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Sample records for antiferromagnetic spin fluctuations

  1. Hole pairing induced by antiferromagnetic spin fluctuations

    International Nuclear Information System (INIS)

    Su, Z.B.; Yu Lu; Dong, J.M.; Tosatti, E.

    1987-08-01

    The effective interaction induced by antiferromagnetic spin fluctuations is considered in the random phase approximation in the context of the recently discovered high T c oxide superconductors. This effective attraction favours a triplet pairing of holes. The implications of such pairing mechanism are discussed in connection with the current experimental observations. (author). 30 refs, 2 figs

  2. Ab initio calculations of incommensurate antiferromagnetic spin fluctuations in hcp iron under pressure

    Science.gov (United States)

    Thakor, V.; Staunton, J. B.; Poulter, J.; Ostanin, S.; Ginatempo, B.; Bruno, Ezio

    2003-05-01

    We present ab initio calculations of the static paramagnetic spin susceptibility for hcp iron at finite temperatures and for a range of pressures. The dominant magnetic fluctuations in hcp Fe are found to be incommensurate antiferromagnetic, characterized by the wave vector qinc=(0.56,0.22,0). We show that qinc is linked to a Fermi-surface nesting feature. For the lowest pressure ˜16 GPa at which hcp Fe forms, we find that these modes become unstable below a Néel temperature (TN) of 69 K. TN rapidly diminishes with increasing pressure. We therefore predict that hcp Fe will be found to have an incommensurate spin-density-wave-ordered state over a small pressure range starting with the onset of hcp phase. We note the coincidence with the superconductivity recently found in this material.

  3. Quantum fluctuations in the competition among spin glass, antiferromagnetism and local pairing superconductivity

    International Nuclear Information System (INIS)

    Magalhaes, S.G.; Zimmer, F.M.; Kipper, C.J.; Calegari, E.J.

    2007-01-01

    The competition among spin glass (SG), antiferromagnetism (AF) and local pairing superconductivity (PAIR) is studied in a two-sublattice fermionic Ising SG model with a local BCS pairing interaction in the presence of a transverse magnetic field Γ. The spins in different sublattices interact with Gaussian random couplings with an antiferromagnetic mean. The problem is formulated in a Grassmann path integral formalism. The static ansatz and the replica symmetry are used to obtain the half-filling thermodynamic potential. The results are shown in phase diagrams that exhibit a complex transition line separating the PAIR phase from the others. This line is second order at high temperature which ends in a tricritical point. The presence of Γ affects deeply the transition lines

  4. Antiferromagnetic spin-orbitronics

    KAUST Repository

    Manchon, Aurelien

    2015-05-01

    Antiferromagnets have long remained an intriguing and exotic state of matter, whose application has been restricted to enabling interfacial exchange bias in metallic and tunneling spin-valves [1]. Their role in the expanding field of applied spintronics has been mostly passive and the in-depth investigation of their basic properties mostly considered from a fundamental perspective.

  5. Antiferromagnetic spin Seebeck effect.

    Energy Technology Data Exchange (ETDEWEB)

    Wu, Stephen M.; Zhang, Wei; KC, Amit; Borisov, Pavel; Pearson, John E.; Jiang, J. Samuel; Lederman, David; Hoffmann, Axel; Bhattacharya, Anand

    2016-03-03

    We report on the observation of the spin Seebeck effect in antiferromagnetic MnF2. A device scale on-chip heater is deposited on a bilayer of MnF2 (110) (30nm)/Pt (4 nm) grown by molecular beam epitaxy on a MgF2(110) substrate. Using Pt as a spin detector layer, it is possible to measure the thermally generated spin current from MnF2 through the inverse spin Hall effect. The low temperature (2–80 K) and high magnetic field (up to 140 kOe) regime is explored. A clear spin-flop transition corresponding to the sudden rotation of antiferromagnetic spins out of the easy axis is observed in the spin Seebeck signal when large magnetic fields (>9T) are applied parallel to the easy axis of the MnF2 thin film. When the magnetic field is applied perpendicular to the easy axis, the spin-flop transition is absent, as expected.

  6. Spin Dynamics and Critical Fluctuations in a Two-Dimensional Random Antiferromagnet

    DEFF Research Database (Denmark)

    Als-Nielsen, Jens Aage; Birgeneau, R. J.; Guggenheim, H. J.

    1975-01-01

    A comprehensive elastic- and inelastic-neutron-scattering study of the binary mixed antiferromagnet Rb2Mn0.5Ni0.5F4 has been carried out. The pure materials, Rb2MnF4 and Rb2NiF4 are [2d] near-Heisenberg antiferromagnets of the K2NiF4 type. Elastic-scattering experiments demonstrate that the Mn...... like the sublattice magnetization while the excitations at larger wave vectors remain well defined through TN and only slightly renormalized from their T=0 energies. Critical scattering measurements of the staggered susceptibility and the correlation length have been carried out between 69 and 120 K...

  7. Spin fluctuations and the

    Directory of Open Access Journals (Sweden)

    V.M. Loktev

    2008-09-01

    Full Text Available We analyze the spectral properties of a phenomenological model for a weakly doped two-dimensional antiferromagnet, in which the carriers move within one of the two sublattices where they were introduced. Such a constraint results in the free carrier spectra with the maxima at k=(± π/2 , ± π/2 observed in some cuprates. We consider the spectral properties of the model by taking into account fluctuations of the spins in the antiferromagnetic background. We show that such fluctuations lead to a non-pole-like structure of the single-hole Green's function and these fluctuations can be responsible for some anomalous "strange metal" properties of underdoped cuprates in the nonsuperconducting regime.

  8. Neutron scattering studies of two-dimensional antiferromagnetic spin fluctuations in insulating and superconducting S = 1/2 systems

    Energy Technology Data Exchange (ETDEWEB)

    Bech Christensen, N

    2005-01-01

    Time-of-flight and polarized triple axis neutron scattering is used to probe the spin excitations of Cu(DCOO){sub 2}x4D{sub 2}O and La{sub 2-x}Sr{sub x}CuO{sub 4}. The first part of the thesis contains an investigation of the excitation spectrum of the square lattice S = 1/2 Heisenberg antiferromagnet Cu(DCOO){sub 2}4D{sub 2}O. Along the antiferromagnetic zone boundary a pronounced intensity variation is found for the dominant single-magnon excitations. This variation tracks an already known zone boundary dispersion. Using polarization analysis to separate the components of the excitation spectrum, a continuum of longitudinally polarized multimagnon excitations is discovered at energies above the single-magnon branch. At low energies, the findings are well described by linear spin wave theory. At high energies, linear spin wave theory fails and instead the data are very well accounted for by state-of-the-art Quantum Monte Carlo computations. In the second part of the thesis, the spin excitation spectra of the high temperature superconductors La{sub 1.90}Sr{sub 0.10}CuO{sub 4} and La{sub 1.84}Sr{sub 0.16}Cu characterized. The main discovery is that the excitations are dispersive at both doping levels. The dispersion strongly resembles that seen in other high-T{sub c} superconductors. The presence of dispersive excitations does not require superconductivity to exist. For La{sub 1.84}Sr{sub 0.16}CuO{sub 4}, but not for La{sub 1.90}Sr{sub 0.10}CuO{sub 4}, the onset superconductivity gives rise to a spectral weight shift which displays qualitative and quantitative similarities to the resonance mode observed in other high-T{sub c} superconductors. (au)

  9. Neutron scattering studies of two-dimensional antiferromagnetic spin fluctuations in insulating and superconducting S = ½ systems

    DEFF Research Database (Denmark)

    Christensen, Niels Bech

    Time-of-flight and polarized triple axis neutron scattering is used to probe the spin excitations of Cu(DCOO)_2_·_4D_2O and La_2_-_xSr_xCuO_4. The first part of the thesis contains an investigation of the excitation spectrum of the square lattice S = 1/2Heisenberg antiferromagnet Cu(DCOO)_2_·_4D_2O....... Along the antiferromagnetic zone boundary a pronounced intensity variation is found for the dominant single-magnon excitations. This variation tracks an already known zone boundary dispersion. Usingpolarization analysis to separate the components of the excitation spectrum, a continuum of longitudinally...... computations. In the second part of the thesis, the spin excitation spectra of the hightemperature superconductors La_1_._9_0Sr_0_._1_0CuO_4 and La_1_._8_4Sr_0_._1_6CuO_4 are characterized. The main discovery is that the excitations are dispersive at both doping levels. The dispersion strongly resembles...

  10. Spin structures in antiferromagnetic nanoparticles

    DEFF Research Database (Denmark)

    Brok, Erik

    a detailed knowledge of it can be important for applications of antiferromagnetic nanoparticles for example combined with ferromagnetic nanoparticles in nanocomposite devices. In this thesis the magnetic structure, in particular the orientation of the spins in the antiferromagnetic sublattices......, proposed to explain the unusual magnetic properties of the mineral. In summary the thesis have demonstrated methods for investigation of spin structures in magnetic nanoparticles. In particular, the classical model of the temperature dependence of canted spin structures sucessfully explains many...... experimental observations of anomalous temperature dependence in nanoparticle and bulk systems. Morover, XY Z neutron polarisation analysis have been demonstrated to be an effective way of investigating the magnetic properties of antiferromagnetic nanoparticles, significantly improving the unpolarised neutron...

  11. Spin Structure Analyses of Antiferromagnets

    International Nuclear Information System (INIS)

    Chung, Jae Ho; Song, Young Sang; Lee, Hak Bong

    2010-05-01

    We have synthesized series of powder sample of incommensurate antiferromagnetic multiferroics, (Mn, Co)WO 4 and Al doped Ba 0.5 Sr 1.5 Zn 2 Fe 12 O 22 , incommensurate antiferromagnetic multiferroics. Their spin structure was studied by using the HRPD. In addition, we have synthesized series of crystalline samples of incommensurate multiferroics, (Mn, Co)WO 4 and olivines. Their spin structure was investigated using neutron diffraction under high magnetic field. As a result, we were able to draw the phase diagram of (Mn, Co)WO 4 as a function of composition and temperature. We learned the how the spin structure changes with increased ionic substitution. Finally we have drawn the phase diagram of the multicritical olivine Mn2SiS4/Mn2GeS4 as a function of filed and temperature through the spin structure studies

  12. 89Y NMR observation of ferromagnetic and antiferromagnetic spin fluctuations in the collapsed tetragonal phase of YFe2(Ge,Si)2

    Science.gov (United States)

    Srpčič, J.; Jeglič, P.; Felner, I.; Lv, Bing; Chu, C. W.; Arčon, D.

    2017-11-01

    The surprising discovery of tripling the superconducting critical temperature of KFe2As2 at high pressures has led to an intriguing question of how the superconductivity in the collapsed tetragonal phase differs from that in the noncollapsed phases of Fe-based superconductors. Here we report a 89Y nuclear magnetic resonance study of YFe2GexSi2 -x compounds whose electronic structure is similar to that of iron-pnictide collapsed tetragonal phases already at ambient pressure. We find that Fe(Ge,Si) layers show ferromagnetic spin fluctuations, whereas the layers are coupled antiferromagnetically. Furthermore, localized moments attributed either to Fe interstitial or antisite defects may account for magnetic impurity pair-breaking effects, thus explaining the substantial variation of superconductivity among different YFe2Ge2 samples.

  13. Spin diffusion and torques in disordered antiferromagnets

    KAUST Repository

    Manchon, Aurelien

    2017-02-01

    We have developed a drift-diffusion equation of spin transport in collinear bipartite metallic antiferromagnets. Starting from a model tight-binding Hamiltonian, we obtain the quantum kinetic equation within Keldysh formalism and expand it to the lowest order in spatial gradient using Wigner expansion method. In the diffusive limit, these equations track the spatio-temporal evolution of the spin accumulations and spin currents on each sublattice of the antiferromagnet. We use these equations to address the nature of the spin transfer torque in (i) a spin-valve composed of a ferromagnet and an antiferromagnet, (ii) a metallic bilayer consisting of an antiferromagnet adjacent to a heavy metal possessing spin Hall effect, and in (iii) a single antiferromagnet possessing spin Hall effect. We show that the latter can experience a self-torque thanks to the non-vanishing spin Hall effect in the antiferromagnet.

  14. Antiferromagnetic spin fluctuations and unconventional nodeless superconductivity in an iron-based new superconductor (Ca4Al2O(6-y))(Fe2As2): 75As nuclear quadrupole resonance study.

    Science.gov (United States)

    Kinouchi, H; Mukuda, H; Yashima, M; Kitaoka, Y; Shirage, P M; Eisaki, H; Iyo, A

    2011-07-22

    We report 75As nuclear quadrupole resonance studies on (Ca4Al2O(6-y))(Fe2As2) with T(c) = 27  K. Measurement of nuclear-spin-relaxation rate 1/T1 has revealed a significant development of two-dimensional antiferromagnetic spin fluctuations down to T(c) in association with the smallest As-Fe-As bond angle. Below T(c), the temperature dependence of 1/T1 without any trace of the coherence peak is well accounted for by a nodeless s(±)-wave multiple-gaps model. From the fact that its T(c) is comparable to T(c) = 28  K in the optimally doped LaFeAsO(1-y) in which antiferromagnetic spin fluctuations are not dominant, we remark that antiferromagnetic spin fluctuations are not a unique factor for enhancing T(c) among Fe-based superconductors, but a condition for optimizing superconductivity should be addressed from the lattice structure point of view.

  15. Antiferromagnetic Spin Wave Field-Effect Transistor

    Science.gov (United States)

    Cheng, Ran; Daniels, Matthew W.; Zhu, Jian-Gang; Xiao, Di

    2016-01-01

    In a collinear antiferromagnet with easy-axis anisotropy, symmetry dictates that the spin wave modes must be doubly degenerate. Theses two modes, distinguished by their opposite polarization and available only in antiferromagnets, give rise to a novel degree of freedom to encode and process information. We show that the spin wave polarization can be manipulated by an electric field induced Dzyaloshinskii-Moriya interaction and magnetic anisotropy. We propose a prototype spin wave field-effect transistor which realizes a gate-tunable magnonic analog of the Faraday effect, and demonstrate its application in THz signal modulation. Our findings open up the exciting possibility of digital data processing utilizing antiferromagnetic spin waves and enable the direct projection of optical computing concepts onto the mesoscopic scale. PMID:27048928

  16. Heat-driven spin torques in antiferromagnets

    Science.gov (United States)

    Białek, Marcin; Bréchet, Sylvain; Ansermet, Jean-Philippe

    2018-04-01

    Heat-driven magnetization damping, which is a linear function of a temperature gradient, is predicted in antiferromagnets by considering the sublattice dynamics subjected to a heat-driven spin torque. This points to the possibility of achieving spin torque oscillator behavior. The model is based on the magnetic Seebeck effect acting on sublattices which are exchange coupled. The heat-driven spin torque is estimated and the feasibility of detecting this effect is discussed.

  17. Spin transport and spin torque in antiferromagnetic devices

    Science.gov (United States)

    Železný, J.; Wadley, P.; Olejník, K.; Hoffmann, A.; Ohno, H.

    2018-03-01

    Ferromagnets are key materials for sensing and memory applications. In contrast, antiferromagnets, which represent the more common form of magnetically ordered materials, have found less practical application beyond their use for establishing reference magnetic orientations via exchange bias. This might change in the future due to the recent progress in materials research and discoveries of antiferromagnetic spintronic phenomena suitable for device applications. Experimental demonstration of the electrical switching and detection of the Néel order open a route towards memory devices based on antiferromagnets. Apart from the radiation and magnetic-field hardness, memory cells fabricated from antiferromagnets can be inherently multilevel, which could be used for neuromorphic computing. Switching speeds attainable in antiferromagnets far exceed those of ferromagnetic and semiconductor memory technologies. Here, we review the recent progress in electronic spin-transport and spin-torque phenomena in antiferromagnets that are dominantly of the relativistic quantum-mechanical origin. We discuss their utility in pure antiferromagnetic or hybrid ferromagnetic/antiferromagnetic memory devices.

  18. Spin Transport in Ferromagnetic and Antiferromagnetic Textures

    KAUST Repository

    Akosa, Collins A.

    2016-12-07

    In this dissertation, we provide an accurate description of spin transport in magnetic textures and in particular, we investigate in detail, the nature of spin torque and magnetic damping in such systems. Indeed, as will be further discussed in this thesis, the current-driven velocity of magnetic textures is related to the ratio between the so-called non-adiabatic torque and magnetic damping. Uncovering the physics underlying these phenomena can lead to the optimal design of magnetic systems with improved efficiency. We identified three interesting classes of systems which have attracted enormous research interest (i) Magnetic textures in systems with broken inversion symmetry: We investigate the nature of magnetic damping in non-centrosymmetric ferromagnets. Based on phenomenological and microscopic derivations, we show that the magnetic damping becomes chiral, i.e. depends on the chirality of the magnetic texture. (ii) Ferromagnetic domain walls, skyrmions and vortices: We address the physics of spin transport in sharp disordered magnetic domain walls and vortex cores. We demonstrate that upon spin-independent scattering, the non-adiabatic torque can be significantly enhanced. Such an enhancement is large for vortex cores compared to transverse domain walls. We also show that the topological spin currents owing in these structures dramatically enhances the non-adiabaticity, an effect unique to non-trivial topological textures (iii) Antiferromagnetic skyrmions: We extend this study to antiferromagnetic skyrmions and show that such an enhanced topological torque also exist in these systems. Even more interestingly, while such a non-adiabatic torque inuences the undesirable transverse velocity of ferromagnetic skyrmions, in antiferromagnetic skyrmions, the topological non-adiabatic torque directly determines the longitudinal velocity. As a consequence, scaling down the antiferromagnetic skyrmion results in a much more efficient spin torque.

  19. High-field spin dynamics of antiferromagnetic quantum spin chains

    DEFF Research Database (Denmark)

    Enderle, M.; Regnault, L.P.; Broholm, C.

    2000-01-01

    present recent work on the high-field spin dynamics of the S = I antiferromagnetic Heisenberg chains NENP (Haldane ground state) and CsNiCl3 (quasi-1D HAF close to the quantum critical point), the uniform S = 1/2 chain CTS, and the spin-Peierls system CuGeO3. (C) 2000 Elsevier Science B,V. All rights......The characteristic internal order of macroscopic quantum ground states in one-dimensional spin systems is usually not directly accessible, but reflected in the spin dynamics and the field dependence of the magnetic excitations. In high magnetic fields quantum phase transitions are expected. We...

  20. Spin-Mechanical Inertia in Antiferromagnet

    Science.gov (United States)

    Cheng, Ran; Wu, Xiaochuan; Xiao, Di

    Interplay between spin dynamics and mechanical motions is responsible for numerous striking phenomena, which has shaped a rapidly expanding field known as spin-mechanics. The guiding principle of this field has been the conservation of angular momentum that involves both quantum spins and classical mechanical rotations. However, in an antiferromagnet, the macroscopic magnetization vanishes while the order parameter (Néel order) does not carry an angular momentum. It is therefore not clear whether the order parameter dynamics has any mechanical consequence as its ferromagnetic counterparts. Here we demonstrate that the Néel order dynamics affects the mechanical motion of a rigid body by modifying its inertia tensor in the presence of strong magnetocrystalline anisotropy. This effect depends on temperature when magnon excitations are considered. Such a spin-mechanical inertia can produce measurable consequences at nanometer scales. Our discovery establishes spin-mechanical inertia as an essential ingredient to properly describe spin-mechanical effects in AFs, which supplements the known governing physics from angular momentum conservation. This work was supported by the DOE, Basic Energy Sciences, Grant No. DE-SC0012509. D.X. also acknowledges support from a Research Corporation for Science Advancement Cottrell Scholar Award.

  1. Robust spin transfer torque in antiferromagnetic tunnel junctions

    KAUST Repository

    Saidaoui, Hamed Ben Mohamed

    2017-04-18

    We theoretically study the current-induced spin torque in antiferromagnetic tunnel junctions, composed of two semi-infinite antiferromagnetic layers separated by a tunnel barrier, in both clean and disordered regimes. We find that the torque enabling electrical manipulation of the Néel antiferromagnetic order parameter is out of plane, ∼n×p, while the torque competing with the antiferromagnetic exchange is in plane, ∼n×(p×n). Here, p and n are the Néel order parameter direction of the reference and free layers, respectively. Their bias dependence shows behavior similar to that in ferromagnetic tunnel junctions, the in-plane torque being mostly linear in bias, while the out-of-plane torque is quadratic. Most importantly, we find that the spin transfer torque in antiferromagnetic tunnel junctions is much more robust against disorder than that in antiferromagnetic metallic spin valves due to the tunneling nature of spin transport.

  2. Dynamics of antiferromagnetic skyrmion driven by the spin Hall effect

    Science.gov (United States)

    Jin, Chendong; Song, Chengkun; Wang, Jianbo; Liu, Qingfang

    2016-10-01

    Magnetic skyrmion moved by the spin-Hall effect is promising for the application of the generation racetrack memories. However, the Magnus force causes a deflected motion of skyrmion, which limits its application. Here, we create an antiferromagnetic skyrmion by injecting a spin-polarized pulse in the nanostripe and investigate the spin Hall effect-induced motion of antiferromagnetic skyrmion by micromagnetic simulations. In contrast to ferromagnetic skyrmion, we find that the antiferromagnetic skyrmion has three evident advantages: (i) the minimum driving current density of antiferromagnetic skyrmion is about two orders smaller than the ferromagnetic skyrmion; (ii) the velocity of the antiferromagnetic skyrmion is about 57 times larger than the ferromagnetic skyrmion driven by the same value of current density; (iii) antiferromagnetic skyrmion can be driven by the spin Hall effect without the influence of Magnus force. In addition, antiferromagnetic skyrmion can move around the pinning sites due to its property of topological protection. Our results present the understanding of antiferromagnetic skyrmion motion driven by the spin Hall effect and may also contribute to the development of antiferromagnetic skyrmion-based racetrack memories.

  3. Spin Currents and Spin Orbit Torques in Ferromagnets and Antiferromagnets

    Science.gov (United States)

    Hung, Yu-Ming

    This thesis focuses on the interactions of spin currents and materials with magnetic order, e.g., ferromagnetic and antiferromagnetic thin films. The spin current is generated in two ways. First by spin-polarized conduction-electrons associated with the spin Hall effect in heavy metals (HMs) and, second, by exciting spin-waves in ferrimagnetic insulators using a microwave frequency magnetic field. A conduction-electron spin current can be generated by spin-orbit coupling in a heavy non-magnetic metal and transfer its spin angular momentum to a ferromagnet, providing a means of reversing the magnetization of perpendicularly magnetized ultrathin films with currents that flow in the plane of the layers. The torques on the magnetization are known as spin-orbit torques (SOT). In the first part of my thesis project I investigated and contrasted the quasistatic (slowly swept current) and pulsed current-induced switching characteristics of micrometer scale Hall crosses consisting of very thin (thesis project studies and considers applications of SOT-driven domain wall (DW) motion in a perpendicularly magnetized ultrathin ferromagnet sandwiched between a heavy metal and an oxide. My experiment results demonstrate that the DW motion can be explained by a combination of the spin Hall effect, which generates a SOT, and Dzyaloshinskii-Moriya interaction, which stabilizes chiral Neel-type DW. Based on SOT-driven DW motion and magnetic coupling between electrically isolated ferromagnetic elements, I proposed a new type of spin logic devices. I then demonstrate the device operation by using micromagnetic modeling which involves studying the magnetic coupling induced by fringe fields from chiral DWs in perpendicularly magnetized nanowires. The last part of my thesis project reports spin transport and spin-Hall magnetoresistance (SMR) in yttrium iron garnet Y3Fe5O 12 (YIG)/NiO/Pt trilayers with varied NiO thickness. To characterize the spin transport through NiO we excite

  4. Spin wave analysis to the spatially-anisotropic Heisenberg antiferromagnet on triangular lattice

    OpenAIRE

    Trumper, Adolfo E.

    1998-01-01

    We study the phase diagram at T=0 of the antiferromagnetic Heisenberg model on the triangular lattice with spatially-anisotropic interactions. For values of the anisotropy very close to J_alpha/J_beta=0.50, conventional spin wave theory predicts that quantum fluctuations melt the classical structures, for S=1/2. For the regime J_beta

  5. Spin Hall magnetoresistance in antiferromagnet/normal metal bilayers

    KAUST Repository

    Manchon, Aurelien

    2017-01-01

    We investigate the emergence of spin Hall magnetoresistance in a magnetic bilayer composed of a normal metal adjacent to an antiferromagnet. Based on a recently derived drift diffusion equation, we show that the resistance of the bilayer depends on the relative angle between the direction transverse to the current flow and the Néel order parameter. While this effect presents striking similarities with the spin Hall magnetoresistance recently reported in ferromagnetic bilayers, its physical origin is attributed to the anisotropic spin relaxation of itinerant spins in the antiferromagnet.

  6. Quantum Spin Liquids in Frustrated Spin-1 Diamond Antiferromagnets

    Science.gov (United States)

    Buessen, Finn Lasse; Hering, Max; Reuther, Johannes; Trebst, Simon

    2018-01-01

    Motivated by the recent synthesis of the spin-1 A -site spinel NiRh2 O4 , we investigate the classical to quantum crossover of a frustrated J1-J2 Heisenberg model on the diamond lattice upon varying the spin length S . Applying a recently developed pseudospin functional renormalization group approach for arbitrary spin-S magnets, we find that systems with S ≥3 /2 reside in the classical regime, where the low-temperature physics is dominated by the formation of coplanar spirals and a thermal (order-by-disorder) transition. For smaller local moments S =1 or S =1 /2 , we find that the system evades a thermal ordering transition and forms a quantum spiral spin liquid where the fluctuations are restricted to characteristic momentum-space surfaces. For the tetragonal phase of NiRh2 O4 , a modified J1-J2--J2⊥ exchange model is found to favor a conventionally ordered Néel state (for arbitrary spin S ), even in the presence of a strong local single-ion spin anisotropy, and it requires additional sources of frustration to explain the experimentally observed absence of a thermal ordering transition.

  7. Spin transfer torque in antiferromagnetic spin valves: From clean to disordered regimes

    KAUST Repository

    Saidaoui, Hamed Ben Mohamed

    2014-05-28

    Current-driven spin torques in metallic spin valves composed of antiferromagnets are theoretically studied using the nonequilibrium Green\\'s function method implemented on a tight-binding model. We focus our attention on G-type and L-type antiferromagnets in both clean and disordered regimes. In such structures, spin torques can either rotate the magnetic order parameter coherently (coherent torque) or compete with the internal antiferromagnetic exchange (exchange torque). We show that, depending on the symmetry of the spin valve, the coherent and exchange torques can either be in the plane, ∝n×(q×n) or out of the plane ∝n×q, where q and n are the directions of the order parameter of the polarizer and the free antiferromagnetic layers, respectively. Although disorder conserves the symmetry of the torques, it strongly reduces the torque magnitude, pointing out the need for momentum conservation to ensure strong spin torque in antiferromagnetic spin valves.

  8. Magnetic correlations and quantum criticality in the insulating antiferromagnetic, insulating spin liquid, renormalized Fermi liquid, and metallic antiferromagnetic phases of the Mott system V2O3

    Science.gov (United States)

    Bao, Wei; Broholm, C.; Aeppli, G.; Carter, S. A.; Dai, P.; Rosenbaum, T. F.; Honig, J. M.; Metcalf, P.; Trevino, S. F.

    1998-11-01

    Magnetic correlations in all four phases of pure and doped vanadium sesquioxide (V2O3) have been examined by magnetic thermal-neutron scattering. Specifically, we have studied the antiferromagnetic and paramagnetic phases of metallic V2-yO3, the antiferromagnetic insulating and paramagnetic metallic phases of stoichiometric V2O3, and the antiferromagnetic and paramagnetic phases of insulating V1.944Cr0.056O3. While the antiferromagnetic insulator can be accounted for by a localized Heisenberg spin model, the long-range order in the antiferromagnetic metal is an incommensurate spin-density wave, resulting from a Fermi surface nesting instability. Spin dynamics in the strongly correlated metal are dominated by spin fluctuations with a ``single lobe'' spectrum in the Stoner electron-hole continuum. Furthermore, our results in metallic V2O3 represent an unprecedentedly complete characterization of the spin fluctuations near a metallic quantum critical point, and provide quantitative support for the self-consistent renormalization theory for itinerant antiferromagnets in the small moment limit. Dynamic magnetic correlations for ħωantiferromagnetic insulator, from the paramagnetic metal and the paramagnetic insulator, introduces a sudden switching of magnetic correlations to a different spatial periodicity which indicates a sudden change in the underlying spin Hamiltonian. To describe this phase transition and also the unusual short-range order in the paramagnetic state, it seems necessary to take into account the orbital degrees of freedom associated with the degenerate d orbitals at the Fermi level in V2O3.

  9. Spin waves in antiferromagnetic FeF2

    DEFF Research Database (Denmark)

    Hutchings, M T; Rainford, B.D.; Guggenheim, H J

    1970-01-01

    Spin-wave dispersion in antiferromagnetic FeF2 has been investigated by inelastic neutron scattering using a chopper time-of-flight spectrometer. The single mode observed has a relatively flat dispersion curve rising from 53 cm-1 at the zone centre to 79 cm-1 at the zone boundary. A spin...

  10. Spin transfer and spin pumping in disordered normal metal-antiferromagnetic insulator systems

    Science.gov (United States)

    Gulbrandsen, Sverre A.; Brataas, Arne

    2018-02-01

    We consider an antiferromagnetic insulator that is in contact with a metal. Spin accumulation in the metal can induce spin-transfer torques on the staggered field and on the magnetization in the antiferromagnet. These torques relate to spin pumping: the emission of spin currents into the metal by a precessing antiferromagnet. We investigate how the various components of the spin-transfer torque are affected by spin-independent disorder and spin-flip scattering in the metal. Spin-conserving disorder reduces the coupling between the spins in the antiferromagnet and the itinerant spins in the metal in a manner similar to Ohm's law. Spin-flip scattering leads to spin-memory loss with a reduced spin-transfer torque. We discuss the concept of a staggered spin current and argue that it is not a conserved quantity. Away from the interface, the staggered spin current varies around a 0 mean in an irregular manner. A network model explains the rapid decay of the staggered spin current.

  11. Role of the antiferromagnetic bulk spins in exchange bias

    Energy Technology Data Exchange (ETDEWEB)

    Schuller, Ivan K. [Center for Advanced Nanoscience and Physics Department, University of California San Diego, La Jolla, CA 92093 (United States); Morales, Rafael, E-mail: rafael.morales@ehu.es [Department of Chemical-Physics & BCMaterials, University of the Basque Country UPV/EHU (Spain); IKERBASQUE, Basque Foundation for Science, 48011 Bilbao (Spain); Batlle, Xavier [Departament Física Fonamental and Institut de Nanociència i Nanotecnologia, Universitat de Barcelona, c/ Martí i Franqués s/n, 08028 Barcelona, Catalonia (Spain); Nowak, Ulrich [Department of Physics, University of Konstanz, 78464 Konstanz (Germany); Güntherodt, Gernot [Physics Institute (IIA), RWTH Aachen University, Campus RWTH-Melaten, 52074 Aachen (Germany)

    2016-10-15

    This “Critical Focused Issue” presents a brief review of experiments and models which describe the origin of exchange bias in epitaxial or textured ferromagnetic/antiferromagnetic bilayers. Evidence is presented which clearly indicates that inner, uncompensated, pinned moments in the bulk of the antiferromagnet (AFM) play a very important role in setting the magnitude of the exchange bias. A critical evaluation of the extensive literature in the field indicates that it is useful to think of this bulk, pinned uncompensated moments as a new type of a ferromagnet which has a low total moment, an ordering temperature given by the AFM Néel temperature, with parallel aligned moments randomly distributed on the regular AFM lattice. - Highlights: • We address the role of bulk antiferromagnetic spins in the exchange bias phenomenon. • Significant experiments on how bulk AFM spins determine exchange bias are highlighted. • We explain the model that accounts for experimental results.

  12. Spin Hall effects in metallic antiferromagnets – perspectives for future spin-orbitronics

    Directory of Open Access Journals (Sweden)

    Joseph Sklenar

    2016-05-01

    Full Text Available We investigate angular dependent spin-orbit torques from the spin Hall effect in a metallic antiferromagnet using the spin-torque ferromagnetic resonance technique. The large spin Hall effect exists in PtMn, a prototypical CuAu-I-type metallic antiferromagnet. By applying epitaxial growth, we previously reported an appreciable difference in spin-orbit torques for c- and a-axis orientated samples, implying anisotropic effects in magnetically ordered materials. In this work we demonstrate through bipolar-magnetic-field experiments a small but noticeable asymmetric behavior in the spin-transfer-torque that appears as a hysteresis effect. We also suggest that metallic antiferromagnets may be good candidates for the investigation of various unidirectional effects related to novel spin-orbitronics phenomena.

  13. Neutron spin-echo study of the critical dynamics of spin-5/2 antiferromagnets in two and three dimensions

    Science.gov (United States)

    Tseng, K. F.; Keller, T.; Walters, A. C.; Birgeneau, R. J.; Keimer, B.

    2016-07-01

    We report a neutron spin-echo study of the critical dynamics in the S =5/2 antiferromagnets MnF2 and Rb2MnF4 with three-dimensional (3D) and two-dimensional (2D) spin systems, respectively, in zero external field. Both compounds are Heisenberg antiferromagnets with a small uniaxial anisotropy resulting from dipolar spin-spin interactions, which leads to a crossover in the critical dynamics close to the Néel temperature, TN. By taking advantage of the μ eV energy resolution of the spin-echo spectrometer, we have determined the dynamical critical exponents z for both longitudinal and transverse fluctuations. In MnF2, both the characteristic temperature for crossover from 3D Heisenberg to 3D Ising behavior and the exponents z in both regimes are consistent with predictions from the dynamical scaling theory. The amplitude ratio of longitudinal and transverse fluctuations also agrees with predictions. In Rb2MnF4 , the critical dynamics crosses over from the expected 2D Heisenberg behavior for T ≫TN to a scaling regime with exponent z =1.387 (4 ) , which has not been predicted by theory and may indicate the influence of long-range dipolar interactions.

  14. Pure spin current manipulation in antiferromagnetically exchange coupled heterostructures

    Science.gov (United States)

    Avilés-Félix, L.; Butera, A.; González-Chávez, D. E.; Sommer, R. L.; Gómez, J. E.

    2018-03-01

    We present a model to describe the spin currents generated by ferromagnet/spacer/ferromagnet exchange coupled trilayer systems and heavy metal layers with strong spin-orbit coupling. By exploiting the magnitude of the exchange coupling (oscillatory RKKY-like coupling) and the spin-flop transition in the magnetization process, it has been possible to produce spin currents polarized in arbitrary directions. The spin-flop transition of the trilayer system originates pure spin currents whose polarization vector depends on the exchange field and the magnetization equilibrium angles. We also discuss a protocol to control the polarization sign of the pure spin current injected into the metallic layer by changing the initial conditions of magnetization of the ferromagnetic layers previously to the spin pumping and inverse spin Hall effect experiments. The small differences in the ferromagnetic layers lead to a change in the magnetization vector rotation that permits the control of the sign of the induced voltage components due to the inverse spin Hall effect. Our results can lead to important advances in hybrid spintronic devices with new functionalities, particularly, the ability to control microscopic parameters such as the polarization direction and the sign of the pure spin current through the variation of macroscopic parameters, such as the external magnetic field or the thickness of the spacer in antiferromagnetic exchange coupled systems.

  15. Critical temperature and the transition from quantum to classical order parameter fluctuations in the three-dimensional Heisenberg antiferromagnet

    OpenAIRE

    Sandvik, A. W.

    1998-01-01

    We present results of extensive quantum Monte Carlo simulations of the three-dimensional (3D) S=1/2 Heisenberg antiferromagnet. Finite-size scaling of the spin stiffness and the sublattice magnetization gives the critical temperature Tc/J = 0.946 +/- 0.001. The critical behavior is consistent with the classical 3D Heisenberg universality class, as expected. We discuss the general nature of the transition from quantum mechanical to classical (thermal) order parameter fluctuations at a continuo...

  16. Spin-current noise from fluctuation relations

    Energy Technology Data Exchange (ETDEWEB)

    Lim, Jong Soo [Institut de Fisica Interdisciplinària i Sistemes Complexos IFISC (UIB-CSIC), E-07122 Palma de Mallorca (Spain); Sánchez, David; López, Rosa [Institut de Fisica Interdisciplinària i Sistemes Complexos IFISC (UIB-CSIC), E-07122 Palma de Mallorca, Spain and Departement de Fisica, Universitat de les Illes Balears, E-07122 Palma de Mallorca (Spain)

    2013-12-04

    We present fluctuation relations that connect spin-polarized current and noise in mesoscopic conductors. In linear response, these relations are equivalent to the fluctuation-dissipation theorem that relates equilibrium current-current correlations to the linear conductance. More interestingly, in the weakly nonlinear regime of transport, these relations establish a connection between the leading-order rectification spin conductance, the spin noise susceptibility and the third cumulant of spin current fluctuations at equilibrium. Our results are valid even for systems in the presence of magnetic fields and coupled to ferromagnetic electrodes.

  17. Healing of defects in random antiferromagnetic spin chains

    Science.gov (United States)

    Vasseur, R.; Roshani, A.; Haas, S.; Saleur, H.

    2017-09-01

    We study the effects of a weakened link in random antiferromagnetic spin chains. We show that healing occurs, and that homogeneity is restored at low energy, in a way that is qualitatively similar to the fate of impurities in clean ferromagnetic spin chains, or in Luttinger liquids with attractive interactions. Healing in the random case occurs even without interactions, and is characteristic of the random singlet phase. Using real-space renormalization group and exact diagonalization methods, we characterize this universal healing crossover by studying the entanglement across the weak link. We identify a crossover healing length L\\star that separates a regime where the system is cut in half by the weak link from a fixed point where the spin chain is healed. Our results open the way to the study of impurity physics in disordered spin chains.

  18. Terahertz-Driven Nonlinear Spin Response of Antiferromagnetic Nickel Oxide

    Science.gov (United States)

    Baierl, S.; Mentink, J. H.; Hohenleutner, M.; Braun, L.; Do, T.-M.; Lange, C.; Sell, A.; Fiebig, M.; Woltersdorf, G.; Kampfrath, T.; Huber, R.

    2016-11-01

    Terahertz magnetic fields with amplitudes of up to 0.4 Tesla drive magnon resonances in nickel oxide while the induced dynamics is recorded by femtosecond magneto-optical probing. We observe distinct spin-mediated optical nonlinearities, including oscillations at the second harmonic of the 1 THz magnon mode. The latter originate from coherent dynamics of the longitudinal component of the antiferromagnetic order parameter, which are probed by magneto-optical effects of second order in the spin deflection. These observations allow us to dynamically disentangle electronic from lattice-related contributions to magnetic linear birefringence and dichroism—information so far only accessible by ultrafast THz spin control. The nonlinearities discussed here foreshadow physics that will become essential in future subcycle spin switching.

  19. Antiferromagnetic phase transition and spin correlations in NiO

    DEFF Research Database (Denmark)

    Chatterji, Tapan; McIntyre, G.J.; Lindgård, Per-Anker

    2009-01-01

    We have investigated the antiferromagnetic (AF) phase transition and spin correlations in NiO by high-temperature neutron diffraction below and above TN. We show that AF phase transition is a continuous second-order transition within our experimental resolution. The spin correlations manifested...... by the strong diffuse magnetic scattering persist well above TN530 K and could still be observed at T=800 K which is about 1.5TN. We argue that the strong spin correlations above TN are due to the topological frustration of the spins on a fcc lattice. The Néel temperature is substantially reduced...... by this process. We determined the critical exponents =0.328±0.002 and =0.64±0.03 and the Néel temperature TN=530±1 K. These critical exponents suggest that NiO should be regarded as a 3dXY system...

  20. Distortion of frustrated spin cluster caused by quantum fluctuation due to magneto-elastic coupling

    International Nuclear Information System (INIS)

    Terao, Kiyosi; Honda, Ikumi

    2007-01-01

    We study the effects of magneto-elastic coupling on frustrated spin states of the antiferromagnetic Heisenberg model on a regular triangle and tetrahedron made of spin 1/2 or 1. Displacement of spin is considered as a quantum-mechanical variable. Distortion of clusters occurs through quantum fluctuation of normal modes caused by magneto-elastic coupling. The nonmagnetic phase transitions of vanadium and chromium spinels are discussed

  1. Spin freezing in the geometrically frustrated pyrochlore antiferromagnet Tb2Mo2O7

    DEFF Research Database (Denmark)

    Gaulin, B.D.; Reimers, J.N.; Mason, T.E.

    1992-01-01

    The magnetic metal ions in the cubic pyrochlore Tb2Mo2O7 form an infinite three-dimensional network of corner-sharing tetrahedra with a very high potential for frustration in the presence of antiferromagnetism. We have performed neutron scattering measurements which show short-range spatial...... correlations that develop continuously with decreasing temperature, while the characteristic time scale for the fluctuating moments decreases dramatically below T(f) is similar to 25 K. Therefore, this pure material, which possesses frustration that is purely geometrical in origin, displays a spin-glass state...

  2. Scattering bottleneck for spin dynamics in metallic helical antiferromagnetic dysprosium

    Science.gov (United States)

    Langner, M. C.; Roy, S.; Kemper, A. F.; Chuang, Y.-D.; Mishra, S. K.; Versteeg, R. B.; Zhu, Y.; Hertlein, M. P.; Glover, T. E.; Dumesnil, K.; Schoenlein, R. W.

    2015-11-01

    Ultrafast studies of magnetization dynamics have revealed fundamental processes that govern spin dynamics, and the emergence of time-resolved x-ray techniques has extended these studies to long-range spin structures that result from interactions with competing symmetries. By combining time-resolved resonant x-ray scattering and ultrafast magneto-optical Kerr studies, we show that the dynamics of the core spins in the helical magnetic structure occur on much longer time scales than the excitation of conduction electrons in the lanthanide metal Dy. The observed spin behavior differs markedly from that observed in the ferromagnetic phase of other lanthanide metals or transition metals and is strongly dependent on temperature and excitation fluence. This unique behavior results from coupling of the real-space helical spin structure to the shape of the conduction electron Fermi surface in momentum space, which creates a bottleneck in spin scattering events that transfer the valence excitation to the core spins. The dependence of the dynamics on the intersite interactions renders the helical ordering much more robust to perturbations than simple ferromagnetic or antiferromagnetic ordering, where dynamics are driven primarily by on-site interactions.

  3. Spin stiffness of frustrated Heisenberg antiferromagnets: Finite size scaling

    International Nuclear Information System (INIS)

    Feiguin, A.E.; Gazza, C.J.; Trumper, A.E.

    1995-07-01

    We calculate the spin stiffness of the S = 1/2 frustrated Heisenberg antiferromagnet on finite square lattices by means of the Schwinger - boson approach. COmparison with recent exact numerical results reveals that the observed lack of scaling with lattice size for intermediate to large frustration cannot be taken as an indication of absence of Neel order. This lack of scaling is already apparent for small frustration and is a finite lattice effect. Our results also indicate that the expected behaviour is regained for larger lattices than those considered in numerical studies. (author). 18 refs, 2 figs

  4. Properties of Haldane Excitations and Multiparticle States in the Antiferromagnetic Spin-1 Chain Compound CsNiCl3

    International Nuclear Information System (INIS)

    Kenzelmann, M.; Cowley, R.A.; Buyers, W.J.L.; Tun, Z.; Coldea, Radu; Enderle, M.

    2002-01-01

    We report inelastic time-of-flight and triple-axis neutron scattering measurements of the excitation spectrum of the coupled antiferromagnetic spin-1 Heisenberg chain system CsNiCl 3 . Measurements over a wide range of wave-vector transfers along the chain confirm that above T N CsNiCl 3 is in a quantum-disordered phase with an energy gap in the excitation spectrum. The spin correlations fall off exponentially with increasing distance with a correlation length ζ = 4.0(2) sites at T = 6.2K. This is shorter than the correlation length for an antiferromagnetic spin-1 Heisenberg chain at this temperature, suggesting that the correlations perpendicular to the chain direction and associated with the interchain coupling lower the single-chain correlation length. A multiparticle continuum is observed in the quantum-disordered phase in the region in reciprocal space where antiferromagnetic fluctuations are strongest, extending in energy up to twice the maximum of the dispersion of the well-defined triplet excitations. We show that the continuum satisfies the Hohenberg-Brinkman sum rule. The dependence of the multiparticle continuum on the chain wave vector resembles that of the two-spinon continuum in antiferromagnetic spin-1/2 Heisenberg chains. This suggests the presence of spin-1/2 degrees of freedom in CsNiCl 3 for T ∼< 12 K, possibly caused by multiply frustrated interchain interactions.

  5. Frustrated spin-1/2 ladder with ferro- and antiferromagnetic legs

    Science.gov (United States)

    Maiti, Debasmita; Dey, Dayasindhu; Kumar, Manoranjan

    2018-01-01

    Two-leg spin-1/2 ladder systems consisting of a ferromagnetic leg and an antiferromagnetic leg are considered where the spins on the legs interact through antiferromagnetic rung couplings J1 . These ladders can have two geometrical arrangements either zigzag or normal ladder and these systems are frustrated irrespective of their geometry. This frustration gives rise to incommensurate spin density wave, dimer and spin fluid phases in the ground state. The magnetization in the systems decreases linearly with J12, and the systems show an incommensurate phase for 0.0 spin-spin correlation functions in the incommensurate phase follow power law decay which is very similar to Heisenberg antiferromagnetic chain in external magnetic field. In large J1 limit, the normal ladder behaves like a collection of singlet dimers, whereas the zigzag ladder behaves as a one dimensional spin-1/2 antiferromagnetic chain.

  6. Studies of diluted antiferromagnets MnxMg1-xTiO3 with x=0.55 and 0.70 by muon spin relaxation method

    International Nuclear Information System (INIS)

    Fukaya, A.; Ito, A.; Torikai, E.; Nishiyama, K.; Nagamine, K.

    1997-01-01

    Longitudinal fields μSR measurements have been performed in order to probe the spin dynamics in the diluted antiferromagnets Mn x Mg 1-x TiO 3 with x=0.70 and 0.55. In the x=0.70 sample which forms the antiferromagnetic long-range order, the static and fluctuating fields coexist at the muon stopping site below T N . On the other hand, in the x=0.55 sample which shows the spin-glass behavior, the local fields fluctuate rather fast even below T SG . We infer that this drastic change occurs when Mn x Mg 1-x TiO 3 transforms from an antiferromagnetic system to a spin-glass system by dilution

  7. Superconductivity mediated by quantum critical antiferromagnetic fluctuations: The rise and fall of hot spots

    Science.gov (United States)

    Wang, Xiaoyu; Schattner, Yoni; Berg, Erez; Fernandes, Rafael M.

    2017-05-01

    In several unconventional superconductors, the highest superconducting transition temperature Tc is found in a region of the phase diagram where the antiferromagnetic transition temperature extrapolates to zero, signaling a putative quantum critical point. The elucidation of the interplay between these two phenomena—high-Tc superconductivity and magnetic quantum criticality—remains an important piece of the complex puzzle of unconventional superconductivity. In this paper, we combine sign-problem-free quantum Monte Carlo simulations and field-theoretical analytical calculations to unveil the microscopic mechanism responsible for the superconducting instability of a general low-energy model, called the spin-fermion model. In this approach, low-energy electronic states interact with each other via the exchange of quantum critical magnetic fluctuations. We find that even in the regime of moderately strong interactions, both the superconducting transition temperature and the pairing susceptibility are governed not by the properties of the entire Fermi surface, but instead by the properties of small portions of the Fermi surface called hot spots. Moreover, Tc increases with increasing interaction strength, until it starts to saturate at the crossover from hot-spots-dominated to Fermi-surface-dominated pairing. Our work provides not only invaluable insights into the system parameters that most strongly affect Tc, but also important benchmarks to assess the origin of superconductivity in both microscopic models and actual materials.

  8. Correlation functions of electronic and nuclear spins in a Heisenberg antiferromagnet semi-infinite medium

    International Nuclear Information System (INIS)

    Sarmento, E.F.

    1981-01-01

    Results are found for the dynamical correlation functions (or its corresponding Green's functions) among any combination including operator pairs of electronic and nuclear spins in an antiferromagnet semi-infinite medium, at low temperatures T [pt

  9. Spin waves treatment of the antiferromagnetic ground state of two Ising-like systems

    Directory of Open Access Journals (Sweden)

    Adegoke Kunle

    2014-01-01

    Full Text Available Using Anderson's spin wave theory, we derive expressions for the ground state energy of two Ising-like systems. Antiferromagnetic long range order is predicted for one of the systems.

  10. Spin-orbit torque in two-dimensional antiferromagnetic topological insulators

    KAUST Repository

    Ghosh, Sumit

    2017-01-24

    We investigate spin transport in two-dimensional ferromagnetic (FTI) and antiferromagnetic (AFTI) topological insulators. In the presence of an in-plane magnetization AFTI supports zero energy modes, which enables topologically protected edge conduction at low energy. We address the nature of current-driven spin torque in these structures and study the impact of spin-independent disorder. Interestingly, upon strong disorder the spin torque develops an antidamping component (i.e., even upon magnetization reversal) along the edges, which could enable current-driven manipulation of the antiferromagnetic order parameter. This antidamping torque decreases when increasing the system size and when the system enters the trivial insulator regime.

  11. Superconductivity, Antiferromagnetism, and Neutron Scattering

    OpenAIRE

    Tranquada, John M.; Xu, Guangyong; Zaliznyak, Igor A.

    2013-01-01

    High-temperature superconductivity in both the copper-oxide and the iron-pnictide/chalcogenide systems occurs in close proximity to antiferromagnetically ordered states. Neutron scattering has been an essential technique for characterizing the spin correlations in the antiferromagnetic phases and for demonstrating how the spin fluctuations persist in the superconductors. While the nature of the spin correlations in the superconductors remains controversial, the neutron scattering measurements...

  12. Superconductivity, antiferromagnetism, and neutron scattering

    International Nuclear Information System (INIS)

    Tranquada, John M.; Xu, Guangyong; Zaliznyak, Igor A.

    2014-01-01

    High-temperature superconductivity in both the copper-oxide and the iron–pnictide/chalcogenide systems occurs in close proximity to antiferromagnetically ordered states. Neutron scattering has been an essential technique for characterizing the spin correlations in the antiferromagnetic phases and for demonstrating how the spin fluctuations persist in the superconductors. While the nature of the spin correlations in the superconductors remains controversial, the neutron scattering measurements of magnetic excitations over broad ranges of energy and momentum transfers provide important constraints on the theoretical options. We present an overview of the neutron scattering work on high-temperature superconductors and discuss some of the outstanding issues. - Highlights: • High-temperature superconductivity is closely associated with antiferromagnetism. • Antiferromagnetic spin fluctuations coexist with the superconductivity. • Neutron scattering is essential for characterising the full spectrum of spin excitations

  13. Odd number of coupled antiferromagnetic anisotropic Heisenberg chains: Spin wave theory

    International Nuclear Information System (INIS)

    Benyoussef, A.

    1996-10-01

    The effect of the chain and perpendicular anisotropies on the energy gap for odd number of coupled quantum spin-1/2 antiferromagnetic anisotropic Heisenberg chains is investigated using a spin wave theory. The energy gap opens above a critical anisotropic value. The known results of the isotropic case have been obtained. (author). 11 refs, 4 figs

  14. Persistent nonequilibrium dynamics of the thermal energies in the spin and phonon systems of an antiferromagnet

    Directory of Open Access Journals (Sweden)

    A. von Reppert

    2016-09-01

    Full Text Available We present a temperature and fluence dependent Ultrafast X-Ray Diffraction study of a laser-heated antiferromagnetic dysprosium thin film. The loss of antiferromagnetic order is evidenced by a pronounced lattice contraction. We devise a method to determine the energy flow between the phonon and spin system from calibrated Bragg peak positions in thermal equilibrium. Reestablishing the magnetic order is much slower than the cooling of the lattice, especially around the Néel temperature. Despite the pronounced magnetostriction, the transfer of energy from the spin system to the phonons in Dy is slow after the spin-order is lost.

  15. Magnetic correlations and quantum criticality in the insulating antiferromagnetic, insulating spin liquid, renormalized Fermi liquid, and metallic antiferromagnetic phases of the Mott system V{sub 2}O{sub 3}

    Energy Technology Data Exchange (ETDEWEB)

    Bao, W. [Physics Department, Brookhaven National Laboratory, Upton, New York 11973 (United States); Broholm, C. [Department of Physics and Astronomy, The Johns Hopkins University, Baltimore, Maryland 21218 (United States)]|[Center for Neutron Research, National Institute of Standards and Technology, Gaithersburg, Maryland 20899 (United States); Aeppli, G. [NEC, 4 Independence Way, Princeton, New Jersey 08540 (United States); Carter, S.A. [Department of Physics, University of California, Santa Cruz, California 95064 (United States); Dai, P. [Solid State Division, Oak Ridge National Laboratory, Oak Ridge, Tennessee 37831 (United States); Rosenbaum, T.F. [James Franck Institute and Department of Physics, University of Chicago, Chicago, Illinois 60637 (United States); Honig, J.M.; Metcalf, P. [Department of Chemistry, Purdue University, West Lafayette, Indiana 47907 (United States); Trevino, S.F. [United States Army Research Laboratory, Adelphi, Maryland 20783 (United States)]|[Center for Neutron Research, National Institute of Standards and Technology, Gaithersburg, Maryland 20899 (United States)

    1998-11-01

    Magnetic correlations in all four phases of pure and doped vanadium sesquioxide (V{sub 2}O{sub 3}) have been examined by magnetic thermal-neutron scattering. Specifically, we have studied the antiferromagnetic and paramagnetic phases of metallic V{sub 2{minus}y}O{sub 3}, the antiferromagnetic insulating and paramagnetic metallic phases of stoichiometric V{sub 2}O{sub 3}, and the antiferromagnetic and paramagnetic phases of insulating V{sub 1.944}Cr{sub 0.056}O{sub 3}. While the antiferromagnetic insulator can be accounted for by a localized Heisenberg spin model, the long-range order in the antiferromagnetic metal is an incommensurate spin-density wave, resulting from a Fermi surface nesting instability. Spin dynamics in the strongly correlated metal are dominated by spin fluctuations with a {open_quotes}single lobe{close_quotes} spectrum in the Stoner electron-hole continuum. Furthermore, our results in metallic V{sub 2}O{sub 3} represent an unprecedentedly complete characterization of the spin fluctuations near a metallic quantum critical point, and provide quantitative support for the self-consistent renormalization theory for itinerant antiferromagnets in the small moment limit. Dynamic magnetic correlations for {h_bar}{omega}{lt}k{sub B}T in the paramagnetic insulator carry substantial magnetic spectral weight. However, they are extremely short-ranged, extending only to the nearest neighbors. The phase transition to the antiferromagnetic insulator, from the paramagnetic metal and the paramagnetic insulator, introduces a sudden switching of magnetic correlations to a different spatial periodicity which indicates a sudden change in the underlying spin Hamiltonian. To describe this phase transition and also the unusual short-range order in the paramagnetic state, it seems necessary to take into account the orbital degrees of freedom associated with the degenerate {ital d} orbitals at the Fermi level in V{sub 2}O{sub 3}. {copyright} {ital 1998} {ital The American

  16. Antiferromagnetism in the Hubbard model using a cluster slave-spin method

    Science.gov (United States)

    Lee, Wei-Cheng; Lee, Ting-Kuo

    2017-09-01

    The cluster slave-spin method is introduced to systematically investigate the solutions of the Hubbard model including the symmetry-broken phases. In this method, the electron operator is factorized into a fermionic spinon describing the physical spin and a slave-spin describing the charge fluctuations. Following the U (1 ) formalism derived by Yu and Si [Phys. Rev. B 86, 085104 (2012), 10.1103/PhysRevB.86.085104], it is shown that the self-consistent equations to explore various symmetry-broken density wave states can be constructed in general with a cluster of multiple slave-spin sites. We employ this method to study the antiferromagnetic (AFM) state in the single band Hubbard model with the two- and four-site clusters of slave spins. While the Hubbard gap, the charge gap due to the doubly occupied states, scales with the Hubbard interaction U as expected, the AFM gap Δ , the gap in the spinon dispersion in the AFM state, exhibits a crossover from the weak- to strong-coupling behaviors as U increases. Our cluster slave-spin method reproduces not only the traditional mean-field behavior of Δ ˜U in the weak-coupling limit, but also the behavior of Δ ˜t2/U predicted by the superexchange mechanism in the strong-coupling limit. In addition, the holon-doublon correlator as functions of U and doping x is also computed, which exhibits a strong tendency toward the holon-doublon binding in the strong coupling regime. We further show that the quasiparticle weight obtained by the cluster slave-spin method is in a good agreement with the generalized Gutzwiller approximation in both AFM and paramagnetic states, and the results can be improved beyond the generalized Gutzwiller approximation as the cluster is enlarged from a single site to four sites. Our results demonstrate that the cluster slave-spin method can be a powerful tool to systematically investigate the strongly correlated system.

  17. Real-space imaging of non-collinear antiferromagnetic order with a single-spin magnetometer

    Science.gov (United States)

    Gross, I.; Akhtar, W.; Garcia, V.; Martínez, L. J.; Chouaieb, S.; Garcia, K.; Carrétéro, C.; Barthélémy, A.; Appel, P.; Maletinsky, P.; Kim, J.-V.; Chauleau, J. Y.; Jaouen, N.; Viret, M.; Bibes, M.; Fusil, S.; Jacques, V.

    2017-09-01

    Although ferromagnets have many applications, their large magnetization and the resulting energy cost for switching magnetic moments bring into question their suitability for reliable low-power spintronic devices. Non-collinear antiferromagnetic systems do not suffer from this problem, and often have extra functionalities: non-collinear spin order may break space-inversion symmetry and thus allow electric-field control of magnetism, or may produce emergent spin-orbit effects that enable efficient spin-charge interconversion. To harness these traits for next-generation spintronics, the nanoscale control and imaging capabilities that are now routine for ferromagnets must be developed for antiferromagnetic systems. Here, using a non-invasive, scanning single-spin magnetometer based on a nitrogen-vacancy defect in diamond, we demonstrate real-space visualization of non-collinear antiferromagnetic order in a magnetic thin film at room temperature. We image the spin cycloid of a multiferroic bismuth ferrite (BiFeO3) thin film and extract a period of about 70 nanometres, consistent with values determined by macroscopic diffraction. In addition, we take advantage of the magnetoelectric coupling present in BiFeO3 to manipulate the cycloid propagation direction by an electric field. Besides highlighting the potential of nitrogen-vacancy magnetometry for imaging complex antiferromagnetic orders at the nanoscale, these results demonstrate how BiFeO3 can be used in the design of reconfigurable nanoscale spin textures.

  18. Correlation functions of electronic and nuclear spins in a Heisenberg antiferromagnet semi-infinite media

    International Nuclear Information System (INIS)

    Sarmento, E.F.

    1980-01-01

    Results are found for the correlation dynamic functions (or the correspondent green functions) between any combination including pairs of electronic anel nuclear spin operators in an antiferromagnet semi-infinite media., at low temperature T N . These correlation functions, are used to investigate, at the same time, the properties of surface spin waves in volume and surface. The dispersion relatons of nuclear and electronic spin waves coupled modes, in surface are found, resolving a system of linearized equatons of spin operators a system of linearized equations of spin operators. (author) [pt

  19. Simultaneous optimization of spin fluctuations and superconductivity under pressure in an iron-based superconductor.

    Science.gov (United States)

    Ji, G F; Zhang, J S; Ma, Long; Fan, P; Wang, P S; Dai, J; Tan, G T; Song, Y; Zhang, C L; Dai, Pengcheng; Normand, B; Yu, Weiqiang

    2013-09-06

    We present a high-pressure NMR study of the overdoped iron pnictide superconductor NaFe0.94Co0.06As. The low-energy antiferromagnetic spin fluctuations in the normal state, manifest as the Curie-Weiss upturn in the spin-lattice relaxation rate 1/(75)T1T, first increase strongly with pressure but fall again at P>Popt=2.2  GPa. Neither long-ranged magnetic order nor a structural phase transition is encountered up to 2.5 GPa. The superconducting transition temperature Tc shows a pressure dependence identical to the spin fluctuations. Our observations demonstrate that magnetic correlations and superconductivity are optimized simultaneously as a function of the electronic structure, thereby supporting very strongly a magnetic origin of superconductivity.

  20. Spin-Hall effect and emergent antiferromagnetic phase transition in n-Si

    Science.gov (United States)

    Lou, Paul C.; Kumar, Sandeep

    2018-04-01

    Spin current experiences minimal dephasing and scattering in Si due to small spin-orbit coupling and spin-lattice interactions is the primary source of spin relaxation. We hypothesize that if the specimen dimension is of the same order as the spin diffusion length then spin polarization will lead to non-equilibrium spin accumulation and emergent phase transition. In n-Si, spin diffusion length has been reported up to 6 μm. The spin accumulation in Si will modify the thermal transport behavior of Si, which can be detected with thermal characterization. In this study, we report observation of spin-Hall effect and emergent antiferromagnetic phase transition behavior using magneto-electro-thermal transport characterization. The freestanding Pd (1 nm)/Ni80Fe20 (75 nm)/MgO (1 nm)/n-Si (2 μm) thin film specimen exhibits a magnetic field dependent thermal transport and spin-Hall magnetoresistance behavior attributed to Rashba effect. An emergent phase transition is discovered using self-heating 3ω method, which shows a diverging behavior at 270 K as a function of temperature similar to a second order phase transition. We propose that spin-Hall effect leads to the spin accumulation and resulting emergent antiferromagnetic phase transition. We propose that the length scale for Rashba effect can be equal to the spin diffusion length and two-dimensional electron gas is not essential for it. The emergent antiferromagnetic phase transition is attributed to the site inversion asymmetry in diamond cubic Si lattice.

  1. Spin polaron in two-dimensional antiferromagnetics - from local singlet to compound quasi-particle

    CERN Document Server

    Barabanov, A F; Belemuk, A M

    2002-01-01

    The basic theoretical concepts, related to the spin polaron scenario for the charge excitations in the two-dimensional antiferromagnetics, are presented. The distinctive peculiarity of the developed approach consists in consideration of the local polaron as the zero approximation for the quasi-particles. On the following stage this excitation is coated into the antiferromagnetic spin waves and the radius intermediate polaron is formed. The method makes it possible to continuously describe the transition from the zero temperatures to the finite ones and to consider the wide doping range. The above approach explains basic results of the ARPES-experiments in the CuO sub 2 plane

  2. Itinerant spin dynamics in iron-based superconductors and cerium-based heavy-fermion antiferromagnets

    International Nuclear Information System (INIS)

    Friemel, Gerd

    2014-01-01

    This thesis contains a comprehensive study of the spin excitations by inelastic neutron scattering (INS) in two different correlated electron systems: the alkali-metal iron selenide superconductors (FeSe122) A x Fe 2-y Se 2 (A=K, Rb, Cs) and the heavy-fermion antiferromagnet CeB6. Both systems exhibit intense modes in their spin-fluctuation spectrum below their respective transition temperatures that can be derived from the spin dynamics of the itinerant quasiparticles. However, the implications of these observations, presented here, are different for each particular compound. The A x Fe 2-y Se 2 superconductors, with a uniform T c of 32 K, belong to a qualitative new family of superconductors. They possess a distinctly different Fermi surface compared to the iron-arsenide-based analogues XFe 2 As 2 (X=Ca, Sr, Ba). Instead of the central hole pockets at Γ and the electron pockets at X((1)/(2) 0), which are nested by the Q AFM = ((1)/(2) 0) vector, there exist only large electron pockets at the X point. Therefore, the magnetic instability along Q AFM that presumably provides the pairing glue for the superconductivity in the shape of spin fluctuations is absent in the FeSe122. The search for spin fluctuations by INS was motivated by a theoretical analysis that predicted their presence at an incommensurate wave vector near Q = (0.5 δ), δ = 0.3125 which results from a quasinesting by Q between the flat parts of the electron pockets. Two samples, namely Rb 0.8 Fe 1.6 Se 2 and K 0.77 Fe 1.85 Se 2 , were prepared and both showed a sizable anisotropic magnetic response at Q sf = ((1)/(2) (1)/(4)) in the normal state. Furthermore, upon entering the superconducting (SC) state a strong excitation appears at ℎω res = 14 meV in the spectrum at Q sf , which is referred to as magnetic resonant mode. This mode is interpreted as a bound spin-1 exciton below the SC charge gap. Its presence implies an unconventional order parameter, which changes the sign between the electron

  3. Itinerant spin dynamics in iron-based superconductors and cerium-based heavy-fermion antiferromagnets

    Energy Technology Data Exchange (ETDEWEB)

    Friemel, Gerd

    2014-05-26

    This thesis contains a comprehensive study of the spin excitations by inelastic neutron scattering (INS) in two different correlated electron systems: the alkali-metal iron selenide superconductors (FeSe122) A{sub x}Fe{sub 2-y}Se{sub 2} (A=K, Rb, Cs) and the heavy-fermion antiferromagnet CeB6. Both systems exhibit intense modes in their spin-fluctuation spectrum below their respective transition temperatures that can be derived from the spin dynamics of the itinerant quasiparticles. However, the implications of these observations, presented here, are different for each particular compound. The A{sub x}Fe{sub 2-y}Se{sub 2} superconductors, with a uniform T{sub c} of 32 K, belong to a qualitative new family of superconductors. They possess a distinctly different Fermi surface compared to the iron-arsenide-based analogues XFe{sub 2}As{sub 2} (X=Ca, Sr, Ba). Instead of the central hole pockets at Γ and the electron pockets at X((1)/(2) 0), which are nested by the Q{sub AFM} = ((1)/(2) 0) vector, there exist only large electron pockets at the X point. Therefore, the magnetic instability along Q{sub AFM} that presumably provides the pairing glue for the superconductivity in the shape of spin fluctuations is absent in the FeSe122. The search for spin fluctuations by INS was motivated by a theoretical analysis that predicted their presence at an incommensurate wave vector near Q = (0.5 δ), δ = 0.3125 which results from a quasinesting by Q between the flat parts of the electron pockets. Two samples, namely Rb{sub 0.8}Fe{sub 1.6}Se{sub 2} and K{sub 0.77}Fe{sub 1.85}Se{sub 2}, were prepared and both showed a sizable anisotropic magnetic response at Q{sub sf} = ((1)/(2) (1)/(4)) in the normal state. Furthermore, upon entering the superconducting (SC) state a strong excitation appears at ℎω{sub res} = 14 meV in the spectrum at Q{sub sf}, which is referred to as magnetic resonant mode. This mode is interpreted as a bound spin-1 exciton below the SC charge gap. Its presence

  4. Spin-orbit torques in locally and globally noncentrosymmetric crystals: Antiferromagnets and ferromagnets

    KAUST Repository

    Železný, J.

    2017-01-10

    One of the main obstacles that prevents practical applications of antiferromagnets is the difficulty of manipulating the magnetic order parameter. Recently, following the theoretical prediction [J. Železný, Phys. Rev. Lett. 113, 157201 (2014)]PRLTAO0031-900710.1103/PhysRevLett.113.157201, the electrical switching of magnetic moments in an antiferromagnet was demonstrated [P. Wadley, Science 351, 587 (2016)]SCIEAS0036-807510.1126/science.aab1031. The switching is due to the so-called spin-orbit torque, which has been extensively studied in ferromagnets. In this phenomena a nonequilibrium spin-polarization exchange coupled to the ordered local moments is induced by current, hence exerting a torque on the order parameter. Here we give a general systematic analysis of the symmetry of the spin-orbit torque in locally and globally noncentrosymmetric crystals. We study when the symmetry allows for a nonzero torque, when is the torque effective, and its dependence on the applied current direction and orientation of magnetic moments. For comparison, we consider both antiferromagnetic and ferromagnetic orders. In two representative model crystals we perform microscopic calculations of the spin-orbit torque to illustrate its symmetry properties and to highlight conditions under which the spin-orbit torque can be efficient for manipulating antiferromagnetic moments.

  5. Nonlocally sensing the magnetic states of nanoscale antiferromagnets with an atomic spin sensor.

    Science.gov (United States)

    Yan, Shichao; Malavolti, Luigi; Burgess, Jacob A J; Droghetti, Andrea; Rubio, Angel; Loth, Sebastian

    2017-05-01

    The ability to sense the magnetic state of individual magnetic nano-objects is a key capability for powerful applications ranging from readout of ultradense magnetic memory to the measurement of spins in complex structures with nanometer precision. Magnetic nano-objects require extremely sensitive sensors and detection methods. We create an atomic spin sensor consisting of three Fe atoms and show that it can detect nanoscale antiferromagnets through minute, surface-mediated magnetic interaction. Coupling, even to an object with no net spin and having vanishing dipolar stray field, modifies the transition matrix element between two spin states of the Fe atom-based spin sensor that changes the sensor's spin relaxation time. The sensor can detect nanoscale antiferromagnets at up to a 3-nm distance and achieves an energy resolution of 10 μeV, surpassing the thermal limit of conventional scanning probe spectroscopy. This scheme permits simultaneous sensing of multiple antiferromagnets with a single-spin sensor integrated onto the surface.

  6. Spin configuration in a frustrated ferromagnetic/antiferromagnetic thin-film system

    Energy Technology Data Exchange (ETDEWEB)

    Yamada, T K [Faculty of Science, Gakushuin University, 171-8588 Mejiro, Tokyo (Japan); MartInez, E [Fachbereich Physik, Universitaet Osnabrueck, D-49069 Osnabrueck (Germany); Vega, A [Departamento de Fisica Teorica, Atomica y Optica, Universidad de Valladolid, 47011 Valladolid (Spain); Robles, R [Department of Physics, Uppsala University, SE-75121 (Sweden); Stoeffler, D [Institut de Physique et Chimie des Materiaux de Strasbourg (UMR C7504 CNRS-ULP), Strasbourg (France); Parga, A L Vazquez de [Departamento de Fisica de la Materia Condensada, Universidad Autonoma de Madrid, Cantoblanco 28049, Madrid (Spain); Mizoguchi, T [Faculty of Science, Gakushuin University, 171-8588 Mejiro, Tokyo (Japan); Kempen, H van [Institute for Molecules and Materials, Radboud University, Toernooiveld 1, 6525 ED Nijmegen (Netherlands)

    2007-06-13

    We have studied the magnetic configuration in ultrathin antiferromagnetic Mn films grown around monoatomic steps on an Fe(001) surface by spin-polarized scanning tunnelling microscopy/spectroscopy and ab initio-parameterized self-consistent real-space tight-binding calculations in which the spin quantization axis is independent for each site, thus allowing noncollinear magnetism. Mn grown on Fe(001) presents a layered antiferromagnetic structure. In the regions where the Mn films overgrows Fe steps the magnetization of the surface layer is reversed across the steps. Around these defects a frustration of the antiferromagnetic order occurs. Due to the weakened magnetic coupling at the central Mn layers, the amount of frustration is smaller than in Cr, and the width of the wall induced by the step does not change with the thickness, at least for coverages up to seven monolayers.

  7. Ferromagnetic and Antiferromagnetic Coupling of Spin Molecular Interfaces with High Thermal Stability.

    Science.gov (United States)

    Avvisati, Giulia; Cardoso, Claudia; Varsano, Daniele; Ferretti, Andrea; Gargiani, Pierluigi; Betti, Maria Grazia

    2018-03-26

    We report an advanced organic spin-interface architecture with magnetic remanence at room temperature, constituted by metal phthalocyanine molecules magnetically coupled with Co layer(s), mediated by graphene. Fe- and Cu-phthalocyanines assembled on graphene/Co have identical structural configurations, but FePc couples antiferromagnetically with Co up to room temperature, while CuPc couples ferromagnetically with weaker coupling and thermal stability, as deduced by element-selective X-ray magnetic circular dichroic signals. The robust antiferromagnetic coupling is stabilized by a superexchange interaction, driven by the out-of-plane molecular orbitals responsible of the magnetic ground state and electronically decoupled from the underlying metal via the graphene layer, as confirmed by ab initio theoretical predictions. These archetypal spin interfaces can be prototypes to demonstrate how antiferromagnetic and/or ferromagnetic coupling can be optimized by selecting the molecular orbital symmetry.

  8. Antiferromagnetic Spin Coupling between Rare Earth Adatoms and Iron Islands Probed by Spin-Polarized Tunneling.

    Science.gov (United States)

    Coffey, David; Diez-Ferrer, José Luis; Serrate, David; Ciria, Miguel; de la Fuente, César; Arnaudas, José Ignacio

    2015-09-03

    High-density magnetic storage or quantum computing could be achieved using small magnets with large magnetic anisotropy, a requirement that rare-earth iron alloys fulfill in bulk. This compelling property demands a thorough investigation of the magnetism in low dimensional rare-earth iron structures. Here, we report on the magnetic coupling between 4f single atoms and a 3d magnetic nanoisland. Thulium and lutetium adatoms deposited on iron monolayer islands pseudomorphically grown on W(110) have been investigated at low temperature with scanning tunneling microscopy and spectroscopy. The spin-polarized current indicates that both kind of adatoms have in-plane magnetic moments, which couple antiferromagnetically with their underlying iron islands. Our first-principles calculations explain the observed behavior, predicting an antiparallel coupling of the induced 5d electrons magnetic moment of the lanthanides with the 3d magnetic moment of iron, as well as their in-plane orientation, and pointing to a non-contribution of 4f electrons to the spin-polarized tunneling processes in rare earths.

  9. The Multisite Antiferromagnetic Ising Spin Model and Universality of Feigenbaum Constants

    OpenAIRE

    Ananikian, N. S.; Lusiniants, R. R.; Oganessyan, K. A.

    1994-01-01

    The Feigenbaum constants $\\alpha$ and $\\delta$ for the three-site antiferromagnetic Ising spin model on Husimi tree are calculated. It is shown that the numerical values of these constants for this real physical system coincide with the famous universal Feigenbaum constants with high accuracy. The quantitative description from ordering to chaos is also obtained.

  10. Spin-transfer torques in antiferromagnetic textures: efficiency and quantification method

    Czech Academy of Sciences Publication Activity Database

    Yamane, Y.; Ieda, J.; Sinova, Jairo

    2016-01-01

    Roč. 94, č. 5 (2016), 1-8, č. článku 054409. ISSN 2469-9950 R&D Projects: GA ČR GB14-37427G Institutional support: RVO:68378271 Keywords : spin-transfer torques * antiferromagnets Subject RIV: BL - Plasma and Gas Discharge Physics Impact factor: 3.836, year: 2016

  11. Strong Coupling of Microwave Photons to Antiferromagnetic Fluctuations in an Organic Magnet

    Science.gov (United States)

    Mergenthaler, Matthias; Liu, Junjie; Le Roy, Jennifer J.; Ares, Natalia; Thompson, Amber L.; Bogani, Lapo; Luis, Fernando; Blundell, Stephen J.; Lancaster, Tom; Ardavan, Arzhang; Briggs, G. Andrew D.; Leek, Peter J.; Laird, Edward A.

    2017-10-01

    Coupling between a crystal of di(phenyl)-(2,4,6-trinitrophenyl)iminoazanium radicals and a superconducting microwave resonator is investigated in a circuit quantum electrodynamics (circuit QED) architecture. The crystal exhibits paramagnetic behavior above 4 K, with antiferromagnetic correlations appearing below this temperature, and we demonstrate strong coupling at base temperature. The magnetic resonance acquires a field angle dependence as the crystal is cooled down, indicating anisotropy of the exchange interactions. These results show that multispin modes in organic crystals are suitable for circuit QED, offering a platform for their coherent manipulation. They also utilize the circuit QED architecture as a way to probe spin correlations at low temperature.

  12. Low-frequency spin dynamics and NMR spin-lattice relaxation in antiferromagnetic rings

    Science.gov (United States)

    Itou, T.; Sagane, T.; Oyamada, A.; Maegawa, S.; Igarashi, S.; Yukawa, Y.

    2011-01-01

    We develop a general theory of the spin dynamics of Heisenberg antiferromagnetic rings (HAFRs) that explains the mechanism of NMR spin-lattice relaxation at low temperatures. In HAFRs, the imaginary parts of the q-summed dynamic spin susceptibilities parallel and perpendicular to an applied static field, χsum∥″(ω) and χsum⊥″(ω), are composed of the sum of many slightly broadened δ-functional modes at many frequencies. The NMR relaxation is caused by the quasielastic mode in χsum∥″(ω) at around zero frequency. This quasielastic mode is characterized by two physical quantities, intensity P0∥ and frequency width Γ0∥. Although P0∥ has to date been assumed to be identical to the uniform static susceptibility, we point out that the two quantities are not identical. Without making this unreliable assumption for P0∥, we demonstrate experimentally how P0∥ and Γ0∥ behave, by analyzing the NMR relaxation rates of two different nuclei, H1 and C13, in a real HAFR. This analysis is more rigorous and thus can be used to estimate Γ0∥ and P0∥ more precisely than previously possible. We find that the temperature dependence of P0∥ exhibits activation-type behavior reflecting the first excitation gap. We also find that Γ0∥ decreases monotonically on cooling but saturates to a nonzero value at zero temperature. This strongly suggests that Γ0∥ is dominated not only by the electron-phonon interactions but also by internanomagnet dipole interactions, which have been neglected to date.

  13. Effect of antiferromagnetic interfacial coupling on spin-wave resonance frequency of multi-layer film

    Energy Technology Data Exchange (ETDEWEB)

    Qiu, Rong-ke, E-mail: rkqiu@163.com; Cai, Wei

    2017-08-15

    Highlights: • A quantum approach is developed to study the SWR of a bicomponent multi-layer films. • The comparison of the SWR in films with FM and AFM interfacial coupling has been made. • The present results show the method to enhance and adjust the SWR frequency of films. - Abstract: We investigate the spin-wave resonance (SWR) frequency in a bicomponent bilayer and triple-layer films with antiferromagnetic or ferromagnetic interfacial couplings, as function of interfacial coupling, surface anisotropy, interface anisotropy, thickness and external magnetic field, using the linear spin-wave approximation and Green’s function technique. The microwave properties for multi-layer magnetic film with antiferromagnetic interfacial coupling is different from those for multi-layer magnetic film with ferromagnetic interfacial coupling. For the bilayer film with antiferromagnetic interfacial couplings, as the lower (upper) surface anisotropy increases, only the SWR frequencies of the odd (even) number modes increase. The lower (upper) surface anisotropy does not affect the SWR frequencies of the even (odd) number modes{sub .} For the multi-layer film with antiferromagnetic interfacial coupling, the SWR frequency of modes m = 1, 3 and 4 decreases while that of mode m = 2 increases with increasing thickness of the film within a proper parameter region. The present results could be useful in enhancing our fundamental understanding and show the method to enhance and adjust the SWR frequency of bicomponent multi-layer magnetic films with antiferromagnetic or ferromagnetic interfacial coupling.

  14. Magnetic order, magnetic correlations, and spin dynamics in the pyrochlore antiferromagnet Er2Ti2O7

    Science.gov (United States)

    Dalmas de Réotier, P.; Yaouanc, A.; Chapuis, Y.; Curnoe, S. H.; Grenier, B.; Ressouche, E.; Marin, C.; Lago, J.; Baines, C.; Giblin, S. R.

    2012-09-01

    Er2Ti2O7 is believed to be a realization of an XY antiferromagnet on a frustrated lattice of corner-sharing regular tetrahedra. It is presented as an example of the order-by-disorder mechanism in which fluctuations lift the degeneracy of the ground state, leading to an ordered state. Here we report detailed measurements of the low-temperature magnetic properties of Er2Ti2O7, which displays a second-order phase transition at TN≃1.2 K with coexisting short- and long-range orders. Magnetic susceptibility studies show that there is no spin-glass-like irreversible effect. Heat capacity measurements reveal that the paramagnetic critical exponent is typical of a 3-dimensional XY magnet while the low-temperature specific heat sets an upper limit on the possible spin-gap value and provides an estimate for the spin-wave velocity. Muon spin relaxation measurements show the presence of spin dynamics in the nanosecond time scale down to 21 mK. This time range is intermediate between the shorter time characterizing the spin dynamics in Tb2Sn2O7, which also displays long- and short-range magnetic order, and the time scale typical of conventional magnets. Hence the ground state is characterized by exotic spin dynamics. We determine the parameters of a symmetry-dictated Hamiltonian restricted to the spins in a tetrahedron, by fitting the paramagnetic diffuse neutron scattering intensity for two reciprocal lattice planes. These data are recorded in a temperature region where the assumption that the correlations are limited to nearest neighbors is fair.

  15. Spin Liquid State in the 3D Frustrated Antiferromagnet PbCuTe_{2}O_{6}: NMR and Muon Spin Relaxation Studies.

    Science.gov (United States)

    Khuntia, P; Bert, F; Mendels, P; Koteswararao, B; Mahajan, A V; Baenitz, M; Chou, F C; Baines, C; Amato, A; Furukawa, Y

    2016-03-11

    PbCuTe_{2}O_{6} is a rare example of a spin liquid candidate featuring a three-dimensional magnetic lattice. Strong geometric frustration arises from the dominant antiferromagnetic interaction that generates a hyperkagome network of Cu^{2+} ions although additional interactions enhance the magnetic lattice connectivity. Through a combination of magnetization measurements and local probe investigations by NMR and muon spin relaxation down to 20 mK, we provide robust evidence for the absence of magnetic freezing in the ground state. The local spin susceptibility probed by the NMR shift hardly deviates from the macroscopic one down to 1 K pointing to a homogeneous magnetic system with a low defect concentration. The saturation of the NMR shift and the sublinear power law temperature (T) evolution of the 1/T_{1} NMR relaxation rate at low T point to a nonsinglet ground state favoring a gapless fermionic description of the magnetic excitations. Below 1 K a pronounced slowing down of the spin dynamics is witnessed, which may signal a reconstruction of spinon Fermi surface. Nonetheless, the compound remains in a fluctuating spin liquid state down to the lowest temperature of the present investigation.

  16. Spin-lattice effects in selected antiferromagnetic materials

    Czech Academy of Sciences Publication Activity Database

    Zherlitsyn, S.; Yasin, S.; Wosnitza, J.; Zvyagin, A.A.; Andreev, Alexander V.; Tsurkan, V.

    2014-01-01

    Roč. 40, č. 2 (2014), s. 123-133 ISSN 1063-777X R&D Projects: GA ČR GAP204/12/0150 Grant - others:AVČR(CZ) M100101203 Keywords : low-dimensional spin systems * frustrated chromium spinels * spin-strain interaction * uranium-based compounds Subject RIV: BM - Solid Matter Physics ; Magnetism Impact factor: 0.786, year: 2014

  17. Distinct nature of orbital-selective Mott phases dominated by low-energy local spin fluctuations

    Science.gov (United States)

    Song, Ze-Yi; Jiang, Xiu-Cai; Lin, Hai-Qing; Zhang, Yu-Zhong

    2017-12-01

    Quantum orbital-selective Mott (OSM) transitions are investigated within dynamical mean-field theory based on a two-orbital Hubbard model with different bandwidth at half filling. We find two distinct OSM phases both showing coexistence of itinerant electrons and localized spins, dependent on whether the Hund's coupling is full or of Ising type. The critical values and the nature of the OSM transitions are efficiently determined by entanglement entropy. We reveal that vanishing of the Kondo energy scale evidenced by absence of local spin fluctuations at low frequency in local dynamical spin susceptibility is responsible for the appearance of non-Fermi-liquid OSM phase in Ising Hund's coupling case. We argue that this scenario can also be applied to account for emergent quantum non-Fermi liquid in the one-band Hubbard model when short-range antiferromagnetic order is considered.

  18. Magnetic Raman Scattering in Two-Dimensional Spin-1/2 Heisenberg Antiferromagnets: Explanation of the Spectral Shape Anomaly

    Science.gov (United States)

    Nori, F.; Merlin, R.; Haas, S.; Sandvick, A.; Dagotto, E.

    1996-03-01

    We calculate(F. Nori, R.Merlin, S. Haas, A.W. Sandvik, and E. Dagotto, Physical Review Letters) 75, 553 (1995). the Raman spectrum of the two-dimensional (2D) spin-1/2 Heisenberg antiferromagnet by exact diagonalization and quantum Monte Carlo techniques on clusters of up to 144 sites. On a 16-site cluster, we consider the phonon-magnon interaction which leads to random fluctuations of the exchange integral. Results are in good agreement with experiments on various high-Tc precursors, such as La_2CuO4 and YBa_2Cu_3O_6.2. In particular, our calculations reproduce the broad lineshape of the two-magnon peak, the asymmetry about its maximum, the existence of spectral weight at high energies, and the observation of nominally forbidden A_1g scattering.

  19. Chiral Spin Liquid on a Kagome Antiferromagnet Induced by the Dzyaloshinskii-Moriya Interaction

    Science.gov (United States)

    Messio, Laura; Bieri, Samuel; Lhuillier, Claire; Bernu, Bernard

    2017-06-01

    The quantum spin liquid material herbertsmithite is described by an antiferromagnetic Heisenberg model on the kagome lattice with a non-negligible Dzyaloshinskii-Moriya interaction (DMI). A well-established phase transition to the q =0 long-range order occurs in this model when the DMI strength increases, but the precise nature of a small-DMI phase remains controversial. Here, we describe a new phase obtained from Schwinger-boson mean-field theory that is stable at small DMI, and which can explain the dispersionless spectrum seen in the inelastic neutron scattering experiment by Han et al. [Nature (London) 492, 406 (2012), 10.1038/nature11659]. It is a time-reversal symmetry breaking Z2 spin liquid, with the unique property of a small and constant spin gap in an extended region of the Brillouin zone. The phase diagram as a function of DMI and spin size is given, and dynamical spin structure factors are presented.

  20. Self-consistent hole motion and spin excitations in a quantum antiferromagnet

    International Nuclear Information System (INIS)

    Su, Z.B.; Yu, L.; Li, Y.M.; Lai, W.Y.

    1989-12-01

    A new quantum Bogoliubov-de Gennes (BdeG) formalism is developed to study the self-consistent motion of holes and spin excitations in a quantum antiferromagnet within the generalized t-J model. On the one hand, the effects of local distortion of spin configurations and the renormalization of the hole motion due to virtual excitations of the distorted spin background are treated on an equal footing to obtain the hole wave function and its spectrum, as well as the effective mass for a propagating hole. On the other hand, the change of the spin excitation spectrum and the spin correlations due to the presence of dynamical holes are studied within the same adiabatic approximation. The stability of the hole states with respect to such changes justifies the self-consistency of the proposed formalism. (author). 25 refs, 6 figs, 1 tab

  1. Dynamical Negative Differential Resistance in Antiferromagnetically Coupled Few-Atom Spin Chains

    Science.gov (United States)

    Rolf-Pissarczyk, Steffen; Yan, Shichao; Malavolti, Luigi; Burgess, Jacob A. J.; McMurtrie, Gregory; Loth, Sebastian

    2017-11-01

    We present the appearance of negative differential resistance (NDR) in spin-dependent electron transport through a few-atom spin chain. A chain of three antiferromagnetically coupled Fe atoms (Fe trimer) was positioned on a Cu2 N /Cu (100 ) surface and contacted with the spin-polarized tip of a scanning tunneling microscope, thus coupling the Fe trimer to one nonmagnetic and one magnetic lead. Pronounced NDR appears at the low bias of 7 mV, where inelastic electron tunneling dynamically locks the atomic spin in a long-lived excited state. This causes a rapid increase of the magnetoresistance between the spin-polarized tip and Fe trimer and quenches elastic tunneling. By varying the coupling strength between the tip and Fe trimer, we find that in this transport regime the dynamic locking of the Fe trimer competes with magnetic exchange interaction, which statically forces the Fe trimer into its high-magnetoresistance state and removes the NDR.

  2. Muon Spin Relaxation Evidence for the U(1) Quantum Spin-Liquid Ground State in the Triangular Antiferromagnet YbMgGaO_{4}.

    Science.gov (United States)

    Li, Yuesheng; Adroja, Devashibhai; Biswas, Pabitra K; Baker, Peter J; Zhang, Qian; Liu, Juanjuan; Tsirlin, Alexander A; Gegenwart, Philipp; Zhang, Qingming

    2016-08-26

    Muon spin relaxation (μSR) experiments on single crystals of the structurally perfect triangular antiferromagnet YbMgGaO_{4} indicate the absence of both static long-range magnetic order and spin freezing down to 0.048 K in a zero field. Below 0.4 K, the μ^{+} spin relaxation rates, which are proportional to the dynamic correlation function of the Yb^{3+} spins, exhibit temperature-independent plateaus. All these μSR results unequivocally support the formation of a gapless U(1) quantum spin liquid ground state in the triangular antiferromagnet YbMgGaO_{4}.

  3. su(1,2) Algebraic Structure of XYZ Antiferromagnetic Model in Linear Spin-Wave Frame

    International Nuclear Information System (INIS)

    Jin Shuo; Xie Binghao; Yu Zhaoxian; Hou Jingmin

    2008-01-01

    The XYZ antiferromagnetic model in linear spin-wave frame is shown explicitly to have an su(1,2) algebraic structure: the Hamiltonian can be written as a linear function of the su(1,2) algebra generators. Based on it, the energy eigenvalues are obtained by making use of the similar transformations, and the algebraic diagonalization method is investigated. Some numerical solutions are given, and the results indicate that only one group solution could be accepted in physics

  4. Spin-orbit coupling induced anisotropy effects in bimetallic antiferromagnets: A route towards antiferromagnetic spintronics

    Czech Academy of Sciences Publication Activity Database

    Shick, Alexander; Khmelevskyi, S.; Mryasov, O. N.; Wunderlich, J.; Jungwirth, Tomáš

    2010-01-01

    Roč. 81, č. 21 (2010), 212409/1-212409/4 ISSN 1098-0121 R&D Projects: GA AV ČR IAA100100912; GA ČR GA202/07/0456; GA AV ČR KAN400100652; GA ČR GEFON/06/E002 EU Projects: European Commission(XE) 215368 - SemiSpinNet; European Commission(XE) 214499 - NAMASTE Grant - others:AV ČR(CZ) AP0801 Program:Akademická prémie - Praemium Academiae Institutional research plan: CEZ:AV0Z10100520; CEZ:AV0Z10100521 Keywords : magnetic anisotropy * tunneling anisotropic magneto-resistance * exchange bias Subject RIV: BM - Solid Matter Physics ; Magnetism Impact factor: 3.772, year: 2010 http://link.aps.org/doi/10.1103/PhysRevB.81.212409

  5. Antiferromagnetism of La2CuO(4-y) studied by muon-spin rotation

    Science.gov (United States)

    Uemura, Y. J.; Kossler, W. J.; Yu, X. H.; Kempton, J. R.; Schone, H. E.

    1987-01-01

    Zero-field spin precession of positive muons has been observed in the antiferromagnetic state of La2CuO(4-y). Sharp onsets of the sublattice magnetization are found at temperatures close to those of the susceptibility maxima of different specimens. The long-lived precession signal indicates a microscopically homogeneous distribution of spin density at each Cu atom below the Neel temperature. A combination of the present results and neutron-scattering studies indicates the ordered moment per Cu atom to be significantly less than 1 mu(B).

  6. Universal spin-polarization fluctuations in one-dimensional wires with magnetic impurities

    DEFF Research Database (Denmark)

    Mortensen, Asger; Egues, J.C.

    2002-01-01

    -flip suppresses conductance fluctuations while enhancing spin-polarization fluctuations. More importantly, spin-polarization fluctuations attain a universal value 1/3 for large enough spin-flip strengths. This intrinsic spin-polarization fluctuation may pose a severe limiting factor to the realization of steady...

  7. Extended dynamic spin-fluctuation theory of metallic magnetism

    Energy Technology Data Exchange (ETDEWEB)

    Melnikov, N B [Moscow State University, Moscow 119991 (Russian Federation); Reser, B I; Grebennikov, V I, E-mail: melnikov@cs.msu.su, E-mail: reser@imp.uran.ru, E-mail: greben@imp.uran.ru [Institute of Metal Physics, Ural Branch of the Russian Academy of Sciences, Ekaterinburg 620990 (Russian Federation)

    2011-07-13

    A dynamic spin-fluctuation theory that directly takes into account nonlocality of thermal spin fluctuations and their mode-mode interactions is developed. The Gaussian approximation in the theory is improved by a self-consistent renormalization of the mean field and spin susceptibility due to the third- and fourth-order terms of the free energy, respectively. This eliminates the fictitious first-order phase transition, which is typical for the Gaussian approximation, and yields a proper second-order phase transition. The effect of nonlocal spin correlations is enhanced by taking into account uniform fluctuations in the single-site mean Green function. Explicit computational formulae for basic magnetic characteristics are obtained. The extended theory is applied to the calculation of magnetic properties of Fe-Ni Invar. Almost full agreement with experiment is achieved for the magnetization, Curie temperature, and local and effective magnetic moments.

  8. Antiferromagnetic spintronics

    Science.gov (United States)

    Baltz, V.; Manchon, A.; Tsoi, M.; Moriyama, T.; Ono, T.; Tserkovnyak, Y.

    2018-01-01

    Antiferromagnetic materials could represent the future of spintronic applications thanks to the numerous interesting features they combine: they are robust against perturbation due to magnetic fields, produce no stray fields, display ultrafast dynamics, and are capable of generating large magnetotransport effects. Intense research efforts over the past decade have been invested in unraveling spin transport properties in antiferromagnetic materials. Whether spin transport can be used to drive the antiferromagnetic order and how subsequent variations can be detected are some of the thrilling challenges currently being addressed. Antiferromagnetic spintronics started out with studies on spin transfer and has undergone a definite revival in the last few years with the publication of pioneering articles on the use of spin-orbit interactions in antiferromagnets. This paradigm shift offers possibilities for radically new concepts for spin manipulation in electronics. Central to these endeavors are the need for predictive models, relevant disruptive materials, and new experimental designs. This paper reviews the most prominent spintronic effects described based on theoretical and experimental analysis of antiferromagnetic materials. It also details some of the remaining bottlenecks and suggests possible avenues for future research. This review covers both spin-transfer-related effects, such as spin-transfer torque, spin penetration length, domain-wall motion, and "magnetization" dynamics, and spin-orbit related phenomena, such as (tunnel) anisotropic magnetoresistance, spin Hall, and inverse spin galvanic effects. Effects related to spin caloritronics, such as the spin Seebeck effect, are linked to the transport of magnons in antiferromagnets. The propagation of spin waves and spin superfluids in antiferromagnets is also covered.

  9. Current-induced spin-orbit torques in ferromagnetic and antiferromagnetic systems

    KAUST Repository

    Manchon, Aurelien

    2018-01-29

    Spin-orbit coupling in inversion-asymmetric magnetic crystals and structures has emerged as a powerful tool to generate complex magnetic textures, interconvert charge and spin under applied current, and control magnetization dynamics. Current-induced spin-orbit torques mediate the transfer of angular momentum from the lattice to the spin system, leading to sustained magnetic oscillations or switching of ferromagnetic as well as antiferromagnetic structures. The manipulation of magnetic order, domain walls and skyrmions by spin-orbit torques provides evidence of the microscopic interactions between charge and spin in a variety of materials and opens novel strategies to design spintronic devices with potentially high impact in data storage, nonvolatile logic, and magnonic applications. This paper reviews recent progress in the field of spin-orbitronics, focusing on theoretical models, material properties, and experimental results obtained on bulk noncentrosymmetric conductors and multilayer heterostructures, including metals, semiconductors, and topological insulator systems. Relevant aspects for improving the understanding and optimizing the efficiency of nonequilibrium spin-orbit phenomena in future nanoscale devices are also discussed.

  10. Generalized theory of spin fluctuations in itinerant electron magnets: Crucial role of spin anharmonicity

    International Nuclear Information System (INIS)

    Solontsov, A.

    2015-01-01

    The paper critically overviews the recent developments of the theory of spatially dispersive spin fluctuations (SF) in itinerant electron magnetism with particular emphasis on spin-fluctuation coupling or spin anharmonicity. It is argued that the conventional self-consistent renormalized (SCR) theory of spin fluctuations is usually used aside of the range of its applicability actually defined by the constraint of weak spin anharmonicity based on the random phase approximation (RPA) arguments. An essential step in understanding SF in itinerant magnets beyond RPA-like arguments was made recently within the soft-mode theory of SF accounting for strong spin anharmonicity caused by zero-point SF. In the present paper we generalize it to apply for a wider range of temperatures and regimes of SF and show it to lead to qualitatively new results caused by zero-point effects. - Highlights: • We review the spin-fluctuation theory of itinerant electron magnets with account of zero-point effects. • We generalize the existing theory to account for different regimes of spin fluctuations. • We show that zero-point spin fluctuations play a crucial role in both low- and high-temperature properties of metallic magnets. • We argue that a new scheme of calculation of ground state properties of magnets is needed including zero-point effects

  11. Spin fluctuations in EuS

    International Nuclear Information System (INIS)

    Hartmann, A.

    1996-02-01

    Demagnetization effects break the isotropy of spin waves. During spring 1995, Peter Boeni et al. performed polarized neutron measurements on EuS using the triple axis spectrometer IN14 at the ILL in Grenoble, in order to investigate the influence of dipolar interactions on the spin waves. In the following work the analysis of the experimental data is described. (author) 25 figs., 2 tabs., 9 refs

  12. Geometric phase of a central spin coupled to an antiferromagnetic environment

    International Nuclear Information System (INIS)

    Yuan Xiaozhong; Zhu Kadi; Goan, H.-S.

    2010-01-01

    Using the spin-wave approximation, we study the geometric phase (GP) of a central spin (signal qubit) coupled to an antiferromagnetic (AF) environment under the application of an external global magnetic field. The external magnetic field affects the GP of the qubit directly and also indirectly through its effect on the AF environment. We find that when the applied magnetic field is increased to the critical magnetic field point, the AF environment undergoes a spin-flop transition, a first-order phase transition, and at the same time the GP of the qubit changes abruptly to zero. This sensitive change of the GP of a signal qubit to the parameter change of a many-body environment near its critical point may serve as another efficient tool or witness to study the many-body phase transition. The influences of the AF environment temperature and crystal anisotropy field on the GP are also investigated.

  13. RVB signatures in the spin dynamics of the square-lattice Heisenberg antiferromagnet

    Science.gov (United States)

    Ghioldi, E. A.; Gonzalez, M. G.; Manuel, L. O.; Trumper, A. E.

    2016-03-01

    We investigate the spin dynamics of the square-lattice spin-\\frac{1}{2} Heisenberg antiferromagnet by means of an improved mean-field Schwinger boson calculation. By identifying both, the long-range Néel and the RVB-like components of the ground state, we propose an educated guess for the mean-field magnetic excitation consisting on a linear combination of local and bond spin flips to compute the dynamical structure factor. Our main result is that when this magnetic excitation is optimized in such a way that the corresponding sum rule is fulfilled, we recover the low- and high-energy spectral weight features of the experimental spectrum. In particular, the anomalous spectral weight depletion at (π,0) found in recent inelastic neutron scattering experiments can be attributed to the interference of the triplet bond excitations of the RVB component of the ground state. We conclude that the Schwinger boson theory seems to be a good candidate to adequately interpret the dynamic properties of the square-lattice Heisenberg antiferromagnet.

  14. Persistence of the gapless spin liquid in the breathing kagome Heisenberg antiferromagnet

    Science.gov (United States)

    Iqbal, Yasir; Poilblanc, Didier; Thomale, Ronny; Becca, Federico

    2018-03-01

    The nature of the ground state of the spin S =1 /2 Heisenberg antiferromagnet on the kagome lattice with breathing anisotropy (i.e., with different superexchange couplings J▵ and J▿ within elementary up- and down-pointing triangles) is investigated within the framework of Gutzwiller projected fermionic wave functions and Monte Carlo methods. We analyze the stability of the U(1 ) Dirac spin liquid with respect to the presence of fermionic pairing that leads to a gapped Z2 spin liquid. For several values of the ratio J▿/J▵ , the size scaling of the energy gain due to the pairing fields and the variational parameters are reported. Our results show that the energy gain of the gapped spin liquid with respect to the gapless state either vanishes for large enough system size or scales to zero in the thermodynamic limit. Similarly, the optimized pairing amplitudes (responsible for opening the spin gap) are shown to vanish in the thermodynamic limit. Our outcome is corroborated by the application of one and two Lanczos steps to the gapless and gapped wave functions, for which no energy gain of the gapped state is detected when improving the quality of the variational states. Finally, we discuss the competition with the "simplex" Z2 resonating-valence-bond spin liquid, valence-bond crystal, and nematic states in the strongly anisotropic regime, i.e., J▿≪J▵ .

  15. Magnetoresistance in RCo2 spin-fluctuation systems

    International Nuclear Information System (INIS)

    Gratz, E.; Nowotny, H.; Enser, J.; Bauer, E.; Hense, K.

    2004-01-01

    The effect of the spin fluctuations on the field and temperature dependence of the magnetoresistance in ScCo 2 and LuCo 2 was studied. The experimental data where explained assuming two competing mechanisms determining the magnetoresistance of these substances. One is the 'normal magnetoresistance' caused by the influence of the Lorentz force on conduction electron trajectories. The other is due to the suppression of the spin fluctuations caused by an external magnetic field. This interplay give rise to a pronounced drop of the magnetoresistance towards the lower temperature range

  16. Multicritical phase diagrams of the antiferromagnetic spin-3/2 Blume-Capel model

    Energy Technology Data Exchange (ETDEWEB)

    Keskin, Mustafa [Department of Physics, Erciyes University, 38039 Kayseri (Turkey)]. E-mail: keskin@erciyes.edu.tr; Ali Pinar, M. [Institute of Science, Erciyes University, 38039 Kayseri (Turkey); Erdinc, Ahmet [Department of Physics, Erciyes University, 38039 Kayseri (Turkey); Canko, Osman [Department of Physics, Erciyes University, 38039 Kayseri (Turkey)

    2006-04-24

    The antiferromagnetic spin-3/2 Blume-Capel model in an external magnetic field is investigated, and the phase diagrams are obtained in detail by using the cluster variation method. The model exhibits distinct critical regions, including the first-order, second-order and special points: two double critical points, a critical end point, a tricritical point and a zero-temperature critical point. The new phase diagram topology is also found that was not obtained previously. Comparison of the results with those of other studies on this, and closely related systems, is made.

  17. Multicritical phase diagrams of the antiferromagnetic spin-3/2 Blume-Capel model

    International Nuclear Information System (INIS)

    Keskin, Mustafa; Ali Pinar, M.; Erdinc, Ahmet; Canko, Osman

    2006-01-01

    The antiferromagnetic spin-3/2 Blume-Capel model in an external magnetic field is investigated, and the phase diagrams are obtained in detail by using the cluster variation method. The model exhibits distinct critical regions, including the first-order, second-order and special points: two double critical points, a critical end point, a tricritical point and a zero-temperature critical point. The new phase diagram topology is also found that was not obtained previously. Comparison of the results with those of other studies on this, and closely related systems, is made

  18. Magnetic fluctuations above the Neel temperature in {kappa}-(BEDT-TTF){sub 2}Cu[N(CN){sub 2}]Cl, a quasi-2D Heisenberg antiferromagnet with Dzyaloshinskii-Moriya interaction

    Energy Technology Data Exchange (ETDEWEB)

    Antal, Agnes; Feher, Titusz; Janossy, Andras [Budapest University of Technology and Economics, Institute of Physics and Condensed Matter Research Group of the Hungarian Academy of Sciences, P.O. Box 91, 1521 Budapest (Hungary); Nafradi, Balint; Forro, Laszlo [Institute of Physics of Complex Matter, FBS, Swiss Federal Institute of Technology (EPFL), 1015 Lausanne (Switzerland)

    2012-05-15

    We report on magnetic fluctuations studied by electron spin resonance (ESR) spectroscopy in the layered organic crystal {kappa}-(BEDT-TTF){sub 2}Cu[N(CN){sub 2}]Cl. A line broadening above the antiferromagnetic ordering temperature, T{sub N} = 23 K is attributed to two-dimensional magnetic fluctuations of a staggered magnetization induced by the interplay of the magnetic field and the Dzyaloshinskii-Moriya (DM) interaction. (Copyright copyright 2012 WILEY-VCH Verlag GmbH and Co. KGaA, Weinheim)

  19. Thermal Transport and Magnetotransport Properties of CuCr1-xMgxO2 with a Spin-3/2 Antiferromagnetic Triangular Lattice

    Science.gov (United States)

    Okuda, Tetsuji; Oozono, Satoshi; Kihara, Takumi; Tokunaga, Masashi

    2013-01-01

    We have investigated the thermal conductivity (κ) and magnetoresistance (MR) of non-doped and hole-doped delafossite CuCrO2 with a spin-3/2 antiferromagnetic (AF) triangular sublattice. The phonon mean free path above the Néel temperature (TN) deduced from κ and lattice specific heat is almost identical to the magnetic correlation length, which indicates that, for both compounds, spin fluctuation enhanced in a geometrically frustrated lattice is strongly coupled with acoustic phonon above TN. κ below TN is significantly suppressed by Mg substitution, suggesting the introduction of some disorder into the 120° Néel state. For the hole-doped CuCr0.97Mg0.03O2, a negative MR is observed above TN, which is enhanced with a decrease in T toward TN, while a component of positive MR appears below TN and the residual negative MR component is observed in a high magnetic field, indicating that spin fluctuation coupled with electrical conductivity is critically enhanced above TN and remains below TN. These results evidence that the 120° Néel state is partially disordered by a doped itinerant hole coupled with spin fluctuation, although AF transition is certainly promoted. The dynamic partial disorder may stabilize the Néel order through an order-by-disorder mechanism.

  20. Effect of Noise on the Decoherence of a Central Electron Spin Coupled to an Antiferromagnetic Spin Bath

    Directory of Open Access Journals (Sweden)

    G. C. Fouokeng

    2014-01-01

    Full Text Available We analyze the influence of a two-state autocorrelated noise on the decoherence and on the tunneling Landau-Zener (LZ transitions during a two-level crossing of a central electron spin (CES coupled to a one dimensional anisotropic-antiferomagnetic spin, driven by a time-dependent global external magnetic field. The energy splitting of the coupled spin system is found through an approach that computes the noise-averaged frequency. At low magnetic field intensity, the decoherence (or entangled state of a coupled spin system is dominated by the noise intensity. The effects of the magnetic field pulse and the spin gap antiferromagnetic material used suggest to us that they may be used as tools for the direct observation of the tunneling splitting through the LZ transitions in the sudden limit. We found that the dynamical frequencies display basin-like behavior decay with time, with the birth of entanglement, while the LZ transition probability shows Gaussian shape.

  1. Padé approximations for the magnetic susceptibilities of Heisenberg antiferromagnetic spin chains for various spin values

    International Nuclear Information System (INIS)

    Law, J M; Benner, H; Kremer, R K

    2013-01-01

    The temperature dependence of the spin susceptibilities of S = 1, 3/2 , 2, 5/2 and 7/2 Heisenberg antiferromagnetic 1D spins chains with nearest-neighbor coupling was simulated via quantum Monte Carlo calculations, within the reduced temperature range of 0.005 ≤ T* ≤ 100, and fitted to a Padé approximation with deviations between the simulated and fitted data of the same order of magnitude as or smaller than the quantum Monte Carlo simulation error. To demonstrate the practicality of our theoretical findings, we compare these results with the susceptibility of the well known 1D chain compound TMMC ([(CH 3 ) 4 N[MnCl 3

  2. Influence of spin and charge fluctuations on spectra of the two-dimensional Hubbard model

    Science.gov (United States)

    Sherman, A.

    2018-05-01

    The influence of spin and charge fluctuations on spectra of the two-dimensional fermionic Hubbard model is considered using the strong coupling diagram technique. Infinite sequences of diagrams containing ladder inserts, which describe the interaction of electrons with these fluctuations, are summed, and obtained equations are self-consistently solved for the ranges of Hubbard repulsions , temperatures and electron concentrations with t the intersite hopping constant. For all considered U the system exhibits a transition to the long-range antiferromagnetic order at . At the same time no indication of charge ordering is observed. Obtained solutions agree satisfactorily with results of other approaches and obey moments sum rules. In the considered region of the U-T plane, the curve separating metallic solutions passes from at the highest temperatures to U  =  2t at for half-filling. If only short-range fluctuations are allowed for the remaining part of this region is occupied by insulating solutions. Taking into account long-range fluctuations leads to strengthening of maxima tails, which transform a part of insulating solutions into bad-metal states. For low T, obtained results allow us to trace the gradual transition from the regime of strong correlations with the pronounced four-band structure and well-defined Mott gap for to the Slater regime of weak correlations with the spectral intensity having a dip along the boundary of the magnetic Brillouin zone due to an antiferromagnetic ordering for . For and doping leads to the occurrence of a pseudogap near the Fermi level, which is a consequence of the splitting out of a narrow band from a Hubbard subband. Obtained spectra feature waterfalls and Fermi arcs, which are similar to those observed in hole-doped cuprates.

  3. Antiferromagnetic spintronics

    KAUST Repository

    Baltz, V.

    2018-02-15

    Antiferromagnetic materials could represent the future of spintronic applications thanks to the numerous interesting features they combine: they are robust against perturbation due to magnetic fields, produce no stray fields, display ultrafast dynamics, and are capable of generating large magnetotransport effects. Intense research efforts over the past decade have been invested in unraveling spin transport properties in antiferromagnetic materials. Whether spin transport can be used to drive the antiferromagnetic order and how subsequent variations can be detected are some of the thrilling challenges currently being addressed. Antiferromagnetic spintronics started out with studies on spin transfer and has undergone a definite revival in the last few years with the publication of pioneering articles on the use of spin-orbit interactions in antiferromagnets. This paradigm shift offers possibilities for radically new concepts for spin manipulation in electronics. Central to these endeavors are the need for predictive models, relevant disruptive materials, and new experimental designs. This paper reviews the most prominent spintronic effects described based on theoretical and experimental analysis of antiferromagnetic materials. It also details some of the remaining bottlenecks and suggests possible avenues for future research. This review covers both spin-transfer-related effects, such as spin-transfer torque, spin penetration length, domain-wall motion, and

  4. Parametric excitation of nuclear spin waves in MnCO3 antiferromagnetic crystals

    International Nuclear Information System (INIS)

    Govorkov, S.A.; Tulin, V.A.

    1976-01-01

    Parametric excitation of nuclear spin waves in the antiferromagnetic crystal MnCO 3 is investigated at 1080 MHz by the parallel pumping technique. Two threshold processes are observed in the experiments. One refers to spin wave excitation in a nuclear magnetic system and the other to excitation of magneto-elastic waves. The post-threshold sample susceptibility in such processes is studied. After the second threshold a very pronounced overheating of the nuclear magnetic system of the sample with respect to the lattice is observed. The nature of these overheating phenomena shows that two magneto-elastic oscillation branches are excited in the second threshold process. The dependence of the threshold field on wave vector is more complicated in a small magnetic field due to magnetization processes in the sample. In a large magnetic field complications are evoked by the magneto-elastic coupling

  5. Thermal conductivity of a quantum spin-1/2 antiferromagnetic chain with magnetic impurities

    International Nuclear Information System (INIS)

    Zviagin, A.A.

    2008-01-01

    We present an exact theory that describes how magnetic impurities change the behavior of the thermal conductivity for the integrable Heisenberg antiferromagnetic quantum spin-1/2 chain. Single magnetic impurities and a large concentration of impurities with similar values of the couplings to the host chain (a weak disorder) do not change the linear-in-temperature low-T behavior of the thermal conductivity: Only the slope of that behavior becomes smaller, compared to the homogeneous case. The strong disorder in the distribution of the impurity-host couplings produces more rapid temperature growth of the thermal conductivity, compared to the linear-in-T dependence of the homogeneous chain and the chain with weak disorder. Recent experiments on the thermal conductivity in inhomogeneous quasi-one-dimensional quantum spin systems manifest qualitative agreement with our results

  6. Temperature dependence of fluctuation time scales in spin glasses

    DEFF Research Database (Denmark)

    Kenning, Gregory G.; Bowen, J.; Sibani, Paolo

    2010-01-01

    Using a series of fast cooling protocols we have probed aging effects in the spin glass state as a function of temperature. Analyzing the logarithmic decay found at very long time scales within a simple phenomenological barrier model, leads to the extraction of the fluctuation time scale of the s...

  7. Direct evidence of spin frustration in the fcc antiferromagnet NiS sub 2

    CERN Document Server

    Matsuura, M; Endoh, Y; Hirota, K; Yamada, K

    2002-01-01

    NiS sub 2 is a well-known Mott insulator with anomalous antiferromagnetic long-range order of coexistent type I (Q sub M =(1,0,0), T sub N sub 1 =40 K) and type II (Q sub M =(1/2,1/2,1/2), T sub N sub 2 =30 K). Extensive neutron-scattering measurements reveal that magnetism in NiS sub 2 is governed by geometrical spin frustration, resulting in magnetic diffuse scattering extending along the fcc zone boundary. Although the diffuse scattering exists at temperatures as high as 250 K (6T sub N sub 1), it disappears rapidly below T sub N sub 2 , associated with minor crystal distortion. We observed a clear energy gap in addition to the low-energy spin-wave excitation at significantly below 30 K, and obtain evidence that degeneracy due to the coexistence of the two types of antiferromagnetism is relieved in the ground state via the reduction in symmetry due to distortion. (orig.)

  8. Evolution of spin excitations in a gapped antiferromagnet from the quantum to the high-temperature limit

    DEFF Research Database (Denmark)

    Kenzelmann, M.; Cowley, R.A.; Buyers, W.J.L.

    2002-01-01

    We have mapped from the quantum to the classical limit the spin excitation spectrum of the antiferromagnetic spin-1 Heisenberg chain system CsNiCl3 in its paramagnetic phase from T=5 to 200 K. Neutron scattering shows that the excitations are resonant and dispersive up to at least T=70 Ksimilar...... or equal to2.7J, but broaden considerably with increasing temperature. The dispersion flattens out with increasing temperature as the resonance energy Delta at the antiferromagnetic wave vector increases and the maximum in the dispersion decreases. The correlation length xi between T=12 and 50 K...

  9. Theory of spin-fluctuation induced superconductivity in iron-based superconductors

    International Nuclear Information System (INIS)

    Zhang, Junhua

    2011-01-01

    In this dissertation we focus on the investigation of the pairing mechanism in the recently discovered high-temperature superconductor, iron pnictides. Due to the proximity to magnetic instability of the system, we considered short-range spin fluctuations as the major mediating source to induce superconductivity. Our calculation supports the magnetic fluctuations as a strong candidate that drives Cooper-pair formation in this material. We find the corresponding order parameter to be of the so-called ss-wave type and show its evolution with temperature as well as the capability of supporting high transition temperature up to several tens of Kelvin. On the other hand, our itinerant model calculation shows pronounced spin correlation at the observed antiferromagnetic ordering wave vector, indicating the underlying electronic structure in favor of antiferromagnetic state. Therefore, the electronic degrees of freedom could participate both in the magnetic and in the superconducting properties. Our work shows that the interplay between magnetism and superconductivity plays an important role to the understanding of the rich physics in this material. The magnetic-excitation spectrum carries important information on the nature of magnetism and the characteristics of superconductivity. We analyze the spin excitation spectrum in the normal and superconducting states of iron pnictides in the magnetic scenario. As a consequence of the sign-reversed gap structure obtained in the above, a spin resonance mode appears below the superconducting transition temperature. The calculated resonance energy, scaled with the gap magnitude and the magnetic correlation length, agrees well with the inelastic neutron scattering (INS) measurements. More interestingly, we find a common feature of those short-range spin fluctuations that are capable of inducing a fully gapped ss state is the momentum anisotropy with elongated span along the direction transverse to the antiferromagnetic momentum

  10. Magnetic structure and spin dynamics of the quasi-one-dimensional spin-chain antiferromagnet BaCo2V2O8

    DEFF Research Database (Denmark)

    Kawasaki, Yu; Gavilano, Jorge L.; Keller, Lukas

    2011-01-01

    We report a neutron diffraction and muon spin relaxation mu SR study of static and dynamical magnetic properties of BaCo2V2O8, a quasi-one-dimensional spin-chain system. A proposed model for the antiferromagnetic structure includes: a propagation vector (k) over right arrow (AF) = (0......,0,1), independent of external magnetic fields for fields below a critical value H-c(T). The ordered moments of 2.18 mu(B) per Co ion are aligned along the crystallographic c axis. Within the screw chains, along the c axis, the moments are arranged antiferromagnetically. In the basal planes the spins are arranged...... ferromagnetically (forming zigzag paths) along one of the axes and antiferromagnetically along the other. The temperature dependence of the sublattice magnetization is consistent with the expectations of the three-dimensional (3D) Ising model. A similar behavior is observed for the internal static fields...

  11. Search for the Heisenberg spin glass on rewired cubic lattices with antiferromagnetic interaction

    International Nuclear Information System (INIS)

    Surungan, Tasrief

    2016-01-01

    Spin glass (SG) is a typical magnetic system which is mainly characterized by a frozen random spin orientation at low temperatures. Frustration and randomness are considered to be the key ingredients for the existence of SGs. Previously, Bartolozzi et al . [Phys. Rev. B73, 224419 (2006)] found that the antiferromagnetic (AF) Ising spins on scale free network (SFN) exhibited SG behavior. This is purely AF system, a new type of SG different from the canonical one which requires the presence of both FM and AF couplings. In this new system, frustration is purely due to a topological factor and its randomness is brought by irregular connectivity. Recently, it was reported that the AF Heisenberg model on SFN exhibited SG behavior [Surungan et al ., JPCS, 640, 012005 (2015)/doi:10.1088/1742-6596/640/1/012005]. In order to accommodate the notion of spatial dimension, we further investigated this type of system by studying an AF Heisenberg model on rewired cubic lattices, constructed by adding one extra bond randomly connecting each spin to one of its next-nearest neighbors. We used Replica Exchange algorithm of Monte Carlo Method and calculated the SG order parameter to search for the existence of SG phase. (paper)

  12. Role of the antiferromagnetic pinning layer on spin wave properties in IrMn/NiFe based spin-valves

    Energy Technology Data Exchange (ETDEWEB)

    Gubbiotti, G., E-mail: gubbiotti@fisica.unipg.it; Tacchi, S. [Istituto Officina dei Materiali del CNR (IOM-CNR), Unità di Perugia, I-06123 Perugia (Italy); Del Bianco, L. [Department of Physics and Astronomy, University of Bologna, I-40127 Bologna (Italy); Department of Physics and Earth Sciences and CNISM, University of Ferrara, I-44122 Ferrara (Italy); Bonfiglioli, E.; Giovannini, L.; Spizzo, F.; Zivieri, R. [Department of Physics and Earth Sciences and CNISM, University of Ferrara, I-44122 Ferrara (Italy); Tamisari, M. [Department of Physics and Earth Sciences and CNISM, University of Ferrara, I-44122 Ferrara (Italy); Dipartimento di Fisica e Geologia, Università di Perugia, I-06123 Perugia (Italy)

    2015-05-07

    Brillouin light scattering (BLS) was exploited to study the spin wave properties of spin-valve (SV) type samples basically consisting of two 5 nm-thick NiFe layers (separated by a Cu spacer of 5 nm), differently biased through the interface exchange coupling with an antiferromagnetic IrMn layer. Three samples were investigated: a reference SV sample, without IrMn (reference); one sample with an IrMn underlayer (10 nm thick) coupled to the bottom NiFe film; one sample with IrMn underlayer and overlayer of different thickness (10 nm and 6 nm), coupled to the bottom and top NiFe film, respectively. The exchange coupling with the IrMn, causing the insurgence of the exchange bias effect, allowed the relative orientation of the NiFe magnetization vectors to be controlled by an external magnetic field, as assessed through hysteresis loop measurements by magneto-optic magnetometry. Thus, BLS spectra were acquired by sweeping the magnetic field so as to encompass both the parallel and antiparallel alignment of the NiFe layers. The BLS results, well reproduced by the presented theoretical model, clearly revealed the combined effects on the spin dynamic properties of the dipolar interaction between the two NiFe films and of the interface IrMn/NiFe exchange coupling.

  13. Zero sound and spin fluctuations in liquid helium-3

    International Nuclear Information System (INIS)

    Aldrich, C.H. III; Pethick, C.J.; Pines, D.

    1976-01-01

    The density fluctuation spectrum of 3 He is calculated using a generalized polarization potential approach and shown to yield both zero sound and quasiparticle spectra in good agreement with the recent neutron scattering experiments. Landau Fermi-liquid theory is used to calculate the spin density fluctuation spectrum; and sum-rule arguments are presented which enable us to establish the qualitative nature of this spectrum at larger wave vectors with results in good qualitative agreement with the recent experiment of Skold et al

  14. Spin waves and phonons in a paraelectric antiferromagnet EuTiO3

    Science.gov (United States)

    Cao, Huibo; Hong, Jiawang; Delaire, Olivier; Hahn, Steven; Ehlers, Georg; Chi, Songxue; Garlea, Vasile; Fernandez-Baca, Jaime; Chakoumakos, Bryan; Yan, Jiaqiang; Sales, Brian

    2015-03-01

    Perovskite titanates ATiO3 (A=Ba,Pb,Sr,Ca,Cd,or Eu) are widely studied for their interesting instabilities and broad applications. A ferroelectric (FE) transition occurs in Ba, Pb, and Cd titanates, but not in SrTiO3 (STO) or EuTiO3 (ETO). In the case of STO, fluctuations yield a quantum paraelectric state, but whether ETO is quantum paraelectric remains an open question. Despite a number of similarities with well-studied STO, ETO is also unique owing to the magnetic Eu ions. By applying a tuning parameter, such as bi-axial tension, ETO can be turned into a FE ferromagnet, the ideal multiferroic. [J. H. Lee, et al., Nature 466, 954 (2010)] Studies of spin-spin and spin-lattice couplings in ETO are of great interest not only from a fundamental standpoint, but also for technological applications. We successfully grew a large, high-quality isotopically-enriched ETO crystal for neutron scattering. The crystal and magnetic structures were characterized with single crystal diffraction at HB-3A at HFIR at ORNL. The spin waves and phonons were measured in the temperature range of 1.5-400 K with CNCS at SNS and HB-3 at HFIR at ORNL. In this presentation, we will discuss structural instabilities, spin-spin interactions, and spin-phonon couplings in ETO. This work was supported by Office of Basic Energy Sciences, U.S. Department of Energy.

  15. Spin reorientation and Ce-Mn coupling in antiferromagnetic oxypnictide CeMnAsO

    Science.gov (United States)

    Vaknin, David; Zhang, Qiang; Peterson, Spencer; Dennis, Kevin; Tian, Wei

    2015-03-01

    Structure and complex magnetic properties of CeMnAsO, a parent compound of the ``1111''-type oxypnictides, have been investigated using neutron powder diffraction and magnetization measurements. Whereas there is no structural transition from the P4/nmm tetragonal phase below 420 K, CeMnAsO undergoes a C-type antiferromagnetic order with Mn2+ (S = 5 / 2) moments pointing along the c-axis below a relatively high Néel temperature of TN = 345 K. Below TSR = 35 K, two instantaneous transitions occur where the Mn moments reorient to the ab-plane preserving the C-type magnetic order, and Ce moments undergo long-range AFM ordering with moments in the ab-plane. Another transition to a noncollinear magnetic structure occurs below 7 K. We find that CeMnAsO primarily falls into the category of a local-moment antiferromagnetic insulator in which the nearest-neighbor interaction (J1) is dominant. The spin reorientation transition driven by the coupling between rare earth Ce and transition metal seems to be common to Mn, Fe and Cr ion,but not to Co and Ni ions in the iso-structural oxypnictides. Supported by the Office of Basic Energy Sciences, US-DOE, Number DE-AC02-07CH11358.

  16. A separation of antiferromagnetic spin motion modes in the training effect of exchange biased Co/CoO film with in-plane anisotropy

    International Nuclear Information System (INIS)

    Wu, R.; Yun, C.; Ding, S. L.; Wen, X.; Liu, S. Q.; Wang, C. S.; Han, J. Z.; Du, H. L.; Yang, J. B.

    2016-01-01

    The motion of antiferromagnetic interfacial spins is investigated through the temperature evolution of training effect in a Co/CoO film with in-plane biaxial anisotropy. Significant differences in the training effect and its temperature dependence are observed in the magnetic easy axis and hard axis (HA) and ascribed to the different motion modes of antiferromagnetic interfacial spins, the collective spin cluster rotation (CSR) and the single spin reversal (SSR), caused by different magnetization reversal modes of ferromagnetic layer. These motion modes of antiferromagnetic spins are successfully separated using a combination of an exponential function and a classic n −1/2 function. A larger CSR to SSR ratio and a shorter lifetime of CSR found in the HA indicates that the domain rotation in the ferromagnetic layer tends to activate and accelerate a CSR mode in the antiferromagnetic spins.

  17. Search for the Heisenberg spin glass on rewired square lattices with antiferromagnetic interaction

    International Nuclear Information System (INIS)

    Surungan, Tasrief; Bansawang, B.J.; Tahir, Dahlang

    2016-01-01

    Spin glass (SG) is a typical magnetic system with frozen random spin orientation at low temperatures. The system exhibits rich physical properties, such as infinite number of ground states, memory effect, and aging phenomena. There are two main ingredients considered to be pivotal for the existence of SG behavior, namely, frustration and randomness. For the canonical SG system, frustration is led by the presence of competing interaction between ferromagnetic (FM) and antiferromagnetic (AF) couplings. Previously, Bartolozzi et al. [Phys. Rev. B73, 224419 (2006)], reported the SG properties of the AF Ising spins on scale free network (SFN). It is a new type of SG, different from the canonical one which requires the presence of both FM and AF couplings. In this new system, frustration is purely caused by the topological factor and its randomness is related to the irregular connectvity. Recently, Surungan et. al. [Journal of Physics: Conference Series, 640, 012001 (2015)] reported SG bahavior of AF Heisenberg model on SFN. We further investigate this type of system by studying an AF Heisenberg model on rewired square lattices. We used Replica Exchange algorithm of Monte Carlo Method and calculated the SG order parameter to search for the existence of SG phase.

  18. An S=1/2 impurity spin in the antiferromagnetic S=1 bond-alternating chain

    Energy Technology Data Exchange (ETDEWEB)

    Ogawa, Nobuyuki [Gifu National College of Technology, Dept. of Fundamental Science, Gifu (Japan); Hikihara, Toshiya [National Inst. for Materials Science, Computational Material Research Group, Tsukuba, Ibaraki (Japan); Kaburagi, Makoto [Kobe Univ., Faculty of Cross-Cultural Studies, Kobe, Hyogo (Japan); Tonegawa, Takashi [Fukui Univ. of Technology, Dept. of Mechanical Engineering, Fukui (Japan)

    2002-06-01

    We explore low-lying excited states as well as the ground state of the antiferromagnetic S=1 bond-alternating chain with an S=1/2 impurity spin. For the case where the ground-state phase of the host system is the Haldane phase, we review a numerical analysis of the electron-spin-resonance experimental results on the NENP: Cu{sup 2+} system. For the case where the ground-state phase of the host system is the dimer phase, on the other hand, we calculate, using the exact-diagonalization method, the dependences of the energy differences between the ground and low-lying excited states upon both the impurity-host exchange constant and the single-ion-type anisotropy constant, and also calculate, using the density-matrix renormalization-group method, the external-magnetic-field dependence of the impurity-spin magnetization in the ground state. In these calculations, we keep the NTENP: Cu{sup 2+} system in mind to choose the value of the bond-alternation parameter. We find that a few low-lying excited states which are expected from the valence-bond-solid picture appear as the impurity states in the energy gap between the singlet ground and triplet first-excited states (the dimer gap). Furthermore, for certain values of the above constants, we find that the impurity-spin magnetization shows a clear jump at a magnetic field which is in the dimer-gap region or in the magnetization-plateau region of the host system, and also that the impurity-spin magnetization has a magnetic-field region where it decreases as a function of the magnetic field. (author)

  19. Frustrated spin-1/2 Ising antiferromagnet on a square lattice in a transverse field

    Science.gov (United States)

    Bobák, A.; Jurčišinová, E.; Jurčišin, M.; Žukovič, M.

    2018-02-01

    We investigate the phase transitions and tricritical behaviors of the frustrated Ising antiferromagnet with first- (J1<0 ) and second- (J2<0 ) nearest-neighbor interactions in a transverse field Ω on the square lattice using an effective-field theory with correlations based on a single-spin approximation. We have proposed a functional for the free energy to obtain the phase diagram in the T -R (R =J2/|J1| ) or T -Ω planes. It is shown that due to the transverse field the phase transition between ordered and disordered phases changes in the tricritical point (TCP) from the second order to the first order. The longitudinal and transverse magnetizations are also studied for selected values of R and Ω . In particular, the variation of TCP at the ground state in the three-dimensional space is constructed. For some special cases, values of the critical temperature and the critical transverse field have been determined analytically.

  20. Coexistence of antiferromagnetism and spin polarization in double perovskite SrLaVMoO6

    International Nuclear Information System (INIS)

    Asano, H; Gotoh, H; Matsushima, H; Takeda, Y; Zhong, J; Rajanikanth, A; Hono, K

    2010-01-01

    The magnetic and transport properties of SrLaVMoO 6 bulk samples with an ordered double perovskite structure have been investigated. Magnetization measurements have indicated that the SrLaVMoO 6 compound exhibits a cusp at 125 K, which is attributable to an antiferromagnetic transition. Electrical resistivity ρ for the compound showed metallic temperature dependence from 10 to 300 K, and a spin polarization P value was measured to be 0.50 using the point-contact Andreev reflection (PCAR) technique. It has been found from X-ray photoemission spectroscopy (XPS) study that SrLaVMoO 6 closely resembles the half-metallic Sr 2 FeMoO 6 in the electronic state of the Mo.

  1. A spin-valve-like magnetoresistance of an antiferromagnet-based tunnel junction

    Czech Academy of Sciences Publication Activity Database

    Park, B.G.; Wunderlich, Joerg; Martí, X.; Holý, V.; Kurosaki, Y.; Yamada, M.; Yamamoto, H.; Nishide, A.; Hayakawa, J.; Takahashi, H.; Shick, Alexander; Jungwirth, Tomáš

    2011-01-01

    Roč. 10, č. 5 (2011), s. 347-351 ISSN 1476-1122 R&D Projects: GA AV ČR KAN400100652; GA MŠk LC510; GA MŠk(CZ) 7E08087 EU Projects: European Commission(XE) 268066 - 0MSPIN; European Commission(XE) 214499 - NAMASTE; European Commission(XE) 215368 - SemiSpinNet Grant - others:AV ČR(CZ) AP0801 Program:Akademická prémie - Praemium Academiae Institutional research plan: CEZ:AV0Z10100521; CEZ:AV0Z10100520 Keywords : spintronics * antiferromagnets Subject RIV: BM - Solid Matter Physics ; Magnetism Impact factor: 32.841, year: 2011

  2. Theory of Topological Spin Hall Effect in Antiferromagnetic Skyrmion: Impact on Current-induced Motion

    KAUST Repository

    Akosa, Collins Ashu

    2017-09-09

    We demonstrate that the nontrivial magnetic texture of antiferromagnetic skyrmions (AFM-Sks) promotes a non-vanishing topological spin Hall effect (TSHE) on the flowing electrons. This results in a substantial enhancement of the non-adiabatic torque and hence improves the skyrmion mobility. This non-adiabatic torque increases when decreasing the skyrmion size, and therefore scaling down results in a much higher torque efficiency. In clean AFM-Sks, we find a significant boost of the TSHE close to van Hove singularity. Interestingly, this effect is enhanced away from the band gap in the presence of non-magnetic interstitial defects. Furthermore, unlike their ferromagnetic counterpart, TSHE in AFM-Sks increases with increase in disorder strength thus opening promising avenues for materials engineering of this effect.

  3. Calorimetric evidence for localized spin fluctuations in UA12

    International Nuclear Information System (INIS)

    Trainor, R.J.; Brodsky, M.B.; Isaacs, L.L.

    1974-01-01

    Results of heat capacity measurements on UAl 2 between 1.8 and 400 0 K are presented. The data are compared with recent resistivity and susceptibility measurements which indicate the existence of localized spin fluctuations in a narrow 5f band. Below about 50 0 K the electronic contribution to the heat capacity becomes large, equivalent to γ approximately 70 mJ/mole-K 2 . Below 6 0 K there is an upturn in C/T which is proportional to T 2 log (T/T/sub SF/), where T/sub SF/ = 10.6 0 K is identified as the spin fluctuation temperature. Extrapolation of this term to zero temperature yields m*/m approximately 2 for the spin-fluctuation mass enhancement. At 300 0 K, UAl 2 exhibits more typical metallic behavior, with γ approximately 15 mJ/mole-K 2 . Data are also presented for nonmagnetic URh 3 ; at low temperatures C = γT + βT 3 , with γ = 14.5 mJ/mole-K 2 and β corresponding to theta/sub D/ = 336 0 K. (U.S.)

  4. Magnetotransport property of the hole-doped delafossite CuCr0.97Mg0.03O2 with a Spin-3/2 antiferromagnetic triangular sublattice

    Science.gov (United States)

    Okuda, Tetsuji; Oozono, Satoshi; Kihara, Takumi; Tokunaga, Masashi

    2013-06-01

    The magnetotransport property of a hole-doped delafossite CuCr0.97Mg0.03O2 with a spin-3/2 antiferromagnetic (AF) triangular sublattice was investigated by using a pulsed high magnetic field. A dramatic change of magnetoresistance was observed with a variation of temperature, which indicates that a spin fluctuation due to a competition between the AF and the ferromagnetic Hund's interactions is enhanced at temperatures around the Néel temperatures ( T N). The competition may lead to a partially-disordered state at temperatures below T N which may cause a nontrivial promotion of a 120° Néel state.

  5. Quantum antiferromagnetic Heisenberg half-odd-integer spin model as the entanglement Hamiltonian of the integer-spin Affleck-Kennedy-Lieb-Tasaki states

    Science.gov (United States)

    Rao, Wen-Jia; Zhang, Guang-Ming; Yang, Kun

    2016-03-01

    Applying a symmetric bulk bipartition to the one-dimensional Affleck-Kennedy-Lieb-Tasaki valence-bond solid (VBS) states for the integer spin-S Haldane gapped phase, we can create an array of fractionalized spin-S /2 edge states with the super unit cell l in the reduced bulk system, and the topological properties encoded in the VBS wave functions can be revealed. The entanglement Hamiltonian (EH) with even l corresponds to the quantum antiferromagnetic Heisenberg spin-S /2 model. For the even integer spins, the EH still describes the Haldane gapped phase. For the odd integer spins, however, the EH just corresponds to the quantum antiferromagnetic Heisenberg half-odd integer-spin model with spinon excitations, characterizing the critical point separating the topological Haldane phase from the trivial gapped phase. Our results thus demonstrate that the topological bulk property not only determines its fractionalized edge states but also the quantum criticality associated with the topological phase, where the elementary excitations are precisely those fractionalized edge degrees of freedom confined in the bulk of the topological phase.

  6. Surface-spin magnetism of antiferromagnetic NiO in nanoparticle and bulk morphology

    International Nuclear Information System (INIS)

    Jagodic, M; Jaglicic, Z; Jelen, A; Dolinsek, J; Lee, Jin Bae; Kim, Hae Jin; Kim, Young-Min

    2009-01-01

    The surface-spin magnetism of the antiferromagnetic (AFM) material NiO in nanoparticle and bulk morphology was investigated by magnetic measurements (temperature-dependent zero-field-cooled (zfc) and field-cooled (fc) dc susceptibility, ac susceptibility and zfc and fc hysteresis loops). We addressed the question of whether the multisublattice ordering of the uncompensated surface spins and the exchange bias (EB) effect are only present in the nanoparticles, originating from their high surface-to-volume ratio or if these surface phenomena are generally present in the AFM materials regardless of their bulky or nanoparticle morphology, but the effect is just too small to be detected experimentally in the bulk due to a very small surface magnetization. Performing experiments on the NiO nanoparticles of different sizes and bulk NiO grains, we show that coercivity enhancement and hysteresis loop shift in the fc experiments, considered to be the key experimental manifestations of multisublattice ordering and the EB effect, are true nanoscale phenomena only present in the nanoparticles and absent in the bulk.

  7. Terahertz-Frequency Spin Hall Auto-oscillator Based on a Canted Antiferromagnet

    Science.gov (United States)

    Sulymenko, O. R.; Prokopenko, O. V.; Tiberkevich, V. S.; Slavin, A. N.; Ivanov, B. A.; Khymyn, R. S.

    2017-12-01

    We propose a design of a terahertz-frequency signal generator based on a layered structure consisting of a current-driven platinum (Pt) layer and a layer of an antiferromagnet (AFM) with easy-plane anisotropy, where the magnetization vectors of the AFM sublattices are canted inside the easy plane by the Dzyaloshinskii-Moriya interaction (DMI). The dc electric current flowing in the Pt layer creates due to the spin Hall effect, a perpendicular spin current that, being injected in the AFM layer, tilts the DMI-canted AFM sublattices out of the easy plane, thus exposing them to the action of a strong internal exchange magnetic field of the AFM. The sublattice magnetizations, along with the small net magnetization vector mDMI of the canted AFM, start to rotate about the hard anisotropy axis of the AFM with the terahertz frequency proportional to the injected spin current and the AFM exchange field. The rotation of the small net magnetization mDMI results in the terahertz-frequency dipolar radiation that can be directly received by an adjacent (e.g., dielectric) resonator. We demonstrate theoretically that the radiation frequencies in the range f =0.05 - 2 THz are possible at the experimentally reachable magnitudes of the driving current density, and we evaluate the power of the signal radiated into different types of resonators. This power increases with the increase of frequency f , and it can exceed 1 μ W at f ˜0.5 THz for a typical dielectric resonator of the electric permittivity ɛ ˜10 and a quality factor Q ˜750 .

  8. Quantum corrections to the spin-correlation function and the spin-stiffness constant in a two-dimensional Heisenberg antiferromagnet at zero temperature

    International Nuclear Information System (INIS)

    Igarashi, J.; Watabe, A.

    1991-01-01

    Quantum corrections to the longitudinal spin-correlation function and the spin-stiffness constant are calculated up to 1/(2S) 2 in a two-dimensional Heisenberg antiferromagnet at zero temperature by using the Holstein-Primakoff transformation. The equal-time longitudinal spin-correlation function is found to compensate almost entirely the reduction caused by the second-order correction in the transverse spin-correlation function, making the spherically averaged correlation function very close to the value given by linear spin-wave theory. In the spin-stiffness constant, a partial cancellation is found between the ''paramagnetic'' and ''diamagnetic'' terms, leading to a small second-order correction

  9. Single-pulse terahertz coherent control of spin resonance in the canted antiferromagnet YFeO3, mediated by dielectric anisotropy

    DEFF Research Database (Denmark)

    Jin, Zuanming; Mics, Zoltán; Ma, Guohong

    2013-01-01

    We report on the coherent control of terahertz (THz) spin waves in a canted antiferromagnet yttrium orthoferrite, YFeO3, associated with a quasiferromagnetic (quasi-FM) spin resonance at a frequency of 0.3 THz, using a single-incident THz pulse. The spin resonance is excited impulsively by the ma...... polarization of the THz oscillation at the spin resonance frequency, suggests a key role of magnon–phonon coupling in spin-wave energy dissipation....

  10. Superconducting fluctuations in systems with Rashba-spin-orbit coupling

    Energy Technology Data Exchange (ETDEWEB)

    Beyl, Stefan [Institut fuer Theoretische Physik und Astrophysik, Universitaet Wuerzburg (Germany); Orth, Peter P.; Scheurer, Mathias; Schmalian, Joerg [Institut fuer Theorie der Kondensierten Materie, Karlsruher Institut fuer Technologie (Germany)

    2015-07-01

    We investigate the BEC-BCS crossover in a two-dimensional system with Rashba-spin-orbit coupling. To include the effects of phase and amplitude fluctuations of the superconducting order parameter we perform a loop expansion of the effective field theory. We analyze in particular the probability of a low density superconducting quantum phase transition. The theory is relevant to LaAlO{sub 3}/SrTiO{sub 3} interfaces and two-dimensional cold atom systems with synthetic gauge fields.

  11. Antiferromagnetic versus spin-glass like behavior in MnIn{sub 2}S{sub 4}

    Energy Technology Data Exchange (ETDEWEB)

    Sagredo, V. [Laboratorio de Magnetismo, Departamento de Fisica, Facultad de Ciencias, Universidad de los Andes, Merida (Venezuela)]. E-mail: sagredo@ula.ve; Moron, M.C. [Instituto de Ciencia de Materiales de Aragon, C.S.I.C.-Universidad de Zaragoza, E-50009, Zaragoza (Spain); Betancourt, L. [Laboratorio de Magnetismo, Departamento de Fisica, Facultad de Ciencias, Universidad de los Andes, Merida (Venezuela); Delgado, G.E. [Laboratorio de Cristalografia, Departamento de Quimica, Facultad de Ciencias, Universidad de los Andes, Merida (Venezuela)

    2007-05-15

    The low-temperature magnetic properties of MnIn{sub 2}S{sub 4} have been studied using AC magnetic susceptibility and magnetization experiments. High-temperature susceptibility fits indicate the presence of antiferromagnetic interactions. Low-field magnetization data show a peak at 5.6{+-}0.1 K, below which strong irreversibility is observed between zero-field-cooled (ZFC) and field-cooled (FC) cycles suggesting that the observed peak corresponds to a spin-glass-like transition instead of the antiferromagnetic one previously reported. Further evidence of this magnetic state comes from AC susceptibility data at different frequencies. The in-phase component {chi}'(T) exhibits the behavior expected of spin glasses, i.e. a shift of the cusp to higher temperatures for higher frequencies.

  12. Quantum-Classical Phase Transition of the Escape Rate of Two-Sublattice Antiferromagnetic Large Spins

    Science.gov (United States)

    Owerre, Solomon Akaraka; Paranjape, M. B.

    2014-11-01

    The Hamiltonian of a two-sublattice antiferromagnetic spins, with single (hard-axis) and double ion anisotropies described by H = J {\\hat S}1...\\hatS 2-2Jz \\hat {S}1z\\hat {S}2z+K(\\hat {S}1z2 +\\hat {S}2z2) is investigated using the method of effective potential. The problem is mapped to a single particle quantum-mechanical Hamiltonian in terms of the relative coordinate and reduced mass. We study the quantum-classical phase transition of the escape rate of this model. We show that the first-order phase transition for this model sets in at the critical value Jc = (Kc+Jz, c)/2 while for the anisotropic Heisenberg coupling H = J(S1xS2x +S1yS2y) + JzS1zS2z + K(S1z2+ S2z2) we obtain Jc = (2Kc-Jz, c)/3. The phase diagrams of the transition are also studied.

  13. Spin glass behavior of the antiferromagnetic Heisenberg model on scale free network

    International Nuclear Information System (INIS)

    Surungan, Tasrief; Zen, Freddy P; Williams, Anthony G

    2015-01-01

    Randomness and frustration are considered to be the key ingredients for the existence of spin glass (SG) phase. In a canonical system, these ingredients are realized by the random mixture of ferromagnetic (FM) and antiferromagnetic (AF) couplings. The study by Bartolozzi et al. [Phys. Rev. B73, 224419 (2006)] who observed the presence of SG phase on the AF Ising model on scale free network (SFN) is stimulating. It is a new type of SG system where randomness and frustration are not caused by the presence of FM and AF couplings. To further elaborate this type of system, here we study Heisenberg model on AF SFN and search for the SG phase. The canonical SG Heisenberg model is not observed in d-dimensional regular lattices for (d ≤ 3). We can make an analogy for the connectivity density (m) of SFN with the dimensionality of the regular lattice. It should be plausible to find the critical value of m for the existence of SG behaviour, analogous to the lower critical dimension (d l ) for the canonical SG systems. Here we study system with m = 2, 3, 4 and 5. We used Replica Exchange algorithm of Monte Carlo Method and calculated the SG order parameter. We observed SG phase for each value of m and estimated its corersponding critical temperature. (paper)

  14. Antiferromagnetic ordering in spin-chain multiferroic Gd{sub 2}BaNiO{sub 5} studied by electronic spin resonance

    Energy Technology Data Exchange (ETDEWEB)

    Guo, Y. M.; Ruan, M. Y.; Cheng, J. J.; Sun, Y. C. [Wuhan National High Magnetic Field Center, Huazhong University of Science and Technology, Wuhan 430074 (China); School of Physics, Huazhong University of Science and Technology, Wuhan 430074 (China); Ouyang, Z. W., E-mail: zwouyang@mail.hust.edu.cn; Xia, Z. C. [Wuhan National High Magnetic Field Center, Huazhong University of Science and Technology, Wuhan 430074 (China); Rao, G. H. [School of Materials Science and Engineering, Guilin University of Electronic Technology, Guilin 541004 (China)

    2015-06-14

    High-field electron spin resonance (ESR) has been employed to study the antiferromagnetic (AFM) ordering state (T < T{sub N} = 55 K) of spin-chain multiferroic Gd{sub 2}BaNiO{sub 5}. The spin reorientation at T{sub SR} = 24 K is well characterized by the temperature-dependent ESR spectra. The magnetization data evidence a field-induced spin-flop transition at 2 K. The frequency-field relationship of the ESR data can be explained by conventional AFM resonance theory with uniaxial anisotropy, in good agreement with magnetization data. Related discussion on zero-field spin gap is presented.

  15. Dynamic magnetic behavior of the mixed spin (2, 5/2) Ising system with antiferromagnetic/antiferromagnetic interactions on a bilayer square lattice

    International Nuclear Information System (INIS)

    Ertaş Mehmet; Keskin Mustafa

    2013-01-01

    Using the mean-field theory and Glauber-type stochastic dynamics, we study the dynamic magnetic properties of the mixed spin (2, 5/2) Ising system for the antiferromagnetic/antiferromagnetic (AFM/AFM) interactions on the bilayer square lattice under a time varying (sinusoidal) magnetic field. The time dependence of average magnetizations and the thermal variation of the dynamic magnetizations are examined to calculate the dynamic phase diagrams. The dynamic phase diagrams are presented in the reduced temperature and magnetic field amplitude plane and the effects of interlayer coupling interaction on the critical behavior of the system are investigated. We also investigate the influence of the frequency and find that the system displays richer dynamic critical behavior for higher values of frequency than that of the lower values of it. We perform a comparison with the ferromagnetic/ferromagnetic (FM/FM) and AFM/FM interactions in order to see the effects of AFM/AFM interaction and observe that the system displays richer and more interesting dynamic critical behaviors for the AFM/AFM interaction than those for the FM/FM and AFM/FM interactions. (general)

  16. Magnetization plateaus in the spin-1/2 antiferromagnetic Heisenberg model on a kagome-strip chain

    Science.gov (United States)

    Morita, Katsuhiro; Sugimoto, Takanori; Sota, Shigetoshi; Tohyama, Takami

    2018-01-01

    The spin-1/2 Heisenberg model on a kagome lattice is a typical frustrated quantum spin system. The basic structure of a kagome lattice is also present in the kagome-strip lattice in one dimension, where a similar type of frustration is expected. We thus study the magnetization plateaus of the spin-1/2 Heisenberg model on a kagome-strip chain with three-independent antiferromagnetic exchange interactions using the density-matrix renormalization-group method. In a certain range of exchange parameters, we find twelve kinds of magnetization plateaus, nine of which have magnetic structures breaking translational and/or reflection symmetry spontaneously. The structures are classified by an array of five-site unit cells with specific bond-spin correlations. In a case with a nontrivial plateau, namely a 3/10 plateau, we find long-period magnetic structure with a period of four unit cells.

  17. Microscopic theory of the nearest-neighbor valence bond sector of the spin-1/2 kagome antiferromagnet

    Science.gov (United States)

    Ralko, Arnaud; Mila, Frédéric; Rousochatzakis, Ioannis

    2018-03-01

    The spin-1/2 Heisenberg model on the kagome lattice, which is closely realized in layered Mott insulators such as ZnCu3(OH) 6Cl2 , is one of the oldest and most enigmatic spin-1/2 lattice models. While the numerical evidence has accumulated in favor of a quantum spin liquid, the debate is still open as to whether it is a Z2 spin liquid with very short-range correlations (some kind of resonating valence bond spin liquid), or an algebraic spin liquid with power-law correlations. To address this issue, we have pushed the program started by Rokhsar and Kivelson in their derivation of the effective quantum dimer model description of Heisenberg models to unprecedented accuracy for the spin-1/2 kagome, by including all the most important virtual singlet contributions on top of the orthogonalization of the nearest-neighbor valence bond singlet basis. Quite remarkably, the resulting picture is a competition between a Z2 spin liquid and a diamond valence bond crystal with a 12-site unit cell, as in the density-matrix renormalization group simulations of Yan et al. Furthermore, we found that, on cylinders of finite diameter d , there is a transition between the Z2 spin liquid at small d and the diamond valence bond crystal at large d , the prediction of the present microscopic description for the two-dimensional lattice. These results show that, if the ground state of the spin-1/2 kagome antiferromagnet can be described by nearest-neighbor singlet dimers, it is a diamond valence bond crystal, and, a contrario, that, if the system is a quantum spin liquid, it has to involve long-range singlets, consistent with the algebraic spin liquid scenario.

  18. Anisotropic phase diagram and spin fluctuations of the hyperkagome magnet Gd3Ga5O12 as revealed by sound velocity measurements

    Science.gov (United States)

    Rousseau, Alexandre; Parent, Jean-Michel; Quilliam, Jeffrey A.

    2017-08-01

    Sound velocity and attenuation measurements on the frustrated garnet material Gd3Ga5O12 (GGG) are presented as a function of field and temperature, with two different magnetic field orientations: [100 ] and [110 ] . We demonstrate that the phase diagram is highly anisotropic, with two distinct field-induced ordered phases for H ||[110 ] and only one for H ||[100 ] . Extensive lattice softening is found to occur at low fields, which can be associated with spin fluctuations. However, deep within the spin liquid phase a low-temperature stiffening of the lattice and reduced attenuation provide evidence for a spin gap which may be related to short-range antiferromagnetic correlations over minimal ten-spin loops.

  19. Antiferromagnetic skyrmions

    Science.gov (United States)

    Tretiakov, Oleg; Barker, Joseph

    Skyrmions are topologically protected entities in magnetic materials which have the potential to be used in spintronics for information storage and processing. However, skyrmions in ferromagnets have some intrinsic difficulties which must be overcome to use them for spintronic applications, such as the inability to move straight along current. We show that skyrmions can also be stabilized and manipulated in antiferromagnetic materials. An antiferromagnetic skyrmion is a compound topological object with a similar but of opposite sign spin texture on each sublattice, which e.g. results in a complete cancelation of the Magnus force. We find that the composite nature of antiferromagnetic skyrmions gives rise to different dynamical behavior, both due to an applied current and temperature effects. O.A.T. and J.B. acknowledge support by the Grants-in-Aid for Scientific Research (Nos. 25800184, 25247056, 25220910 and 15H01009) from the Ministry of Education, Culture, Sports, Science and Technology (MEXT) of Japan and SpinNet.

  20. Spin-flip transition and Faraday effect in antiferromagnet KMnF3 in megagauss magnetic field

    International Nuclear Information System (INIS)

    Mukhin, A.A.; Plis, V.I.; Popov, A.I.; Zvezdin, A.K.; Platonov, V.; Tatsenko, O.M.

    1998-01-01

    Faraday effect in the antiferromagnet KMnF 3 has been investigated in pulse explosive fields up to 500 T at T=78 K. The laser wavelength 0.63 μm was used in the experiment. The magnetic field dependence of Faraday rotation in this antiferromagnet shows a unique feature of a lack of saturation effect in the fields up to 500 T whereas critical field of spin-flip transition is about 120 T. The theoretical analysis of microscopic nature of Faraday rotation, including the diamagnetic, magneto-dipole and paramagnetic mechanisms has been performed. The strong competition of these mechanisms is important to explain the extremely small value of the effect and its unusual magnetic field dependence

  1. Effective S =2 antiferromagnetic spin chain in the salt (o -MePy-V)FeCl4

    Science.gov (United States)

    Iwasaki, Y.; Kida, T.; Hagiwara, M.; Kawakami, T.; Hosokoshi, Y.; Tamekuni, Y.; Yamaguchi, H.

    2018-02-01

    We present a model compound for the S =2 antiferromagnetic (AF) spin chain composed of the salt (o -MePy-V ) FeCl4 . Ab initio molecular-orbital calculations indicate the formation of a partially stacked two-dimensional (2D) spin model comprising five types of exchange interactions between S =1 /2 and S =5 /2 spins, which locate on verdazyl radical and Fe ion, respectively. The magnetic properties of the synthesized crystals indicate that the dominant interaction between the S =1 /2 and S =5 /2 spins stabilizes an S =2 spin in the low-temperature region, and an effective S =2 AF chain is formed for T ≪10 K and H chain. At higher fields above quantitatively 4 T, the magnetization curve assumes two-thirds of the full saturation value for fields between 4 and 20 T, and approaches saturation at ˜40 T. The spin model in the high-field region can be considered as a quasi-2D S =1 /2 honeycomb lattice under an effective internal field caused by the fully polarized S =5 /2 spin.

  2. Direct Observation of Localized Spin Antiferromagnetic Transition in PdCrO2 by Angle-Resolved Photoemission Spectroscopy

    Science.gov (United States)

    Noh, Han-Jin; Jeong, Jinwon; Chang, Bin; Jeong, Dahee; Moon, Hyun Sook; Cho, En-Jin; Ok, Jong Mok; Kim, Jun Sung; Kim, Kyoo; Min, B. I.; Lee, Han-Koo; Kim, Jae-Young; Park, Byeong-Gyu; Kim, Hyeong-Do; Lee, Seongsu

    2014-01-01

    We report the first case of the successful measurements of a localized spin antiferromagnetic transition in delafossite-type PdCrO2 by angle-resolved photoemission spectroscopy (ARPES). This demonstrates how to circumvent the shortcomings of ARPES for investigation of magnetism involved with localized spins in limited size of two-dimensional crystals or multi-layer thin films that neutron scattering can hardly study due to lack of bulk compared to surface. Also, our observations give direct evidence for the spin ordering pattern of Cr3+ ions in PdCrO2 suggested by neutron diffraction and quantum oscillation measurements, and provide a strong constraint that has to be satisfied by a microscopic mechanism for the unconventional anomalous Hall effect recently reported in this system. PMID:24419488

  3. Spin liquid in a single crystal of the frustrated diamond lattice antiferromagnet CoAl2O4

    DEFF Research Database (Denmark)

    Zaharko, O.; Christensen, Niels Bech; Cervellino, A.

    2011-01-01

    We study the evidence for spin liquid in the frustrated diamond lattice antiferromagnet CoAl2O4 by means of single-crystal neutron scattering in zero and applied magnetic fields. The magnetically ordered phase appearing below T-N = 8 K remains nonconventional down to 1.5 K. The magnetic Bragg peaks...... at the q = 0 positions are broad and their line shapes have strong Lorentzian contributions. Additionally, the peaks are connected by weak diffuse streaks oriented along the directions. The observed short-range magnetic correlations are explained within the spiral spin-liquid model. The specific...... shape of the energy landscape of the system, with an extremely flat energy minimum around q = 0 and many low-lying excited spiral states with q = , results in thermal population of this manifold at finite temperatures. The agreement between the experimental results and the spiral spin-liquid model...

  4. Unusual magnetic excitations in the weakly ordered spin- 12 chain antiferromagnet Sr2CuO3: Possible evidence for Goldstone magnon coupled with the amplitude mode

    International Nuclear Information System (INIS)

    Sergeicheva, E. G.; Sosin, S. S.; Prozorova, L. A.; Gu, G. D.; Zaliznyak, I. A.

    2017-01-01

    We report on an electron spin resonance (ESR) study of a nearly one-dimensional (1D) spin-1/2 chain antiferromagnet, Sr 2 CuO 3 , with extremely weak magnetic ordering. The ESR spectra at T > T N , in the disordered Luttinger-spin-liquid phase, reveal nearly ideal Heisenberg-chain behavior with only a very small, field-independent linewidth, ~1/T. In the ordered state, below T N , we identify field-dependent antiferromagnetic resonance modes, which are well described by pseudo-Goldstone magnons in the model of a collinear biaxial antiferromagnet. Additionally, we observe a major resonant mode with unusual and strongly anisotropic properties, which is not anticipated by the conventional theory of Goldstone spin waves. Lastly, we propose that this unexpected magnetic excitation can be attributed to a field-independent magnon mode renormalized due to its interaction with the high-energy amplitude (Higgs) mode in the regime of weak spontaneous symmetry breaking.

  5. Topological antiferromagnetic spintronics

    Science.gov (United States)

    Šmejkal, Libor; Mokrousov, Yuriy; Yan, Binghai; MacDonald, Allan H.

    2018-03-01

    The recent demonstrations of electrical manipulation and detection of antiferromagnetic spins have opened up a new chapter in the story of spintronics. Here, we review the emerging research field that is exploring the links between antiferromagnetic spintronics and topological structures in real and momentum space. Active topics include proposals to realize Majorana fermions in antiferromagnetic topological superconductors, to control topological protection and Dirac points by manipulating antiferromagnetic order parameters, and to exploit the anomalous and topological Hall effects of zero-net-moment antiferromagnets. We explain the basic concepts behind these proposals, and discuss potential applications of topological antiferromagnetic spintronics.

  6. Photoinduced Coherent Spin Fluctuation in Primary Dynamics of Insulator to Metal Transition in Perovskite Cobalt Oxide

    Directory of Open Access Journals (Sweden)

    Arima T.

    2013-03-01

    Full Text Available Coherent spin fluctuation was detected in the photoinduced Mott insulator-metal transition in perovskite cobalt oxide by using 3 optical-cycle infrared pulse. Such coherent spin fluctuation is driven by the perovskite distortion changing orbital gap.

  7. Perspectives of antiferromagnetic spintronics

    Science.gov (United States)

    Jungfleisch, Matthias B.; Zhang, Wei; Hoffmann, Axel

    2018-04-01

    Antiferromagnets are promising for future spintronic applications owing to their advantageous properties: They are magnetically ordered, but neighboring magnetic moments point in opposite directions, which results in zero net magnetization. This means antiferromagnets produce no stray fields and are insensitive to external magnetic field perturbations. Furthermore, they show intrinsic high frequency dynamics, exhibit considerable spin-orbit and magneto-transport effects. Over the past decade, it has been realized that antiferromagnets have more to offer than just being utilized as passive components in exchange bias applications. This development resulted in a paradigm shift, which opens the pathway to novel concepts using antiferromagnets for spin-based technologies and applications. This article gives a broad perspective on antiferromagnetic spintronics. In particular, the manipulation and detection of antiferromagnetic states by spintronics effects, as well as spin transport and dynamics in antiferromagnetic materials will be discussed. We will also outline current challenges and future research directions in this emerging field.

  8. Effect of spin fluctuations in magnetocaloric and magnetoresistance properties of Dy10Co20Si70 alloy

    Science.gov (United States)

    Rashid, T. P.; Arun, K.; Curlik, Ivan; Ilkovic, Sergej; Reiffers, Marian; Dzubinska, Andrea; Nagalakshmi, R.

    2017-09-01

    Systematic investigations on the structure, magnetic, thermodynamic, magnetocaloric and magnetoresistance (MR) properties of the arc melted Dy10Co20Si70 alloy are presented. The Dy10Co20Si70 alloy crystallizes in tetragonal BaNiSn3-type DyCoSi3 (space group = I4mm; No. 107) as a major phase and CaF2-type CoSi2 (space group = Fm-3m; No. 225) and C-type Si (space group = Fd-3m; No. 227) as minor phases. The title compound exhibits multiple magnetic transitions having antiferromagnetic ordering at temperatures, viz., T1 = 10.8 K, T2 = 8.8 K and T3 = 3.3 K. The magnetic and thermodynamic studies confirm these magnetic anomalies in the compound. The large value of maximum magnetic entropy change, -ΔSMM a x = 16.4 and 26.6 J/kg K for the field change ΔH of 50 and 90 kOe, respectively, observed in the compound is associated with field induced magnetic transitions. Asymmetric broadening of the magnetic entropy change peaks above the ordering temperatures resulting in significant refrigerant capacities of 361 and 868 J/kg for ΔH = 50 and 90 kOe, respectively, in the compound is due to the spin fluctuation effect. The sign reversal in MR measurements is attributed to the field induced antiferromagnetic to ferromagnetic transition. A large positive MR (42% in 90 kOe) is observed at 2 K. The H2 dependence of both the magnetocaloric effect (MCE) and MR in the paramagnetic regime indicates the role of the applied magnetic field in suppressing the spin fluctuations. The large MCE and MR together with no thermal or magnetic hysteresis establish this new compound as an attractive multifunctional magnetic material.

  9. Collective modes and spin fluctuations for spin-triplet superconducting state in Sr2RuO4

    International Nuclear Information System (INIS)

    Tewordt, L.

    1999-01-01

    First the authors calculate the collective order parameter modes for the most promising candidates of spin-triplet p-wave pairing states in the layered perovskite structure of Sr 2 RuO 4 . The pairing interaction and accordingly the equations for the order parameter fluctuations are decomposed in terms of spin-triplet pairing states corresponding to the irreducible representations of the point group D 4h . Asymmetric pairing interaction and spin-orbit coupling give rise to finite frequencies of the original Goldstone modes corresponding to broken rotational symmetry. These fluctuations of the rvec d-vector within the basal plane can be excited by external fields lying in the plane and coupling to spin density. The fluctuations of the amplitude of the rvec d-vector perpendicular to the basal plane have frequency ω = 2Δ 0 for the state without nodes and ω = √3 Δ 0 for the state with nodes (Δ 0 is the amplitude of the gap). These modes couple to charge density by electron-hole asymmetry at the Fermi surface. In the second part the author develops the self-consistent FLEX (fluctuation exchange) approximation for spin-triplet pairing mediated by exchange of spin fluctuations. At T c the pairing interaction is only one third of that for singlet-pairing. Below T c the feed-back effect stabilizes the spin-triplet state with rvec d-vector perpendicular to the basal plane

  10. Low temperature magnetic properties and spin dynamics in single crystals of Cr{sub 8}Zn antiferromagnetic molecular rings

    Energy Technology Data Exchange (ETDEWEB)

    Adelnia, Fatemeh [Dipartimento di Fisica, Università degli Studi di Milano and INSTM, I-20133 Milano (Italy); Dipartimento di Fisica, Università degli Studi di Pavia and INSTM, I-27100 Pavia (Italy); Chiesa, Alessandro; Bordignon, Sara; Carretta, Stefano [Dipartimento di Fisica e Scienze della Terra, Università degli Studi di Parma, I-43124 Parma (Italy); Ghirri, Alberto; Candini, Andrea [CNR Institute Nanosciences S3, I- 41125 Modena (Italy); Cervetti, Christian [Dipartimento di Scienze Fisiche, Informatiche, Matematiche, Università di Modena e Reggio Emilia, I-41125 Modena (Italy); Evangelisti, Marco [CNR Institute Nanosciences S3, I- 41125 Modena (Italy); Dipartimento di Scienze Fisiche, Informatiche, Matematiche, Università di Modena e Reggio Emilia, I-41125 Modena (Italy); Instituto de Ciencia de Materiales de Aragón and Departamento de Física de la Materia Condensada, CSIC-Universidad de Zaragoza, 50009 Zaragoza (Spain); Affronte, Marco [CNR Institute Nanosciences S3, I- 41125 Modena (Italy); Dipartimento di Scienze Fisiche, Informatiche, Matematiche, Università di Modena e Reggio Emilia, I-41125 Modena (Italy); Sheikin, Ilya [Grenoble High Magnetic Field Laboratory, CNRS-LNCMI, 25, B.P. 166, 38042 Grenoble Cedex 9 (France); Winpenny, Richard; Timco, Grigore [The Lewis Magnetism Laboratory, The University of Manchester, M13 9PL Manchester (United Kingdom); Borsa, Ferdinando [Dipartimento di Fisica, Università degli Studi di Pavia and INSTM, I-27100 Pavia (Italy); and others

    2015-12-28

    A detailed experimental investigation of the effects giving rise to the magnetic energy level structure in the vicinity of the level crossing (LC) at low temperature is reported for the open antiferromagnetic molecular ring Cr{sub 8}Zn. The study is conducted by means of thermodynamic techniques (torque magnetometry, magnetization and specific heat measurements) and microscopic techniques (nuclear magnetic resonance line width, nuclear spin lattice, and spin-spin relaxation measurements). The experimental results are shown to be in excellent agreement with theoretical calculations based on a minimal spin model Hamiltonian, which includes a Dzyaloshinskii-Moriya interaction. The first ground state level crossing at μ{sub 0}H{sub c1} = 2.15 T is found to be an almost true LC while the second LC at μ{sub 0}H{sub c2} = 6.95 T has an anti-crossing gap of Δ{sub 12} = 0.19 K. In addition, both NMR and specific heat measurements show the presence of a level anti-crossing between excited states at μ{sub 0}H = 4.5 T as predicted by the theory. In all cases, the fit of the experimental data is improved by introducing a distribution of the isotropic exchange couplings (J), i.e., using a J strain model. The peaks at the first and second LCs in the nuclear spin-lattice relaxation rate are dominated by inelastic scattering and a value of Γ ∼ 10{sup 10} rad/s is inferred for the life time broadening of the excited state of the open ring, due to spin phonon interaction. A loss of NMR signal (wipe-out effect) is observed for the first time at LC and is explained by the enhancement of the spin-spin relaxation rate due to the inelastic scattering.

  11. Single reference Coupled Cluster treatment of nearly degenerate problems: Cohesive energy of antiferromagnetic lattices of spin 1 centers

    International Nuclear Information System (INIS)

    Malrieu, Jean-Paul

    2012-01-01

    Lattices of antiferromagnetically coupled spins, ruled by Heisenberg Hamiltonians, are intrinsically highly degenerate systems. The present work tries to estimate the ground state energy of regular bipartite spin lattices of S = 1 sites from a single reference Coupled Cluster expansion starting from a Néel function, taken as reference. The simultaneous changes of spin momentum on adjacent sites play the role of the double excitations in molecular electronic problems. Propagation of the spin changes plays the same role as the triple excitations. The treatment takes care of the deviation of multiple excitation energies from additivity. Specific difficulties appear for 1D chains, which are not due to a near degeneracy between the reference and the vectors which directly interact with it but to the complexity of the processes which lead to the low energy configurations where a consistent reversed-Néel domain is created inside the Néel starting spin wave. Despite these difficulties a reasonable value of the cohesive energy is obtained.

  12. Single reference Coupled Cluster treatment of nearly degenerate problems: Cohesive energy of antiferromagnetic lattices of spin 1 centers

    Science.gov (United States)

    Malrieu, Jean-Paul

    2012-06-01

    Lattices of antiferromagnetically coupled spins, ruled by Heisenberg Hamiltonians, are intrinsically highly degenerate systems. The present work tries to estimate the ground state energy of regular bipartite spin lattices of S = 1 sites from a single reference Coupled Cluster expansion starting from a Néel function, taken as reference. The simultaneous changes of spin momentum on adjacent sites play the role of the double excitations in molecular electronic problems. Propagation of the spin changes plays the same role as the triple excitations. The treatment takes care of the deviation of multiple excitation energies from additivity. Specific difficulties appear for 1D chains, which are not due to a near degeneracy between the reference and the vectors which directly interact with it but to the complexity of the processes which lead to the low energy configurations where a consistent reversed-Néel domain is created inside the Néel starting spin wave. Despite these difficulties a reasonable value of the cohesive energy is obtained.

  13. Fractional Spin Fluctuations as a Precursor of Quantum Spin Liquids: Majorana Dynamical Mean-Field Study for the Kitaev Model.

    Science.gov (United States)

    Yoshitake, Junki; Nasu, Joji; Motome, Yukitoshi

    2016-10-07

    Experimental identification of quantum spin liquids remains a challenge, as the pristine nature is to be seen in asymptotically low temperatures. We here theoretically show that the precursor of quantum spin liquids appears in the spin dynamics in the paramagnetic state over a wide temperature range. Using the cluster dynamical mean-field theory and the continuous-time quantum Monte Carlo method, which are newly developed in the Majorana fermion representation, we calculate the dynamical spin structure factor, relaxation rate in nuclear magnetic resonance, and magnetic susceptibility for the honeycomb Kitaev model whose ground state is a canonical example of the quantum spin liquid. We find that dynamical spin correlations show peculiar temperature and frequency dependence even below the temperature where static correlations saturate. The results provide the experimentally accessible symptoms of the fluctuating fractionalized spins evincing the quantum spin liquids.

  14. Investigation of the spin-1 honeycomb antiferromagnet BaNi2V2O8 with easy-plane anisotropy

    Science.gov (United States)

    Klyushina, E. S.; Lake, B.; Islam, A. T. M. N.; Park, J. T.; Schneidewind, A.; Guidi, T.; Goremychkin, E. A.; Klemke, B.; Mânsson, M.

    2017-12-01

    The magnetic properties of the two-dimensional, S =1 honeycomb antiferromagnet BaNi2V2O8 have been comprehensively studied using dc susceptibility measurements and inelastic neutron scattering techniques. The magnetic excitation spectrum is found to be dispersionless within experimental resolution between the honeycomb layers, while it disperses strongly within the honeycomb plane where it consists of two gapped spin-wave modes. The magnetic excitations are compared to linear spin-wave theory allowing the Hamiltonian to be determined. The first- and second-neighbor magnetic exchange interactions are antiferromagnetic and lie within the ranges 10.90 meV ≤Jn≤13.35 meV and 0.85 meV ≤Jn n≤1.65 meV, respectively. The interplane coupling Jout is four orders of magnitude weaker than the intraplane interactions, confirming the highly two-dimensional magnetic behavior of this compound. The sizes of the energy gaps are used to extract the magnetic anisotropies and reveal substantial easy-plane anisotropy and a very weak in-plane easy-axis anisotropy. Together these results reveal that BaNi2V2O8 is a candidate compound for the investigation of vortex excitations and Berezinsky-Kosterliz-Thouless phenomenon.

  15. Perspectives of Antiferromagnetic Spintronics

    Energy Technology Data Exchange (ETDEWEB)

    Jungfleisch, Matthias B.; Zhang, Wei; Hoffmann, Axel

    2018-04-05

    Antiferromagnets are promising for future spintronics applications owing to their interesting properties: They are magnetically ordered, but neighboring magnetic moments point in opposite directions which results in zero net magneti- zation. This means antiferromagnets produce no stray fields and are insensitive to external magnetic field perturbations. Furthermore, they show intrinsic high frequency dynamics, exhibit considerable spin-orbit and magneto-transport effects. Over the past decade, it has been realized that antiferromagnets have more to offer than just being utilized as passive components in exchange bias applications. This development resulted in a paradigm shift, which opens the pathway to novel concepts using antiferromagnets for spin-based technologies and applications. This article gives a broad per- spective on antiferromagnetic spintronics. In particular, the manipulation and detection of anitferromagnetic states by spintronics effects, as well as spin transport and dynamics in antiferromagnetic materials will be discussed. We will also outline current challenges and future research directions in this emerging field.

  16. Density of states and phase diagram of the antiferromagnetic spin chain with Dzyaloshinsky-Moriya interaction and spin-phonon coupling

    International Nuclear Information System (INIS)

    Wang Qin; Chen Hong; Zheng Hang

    2007-01-01

    The effects of DM interaction on the density-of-states, the dimerization and the phase diagram in the antiferromagnetic Heisenberg chain coupled with quantum phonons have been studied by a nonadiabatic analytical approach. The results show that the effect of the DM interaction is to increase the staggered antisymmetric spin exchange interaction order but to decrease the spin dimerization and their competitions result in the lattice dimerization ordering parameter to increase for large staggered DM interaction parameter β and decrease for small β. A crossover of β exists in which the dimerization ordering parameter changes non-monotonously. As the DM interaction parameter D increases, depending on the appropriate values of spin-phonon coupling, phonon frequency and β, the system undergoes phase transition from spin gapless state to gapped state or reversely and can even reenter between the two states. The relation between the phonon-staggered ordering parameter, the spin-dimer order parameter and the staggered DM interaction order parameter gives clearly their contributing weights to the lattice dimerization

  17. Gapped paramagnetic state in a frustrated spin-1/2 Heisenberg antiferromagnet on the cross-striped square lattice

    Science.gov (United States)

    Li, P. H. Y.; Bishop, R. F.

    2018-03-01

    We implement the coupled cluster method to very high orders of approximation to study the spin-1/2 J1 -J2 Heisenberg model on a cross-striped square lattice. Every nearest-neighbour pair of sites on the square lattice has an isotropic antiferromagnetic exchange bond of strength J1 > 0 , while the basic square plaquettes in alternate columns have either both or neither next-nearest-neighbour (diagonal) pairs of sites connected by an equivalent frustrating bond of strength J2 ≡ αJ1 > 0 . By studying the magnetic order parameter (i.e., the average local on-site magnetization) in the range 0 ≤ α ≤ 1 of the frustration parameter we find that the quasiclassical antiferromagnetic Néel and (so-called) double Néel states form the stable ground-state phases in the respective regions α α1bc = 0.615(5) . The double Néel state has Néel (⋯ ↑↓↑↓ ⋯) ordering along the (column) direction parallel to the stripes of squares with both or no J2 bonds, and spins alternating in a pairwise (⋯ ↑↑↓↓↑↑↓↓ ⋯) fashion along the perpendicular (row) direction, so that the parallel pairs occur on squares with both J2 bonds present. Further explicit calculations of both the triplet spin gap and the zero-field uniform transverse magnetic susceptibility provide compelling evidence that the ground-state phase over all or most of the intermediate regime α1ac state with no discernible long-range magnetic order.

  18. The anisotropic quantum spin-1/2 Heisenberg antiferromagnet in the presence of a longitudinal field on a bcc lattice

    Energy Technology Data Exchange (ETDEWEB)

    Neto, Minos A., E-mail: minos@pq.cnpq.br [Departamento de Fisica, Universidade Federal do Amazonas, 3000, Japiim, Manaus, 69077-000 AM (Brazil); Roberto Viana, J., E-mail: vianafisica@bol.com.br [Departamento de Fisica, Universidade Federal do Amazonas, 3000, Japiim, Manaus, 69077-000 AM (Brazil); Ricardo de Sousa, J., E-mail: jsousa@edu.ufam.br [Departamento de Fisica, Universidade Federal do Amazonas, 3000, Japiim, Manaus, 69077-000 AM (Brazil); National Institute of Science and Technology for Complex Systems, 3000, Japiim, Manaus, 69077-000 AM (Brazil)

    2012-08-15

    In this work we study the critical behavior of the quantum spin-1/2 anisotropic Heisenberg antiferromagnet in the presence of a longitudinal field on a body centered cubic (bcc) lattice as a function of temperature, anisotropy parameter ({Delta}) and magnetic field (H), where {Delta}=0 and 1 correspond the isotropic Heisenberg and Ising models, respectively. We use the framework of the differential operator technique in the effective-field theory with finite cluster of N=4 spins (EFT-4). The staggered m{sub s}=(m{sub A}-m{sub B})/2 and total m=(m{sub A}+m{sub B})/2 magnetizations are numerically calculated, where in the limit of m{sub s}{yields}0 the critical line T{sub N}(H,{Delta}) is obtained. The phase diagram in the T-H plane is discussed as a function of the parameter {Delta} for all values of H Element-Of [0,H{sub c}({Delta})], where H{sub c}({Delta}) correspond the critical field (T{sub N}=0). Special focus is given in the low temperature region, where a reentrant behavior is observed around of H=H{sub c}({Delta}){>=}H{sub c}({Delta}=1)=8J in the Ising limit, results in accordance with Monte Carlo simulation, and also was observed for all values of {Delta} Element-Of [0,1]. This reentrant behavior increases with increase of the anisotropy parameter {Delta}. In the limit of low field, our results for the Heisenberg limit are compared with series expansion values. - Highlights: Black-Right-Pointing-Pointer In the lat decade there has been a great interest in the physics of the quantum phase transition in spins system. Black-Right-Pointing-Pointer Effective-field theory in cluster with N=4 spins is generalized to treat the quantum spin-1/2 Heisenberg model. Black-Right-Pointing-Pointer We have obtained phase diagram at finite temperature for the quantum spin-1/2 antiferromagnet Heisenberg model as a bcc lattice.

  19. Weakly spin-dependent band structures of antiferromagnetic perovskite LaMO3(M  =  Cr, Mn, Fe).

    Science.gov (United States)

    Okugawa, Takuya; Ohno, Kaoru; Noda, Yusuke; Nakamura, Shinichiro

    2018-02-21

    We investigate the spin-dependent electronic states of antiferromagnetic (AFM) lanthanum chromite (LaCrO 3 ), lanthanum manganite (LaMnO 3 ), and lanthanum ferrite (LaFeO 3 ) using spin-polarized first-principles density functional theory with Hubbard U correction. The band structures are calculated for 15 types of their different AFM structures. It is verified for these structures that there is a very simple rule to identify which wave number [Formula: see text] exhibits spin splitting or degeneracy in the band structure. This rule uses the symmetry operations that map the up-spin atoms onto the down-spin atoms. The resulting spin splitting is very small for the most stable spin configuration of the most stable experimental structure. We discuss a plausible benefit of this characteristic, i.e. the direction-independence of the spin current, in electrode applications.

  20. Exchange and spin-fluctuation superconducting pairing in the strong correlation limit of the Hubbard model

    International Nuclear Information System (INIS)

    Plakida, N. M.; Anton, L.; Adam, S. . Department of Theoretical Physics, Horia Hulubei National Institute for Physics and Nuclear Engineering, PO Box MG-6, RO-76900 Bucharest - Magurele; RO); Adam, Gh. . Department of Theoretical Physics, Horia Hulubei National Institute for Physics and Nuclear Engineering, PO Box MG-6, RO-76900 Bucharest - Magurele; RO)

    2001-01-01

    contrast, the exchange interaction is maximal along the above mentioned lines inside BZ and it couples the electrons (holes) in a much broader energy shell, of the order of the bandwidth W= 8 t eff due to the interband hopping where the retardation effects are unimportant. Samplings of the wave-vector behavior of the order parameters Φ 22 (k) over the first quadrant of the BZ at several temperatures show the occurrence of a peculiar d x 2 -y 2 -wave gap pattern which strongly depends on the type of the involved interactions. In conclusion, the present investigation points to the existence of a singlet d x 2 -y 2 -wave superconducting pairing for holes or electrons in the two-band Hubbard model mediated by the exchange interaction and antiferromagnetic spin-fluctuation scattering induced by the kinematic interaction, characteristic to the Hubbard model. These mechanisms of superconducting pairing are absent in the fermionic models. Our results agree with the recent investigations of the Hubbard model within the dynamical cluster approximation, where the self-energy has been calculated in the non-crossing approximation for the 4-cluster model. (authors)

  1. Valence and Spin fluctuations in Mn-doped ferroelectric BaTiO3

    OpenAIRE

    Mandal, Subhasish; Cohen, R. E.; Haule, K.

    2018-01-01

    We study Mn substitution for Ti in BaTiO$_3$ with and without compensating oxygen vacancies using density functional theory (DFT) in combination with dynamical mean field theory (DMFT). We find strong charge and spin fluctuations. Without compensating oxygen vacancies, the ground state is found to be a quantum superposition of two distinct atomic valences, 3{\\it d}$^4$ and 3{\\it d}$^5$. Introducing a compensating oxygen vacancy at a neighboring site reduces both charge and spin fluctuations d...

  2. Superconductivity, Antiferromagnetism, and Kinetic Correlation in Strongly Correlated Electron Systems

    Directory of Open Access Journals (Sweden)

    Takashi Yanagisawa

    2015-01-01

    Full Text Available We investigate the ground state of two-dimensional Hubbard model on the basis of the variational Monte Carlo method. We use wave functions that include kinetic correlation and doublon-holon correlation beyond the Gutzwiller ansatz. It is still not clear whether the Hubbard model accounts for high-temperature superconductivity. The antiferromagnetic correlation plays a key role in the study of pairing mechanism because the superconductive phase exists usually close to the antiferromagnetic phase. We investigate the stability of the antiferromagnetic state when holes are doped as a function of the Coulomb repulsion U. We show that the antiferromagnetic correlation is suppressed as U is increased exceeding the bandwidth. High-temperature superconductivity is possible in this region with enhanced antiferromagnetic spin fluctuation and pairing interaction.

  3. Spin-orbit torques in locally and globally noncentrosymmetric crystals: antiferromagnets and ferromagnets

    Czech Academy of Sciences Publication Activity Database

    Železný, Jakub; Gao, H.; Manchon, A.; Freimuth, F.; Mokrousov, Y.; Zemen, J.; Mašek, Jan; Sinova, Jairo; Jungwirth, Tomáš

    2017-01-01

    Roč. 95, č. 1 (2017), 1-18, č. článku 014403. ISSN 2469-9950 R&D Projects: GA MŠk LM2015087; GA ČR GB14-37427G; GA MŠk(CZ) LM2011026 EU Projects: European Commission(XE) 268066 - 0MSPIN Institutional support: RVO:68378271 Keywords : spintronics * antiferromagnets Subject RIV: BM - Solid Matter Physics ; Magnetism Impact factor: 3.836, year: 2016

  4. High antiferromagnetic domain wall velocity induced by Néel spin-orbit torques

    Czech Academy of Sciences Publication Activity Database

    Gomonay, O.; Jungwirth, Tomáš; Sinova, Jairo

    2016-01-01

    Roč. 117, č. 1 (2016), 1-5, č. článku 017202. ISSN 0031-9007 R&D Projects: GA MŠk(CZ) LM2011026; GA ČR GB14-37427G EU Projects: European Commission(XE) 268066 - 0MSPIN Institutional support: RVO:68378271 Keywords : spintronics * domain walls * antiferromagnets Subject RIV: BM - Solid Matter Physics ; Magnetism Impact factor: 8.462, year: 2016

  5. Control of antiferromagnetic spin axis orientation in bilayer Fe/CuMnAs films

    Czech Academy of Sciences Publication Activity Database

    Wadley, P.; Edmonds, K. W.; Shahedkhah, M.R.; Campion, R. P.; Gallagher, B. L.; Železný, Jakub; Kuneš, Jan; Novák, Vít; Jungwirth, Tomáš; Saidl, Vít; Němec, P.; Maccherozzi, F.; Dhesi, S.S.

    2017-01-01

    Roč. 7, Sep (2017), 1-6, č. článku 11147. ISSN 2045-2322 R&D Projects: GA MŠk LM2015087; GA ČR GB14-37427G Institutional support: RVO:68378271 Keywords : antiferromagnetic spintronics * exchange coupling Subject RIV: BM - Solid Matter Physics ; Magnetism OBOR OECD: Condensed matter physics (including formerly solid state physics, supercond.) Impact factor: 4.259, year: 2016

  6. Spin correlations in the 2D Heisenberg antiferromagnet Sr2CuO2Cl2: Neutron scattering, Monte Carlo simulation, and theory

    International Nuclear Information System (INIS)

    Greven, M.; Birgeneau, R.J.; Endoh, Y.; Kastner, M.A.; Keimer, B.; Matsuda, M.; Shirane, G.; Thurston, T.R.

    1994-01-01

    We report a neutron scattering study of the spin correlations in the model 2D, S=1/2, square-lattice Heisenberg antiferromagnetic Sr 2 CuO 2 Cl 2 . The spin correlation lengths obtained agree quantitatively with values deduced from Monte Carlo simulations over a wide range of temperature. The combined data, which cover the length scale from 1 to 200 lattice constants, are predicted accurately with no adjustable parameters by renormalized classical theory for the quantum nonlinear sigma model

  7. Characterisation of spin-waves in copper(II) deuteroformate tetradeuterate: A square ¤S¤=1/2 Heisenberg antiferromagnet

    DEFF Research Database (Denmark)

    Clarke, S.J.; Harrison, A.; Mason, T.E.

    1999-01-01

    Copper(II) formate tetrahydrate (CFTH) is a model square S = 1/2 Heisenberg antiferromagnet with T-N = 16.54 +/- 0.05 K. The dispersion of spin-waves in the magnetic layers of a fully deuterated sample of this material has been mapped at 4.3 K by inelastic neutron scattering from the zone centre...

  8. Erratum : Critical Properties of Spin-1 Antiferromagnetic Heisenberg Chains with Bond Alternation and Uniaxial Single-Ion-Type Anisotropy (vol 69, pg 237, 2000)

    OpenAIRE

    Chen, Wei; 飛田, 和男; Sanctuary, Bryan C.

    2008-01-01

    Original Paper :Critical Properties of Spin-1 Antiferromagnetic Heisenberg Chains with Bond Alternation and Uniaxial Single-Ion-Type AnisotropyWei Chen, Kazuo Hida and Bryan Clifford Sanctuary Journal of the Physical Society of Japan 69 (2000) pp.237-241

  9. Imaging the real space structure of the spin fluctuations in an iron-based superconductor.

    Science.gov (United States)

    Chi, Shun; Aluru, Ramakrishna; Grothe, Stephanie; Kreisel, A; Singh, Udai Raj; Andersen, Brian M; Hardy, W N; Liang, Ruixing; Bonn, D A; Burke, S A; Wahl, Peter

    2017-06-29

    Spin fluctuations are a leading candidate for the pairing mechanism in high temperature superconductors, supported by the common appearance of a distinct resonance in the spin susceptibility across the cuprates, iron-based superconductors and many heavy fermion materials. The information we have about the spin resonance comes almost exclusively from neutron scattering. Here we demonstrate that by using low-temperature scanning tunnelling microscopy and spectroscopy we can characterize the spin resonance in real space. We show that inelastic tunnelling leads to the characteristic dip-hump feature seen in tunnelling spectra in high temperature superconductors and that this feature arises from excitations of the spin fluctuations. Spatial mapping of this feature near defects allows us to probe non-local properties of the spin susceptibility and to image its real space structure.

  10. Imaging the real space structure of the spin fluctuations in an iron-based superconductor

    Science.gov (United States)

    Chi, Shun; Aluru, Ramakrishna; Grothe, Stephanie; Kreisel, A.; Singh, Udai Raj; Andersen, Brian M.; Hardy, W. N.; Liang, Ruixing; Bonn, D. A.; Burke, S. A.; Wahl, Peter

    2017-06-01

    Spin fluctuations are a leading candidate for the pairing mechanism in high temperature superconductors, supported by the common appearance of a distinct resonance in the spin susceptibility across the cuprates, iron-based superconductors and many heavy fermion materials. The information we have about the spin resonance comes almost exclusively from neutron scattering. Here we demonstrate that by using low-temperature scanning tunnelling microscopy and spectroscopy we can characterize the spin resonance in real space. We show that inelastic tunnelling leads to the characteristic dip-hump feature seen in tunnelling spectra in high temperature superconductors and that this feature arises from excitations of the spin fluctuations. Spatial mapping of this feature near defects allows us to probe non-local properties of the spin susceptibility and to image its real space structure.

  11. Magnetization process and magnetocaloric effect in geometrically frustrated Ising antiferromagnet and spin ice models on a 'Star of David' nanocluster

    Science.gov (United States)

    Žukovič, M.; Semjan, M.

    2018-04-01

    Magnetic and magnetocaloric properties of geometrically frustrated antiferromagnetic Ising (IA) and ferromagnetic spin ice (SI) models on a nanocluster with a 'Star of David' topology, including next-nearest-neighbor (NNN) interactions, are studied by an exact enumeration. In an external field applied in characteristic directions of the respective models, depending on the NNN interaction sign and magnitude, the ground state magnetization of the IA model is found to display up to three intermediate plateaus at fractional values of the saturation magnetization, while the SI model shows only one zero-magnetization plateau and only for the antiferromagnetic NNN coupling. A giant magnetocaloric effect is revealed in the IA model with the NNN interaction either absent or equal to the nearest-neighbor coupling. The latter is characterized by abrupt isothermal entropy changes at low temperatures and infinitely fast adiabatic temperature variations for specific entropy values in the processes when the magnetic field either vanishes or tends to the critical values related to the magnetization jumps.

  12. Spin frustration and magnetic ordering in triangular lattice antiferromagnet Ca3CoNb2O9

    Science.gov (United States)

    Dai, Jia; Zhou, Ping; Wang, Peng-Shuai; Pang, Fei; Munsie, Tim J.; Luke, Graeme M.; Zhang, Jin-Shan; Yu, Wei-Qiang

    2015-12-01

    We synthesized a quasi-two-dimensional distorted triangular lattice antiferromagnet Ca3CoNb2O9, in which the effective spin of Co2+ is 1/2 at low temperatures, whose magnetic properties were studied by dc susceptibility and magnetization techniques. The x-ray diffraction confirms the quality of our powder samples. The large Weiss constant θCW˜ -55 K and the low Neel temperature TN˜ 1.45 K give a frustration factor f = | θCW/TN | ≈ 38, suggesting that Ca3CoNb2O9 resides in strong frustration regime. Slightly below TN, deviation between the susceptibility data under zero-field cooling (ZFC) and field cooling (FC) is observed. A new magnetic state with 1/3 of the saturate magnetization Ms is suggested in the magnetization curve at 0.46 K. Our study indicates that Ca3CoNb2O9 is an interesting material to investigate magnetism in triangular lattice antiferromagnets with weak anisotropy. Project supported by the National Natural Science Foundation of China (Grant Nos. 11374364 and 11222433), the National Basic Research Program of China (Grant No. 2011CBA00112). Research at McMaster University supported by the Natural Sciences and Engineering Research Council. Work at North China Electric Power University supported by the Scientific Research Foundation for the Returned Overseas Chinese Scholars, State Education Ministry.

  13. Fullerene/layered antiferromagnetic reconstructed spinterface: Subsurface layer dominates molecular orbitals' spin-split and large induced magnetic moment

    Science.gov (United States)

    Shao, Yangfan; Pang, Rui; Pan, Hui; Shi, Xingqiang

    2018-03-01

    The interfaces between organic molecules and magnetic metals have gained increasing interest for both fundamental reasons and applications. Among them, the C60/layered antiferromagnetic (AFM) interfaces have been studied only for C60 bonded to the outermost ferromagnetic layer [S. L. Kawahara et al., Nano Lett. 12, 4558 (2012) and D. Li et al., Phys. Rev. B 93, 085425 (2016)]. Here, via density functional theory calculations combined with evidence from the literature, we demonstrate that C60 adsorption can reconstruct the layered-AFM Cr(001) surface at elevated annealing temperatures so that C60 bonds to both the outermost and the subsurface Cr layers in opposite spin directions. Surface reconstruction drastically changes the adsorbed molecule spintronic properties: (1) the spin-split p-d hybridization involves multi-orbitals of C60 and top two layers of Cr with opposite spin-polarization, (2) the subsurface Cr atom dominates the C60 electronic properties, and (3) the reconstruction induces a large magnetic moment of 0.58 μB in C60 as a synergistic effect of the top two Cr layers. The induced magnetic moment in C60 can be explained by the magnetic direct-exchange mechanism, which can be generalized to other C60/magnetic metal systems. Understanding these complex hybridization behaviors is a crucial step for molecular spintronic applications.

  14. Mechanism of Basal-Plane Antiferromagnetism in the Spin-Orbit Driven Iridate Ba_{2}IrO_{4}

    Directory of Open Access Journals (Sweden)

    Vamshi M. Katukuri

    2014-06-01

    Full Text Available By ab initio many-body quantum chemistry calculations, we determine the strength of the symmetric anisotropy in the 5d^{5} j≈1/2 layered material Ba_{2}IrO_{4}. While the calculated anisotropic couplings come out in the range of a few meV, orders of magnitude stronger than in analogous 3d transition-metal compounds, the Heisenberg superexchange still defines the largest energy scale. The ab initio results reveal that individual layers of Ba_{2}IrO_{4} provide a close realization of the quantum spin-1/2 Heisenberg-compass model on the square lattice. We show that the experimentally observed basal-plane antiferromagnetism can be accounted for by including additional interlayer interactions and the associated order-by-disorder quantum-mechanical effects, in analogy to undoped layered cuprates.

  15. Writing and reading antiferromagnetic Mn2Au by Néel spin-orbit torques and large anisotropic magnetoresistance.

    Science.gov (United States)

    Bodnar, S Yu; Šmejkal, L; Turek, I; Jungwirth, T; Gomonay, O; Sinova, J; Sapozhnik, A A; Elmers, H-J; Kläui, M; Jourdan, M

    2018-01-24

    Using antiferromagnets as active elements in spintronics requires the ability to manipulate and read-out the Néel vector orientation. Here we demonstrate for Mn 2 Au, a good conductor with a high ordering temperature suitable for applications, reproducible switching using current pulse generated bulk spin-orbit torques and read-out by magnetoresistance measurements. Reversible and consistent changes of the longitudinal resistance and planar Hall voltage of star-patterned epitaxial Mn 2 Au(001) thin films were generated by pulse current densities of ≃10 7  A/cm 2 . The symmetry of the torques agrees with theoretical predictions and a large read-out magnetoresistance effect of more than ≃6% is reproduced by ab initio transport calculations.

  16. Beyond Gaussian approximation in the spin-fluctuation theory of metallic ferromagnetism

    Energy Technology Data Exchange (ETDEWEB)

    Reser, B I; Grebennikov, V I [Institute of Metal Physics, Russian Academy of Sciences, Ekaterinburg (Russian Federation); Melnikov, N B, E-mail: reser@imp.uran.r [Lomonosov Moscow State University, Moscow (Russian Federation)

    2010-01-15

    A characteristic feature of the Gaussian spin-fluctuation theory is the jump transition into the paramagnetic state. We eliminate the jump and obtain a continuous second-order phase transition by taking into account the high-order terms of the free energy of electrons in the fluctuating exchange field. The third-order term of the free energy yields a renormalization of the mean field, and fourth-order term, responsible for the interaction of the fluctuations, gives a renormalization of the spin susceptibility. The extended theory is applied to the calculation of magnetic properties of Fe-Ni Invar.

  17. Effects of spin fluctuations and anomalous thermal expansion of δ-Pu

    Energy Technology Data Exchange (ETDEWEB)

    Solontsov, A.; Antropov, V. P.

    2010-06-02

    We suggest a model for the magnetic dynamics of {delta} plutonium and its alloys in order to show that the dynamical fluctuations of the magnetization density, or spin fluctuations, may be responsible for the anomalies of their observed thermal expansion. We show that due to strong magnetoelastic coupling, spin fluctuations may essentially contribute to the volume strain by giving a negative magnetovolume contribution that is proportional to the squared local magnetic moment and the magnetic Gruneisen constant which is negative in {delta} plutonium. In the presented model, the local magnetic moment increases as the temperature rises, resulting in the interplay between the positive contributions to the volume strain from the lattice and the negative contribution from spin fluctuations, and finally leads to the Invar anomaly or to the negative coefficient of thermal expansion. Our results agree closely with the measured thermal-expansion data for Pu-Ga alloys.

  18. Spin reorientation and Ce-Mn coupling in antiferromagnetic oxypnictide CeMnAsO

    OpenAIRE

    Zhang, Qiang; Tian, Wei; Peterson, Spencer G.; Dennis, Kevin W.; Vaknin, David

    2014-01-01

    Structure and magnetic properties of high-quality polycrystlline CeMnAsO, a parent compound of the "1111"-type oxypnictides, have been investigated using neutron powder diffraction and magnetization measurements. We find that CeMnAsO undergoes a C-type antiferromagnetic order with Mn$^{2+}$ ($S=5/2$) moments pointing along the \\textit{c}-axis below a relatively high N\\'{e}el temperature of $T_{\\rm N} = 345$ K. Below $T_{\\rm SR} = 35$ K, two instantaneous transitions occur where the Mn moments...

  19. Electric control of Dirac quasiparticles by spin-orbit torque in an antiferromagnet

    Czech Academy of Sciences Publication Activity Database

    Šmejkal, Libor; Železný, Jakub; Sinova, Jairo; Jungwirth, Tomáš

    2017-01-01

    Roč. 118, č. 10 (2017), 1-5, č. článku 106402. ISSN 0031-9007 R&D Projects: GA MŠk LM2015087; GA ČR GB14-37427G EU Projects: European Commission(XE) 610115 - SC2 Institutional support: RVO:68378271 Keywords : spintronics * topological Dirac fermions * antiferromagnets Subject RIV: BM - Solid Matter Physics ; Magnetism OBOR OECD: Condensed matter physics (including formerly solid state physics , supercond.) Impact factor: 8.462, year: 2016

  20. Magnetic correlations of the quasi-one-dimensional half-integer spin-chain antiferromagnets Sr$M_2$V$_2$O$_8$ ($M$ = Co, Mn)

    OpenAIRE

    Bera, A. K.; Lake, B.; Stein, W. -D.; Zander, S.

    2014-01-01

    Magnetic correlations of two iso-structural quasi-one-dimensional (1D) antiferromagnetic spin-chain compounds Sr$M_2$V$_2$O$_8$ ($M$ = Co, Mn) have been investigated by magnetization and powder neutron diffraction. Two different collinear antiferromagnetic (AFM) structures, characterized by the propagation vectors, $k$ = (0 0 1) and $k$ = (0 0 0), have been found below $\\sim$ 5.2 K and $\\sim$ 42.2 K for the Co- and Mn-compounds, respectively. For the Mn-compound, AFM chains (along the $c$ axi...

  1. Superconductivity by charge and spin fluctuations in strongly correlated systems

    Energy Technology Data Exchange (ETDEWEB)

    Costa-Quintana, J. [Universitat Autonoma de Barcelona (Spain). Grup d`Electromagnetisme; Gonzalez-Leon, E. [Universitat Autonoma de Barcelona (Spain). Grup d`Electromagnetisme; Lopez Aguilar, F. [Universitat Autonoma de Barcelona (Spain). Grup d`Electromagnetisme; Puig-Puig, L. [Universitat Autonoma de Barcelona (Spain). Grup d`Electromagnetisme; Sanchez-Lopez, M.M. [Universitat Autonoma de Barcelona (Spain). Grup d`Electromagnetisme

    1995-02-01

    We obtain the effective potential from a screened coulombian interaction considering separately the interaction between fermions with parallel and antiparallel spins. In both cases we analyze the possibility of obtaining superconductivity. ((orig.)).

  2. Protocol for generating multiphoton entangled states from quantum dots in the presence of nuclear spin fluctuations

    Science.gov (United States)

    Denning, Emil V.; Iles-Smith, Jake; McCutcheon, Dara P. S.; Mork, Jesper

    2017-12-01

    Multiphoton entangled states are a crucial resource for many applications in quantum information science. Semiconductor quantum dots offer a promising route to generate such states by mediating photon-photon correlations via a confined electron spin, but dephasing caused by the host nuclear spin environment typically limits coherence (and hence entanglement) between photons to the spin T2* time of a few nanoseconds. We propose a protocol for the deterministic generation of multiphoton entangled states that is inherently robust against the dominating slow nuclear spin environment fluctuations, meaning that coherence and entanglement is instead limited only by the much longer spin T2 time of microseconds. Unlike previous protocols, the present scheme allows for the generation of very low error probability polarization encoded three-photon GHZ states and larger entangled states, without the need for spin echo or nuclear spin calming techniques.

  3. Phase diagrams of antiferromagnetic spin-1 bosons on a square optical lattice with the quadratic Zeeman effect

    Science.gov (United States)

    de Forges de Parny, L.; Rousseau, V. G.

    2018-02-01

    We study the quadratic Zeeman effect (QZE) in a system of antiferromagnetic spin-1 bosons on a square lattice and derive the ground-state phase diagrams by means of quantum Monte Carlo simulations and mean-field treatment. The QZE imbalances the populations of the magnetic sublevels σ =±1 and σ =0 , and therefore affects the magnetic and mobility properties of the phases. Both methods show that the tip of the even Mott lobes, stabilized by singlet state, is destroyed when turning on the QZE, thus leaving the space to the superfluid phase. Contrariwise, the tips of odd Mott lobes remain unaffected. Therefore, the Mott-superfluid transition with even filling strongly depends on the strength of the QZE, and we show that the QZE can act as a control parameter for this transition at fixed hopping. Using quantum Monte Carlo simulations, we elucidate the nature of the phase transitions and examine in detail the nematic order: the first-order Mott-superfluid transition with even filling observed in the absence of QZE becomes second order for weak QZE, in contradistinction to our mean-field results which predict a first-order transition in a larger range of QZE. Furthermore, a spin nematic order with director along the z axis is found in the odd Mott lobes and in the superfluid phase for energetically favored σ =±1 states. In the superfluid phase with even filling, the x y components of the nematic director remain finite only for moderate QZE.

  4. Inelastic neutron scattering study of a nonmagnetic collapsed tetragonal phase in nonsuperconducting CaFe2As2: evidence of the impact of spin fluctuations on superconductivity in the iron-arsenide compounds.

    Science.gov (United States)

    Soh, J H; Tucker, G S; Pratt, D K; Abernathy, D L; Stone, M B; Ran, S; Bud'ko, S L; Canfield, P C; Kreyssig, A; McQueeney, R J; Goldman, A I

    2013-11-27

    The relationship between antiferromagnetic spin fluctuations and superconductivity has become a central topic of research in studies of superconductivity in the iron pnictides. We present unambiguous evidence of the absence of magnetic fluctuations in the nonsuperconducting collapsed tetragonal phase of CaFe2As2 via inelastic neutron scattering time-of-flight data, which is consistent with the view that spin fluctuations are a necessary ingredient for unconventional superconductivity in the iron pnictides. We demonstrate that the collapsed tetragonal phase of CaFe2As2 is nonmagnetic, and discuss this result in light of recent reports of high-temperature superconductivity in the collapsed tetragonal phase of closely related compounds.

  5. Strong anisotropic anomalous Hall effect and spin Hall effect in the chiral antiferromagnetic compounds Mn3X (X =Ge , Sn, Ga, Ir, Rh, and Pt)

    Science.gov (United States)

    Zhang, Yang; Sun, Yan; Yang, Hao; Železný, Jakub; Parkin, Stuart P. P.; Felser, Claudia; Yan, Binghai

    2017-02-01

    We have carried out a comprehensive study of the intrinsic anomalous Hall effect and spin Hall effect of several chiral antiferromagnetic compounds Mn3X (X = Ge, Sn, Ga, Ir, Rh and Pt) by ab initio band structure and Berry phase calculations. These studies reveal large and anisotropic values of both the intrinsic anomalous Hall effect and spin Hall effect. The Mn3X materials exhibit a noncollinear antiferromagnetic order which, to avoid geometrical frustration, forms planes of Mn moments that are arranged in a Kagome-type lattice. With respect to these Kagome planes, we find that both the anomalous Hall conductivity (AHC) and the spin Hall conductivity (SHC) are quite anisotropic for any of these materials. Based on our calculations, we propose how to maximize AHC and SHC for different materials. The band structures and corresponding electron filling, that we show are essential to determine the AHC and SHC, are compared for these different compounds. We point out that Mn3Ga shows a large SHC of about 600 (ℏ /e ) (Ωcm) -1 . Our work provides insights into the realization of strong anomalous Hall effects and spin Hall effects in chiral antiferromagnetic materials.

  6. Protocol for generating multiphoton entangled states from quantum dots in the presence of nuclear spin fluctuations

    DEFF Research Database (Denmark)

    Denning, Emil Vosmar; Iles-Smith, Jake; McCutcheon, Dara P. S.

    2017-01-01

    Multiphoton entangled states are a crucial resource for many applications inquantum information science. Semiconductor quantum dots offer a promising route to generate such states by mediating photon-photon correlations via a confinedelectron spin, but dephasing caused by the host nuclear spin...... environment typically limits coherence (and hence entanglement) between photons to the spin T2* time of a few nanoseconds. We propose a protocol for the deterministic generation of multiphoton entangled states that is inherently robust against the dominating slow nuclear spin environment fluctuations, meaning...... that coherence and entanglement is instead limited only by the much longer spin T2 time of microseconds. Unlike previous protocols, the present schemeallows for the generation of very low error probability polarisation encoded three-photon GHZ states and larger entangled states, without the need for spin echo...

  7. Spin fluctuations and low temperature features of thermal coefficient of linear expansion of iron monosilicide

    International Nuclear Information System (INIS)

    Volkov, A.G.; Kortov, S.V.; Povzner, A.A.

    1996-01-01

    The low temperature measurements of thermal coefficient of linear expansion of strong paramagnet FeSi are carried out. The results obtained are discussed with in the framework of spin-fluctuation theory. It is shown that electronic part of the thermal coefficient of linear expansion is negative in the range of temperatures lower that of the semiconductor-metal phase transition. In metal phase it becomes positive. This specific features of the thermal coefficient is explained by the spin-fluctuation renormalization of d-electronic states density

  8. Zitterbewegung with spin-orbit coupled ultracold atoms in a fluctuating optical lattice

    OpenAIRE

    Argonov, V. Yu.; Makarov, D. V.

    2015-01-01

    Dynamics of non-interacting ultracold atoms with artificial spin-orbit coupling is considered. Spin-orbit coupling is created using two moving optical lattices with orthogonal polarizations. Our main goal is to study influence of lattice noise on Rabi oscillations. Special attention is paid to the phenomenon of the Zitterbewegung being trembling motion caused by Rabi transitions between states with different velocities. Phase and amplitude fluctuations of lattices are modelled by means of the...

  9. Critical and reentrant behavior of the spin quantum 1/2 anisotropic Heisenberg antiferromagnet model with Dzyaloshinskii–Moriya interaction in a longitudinal magnetic field

    Energy Technology Data Exchange (ETDEWEB)

    Parente, Walter E.F.; Pacobahyba, J.T.M.; Araújo, Ijanílio G. [Departamento de Física, Universidade Federal de Roraima, BR 174, Km 12. Bairro Monte Cristo. CEP: 69300-000 Boa Vista, Roraima (Brazil); Neto, Minos A., E-mail: minos@pq.cnpq.br [Universidade Federal do Amazonas, Departamento de Física, 3000, Japiim, 69077-000, Manaus-AM (Brazil); Ricardo de Sousa, J. [Universidade Federal do Amazonas, Departamento de Física, 3000, Japiim, 69077-000, Manaus-AM (Brazil); National Institute of Science and Technology for Complex Systems, 3000, Japiim, 69077-000, Manaus-AM (Brazil); Akinci, Ümit [Department of Physics, Dokuz Eylül University, Tr-35160 Izmir (Turkey)

    2014-04-15

    In this paper we study the quantum spin-1/2 anisotropic Heisenberg antiferromagnet model in the presence of a Dzyaloshinskii–Moriya interaction (D) and a uniform longitudinal (H) magnetic field. Using the effective-field theory with a finite cluster N=2 spin (EFT-2) we calculate the phase diagrams in the H−T and D−T planes on a simple cubic lattice (z=6). We have only observed second order phase transitions for values between Δ∈[0,1], where the cases were analysed: Ising (Δ=1), anisotropic Heisenberg (Δ=0.6) and isotropic Heisenberg (Δ=0). - Highlights: • Anisotropic Heisenberg antiferromagnet on a simple cubic lattice. • Effective-field theory. • Dzyaloshinskii–Moriya interaction.

  10. Spin model for nontrivial types of magnetic order in inverse-perovskite antiferromagnets

    Science.gov (United States)

    Mochizuki, Masahito; Kobayashi, Masaya; Okabe, Reoya; Yamamoto, Daisuke

    2018-02-01

    Nontrivial magnetic orders in the inverse-perovskite manganese nitrides are theoretically studied by constructing a classical spin model describing the magnetic anisotropy and frustrated exchange interactions inherent in specific crystal and electronic structures of these materials. With a replica-exchange Monte Carlo technique, a theoretical analysis of this model reproduces the experimentally observed triangular Γ5 g and Γ4 g spin-ordered patterns and the systematic evolution of magnetic orders. Our Rapid Communication solves a 40-year-old problem of nontrivial magnetism for the inverse-perovskite manganese nitrides and provides a firm basis for clarifying the magnetism-driven negative thermal expansion phenomenon discovered in this class of materials.

  11. Antiferromagnetic spin correlations in (Nd,Pr)2-xCexCuO4

    International Nuclear Information System (INIS)

    Thurston, T.R.; Matsuda, M.; Kakurai, K.; Yamada, K.; Endoh, Y.; Birgeneau, R.J.; Gehring, P.M.; Hidaka, Y.; Kastner, M.A.; Murakami, T.; Shirane, G.

    1990-01-01

    Neutron-scattering measurements have been performed on (Nd,Pr) 2-x Ce x CuO 4 (0.0 2 CuO 4 albeit with renormalized spin stiffness constants ρ s . Thus, in the nonsuperconducting doping regime the hole- and electron-doped systems exhibit analogous magnetic behavior except for the drastically different dopant-concentration scales for the destruction of magnetic order

  12. Spin-valves with modified synthetic antiferromagnets exhibiting an enhanced bias point control capability at submicrometer dimensions

    International Nuclear Information System (INIS)

    Park, J.-S.; Lee, S.-R.; Kim, Y.K.

    2004-01-01

    Bias point control is of practical importance for operating read sensors for magnetic recording and magnetic random access memory devices. To attain bias point control capability, in particular, at submicrometer cell size, a modified synthetic antiferromagnet-based spin-valve (MSSV) structure was devised. A series of calculations were carried out to investigate the effect of size variation on their MR transfer behaviors. The cell dimension was varied from 10 to 0.05 μm. The typical MSSV comprises IrMn (9.0)/CoFe (P1, 1.5)/Ru (0.7)/CoFe (P2, 3.0)/Ru (0.7)/CoFe (P3, 1.5)/Cu (2.8)/CoFe (1.6)/NiFe (3.2) (in nm). As the cell size decreased, the bias point in the MSSV maintained nearly zero regardless of the cell size. The bias point was further tuned by varying the P3 layer thickness. Moreover, the effective exchange field (H ex.eff ) of the MSSV was much larger than that of the conventional SSV. The field sensitivity of the MSSV was very high indicating that the free layer can rotate more sharply

  13. Spin-valves with modified synthetic antiferromagnets exhibiting an enhanced bias point control capability at submicrometer dimensions

    Science.gov (United States)

    Park, Jeong-Suk; Lee, Seong-Rae; Kim, Young Keun

    2004-08-01

    Bias point control is of practical importance for operating read sensors for magnetic recording and magnetic random access memory devices. To attain bias point control capability, in particular, at submicrometer cell size, a modified synthetic antiferromagnet-based spin-valve (MSSV) structure was devised. A series of calculations were carried out to investigate the effect of size variation on their MR transfer behaviors. The cell dimension was varied from 10 to 0.05 μm. The typical MSSV comprises IrMn (9.0)/CoFe (P1, 1.5)/Ru (0.7)/CoFe (P2, 3.0)/Ru (0.7)/CoFe (P3, 1.5)/Cu (2.8)/CoFe (1.6)/NiFe (3.2) (in nm). As the cell size decreased, the bias point in the MSSV maintained nearly zero regardless of the cell size. The bias point was further tuned by varying the P3 layer thickness. Moreover, the effective exchange field ( Hex.eff) of the MSSV was much larger than that of the conventional SSV. The field sensitivity of the MSSV was very high indicating that the free layer can rotate more sharply.

  14. Low temperature ballistic spin transport in the S=1/2 antiferromagnetic Heisenberg chain compound SrCuO{sub 2}

    Energy Technology Data Exchange (ETDEWEB)

    Maeter, H.; Klauss, H.H. [Institut fuer Festkoerperphysik, TU Dresden (Germany); Zvyagin, A.A. [Institut fuer Festkoerperphysik, TU Dresden (Germany); Institute for Low Temperature Physics and Engineering, NAS of Ukraine, Kharkov (Ukraine); Luetkens, H.; Pascua, G.; Shermadini, Z. [Laboratory for Muon-Spin Spectroscopy, Paul Scherrer Institute, Villigen (Switzerland); Hess, C.; Hlubek, N.; Buechner, B. [Leibniz-Institut fuer Festkoerper- und Werkstoffforschung, Dresden (Germany); Saint-Matin, R.; Revcolevschi, A. [Laboratoire de Physico-Chimie de L' Etat Solide, ICMMO, UMR 8182, Universite Paris-Sud, Orsay (France)

    2011-07-01

    For one-dimensional quantum spin chain systems recent experimental and theoretical studies indicate unexpectedly large, in some cases diverging spin and heat transport coefficients. Local probes, like e.g. muon spin relaxation ({mu}SR) can indirectly characterize the spin transport properties of low dimensional systems via the magnetic field dependence of the spin lattice relaxation rate {lambda}(B). For diffusive spin transport {lambda}{proportional_to}B{sup -0.5} is expected. For the ground state of the isotropic spin-1/2 antiferromagnetic Heisenberg chain the eigenstates of the Heisenberg Hamiltonian dominate the spin transport, which is then ballistic. Using the Mueller ansatz {lambda}{proportional_to}B{sup -1} is expected in this case. For SrCuO{sub 2} we find {lambda}{proportional_to}B{sup -0.9(3)}. This result is temperature independent for 5 K{<=}T {<=}300 K. Within conformal field theory and using the Mueller ansatz we conclude ballistic spin transport in SrCuO{sub 2}.

  15. Doping dependence of spin fluctuations and electron correlations in iron pnictides

    Czech Academy of Sciences Publication Activity Database

    Ikeda, H.; Arita, R.; Kuneš, Jan

    2010-01-01

    Roč. 82, č. 2 (2010), 024508/1-024508/6 ISSN 1098-0121 Institutional research plan: CEZ:AV0Z10100521 Keywords : iron pnicitdes * dynamic spin susceptibility * fluctuation- exchange approximation Subject RIV: BM - Solid Matter Physics ; Magnetism Impact factor: 3.772, year: 2010 http://prb.aps.org/abstract/PRB/v82/i2/e024508

  16. Spin fluctuations and superconductivity in Mo.sub.3./sub.Sb.sub.7./sub..

    Czech Academy of Sciences Publication Activity Database

    Candolfi, C.; Lenoir, B.; Dauscher, A.; Bellouard, C.; Hejtmánek, Jiří; Šantavá, Eva; Tobola, J.

    2007-01-01

    Roč. 99, č. 3 (2007), 037006/1-037006/4 ISSN 0031-9007 Institutional research plan: CEZ:AV0Z10100521 Keywords : spin fluctuations * paramagnons * superconductivity Subject RIV: BM - Solid Matter Physics ; Magnetism Impact factor: 6.944, year: 2007

  17. Itinerant ferromagnetism in actinide 5 f -electron systems: Phenomenological analysis with spin fluctuation theory

    Science.gov (United States)

    Tateiwa, Naoyuki; Pospíšil, Jiří; Haga, Yoshinori; Sakai, Hironori; Matsuda, Tatsuma D.; Yamamoto, Etsuji

    2017-07-01

    We have carried out an analysis of magnetic data in 69 uranium, 7 neptunium, and 4 plutonium ferromagnets with the spin fluctuation theory developed by Takahashi [Y. Takahashi, J. Phys. Soc. Jpn. 55, 3553 (1986), 10.1143/JPSJ.55.3553]. The basic and spin fluctuation parameters of the actinide ferromagnets are determined and the applicability of the spin fluctuation theory to actinide 5 f system has been discussed. Itinerant ferromagnets of the 3 d transition metals and their intermetallics follow a generalized Rhodes-Wohlfarth relation between peff/ps and TC/T0 , viz., peff/ps∝(TC/T0) -3 /2 . Here, ps, peff, TC, and T0 are the spontaneous and effective magnetic moments, the Curie temperature, and the width of spin fluctuation spectrum in energy space, respectively. The same relation is satisfied for TC/T0uranium and neptunium ferromagnets below (TC/T0)kink=0.32 ±0.02 , where a kink structure appears in relation between the two quantities. ps increases more weakly above (TC/T0)kink. A possible interpretation with the TC/T0 dependence of ps is given.

  18. Effect of spatial spin modulation on relaxation and NMR frequencies of sup 5 sup 7 Fe nuclei in ferroelectric antiferromagnetic BiFeO sub 3

    CERN Document Server

    Zalessky, A V; Zvezdin, A K; Gippius, A A; Morozova, E N; Khozeev, D F; Bush, A S; Pokatilov, V S

    2002-01-01

    The NMR spectra on the iron nuclei in the BiFeO sub 3 antiferromagnetic sample enriched by the sup 5 sup 7 Fe (95.43%) with the spatially-modulated magnetic structure are studied. It is established that the cycloid-type spin modulation in the BiFeO sub 3 produces spatial modulation of the nuclear spin-spin relaxation velocity and leads to the spectral nonuniform widening of the NMR local line. It is determined also that the local magnetic moments of the iron ions on various cycloid sections differently depend on temperature which testifies to different character of the spin waves excitation. The analogy of the experimental results with the NMR regularities in the Bloch wall is discussed

  19. Enhanced quantum spin fluctuations in a binary Bose-Einstein condensate

    Science.gov (United States)

    Bisset, R. N.; Kevrekidis, P. G.; Ticknor, C.

    2018-02-01

    For quantum fluids, the role of quantum fluctuations may be significant in several regimes such as when the dimensionality is low, the density is high, the interactions are strong, or for low particle numbers. In this paper, we propose a fundamentally different regime for enhanced quantum fluctuations without being restricted by any of the above conditions. Instead, our scheme relies on the engineering of an effective attractive interaction in a dilute, two-component Bose-Einstein condensate (BEC) consisting of thousands of atoms. In such a regime, the quantum spin fluctuations are significantly enhanced (atom bunching with respect to the noninteracting limit) since they act to reduce the interaction energy, a remarkable property given that spin fluctuations are normally suppressed (antibunching) at zero temperature. In contrast to the case of true attractive interactions, our approach is not vulnerable to BEC collapse. We numerically demonstrate that these quantum fluctuations are experimentally accessible by either spin or single-component Bragg spectroscopy, offering a useful platform on which to test beyond-mean-field theories. We also develop a variational model and use it to analytically predict the shift of the immiscibility critical point, finding good agreement with our numerics.

  20. Topological-Sector Fluctuations and Curie-Law Crossover in Spin Ice

    Directory of Open Access Journals (Sweden)

    L. D. C. Jaubert

    2013-02-01

    Full Text Available At low temperatures, a spin ice enters a Coulomb phase—a state with algebraic correlations and topologically constrained spin configurations. We show how analytical and numerical approaches for model spin-ice systems reveal a crossover between two Curie laws. One of these laws characterizes the high-temperature paramagnetic regime, while the other, which we call the “spin-liquid Curie law,” characterizes the low-temperature Coulomb-phase regime, which provides implicit evidence that the topological sector fluctuates. We compare our theory with experiment for Ho_{2}Ti_{2}O_{7}, where this process leads to a nonstandard temperature evolution of the bulk susceptibility and the wave-vector-dependent magnetic susceptibility, as measured by neutron scattering. Theory and experiment agree for bulk quantities and at large scattering wave vectors, but differences at small wave vectors indicate that the classical spin-ice states are not equally populated at low temperatures. More generally, the crossover appears to be a generic property of the emergent gauge field for a classical spin liquid, and it sheds light on the experimental difficulty of measuring a precise Curie-Weiss temperature in frustrated materials. The susceptibility at finite wave vectors is shown to be a local probe of fluctuations among topological sectors on varying length scales.

  1. Observation of layered antiferromagnetism in self-assembled parallel NiSi nanowire arrays on Si(110) by spin-polarized scanning tunneling spectromicroscopy

    Science.gov (United States)

    Hong, Ie-Hong; Hsu, Hsin-Zan

    2018-03-01

    The layered antiferromagnetism of parallel nanowire (NW) arrays self-assembled on Si(110) have been observed at room temperature by direct imaging of both the topographies and magnetic domains using spin-polarized scanning tunneling microscopy/spectroscopy (SP-STM/STS). The topographic STM images reveal that the self-assembled unidirectional and parallel NiSi NWs grow into the Si(110) substrate along the [\\bar{1}10] direction (i.e. the endotaxial growth) and exhibit multiple-layer growth. The spatially-resolved SP-STS maps show that these parallel NiSi NWs of different heights produce two opposite magnetic domains, depending on the heights of either even or odd layers in the layer stack of the NiSi NWs. This layer-wise antiferromagnetic structure can be attributed to an antiferromagnetic interlayer exchange coupling between the adjacent layers in the multiple-layer NiSi NW with a B2 (CsCl-type) crystal structure. Such an endotaxial heterostructure of parallel magnetic NiSi NW arrays with a layered antiferromagnetic ordering in Si(110) provides a new and important perspective for the development of novel Si-based spintronic nanodevices.

  2. Magnetic fluctuations in heavy-fermion metals

    DEFF Research Database (Denmark)

    Mason, T.E.; Petersen, T.; Aeppli, G.

    1995-01-01

    , the nature of the antiferromagnetic order and magnetic fluctuations is qualitatively quite different. UPd2Al3 resembles a rare earth magnetic system with coupling of the 4f electrons to the conduction electrons manifested in a broadening of otherwise conventional spin wave excitations. This is in marked...

  3. Partially disordered state and spin-lattice coupling in an S=3/2 triangular lattice antiferromagnet Ag2CrO2

    Science.gov (United States)

    Matsuda, M.; Yoshida, H.; Isobe, M.; de La Cruz, C.; Fishman, R. S.

    2012-02-01

    Ag2CrO2 consists of triangular lattice planes of CrO2, which are well separated by the metallic Ag2 layers. [1] This compound is an S=3/2 frustrated triangular lattice antiferromagnet without orbital degree of freedom. We performed neutron diffraction experiments on a powder sample of Ag2CrO2 on a neutron powder diffractometer HB-2A and a triple-axis neutron spectrometer HB-1, installed at HFIR in Oak Ridge National Laboratory. With decreasing temperature, a short-range 4-sublatice spin state develops. However, a long-range partially disordered state with 5 sublattices abruptly appears at TN=24 K, accompanied by a structural distortion, and persists at least down to 2 K. The spin-lattice coupling stabilizes the anomalous state, which is expected to appear only in limited ranges of further-neighbor interactions and temperature. It was found that the spin-lattice coupling is a common feature in triangular lattice antiferromagnets with multiple-sublattice spin states, since the triangular lattice is elastic. [4pt] [1] H. Yoshida et al., to appear in J. Phys. Soc. Jpn.

  4. Thermal and quantal isospin and spin fluctuations in heavy ion reactions

    International Nuclear Information System (INIS)

    Moretto, L.G.

    1980-01-01

    The isobaric charge distributions are discussed in terms of quantal and classical isospin fluctuations. The roles of mass asymmetry and of the higher giant isovector modes are treated within the framework of a cylinder model that is worked out exactly. Spin fluctuations are considered first in terms of quantal fluctuations in a cylinder model and second in terms of thermal fluctuations in a two-sphere model. The results are applied to the calculation of in- and out-of-plane angular distributions for sequential fission, alpha and gamma decay. Analytical expressions are obtained for the angular distributions. The theoretical predictions are compared with experimental results for sequential fission, alpha, and gamma angular distributions. 23 figures

  5. Superconductivity from magnetic fluctuations in FeTe{sub 1-x}Se{sub x}-feedback of double stripe magnetism on itinerant spin excitations

    Energy Technology Data Exchange (ETDEWEB)

    Mardani, Masoud; Moessner, Roderich [Max Planck Institute for the Physics of Complex Systems, Dresden (Germany); Knolle, Johannes [TCM Group, Cavendish Laboratory, University of Cambridge (United Kingdom); Eremin, Ilya [Institute for Theoretical Physics III, Ruhr-Universitaet Bochum (Germany)

    2015-07-01

    Iron-chalcogenide superconductors exhibit an unusual double stripe antiferromagnetic parent phase with ordering vector Q{sub AF} = (π/2,π/2) (in the one iron unit cell). In addition, magnetic excitations in optimally doped systems are peaked at momenta Q{sub SF} = (π,0)/(0,π), which is in contrast to most other families of iron-based superconductors. There, both the magnetic order of the parent compounds and the magnetic fluctuations in the superconducting state have the same momentum Q{sub SF}, which is taken as a strong argument in favor of spin-fluctuation induced superconductivity. Here, we model iron-chalcogenides as a system of itinerant electrons coupled to localized electrons responsible for the double stripe magnetism. We study the feedback of this unusual magnetic order on the itinerant spin excitations at Q{sub SF} and show that they increase with decreasing magnetism. We make connection to recent INS experiments and reproduce qualitatively the behavior of magnetic excitations in FeTe{sub 1-x}Se{sub x} from x=0 towards x=0.4.

  6. Large spin fluctuations and moment-volume coupling in Fe in an fcc environment

    International Nuclear Information System (INIS)

    Acet, M.; Wassermann, E.F.

    1999-01-01

    Complete text of publication follows. Polarized paramagnetic neutron diffraction experiments show that the persisting ferromagnetic correlations above the Curie temperature and the associated magnetic moment of fcc Fe 1-x Ni x alloys with x > 0.30 weaken with increasing temperature reflecting a temperature dependence of the band splitting. In alloys with x ≤ 0.30 the magnetic moment becomes more temperature insensitive and, as the pure Fe concentration is reached, it begins to increase with increasing temperature [1]. The observed property is attributed to a combination of effects arising from spin fluctuations pertinent to itinerant system and to moment-volume fluctuations arising from low-spin to high-spin transitions in systems incorporating a high concentration of fcc-Fe. The experiments are extended to broader fcc stability temperature ranges by using and Fe 0.77 Ni 0.13 Mn 0.07 C 0.03 alloy and further and more clear evidence for the temperature driven low-spin to high-spin transitions is shown. (author) [1] M. Acet, E.F. Wassermann, K. Andersen, A. Murani and O. Schaerpf, Europhys. Lett., 40 (1997) 93

  7. Quasi-2D J1-J2 antiferromagnet Zn2VO(PO4)2 and its Ti-substituted derivative: A spin-wave analysis

    Science.gov (United States)

    Kar, Satyaki; Saha-Dasgupta, Tanusri

    2014-01-01

    In this study, we present non-linear spin wave analysis of a quasi-2D spin-{1}/{2}J1-J2 antiferromagnet at the parameter regime relevant for the recently studied compound Zn2VO(PO4)2. We obtain the temperature dependence of the spin wave energy, susceptibility and magnetization using Green's function technique and Tyablikov's decoupling or Hartree-Fock factorization. The comparison of our numerical results with the experimental findings is discussed. Magnetic structure factor is calculated and compared with powder neutron diffraction data. We also study the spin wave behavior of the compound Zn2Ti0.25V0.75O(PO4)2 obtained by partial chemical substitution of Ti at V sites of the compound Zn2VO(PO4)2 [Kanungo, et al., Phys. Rev. B 87 (2013) 054431]. Due to the superlattice structure of the spin lattice, the substituted compound possesses multiple spin wave modes. The spin wave analysis confirms the quasi-1D nature of the substituted system.

  8. Glass-like recovery of antiferromagnetic spin ordering in a photo-excited manganite Pr0.7Ca0.3MnO3

    Energy Technology Data Exchange (ETDEWEB)

    Zhou, S. Y.; Langner, M. C.; Zhu, Y.; Chuang, Y. -D.; Rini, M.; Glover, T. E.; Hertlein, M. P.; Gonzalez, A.G. Cruz; Tahir, N.; Tomioka, Y.; Tokura, Y.; Hussain, Z.; Schoenlein, R. W.

    2014-01-16

    Electronic orderings of charges, orbitals and spins are observed in many strongly correlated electron materials, and revealing their dynamics is a critical step toward understanding the underlying physics of important emergent phenomena. Here we use time-resolved resonant soft x-ray scattering spectroscopy to probe the dynamics of antiferromagnetic spin ordering in the manganite Pr0:7Ca0:3MnO3 following ultrafast photo-exitation. Our studies reveal a glass-like recovery of the spin ordering and a crossover in the dimensionality of the restoring interaction from quasi-1D at low pump fluence to 3D at high pump fluence. This behavior arises from the metastable state created by photo-excitation, a state characterized by spin disordered metallic droplets within the larger charge- and spin-ordered insulating domains. Comparison with time-resolved resistivity measurements suggests that the collapse of spin ordering is correlated with the insulator-to-metal transition, but the recovery of the insulating phase does not depend on the re-establishment of the spin ordering.

  9. Finite-dimensional colored fluctuation-dissipation theorem for spin systems

    Science.gov (United States)

    Nicolis, Stam; Thibaudeau, Pascal; Tranchida, Julien

    2017-05-01

    When nano-magnets are coupled to random external sources, their magnetization becomes a random variable, whose properties are defined by an induced probability density, that can be reconstructed from its moments, using the Langevin equation, for mapping the noise to the dynamical degrees of freedom. When the spin dynamics is discretized in time, a general fluctuation-dissipation theorem, valid for non-Markovian noise, can be established, even when zero modes are present. We discuss the subtleties that arise, when Gilbert damping is present and the mapping between noise and spin degrees of freedom is non-linear.

  10. Study on spin and charge fluctuations in {tau} -type organic conductor

    Energy Technology Data Exchange (ETDEWEB)

    Aizawa, Hirohito [Institute of Physics, Kanagawa University, Yokohama 221-8686 (Japan); Kuroki, Kazuhiko [Department of Engineering Science, The University of Electro-Communications, Chofu, Tokyo 182-8585 (Japan)

    2012-05-15

    We theoretically study the possibility of the ferromagnetic behavior in a quasi-two-dimensional organic conductor, {tau} -(EDO-S,S -DMEDT-TTF){sub 2}(AuBr{sub 2}){sub 1+y} with y {approx} 0.875. We adopt a two-band extended Hubbard model, whose band dispersion nicely reproduces the ab initio band structure. We consider both on-site and nearest neighbor off-site repulsive interactions. By applying the random phase approximation, we find that both spin and charge susceptibilities are maximized at Q = (0, 0). Although this can be an indication of pure antiferromagnetism since two sites are present in a unit cell, the divergence of the susceptibilities at the origin of the k -space can also be related to the ferromagnetic behavior observed in this organic conductor. (copyright 2012 WILEY-VCH Verlag GmbH and Co. KGaA, Weinheim) (orig.)

  11. Magnetotransport evidence for irreversible spin reorientation in the collinear antiferromagnetic state of underdoped Nd2 -xCexCuO4

    Science.gov (United States)

    Dorantes, A.; Alshemi, A.; Huang, Z.; Erb, A.; Helm, T.; Kartsovnik, M. V.

    2018-02-01

    We make use of the strong spin-charge coupling in the electron-doped cuprate Nd2 -xCexCuO4 to probe changes in its spin system via magnetotransport measurements. We present a detailed study of the out-of-plane magnetoresistance in underdoped single crystals of this compound, including the nonsuperconducting, 0.05 ≤x ≤0.115 , and superconducting, 0.12 ≤x ≤0.13 , compositions. Special focus is put on the dependence of the magnetoresistance on the field orientation in the plane of the CuO2 layers. In addition to the kink at the field-induced transition between the noncollinear and collinear antiferromagnetic configurations, a sharp irreversible feature is found in the angle-dependent magnetoresistance of all samples in the high-field regime, at field orientations around the Cu-O-Cu direction. The obtained behavior can be explained in terms of field-induced reorientation of Cu2 + spins within the collinear antiferromagnetic state. It is therefore considered an unambiguous indication of the long-range magnetic order.

  12. Universal scaling of Néel temperature, staggered magnetization density, and spin-wave velocity of three-dimensional disordered and clean quantum antiferromagnets

    Science.gov (United States)

    Tan, D.-R.; Jiang, F.-J.

    2017-02-01

    The Néel temperature, staggered magnetization density, as well as the spin-wave velocity of a three-dimensional (3D) quantum Heisenberg model with antiferromagnetic disorder (randomness) are calculated using first-principles nonperturbative quantum Monte Carlo simulations. In particular, we examine the validity of universal scaling relations that are related to these three studied physical quantities. These relations are relevant to experimental data and are firmly established for clean (regular) 3D dimerized spin-1/2 Heisenberg models. Remarkably, our numerical results show that the considered scaling relations remain true for the investigated model with the introduced disorder. In addition, while the presence of disorder may change the physical properties of regular dimerized models, hence leading to different critical theories, both the obtained data of Néel temperature and staggered magnetization density in our study are fully compatible with the expected critical behavior for clean dimerized systems. As a result, it is persuasive to conclude that the related quantum phase transitions of the considered disordered model and its clean analogues are governed by the same critical theory, which is not always the case in general. Finally, we also find smooth scaling curves even emerging when both the data of the investigated disordered model as well as its associated clean system are taken into account concurrently. This in turn implies that, while in a restricted sense, the considered scaling relations for 3D spin-1/2 antiferromagnets are indeed universal.

  13. Magnetic phase diagram and multiferroicity of Ba3MnNb2O9: A spin-5/2 triangular lattice antiferromagnet with weak easy-axis anisotropy

    Science.gov (United States)

    Lee, M.; Choi, E. S.; Huang, X.; Ma, J.; Dela Cruz, C. R.; Matsuda, M.; Tian, W.; Dun, Z. L.; Dong, S.; Zhou, H. D.

    2015-03-01

    We have performed magnetic, electric, thermal, and neutron powder diffraction (NPD) experiments as well as density functional theory (DFT) calculations on Ba3MnNb2O9. All results suggest that Ba3MnNb2O9 is a spin-5/2 triangular lattice antiferromagnet (TLAF) with weak easy-axis anisotropy. At zero field, we observed a narrow two-step transition at TN 1 = 3.4 K and TN 2 = 3.0 K. The neutron diffraction measurement and the DFT calculation indicate a 120° spin structure in the ab plane with out-of-plane canting at low temperatures. With increasing magnetic field, the 120° spin structure evolves into up-up-down (uud) and oblique phase showing successive magnetic phase transitions, which fits well to the theoretical prediction for the 2D Heisenberg TLAF with classical spins. Multiferroicity is observed when the spins are not collinear but suppressed in the uud and the oblique phase. We discuss the results in comparison with our previous works on its sister compounds with small spins, Ba3NiNb2O9 (S = 1) (J. Hwang et al ., Phys. Rev. Lett. 109, 257205 (2012) and Ba3CoNb2O9 (S = 1/2) (M. Lee et al ., Phys. Rev. B 89, 104420 (2014)). NHMFL is supported by NSF, the state of Florida and US DOE. ORNL HFIR was sponsored by U.S. DOE.

  14. Surface and step dynamics of a semi-infinite insulating antiferromagnet system

    CERN Document Server

    Tamine, M

    2003-01-01

    We have carried out a theoretical study of the localized spin-wave modes near the surface step of the insulating Heisenberg antiferromagnet. In this work, we study the full magnetic problem arising from the absence of translational symmetry due to the presence of a magnetic surface and step. The calculation concerns in particular the spin fluctuation dynamics and employs the matching procedure in the random-phase approximation. Only the nearest neighbours exchange interactions are considered between the spins in the model. The analytical formalism presented here determines the bulk and evanescent spin fluctuation fields in the two-dimensional plane normal to the surface and step regions. The results are used to calculate the localized modes of magnons associated with the step and surface terraces. The present model may be generalized to treat the spin fluctuations dynamics of other extended surface imperfections or nanostructures, provided they preserve the translation symmetry of the ordered spins along a di...

  15. Classification for the universal scaling of Néel temperature and staggered magnetization density of three-dimensional dimerized spin-1/2 antiferromagnets

    Science.gov (United States)

    Tan, D.-R.; Li, C.-D.; Jiang, F.-J.

    2018-03-01

    Inspired by the recent theoretical development relevant to the experimental data of TlCuCl3, particularly those associated with the universal scaling between the Néel temperature TN and the staggered magnetization density Ms, we carry out a detailed investigation of three-dimensional (3D) dimerized quantum antiferromagnets using the first-principles quantum Monte Carlo calculations. Through this study we wish to better understand the microscopic effects on these scaling relations of TN and Ms, hence to shed light on some of the observed inconsistency between the theoretical and the experimental results. Remarkably, for the considered 3D dimerized models, we find that the established universal scaling relations are not only valid, but can each be categorized within its kind by the amount of stronger antiferromagnetic couplings connected to each spin. Convincing numerical evidence is provided to support the validity of this classification scheme. Based on all the related results known in the literature, we further argue that the proposed categorization for the universal scaling investigated in our paper should be applicable for 3D dimerized spin systems with (certain kinds of) quenched disorder and (or) on lattice geometries other than those considered here. The relevance of the outcomes presented in this investigation to the experiments of TlCuCl3 is briefly discussed as well.

  16. Magnetic phase diagrams of classical triangular and kagome antiferromagnets

    Energy Technology Data Exchange (ETDEWEB)

    Gvozdikova, M V [Department of Physics, Kharkov National University, 61077 Kharkov (Ukraine); Melchy, P-E; Zhitomirsky, M E, E-mail: mike.zhitomirsky@cea.fr [Service de Physique Statistique, Magnetisme et Supraconductivite, UMR-E9001 CEA-INAC/UJF, 17 rue des Martyrs, 38054 Grenoble (France)

    2011-04-27

    We investigate the effect of geometrical frustration on the H-T phase diagrams of the classical Heisenberg antiferromagnets on triangular and kagome lattices. The phase diagrams for the two models are obtained from large-scale Monte Carlo simulations. For the kagome antiferromagnet, thermal fluctuations are unable to lift degeneracy completely and stabilize translationally disordered multipolar phases. We find a substantial difference in the temperature scales of the order by disorder effect related to different degeneracy of the low- and the high-field classical ground states in the kagome antiferromagnet. In the low-field regime, the Kosterlitz-Thouless transition into a spin-nematic phase is produced by unbinding of half-quantum vortices.

  17. Does long-range antiferromagnetism help or inhibit superconductivity?

    Science.gov (United States)

    Arrachea, Liliana; Aligia, A. A.

    1998-07-01

    We analyze the possible existence of a superconducting state in a background with long-range antiferromagnetism. We consider a generalized Hubbard model with nearest-neighbor correlated hopping in a square lattice. Near half filling, the model exhibits a d-wave-Bardeen-Cooper-Schrieffer (BCS) solution in the paramagnetic state. The superconducting solution would be enhanced by the antiferromagnetic background if the contribution of triplet pairs with d-wave symmetry and total momentum ( π, π) could be neglected. However, we find that due to their contribution, the coexistence of superconductivity and long-range antiferromagnetism is ruled out for large values of the Coulomb repulsion U. Spin-density wave fluctuations (SDWF) do not change this result.

  18. Anisotropic spin fluctuations in heavy-fermion superconductor CeCoIn sub 5. In-NQR and Co-NMR studies

    CERN Document Server

    Kawasaki, Y; Yashima, M

    2003-01-01

    We report In-NQR and Co-NMR experiments of CeCoIn sub 5 that undergoes a superconducting transition with a record high T sub c =2.3 K to date among heavy-fermion superconductors. At zero magnetic field, an anomalous temperature (T) dependence of nuclear spin-lattice relaxation rate 1/T sub 1 of sup 1 sup 1 sup 5 In is explained by the relation 1/T sub 1 propor to T centre dot chi sub Q (T) sup 3 sup / sup 4 based on the anisotropic spin-fluctuations model in case of the proximity to an antiferromagnetic (AFM) quantum critical point (QCP). The novel behavior of 1/T sub 1 - T sup 1 sup / sup 4 over a wide T range of T sub c < T < 40 K arises because the staggered susceptibility almost follows the Curie law chi sub Q (T) propor to 1/(T + theta) with theta=0.6 K and hence 1/T sub 1 propor to T/(T + 0.6) sup 3 sup / sup 4 - T sup 1 sup / sup 4 for theta < T. We highlight that the behavior 1/T sub 1 - T sup 1 sup / sup 4 is due to the proximity to the anisotropic AFM QCP relevant with its layered structure...

  19. Zitterbewegung with spin-orbit coupled ultracold atoms in a fluctuating optical lattice

    Science.gov (United States)

    Argonov, V. Yu; Makarov, D. V.

    2016-09-01

    The dynamics of non-interacting ultracold atoms with artificial spin-orbit coupling is considered. Spin-orbit coupling is created using two moving optical lattices with orthogonal polarizations. Our main goal is to study influence of lattice noise on Rabi oscillations. Special attention is paid to the phenomenon of the Zitterbewegung being trembling motion caused by Rabi transitions between states with different velocities. Phase and amplitude fluctuations of lattices are modelled by means of the two-dimensional stochastic Ornstein-Uhlenbeck process, also known as harmonic noise. In the the noiseless case the problem is solved analytically in terms of the momentum representation. It is shown that lattice noise significantly extends duration of the Zitterbewegung as compared to the noiseless case. This effect originates from noise-induced decoherence of Rabi oscillations.

  20. Superconductivity and spin fluctuations in M-Zr metallic glasses (M = Cu, Ni, Co, and Fe)

    International Nuclear Information System (INIS)

    Altounian, Z.; Strom-Olsen, J.O.

    1983-01-01

    The superconducting transition temperature, upper critical field, and magnetic susceptibility have been measured in four binary metallic glass systems: Cu-Zr, Ni-Zr, Co-Zr, and Fe-Zr. For each alloy system, a full and continuous range of Zr-rich compositions accessible by melt spinning has been examined. For Cu-Zr, the range is 0.75>x>0.30; for Ni-Zr, 0.80>x>0.30; for Co-Zr, 0.80>x>0.48, and for Fe-Zr, 0.80>x>0.55 (x being the concentration of Zr in at. %). The results show clearly the influence of spin fluctuations in reducing the superconducting transition temperature. The data have been successfully analyzed using a modified form of the McMillan equation together with expressions for the Stoner enhanced magnetic susceptibility and the Ginsburg-Landau-Abrikosov-Gor'kov expression for the upper critical field

  1. Short-range order above the Curie temperature in the dynamic spin-fluctuation theory

    International Nuclear Information System (INIS)

    Melnikov, N.B.; Reser, B.I.

    2016-01-01

    Based on the dynamic spin-fluctuation theory, we study the spin-density correlations in the ferromagnetic metals. We obtain computational formulae for the correlation function and correlation radius in different approximations of the theory. Using these formulae, we calculate the magnetic short-range order above the Curie temperature in bcc Fe. Results of the calculation confirm our theoretical prediction that the inverse correlation radius increases linearly with temperature for T sufficiently large. The calculated short-range order is small but sufficient to correctly describe neutron scattering experiments. A considerable amount of the short-range order is shown to persist up to temperatures much higher than the Curie temperature. - Highlights: • We study the spin correlations in ferromagnetic metals above the Curie temperature. • We derive computational formulae for the spin correlator and correlation radius. • The correlation radius decreases inversely with temperature over a wide interval. • The calculated short-range order in Fe is small, in agreement with experiment. • A considerable amount of short-range order in Fe persists up to high temperatures.

  2. Two spin-canting textures in the antiferromagnetic phase AF1 of MnWO4 based on the new polar atomistic model in P2

    Science.gov (United States)

    Park, S.-H.; Liu, B.-Q.; Behal, D.; Pedersen, B.; Schneidewind, A.

    2018-04-01

    The low temperature antiferromagnetic (AF) phase of MnWO4 (the so-called AF1 phase) exhibits different spin-canting configurations at two Mn2+ sublattices of the (3  +  1)-dimensional magnetic structure. The suggested superspace group {{\\boldsymbol P}}2.1^\\prime(α, 1/2, γ)0s is a significant consequence of the polar space group {{\\boldsymbol P}} 2 true for the nuclear structure of MnWO4. Density functional theory calculations showed that its ground state prefers this two spin-canting system. The structural difference between two independent atomic sites for Mn (Mn a , Mn b ) is too small to allow microscopically detectable electric polarisation. However, this hidden intrinsic polar character allows AF1 two commensurately modulated spin-canting textures. This is considered as the prerequisite onset of the improper ferroelectricity enhanced by the helical spin order in the multiferroic phase AF2 of MnWO4.

  3. Focused issue on antiferromagnetic spintronics: An overview (Part of a collection of reviews on antiferromagnetic spintronics)

    KAUST Repository

    Jungwirth, T.

    2017-05-30

    This focused issue attempts to provide a comprehensive introduction into the field of antiferromagnetic spintronics. Apart from the brief overview below, it features five review articles. The intention is to cover in a coherent and complementary way key physical aspects of the antiferromagnetic spintronics research. These range from microelectronic memory devices and optical manipulation and detection of antiferromagnetic spins, to the fundamentals of antiferromagnetic dynamics in uniform or spin-textured systems, and to the interplay of antiferromagnetic spintronics with topological phenomena. The antiferromagnetic ordering can take a number of forms including fully compensated collinear, non-collinear, and non-coplanar magnetic lattices, compensated and uncompensated ferrimagnets, or metamagnetic materials hosting an antiferromagnetic to ferromagnetic phase transition. Apart from the variety of distinct magnetic crystal structures, the focused issue also encompasses spintronic phenomena and devices studied in antiferromagnet/ferromagnet heterostructures and in synthetic antiferromagnets.

  4. Magnetic fluctuations in UNi4B

    DEFF Research Database (Denmark)

    Mentink, S.A.M.; Mason, T.E.; Buyers, W.J.L.

    1997-01-01

    We investigate the magnetic fluctuation spectrum of the geometrically frustrated antiferromagnetic compound UNi4B, which partially orders below T-N = 20 K. An overdamped spin excitation is observed at the AF wave vector around 2.4 meV. Low-frequency, weakly Q-dependent inelastic scattering...

  5. Stable magnetic remanence in antiferromagnetic goethite.

    Science.gov (United States)

    Strangway, D W; McMahon, B E; Honea, R M

    1967-11-10

    Goethite, known to be antiferromagnetic, acquires thermoremanent magnetization at its Neel temperature of 120 degrees C. This remanence, extremely stable, is due to the presence of unbalanced spins in the antiferromagnetic structure; the spins may result from grain size, imperfections, or impurities.

  6. Properties of spin-1/2 triangular-lattice antiferromagnets CuY2Ge2O8 and CuLa2Ge2O8

    Science.gov (United States)

    Cho, Hwanbeom; Kratochvílová, Marie; Sim, Hasung; Choi, Ki-Young; Kim, Choong Hyun; Paulsen, Carley; Avdeev, Maxim; Peets, Darren C.; Jo, Younghun; Lee, Sanghyun; Noda, Yukio; Lawler, Michael J.; Park, Je-Geun

    2017-04-01

    We found new two-dimensional (2D) quantum (S =1 /2 ) antiferromagnetic systems: Cu R E2G e2O8 (R E =Y and La). According to our analysis of high-resolution x-ray and neutron diffraction experiments, the Cu network of Cu R E2G e2O8 (R E =Y and La) exhibits a 2D triangular lattice linked via weak bonds along the perpendicular b axis. Our bulk characterizations from 0.08 to 400 K show that they undergo a long-range order at 0.51(1) and 1.09(4) K for the Y and La systems, respectively. Interestingly, they also exhibit field induced phase transitions. For theoretical understanding, we carried out the density functional theory (DFT) band calculations to find that they are typical charge-transfer-type insulators with a gap of Eg≅2 eV . Taken together, our observations make Cu R E2G e2O8 (R E =Y and La) additional examples of low-dimensional quantum spin triangular antiferromagnets with the low-temperature magnetic ordering.

  7. The spinning dancer illusion and spontaneous brain fluctuations: an fMRI study.

    Science.gov (United States)

    Bernal, Byron; Guillen, Magno; Marquez, Juan Camilo

    2014-01-01

    The brain activation associated with the Spinning Dancer Illusion, a cognitive visual illusion, is not entirely known. Inferences from other study modalities point to the involvement of the dorso-parieto-occipital areas in the spontaneous switchings of perception in other bistable non-kinetic illusions. fMRI is a mature technique used to investigate the brain responses associated with mental changes. Resting-state fMRI is a novel technique that may help ascertain the effects of spontaneous brain changes in the top-down regulation of visual perception. The purpose of this report is to describe the brain activation associated with the subjective illusory changes of perception of a kinetic bistable stimulus. We hypothesize that there is a relationship between the perception phases with the very slow cortical spontaneous fluctuations, recently described. A single normal subject who was trained to produce voluntarily perception phase switches underwent a series of fMRI studies whose blocks were either defined post-hoc or accordingly with a predefined timeline to assess spontaneous and voluntarily evoked visual perception switches, respectively. Correlation of findings with resting-state fMRI and independent component analysis of the task series was sought. Phases of the rotation direction were found associated with right parietal activity. Independent component analysis of the task series and their comparison with basal resting-state components suggest that this activity is related to one of the very slow spontaneous brain fluctuations. The spontaneous fluctuations of the cortical activity may explain the subjective changes in perception of direction of the Spinning Dancer Illusion. This observation is a proof-of-principle, suggesting that the spontaneous brain oscillations may influence top-down sensory regulation.

  8. Performance comparison of dynamical decoupling sequences for a qubit in a rapidly fluctuating spin bath

    International Nuclear Information System (INIS)

    Alvarez, Gonzalo A.; Suter, Dieter; Ajoy, Ashok; Peng Xinhua

    2010-01-01

    Avoiding the loss of coherence of quantum mechanical states is an important prerequisite for quantum information processing. Dynamical decoupling (DD) is one of the most effective experimental methods for maintaining coherence, especially when one can access only the qubit system and not its environment (bath). It involves the application of pulses to the system whose net effect is a reversal of the system-environment interaction. In any real system, however, the environment is not static, and therefore the reversal of the system-environment interaction becomes imperfect if the spacing between refocusing pulses becomes comparable to or longer than the correlation time of the environment. The efficiency of the refocusing improves therefore if the spacing between the pulses is reduced. Here, we quantify the efficiency of different DD sequences in preserving different quantum states. We use 13 C nuclear spins as qubits and an environment of 1 H nuclear spins as the environment, which couples to the qubit via magnetic dipole-dipole couplings. Strong dipole-dipole couplings between the proton spins result in a rapidly fluctuating environment with a correlation time of the order of 100 μs. Our experimental results show that short delays between the pulses yield better performance if they are compared with the bath correlation time. However, as the pulse spacing becomes shorter than the bath correlation time, an optimum is reached. For even shorter delays, the pulse imperfections dominate over the decoherence losses and cause the quantum state to decay.

  9. NMR on the antiferromagnetic S=1/2 Heisenberg spin chain Sr{sub 2}CuO{sub 3} under the impact of Ni impurities

    Energy Technology Data Exchange (ETDEWEB)

    Utz, Yannic; Hammerath, Franziska; Nishimoto, Satoshi; Drechsler, Stefan-Ludwig; Hess, Christian; Buechner, Bernd; Grafe, Hans-Joachim [IFW Dresden (Germany); Beesetty, Neela Sekhar; Saint-Martin, Romuald; Revcolevschi, Alexandre [SP2M-ICMMO UMR-CNRS, Universite Paris-Sud (France)

    2015-07-01

    We present {sup 63}Cu NMR measurements on single crystals of Sr{sub 2}CuO{sub 3} doped with different amounts of nickel and compare them to numerical DMRG results. The parent compound contains copper-oxygen chains with S=1/2 on the copper site coupled by a large antiferromagnetic exchange coupling J ∼ 2000 K and is known to be a good realization of the 1D Heisenberg model. The measurements show that replacing only a few of the S=1/2 Cu ions with S=1 Ni has a major impact on the magnetic properties of the spin chain system. An unusual line broadening in the low temperature NMR spectra reveals the existence of an impurity-induced local alternating magnetization (LAM), and exponentially decaying spin-lattice relaxation rates T{sup -1}{sub 1} towards low temperatures indicate the opening of a spin gap similar to Ca-doped Sr{sub 2}CuO{sub 3}. While the T{sup -1}{sub 1} measurements could be explained by pure chain segmentation, as expected for a S=0 impurity, the spectra can only be understood by taking the nickel.

  10. Zn and Ni substitutional effects on spin fluctuations in YBa sub 2 Cu sub 3 O sub 7 by sup 6 sup 3 sup , sup 6 sup 5 Cu NQR

    CERN Document Server

    Han, K S; Mean, B J; Lee, K H; Seo, S W; Lee, M H; Lee, W C

    2000-01-01

    We have prepared Zn- and Ni-substituted YBa sub 2 Cu sub 3 O sub 7 (YBa sub 2 Cu sub 3 sub - sub x M sub x O sub 7 , M=Zn or Ni, x=0.00 approx 0.09) and performed sup 6 sup 3 sup , sup 6 sup 5 Cu nuclear quadrupole resonance (NQR) measurements for the plane site at 300 and 100 K. Substitutional effects on the relaxation rates are markedly different. Both the spin-lattice and the spin-spin relaxation rates decrease for Zn-doped YBCO. However, those increase for Ni-doped YBCO. This contrast in local electronic dynamics provides clear microscopic evidence that Zn forms no local moment while Ni develops a local moment. Consequently, the antiferromagnetic spin fluctuation is suppressed by Zn doping whereas it is preserved by Ni doping. This is also confirmed by the ratio of the sup 6 sup 3 sup , sup 6 sup 5 Cu spin-lattice relaxation rates for the plane coppers.

  11. Low-energy spin fluctuations in the non-Fermi-liquid compound YbRh2Si2

    Directory of Open Access Journals (Sweden)

    O. Stockert et al

    2007-01-01

    Full Text Available We report on inelastic neutron scattering experiments on YbRh2Si2 powder to study the low-energy spin dynamics at temperatures between T=0.8 and 22 K. The low-energy magnetic response is quasielastic. However, it exhibits an unusual form not modelled by a simple relaxation rate yielding a Lorentzian lineshape, but can satisfactorily be described by a phenomenological model involving a distribution of relaxation rates. The lower bound of the relaxation rates varies roughly linear with temperature indicating a pronounced slowing down of the critical modes above the antiferromagnetic ordering temperature TNapprox70 mK.

  12. Spin disorder and order in quasi-2D triangular Heisenberg antiferromagnets: comparative study of FeGa2S4, Fe2Ga2S5, and NiGa2S4.

    Science.gov (United States)

    Nakatsuji, S; Tonomura, H; Onuma, K; Nambu, Y; Sakai, O; Maeno, Y; Macaluso, R T; Chan, Julia Y

    2007-10-12

    Our single crystal study reveals that the single-layer S=2 triangular Heisenberg antiferromagnet FeGa2S4 forms a frozen spin-disordered state, similar to the S=1 isostructural magnet NiGa2S4. In this state, the magnetic specific heat C{M} is not only insensitive to the field, but shows a T2 dependence that scales to C{M} of NiGa2S4, suggesting the same underlying mechanism of the 2D coherent behavior. In contrast, the bilayer system Fe2Ga2S5 exhibits a 3D antiferromagnetic order.

  13. Reduced interface spin polarization by antiferromagnetically coupled Mn segregated to the C o2MnSi /GaAs (001) interface

    Science.gov (United States)

    Rath, Ashutosh; Sivakumar, Chockalingam; Sun, C.; Patel, Sahil J.; Jeong, Jong Seok; Feng, J.; Stecklein, G.; Crowell, Paul A.; Palmstrøm, Chris J.; Butler, William H.; Voyles, Paul M.

    2018-01-01

    We have investigated the interfacial structure and its correlation with the calculated spin polarization in C o2MnSi /GaAs(001) lateral spin valves. C o2MnSi (CMS) films were grown on As-terminated c(4 ×4 ) GaAs(100) by molecular beam epitaxy using different first atomic layers: MnSi, Co, and Mn. Atomically resolved Z -contrast scanning transmission electron microscopy (STEM) imaging and electron energy loss spectroscopy (EELS) were used to develop atomic structural models of the CMS/GaAs interfaces that were used as inputs for first-principles calculations to understand the magnetic and electronic properties of the interface. First-principles structures were relaxed and then validated by comparing experimental and simulated high-resolution STEM images. STEM-EELS results show that all three films have similar six atomic layer thick, Mn- and As-rich multilayer interfaces. However, the Co-initiated interface contains a M n2As -like layer, which is antiferromagnetic, and which is not present in the other two interfaces. Density functional theory calculations show a higher degree of interface spin polarization in the Mn- and MnSi-initiated cases, compared to the Co-initiated case, although none of the interfaces are half-metallic. The loss of half-metallicity is attributed, at least in part, to the segregation of Mn at the interface, which leads to the formation of interface states. The implications for the performance of lateral spin valves based on these interfaces are discussed briefly.

  14. Nonlinear spin fluctuations in the Fermi liquid of itinerant electron ferromagnets

    International Nuclear Information System (INIS)

    Solontsov, A.; Lacroix, C.

    2003-01-01

    A microscopic derivation of nonlinear equations of magnetic dynamics for itinerant ferromagnets is presented within the electron Fermi liquid model accounting for both long-range Coulomb and short-range interactions of quasiparticles, which founds the basis for the phenomenological description of nonlinear spin fluctuations (SF) using the Ginsburg-Landau formalism. Crystal lattice is shown to play a significant role screening the long-range Coulomb interaction and affecting magnetic dynamics. The spectrum of longitudinal SF with account of nonlinear mode-mode coupling is shown to result from an interplay of quasielastic SF and inelastic excitations near the magnon frequencies, both having mainly the nonlinear nature and arising due to their emission (absorption) by magnons

  15. Phenomenological approach to spin fluctuations in itinerant magnets and superconductors from ab initio calculations

    Energy Technology Data Exchange (ETDEWEB)

    Ortenzi, Luciano

    2013-10-17

    In this thesis I study the interplay between magnetism and superconductivity in itinerant magnets and superconductors. I do this by applying a semiphenomenological method to four representative compounds. In particular I use the discrepancies (whenever present) between density functional theory (DFT) calculations and the experiments in order to construct phenomenological models which explain the magnetic, superconducting and optical properties of four representative systems. I focus my attention on the superconducting and normal state properties of the recently discovered APt3P superconductors, on superconducting hole-doped CuBiSO, on the optical properties of LaFePO and finally on the ferromagnetic-paramagnetic transition of Ni3Al under pressure. At the end I present a new method which aims to describe the effect of spin fluctuations in itinerant magnets and superconductors that can be used to monitor the evolution of the electronic structure from non magnetic to magnetic in systems close to a quantum critical point.

  16. Pressure dependence of critical temperature of bulk FeSe from spin fluctuation theory

    Science.gov (United States)

    Hirschfeld, Peter; Kreisel, Andreas; Wang, Yan; Tomic, Milan; Jeschke, Harald; Jacko, Anthony; Valenti, Roser; Maier, Thomas; Scalapino, Douglas

    2013-03-01

    The critical temperature of the 8K superconductor FeSe is extremely sensitive to pressure, rising to a maximum of 40K at about 10GPa. We test the ability of the current generation of fluctuation exchange pairing theories to account for this effect, by downfolding the density functional theory electronic structure for each pressure to a tight binding model. The Fermi surface found in such a procedure is then used with fixed Hubbard parameters to determine the pairing strength using the random phase approximation for the spin singlet pairing vertex. We find that the evolution of the Fermi surface captured by such an approach is alone not sufficient to explain the observed pressure dependence, and discuss alternative approaches. PJH, YW, AK were supported by DOE DE-FG02-05ER46236, the financial support of MT, HJ, and RV from the DFG Schwerpunktprogramm 1458 is kindly acknowledged.

  17. Critical slowing down of spin fluctuations in BiFeO3

    International Nuclear Information System (INIS)

    Scott, J F; Singh, M K; Katiyar, R S

    2008-01-01

    In earlier work we reported the discovery of phase transitions in BiFeO 3 evidenced by divergences in the magnon light-scattering cross-sections at 140 and 201 K (Singh et al 2008 J. Phys.: Condens. Matter 20 252203) and fitted these intensity data to critical exponents α = 0.06 and α' = 0.10 (Scott et al 2008 J. Phys.: Condens. Matter 20 322203), under the assumption that the transitions are strongly magnetoelastic (Redfern et al 2008 at press) and couple to strain divergences through the Pippard relationship (Pippard 1956 Phil. Mag. 1 473). In the present paper we extend those criticality studies to examine the magnon linewidths, which exhibit critical slowing down (and hence linewidth narrowing) of spin fluctuations. The linewidth data near the two transitions are qualitatively different and we cannot reliably extract a critical exponent ν, although the mean field value ν = 1/2 gives a good fit near the lower transition.

  18. Static and dynamic spin fluctuations in the spin glass doping regime in La2-xSrxCuO4+y

    International Nuclear Information System (INIS)

    Birgeneau, R.J.; Belk, N.; Kastner, M.A.; Keimer, B.; Shirane, G.

    1991-01-01

    We review the results of neutron scattering studies of the static and dynamic spin fluctuations crystals of La 2-x Sr x CuO 4+δ in the doping regime intermediate between the Neel and superconducting regions. In this regime the in-plane resistance is linear in temperature down to ∼80 K with a crossover due to logarithmic conductance effects at lower temperatures. The static spin correlations are well-described by a simple model in which the inverse correlation length κ(x,T) =κ(x,0) + κ(0,T). The most dramatic new result is the discovery by Keimer et al. that the dynamic spin fluctuations exhibit a temperature dependence which is a simple function of ω/T for temperatures 10 K≤T≤500 K for a wide range of energies. This scaling leads to a natural explanation of a variety of normal state properties of the copper oxides. 21 refs., 4 figs

  19. Numerical study of the enlarged O(5) symmetry of the 3D antiferromagnetic RP2 spin model

    International Nuclear Information System (INIS)

    Fernandez, L.A.; Martin-Mayor, V.; Sciretti, D.; Tarancon, A.; Velasco, J.L.

    2005-01-01

    We investigate by means of Monte Carlo simulation and finite-size scaling analysis the critical properties of the three-dimensional O(5) non-linear σ model and of the antiferromagnetic RP 2 model, both of them regularized on a lattice. High accuracy estimates are obtained for the critical exponents, universal dimensionless quantities and critical couplings. It is concluded that both models belong to the same universality class, provided that rather non-standard identifications are made for the momentum-space propagator of the RP 2 model. We have also investigated the phase diagram of the RP 2 model extended by a second-neighbor interaction. A rich phase diagram is found, where most of the phase transitions are of the first order

  20. Neutron Inelastic Scattering Study of Transverse Spin Fluctuations in CsNiF3: a Soliton-only Central Peak

    DEFF Research Database (Denmark)

    Steiner, M.; Kakurai, K.; Knop, W.

    1982-01-01

    We have observed a quasi-elastic contribution to the spectrum of the transverse spin fluctuations Sperp;(Q, ω), perpendicular to an applied magnetic field in the easy plane of the one-dimensional ferromagnet CsNiF3. According to the present theoretical understanding this contribution is due solely...

  1. High-order study of the quantum critical behavior of a frustrated spin-1/2 antiferromagnet on a stacked honeycomb bilayer

    Science.gov (United States)

    Bishop, R. F.; Li, P. H. Y.

    2017-12-01

    We study a frustrated spin-1/2 J1-J2-J3-J1⊥ Heisenberg antiferromagnet on an A A -stacked bilayer honeycomb lattice. In each layer we consider nearest-neighbor (NN), next-nearest-neighbor, and next-next-nearest-neighbor antiferromagnetic (AFM) exchange couplings J1,J2 , and J3, respectively. The two layers are coupled with an AFM NN exchange coupling J1⊥≡δ J1 . The model is studied for arbitrary values of δ along the line J3=J2≡α J1 that includes the most highly frustrated point at α =1/2 , where the classical ground state is macroscopically degenerate. The coupled cluster method is used at high orders of approximation to calculate the magnetic order parameter and the triplet spin gap. We are thereby able to give an accurate description of the quantum phase diagram of the model in the α δ plane in the window 0 ≤α ≤1 ,0 ≤δ ≤1 . This includes two AFM phases with Néel and striped order, and an intermediate gapped paramagnetic phase that exhibits various forms of valence-bond crystalline order. We obtain accurate estimations of the two phase boundaries, δ =δci(α) , or equivalently, α =αc i(δ ) , with i =1 (Néel) and 2 (striped). The two boundaries exhibit an "avoided crossing" behavior with both curves being re-entrant. Thus, in this α δ window, Néel order exists only for values of δ in the range δc1 (α ) , with δc1 0 for αc 1(0 ) ≈0.49 (1 ) , and striped order similarly exists only for values of δ in the range δc2 (α ) , with δc2 αc2(0) ≈0.600 (5 ) and δc2 0 for αc 2(0 ) >α >α2<≈0.56 (1 ) .

  2. Elastic properties of paramagnetic austenitic steel at finite temperature: Longitudinal spin fluctuations in multicomponent alloys

    Science.gov (United States)

    Dong, Zhihua; Schönecker, Stephan; Chen, Dengfu; Li, Wei; Long, Mujun; Vitos, Levente

    2017-11-01

    We propose a first-principles framework for longitudinal spin fluctuations (LSFs) in disordered paramagnetic (PM) multicomponent alloy systems and apply it to investigate the influence of LSFs on the temperature dependence of two elastic constants of PM austenitic stainless steel Fe15Cr15Ni. The magnetic model considers individual fluctuating moments in a static PM medium with first-principles-derived LSF energetics in conjunction with describing chemical disorder and randomness of the transverse magnetic component in the single-site alloy formalism and disordered local moment (DLM) picture. A temperature-sensitive mean magnetic moment is adopted to accurately represent the LSF state in the elastic-constant calculations. We make evident that magnetic interactions between an LSF impurity and the PM medium are weak in the present steel alloy. This allows gaining accurate LSF energetics and mean magnetic moments already through a perturbation from the static DLM moments instead of a tedious self-consistent procedure. We find that LSFs systematically lower the cubic shear elastic constants c' and c44 by ˜6 GPa in the temperature interval 300-1600 K, whereas the predominant mechanism for the softening of both elastic constants with temperature is the magneto-volume coupling due to thermal lattice expansion. We find that non-negligible local magnetic moments of Cr and Ni are thermally induced by LSFs, but they exert only a small influence on the elastic properties. The proposed framework exhibits high flexibility in accurately accounting for finite-temperature magnetism and its impact on the mechanical properties of PM multicomponent alloys.

  3. Pairing versus phase coherence of doped holes in distinct quantum spin backgrounds

    Science.gov (United States)

    Zhu, Zheng; Sheng, D. N.; Weng, Zheng-Yu

    2018-03-01

    We examine the pairing structure of holes injected into two distinct spin backgrounds: a short-range antiferromagnetic phase versus a symmetry protected topological phase. Based on density matrix renormalization group (DMRG) simulation, we find that although there is a strong binding between two holes in both phases, phase fluctuations can significantly influence the pair-pair correlation depending on the spin-spin correlation in the background. Here the phase fluctuation is identified as an intrinsic string operator nonlocally controlled by the spins. We show that while the pairing amplitude is generally large, the coherent Cooper pairing can be substantially weakened by the phase fluctuation in the symmetry-protected topological phase, in contrast to the short-range antiferromagnetic phase. It provides an example of a non-BCS mechanism for pairing, in which the paring phase coherence is determined by the underlying spin state self-consistently, bearing an interesting resemblance to the pseudogap physics in the cuprate.

  4. Neutron spin-echo studies on dynamic and static fluctuations in two types of poly(vinyl alcohol) gels

    International Nuclear Information System (INIS)

    Kanaya, T.; Takahashi, N.; Nishida, K.; Seto, H.; Nagao, M.; Takeda, T.

    2005-01-01

    We report neutron spin-echo measurements on two types of poly(vinyl alcohol) (PVA) gels. The first is PVA gel in a mixture of dimethyl sulfoxide (DMSO) and water with volume ratio 60/40, and the second is PVA gel in an aqueous borax solution. The observed normalized intermediate scattering functions I(Q,t)/I(Q,0) are very different between them. The former I(Q,t)/I(Q,0) shows a nondecaying component in addition to a fast decay, but the latter does not have the nondecaying one. This clearly indicates that the fluctuations in the former PVA gel consist of static and dynamic fluctuations whereas the latter PVA gel does include only the dynamic fluctuations. The dynamic fluctuations of the former and latter gels have been analyzed in terms of a restricted motion in the network and Zimm motion, respectively, and the origins of these motions will be discussed

  5. Soft modes in the easy plane pyrochlore antiferromagnet

    International Nuclear Information System (INIS)

    Champion, J D M; Holdsworth, P C W

    2004-01-01

    Thermal fluctuations lift the high ground state degeneracy of the classical nearest neighbour pyrochlore antiferromagnet, with easy plane anisotropy, giving a first-order phase transition to a long range ordered state. We show, from spin wave analysis and numerical simulation, that even below this transition a continuous manifold of states, of dimension N 2/3 , exist (N is the number of degrees of freedom). As the temperature goes to zero a further 'order by disorder' selection is made from this manifold. The pyrochlore antiferromagnet Er 2 Ti 2 O 7 is believed to have an easy plane anisotropy and is reported to have the same magnetic structure. This is perhaps surprising, given that the dipole interaction lifts the degeneracy of the classical model in favour of a different structure. We interpret our results in the light of these facts

  6. Linearized Jastrow-style fluctuations on spin-projected Hartree-Fock.

    Science.gov (United States)

    Henderson, Thomas M; Scuseria, Gustavo E

    2013-12-21

    The accurate and efficient description of strong electronic correlations remains an important objective in electronic structure theory. Projected Hartree-Fock theory, where symmetries of the Hamiltonian are deliberately broken and projectively restored, all with a mean-field computational scaling, shows considerable promise in this regard. However, the method is neither size extensive nor size consistent; in other words, the correlation energy per particle beyond broken-symmetry mean field vanishes in the thermodynamic limit, and the dissociation limit of a molecule is not the sum of the fragment energies. These two problems are closely related. Recently, Neuscamman [Phys. Rev. Lett. 109, 203001 (2012)] has proposed a method to cure the lack of size consistency in the context of the antisymmetrized geminal power wave function (equivalent to number-projected Hartree-Fock-Bogoliubov) by using a Jastrow-type correlator in Hilbert space. Here, we apply the basic idea in the context of projected Hartree-Fock theory, linearizing the correlator for computational simplicity but extending it to include spin fluctuations. Results are presented for the Hubbard Hamiltonian and for some simple molecular systems.

  7. Linearized Jastrow-style fluctuations on spin-projected Hartree-Fock

    International Nuclear Information System (INIS)

    Henderson, Thomas M.; Scuseria, Gustavo E.

    2013-01-01

    The accurate and efficient description of strong electronic correlations remains an important objective in electronic structure theory. Projected Hartree-Fock theory, where symmetries of the Hamiltonian are deliberately broken and projectively restored, all with a mean-field computational scaling, shows considerable promise in this regard. However, the method is neither size extensive nor size consistent; in other words, the correlation energy per particle beyond broken-symmetry mean field vanishes in the thermodynamic limit, and the dissociation limit of a molecule is not the sum of the fragment energies. These two problems are closely related. Recently, Neuscamman [Phys. Rev. Lett. 109, 203001 (2012)] has proposed a method to cure the lack of size consistency in the context of the antisymmetrized geminal power wave function (equivalent to number-projected Hartree-Fock-Bogoliubov) by using a Jastrow-type correlator in Hilbert space. Here, we apply the basic idea in the context of projected Hartree-Fock theory, linearizing the correlator for computational simplicity but extending it to include spin fluctuations. Results are presented for the Hubbard Hamiltonian and for some simple molecular systems

  8. Weak doping dependence of the antiferromagnetic coupling between nearest-neighbor Mn2 + spins in (Ba1 -xKx) (Zn1-yMny) 2As2

    Science.gov (United States)

    Surmach, M. A.; Chen, B. J.; Deng, Z.; Jin, C. Q.; Glasbrenner, J. K.; Mazin, I. I.; Ivanov, A.; Inosov, D. S.

    2018-03-01

    Dilute magnetic semiconductors (DMS) are nonmagnetic semiconductors doped with magnetic transition metals. The recently discovered DMS material (Ba1 -xKx) (Zn1-yMny) 2As2 offers a unique and versatile control of the Curie temperature TC by decoupling the spin (Mn2 +, S =5 /2 ) and charge (K+) doping in different crystallographic layers. In an attempt to describe from first-principles calculations the role of hole doping in stabilizing ferromagnetic order, it was recently suggested that the antiferromagnetic exchange coupling J between the nearest-neighbor Mn ions would experience a nearly twofold suppression upon doping 20% of holes by potassium substitution. At the same time, further-neighbor interactions become increasingly ferromagnetic upon doping, leading to a rapid increase of TC. Using inelastic neutron scattering, we have observed a localized magnetic excitation at about 13 meV associated with the destruction of the nearest-neighbor Mn-Mn singlet ground state. Hole doping results in a notable broadening of this peak, evidencing significant particle-hole damping, but with only a minor change in the peak position. We argue that this unexpected result can be explained by a combined effect of superexchange and double-exchange interactions.

  9. Mean Field Theory of a Coupled Heisenberg Model and Its Application to an Organic Antiferromagnet with Magnetic Anions

    Science.gov (United States)

    Ito, Kazuhiro; Shimahara, Hiroshi

    2016-02-01

    We examine the mean field theory of a uniaxial coupled Heisenberg antiferromagnet with two subsystems, one of which consists of strongly interacting small spins and the other consists of weakly interacting large spins. We reanalyze the experimental data of specific heat and magnetic susceptibility obtained by previous authors for the organic compound λ-(BETS)2FeCl4 at low temperatures, where BETS stands for bis(ethylenedithio)tetraselenafulvalene. The model parameters for this compound are evaluated, where the applicability of the theory is checked. As a result, it is found that J1 ≫ J12 ≫ J2, where J1, J2, and J12 denote the exchange coupling constant between π spins, that between 3d spins, and that between π and 3d spins, respectively. At the low-temperature limit, both sublattice magnetizations of the 3d and π spins are saturated, and the present model is reduced to the Schottky model, which successfully explains experimental observations in previous studies. As temperature increases, fluctuations of 3d spins increase, while π spins remain almost saturated. Near the critical temperature, both spins fluctuate significantly, and thus the mean field approximation breaks down. It is revealed that the magnetic anisotropy, which may be crucial to the antiferromagnetic long-range order, originates from J12 rather than from J2 and that the angle between the magnetic easy-axis and the crystal c-axis is approximately 26-27° in the present effective model.

  10. Antiferromagnetic ordering in superconducting YBa2Cu3O6.5

    DEFF Research Database (Denmark)

    Sidis, Y.; Ulrich, C.; Bourges, P.

    2001-01-01

    Commensurate antiferromagnetic ordering has been observed in the superconducting high-T-c. cuprate YBa2Cu3O6.5 (T-c = 55 K) by polarized and unpolarized elastic neutron scattering. The magnetic peak intensity exhibits a marked enhancement at T-c. Zero-field muon-spin-resonance experiments...... demonstrate that the staggered magnetization is not truly static but fluctuates on a nanosecond time scale. These results point towards an unusual spin density wave state coexisting with superconductivity....

  11. Antiferromagnetic spintronics

    Czech Academy of Sciences Publication Activity Database

    Jungwirth, Tomáš; Martí, Xavier; Wadley, P.; Wunderlich, Joerg

    2016-01-01

    Roč. 11, č. 3 (2016), 231-241 ISSN 1748-3387 R&D Projects: GA MŠk(CZ) LM2011026; GA ČR GB14-37427G EU Projects: European Commission(XE) 268066 - 0MSPIN Institutional support: RVO:68378271 Keywords : antiferromagnets * spintronics Subject RIV: BM - Solid Matter Physics ; Magnetism Impact factor: 38.986, year: 2016

  12. Antiferromagnetism and hot spots in CeIn3

    Science.gov (United States)

    Grigoriev, Pavel; Gor'kov, Lev

    2006-03-01

    Enormous mass enhancement at ``hot spots'' on the Fermi surface (FS) of the antiferromagnetic CeIn3 has been reported at strong magnetic field near its antiferromagnetic quantum critical point [T. Ebihara et al., Phys. Rev. Lett. 93, 246401 (2004)]. The effect was ascribed to anomalous spin fluctuations at these spots owing to peculiar strong many-body interactions. The ``hot spots'' lie at the positions on FS same as in non-magnetic LaIn3 where the narrow necks are protruded, thus, hinting on their possible relation. Assuming that in paramagnetic phase CeIn3 has similar spectrum, we study the influence of the antiferromagnetic ordering (AFM) on the energy spectrum of CeIn3 and show that its FS undergoes a topological change at the onset of AFM. The necks at the ``hot spots'' are truncated by the AFM, thus restoring the almost spherical d-part of the FS of CeIn3. Applied field suppresses the AFM and restores the necks on the FS (so-called 2.5-order phase transition) leading to logarithmic divergence of the dHvA effective mass when the electron trajectory passes near or through the restored necks. This effect fully explains the observed dHvA mass enhancement in the ``hot spots'' in the frameworks of one-particle approximation and leads to the predictions concerning the spin-dependence of the effective electron mass.

  13. Conductance Fluctuations in Disordered 2D Topological Insulator Wires: From Quantum Spin-Hall to Ordinary Phases

    Science.gov (United States)

    Hsu, Hsiu-Chuan; Kleftogiannis, Ioannis; Guo, Guang-Yu; Gopar, Víctor A.

    2018-03-01

    Impurities and defects are ubiquitous in topological insulators (TIs) and thus understanding the effects of disorder on electronic transport is important. We calculate the distribution of the random conductance fluctuations P(G) of disordered 2D TI wires modeled by the Bernevig-Hughes-Zhang (BHZ) Hamiltonian with realistic parameters. As we show, the disorder drives the TIs into different regimes: metal (M), quantum spin-Hall insulator (QSHI), and ordinary insulator (OI). By varying the disorder strength and Fermi energy, we calculate analytically and numerically P(G) across the entire phase diagram. The conductance fluctuations follow the statistics of the unitary universality class β = 2. At strong disorder and high energy, however, the size of the fluctuations δG reaches the universal value of the orthogonal symmetry class (β = 1). At the QSHI-M and QSHI-OI crossovers, the interplay between edge and bulk states plays a key role in the statistical properties of the conductance.

  14. Coexistence of antiferromagnetic and ferromagnetic spin correlations in Ca(Fe1-xCox)2As2 revealed by As75 nuclear magnetic resonance

    Energy Technology Data Exchange (ETDEWEB)

    Cui, J.; Wiecki, P.; Ran, S.; Bud' ko, S. L.; Canfield, P. C.; Furukawa, Y.

    2016-11-22

    Recent nuclear magnetic resonance (NMR) measurements revealed the coexistence of stripe-type antiferromagnetic (AFM) and ferromagnetic (FM) spin correlations in both the hole- and electron-doped BaFe 2 As 2 families of iron-pnictide superconductors by a Korringa ratio analysis. Motivated by the NMR work, we investigate the possible existence of FM fluctuations in another iron-pnictide superconducting family, Ca ( Fe 1 - x Co x ) 2 As 2 . We reanalyzed our previously reported data in terms of the Korringa ratio and found clear evidence for the coexistence of stripe-type AFM and FM spin correlations in the electron-doped CaFe 2 As 2 system. These NMR data indicate that FM fluctuations exist in general in iron-pnictide superconducting families and thus must be included to capture the phenomenology of the iron pnictides.

  15. Role of disorder in the multi-critical region of d-wave superconductivity and antiferromagnetism

    International Nuclear Information System (INIS)

    Yanase, Youichi; Ogata, Masao

    2007-01-01

    We investigate the disorder-induced microscopic inhomogeneity in the multi-critical region of d-wave superconductivity and antiferromagnetism on the basis of the microscopic t-t ' -U-V model. We find that a small amount of point disorder induces the nano-scale inhomogeneity of spin and superconducting fluctuations when the coherence length of superconductivity is remarkably short as in the under-doped cuprates. Then, the two fluctuations spatially segregate to avoid their competition. We show the remarkable electron-hole asymmetry in high-T c cuprates where the quite different spatial structure is expected in the electron-doped materials

  16. Doping Dependence of Collective Spin and Orbital Excitations in the Spin-1 Quantum Antiferromagnet La2 -xSrxNiO4 Observed by X Rays

    Science.gov (United States)

    Fabbris, G.; Meyers, D.; Xu, L.; Katukuri, V. M.; Hozoi, L.; Liu, X.; Chen, Z.-Y.; Okamoto, J.; Schmitt, T.; Uldry, A.; Delley, B.; Gu, G. D.; Prabhakaran, D.; Boothroyd, A. T.; van den Brink, J.; Huang, D. J.; Dean, M. P. M.

    2017-04-01

    We report the first empirical demonstration that resonant inelastic x-ray scattering (RIXS) is sensitive to collective magnetic excitations in S =1 systems by probing the Ni L3 edge of La2 -xSrxNiO4 (x =0 , 0.33, 0.45). The magnetic excitation peak is asymmetric, indicating the presence of single and multi-spin-flip excitations. As the hole doping level is increased, the zone boundary magnon energy is suppressed at a much larger rate than that in hole doped cuprates. Based on the analysis of the orbital and charge excitations observed by RIXS, we argue that this difference is related to the orbital character of the doped holes in these two families. This work establishes RIXS as a probe of fundamental magnetic interactions in nickelates opening the way towards studies of heterostructures and ultrafast pump-probe experiments.

  17. Doping Dependence of Collective Spin and Orbital Excitations in the Spin-1 Quantum Antiferromagnet La_{2-x}Sr_{x}NiO_{4} Observed by X Rays.

    Science.gov (United States)

    Fabbris, G; Meyers, D; Xu, L; Katukuri, V M; Hozoi, L; Liu, X; Chen, Z-Y; Okamoto, J; Schmitt, T; Uldry, A; Delley, B; Gu, G D; Prabhakaran, D; Boothroyd, A T; van den Brink, J; Huang, D J; Dean, M P M

    2017-04-14

    We report the first empirical demonstration that resonant inelastic x-ray scattering (RIXS) is sensitive to collective magnetic excitations in S=1 systems by probing the Ni L_{3} edge of La_{2-x}Sr_{x}NiO_{4} (x=0, 0.33, 0.45). The magnetic excitation peak is asymmetric, indicating the presence of single and multi-spin-flip excitations. As the hole doping level is increased, the zone boundary magnon energy is suppressed at a much larger rate than that in hole doped cuprates. Based on the analysis of the orbital and charge excitations observed by RIXS, we argue that this difference is related to the orbital character of the doped holes in these two families. This work establishes RIXS as a probe of fundamental magnetic interactions in nickelates opening the way towards studies of heterostructures and ultrafast pump-probe experiments.

  18. Effects of impurities and vortices on the low-energy spin excitations in high-Tc materials

    DEFF Research Database (Denmark)

    Andersen, Brian Møller; Graser, S.; Schmid, M.

    2011-01-01

    We review a theoretical scenario for the origin of the spin-glass phase of underdoped cuprate materials. In particular it is shown how disorder in a correlated d-wave superconductor generates a magnetic phase by inducing local droplets of antiferromagnetic order which eventually merge and form a ...... disorder and/or applied magnetic fields lead to a slowing down of the dynamical spin fluctuations in agreement with neutron scattering and muon spin rotation (mSR) experiments....

  19. Coexistence of magnetic fluctuations and superconductivity in the pnictide high temperature superconductor SmFeAsO1-xFx measured by muon spin rotation.

    Science.gov (United States)

    Drew, A J; Pratt, F L; Lancaster, T; Blundell, S J; Baker, P J; Liu, R H; Wu, G; Chen, X H; Watanabe, I; Malik, V K; Dubroka, A; Kim, K W; Rössle, M; Bernhard, C

    2008-08-29

    Muon spin rotation experiments were performed on the pnictide high temperature superconductor SmFeAsO1-xFx with x=0.18 and 0.3. We observed an unusual enhancement of slow spin fluctuations in the vicinity of the superconducting transition which suggests that the spin fluctuations contribute to the formation of an unconventional superconducting state. An estimate of the in-plane penetration depth lambda ab(0)=190(5) nm was obtained, which confirms that the pnictide superconductors obey an Uemura-style relationship between Tc and lambda ab(0);(-2).

  20. Spin wave collapse and incommensurate fluctuations in URu2Si2

    DEFF Research Database (Denmark)

    Buyers, W.J.L.; Tun, Z.; Petersen, T.

    1994-01-01

    To test if the T(N) = 17.7 K transition in URu2Si2 is driven by a divergence of a magnetic order parameter we performed high-resolution neutron scattering. At the ordering wave vector the spin-wave energy collapsed. and the susceptibility diverged as T(N) was approached. This confirms...... that the order parameter is the magnetic dipole, as shown by recent symmetry arguments and polarized neutron experiments [1]. We also observe incommensurate fluctuations, suggesting that competing temperature-dependent interactions may influence this weak-moment transition....

  1. Correlation driven charge and spin fluctuations in LaCoO{sub 3}

    Energy Technology Data Exchange (ETDEWEB)

    Karolak, Michael [Institut fuer Theoretische Physik und Astrophysik, Universitaet Wuerzburg, Am Hubland, 97074 Wuerzburg (Germany); Izquierdo, Manuel [European XFEL GmbH, Albert-Einstein-Ring 19, 22761 Hamburg (Germany); Synchrotron Soleil, L' Orme des Merisiers St-Aubin, BP-48, 91192, Gif-sur-Yvette (France); Institut fuer Theoretische Physik, Universitaet Hamburg, Jungiusstrasse 9, 20355 Hamburg (Germany); Molodtsov, Serguei L. [European XFEL GmbH, Albert-Einstein-Ring 19, 22761 Hamburg (Germany); Institute of Experimental Physics, Technische Universitaet Bergakademie Freiberg, 09599 Freiberg (Germany); ITMO University, Kronverkskiy pr. 49, 197101 St. Petersburg (Russian Federation); Lichtenstein, Alexander I. [Institut fuer Theoretische Physik, Universitaet Hamburg, Jungiusstrasse 9, 20355 Hamburg (Germany)

    2015-07-01

    The spin transition in LaCoO{sub 3} has been investigated within the DFT+DMFT formalism using continuous time quantum Monte Carlo. Calculations on the experimental rhombohedral atomic structure with two Co sites per unit cell show that an independent treatment of the Co atoms results in a ground state with charge imbalance induced by electronic correlations. Each atom shows a contribution from either a d{sup 5} or a d{sup 7} state in addition to the main d{sup 6} state. These charged states play a relevant role in the spin transition which can be understood as a low spin-high spin (LS-HS) transition with significant contributions (∝ 10%) to the LS and HS states of d{sup 5} and d{sup 7} states. A thermodynamic analysis reveals that the introduction of charge imbalance significantly lowers the total energy of the system.

  2. Constructing a magnetic handle for antiferromagnetic manganites

    Science.gov (United States)

    Glavic, Artur; Dixit, Hemant; Cooper, Valentino R.; Aczel, Adam A.

    2016-04-01

    An intrinsic property of antiferromagnetic materials is the compensation of the magnetic moments from the individual atoms that prohibits the direct interaction of the spin lattice with an external magnetic field. To overcome this limitation we have created artificial spin structures by heteroepitaxy between two bulk antiferromagnets SrMnO3 and NdMnO3. Here, we demonstrate that charge transfer at the interface results in the creation of thin ferromagnetic layers adjacent to A -type antiferromagnetism in thick NdMnO3 layers. A novel interference based neutron diffraction technique and polarized neutron reflectometry are used to confirm the presence of ferromagnetism in the SrMnO3 layers and to probe the relative alignment of antiferromagnetic spins induced by the coupling at the ferro- to antiferromagnet interface. A density functional theory analysis of the driving forces for the exchange reveals strong ferromagnetic interfacial coupling through quantifiable short range charge transfer. These results confirm a layer-by-layer control of magnetic arrangements that constitutes a promising step on a path towards isothermal magnetic control of antiferromagnetic arrangements as would be necessary in spin-based heterostructures like multiferroic devices.

  3. Spin fluctuations in EuS; Spinfluktuationen in EuS

    Energy Technology Data Exchange (ETDEWEB)

    Hartmann, A. [Paul Scherrer Inst. (PSI), Villigen (Switzerland)

    1996-02-01

    Demagnetization effects break the isotropy of spin waves. During spring 1995, Peter Boeni et al. performed polarized neutron measurements on EuS using the triple axis spectrometer IN14 at the ILL in Grenoble, in order to investigate the influence of dipolar interactions on the spin waves. In the following work the analysis of the experimental data is described. (author) 25 figs., 2 tabs., 9 refs.

  4. Breakdown of antiferromagnet order in polycrystalline NiFe/NiO bilayers probed with acoustic emission

    Science.gov (United States)

    Lebyodkin, M. A.; Lebedkina, T. A.; Shashkov, I. V.; Gornakov, V. S.

    2017-07-01

    Magnetization reversal of polycrystalline NiFe/NiO bilayers was investigated using magneto-optical indicator film imaging and acoustic emission techniques. Sporadic acoustic signals were detected in a constant magnetic field after the magnetization reversal. It is suggested that they are related to elastic waves excited by sharp shocks in the NiO layer with strong magnetostriction. Their probability depends on the history and number of repetitions of the field cycling, thus testifying the thermal-activation nature of the long-time relaxation of an antiferromagnetic order. These results provide evidence of spontaneous thermally activated switching of the antiferromagnetic order in NiO grains during magnetization reversal in ferromagnet/antiferromagnet (FM/AFM) heterostructures. The respective deformation modes are discussed in terms of the thermal fluctuation aftereffect in the Fulcomer and Charap model which predicts that irreversible breakdown of the original spin orientation can take place in some antiferromagnetic grains with disordered anisotropy axes during magnetization reversal of exchange-coupled FM/AFM structures. The spin reorientation in the saturated state may induce abrupt distortion of isolated metastable grains because of the NiO magnetostriction, leading to excitation of shock waves and formation of plate (or Lamb) waves.

  5. Stabilization of Long-Range Order by Additional Anisotropic Spins in Two-Dimensional Isotropic Heisenberg Antiferromagnets —A Possible Model of an Organic Compound with Magnetic Anions—

    Science.gov (United States)

    Shimahara, Hiroshi; Ito, Kazuhiro

    2014-11-01

    We examine a two-dimensional (2D) coupled antiferromagnetic (AF) Heisenberg model that consists of two subsystems: an isotropic S = 1/2 spin subsystem with strong AF exchange interactions (main system), and a uniaxial S = 5/2 spin subsystem with weak exchange interactions. This model is an example in which additional semiclassical degrees of freedom affect a quantum system; it also describes a possible stabilization mechanism of AF long-range order (LRO) in the 2D organic compound λ-(BETS)2FeCl4, where BETS stands for bis(ethylenedithio)tetraselenafulvalene. Previous experimental studies have revealed that 3d spins on FeCl4 anions passively follow the AF LRO of the π-electron system in the BETS layers, although the AF LRO is stabilized by the 3d spins themselves. To explain this paradoxical behavior, we examine a scenario in which the uniaxial anisotropy of the 3d spins stabilizes the AF LRO on an isotropic 2D π-spin system. We extend Green's function theory, called the Tyablikov approximation, to the present system, which describes spin-wave excitations and is consistent with the Mermin-Wagner theorem. It is shown that even extremely weak interactions with the uniaxial subsystem efficiently stabilize the AF LRO in the main system, even in the absence of AF exchange interactions in the uniaxial subsystem. The AF LRO is triggered by the uniaxial subsystem, but the sublattice magnetization remains smaller than that of the main system in the high-temperature region. These results are consistent with experimental data for λ-(BETS)2FeCl4 and λ-(BETS)2GaCl4; the latter does not have the 3d spins and does not exhibit the AF LRO.

  6. Advanced first-principles theory of superconductivity including both lattice vibrations and spin fluctuations: The case of FeB4

    Science.gov (United States)

    Bekaert, J.; Aperis, A.; Partoens, B.; Oppeneer, P. M.; Milošević, M. V.

    2018-01-01

    We present an advanced method to study spin fluctuations in superconductors quantitatively and entirely from first principles. This method can be generally applied to materials where electron-phonon coupling and spin fluctuations coexist. We employ it here to examine the recently synthesized superconductor iron tetraboride (FeB4) with experimental Tc˜2.4 K [H. Gou et al., Phys. Rev. Lett. 111, 157002 (2013), 10.1103/PhysRevLett.111.157002]. We prove that FeB4 is particularly prone to ferromagnetic spin fluctuations due to the presence of iron, resulting in a large Stoner interaction strength, I =1.5 eV, as calculated from first principles. The other important factor is its Fermi surface that consists of three separate sheets, among which two are nested ellipsoids. The resulting susceptibility has a ferromagnetic peak around q =0 , from which we calculated the repulsive interaction between Cooper pair electrons using the random phase approximation. Subsequently, we combined the electron-phonon interaction calculated from first principles with the spin fluctuation interaction in fully anisotropic Eliashberg theory calculations. We show that the resulting superconducting gap spectrum is conventional, yet very strongly depleted due to coupling to the spin fluctuations. The critical temperature decreases from Tc=41 K, if they are not taken into account, to Tc=1.7 K, in good agreement with the experimental value.

  7. Classical Antiferromagnetism in Kinetically Frustrated Electronic Models

    Science.gov (United States)

    Sposetti, C. N.; Bravo, B.; Trumper, A. E.; Gazza, C. J.; Manuel, L. O.

    2014-05-01

    We study, by means of the density matrix renormalization group, the infinite U Hubbard model—with one hole doped away from half filling—in triangular and square lattices with frustrated hoppings, which invalidate Nagaoka's theorem. We find that these kinetically frustrated models have antiferromagnetic ground states with classical local magnetization in the thermodynamic limit. We identify the mechanism of this kinetic antiferromagnetism with the release of the kinetic energy frustration, as the hole moves in the established antiferromagnetic background. This release can occur in two different ways: by a nontrivial spin Berry phase acquired by the hole, or by the effective vanishing of the hopping amplitude along the frustrating loops.

  8. Magnetic fluctuations and correlations in MnSi : Evidence for a chiral skyrmion spin liquid phase

    NARCIS (Netherlands)

    Pappas, C.; Lelièvre-Berna, E.; Bentley, P.; Falus, P.; Fouquet, P.; Farago, B.

    2011-01-01

    We present a comprehensive analysis of high-resolution neutron scattering data involving neutron spin echo spectroscopy and spherical polarimetry, which confirm the first-order nature of the helical transition in MnSi. The experiments reveal the existence of a totally chiral dynamic phase in a very

  9. NMR study of spin fluctuations and superconductivity in LaFeAsO1-xHx

    Science.gov (United States)

    Fujiwara, Naoki; Sakurai, Ryosuke; Iimura, Soushi; Matsuishi, Satoru; Hosono, Hideo; Yamakawa, Yoichi; Kontani, Hiroshi

    2013-03-01

    We have performed NMR measurements in LaFeAsO1-xHx, an isomorphic compound of LaFeAsO1-xFx. LaFeAsO1-xHx is most recently known for having double superconducting (SC) domes on H doping. LaFeAsO1-xHx is an electron- doped system, and protons act as H-1 as well as F-1. The first SC dome is very similar between F and H doping, suggesting that H doping supplies the same amount of electrons as F doping. Interestingly, an excess amount of H up to x=0.5 can be replaced with O2-. In the H-overdoped regime (x > 0 . 2), LaFeAsO1-xHx undergoes the second superconducting state. We measured the relaxation rate of LaFeAsO1-xHx for x=0.2 and 0.4, and fond an anomalous electronic state; spin fluctuations measured from 1 /T1 T is enhanced with increasing the doping level from x = 0 . 2 to 0.4. The enhancement of spin fluctuations with increasing carrier doping is a new phenomenon that has not observed in LaFeAsO1-xFx in which the upper limit of the doping level is at most x = 0 . 2 . We will discuss the phenomenon in relation to superconductivity. Grant (KAKENHI 23340101) from the Ministry of Education, Sports and Science, Japan

  10. Thermodynamic properties of paramagnetic α - and β -Mn from first principles: The effect of transverse spin fluctuations

    Science.gov (United States)

    Ehteshami, Hossein; Korzhavyi, Pavel A.

    2017-12-01

    First-principles-based thermodynamic modeling of cubic α and β phases of Mn represent a challenge due to their structural complexity and the necessity of simultaneous treatment of several types of disorder (electronic, magnetic, and vibrational) that have very different characteristic time scales. Here we employ mean-field theoretical models to describe the different types of disorder and then we connect each layer of theory to the others using the adiabatic principle of separating faster and slower degrees of freedom. The slowest (vibrational) degrees of freedom are treated using the Moruzzi, Janak, and Schwarz formalism [Phys. Rev. B 37, 790 (1988), 10.1103/PhysRevB.37.790] of the Debye-Grüneisen model parametrized based on the first-principles calculated equation of state which includes the free-energy contributions due to the fast (electronic and magnetic) degrees of freedom via the Fermi-Dirac distribution function and a mean-field theory of transverse spin fluctuations. The magnetic contribution due to transverse spin fluctuations has been computed self-consistently within the disordered local moment picture of the paramagnetic state. The obtained results for thermodynamic properties such as lattice parameter, linear thermal expansion coefficient, and heat capacity of both phases show a good agreement with available experimental data. We also tested the assumption about the nature (localized versus delocalized) of magnetic moment on site IV in α -Mn and site I in β -Mn on the thermodynamic properties of these two phases. Similar to the findings of experimental studies, we conclude that magnetic moment on site IV in α -Mn is not of a localized character. However, a similar analysis suggests that the magnetic moment of site I in β -Mn should be treated as localized.

  11. The low-temperature phase of the Heisenberg antiferromagnet in a fermionic representation

    International Nuclear Information System (INIS)

    Azakov, S.; Dilaver, M.; Oztas, A.M.

    1999-09-01

    Thermal properties of the ordered phase of the spin 1/2 isotropic Heisenberg Antiferromagnet on a d-dimensional hypercubical lattice are studied within the fermionic representation when the constraint of a single occupancy condition is taken into account by the method suggested by Popov and Fedotov. Using a saddle point approximation in the path integral approach we discuss not only the leading order but also the fluctuations around the saddle point at one-loop level. The influence of taking into account the single occupancy condition is discussed at all steps. (author)

  12. Field-controlled magnetic order in the quantum spin-ladder system (Hpip)2CuBr4

    DEFF Research Database (Denmark)

    Thielemann, B.; Rüegg, C.; Kiefer, K.

    2009-01-01

    Neutron diffraction is used to investigate the field-induced, antiferromagnetically ordered state in the two-leg spin-ladder material (Hpip)(2)CuBr4. This "classical" phase, a consequence of weak interladder coupling, is nevertheless highly unconventional: its properties are influenced strongly b...... the quantum fluctuation corrections to the mean-field interaction.......Neutron diffraction is used to investigate the field-induced, antiferromagnetically ordered state in the two-leg spin-ladder material (Hpip)(2)CuBr4. This "classical" phase, a consequence of weak interladder coupling, is nevertheless highly unconventional: its properties are influenced strongly...

  13. Emergent criticality and Friedan scaling in a two-dimensional frustrated Heisenberg antiferromagnet

    Science.gov (United States)

    Orth, Peter P.; Chandra, Premala; Coleman, Piers; Schmalian, Jörg

    2014-03-01

    We study a two-dimensional frustrated Heisenberg antiferromagnet on the windmill lattice consisting of triangular and dual honeycomb lattice sites. In the classical ground state, the spins on different sublattices are decoupled, but quantum and thermal fluctuations drive the system into a coplanar state via an "order from disorder" mechanism. We obtain the finite temperature phase diagram using renormalization group approaches. In the coplanar regime, the relative U(1) phase between the spins on the two sublattices decouples from the remaining degrees of freedom, and is described by a six-state clock model with an emergent critical phase. At lower temperatures, the system enters a Z6 broken phase with long-range phase correlations. We derive these results by two distinct renormalization group approaches to two-dimensional magnetism: Wilson-Polyakov scaling and Friedan's geometric approach to nonlinear sigma models where the scaling of the spin stiffnesses is governed by the Ricci flow of a 4D metric tensor.

  14. Exchange bias in diluted-antiferromagnet/antiferromagnet bilayers

    International Nuclear Information System (INIS)

    Mao, Zhongquan; Zhan, Xiaozhi; Chen, Xi

    2015-01-01

    The hysteresis-loop properties of a diluted-antiferromagnetic (DAF) layer exchange coupling to an antiferromagnetic (AF) layer are investigated by means of numerical simulations. Remarkable loop shift and coercivity enhancement are observed in such DAF/AF bilayers, while they are absent in the uncoupled DAF single layer. The influences of pinned domains, dilution, cooling field and DAF layer thickness on the loop shift are investigated systematically. The result unambiguously confirms an exchange bias (EB) effect in the DAF/AF bilayers. It also reveals that the EB effect originates from the pinned AF domains within the DAF layer. In contrast to conventional EB systems, frozen uncompensated spins are not found at the interface of the AF pinning layer. (paper)

  15. Long Range Order and Spin-Fluctuations in Strongly Correlated Electron System with Valence Instability

    Science.gov (United States)

    Alekseev, P. A.; Menushenkov, A. P.; Mignot, J.-M.; Nemkovski, K. S.; Yaroslavtsev, A. A.; Kozlenko, D. P.

    Rare-earth based strongly correlated electron systems (SCES) exhibit a large variety of different ground states, ranging from the simple paramagnetism of crystal-field-split f-electron multiplets to highly unconventional Kondo-insulator states with a combination of charge gap, spin gap and valence instability, in which long-range magnetic order can eventually arise from an initially singlet state. The physical background for these properties of the electron subsystem may be clarified by performing detailed neutron scattering experiments, namely magnetic neutron scattering spectroscopy and diffraction. This report reviews the results of the previous and new experimental studies on a number of rare-earth intermetallic compounds, which shed light on peculiar features of those unusual ground states.

  16. Spin fluctuation effects on the conductance through a single Pd atom contact

    International Nuclear Information System (INIS)

    Romero, M A; Goldberg, E C; Gomez-Carrillo, S C; Bolcatto, P G

    2009-01-01

    A controversy about the conductance through single atoms still exists. There are many experiments where values lower than the quantum unity G 0 = 2e 2 /h have been found associated to Kondo regimes with high Kondo temperatures. Specifically in the Pd single atom contact, conductance values close to G 0 /2 at room temperature have been reported. In this work we propose a theoretical analysis of a break junction of Pd where the charge fluctuation in the single atom contact is limited to the most probable one: d 10 ↔d 9 . The projected density of states and the characteristics of the electron transport are calculated by using a realistic description of the interacting system. A Kondo regime is found where the conductance values and their dependence on temperature are in good agreement with the experimental trends observed in the conduction of single molecule transistors based on transition metal coordination complexes.

  17. Strong antiferromagnetic coupling of spins in the (MDABCO+)(C60·-) salt with 3D close packing of the C60·- radical anions (MDABCO+: N-methyldiazabicyclooctanium cation).

    Science.gov (United States)

    Konarev, Dmitri V; Khasanov, Salavat S; Otsuka, Akihiro; Yamochi, Hideki; Saito, Gunzi; Lyubovskaya, Rimma N

    2014-06-01

    A new salt, (MDABCO(+))(C60(·-)) (1; MDABCO(+) = N-methyldiazabicyclooctanium cation), was obtained as single crystals. The crystal structure of 1 determined at 250 and 100 K showed 3D close packing of fullerenes with eight fullerene neighbors for each C60(·-). These neighbors are located at 10.01-10.11 Å center-to-center distances (250 K) and van der Waals interfullerene C⋅⋅⋅C contacts are formed with four fullerene neighbors arranged in the bc plane. Fullerene ordering observed below 160 K is accompanied by the appearance of one and a half independent C60(·-) and trebling of the unit cell along the b axis. Fullerenes are packed closer to each other at 100 K. As a result, fullerenes are located in the three-dimensional packing at 9.91-10.12 Å center-to-center distances and 18 short interfullerene C⋅⋅⋅C contacts are formed for each C60(·-). Although they are closed packed, fullerenes are not dimerized down to 1.9 K. Magnetic data indicate strong antiferromagnetic coupling of spins in the 70-300 K range with a Weiss temperature of Θ = -118 K. Magnetic susceptibility shows a round maximum at 46 K. Such behavior can be described well by the Heisenberg model for square two-dimensional antiferromagnetic coupling of spins with an exchange interaction of J/kB = -25.3 K. This magnetic coupling is one of the strongest observed for C60(·-) salts. © 2014 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

  18. Charge stripes and spin correlations in copper-oxide superconductors

    OpenAIRE

    Tranquada, J. M.

    1997-01-01

    Recent neutron diffraction studies have yielded evidence that, in a particular cuprate family, holes doped into the CuO(2) planes segregate into stripes that separate antiferromagnetic domains. Here it is shown that such a picture provides a quantitatively consistent interpretation of the spin fluctuations measured by neutron scattering in La(1.85)Sr(0.15)CuO(4) and YBa(2)Cu(3)O(6+x).

  19. Magnetic Hamiltonian and phase diagram of the quantum spin liquid Ca10Cr7O28

    Science.gov (United States)

    Balz, Christian; Lake, Bella; Nazmul Islam, A. T. M.; Singh, Yogesh; Rodriguez-Rivera, Jose A.; Guidi, Tatiana; Wheeler, Elisa M.; Simeoni, Giovanna G.; Ryll, Hanjo

    2017-05-01

    A spin liquid is a new state of matter with topological order where the spin moments continue to fluctuate coherently down to the lowest temperatures rather than develop static long-range magnetic order as found in conventional magnets. For spin liquid behavior to arise in a material the magnetic Hamiltonian must be "frustrated", where the combination of lattice geometry, interactions, and anisotropies gives rise to competing spin arrangements in the ground state. Theoretical Hamiltonians which produce spin liquids are spin ice, the Kitaev honeycomb model, and the kagome antiferromagnet. Spin liquid behavior, however, in real materials is rare because they can only approximate these Hamiltonians and often have weak higher-order terms that destroy the spin liquid state. Ca10Cr7O28 is a new quantum spin liquid candidate with magnetic Cr5 + ions that possess quantum spin number S =½ . The spins are entirely dynamic in the ground state and the excitation spectrum is broad and diffuse, as is typical of spinons which are the excitations of a spin liquid. In this paper we determine the Hamiltonian of Ca10Cr7O28 using inelastic neutron scattering under high magnetic field to induce a field-polarized paramagnetic ground state and spin-wave excitations that can be fitted to extract the interactions. We further explore the phase diagram by using inelastic neutron scattering and heat capacity measurements and establish the boundaries of the spin liquid phase as a function of magnetic field and temperature. Our results show that Ca10Cr7O28 consists of distorted kagome bilayers with several isotropic ferromagnetic and antiferromagnetic interactions where, unexpectedly, the ferromagnetic interactions are stronger than the antiferromagnetic ones. This complex Hamiltonian does not correspond to any known spin liquid model and points to new directions in the search for quantum spin liquid behavior.

  20. Spin-1/2 Triangular-Lattice Heisenberg Antiferromagnet with √{3} × √{3} -Type Distortion — Behavior around the Boundaries of the Intermediate Phase

    Science.gov (United States)

    Shimada, Alisa; Nakano, Hiroki; Sakai, Tôru; Yoshimura, Kazuyoshi

    2018-03-01

    The S = 1/2 triangular-lattice Heisenberg antiferromagnet with distortion is investigated by the numerical-diagonalization method. The examined distortion type is √{3} × √{3} . We study the case when the distortion connects the undistorted triangular lattice and the dice lattice. For the intermediate phase reported previously in this system, we obtain results of the boundaries of the intermediate phase for a larger system than those in the previous report and examine the system size dependence of the boundaries in detail. We also report the specific heat of this system, which shows a marked peak structure related to the appearance of the intermediate state.

  1. Femtosecond optomagnetism in dielectric antiferromagnets

    Science.gov (United States)

    Bossini, D.; Rasing, Th

    2017-02-01

    Optical femtosecond manipulation of magnetic order is attractive for the development of new concepts for ultrafast magnetic recording. Theoretical and experimental investigations in this research area aim at establishing a physical understanding of magnetic media in light-induced non-equilibrium states. Such a quest requires one to adjust the theory of magnetism, since the thermodynamical concepts of elementary excitations and spin alignment determined by the exchange interaction are not applicable on the femtosecond time-scale after the photo-excitation. Here we report some key milestones concerning the femtosecond optical control of spins in dielectric antiferromagnets, whose spin dynamics is by nature faster than that of ferromagnets and can be triggered even without any laser heating. The recent progress of the opto-magnetic effect in the sub-wavelength regime makes this exciting research area even more promising, in terms of both fundamental breakthroughs and technological perspectives.

  2. Dynamic zero modes of Dirac fermions and competing singlet phases of antiferromagnetic order

    Science.gov (United States)

    Goswami, Pallab; Si, Qimiao

    2017-06-01

    In quantum spin systems, singlet phases often develop in the vicinity of an antiferromagnetic order. Typical settings for such problems arise when itinerant fermions are also present. In this paper, we develop a theoretical framework for addressing such competing orders in an itinerant system, described by Dirac fermions strongly coupled to an O(3) nonlinear sigma model. We focus on two spatial dimensions, where upon disordering the antiferromagnetic order by quantum fluctuations the singular tunneling events also known as (anti)hedgehogs can nucleate competing singlet orders in the paramagnetic phase. In the presence of an isolated hedgehog configuration of the nonlinear sigma model field, we show that the fermion determinant vanishes as the dynamic Euclidean Dirac operator supports fermion zero modes of definite chirality. This provides a topological mechanism for suppressing the tunneling events. Using the methodology of quantum chromodynamics, we evaluate the fermion determinant in the close proximity of magnetic quantum phase transition, when the antiferromagnetic order-parameter field can be described by a dilute gas of hedgehogs and antihedgehogs. We show how the precise nature of emergent singlet order is determined by the overlap between dynamic fermion zero modes of opposite chirality, localized on the hedgehogs and antihedgehogs. For a Kondo-Heisenberg model on the honeycomb lattice, we demonstrate the competition between spin Peierls order and Kondo singlet formation, thereby elucidating its global phase diagram. We also discuss other physical problems that can be addressed within this general framework.

  3. Reciprocal propagation of surface modes in an antiferromagnetic film

    International Nuclear Information System (INIS)

    Oliveira, F.A.; Amato, M.A.

    1987-09-01

    Linear response theory is used to evaluate the Green's functions describing the fluctuations in an antiferromagnetic film at zero applied field. It is shown the similarities between the dielectric and magnetic excitations. (Author) [pt

  4. Thermoinduced magnetization in nanoparticles of antiferromagnetic materials

    DEFF Research Database (Denmark)

    Mørup, Steen; Frandsen, Cathrine

    2004-01-01

    We show that there is a thermoinduced contribution to the magnetic moment of nanoparticles of antiferromagnetic materials. It arises from thermal excitations of the uniform spin-precession mode, and it has the unusual property that its magnitude increases with increasing temperature. This has...

  5. The electronic structure of antiferromagnetic chromium

    DEFF Research Database (Denmark)

    Skriver, Hans Lomholt

    1981-01-01

    The author has used the local spin density formalism to perform self-consistent calculations of the electronic structure of chromium in the non-magnetic and commensurate antiferromagnetic phases, as a function of the lattice parameter. A change of a few per cent in the atomic radius brings...

  6. High-T_{c} Superconductivity in FeSe at High Pressure: Dominant Hole Carriers and Enhanced Spin Fluctuations.

    Science.gov (United States)

    Sun, J P; Ye, G Z; Shahi, P; Yan, J-Q; Matsuura, K; Kontani, H; Zhang, G M; Zhou, Q; Sales, B C; Shibauchi, T; Uwatoko, Y; Singh, D J; Cheng, J-G

    2017-04-07

    The importance of electron-hole interband interactions is widely acknowledged for iron-pnictide superconductors with high transition temperatures (T_{c}). However, the absence of hole pockets near the Fermi level of the iron-selenide (FeSe) derived high-T_{c} superconductors raises a fundamental question of whether iron pnictides and chalcogenides have different pairing mechanisms. Here, we study the properties of electronic structure in the high-T_{c} phase induced by pressure in bulk FeSe from magnetotransport measurements and first-principles calculations. With increasing pressure, the low-T_{c} superconducting phase transforms into the high-T_{c} phase, where we find the normal-state Hall resistivity changes sign from negative to positive, demonstrating dominant hole carriers in contrast to other FeSe-derived high-T_{c} systems. Moreover, the Hall coefficient is enlarged and the magnetoresistance exhibits anomalous scaling behaviors, evidencing strongly enhanced interband spin fluctuations in the high-T_{c} phase. These results in FeSe highlight similarities with high-T_{c} phases of iron pnictides, constituting a step toward a unified understanding of iron-based superconductivity.

  7. Improving cerebral blood flow quantification for arterial spin labeled perfusion MRI by removing residual motion artifacts and global signal fluctuations.

    Science.gov (United States)

    Wang, Ze

    2012-12-01

    Denoising is critical to improving the quality and stability of cerebral blood flow (CBF) quantification in arterial spin labeled (ASL) perfusion magnetic resonance imaging (MRI) due to the intrinsic low signal-to-noise-ratio (SNR) of ASL data. Previous studies have been focused on reducing the spatial or temporal noise using standard filtering techniques, and less attention has been paid to two global nuisance effects, the residual motion artifacts and the global signal fluctuations. Since both nuisances affect the whole brain, removing them in advance should enhance the CBF quantification quality for ASL MRI. The purpose of this paper was to assess this potential benefit. Three methods were proposed to suppress each or both of the two global nuisances. Their performances for CBF quantification were validated using ASL data acquired from 13 subjects. Evaluation results showed that covarying out both global nuisances significantly improved temporal SNR and test-retest stability of CBF measurement. Although the concept of removing both nuisances is not technically novel per se, this paper clearly showed the benefits for ASL CBF quantification. Dissemination of the proposed methods in a free ASL data processing toolbox should be of interest to a broad range of ASL users. Copyright © 2012 Elsevier Inc. All rights reserved.

  8. Quasiparticle excitations in frustrated antiferromagnets

    Energy Technology Data Exchange (ETDEWEB)

    Trumper, Adolfo E. [Instituto de Fisica Rosario (CONICET) Universidad Nacional de Rosario, Boulevard 27 de Febrero 210 bis, 2000 Rosario (Argentina)]. E-mail: trumper@ifir.edu.ar; Gazza, Claudio J. [Instituto de Fisica Rosario (CONICET) Universidad Nacional de Rosario, Boulevard 27 de Febrero 210 bis, 2000 Rosario (Argentina); Manuel, Luis O. [Instituto de Fisica Rosario (CONICET) Universidad Nacional de Rosario, Boulevard 27 de Febrero 210 bis, 2000 Rosario (Argentina)]. E-mail: manuel@ifir.edu.ar

    2004-12-31

    We have computed the quasiparticle wave function corresponding to a hole injected in a triangular antiferromagnet. We have taken into account multi-magnon contributions within the self-consistent Born approximation. We have found qualitative differences, under sign reversal of the integral transfer t, regarding the multi-magnon components and the own existence of the quasiparticle excitations. Such differences are due to the subtle interplay between magnon-assisted and free hopping mechanisms. We conclude that the conventional quasiparticle picture can be broken by geometrical frustration without invoking spin liquid phases.

  9. Quasiparticle excitations in frustrated antiferromagnets

    Science.gov (United States)

    Trumper, Adolfo E.; Gazza, Claudio J.; Manuel, Luis O.

    2004-12-01

    We have computed the quasiparticle wave function corresponding to a hole injected in a triangular antiferromagnet. We have taken into account multi-magnon contributions within the self-consistent Born approximation. We have found qualitative differences, under sign reversal of the integral transfer t, regarding the multi-magnon components and the own existence of the quasiparticle excitations. Such differences are due to the subtle interplay between magnon-assisted and free hopping mechanisms. We conclude that the conventional quasiparticle picture can be broken by geometrical frustration without invoking spin liquid phases.

  10. Quasiparticle excitations in frustrated antiferromagnets

    International Nuclear Information System (INIS)

    Trumper, Adolfo E.; Gazza, Claudio J.; Manuel, Luis O.

    2004-01-01

    We have computed the quasiparticle wave function corresponding to a hole injected in a triangular antiferromagnet. We have taken into account multi-magnon contributions within the self-consistent Born approximation. We have found qualitative differences, under sign reversal of the integral transfer t, regarding the multi-magnon components and the own existence of the quasiparticle excitations. Such differences are due to the subtle interplay between magnon-assisted and free hopping mechanisms. We conclude that the conventional quasiparticle picture can be broken by geometrical frustration without invoking spin liquid phases

  11. Spin-fluctuation mediated superconductivity and magnetic order in the cuprate La1.88Sr0.12CuO4

    DEFF Research Database (Denmark)

    Rømer, Astrid Tranum

    High-temperature superconductivity in cuprates emerges as one out of many electronic phases when doping the antiferromagnetic Mott insulator La2CuO4 away from half _lling. The description of the superconducting phase is therefore complicated by intertwined electronic orders that compete...... with superconductivity. However, it is possible that the tendency towards additional ordering phenomena is a necessary condition for unconventional superconductivity to develop. Indeed most superconductors discovered throughout the last 29 years, including also the recently discovered class of iron-based superconductors......, show a very rich electronic phase diagram. A common feature that characterizes both cuprates, heavy fermions, and iron pnictides is the proximity to magnetic order. Therefore, the idea of spin-uctuation mediated pairing is a popular paradigm proposed for unconventional superconductivity. A _ngerprint...

  12. Detecting quantum critical points using bipartite fluctuations.

    Science.gov (United States)

    Rachel, Stephan; Laflorencie, Nicolas; Song, H Francis; Le Hur, Karyn

    2012-03-16

    We show that the concept of bipartite fluctuations F provides a very efficient tool to detect quantum phase transitions in strongly correlated systems. Using state-of-the-art numerical techniques complemented with analytical arguments, we investigate paradigmatic examples for both quantum spins and bosons. As compared to the von Neumann entanglement entropy, we observe that F allows us to find quantum critical points with much better accuracy in one dimension. We further demonstrate that F can be successfully applied to the detection of quantum criticality in higher dimensions with no prior knowledge of the universality class of the transition. Promising approaches to experimentally access fluctuations are discussed for quantum antiferromagnets and cold gases.

  13. Spin dynamics and structural phase transitions in quasi-2D R sub 2 CuO sub 4 (R=Pr, Sm and Eu) antiferromagnetics

    CERN Document Server

    Golovenchits, E I

    2001-01-01

    One studied spin dynamics and dynamics of lattice in R sub 2 CuO sub 4 (R = Pr, Sm, and Eu) crystals within 20-250 GHz frequency range and within 50350 K temperature interval. One detected abrupt variation of absorption coefficient within wide range of frequencies above 120 GHz at 20, 80 and 150 K temperatures in R sub 2 CuO sub 4 (R = Pr, Sm, and Eu), respectively. Absorption jumpings result from structural phase transitions. Wide ranges of spin-wave excitations were observed in all examined crystals in high-temperature phase. Close to temperatures of phase transitions within wide range of frequencies including frequencies corresponding to ranges of spin-wave excitations one observed lines of a absorption caused by lattice dynamics

  14. Frozen concentration fluctuations in a poly(N-isopropyl acrylamide) gel studied by neutron spin echo and small-angle neutron scattering

    CERN Document Server

    Koizumi, S; Richter, D; Schwahn, D; Faragó, B; Annaka, M

    2002-01-01

    By employing neutron spin echo and small-angle neutron scattering, we determined the structure factor of the frozen concentration fluctuations on nano-length scales in a swollen poly(N-isopropyl acrylamide) gel. The frozen contribution, showing a plateau at the low scattering wavenumber q (0.02 A sup - sup 1), is intimately related to the abnormal butterfly scattering pattern appearing at low q under deformation. (orig.)

  15. Quantum spin quadrumer

    Science.gov (United States)

    Khatua, Subhankar; Shankar, R.; Ganesh, R.

    2018-02-01

    A fundamental motif in frustrated magnetism is the fully mutually coupled cluster of N spins, with each spin coupled to every other spin. Clusters with N =2 and 3 have been extensively studied as building blocks of square and triangular lattice antiferromagnets. In both cases, large-S semiclassical descriptions have been fruitfully constructed, providing insights into the physics of macroscopic magnetic systems. Here, we develop a semiclassical theory for the N =4 cluster. This problem has rich mathematical structure with a ground-state space that has nontrivial topology. We show that ground states are appropriately parametrized by a unit vector order parameter and a rotation matrix. Remarkably, in the low-energy description, the physics of the cluster reduces to that of an emergent free spin-S spin and a rigid rotor. This successfully explains the spectrum of the quadrumer and its associated degeneracies. However, this mapping does not hold in the vicinity of collinear ground states due to a subtle effect that arises from the nonmanifold nature of the ground-state space. We demonstrate this by an analysis of soft fluctuations, showing that collinear states have a larger number of soft modes. Nevertheless, as these singularities only occur on a subset of measure zero, the mapping to a spin and a rotor provides a good description of the quadrumer. We interpret thermodynamic properties of the quadrumer that are accessible in molecular magnets, in terms of the rotor and spin degrees of freedom. Our study paves the way for field theoretic descriptions of systems such as pyrochlore magnets.

  16. Novel domain wall dynamics in synthetic antiferromagnets

    Science.gov (United States)

    Yang, See-Hun; Parkin, Stuart

    2017-08-01

    In this article, we review fascinating new mechanisms on recently observed remarkable current driven domain wall motion in nanowires formed from perpendicularly magnetized synthetic antiferromagnets interfaced with heavy metallic layers, sources of spin-orbit torques. All the associated torques such as volumetric adiabatic and non-adiabatic spin-transfer-torque, spin-orbit torques, shape anisotropy field torques, Dzyaloshinkii-Moriya interaction torques and most importantly a new powerful torque, exchange coupling torque, will be discussed based on an analytical model that provides an intuitive description of domain wall dynamics in synthetic ferromagnets as well as synthetic antiferromagnets. In addition, the current driven DW motion in the presence of in-plane fields will be investigated, thus deepening our knowledge about the role of the exchange coupling torque, which will be of potential use for application to various novel spintronic devices.

  17. Measurement of spin amplitudes of neutron scattering on 159Tb by neutron diffraction method in antiferromagnets at ultra-low temperature

    International Nuclear Information System (INIS)

    Akopyan, G.G.; Alfimenkov, V.P.; Lason', L.; Ovchinnikov, O.N.; Sharapov, Eh.I.

    1975-01-01

    The measurement results are presented of the spin-spin amplitude for 159 Tb performed by the method of neutron diffraction by the flight time in the IBR-30 pulse reactor with samples cooled down to ultralow temperatures in a cryostat with 3 He dissolved in 4 He. The scattering angle has been fixed, neutrons incident upon the sample had a continuous energy spectrum, and the wave length satisfying the Bragg-Wolf condition has been determined by the neutron flight time required for given distance. Small-sized helium counters served as detectors. Preliminary measurements have been done with terbium dioxide and cobalt oxide whose intraatomic field values are not high. For main measurements TbAg intermetal has been chosen in which the magnetic field on a terbium nuclei is much greater. The difference of spin amplitudes of the thermal neutron scattering by terbium nuclei appeared to be equal to αsub(+-)αsub(-)=(0.35+-0.14) fermi. The spin-noncoherent scattering cross section has been obtained to be sigmasub(inc)=5+-4 mbn. The experiments have shown that the method is highly sensitive to a temperature

  18. Magnetic structure of MgCu2O3 and doping-induced spin reorientation in Mg1-x/2LixCu2-x/2O3

    DEFF Research Database (Denmark)

    Winkelmann, M.; Graf, H.A.; Andersen, N.H.

    1994-01-01

    is similar to the one producing an infinitely degenerate state in antiferromagnetic fcc lattices. Doping experiments with Li clearly demonstrate the importance of spin fluctuations and fluctuations of the local exchange fields for lifting the degeneracy in such a system. A remarkably small amount of Li...... (about 2 mole % Li) is sufficient to disturb the magnetic lattice in such a way that the almost collinear spin arrangement changes into an arrangement where the spins of one sublattice are strongly canted with respect to the spins of the other sublattice....

  19. Temperature-dependent striped antiferromagnetism of LaFeAsO in a Green's function approach

    International Nuclear Information System (INIS)

    Liu Guibin; Liu Banggui

    2009-01-01

    We use a Green's function method to study the temperature-dependent average moment and magnetic phase-transition temperature of the striped antiferromagnetism of LaFeAsO, and other similar compounds, as the parents of FeAs-based superconductors. We consider the nearest and the next-nearest couplings in the FeAs layer, and the nearest coupling for inter-layer spin interaction. The dependence of the transition temperature T N and the zero-temperature average spin on the interaction constants is investigated. We obtain an analytical expression for T N and determine our temperature-dependent average spin from zero temperature to T N in terms of unified self-consistent equations. For LaFeAsO, we obtain a reasonable estimation of the coupling interactions with the experimental transition temperature T N = 138 K. Our results also show that a non-zero antiferromagnetic (AFM) inter-layer coupling is essential for the existence of a non-zero T N , and the many-body AFM fluctuations reduce substantially the low-temperature magnetic moment per Fe towards the experimental value. Our Green's function approach can be used for other FeAs-based parent compounds and these results should be useful to understand the physical properties of FeAs-based superconductors.

  20. Spins in the Vortices of a High Temperature Superconductor

    OpenAIRE

    Lake, B; Aeppli, G; Clausen, KN; McMorrow, DF; Lefmann, K; Hussey, NE; Mangkorntong, N; Nohara, M; Takagi, H; Mason, TE; Schröder, A

    2002-01-01

    Neutron scattering is used to characterise the magnetism of the vortices for the optimally doped high-temperature superconductor La(2-x)Sr(x)CuO(4) (x=0.163) in an applied magnetic field. As temperature is reduced, low frequency spin fluctuations first disappear with the loss of vortex mobility, but then reappear. We find that the vortex state can be regarded as an inhomogeneous mixture of a superconducting spin fluid and a material containing a nearly ordered antiferromagnet. These experimen...

  1. Charge dynamics of the antiferromagnetically ordered Mott insulator

    International Nuclear Information System (INIS)

    Han, Xing-Jie; Li, Xin; Chen, Jing; Liao, Hai-Jun; Xiang, Tao; Liu, Yu; Liu, Zhi-Yuan; Xie, Zhi-Yuan; Normand, B

    2016-01-01

    We introduce a slave-fermion formulation in which to study the charge dynamics of the half-filled Hubbard model on the square lattice. In this description, the charge degrees of freedom are represented by fermionic holons and doublons and the Mott-insulating characteristics of the ground state are the consequence of holon–doublon bound-state formation. The bosonic spin degrees of freedom are described by the antiferromagnetic Heisenberg model, yielding long-ranged (Néel) magnetic order at zero temperature. Within this framework and in the self-consistent Born approximation, we perform systematic calculations of the average double occupancy, the electronic density of states, the spectral function and the optical conductivity. Qualitatively, our method reproduces the lower and upper Hubbard bands, the spectral-weight transfer into a coherent quasiparticle band at their lower edges and the renormalisation of the Mott gap, which is associated with holon–doublon binding, due to the interactions of both quasiparticle species with the magnons. The zeros of the Green function at the chemical potential give the Luttinger volume, the poles of the self-energy reflect the underlying quasiparticle dispersion with a spin-renormalised hopping parameter and the optical gap is directly related to the Mott gap. Quantitatively, the square-lattice Hubbard model is one of the best-characterised problems in correlated condensed matter and many numerical calculations, all with different strengths and weaknesses, exist with which to benchmark our approach. From the semi-quantitative accuracy of our results for all but the weakest interaction strengths, we conclude that a self-consistent treatment of the spin-fluctuation effects on the charge degrees of freedom captures all the essential physics of the antiferromagnetic Mott–Hubbard insulator. We remark in addition that an analytical approximation with these properties serves a vital function in developing a full understanding of

  2. Charge dynamics of the antiferromagnetically ordered Mott insulator

    Science.gov (United States)

    Han, Xing-Jie; Liu, Yu; Liu, Zhi-Yuan; Li, Xin; Chen, Jing; Liao, Hai-Jun; Xie, Zhi-Yuan; Normand, B.; Xiang, Tao

    2016-10-01

    We introduce a slave-fermion formulation in which to study the charge dynamics of the half-filled Hubbard model on the square lattice. In this description, the charge degrees of freedom are represented by fermionic holons and doublons and the Mott-insulating characteristics of the ground state are the consequence of holon-doublon bound-state formation. The bosonic spin degrees of freedom are described by the antiferromagnetic Heisenberg model, yielding long-ranged (Néel) magnetic order at zero temperature. Within this framework and in the self-consistent Born approximation, we perform systematic calculations of the average double occupancy, the electronic density of states, the spectral function and the optical conductivity. Qualitatively, our method reproduces the lower and upper Hubbard bands, the spectral-weight transfer into a coherent quasiparticle band at their lower edges and the renormalisation of the Mott gap, which is associated with holon-doublon binding, due to the interactions of both quasiparticle species with the magnons. The zeros of the Green function at the chemical potential give the Luttinger volume, the poles of the self-energy reflect the underlying quasiparticle dispersion with a spin-renormalised hopping parameter and the optical gap is directly related to the Mott gap. Quantitatively, the square-lattice Hubbard model is one of the best-characterised problems in correlated condensed matter and many numerical calculations, all with different strengths and weaknesses, exist with which to benchmark our approach. From the semi-quantitative accuracy of our results for all but the weakest interaction strengths, we conclude that a self-consistent treatment of the spin-fluctuation effects on the charge degrees of freedom captures all the essential physics of the antiferromagnetic Mott-Hubbard insulator. We remark in addition that an analytical approximation with these properties serves a vital function in developing a full understanding of the

  3. Anti-ferromagnetic Heisenberg model on bilayer honeycomb

    International Nuclear Information System (INIS)

    Shoja, M.; Shahbazi, F.

    2012-01-01

    Recent experiment on spin-3/2 bilayer honeycomb lattice antiferromagnet Bi 3 Mn 4 O 12 (NO 3 ) shows a spin liquid behavior down to very low temperatures. This behavior can be ascribed to the frustration effect due to competitions between first and second nearest neighbour's antiferromagnet interaction. Motivated by the experiment, we study J 1 -J 2 Antiferromagnet Heisenberg model, using Mean field Theory. This calculation shows highly degenerate ground state. We also calculate the effect of second nearest neighbor through z direction and show these neighbors also increase frustration in these systems. Because of these degenerate ground state in these systems, spins can't find any ground state to be freeze in low temperatures. This behavior shows a novel spin liquid state down to very low temperatures.

  4. Antiferromagnetic order in hybrid electromagnetic metamaterials

    Science.gov (United States)

    Miroshnichenko, Andrey E.; Filonov, Dmitry; Lukyanchuk, Boris; Kivshar, Yuri

    2017-08-01

    We demonstrate experimentally a new type of order in optical magnetism resembling the staggered structure of spins in antiferromagnetic ordered materials. We study hybrid electromagnetic metasurfaces created by assembling hybrid meta-atoms formed by metallic split-ring resonators and dielectric particles with a high refractive index, both supporting optically-induced magnetic dipole resonances of different origin. Each pair (or ‘metamolecule’) is characterized by two interacting magnetic dipole moments with the distance-dependent magnetization resembling the spin exchange interaction in magnetic materials. By directly mapping the structure of the electromagnetic fields, we demonstrate experimentally that strong coupling between the optically-induced magnetic moments of different origin can flip the magnetisation orientation in a metamolecule creating an antiferromagnetic lattice of staggered optically-induced magnetic moments in hybrid metasurfaces.

  5. Robustness of dynamic magnetism in the triangle-based antiferromagnets Ba3Ru1- x Ir x Ti2O9 ( x = 0.5 and 0.8)

    Science.gov (United States)

    Lee, W.-J.; Do, S.-H.; Lee, S.; Choi, Y.-S.; Choi, K.-Y.; Yoon, Sungwon; Suh, Byoungjin; Jang, Zeehoon

    2018-01-01

    We report on the spin dynamics of the strong spin-orbit coupled antiferromagnets Ba3Ru1- x Ir x Ti2O9 ( x = 0.5 and 0.8), which comprise a mixture of edge- and corner-sharing triangles. Muon spin-relaxation measurements give no hints of long-range magnetic order down to 25 mK. Rather, the muon spin-relaxation rates λ( T) show persistent spin dynamics below 1 K, indicating that fast fluctuations are dominant in spite of Ir4+( J eff = 1/2)/Ru4+( S = 1) randomness. The muon spin depolarization of both compounds is well described by a stretched exponential function with the stretching exponent β = 0.4 (0.6) for x = 0.5 (0.8) at low temperatures, which is larger than β = 1/3 expected for a spin glass. Our results suggest that randomness in the spin number and the exchange interaction induces a partial spin freezing, but the majority of spins remain dynamically fluctuating.

  6. Magnetic anisotropy and spin fluctuations in the paramagnetic dimer [Fe(OMe)(dpm)2]2: Moessbauer spectroscopy and ab initio calculations

    International Nuclear Information System (INIS)

    Cianchi, L.; Del Giallo, F.; Moretti, P.; Spina, G.; Mancini, M.; Caneschi, A.; Lantieri, M.

    2008-01-01

    The magnetic anisotropy and the spin fluctuations of the paramagnetic molecule [Fe(OMe)(dpm) 2 ] 2 are analyzed by means of Moessbauer spectroscopy in the temperature range [7.6-33] K. Spectra in the presence of a 5 T magnetic field directed along the γ rays were collected, by using a sample of pseudo-single crystal prepared by oriented grains. From the fits of the spectra, the hyperfine parameters are determined. Fits give also the value and direction of the magnetic anisotropy, referred to the electric field gradient (EFG) principal axes. The latter, together with the EFG components, were evaluated by means of ROHF ab initio calculations. Lastly, the rate of the spin transitions in function of T is discussed

  7. The case for spin-fluctuation induced pairing in Ba{sub 1-x}K{sub x}Fe{sub 2}As{sub 2}

    Energy Technology Data Exchange (ETDEWEB)

    Boehm, Thomas U.

    2017-03-07

    The microscopic mechanism and the experimental identification of unconventional superconductivity is one of the most vexing problems of contemporary condensed matter physics. Raman spectroscopy provides a new avenue for this quest by accessing the hierarchy of superconducting pairing propensities. The doping-dependent study of competing pairing channels in Ba{sub 1-x}K{sub x}Fe{sub 2}As{sub 2} for 0.22 ≤ x ≤ 0.70 is one of the main aspects of this thesis. The observations demonstrate the importance of spin fluctuations for Cooper pairing.

  8. Superconducting pairing of spin polarons in the t - J model

    International Nuclear Information System (INIS)

    Plakida, N.M.; Horsch, P.; Liechtenstein, A.; Oudovenko, V.S.

    1995-07-01

    A spin polaron model derived from the t - J model on a two-sublattice antiferromagnet is considered. The self-consistent Born approximation for the matrix Green functions for doped holes (spin polarons) and magnons is used to study temperature and doping dependence of the quasi-particle hole spectrum and superconducting pairing of two holes on different sublattices. A numerical solution of the self-consistent system of equations by the fast Fourier transformation method shows a strong renormalization of the quasi-particle hole spectrum due to spin fluctuations, and a singlet superconducting pairing of d-wave symmetry with maximal T c ∼ 0.01t around the hole concentration 0.25. We argue that the superconducting pairing of spin polarons for the model with strong electron correlations represents the mechanism of high-temperature superconductivity. (author). 26 refs, 10 figs

  9. Calculations of Exchange Bias in Thin Films with Ferromagnetic/Antiferromagnetic Interfaces

    Science.gov (United States)

    Koon, N. C.

    1997-06-01

    A microscopic explanation of exchange bias in thin films with compensated ferro/antiferromagnetic interfaces is presented. Full micromagnetic calculations show the interfacial exchange coupling to be relatively strong with a perpendicular orientation between the ferro/antiferromagnetic axis directions, similar to the classic ``spin-flop'' state in bulk antiferromagnets. With reasonable parameters the calculations predict bias fields comparable to those observed and provide a possible explanation for both anomalous high field rotational hysteresis and recently discovered ``positive'' exchange bias.

  10. Quantum spin liquid and spin ice states in new pyrochlores

    Science.gov (United States)

    Sibille, Romain

    Magnetic systems with competing interactions can adopt exotic ground states. A particularly promising class is that of the geometrically frustrated magnets, such as the A2B2O7 pyrochlores, in which unusual spin liquids appear. Some of these phases feature short-range correlated states analogous to a Coulomb phase and give rise to emergent quasiparticle excitations. Although cases like the classical spin ice are reasonably well understood, the theoretical expectation is that quantum fluctuations lead to novel phases which are quantum spin liquids (QSLs). For instance, the quantum spin ice (QSI) is a generalization of the classical spin ice state to include quantum fluctuations, such that the effective theory becomes emergent quantum electrodynamics - the classical monopoles become coherent quantum quasiparticles, and a novel excitation playing the role of the photon appears. In this talk, I will present results on three novel materials with potential for QSL states. Each of them corresponds to a way to potentially strengthen the role of quantum fluctuations on the ground state properties of pyrochlore magnets. Firstly, I will demonstrate that, in Tb2Hf2O7, where a sizeable gap isolates the non-Kramers ground state doublet at low temperature, a large amount of anion Frenkel disorder leads to quenched random crystal fields and disordered magnetic interactions. The detailed study of this material demonstrates that disorder can play a crucial role in preventing long-range magnetic order at low temperatures, and instead induces a strongly-fluctuating Coulomb spin liquid with defect-induced frozen magnetic degrees of freedom. Secondly, I will present results on another QSL candidate based on non-Kramers ions, Pr2Hf2O7, which displays striking characteristics of the ferromagnetic correlations expected in a QSI. Finally, in the pyrochlore Ce2Sn2O7, where macroscopic measurements suggest an antiferromagnetic liquid ground state with quantum fluctuations, I will present

  11. Magnonic topological insulators in antiferromagnets

    Science.gov (United States)

    Nakata, Kouki; Kim, Se Kwon; Klinovaja, Jelena; Loss, Daniel

    2017-12-01

    Extending the notion of symmetry protected topological phases to insulating antiferromagnets (AFs) described in terms of opposite magnetic dipole moments associated with the magnetic N e ´el order, we establish a bosonic counterpart of topological insulators in semiconductors. Making use of the Aharonov-Casher effect, induced by electric field gradients, we propose a magnonic analog of the quantum spin Hall effect (magnonic QSHE) for edge states that carry helical magnons. We show that such up and down magnons form the same Landau levels and perform cyclotron motion with the same frequency but propagate in opposite direction. The insulating AF becomes characterized by a topological Z2 number consisting of the Chern integer associated with each helical magnon edge state. Focusing on the topological Hall phase for magnons, we study bulk magnon effects such as magnonic spin, thermal, Nernst, and Ettinghausen effects, as well as the thermomagnetic properties of helical magnon transport both in topologically trivial and nontrivial bulk AFs and establish the magnonic Wiedemann-Franz law. We show that our predictions are within experimental reach with current device and measurement techniques.

  12. Spin-charge separation in the t-J model: Magnetic and transport anomalies

    International Nuclear Information System (INIS)

    Weng, Z.Y.; Sheng, D.N.; Ting, C.S.

    1995-01-01

    A real spin-charge separation scheme is found based on a saddle-point state of the t-J model. In the one-dimensional (1D) case, such a saddle-point reproduces the correct asymptotic correlations at the strong-coupling fixed point of the model. In the two-dimensional (2D) case, the transverse gauge field confining spinon and holon is shown to be gapped at finite doping so that a spin-charge deconfinement is obtained for its first time in 2D. The gap in the gauge fluctuation disappears at half-filling limit, where a long-range antiferromagnetic order is recovered at zero temperature and spinons become confined. The most interesting features of spin dynamics and transport are exhibited at finite doping where exotic residual couplings between spin and charge degrees of freedom lead to systematic anomalies with regard to a Fermi-liquid system. In spin dynamics, a commensurate antiferromagnetic fluctuation with a small, doping-dependent energy scale is found, which is characterized in momentum space by a Gaussian peak at (π/a,π/a) with a doping-dependent width. This commensurate magnetic fluctuation contributes a non-Korringa behavior for the NMR spin-lattice relaxation rate. There also exists a characteristic temperature scale below thich a pseudogap behavior appears in the spin dynamics. Furthermore, an incommensurate magnetic fluctuation is also obtained at a finite energy regime. In the transport, a strong-range phase intereference leads to an effective holon Lagrangian which can give rise to a series of interesting phenomena including linear-T resistivity and a T 2 Hall angle. We discuss the striking similarities of these theoretical features with those found in the high-T c cuprates and give a consistent picture for the latter. Electronic properties like Fermi surface and superconducting pairing in this framework are also discussed

  13. Electrical manipulation of a ferromagnet by an antiferromagnet

    Science.gov (United States)

    Tshitoyan, V.; Ciccarelli, C.; Mihai, A. P.; Ali, M.; Irvine, A. C.; Moore, T. A.; Jungwirth, T.; Ferguson, A. J.

    Several recent studies of antiferromagnetic (AFM) spintronics have focused on transmission and detection of spin-currents in AFMs. Efficient spin transmission through AFMs was inferred from experiments in FM/AFM/NM (normal metal) structures. Measurements in FM/AFM bilayers have demonstrated that a metallic AFM can also act as an efficient ISHE detector of the spin-current, with spin-Hall angles comparable to heavy NMs. Here we demonstrate that an antiferromagnet can be employed for a highly efficient electrical manipulation of a ferromagnet. We use an all-electrical excitation and detection technique of ferromagnetic resonance in a NiFe/IrMn bilayer. We observe antidamping-like spin torque acting on the NiFe generated by the in-plane current driven through the IrMn antiferromagnet. A large enhancement of the torque, characterized by an effective spin-Hall angle exceeding most heavy transition metals, correlates with the presence of the exchange-bias field at the NiFe/IrMn interface. It highlights that, in addition to strong spin-orbit coupling, the AFM order in IrMn governs the observed phenomenon.

  14. Spin and isospin fluctuations in heavy ion collisions and their dependence upon the shape of the dinuclear complex

    International Nuclear Information System (INIS)

    Moretto, L.G.

    1980-08-01

    The relevance of higher multipoles of giant isovector modes in the charge distribution of deep inelastic fragments is discussed and found to depend strongly on mass asymmetry. The sources of angular momentum fluctuations are investigated. Quantal effects are considered as well as effects arising from non-equilibrium and equilibrium statistical fluctuations. A model based upon equilibrium statistical mechanics is considered in detail, and used to predict both 2nd moments of the angular momentum distributions and the angular momentum misalignment. Analytical expressions are derived to calculate the angular distributions of sequentially emitted particles, fission fragments, as well as gamma rays in terms of the angular momentum misalignment. Recent data on the angular distributions of sequential alphas, fission and gamma rays are analyzed in terms of the model. 29 figures, 1 table

  15. Spin and isospin fluctuations in heavy ion collisions and their dependence upon the shape of the dinuclear complex

    Energy Technology Data Exchange (ETDEWEB)

    Moretto, L.G.

    1980-08-01

    The relevance of higher multipoles of giant isovector modes in the charge distribution of deep inelastic fragments is discussed and found to depend strongly on mass asymmetry. The sources of angular momentum fluctuations are investigated. Quantal effects are considered as well as effects arising from non-equilibrium and equilibrium statistical fluctuations. A model based upon equilibrium statistical mechanics is considered in detail, and used to predict both 2nd moments of the angular momentum distributions and the angular momentum misalignment. Analytical expressions are derived to calculate the angular distributions of sequentially emitted particles, fission fragments, as well as gamma rays in terms of the angular momentum misalignment. Recent data on the angular distributions of sequential alphas, fission and gamma rays are analyzed in terms of the model. 29 figures, 1 table.

  16. Nanoparticles of antiferromagnetic materials

    DEFF Research Database (Denmark)

    Madsen, Daniel Esmarch

    2008-01-01

    I denne Ph.D. afhandling studeres forskellige egenskaber ved antiferromagnetiske nanopartikler. I en ideel antiferromagnet er spinnene orienteret således at der ikke er et resulterende magnetisk moment. I nanopartikler af antiferromagnetiske materialer er denne kompensation på grund af forskellig...

  17. Prospect for antiferromagnetic spintronics

    Czech Academy of Sciences Publication Activity Database

    Martí, Xavier; Fina, I.; Jungwirth, Tomáš

    2015-01-01

    Roč. 51, č. 4 (2015), s. 2900104 ISSN 0018-9464 R&D Projects: GA MŠk(CZ) LM2011026; GA ČR GB14-37427G EU Projects: European Commission(XE) 268066 - 0MSPIN Institutional support: RVO:68378271 Keywords : spintronics * antiferromagnets Subject RIV: BM - Solid Matter Physics ; Magnetism Impact factor: 1.277, year: 2015

  18. Synthetic antiferromagnetic spintronics

    Science.gov (United States)

    Duine, R. A.; Lee, Kyung-Jin; Parkin, Stuart S. P.; Stiles, M. D.

    2018-03-01

    Spintronic and nanomagnetic devices often derive their functionality from layers of different materials and the interfaces between them. We discuss the opportunities that arise from synthetic antiferromagnets consisting of two or more ferromagnetic layers that are separated by metallic spacers or tunnel barriers and have antiparallel magnetizations.

  19. Kinetically inhibited order in a diamond-lattice antiferromagnet

    Science.gov (United States)

    MacDougall, Gregory J.; Gout, Delphine; Zarestky, Jerel L.; Ehlers, Georg; Podlesnyak, Andrey; McGuire, Michael A.; Mandrus, David; Nagler, Stephen E.

    2011-01-01

    Frustrated magnetic systems exhibit highly degenerate ground states and strong fluctuations, often leading to new physics. An intriguing example of current interest is the antiferromagnet on a diamond lattice, realized physically in A-site spinel materials. This is a prototypical system in three dimensions where frustration arises from competing interactions rather than purely geometric constraints, and theory suggests the possibility of unusual magnetic order at low temperature. Here, we present a comprehensive single-crystal neutron scattering study of CoAl2O4, a highly frustrated A-site spinel. We observe strong diffuse scattering that peaks at wavevectors associated with Néel ordering. Below the temperature T∗ = 6.5 K, there is a dramatic change in the elastic scattering lineshape accompanied by the emergence of well-defined spin-wave excitations. T∗ had previously been associated with the onset of glassy behavior. Our new results suggest instead that T∗ signifies a first-order phase transition, but with true long-range order inhibited by the kinetic freezing of domain walls. This scenario might be expected to occur widely in frustrated systems containing first-order phase transitions and is a natural explanation for existing reports of anomalous glassy behavior in other materials. PMID:21896723

  20. Spin-polarized current in noncollinear antiferromagnets

    Czech Academy of Sciences Publication Activity Database

    Železný, Jakub; Zhang, Y.; Felser, C.; Yan, B.

    2017-01-01

    Roč. 119, č. 18 (2017), s. 1-7, č. článku 187204. ISSN 0031-9007 Institutional support: RVO:68378271 Keywords : anisotropic magnetoresistance * wannier functions * room-temperature * torques * spintronics Subject RIV: BM - Solid Matter Physics ; Magnetism OBOR OECD: Condensed matter physics (including formerly solid state physics, supercond.) Impact factor: 8.462, year: 2016

  1. Is gadolinium a helical antiferromagnet or a collinear ferromagnet?

    Indian Academy of Sciences (India)

    as low as 15 Oe suffice to transform the helical antiferromagnetism into collinear ferro- magnetism. This picture of the spin structure in Gd had to be discarded after subsequent. £Article presented at the International Symposium on Advances in Superconductivity and Mag- netism: Materials, Mechanisms and Devices, ...

  2. Observation of Antiferromagnetic Resonance in an Organic Superconductor

    DEFF Research Database (Denmark)

    Torrance, J. B.; Pedersen, H. J.; Bechgaard, K.

    1982-01-01

    Anomalous microwave absorption has been observed in the organic superconductor TMTSF2AsF6 (TMTSF: tetramethyltetraselenafulvalene) below its metal-nonmetal transition near 12 K. This absorption is unambiguously identified as antiferromagnetic resonance by the excellent agreement between a spin...

  3. Monopoles in an Antiferromagnetic Bose-Einstein Condensate

    NARCIS (Netherlands)

    Stoof, H.T.C.; Vliegen, E.; Al Khawaja, U.

    2001-01-01

    We show that even in three dimensions an antiferromagnetic spin-1 Bose-Einstein condensate, which can, for instance, be created with 23Na atoms in an optical trap, has not only singular linelike vortex excitations, but also allows for singular pointlike topological excitations, i.e., monopoles

  4. Ferro- and antiferro-magnetism in (Np, Pu)BC

    Czech Academy of Sciences Publication Activity Database

    Klimczuk, T.; Shick, Alexander; Kozub, Agnieszka L.; Griveau, J.C.; Colineau, E.; Falmbigl, M.; Wastin, F.; Rogl, P.

    2015-01-01

    Roč. 3, č. 4 (2015), "041803-1"-"041803-9" ISSN 2166-532X R&D Projects: GA ČR GA15-07172S Institutional support: RVO:68378271 Keywords : ferromagetism * antiferromagnetism * magnetic anisotropy * strong electron correlations * spin-orbit coupling Subject RIV: BM - Solid Matter Physics ; Magnetism Impact factor: 4.323, year: 2015

  5. Broken discrete and continuous symmetries in two-dimensional spiral antiferromagnets

    International Nuclear Information System (INIS)

    Mezio, A; Sposetti, C N; Manuel, L O; Trumper, A E

    2013-01-01

    We study the occurrence of symmetry breaking, at zero and finite temperatures, in the J 1 –J 3 antiferromagnetic Heisenberg model on the square lattice using Schwinger boson mean field theory. For spin- 1/2 the ground state always breaks the SU(2) symmetry with a continuous quasi-critical transition at J 3 /J 1 ∼ 0.38, from Néel to spiral long range order, although local spin fluctuation considerations suggest an intermediate disordered regime around 0.35 ≲ J 3 /J 1 ≲ 0.5, in qualitative agreement with recent numerical results. At low temperatures we find a Z 2 broken symmetry region with short range spiral order characterized by an Ising-like nematic order parameter that compares qualitatively well with classical Monte Carlo results. At intermediate temperatures the phase diagram shows regions with collinear short range orders: for J 3 /J 1 3 /J 1 > 1 a novel phase consisting of four decoupled third neighbour sublattices with Néel (π,π) correlations in each one. We conclude that the effect of quantum and thermal fluctuations is to favour collinear correlations even in the strongly frustrated regime. (paper)

  6. Broken discrete and continuous symmetries in two-dimensional spiral antiferromagnets

    Science.gov (United States)

    Mezio, A.; Sposetti, C. N.; Manuel, L. O.; Trumper, A. E.

    2013-11-01

    We study the occurrence of symmetry breaking, at zero and finite temperatures, in the J1-J3 antiferromagnetic Heisenberg model on the square lattice using Schwinger boson mean field theory. For spin-\\frac{1}{2} the ground state always breaks the SU(2) symmetry with a continuous quasi-critical transition at J3/J1 ˜ 0.38, from Néel to spiral long range order, although local spin fluctuation considerations suggest an intermediate disordered regime around 0.35 ≲ J3/J1 ≲ 0.5, in qualitative agreement with recent numerical results. At low temperatures we find a Z2 broken symmetry region with short range spiral order characterized by an Ising-like nematic order parameter that compares qualitatively well with classical Monte Carlo results. At intermediate temperatures the phase diagram shows regions with collinear short range orders: for J3/J1 1 a novel phase consisting of four decoupled third neighbour sublattices with Néel (π,π) correlations in each one. We conclude that the effect of quantum and thermal fluctuations is to favour collinear correlations even in the strongly frustrated regime.

  7. Superfluid and antiferromagnetic phases in ultracold fermionic quantum gases

    Energy Technology Data Exchange (ETDEWEB)

    Gottwald, Tobias

    2010-08-27

    domain wall formation, antiferromagnetically induced density shifts, and we show the relevant role of spin-imbalance for antiferromagnetic states. Since the first step for understanding the physics of the examined models was the application of a mean field approximation, we analyze the effect of including the second order terms of the weak coupling perturbation expansion for the repulsive model. We show that our results survive the influence of quantum fluctuations and show that the renormalization factors for order parameters and critical temperatures lead to a weaker influence of the fluctuations on the results in finite sized systems than on the results in the thermodynamical limit. Furthermore, in the context of second order theory we address the question whether results obtained in the dynamical mean field theory (DMFT), which is meanwhile a frequently used method for describing trapped systems, survive the effect of the non-local Feynman diagrams neglected in DMFT. (orig.)

  8. Superfluid and antiferromagnetic phases in ultracold fermionic quantum gases

    International Nuclear Information System (INIS)

    Gottwald, Tobias

    2010-01-01

    domain wall formation, antiferromagnetically induced density shifts, and we show the relevant role of spin-imbalance for antiferromagnetic states. Since the first step for understanding the physics of the examined models was the application of a mean field approximation, we analyze the effect of including the second order terms of the weak coupling perturbation expansion for the repulsive model. We show that our results survive the influence of quantum fluctuations and show that the renormalization factors for order parameters and critical temperatures lead to a weaker influence of the fluctuations on the results in finite sized systems than on the results in the thermodynamical limit. Furthermore, in the context of second order theory we address the question whether results obtained in the dynamical mean field theory (DMFT), which is meanwhile a frequently used method for describing trapped systems, survive the effect of the non-local Feynman diagrams neglected in DMFT. (orig.)

  9. Untersuchung der magnetischen und strukturellen Eigenschaften der beiden niedrigdimensionalen Antiferromagnete TiPO4 und CrOCl

    OpenAIRE

    Reuvekamp, Patrick Gerald

    2014-01-01

    Titanium (III) phosphate TiPO4 (3d1 electronic configuration with S = 1/2) is a one-dimensional quantum antiferromagnet exhibiting non-conventional spin-Peierls behaviour at low temperatures. Chromium oxychloride CrOCl (3d3 electronic configuration with S = 3/2) is a two-dimensional antiferromagnet consisting of ferromagnetic spin chains interconnected by competing anti and ferromagnetic spin exchanges interactions. The magnetic and the structural properties of these compounds are intimately ...

  10. Walls, anomalies, and deconfinement in quantum antiferromagnets

    Science.gov (United States)

    Komargodski, Zohar; Sulejmanpasic, Tin; Ünsal, Mithat

    2018-02-01

    We consider the Abelian-Higgs model in 2 +1 dimensions with instanton-monopole defects. This model is closely related to the phases of quantum antiferromagnets. In the presence of Z2 preserving monopole operators, there are two confining ground states in the monopole phase, corresponding to the valence bond solid (VBS) phase of quantum magnets. We show that the domain wall carries a 't Hooft anomaly in this case. The anomaly can be saturated by, e.g., charge-conjugation breaking on the wall or by the domain wall theory becoming gapless (a gapless model that saturates the anomaly is S U (2) 1 WZW). Either way the fundamental scalar particles (i.e., spinons) which are confined in the bulk are deconfined on the domain wall. This Z2 phase can be realized either with spin-1/2 on a rectangular lattice or spin-1 on a square lattice. In both cases the domain wall contains spin-1/2 particles (which are absent in the bulk). We discuss the possible relation to recent lattice simulations of domain walls in VBS. We further generalize the discussion to Abrikosov-Nielsen-Olsen (ANO) vortices in a dual superconductor of the Abelian-Higgs model in 3 +1 dimensions and to the easy-plane limit of antiferromagnets. In the latter case the wall can undergo a variant of the BKT transition (consistent with the anomalies) while the bulk is still gapped. The same is true for the easy-axis limit of antiferromagnets. We also touch upon some analogies to Yang-Mills theory.

  11. Correlations, spin dynamics, defects: the highly-frustrated Kagome bilayer

    International Nuclear Information System (INIS)

    Bono, David; Limot, Laurent; Mendels, Philippe; Collin Gaston; Blanchard Nicole

    2005-01-01

    The SrCr 9p Ga 1 -2 -9p O 19 and Ba 2 Sn 2 ZnGa 10-7p Cr 7p O 22 compounds are two highly-frustrated magnets possessing a quasi-two-dimensional Kagome bilayer of spin 3/2 chromium ions with antiferromagnetic interactions. Their magnetic susceptibility was measured by local nuclear magnetic resonance and nonlocal (SQUID) techniques, and their low-temperature spin dynamics by muon spin resonance. Consistent with the theoretical picture drawn for geometrically frustrated systems, the Kagome bilayer is shown here to exhibit: (i) short range spin-spin correlations down to a temperature much lower than the Curie-Weiss temperature, no conventional long-range transition occurring; (ii) a Curie contribution to the susceptibility from paramagnetic defects generated by spin vacancies; (iii) low-temperature spin fluctuations, at least down to 30 mK, which are a trademark of a dynamical ground state. These properties point to a spin-liquid ground state, possibly built on resonating valence bonds with unconfined spinons as the magnetic excitations

  12. Thermoelectric properties of layered antiferromagnetic CuCrSe2

    International Nuclear Information System (INIS)

    Tewari, Girish C.; Tripathi, T.S.; Yamauchi, Hisao; Karppinen, Maarit

    2014-01-01

    Here we study thermoelectric and magnetic properties of CuCrSe 2 samples sintered at various temperatures. Structural analysis with XRD shows an order-disorder transition for Cr atoms when the sintering temperature is increased above 1273 K. Metal-like electrical resistivity and anomalously large Seebeck coefficient are found about room temperature. Analysis of electrical conductivity and Seebeck coefficient of the partially-disordered phase suggests hopping conduction of charge carriers. For both the ordered and disordered phases magnetic susceptibility follows Curie–Weiss temperature dependence at high temperatures above 150 K and shows an antiferromagnetic transition around 55 K. For the disordered phase, the effective magnetic moment is determined at 3.62 μ B ; this low value in comparison to the spin only value for Cr 3+ of 3.89 μ B indicates spin fluctuations in the paramagnetic state. The thermal conductivity in these phases is low and dominated by the lattice contribution. Values for the thermoelectric figure of merit (ZT) at room temperature are estimated to be 0.17 and 0.05 for the ordered and disordered phases, respectively. - Highlights: • Thermoelectric and magnetic properties of CuCrSe 2 samples are investigated. • The properties strongly depend on the degree of order of chromium atoms. • The degree of order is controlled by the sintering temperature. • Room-temperature figure of merit is estimated at 0.17 for the ordered phase. • For the disordered phase the figure of merit is lower

  13. Concepts of antiferromagnetic spintronics

    Czech Academy of Sciences Publication Activity Database

    Gomonay, O.; Jungwirth, Tomáš; Sinova, Jairo

    2017-01-01

    Roč. 11, č. 4 (2017), 1-8, č. článku 1700022. ISSN 1862-6254 R&D Projects: GA MŠk LM2015087; GA ČR GB14-37427G Institutional support: RVO:68378271 Keywords : spintronics * antiferromagnets Subject RIV: BM - Solid Matter Physics ; Magnetism OBOR OECD: Condensed matter physics (including formerly solid state physics, supercond.) Impact factor: 3.032, year: 2016

  14. Isothermal anisotropic magnetoresistance in antiferromagnetic metallic IrMn.

    Science.gov (United States)

    Galceran, R; Fina, I; Cisneros-Fernández, J; Bozzo, B; Frontera, C; López-Mir, L; Deniz, H; Park, K-W; Park, B-G; Balcells, Ll; Martí, X; Jungwirth, T; Martínez, B

    2016-10-20

    Antiferromagnetic spintronics is an emerging field; antiferromagnets can improve the functionalities of ferromagnets with higher response times, and having the information shielded against external magnetic field. Moreover, a large list of aniferromagnetic semiconductors and metals with Néel temperatures above room temperature exists. In the present manuscript, we persevere in the quest for the limits of how large can anisotropic magnetoresistance be in antiferromagnetic materials with very large spin-orbit coupling. We selected IrMn as a prime example of first-class moment (Mn) and spin-orbit (Ir) combination. Isothermal magnetotransport measurements in an antiferromagnetic-metal(IrMn)/ferromagnetic-insulator thin film bilayer have been performed. The metal/insulator structure with magnetic coupling between both layers allows the measurement of the modulation of the transport properties exclusively in the antiferromagnetic layer. Anisotropic magnetoresistance as large as 0.15% has been found, which is much larger than that for a bare IrMn layer. Interestingly, it has been observed that anisotropic magnetoresistance is strongly influenced by the field cooling conditions, signaling the dependence of the found response on the formation of domains at the magnetic ordering temperature.

  15. Relativistic Néel-Order Fields Induced by Electrical Current in Antiferromagnets

    KAUST Repository

    Železný, J.

    2014-10-06

    We predict that a lateral electrical current in antiferromagnets can induce nonequilibrium Néel-order fields, i.e., fields whose sign alternates between the spin sublattices, which can trigger ultrafast spin-axis reorientation. Based on microscopic transport theory calculations we identify staggered current-induced fields analogous to the intraband and to the intrinsic interband spin-orbit fields previously reported in ferromagnets with a broken inversion-symmetry crystal. To illustrate their rich physics and utility, we consider bulk Mn2Au with the two spin sublattices forming inversion partners, and a 2D square-lattice antiferromagnet with broken structural inversion symmetry modeled by a Rashba spin-orbit coupling. We propose an antiferromagnetic memory device with electrical writing and reading.

  16. Brownian motion and entropic torque driven motion of domain walls in antiferromagnets

    Science.gov (United States)

    Yan, Zhengren; Chen, Zhiyuan; Qin, Minghui; Lu, Xubing; Gao, Xingsen; Liu, Junming

    2018-02-01

    We study the spin dynamics in antiferromagnetic nanowire under an applied temperature gradient using micromagnetic simulations on a classical spin model with a uniaxial anisotropy. The entropic torque driven domain-wall motion and the Brownian motion are discussed in detail, and their competition determines the antiferromagnetic wall motion towards the hotter or colder region. Furthermore, the spin dynamics in an antiferromagnet can be well tuned by the anisotropy and the temperature gradient. Thus, this paper not only strengthens the main conclusions obtained in earlier works [Kim et al., Phys. Rev. B 92, 020402(R) (2015), 10.1103/PhysRevB.92.020402; Selzer et al., Phys. Rev. Lett. 117, 107201 (2016), 10.1103/PhysRevLett.117.107201], but more importantly gives the concrete conditions under which these conclusions apply, respectively. Our results may provide useful information on the antiferromagnetic spintronics for future experiments and storage device design.

  17. Topological Excitations in Quantum Spin Systems

    Directory of Open Access Journals (Sweden)

    Ranjan Chaudhury

    2013-01-01

    Full Text Available The origin and significance of topological excitations in quantum spin models in low dimensions are presented in detail. Besides a general review, our own work in this area is described in great depth. Apart from theoretical analysis of the existence and properties of spin vortices and antivortices, the possible experimental consequences and signatures are also highlighted. In particular, the distinguishing features between the even and odd charged topological excitations are brought out through a detailed analysis of the topological term in the quantum action. Moreover, an interesting symmetry property is predicted between the excitations from a ferromagnetic model and an antiferromagnetic model. Through a novel approach of ours, a bridge is established between field theoretical formalism and the well-known statistical mechanical treatment of Berezinskii-Kosterlitz-Thouless (BKT transition involving these topological excitations. Furthermore, a detailed phenomenological analysis of the experimentally observed static and dynamic magnetic properties of the layered magnetic materials, possessing XY anisotropy in the in-plane spin-spin couplings, is undertaken to test the theoretical predictions regarding the behaviour of these excitations. The importance and the crucial role of quantum spin fluctuations in these studies are also brought out very clearly by our analysis.

  18. Quantum phase transitions in effective spin-ladder models for graphene zigzag nanoribbons

    Science.gov (United States)

    Koop, Cornelie; Wessel, Stefan

    2017-10-01

    We examine the magnetic correlations in quantum spin models that were derived recently as effective low-energy theories for electronic correlation effects on the edge states of graphene nanoribbons. For this purpose, we employ quantum Monte Carlo simulations to access the large-distance properties, accounting for quantum fluctuations beyond mean-field-theory approaches to edge magnetism. For certain chiral nanoribbons, antiferromagnetic interedge couplings were previously found to induce a gapped quantum disordered ground state of the effective spin model. We find that the extended nature of the intraedge couplings in the effective spin model for zigzag nanoribbons leads to a quantum phase transition at a large, finite value of the interedge coupling. This quantum critical point separates the quantum disordered region from a gapless phase of stable edge magnetism at weak intraedge coupling, which includes the ground states of spin-ladder models for wide zigzag nanoribbons. To study the quantum critical behavior, the effective spin model can be related to a model of two antiferromagnetically coupled Haldane-Shastry spin-half chains with long-ranged ferromagnetic intrachain couplings. The results for the critical exponents are compared also to several recent renormalization-group calculations for related long-ranged interacting quantum systems.

  19. Weyl magnons in noncoplanar stacked kagome antiferromagnets

    Science.gov (United States)

    Owerre, S. A.

    2018-03-01

    Weyl nodes have been experimentally realized in photonic, electronic, and phononic crystals. However, magnonic Weyl nodes are yet to be seen experimentally. In this paper, we propose Weyl magnon nodes in noncoplanar stacked frustrated kagome antiferromagnets, naturally available in various real materials. Most crucially, the Weyl nodes in the current system occur at the lowest excitation and possess a topological thermal Hall effect, therefore they are experimentally accessible at low temperatures due to the population effect of bosonic quasiparticles. In stark contrast to other magnetic systems, the current Weyl nodes do not rely on time-reversal symmetry breaking by the magnetic order. Rather, they result from explicit macroscopically broken time reversal symmetry by the scalar spin chirality of noncoplanar spin textures and can be generalized to chiral spin liquid states. Moreover, the scalar spin chirality gives a real space Berry curvature which is not available in previously studied magnetic Weyl systems. We show the existence of magnon arc surface states connecting projected Weyl magnon nodes on the surface Brillouin zone. We also uncover the first realization of triply-degenerate nodal magnon point in the noncollinear regime with zero scalar spin chirality.

  20. Misjudging frustrations in spin liquids from oversimplified use of Curie-Weiss law

    Energy Technology Data Exchange (ETDEWEB)

    Nag, Abhishek, E-mail: msan@iacs.res.in [Department of Materials Science, Indian Association for the Cultivation of Science, Jadavpur, Kolkata 700032 (India); Ray, Sugata [Department of Materials Science, Indian Association for the Cultivation of Science, Jadavpur, Kolkata 700032 (India); Centre for Advanced Materials, Indian Association for the Cultivation of Science, Jadavpur, Kolkata 700032 (India)

    2017-02-15

    Absence of a single smoking-gun experiment to identify a quantum spin liquid, has kept their characterisation difficult till date. Featureless dc magnetic susceptibility and large antiferromagnetic frustration are always considered as the essential pointers to these systems. However, we show that the amount of frustration estimated by using generalised Curie-Weiss law on these susceptibility data are prone to errors and thus should be dealt with caution. We measure and analyse susceptibility data of Ba{sub 3}ZnIr{sub 2}O{sub 9}, a spin orbital liquid candidate and Gd{sub 2}O{sub 3}, a 1.5 K antiferromagnet and show the distinguishing features between them. A continuous and significant change in Curie and Weiss constants is seen to take place in Ba{sub 3}ZnIr{sub 2}O{sub 9} and other reported spin liquids with the change in the range of fitting temperatures showing the need of a temperature ‘range-of-fit’ analysis before commenting on the Weiss constants of spin liquids. The variation observed is similar to fluctuations among topological sectors persisting over a range of temperature in spin-ice candidates. On the other hand, even though we find correlations to exist at even 100 times the ordering temperature in Gd{sub 2}O{sub 3}, no such fluctuation is observed which may be used as an additional distinguishing signature of spin liquids over similarly featureless correlated paramagnets. - Highlights: • Curie-Weiss fitting may give erroneous frustration parameters in spin-liquids. • The results depend upon choice of fitting method and temperature range used. • More appropriate method is to use a ʽrange of fit’ analysis. • Can distinguish between spin-liquids and correlated paramagnets.

  1. Development of antiferromagnetic Heusler alloys for the replacement of iridium as a critically raw material

    Science.gov (United States)

    Hirohata, Atsufumi; Huminiuc, Teodor; Sinclair, John; Wu, Haokaifeng; Samiepour, Marjan; Vallejo-Fernandez, Gonzalo; O'Grady, Kevin; Balluf, Jan; Meinert, Markus; Reiss, Günter; Simon, Eszter; Khmelevskyi, Sergii; Szunyogh, Laszlo; Yanes Díaz, Rocio; Nowak, Ulrich; Tsuchiya, Tomoki; Sugiyama, Tomoko; Kubota, Takahide; Takanashi, Koki; Inami, Nobuhito; Ono, Kanta

    2017-11-01

    As a platinum group metal, iridium (Ir) is the scarcest element on the earth but it has been widely used as an antiferromagnetic layer in magnetic recording, crucibles and spark plugs due to its high melting point. In magnetic recording, antiferromagnetic layers have been used to pin its neighbouring ferromagnetic layer in a spin-valve read head in a hard disk drive for example. Recently, antiferromagnetic layers have also been found to induce a spin-polarised electrical current. In these devices, the most commonly used antiferromagnet is an Ir-Mn alloy because of its corrosion resistance and the reliable magnetic pinning of adjacent ferromagnetic layers. It is therefore crucial to explore new antiferromagnetic materials without critical raw materials. In this review, recent research on new antiferromagnetic Heusler alloys and their exchange interactions along the plane normal is discussed. These new antiferromagnets are characterised by very sensitive magnetic and electrical measurement techniques recently developed to determine their characteristic temperatures together with atomic structural analysis. Mn-based alloys and compounds are found to be most promising based on their robustness against atomic disordering and large pinning strength up to 1.4 kOe, which is comparable with that for Ir-Mn. The search for new antiferromagnetic films and their characterisation are useful for further miniaturisation and development of spintronic devices in a sustainable manner.

  2. Absence of low energy magnetic spin-fluctuations in isovalently and aliovalently doped LaCo2B2 superconducting compounds

    Science.gov (United States)

    Majumder, M.; Ghoshray, A.; Khuntia, P.; Mazumdar, C.; Poddar, A.; Baenitz, M.; Ghoshray, K.

    2016-09-01

    Magnetization, resistivity and 11B, 59Co NMR measurements have been performed on the Pauli paramagnet \\text{LaC}{{\\text{o}}2}{{\\text{B}}2} , and the superconductors \\text{L}{{\\text{a}}0.9}{{\\text{Y}}0.1}\\text{C}{{\\text{o}}2}{{\\text{B}}2} ({{T}\\text{c}}≈ 4.2 K) and \\text{La}{{≤ft(\\text{C}{{\\text{o}}0.7}\\text{F}{{\\text{e}}0.3}\\right)}2}{{\\text{B}}2} ({{T}\\text{c}}≈ 5.8 K). The site selective NMR experiment reveals the multiband nature of the Fermi surface in these systems. The temperature independent Knight shift and 1/T 1 T clearly indicate the absence of correlated low energy magnetic spin-fluctuations in the normal state, which is in contrast to other Fe-based pnictides. The density of states (DOS) of Co 3d electrons has been enhanced in superconducting \\text{L}{{\\text{a}}0.9}{{\\text{Y}}0.1}\\text{C}{{\\text{o}}2}{{\\text{B}}2} and \\text{La}{{≤ft(\\text{C}{{\\text{o}}0.7}\\text{F}{{\\text{e}}0.3}\\right)}2}{{\\text{B}}2} with respect to the non superconducting reference compound \\text{LaC}{{\\text{o}}2}{{\\text{B}}2} . The occurrence of superconductivity is related to the DOS enhancement.

  3. Fluctuation-induced first-order transition in Eu-based trillium lattices

    Science.gov (United States)

    Franco, Diego G.; Prots, Yurii; Geibel, Christoph; Seiro, Silvia

    2017-07-01

    Among spin arrangements prone to geometric frustration, the so-called trillium lattice has not been very intensively investigated. A few theoretical works show that it is at the border between a degenerate, an only partially ordered, and a fully ordered ground state. However, only few compounds with this structure have been studied, and there is presently no good example of a trillium lattice with an antiferromagnetic ground state and clear evidence for frustration effects. We present magnetic and specific heat measurements on two realizations of a trillium lattice of local spins, EuPtSi and EuPtGe. Both compounds exhibit a similar magnetic behavior, with Eu2 + moments ordering antiferromagnetically at TN=4.1 K (EuPtSi) and 3.3 K (EuPtGe), albeit retaining a considerable amount of entropy in strong magnetic fluctuations extending to temperatures well above TN. The magnetic entropy reaches only roughly half of R ln8 at TN. These fluctuations are presumably the source for the pronounced first-order character of the transition at TN and are likely due to magnetic frustration. Thus, EuPtSi and EuPtGe open a new door to experimental studies of frustration effects in the trillium lattice and provide a testing ground for theoretical predictions.

  4. Effective Hamiltonian and low-lying eigenenergy clustering patterns of four-sublattice antiferromagnets

    DEFF Research Database (Denmark)

    Zhang, N.G.; Henley, C.L.; Rischel, C.

    2002-01-01

    We study the low-lying eigenenergy clustering patterns of quantum antiferromagnets with p sublattices (in particular p = 4). We treat each sublattice as a large spin, and using second-order degenerate perturbation theory, we derive the effective (biquadratic) Hamiltonian coupling the p large spins....... In order to compare with exact diagonalizations, the Hamiltonian is explicitly written for a finite-size lattice, and it contains information on energies of excited states as well as the ground state. The result is applied to the face-centered-cubic Type-I antiferromagnet of spin 1/2, including second...

  5. Nuclear spin pumping and electron spin susceptibilities

    NARCIS (Netherlands)

    Danon, J.; Nazarov, Y.V.

    2011-01-01

    In this work we present a new formalism to evaluate the nuclear spin dynamics driven by hyperfine interaction with nonequilibrium electron spins. To describe the dynamics up to second order in the hyperfine coupling it suffices to evaluate the susceptibility and fluctuations of the electron spin.

  6. Expansivity and heat capacity data for Lu and Sc crystals from 1 to 300 K: Spin-fluctuation and electron-phonon effects

    International Nuclear Information System (INIS)

    Swenson, C.A.

    1996-01-01

    Linear thermal expansivity (α) measurements from 1 to 300 K and heat capacity (C p ) measurements from 1 to 110 K are reported for single crystals of the hexagonal scandium and lutetium metals; the C p data were combined with previous data to obtain smooth representations to 305 K for Lu and 350 K for Sc. The Θ 0 close-quote s (352 and 190 K, respectively, for Sc and Lu) and γ close-quote s (10.38 and 8.30 mJ/molK 2 , respectively for Sc and Lu) are in reasonable agreement with previous data of various kinds. Electronic contributions are much larger for the α close-quote s than for the C p close-quote s, with the large anisotropies of the α close-quote s primarily electronic in origin. The equivalent Debye Θ close-quote s for the lattice C p close-quote s and the Grueneisen parameters Γ for the lattice α close-quote s both show an unexpected T dependence at open-quote open-quote high close-quote close-quote T (T approx-gt Θ 0 /2), which can be associated with the disappearance of spin-fluctuation and electron-phonon enhancements to the electronic properties; this effect has been reported previously for Sc C ν close-quote s by Pleschiutschnig et al. [Phys. Rev. B 44, 6794 (1991)]. While the resulting high-temperature open-quote open-quote bare close-quote close-quote or open-quote open-quote density of states close-quote close-quote γ for Sc, γ b =5.75(25) mJ/molK 2 , is slightly larger than that calculated recently by Goetz and Winter [J. Phys. Condens. Matter 5, 1721 (1993)], the magnitude of the sum (γ spin +γep) agrees well. For Lu, for which no recent calculations exist, γ b =5.50(25) mJ/molK 2 . (Abstract Truncated)

  7. Expansivity and heat capacity data for Lu and Sc crystals from 1 to 300 K: Spin-fluctuation and electron-phonon effects

    Energy Technology Data Exchange (ETDEWEB)

    Swenson, C.A. [Ames Laboratory and Department of Physics and Astronomy, Iowa State University, Ames, Iowa 50011 (United States)

    1996-02-01

    Linear thermal expansivity ({alpha}) measurements from 1 to 300 K and heat capacity ({ital C}{sub {ital p}}) measurements from 1 to 110 K are reported for single crystals of the hexagonal scandium and lutetium metals; the {ital C}{sub {ital p}} data were combined with previous data to obtain smooth representations to 305 K for Lu and 350 K for Sc. The {Theta}{sub 0}{close_quote}s (352 and 190 K, respectively, for Sc and Lu) and {gamma}{close_quote}s (10.38 and 8.30 mJ/molK{sup 2}, respectively for Sc and Lu) are in reasonable agreement with previous data of various kinds. Electronic contributions are much larger for the {alpha}{close_quote}s than for the {ital C}{sub {ital p}}{close_quote}s, with the large anisotropies of the {alpha}{close_quote}s primarily electronic in origin. The equivalent Debye {Theta}{close_quote}s for the lattice {ital C}{sub {ital p}}{close_quote}s and the Gr{umlt u}neisen parameters {Gamma} for the lattice {alpha}{close_quote}s both show an unexpected {ital T} dependence at {open_quote}{open_quote}high{close_quote}{close_quote} {ital T} ({ital T}{approx_gt}{Theta}{sub 0}/2), which can be associated with the disappearance of spin-fluctuation and electron-phonon enhancements to the electronic properties; this effect has been reported previously for Sc {ital C}{sub {nu}}{close_quote}s by Pleschiutschnig {ital et} {ital al}. [Phys. Rev. B {bold 44}, 6794 (1991)]. While the resulting high-temperature {open_quote}{open_quote}bare{close_quote}{close_quote} or {open_quote}{open_quote}density of states{close_quote}{close_quote} {gamma} for Sc, {gamma}{sub {ital b}}=5.75(25) mJ/molK{sup 2}, is slightly larger than that calculated recently by G{umlt o}tz and Winter [J. Phys. Condens. Matter {bold 5}, 1721 (1993)], the magnitude of the sum ({gamma}{sub spin}+{gamma}{ital ep}) agrees well. For Lu, for which no recent calculations exist, {gamma}{sub {ital b}}=5.50(25) mJ/molK{sup 2}. (Abstract Truncated)

  8. Ab initio dynamical exchange interactions in frustrated antiferromagnets

    Science.gov (United States)

    Simoni, Jacopo; Stamenova, Maria; Sanvito, Stefano

    2017-08-01

    The ultrafast response to an optical pulse excitation of the spin-spin exchange interaction in transition metal antiferromagnets is studied within the framework of the time-dependent spin-density functional theory. We propose a formulation for the full dynamical exchange interaction, which is nonlocal in space, and it is derived starting from ab initio arguments. Then, we investigate the effect of the laser pulse on the onset of the dynamical process. It is found that we can distinguish two types of excitations, both activated immediately after the action of the laser pulse. While the first one can be associated to a Stoner-like excitation and involves the transfer of spin from one site to another, the second one is related to the ultrafast modification of a Heisenberg-like exchange interaction and can trigger the formation of spin waves in the first few hundred femtoseconds of the time evolution.

  9. Spin-glass transition in disordered terbium

    International Nuclear Information System (INIS)

    Hauser, J.J.

    1985-01-01

    While crystalline Tb is a helix antiferromagnet with a Neel temperature of 229 K which becomes ferromagnetic at 222 K, disordered Tb exhibits a spin-glass transition. The spin-glass freezing temperature ranges from 183 to 53 K, the lowest temperatures corresponding to the greatest degree of atomic disorder. These experiments constitute the first evidence for an elemental spin-glass. (author)

  10. Metrologically useful states of spin-1 Bose condensates with macroscopic magnetization

    Science.gov (United States)

    Kajtoch, Dariusz; Pawłowski, Krzysztof; Witkowska, Emilia

    2018-02-01

    We study theoretically the usefulness of spin-1 Bose condensates with macroscopic magnetization in a homogeneous magnetic field for quantum metrology. We demonstrate Heisenberg scaling of the quantum Fisher information for states in thermal equilibrium. The scaling applies to both antiferromagnetic and ferromagnetic interactions. The effect preserves as long as fluctuations of magnetization are sufficiently small. Scaling of the quantum Fisher information with the total particle number is derived within the mean-field approach in the zero-temperature limit and exactly in the high-magnetic-field limit for any temperature. The precision gain is intuitively explained owing to subtle features of the quasidistribution function in the phase space.

  11. dx^2-y^2 paring symmetry of heavy fermion CeIrIn5 remote from antiferromagnetic quantum critical point

    Science.gov (United States)

    Kasahara, Yuichi; Iwasawa, T.; Shimizu, Y.; Shishido, H.; Shibauchi, T.; Vekhter, I.; Matsuda, Y.

    2008-03-01

    Quasi-two dimensional heavy Fermion CeIrIn5 involves two distinct superconducting domes in the phase diagram, which appear as a function of pressure or Rh substitution of Ir. In the analogy to CeCu2Si2, two distinct superconducting domes with different symmetry has been invoked. We report on the results of low-temperature thermal transport of CeIrIn5 in the second dome, which locates away from an antiferromagnetic quantum critical point. The thermal conductivity is measured under a magnetic field rotated with respect to the crystal axes, which give direct evidence for superconducting gap structure. Clear fourfold oscillation with minima at [110] and [1-10] directions is observed as rotating magnetic field within the basal ab-plane, while no oscillation is observed within the bc-plane. In sharp contrast to previous reports that suggested Eg symmetry with horizontal line node within the ab-plane [1], our results are most consistent with dx^2- y^2 symmetry with vertical line nodes along the c-axis. These results imply that two superconducting domes have the same gap symmetry which appears to be mediated by antiferromagnetic spin fluctuations. [1] H. Shakeripour et al., Phys. Rev. Lett. 99, 187004 (2007).

  12. Biaxial-stress-driven full spin polarization in ferromagnetic hexagonal chromium telluride

    Energy Technology Data Exchange (ETDEWEB)

    Xiao, Xiang-Bo; Li, Jun [Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences, Beijing 100190 (China); Liu, Bang-Gui, E-mail: bgliu@iphy.ac.cn [Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences, Beijing 100190 (China); School of Physical Sciences, University of Chinese Academy of Sciences, Beijing 100190 (China)

    2017-03-15

    It is important to spintronics to achieve fully-spin-polarized magnetic materials that are stable and can be easily fabricated. Here, through systematical density-functional-theory investigations, we achieve high and even full spin polarization for carriers in the ground-state phase of CrTe by applying tensile biaxial stress. The resulting strain is tensile in the xy plane and compressive in the z axis. With the in-plane tensile strain increasing, the ferromagnetic order is stable against antiferromagnetic fluctuations, and a half-metallic ferromagnetism is achieved at an in-plane strain of 4.8%. With the spin-orbit coupling taken into account, the spin polarization is equivalent to 97% at the electronic transition point, and then becomes 100.0% at the in-plane strain of 6.0%. These make us believe that the full-spin-polarized ferromagnetism in this stable and easily-realizable hexagonal phase could be realized soon, and applied in spintronics. - Highlights: • Full spin polarization in the hexagonal ground-state phase of CrTe by biaxial stress. • The stress produces in-plane tensile strain and perpendicular compressive strain. • Reliable electronic structure is calculated with improved exchange functional. • Spin polarization is calculated with spin-orbit coupling taken into account.

  13. Dynamic rotor mode in antiferromagnetic nanoparticles

    DEFF Research Database (Denmark)

    Lefmann, Kim; Jacobsen, H.; Garde, J.

    2015-01-01

    measured neutron data and reveal that thermally activated spin canting gives rise to an unusual type of coherent magnetic precession mode. This "rotor" mode can be seen as a high-temperature version of superparamagnetism and is driven by exchange interactions between the two magnetic sublattices......We present experimental, numerical, and theoretical evidence for an unusual mode of antiferromagnetic dynamics in nanoparticles. Elastic neutron scattering experiments on 8-nm particles of hematite display a loss of diffraction intensity with temperature, the intensity vanishing around 150 K....... The frequency of the rotor mode behaves in fair agreement with a simple analytical model, based on a high-temperature approximation of the generally accepted Hamiltonian of the system. The extracted model parameters, such as the magnetic interaction and the axial anisotropy, are in excellent agreement...

  14. Electrical manipulation of ferromagnetic NiFe by antiferromagnetic IrMn

    Science.gov (United States)

    Tshitoyan, V.; Ciccarelli, C.; Mihai, A. P.; Ali, M.; Irvine, A. C.; Moore, T. A.; Jungwirth, T.; Ferguson, A. J.

    2015-12-01

    We demonstrate that an antiferromagnet can be employed for a highly efficient electrical manipulation of a ferromagnet. In our study, we use an electrical detection technique of the ferromagnetic resonance driven by an in-plane ac current in a NiFe/IrMn bilayer. At room temperature, we observe antidampinglike spin torque acting on the NiFe ferromagnet, generated by an in-plane current driven through the IrMn antiferromagnet. A large enhancement of the torque, characterized by an effective spin-Hall angle exceeding most heavy transition metals, correlates with the presence of the exchange-bias field at the NiFe/IrMn interface. It highlights that, in addition to the strong spin-orbit coupling, the antiferromagnetic order in IrMn governs the observed phenomenon.

  15. Modeling of exchange bias in the antiferromagnetic (core)/ferromagnetic (shell) nanoparticles with specialized shapes

    International Nuclear Information System (INIS)

    Hu Yong; Liu Yan; Du An

    2011-01-01

    Zero-field-cooled (ZFC) and field-cooled (FC) hysteresis loops of egg- and ellipsoid-shaped nanoparticles with inverted ferromagnetic (FM)-antiferromagnetic (AFM) core-shell morphologies are simulated using a modified Monte Carlo method, which takes into account both the thermal fluctuations and energy barriers during the rotation of spin. Pronounced exchange bias (EB) fields and reduced coercivities are obtained in the FC hysteresis loops. The analysis of the microscopic spin configurations allows us to conclude that the magnetization reversal occurs by means of the nucleation process during both the ZFC and FC hysteresis branches. The nucleation takes place in the form of 'sparks' resulting from the energy competition and the morphology of the nanoparticle. The appearance of EB in the FC hysteresis loops is only dependent on that the movements of 'sparks' driven by magnetic field at both branches of hysteresis loops are not along the same axis, which is independent of the strength of AFM anisotropy. The tilt of 'spark' movement with respect to the symmetric axis implies the existence of additional unidirectional anisotropy at the AFM/FM interfaces as a consequence of the surplus magnetization in the AFM core, which is the commonly accepted origin of EB. Our simulations allow us to clarify the microscopic mechanisms of the observed EB behavior, not accessible in experiments. - Highlights: → A modified Monte Carlo method considers thermal fluctuations and energy barriers. → Egg and ellipsoid nanoparticles with inverted core-shell morphology are studied. → Pronounced exchange bias fields and reduced coercivities may be detected. → 'Sparks' representing nucleation sites due to energy competition are observed. → 'Sparks' can reflect or check directly and vividly the origin of exchange bias.

  16. Temperature dependence of magnetic excitations in the frustrated antiferromagnetic spinel ZnMn2O4

    Science.gov (United States)

    Chang, Hun; Hwang, In-Yong; Chung, Jae-Ho; Stewart, J. Ross; Higemoto, Wataru; Miyake, Yasuhiro

    2018-01-01

    We report the temperature-dependent evolution of spin ordering and excitations of the frustrated tetragonal (c >a ) spinel ZnMn2O4 across the two-dimensional antiferromagnetic transition. Muon spin relaxation indicates full development of ordered magnetic moments immediately below TN=62.7 (2 ) K in spite of the apparent low-dimensional ordering. Using inelastic neutron scattering, we obtained the spin Hamiltonian accounting for the temperature-dependent spin excitations. The damped spin waves at high temperature exhibit a continuous increase in their lifetime on cooling across TN. In contrast, the finite anisotropy gap appears suddenly below TN indicating that single-ion anisotropy stabilizes the antiferromagnetic chains. We also observed the frustrated out-of-plane exchange contributing to the high-energy modes.

  17. Ground State of Quasi-One Dimensional Competing Spin Chain Cs2Cu2Mo3O12 at zero and Finite Fields

    Science.gov (United States)

    Matsui, Kazuki; Goto, Takayuki; Angel, Julia; Watanabe, Isao; Sasaki, Takahiko; Hase, Masashi

    The ground state of competing-spin-chain Cs2Cu2Mo3O12 with the ferromagnetic exchange interaction J1 = -93 K on nearest-neighboring spins and the antiferromagnetic one J2 = +33 K on next-nearest-neighboring spins was investigated by ZF/LF-μSR and 133Cs-NMR in the 3He temperature range. The zero-field μSR relaxation rate λ shows a significant increase below 1.85 K, suggesting the existence of magnetic order, which is consistent with the recent report on the specific heat. However, LF decoupling data at the lowest temperature 0.3 K indicate that the spins fluctuate dynamically, suggesting that the system is in a quasi-static ordered state under zero field. This idea is further supported by the fact that the broadening in NMR spectra below TN is weakened at low field below 2 T.

  18. Studies of a Large Odd-Numbered Odd-Electron Metal Ring: Inelastic Neutron Scattering and Muon Spin Relaxation Spectroscopy of Cr8 Mn.

    Science.gov (United States)

    Baker, Michael L; Lancaster, Tom; Chiesa, Alessandro; Amoretti, Giuseppe; Baker, Peter J; Barker, Claire; Blundell, Stephen J; Carretta, Stefano; Collison, David; Güdel, Hans U; Guidi, Tatiana; McInnes, Eric J L; Möller, Johannes S; Mutka, Hannu; Ollivier, Jacques; Pratt, Francis L; Santini, Paolo; Tuna, Floriana; Tregenna-Piggott, Philip L W; Vitorica-Yrezabal, Iñigo J; Timco, Grigore A; Winpenny, Richard E P

    2016-01-26

    The spin dynamics of Cr8 Mn, a nine-membered antiferromagnetic (AF) molecular nanomagnet, are investigated. Cr8 Mn is a rare example of a large odd-membered AF ring, and has an odd-number of 3d-electrons present. Odd-membered AF rings are unusual and of interest due to the presence of competing exchange interactions that result in frustrated-spin ground states. The chemical synthesis and structures of two Cr8 Mn variants that differ only in their crystal packing are reported. Evidence of spin frustration is investigated by inelastic neutron scattering (INS) and muon spin relaxation spectroscopy (μSR). From INS studies we accurately determine an appropriate microscopic spin Hamiltonian and we show that μSR is sensitive to the ground-spin-state crossing from S=1/2 to S=3/2 in Cr8 Mn. The estimated width of the muon asymmetry resonance is consistent with the presence of an avoided crossing. The investigation of the internal spin structure of the ground state, through the analysis of spin-pair correlations and scalar-spin chirality, shows a non-collinear spin structure that fluctuates between non-planar states of opposite chiralities. © 2016 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

  19. Zigzag antiferromagnetic ground state with anisotropic correlation lengths in the quasi-two-dimensional honeycomb lattice compound N a2C o2Te O6

    Science.gov (United States)

    Bera, A. K.; Yusuf, S. M.; Kumar, Amit; Ritter, C.

    2017-03-01

    The crystal structure, magnetic ground state, and the temperature-dependent microscopic spin-spin correlations of the frustrated honeycomb lattice antiferromagnet N a2C o2Te O6 have been investigated by powder neutron diffraction. A long-range antiferromagnetic (AFM) ordering has been found below TN˜24.8 K . The magnetic ground state, determined to be zigzag antiferromagnetic and characterized by a propagation vector k =(1 /2 0 0 ) , occurs due to the competing exchange interactions up to third-nearest neighbors within the honeycomb lattice. The exceptional existence of a limited magnetic correlation length along the c axis (perpendicular to the honeycomb layers in the a b planes) has been found even at 1.8 K, well below the TN˜24.8 K . The observed limited correlation along the c axis is explained by the disorder distribution of the Na ions within the intermediate layers between honeycomb planes. The reduced ordered moments mCo (1 )=2.77 (3 ) μB/C o2 + and mCo (2 )=2.45 (2 ) μB/C o2 + at 1.8 K reflect the persistence of spin fluctuations in the ordered state. Above TN˜24.8 K , the presence of short-range magnetic correlations, manifested by broad diffuse magnetic peaks in the diffraction patterns, has been found. Reverse Monte Carlo analysis of the experimental diffuse magnetic scattering data reveals that the spin correlations are mainly confined within the two-dimensional honeycomb layers (a b plane) with a correlation length of ˜12 Å at 25 K. The nature of the spin arrangements is found to be similar in both the short-range and long-range ordered magnetic states. This implies that the short-range correlation grows with decreasing temperature and leads to the zigzag AFM ordering at T ≤TN . The present study provides a comprehensive picture of the magnetic correlations over the temperature range above and below the TN and their relation to the crystal structure. The role of intermediate soft Na layers on the magnetic coupling between honeycomb planes is

  20. One dimensionalization in the spin-1 Heisenberg model on the anisotropic triangular lattice

    Science.gov (United States)

    Gonzalez, M. G.; Ghioldi, E. A.; Gazza, C. J.; Manuel, L. O.; Trumper, A. E.

    2017-11-01

    We investigate the effect of dimensional crossover in the ground state of the antiferromagnetic spin-1 Heisenberg model on the anisotropic triangular lattice that interpolates between the regime of weakly coupled Haldane chains (J'≪J ) and the isotropic triangular lattice (J'=J ). We use the density-matrix renormalization group (DMRG) and Schwinger boson theory performed at the Gaussian correction level above the saddle-point solution. Our DMRG results show an abrupt transition between decoupled spin chains and the spirally ordered regime at (J'/J) c˜0.42 , signaled by the sudden closing of the spin gap. Coming from the magnetically ordered side, the computation of the spin stiffness within Schwinger boson theory predicts the instability of the spiral magnetic order toward a magnetically disordered phase with one-dimensional features at (J'/J) c˜0.43 . The agreement of these complementary methods, along with the strong difference found between the intra- and the interchain DMRG short spin-spin correlations for sufficiently large values of the interchain coupling, suggests that the interplay between the quantum fluctuations and the dimensional crossover effects gives rise to the one-dimensionalization phenomenon in this frustrated spin-1 Hamiltonian.

  1. Fermionic Hubbard model with Rashba or Dresselhaus spin-orbit coupling

    Science.gov (United States)

    Sun, Fadi; Ye, Jinwu; Liu, Wu-Ming

    2017-06-01

    In this work, we investigate the possible dramatic effects of Rashba or Dresselhaus spin-orbit coupling (SOC) on the fermionic Hubbard model in a two-dimensional square lattice. In the strong coupling limit, it leads to the rotated antiferromagnetic Heisenberg model which is a new class of quantum spin model. For a special equivalent class, we identify a new spin-orbital entangled commensurate ground (Y-y) state subject to strong quantum fluctuations at T = 0. We evaluate the quantum fluctuations by the spin wave expansion up to order 1/{S}2. In some SOC parameter regimes, the Y-y state supports a massive relativistic incommensurate magnon (C-IC) with its two gap minima positions continuously tuned by the SOC parameters. The C-IC magnons dominate all the low temperature thermodynamic quantities and also lead to the separation of the peak positions between the longitudinal and the transverse spin structure factors. In the weak coupling limit, any weak repulsive interaction also leads to a weak Y-y state. There is only a crossover from the weak to the strong coupling. High temperature expansions of the specific heats in both weak and strong coupling are presented. The dramatic roles to be played by these C-IC magnons at generic SOC parameters or under various external probes are hinted at. Experimental applications to both layered noncentrosymmetric materials and cold atoms are discussed.

  2. Unconventional spin order in the triangular lattice system NaCrO2: A neutron scattering study

    International Nuclear Information System (INIS)

    Hsieh, D.; Qian, D.; Berger, R.F.; Cava, R.J.; Lynn, J.W.; Huang, Q.; Hasan, M.Z.

    2008-01-01

    We report high resolution neutron scattering measurements on the rhombohedrally stacked triangular antiferromagnet NaCrO 2 which has recently been shown to exhibit an unusually broad fluctuating cross-over regime extending far below the onset of spin freezing at T c . Our results show that at T c purely two-dimensional quasi-static spin correlations of the 120 o type exist. Below some cross-over temperature (T∼0.75T c ) a small incommensuration develops which helps resolve the inter-layer spin frustration and drives short-range three-dimensional magnetic order. This incommensuration assisted dimensional cross-over suggests that inter-layer frustration is responsible for stabilizing the rare 2D correlated phase above 0.75T c

  3. Antiferromagnetic Skyrmion: Stability, Creation and Manipulation

    Science.gov (United States)

    Zhang, Xichao; Zhou, Yan; Ezawa, Motohiko

    2016-04-01

    Magnetic skyrmions are particle-like topological excitations in ferromagnets, which have the topo-logical number Q = ± 1, and hence show the skyrmion Hall effect (SkHE) due to the Magnus force effect originating from the topology. Here, we propose the counterpart of the magnetic skyrmion in the antiferromagnetic (AFM) system, that is, the AFM skyrmion, which is topologically protected but without showing the SkHE. Two approaches for creating the AFM skyrmion have been described based on micromagnetic lattice simulations: (i) by injecting a vertical spin-polarized current to a nanodisk with the AFM ground state; (ii) by converting an AFM domain-wall pair in a nanowire junction. It is demonstrated that the AFM skyrmion, driven by the spin-polarized current, can move straightly over long distance, benefiting from the absence of the SkHE. Our results will open a new strategy on designing the novel spintronic devices based on AFM materials.

  4. Magnetic Nanostructures Spin Dynamics and Spin Transport

    CERN Document Server

    Farle, Michael

    2013-01-01

    Nanomagnetism and spintronics is a rapidly expanding and increasingly important field of research with many applications already on the market and many more to be expected in the near future. This field started in the mid-1980s with the discovery of the GMR effect, recently awarded with the Nobel prize to Albert Fert and Peter Grünberg. The present volume covers the most important and most timely aspects of magnetic heterostructures, including spin torque effects, spin injection, spin transport, spin fluctuations, proximity effects, and electrical control of spin valves. The chapters are written by internationally recognized experts in their respective fields and provide an overview of the latest status.

  5. Anomalous Hall-like effect probe of antiferromagnetic domain wall.

    Science.gov (United States)

    Lang, Lili; Qiu, Xuepeng; Zhou, Shiming

    2018-01-10

    Of crucial importance to antiferromagnetic (AF) spintronic devices, AF domain wall (AFDW), created in exchange biased Y 3 Fe 5 O 12 /Ni 0.50 Co 0.50 O (NiCoO)/Pt, is characterized by anomalous Hall-like effect through magnetic proximity effect and spin Hall magnetoresistance at NiCoO/Pt interface. The AFDW thickness, in the order of nanometers, has been for the first time proved in experiments to increase with increasing temperature. AF spins within AFDW show the same chirality in decent and ascent branches of ferromagnetic magnetization reversal process. Moreover, the uncompensated magnetic moment at the NiCoO/Pt interface is of perpendicular magnetization anisotropy and changes linearly in magnitude with temperature due to the reduced coordination of the magnetic atoms on the AF surface. This work will help to clarify the mechanism of the spin current propagation in AF materials and fully understand the physics behind exchange bias.

  6. Superconductivity and antiferromagnetism in cuprates and pnictides: Evidence of the role of Coulomb correlation

    International Nuclear Information System (INIS)

    Fan, J.D.; Malozovsky, Y.M.

    2013-01-01

    Highlights: • In a layered 2D cuprates the long-range order antiferromagnetism is driven mainly by the Van Hove singularity. • The long-range antiferromagnetism quickly disappear with doping away from the Van Hove singularity. • For pnictides the antiferromagnetism exists as a result of the nesting condition. • Since the doping steadily changes the nesting conditions, the antiferromagnetism and superconductivity may coexist. -- Abstract: We consider the Hubbard model in terms of the perturbative diagrammatic approach (UN F ⩽1) where the interaction between two electrons with antiparallel spins in the lowest order of perturbation is described by the short-range repulsive contact (on-site) interaction (U>0). We argue that in layered 2D cuprates the long-range order antiferromagnetism is driven mainly by the Van Hove singularity, whereas in the case of pnictides the antiferromagnetism exists as a result of the nesting condition. We show that when the interaction is quite strong (UN F ≈1) in the case of the Van Hove singularity the electron system undergoes the antiferromagnetic phase transition with the log-range order parameter and large insulating gap. The long-range antiferromagnetism quickly disappear, as shown, with the doping away from the Van Hove singularity, but the antiferromagnetic short-range correlation persists (UN F < 1) due to Coulomb repulsive interaction which is the mechanism for superconductivity in cuprates. We argue that in the case of pnictides the antiferromagnetism appears when the nesting conditions for the Fermi surface are met. Since the doping steadily changes the nesting conditions, the antiferromagnetism and superconductivity may coexist as has been observed in pnictides. We show that the proximity of the antiferromagnetism and superconductivity implies the repulsive interaction between electrons, which turns into attractive between quasiparticles as shown by the authors in the article published on the same issue as this one

  7. Large anomalous Hall effect in a non-collinear antiferromagnet at room temperature

    Science.gov (United States)

    Nakatsuji, Satoru; Kiyohara, Naoki; Higo, Tomoya

    2015-11-01

    In ferromagnetic conductors, an electric current may induce a transverse voltage drop in zero applied magnetic field: this anomalous Hall effect is observed to be proportional to magnetization, and thus is not usually seen in antiferromagnets in zero field. Recent developments in theory and experiment have provided a framework for understanding the anomalous Hall effect using Berry-phase concepts, and this perspective has led to predictions that, under certain conditions, a large anomalous Hall effect may appear in spin liquids and antiferromagnets without net spin magnetization. Although such a spontaneous Hall effect has now been observed in a spin liquid state, a zero-field anomalous Hall effect has hitherto not been reported for antiferromagnets. Here we report empirical evidence for a large anomalous Hall effect in an antiferromagnet that has vanishingly small magnetization. In particular, we find that Mn3Sn, an antiferromagnet that has a non-collinear 120-degree spin order, exhibits a large anomalous Hall conductivity of around 20 per ohm per centimetre at room temperature and more than 100 per ohm per centimetre at low temperatures, reaching the same order of magnitude as in ferromagnetic metals. Notably, the chiral antiferromagnetic state has a very weak and soft ferromagnetic moment of about 0.002 Bohr magnetons per Mn atom (refs 10, 12), allowing us to switch the sign of the Hall effect with a small magnetic field of around a few hundred oersted. This soft response of the large anomalous Hall effect could be useful for various applications including spintronics—for example, to develop a memory device that produces almost no perturbing stray fields.

  8. 't Hooft-Polyakov monopoles in an antiferromagnetic Bose-Einstein condensate

    NARCIS (Netherlands)

    Stoof, H.T.C.; Vliegen, E.; Al Khawaja, U.

    2001-01-01

    We show that an antiferromagnetic spin-1 Bose-Einstein condensate, which can for instance be created with 23-Na atoms in an optical trap, has not only singular line-like vortex excitations, but also allows for singular point-like topological excitations, i.e., 't Hooft-Polyakov monopoles. We discuss

  9. The dynamical frustration of interlayer excitons delocalizing in bilayer quantum antiferromagnets

    NARCIS (Netherlands)

    Rademaker, L.; Wu, K.; Hilgenkamp, H.; Zaanen, J.

    2012-01-01

    Using the self-consistent Born approximation we study the delocalization of interlayer excitons in the bilayer Heisenberg quantum antiferromagnet. Under realistic conditions we find that the coupling between the exciton motion and the spin system is strongly enhanced as compared to the case of a

  10. Construction and study of exact ground states for a class of quantum antiferromagnets

    International Nuclear Information System (INIS)

    Fannes, M.

    1989-01-01

    Techniques of quantum probability are used to construct the exact ground states for a class of quantum spin systems in one dimension. This class in particular contains the antiferromagnetic models introduced by various authors under the name of VBS-models. The construction permits a detailed study of these ground states. (A.C.A.S.) [pt

  11. Using random boundary conditions to simulate disordered quantum spin models in two-dimensional systems

    Science.gov (United States)

    Yuste, A.; Moreno-Cardoner, M.; Sanpera, A.

    2017-05-01

    Disordered quantum antiferromagnets in two-dimensional compounds have been a focus of interest in the last years due to their exotic properties. However, with very few exceptions, the ground states of the corresponding Hamiltonians are notoriously difficult to simulate making their characterization and detection very elusive, both theoretically and experimentally. Here we propose a method to signal quantum disordered antiferromagnets by doing exact diagonalization in small lattices using random boundary conditions and averaging the observables of interest over the different disorder realizations. We apply our method to study the Heisenberg spin-1/2 model in an anisotropic triangular lattice. In this model, the competition between frustration and quantum fluctuations might lead to some spin-liquid phases as predicted from different methods ranging from spin-wave mean-field theory to 2D-DMRG or PEPS. Our method accurately reproduces the ordered phases expected of the model and signals quantum disordered phases by the presence of a large number of quasidegenerate ground states together with an undefined local order parameter. The method presents a weak dependence on finite-size effects.

  12. How to manipulate magnetic states of antiferromagnets

    Science.gov (United States)

    Song, Cheng; You, Yunfeng; Chen, Xianzhe; Zhou, Xiaofeng; Wang, Yuyan; Pan, Feng

    2018-03-01

    Antiferromagnetic materials, which have drawn considerable attention recently, have fascinating features: they are robust against perturbation, produce no stray fields, and exhibit ultrafast dynamics. Discerning how to efficiently manipulate the magnetic state of an antiferromagnet is key to the development of antiferromagnetic spintronics. In this review, we introduce four main methods (magnetic, strain, electrical, and optical) to mediate the magnetic states and elaborate on intrinsic origins of different antiferromagnetic materials. Magnetic control includes a strong magnetic field, exchange bias, and field cooling, which are traditional and basic. Strain control involves the magnetic anisotropy effect or metamagnetic transition. Electrical control can be divided into two parts, electric field and electric current, both of which are convenient for practical applications. Optical control includes thermal and electronic excitation, an inertia-driven mechanism, and terahertz laser control, with the potential for ultrafast antiferromagnetic manipulation. This review sheds light on effective usage of antiferromagnets and provides a new perspective on antiferromagnetic spintronics.

  13. Colossal magnetodielectric effect and spin flop in magnetoelectric Co4Nb2O9 crystal

    International Nuclear Information System (INIS)

    Yin, L. H.; Yang, J.; Dai, J. M.; Song, W. H.; Zhu, X. B.; Zou, Y. M.; Sun, Y. P.

    2016-01-01

    We have investigated the detailed magnetic, magnetoelectric (ME), magnetodielectric (MD) and thermal expansion properties in Co 4 Nb 2 O 9 crystal. A magnetic-field-induced spin flop was observed below antiferromagnetic (AFM) transition temperature T N . Dielectric constant at applied magnetic field nearly diverges around the AFM transition, giving rise to a colossal MD effect as high as ∼138% around T N . Theoretical analysis of the ME and MD data revealed a major contribution of critical spin fluctuation to the colossal MD effect in Co 4 Nb 2 O 9 . These results suggest that linear ME materials with large ME coupling might be potentially used to realize large MD effect for future application.

  14. Spin Dynamics and Quantum Tunneling in Fe8 Nanomagnet and in AFM Rings by NMR

    Energy Technology Data Exchange (ETDEWEB)

    Ho-Baek, Seung [Iowa State Univ., Ames, IA (United States)

    2004-01-01

    In this thesis, our main interest has been to investigate the spin dynamics and quantum tunneling in single molecule magnets (SMMs), For this we have selected two different classes of SMMs: a ferrimagnetic total high spin S = 10 cluster Fe8 and antiferromagnetic (AFM) ring-type clusters. For Fe8, our efforts have been devoted to the investigation of the quantum tunneling of magnetization in the very low temperature region. The most remarkable experimental finding in Fe8 is that the nuclear spin-lattice relaxation rate (1/T{sub l}) at low temperatures takes place via strong collision mechanism, and thus it allows to measure directly the tunneling rate vs T and H for the first time. For AFM rings, we have shown that 1/T{sub l} probes the thermal fluctuations of the magnetization in the intermediate temperature range. We find that the fluctuations are dominated by a single characteristic frequency which has a power law T-dependence indicative of fluctuations due to electron-acoustic phonon interactions.

  15. Spin Dynamics and Quantum Tunneling in Fe8 Nanomagnet and in AFM Rings by NMR

    International Nuclear Information System (INIS)

    Seung-Ho-Baek

    2004-01-01

    In this thesis, our main interest has been to investigate the spin dynamics and quantum tunneling in single molecule magnets (SMMs), For this we have selected two different classes of SMMs: a ferrimagnetic total high spin S = 10 cluster Fe8 and antiferromagnetic (AFM) ring-type clusters. For Fe8, our efforts have been devoted to the investigation of the quantum tunneling of magnetization in the very low temperature region. The most remarkable experimental finding in Fe8 is that the nuclear spin-lattice relaxation rate (1/T l ) at low temperatures takes place via strong collision mechanism, and thus it allows to measure directly the tunneling rate vs T and H for the first time. For AFM rings, we have shown that 1/T l probes the thermal fluctuations of the magnetization in the intermediate temperature range. We find that the fluctuations are dominated by a single characteristic frequency which has a power law T-dependence indicative of fluctuations due to electron-acoustic phonon interactions

  16. Spin dynamics and quantum tunneling in Fe8 nanomagnet and in AFM rings by NMR

    Science.gov (United States)

    Baek, Seung-Ho

    In this thesis, our main interest has been to investigate the spin dynamics and quantum tunneling in single molecule magnets (SMMs). For this we have selected two different classes of SMMs: a ferromagnetic total high spin S = 10 cluster Fe8 and antiferromagnetic (AFM) ring-type clusters. For Fe8, our efforts have been devoted to the investigation of the quantum tunneling of magnetization in the very low temperature region. The most remarkable experimental finding in Fe8 is that the nuclear spin-lattice relaxation rate (1/T1) at low temperatures takes place via strong collision mechanism, and thus it allows to measure directly the tunneling rate vs. T and H for the first time. For AFM rings, we have shown that 1/T1 probes the thermal fluctuations of the magnetization in the intermediate temperature range. We find that the fluctuations are dominated by a single characteristic frequency which has a power-law T-dependence indicative of fluctuations due to electron-acoustic phonon interactions.

  17. Two-dimensional magnetism in the triangular antiferromagnet NiGa2S4

    International Nuclear Information System (INIS)

    Nambu, Yusuke

    2013-01-01

    At sufficiently low temperatures, electron spins in normal magnets generally order into some fashion, for instance, ferromagnetic and antiferromagnetic. Geometrical frustration and/or reduced dimensionality can suppress such conventional orders, and occasionally induce unknown states of matter. This is the case for the two-dimensional (2D) triangular antiferromagnet Ni(Ga 2 S 4 , in which S=1 nickel spins do not order, instead show an exotic magnetism. We found (1) a resonant critical slowing down toward T*=8.5 K followed by a viscous spin liquid behavior, and (2) a spin-size dependent ground state. To elucidate (1), spin dynamics ranging from 10 -13 to 10 0 seconds were quantitatively explored through the experimental techniques such as inelastic neutron scattering, backscattering, neutron spin echo, ac and nonlinear susceptibilities. The finding of (2) is evidenced by impurity effects. Integer spins substituted systems such as zinc and iron ions retain a quadratic temperature dependence of the magnetic specific heat as for the parent compound. However, substitutions of half-odd integer spins, cobalt and manganese ions, eventually induce a distinct behavior, indicating an importance of integer size of spins to stabilize the 2D magnetism realized in NiGa 2 S 4 . The article gives our experimental findings and as well as some relevant theoretical scenarios. (author)

  18. Far-from-Equilibrium Field Theory of Many-Body Quantum Spin Systems: Prethermalization and Relaxation of Spin Spiral States in Three Dimensions

    Directory of Open Access Journals (Sweden)

    Mehrtash Babadi

    2015-10-01

    Full Text Available We study theoretically the far-from-equilibrium relaxation dynamics of spin spiral states in the three-dimensional isotropic Heisenberg model. The investigated problem serves as an archetype for understanding quantum dynamics of isolated many-body systems in the vicinity of a spontaneously broken continuous symmetry. We present a field-theoretical formalism that systematically improves on the mean field for describing the real-time quantum dynamics of generic spin-1/2 systems. This is achieved by mapping spins to Majorana fermions followed by a 1/N expansion of the resulting two-particle-irreducible effective action. Our analysis reveals rich fluctuation-induced relaxation dynamics in the unitary evolution of spin spiral states. In particular, we find the sudden appearance of long-lived prethermalized plateaus with diverging lifetimes as the spiral winding is tuned toward the thermodynamically stable ferro- or antiferromagnetic phases. The emerging prethermalized states are characterized by different bosonic modes being thermally populated at different effective temperatures and by a hierarchical relaxation process reminiscent of glassy systems. Spin-spin correlators found by solving the nonequilibrium Bethe-Salpeter equation provide further insight into the dynamic formation of correlations, the fate of unstable collective modes, and the emergence of fluctuation-dissipation relations. Our predictions can be verified experimentally using recent realizations of spin spiral states with ultracold atoms in a quantum gas microscope [S. Hild et al., Phys. Rev. Lett. 113, 147205 (2014PRLTAO0031-900710.1103/PhysRevLett.113.147205].

  19. Room-temperature antiferromagnetism in CuMnAs

    Czech Academy of Sciences Publication Activity Database

    Máca, František; Mašek, Jan; Stelmakhovych, O.; Martí, X.; Reichlová, Helena; Uhlířová, K.; Beran, Přemysl; Wadley, P.; Novák, Vít; Jungwirth, Tomáš

    2012-01-01

    Roč. 324, č. 8 (2012), s. 1606-1612 ISSN 0304-8853 R&D Projects: GA MŠk LC510 EU Projects: European Commission(XE) 215368 - SemiSpinNet; European Commission(XE) 268066 - 0MSPIN Grant - others:AV ČR(CZ) AP0801 Program:Akademická prémie - Praemium Academiae Institutional research plan: CEZ:AV0Z10100520; CEZ:AV0Z10100521; CEZ:AV0Z10480505 Keywords : antiferromagnetic semiconductors * spintronics * molecular beam epitaxy Subject RIV: BM - Solid Matter Physics ; Magnetism Impact factor: 1.826, year: 2012

  20. Thermoelectric properties of layered antiferromagnetic CuCrSe{sub 2}

    Energy Technology Data Exchange (ETDEWEB)

    Tewari, Girish C. [Department of Chemistry, Aalto University, P.O. Box 16100, FI-00076 Aalto (Finland); Tripathi, T.S. [Department of Physics, National University of Singapore, 117542 Singapore (Singapore); Yamauchi, Hisao [Department of Chemistry, Aalto University, P.O. Box 16100, FI-00076 Aalto (Finland); Karppinen, Maarit, E-mail: maarit.karppinen@aalto.fi [Department of Chemistry, Aalto University, P.O. Box 16100, FI-00076 Aalto (Finland)

    2014-05-01

    Here we study thermoelectric and magnetic properties of CuCrSe{sub 2} samples sintered at various temperatures. Structural analysis with XRD shows an order-disorder transition for Cr atoms when the sintering temperature is increased above 1273 K. Metal-like electrical resistivity and anomalously large Seebeck coefficient are found about room temperature. Analysis of electrical conductivity and Seebeck coefficient of the partially-disordered phase suggests hopping conduction of charge carriers. For both the ordered and disordered phases magnetic susceptibility follows Curie–Weiss temperature dependence at high temperatures above 150 K and shows an antiferromagnetic transition around 55 K. For the disordered phase, the effective magnetic moment is determined at 3.62 μ{sub B}; this low value in comparison to the spin only value for Cr{sup 3+} of 3.89 μ{sub B} indicates spin fluctuations in the paramagnetic state. The thermal conductivity in these phases is low and dominated by the lattice contribution. Values for the thermoelectric figure of merit (ZT) at room temperature are estimated to be 0.17 and 0.05 for the ordered and disordered phases, respectively. - Highlights: • Thermoelectric and magnetic properties of CuCrSe{sub 2} samples are investigated. • The properties strongly depend on the degree of order of chromium atoms. • The degree of order is controlled by the sintering temperature. • Room-temperature figure of merit is estimated at 0.17 for the ordered phase. • For the disordered phase the figure of merit is lower.

  1. Room-temperature antiferromagnetic memory resistor.

    Science.gov (United States)

    Marti, X; Fina, I; Frontera, C; Liu, Jian; Wadley, P; He, Q; Paull, R J; Clarkson, J D; Kudrnovský, J; Turek, I; Kuneš, J; Yi, D; Chu, J-H; Nelson, C T; You, L; Arenholz, E; Salahuddin, S; Fontcuberta, J; Jungwirth, T; Ramesh, R

    2014-04-01

    The bistability of ordered spin states in ferromagnets provides the basis for magnetic memory functionality. The latest generation of magnetic random access memories rely on an efficient approach in which magnetic fields are replaced by electrical means for writing and reading the information in ferromagnets. This concept may eventually reduce the sensitivity of ferromagnets to magnetic field perturbations to being a weakness for data retention and the ferromagnetic stray fields to an obstacle for high-density memory integration. Here we report a room-temperature bistable antiferromagnetic (AFM) memory that produces negligible stray fields and is insensitive to strong magnetic fields. We use a resistor made of a FeRh AFM, which orders ferromagnetically roughly 100 K above room temperature, and therefore allows us to set different collective directions for the Fe moments by applied magnetic field. On cooling to room temperature, AFM order sets in with the direction of the AFM moments predetermined by the field and moment direction in the high-temperature ferromagnetic state. For electrical reading, we use an AFM analogue of the anisotropic magnetoresistance. Our microscopic theory modelling confirms that this archetypical spintronic effect, discovered more than 150 years ago in ferromagnets, is also present in AFMs. Our work demonstrates the feasibility of fabricating room-temperature spintronic memories with AFMs, which in turn expands the base of available magnetic materials for devices with properties that cannot be achieved with ferromagnets.

  2. Landau model for the multiferroic delafossite antiferromagnets

    Energy Technology Data Exchange (ETDEWEB)

    Ribeiro, J.L, E-mail: jlr@fisica.uminho.pt [Centro de Física da Universidade do Minho, 4710-057 Braga (Portugal); Perez-Mato, J.M [Dpto. de Física de la Materia Condensada, Facultad de Ciencia y Tecnología, Universidad del País Vasco, Apartado 644, 48080 Bilbao (Spain); Vieira, L.G [Centro de Física da Universidade do Minho, 4710-057 Braga (Portugal)

    2016-10-15

    A symmetry based framework is used to describe the complex phase diagrams observed in the multiferroic delafossite compounds. A free energy Landau functional is derived from the analysis of the transformation properties of the most general incommensurate magnetic spin order parameter. A principle of maximal symmetry is invoked and the stability of each of the different higher symmetry phases considered. The competition between different potential ground states is analysed within the scope of a simplified model, which emphasizes the role of the symmetry allowed phase dependent biquadratic couplings. The cross-over between the different competing states is also discussed. The results show that the diverse set of phase diagrams that are experimentally observed in this class of triangular lattice antiferromagnets and, in particular, the stabilization of magnetically induced ferroelectric states, can be well interpreted and described within this integrated phenomenological approximation. - Highlights: • Symmetry considerations are used to analyze the phase diagrams of the compounds. • The competition between possible ground states is discussed. • The field induced transitions between competing states are described.

  3. Coupled Quantum Fluctuations and Quantum Annealing

    Science.gov (United States)

    Hormozi, Layla; Kerman, Jamie

    We study the relative effectiveness of coupled quantum fluctuations, compared to single spin fluctuations, in the performance of quantum annealing. We focus on problem Hamiltonians resembling the the Sherrington-Kirkpatrick model of Ising spin glass and compare the effectiveness of different types of fluctuations by numerically calculating the relative success probabilities and residual energies in fully-connected spin systems. We find that for a small class of instances coupled fluctuations can provide improvement over single spin fluctuations and analyze the properties of the corresponding class. Disclaimer: This research was funded by ODNI, IARPA via MIT Lincoln Laboratory under Air Force Contract No. FA8721-05-C-0002. The views and conclusions contained herein are those of the authors and should not be interpreted as necessarily representing the official policies or endorsements, either expressed or implied, of ODNI, IARPA, or the US Government.

  4. Glassy low-energy spin fluctuations and anisotropy gap in La1.88Sr0.12CuO4

    DEFF Research Database (Denmark)

    Rømer, A. T.; Chang, J.; Christensen, Niels Bech

    2013-01-01

    between the ordering temperature TN ≃ Tc inferred from elastic neutron scattering and the freezing temperature Tf ≃ 11 K obtained from muon spin rotation studies. The magnetic field independence of the observed excitation spectrum as well as the observation of a partial suppression of magnetic spectral...... that the significant enhancement in a magnetic field of nominally elastic incommensurate scattering is caused by strictly inelastic scattering-at least in the temperature range between Tf and Tc - which is not resolved in the present experiment. Combining the results obtained from our study of La1.88Sr0.12CuO4......We present high-resolution triple-axis neutron scattering studies of the high-temperature superconductorLa1.88Sr0.12CuO4 (Tc = 27 K). The temperature dependence of the low-energy incommensurate magnetic fluctuations reveals distinctly glassy features. The glassiness is confirmed by the difference...

  5. Spin Hall noise

    NARCIS (Netherlands)

    Kamra, A.; Witek, F.P.; Meyer, S.; Huebl, H.; Geprägs, S.; Gross, R.; Bauer, G.E.W.; Goennenwein, S.T.B.

    2014-01-01

    We measure the low-frequency thermal fluctuations of pure spin current in a platinum film deposited on yttrium iron garnet via the inverse spin Hall effect (ISHE)-mediated voltage noise as a function of the angle ? between the magnetization and the transport direction. The results are consistent

  6. Dynamics of Coupled Quantum Spin Chains

    International Nuclear Information System (INIS)

    Schulz, H.J.

    1996-01-01

    Static and dynamical properties of weakly coupled antiferromagnetic spin chains are treated using a mean-field approximation for the interchain coupling and exact results for the resulting effective one-dimensional problem. Results for staggered magnetization, Nacute eel temperature, and spin wave excitations are in agreement with experiments on KCuF 3 . The existence of a narrow longitudinal mode is predicted. The results are in agreement with general scaling arguments, contrary to spin wave theory. copyright 1996 The American Physical Society

  7. Magnetic correlations in the intermetallic antiferromagnet Nd3Co4Sn13

    Science.gov (United States)

    Wang, C. W.; Lin, J. W.; Lue, C. S.; Liu, H. F.; Kuo, C. N.; Mole, R. A.; Gardner, J. S.

    2017-11-01

    Specific heat, magnetic susceptibility, and neutron scattering have been used to investigate the nature of the spin system in the antiferromagnet Nd3Co4Sn13. At room temperature Nd3Co4Sn13 has a cubic, Pm-3n structure similar to Yb3Rh4Sn13. Antiferromagnetic interactions between, Nd3+ ions dominate the magnetic character of this sample and at 2.4 K the Nd spins enter a long range order state with a magnetic propagation vector q  =  (0 0 0) with an ordered moment of 1.78(2) µ B at 1.5 K. The magnetic Bragg intensity grows very slowly below 1 K, reaching ~2.4 µ B at 350 mK. The average magnetic Nd3+ configuration corresponds to the 3D irreducible representation Γ7. This magnetic structure can be viewed as three sublattices of antiferromagnetic spin chains coupled with each other in the 120°-configuration. A well-defined magnetic excitation was measured around the 1 1 1 zone centre and the resulting dispersion curve is appropriate for an antiferromagnet with a gap of 0.20(1) meV.

  8. A mean field study of the quasi-one-dimensional antiferromagnetic anisotropic Heisenberg model

    International Nuclear Information System (INIS)

    Benyoussef, A.

    1996-10-01

    The effect of the chain and the dimer anisotropies on the ground state energy and the energy gap of the spin-1/2 quasi-one-dimensional antiferromagnetic Heisenberg model is investigated using a mean field theory. The dependence of the magnetization and the effective hopping parameters on the anisotropy α xy (=J xy perpendicular /J xy parallel ) are presented for several values of the chain anisotropy. However, such a system exhibits a transition from antiferromagnetic ordered to disordered phases for arbitrary chain anisotropy and dimer anisotropy. (author). 22 refs, 11 figs

  9. Ground-state candidate for the classical dipolar kagome Ising antiferromagnet

    Science.gov (United States)

    Chioar, I. A.; Rougemaille, N.; Canals, B.

    2016-06-01

    We have investigated the low-temperature thermodynamic properties of the classical dipolar kagome Ising antiferromagnet using Monte Carlo simulations, in the quest for the ground-state manifold. In spite of the limitations of a single-spin-flip approach, we managed to identify certain ordering patterns in the low-temperature regime and we propose a candidate for this unknown state. This configuration presents some intriguing features and is fully compatible with the extrapolations of the at-equilibrium thermodynamic behavior sampled so far, making it a very likely choice for the dipolar long-range ordered state of the classical kagome Ising antiferromagnet.

  10. Spintronic materials and devices based on antiferromagnetic metals

    Directory of Open Access Journals (Sweden)

    Y.Y. Wang

    2017-04-01

    Full Text Available In this paper, we review our recent experimental developments on antiferromagnet (AFM spintronics mainly comprising Mn-based noncollinear AFM metals. IrMn-based tunnel junctions and Hall devices have been investigated to explore the manipulation of AFM moments by magnetic fields, ferromagnetic materials and electric fields. Room-temperature tunneling anisotropic magnetoresistance based on IrMn as well as FeMn has been successfully achieved, and electrical control of the AFM exchange spring is realized by adopting ionic liquid. In addition, promising spin-orbit effects in AFM as well as spin transfer via AFM spin waves reported by different groups have also been reviewed, indicating that the AFM can serve as an efficient spin current source. To explore the crucial role of AFM acting as efficient generators, transmitters, and detectors of spin currents is an emerging topic in the field of magnetism today. AFM metals are now ready to join the rapidly developing fields of basic and applied spintronics, enriching this area of solid-state physics and microelectronics.

  11. Magnetic fluctuations and superconducting properties of CaKFe4As4 studied by 75As NMR

    Science.gov (United States)

    Cui, J.; Ding, Q.-P.; Meier, W. R.; Böhmer, A. E.; Kong, T.; Borisov, V.; Lee, Y.; Bud'ko, S. L.; Valentí, R.; Canfield, P. C.; Furukawa, Y.

    2017-09-01

    We report 75As nuclear magnetic resonance (NMR) studies on a new iron-based superconductor, CaKFe4As4 , with Tc=35 K. 75As NMR spectra show two distinct lines corresponding to the As(1) and As(2) sites close to the K and Ca layers, respectively, revealing that K and Ca layers are well ordered without site inversions. We found that nuclear quadrupole frequencies νQ of the As(1) and As(2) sites show an opposite temperature T dependence. Nearly T independent behavior of the Knight shifts K is observed in the normal state, and a sudden decrease in K in the superconducting (SC) state suggests spin-singlet Cooper pairs. 75As spin-lattice relaxation rates 1 /T1 show a power-law T dependence with different exponents for the two As sites. The isotropic antiferromagnetic spin fluctuations characterized by the wave vector q =(π ,0 ) or (0 ,π ) in the single-iron Brillouin zone notation are revealed by 1 /T1T and K measurements. Such magnetic fluctuations are necessary to explain the observed temperature dependence of the 75As quadrupole frequencies, as evidenced by our first-principles calculations. In the SC state, 1 /T1 shows a rapid decrease below Tc without a Hebel-Slichter peak and decreases exponentially at low T , consistent with an s± nodeless two-gap superconductor.

  12. Metamagnetic phase transition of the antiferromagnetic Heisenberg icosahedron.

    Science.gov (United States)

    Schröder, Christian; Schmidt, Heinz-Jürgen; Schnack, Jürgen; Luban, Marshall

    2005-05-27

    The observation of hysteresis effects in single molecule magnets like Mn12-acetate has initiated ideas of future applications in storage technology. The appearance of a hysteresis loop in such compounds is an outcome of their magnetic anisotropy. In this Letter we report that magnetic hysteresis occurs in a spin system without any anisotropy, specifically where spins mounted on the vertices of an icosahedron are coupled by antiferromagnetic isotropic nearest-neighbor Heisenberg interaction giving rise to geometric frustration. At T = 0 this system undergoes a first-order metamagnetic phase transition at a critical field Bc between two distinct families of ground state configurations. The metastable phase of the system is characterized by a temperature and field dependent survival probability distribution.

  13. Evolution of topological features in finite antiferromagnetic Heisenberg chains

    International Nuclear Information System (INIS)

    Chen Changfeng

    2003-01-01

    We examine the behavior of nonlocal topological order in finite antiferromagnetic Heisenberg chains using the density matrix renormalization group techniques. We find that chains with even and odd site parity show very different behavior in the topological string order parameter, reflecting interesting interplay of the intrinsic magnetic correlation and the topological term in the chains. Analysis of the calculated string order parameter as a function of the chain length and the topological angle indicates that S=1/2 and S=1 chains show special behavior while all S>1 chains have similar topological structure. This result supports an earlier conjecture on the classification of quantum spin chains based on an analysis of their phase diagrams. Implications of the topological behavior in finite quantum spin chains are discussed

  14. Magnetocaloric properties of a frustrated Blume-Capel antiferromagnet

    Directory of Open Access Journals (Sweden)

    Žukovič Milan

    2014-07-01

    Full Text Available Low-temperature magnetization processes and magnetocaloric properties of a geometrically frustrated spin-1 Blume-Capel model on a triangular lattice are studied by Monte Carlo simulations. The model is found to display qualitatively different behavior depending on the sign of the single-ion anisotropy D. For positive values of D we observe two magnetization plateaus, similar to the spin-1/2 Ising antiferromagnet, and negative isothermal entropy changes for any field intensity. For a range of small negative values of D there are four magnetization plateaus and the entropy changes can be either negative or positive, depending on the field. If D is negative but large in absolute value then the entropy changes are solely positive.

  15. Magnetic structure and interactions in the quasi-1D antiferromagnet CaV{sub 2}O{sub 4}

    Energy Technology Data Exchange (ETDEWEB)

    Pieper, Oliver; Lake, Bella [Helmholtz-Zentrum Berlin fuer Materialien und Energie, Berlin (Germany); Technische Universitaet Berlin, Institut fuer Festkoerperphysik, Berlin (Germany); Daoud-Aladine, Aziz [ISIS Facility, Rutherford Appleton Lab., Chilton (United Kingdom); Reehuis, Manfred [Helmholtz-Zentrum Berlin fuer Materialien und Energie, Berlin (Germany); Max-Planck-Institut fuer Festkoerperforschung, Stuttgart (Germany); Prokes, Karel; Klemke, Bastian; Kiefer, Klaus [Helmholtz-Zentrum Berlin fuer Materialien und Energie, Berlin (Germany); Yan, Jiaqiang; Niazi, Asad; Johnston, David C. [Ames Lab., Departement of Physics and Astronomy, Iowa State University, Ames (United States); Honecker, Andreas [Universitaet Goettingen, Institut fuer Theoretische Physik, Goettingen (Germany)

    2009-07-01

    CaV{sub 2}O{sub 4} is a spin-1 antiferromagnet where the magnetic vanadium ions are arranged on quasi-one-dimensional zig-zag chains with frustrated antiferromagnetic exchange interactions. Here we present high temperature susceptibility and single-crystal neutron diffraction measurements, which are used to deduce the magnetic structure, dominant exchange interactions and orbital configurations. The results suggest that at high temperatures of CaV{sub 2}O{sub 4}, the zig-zags behave as Haldane chains but at low temperatures, orbital ordering lifts the exchange frustration and the zig-zags become spin-1 ladders.

  16. Variational treatment of the Shastry-Sutherland antiferromagnet using Projected Entangled Pair States (PEPS)

    OpenAIRE

    Isacsson, A.; Syljuasen, O. F.

    2006-01-01

    We have applied a variational algorithm based on Projected Entangled Pair States (PEPS) to a two dimensional frustrated spin system, the spin-1/2 antiferromagnetic Heisenberg model on the Shastry-Sutherland lattice. We use the class of PEPS with internal tensor dimension D=2, the first step beyond product states (D=1 PEPS). We have found that the D=2 variational PEPS algorithm is able to capture the physics in both the valence-bond crystal and the Neel ordered state. Also the spin-textures gi...

  17. Electrical control of antiferromagnetic metal up to 15 nm

    Science.gov (United States)

    Zhang, PengXiang; Yin, GuFan; Wang, YuYan; Cui, Bin; Pan, Feng; Song, Cheng

    2016-08-01

    Manipulation of antiferromagnetic (AFM) spins by electrical means is on great demand to develop the AFM spintronics with low power consumption. Here we report a reversible electrical control of antiferromagnetic moments of FeMn up to 15 nm, using an ionic liquid to exert a substantial electric-field effect. The manipulation is demonstrated by the modulation of exchange spring in [Co/Pt]/FeMn system, where AFM moments in FeMn pin the magnetization rotation of Co/Pt. By carrier injection or extraction, the magnetic anisotropy of the top layer in FeMn is modulated to influence the whole exchange spring and then passes its influence to the [Co/Pt]/FeMn interface, through a distance up to the length of exchange spring that fully screens electric field. Comparing FeMn to IrMn, despite the opposite dependence of exchange bias on gate voltages, the same correlation between carrier density and exchange spring stiffness is demonstrated. Besides the fundamental significance of modulating the spin structures in metallic AFM via all-electrical fashion, the present finding would advance the development of low-power-consumption AFM spintronics.

  18. Anisotropic Magnetoresistance in Antiferromagnetic Sr_{2}IrO_{4}

    Directory of Open Access Journals (Sweden)

    C. Wang

    2014-11-01

    Full Text Available We report point-contact measurements of anisotropic magnetoresistance (AMR in a single crystal of antiferromagnetic Mott insulator Sr_{2}IrO_{4}. The point-contact technique is used here as a local probe of magnetotransport properties on the nanoscale. The measurements at liquid nitrogen temperature reveal negative magnetoresistances (up to 28% for modest magnetic fields (250 mT applied within the IrO_{2} a-b plane and electric currents flowing perpendicular to the plane. The angular dependence of magnetoresistance shows a crossover from fourfold to twofold symmetry in response to an increasing magnetic field with angular variations in resistance from 1% to 14%. We tentatively attribute the fourfold symmetry to the crystalline component of AMR and the field-induced transition to the effects of applied field on the canting of antiferromagnetic-coupled moments in Sr_{2}IrO_{4}. The observed AMR is very large compared to the crystalline AMRs in 3d transition metal alloys or oxides (0.1%–0.5% and can be associated with the large spin-orbit interactions in this 5d oxide while the transition provides evidence of correlations between electronic transport, magnetic order, and orbital states. The finding of this work opens an entirely new avenue to not only gain a new insight into physics associated with spin-orbit coupling but also to better harness the power of spintronics in a more technically favorable fashion.

  19. Exact Solutions for Correlations in the Kagomé Ising Antiferromagnet

    Science.gov (United States)

    Barry, J. H.; Khatun, M.

    The kagomé Ising antiferromagnet is highly frustrated with its pair correlation decaying exponentially at large distance for all temperatures including absolute zero. Hence, the spin system does not support long-range orderings and is devoid of any phase transition. One proves, via local star-triangle and decoration-decimation transformations, that correlations in the kagomé Ising antiferromagnet at arbitrary temperatures can be represented as linear combinations of correlations in the honeycomb Ising ferromagnet at high temperatures (disordered region). Existent knowledge of all honeycomb Ising correlations upon a select (spatially compact) 10-site cluster is thus sufficient to determine all present kagomé Ising correlations upon an associated 9-site cluster. Examples of resulting exact solutions for pair and multisite correlations in the kagomé Ising antiferromagnet are presented at all temperatures. Applications include joint configuration probabilities, thermodynamic response functions such as the specific heat and the initial perpendicular susceptibility, and the inelastic neutron scattering function.

  20. Static and Dynamical Properties of Antiferromagnetic Skyrmions in the Presence of Applied Current and Temperature

    Science.gov (United States)

    Barker, Joseph; Tretiakov, Oleg A.

    2016-04-01

    Skyrmions are topologically protected entities in magnetic materials which have the potential to be used in spintronics for information storage and processing. However, Skyrmions in ferromagnets have some intrinsic difficulties which must be overcome to use them for spintronic applications, such as the inability to move straight along current. We show that Skyrmions can also be stabilized and manipulated in antiferromagnetic materials. An antiferromagnetic Skyrmion is a compound topological object with a similar but of opposite sign spin texture on each sublattice, which, e.g., results in a complete cancellation of the Magnus force. We find that the composite nature of antiferromagnetic Skyrmions gives rise to different dynamical behavior due to both an applied current and temperature effects.

  1. Scaling relations of three-dimensional random-exchange quantum antiferromagnets

    Science.gov (United States)

    Tan, Deng-Ruei; Jiang, Fu-Jiun

    2015-11-01

    The thermal and ground state properties of a class of three-dimensional (3D) random-exchange spin-1/2 antiferromagnets are studied using first principles quantum Monte Carlo method. Our motivation is to examine whether the newly discovered universal scaling properties, which connect the Néel temperature and the staggered magnetization density, for the clean 3D quantum dimerized Heisenberg models remain valid for the random-exchange models considered here. Remarkably, similar to the clean systems, our Monte Carlo results indicate that these scaling relations also emerge for the considered models with the introduced antiferromagnetic randomness. The scope of the validity of these scaling properties for the 3D quantum antiferromagnets is investigated as well.

  2. Magnetism in the iron-based superconductors: The determination of spin-nematic fluctuations as the primary order parameter and its implications for unconventional superconductivity

    Science.gov (United States)

    Taddei, Keith M.

    With nearly innumerable applications, superconductivity stands as a holy grail in the research of quantum phenomena. Understanding the mechanism that begets the fabled pairing of electrons which leads to zero resistance is the most significant undertaking in order to bring to fruition all of superconductivity's splendor. Yet the interaction which couples electrons in the most promising family of superconductors known as unconventional superconductors, which show the highest Tc's and largest upper critical fields remains a mystery. Intense study over the past several decades on the cuprate superconductors has allowed for the identification of several candidate mechanisms --- cardinal of which is magnetic fluctuations --- however as of yet the question still remains. Recently, the discovery of the iron-based superconductors has provided another fruitful avenue through which this mechanism can be probed. Excitingly in these materials superconductivity not only arises near a magnetic instability - a situation which is expected to be particularly suited for engendering superconductivity should magnetic fluctuations be the pairing mechanism - but also exhibit the microscopic co-existence of the two presumably adversarial phenomena. In the work presented here the powerful techniques of neutron and x-ray diffraction will be used to study two particularly interesting members of this family: the intercalated iron-selenide CsxFe 2--xSe2 and two members of the iron-arsenide 122 family (BaFe2(As1--xPx)2 and Sr1--xNaxFe2As 2). Though isostructural at high temperatures, these two materials behave remarkably differently and the idiosyncratic manifestations of superconductivity and ordered magnetism in either give clues as to how the latter might stabilize the former. The iron-selenides will be shown to exhibit a complex phase space with phase separation leading to stabilization of magnetism and superconductivity in separate phases. The structure, behavior and complex vacancy

  3. Spin thermoelectric effects in organic single-molecule devices

    Energy Technology Data Exchange (ETDEWEB)

    Wang, H.L.; Wang, M.X.; Qian, C.; Hong, X.K.; Zhang, D.B.; Liu, Y.S.; Yang, X.F., E-mail: xfyang@cslg.edu.cn

    2017-05-25

    Highlights: • A stronger spin thermoelectric performance in a polyacetylene device is observed. • For the antiferromagnetic (AFM) ordering, a transport gap is opened. Thus the thermoelectric effects are largely enhanced. - Abstract: The spin thermoelectric performance of a polyacetylene chain bridging two zigzag graphene nanoribbons (ZGNRs) is investigated based on first principles method. Two different edge spin arrangements in ZGNRs are considered. For ferromagnetic (FM) ordering, transmission eigenstates with different spin indices distributed below and above Fermi level are observed, leading directly to a strong spin thermoelectric effect in a wide temperature range. With the edge spins arranged in the antiferromagnetic (AFM) ordering, an obvious transport gap appears in the system, which greatly enhances the thermoelectric effects. The presence of a small spin splitting also induces a spin thermoelectric effect greater than the charge thermoelectric effect in certain temperature range. In general, the single-molecule junction exhibits the potential to be used for the design of perfect thermospin devices.

  4. The fluctuating gap model

    International Nuclear Information System (INIS)

    Cao, Xiaobin

    2011-01-01

    The quasi-one-dimensional systems exhibit some unusual phenomenon, such as the Peierls instability, the pseudogap phenomena and the absence of a Fermi-Dirac distribution function line shape in the photoemission spectroscopy. Ever since the discovery of materials with highly anisotropic properties, it has been recognized that fluctuations play an important role above the three-dimensional phase transition. This regime where the precursor fluctuations are presented can be described by the so called fluctuating gap model (FGM) which was derived from the Froehlich Hamiltonian to study the low energy physics of the one-dimensional electron-phonon system. Not only is the FGM of great interest in the context of quasi-one-dimensional materials, liquid metal and spin waves above T c in ferromagnets, but also in the semiclassical approximation of superconductivity, it is possible to replace the original three-dimensional problem by a directional average over effectively one-dimensional problem which in the weak coupling limit is described by the FGM. In this work, we investigate the FGM in a wide temperature range with different statistics of the order parameter fluctuations. We derive a formally exact solution to this problem and calculate the density of states, the spectral function and the optical conductivity. In our calculation, we show that a Dyson singularity appears in the low energy density of states for Gaussian fluctuations in the commensurate case. In the incommensurate case, there is no such kind of singularity, and the zero frequency density of states varies differently as a function of the correlation lengths for different statistics of the order parameter fluctuations. Using the density of states we calculated with non-Gaussian order parameter fluctuations, we are able to calculate the static spin susceptibility which agrees with the experimental data very well. In the calculation of the spectral functions, we show that as the correlation increases, the quasi

  5. The fluctuating gap model

    Energy Technology Data Exchange (ETDEWEB)

    Cao, Xiaobin

    2011-01-15

    The quasi-one-dimensional systems exhibit some unusual phenomenon, such as the Peierls instability, the pseudogap phenomena and the absence of a Fermi-Dirac distribution function line shape in the photoemission spectroscopy. Ever since the discovery of materials with highly anisotropic properties, it has been recognized that fluctuations play an important role above the three-dimensional phase transition. This regime where the precursor fluctuations are presented can be described by the so called fluctuating gap model (FGM) which was derived from the Froehlich Hamiltonian to study the low energy physics of the one-dimensional electron-phonon system. Not only is the FGM of great interest in the context of quasi-one-dimensional materials, liquid metal and spin waves above T{sub c} in ferromagnets, but also in the semiclassical approximation of superconductivity, it is possible to replace the original three-dimensional problem by a directional average over effectively one-dimensional problem which in the weak coupling limit is described by the FGM. In this work, we investigate the FGM in a wide temperature range with different statistics of the order parameter fluctuations. We derive a formally exact solution to this problem and calculate the density of states, the spectral function and the optical conductivity. In our calculation, we show that a Dyson singularity appears in the low energy density of states for Gaussian fluctuations in the commensurate case. In the incommensurate case, there is no such kind of singularity, and the zero frequency density of states varies differently as a function of the correlation lengths for different statistics of the order parameter fluctuations. Using the density of states we calculated with non-Gaussian order parameter fluctuations, we are able to calculate the static spin susceptibility which agrees with the experimental data very well. In the calculation of the spectral functions, we show that as the correlation increases, the

  6. Magnons, Spin Current and Spin Seebeck Effect

    Science.gov (United States)

    Maekawa, Sadamichi

    2012-02-01

    When metals and semiconductors are placed in a temperature gradient, the electric voltage is generated. This mechanism to convert heat into electricity, the so-called Seebeck effect, has attracted much attention recently as the mechanism for utilizing wasted heat energy. [1]. Ferromagnetic insulators are good conductors of spin current, i.e., the flow of electron spins [2]. When they are placed in a temperature gradient, generated are magnons, spin current and the spin voltage [3], i.e., spin accumulation. Once the spin voltage is converted into the electric voltage by inverse spin Hall effect in attached metal films such as Pt, the electric voltage is obtained from heat energy [4-5]. This is called the spin Seebeck effect. Here, we present the linear-response theory of spin Seebeck effect based on the fluctuation-dissipation theorem [6-8] and discuss a variety of the devices. [4pt] [1] S. Maekawa et al, Physics of Transition Metal Oxides (Springer, 2004). [0pt] [2] S. Maekawa: Nature Materials 8, 777 (2009). [0pt] [3] Concept in Spin Electronics, eds. S. Maekawa (Oxford University Press, 2006). [0pt] [4] K. Uchida et al., Nature 455, 778 (2008). [0pt] [5] K. Uchida et al., Nature Materials 9, 894 (2010) [0pt] [6] H. Adachi et al., APL 97, 252506 (2010) and Phys. Rev. B 83, 094410 (2011). [0pt] [7] J. Ohe et al., Phys. Rev. B (2011) [0pt] [8] K. Uchida et al., Appl. Phys. Lett. 97, 104419 (2010).

  7. SPIN SUSCEPTIBILITY IN HIGH - TC SUPERCONDUCTIVITY

    African Journals Online (AJOL)

    USER

    2012-07-05

    Jul 5, 2012 ... Anderson (KGA)rules(Suzuki,Suzuki,2009) will upturn the. Cu spins. It turns that this process introduces the now measurable spin fluctuations in the cuprates. The AFM sublattices contain two spin magnetic moments as we know and according to basic theory of magnetism, equal and opposite spin currents ...

  8. GPU-Accelerated Population Annealing Algorithm: Frustrated Ising Antiferromagnet on the Stacked Triangular Lattice

    Directory of Open Access Journals (Sweden)

    Borovský Michal

    2016-01-01

    Full Text Available The population annealing algorithm is a novel approach to study systems with rough free-energy landscapes, such as spin glasses. It combines the power of simulated annealing, Boltzmann weighted differential reproduction and sequential Monte Carlo process to bring the population of replicas to the equilibrium even in the low-temperature region. Moreover, it provides a very good estimate of the free energy. The fact that population annealing algorithm is performed over a large number of replicas with many spin updates, makes it a good candidate for massive parallelism. We chose the GPU programming using a CUDA implementation to create a highly optimized simulation. It has been previously shown for the frustrated Ising antiferromagnet on the stacked triangular lattice with a ferromagnetic interlayer coupling, that standard Markov Chain Monte Carlo simulations fail to equilibrate at low temperatures due to the effect of kinetic freezing of the ferromagnetically ordered chains. We applied the population annealing to study the case with the isotropic intra- and interlayer antiferromagnetic coupling (J2/|J1| = −1. The reached ground states correspond to non-magnetic degenerate states, where chains are antiferromagnetically ordered, but there is no long-range ordering between them, which is analogical with Wannier phase of the 2D triangular Ising antiferromagnet.

  9. Breatherlike electromagnetic wave propagation in an antiferromagnetic medium with Dzyaloshinsky-Moriya interaction

    International Nuclear Information System (INIS)

    Kavitha, L.; Saravanan, M.; Srividya, B.; Gopi, D.

    2011-01-01

    We investigate the nature of propagation of electromagnetic waves (EMWs) in an antiferromagnetic medium with Dzyaloshinsky-Moriya (DM) interaction environment. The interplay of bilinear and DM exchange spin coupling with the magnetic field component of the EMW has been studied by solving Maxwell's equations coupled with a nonlinear spin equation for the magnetization of the medium. We made a nonuniform expansion of the magnetization and magnetic field along the direction of propagation of EMW, in the framework of reductive perturbation method, and the dynamics of the system is found to be governed by a generalized derivative nonlinear Schroedinger (DNLS) equation. We employ the Jacobi-elliptic function method to solve the DNLS equation, and the electromagnetic wave propagation in an antiferromagnetic medium is governed by the breatherlike spatially and temporally coherent localized modes under the influence of DM interaction parameter.

  10. Quantum critical scaling and fluctuations in Kondo lattice materials

    Science.gov (United States)

    Yang, Yi-feng; Pines, David; Lonzarich, Gilbert

    2017-01-01

    We propose a phenomenological framework for three classes of Kondo lattice materials that incorporates the interplay between the fluctuations associated with the antiferromagnetic quantum critical point and those produced by the hybridization quantum critical point that marks the end of local moment behavior. We show that these fluctuations give rise to two distinct regions of quantum critical scaling: Hybridization fluctuations are responsible for the logarithmic scaling in the density of states of the heavy electron Kondo liquid that emerges below the coherence temperature T∗, whereas the unconventional power law scaling in the resistivity that emerges at lower temperatures below TQC may reflect the combined effects of hybridization and antiferromagnetic quantum critical fluctuations. Our framework is supported by experimental measurements on CeCoIn5, CeRhIn5, and other heavy electron materials. PMID:28559308

  11. Magnetic Phase Transitions in Quantum Ising Model with Annealed Antiferromagnetic Bond Randomness

    Science.gov (United States)

    Shi, Zhu-pei; Tao, Rui-bao

    1990-06-01

    The effect of annealed antiferromagnetic bond randomness on the phase transitions of the Quantum Ising Model (QIM) is studied by using mean-field renormalization group method. It is argued that bond randomness drastically alters multicritical phase diagram via transverse field. Multicritical points and coexistence region of ferromagnetic and antiferromagnetic case exist only at weak transverse field, and are entirely eliminated at strong transverse field. The coexistence region diminishes in reducing the fluctuation interaction. This physical picture demonstrates that the competition between transverse field and exchange interaction and fluctuation interaction via bond randomness play an important role in generating multiphase structure. Another consequence of competition is that tricritical points of first-second order phase transitions are not entirely eliminated by bond randomness in two-dimensional QIM. The project supported by the Foundation of Doctoral Education.

  12. Spin texture motion in antiferromagnetic and ferromagnetic nanowires

    Czech Academy of Sciences Publication Activity Database

    Rodrigues, D.R.; Everschor-Sitte, K.; Tretiakov, O.A.; Sinova, Jairo; Abanov, A.

    2017-01-01

    Roč. 95, č. 17 (2017), s. 1-7, č. článku 174408. ISSN 2469-9950 R&D Projects: GA ČR GB14-37427G EU Projects: European Commission(XE) 610115 - SC2 Institutional support: RVO:68378271 Keywords : orbit torques * magnetization * spintronics Subject RIV: BM - Solid Matter Physics ; Magnetism OBOR OECD: Condensed matter physics (including formerly solid state physics, supercond.) Impact factor: 3.836, year: 2016

  13. Spinon confinement in the quasi-1D Ising-like antiferromagnet SrCo{sub 2}V{sub 2}O{sub 8}

    Energy Technology Data Exchange (ETDEWEB)

    Wang, Zhe; Schmidt, Michael; Loidl, Alois; Deisenhofer, Joachim [Experimental Physics V, Center for Electronic Correlations and Magnetism, University of Augsburg, Augsburg (Germany); Bera, Anup Kumar [Helmholtz-Zentrum Berlin fuer Materialien und Energie, Berlin (Germany); Lake, Bella [Helmholtz-Zentrum Berlin fuer Materialien und Energie, Berlin (Germany); Institut fuer Festkoerperphysik, Technische Universitaet Berlin, Berlin (Germany)

    2015-07-01

    Using THz transmission spectroscopy in magnetic field, we have investigated low-energy magnetic excitations in the quasi-one-dimensional Ising-like XXZ antiferromagnet SrCo{sub 2}V{sub 2}O{sub 8}. Spinon-pair excitations on the antiferromagnetic ground state have been observed in the XXZ antiferromagnet. Spinon-pair bound states with entangled spin-orbit moment S = 1 are determined unambiguously. The hierarchy of the spinon-pair boundstates can be described by a one-dimensional Schroedinger equation with a linear confinement potential imposed by the interchain interaction.

  14. Magnetic hysteresis and domain wall dynamics in single chain magnets with antiferromagnetic interchain coupling

    Energy Technology Data Exchange (ETDEWEB)

    Bukharov, A A; Ovchinnikov, A S; Baranov, N V [Department of Physics, Ural State University, Ekaterinburg, 620083 (Russian Federation); Inoue, K [Institute for Advanced Materials Research, Hiroshima University, Hiroshima (Japan)

    2010-11-03

    Using Monte Carlo simulations we investigate magnetic hysteresis in two- and three-dimensional systems of weakly antiferromagnetically coupled spin chains based on a scenario of domain wall (kink) motion within the chains. By adapting the model of walkers to simulate the domain wall dynamics and using the Ising-like dipole-dipole model, we study the effects of interchain coupling, temperature and anisotropy axis direction on hysteresis curves.

  15. Photo-induced antiferromagnetic interlayer coupling in Fe superlattices with iron silicide spacers

    Energy Technology Data Exchange (ETDEWEB)

    Mattson, J.E.; Fullerton, E.E.; Kumar, S.; Lee, S.R.; Sowers, C.H.; Grimsditch, M.; Bader, S.D. [Argonne National Lab., IL (United States); Parker, F.T. [California Univ., San Diego, La Jolla, CA (United States). Center for Magnetic Recording Research

    1993-09-01

    Sputtered Fe/FeSi films possessing antiferromagnetic (AF) interlayer coupling at room temperature develop ferromagnetic remanence when cooled below 100K, but the AF coupling can be restored at low temperature by exposure to visible light of sufficient intensity (>10 mW/mm{sup 2}). We attribute these effects to charge carriers in the FeSi spacer layer which, when thermally or photo-generated, are capable of communicating spin information between the Fe layers.

  16. Remanent Magnetization: Signature of Many-Body Localization in Quantum Antiferromagnets

    Science.gov (United States)

    Ros, V.; Müller, M.

    2017-06-01

    We study the remanent magnetization in antiferromagnetic, many-body localized quantum spin chains, initialized in a fully magnetized state. Its long time limit is an order parameter for the localization transition, which is readily accessible by standard experimental probes in magnets. We analytically calculate its value in the strong-disorder regime exploiting the explicit construction of quasilocal conserved quantities of the localized phase. We discuss analogies in cold atomic systems.

  17. Magnetotransport and Antiferromagnetic Behavior in ErP Epitaxial Layers on GaInP(001)

    Science.gov (United States)

    Nakamura, A.; Ito, T.; Ohnishi, H.; Koizumi, A.; Takeda, Y.

    2007-04-01

    We have investigated transport and magnetic properties in ErP ultrathin films grown on the GaInP (001) surface. Hall resistance and transverse magnetoresistance measurements yield the carrier density of ˜1.4×1020 cm-3 and the electron and hole mobilities of 1250-1450 cm2/Vs at 10 K. The resistivity anomaly in the longitudinal megnetoresistance is interpreted in terms of the spin-disorder scattering in the antiferromagnetic phase below 3.5 K.

  18. Field-Induced Magnetostructural Transitions in Antiferromagnetic Fe1+ y Te1- x S x

    Science.gov (United States)

    Tokunaga, M.; Kihara, T.; Mizuguchi, Y.; Takano, Y.

    2013-03-01

    Transport and structural properties of Fe1+ y Te1- x S x were studied in pulsed magnetic fields. Application of high magnetic fields induces first order transitions showing positive magnetoresistance effects in the antiferromagnetic phase. Polarizing microscope images taken at high magnetic fields revealed the concomitant melting of the orbital order. These results indicate the importance of crossed coupling between spin and lattice or orbital degrees of freedom in this compound.

  19. Low-temperature spin dynamics of a valence bond glass in Ba2YMoO6

    Science.gov (United States)

    de Vries, M. A.; Piatek, J. O.; Misek, M.; Lord, J. S.; Rønnow, H. M.; Bos, J.-W. G.

    2013-04-01

    We carried out ac magnetic susceptibility measurements and muon spin relaxation spectroscopy on the cubic double perovskite Ba2YMoO6, down to 50 mK. Below ∼1 K the muon relaxation is typical of a magnetic insulator with a spin-liquid type ground state, i.e. without broken symmetries or frozen moments. However, the ac susceptibility revealed a dilute-spin-glass-like transition below ∼1 K. Antiferromagnetically coupled Mo5+ 4d1 electrons in triply degenerate t2g orbitals are in this material arranged in a geometrically frustrated fcc lattice. Bulk magnetic susceptibility data has previously been interpreted in terms of a freezing to a heterogeneous state with non-magnetic sites where 4d1 electrons have paired in spin-singlets dimers, and residual unpaired Mo5+ 4d1 electron spins. Based on the magnetic heat capacity data it has been suggested that this heterogeneity is the result of kinetic constraints intrinsic to the physics of the pure system (possibly due to topological overprotection) leading to a self-induced glass of valence bonds between neighbouring 4d1 electrons. The muon spin relaxation (μSR) unambiguously points to a heterogeneous state with a static arrangement of unpaired electrons in a background of (valence bond) dimers between the majority of Mo5+ 4d electrons. The ac susceptibility data indicate that the residual magnetic moments freeze into a dilute-spin-glass-like state. This is in apparent contradiction with the muon-spin decoupling at 50 mK in fields up to 200 mT, which indicates that, remarkably, the time scale of the field fluctuations from the residual moments is ∼5 ns. Comparable behaviour has been observed in other geometrically frustrated magnets with spin-liquid-like behaviour and the implications of our observations on Ba2YMoO6 are discussed in this context.

  20. Prediction for spin Fano factor generated by biased quantum spin chains

    Science.gov (United States)

    Aftergood, Joshua; Takei, So

    We theoretically study noise in the spin current injected into a normal metal from a 1D Heisenberg spin- 1 / 2 antiferromagnet. We consider the noise generated in two separate scenarios: first by inducing an over-population of one chiral mode relative to the other in the spin chain at uniform temperature, and second by elevating the temperature of the spin chain relative to the metal, i.e., by way of the spin Seebeck effect. We compute excess noise in the normal metal generated by the coupling to the spin chain and predict the spin Fano factor, defined as the noise in the spin current normalized by the average spin current, for both scenarios. The authors thank the PSC-CUNY Research Award Program for its support.

  1. Muon spin rotation study of magnetism and superconductivity in Ba(Fe1-xCox)2As2 single crystals

    DEFF Research Database (Denmark)

    Bernhard, C.; Wang, C. N.; Nuccio, L.

    2012-01-01

    Using muon spin rotation (μSR) we investigated the magnetic and superconducting properties of a series of Ba(Fe1−xCox)2As2 single crystals with 0 ≤x ≤0.15. Our study details how the antiferromagnetic order is suppressed upon Co substitution and how it coexists with superconductivity. In the nonsu......Using muon spin rotation (μSR) we investigated the magnetic and superconducting properties of a series of Ba(Fe1−xCox)2As2 single crystals with 0 ≤x ≤0.15. Our study details how the antiferromagnetic order is suppressed upon Co substitution and how it coexists with superconductivity...... caused by the randomly distributed Co atoms. A different kind of magnetic order that was also previously identified [C. Bernhard et al., New J. Phys. 11, 055050 (2009)] occurs at 0.055 magnetic order develops here only in parts of the sample volume...... and it seems to cooperate with superconductivity since its onset temperature coincides with Tc. Even in the strongly overdoped regime at x = 0.11, where the static magnetic order has disappeared, we find that the low-energy spin fluctuations are anomalously enhanced below Tc. These findings point toward...

  2. Spin coupling in zigzag Wigner crystals

    International Nuclear Information System (INIS)

    Klironomos, A. D.; Meyer, J. S.; Hikihara, T.; Matveev, K. A.

    2007-01-01

    We consider interacting electrons in a quantum wire in the case of a shallow confining potential and low electron density. In a certain range of densities, the electrons form a two-row (zigzag) Wigner crystal whose spin properties are determined by nearest and next-nearest neighbor exchange as well as by three- and four-particle ring exchange processes. The phase diagram of the resulting zigzag spin chain has regions of complete spin polarization and partial spin polarization in addition to a number of unpolarized phases, including antiferromagnetism and dimer order as well as a novel phase generated by the four-particle ring exchange

  3. Strain fields and electronic structure of antiferromagnetic CrN

    Science.gov (United States)

    Rojas, Tomas; Ulloa, Sergio E.

    2017-09-01

    We present a theoretical analysis of the role that strain plays on the electronic structure of chromium nitride (CrN) crystals. We use local spin-density approximation + U calculations to study the elastic constants, deformation potentials, and strain dependence of electron and hole masses near the fundamental gap. We consider the lowest energy antiferromagnetic models believed to describe CrN at low temperatures, and apply strain along different directions. We find relatively large deformation potentials for all models, and find increasing gaps for tensile strain along most directions. Most interestingly, we find that compressive strains should be able to close the relatively small indirect gap (≃100 meV) at moderate amplitudes ≃1.3 % . We also find large and anisotropic changes in the effective masses with strain, with principal axes closely related to the magnetic ordering of neighboring layers in the antiferromagnet. It would be interesting to consider the role that these effects may have on typical film growth on different substrates, and the possibility of monitoring optical and transport properties of thin films as strain is applied.

  4. Unusual spin frozen state in a frustrated pyrochlore system NaCaCo{sub 2}F{sub 7} as observed by NMR

    Energy Technology Data Exchange (ETDEWEB)

    Sarkar, R.; Brueckner, F.; Klauss, H.H. [IFP, TU Dresden (Germany); Krizan, J.W.; Cava, R.J. [Department of Chemistry, Princeton University, Princeton, NJ (United States)

    2016-07-01

    We present {sup 23}Na -and {sup 19}F NMR results on the magnetically frustrated pyrochlore NaCaCo{sub 2}F{sub 7} with a frustration index of f = θ{sub CW}/T{sub f} ∝ 56. Recent neutron scattering experiments proposed XY like antiferromagnetic spin clusters at low energies in NaCaCo{sub 2}F{sub 7}. {sup 23}Na NMR -spectra reveal the presence of two magnetically non equivalent Na sites in conjunction with the local Co{sup 2+} spin structure. Below 3.6 K both the {sup 23}Na -and {sup 19}F spectra broaden due to the formation of static spin correlations. A huge reduction of the {sup 19}F -and {sup 23}Na NMR signal intensity hints at a quasi-static field distribution in NaCaCo{sub 2}F{sub 7} in this regime. The {sup 19}F spin-lattice relaxation rate {sup 19}(1/T{sub 1}) exhibits a peak at around 2.9 K, at the same temperature range where ac and dc susceptibility data show a broad maximum. The character of the spin fluctuation appears to be isotropic. The overall temperature dependence of {sup 19}(1/T{sub 1}) can be described by the BPP theory considering a fluctuating hyperfine field with an autocorrelation function. The correlation time of the autocorrelation function exhibits an activation behavior further indicating the spin-frozen state. While the present NMR studies suggest the spin frozen state at low temperatures, μSR investigations however reveal the presence of so called persistent spin dynamics down to 20 mK implying an exotic ground state in NaCaCo{sub 2}F{sub 7}.

  5. Synthetic antiferromagnetic nanoparticles with tunable susceptibilities

    Science.gov (United States)

    Hu, Wei; Wilson, Robert J.; Earhart, Christopher M.; Koh, Ai Leen; Sinclair, Robert; Wang, Shan X.

    2009-01-01

    High-moment monodisperse disk-shaped Co–Fe magnetic nanoparticles, stable in aqueous solution, were physically fabricated by using nanoimprinted templates and vacuum deposition techniques. These multilayer synthetic antiferromagnetic nanoparticles exhibit nearly zero magnetic remanence and coercivity, and susceptibilities which can be tuned by exploiting interlayer magnetic interactions. In addition, a low cost method of scaling up the production of sub-100 nm synthetic antiferromagnetic nanoparticles is demonstrated. PMID:19529797

  6. Faraday rotation echo spectroscopy and detection of quantum fluctuations.

    Science.gov (United States)

    Chen, Shao-Wen; Liu, Ren-Bao

    2014-04-15

    Central spin decoherence is useful for detecting many-body physics in environments and moreover, the spin echo control can remove the effects of static thermal fluctuations so that the quantum fluctuations are revealed. The central spin decoherence approach, however, is feasible only in some special configurations and often requires uniform coupling between the central spin and individual spins in the baths, which are very challenging in experiments. Here, by making analogue between central spin decoherence and depolarization of photons, we propose a scheme of Faraday rotation echo spectroscopy (FRES) for studying quantum fluctuations in interacting spin systems. The echo control of the photon polarization is realized by flipping the polarization with a birefringence crystal. The FRES, similar to spin echo in magnetic resonance spectroscopy, can suppress the effects of the static magnetic fluctuations and therefore reveal dynamical magnetic fluctuations. We apply the scheme to a rare-earth compound LiHoF4 and calculate the echo signal, which is related to the quantum fluctuations of the system. We observe enhanced signals at the phase boundary. The FRES should be useful for studying quantum fluctuations in a broad range of spin systems, including cold atoms, quantum dots, solid-state impurities, and transparent magnetic materials.

  7. Antiferromagnetic bipolar semiconductor LaMnPO with ZrCuSiAs-type structure

    OpenAIRE

    Yanagi, Hiroshi; Watanabe, Takumi; Kodama, Katsuaki; Iikubo, Satoshi; Shamoto, Shin-ichi; Kamiya, Toshio; Hirano, Masahiro; Hosono, Hideo

    2009-01-01

    Electronic and magnetic properties of a layered compound LaMnPO are examined in relation to a newly discovered iso-structural superconductor LaFeAs(P)O. Neutron diffraction measurements, together with temperature dependent magnetic susceptibility, clarify that LaMnPO is an antiferromagnet at least up to 375 K. The spin moment of a Mn ion is determined to be 2.26  µB at room temperature, and the spin configuration is antiparallel in the Mn–P plane and parallel between the Mn–P planes, which is...

  8. Monte Carlo study of four-spinon dynamic structure function in antiferromagnetic Heisenberg model

    International Nuclear Information System (INIS)

    Si-Lakhal, B.; Abada, A.

    2003-11-01

    Using Monte Carlo integration methods, we describe the behavior of the exact four-s pinon dynamic structure function S 4 in the antiferromagnetic spin 1/2 Heisenberg quantum spin chain as a function of the neutron energy ω and momentum transfer k. We also determine the fourspinon continuum, the extent of the region in the (k, ω) plane outside which S 4 is identically zero. In each case, the behavior of S 4 is shown to be consistent with the four-spinon continuum and compared to the one of the exact two-spinon dynamic structure function S 2 . Overall shape similarity is noted. (author)

  9. Double-Exchange Interaction in Optically Induced Nonequilibrium State: A Conversion from Ferromagnetic to Antiferromagnetic Structure

    Science.gov (United States)

    Ono, Atsushi; Ishihara, Sumio

    2017-11-01

    The double-exchange (DE) interaction, that is, a ferromagnetic (FM) interaction due to a combination of electron motion and the Hund coupling, is a well-known source of a wide class of FM orders. Here, we show that the DE interaction in highly photoexcited states is antiferromagnetic (AFM). Transient dynamics of quantum electrons coupled with classical spins are analyzed. An ac field applied to a metallic FM state results in an almost perfect Néel state. A time characterizing the FM-to-AFM conversion is scaled by light amplitude and frequency. This hidden AFM interaction is attributable to the electron-spin coupling under nonequilibrium electron distribution.

  10. Long lived excitations in fully compensated antiferromagnetic nanomagnets

    Science.gov (United States)

    Burgess, Jacob; Malavolti, Luigi; Rolf-Pissarczyk, Steffen; McMurtrie, Gregory; Yan, Shichao; Loth, Sebastian

    Extensive interest is directed towards finding long lived states in atomic scale magnetic structures. Applications include classical and quantum spintronics schemes. Here we use a recently described method of applying a single atom exchange bias, using a magnetic scanning tunneling microscope tip, to control the quantum states of fully compensated nano-antiferromagnetic atomic chains. We apply time-resolved spin-polarized scanning tunneling microscopy to measure the energy relaxation of the chains as a function of the tip interaction strength. With strong coupling to the microscope tip, the excited state lifetimes can extend to the millisecond scale. Center for Free Electron Laser Science, Max Planck Society, Deutsches Elektronen-Synchrotron, Alexander von Humboldt Foundation, Natural Sciences and Engineering Research Council of Canada.

  11. Performance of synthetic antiferromagnetic racetrack memory: domain wall versus skyrmion

    KAUST Repository

    Tomasello, R

    2017-06-20

    A storage scheme based on racetrack memory, where the information can be coded in a domain or a skyrmion, seems to be an alternative to conventional hard disk drive for high density storage. Here, we perform a full micromagnetic study of the performance of synthetic antiferromagnetic (SAF) racetrack memory in terms of velocity and sensitivity to defects by using experimental parameters. We find that, to stabilize a SAF skyrmion, the Dzyaloshinskii–Moriya interaction in the top and the bottom ferromagnet should have an opposite sign. The velocity of SAF skyrmions and SAF Néel domain walls are of the same order and can reach values larger than 1200 m s−1 if a spin–orbit torque from the spin-Hall effect with opposite sign is applied to both ferromagnets. The presence of disordered anisotropy in the form of randomly distributed grains introduces a threshold current for both SAF skyrmions and SAF domain walls motions.

  12. Producing coherent excitations in pumped Mott antiferromagnetic insulators

    Science.gov (United States)

    Wang, Yao; Claassen, Martin; Moritz, B.; Devereaux, T. P.

    2017-12-01

    Nonequilibrium dynamics in correlated materials has attracted attention due to the possibility of characterizing, tuning, and creating complex ordered states. To understand the photoinduced microscopic dynamics, especially the linkage under realistic pump conditions between transient states and remnant elementary excitations, we performed nonperturbative simulations of various time-resolved spectroscopies. We used the Mott antiferromagnetic insulator as a model platform. The transient dynamics of multiparticle excitations can be attributed to the interplay between Floquet virtual states and a modification of the density of states, in which interactions induce a spectral weight transfer. Using an autocorrelation of the time-dependent spectral function, we show that resonance of the virtual states with the upper Hubbard band in the Mott insulator provides the route towards manipulating the electronic distribution and modifying charge and spin excitations. Our results link transient dynamics to the nature of many-body excitations and provide an opportunity to design nonequilibrium states of matter via tuned laser pulses.

  13. Antiferromagnetic order in the Hubbard model on the Penrose lattice

    Science.gov (United States)

    Koga, Akihisa; Tsunetsugu, Hirokazu

    2017-12-01

    We study an antiferromagnetic order in the ground state of the half-filled Hubbard model on the Penrose lattice and investigate the effects of quasiperiodic lattice structure. In the limit of infinitesimal Coulomb repulsion U →+0 , the staggered magnetizations persist to be finite, and their values are determined by confined states, which are strictly localized with thermodynamics degeneracy. The magnetizations exhibit an exotic spatial pattern, and have the same sign in each of cluster regions, the size of which ranges from 31 sites to infinity. With increasing U , they continuously evolve to those of the corresponding spin model in the U =∞ limit. In both limits of U , local magnetizations exhibit a fairly intricate spatial pattern that reflects the quasiperiodic structure, but the pattern differs between the two limits. We have analyzed this pattern change by a mode analysis by the singular value decomposition method for the fractal-like magnetization pattern projected into the perpendicular space.

  14. Suppression of tunneling by interference in half-integer--spin particles

    OpenAIRE

    Loss, Daniel; DiVincenzo, David P.; Grinstein, G.

    1992-01-01

    Within a wide class of ferromagnetic and antiferromagnetic systems, quantum tunneling of magnetization direction is spin-parity dependent: it vanishes for magnetic particles with half-integer spin, but is allowed for integer spin. A coherent-state path integral calculation shows that this topological effect results from interference between tunneling paths.

  15. Quantum fluctuations

    International Nuclear Information System (INIS)

    Reynaud, S.; Giacobino, S.; Zinn-Justin, J.

    1997-01-01

    This course is dedicated to present in a pedagogical manner the recent developments in peculiar fields concerned by quantum fluctuations: quantum noise in optics, light propagation through dielectric media, sub-Poissonian light generated by lasers and masers, quantum non-demolition measurements, quantum electrodynamics applied to cavities and electrical circuits involving superconducting tunnel junctions. (A.C.)

  16. Polarized neutron powder diffraction studies of antiferromagnetic order in bulk and nanoparticle NiO

    DEFF Research Database (Denmark)

    Brok, Erik; Lefmann, Kim; Deen, Pascale P.

    2015-01-01

    In many materials it remains a challenge to reveal the nature of magnetic correlations, including antiferromagnetism and spin disorder. Revealing the spin structure in magnetic nanoparticles is further complicated by the large incoherent neutron scattering cross section from water adsorbed...... surface contribution to the magnetic anisotropy. Here we explore the potential use of polarized neutron diffraction to reveal the magnetic structure in NiO bulk and nanoparticle powders by applying the XYZ-polarization analysis method. Our investigations address in particular the spin orientation in bulk...... at the particle surfaces and by the broadening of diffraction peaks due to the finite crystallite size. Moreover, the spin structure in magnetic nanoparticles may deviate significantly from that of the corresponding bulk material because of the low-symmetry surroundings of surface atoms and the large relative...

  17. Low temperature properties of the triangular-lattice antiferromagnet: a bosonic spinon theory

    Science.gov (United States)

    Mezio, A.; Manuel, L. O.; Singh, R. R. P.; Trumper, A. E.

    2012-12-01

    We study the low temperature properties of the triangular-lattice Heisenberg antiferromagnet with a mean field Schwinger spin-\\frac {1}{2} boson scheme that reproduces quantitatively the zero temperature energy spectrum derived previously using series expansions. By analyzing the spin-spin and the boson density-density dynamical structure factors, we identify the unphysical spin excitations that come from the relaxation of the local constraint on bosons. This allows us to reconstruct a free energy based on the physical excitations only, whose predictions for entropy and uniform susceptibility seem to be reliable within the temperature range 0 ⩽ T ≲ 0.3J, which is difficult to access by other methods. The high values of entropy, also found in high temperature expansion studies, can be attributed to the roton-like narrowed dispersion at finite temperatures.

  18. The phase diagrams and the order parameters of the diluted superlattice with antiferromagnetic interface coupling

    International Nuclear Information System (INIS)

    Oubelkacem, A.; El Aouad, N.; Bentaleb, M.; Laaboudi, B.; Saber, M.

    2004-01-01

    Using the effective field theory with a probability distribution technique that accounts for the self-spin correlation functions, the magnetic properties of the diluted Ising superlattice consisting of two ferromagnetic materials A and B, with L a layers of diluted spins S a =((1)/(2)) and L b layers of diluted spins S b =1 with antiferromagnetic interface coupling are examined. For fixed values of the reduced exchange interactions and the concentration c of magnetic atoms, the phase diagrams, the two sublattice magnetizations and the total magnetization for the superlattice with the same spin S a =S b =((1)/(2)) and for S a =((1)/(2)), S b =1 are studied as a function of the temperature. We find a number of characteristic phenomena. In particular, the effect of the concentration c of magnetic atoms, the interlayer coupling and the layer thickness on both the compensation temperature and the magnetization profiles are clarified

  19. Logarithmic corrections from ferromagnetic impurity ending bonds of open antiferromagnetic host chains

    International Nuclear Information System (INIS)

    Lou Jizhong; Qin Shaojin; Su Zhaobin; Dai Jianhui; Yu Lu

    2000-06-01

    We analyze the logarithmic corrections due to ferromagnetic impurity ending bonds of open spin 1/2 antiferromagnetic chains, using the density matrix renormalization group technique. A universal finite size scaling ∼ 1/L log L for impurity contributions in the quasi-degenerate ground state energy is demonstrated for a zigzag spin 1/2 chain at the critical next nearest neighbor coupling and the standard Heisenberg spin 1/2 chain, in the long chain limit. Using an exact solution for the latter case it is argued that one can extract the impurity contributions to the entropy and specific heat from the scaling analysis. It is also shown that a pure spin 3/2 open Heisenberg chain belongs to the same universality class. (author)

  20. Experimental Realization of a Quantum Spin Pump

    DEFF Research Database (Denmark)

    Watson, Susan; Potok, R.; M. Marcus, C.

    2003-01-01

    We demonstrate the operation of a quantum spin pump based on cyclic radio-frequency excitation of a GaAs quantum dot, including the ability to pump pure spin without pumping charge. The device takes advantage of bidirectional mesoscopic fluctuations of pumped current, made spin......-dependent by the application of an in-plane Zeeman field. Spin currents are measured by placing the pump in a focusing geometry with a spin-selective collector....

  1. Magnetic structure and interactions in the quasi-one-dimensional antiferromagnet CaV2O4

    Science.gov (United States)

    Pieper, O.; Lake, B.; Daoud-Aladine, A.; Reehuis, M.; Prokeš, K.; Klemke, B.; Kiefer, K.; Yan, J. Q.; Niazi, A.; Johnston, D. C.; Honecker, A.

    2009-05-01

    CaV2O4 is a spin-1 antiferromagnet, where the magnetic vanadium ions have an orbital degree of freedom and are arranged on quasi-one-dimensional zigzag chains. The first- and second-neighbor vanadium separations are approximately equal suggesting frustrated antiferromagnetic exchange interactions. High-temperature susceptibility and single-crystal neutron-diffraction measurements are used to deduce the dominant exchange paths and orbital configurations. The results suggest that at high temperatures CaV2O4 behaves as a Haldane chain, but at low temperatures, it is a spin-1 ladder. These two magnetic structures are explained by different orbital configurations and show how orbital ordering can drive a system from one exotic spin Hamiltonian to another.

  2. Paramagnetic Spin Correlations in CaFe2As2 Single Crystals

    International Nuclear Information System (INIS)

    Omar Diallo, Souleymane; Pratt, Daniel; Fernandes, Rafael; Tian, Wei; Zarestky, J.L.; Lumsden, Mark D.; Perring, T.G.; Broholm, C.; Ni, Ni; Budko, S.L.; Canfield, Paul; Li, Haifeng; Vaknin, D.; Kreyssig, A.; Goldman, A.I.; Mcqueeney, R.J.

    2010-01-01

    Magnetic correlations in the paramagnetic phase of CaFe2As2(TN=172 K) have been examined by means of inelastic neutron scattering from 180 K ( 1.05TN) up to 300 K (1.8TN). Despite the first-order nature of the magnetic ordering, strong but short-ranged antiferromagnetic (AFM) correlations are clearly observed. These correlations, which consist of quasielastic scattering centered at the wave vector QAFM of the low-temperature AFM structure, are observed up to the highest measured temperature of 300 K and at high energy transfer ( >60 meV). The L dependence of the scattering implies rather weak interlayer coupling in the tetragonal c direction corresponding to nearly two-dimensional fluctuations in the (ab) plane. The spin correlation lengths within the Fe layer are found to be anisotropic, consistent with underlying fluctuations of the AFM stripe structure. Similar to the cobalt-doped superconducting BaFe2As2 compounds, these experimental features can be adequately reproduced by a scattering model that describes short-ranged and anisotropic spin correlations with overdamped dynamics.

  3. Unified molecular field theory for collinear and noncollinear Heisenberg antiferromagnets

    Science.gov (United States)

    Johnston, David C.

    2015-02-01

    A unified molecular field theory (MFT) is presented that applies to both collinear and planar noncollinear Heisenberg antiferromagnets (AFs) on the same footing. The spins in the system are assumed to be identical and crystallographically equivalent. This formulation allows calculations of the anisotropic magnetic susceptibility χ versus temperature T below the AF ordering temperature TN to be carried out for arbitrary Heisenberg exchange interactions Ji j between arbitrary neighbors j of a given spin i without recourse to magnetic sublattices. The Weiss temperature θp in the Curie-Weiss law is written in terms of the Ji j values and TN in terms of the Ji j values and an assumed AF structure. Other magnetic and thermal properties are then expressed in terms of quantities easily accessible from experiment as laws of corresponding states for a given spin S . For collinear ordering these properties are the reduced temperature t =T /TN , the ratio f =θp/TN , and S . For planar noncollinear helical or cycloidal ordering, an additional parameter is the wave vector of the helix or cycloid. The MFT is also applicable to AFs with other AF structures. The MFT predicts that χ (T ≤TN) of noncollinear 120∘ spin structures on triangular lattices is isotropic and independent of S and T and thus clarifies the origin of this universally observed behavior. The high-field magnetization and heat capacity for fields applied perpendicular to the ordering axis (collinear AFs) and ordering plane (planar noncollinear AFs) are also calculated and expressed for both types of AF structures as laws of corresponding states for a given S , and the reduced perpendicular field versus reduced temperature phase diagram is constructed.

  4. Itinerant Antiferromagnetism in RuO_{2}.

    Science.gov (United States)

    Berlijn, T; Snijders, P C; Delaire, O; Zhou, H-D; Maier, T A; Cao, H-B; Chi, S-X; Matsuda, M; Wang, Y; Koehler, M R; Kent, P R C; Weitering, H H

    2017-02-17

    Bulk rutile RuO_{2} has long been considered a Pauli paramagnet. Here we report that RuO_{2} exhibits a hitherto undetected lattice distortion below approximately 900 K. The distortion is accompanied by antiferromagnetic order up to at least 300 K with a small room temperature magnetic moment of approximately 0.05μ_{B} as evidenced by polarized neutron diffraction. Density functional theory plus U (DFT+U) calculations indicate that antiferromagnetism is favored even for small values of the Hubbard U of the order of 1 eV. The antiferromagnetism may be traced to a Fermi surface instability, lifting the band degeneracy imposed by the rutile crystal field. The combination of high Néel temperature and small itinerant moments make RuO_{2} unique among ruthenate compounds and among oxide materials in general.

  5. Itinerant Antiferromagnetism in RuO2

    Science.gov (United States)

    Berlijn, T.; Snijders, P. C.; Delaire, O.; Zhou, H.-D.; Maier, T. A.; Cao, H.-B.; Chi, S.-X.; Matsuda, M.; Wang, Y.; Koehler, M. R.; Kent, P. R. C.; Weitering, H. H.

    2017-02-01

    Bulk rutile RuO2 has long been considered a Pauli paramagnet. Here we report that RuO2 exhibits a hitherto undetected lattice distortion below approximately 900 K. The distortion is accompanied by antiferromagnetic order up to at least 300 K with a small room temperature magnetic moment of approximately 0.05 μB as evidenced by polarized neutron diffraction. Density functional theory plus U (DFT +U ) calculations indicate that antiferromagnetism is favored even for small values of the Hubbard U of the order of 1 eV. The antiferromagnetism may be traced to a Fermi surface instability, lifting the band degeneracy imposed by the rutile crystal field. The combination of high Néel temperature and small itinerant moments make RuO2 unique among ruthenate compounds and among oxide materials in general.

  6. Magnetoresistance and Anti-Ferromagnetic Coupling in FM-Graphene-FM Trilayers

    Science.gov (United States)

    Cobas, Enrique D.; van't Erve, Olaf M. J.; Cheng, Shu-Fan; Jonker, Berend T.

    Both high-magnetoresistance(MR) minority spin filtering and anti-ferromagnetic (AFM) coupling have been predicted for FM|Graphene|FM vertical heterostructures. Our previous experiments demonstrated ordinary magnetoresistance in NiFe-Graphene-Co heterostructures and no evident AFM coupling. Here we present experimental results that confirm both MR minority spin filtering and AFM coupling in high-quality FM|Graphene|FM heterostructures. The heterostructures were fabricated by a combination of sputtering, chemical vapor deposition and electron beam evaporation. The stack was patterned into symmetric cross-bar structures using Ar ion milling. Measurements show negative magnetoresistance in excess of 10 percent, confirming spin-filtering, and weak anti-ferromagnetic coupling throughout the temperature range 15K to 300K. The temperature dependence of the MR was studied and found consistent with thermal excitation of spin waves in the ferromagnetic electrodes. Junction resistance-area products are in the range of 10 Ωcm2. These heterostructures provide a fast and low-power magnetic field sensor in the sub-100 Oe range and are a step towards high-MR low RA-product MRAM junctions.

  7. Spin wave mediated interaction as a mechanism of pairs formation in iron-based superconductors

    Science.gov (United States)

    Lima, Leonardo S.

    2018-03-01

    The spin wave mediated interaction between electrons has been proposed as mechanism to formation of electron pairs in iron-based superconductors. We employe the diagrammatic expansion to calculate the binding energy of electrons pairs mediated by spin wave. Therefore, we propose the coupling of electrons in high-temperature superconductors mediated by spin waves, since that is well known that this class of superconductors materials if relates with spin-1/2 two-dimensional antiferromagnets, where it is well known there be an interplay between antiferromagnetism 2D and high-temperature superconductivity.

  8. Higher-spin cluster algorithms: the Heisenberg spin and U(1) quantum link models

    Energy Technology Data Exchange (ETDEWEB)

    Chudnovsky, V

    2000-03-01

    I discuss here how the highly-efficient spin-1/2 cluster algorithm for the Heisenberg antiferromagnet may be extended to higher-dimensional representations; some numerical results are provided. The same extensions can be used for the U(1) flux cluster algorithm, but have not yielded signals of the desired Coulomb phase of the system.

  9. Higher-spin cluster algorithms: the Heisenberg spin and U(1) quantum link models

    International Nuclear Information System (INIS)

    Chudnovsky, V.

    2000-01-01

    I discuss here how the highly-efficient spin-1/2 cluster algorithm for the Heisenberg antiferromagnet may be extended to higher-dimensional representations; some numerical results are provided. The same extensions can be used for the U(1) flux cluster algorithm, but have not yielded signals of the desired Coulomb phase of the system

  10. Successive magnetic phase transitions and multiferroicity in quasi-two-dimensional triangular lattice Heisenberg antiferromagnets Ba3CoNb2O9 and Ba3MnNb2O9

    Science.gov (United States)

    Lee, M.; Hwang, J.; Choi, E. S.; Ma, J.; Dela Cruz, C. R.; Zhu, M.; Ke, X.; Dun, Z. L.; Zhou, H. D.

    2014-03-01

    We have measured magnetic, dielectric and thermodynamic properties of quasi-two-dimensional triangular lattice antiferromagnet (TLAF), Ba3CoNb2O9 (S = 1/2) and Ba3MnNb2O9 (S = 3/2). At zero magnetic field, Ba3CoNb2O9 undergoes a two-step transition at 1.36 K and 1.10 K and enters a 120 degree ordered state. By applying magnetic fields, a series of magnetic phases with fractional saturation magnetization (1/3, 1/2, 2/3 (or √{ 3}/3Ms) are observed. The collinear spin phase with 1/3 Ms becomes more robust at lower temperatures due to quantum fluctuations. For Ba3MnNb2O9, the 120 degree ordered state is stabilized below 3.10 K at zero field. Under the magnetic field, successive magnetic phase transitions are observed with fractional magnetization 1/3 and 1/2 Ms. The 1/3 Ms phase becomes more stable at higher temperatures due to thermal fluctuations. The ferroelectricity emerges in all spin states in both compounds regardless of the spin chirality. Therefore, Ba3CoNb2O9andBa3MnNb2O9 are unique TLAFs exhibiting not only a series of magnetic phase transitions but also multiferroicity. NHMFL is supported by NSF, the State of Florida and US DOE. ORNL HFIR was sponsored by U.S. DOE.

  11. Improved Hard-Spin Mean-Field Approach for Frustrated XY Models

    Science.gov (United States)

    Behzadi, Azad E.; McKay, Susan R.

    1998-03-01

    We have modified the hard-spin mean-field approaches previously used on frustrated Ising(R.R. Netz and A.N. Berker, Phys. Rev. Lett. 66), 377 (1991). and XY (J.E. Tesiero, Physics M.S. thesis, U. of Maine (1995).) models to include self-consistent Gaussian fluctuations in the direction of each nearest-neighbor spin. This method, applied to the family of frustrated XY models on a square lattice with variable ratio of antiferromagnetic to ferromagnetic interaction strength, η, shows excellent agreement with Monte Carlo results on the same system(B. Berge et al., Phys. Rev. B 34), 3177 (1986).. For η=0.5 and 0.6, two specific heat peaks are clearly present, with the Ising transition occurring at lower temperature. The Ising transition is signaled by a nonzero chirality, while the Kosterlitz-Thouless (KT) transition shows nonzero helicity modulus and sublattice magnetizations. The specific heat shows a sharp, dominant peak at the Ising transition and a smaller, more rounded peak at the KT transition. For η=1.5, the specific heat has its most pronounced peak at T=0.45, the same location as the η=1 case, again in agreement with Monte Carlo simulations. Results presented are obtained from both the Monte Carlo implementation of this hard-spin mean-field approach and from solving the local magnetization equations self-consistently.

  12. Large anomalous Hall effect driven by a nonvanishing Berry curvature in the noncolinear antiferromagnet Mn3Ge.

    Science.gov (United States)

    Nayak, Ajaya K; Fischer, Julia Erika; Sun, Yan; Yan, Binghai; Karel, Julie; Komarek, Alexander C; Shekhar, Chandra; Kumar, Nitesh; Schnelle, Walter; Kübler, Jürgen; Felser, Claudia; Parkin, Stuart S P

    2016-04-01

    It is well established that the anomalous Hall effect displayed by a ferromagnet scales with its magnetization. Therefore, an antiferromagnet that has no net magnetization should exhibit no anomalous Hall effect. We show that the noncolinear triangular antiferromagnet Mn3Ge exhibits a large anomalous Hall effect comparable to that of ferromagnetic metals; the magnitude of the anomalous conductivity is ~500 (ohm·cm)(-1) at 2 K and ~50 (ohm·cm)(-1) at room temperature. The angular dependence of the anomalous Hall effect measurements confirms that the small residual in-plane magnetic moment has no role in the observed effect except to control the chirality of the spin triangular structure. Our theoretical calculations demonstrate that the large anomalous Hall effect in Mn3Ge originates from a nonvanishing Berry curvature that arises from the chiral spin structure, and that also results in a large spin Hall effect of 1100 (ħ/e) (ohm·cm)(-1), comparable to that of platinum. The present results pave the way toward the realization of room temperature antiferromagnetic spintronics and spin Hall effect-based data storage devices.

  13. Feedback control of noise in spin valves by the spin-transfer torque

    NARCIS (Netherlands)

    Bandopadyay, S.; Brataas, A.; Bauer, G.E.W.

    2011-01-01

    The miniaturization of magnetic read heads and random access memory elements makes them vulnerable to thermal fluctuations. We demonstrate how current-induced spin-transfer torques can be used to suppress the effects of thermal fluctuations. This enhances the fidelity of perpendicular magnetic spin

  14. Efficient density matrix renormalization group algorithm to study Y junctions with integer and half-integer spin

    KAUST Repository

    Kumar, Manoranjan

    2016-02-03

    An efficient density matrix renormalization group (DMRG) algorithm is presented and applied to Y junctions, systems with three arms of n sites that meet at a central site. The accuracy is comparable to DMRG of chains. As in chains, new sites are always bonded to the most recently added sites and the superblock Hamiltonian contains only new or once renormalized operators. Junctions of up to N=3n+1≈500 sites are studied with antiferromagnetic (AF) Heisenberg exchange J between nearest-neighbor spins S or electron transfer t between nearest neighbors in half-filled Hubbard models. Exchange or electron transfer is exclusively between sites in two sublattices with NA≠NB. The ground state (GS) and spin densities ρr=⟨Szr⟩ at site r are quite different for junctions with S=1/2, 1, 3/2, and 2. The GS has finite total spin SG=2S(S) for even (odd) N and for MG=SG in the SG spin manifold, ρr>0(<0) at sites of the larger (smaller) sublattice. S=1/2 junctions have delocalized states and decreasing spin densities with increasing N. S=1 junctions have four localized Sz=1/2 states at the end of each arm and centered on the junction, consistent with localized states in S=1 chains with finite Haldane gap. The GS of S=3/2 or 2 junctions of up to 500 spins is a spin density wave with increased amplitude at the ends of arms or near the junction. Quantum fluctuations completely suppress AF order in S=1/2 or 1 junctions, as well as in half-filled Hubbard junctions, but reduce rather than suppress AF order in S=3/2 or 2 junctions.

  15. Magnon condensation and spin superfluidity

    Science.gov (United States)

    Bunkov, Yury M.; Safonov, Vladimir L.

    2018-04-01

    We consider the Bose-Einstein condensation (BEC) of quasi-equilibrium magnons which leads to spin superfluidity, the coherent quantum transfer of magnetization in magnetic material. The critical conditions for excited magnon density in ferro- and antiferromagnets, bulk and thin films, are estimated and discussed. It was demonstrated that only the highly populated region of the spectrum is responsible for the emergence of any BEC. This finding substantially simplifies the BEC theoretical analysis and is surely to be used for simulations. It is shown that the conditions of magnon BEC in the perpendicular magnetized YIG thin film is fulfillied at small angle, when signals are treated as excited spin waves. We also predict that the magnon BEC should occur in the antiferromagnetic hematite at room temperature at much lower excited magnon density compared to that of ferromagnetic YIG. Bogoliubov's theory of Bose-Einstein condensate is generalized to the case of multi-particle interactions. The six-magnon repulsive interaction may be responsible for the BEC stability in ferro- and antiferromagnets where the four-magnon interaction is attractive.

  16. Orbital Contribution in 5f itinerant antiferromagnet UNiGa5 and UPtGa_5

    Science.gov (United States)

    Kaneko, Koji; Metoki, Naoto; Tokiwa, Yoshihumi; Haga, Yoshinori; Ishii, Yoshinobu; Bernhoeft, Nicholas; Lander, Gerard H.; O¯nuki, Yoshichika

    2003-03-01

    UNiGa5 and UPtGa5 which are isostructural to the heavy fermion superconductor PuCoGa5 exhibit itinerant antiferromagnetism with T_N=86 K and 26 K, respectively. Note that the nearest neighbor coupling of magnetic moments within the (0 0 1) plane is different between these iso-electronic compounds. In this work, the itinerant antiferromagnetism of UNiGa5 and UPtGa5 were studied in terms of magneto-striction and magnetic form factors. The neutron diffraction reveals the existence of remarkable magneto-strictions around T_N, indicating the large spin-orbit coupling in this system. The magnetic form factors of both compounds show that the orbital moments are quenched systematically corresponding to their behavior in the magnetic susceptibility. The result indicates the important role of orbital moment on the itinerancy of 5f electron in this system.

  17. The antiferromagnetic form factor of La2NiO4

    International Nuclear Information System (INIS)

    Wang, X.L.; Stassis, C.; Johnston, D.C.; Leung, T.C.; Ye, J.; Harmon, B.N.; Lander, G.H.; Schultz, A.J.; Loong, C.; Honig, J.M.

    1991-01-01

    Neutron-diffraction techniques have been used to study the antiferromagnetic form factor of a La 2 NiO 4 single crystal at 15 K. The antiferromagnetic form factor was obtained by measuring the integrated intensities of 16 magnetic reflections. A plateau is clearly seen at low Q (up to 3 A -1 ) in the experimentally determined form factor, similar to those observed for La 2 CuO 4 and Sr 2 CuO 2 Cl 2 . As in the case of these latter compounds, the fit of the experimental data by a Ni 2+ ionic form factor is not satisfactory. The experimental data are compared with a recent spin-polarized band calculation and with a covalency model

  18. Neutron experiments on antiferromagnetic nuclear order in silver at picokelvin temperatures

    DEFF Research Database (Denmark)

    Tuoriniemi, J.T.; Nummila, K.K.; Vuorinen, R.T.

    1995-01-01

    Spontaneous long-range nuclear antiferromagnetic order in the spin-1/2 system of silver nuclei was observed by neutron diffraction on a single crystal of Ag-109. A structure with the ordering vector k = (2 pi/a) (0,0,1) developed when the antiferromagnetic state was entered by adiabatic...... demagnetization along the [001] axis. No domains of the other two symmetry-equivalent k vectors, (2 pi/a) (0,1,0) and (2 pi/a) (1,0,0), formed during warmup in zero field. Nuclear susceptibility and entropy were found by neutron transmission. In B = 0, the critical entropy of ordering was S-c = (0.54 +/- 0.03)R...

  19. Magnetostriction and Magnetostructural Domains in Antiferromagnetic YBa2 Cu3 O6

    Science.gov (United States)

    Náfrádi, B.; Keller, T.; Hardy, F.; Meingast, C.; Erb, A.; Keimer, B.

    2016-01-01

    We use high-resolution neutron Larmor diffraction and capacitative dilatometry to investigate spontaneous and forced magnetostriction in undoped, antiferromagnetic YBa2 Cu3 O6.0 , the parent compound of a prominent family of high-temperature superconductors. Upon cooling below the Néel temperature TN=420 K , Larmor diffraction reveals the formation of magnetostructural domains of characteristic size ˜240 nm . In the antiferromagnetic state, dilatometry reveals a minute (4 ×10-6) orthorhombic distortion of the crystal lattice in external magnetic fields. We attribute these observations to exchange striction and spin-orbit coupling induced magnetostriction, respectively, and show that they have an important influence on the thermal and charge transport properties of undoped and lightly doped cuprates.

  20. Tunnelling anisotropic magnetoresistance due to antiferromagnetic CoO tunnel barriers

    Science.gov (United States)

    Wang, K.; Sanderink, J. G. M.; Bolhuis, T.; van der Wiel, W. G.; de Jong, M. P.

    2015-01-01

    A new approach in spintronics is based on spin-polarized charge transport phenomena governed by antiferromagnetic (AFM) materials. Recent studies have demonstrated the feasibility of this approach for AFM metals and semiconductors. We report tunneling anisotropic magnetoresistance (TAMR) due to the rotation of antiferromagnetic moments of an insulating CoO layer, incorporated into a tunnel junction consisting of sapphire(substrate)/fcc-Co/CoO/AlOx/Al. The ferromagnetic Co layer is exchange coupled to the AFM CoO layer and drives rotation of the AFM moments in an external magnetic field. The results may help pave the way towards the development of spintronic devices based on AFM insulators. PMID:26486931

  1. Correlated electric-field induced reversal of antiferromagnetic order and surface magnetization in magnetoelectric Cr2O3

    Science.gov (United States)

    Wang, Junlei; Singh, Uday; Binek, Christian

    The electric-field-induced Faraday effect in magnetoelectrics comprises a superimposition of linear electric field responses with temperature dependencies of the linear magnetoelectric susceptibility and the antiferromagnetic order parameter. The tunability of the relative strength between the two contributions leads to a table-top set-up allowing to measure voltage-controlled selection and temperature dependence of the antiferromagnetic order parameter. Simultaneous measurement of the polar Kerr effect and the electric-field-induced Faraday effect is utilized to investigate correlated formation and switching of the surface magnetization and bulk antiferromagnetic order in Cr2O3 The correlated reversal of surface or boundary magnetization in response to voltage-controlled reversal of the bulk antiferromagnetic order parameter is of key importance for applications in spintronic devices such as the magnetoelectric MRAM. The Faraday rotation per applied voltage is independent of the sample thickness making the method scalable and versatile for thin film investigations. Scalability, compactness, and simplicity of the data analysis combined with low photon flux requirements make the Faraday approach advantageous for the investigation of the otherwise difficult to access voltage-controlled switching of antiferromagnetic domain states in magnetoelectric thin films. Acknowledgment: This project was supported by SRC through CNFD, an SRC-NRI Center, by C-SPIN, part of STARnet, and by the NSF through MRSEC DMR-0820521.

  2. Anisotropy modulated stepwise magnetization in triangular Heisenberg antiferromagnet

    International Nuclear Information System (INIS)

    Yao Xiaoyan; Liu Junming; Lo, Veng Cheong

    2011-01-01

    During the course of tuning anisotropy from Ising type to zero, the variation of magnetization (M) steps against magnetic field (h) is investigated in a triangular antiferromagnetic Heisenberg model using Monte Carlo techniques. It is revealed that the anisotropy is an essential key to induce the temperature-dependent stepwise M(h) curve observed in frustrated magnetic system, and it can be employed to modulate this steplike magnetic behavior effectively. When the anisotropy is strengthened, a ground state transition occurs from the homogeneous 120 o triangular structure to the collinear partially disordered antiferromagnetic state. No M step is detected in the system without anisotropy. But if the anisotropy is nonzero, the M 0 /3 step (where M 0 is the saturated M) will emerge on M(h) curve, which is due to an h-induced quasi-collinear ferrimagnetic state. This M 0 /3 step can be extended by increasing the anisotropy. When the M 0 /3 plateau dominates the h-range broad enough, the equidistant metastable substeps, which originates from the disorders frozen in the frustrated collinear spin structure, appear to be superposed on the M 0 /3 plateau. Thus the system with a strong anisotropy presents the whole temperature evolution of stepwise M(h) curve in quantitative agreement with the experiments of Ca 3 Co 2 O 6 . - Highlights: → Variation of M steps is investigated by tuning anisotropy from Ising type to zero. → Anisotropy is essential to induce T-dependent multistep M against magnetic field. → Simulation with strong anisotropy reproduces T-evolution of M steps in Ca 3 Co 2 O 6 . → Metastable substeps at low T can be enhanced by increasing anisotropy.

  3. Antiferromagnetic noise correlations in optical lattices

    DEFF Research Database (Denmark)

    Bruun, Niels Bohr International Academy, University of Copenhagen, DK-2100 Copenhagen Ø, Denmark, Georg Morten; Syljuåsen, F. T.; Pedersen, K. G. L.

    2009-01-01

    We analyze how noise correlations probed by time-of-flight experiments reveal antiferromagnetic (AF) correlations of fermionic atoms in two-dimensional and three-dimensional optical lattices. Combining analytical and quantum Monte Carlo calculations using experimentally realistic parameters, we s...

  4. Antiferromagnetism in chromium alloy single crystals

    DEFF Research Database (Denmark)

    Bjerrum Møller, Hans; Trego, A.L.; Mackintosh, A.R.

    1965-01-01

    The antiferromagnetism of single crystals of dilute alloys of V, Mn and Re in Cr has been studied at 95°K and 300°K by neutron diffraction. The addition of V causes the diffraction peaks to decrease in intensity and move away from (100), while Mn and Re cause them to increase and approach (100) s...

  5. Low temperature properties of the triangular-lattice antiferromagnet: a bosonic spinon theory

    International Nuclear Information System (INIS)

    Mezio, A; Manuel, L O; Trumper, A E; Singh, R R P

    2012-01-01

    We study the low temperature properties of the triangular-lattice Heisenberg antiferromagnet with a mean field Schwinger spin- 1/2 boson scheme that reproduces quantitatively the zero temperature energy spectrum derived previously using series expansions. By analyzing the spin–spin and the boson density–density dynamical structure factors, we identify the unphysical spin excitations that come from the relaxation of the local constraint on bosons. This allows us to reconstruct a free energy based on the physical excitations only, whose predictions for entropy and uniform susceptibility seem to be reliable within the temperature range 0 ⩽ T ≲ 0.3J, which is difficult to access by other methods. The high values of entropy, also found in high temperature expansion studies, can be attributed to the roton-like narrowed dispersion at finite temperatures. (paper)

  6. The phase diagrams and the order parameters of the diluted transverse superlattice with antiferromagnetic interface coupling

    International Nuclear Information System (INIS)

    Oubelkacem, A.; El Aouad, N.; Benaboud, A.; Saber, M.

    2004-01-01

    Using the effective field theory with a probability distribution technique that accounts for the self-spin correlation functions, the magnetic properties of the Ising superlattice consisting of two ferromagnetic materials A and B, with L a layers of diluted spins S a =((1)/(2)) and L b layers of diluted spins S b =1 in an applied transverse field Ω with antiferromagnetic interface coupling are examined. For fixed values of the reduced exchange interactions and the concentration c of magnetic atoms, the phase diagrams and the total magnetization for the superlattice are studied as a function of the transverse field and the temperature. We find a number of characteristic phenomena. In particular, the effect of the concentration c of magnetic atoms, the interlayer coupling and the transverse field on both the compensation temperature and the magnetization profiles are clarified. Some of them may be related to the experimental works of rare-earth (RE)/transition metal (TM) multilayer films

  7. Enhanced exchange bias fields for CoO/Co bilayers: influence of antiferromagnetic grains and mechanisms

    Energy Technology Data Exchange (ETDEWEB)

    Chang, Cheng-Hsun-Tony; Chang, Shin-Chen [Department of Physics, National Taiwan Normal University, Taipei 116, Taiwan (China); Tsay, Jyh-Shen, E-mail: jstsay@phy.ntnu.edu.tw [Department of Physics, National Taiwan Normal University, Taipei 116, Taiwan (China); Yao, Yeong-Der [Institute of Physics, Academia Sinica, Nankang, Taipei 11529, Taiwan (China)

    2017-05-31

    Highlights: • An antiferromagnetic grain model on exchange bias phenomena is proposed. • Grain size and grain density are considered. • For smaller grain size, the dependence of t{sub CoO} on T{sub B} showed a less pronounced variation. • An increased grain density is responsible for the enhancement in the exchange bias fields. - Abstract: The emergence and optimization of devices that can be applied to spintronics have attracted considerable interest, and both experimental and theoretical approaches have been used in studies of exchange bias phenomena. A survey of the literature indicates that great efforts have been devoted to improving exchange bias fields, while only limited attempts have been made to control the temperature dependence of exchange bias. In this study, the influence of antiferromagnetic grains on exchange bias phenomena in CoO/Co bilayers on a semiconductor surface was investigated. Based on an antiferromagnetic grain model, a correlation between grain size, grain density, blocking temperature, and the exchange bias field was established. For crystallites with a smaller median diameter, the dependence of the thickness of the CoO layer on blocking temperature showed a less pronounced variation. This is due to the larger thermal agitation of the atomic spin moments in the grain, which causes a weaker exchange coupling between atomic spin moments. The enhanced density of antiferromagnetic/ferromagnetic pinning sites resulting from an increased grain density is responsible for the enhancement in the exchange bias fields. The results reported herein provide insights into our knowledge related to controlling the temperature dependence of exchange bias and related mechanisms.

  8. Superconductivity in the background of disordered flux state of spins

    International Nuclear Information System (INIS)

    Feng Shiping; Guo Rui; Han Fei

    1992-01-01

    The phase diagram of the copper oxide materials with the antiferromagnetic and the superconducting properties as a function of doping δ is obtained in the framework of the t-J model by using the Schwinger boson-slave fermion theory. The results show that the spiral order of spins competes and coexists with superconductivity for small doping δ. For large doping δ, superconductivity appears, which may be caused by the occurrence of a disordered flux state of spins. The phase diagram suggests a strong relationship between antiferromagnetism and superconductivity. (orig.)

  9. Spin-orbit mediated control of spin qubits

    DEFF Research Database (Denmark)

    Flindt, Christian; Sørensen, A.S; Flensberg, Karsten

    2006-01-01

    We propose to use the spin-orbit interaction as a means to control electron spins in quantum dots, enabling both single-qubit and two-qubit operations. Very fast single-qubit operations may be achieved by temporarily displacing the electrons. For two-qubit operations the coupling mechanism is based...... on a combination of the spin-orbit coupling and the mutual long-ranged Coulomb interaction. Compared to existing schemes using the exchange coupling, the spin-orbit induced coupling is less sensitive to random electrical fluctuations in the electrodes defining the quantum dots....

  10. Na4Ir3O8 as a 3D spin liquid with fermionic spinons.

    Science.gov (United States)

    Zhou, Yi; Lee, Patrick A; Ng, Tai-Kai; Zhang, Fu-Chun

    2008-11-07

    Spin liquid states for the spin-1/2 antiferromagnetic Heisenberg model on a hyperkagome lattice are studied. We classify and study flux states according to symmetries. Applying this model to Na4Ir3O8, we propose that the high temperature state may be described by a spinon Fermi surface, which forms a paired state with line nodes below 20 K. The possible mixed spin singlet and spin triplet pairing states are discussed according to the lattice symmetry which breaks inversion.

  11. Interlayer coupling between out-of-plane magnetized multilayers across a thin antiferromagnetic spacer

    Energy Technology Data Exchange (ETDEWEB)

    Moritz, J., E-mail: jerome.moritz@cea.fr [SPINTEC, UMR CEA/CNRS/UJF/Grenoble-INP, Grenoble (France); Bacher, P. [LEMTA, UMR CNRS-INPL-UHP, ESSTIN, 2, rue Jean Lamour, Vandoeuvre Les Nancy Cedex F-54519 (France); Auffret, S.; Dieny, B. [SPINTEC, UMR CEA/CNRS/UJF/Grenoble-INP, Grenoble (France)

    2011-10-15

    The interlayer exchange coupling between Co/Pt perpendicular-to-plane magnetized layers across a thin IrMn spacer layer was experimentally studied. In contrast to earlier studies on interlayer coupling through antiferromagnetic NiO, which revealed an oscillatory coupling behavior as a function of NiO thickness, a ferromagnetic coupling was observed here in the range of IrMn thickness between 0.6 and 1.5 nm and antiferromagnetic between 1.5 and 2.5 nm. The antiferromagnetic coupling is attributed to an orange peel magnetostatic mechanism whereas the ferromagnetic coupling is attributed to an out-of-plane polarization of the antiferromagnetic IrMn layer induced by the interfacial exchange interaction with the adjacent out-of-plane ferromagnetic layers. Measurements of hysteresis loops versus temperature show that the coupling vanishes at 510 K for t{sub IrMn}=1 nm. This critical temperature is far below the Neel temperature of bulk IrMn, but above the blocking temperature of IrMn/Co bilayers at such thickness. Using a one-dimensional model describing a partial domain wall in the antiferromagnet, we explain the coupling in terms of an out-of-plane tilt of the Mn moments at the IrMn/(Co/Pt) interfaces yielding a weak net polarization of the IrMn. Finally, the non-oscillatory decay of the coupling was attributed to the compensated spin structure of the IrMn in the parallel to the interfaces. - Highlights: > Interlayer coupling between Pt/Co multilayer separated by thin IrMn film is studied. > Coupling is ferromagnetic at low thickness of IrMn (between 0.6 and 1.2 nm). > Coupling vanishes between the blocking and the Neel temperature of IrMn. > We model the coupling by considering a tilt of the interfacial IrMn spins. > Non-oscillatory coupling is attributed to the compensated spin structure of IrMn.

  12. Magnetism, chemical bonding and hyperfine properties in the nanoscale antiferromagnet [Fe(O Me)2(O2 C C H2 Cl)]10

    International Nuclear Information System (INIS)

    Zeng, Z.; Duan, Y.; Guenzburger, Diana

    1996-09-01

    The electronic and magnetic properties of the nanometer-size antiferromagnet (the ferric wheel molecule) are investigated with the first-principles spin-polarized Discrete Variational Method, in the framework of Density Functional theory. Magnetic moments, densities of the states and charge and spin-density maps are obtained. The Moessbauer hyperfine parameters Isomer shift, Quadrupole Splitting and Hyperfine Field are obtained from the calculations and compared to reported experimental values when available. (author). 33 refs., 8 figs., 4 tabs

  13. Spin noise spectroscopy beyond thermal equilibrium and linear response.

    Science.gov (United States)

    Glasenapp, P; Sinitsyn, N A; Yang, Luyi; Rickel, D G; Roy, D; Greilich, A; Bayer, M; Crooker, S A

    2014-10-10

    Per the fluctuation-dissipation theorem, the information obtained from spin fluctuation studies in thermal equilibrium is necessarily constrained by the system's linear response functions. However, by including weak radio frequency magnetic fields, we demonstrate that intrinsic and random spin fluctuations even in strictly unpolarized ensembles can reveal underlying patterns of correlation and coupling beyond linear response, and can be used to study nonequilibrium and even multiphoton coherent spin phenomena. We demonstrate this capability in a classical vapor of (41)K alkali atoms, where spin fluctuations alone directly reveal Rabi splittings, the formation of Mollow triplets and Autler-Townes doublets, ac Zeeman shifts, and even nonlinear multiphoton coherences.

  14. [mu]SR magnetic response in frustrated antiferromagnets of type RMn[sub 2] (R = rare earth)

    Energy Technology Data Exchange (ETDEWEB)

    Weber, M. (Physics Dept., TU Munich, Garching (Germany)); Asch, L. (Physics Dept., TU Munich, Garching (Germany)); Kratzer, A. (Physics Dept., TU Munich, Garching (Germany)); Kalvius, G.M. (Physics Dept., TU Munich, Garching (Germany)); Muench, K.H. (Physics Dept., TU Munich, Garching (Germany)); Ballou, R. (Lab. Louis Neel, CNRS, 38 Grenoble (France)); Deportes, J. (Lab. Louis Neel, CNRS, 38 Grenoble (France)); Waeppling, R. (Dept. of Physics, Univ. of Uppsala (Sweden)); Litterst, F.J. (Inst. for Metal Physics, TU Braunschweig (Germany)); Klauss, H.H. (Inst. for Metal Physics, TU Braunschweig (Germany)); Niedermayer, C. (Faculty for Physics, Univ. Konstanz (Germany)); Chappert, J. (CEA/DRFMC, CEN Grenoble, 38 (France))

    1994-07-01

    Zero, longitudinal and transverse field [mu]SR was carried out in the antiferromagnets YMn[sub 2], Y[sub 0.95] Tb[sub 0.15] Mn[sub 2], Y[sub 0.9]Tb[sub 0.1]Mn[sub 2], Y[sub 0.99] Sc[sub 0.01] Mn[sub 2], Y[sub 0.98]Sc[sub 0.02]Mn[sub 2] and TbMn[sub 2]. The dynamics of Mn magnetic moments above T[sub N] is typical for an itinerant antiferromagnet. Within a certain temperature range above T[sub N] part of the material enters a randomly ordered (spin glass like) magnetic state as an out-come of frustration. At temperatures above [approx] 150 K the muon spin relaxation rate indicates that the muon has become mobile. (orig.)

  15. Ferromagnetic nature in low-dimensional S = 1 antiferromagnetic Li2Ni(WO4)2 nanoparticles

    Science.gov (United States)

    Panneer Muthuselvam, I.; Sankar, R.; Narsinga Rao, G.; Karna, Sunil K.; Chou, F. C.

    2018-03-01

    We report the magnetic behaviour of ball-milled nanoparticles of antiferromagnetic spin-1 Li2Ni(WO4)2 system by magnetic susceptibility and neutron diffraction measurements. Bulk sample shows indicators of two successive three dimensional (3D) antiferromagnetic (AF) ordering at TN1 ∼ 18K and TN2 ∼ 13K in χ (T). The magnetic susceptibility and neutron diffraction measurements indicate that no long-range magnetic order is detected when bulk sample is reduced to nano size particles, despite of the identical crystal structures. The super-super exchange interaction is proposed being disrupted as a result of cell volume expansion in nanoparticles. The Zero-Field-Cooled (ZFC) and Field-Cooled (FC) curve bifurcation and M(H) curve of nanoparticle reveal that the weak ferromagnetic behavior exists at low temperature because of spin disorder on the surface of nanoparticle.

  16. Er2Ti2O7: Evidence of quantum order by disorder in a frustrated antiferromagnet

    DEFF Research Database (Denmark)

    Champion, J.D.M.; Harris, M.J.; Holdsworth, P.C.W.

    2003-01-01

    Er(2)Ti(2)O(7) has been suggested to be a realization of the frustrated XY pyrochlore lattice antiferromagnet, for which theory predicts fluctuation-induced symmetry breaking in a highly degenerate ground state manifold. We present a theoretical analysis of the classical model compared...

  17. Antiferromagnetic bipolar semiconductor LaMnPO with ZrCuSiAs-type structure

    Science.gov (United States)

    Yanagi, Hiroshi; Watanabe, Takumi; Kodama, Katsuaki; Iikubo, Satoshi; Shamoto, Shin-ichi; Kamiya, Toshio; Hirano, Masahiro; Hosono, Hideo

    2009-05-01

    Electronic and magnetic properties of a layered compound LaMnPO are examined in relation to a newly discovered iso-structural superconductor LaFeAs(P)O. Neutron diffraction measurements, together with temperature dependent magnetic susceptibility, clarify that LaMnPO is an antiferromagnet at least up to 375 K. The spin moment of a Mn ion is determined to be 2.26 μB at room temperature, and the spin configuration is antiparallel in the Mn-P plane and parallel between the Mn-P planes, which is rather different from that of LaFeAsO. Optical absorption spectra, photoemission spectra, and temperature dependent electrical conductivity indicate that LaMnPO is a semiconductor. Furthermore, nominally undoped LaMnPO exhibits n-type conduction while the conduction type is changed by doping of Cu or Ca to the La sites, indicating that LaMnPO is a bipolar conductor. Density functional calculation using the GGA+U approximation supports the above conclusions; the electronic band structure has an open band gap and the antiferromagnetic spin configuration is more stable than the ferromagnetic one.

  18. Strongly Coupled Systems: From Quantum Antiferromagnets To Unified Models For Superconductors

    CERN Document Server

    Chudnovsky, V

    2002-01-01

    I discuss the significance of the antiferromagnetic Heisenberg model (AFHM) in both high-energy and condensed-matter physics, and proceed to describe an efficient cluster algorithm used to simulate the AFHM. This is one of two algorithms with which my collaborators and I were able to obtain numerical results that definitively confirm that chiral perturbation theory, corrected for cutoff effects in the AFHM, leads to a correct field-theoretical description of the low- temperature behavior of the spin correlation length in various spin representations S. Using a finite-size-scaling technique, we explored correlation lengths of up to 105 lattice spacings for spins S = 1 and 5/2. We show how the recent prediction of cutoff effects by P. Hasenfratz is approached for moderate correlation lengths, and smoothly connects with other approaches to modeling the AFHM at smaller correlation lengths. I also simulate and discuss classical antiferromagnetic systems with simultaneous SO(M) and SO( N) symmetries, which have bee...

  19. Strongly Coupled Systems From Quantum Antiferromagnets To Unified Models For Superconductors

    CERN Document Server

    Chudnovsky, V

    2002-01-01

    I discuss the significance of the antiferromagnetic Heisenberg model (AFHM) in both high-energy and condensed-matter physics, and proceed to describe an efficient cluster algorithm used to simulate the AFHM. This is one of two algorithms with which my collaborators and I were able to obtain numerical results that definitively confirm that chiral perturbation theory, corrected for cutoff effects in the AFHM, leads to a correct field-theoretical description of the low- temperature behavior of the spin correlation length in various spin representations S. Using a finite-size-scaling technique, we explored correlation lengths of up to 105 lattice spacings for spins S = 1 and 5/2. We show how the recent prediction of cutoff effects by P. Hasenfratz is approached for moderate correlation lengths, and smoothly connects with other approaches to modeling the AFHM at smaller correlation lengths. I also simulate and discuss classical antiferromagnetic systems with simultaneous SO(M) and SO( N) symmetries, which have bee...

  20. Fluctuation analysis

    International Nuclear Information System (INIS)

    Clarke, J.

    1980-01-01

    This paper briefly reviews sources of noise in Josephson junctions, and the limits they impose on the sensitivity of dc and rf SQUIDS. The results are strictly valid only for a resistively shunted junction (RSJ) with zero capacitance, but should be applicable to point contact junctions and microbridges in so far as these devices can be approximated by the RSJ model. Fluctuations arising from Nyquist noise in the resistive shunt of a single junction are discussed in the limit eI/sub o/R/k/sub B/T << 1 in which a classical treatment is appropriate, and then extend the treatment to the limit eI/sub o/R/k/sub B/T greater than or equal to 1 in which quantum effects become important. The Nyquist limit theory is used to calculate the noise in a dc SQUID, and the results are compared with a number of practical devices. The quantum limit is briefly considered. Results for the predicted sensitivity of rf SQUIDS are presented, and also compared with a number of practical devices. Finally, the importance of l/f noise (f is the frequency) in limiting the low frequency performance of SQUIDS is discussed

  1. Magnons versus free spinons in finite quantum frustrated antiferromagnets

    Energy Technology Data Exchange (ETDEWEB)

    Hamad, I.J.; Manuel, L.O. [Instituto de Fisica Rosario (CONICET) and Universidad Nacional de Rosario, Boulevard 27 de Febrero 210 bis, 2000 Rosario (Argentina); Trumper, A.E., E-mail: trumper@ifir-conicet.gov.a [Instituto de Fisica Rosario (CONICET) and Universidad Nacional de Rosario, Boulevard 27 de Febrero 210 bis, 2000 Rosario (Argentina)

    2009-10-01

    We have investigated the validity of doping with a vacancy the J{sub 1}-J{sub 3} frustrated Heisenberg model on a finite square lattice as a way to test the existence of fractional spin excitations. Using a generalized t-J{sub 1}-J{sub 3} model we have computed the vacancy spectral functions in the self-consistent Born approximation. We have found that by including spiral fluctuations in the magnetic ground state, the spectral functions on finite systems agree very well with the unbiased exact ones. In contrast to the recent proposal that the quasiparticle weight reduction could be a signal of a spinon free excitation in finite systems, we have found strong evidence that such a reduction is due to the existence of spiral fluctuations.

  2. Magnons versus free spinons in finite quantum frustrated antiferromagnets

    International Nuclear Information System (INIS)

    Hamad, I.J.; Manuel, L.O.; Trumper, A.E.

    2009-01-01

    We have investigated the validity of doping with a vacancy the J 1 -J 3 frustrated Heisenberg model on a finite square lattice as a way to test the existence of fractional spin excitations. Using a generalized t-J 1 -J 3 model we have computed the vacancy spectral functions in the self-consistent Born approximation. We have found that by including spiral fluctuations in the magnetic ground state, the spectral functions on finite systems agree very well with the unbiased exact ones. In contrast to the recent proposal that the quasiparticle weight reduction could be a signal of a spinon free excitation in finite systems, we have found strong evidence that such a reduction is due to the existence of spiral fluctuations.

  3. Magnons versus free spinons in finite quantum frustrated antiferromagnets

    Science.gov (United States)

    Hamad, I. J.; Manuel, L. O.; Trumper, A. E.

    2009-10-01

    We have investigated the validity of doping with a vacancy the J1-J3 frustrated Heisenberg model on a finite square lattice as a way to test the existence of fractional spin excitations. Using a generalized t-J1-J3 model we have computed the vacancy spectral functions in the self-consistent Born approximation. We have found that by including spiral fluctuations in the magnetic ground state, the spectral functions on finite systems agree very well with the unbiased exact ones. In contrast to the recent proposal that the quasiparticle weight reduction could be a signal of a spinon free excitation in finite systems, we have found strong evidence that such a reduction is due to the existence of spiral fluctuations.

  4. Oxygen-induced immediate onset of the antiferromagnetic stacking in thin Cr films on Fe(001)

    Energy Technology Data Exchange (ETDEWEB)

    Berti, Giulia, E-mail: giulia.berti@polimi.it; Brambilla, Alberto; Calloni, Alberto; Bussetti, Gianlorenzo; Finazzi, Marco; Duò, Lamberto; Ciccacci, Franco [Dipartimento di Fisica, Politecnico di Milano, Piazza Leonardo da Vinci 32, I-20133 Milano (Italy)

    2015-04-20

    We investigated the magnetic coupling of ultra-thin Cr films grown at 600 K on a Fe(001)-p(1 × 1)O substrate by means of spin-polarized photoemission spectroscopy. Our findings show that the expected antiferromagnetic stacking of the magnetization in Cr(001) layers occurs right from the first atomic layer at the Cr/Fe interface. This is at variance with all previous observations in similar systems, prepared in oxygen-free conditions, which always reported on a delayed onset of the magnetic oscillations due to the occurrence of significant chemical alloying at the interface, which is substantially absent in our preparation.

  5. Magnetic study of a few antiferromagnets in very-strong pulsed fields (450 kOE)

    International Nuclear Information System (INIS)

    Krebs, J.

    1968-01-01

    In this thesis we describe a pulsed field device with which we obtain magnetization curves up to 450 kOE at all temperatures between 1. 6 and 300. We have studied the 'spin-flopping'(and therefore the anisotropy) in MnF 2 versus temperature, below the Neel point. We have also studied the antiferromagnets MnSO 4 . and MnSO 4 .H 2 O which have revealed saturation fields respectively of 250 kOE and 320 kOE. (author) [fr

  6. Optimized RVB states of the 2-d antiferromagnet: ground state and excitation spectrum

    Science.gov (United States)

    Chen, Yong-Cong; Xiu, Kai

    1993-10-01

    The Gutzwiller projection of the Schwinger-boson mean-field solution of the 2-d spin- {1}/{2} antiferromagnet in a square lattice is shown to produce the optimized, parameter-free RVB ground state. We get -0.6688 J/site and 0.311 for the energy and the staggered magnetization. The spectrum of the excited states is found to be linear and gapless near k≅0. Our calculation suggests, upon breaking of the rotational symmetry, ɛ k≅2JZ r1-γ 2k with Zr≅1.23.

  7. Emergent Power-Law Phase in the 2D Heisenberg Windmill Antiferromagnet: A Computational Experiment

    Science.gov (United States)

    Jeevanesan, Bhilahari; Chandra, Premala; Coleman, Piers; Orth, Peter P.

    2015-10-01

    In an extensive computational experiment, we test Polyakov's conjecture that under certain circumstances an isotropic Heisenberg model can develop algebraic spin correlations. We demonstrate the emergence of a multispin U(1) order parameter in a Heisenberg antiferromagnet on interpenetrating honeycomb and triangular lattices. The correlations of this relative phase angle are observed to decay algebraically at intermediate temperatures in an extended critical phase. Using finite-size scaling we show that both phase transitions are of the Berezinskii-Kosterlitz-Thouless type, and at lower temperatures we find long-range Z6 order.

  8. Renormalization-group studies of antiferromagnetic chains. I. Nearest-neighbor interactions

    International Nuclear Information System (INIS)

    Rabin, J.M.

    1980-01-01

    The real-space renormalization-group method introduced by workers at the Stanford Linear Accelerator Center (SLAC) is used to study one-dimensional antiferromagnetic chains at zero temperature. Calculations using three-site blocks (for the Heisenberg-Ising model) and two-site blocks (for the isotropic Heisenberg model) are compared with exact results. In connection with the two-site calculation a duality transformation is introduced under which the isotropic Heisenberg model is self-dual. Such duality transformations can be defined for models other than those considered here, and may be useful in various block-spin calculations

  9. Inducing spin-dependent tunneling to probe magnetic correlations in optical lattices

    DEFF Research Database (Denmark)

    Pedersen, Kim Georg Lind; Andersen, Brian Møller; Bruun, Georg Morten

    2012-01-01

    We suggest a simple experimental method for probing antiferromagnetic spin correlations of two-component Fermi gases in optical lattices. The method relies on a spin selective Raman transition to excite atoms of one spin species to their first excited vibrational mode where the tunneling is large....... The resulting difference in the tunneling dynamics of the two spin species can then be exploited, to reveal the spin correlations by measuring the number of doubly occupied lattice sites at a later time. We perform quantum Monte Carlo simulations of the spin system and solve the optical lattice dynamics...... numerically to show how the timed probe can be used to identify antiferromagnetic spin correlations in optical lattices....

  10. Dimensional Reduction in Quantum Dipolar Antiferromagnets

    Science.gov (United States)

    Babkevich, P.; Jeong, M.; Matsumoto, Y.; Kovacevic, I.; Finco, A.; Toft-Petersen, R.; Ritter, C.; Mânsson, M.; Nakatsuji, S.; Rønnow, H. M.

    2016-05-01

    We report ac susceptibility, specific heat, and neutron scattering measurements on a dipolar-coupled antiferromagnet LiYbF4 . For the thermal transition, the order-parameter critical exponent is found to be 0.20(1) and the specific-heat critical exponent -0.25 (1 ) . The exponents agree with the 2D X Y /h4 universality class despite the lack of apparent two-dimensionality in the structure. The order-parameter exponent for the quantum phase transitions is found to be 0.35(1) corresponding to (2 +1 )D . These results are in line with those found for LiErF4 which has the same crystal structure, but largely different TN, crystal field environment and hyperfine interactions. Our results therefore experimentally establish that the dimensional reduction is universal to quantum dipolar antiferromagnets on a distorted diamond lattice.

  11. Antiferromagnetic exchange mechanism of superconductivity in cuprates

    CERN Document Server

    Plakida, N M

    2001-01-01

    One examines theory of superconducting coupling resulted from antiferromagnetic exchange in terms of which one explains strong dependence of T sub c superconducting transition temperature on alpha lattice constant. Calculations are based on the Hubbard p-d two-region model within strong correlation limit. DELTA pd excitation high energy at antiferromagnetic exchange of two particles from different Hubbard subregions results in suppression o delay effects and in coupling of all particles in conductivity subregion with Fermi energy E sub F >= DELTA pd : T sub c approx = E sub F exp(-1/lambda), where lambda propor to J. T sub c (alpha) and isotopic effect are explained by J exchange interaction dependence on alpha and on zero oscillations of oxygen ions

  12. Magnetic behaviour of interacting antiferromagnetic nanoparticles

    International Nuclear Information System (INIS)

    Markovich, V; Jung, G; Gorodetsky, G; Puzniak, R; Wisniewski, A; Skourski, Y; Mogilyanski, D

    2012-01-01

    Magnetic properties of interacting La 0.2 Ca 0.8 MnO 3 nanoparticles have been investigated. The field-induced transition from antiferromagnetic (AFM) to ferromagnetic (FM) state in the La 0.2 Ca 0.8 MnO 3 bulk has been observed at exceptionally high magnetic fields. For large particles, the field-induced transition widens while magnetization progressively decreases. In small particles the transition is almost fully suppressed. The thermoremanence and isothermoremanence curves constitute fingerprints of irreversible magnetization originating from nanoparticle shells. We have ascribed the magnetic behaviour of nanoparticles to a core-shell scenario with two main magnetic contributions; one attributed to the formation of a collective state formed by FM clusters in frustrated coordination at the surfaces of interacting AFM nanoparticles and the other associated with inner core behaviour as a two-dimensional diluted antiferromagnet. (paper)

  13. Scaling of magnetic fluctuations near a quantum phase transition

    DEFF Research Database (Denmark)

    Schröder, A.; Aeppli, G.; Bucher, E.

    1998-01-01

    We use inelastic neutron scattering to measure the magnetic fluctuations in a single crystal of the heavy fermion alloy CeCu5.9Au0.1 close to the antiferromagnetic quantum critical point. The energy (E), wave vector (Q), and temperature (T) dependent spectra obey E/T scaling at Q near (1...... and the thermodynamics can be understood in terms of a quantum Lifshitz point....

  14. Magnetic Properties of Nanoparticles of Antiferromagnetic Materials

    DEFF Research Database (Denmark)

    Mørup, Steen; Frandsen, Cathrine; Bødker, Franz

    2003-01-01

    The magnetic properties of antiferromagnetic nanoparticles have been studied by Mossbauer spectroscopy and neutron scattering. Temperature series of Mossbauer spectra of non-interacting, superparamagnetic hematite nanoparticles were fitted by use of the Blume-Tjon relaxation model. It has been...... found that the magnetic anisotropy energy constant increases significantly with decreasing particle size. Neutron scattering experiments on similar samples give new information on both superparamagnetic relaxation and collective magnetic excitations. There is good agreement between the values...

  15. Electron spin resonance insight into broadband absorption of the Cu3Bi(SeO32O2Br metamagnet

    Directory of Open Access Journals (Sweden)

    A. Zorko

    2016-05-01

    Full Text Available Metamagnets, which exhibit a transition from a low-magnetization to a high-magnetization state induced by the applied magnetic field, have recently been highlighted as promising materials for controllable broadband absorption. Here we show results of a multifrequency electron spin resonance (ESR investigation of the Cu3Bi(SeO32O2Br planar metamagnet on the kagome lattice. Its mixed antiferromagnetic/ferromagnetic phase is stabilized in a finite range of applied fields around 0.8 T at low temperatures and is characterized by enhanced microwave absorption. The absorption signal is non-resonant and its boundaries correspond to two critical fields that determine the mixed phase. With decreasing temperature these increase like the sublattice magnetization of the antiferromagnetic phase and show no frequency dependence between 100 and 480 GHz. On the contrary, we find that the critical fields depend on the magnetic-field sweeping direction. In particular, the higher critical field, which corresponds to the transition from the mixed to the ferromagnetic phase, shows a pronounced hysteresis effect, while such a hysteresis is absent for the lower critical field. The observed hysteresis is enhanced at lower temperatures, which suggests that thermal fluctuations play an important role in destabilizing the highly absorbing mixed phase.

  16. Frustrated antiferromagnets at high fields: Bose-Einstein condensation in degenerate spectra

    International Nuclear Information System (INIS)

    Jackeli, G.; Zhitomirsky, M.E.

    2004-01-01

    Quantum phase transition at the saturation field is studied for a class of frustrated quantum antiferromagnets. The considered models include (i) the J 1 -J 2 frustrated square-lattice antiferromagnet with J 2 =(1/2)J 1 and (ii) the nearest-neighbor Heisenberg antiferromagnet on a face centered cubic lattice. In the fully saturated phase the magnon spectra for the two models have lines of degenerate minima. Transition into a partially magnetized state is treated via a mapping to a dilute gas of hard-core bosons and by complementary spin-wave calculations. Momentum dependence of the exact four-point boson vertex removes the degeneracy of the single-particle excitation spectra and selects the ordering wave vectors at (π,π) and (π,0,0) for the two models. We predict a unique form for the magnetization curve ΔM=S-M≅μ (d-1)/2 (logμ) (d-1) , where μ is a distance from the quantum critical point

  17. Quantum spin dynamics in molecular magnets

    International Nuclear Information System (INIS)

    Leuenberger, M.N.; Meier, F.; Loss, D.

    2003-01-01

    The detailed theoretical understanding of quantum spin dynamics in various molecular magnets is an important step on the roadway to technological applications of these systems. Quantum effects in both ferromagnetic and antiferromagnetic molecular clusters are, by now, theoretically well understood. Ferromagnetic molecular clusters allow one to study the interplay of incoherent quantum tunneling and thermally activated transitions between states with different spin orientation. The Berry phase oscillations found in Fe 8 are signatures of the quantum mechanical interference of different tunneling paths. Antiferromagnetic molecular clusters are promising candidates for the observation of coherent quantum tunneling on the mesoscopic scale. Although challenging, application of molecular magnetic clusters for data storage and quantum data processing are within experimental reach already with present day technology. Refs. 77 (author)

  18. Spin orientation in solid solution hematite-ilmenite

    DEFF Research Database (Denmark)

    Brok, Erik; Frandsen, Cathrine; Lefmann, Kim

    2017-01-01

    temperature range below the Néel temperature and does not depend systematically on Ti-content. The results indicate that the out-of-plane spin component is an intrinsic feature of hematite itself, with an origin not yet fully understood, but consistent with group theory. This represents a major shift...... spectroscopy. The usually assumed magnetic structure of hematite within this temperature range is antiferromagnetic with the spins confined to the basal plane of the hexagonal structure; however, an out-of-plane spin component is allowed by the symmetry of the system and has been observed in recent studies......The spin orientation in synthetic hematite-ilmenite samples and in a sample of natural hematite was studied from room temperature to above the antiferromagnetic-paramagnetic phase transition (the Néel temperature; TN ≈ 600–950 K) by neutron powder diffraction and at room temperature by Mössbauer...

  19. Fermi Surface, Pressure-Induced Antiferromagnetic Order, and Superconductivity in FeSe

    Science.gov (United States)

    Ishizuka, Jun; Yamada, Takemi; Yanagi, Yuki; Ōno, Yoshiaki

    2018-01-01

    The pressure dependence of the structural (Ts), antiferromagnetic (Tm), and superconducting (Tc) transition temperatures in FeSe is investigated on the basis of the 16-band d-p model. At ambient pressure, a shallow hole pocket disappears due to the correlation effect, as observed in the angular-resolved photoemission spectroscopy (ARPES) and quantum oscillation (QO) experiments, resulting in the suppression of the antiferromagnetic order, in contrast to the other iron pnictides. The orbital-polarization interaction between the Fe d orbital and Se p orbital is found to drive the ferro-orbital order responsible for the structural transition without accompanying the antiferromagnetic order. The pressure dependence of the Fermi surfaces is derived from the first-principles calculation and is found to well account for the opposite pressure dependences of Ts and Tm, around which the enhanced orbital and magnetic fluctuations cause the double-dome structure of the eigenvalue λ in the Eliashberg equation, as consistent with that of Tc in FeSe.

  20. Mixed spin Ising model with four-spin interaction and random crystal field

    Energy Technology Data Exchange (ETDEWEB)

    Benayad, N., E-mail: n.benayad@fsac.ac.ma [Groupe de Mecanique Statistique, Laboratoire de physique theorique et appliquee, Faculte des sciences-Aien Chock, Universite Hassan II-Casablanca, B.P 5366 Maarif, Casablanca 20100 (Morocco); Laboratoire de physique des hautes energies et de la matiere condensee, Faculte des sciences-Aien Chock, Universite Hassan II-Casablanca, B.P 5366 Maarif, Casablanca 20100 (Morocco); Ghliyem, M. [Groupe de Mecanique Statistique, Laboratoire de physique theorique et appliquee, Faculte des sciences-Aien Chock, Universite Hassan II-Casablanca, B.P 5366 Maarif, Casablanca 20100 (Morocco); Laboratoire de physique des hautes energies et de la matiere condensee, Faculte des sciences-Aien Chock, Universite Hassan II-Casablanca, B.P 5366 Maarif, Casablanca 20100 (Morocco)

    2012-01-01

    The effects of fluctuations of the crystal field on the phase diagram of the mixed spin-1/2 and spin-1 Ising model with four-spin interactions are investigated within the finite cluster approximation based on a single-site cluster theory. The state equations are derived for the two-dimensional square lattice. It has been found that the system exhibits a variety of interesting features resulting from the fluctuation of the crystal field interactions. In particular, for low mean value D of the crystal field, the critical temperature is not very sensitive to fluctuations and all transitions are of second order for any value of the four-spin interactions. But for relatively high D, the transition temperature depends on the fluctuation of the crystal field, and the system undergoes tricritical behaviour for any strength of the four-spin interactions. We have also found that the model may exhibit reentrance for appropriate values of the system parameters.