluctuation correlators near the Neel point is studied. These magnitudes are shown to increase with the critical index r=-1 [ru

  19. NMR study of spin fluctuations and superconductivity in LaFeAsO1-xHx

    Science.gov (United States)

    Fujiwara, Naoki; Sakurai, Ryosuke; Iimura, Soushi; Matsuishi, Satoru; Hosono, Hideo; Yamakawa, Yoichi; Kontani, Hiroshi

    2013-03-01

    We have performed NMR measurements in LaFeAsO1-xHx, an isomorphic compound of LaFeAsO1-xFx. LaFeAsO1-xHx is most recently known for having double superconducting (SC) domes on H doping. LaFeAsO1-xHx is an electron- doped system, and protons act as H-1 as well as F-1. The first SC dome is very similar between F and H doping, suggesting that H doping supplies the same amount of electrons as F doping. Interestingly, an excess amount of H up to x=0.5 can be replaced with O2-. In the H-overdoped regime (x > 0 . 2), LaFeAsO1-xHx undergoes the second superconducting state. We measured the relaxation rate of LaFeAsO1-xHx for x=0.2 and 0.4, and fond an anomalous electronic state; spin fluctuations measured from 1 /T1 T is enhanced with increasing the doping level from x = 0 . 2 to 0.4. The enhancement of spin fluctuations with increasing carrier doping is a new phenomenon that has not observed in LaFeAsO1-xFx in which the upper limit of the doping level is at most x = 0 . 2 . We will discuss the phenomenon in relation to superconductivity. Grant (KAKENHI 23340101) from the Ministry of Education, Sports and Science, Japan

  20. Thermodynamic properties of paramagnetic α - and β -Mn from first principles: The effect of transverse spin fluctuations

    Science.gov (United States)

    Ehteshami, Hossein; Korzhavyi, Pavel A.

    2017-12-01

    First-principles-based thermodynamic modeling of cubic α and β phases of Mn represent a challenge due to their structural complexity and the necessity of simultaneous treatment of several types of disorder (electronic, magnetic, and vibrational) that have very different characteristic time scales. Here we employ mean-field theoretical models to describe the different types of disorder and then we connect each layer of theory to the others using the adiabatic principle of separating faster and slower degrees of freedom. The slowest (vibrational) degrees of freedom are treated using the Moruzzi, Janak, and Schwarz formalism [Phys. Rev. B 37, 790 (1988), 10.1103/PhysRevB.37.790] of the Debye-Grüneisen model parametrized based on the first-principles calculated equation of state which includes the free-energy contributions due to the fast (electronic and magnetic) degrees of freedom via the Fermi-Dirac distribution function and a mean-field theory of transverse spin fluctuations. The magnetic contribution due to transverse spin fluctuations has been computed self-consistently within the disordered local moment picture of the paramagnetic state. The obtained results for thermodynamic properties such as lattice parameter, linear thermal expansion coefficient, and heat capacity of both phases show a good agreement with available experimental data. We also tested the assumption about the nature (localized versus delocalized) of magnetic moment on site IV in α -Mn and site I in β -Mn on the thermodynamic properties of these two phases. Similar to the findings of experimental studies, we conclude that magnetic moment on site IV in α -Mn is not of a localized character. However, a similar analysis suggests that the magnetic moment of site I in β -Mn should be treated as localized.

  1. Ti{sub 3}CrCu{sub 4}: A possible 2-D ferromagnetic spin fluctuating system

    Energy Technology Data Exchange (ETDEWEB)

    Dhar, S. K.; Kulkarni, R.; Goyal, Neeraj [Department of Condensed Matter Physics & Materials Science, T.I.F.R., Homi Bhabha Road, Colaba, Mumbai, 400005 (India); Provino, A.; Manfrinetti, P. [Department of Chemistry, University of Genova, Via Dodecaneso 31, 16146 Genova (Italy); Paudyal, D. [The Ames Laboratory, US Department of Energy, Iowa State University, Ames, IA 50011-3020 (United States)

    2016-05-15

    Ti{sub 3}CrCu{sub 4} is a new ternary compound which crystallizes in the tetragonal Ti{sub 3}Pd{sub 5} structure type. The Cr atoms form square nets in the a-b plane (a = 3.124 Å) which are separated by an unusually large distance c = 11.228 Å along the tetragonal axis, thus forming a -2-D Cr-sublattice. The paramagnetic susceptibility is characterized by a low effective moment, μ{sub eff} = 1.1 μ{sub B}, a low paramagnetic Curie temperature θ{sub P} (below 7 K) and a temperature independent χ{sub 0} = 6.7 x 10{sup −4} emu/mol. The magnetization at 1.8 K increases rapidly with field nearly saturating to 0.2 μ{sub B}/f.u. The zero field heat capacity C/T shows an upturn below 7 K (∼190 mJ/mol K{sup 2} at ∼0.1K) which is suppressed in applied magnetic fields and interpreted as suggesting the presence of spin fluctuations. The resistivity at low temperatures shows non-Fermi liquid behavior. Overall, the experimental data thus reveal an unusual magnetic state in Ti{sub 3}CrCu{sub 4}, which likely has its origin in the layered nature of the Cr sub-lattice and ferromagnetic spin fluctuations. Density functional theoretical calculations reveal a sharp Cr density of states peak just above the Fermi level, indicating the propensity of Ti{sub 3}CrCu{sub 4} to become magnetic.

  2. Emergent criticality and Friedan scaling in a two-dimensional frustrated Heisenberg antiferromagnet

    Science.gov (United States)

    Orth, Peter P.; Chandra, Premala; Coleman, Piers; Schmalian, Jörg

    2014-03-01

    We study a two-dimensional frustrated Heisenberg antiferromagnet on the windmill lattice consisting of triangular and dual honeycomb lattice sites. In the classical ground state, the spins on different sublattices are decoupled, but quantum and thermal fluctuations drive the system into a coplanar state via an "order from disorder" mechanism. We obtain the finite temperature phase diagram using renormalization group approaches. In the coplanar regime, the relative U(1) phase between the spins on the two sublattices decouples from the remaining degrees of freedom, and is described by a six-state clock model with an emergent critical phase. At lower temperatures, the system enters a Z6 broken phase with long-range phase correlations. We derive these results by two distinct renormalization group approaches to two-dimensional magnetism: Wilson-Polyakov scaling and Friedan's geometric approach to nonlinear sigma models where the scaling of the spin stiffnesses is governed by the Ricci flow of a 4D metric tensor.

  3. Spin systems

    CERN Document Server

    Caspers, W J

    1989-01-01

    This book is about spin systems as models for magnetic materials, especially antiferromagnetic lattices. Spin-systems are well-defined models, for which, in special cases, exact properties may be derived. These special cases are for the greater part, one- dimensional and restricted in their applicability, but they may give insight into general properties that also exist in higher dimension. This work pays special attention to qualitative differences between spin lattices of different dimensions. It also replaces the traditional picture of an (ordered) antiferromagnetic state of a Heisenberg sy

  4. Reciprocal propagation of surface modes in an antiferromagnetic film

    International Nuclear Information System (INIS)

    Oliveira, F.A.; Amato, M.A.

    1987-09-01

    Linear response theory is used to evaluate the Green's functions describing the fluctuations in an antiferromagnetic film at zero applied field. It is shown the similarities between the dielectric and magnetic excitations. (Author) [pt

  5. Parametric instability of spinning elastic rings excited by fluctuating space-fixed stiffnesses

    Science.gov (United States)

    Liu, Chunguang; Cooley, Christopher G.; Parker, Robert G.

    2017-07-01

    This study investigates the vibration of rotating elastic rings that are dynamically excited by an arbitrary number of space-fixed discrete stiffnesses with periodically fluctuating stiffnesses. The rotating, elastic ring is modeled using thin-ring theory with radial and tangential deformations. Primary and combination instability regions are determined in closed-form using the method of multiple scales. The ratio of peak-to-peak fluctuation to average discrete stiffness is used as the perturbation parameter, so the resulting perturbation analysis is not limited to small mean values of discrete stiffnesses. The natural frequencies and vibration modes are determined by discretizing the governing equations using Galerkin's method. Results are demonstrated for compliant gear applications. The perturbation results are validated by direct numerical integration of the equations of motion and Floquet theory. The bandwidths of the instability regions correlate with the fractional strain energy stored in the discrete stiffnesses. For rings with multiple discrete stiffnesses, the phase differences between them can eliminate large amplitude response under certain conditions.

  6. Spin-1/2 Triangular-Lattice Heisenberg Antiferromagnet with √{3} × √{3} -Type Distortion — Behavior around the Boundaries of the Intermediate Phase

    Science.gov (United States)

    Shimada, Alisa; Nakano, Hiroki; Sakai, Tôru; Yoshimura, Kazuyoshi

    2018-03-01

    The S = 1/2 triangular-lattice Heisenberg antiferromagnet with distortion is investigated by the numerical-diagonalization method. The examined distortion type is √{3} × √{3} . We study the case when the distortion connects the undistorted triangular lattice and the dice lattice. For the intermediate phase reported previously in this system, we obtain results of the boundaries of the intermediate phase for a larger system than those in the previous report and examine the system size dependence of the boundaries in detail. We also report the specific heat of this system, which shows a marked peak structure related to the appearance of the intermediate state.

  7. Spin fluctuation effects on the conductance through a single Pd atom contact

    International Nuclear Information System (INIS)

    Romero, M A; Goldberg, E C; Gomez-Carrillo, S C; Bolcatto, P G

    2009-01-01

    A controversy about the conductance through single atoms still exists. There are many experiments where values lower than the quantum unity G 0 = 2e 2 /h have been found associated to Kondo regimes with high Kondo temperatures. Specifically in the Pd single atom contact, conductance values close to G 0 /2 at room temperature have been reported. In this work we propose a theoretical analysis of a break junction of Pd where the charge fluctuation in the single atom contact is limited to the most probable one: d 10 ↔d 9 . The projected density of states and the characteristics of the electron transport are calculated by using a realistic description of the interacting system. A Kondo regime is found where the conductance values and their dependence on temperature are in good agreement with the experimental trends observed in the conduction of single molecule transistors based on transition metal coordination complexes.

  8. The electronic structure of antiferromagnetic chromium

    DEFF Research Database (Denmark)

    Skriver, Hans Lomholt

    1981-01-01

    The author has used the local spin density formalism to perform self-consistent calculations of the electronic structure of chromium in the non-magnetic and commensurate antiferromagnetic phases, as a function of the lattice parameter. A change of a few per cent in the atomic radius brings...

  9. Thermoinduced magnetization in nanoparticles of antiferromagnetic materials

    DEFF Research Database (Denmark)

    Mørup, Steen; Frandsen, Cathrine

    2004-01-01

    We show that there is a thermoinduced contribution to the magnetic moment of nanoparticles of antiferromagnetic materials. It arises from thermal excitations of the uniform spin-precession mode, and it has the unusual property that its magnitude increases with increasing temperature. This has...

  10. Antiferromagnetism and d-wave superconductivity in the Hubbard model

    Energy Technology Data Exchange (ETDEWEB)

    Krahl, H.C.

    2007-07-25

    The two-dimensional Hubbard model is a promising effective model for the electronic degrees of freedom in the copper-oxide planes of high temperature superconductors. We present a functional renormalization group approach to this model with focus on antiferromagnetism and d-wave superconductivity. In order to make the relevant degrees of freedom more explicitly accessible on all length scales, we introduce composite bosonic fields mediating the interaction between the fermions. Spontaneous symmetry breaking is reflected in a non-vanishing expectation value of a bosonic field. The emergence of a coupling in the d-wave pairing channel triggered by spin wave fluctuations is demonstrated. Furthermore, the highest temperature at which the interaction strength for the electrons diverges in the renormalization flow is calculated for both antiferromagnetism and d-wave superconductivity over a wide range of doping. This ''pseudo-critical'' temperature signals the onset of local ordering. Moreover, the temperature dependence of d-wave superconducting order is studied within a simplified model characterized by a single coupling in the d-wave pairing channel. The phase transition within this model is found to be of the Kosterlitz-Thouless type. (orig.)

  11. μSR Study of the Unusual Magnetic Ordering in the Frustrated Antiferromagnet Zn(CrxGa1-x)2O4

    International Nuclear Information System (INIS)

    Kikuchi, H.; Fukushima, H.; Higemoto, W.; Nishiyama, K.

    2001-01-01

    μSR spectra on the spin frustrating spinel antiferromagnet Zn(Cr x Ga 1-x ) 2 O 4 (x=0.9,1.0) have been measured. For x=1.0 compound, both the relaxation rate and the initial asymmetry showed distinct anomalies at the Neel temperature. The magnetic susceptibility for the x=0.9 compound was known to have a faint peak at around 12 K, whose origin was not clear so far. Our μSR study revealed that this temperature is the onset temperature of development of the magnetic correlation accompanied by appreciable spin fluctuations.

  12. SU (N ) spin-wave theory: Application to spin-orbital Mott insulators

    Science.gov (United States)

    Dong, Zhao-Yang; Wang, Wei; Li, Jian-Xin

    2018-05-01

    We present the application of the SU (N ) spin-wave theory to spin-orbital Mott insulators whose ground states exhibit magnetic orders. When taking both spin and orbital degrees of freedom into account rather than projecting Hilbert space onto the Kramers doublet, which is the lowest spin-orbital locked energy levels, the SU (N ) spin-wave theory should take the place of the SU (2 ) one due to the inevitable spin-orbital multipole exchange interactions. To implement the application, we introduce an efficient general local mean-field method, which involves all local fluctuations, and develop the SU (N ) linear spin-wave theory. Our approach is tested firstly by calculating the multipolar spin-wave spectra of the SU (4 ) antiferromagnetic model. Then, we apply it to spin-orbital Mott insulators. It is revealed that the Hund's coupling would influence the effectiveness of the isospin-1 /2 picture when the spin-orbital coupling is not large enough. We further carry out the SU (N ) spin-wave calculations of two materials, α -RuCl3 and Sr2IrO4 , and find that the magnonic and spin-orbital excitations are consistent with experiments.

  13. Theoretical modeling of diluted antiferromagnetic systems

    International Nuclear Information System (INIS)

    Pozo, J; Elgueta, R; Acevedo, R

    2000-01-01

    Some magnetic properties of a Diluted Antiferromagnetic System (DAFS) are studied. The model of the two sub-networks for antiferromagnetism is used and a Heisenberg Hamiltonian type is proposed, where the square operators are expressed in terms of boson operators with the approach of spin waves. The behavior of the diluted system's fundamental state depends basically on the competition effect between the anisotropy field and the Weiss molecular field. The approach used allows the diluted system to be worked for strong anisotropies as well as when these are very weak

  14. Mn induced ferromagnetism spin fluctuation enhancement in Sr{sub 2}Ru{sub 1−x}Mn{sub x}O{sub 4}

    Energy Technology Data Exchange (ETDEWEB)

    Zheng, Long; Cai, Jinzhu; Xie, Qiyun; Lv, Bin [Laboratory of Solid State Microstructures and Department of Physics, Nanjing University, Nanjing 210093 (China); Mao, Z.Q. [Department of Physics and Engineering Physics, Tulane University, New Orleans, LA 70118 (United States); Wu, X.S., E-mail: xswu@nju.edu.cn [Laboratory of Solid State Microstructures and Department of Physics, Nanjing University, Nanjing 210093 (China)

    2013-09-15

    We establish that Sr{sub 2}RuO{sub 4} is extremely close to incommensurate spin density wave instability. With increasing Mn content, the RuO{sub 6} octahedron in the unit cell varies. The octahedron of RuO{sub 6} contracts along c-axis for x<0.20, Mn element mainly showing the +3 chemical valence (Mn{sup 3+}), and it expands along c-axis with further increasing Mn content (x>0.20), and Mn element shows the +4 chemical valence (Mn{sup 4+}). Spin-glass-related ferromagnetism enhancement is observed for x>0.20, which indicates the critical ferromagnetic spin fluctuation due to Mn doping in Sr{sub 2}Ru{sub 1−x}Mn{sub x}O{sub 4}. - Highlights: • The chemical valence of Mn ions changed from Mn{sup 3+} to Mn{sup 4+} with the increase of Mn content. • Spin-glass-related ferromagnetism enhancement behavior is observed. • The electrical resistivity can be fitted using Mott's variable-range hopping model. • The evolution of octahedron with increase of Mn content is given. • The spin fluctuation effect plays an important role in the magnetic property.

  15. Detecting quantum critical points using bipartite fluctuations.

    Science.gov (United States)

    Rachel, Stephan; Laflorencie, Nicolas; Song, H Francis; Le Hur, Karyn

    2012-03-16

    We show that the concept of bipartite fluctuations F provides a very efficient tool to detect quantum phase transitions in strongly correlated systems. Using state-of-the-art numerical techniques complemented with analytical arguments, we investigate paradigmatic examples for both quantum spins and bosons. As compared to the von Neumann entanglement entropy, we observe that F allows us to find quantum critical points with much better accuracy in one dimension. We further demonstrate that F can be successfully applied to the detection of quantum criticality in higher dimensions with no prior knowledge of the universality class of the transition. Promising approaches to experimentally access fluctuations are discussed for quantum antiferromagnets and cold gases.

  16. Charge dynamics of the antiferromagnetically ordered Mott insulator

    International Nuclear Information System (INIS)

    Han, Xing-Jie; Li, Xin; Chen, Jing; Liao, Hai-Jun; Xiang, Tao; Liu, Yu; Liu, Zhi-Yuan; Xie, Zhi-Yuan; Normand, B

    2016-01-01

    We introduce a slave-fermion formulation in which to study the charge dynamics of the half-filled Hubbard model on the square lattice. In this description, the charge degrees of freedom are represented by fermionic holons and doublons and the Mott-insulating characteristics of the ground state are the consequence of holon–doublon bound-state formation. The bosonic spin degrees of freedom are described by the antiferromagnetic Heisenberg model, yielding long-ranged (Néel) magnetic order at zero temperature. Within this framework and in the self-consistent Born approximation, we perform systematic calculations of the average double occupancy, the electronic density of states, the spectral function and the optical conductivity. Qualitatively, our method reproduces the lower and upper Hubbard bands, the spectral-weight transfer into a coherent quasiparticle band at their lower edges and the renormalisation of the Mott gap, which is associated with holon–doublon binding, due to the interactions of both quasiparticle species with the magnons. The zeros of the Green function at the chemical potential give the Luttinger volume, the poles of the self-energy reflect the underlying quasiparticle dispersion with a spin-renormalised hopping parameter and the optical gap is directly related to the Mott gap. Quantitatively, the square-lattice Hubbard model is one of the best-characterised problems in correlated condensed matter and many numerical calculations, all with different strengths and weaknesses, exist with which to benchmark our approach. From the semi-quantitative accuracy of our results for all but the weakest interaction strengths, we conclude that a self-consistent treatment of the spin-fluctuation effects on the charge degrees of freedom captures all the essential physics of the antiferromagnetic Mott–Hubbard insulator. We remark in addition that an analytical approximation with these properties serves a vital function in developing a full understanding of

  17. Charge dynamics of the antiferromagnetically ordered Mott insulator

    Science.gov (United States)

    Han, Xing-Jie; Liu, Yu; Liu, Zhi-Yuan; Li, Xin; Chen, Jing; Liao, Hai-Jun; Xie, Zhi-Yuan; Normand, B.; Xiang, Tao

    2016-10-01

    We introduce a slave-fermion formulation in which to study the charge dynamics of the half-filled Hubbard model on the square lattice. In this description, the charge degrees of freedom are represented by fermionic holons and doublons and the Mott-insulating characteristics of the ground state are the consequence of holon-doublon bound-state formation. The bosonic spin degrees of freedom are described by the antiferromagnetic Heisenberg model, yielding long-ranged (Néel) magnetic order at zero temperature. Within this framework and in the self-consistent Born approximation, we perform systematic calculations of the average double occupancy, the electronic density of states, the spectral function and the optical conductivity. Qualitatively, our method reproduces the lower and upper Hubbard bands, the spectral-weight transfer into a coherent quasiparticle band at their lower edges and the renormalisation of the Mott gap, which is associated with holon-doublon binding, due to the interactions of both quasiparticle species with the magnons. The zeros of the Green function at the chemical potential give the Luttinger volume, the poles of the self-energy reflect the underlying quasiparticle dispersion with a spin-renormalised hopping parameter and the optical gap is directly related to the Mott gap. Quantitatively, the square-lattice Hubbard model is one of the best-characterised problems in correlated condensed matter and many numerical calculations, all with different strengths and weaknesses, exist with which to benchmark our approach. From the semi-quantitative accuracy of our results for all but the weakest interaction strengths, we conclude that a self-consistent treatment of the spin-fluctuation effects on the charge degrees of freedom captures all the essential physics of the antiferromagnetic Mott-Hubbard insulator. We remark in addition that an analytical approximation with these properties serves a vital function in developing a full understanding of the

  18. Temperature-dependent striped antiferromagnetism of LaFeAsO in a Green's function approach

    International Nuclear Information System (INIS)

    Liu Guibin; Liu Banggui

    2009-01-01

    We use a Green's function method to study the temperature-dependent average moment and magnetic phase-transition temperature of the striped antiferromagnetism of LaFeAsO, and other similar compounds, as the parents of FeAs-based superconductors. We consider the nearest and the next-nearest couplings in the FeAs layer, and the nearest coupling for inter-layer spin interaction. The dependence of the transition temperature T N and the zero-temperature average spin on the interaction constants is investigated. We obtain an analytical expression for T N and determine our temperature-dependent average spin from zero temperature to T N in terms of unified self-consistent equations. For LaFeAsO, we obtain a reasonable estimation of the coupling interactions with the experimental transition temperature T N = 138 K. Our results also show that a non-zero antiferromagnetic (AFM) inter-layer coupling is essential for the existence of a non-zero T N , and the many-body AFM fluctuations reduce substantially the low-temperature magnetic moment per Fe towards the experimental value. Our Green's function approach can be used for other FeAs-based parent compounds and these results should be useful to understand the physical properties of FeAs-based superconductors.

  19. Frozen concentration fluctuations in a poly(N-isopropyl acrylamide) gel studied by neutron spin echo and small-angle neutron scattering

    CERN Document Server

    Koizumi, S; Richter, D; Schwahn, D; Faragó, B; Annaka, M

    2002-01-01

    By employing neutron spin echo and small-angle neutron scattering, we determined the structure factor of the frozen concentration fluctuations on nano-length scales in a swollen poly(N-isopropyl acrylamide) gel. The frozen contribution, showing a plateau at the low scattering wavenumber q (0.02 A sup - sup 1), is intimately related to the abnormal butterfly scattering pattern appearing at low q under deformation. (orig.)

  20. Spins in the vortices of a high-temperature superconductor

    DEFF Research Database (Denmark)

    Lake, B.; Aeppli, G.; Clausen, K.N.

    2001-01-01

    Neutron scattering is used to characterize the magnetism of the vortices for the optimally doped high-temperature superconductor La2-xSrxCuO4 (x = 0.163) in an applied magnetic field. As temperature is reduced, Low-frequency spin fluctuations first disappear with the loss of vortex mobility......, but then reappear. We find that the vortex state can be regarded as an inhomogeneous mixture of a superconducting spin fluid and a material containing a nearly ordered antiferromagnet. These experiments show that as for many other properties of cuprate superconductors, the important underlying microscopic forces...

  1. Enhanced superconducting transition temperature in hyper-interlayer-expanded FeSe despite the suppressed electronic nematic order and spin fluctuations

    Science.gov (United States)

    Hrovat, Matevž Majcen; Jeglič, Peter; Klanjšek, Martin; Hatakeda, Takehiro; Noji, Takashi; Tanabe, Yoichi; Urata, Takahiro; Huynh, Khuong K.; Koike, Yoji; Tanigaki, Katsumi; Arčon, Denis

    2015-09-01

    The superconducting critical temperature, Tc, of FeSe can be dramatically enhanced by intercalation of a molecular spacer layer. Here we report on a 77Se,7Li , and 1H nuclear magnetic resonance (NMR) study of the powdered hyper-interlayer-expanded Lix(C2H8N2) yFe2 -zSe2 with a nearly optimal Tc=45 K. The absence of any shift in the 7Li and 1H NMR spectra indicates a complete decoupling of interlayer units from the conduction electrons in FeSe layers, whereas nearly temperature-independent 7Li and 1H spin-lattice relaxation rates are consistent with the non-negligible concentration of Fe impurities present in the insulating interlayer space. On the other hand, the strong temperature dependence of 77Se NMR shift and spin-lattice relaxation rate, 1 /77T1 , is attributed to the holelike bands close to the Fermi energy. 1 /77T1 shows no additional anisotropy that would account for the onset of electronic nematic order down to Tc. Similarly, no enhancement in 1 /77T1 due to the spin fluctuations could be found in the normal state. Yet, a characteristic power-law dependence 1 /77T1∝T4.5 still complies with the Cooper pairing mediated by spin fluctuations.

  2. Singlet ground-state fluctuations in praseodymium observed by muon spin relaxation in PrP and PrP0.9

    International Nuclear Information System (INIS)

    Noakes, D R; Waeppling, R; Kalvius, G M; Jr, M F White; Stronach, C E

    2005-01-01

    Muon spin relaxation (μSR) in the singlet ground-state compounds PrP and PrP 0.9 reveals the unusual situation of a Lorentzian local field distribution with fast-fluctuation-limit strong-collision dynamics, a case that does not show motional narrowing. Contrary to publications by others, where PrP 0.9 was asserted to have vacancy-induced spin-glass freezing, no spin-glass freezing is seen in PrP 0.9 or PrP down to ≤100mK. This was confirmed by magnetization measurements on these same samples. In both compounds, the muon spin relaxation rate does increase as temperature decreases, demonstrating increasing strength of the paramagnetic response. A Monte Carlo model of fluctuations of Pr ions out of their crystalline-electric-field singlet ground states into their magnetic excited states (and back down again) produces the strong-collision-dynamic Lorentzian relaxation functions observed at each individual temperature but not the observed temperature dependence. This model contains no exchange interaction, and so predicts decreasing paramagnetic response as the temperature decreases, contrary to the temperature dependence observed. Comparison of the simulations to the data suggests that the exchange interaction is causing the system to approach magnetic freezing (by mode softening), but fails to complete the process

  3. Anti-ferromagnetic Heisenberg model on bilayer honeycomb

    International Nuclear Information System (INIS)

    Shoja, M.; Shahbazi, F.

    2012-01-01

    Recent experiment on spin-3/2 bilayer honeycomb lattice antiferromagnet Bi 3 Mn 4 O 12 (NO 3 ) shows a spin liquid behavior down to very low temperatures. This behavior can be ascribed to the frustration effect due to competitions between first and second nearest neighbour's antiferromagnet interaction. Motivated by the experiment, we study J 1 -J 2 Antiferromagnet Heisenberg model, using Mean field Theory. This calculation shows highly degenerate ground state. We also calculate the effect of second nearest neighbor through z direction and show these neighbors also increase frustration in these systems. Because of these degenerate ground state in these systems, spins can't find any ground state to be freeze in low temperatures. This behavior shows a novel spin liquid state down to very low temperatures.

  4. Effect of Dzyaloshinskii-Moriya on Magnetic orders of J_1-J_2 Antiferromagnetic Heisenberg model

    Directory of Open Access Journals (Sweden)

    Fariba Masoudi

    2017-11-01

    Full Text Available Motivated by recent experiments that detects Dzyaloshinskii-Moriya (DM interaction in , we study the effects of DM interaction on magnetic orders of J1-J2 antiferromagnetic Heisenberg model. First, we find the classical phase diagram of the model using Luttinger-Tisza approximation. In this approximation, the classical phase diagram has two phases. For , the model has canted Neel and DM interaction cants the spins of one on the subluttices. The ground state of model is classically degenerate for , including infinit numbers of vorticity vectors that are able to minimize the model. This phase is important because of the probability of the existence of quantum spin liquid in this region. To investigate the effect of quantum fluctuation on the stability of the classical phase diagram, linear spin wave theory of  Holstein-Primakoff is used. The results show that in the classical degeneracy regime, the quantum fluctuations for  cause spiral order in this region. The ground state of model remains disorder for, and this region is a good place for finding quantum spin liquid

  5. Antiferromagnetic transition in graphene functionalized with nitroaniline

    Science.gov (United States)

    Komlev, Anton A.; Makarova, Tatiana L.; Lahderanta, Erkki; Semenikhin, Petr Valeryevich; Veinger, Anatoly I.; Kochman, Igor V.; Magnani, Giacomo; Bertoni, Giovanni; Pontiroli, Daniele; Ricco, Mauro

    2017-07-01

    Magnetic properties of graphene nanostructures functionalized with aromatic radicals were investigated by electron spin resonance (ESR) and superconducting quantum interference device (SQUID) techniques. Three types of functionalized graphene samples were investigated (functionalization was performed by 4-bromoaniline, 4-nitroaniline, or 4-chloroaniline). According to SQUID measurements, in case of functionalization by nitroaniline, sharp change in temperature dependence of magnetic susceptibility was observed near 120 K. Such behavior was explained as antiferromagnetic ordering. The same but more extended effect was observed in ESR measurements below 160 K. In the ESR measurements, only one resonance line with g-factor equal to 2.003 was observed. Based on the temperature dependencies of spin concentration and resonance position and intensity, the effect was explained as antiferromagnetic ordering along the extended defects on the basal planes of the graphene.

  6. Entanglement in a Dimerized Antiferromagnetic Heisenberg Chain

    OpenAIRE

    Hao, Xiang; Zhu, Shiqun

    2008-01-01

    The entanglement properties in an antiferromagnetic dimerized Heisenberg spin-1/2 chain are investigated. The entanglement gap, which is the difference between the ground-state energy and the minimal energy that any separable state can attain, is calculated to detect the entanglement. It is found that the entanglement gap can be increased by varying the alternation parameter. Through thermal energy, the witness of the entanglement can determine a characteristic temperature below that an entan...

  7. Robustness of dynamic magnetism in the triangle-based antiferromagnets Ba3Ru1- x Ir x Ti2O9 ( x = 0.5 and 0.8)

    Science.gov (United States)

    Lee, W.-J.; Do, S.-H.; Lee, S.; Choi, Y.-S.; Choi, K.-Y.; Yoon, Sungwon; Suh, Byoungjin; Jang, Zeehoon

    2018-01-01

    We report on the spin dynamics of the strong spin-orbit coupled antiferromagnets Ba3Ru1- x Ir x Ti2O9 ( x = 0.5 and 0.8), which comprise a mixture of edge- and corner-sharing triangles. Muon spin-relaxation measurements give no hints of long-range magnetic order down to 25 mK. Rather, the muon spin-relaxation rates λ( T) show persistent spin dynamics below 1 K, indicating that fast fluctuations are dominant in spite of Ir4+( J eff = 1/2)/Ru4+( S = 1) randomness. The muon spin depolarization of both compounds is well described by a stretched exponential function with the stretching exponent β = 0.4 (0.6) for x = 0.5 (0.8) at low temperatures, which is larger than β = 1/3 expected for a spin glass. Our results suggest that randomness in the spin number and the exchange interaction induces a partial spin freezing, but the majority of spins remain dynamically fluctuating.

  8. Narrow and broad solitons in the antiferromagnetic chains of CsCoCl3 and TMMC

    International Nuclear Information System (INIS)

    Boucher, J.P.; Regnault, L.P.; Pires, A.; Rossat-Mignod, J.; Henry, Y.; Bouillot, J.; Stirling, W.G.; Renard, J.P.

    1984-06-01

    The two quasi one-dimensional (1D) compounds CsCoCl 3 and (CH 3 ) 4 NMnCl 3 (TMMC) are almost ideal systems in which to study soliton excitations. Both they have antiferromagnetic (AF) couplings in the chains and at low temperature they exhibit an Ising symmetry favourable for the occurence of solitons. This symmetry is an intrinsic property of CsCoCl 3 while in TMMC it is only achieved by the application of an external magnetic field H perpendicular to the chains. In the lD short range order regime two energetically equivalent configurations are expected for the spins. Solitons can be seen as Bloch walls separating ordered domains and allowing the spins to pass from one configuration to the other. In the case of a ''strong'' Ising symmetry (CsCoCl 3 ) the walls are reduced to one lattice unit (''narrow'' solitons) while in the case of a ''weak'' Ising symmetry (TMMC) the walls extend over several lattice units (10 to 30) (''broad'' solitons). To maintain a paramagnetic state, these walls move rapidly along the chains inducing characteristic fluctuations. The investigation of these two compounds, CsCoCl 3 and TMMC illustrates the advantage of antiferromagnets as the AF mode yields an accurate determination of the soliton regime. Narrow and broad solitons are observed to behave very similarly

  9. The case for spin-fluctuation induced pairing in Ba{sub 1-x}K{sub x}Fe{sub 2}As{sub 2}

    Energy Technology Data Exchange (ETDEWEB)

    Boehm, Thomas U.

    2017-03-07

    The microscopic mechanism and the experimental identification of unconventional superconductivity is one of the most vexing problems of contemporary condensed matter physics. Raman spectroscopy provides a new avenue for this quest by accessing the hierarchy of superconducting pairing propensities. The doping-dependent study of competing pairing channels in Ba{sub 1-x}K{sub x}Fe{sub 2}As{sub 2} for 0.22 ≤ x ≤ 0.70 is one of the main aspects of this thesis. The observations demonstrate the importance of spin fluctuations for Cooper pairing.

  10. Long range order in the ground state of two-dimensional antiferromagnets

    International Nuclear Information System (INIS)

    Neves, E.J.; Perez, J.F.

    1985-01-01

    The existence of long range order is shown in the ground state of the two-dimensional isotropic Heisenberg antiferromagnet for S >= 3/2. The method yields also long range order for the ground state of a larger class of anisotropic quantum antiferromagnetic spin systems with or without transverse magnetic fields. (Author) [pt

  11. Weyl magnons in breathing pyrochlore antiferromagnets

    Science.gov (United States)

    Li, Fei-Ye; Li, Yao-Dong; Kim, Yong Baek; Balents, Leon; Yu, Yue; Chen, Gang

    2016-01-01

    Frustrated quantum magnets not only provide exotic ground states and unusual magnetic structures, but also support unconventional excitations in many cases. Using a physically relevant spin model for a breathing pyrochlore lattice, we discuss the presence of topological linear band crossings of magnons in antiferromagnets. These are the analogues of Weyl fermions in electronic systems, which we dub Weyl magnons. The bulk Weyl magnon implies the presence of chiral magnon surface states forming arcs at finite energy. We argue that such antiferromagnets present a unique example, in which Weyl points can be manipulated in situ in the laboratory by applied fields. We discuss their appearance specifically in the breathing pyrochlore lattice, and give some general discussion of conditions to find Weyl magnons, and how they may be probed experimentally. Our work may inspire a re-examination of the magnetic excitations in many magnetically ordered systems. PMID:27650053

  12. Nanoparticles of antiferromagnetic materials

    DEFF Research Database (Denmark)

    Madsen, Daniel Esmarch

    2008-01-01

    I denne Ph.D. afhandling studeres forskellige egenskaber ved antiferromagnetiske nanopartikler. I en ideel antiferromagnet er spinnene orienteret således at der ikke er et resulterende magnetisk moment. I nanopartikler af antiferromagnetiske materialer er denne kompensation på grund af forskellig...

  13. Prospect for antiferromagnetic spintronics

    Czech Academy of Sciences Publication Activity Database

    Martí, Xavier; Fina, I.; Jungwirth, Tomáš

    2015-01-01

    Roč. 51, č. 4 (2015), s. 2900104 ISSN 0018-9464 R&D Projects: GA MŠk(CZ) LM2011026; GA ČR GB14-37427G EU Projects: European Commission(XE) 268066 - 0MSPIN Institutional support: RVO:68378271 Keywords : spintronics * antiferromagnets Subject RIV: BM - Solid Matter Physics ; Magnetism Impact factor: 1.277, year: 2015

  14. Adiabatic physics of an exchange-coupled spin-dimer system: Magnetocaloric effect, zero-point fluctuations, and possible two-dimensional universal behavior

    International Nuclear Information System (INIS)

    Brambleby, J.; Goddard, P. A.; Singleton, John; Jaime, Marcelo; Lancaster, T.

    2017-01-01

    We present the magnetic and thermal properties of the bosonic-superfluid phase in a spin-dimer network using both quasistatic and rapidly changing pulsed magnetic fields. The entropy derived from a heat-capacity study reveals that the pulsed-field measurements are strongly adiabatic in nature and are responsible for the onset of a significant magnetocaloric effect (MCE). In contrast to previous predictions we show that the MCE is not just confined to the critical regions, but occurs for all fields greater than zero at sufficiently low temperatures. We explain the MCE using a model of the thermal occupation of exchange-coupled dimer spin states and highlight that failure to take this effect into account inevitably leads to incorrect interpretations of experimental results. In addition, the heat capacity in our material is suggestive of an extraordinary contribution from zero-point fluctuations and appears to indicate universal behavior with different critical exponents at the two field-induced critical points. Finally, the data at the upper critical point, combined with the layered structure of the system, are consistent with a two-dimensional nature of spin excitations in the system.

  15. Topological term of the antiferromagnetic Heisenberg model in 2+1 dimension

    International Nuclear Information System (INIS)

    Wu Ke; Yu Lu; Zhu Chuanjie

    1988-05-01

    It is shown in this note that the two different ways of introducing the topological term in the discussion of the spin 1/2 antiferromagnetic Heisenberg model are identical to each other. (author). 12 refs

  16. Electron-phonon and spin-phonon coupling in NaV2O5 : Charge fluctuations effects

    NARCIS (Netherlands)

    Sherman, E.Ya.; Fischer, M.; Lemmens, P; Loosdrecht, P.H.M. van; Güntherodt, G.

    1999-01-01

    We show that the asymmetric crystal environment of the V site in the ladder compound NaV2O5 leads to a strong coupling of vanadium 3d electrons to phonons. This coupling causes fluctuations of the charge on the V ions, and favors a transition to a charge-ordered state at low temperatures. In the low

  17. Kinetically Inhibited Order in a Diamond-Lattice Antiferromagnet

    International Nuclear Information System (INIS)

    MacDougall, Gregory J.; Gout, Delphine J.; Zarestky, Jerel L.; Ehlers, Georg; Podlesnyak, Andrey A.; McGuire, Michael A.; Mandrus, David; Nagler, Stephen E.

    2011-01-01

    Frustrated magnetic systems exhibit highly degenerate ground states and strong fluctuations, often leading to new physics. An intriguing example of current interest is the antiferromagnet on a diamond lattice, realized physically in the A-site spinel materials. This is a prototypical system in three dimensions where frustration arises from competing interactions rather than purely geometric constraints, and theory suggests the possibility of novel order at low temperature. Here we present a comprehensive single crystal neutron scattering study CoAl2O4, a highly frustrated A-site spinel. We observe strong diffuse scattering that peaks at wavevectors associated with Neel ordering. Below the temperature T*=6.5K, there is a dramatic change in elastic scattering lineshape accompanied by the emergence of well-defined spin-wave excitations. T* had previously been associated with the onset of glassy behavior. Our new results suggest instead that in fact T* signifies a first-order phase transition, but with true long-range order inhibited by the kinetic freezing of domain walls. This scenario might be expected to occur widely in frustrated systems containing first-order phase transitions and is a natural explanation for existing reports of anomalous glassy behavior in other materials.

  18. Spin currents and magnon dynamics in insulating magnets

    Science.gov (United States)

    Nakata, Kouki; Simon, Pascal; Loss, Daniel

    2017-03-01

    Nambu-Goldstone theorem provides gapless modes to both relativistic and nonrelativistic systems. The Nambu-Goldstone bosons in insulating magnets are called magnons or spin-waves and play a key role in magnetization transport. We review here our past works on magnetization transport in insulating magnets and also add new insights, with a particular focus on magnon transport. We summarize in detail the magnon counterparts of electron transport, such as the Wiedemann-Franz law, the Onsager reciprocal relation between the Seebeck and Peltier coefficients, the Hall effects, the superconducting state, the Josephson effects, and the persistent quantized current in a ring to list a few. Focusing on the electromagnetism of moving magnons, i.e. magnetic dipoles, we theoretically propose a way to directly measure magnon currents. As a consequence of the Mermin-Wagner-Hohenberg theorem, spin transport is drastically altered in one-dimensional antiferromagnetic (AF) spin-1/2 chains; where the Néel order is destroyed by quantum fluctuations and a quasiparticle magnon-like picture breaks down. Instead, the low-energy collective excitations of the AF spin chain are described by a Tomonaga-Luttinger liquid (TLL) which provides the spin transport properties in such antiferromagnets some universal features at low enough temperature. Finally, we enumerate open issues and provide a platform to discuss the future directions of magnonics.

  19. Spin currents and magnon dynamics in insulating magnets

    International Nuclear Information System (INIS)

    Nakata, Kouki; Loss, Daniel; Simon, Pascal

    2017-01-01

    Nambu–Goldstone theorem provides gapless modes to both relativistic and nonrelativistic systems. The Nambu–Goldstone bosons in insulating magnets are called magnons or spin-waves and play a key role in magnetization transport. We review here our past works on magnetization transport in insulating magnets and also add new insights, with a particular focus on magnon transport. We summarize in detail the magnon counterparts of electron transport, such as the Wiedemann–Franz law, the Onsager reciprocal relation between the Seebeck and Peltier coefficients, the Hall effects, the superconducting state, the Josephson effects, and the persistent quantized current in a ring to list a few. Focusing on the electromagnetism of moving magnons, i.e. magnetic dipoles, we theoretically propose a way to directly measure magnon currents. As a consequence of the Mermin–Wagner–Hohenberg theorem, spin transport is drastically altered in one-dimensional antiferromagnetic (AF) spin-1/2 chains; where the Néel order is destroyed by quantum fluctuations and a quasiparticle magnon-like picture breaks down. Instead, the low-energy collective excitations of the AF spin chain are described by a Tomonaga–Luttinger liquid (TLL) which provides the spin transport properties in such antiferromagnets some universal features at low enough temperature. Finally, we enumerate open issues and provide a platform to discuss the future directions of magnonics. (paper)

  20. Spin Transport in Ferromagnetic and Antiferromagnetic Textures

    KAUST Repository

    Akosa, Collins Ashu

    2016-01-01

    in this thesis, the current-driven velocity of magnetic textures is related to the ratio between the so-called non-adiabatic torque and magnetic damping. Uncovering the physics underlying these phenomena can lead to the optimal design of magnetic systems

  1. Spin-polarized current in noncollinear antiferromagnets

    Czech Academy of Sciences Publication Activity Database

    Železný, Jakub; Zhang, Y.; Felser, C.; Yan, B.

    2017-01-01

    Roč. 119, č. 18 (2017), s. 1-7, č. článku 187204. ISSN 0031-9007 Institutional support: RVO:68378271 Keywords : anisotropic magnetoresistance * wannier functions * room-temperature * torques * spintronics Subject RIV: BM - Solid Matter Physics ; Magnetism OBOR OECD: Condensed matter physics (including formerly solid state physics, supercond.) Impact factor: 8.462, year: 2016

  2. Observation of Antiferromagnetic Resonance in an Organic Superconductor

    DEFF Research Database (Denmark)

    Torrance, J. B.; Pedersen, H. J.; Bechgaard, K.

    1982-01-01

    Anomalous microwave absorption has been observed in the organic superconductor TMTSF2AsF6 (TMTSF: tetramethyltetraselenafulvalene) below its metal-nonmetal transition near 12 K. This absorption is unambiguously identified as antiferromagnetic resonance by the excellent agreement between a spin...

  3. Ferro- and antiferro-magnetism in (Np, Pu)BC

    Czech Academy of Sciences Publication Activity Database

    Klimczuk, T.; Shick, Alexander; Kozub, Agnieszka L.; Griveau, J.C.; Colineau, E.; Falmbigl, M.; Wastin, F.; Rogl, P.

    2015-01-01

    Roč. 3, č. 4 (2015), "041803-1"-"041803-9" ISSN 2166-532X R&D Projects: GA ČR GA15-07172S Institutional support: RVO:68378271 Keywords : ferromagetism * antiferromagnetism * magnetic anisotropy * strong electron correlations * spin-orbit coupling Subject RIV: BM - Solid Matter Physics ; Magnetism Impact factor: 4.323, year: 2015

  4. Spin and isospin fluctuations in heavy ion collisions and their dependence upon the shape of the dinuclear complex

    Energy Technology Data Exchange (ETDEWEB)

    Moretto, L.G.

    1980-08-01

    The relevance of higher multipoles of giant isovector modes in the charge distribution of deep inelastic fragments is discussed and found to depend strongly on mass asymmetry. The sources of angular momentum fluctuations are investigated. Quantal effects are considered as well as effects arising from non-equilibrium and equilibrium statistical fluctuations. A model based upon equilibrium statistical mechanics is considered in detail, and used to predict both 2nd moments of the angular momentum distributions and the angular momentum misalignment. Analytical expressions are derived to calculate the angular distributions of sequentially emitted particles, fission fragments, as well as gamma rays in terms of the angular momentum misalignment. Recent data on the angular distributions of sequential alphas, fission and gamma rays are analyzed in terms of the model. 29 figures, 1 table.

  5. Spin and isospin fluctuations in heavy ion collisions and their dependence upon the shape of the dinuclear complex

    International Nuclear Information System (INIS)

    Moretto, L.G.

    1980-08-01

    The relevance of higher multipoles of giant isovector modes in the charge distribution of deep inelastic fragments is discussed and found to depend strongly on mass asymmetry. The sources of angular momentum fluctuations are investigated. Quantal effects are considered as well as effects arising from non-equilibrium and equilibrium statistical fluctuations. A model based upon equilibrium statistical mechanics is considered in detail, and used to predict both 2nd moments of the angular momentum distributions and the angular momentum misalignment. Analytical expressions are derived to calculate the angular distributions of sequentially emitted particles, fission fragments, as well as gamma rays in terms of the angular momentum misalignment. Recent data on the angular distributions of sequential alphas, fission and gamma rays are analyzed in terms of the model. 29 figures, 1 table

  6. Superfluid and antiferromagnetic phases in ultracold fermionic quantum gases

    International Nuclear Information System (INIS)

    Gottwald, Tobias

    2010-01-01

    domain wall formation, antiferromagnetically induced density shifts, and we show the relevant role of spin-imbalance for antiferromagnetic states. Since the first step for understanding the physics of the examined models was the application of a mean field approximation, we analyze the effect of including the second order terms of the weak coupling perturbation expansion for the repulsive model. We show that our results survive the influence of quantum fluctuations and show that the renormalization factors for order parameters and critical temperatures lead to a weaker influence of the fluctuations on the results in finite sized systems than on the results in the thermodynamical limit. Furthermore, in the context of second order theory we address the question whether results obtained in the dynamical mean field theory (DMFT), which is meanwhile a frequently used method for describing trapped systems, survive the effect of the non-local Feynman diagrams neglected in DMFT. (orig.)

  7. Superfluid and antiferromagnetic phases in ultracold fermionic quantum gases

    Energy Technology Data Exchange (ETDEWEB)

    Gottwald, Tobias

    2010-08-27

    domain wall formation, antiferromagnetically induced density shifts, and we show the relevant role of spin-imbalance for antiferromagnetic states. Since the first step for understanding the physics of the examined models was the application of a mean field approximation, we analyze the effect of including the second order terms of the weak coupling perturbation expansion for the repulsive model. We show that our results survive the influence of quantum fluctuations and show that the renormalization factors for order parameters and critical temperatures lead to a weaker influence of the fluctuations on the results in finite sized systems than on the results in the thermodynamical limit. Furthermore, in the context of second order theory we address the question whether results obtained in the dynamical mean field theory (DMFT), which is meanwhile a frequently used method for describing trapped systems, survive the effect of the non-local Feynman diagrams neglected in DMFT. (orig.)

  8. Concepts of antiferromagnetic spintronics

    Czech Academy of Sciences Publication Activity Database

    Gomonay, O.; Jungwirth, Tomáš; Sinova, Jairo

    2017-01-01

    Roč. 11, č. 4 (2017), 1-8, č. článku 1700022. ISSN 1862-6254 R&D Projects: GA MŠk LM2015087; GA ČR GB14-37427G Institutional support: RVO:68378271 Keywords : spintronics * antiferromagnets Subject RIV: BM - Solid Matter Physics ; Magnetism OBOR OECD: Condensed matter physics (including formerly solid state physics, supercond.) Impact factor: 3.032, year: 2016

  9. Roles of spin fluctuation and frustration in the superconductivity of β-(BDA-TTP)2X (X=SbF6,AsF6) under uniaxial compression

    Science.gov (United States)

    Ito, Hiroshi; Ishihara, Tetsuo; Tanaka, Hisaaki; Kuroda, Shin-Ichi; Suzuki, Takeo; Onari, Seiichiro; Tanaka, Yukio; Yamada, Jun-Ichi; Kikuchi, Koichi

    2008-11-01

    β -type BDA-TTP [ BDA-TTP=2,5 -bis(1,3-dithian-2-ylidene)-1,3,4,6-tetrathiapentalene] salts possess high transition temperatures TC reaching 7 K among organic superconductors. TC of β-(BDA-TTP)2X (X=SbF6,AsF6) is studied by resistive measurements under uniaxial compression. TC once increases and takes a maximum under compression parallel to the donor stack while it decreases under compression perpendicular to the donor stack. These results are in agreement with the half-filled Hubbard model on the triangular lattice in which the compression controls the spin fluctuation and frustration in the weak pressure region.

  10. Electronic structure, superconductivity, and spin fluctuations in the A15 compounds A3B: A = V, Nb; B = Ir,Pt,Au

    International Nuclear Information System (INIS)

    Jarlborg, T.; Junod, A.; Peter, M.

    1983-01-01

    The electronic structure of six A15 compounds V 3 Ir, V 3 Pt, V 3 Au, Nb 3 Ir, Nb 3 Pt, and Nb 3 Au has been determined by means of self-consistent semirelativistic linear muffin-tin orbital band calculations. Parameters related to superconductivity such as electron-phonon coupling, transition temperature, electronic specific heat, and magnetic exchange enhancement are derived from the electronic-structure results. Generally the results obtained agree well with experimental values, with the exception of Nb 3 Pt and V 3 Au. In the former compound the density of states (DOS) has a sharp increase at E/sub F/ making the exact DOS value uncertain. In V 3 Au the high calculated T/sub c/ and the Stoner factor indicate that spin fluctuations may be limiting the T/sub c/. .AE

  11. Analytic evidence of the equivalence of the alternating Heisenberg spin chain to the mixed spin (1, 1/2) Heisenberg chain

    International Nuclear Information System (INIS)

    Jiang Jianjun; Liu Yongjun; Tang Fei; Yang Cuihong

    2011-01-01

    We investigated the properties of the spin-1/2 ferromagnetic-antiferromagnetic-antiferromagnetic alternating Heisenberg chain using the spin-wave theory. The spin-wave excitation spectra, the sublattice magnetizations and the local bond energies of the model are calculated to be compared with the corresponding properties of the mixed spin (1, 1/2) chain for a range of α. The results demonstrate that all the properties show similar behaviours in the small α limit, so the properties of the mixed spin (1, 1/2) chain can be described using the spin-1/2 ferromagnetic-antiferromagnetic-antiferromagnetic alternating Heisenberg chain. -- Research Highlights: →The spin-wave excitation spectra, the sublattice magnetizations and the local bond energies of the spin-1/2 ferromagnetic-antiferromagnetic-antiferromagnetic alternating Heisenberg chain are calculated. →In the small α limit, the properties of the mixed spin (1,1/2) chain can be described using the spin-1/2 ferromagnetic-antiferromagnetic-antiferromagnetic alternating Heisenberg chain. →The spin-1/2 ferromagnetic-antiferromagnetic-antiferromagnetic alternating Heisenberg chain may be of interest for some real quasi-one-dimensional molecular magnetic materials.

  12. Isothermal anisotropic magnetoresistance in antiferromagnetic metallic IrMn.

    Science.gov (United States)

    Galceran, R; Fina, I; Cisneros-Fernández, J; Bozzo, B; Frontera, C; López-Mir, L; Deniz, H; Park, K-W; Park, B-G; Balcells, Ll; Martí, X; Jungwirth, T; Martínez, B

    2016-10-20

    Antiferromagnetic spintronics is an emerging field; antiferromagnets can improve the functionalities of ferromagnets with higher response times, and having the information shielded against external magnetic field. Moreover, a large list of aniferromagnetic semiconductors and metals with Néel temperatures above room temperature exists. In the present manuscript, we persevere in the quest for the limits of how large can anisotropic magnetoresistance be in antiferromagnetic materials with very large spin-orbit coupling. We selected IrMn as a prime example of first-class moment (Mn) and spin-orbit (Ir) combination. Isothermal magnetotransport measurements in an antiferromagnetic-metal(IrMn)/ferromagnetic-insulator thin film bilayer have been performed. The metal/insulator structure with magnetic coupling between both layers allows the measurement of the modulation of the transport properties exclusively in the antiferromagnetic layer. Anisotropic magnetoresistance as large as 0.15% has been found, which is much larger than that for a bare IrMn layer. Interestingly, it has been observed that anisotropic magnetoresistance is strongly influenced by the field cooling conditions, signaling the dependence of the found response on the formation of domains at the magnetic ordering temperature.

  13. Thermoelectric properties of layered antiferromagnetic CuCrSe2

    International Nuclear Information System (INIS)

    Tewari, Girish C.; Tripathi, T.S.; Yamauchi, Hisao; Karppinen, Maarit

    2014-01-01

    Here we study thermoelectric and magnetic properties of CuCrSe 2 samples sintered at various temperatures. Structural analysis with XRD shows an order-disorder transition for Cr atoms when the sintering temperature is increased above 1273 K. Metal-like electrical resistivity and anomalously large Seebeck coefficient are found about room temperature. Analysis of electrical conductivity and Seebeck coefficient of the partially-disordered phase suggests hopping conduction of charge carriers. For both the ordered and disordered phases magnetic susceptibility follows Curie–Weiss temperature dependence at high temperatures above 150 K and shows an antiferromagnetic transition around 55 K. For the disordered phase, the effective magnetic moment is determined at 3.62 μ B ; this low value in comparison to the spin only value for Cr 3+ of 3.89 μ B indicates spin fluctuations in the paramagnetic state. The thermal conductivity in these phases is low and dominated by the lattice contribution. Values for the thermoelectric figure of merit (ZT) at room temperature are estimated to be 0.17 and 0.05 for the ordered and disordered phases, respectively. - Highlights: • Thermoelectric and magnetic properties of CuCrSe 2 samples are investigated. • The properties strongly depend on the degree of order of chromium atoms. • The degree of order is controlled by the sintering temperature. • Room-temperature figure of merit is estimated at 0.17 for the ordered phase. • For the disordered phase the figure of merit is lower

  14. Exact mapping of the dx2-y2 Cooper-pair wavefunction onto the spin fluctuations in cuprates: the Fermi surface as a driver for 'high Tc' superconductivity

    International Nuclear Information System (INIS)

    McDonald, Ross D; Harrison, Neil; Singleton, John

    2009-01-01

    We propose that the extraordinarily high superconducting transition temperatures in the cuprates are driven by an exact mapping of the d x 2 -y 2 Cooper-pair wavefunction onto the incommensurate spin fluctuations observed in neutron-scattering experiments. This is manifested in the direct correspondence between the inverse of the incommensurability factor δ seen in inelastic neutron-scattering experiments and the measured superconducting coherence length ξ 0 . Strikingly, the relationship between ξ 0 and δ is valid for both La 2-x Sr x CuO 4 and YBa 2 Cu 3 O 7-x , suggesting a common mechanism for superconductivity across the entire hole-doped cuprate family. Using data from recent quantum-oscillation experiments in the cuprates, we propose that the fluctuations responsible for superconductivity are driven by a Fermi-surface instability. On the basis of these findings, one can specify the optimal characteristics of a solid that will exhibit 'high T c ' superconductivity. (fast track communication)

  15. Quasistatic antiferromagnetism in the quantum wells of SmTiO3/SrTiO3 heterostructures

    Science.gov (United States)

    Need, Ryan F.; Marshall, Patrick B.; Kenney, Eric; Suter, Andreas; Prokscha, Thomas; Salman, Zaher; Kirby, Brian J.; Stemmer, Susanne; Graf, Michael J.; Wilson, Stephen D.

    2018-03-01

    High carrier density quantum wells embedded within a Mott insulating matrix present a rich arena for exploring unconventional electronic phase behavior ranging from non-Fermi-liquid transport and signatures of quantum criticality to pseudogap formation. Probing the proposed connection between unconventional magnetotransport and incipient electronic order within these quantum wells has however remained an enduring challenge due to the ultra-thin layer thicknesses required. Here we address this challenge by exploring the magnetic properties of high-density SrTiO3 quantum wells embedded within the antiferromagnetic Mott insulator SmTiO3 via muon spin relaxation and polarized neutron reflectometry measurements. The one electron per planar unit cell acquired by the nominal d0 band insulator SrTiO3 when embedded within a d1 Mott SmTiO3 matrix exhibits slow magnetic fluctuations that begin to freeze into a quasistatic spin state below a critical temperature T*. The appearance of this quasistatic well magnetism coincides with the previously reported opening of a pseudogap in the tunneling spectra of high carrier density wells inside this film architecture. Our data suggest a common origin of the pseudogap phase behavior in this quantum critical oxide heterostructure with those observed in bulk Mott materials close to an antiferromagnetic instability.

  16. Relativistic Néel-Order Fields Induced by Electrical Current in Antiferromagnets

    KAUST Repository

    Železný, J.

    2014-10-06

    We predict that a lateral electrical current in antiferromagnets can induce nonequilibrium Néel-order fields, i.e., fields whose sign alternates between the spin sublattices, which can trigger ultrafast spin-axis reorientation. Based on microscopic transport theory calculations we identify staggered current-induced fields analogous to the intraband and to the intrinsic interband spin-orbit fields previously reported in ferromagnets with a broken inversion-symmetry crystal. To illustrate their rich physics and utility, we consider bulk Mn2Au with the two spin sublattices forming inversion partners, and a 2D square-lattice antiferromagnet with broken structural inversion symmetry modeled by a Rashba spin-orbit coupling. We propose an antiferromagnetic memory device with electrical writing and reading.

  17. Relativistic Néel-Order Fields Induced by Electrical Current in Antiferromagnets

    KAUST Repository

    Železný , J.; Gao, H.; Vý borný , K.; Zemen, J.; Mašek, J.; Manchon, Aurelien; Wunderlich, J.; Sinova, Jairo; Jungwirth, T.

    2014-01-01

    We predict that a lateral electrical current in antiferromagnets can induce nonequilibrium Néel-order fields, i.e., fields whose sign alternates between the spin sublattices, which can trigger ultrafast spin-axis reorientation. Based on microscopic transport theory calculations we identify staggered current-induced fields analogous to the intraband and to the intrinsic interband spin-orbit fields previously reported in ferromagnets with a broken inversion-symmetry crystal. To illustrate their rich physics and utility, we consider bulk Mn2Au with the two spin sublattices forming inversion partners, and a 2D square-lattice antiferromagnet with broken structural inversion symmetry modeled by a Rashba spin-orbit coupling. We propose an antiferromagnetic memory device with electrical writing and reading.

  18. Can one observe by μ SR the transition from uncorrelated to correlated spin fluctuations? Example: Nd1.4Ce0.2Sr0.4CuO4-δ

    International Nuclear Information System (INIS)

    Pinkpank, M.; Amato, A.; Gygax, F.N.; Schenck, A.; Henggeler, W.; Fischer, P.

    1997-01-01

    μSR-measurements in ZF and LF on Nd 1.4 Ce 0.2 Sr 0.4 CuO 4-δ show a sharp increase of the depolarisation rate (λ) below ∼ 2K. This increase can be explained by the transition from uncorrelated to correlated spin fluctuations, which is in agreement with results obtained by neutron scattering

  19. Impurity-induced staggered polarization and antiferromagnetic order in spin-12 Heisenberg two-leg ladder compound SrCu2O3: Extensive Cu NMR and NQR studies

    Science.gov (United States)

    Ohsugi, S.; Tokunaga, Y.; Ishida, K.; Kitaoka, Y.; Azuma, M.; Fujishiro, Y.; Takano, M.

    1999-08-01

    We report characteristics of impurity-induced staggered polarization (IISP) and antiferromagnetic long-range order (AF-LRO) in the gapped spin-1/2 Heisenberg two-leg ladder compound SrCu2O3 (Sr123). We have carried out comprehensive NMR and NQR investigations on three impurity-doped systems, Sr(Cu1-xMx)2O3 (M=Zn, Ni) with xIISP along the leg was found to be much longer than ξ0/a in x=0.001 and 0.005. The notable result is that ξs/a that was found to be T independent is scaled to mean distances DAV=1/(2x) between the Zn and Ni impurities and DAV=1/x between the La impurities. When DAV=500 for x=0.001 (Zn doping), ξs/a~50 is estimated. The significantly broadened NQR spectrum has provided unambiguous evidence for the AF-LRO in the Zn and Ni doping (x=0.01 and 0.02). Rather uniform AF moments at the middle Cu sites between the impurities are estimated to be about 0.04μB at 1.4 K along the a axis. By assuming that exponential decay constants of AF moments are equivalent to ξs/a's for the IISP, the size of an AF moment next to the impurity is deduced as SAF~1/4. We propose that these exponential distributions of IISP and AF moments along the two-leg suggest that an interladder interaction is in a weakly coupled quasi-one-dimensional (WC-Q1D) regime. The formula of TN=J0exp(-DAV/(ξs/a)) based on the WC-Q1D model explains TN(exp)=3 K (x=0.01) and 5.8 K (x=0.02) quantitatively and predicts to be as small as TN=0.09 K for x=0.001 using J0=2000 K. On the other hand, there is no evidence of AF-LRO for the La doping (x=0.02 and 0.03) down to 1.4 K, nevertheless their ξs/a's are almost equivalent to those in the Zn and Ni doping (x=0.01 and 0.02). We remark that the Q1D-IISP is dramatically enhanced by the interladder interaction even though so weak, once the impurity breaks up the quantum coherence in the short-range resonating valence bond (RVB) state with the gap. On the one hand, we propose that TN is determined by a strength of the interladder interaction and a size

  20. Ising antiferromagnet on the Archimedean lattices

    Science.gov (United States)

    Yu, Unjong

    2015-06-01

    Geometric frustration effects were studied systematically with the Ising antiferromagnet on the 11 Archimedean lattices using the Monte Carlo methods. The Wang-Landau algorithm for static properties (specific heat and residual entropy) and the Metropolis algorithm for a freezing order parameter were adopted. The exact residual entropy was also found. Based on the degree of frustration and dynamic properties, ground states of them were determined. The Shastry-Sutherland lattice and the trellis lattice are weakly frustrated and have two- and one-dimensional long-range-ordered ground states, respectively. The bounce, maple-leaf, and star lattices have the spin ice phase. The spin liquid phase appears in the triangular and kagome lattices.

  1. Weyl magnons in noncoplanar stacked kagome antiferromagnets

    Science.gov (United States)

    Owerre, S. A.

    2018-03-01

    Weyl nodes have been experimentally realized in photonic, electronic, and phononic crystals. However, magnonic Weyl nodes are yet to be seen experimentally. In this paper, we propose Weyl magnon nodes in noncoplanar stacked frustrated kagome antiferromagnets, naturally available in various real materials. Most crucially, the Weyl nodes in the current system occur at the lowest excitation and possess a topological thermal Hall effect, therefore they are experimentally accessible at low temperatures due to the population effect of bosonic quasiparticles. In stark contrast to other magnetic systems, the current Weyl nodes do not rely on time-reversal symmetry breaking by the magnetic order. Rather, they result from explicit macroscopically broken time reversal symmetry by the scalar spin chirality of noncoplanar spin textures and can be generalized to chiral spin liquid states. Moreover, the scalar spin chirality gives a real space Berry curvature which is not available in previously studied magnetic Weyl systems. We show the existence of magnon arc surface states connecting projected Weyl magnon nodes on the surface Brillouin zone. We also uncover the first realization of triply-degenerate nodal magnon point in the noncollinear regime with zero scalar spin chirality.

  2. Quantum disordered phase in a doped antiferromagnet

    International Nuclear Information System (INIS)

    Kuebert, C.; Muramatsu, A.

    1995-01-01

    A quantitative description of the transition to a quantum disordered phase in a doped antiferromagnet is obtained for the long-wavelength limit of the spin-fermion model, which is given by the O(3) non-linear σ model, a free fermionic part and current-current interactions. By choosing local spin quantization axes for the fermionic spinor we show that the low-energy limit of the model is equivalent to a U(1) gauge theory, where both the bosonic and fermionic degrees of freedom are minimally coupled to a vector gauge field. Within a large-N expansion, the strength of the gauge fields is found to be determined by the gap in the spin-wave spectrum, which is dynamically generated. The explicit doping dependence of the spin-gap is determined as a function of the parameters of the original model. As a consequence of the above, the gauge-fields mediate a long-range interaction among dopant holes and S-1/2 magnetic excitations only in the quantum disordered phase. The possible bound-states in this regime correspond to charge-spin separation and pairing

  3. Antiferromagnetism of nuclear matter in the model with effective Gogny interaction

    International Nuclear Information System (INIS)

    Isayev, A.A.; Yang, J.

    2006-01-01

    The possibility of ferromagnetic (FM) antiferromagnetic (AFM) phase transitions in symmetric nuclear matter is analyzed within the framework of a Fermi-liquid theory with the effective Gogny interaction. It is shown that at some critical density nuclear matter undergoes a phase transition to the AFM spin state. The self-consistent equations of spin-polarized nuclear matter have no solutions corresponding to FM spin ordering and, hence, the FM transition does not appear. The AFM spin state properties are investigated [ru

  4. Quantum phase transitions in effective spin-ladder models for graphene zigzag nanoribbons

    Science.gov (United States)

    Koop, Cornelie; Wessel, Stefan

    2017-10-01

    We examine the magnetic correlations in quantum spin models that were derived recently as effective low-energy theories for electronic correlation effects on the edge states of graphene nanoribbons. For this purpose, we employ quantum Monte Carlo simulations to access the large-distance properties, accounting for quantum fluctuations beyond mean-field-theory approaches to edge magnetism. For certain chiral nanoribbons, antiferromagnetic interedge couplings were previously found to induce a gapped quantum disordered ground state of the effective spin model. We find that the extended nature of the intraedge couplings in the effective spin model for zigzag nanoribbons leads to a quantum phase transition at a large, finite value of the interedge coupling. This quantum critical point separates the quantum disordered region from a gapless phase of stable edge magnetism at weak intraedge coupling, which includes the ground states of spin-ladder models for wide zigzag nanoribbons. To study the quantum critical behavior, the effective spin model can be related to a model of two antiferromagnetically coupled Haldane-Shastry spin-half chains with long-ranged ferromagnetic intrachain couplings. The results for the critical exponents are compared also to several recent renormalization-group calculations for related long-ranged interacting quantum systems.

  5. Misjudging frustrations in spin liquids from oversimplified use of Curie-Weiss law

    Energy Technology Data Exchange (ETDEWEB)

    Nag, Abhishek, E-mail: msan@iacs.res.in [Department of Materials Science, Indian Association for the Cultivation of Science, Jadavpur, Kolkata 700032 (India); Ray, Sugata [Department of Materials Science, Indian Association for the Cultivation of Science, Jadavpur, Kolkata 700032 (India); Centre for Advanced Materials, Indian Association for the Cultivation of Science, Jadavpur, Kolkata 700032 (India)

    2017-02-15

    Absence of a single smoking-gun experiment to identify a quantum spin liquid, has kept their characterisation difficult till date. Featureless dc magnetic susceptibility and large antiferromagnetic frustration are always considered as the essential pointers to these systems. However, we show that the amount of frustration estimated by using generalised Curie-Weiss law on these susceptibility data are prone to errors and thus should be dealt with caution. We measure and analyse susceptibility data of Ba{sub 3}ZnIr{sub 2}O{sub 9}, a spin orbital liquid candidate and Gd{sub 2}O{sub 3}, a 1.5 K antiferromagnet and show the distinguishing features between them. A continuous and significant change in Curie and Weiss constants is seen to take place in Ba{sub 3}ZnIr{sub 2}O{sub 9} and other reported spin liquids with the change in the range of fitting temperatures showing the need of a temperature ‘range-of-fit’ analysis before commenting on the Weiss constants of spin liquids. The variation observed is similar to fluctuations among topological sectors persisting over a range of temperature in spin-ice candidates. On the other hand, even though we find correlations to exist at even 100 times the ordering temperature in Gd{sub 2}O{sub 3}, no such fluctuation is observed which may be used as an additional distinguishing signature of spin liquids over similarly featureless correlated paramagnets. - Highlights: • Curie-Weiss fitting may give erroneous frustration parameters in spin-liquids. • The results depend upon choice of fitting method and temperature range used. • More appropriate method is to use a ʽrange of fit’ analysis. • Can distinguish between spin-liquids and correlated paramagnets.

  6. Effective Hamiltonian and low-lying eigenenergy clustering patterns of four-sublattice antiferromagnets

    DEFF Research Database (Denmark)

    Zhang, N.G.; Henley, C.L.; Rischel, C.

    2002-01-01

    We study the low-lying eigenenergy clustering patterns of quantum antiferromagnets with p sublattices (in particular p = 4). We treat each sublattice as a large spin, and using second-order degenerate perturbation theory, we derive the effective (biquadratic) Hamiltonian coupling the p large spins....... In order to compare with exact diagonalizations, the Hamiltonian is explicitly written for a finite-size lattice, and it contains information on energies of excited states as well as the ground state. The result is applied to the face-centered-cubic Type-I antiferromagnet of spin 1/2, including second...

  7. Polarized neutron powder diffraction studies of antiferromagnetic order in bulk and nanoparticle NiO

    DEFF Research Database (Denmark)

    Brok, Erik; Lefmann, Kim; Deen, Pascale P.

    2015-01-01

    surface contribution to the magnetic anisotropy. Here we explore the potential use of polarized neutron diffraction to reveal the magnetic structure in NiO bulk and nanoparticle powders by applying the XYZ-polarization analysis method. Our investigations address in particular the spin orientation in bulk....... The results show that polarization analyzed neutron powder diffraction is a viable method to investigate magnetic order in powders of antiferromagnetic nanoparticles.......In many materials it remains a challenge to reveal the nature of magnetic correlations, including antiferromagnetism and spin disorder. Revealing the spin structure in magnetic nanoparticles is further complicated by the large incoherent neutron scattering cross section from water adsorbed...

  8. Electronic structure of the antiferromagnetic phase of Sr2Co2O5

    International Nuclear Information System (INIS)

    Pardo, V.; Botta, P.M.; Baldomir, D.; Rivas, J.; Pineiro, A.; Calle, C. de la; Alonso, J.A.; Arias, J.E.

    2008-01-01

    Ab initio calculations analyze the properties of the G-type antiferromagnetic Sr 2 Co 2 O 5 as a high-spin system. The description of the electronic structure is given; all the Co atoms are in a high-spin state with a small unquenched orbital angular momentum. Thermal analysis on a polycrystalline sample shows a magnetic phase transition at high temperatures

  9. Topics on frustrated spin systems and high-temperature superconductors

    International Nuclear Information System (INIS)

    Lu Yong.

    1990-01-01

    The numerical study of frustrated spin systems using the Monte Carlo simulation method and the analytic study of fluctuation phenomenon of the thermoelectric power near the superconducting transition using Green's function techniques are presented. The first frustrated system considered is the B-site antiferromagnetic (AF) spinel. Based on an Ising model, various thermodynamic and magnetic properties were studied for both the fully frustrated structure and partially frustrated cases of a small tetragonal distortion. When fully frustrated, an interesting short-range order and some unusual scaling behavior were obtained. The other frustrated spin system studied is the magnetic phase of YBa 2 Cu 3 O 6+x via a classical spin model, with appropriate anisotropic exchange couplings and randomly located spins of distribution probability as a function of x. There is a first order boundary between Type 1 and Type 2 in the Ising case, while there is no real phase boundary in the cases of continuous spin. In the study on the thermopower fluctuation, the thermopower was determined by the linear response of the electric and heat currents to an electric field, and the linear responses were in turn calculated from correlation functions of the current

  10. Helical waves in easy-plane antiferromagnets

    Science.gov (United States)

    Semenov, Yuriy G.; Li, Xi-Lai; Xu, Xinyi; Kim, Ki Wook

    2017-12-01

    Effective spin torques can generate the Néel vector oscillations in antiferromagnets (AFMs). Here, it is theoretically shown that these torques applied at one end of a normal AFM strip can excite a helical type of spin wave in the strip whose properties are drastically different from characteristic spin waves. An analysis based on both a Néel vector dynamical equation and the micromagnetic simulation identifies the direction of magnetic anisotropy and the damping factor as the two key parameters determining the dynamics. Helical wave propagation requires the hard axis of the easy-plane AFM to be aligned with the traveling direction, while the damping limits its spatial extent. If the damping is neglected, the calculation leads to a uniform periodic domain wall structure. On the other hand, finite damping decelerates the helical wave rotation around the hard axis, ultimately causing stoppage of its propagation along the strip. With the group velocity staying close to spin-wave velocity at the wave front, the wavelength becomes correspondingly longer away from the excitation point. In a sufficiently short strip, a steady-state oscillation can be established whose frequency is controlled by the waveguide length as well as the excitation energy or torque.

  11. Field-dependent antiferromagnetism and ferromagnetism of the two copper sublattices in Sr2Cu3O4Cl2

    International Nuclear Information System (INIS)

    Kastner, M.A.; Aharony, A.; Birgeneau, R.J.; Chou, F.C.; Entin-Wohlman, O.; Greven, M.; Harris, A.B.; Kim, Y.J.; Lee, Y.S.; Parks, M.E.; Zhu, Q.

    1999-01-01

    The Cu 3 O 4 layer in Sr 2 Cu 3 O 4 Cl 2 is a variant of the square CuO 2 lattice of the high-temperature superconductors, in which the center of every second plaquette contains an extra Cu 2+ ion. The ions that make up the conventional CuO 2 network, called CuI, have CuI-CuI exchange energy ∼130meV, and order antiferromagnetically at about 380 K; the CuII-CuII exchange is only ∼10meV, and the CuII close-quote s order at ∼40K. A study is reported here of the dependence of the magnetization on field, temperature, and crystallographic orientation for this interesting system. We show that the small permanent ferromagnetic moment, that appears when the CuI spins order, and the unusual spin rotation transitions seen most clearly for one particular direction of the magnetic field, are the result of several small bond-dependent anisotropic terms in the spin Hamiltonian that are revealed because of the frustration of the isotropic Heisenberg interaction between CuI and CuII spins. These include a term which favors collinearity of the CuI and CuII spins, which originates from quantum fluctuations, and also the pseudodipolar interaction. Some of these small interactions also come into play in other lamellar cuprates, connected with the high-T c superconductivity materials, and in many spin-chain and spin-ladder compounds. copyright 1999 The American Physical Society

  12. Antiferromagnetism and d-wave superconductivity in (doped) Mott insulators: A wave function approach

    OpenAIRE

    Weng, Z. Y.; Zhou, Y.; Muthukumar, V. N.

    2003-01-01

    We propose a class of wave functions that provide a unified description of antiferromagnetism and d-wave superconductivity in (doped) Mott insulators. The wave function has a Jastrow form and prohibits double occupancies. In the absence of holes, the wave function describes antiferromagnetism accurately. Off diagonal long range order develops at finite doping and the superconducting order parameter has d-wave symmetry. We also show how nodal quasiparticles and neutral spin excitations can be ...

  13. Polarized Neutron Reflectivity Simulation of Ferromagnet/ Antiferromagnet Thin Films

    Energy Technology Data Exchange (ETDEWEB)

    Kim, Ki Yeon; Lee, Jeong Soo

    2008-02-15

    This report investigates the current simulating and fitting programs capable of calculating the polarized neutron reflectivity of the exchange-biased ferromagnet/antiferromagnet magnetic thin films. The adequate programs are selected depending on whether nonspin flip and spin flip reflectivities of magnetic thin films and good user interface are available or not. The exchange-biased systems such as Fe/Cr, Co/CoO, CoFe/IrMn/Py thin films have been simulated successfully with selected programs.

  14. Interface states in stressed semiconductor heterojunction with antiferromagnetic ordering

    International Nuclear Information System (INIS)

    Kantser, V.G.

    1995-08-01

    The stressed heterojunctions with antiferromagnetic ordering in which the constituents have opposite band edge symmetry and their gaps have opposite signs have been investigated. The interface states have been shown to appear in these heterojunctions and they are spin-split. As a result if the Fermi level gets into one of the interface bands then it leads to magnetic ordering in the interface plane. That is if the interface magnetization effect can be observed. (author). 14 refs, 2 figs

  15. Magnetocaloric effect in quantum spin-s chains

    Directory of Open Access Journals (Sweden)

    A. Honecker

    2009-01-01

    Full Text Available We compute the entropy of antiferromagnetic quantum spin-s chains in an external magnetic field using exact diagonalization and Quantum Monte Carlo simulations. The magnetocaloric effect, i. e., temperature variations during adiabatic field changes, can be derived from the isentropes. First, we focus on the example of the spin-s=1 chain and show that one can cool by closing the Haldane gap with a magnetic field. We then move to quantum spin-s chains and demonstrate linear scaling with s close to the saturation field. In passing, we propose a new method to compute many low-lying excited states using the Lanczos recursion.

  16. Spin-glass transition in disordered terbium

    International Nuclear Information System (INIS)

    Hauser, J.J.

    1985-01-01

    While crystalline Tb is a helix antiferromagnet with a Neel temperature of 229 K which becomes ferromagnetic at 222 K, disordered Tb exhibits a spin-glass transition. The spin-glass freezing temperature ranges from 183 to 53 K, the lowest temperatures corresponding to the greatest degree of atomic disorder. These experiments constitute the first evidence for an elemental spin-glass. (author)

  17. Long-range spin deformations around quasiparticles

    International Nuclear Information System (INIS)

    Godfrey, M.; Gunn, M.

    1989-01-01

    The quasi-particle formed by a hole in a Heisenberg antiferromagnet has an associated long-range spin distortion whose amplitude increases with the velocity of the hole. The authors show that the existence and properties of this distortion follow from simple classical arguments based on the long-wavelength equations of motion for the spin system. A similar long-range distortion is found in the quantum-mechanical problem of an electron exchange coupled to a Heisenberg antiferromagnet

  18. Modeling of exchange bias in the antiferromagnetic (core)/ferromagnetic (shell) nanoparticles with specialized shapes

    International Nuclear Information System (INIS)

    Hu Yong; Liu Yan; Du An

    2011-01-01

    Zero-field-cooled (ZFC) and field-cooled (FC) hysteresis loops of egg- and ellipsoid-shaped nanoparticles with inverted ferromagnetic (FM)-antiferromagnetic (AFM) core-shell morphologies are simulated using a modified Monte Carlo method, which takes into account both the thermal fluctuations and energy barriers during the rotation of spin. Pronounced exchange bias (EB) fields and reduced coercivities are obtained in the FC hysteresis loops. The analysis of the microscopic spin configurations allows us to conclude that the magnetization reversal occurs by means of the nucleation process during both the ZFC and FC hysteresis branches. The nucleation takes place in the form of 'sparks' resulting from the energy competition and the morphology of the nanoparticle. The appearance of EB in the FC hysteresis loops is only dependent on that the movements of 'sparks' driven by magnetic field at both branches of hysteresis loops are not along the same axis, which is independent of the strength of AFM anisotropy. The tilt of 'spark' movement with respect to the symmetric axis implies the existence of additional unidirectional anisotropy at the AFM/FM interfaces as a consequence of the surplus magnetization in the AFM core, which is the commonly accepted origin of EB. Our simulations allow us to clarify the microscopic mechanisms of the observed EB behavior, not accessible in experiments. - Highlights: → A modified Monte Carlo method considers thermal fluctuations and energy barriers. → Egg and ellipsoid nanoparticles with inverted core-shell morphology are studied. → Pronounced exchange bias fields and reduced coercivities may be detected. → 'Sparks' representing nucleation sites due to energy competition are observed. → 'Sparks' can reflect or check directly and vividly the origin of exchange bias.

  19. Quantum Heisenberg antiferromagnetic chains with exchange and single-ion anisotropies

    International Nuclear Information System (INIS)

    Peters, D; Selke, W; McCulloch, I P

    2010-01-01

    Using density matrix renormalization group calculations, ground state properties of the spin-1 Heisenberg chain with exchange and quadratic single-ion anisotropies in an external field are studied, for special choices of the two kinds of anisotropies. In particular, the phase diagram includes antiferromagnetic, spin-liquid (or spin-flop), IS2, and supersolid (or biconical) phases. Especially, new features of the spin-liquid and supersolid phases are discussed. Properties of the quantum chains are compared to those of corresponding classical spin chains.

  20. Field-controlled spin current in frustrated spin chains

    Directory of Open Access Journals (Sweden)

    A.K. Kolezhuk

    2009-01-01

    Full Text Available We study states with spontaneous spin current, emerging in frustrated antiferromagnetic spin-S chains subject to a strong external magnetic field. As a numerical tool, we use a non-Abelian symmetry realization of the density matrix renormalization group. The field dependence of the order parameter and the critical exponents are presented for zigzag chains with S=1/2, 1, 3/2, and 2.

  1. ZnFe{sub 2}O{sub 4} antiferromagnetic structure redetermination

    Energy Technology Data Exchange (ETDEWEB)

    Kremenović, Aleksandar, E-mail: akremenovic@rgf.bg.ac.rs [Laboratory for Crystallography, Faculty of Mining and Geology, University of Belgrade, Đušina 7, Belgrade 11000 (Serbia); Antić, Bratislav [Condensed Matter Physics Laboratory, Institute of Nuclear Sciences “Vinča”, University of Belgrade, P.O. Box 522, Belgrade 11001 (Serbia); Vulić, Predrag [Laboratory for Crystallography, Faculty of Mining and Geology, University of Belgrade, Đušina 7, Belgrade 11000 (Serbia); Blanuša, Jovan [Condensed Matter Physics Laboratory, Institute of Nuclear Sciences “Vinča”, University of Belgrade, P.O. Box 522, Belgrade 11001 (Serbia); Tomic, Aleksandra [Condensed Matter Physics Laboratory, Institute of Nuclear Sciences “Vinča”, University of Belgrade, P.O. Box 522, Belgrade 11001 (Serbia); Department of Applied Physics and Applied Mathematics, Columbia University, New York, NY, 10027 (United States)

    2017-03-15

    Magnetic structure of ZnFe{sub 2}O{sub 4} normal spinel is re-examined. Antiferromagnetic structure non-collinear model is established within C{sub a}2 space group having four different crystallographic/magnetic sites for 32 Fe{sup 3+} spins within magnetic unit cell. - Highlights: • Magnetic structure of ZnFe{sub 2}O{sub 4} normal spinel is re-examined. • Antiferromagnetic non-collinear structure model is established within C{sub a}2 space group. • Four different crystallographic/magnetic sites contain 32 Fe{sup 3+} spins within magnetic unit cell.

  2. Antiferromagnetic Skyrmion: Stability, Creation and Manipulation

    Science.gov (United States)

    Zhang, Xichao; Zhou, Yan; Ezawa, Motohiko

    2016-04-01

    Magnetic skyrmions are particle-like topological excitations in ferromagnets, which have the topo-logical number Q = ± 1, and hence show the skyrmion Hall effect (SkHE) due to the Magnus force effect originating from the topology. Here, we propose the counterpart of the magnetic skyrmion in the antiferromagnetic (AFM) system, that is, the AFM skyrmion, which is topologically protected but without showing the SkHE. Two approaches for creating the AFM skyrmion have been described based on micromagnetic lattice simulations: (i) by injecting a vertical spin-polarized current to a nanodisk with the AFM ground state; (ii) by converting an AFM domain-wall pair in a nanowire junction. It is demonstrated that the AFM skyrmion, driven by the spin-polarized current, can move straightly over long distance, benefiting from the absence of the SkHE. Our results will open a new strategy on designing the novel spintronic devices based on AFM materials.

  3. Ground State of Quasi-One Dimensional Competing Spin Chain Cs2Cu2Mo3O12 at zero and Finite Fields

    Science.gov (United States)

    Matsui, Kazuki; Goto, Takayuki; Angel, Julia; Watanabe, Isao; Sasaki, Takahiko; Hase, Masashi

    The ground state of competing-spin-chain Cs2Cu2Mo3O12 with the ferromagnetic exchange interaction J1 = -93 K on nearest-neighboring spins and the antiferromagnetic one J2 = +33 K on next-nearest-neighboring spins was investigated by ZF/LF-μSR and 133Cs-NMR in the 3He temperature range. The zero-field μSR relaxation rate λ shows a significant increase below 1.85 K, suggesting the existence of magnetic order, which is consistent with the recent report on the specific heat. However, LF decoupling data at the lowest temperature 0.3 K indicate that the spins fluctuate dynamically, suggesting that the system is in a quasi-static ordered state under zero field. This idea is further supported by the fact that the broadening in NMR spectra below TN is weakened at low field below 2 T.

  4. Magnetic fluctuations in heavy fermion systems

    International Nuclear Information System (INIS)

    Broholm, C.L.

    1989-06-01

    Magnetic order and fluctuations in the heavy Fermion systems UPt 3 , U 2 Zn 17 and URu 2 Si 2 have been studied by neutron scattering. Single crystalline samples and triple-axis neutron-scattering techniques with energy transfers between 0 and 40 meV and energy resolutions between 0.1 meV and 4 meV have been employed. UPt 3 develops an antiferromagnetically ordered moment of (0.02±0.005) μ B below T N = 5 K which doubles the unit cell in the basal plane and coexists with superconductivity below T c = 0.5 K. The magnetic fluctuations are relaxational, and enhanced at the antiferromagnetic zone center in a low-energy regime. The characteristic zone-center relaxation energy is 0.3 meV. The temperature- and field-dependence of the antiferromagnetic order in the superconducting phase suggest a close relation between these two properties in UPt 3 . U 2 Zn 17 has a broad spectrum of magnetic fluctuations, even below T N = 9.7 K, of which the transverse part below 10 meV is strongly enhanced at the antiferromagnetic zone center. The system has an anomalously extended critical region and the antiferromagnetic phase transition seems to be driven by the temperature-dependence of an effective RKKY interaction, as anticipated theoretically. URu 2 Si 2 , a strongly anisotropic heavy Fermion system, has a high-energy regime of antiferromagnetically-correlated overdamped magnetic fluctuations. Below T N = 17.5 K weak antiferromagnetic order, μ = (0.04±0.01)μ B , with finite correlations along the tetragonal c axis, develops along with a low-energy regime of strongly dispersive singlet-singlet excitations. Below T c = 1 K antiferromagnetism coexists with superconductivity. A phenomenological model describing the exchange-enhanced overdamped magnetic fluctuations of heavy Fermion systems is proposed. Our experimental results are compared to the anomalous bulk properties of heavy Fermion systems, and to magnetic fluctuations in other metallic magnets. (orig.)

  5. Spin-polarized SEM

    International Nuclear Information System (INIS)

    Konoto, Makoto

    2007-01-01

    Development of highly effective evaluation technology of magnetic structures on a nanometric scale is a key to understanding spintronics and related phenomena. A high-resolution spin-polarized scanning electron microscope (spin SEM) developed recently is quite suitable for probing such nanostructures because of the capability of analyzing local magnetization vectors in three dimensions. Utilizing the spin SEM, a layered antiferromagnetic structure with the 1nm-alternation of bilayer-sheet magnetization has been successfully resolved. The real-space imaging with full analysis of the temperature-dependent magnetization vectors will be demonstrated. (author)

  6. Ferrimagnetic-antiferromagnetic phase transition in Mn2–xCrxSb : Electronic structure and electrical and magnetic properties

    NARCIS (Netherlands)

    Wijngaard, Jan; Haas, C.; Groot, R.A. de

    1992-01-01

    Self-consistent spin-polarized energy-band calculations have been performed for Mn2Sb for a ferrimagnetic (FI), ferromagnetic (F), and antiferromagnetic (AF) spin alignment. The calculated local moments on the two types of Mn atoms are in agreement with values obtained from neutron diffraction for

  7. Superconductivity and antiferromagnetism in heavy-electron systems

    International Nuclear Information System (INIS)

    Konno, R.; Ueda, K.

    1989-01-01

    Superconductivity and antiferromagnetism in heavy-electron systems are investigated from a general point of view. First we classify superconducting states in a simple cubic lattice, a body-centered tetragonal lattice, and a hexagonal close-packed lattice, having URu 2 Si 2 and UPt 3 in mind. For that purpose we take an approach to treat the effective couplings in real space. The approach is convenient to discuss the relation between the nature of fluctuations in the system and the superconducting states. When we assume that the antiferromagnetic fluctuations reported by neutron experiments are dominant, the most promising are some of the anisotropic singlet states and there remains the possibility for some triplet states too. Then we discuss the coupling between the two order parameters based on a Ginzburg-Landau theory. We derive a general expression of the coupling term. It is pointed out that the coupling constant can be large in heavy-electron systems. The general trend of the coexistence of the superconductivity and antiferromagnetism is discussed, and it is shown that the anisotropic states are generally more favorable to the coexistence than the conventional isotropic singlet. Experimental data of URu 2 Si 2 and UPt 3 are analyzed by the Ginzburg-Landau theory. According to the analysis URu 2 Si 2 has a small coupling constant and a large condensation energy of the antiferromagnetism. On the other hand, UPt 3 has a large coupling constant and a small condensation energy. It means that the specific-heat anomaly at T N should be small in UPt 3 and its superconductivity is easily destroyed when a large moment is formed

  8. Superconductivity and antiferromagnetism in cuprates and pnictides: Evidence of the role of Coulomb correlation

    International Nuclear Information System (INIS)

    Fan, J.D.; Malozovsky, Y.M.

    2013-01-01

    Highlights: • In a layered 2D cuprates the long-range order antiferromagnetism is driven mainly by the Van Hove singularity. • The long-range antiferromagnetism quickly disappear with doping away from the Van Hove singularity. • For pnictides the antiferromagnetism exists as a result of the nesting condition. • Since the doping steadily changes the nesting conditions, the antiferromagnetism and superconductivity may coexist. -- Abstract: We consider the Hubbard model in terms of the perturbative diagrammatic approach (UN F ⩽1) where the interaction between two electrons with antiparallel spins in the lowest order of perturbation is described by the short-range repulsive contact (on-site) interaction (U>0). We argue that in layered 2D cuprates the long-range order antiferromagnetism is driven mainly by the Van Hove singularity, whereas in the case of pnictides the antiferromagnetism exists as a result of the nesting condition. We show that when the interaction is quite strong (UN F ≈1) in the case of the Van Hove singularity the electron system undergoes the antiferromagnetic phase transition with the log-range order parameter and large insulating gap. The long-range antiferromagnetism quickly disappear, as shown, with the doping away from the Van Hove singularity, but the antiferromagnetic short-range correlation persists (UN F < 1) due to Coulomb repulsive interaction which is the mechanism for superconductivity in cuprates. We argue that in the case of pnictides the antiferromagnetism appears when the nesting conditions for the Fermi surface are met. Since the doping steadily changes the nesting conditions, the antiferromagnetism and superconductivity may coexist as has been observed in pnictides. We show that the proximity of the antiferromagnetism and superconductivity implies the repulsive interaction between electrons, which turns into attractive between quasiparticles as shown by the authors in the article published on the same issue as this one

  9. Uranium nitride: a cubic antiferromagnet with anisotropic critical behavior

    International Nuclear Information System (INIS)

    Buyers, W.J.L.; Holden, T.M.; Svensson, E.C.; Lander, G.H.

    1977-11-01

    Highly anisotropic critical scattering associated with the transition at T/sub N/ = 49.5 K to the type-I antiferromagnetic structure has been observed in uranium nitride. The transverse susceptibility is found to be unobservably small. The longitudinal susceptibility diverges at T/sub N/ and its anisotropy shows that the spins within the (001) ferromagnetic sheets of the [001] domain are much more highly correlated than they are with the spins lying in adjacent (001) sheets. The correlation range within the sheets is much greater than that expected for a Heisenberg system with the same T/sub N/. The rod-like scattering extended along the spin and domain direction is reminiscent of two-dimensional behavior. The results are inconsistent with a simple localized model and may reflect the itinerant nature of the 5f electrons

  10. Quantum oscillations in antiferromagnetic CaFe2As2 on the brink of superconductivity

    International Nuclear Information System (INIS)

    Harrison, N; McDonald, R D; Mielke, C H; Bauer, E D; Ronning, F; Thompson, J D

    2009-01-01

    We report quantum oscillation measurements on CaFe 2 As 2 under strong magnetic fields-recently reported to become superconducting under pressures of as little as a kilobar. The largest observed carrier pocket occupies less than 0.05% of the paramagnetic Brillouin zone volume-consistent with Fermi surface reconstruction caused by antiferromagnetism. On comparing several alkaline earth AFe 2 As 2 antiferromagnets (with A = Ca, Sr and Ba), the dependences of the Fermi surface cross-sectional area F α and the effective mass m α * of the primary observed pocket on the antiferromagnetic/structural transition temperature T s are both found to be consistent with the case for quasiparticles in a conventional spin-density wave model. These findings suggest that the recently proposed strain-enhanced superconductivity in these materials occurs within a broadly conventional spin-density wave phase. (fast track communication)

  11. Fermionic Hubbard model with Rashba or Dresselhaus spin-orbit coupling

    Science.gov (United States)

    Sun, Fadi; Ye, Jinwu; Liu, Wu-Ming

    2017-06-01

    In this work, we investigate the possible dramatic effects of Rashba or Dresselhaus spin-orbit coupling (SOC) on the fermionic Hubbard model in a two-dimensional square lattice. In the strong coupling limit, it leads to the rotated antiferromagnetic Heisenberg model which is a new class of quantum spin model. For a special equivalent class, we identify a new spin-orbital entangled commensurate ground (Y-y) state subject to strong quantum fluctuations at T = 0. We evaluate the quantum fluctuations by the spin wave expansion up to order 1/{S}2. In some SOC parameter regimes, the Y-y state supports a massive relativistic incommensurate magnon (C-IC) with its two gap minima positions continuously tuned by the SOC parameters. The C-IC magnons dominate all the low temperature thermodynamic quantities and also lead to the separation of the peak positions between the longitudinal and the transverse spin structure factors. In the weak coupling limit, any weak repulsive interaction also leads to a weak Y-y state. There is only a crossover from the weak to the strong coupling. High temperature expansions of the specific heats in both weak and strong coupling are presented. The dramatic roles to be played by these C-IC magnons at generic SOC parameters or under various external probes are hinted at. Experimental applications to both layered noncentrosymmetric materials and cold atoms are discussed.

  12. One dimensionalization in the spin-1 Heisenberg model on the anisotropic triangular lattice

    Science.gov (United States)

    Gonzalez, M. G.; Ghioldi, E. A.; Gazza, C. J.; Manuel, L. O.; Trumper, A. E.

    2017-11-01

    We investigate the effect of dimensional crossover in the ground state of the antiferromagnetic spin-1 Heisenberg model on the anisotropic triangular lattice that interpolates between the regime of weakly coupled Haldane chains (J'≪J ) and the isotropic triangular lattice (J'=J ). We use the density-matrix renormalization group (DMRG) and Schwinger boson theory performed at the Gaussian correction level above the saddle-point solution. Our DMRG results show an abrupt transition between decoupled spin chains and the spirally ordered regime at (J'/J) c˜0.42 , signaled by the sudden closing of the spin gap. Coming from the magnetically ordered side, the computation of the spin stiffness within Schwinger boson theory predicts the instability of the spiral magnetic order toward a magnetically disordered phase with one-dimensional features at (J'/J) c˜0.43 . The agreement of these complementary methods, along with the strong difference found between the intra- and the interchain DMRG short spin-spin correlations for sufficiently large values of the interchain coupling, suggests that the interplay between the quantum fluctuations and the dimensional crossover effects gives rise to the one-dimensionalization phenomenon in this frustrated spin-1 Hamiltonian.

  13. Unconventional spin order in the triangular lattice system NaCrO2: A neutron scattering study

    International Nuclear Information System (INIS)

    Hsieh, D.; Qian, D.; Berger, R.F.; Cava, R.J.; Lynn, J.W.; Huang, Q.; Hasan, M.Z.

    2008-01-01

    We report high resolution neutron scattering measurements on the rhombohedrally stacked triangular antiferromagnet NaCrO 2 which has recently been shown to exhibit an unusually broad fluctuating cross-over regime extending far below the onset of spin freezing at T c . Our results show that at T c purely two-dimensional quasi-static spin correlations of the 120 o type exist. Below some cross-over temperature (T∼0.75T c ) a small incommensuration develops which helps resolve the inter-layer spin frustration and drives short-range three-dimensional magnetic order. This incommensuration assisted dimensional cross-over suggests that inter-layer frustration is responsible for stabilizing the rare 2D correlated phase above 0.75T c

  14. Generalized spin-wave theory: Application to the bilinear-biquadratic model

    Science.gov (United States)

    Muniz, Rodrigo A.; Kato, Yasuyuki; Batista, Cristian D.

    2014-08-01

    We present a mathematical framework for the multi-boson approach that has been used several times for treating spin systems. We demonstrate that the multi-boson approach corresponds to a generalization of the traditional spin-wave theory from SU(2) to SU(N), where N is the number of states of the local degree of freedom. Low-energy excitations are waves of the local order parameter that fluctuates in the SU(N) space of unitary transformations of the local spin states, instead of the SU(2) space of local spin rotations. Since the generators of the SU(N) group can be represented as bilinear forms in N-flavored bosons, the low-energy modes of the generalized spin-wave theory (GSWT) are described with N-1 different bosons, which provide a more accurate description of low-energy excitations even for the usual ferromagnetic and antiferromagnetic phases. The generalization enables the treatment of quantum spin systems whose ground states exhibit multipolar ordering as well as the detection of instabilities of magnetically ordered states (dipolar ordering) towards higher multipolar orderings. We illustrate the advantages of the GSWT by applying it to a bilinear-biquadratic model of arbitrary spin S on hypercubic lattices, and then analyzing the spectrum of dipolar phases in order to find their instabilities. In contrast to the known results for S=1 when the biquadratic term in the Hamiltonian is negative, we find that there is no nematic phase between the ferromagnetic or antiferromagnetic orderings for S>1.

  15. Topics on frustrated spin systems and high-temperature superconductors

    International Nuclear Information System (INIS)

    Lu, Yong.

    1990-01-01

    The numerical study of frustrated spin systems using the Monte Carlo simulation method and the analytic study of fluctuation phenomenon of the thermoelectric power near the superconducting transition using Green's function techniques are presented. The first frustrated system considered was the B-site antiferromagnetic (AF) spinel. Based on an Ising model, various thermodynamic and magnetic properties for both the fully frustrated structure and partially frustrated cases of a small tetragonal distortion were studied. When fully frustrated, an interesting short range order and some unusual scaling behavior were obtained. In the two tetragonally distorted cases, contracting and expanding in the crystallographic c-direction, AF long range orders and some hysteresis behavior were found. A general phase diagram was constructed as a function of the degree of the distortion. The other frustrated spin system that was studied is the magnetic phase of YBa2Cu3O(6+x). A classical spin model, was constructed, and various properties in its Ising, Heisenberg, and x-y versions were studied. The susceptibility was calculated as a function of temperature for various values of x. In the study on the thermopower fluctuation, the thermopower was determined by the linear response of the electric and heat currents to an electric field, and the linear responses were in turn calculated from correlation functions of the current

  16. How to manipulate magnetic states of antiferromagnets

    Science.gov (United States)

    Song, Cheng; You, Yunfeng; Chen, Xianzhe; Zhou, Xiaofeng; Wang, Yuyan; Pan, Feng

    2018-03-01

    Antiferromagnetic materials, which have drawn considerable attention recently, have fascinating features: they are robust against perturbation, produce no stray fields, and exhibit ultrafast dynamics. Discerning how to efficiently manipulate the magnetic state of an antiferromagnet is key to the development of antiferromagnetic spintronics. In this review, we introduce four main methods (magnetic, strain, electrical, and optical) to mediate the magnetic states and elaborate on intrinsic origins of different antiferromagnetic materials. Magnetic control includes a strong magnetic field, exchange bias, and field cooling, which are traditional and basic. Strain control involves the magnetic anisotropy effect or metamagnetic transition. Electrical control can be divided into two parts, electric field and electric current, both of which are convenient for practical applications. Optical control includes thermal and electronic excitation, an inertia-driven mechanism, and terahertz laser control, with the potential for ultrafast antiferromagnetic manipulation. This review sheds light on effective usage of antiferromagnets and provides a new perspective on antiferromagnetic spintronics.

  17. Construction and study of exact ground states for a class of quantum antiferromagnets

    International Nuclear Information System (INIS)

    Fannes, M.

    1989-01-01

    Techniques of quantum probability are used to construct the exact ground states for a class of quantum spin systems in one dimension. This class in particular contains the antiferromagnetic models introduced by various authors under the name of VBS-models. The construction permits a detailed study of these ground states. (A.C.A.S.) [pt

  18. Tunnelling anisotropic magnetoresistance due to antiferromagnetic CoO tunnel barriers

    NARCIS (Netherlands)

    Wang, Kai; Sanderink, Johannes G.M.; Bolhuis, Thijs; van der Wiel, Wilfred Gerard; de Jong, Machiel Pieter

    2015-01-01

    A new approach in spintronics is based on spin-polarized charge transport phenomena governed by antiferromagnetic (AFM) materials. Recent studies have demonstrated the feasibility of this approach for AFM metals and semiconductors. We report tunneling anisotropic magnetoresistance (TAMR) due to the

  19. Susceptibility and specific heat of the Heisenberg antiferromagnet on the Kagome lattice

    International Nuclear Information System (INIS)

    Bernhard, B.H.; Canals, B.; Lacroix, C.

    2001-01-01

    The dynamic susceptibility of the S=((1)/(2)) Heisenberg antiferromagnet is calculated on the Kagome lattice by means of a Green's function decoupling scheme. The spin-spin correlation functions decrease exponentially with distance. The specific heat exhibits a single-peak structure with a T 2 dependence at low temperature and the correct high-temperature behaviour. The calculated total change in entropy indicates a ground-state entropy of 0.46 ln 2

  20. Wave function, spectrum and effective mass of holes in 2 D quantum antiferromagnet

    Science.gov (United States)

    Su, Zhao-bin; Ll, Yan-min; Lai, Wu-yan; Yu, Lu

    1989-12-01

    A new quantum Bogoliubov-de Gennes (BdeG) formalism is developed to study the self-consistent motion of holes on an quantum antiferromagnetic (QAFM) background within the generalized t- J model. The local distortion of spin configurations and the renormalization of the hole motion due to virtual excitations of the distorted spin background are treated on an equal footing. The hole wave function and its spectrum, as well as the effective mass for a propagating hole are calculated explicitly.

  1. The Heisenberg antiferromagnet on the square-kagomé lattice

    Directory of Open Access Journals (Sweden)

    J. Richter

    2009-01-01

    Full Text Available We discuss the ground state, the low-lying excitations as well as high-field thermodynamics of the Heisenberg antiferromagnet on the two-dimensional square-kagomé lattice. This magnetic system belongs to the class of highly frustrated spin systems with an infinite non-trivial degeneracy of the classical ground state as it is also known for the Heisenberg antiferromagnet on the kagomé and on the star lattice. The quantum ground state of the spin-half system is a quantum paramagnet with a finite spin gap and with a large number of non-magnetic excitations within this gap. We also discuss the magnetization versus field curve that shows a plateaux as well as a macroscopic magnetization jump to saturation due to independent localized magnon states. These localized states are highly degenerate and lead to interesting features in the low-temperature thermodynamics at high magnetic fields such as an additional low-temperature peak in the specific heat and an enhanced magnetocaloric effect.

  2. Magnetic Nanostructures Spin Dynamics and Spin Transport

    CERN Document Server

    Farle, Michael

    2013-01-01

    Nanomagnetism and spintronics is a rapidly expanding and increasingly important field of research with many applications already on the market and many more to be expected in the near future. This field started in the mid-1980s with the discovery of the GMR effect, recently awarded with the Nobel prize to Albert Fert and Peter Grünberg. The present volume covers the most important and most timely aspects of magnetic heterostructures, including spin torque effects, spin injection, spin transport, spin fluctuations, proximity effects, and electrical control of spin valves. The chapters are written by internationally recognized experts in their respective fields and provide an overview of the latest status.

  3. Analogies between antiferromagnets and antiferroelectrics

    International Nuclear Information System (INIS)

    Enz, C.P.; Matthias, B.T.

    1980-01-01

    Ferro- and antiferromagnetism in the Laves phase TiBesub(2-x) Cusub(x) occurs for 0.1 4 H 2 PO 4 and its solid solutions with TlH 2 PO 4 and with the ferroelectric KH 2 PO 4 are discussed as function of deuteration and of pressure. Another analogy as function of pressure is established with the antiferroelectric perovskite PbZrO 3 . (author)

  4. Localized description of valence fluctuations

    International Nuclear Information System (INIS)

    Alascio, B.; Allub, R.; Aligia, A.

    1979-07-01

    The authors set up a model for intermediate valence equivalent to the ''atomic'' limit of the Anderson Hamiltonian. Detailed analysis of this model shows that most of the essential characteristics of valence fluctuators are already present in this crudely simplified Hamiltonian. The spin-spin and the 4f charge-charge correlation functions are studied and it is shown that it is possible to define a spin fluctuation frequency ωsub(s.f.) and a charge fluctuation frequency ωsub(ch.f.).ωsub(s.f.) and ωsub(ch.f.) can differ considerably for some values of the parameters of the model. The magnetic susceptibility and the specific heat are calculated as functions of temperature and it is shown how the results simulate the behaviour found in valence fluctuators. (author)

  5. Two-dimensional magnetism in the triangular antiferromagnet NiGa2S4

    International Nuclear Information System (INIS)

    Nambu, Yusuke

    2013-01-01

    At sufficiently low temperatures, electron spins in normal magnets generally order into some fashion, for instance, ferromagnetic and antiferromagnetic. Geometrical frustration and/or reduced dimensionality can suppress such conventional orders, and occasionally induce unknown states of matter. This is the case for the two-dimensional (2D) triangular antiferromagnet Ni(Ga 2 S 4 , in which S=1 nickel spins do not order, instead show an exotic magnetism. We found (1) a resonant critical slowing down toward T*=8.5 K followed by a viscous spin liquid behavior, and (2) a spin-size dependent ground state. To elucidate (1), spin dynamics ranging from 10 -13 to 10 0 seconds were quantitatively explored through the experimental techniques such as inelastic neutron scattering, backscattering, neutron spin echo, ac and nonlinear susceptibilities. The finding of (2) is evidenced by impurity effects. Integer spins substituted systems such as zinc and iron ions retain a quadratic temperature dependence of the magnetic specific heat as for the parent compound. However, substitutions of half-odd integer spins, cobalt and manganese ions, eventually induce a distinct behavior, indicating an importance of integer size of spins to stabilize the 2D magnetism realized in NiGa 2 S 4 . The article gives our experimental findings and as well as some relevant theoretical scenarios. (author)

  6. Neutron scattering studies of spin correlations in metallic YBa2Cu3O6+x

    International Nuclear Information System (INIS)

    Tranquada, J.M.

    1991-01-01

    Electron-electron correlations appear to play an important role in determining many properties of the copper oxide superconductors. One significant consequence of the electronic coulomb interactions are spin correlations. In the insulating phases of the layered cuprates, where the antibonding band due to Cu 3d x 2 - y 2 -O 2p σ hybridization in the CuO 2 planes is half filled, long-range antiferromagnetic order is observed. As the layers are doped with holes, the Neel order is rapidly destroyed, but dynamical antiferromagnetic correlations survive. In this paper, I will review some inelastic neutron scattering studies of the spin fluctuations in metallic YBa 2 Cu 3 O 6+x . The paper is organized as follows. In the first section I briefly discuss some background information concerning the phase diagram and spin waves in the insulating phase. Experimental results on metallic YBa 2 Cu 3 O 6+x samples are presented in the second section. The interpretation of these results and their relationship to nuclear magnetic resonance (NMR) studies and to theory are discussed in the final section

  7. Quantum dynamics and entanglement of spins on a square lattice

    DEFF Research Database (Denmark)

    Christensen, Niels Bech; Rønnow, Henrik Moodysson; McMorrow, Desmond Francis

    2007-01-01

    in understanding quantum effects in one-dimensional quantum antiferromagnets, but a complete experimental description of even simple two-dimensional antiferromagnets is lacking. Here we describe a comprehensive set of neutron scattering measurements that reveal a non-spin-wave continuum and strong quantum effects...

  8. Colossal magnetodielectric effect and spin flop in magnetoelectric Co4Nb2O9 crystal

    International Nuclear Information System (INIS)

    Yin, L. H.; Yang, J.; Dai, J. M.; Song, W. H.; Zhu, X. B.; Zou, Y. M.; Sun, Y. P.

    2016-01-01

    We have investigated the detailed magnetic, magnetoelectric (ME), magnetodielectric (MD) and thermal expansion properties in Co 4 Nb 2 O 9 crystal. A magnetic-field-induced spin flop was observed below antiferromagnetic (AFM) transition temperature T N . Dielectric constant at applied magnetic field nearly diverges around the AFM transition, giving rise to a colossal MD effect as high as ∼138% around T N . Theoretical analysis of the ME and MD data revealed a major contribution of critical spin fluctuation to the colossal MD effect in Co 4 Nb 2 O 9 . These results suggest that linear ME materials with large ME coupling might be potentially used to realize large MD effect for future application.

  9. Anomalous enhancement of nuclear spin relaxation rates of 109Ag and 115In at low temperatures in cubic Γ3 ground-state system PrAg2In. First observation of octupole fluctuations of f-electrons

    International Nuclear Information System (INIS)

    Tanida, Hiroshi; Takagi, Shigeru; Suzuki, Hiroyuki S.; Satoh, Isamu; Komatsubara, Takemi

    2006-01-01

    Microscopic properties have been investigated on a cubic nonmagnetic non-Kramers Γ 3 doublet ground-state (GS) system PrAg 2 In by complementarily utilizing 115 In (I=9/2) and 109 Ag (I=1/2) NMR with particular emphasis on the low-frequency (low-ω) dipole and multipole (octupole and/or quadrupole) fluctuations of f-electrons as probed by the nuclear spin relaxation rates 1/ 115 T 1 and 1/ 109 T 1 . We show that 1/ 115 T 1 and 1/ 109 T 1 are anomalously enhanced respectively below≅50 K and ≅100K over those expected for the low-ω dipole fluctuations of the excited magnetic Γ 4 and Γ 5 states in a simple crystalline-electric-field model for a Γ 3 GS system. By comparing 1/( 115 T 1 T) and 1/( 109 T 1 T) and also by considering an invariant form of the hyperfine and/or quadrupole couplings of Γ 3 octupole and/or quadrupole moments with Ag/In nuclear dipole and/or quadrupole moments, we show that Γ 3 octupole fluctuations dominate 1/ 109 T 1 and quadrupole ones can possibly contribute to 1/ 115 T 1 at low T. (author)

  10. Magnetic structure of MgCu2O3 and doping-induced spin reorientation in Mg1-x/2LixCu2-x/2O3

    DEFF Research Database (Denmark)

    Winkelmann, M.; Graf, H.A.; Andersen, N.H.

    1994-01-01

    The magnetic properties of undoped and Li-doped MgCu2O3 single crystals have been studied by magnetic-susceptibility and neutron-diffraction measurements. The pure compound is a semiconductor with an antiferromagnetic ground state (T(N) = 95 K). Above T(N), short-range magnetic correlations within...... the Cu-O chains of the MgCu2O3 structure give rise to a predominantly one-dimensional (1D) magnetic behavior. This is revealed by the quantitative interpretation of the susceptibility measurements. Below T(N), the 3D magnetic structure, derived from neutron-diffraction experiments, can be described...... is similar to the one producing an infinitely degenerate state in antiferromagnetic fcc lattices. Doping experiments with Li clearly demonstrate the importance of spin fluctuations and fluctuations of the local exchange fields for lifting the degeneracy in such a system. A remarkably small amount of Li...

  11. Room-temperature antiferromagnetic memory resistor.

    Science.gov (United States)

    Marti, X; Fina, I; Frontera, C; Liu, Jian; Wadley, P; He, Q; Paull, R J; Clarkson, J D; Kudrnovský, J; Turek, I; Kuneš, J; Yi, D; Chu, J-H; Nelson, C T; You, L; Arenholz, E; Salahuddin, S; Fontcuberta, J; Jungwirth, T; Ramesh, R

    2014-04-01

    The bistability of ordered spin states in ferromagnets provides the basis for magnetic memory functionality. The latest generation of magnetic random access memories rely on an efficient approach in which magnetic fields are replaced by electrical means for writing and reading the information in ferromagnets. This concept may eventually reduce the sensitivity of ferromagnets to magnetic field perturbations to being a weakness for data retention and the ferromagnetic stray fields to an obstacle for high-density memory integration. Here we report a room-temperature bistable antiferromagnetic (AFM) memory that produces negligible stray fields and is insensitive to strong magnetic fields. We use a resistor made of a FeRh AFM, which orders ferromagnetically roughly 100 K above room temperature, and therefore allows us to set different collective directions for the Fe moments by applied magnetic field. On cooling to room temperature, AFM order sets in with the direction of the AFM moments predetermined by the field and moment direction in the high-temperature ferromagnetic state. For electrical reading, we use an AFM analogue of the anisotropic magnetoresistance. Our microscopic theory modelling confirms that this archetypical spintronic effect, discovered more than 150 years ago in ferromagnets, is also present in AFMs. Our work demonstrates the feasibility of fabricating room-temperature spintronic memories with AFMs, which in turn expands the base of available magnetic materials for devices with properties that cannot be achieved with ferromagnets.

  12. Spin Dynamics and Quantum Tunneling in Fe8 Nanomagnet and in AFM Rings by NMR

    International Nuclear Information System (INIS)

    Seung-Ho-Baek

    2004-01-01

    In this thesis, our main interest has been to investigate the spin dynamics and quantum tunneling in single molecule magnets (SMMs), For this we have selected two different classes of SMMs: a ferrimagnetic total high spin S = 10 cluster Fe8 and antiferromagnetic (AFM) ring-type clusters. For Fe8, our efforts have been devoted to the investigation of the quantum tunneling of magnetization in the very low temperature region. The most remarkable experimental finding in Fe8 is that the nuclear spin-lattice relaxation rate (1/T l ) at low temperatures takes place via strong collision mechanism, and thus it allows to measure directly the tunneling rate vs T and H for the first time. For AFM rings, we have shown that 1/T l probes the thermal fluctuations of the magnetization in the intermediate temperature range. We find that the fluctuations are dominated by a single characteristic frequency which has a power law T-dependence indicative of fluctuations due to electron-acoustic phonon interactions

  13. Spin Dynamics and Quantum Tunneling in Fe8 Nanomagnet and in AFM Rings by NMR

    Energy Technology Data Exchange (ETDEWEB)

    Ho-Baek, Seung [Iowa State Univ., Ames, IA (United States)

    2004-01-01

    In this thesis, our main interest has been to investigate the spin dynamics and quantum tunneling in single molecule magnets (SMMs), For this we have selected two different classes of SMMs: a ferrimagnetic total high spin S = 10 cluster Fe8 and antiferromagnetic (AFM) ring-type clusters. For Fe8, our efforts have been devoted to the investigation of the quantum tunneling of magnetization in the very low temperature region. The most remarkable experimental finding in Fe8 is that the nuclear spin-lattice relaxation rate (1/T{sub l}) at low temperatures takes place via strong collision mechanism, and thus it allows to measure directly the tunneling rate vs T and H for the first time. For AFM rings, we have shown that 1/T{sub l} probes the thermal fluctuations of the magnetization in the intermediate temperature range. We find that the fluctuations are dominated by a single characteristic frequency which has a power law T-dependence indicative of fluctuations due to electron-acoustic phonon interactions.

  14. Spin dynamics and quantum tunneling in Fe8 nanomagnet and in AFM rings by NMR

    Science.gov (United States)

    Baek, Seung-Ho

    In this thesis, our main interest has been to investigate the spin dynamics and quantum tunneling in single molecule magnets (SMMs). For this we have selected two different classes of SMMs: a ferromagnetic total high spin S = 10 cluster Fe8 and antiferromagnetic (AFM) ring-type clusters. For Fe8, our efforts have been devoted to the investigation of the quantum tunneling of magnetization in the very low temperature region. The most remarkable experimental finding in Fe8 is that the nuclear spin-lattice relaxation rate (1/T1) at low temperatures takes place via strong collision mechanism, and thus it allows to measure directly the tunneling rate vs. T and H for the first time. For AFM rings, we have shown that 1/T1 probes the thermal fluctuations of the magnetization in the intermediate temperature range. We find that the fluctuations are dominated by a single characteristic frequency which has a power-law T-dependence indicative of fluctuations due to electron-acoustic phonon interactions.

  15. Percolation and spin glass transition

    International Nuclear Information System (INIS)

    Sadiq, A.; Tahir-Kheli, R.A.; Wortis, M.; Bhatti, N.A.

    1980-10-01

    The behaviour of clusters of curved and normal plaquette particles in a bond random, +-J, Ising model is studied in finite square and triangular lattices. Computer results for the concentration of antiferromagnetic bonds when percolating clusters first appears are found to be close to those reported for the occurrence and disappearance of spin glass phases in these systems. (author)

  16. Spin Filtering in Epitaxial Spinel Films with Nanoscale Phase Separation

    KAUST Repository

    Li, Peng; Xia, Chuan; Li, Jun; Zhu, Zhiyong; Wen, Yan; Zhang, Qiang; Zhang, Junwei; Peng, Yong; Alshareef, Husam N.; Zhang, Xixiang

    2017-01-01

    The coexistence of ferromagnetic metallic phase and antiferromagnetic insulating phase in nanoscaled inhomogeneous perovskite oxides accounts for the colossal magnetoresistance. Although the model of spin-polarized electron transport across

  17. Magnetic correlations in the intermetallic antiferromagnet Nd3Co4Sn13

    Science.gov (United States)

    Wang, C. W.; Lin, J. W.; Lue, C. S.; Liu, H. F.; Kuo, C. N.; Mole, R. A.; Gardner, J. S.

    2017-11-01

    Specific heat, magnetic susceptibility, and neutron scattering have been used to investigate the nature of the spin system in the antiferromagnet Nd3Co4Sn13. At room temperature Nd3Co4Sn13 has a cubic, Pm-3n structure similar to Yb3Rh4Sn13. Antiferromagnetic interactions between, Nd3+ ions dominate the magnetic character of this sample and at 2.4 K the Nd spins enter a long range order state with a magnetic propagation vector q  =  (0 0 0) with an ordered moment of 1.78(2) µ B at 1.5 K. The magnetic Bragg intensity grows very slowly below 1 K, reaching ~2.4 µ B at 350 mK. The average magnetic Nd3+ configuration corresponds to the 3D irreducible representation Γ7. This magnetic structure can be viewed as three sublattices of antiferromagnetic spin chains coupled with each other in the 120°-configuration. A well-defined magnetic excitation was measured around the 1 1 1 zone centre and the resulting dispersion curve is appropriate for an antiferromagnet with a gap of 0.20(1) meV.

  18. Antiferromagnetic MnN layer on the MnGa(001) surface

    Energy Technology Data Exchange (ETDEWEB)

    Guerrero-Sánchez, J., E-mail: guerrero@cnyn.unam.mx; Takeuchi, Noboru

    2016-12-30

    Highlights: • A ferromagnetic Gallium terminated surface is stable before N incorporation. • After N incorporation, an antiferromagnetic MnN layer becomes stable in a wide range of chemical potential. • Spin density distribution shows an antiferromagnetic/ferromagnetic (MnN/MnGa) arrangement at the surface. - Abstract: Spin polarized first principles total energy calculations have been applied to study the stability and magnetic properties of the MnGa(001) surface and the formation of a topmost MnN layer with the deposit of nitrogen. Before nitrogen adsorption, surface formation energies show a stable gallium terminated ferromagnetic surface. After incorporation of nitrogen atoms, the antiferromagnetic manganese terminated surface becomes stable due to the formation of a MnN layer (Mn-N bonding at the surface). Spin density distribution shows a ferromagnetic/antiferromagnetic arrangement in the first surface layers. This thermodynamically stable structure may be exploited to growth MnGa/MnN magnetic heterostructures as well as to look for exchange biased systems.

  19. Controlling the switching field in nanomagnets by means of domain-engineered antiferromagnets

    Science.gov (United States)

    Folven, E.; Linder, J.; Gomonay, O. V.; Scholl, A.; Doran, A.; Young, A. T.; Retterer, S. T.; Malik, V. K.; Tybell, T.; Takamura, Y.; Grepstad, J. K.

    2015-09-01

    Using soft x-ray spectromicroscopy, we investigate the magnetic domain structure in embedded nanomagnets defined in L a0.7S r0.3Mn O3 thin films and LaFe O3/L a0.7S r0.3Mn O3 bilayers. We find that shape-controlled antiferromagnetic domain states give rise to a significant reduction of the switching field of the rectangular nanomagnets. This is discussed within the framework of competition between an intrinsic spin-flop coupling and shape anisotropy. The data demonstrates that shape effects in antiferromagnets may be used to control the magnetic properties in nanomagnets.

  20. A mean field study of the quasi-one-dimensional antiferromagnetic anisotropic Heisenberg model

    International Nuclear Information System (INIS)

    Benyoussef, A.

    1996-10-01

    The effect of the chain and the dimer anisotropies on the ground state energy and the energy gap of the spin-1/2 quasi-one-dimensional antiferromagnetic Heisenberg model is investigated using a mean field theory. The dependence of the magnetization and the effective hopping parameters on the anisotropy α xy (=J xy perpendicular /J xy parallel ) are presented for several values of the chain anisotropy. However, such a system exhibits a transition from antiferromagnetic ordered to disordered phases for arbitrary chain anisotropy and dimer anisotropy. (author). 22 refs, 11 figs

  1. Ground-state candidate for the classical dipolar kagome Ising antiferromagnet

    Science.gov (United States)

    Chioar, I. A.; Rougemaille, N.; Canals, B.

    2016-06-01

    We have investigated the low-temperature thermodynamic properties of the classical dipolar kagome Ising antiferromagnet using Monte Carlo simulations, in the quest for the ground-state manifold. In spite of the limitations of a single-spin-flip approach, we managed to identify certain ordering patterns in the low-temperature regime and we propose a candidate for this unknown state. This configuration presents some intriguing features and is fully compatible with the extrapolations of the at-equilibrium thermodynamic behavior sampled so far, making it a very likely choice for the dipolar long-range ordered state of the classical kagome Ising antiferromagnet.

  2. Magnetocaloric properties of a frustrated Blume-Capel antiferromagnet

    Directory of Open Access Journals (Sweden)

    Žukovič Milan

    2014-07-01

    Full Text Available Low-temperature magnetization processes and magnetocaloric properties of a geometrically frustrated spin-1 Blume-Capel model on a triangular lattice are studied by Monte Carlo simulations. The model is found to display qualitatively different behavior depending on the sign of the single-ion anisotropy D. For positive values of D we observe two magnetization plateaus, similar to the spin-1/2 Ising antiferromagnet, and negative isothermal entropy changes for any field intensity. For a range of small negative values of D there are four magnetization plateaus and the entropy changes can be either negative or positive, depending on the field. If D is negative but large in absolute value then the entropy changes are solely positive.

  3. Evolution of topological features in finite antiferromagnetic Heisenberg chains

    International Nuclear Information System (INIS)

    Chen Changfeng

    2003-01-01

    We examine the behavior of nonlocal topological order in finite antiferromagnetic Heisenberg chains using the density matrix renormalization group techniques. We find that chains with even and odd site parity show very different behavior in the topological string order parameter, reflecting interesting interplay of the intrinsic magnetic correlation and the topological term in the chains. Analysis of the calculated string order parameter as a function of the chain length and the topological angle indicates that S=1/2 and S=1 chains show special behavior while all S>1 chains have similar topological structure. This result supports an earlier conjecture on the classification of quantum spin chains based on an analysis of their phase diagrams. Implications of the topological behavior in finite quantum spin chains are discussed

  4. Spintronic materials and devices based on antiferromagnetic metals

    Directory of Open Access Journals (Sweden)

    Y.Y. Wang

    2017-04-01

    Full Text Available In this paper, we review our recent experimental developments on antiferromagnet (AFM spintronics mainly comprising Mn-based noncollinear AFM metals. IrMn-based tunnel junctions and Hall devices have been investigated to explore the manipulation of AFM moments by magnetic fields, ferromagnetic materials and electric fields. Room-temperature tunneling anisotropic magnetoresistance based on IrMn as well as FeMn has been successfully achieved, and electrical control of the AFM exchange spring is realized by adopting ionic liquid. In addition, promising spin-orbit effects in AFM as well as spin transfer via AFM spin waves reported by different groups have also been reviewed, indicating that the AFM can serve as an efficient spin current source. To explore the crucial role of AFM acting as efficient generators, transmitters, and detectors of spin currents is an emerging topic in the field of magnetism today. AFM metals are now ready to join the rapidly developing fields of basic and applied spintronics, enriching this area of solid-state physics and microelectronics.

  5. Spin Current Noise of the Spin Seebeck Effect and Spin Pumping

    Science.gov (United States)

    Matsuo, M.; Ohnuma, Y.; Kato, T.; Maekawa, S.

    2018-01-01

    We theoretically investigate the fluctuation of a pure spin current induced by the spin Seebeck effect and spin pumping in a normal-metal-(NM-)ferromagnet(FM) bilayer system. Starting with a simple ferromagnet-insulator-(FI-)NM interface model with both spin-conserving and non-spin-conserving processes, we derive general expressions of the spin current and the spin-current noise at the interface within second-order perturbation of the FI-NM coupling strength, and estimate them for a yttrium-iron-garnet-platinum interface. We show that the spin-current noise can be used to determine the effective spin carried by a magnon modified by the non-spin-conserving process at the interface. In addition, we show that it provides information on the effective spin of a magnon, heating at the interface under spin pumping, and spin Hall angle of the NM.

  6. Anisotropic Magnetoresistance in Antiferromagnetic Sr_{2}IrO_{4}

    Directory of Open Access Journals (Sweden)

    C. Wang

    2014-11-01

    Full Text Available We report point-contact measurements of anisotropic magnetoresistance (AMR in a single crystal of antiferromagnetic Mott insulator Sr_{2}IrO_{4}. The point-contact technique is used here as a local probe of magnetotransport properties on the nanoscale. The measurements at liquid nitrogen temperature reveal negative magnetoresistances (up to 28% for modest magnetic fields (250 mT applied within the IrO_{2} a-b plane and electric currents flowing perpendicular to the plane. The angular dependence of magnetoresistance shows a crossover from fourfold to twofold symmetry in response to an increasing magnetic field with angular variations in resistance from 1% to 14%. We tentatively attribute the fourfold symmetry to the crystalline component of AMR and the field-induced transition to the effects of applied field on the canting of antiferromagnetic-coupled moments in Sr_{2}IrO_{4}. The observed AMR is very large compared to the crystalline AMRs in 3d transition metal alloys or oxides (0.1%–0.5% and can be associated with the large spin-orbit interactions in this 5d oxide while the transition provides evidence of correlations between electronic transport, magnetic order, and orbital states. The finding of this work opens an entirely new avenue to not only gain a new insight into physics associated with spin-orbit coupling but also to better harness the power of spintronics in a more technically favorable fashion.

  7. Electrical control of antiferromagnetic metal up to 15 nm

    Science.gov (United States)

    Zhang, PengXiang; Yin, GuFan; Wang, YuYan; Cui, Bin; Pan, Feng; Song, Cheng

    2016-08-01

    Manipulation of antiferromagnetic (AFM) spins by electrical means is on great demand to develop the AFM spintronics with low power consumption. Here we report a reversible electrical control of antiferromagnetic moments of FeMn up to 15 nm, using an ionic liquid to exert a substantial electric-field effect. The manipulation is demonstrated by the modulation of exchange spring in [Co/Pt]/FeMn system, where AFM moments in FeMn pin the magnetization rotation of Co/Pt. By carrier injection or extraction, the magnetic anisotropy of the top layer in FeMn is modulated to influence the whole exchange spring and then passes its influence to the [Co/Pt]/FeMn interface, through a distance up to the length of exchange spring that fully screens electric field. Comparing FeMn to IrMn, despite the opposite dependence of exchange bias on gate voltages, the same correlation between carrier density and exchange spring stiffness is demonstrated. Besides the fundamental significance of modulating the spin structures in metallic AFM via all-electrical fashion, the present finding would advance the development of low-power-consumption AFM spintronics.

  8. Spinon confinement in a quasi-one-dimensional XXZ Heisenberg antiferromagnet

    Science.gov (United States)

    Lake, Bella; Bera, Anup K.; Essler, Fabian H. L.; Vanderstraeten, Laurens; Hubig, Claudius; Schollwock, Ulrich; Islam, A. T. M. Nazmul; Schneidewind, Astrid; Quintero-Castro, Diana L.

    Half-integer spin Heisenberg chains constitute a key paradigm for quantum number fractionalization: flipping a spin creates a minimum of two elementary spinon excitations. These have been observed in numerous experiments. We report on inelastic neutron scattering experiments on the quasi-one-dimensional anisotropic spin-1/2 Heisenberg antiferromagnet SrCo2V2O8. These reveal a mechanism for temperature-induced spinon confinement, manifesting itself in the formation of sequences of spinon bound states. A theoretical description of this effect is achieved by a combination of analytical and numerical methods.

  9. Itinerant-electron antiferromagnetism precursor to superconductivity in an organic conductor

    International Nuclear Information System (INIS)

    Walsh, W.M. Jr.; Wudl, F.; Aharon-Shalom, E.; Rupp, L.W. Jr.; Vandenberg, J.M.; Andres, K.; Torrance, J.B.

    1982-01-01

    Below 5.5 K minimally strained crystals of (TMTSF) 2 ClO 4 (TMTSF: tetramethyltetraselenafulvalene) exhibit vanishing spin-resonance intensity and reduced conductivity at low microwave power. More intense microwave electric fields along the needle axis nonlinearly restore both the resonance signal and the conductivity, indicating the presence of charged spin-density waves. Very anisotropic antiferromagnetic resonances are observed at 1.6 K, confirming that an intinerant spin-density-wave state precedes the onset of superconductivity at 1.3 K

  10. The 120° Ordered Phase of Triangular Lattice Antiferromagnetic Heisenberg Model with Long Range Couplings

    International Nuclear Information System (INIS)

    Zhan-Hai, Dong

    2009-01-01

    In order to look for the 120° order phase of triangular lattice Heisenberg antiferromagnet with long range couplings, the Hamiltonian is diagonalized with the Bogoliubov transformation within linear spin-wave approximation. It is found that when the long range spin couplings are taken into account, the transformation is valid only for certain regions in the spin coupling parameter space. These regions just correspond to the 120° (or Néel) ordered phase, which is very different from square lattice in terms of shape, size and topological property

  11. Coupled Quantum Fluctuations and Quantum Annealing

    Science.gov (United States)

    Hormozi, Layla; Kerman, Jamie

    We study the relative effectiveness of coupled quantum fluctuations, compared to single spin fluctuations, in the performance of quantum annealing. We focus on problem Hamiltonians resembling the the Sherrington-Kirkpatrick model of Ising spin glass and compare the effectiveness of different types of fluctuations by numerically calculating the relative success probabilities and residual energies in fully-connected spin systems. We find that for a small class of instances coupled fluctuations can provide improvement over single spin fluctuations and analyze the properties of the corresponding class. Disclaimer: This research was funded by ODNI, IARPA via MIT Lincoln Laboratory under Air Force Contract No. FA8721-05-C-0002. The views and conclusions contained herein are those of the authors and should not be interpreted as necessarily representing the official policies or endorsements, either expressed or implied, of ODNI, IARPA, or the US Government.

  12. Dynamics of Coupled Quantum Spin Chains

    International Nuclear Information System (INIS)

    Schulz, H.J.

    1996-01-01

    Static and dynamical properties of weakly coupled antiferromagnetic spin chains are treated using a mean-field approximation for the interchain coupling and exact results for the resulting effective one-dimensional problem. Results for staggered magnetization, Nacute eel temperature, and spin wave excitations are in agreement with experiments on KCuF 3 . The existence of a narrow longitudinal mode is predicted. The results are in agreement with general scaling arguments, contrary to spin wave theory. copyright 1996 The American Physical Society

  13. NMR studies of spin dynamics in cuprates

    International Nuclear Information System (INIS)

    Takigawa, M.; Mitzi, D.B.

    1994-01-01

    The authors report recent NMR results in cuprates. The oxygen Knight shift and the Cu nuclear spin-lattice relaxation rate in Bi 2.1 Sr 1.94 Ca 0.88 Cu 2.07 O 8+σ single crystals revealed a gapless superconducting state, which can be most naturally explained by a d-wave pairing state and the intrinsic disorder in this material. The Cu nuclear spin-spin relaxation rate in underdoped YBa 2 Cu 3 O 6.63 shows distinct temperature dependence from the spin-lattice relaxation rate, providing direct evidence for a pseudo spin-gap near the antiferromagnetic wave vector

  14. NMR studies of spin dynamics in cuprates

    Science.gov (United States)

    Takigawa, M.; Mitzi, D. B.

    1994-04-01

    We report recent NMR results in cuprates. The oxygen Knight shift and the Cu nuclear spin-lattice relaxation rate in Bi2.1Sr1.94Ca0.88Cu2.07O8+δ single crystals revealed a gapless superconducting state, which can be most naturally explained by a d-wave pairing state and the intrinsic disorder in this material. The Cu nuclear spin-spin relaxation rate in underdoped YBa2Cu3O6.63 shows distinct temperature dependence from the spin-lattice relaxation rate, providing direct evidence for a pseudo spin-gap near the antiferromagnetic wave vector.

  15. GPU-Accelerated Population Annealing Algorithm: Frustrated Ising Antiferromagnet on the Stacked Triangular Lattice

    Directory of Open Access Journals (Sweden)

    Borovský Michal

    2016-01-01

    Full Text Available The population annealing algorithm is a novel approach to study systems with rough free-energy landscapes, such as spin glasses. It combines the power of simulated annealing, Boltzmann weighted differential reproduction and sequential Monte Carlo process to bring the population of replicas to the equilibrium even in the low-temperature region. Moreover, it provides a very good estimate of the free energy. The fact that population annealing algorithm is performed over a large number of replicas with many spin updates, makes it a good candidate for massive parallelism. We chose the GPU programming using a CUDA implementation to create a highly optimized simulation. It has been previously shown for the frustrated Ising antiferromagnet on the stacked triangular lattice with a ferromagnetic interlayer coupling, that standard Markov Chain Monte Carlo simulations fail to equilibrate at low temperatures due to the effect of kinetic freezing of the ferromagnetically ordered chains. We applied the population annealing to study the case with the isotropic intra- and interlayer antiferromagnetic coupling (J2/|J1| = −1. The reached ground states correspond to non-magnetic degenerate states, where chains are antiferromagnetically ordered, but there is no long-range ordering between them, which is analogical with Wannier phase of the 2D triangular Ising antiferromagnet.

  16. Quasi-one-dimensional Heisenberg antiferromagnetic model for an organic polymeric chain

    International Nuclear Information System (INIS)

    Wu, F; Wang, W Z

    2006-01-01

    Using the exact diagonalization technique, we study the properties of the ground state of a spin-1/2 antiferromagnetic Heisenberg model for a zigzag polymer chain with side radicals connected to the even sites. We consider the nearest-neighbour exchange J and the next-nearest-neighbour exchange αJ along the main chain, and J 1 between the even site on the main chain and the radical site. For small α the ground state is ferrimagnetic. For α>α c1 , the ground state is a spiral phase, which is characterized by a peak of the static structure factor S(q) locating at an incommensurate value q max . For α>α c2 , the ground state is antiferromagnetic. With increasing J 1 , α c1 decreases while α c2 has a maximum at about J 1 = 0.5. For very small J 1 and α = 0.5, the spin configuration on the main chain is a product of nearest-neighbour singlets. In the antiferromagnetic phase, if J 1 is large enough the even site and the radical site form a singlet with exchange-decoupling from the odd site while the odd sites approximately form an antiferromagnetic chain

  17. Precessional switching of antiferromagnets by electric field induced Dzyaloshinskii-Moriya torque

    Science.gov (United States)

    Kim, T. H.; Grünberg, P.; Han, S. H.; Cho, B. K.

    2018-05-01

    Antiferromagnetic insulators (AFIs) have attracted much interest from many researchers as promising candidates for use in ultrafast, ultralow-dissipation spintronic devices. As a fast method of reversing magnetization, precessional switching is realized when antiferromagnetic Néel orders l =(s1+s2 )/2 surmount the magnetic anisotropy or potential barrier in a given magnetic system, which is described well by the antiferromagnetic plane pendulum (APP) model. Here, we report that, as an alternative switching scenario, the direct coupling of an electric field with Dzyaloshinskii-Moriya (DM) interaction, which stems from spin-orbit coupling, is exploited for optimal switching. We derive the pendulum equation of motion of antiferromagnets, where DM torque is induced by a pulsed electric field. The temporal DM interaction is found to not only be in the form of magnetic torques (e.g., spin-orbit torque or magnetic field) but also modifies the magnetic potential that limits l 's activity; as a result, appropriate controls (e.g., direction, magnitude, and pulse shape) of the induced DM vector realize deterministic reversal in APP. The results present an approach for the control of a magnetic storage device by means of an electric field.

  18. Hybrid excitations due to crystal field, spin-orbit coupling, and spin waves in LiFePO4

    Science.gov (United States)

    Yiu, Yuen; Le, Manh Duc; Toft-Peterson, Rasmus; Ehlers, Georg; McQueeney, Robert J.; Vaknin, David

    2017-03-01

    We report on the spin waves and crystal field excitations in single crystal LiFePO4 by inelastic neutron scattering over a wide range of temperatures, below and above the antiferromagnetic transition of this system. In particular, we find extra excitations below TN=50 K that are nearly dispersionless and are most intense around magnetic zone centers. We show that these excitations correspond to transitions between thermally occupied excited states of Fe2 + due to splitting of the S =2 levels that arise from the crystal field and spin-orbit interactions. These excitations are further amplified by the highly distorted nature of the oxygen octahedron surrounding the iron atoms. Above TN, magnetic fluctuations are observed up to at least 720 K, with an additional inelastic excitation around 4 meV, which we attribute to single-ion effects, as its intensity weakens slightly at 720 K compared to 100 K, which is consistent with the calculated cross sections using a single-ion model. Our theoretical analysis, using the MF-RPA model, provides both detailed spectra of the Fe d shell and estimates of the average ordered magnetic moment and TN. By applying the MF-RPA model to a number of existing spin-wave results from other Li M PO4 (M =Mn , Co, and Ni), we are able to obtain reasonable predictions for the moment sizes and transition temperatures.

  19. Spin thermoelectric effects in organic single-molecule devices

    Energy Technology Data Exchange (ETDEWEB)

    Wang, H.L.; Wang, M.X.; Qian, C.; Hong, X.K.; Zhang, D.B.; Liu, Y.S.; Yang, X.F., E-mail: xfyang@cslg.edu.cn

    2017-05-25

    Highlights: • A stronger spin thermoelectric performance in a polyacetylene device is observed. • For the antiferromagnetic (AFM) ordering, a transport gap is opened. Thus the thermoelectric effects are largely enhanced. - Abstract: The spin thermoelectric performance of a polyacetylene chain bridging two zigzag graphene nanoribbons (ZGNRs) is investigated based on first principles method. Two different edge spin arrangements in ZGNRs are considered. For ferromagnetic (FM) ordering, transmission eigenstates with different spin indices distributed below and above Fermi level are observed, leading directly to a strong spin thermoelectric effect in a wide temperature range. With the edge spins arranged in the antiferromagnetic (AFM) ordering, an obvious transport gap appears in the system, which greatly enhances the thermoelectric effects. The presence of a small spin splitting also induces a spin thermoelectric effect greater than the charge thermoelectric effect in certain temperature range. In general, the single-molecule junction exhibits the potential to be used for the design of perfect thermospin devices.

  20. 133Cs NMR investigation of 2D frustrated Heisenberg antiferromagnet, Cs2CuCl4

    Science.gov (United States)

    Vachon, M.-A.; Kundhikanjana, W.; Straub, A.; Mitrovic, V. F.; Reyes, A. P.; Kuhns, P.; Coldea, R.; Tylczynski, Z.

    2006-10-01

    We report 133Cs nuclear magnetic resonance (NMR) measurements on the 2D frustrated Heisenberg antiferromagnet Cs2CuCl4 down to 2 K and up to 15 T. We show that 133Cs NMR is a good probe of the magnetic degrees of freedom in this material. Cu spin degrees of freedom are sensed through a strong anisotropic hyperfine coupling. The spin excitation gap opens above the critical saturation field. The gap value was determined from the activation energy of the nuclear spin-lattice relaxation rate in a magnetic field applied parallel to the Cu chains (\\skew3\\hat{b} axis). The values of the g-factor and the saturation field are consistent with the neutron-scattering and magnetization results. The measurements of the spin spin relaxation time are exploited to show that no structural changes occur down to the lowest temperatures investigated.

  1. Excitation spectrum of Heisenberg spin ladders

    International Nuclear Information System (INIS)

    Barnes, T.; Dagotto, E.; Riera, J.; Swanson, E.S.

    1993-01-01

    Heisenberg antiferromagnetic spin ''ladders'' (two coupled spin chains) are low-dimensional magnetic systems which for S=1/2 interpolate between half-integer-spin chains, when the chains are decoupled, and effective integer-spin one-dimensional chains in the strong-coupling limit. The spin-1/2 ladder may be realized in nature by vanadyl pyrophosphate, (VO) 2 P 2 O 7 . In this paper we apply strong-coupling perturbation theory, spin-wave theory, Lanczos techniques, and a Monte Carlo method to determine the ground-state energy and the low-lying excitation spectrum of the ladder. We find evidence of a nonzero spin gap for all interchain couplings J perpendicular >0. A band of spin-triplet excitations above the gap is also analyzed. These excitations are unusual for an antiferromagnet, since their long-wavelength dispersion relation behaves as (k-k 0 ) 2 (in the strong-coupling limit J perpendicular much-gt J, where J is the in-chain antiferromagnetic coupling). Their band is folded, with a minimum energy at k 0 =π, and a maximum between k 1 =π/2 (for J perpendicular =0) and 0 (for J perpendicular =∞). We also give numerical results for the dynamical structure factor S(q,ω), which can be determined in neutron scattering experiments. Finally, possible experimental techniques for studying the excitation spectrum are discussed

  2. The fluctuating gap model

    Energy Technology Data Exchange (ETDEWEB)

    Cao, Xiaobin

    2011-01-15

    The quasi-one-dimensional systems exhibit some unusual phenomenon, such as the Peierls instability, the pseudogap phenomena and the absence of a Fermi-Dirac distribution function line shape in the photoemission spectroscopy. Ever since the discovery of materials with highly anisotropic properties, it has been recognized that fluctuations play an important role above the three-dimensional phase transition. This regime where the precursor fluctuations are presented can be described by the so called fluctuating gap model (FGM) which was derived from the Froehlich Hamiltonian to study the low energy physics of the one-dimensional electron-phonon system. Not only is the FGM of great interest in the context of quasi-one-dimensional materials, liquid metal and spin waves above T{sub c} in ferromagnets, but also in the semiclassical approximation of superconductivity, it is possible to replace the original three-dimensional problem by a directional average over effectively one-dimensional problem which in the weak coupling limit is described by the FGM. In this work, we investigate the FGM in a wide temperature range with different statistics of the order parameter fluctuations. We derive a formally exact solution to this problem and calculate the density of states, the spectral function and the optical conductivity. In our calculation, we show that a Dyson singularity appears in the low energy density of states for Gaussian fluctuations in the commensurate case. In the incommensurate case, there is no such kind of singularity, and the zero frequency density of states varies differently as a function of the correlation lengths for different statistics of the order parameter fluctuations. Using the density of states we calculated with non-Gaussian order parameter fluctuations, we are able to calculate the static spin susceptibility which agrees with the experimental data very well. In the calculation of the spectral functions, we show that as the correlation increases, the

  3. The fluctuating gap model

    International Nuclear Information System (INIS)

    Cao, Xiaobin

    2011-01-01

    The quasi-one-dimensional systems exhibit some unusual phenomenon, such as the Peierls instability, the pseudogap phenomena and the absence of a Fermi-Dirac distribution function line shape in the photoemission spectroscopy. Ever since the discovery of materials with highly anisotropic properties, it has been recognized that fluctuations play an important role above the three-dimensional phase transition. This regime where the precursor fluctuations are presented can be described by the so called fluctuating gap model (FGM) which was derived from the Froehlich Hamiltonian to study the low energy physics of the one-dimensional electron-phonon system. Not only is the FGM of great interest in the context of quasi-one-dimensional materials, liquid metal and spin waves above T c in ferromagnets, but also in the semiclassical approximation of superconductivity, it is possible to replace the original three-dimensional problem by a directional average over effectively one-dimensional problem which in the weak coupling limit is described by the FGM. In this work, we investigate the FGM in a wide temperature range with different statistics of the order parameter fluctuations. We derive a formally exact solution to this problem and calculate the density of states, the spectral function and the optical conductivity. In our calculation, we show that a Dyson singularity appears in the low energy density of states for Gaussian fluctuations in the commensurate case. In the incommensurate case, there is no such kind of singularity, and the zero frequency density of states varies differently as a function of the correlation lengths for different statistics of the order parameter fluctuations. Using the density of states we calculated with non-Gaussian order parameter fluctuations, we are able to calculate the static spin susceptibility which agrees with the experimental data very well. In the calculation of the spectral functions, we show that as the correlation increases, the quasi

  4. Thermal conductivity of the vortex lattice state involving the antiferromagnetism around the core

    International Nuclear Information System (INIS)

    Takigawa, Mitsuaki; Ichioka, Masanori; Machida, Kazushige

    2004-01-01

    The thermal conductivity κ xx is the difference between higher and lower temperature regions, because the spatially-resolved thermal conductivity κ xx (r) is localized around the vortex core at lower temperature and delocalized at higher temperature. On one hand, much attention is focused on the spin and charge ordering around the vortex. When the antiferromagnetism appears around the core, the energy gap suppresses the density of states on the Fermi energy, and the zero-energy peak at the vortex core splits or vanishes. The κ xx under the Neel temperature is suppressed by the antiferromagnetism. We solve the Bogoliubov-de Gennes equation self-consistently by two-dimensional extended Hubbard model including the repulsive interaction U, and calculate the κ xx on the basis of the linear response theory. The picture of the spatial variation of the thermal conductivity κ(r) through the spin resolved local DOS well explains recent experiments

  5. Breatherlike electromagnetic wave propagation in an antiferromagnetic medium with Dzyaloshinsky-Moriya interaction

    International Nuclear Information System (INIS)

    Kavitha, L.; Saravanan, M.; Srividya, B.; Gopi, D.

    2011-01-01

    We investigate the nature of propagation of electromagnetic waves (EMWs) in an antiferromagnetic medium with Dzyaloshinsky-Moriya (DM) interaction environment. The interplay of bilinear and DM exchange spin coupling with the magnetic field component of the EMW has been studied by solving Maxwell's equations coupled with a nonlinear spin equation for the magnetization of the medium. We made a nonuniform expansion of the magnetization and magnetic field along the direction of propagation of EMW, in the framework of reductive perturbation method, and the dynamics of the system is found to be governed by a generalized derivative nonlinear Schroedinger (DNLS) equation. We employ the Jacobi-elliptic function method to solve the DNLS equation, and the electromagnetic wave propagation in an antiferromagnetic medium is governed by the breatherlike spatially and temporally coherent localized modes under the influence of DM interaction parameter.

  6. Magnetic properties of CsCrCl/sub 3/, an antiferromagnetic chain compound with single-ion anisotropy

    Energy Technology Data Exchange (ETDEWEB)

    Day, P; Gregson, A K; Leech, D H [Oxford Univ. (UK). Inorganic Chemistry Lab.; Hutchings, M T [UKAEA Atomic Energy Research Establishment, Harwell. Materials Physics Div.; Rainford, B D [Imperial Coll. of Science and Technology, London (UK). Dept. of Physics

    1979-01-01

    The magnetic structure and excitations of the linear chain hexagonal perovskite salt CsCrCl/sub 3/ have been studied by susceptibility, powder and single crystal neutron diffraction, and coherent inelastic neutron scattering. Below the Neel temperature, Tsub(N) = 16 K, the spins lie in the basal plane with antiferromagnetic ordering along the c-axis chains. At 4.5 K there is strong dispersion of the spin-wave energy along c but no measurable dispersion perpendicular to c.

  7. Contrasting dynamic spin susceptibility models and their relation to high-temperature superconductivity

    International Nuclear Information System (INIS)

    Schuettler, H.; Norman, M.R.

    1996-01-01

    We compare the normal-state resistivities ρ and the critical temperatures T c for superconducting d x 2 -y 2 pairing due to antiferromagnetic (AF) spin fluctuation exchange in the context of two phenomenological dynamical spin susceptibility models for the cuprate high-T c materials, one based on fits to NMR data on Y-Ba-Cu-O (YBCO) proposed by Millis, Monien, and Pines (MMP) and Monthoux and Pines (MP), and the other based on fits to neutron scattering data on YBCO proposed by Radtke, Ullah, Levin, and Norman (RULN). Assuming comparable electronic bandwidths and resistivities in both models, we show that the RULN model gives a much lower d-wave T c (approx-lt 20 K) than the MMP model (with T c ∼100 K). We demonstrate that these profound differences in the T c close-quote s arise from fundamental differences in the spectral weight distributions of the two model susceptibilities at high (>100 meV) frequencies and are not primarily caused by differences in the calculational techniques employed by MP and RULN. Further neutron scattering experiments, to explore the spectral weight distribution at all wave vectors over a sufficiently large excitation energy range, will thus be of crucial importance to resolve the question whether AF spin fluctuation exchange can provide a viable mechanism to account for high-T c superconductivity. Limitations of the Migdal-Eliashberg approach in such models will be discussed. copyright 1996 The American Physical Society

  8. Dynamic rotor mode in antiferromagnetic nanoparticles

    DEFF Research Database (Denmark)

    Lefmann, Kim; Jacobsen, H.; Garde, J.

    2015-01-01

    We present experimental, numerical, and theoretical evidence for an unusual mode of antiferromagnetic dynamics in nanoparticles. Elastic neutron scattering experiments on 8-nm particles of hematite display a loss of diffraction intensity with temperature, the intensity vanishing around 150 K...

  9. Magnetic hysteresis and domain wall dynamics in single chain magnets with antiferromagnetic interchain coupling

    Energy Technology Data Exchange (ETDEWEB)

    Bukharov, A A; Ovchinnikov, A S; Baranov, N V [Department of Physics, Ural State University, Ekaterinburg, 620083 (Russian Federation); Inoue, K [Institute for Advanced Materials Research, Hiroshima University, Hiroshima (Japan)

    2010-11-03

    Using Monte Carlo simulations we investigate magnetic hysteresis in two- and three-dimensional systems of weakly antiferromagnetically coupled spin chains based on a scenario of domain wall (kink) motion within the chains. By adapting the model of walkers to simulate the domain wall dynamics and using the Ising-like dipole-dipole model, we study the effects of interchain coupling, temperature and anisotropy axis direction on hysteresis curves.

  10. Photo-induced antiferromagnetic interlayer coupling in Fe superlattices with iron silicide spacers

    Energy Technology Data Exchange (ETDEWEB)

    Mattson, J.E.; Fullerton, E.E.; Kumar, S.; Lee, S.R.; Sowers, C.H.; Grimsditch, M.; Bader, S.D. [Argonne National Lab., IL (United States); Parker, F.T. [California Univ., San Diego, La Jolla, CA (United States). Center for Magnetic Recording Research

    1993-09-01

    Sputtered Fe/FeSi films possessing antiferromagnetic (AF) interlayer coupling at room temperature develop ferromagnetic remanence when cooled below 100K, but the AF coupling can be restored at low temperature by exposure to visible light of sufficient intensity (>10 mW/mm{sup 2}). We attribute these effects to charge carriers in the FeSi spacer layer which, when thermally or photo-generated, are capable of communicating spin information between the Fe layers.

  11. Energy of the amplitude mode in the bicubic antiferromagnet: Series expansion results

    Science.gov (United States)

    Oitmaa, J.

    2018-05-01

    Series expansion methods are used to study the quantum critical behavior of the bicubic spin-1/2 antiferromagnet. Excitation energies are computed throughout the Brillouin zone, for both the Néel and dimer phases. We compute the energy of the amplitude/Higgs mode and show that it becomes degenerate with the magnon modes at the quantum critical point, as expected on general symmetry grounds.

  12. Spinon Attraction in Spin-1/2 Antiferromagnetic Chains

    International Nuclear Information System (INIS)

    Bernevig, B. A.; Giuliano, D.; Laughlin, R. B.

    2001-01-01

    We derive the representation of the two-spinon wave function for the Haldane-Shastry model in terms of the spinon coordinates. This result allows us to rigorously analyze spinon interaction and its physical effects. We show that spinons attract one another. The attraction gets stronger as the size of the system is increased and, in the thermodynamic limit, determines the power law with which the susceptibility diverges

  13. Spin texture motion in antiferromagnetic and ferromagnetic nanowires

    Czech Academy of Sciences Publication Activity Database

    Rodrigues, D.R.; Everschor-Sitte, K.; Tretiakov, O.A.; Sinova, Jairo; Abanov, A.

    2017-01-01

    Roč. 95, č. 17 (2017), s. 1-7, č. článku 174408. ISSN 2469-9950 R&D Projects: GA ČR GB14-37427G EU Projects: European Commission(XE) 610115 - SC2 Institutional support: RVO:68378271 Keywords : orbit torques * magnetization * spintronics Subject RIV: BM - Solid Matter Physics ; Magnetism OBOR OECD: Condensed matter physics (including formerly solid state physics, supercond.) Impact factor: 3.836, year: 2016

  14. Quantum critical scaling and fluctuations in Kondo lattice materials

    Science.gov (United States)

    Yang, Yi-feng; Pines, David; Lonzarich, Gilbert

    2017-01-01

    We propose a phenomenological framework for three classes of Kondo lattice materials that incorporates the interplay between the fluctuations associated with the antiferromagnetic quantum critical point and those produced by the hybridization quantum critical point that marks the end of local moment behavior. We show that these fluctuations give rise to two distinct regions of quantum critical scaling: Hybridization fluctuations are responsible for the logarithmic scaling in the density of states of the heavy electron Kondo liquid that emerges below the coherence temperature T∗, whereas the unconventional power law scaling in the resistivity that emerges at lower temperatures below TQC may reflect the combined effects of hybridization and antiferromagnetic quantum critical fluctuations. Our framework is supported by experimental measurements on CeCoIn5, CeRhIn5, and other heavy electron materials. PMID:28559308

  15. Quantum spin liquids in the absence of spin-rotation symmetry: Application to herbertsmithite

    Science.gov (United States)

    Dodds, Tyler; Bhattacharjee, Subhro; Kim, Yong Baek

    2013-12-01

    It has been suggested that the nearest-neighbor antiferromagnetic Heisenberg model on the Kagome lattice may be a good starting point for understanding the spin-liquid behavior discovered in herbertsmithite. In this work, we investigate possible quantum spin liquid phases in the presence of spin-rotation symmetry-breaking perturbations such as Dzyaloshinskii-Moriya and Ising interactions, as well as second-neighbor antiferromagnetic Heisenberg interactions. Experiments suggest that such perturbations are likely to be present in herbertsmithite. We use the projective symmetry group analysis within the framework of the slave-fermion construction of quantum spin liquid phases and systematically classify possible spin liquid phases in the presence of perturbations mentioned above. The dynamical spin-structure factor for relevant spin liquid phases is computed and the effect of those perturbations are studied. Our calculations reveal dispersive features in the spin structure factor embedded in a generally diffuse background due to the existence of fractionalized spin-1/2 excitations called spinons. For two of the previously proposed Z2 states, the dispersive features are almost absent, and diffuse scattering dominates over a large energy window throughout the Brillouin zone. This resembles the structure factor observed in recent inelastic neutron-scattering experiments on singlet crystals of herbertsmithite. Furthermore, one of the Z2 states with the spin structure factor with mostly diffuse scattering is gapped, and it may be adiabatically connected to the gapped spin liquid state observed in recent density-matrix renormalization group calculations for the nearest-neighbor antiferromagnetic Heisenberg model. The perturbations mentioned above are found to enhance the diffuse nature of the spin structure factor and reduce the momentum dependencies of the spin gap. We also calculate the electron spin resonance (ESR) absorption spectra that further characterize the role of

  16. Stability of the antiferromagnetic state in the electron doped iridates

    Science.gov (United States)

    Bhowal, Sayantika; Moradi Kurdestany, Jamshid; Satpathy, Sashi

    2018-06-01

    Iridates such as Sr2IrO4 are of considerable interest owing to the formation of the Mott insulating state driven by a large spin–orbit coupling. However, in contrast to the expectation from the Nagaoka theorem that a single doped hole or electron destroys the anti-ferromagnetic (AFM) state of the half-filled Hubbard model in the large U limit, the anti-ferromagnetism persists in the doped Iridates for a large dopant concentration beyond half-filling. With a tight-binding description of the relevant states by the third-neighbor (t 1, t 2, t 3, U) Hubbard model on the square lattice, we examine the stability of the AFM state to the formation of a spin spiral state in the strong coupling limit. The third-neighbor interaction t 3 is important for the description of the Fermi surface of the electron doped system. A phase diagram in the parameter space is obtained for the regions of stability of the AFM state. Our results qualitatively explain the robustness of the AFM state in the electron doped iridate (such as Sr2‑x La x IrO4), observed in many experiments, where the AFM state continues to be stable until a critical dopant concentration.

  17. Magnon-induced superconductivity in a topological insulator coupled to ferromagnetic and antiferromagnetic insulators

    Science.gov (United States)

    Hugdal, Henning G.; Rex, Stefan; Nogueira, Flavio S.; Sudbø, Asle

    2018-05-01

    We study the effective interactions between Dirac fermions on the surface of a three-dimensional topological insulator due to the proximity coupling to the magnetic fluctuations in a ferromagnetic or antiferromagnetic insulator. Our results show that the magnetic fluctuations can mediate attractive interactions between Dirac fermions of both Amperean and BCS types. In the ferromagnetic case, we find pairing between fermions with parallel momenta, so-called Amperean pairing, whenever the effective Lagrangian for the magnetic fluctuations does not contain a quadratic term. The pairing interaction also increases with increasing Fermi momentum and is in agreement with previous studies in the limit of high chemical potential. If a quadratic term is present, the pairing is instead of BCS type above a certain chemical potential. In the antiferromagnetic case, BCS pairing occurs when the ferromagnetic coupling between magnons on the same sublattice exceeds the antiferromagnetic coupling between magnons on different sublattices. Outside this region in parameter space, we again find that Amperean pairing is realized.

  18. Antiferromagnetic order in the Hubbard model on the Penrose lattice

    Science.gov (United States)

    Koga, Akihisa; Tsunetsugu, Hirokazu

    2017-12-01

    We study an antiferromagnetic order in the ground state of the half-filled Hubbard model on the Penrose lattice and investigate the effects of quasiperiodic lattice structure. In the limit of infinitesimal Coulomb repulsion U →+0 , the staggered magnetizations persist to be finite, and their values are determined by confined states, which are strictly localized with thermodynamics degeneracy. The magnetizations exhibit an exotic spatial pattern, and have the same sign in each of cluster regions, the size of which ranges from 31 sites to infinity. With increasing U , they continuously evolve to those of the corresponding spin model in the U =∞ limit. In both limits of U , local magnetizations exhibit a fairly intricate spatial pattern that reflects the quasiperiodic structure, but the pattern differs between the two limits. We have analyzed this pattern change by a mode analysis by the singular value decomposition method for the fractal-like magnetization pattern projected into the perpendicular space.

  19. Performance of synthetic antiferromagnetic racetrack memory: domain wall versus skyrmion

    International Nuclear Information System (INIS)

    Tomasello, R; Puliafito, V; Martinez, E; Manchon, A; Ricci, M; Carpentieri, M; Finocchio, G

    2017-01-01

    A storage scheme based on racetrack memory, where the information can be coded in a domain or a skyrmion, seems to be an alternative to conventional hard disk drive for high density storage. Here, we perform a full micromagnetic study of the performance of synthetic antiferromagnetic (SAF) racetrack memory in terms of velocity and sensitivity to defects by using experimental parameters. We find that, to stabilize a SAF skyrmion, the Dzyaloshinskii–Moriya interaction in the top and the bottom ferromagnet should have an opposite sign. The velocity of SAF skyrmions and SAF Néel domain walls are of the same order and can reach values larger than 1200 m s −1 if a spin–orbit torque from the spin-Hall effect with opposite sign is applied to both ferromagnets. The presence of disordered anisotropy in the form of randomly distributed grains introduces a threshold current for both SAF skyrmions and SAF domain walls motions. (paper)

  20. Performance of synthetic antiferromagnetic racetrack memory: domain wall versus skyrmion

    KAUST Repository

    Tomasello, R

    2017-06-20

    A storage scheme based on racetrack memory, where the information can be coded in a domain or a skyrmion, seems to be an alternative to conventional hard disk drive for high density storage. Here, we perform a full micromagnetic study of the performance of synthetic antiferromagnetic (SAF) racetrack memory in terms of velocity and sensitivity to defects by using experimental parameters. We find that, to stabilize a SAF skyrmion, the Dzyaloshinskii–Moriya interaction in the top and the bottom ferromagnet should have an opposite sign. The velocity of SAF skyrmions and SAF Néel domain walls are of the same order and can reach values larger than 1200 m s−1 if a spin–orbit torque from the spin-Hall effect with opposite sign is applied to both ferromagnets. The presence of disordered anisotropy in the form of randomly distributed grains introduces a threshold current for both SAF skyrmions and SAF domain walls motions.

  1. Equivalence of the O( n) vector ferromagnetic and antiferromagnetic models

    Science.gov (United States)

    Sousa, J. Ricardo de

    The effective-field renormalization group (EFRG) approach is used to find the Néel temperature ( TN) of the O( n) vector model with antiferromagnetic (AF) interaction. The EFRG method is illustrated by employing approximations in which clusters with one ( N‧=1) and two ( N=2) spins are used. The critical temperature TN is obtained as a function of component ( n) and coordination ( z) numbers. For all values of n and z we show that TN= Tc, where Tc is the Curie temperature for the ferromagnetic (F) case. As a comparison, the results of the quantum Heisenberg model ( n=3) with F and AF interactions are also presented, and we find that TN> Tc, which is different from the classical result Tc= TN.

  2. Magnetic field effects of tow-leg Heisenberg antiferromagnetic ladders: Thermodynamic properties

    International Nuclear Information System (INIS)

    Wang Xiaoqun; Yu Lu

    2000-05-01

    Using the recently developed transfer-matrix renormalization group method, we have studied the thermodynamic properties of two-leg antiferromagnetic ladders in the magnetic field. Based on different behavior of magnetization, we found disordered spin liquid, Luttinger liquid, spin-polarized phases and a classical regime depending on magnetic field and temperature. Our calculations in Luttinger liquid regime suggest that both the divergence of the NMR relaxation rate and the anomalous specific heat behavior observed on Cu 2 (C 5 H 12 N 2 ) 2 Cl 4 are due to quasi-one-dimensional effect rather than three-dimensional ordering. (author)

  3. Numerical study of ground state and low lying excitations of quantum antiferromagnets

    International Nuclear Information System (INIS)

    Trivedi, N.; Ceperley, D.M.

    1989-01-01

    The authors have studied, via Green function Monte Carlo (GFMC), the S = 1/2 Heisenberg quantum antiferromagnet in two dimensions on a square lattice. They obtain the ground state energy with only statistical errors E 0 /J = -0.6692(2), the staggered magnetization m † = 0.31(2), and from the long wave length behavior of the structure factor, the spin wave velocity c/c o = 1.14(5). They show that the ground state wave function has long range pair correlations arising from the zero point motion of spin waves

  4. Monte Carlo study of four-spinon dynamic structure function in antiferromagnetic Heisenberg model

    International Nuclear Information System (INIS)

    Si-Lakhal, B.; Abada, A.

    2003-11-01

    Using Monte Carlo integration methods, we describe the behavior of the exact four-s pinon dynamic structure function S 4 in the antiferromagnetic spin 1/2 Heisenberg quantum spin chain as a function of the neutron energy ω and momentum transfer k. We also determine the fourspinon continuum, the extent of the region in the (k, ω) plane outside which S 4 is identically zero. In each case, the behavior of S 4 is shown to be consistent with the four-spinon continuum and compared to the one of the exact two-spinon dynamic structure function S 2 . Overall shape similarity is noted. (author)

  5. Antiferromagnetism in EuPdGe{sub 3}

    Energy Technology Data Exchange (ETDEWEB)

    Albedah, Mohammed A. [Department of Physics, University of Ottawa, Ottawa, Ontario K1N 6N5 (Canada); Al-Qadi, Khalid [Department of Physics, University of Ottawa, Ottawa, Ontario K1N 6N5 (Canada); Department of Mathematics, Statistics and Physics, Qatar University, P.O. Box 2713, Doha (Qatar); Stadnik, Zbigniew M., E-mail: stadnik@uottawa.ca [Department of Physics, University of Ottawa, Ottawa, Ontario K1N 6N5 (Canada); Przewoźnik, Janusz [Solid State Physics Department, Faculty of Physics and Applied Computer Science, AGH University of Science and Technology, 30-059 Kraków (Poland)

    2014-11-15

    Highlights: • We show that EuPdGe{sub 3} crystallizes in the BaNiSn{sub 3}-type structure with the lattice constants a = 4.4457(1) Å and c = 10.1703(2). • We demonstrate that EuPdGe{sub 3} is an antiferromagnet with the Néel temperature T{sub N} = 12.16(1) K. • The temperature dependence of the hyperfine magnetic field follows a S = 7/2 Brillouin function. • We find that the Debye temperature of the studied compound is 199(2) K. - Abstract: The results of X-ray diffraction, magnetic susceptibility and magnetization, and {sup 151}Eu Mössbauer spectroscopy measurements of polycrystalline EuPdGe{sub 3} are reported. EuPdGe{sub 3} crystallizes in the BaNiSn{sub 3}-type tetragonal structure (space group I4mm) with the lattice constants a=4.4457(1)Å and c=10.1703(2)Å. The results are consistent with EuPdGe{sub 3} being an antiferromagnet with the Néel temperature T{sub N}=12.16(1)K and with the Eu spins S=7/2 in the ab plane. The temperature dependence of the magnetic susceptibility above T{sub N} follows the modified Curie-Weiss law with the effective magnetic moment of 7.82(1) μ{sub B} per Eu atom and the paramagnetic Curie temperature of -5.3(1)K indicative of dominant antiferromagnetic interactions. The M(H) isotherms for temperatures approaching T{sub N} from above are indicative of dynamical short-range antiferromagnetic ordering in the sample. The temperature dependence of the hyperfine magnetic field follows a S=7/2 Brillouin function. The principal component of the electric field gradient tensor is shown to increase with decreasing temperature and is well described by a T{sup 3/2} power-law relation. The Debye temperature of EuPdGe{sub 3} determined from the Mössbauer data is 199(2) K.

  6. Giant magneto-spin-Seebeck effect and magnon transfer torques in insulating spin valves

    Science.gov (United States)

    Cheng, Yihong; Chen, Kai; Zhang, Shufeng

    2018-01-01

    We theoretically study magnon transport in an insulating spin valve (ISV) made of an antiferromagnetic insulator sandwiched between two ferromagnetic insulator (FI) layers. In the conventional metal-based spin valve, the electron spins propagate between two metallic ferromagnetic layers, giving rise to giant magnetoresistance and spin transfer torque. Here, the incoherent magnons in the ISV serve as angular momentum carriers and are responsible for the angular momentum transport between two FI layers across the antiferromagnetic spacer. We predict two transport phenomena in the presence of the temperature gradient: a giant magneto-spin-Seebeck effect in which the output voltage signal is controlled by the relative orientation of the two FI layers and magnon transfer torque that can be used for switching the magnetization of the FI layers with a temperature gradient of the order of 0.1 Kelvin per nanometer.

  7. Low-temperature spin dynamics of a valence bond glass in Ba2YMoO6

    International Nuclear Information System (INIS)

    De Vries, M A; Piatek, J O; Rønnow, H M; Misek, M; Lord, J S; Bos, J-W G

    2013-01-01

    We carried out ac magnetic susceptibility measurements and muon spin relaxation spectroscopy on the cubic double perovskite Ba 2 YMoO 6 , down to 50 mK. Below ∼1 K the muon relaxation is typical of a magnetic insulator with a spin-liquid type ground state, i.e. without broken symmetries or frozen moments. However, the ac susceptibility revealed a dilute-spin-glass-like transition below ∼1 K. Antiferromagnetically coupled Mo 5+ 4d 1 electrons in triply degenerate t 2g orbitals are in this material arranged in a geometrically frustrated fcc lattice. Bulk magnetic susceptibility data has previously been interpreted in terms of a freezing to a heterogeneous state with non-magnetic sites where 4d 1 electrons have paired in spin-singlets dimers, and residual unpaired Mo 5+ 4d 1 electron spins. Based on the magnetic heat capacity data it has been suggested that this heterogeneity is the result of kinetic constraints intrinsic to the physics of the pure system (possibly due to topological overprotection) leading to a self-induced glass of valence bonds between neighbouring 4d 1 electrons. The muon spin relaxation (μSR) unambiguously points to a heterogeneous state with a static arrangement of unpaired electrons in a background of (valence bond) dimers between the majority of Mo 5+ 4d electrons. The ac susceptibility data indicate that the residual magnetic moments freeze into a dilute-spin-glass-like state. This is in apparent contradiction with the muon-spin decoupling at 50 mK in fields up to 200 mT, which indicates that, remarkably, the time scale of the field fluctuations from the residual moments is ∼5 ns. Comparable behaviour has been observed in other geometrically frustrated magnets with spin-liquid-like behaviour and the implications of our observations on Ba 2 YMoO 6 are discussed in this context. (paper)

  8. Low-temperature spin dynamics of a valence bond glass in Ba2YMoO6

    Science.gov (United States)

    de Vries, M. A.; Piatek, J. O.; Misek, M.; Lord, J. S.; Rønnow, H. M.; Bos, J.-W. G.

    2013-04-01

    We carried out ac magnetic susceptibility measurements and muon spin relaxation spectroscopy on the cubic double perovskite Ba2YMoO6, down to 50 mK. Below ∼1 K the muon relaxation is typical of a magnetic insulator with a spin-liquid type ground state, i.e. without broken symmetries or frozen moments. However, the ac susceptibility revealed a dilute-spin-glass-like transition below ∼1 K. Antiferromagnetically coupled Mo5+ 4d1 electrons in triply degenerate t2g orbitals are in this material arranged in a geometrically frustrated fcc lattice. Bulk magnetic susceptibility data has previously been interpreted in terms of a freezing to a heterogeneous state with non-magnetic sites where 4d1 electrons have paired in spin-singlets dimers, and residual unpaired Mo5+ 4d1 electron spins. Based on the magnetic heat capacity data it has been suggested that this heterogeneity is the result of kinetic constraints intrinsic to the physics of the pure system (possibly due to topological overprotection) leading to a self-induced glass of valence bonds between neighbouring 4d1 electrons. The muon spin relaxation (μSR) unambiguously points to a heterogeneous state with a static arrangement of unpaired electrons in a background of (valence bond) dimers between the majority of Mo5+ 4d electrons. The ac susceptibility data indicate that the residual magnetic moments freeze into a dilute-spin-glass-like state. This is in apparent contradiction with the muon-spin decoupling at 50 mK in fields up to 200 mT, which indicates that, remarkably, the time scale of the field fluctuations from the residual moments is ∼5 ns. Comparable behaviour has been observed in other geometrically frustrated magnets with spin-liquid-like behaviour and the implications of our observations on Ba2YMoO6 are discussed in this context.

  9. Effect of antiferromagnetic layer thickness on exchange bias, training effect, and magnetotransport properties in ferromagnetic/antiferromagnetic antidot arrays

    Energy Technology Data Exchange (ETDEWEB)

    Gong, W. J.; Liu, W., E-mail: wliu@imr.ac.cn; Feng, J. N.; Zhang, Z. D. [Shenyang National Laboratory for Materials Science, Institute of Metal Research, Chinese Academy of Sciences, Shenyang 110016 (China); Kim, D. S.; Choi, C. J. [Functional Materials Division, Korea Institute of Materials Science, 531 Changwon- daero, Changwon 631-831 (Korea, Republic of)

    2014-04-07

    The effect of antiferromagnetic (AFM) layer on exchange bias (EB), training effect, and magnetotransport properties in ferromagnetic (FM) /AFM nanoscale antidot arrays and sheet films Ag(10 nm)/Co(8 nm)/NiO(t{sub NiO})/Ag(5 nm) at 10 K is studied. The AFM layer thickness dependence of the EB field shows a peak at t{sub NiO} = 2 nm that is explained by using the random field model. The misalignment of magnetic moments in the three-dimensional antidot arrays causes smaller decrease of EB field compared with that in the sheet films for training effect. The anomalous magnetotransport properties, in particular positive magnetoresistance (MR) for antidot arrays but negative MR for sheet films are found. The training effect and magnetotransport properties are strongly affected by the three-dimensional spin-alignment effects in the antidot arrays.

  10. Paramagnetic fluctuations in Pr0.65Ca0.35MnO3 around the charge-ordering temperature

    International Nuclear Information System (INIS)

    Daoud-Aladine, A; Roessli, B; Gvasaliya, S N; Perca, C; Pinsard-Gaudart, L; Rodriguez-Carvajal, J; Revcolevschi, A

    2006-01-01

    We have studied the ferromagnetic and antiferromagnetic fluctuations in the charge-ordered Pr 0.65 Ca 0.35 MnO 3 antiferromagnet by triple-axis neutron spectrometry. Whereas ferromagnetic fluctuations are observed above and below the charge-ordering transition (T CO ), the antiferromagnetic fluctuations develop only below T CO . The dynamical exponent z of both ferromagnetic and antiferromagnetic fluctuations are determined. The ferromagnetic fluctuations are not completely suppressed below T CO and their correlation lengths are short-ranged at all temperatures. The results are discussed with respect to the Zener polaron model recently introduced to describe the charge-ordered state of Pr 0.6 Ca 0.40 MnO 3

  11. Logarithmic corrections from ferromagnetic impurity ending bonds of open antiferromagnetic host chains

    International Nuclear Information System (INIS)

    Lou Jizhong; Qin Shaojin; Su Zhaobin; Dai Jianhui; Yu Lu

    2000-06-01

    We analyze the logarithmic corrections due to ferromagnetic impurity ending bonds of open spin 1/2 antiferromagnetic chains, using the density matrix renormalization group technique. A universal finite size scaling ∼ 1/L log L for impurity contributions in the quasi-degenerate ground state energy is demonstrated for a zigzag spin 1/2 chain at the critical next nearest neighbor coupling and the standard Heisenberg spin 1/2 chain, in the long chain limit. Using an exact solution for the latter case it is argued that one can extract the impurity contributions to the entropy and specific heat from the scaling analysis. It is also shown that a pure spin 3/2 open Heisenberg chain belongs to the same universality class. (author)

  12. The phase diagrams and the order parameters of the diluted superlattice with antiferromagnetic interface coupling

    International Nuclear Information System (INIS)

    Oubelkacem, A.; El Aouad, N.; Bentaleb, M.; Laaboudi, B.; Saber, M.

    2004-01-01

    Using the effective field theory with a probability distribution technique that accounts for the self-spin correlation functions, the magnetic properties of the diluted Ising superlattice consisting of two ferromagnetic materials A and B, with L a layers of diluted spins S a =((1)/(2)) and L b layers of diluted spins S b =1 with antiferromagnetic interface coupling are examined. For fixed values of the reduced exchange interactions and the concentration c of magnetic atoms, the phase diagrams, the two sublattice magnetizations and the total magnetization for the superlattice with the same spin S a =S b =((1)/(2)) and for S a =((1)/(2)), S b =1 are studied as a function of the temperature. We find a number of characteristic phenomena. In particular, the effect of the concentration c of magnetic atoms, the interlayer coupling and the layer thickness on both the compensation temperature and the magnetization profiles are clarified

  13. Unusual spin frozen state in a frustrated pyrochlore system NaCaCo{sub 2}F{sub 7} as observed by NMR

    Energy Technology Data Exchange (ETDEWEB)

    Sarkar, R.; Brueckner, F.; Klauss, H.H. [IFP, TU Dresden (Germany); Krizan, J.W.; Cava, R.J. [Department of Chemistry, Princeton University, Princeton, NJ (United States)

    2016-07-01

    We present {sup 23}Na -and {sup 19}F NMR results on the magnetically frustrated pyrochlore NaCaCo{sub 2}F{sub 7} with a frustration index of f = θ{sub CW}/T{sub f} ∝ 56. Recent neutron scattering experiments proposed XY like antiferromagnetic spin clusters at low energies in NaCaCo{sub 2}F{sub 7}. {sup 23}Na NMR -spectra reveal the presence of two magnetically non equivalent Na sites in conjunction with the local Co{sup 2+} spin structure. Below 3.6 K both the {sup 23}Na -and {sup 19}F spectra broaden due to the formation of static spin correlations. A huge reduction of the {sup 19}F -and {sup 23}Na NMR signal intensity hints at a quasi-static field distribution in NaCaCo{sub 2}F{sub 7} in this regime. The {sup 19}F spin-lattice relaxation rate {sup 19}(1/T{sub 1}) exhibits a peak at around 2.9 K, at the same temperature range where ac and dc susceptibility data show a broad maximum. The character of the spin fluctuation appears to be isotropic. The overall temperature dependence of {sup 19}(1/T{sub 1}) can be described by the BPP theory considering a fluctuating hyperfine field with an autocorrelation function. The correlation time of the autocorrelation function exhibits an activation behavior further indicating the spin-frozen state. While the present NMR studies suggest the spin frozen state at low temperatures, μSR investigations however reveal the presence of so called persistent spin dynamics down to 20 mK implying an exotic ground state in NaCaCo{sub 2}F{sub 7}.

  14. Pressure-induced antiferromagnetic superconductivity in CeNiGe3: A Ge73-NQR study under pressure

    International Nuclear Information System (INIS)

    Harada, A.; Kawasaki, S.; Mukuda, H.; Kitaoka, Y.; Thamizhavel, A.; Okuda, Y.; Settai, R.; Onuki, Y.; Itoh, K.M.; Haller, E.E.; Harima, H.

    2007-01-01

    We report on antiferromagnetic (AF) properties of pressure-induced superconductivity in CeNiGe 3 via the Ge73 nuclear-quadrupole-resonance (NQR) measurements under pressure (P). The NQR-spectrum measurements have revealed that the incommensurate antiferromagnetic ordering is robust against increasing P with the increase of ordered moment and ordering temperature. Nevertheless the measurements of nuclear spin-lattice relaxation rate (1/T 1 ) have pointed to the onset of superconductivity as a consequence of Ce-4f electrons delocalized by applying P. The emergence of superconductivity under the development of AF order suggests that a novel type of superconducting mechanism works in this compound

  15. Faraday rotation echo spectroscopy and detection of quantum fluctuations.

    Science.gov (United States)

    Chen, Shao-Wen; Liu, Ren-Bao

    2014-04-15

    Central spin decoherence is useful for detecting many-body physics in environments and moreover, the spin echo control can remove the effects of static thermal fluctuations so that the quantum fluctuations are revealed. The central spin decoherence approach, however, is feasible only in some special configurations and often requires uniform coupling between the central spin and individual spins in the baths, which are very challenging in experiments. Here, by making analogue between central spin decoherence and depolarization of photons, we propose a scheme of Faraday rotation echo spectroscopy (FRES) for studying quantum fluctuations in interacting spin systems. The echo control of the photon polarization is realized by flipping the polarization with a birefringence crystal. The FRES, similar to spin echo in magnetic resonance spectroscopy, can suppress the effects of the static magnetic fluctuations and therefore reveal dynamical magnetic fluctuations. We apply the scheme to a rare-earth compound LiHoF4 and calculate the echo signal, which is related to the quantum fluctuations of the system. We observe enhanced signals at the phase boundary. The FRES should be useful for studying quantum fluctuations in a broad range of spin systems, including cold atoms, quantum dots, solid-state impurities, and transparent magnetic materials.

  16. Suppression of tunneling by interference in half-integer--spin particles

    OpenAIRE

    Loss, Daniel; DiVincenzo, David P.; Grinstein, G.

    1992-01-01

    Within a wide class of ferromagnetic and antiferromagnetic systems, quantum tunneling of magnetization direction is spin-parity dependent: it vanishes for magnetic particles with half-integer spin, but is allowed for integer spin. A coherent-state path integral calculation shows that this topological effect results from interference between tunneling paths.

  17. Charge ordering and opening of spin gap in NaV2O5

    NARCIS (Netherlands)

    Mostovoy, M.V.; Khomskii, D.I.

    1999-01-01

    We argue that the origin of the phase transition in quasi-one-dimensional antiferromagnet NaV2O5 is not the spin-Peierls (SP) instability, but a charge ordering. The opening of the spin gap and the lattice dimerization, characteristic for the spin-Peierls systems, in NaV2O5 result from the interplay

  18. Quantum fluctuations

    International Nuclear Information System (INIS)

    Reynaud, S.; Giacobino, S.; Zinn-Justin, J.

    1997-01-01

    This course is dedicated to present in a pedagogical manner the recent developments in peculiar fields concerned by quantum fluctuations: quantum noise in optics, light propagation through dielectric media, sub-Poissonian light generated by lasers and masers, quantum non-demolition measurements, quantum electrodynamics applied to cavities and electrical circuits involving superconducting tunnel junctions. (A.C.)

  19. Spin dynamics in CuO and Cu[sub 1[minus][ital x

    Energy Technology Data Exchange (ETDEWEB)

    Carretta, P.; Corti, M.; Rigamonti, A. (Department of Physics Alessandro Volta,' ' University of Pavia, Via Bassi 6, 27100 Pavia (Italy))

    1993-08-01

    [sup 63]Cu nuclear quadrupole resonance (NQR), nuclear antiferromagnetic resonance (AFNMR), and spin-lattice relaxation, as well as [sup 7]Li NMR and relaxation measurements in CuO and in Cu[sub 1[minus][ital x

  20. Anomalous Z2 antiferromagnetic topological phase in pressurized SmB6

    Science.gov (United States)

    Chang, Kai-Wei; Chen, Peng-Jen

    2018-05-01

    Antiferromagnetic materials, whose time-reversal symmetry is broken, can be classified into the Z2 topology if they respect some specific symmetry. Since the theoretical proposal, however, no materials have been found to host such Z2 antiferromagnetic topological (Z2-AFT ) phase to date. Here we demonstrate that the topological Kondo insulator SmB6 can be a Z2-AFT system when pressurized to undergo an antiferromagnetic phase transition. In addition to proposing the possible candidate for a Z2-AFT material, in this work we also illustrate the anomalous topological surface states of the Z2-AFT phase which have not been discussed before. Originating from the interplay between the topological properties and the antiferromagnetic surface magnetization, the topological surface states of the Z2-AFT phase behave differently as compared with those of a topological insulator. Besides, the Z2-AFT insulators are also found promising in the generation of tunable spin currents, which is an important application in spintronics.