WorldWideScience

Sample records for angular resolved photoemission

  1. Bogoliubov Angle, Particle-Hole Mixture and Angular Resolved Photoemission Spectroscopy in Superconductors

    Energy Technology Data Exchange (ETDEWEB)

    Balatsky, A.

    2010-05-04

    Superconducting excitations - Bogoliubov quasiparticles - are the quantum mechanical mixture of negatively charged electron (-e) and positively charged hole (+e). We propose a new observable for Angular Resolved Photoemission Spectroscopy (ARPES) studies that is the manifestation of the particle-hole entanglement of the superconducting quasiparticles. We call this observable a Bogoliubov angle. This angle measures the relative weight of particle and hole amplitude in the superconducting (Bogoliubov) quasiparticle. We show how this quantity can be measured by comparing the ratio of spectral intensities at positive and negative energies.

  2. Direct angle resolved photoemission spectroscopy and ...

    Indian Academy of Sciences (India)

    Keywords. Condensed matter physics; high-c superconductivity; electronic properties; photoemission spectroscopy; angle resolved photoemission spectroscopy; cuprates; films; strain; pulsed laser deposition.

  3. Photoemission Electron Spectroscopy IV: Angle-resolved photoemission spectroscopy

    OpenAIRE

    Lee, J. D.; Nagatomi, T. (Translator); Mizutani, G. (Translator); Endo, K. (Translation Supervisor)

    2010-01-01

    The angle-resolved photoemission spectroscopy (ARPES) is a powerful experimental tool to probe themomentum-resolved electronic structure, i.e., the electronic band dispersion ε(k), of solids and their surfaces. ARPES is also an ideal tool to address the question concerning the electron correlation effect on quasiparticle excitations in the low-dimensional (one- or two-dimensional) correlated electron systems. In this issue, we briefly introduce representative studies of ARPES and their fruitf...

  4. Direct angle resolved photoemission spectroscopy and ...

    Indian Academy of Sciences (India)

    Since 1997 we systematically perform direct angle resolved photoemission spectroscopy (ARPES) on in-situ grown thin (< 30 nm) cuprate films. Specifically, we probe low-energy electronic structure and properties of high-c superconductors (HTSC) under different degrees of epitaxial (compressive vs. tensile) strain.

  5. Angular momentum-induced delays in solid-state photoemission enhanced by intra-atomic interactions.

    Science.gov (United States)

    Siek, Fabian; Neb, Sergej; Bartz, Peter; Hensen, Matthias; Strüber, Christian; Fiechter, Sebastian; Torrent-Sucarrat, Miquel; Silkin, Vyacheslav M; Krasovskii, Eugene E; Kabachnik, Nikolay M; Fritzsche, Stephan; Muiño, Ricardo Díez; Echenique, Pedro M; Kazansky, Andrey K; Müller, Norbert; Pfeiffer, Walter; Heinzmann, Ulrich

    2017-09-22

    Attosecond time-resolved photoemission spectroscopy reveals that photoemission from solids is not yet fully understood. The relative emission delays between four photoemission channels measured for the van der Waals crystal tungsten diselenide (WSe 2 ) can only be explained by accounting for both propagation and intra-atomic delays. The intra-atomic delay depends on the angular momentum of the initial localized state and is determined by intra-atomic interactions. For the studied case of WSe 2 , the photoemission events are time ordered with rising initial-state angular momentum. Including intra-atomic electron-electron interaction and angular momentum of the initial localized state yields excellent agreement between theory and experiment. This has required a revision of existing models for solid-state photoemission, and thus, attosecond time-resolved photoemission from solids provides important benchmarks for improved future photoemission models. Copyright © 2017 The Authors, some rights reserved; exclusive licensee American Association for the Advancement of Science. No claim to original U.S. Government Works.

  6. A spin-resolved photoemission study

    Indian Academy of Sciences (India)

    Stoner vs. spin-mixing behavior in the bulk magnetism of Gd: A spin-resolved photoemission study. K MAITI1,2,∗. , M C MALAGOLI2, A DALLMEYER2 and C CARBONE2,3. 1Tata Institute of Fundamental Research, Homi Bhabha Road, Mumbai 400 005, India. 2Institut für Festkörperforschung, Forschungszentrum Jülich, ...

  7. Angle-resolved photoemission extended fine structure

    International Nuclear Information System (INIS)

    Barton, J.J.

    1985-03-01

    Measurements of the Angle-Resolved Photoemission Extended Fine Structure (ARPEFS) from the S(1s) core level of a c(2 x 2)S/Ni(001) are analyzed to determine the spacing between the S overlayer and the first and second Ni layers. ARPEFS is a type of photoelectron diffraction measurement in which the photoelectron kinetic energy is swept typically from 100 to 600 eV. By using this wide range of intermediate energies we add high precision and theoretical simplification to the advantages of the photoelectron diffraction technique for determining surface structures. We report developments in the theory of photoelectron scattering in the intermediate energy range, measurement of the experimental photoemission spectra, their reduction to ARPEFS, and the surface structure determination from the ARPEFS by combined Fourier and multiple-scattering analyses. 202 refs., 67 figs., 2 tabs

  8. Evidence of the nature of core-level photoemission satellites using angle-resolved photoemission extended fine structure

    International Nuclear Information System (INIS)

    Moler, E.J.; Kellar, S.A.; Huff, W.R.A.

    1997-01-01

    The authors present a unique method of experimentally determining the angular momentum and intrinsic/extrinsic origin of core-level photoemission satellites by examining the satellite diffraction pattern in the Angle Resolved Photoemission Extended Fine Structure (ARPEFS) mode. They show for the first time that satellite peaks not associated with chemically differentiated atomic species display an ARPEFS intensity oscillation. They present ARPEFS data for the carbon 1s from (√3x√3)R30 CO/Cu(111) and p2mg(2xl)CO/Ni(110), nitrogen 1s from c(2x2) N 2 /Ni(100), cobalt 1s from p(1x1)Co/Cu(100), and nickel 3p from clean nickel (111). The satellite peaks and tails of the Doniach-Sunjic line shapes in all cases exhibit ARPEFS curves which indicate an angular momentum identical to the main peak and are of an intrinsic nature

  9. Evidence of the nature of core-level photoemission satellites using angle-resolved photoemission extended fine structure

    Energy Technology Data Exchange (ETDEWEB)

    Moler, E.J.; Kellar, S.A.; Huff, W.R.A. [Lawrence Berkeley National Lab., CA (United States)] [and others

    1997-04-01

    The authors present a unique method of experimentally determining the angular momentum and intrinsic/extrinsic origin of core-level photoemission satellites by examining the satellite diffraction pattern in the Angle Resolved Photoemission Extended Fine Structure (ARPEFS) mode. They show for the first time that satellite peaks not associated with chemically differentiated atomic species display an ARPEFS intensity oscillation. They present ARPEFS data for the carbon 1s from ({radical}3x{radical}3)R30 CO/Cu(111) and p2mg(2xl)CO/Ni(110), nitrogen 1s from c(2x2) N{sub 2}/Ni(100), cobalt 1s from p(1x1)Co/Cu(100), and nickel 3p from clean nickel (111). The satellite peaks and tails of the Doniach-Sunjic line shapes in all cases exhibit ARPEFS curves which indicate an angular momentum identical to the main peak and are of an intrinsic nature.

  10. Radiofrequency encoded angular-resolved light scattering

    DEFF Research Database (Denmark)

    Buckley, Brandon W.; Akbari, Najva; Diebold, Eric D.

    2015-01-01

    The sensitive, specific, and label-free classification of microscopic cells and organisms is one of the outstanding problems in biology. Today, instruments such as the flow cytometer use a combination of light scatter measurements at two distinct angles to infer the size and internal complexity...... of cells at rates of more than 10,000 per second. However, by examining the entire angular light scattering spectrum it is possible to classify cells with higher resolution and specificity. Current approaches to performing these angular spectrum measurements all have significant throughput limitations...... Encoded Angular-resolved Light Scattering (REALS), this technique multiplexes angular light scattering in the radiofrequency domain, such that a single photodetector captures the entire scattering spectrum from a particle over approximately 100 discrete incident angles on a single shot basis. As a proof...

  11. An experimentalist's guide to the matrix element in angle resolved photoemission

    International Nuclear Information System (INIS)

    Moser, Simon

    2017-01-01

    Highlights: • An introduction to the art of angle resolved photoemission is presented. • Matrix element effects are described by a nearly free electron final state model. • ARPES spectral weight of a Bloch band can be calculated from the Fourier transform of its Wannier orbital. • Experimental handedness and improper polarization introduce dichroism. • Instructive showcases from modern ARPES are discussed in detail. - Abstract: Angle resolved photoemission spectroscopy (ARPES) is commonly known as a powerful probe of the one-electron removal spectral function in ordered solid state. With increasing efficiency of light sources and spectrometers, experiments over a wide range of emission angles become more and more common. Consequently, the angular variation of ARPES spectral weight – often times termed “matrix element effect” – enters as an additional source of information. In this tutorial, we develop a simple but instructive free electron final state approach based on the three-step model to describe the intensity distribution in ARPES. We find a compact expression showing that the ARPES spectral weight of a given Bloch band is essentially determined by the momentum distribution (the Fourier transform) of its associated Wannier orbital – times a polarization dependent pre-factor. While the former is giving direct information on the symmetry and shape of the electronic wave function, the latter can give rise to surprising geometric effects. We discuss a variety of modern and instructive experimental showcases for which this simplistic formalism works astonishingly well and discuss the limits of this approach.

  12. Angle-resolved photoemission spectroscopy with quantum gas microscopes

    Science.gov (United States)

    Bohrdt, A.; Greif, D.; Demler, E.; Knap, M.; Grusdt, F.

    2018-03-01

    Quantum gas microscopes are a promising tool to study interacting quantum many-body systems and bridge the gap between theoretical models and real materials. So far, they were limited to measurements of instantaneous correlation functions of the form 〈O ̂(t ) 〉 , even though extensions to frequency-resolved response functions 〈O ̂(t ) O ̂(0 ) 〉 would provide important information about the elementary excitations in a many-body system. For example, single-particle spectral functions, which are usually measured using photoemission experiments in electron systems, contain direct information about fractionalization and the quasiparticle excitation spectrum. Here, we propose a measurement scheme to experimentally access the momentum and energy-resolved spectral function in a quantum gas microscope with currently available techniques. As an example for possible applications, we numerically calculate the spectrum of a single hole excitation in one-dimensional t -J models with isotropic and anisotropic antiferromagnetic couplings. A sharp asymmetry in the distribution of spectral weight appears when a hole is created in an isotropic Heisenberg spin chain. This effect slowly vanishes for anisotropic spin interactions and disappears completely in the case of pure Ising interactions. The asymmetry strongly depends on the total magnetization of the spin chain, which can be tuned in experiments with quantum gas microscopes. An intuitive picture for the observed behavior is provided by a slave-fermion mean-field theory. The key properties of the spectra are visible at currently accessible temperatures.

  13. Time-resolved two-photon photoemission from metal surfaces

    CERN Document Server

    Weinelt, M

    2002-01-01

    The Rydberg-like series of image-potential states is a prototype system for loosely bound electrons at a metal surface. The electronic structure and the femtosecond dynamics of these states is studied by high-resolution energy-and time-resolved two-photon photoemission spectroscopy. The electron trapped in the image potential moves virtually freely laterally to the surface where it is subject to inelastic and quasielastic scattering processes which cause decay of population and phase relaxation. The influence of surface corrugation on these processes has been investigated for adsorbates on Cu(001) and stepped Cu(117) and Cu(119) surfaces which are vicinal to Cu(001). The dynamics depend on both the distance of the electron in front of the surface and the parallel momentum. For CO molecules on Cu(001) inelastic scattering into bulk states and adsorbate-induced resonances determine the decay rate. For small numbers of Cu adatoms on Cu(001) and the vicinal surfaces the decay rate of image-potential states is sig...

  14. Constant Matrix Element Approximation to Time-Resolved Angle-Resolved Photoemission Spectroscopy

    Directory of Open Access Journals (Sweden)

    James K. Freericks

    2016-11-01

    Full Text Available We discuss several issues associated with employing a constant matrix element approximation for the coupling of light to multiband electrons in the context of time-resolved angle-resolved photoemission spectroscopy (TR-ARPES. In particular, we demonstrate that the “constant matrix element approximation” —even when reasonable—only holds for specific choices of the one-electron basis, and changing to other bases, requires including nonconstant corrections to the matrix element. We also discuss some simplifying approximations, where a constant matrix element is employed in multiple bases, and the consequences of this further approximation (especially with respect to the calculated TR-ARPES signal becoming negative. We also discuss issues related to gauge invariance of the final spectra.

  15. Angle-resolved photoemission spectroscopy (ARPES) studies of cuprate superconductors

    Energy Technology Data Exchange (ETDEWEB)

    Palczewski, Ari Deibert [Iowa State Univ., Ames, IA (United States)

    2010-01-01

    This dissertation is comprised of three different angle-resolved photoemission spectroscopy (ARPES) studies on cuprate superconductors. The first study compares the band structure from two different single layer cuprates Tl2Ba2CuO6+δ (Tl2201) Tc,max ~95 K and (Bi1.35Pb0.85)(Sr1.47La0.38)CuO6+δ (Bi2201) Tc,max 35 K. The aim of the study was to provide some insight into the reasons why single layer cuprate's maximum transition temperatures are so different. The study found two major di erences in the band structure. First, the Fermi surface segments close to ( π,0) are more parallel in Tl2201 than in Bi2201. Second, the shadow band usually related to crystal structure is only present in Bi2201, but absent in higher Tc Tl2201. The second study looks at the different ways of doping Bi2Sr2CaCu2O8+δ (Bi2212) in-situ by only changing the post bake-out vacuum conditions and temperature. The aim of the study is to systematically look into the generally overlooked experimental conditions that change the doping of a cleaved sample in ultra high vacuum (UHV) experiments. The study found two major experimental facts. First, in inadequate UHV conditions the carrier concentration of Bi2212 increases with time, due to the absorption of oxygen from CO2/CO molecules, prime contaminants present in UHV systems. Second, in a very clean UHV system at elevated temperatures (above about 200 K), the carrier concentration decreases due to the loss of oxygen atoms from the Bi-O layer. The final study probed the particle-hole symmetry of the pseudogap phase in high temperature superconducting cuprates by looking at the thermally excited bands above the Fermi level. The data showed a particle-hole symmetric pseudogap which symmetrically closes away from the nested FS before the node. The data is consistent with

  16. Angle-resolved photoemission spectroscopy (ARPES) studies of cuprate superconductors

    Energy Technology Data Exchange (ETDEWEB)

    Palczewski, Ari Deibert [Iowa State Univ., Ames, IA (United States)

    2010-01-01

    This dissertation is comprised of three different angle-resolved photoemission spectroscopy (ARPES) studies on cuprate superconductors. The first study compares the band structure from two different single layer cuprates Tl2Ba2CuO6+δ (Tl2201) Tc, max ≈ 95 K and (Bi 1.35Pb0.85)(Sr1.47La0.38)CuO6+δ (Bi2201) Tc, max ≈ 35 K. The aim of the study was to provide some insight into the reasons why single layer cuprate's maximum transition temperatures are so different. The study found two major differences in the band structure. First, the Fermi surface segments close to (π,0) are more parallel in Tl2201 than in Bi2201. Second, the shadow band usually related to crystal structure is only present in Bi2201, but absent in higher Tc Tl2201. The second study looks at the different ways of doping Bi2Sr2CaCu2O8+δ (Bi2212) in-situ by only changing the post bake-out vacuum conditions and temperature. The aim of the study is to systematically look into the generally overlooked experimental conditions that change the doping of a cleaved sample in ultra high vacuum (UHV) experiments. The study found two major experimental facts. First, in inadequate UHV conditions the carrier concentration of Bi2212 increases with time, due to the absorption of oxygen from CO2/CO molecules, prime contaminants present in UHV systems. Second, in a very clean UHV system at elevated temperatures (above about 200 K), the carrier concentration decreases due to the loss of oxygen atoms from the Bi-O layer. The final study probed the particle-hole symmetry of the pseudogap phase in high temperature superconducting cuprates by looking at the thermally excited bands above the Fermi level. The data showed a particle-hole symmetric pseudogap which symmetrically closes away from the nested FS before the node. The data is

  17. Theory of angle-resolved photoemission from the cuprate superconductors

    International Nuclear Information System (INIS)

    Hedegard, P.; Pedersen, M.B.

    1990-01-01

    We show that the photoemission spectrum for an RVB state with bosonic spins and fermionic charges consists of a peak on top of a broad background. The 'Fermi surface' corresponds to hole pockets around certain k-vectors. The theoretical predictions are compared with the available experimental data, and with the results obtained by other approaches. (orig.)

  18. Molecular frame photoelectron angular distribution for oxygen 1s photoemission from CO2 molecules

    International Nuclear Information System (INIS)

    Saito, N; Ueda, K; De Fanis, A

    2005-01-01

    We have measured photoelectron angular distributions in the molecular frame (MF-PADs) for O 1s photoemission from CO 2 , using photoelectron-O + -CO + coincidence momentum imaging. Results for the molecular axis at 0, 45 and 90 0 to the electric vector of the light are reported. The major features of the MF-PADs are fairly well reproduced by calculations employing a relaxed-core Hartree-Fock approach. Weak asymmetric features are seen through a plane perpendicular to the molecular axis and attributed to symmetry lowering by anti-symmetric stretching motion. (letter to the editor)

  19. Gauge invariance in the theoretical description of time-resolved angle-resolved pump/probe photoemission spectroscopy

    Energy Technology Data Exchange (ETDEWEB)

    Freericks, J. K.; Krishnamurthy, H. R.; Sentef, M. A.; Devereaux, T. P.

    2015-10-01

    Nonequilibrium calculations in the presence of an electric field are usually performed in a gauge, and need to be transformed to reveal the gauge-invariant observables. In this work, we discuss the issue of gauge invariance in the context of time-resolved angle-resolved pump/probe photoemission. If the probe is applied while the pump is still on, one must ensure that the calculations of the observed photocurrent are gauge invariant. We also discuss the requirement of the photoemission signal to be positive and the relationship of this constraint to gauge invariance. We end by discussing some technical details related to the perturbative derivation of the photoemission spectra, which involve processes where the pump pulse photoexcites electrons due to nonequilibrium effects.

  20. Electronic structure studies of BaFe2As2 by angle-resolved photoemission spectroscopy

    NARCIS (Netherlands)

    Fink, J.; Thirupathaiah, R.; Ovsyannikov, R.; Dürr, H.A.; Follath, R.; Huang, Y.; de Jong, S.; Golden, M.S.; Zhang, Y.Z.; Jeschke, H.O.; Valentí, R.; Felser, C.; Dastjani Farahani, S.; Rotter, M.; Johrendt, D.

    2009-01-01

    We report high resolution angle-resolved photoemission spectroscopy (ARPES) studies of the electronic structure of BaFe2As2, which is one of the parent compounds of the Fe-pnictide superconductors. ARPES measurements have been performed at 20 and 300 K, corresponding to the orthorhombic

  1. Dynamics of Molecular Orientation Observed Using Angle Resolved Photoemission Spectroscopy during Deposition of Pentacene on Graphite.

    Science.gov (United States)

    Park, Sang Han; Kwon, Soonnam

    2016-04-19

    A real-time method to observe both the structural and the electronic configuration of an organic molecule during deposition is reported for the model system of pentacene on graphite. Structural phase transition of the thin films as a function of coverage is monitored by using in situ angle resolved photoemission spectroscopy (ARPES) results to observe the change of the electronic configuration at the same time. A photoemission theory that uses independent atomic center approximations is introduced to identify the molecular orientation from the ARPES technique. This study provides a practical insight into interpreting ARPES data regarding dynamic changes of molecular orientation during initial growth of molecules on a well-defined surface.

  2. A tunable low-energy photon source for high-resolution angle-resolved photoemission spectroscopy

    International Nuclear Information System (INIS)

    Harter, John W.; Monkman, Eric J.; Shai, Daniel E.; Nie Yuefeng; Uchida, Masaki; Burganov, Bulat; Chatterjee, Shouvik; King, Philip D. C.; Shen, Kyle M.

    2012-01-01

    We describe a tunable low-energy photon source consisting of a laser-driven xenon plasma lamp coupled to a Czerny-Turner monochromator. The combined tunability, brightness, and narrow spectral bandwidth make this light source useful in laboratory-based high-resolution photoemission spectroscopy experiments. The source supplies photons with energies up to ∼7 eV, delivering under typical conditions >10 12 ph/s within a 10 meV spectral bandwidth, which is comparable to helium plasma lamps and many synchrotron beamlines. We first describe the lamp and monochromator system and then characterize its output, with attention to those parameters which are of interest for photoemission experiments. Finally, we present angle-resolved photoemission spectroscopy data using the light source and compare its performance to a conventional helium plasma lamp.

  3. Integrated experimental setup for angle resolved photoemission spectroscopy of transuranic materials.

    Science.gov (United States)

    Graham, Kevin S; Joyce, John J; Durakiewicz, Tomasz

    2013-09-01

    We have developed the Angle Resolved Photoemission Spectroscopy (ARPES) system for transuranic materials. The ARPES transuranic system is an endstation upgrade to the Laser Plasma Light Source (LPLS) at Los Alamos National Laboratory. The LPLS is a tunable light source for photoemission with a photon energy range covering the vacuum ultraviolet (VUV) and soft x-ray regions (27-140 eV). The LPLS was designed and developed for transuranic materials. Transuranic photoemission is currently not permitted at the public synchrotrons worldwide in the VUV energy range due to sample encapsulation requirements. With the addition of the ARPES capability to the LPLS system there is an excellent opportunity to explore new details centered on the electronic structure of actinide and transuranic materials.

  4. Electronic structure of Sr2RuO4 studied by angle-resolved photoemission spectroscopy

    International Nuclear Information System (INIS)

    Iwasawa, H.; Aiura, Y.; Saitoh, T.; Yoshida, Y.; Hase, I.; Ikeda, S.I.; Bando, H.; Kubota, M.; Ono, K.

    2007-01-01

    Electronic structure of the monolayer strontium ruthenate Sr 2 RuO 4 was investigated by high-resolution angle-resolved photoemission spectroscopy. We present photon-energy (hν) dependence of the electronic structure near the Fermi level along the ΓM line. The hν dependence has shown a strong spectral weight modulation of the Ru 4d xy and 4d zx bands

  5. Study of High Temperature Superconductors with Angle-Resolved Photoemission Spectroscopy

    Energy Technology Data Exchange (ETDEWEB)

    Dunn, Lisa

    2003-05-13

    The Angle Resolved Photoemission Spectroscopy (ARPES) recently emerged as a powerful tool for the study of highly correlated materials. This thesis describes the new generation of ARPES experiment, based on the third generation synchrotron radiation source and utilizing very high resolution electron energy and momentum analyzer. This new setup is used to study the physics of high temperature superconductors. New results on the Fermi surfaces, dispersions, scattering rate and superconducting gap in high temperature superconductors are presented.

  6. Electronic structure of superconducting Bi2212 crystal by angle resolved ultra violet photoemission

    International Nuclear Information System (INIS)

    Saini, N.L.; Shrivastava, P.; Garg, K.B.

    1993-01-01

    The electronic structure of a high quality superconducting Bi 2 Sr 2 CaCu 2 Osub(8+δ) (Bi2212) single crystal is studied by angle resolved ultra violet photoemission (ARUPS) using He I (21.2 eV). Our results appear to show two bands crossing the Fermi level in ΓX direction of the Brillouin zone as reported by Takahashi et al. The bands at higher binding energy do not show any appreciable dispersion. The nature of the states near the Fermi level is discussed and the observed band structure is compared with the band structure calculations. (author)

  7. Determination of electronic states in crystalline semiconductors and metals by angle-resolved photoemission

    International Nuclear Information System (INIS)

    Mills, K.A.

    1979-08-01

    An important part of the theoretical description of the solid state is band structure, which relies on the existence of dispersion relations connecting the electronic energy and wavevector in materials with translational symmetry. These relations determine the electronic behavior of such materials. The elaboration of accurate band structures, therefore, is of considerable fundamental and practical importance. Angle-resolved photoemission (ARP) spectroscopy provides the only presently available method for the detailed experimental investigation of band structures. This work is concerned with its application to both semiconducting and metallic single crystals

  8. Spin-resolved photoemission of surface states of W(110)-(1x1)H

    International Nuclear Information System (INIS)

    Hochstrasser, M.; Tobin, J.G.; Rotenberg, Eli; Kevan, S.D.

    2002-01-01

    The surface electronic states of W(110)-(1x1)H have been measured using spin- and angle-resolved photoemission. We directly demonstrate that the surface bands are both split and spin-polarized by the spin-orbit interaction in association with the loss of inversion symmetry near a surface. We observe 100 percent spin polarization of the surface states, with the spins aligned in the plane of the surface and oriented in a circular fashion relative to the S-bar symmetry point. In contrast, no measurable polarization of nearby bulk states is observed

  9. The Verwey transition observed by spin-resolved photoemission electron microscopy

    Energy Technology Data Exchange (ETDEWEB)

    Figuera, Juan de la, E-mail: juan.delafiguera@iqfr.csic.es [Instituto de Química Física “Rocasolano”, CSIC, Madrid E-28006 (Spain); Tusche, Christian [Max Planck Institute of Microstructure Physics, Halle D-06120 (Germany); Forschungszentrum Jülich GmbH, Peter Grünberg Institut (PGI-6), D-52425 Jülich (Germany)

    2017-01-01

    Highlights: • First observations of magnetic domains on magnetite (001) by spin-resolved PEEM. • Spin-polarization through the Verwey transitions does not change appreciably. • Shape and distribution of domains has been observed through the Verwey transition. - Abstract: We have imaged the magnetic domains on magnetite (001) through the Verwey transition by means of spin-resolved photoemission electron microscopy. A He laboratory source is used for illumination. The magnetic domains walls above the Verwey transition are aligned with 〈110〉 in-plane directions. Below the Verwey transition, the domain structure is interpreted as arising from a distribution of areas with different monoclinic c-axis, with linear 180° domain walls within each area and ragged edges when the magnetic domain boundaries coincide with structural domain walls. The domains evolve above the Verwey transition, while they are static below.

  10. Invited Article: High resolution angle resolved photoemission with tabletop 11 eV laser.

    Science.gov (United States)

    He, Yu; Vishik, Inna M; Yi, Ming; Yang, Shuolong; Liu, Zhongkai; Lee, James J; Chen, Sudi; Rebec, Slavko N; Leuenberger, Dominik; Zong, Alfred; Jefferson, C Michael; Moore, Robert G; Kirchmann, Patrick S; Merriam, Andrew J; Shen, Zhi-Xun

    2016-01-01

    We developed a table-top vacuum ultraviolet (VUV) laser with 113.778 nm wavelength (10.897 eV) and demonstrated its viability as a photon source for high resolution angle-resolved photoemission spectroscopy (ARPES). This sub-nanosecond pulsed VUV laser operates at a repetition rate of 10 MHz, provides a flux of 2 × 10(12) photons/s, and enables photoemission with energy and momentum resolutions better than 2 meV and 0.012 Å(-1), respectively. Space-charge induced energy shifts and spectral broadenings can be reduced below 2 meV. The setup reaches electron momenta up to 1.2 Å(-1), granting full access to the first Brillouin zone of most materials. Control over the linear polarization, repetition rate, and photon flux of the VUV source facilitates ARPES investigations of a broad range of quantum materials, bridging the application gap between contemporary low energy laser-based ARPES and synchrotron-based ARPES. We describe the principles and operational characteristics of this source and showcase its performance for rare earth metal tritellurides, high temperature cuprate superconductors, and iron-based superconductors.

  11. Valence-band structure of cubic CdS as determined by angle-resolved photoemission

    Science.gov (United States)

    Stampfl, A. P. J.; Hofmann, Ph.; Schaff, O.; Bradshaw, A. M.

    1997-04-01

    The valence-band structure of cubic CdS along the Γ-Σ-X direction and at all high-symmetry points has been experimentally determined using angle-resolved photoemission and compared to two local density approximation (LDA) calculations as well as to a recent quasiparticle calculation. The Cd 4d level was found to be semibandlike with an energy dispersion of up to 1 eV. The energy difference between the experimental and our calculated linear-muffin-tin orbital (LMTO) LDA energies falls, as expected, along a line of positive gradient. The quasiparticle calculation by Pollmann and co-workers fits the experimental values somewhat better than the LMTO calculation, although a difference of ~1.0 eV was still found to occur for the Cd 4d band. The self-interaction and relaxation-corrected pseudopotential LDA results by the same group give the best fit to within ~+/-0.5 eV for nearly all critical energies measured. Comparison with previously reported photoemission results on the wurtzite structure shows that energies at equivalent symmetry points agree within experimental error.

  12. Soft X-ray angle-resolved photoemission with micro-positioning techniques for metallic V2O3

    Science.gov (United States)

    Fujiwara, Hidenori; Kiss, Takayuki; Wakabayashi, Yuki K.; Nishitani, Yoshito; Mori, Takeo; Nakata, Yuki; Kitayama, Satoshi; Fukushima, Kazuaki; Ikeda, Shinji; Fuchimoto, Hiroto; Minowa, Yosuke; Mo, Sung-Kwan; Denlinger, Jonathan D.; Allen, James W.; Metcalf, Patricia; Imai, Masaki; Yoshimura, Kazuyoshi; Suga, Shigemasa; Muro, Takayuki; Sekiyama, Akira

    2015-01-01

    Soft X-ray angle-resolved photoemission has been performed for metallic V2O3. By combining a microfocus beam (40 µm × 65 µm) and micro-positioning techniques with a long-working-distance microscope, it has been possible to observe band dispersions from tiny cleavage surfaces with a typical size of several tens of µm. The photoemission spectra show a clear position dependence, reflecting the morphology of the cleaved sample surface. By selecting high-quality flat regions on the sample surface, it has been possible to perform band mapping using both photon-energy and polar-angle dependences, opening the door to three-dimensional angle-resolved photoemission spectroscopy for typical three-dimensional correlated materials where large cleavage planes are rarely obtained. PMID:25931096

  13. Modeling angle-resolved photoemission of graphene and black phosphorus nano structures.

    Science.gov (United States)

    Park, Sang Han; Kwon, Soonnam

    2016-05-10

    Angle-resolved photoemission spectroscopy (ARPES) data on electronic structure are difficult to interpret, because various factors such as atomic structure and experimental setup influence the quantum mechanical effects during the measurement. Therefore, we simulated ARPES of nano-sized molecules to corroborate the interpretation of experimental results. Applying the independent atomic-center approximation, we used density functional theory calculations and custom-made simulation code to compute photoelectron intensity in given experimental setups for every atomic orbital in poly-aromatic hydrocarbons of various size, and in a molecule of black phosphorus. The simulation results were validated by comparing them to experimental ARPES for highly-oriented pyrolytic graphite. This database provides the calculation method and every file used during the work flow.

  14. Dimensional Crossover in a Charge Density Wave Material Probed by Angle-Resolved Photoemission Spectroscopy

    Science.gov (United States)

    Nicholson, C. W.; Berthod, C.; Puppin, M.; Berger, H.; Wolf, M.; Hoesch, M.; Monney, C.

    2017-05-01

    High-resolution angle-resolved photoemission spectroscopy data reveal evidence of a crossover from one-dimensional (1D) to three-dimensional (3D) behavior in the prototypical charge density wave (CDW) material NbSe3 . In the low-temperature 3D regime, gaps in the electronic structure are observed due to two incommensurate CDWs, in agreement with x-ray diffraction and electronic-structure calculations. At higher temperatures we observe a spectral weight depletion that approaches the power-law behavior expected in one dimension. From the warping of the quasi-1D Fermi surface at low temperatures, we extract the energy scale of the dimensional crossover. This is corroborated by a detailed analysis of the density of states, which reveals a change in dimensional behavior dependent on binding energy. Our results offer an important insight into the dimensionality of excitations in quasi-1D materials.

  15. Angle-resolved photoemission studies of the superconducting gap symmetry in Fe-based superconductors

    Directory of Open Access Journals (Sweden)

    Y.-B. Huang

    2012-12-01

    Full Text Available The superconducting gap is the fundamental parameter that characterizes the superconducting state, and its symmetry is a direct consequence of the mechanism responsible for Cooper pairing. Here we discuss about angle-resolved photoemission spectroscopy measurements of the superconducting gap in the Fe-based high-temperature superconductors. We show that the superconducting gap is Fermi surface dependent and nodeless with small anisotropy, or more precisely, a function of the momentum location in the Brillouin zone. We show that while this observation seems inconsistent with weak coupling approaches for superconductivity in these materials, it is well supported by strong coupling models and global superconducting gaps. We also suggest that a smaller lifetime of the superconducting Cooper pairs induced by the momentum dependent interband scattering inherent to these materials could affect the residual density of states at low energies, which is critical for a proper evaluation of the superconducting gap.

  16. Angle-resolved photoemission spectra of graphene from first-principles calculations.

    Science.gov (United States)

    Park, Cheol-Hwan; Giustino, Feliciano; Spataru, Catalin D; Cohen, Marvin L; Louie, Steven G

    2009-12-01

    Angle-resolved photoemission spectroscopy (ARPES) is a powerful experimental technique for directly probing electron dynamics in solids. The energy versus momentum dispersion relations and the associated spectral broadenings measured by ARPES provide a wealth of information on quantum many-body interaction effects. In particular, ARPES allows studies of the Coulomb interaction among electrons (electron-electron interactions) and the interaction between electrons and lattice vibrations (electron-phonon interactions). Here, we report ab initio simulations of the ARPES spectra of graphene including both electron-electron and electron-phonon interactions on the same footing. Our calculations reproduce some of the key experimental observations related to many-body effects, including the indication of a mismatch between the upper and lower halves of the Dirac cone.

  17. A brief update of angle-resolved photoemission spectroscopy on a correlated electron system.

    Science.gov (United States)

    Lee, W S; Vishik, I M; Lu, D H; Shen, Z-X

    2009-04-22

    In this paper, we briefly summarize the capabilities of state-of-the-art angle-resolved photoemission spectroscopy (ARPES) in the field of experimental condensed matter physics. Due to the advancement of the detector technology and the high flux light sources, ARPES has become a powerful tool to study the low energy excitations of solids, especially those novel quantum materials in which many-body physics are at play. To benchmark today's state-of-the-art ARPES technique, we demonstrate that the precision of today's ARPES has advanced to a regime comparable to the bulk-sensitive de Haas-van Alphen (dHvA) measurements. Finally, as an example of new discoveries driven by the advancement of the ARPES technique, we summarize some of our recent ARPES measurements on underdoped high-T(c) superconducting cuprates, which have provided further insight into the complex pseudogap problem.

  18. Angle-resolved photoemission spectroscopy for the study of two-dimensional materials

    Science.gov (United States)

    Mo, Sung-Kwan

    2017-03-01

    Quantum systems in confined geometries allow novel physical properties that cannot easily be attained in their bulk form. These properties are governed by the changes in the band structure and the lattice symmetry, and most pronounced in their single layer limit. Angle-resolved photoemission spectroscopy (ARPES) is a direct tool to investigate the underlying changes of band structure to provide essential information for understanding and controlling such properties. In this review, recent progresses in ARPES as a tool to study two-dimensional atomic crystals have been presented. ARPES results from few-layer and bulk crystals of material class often referred as "beyond graphene" are discussed along with the relevant developments in the instrumentation.

  19. Direct observation of superconducting gaps in MgB 2 by angle-resolved photoemission spectroscopy

    Science.gov (United States)

    Souma, S.; Machida, Y.; Sato, T.; Takahashi, T.; Matsui, H.; Wang, S.-C.; Ding, H.; Kaminski, A.; Campuzano, J. C.; Sasaki, S.; Kadowaki, K.

    2004-08-01

    High-resolution angle-resolved photoemission spectroscopy has been carried out to clarify the anomalous superconductivity of MgB 2. We observed three bands crossing the Fermi level, which are ascribed to B2p-σ, π and surface bands. We have succeeded for the first time in directly observing the superconducting gaps of these bands separately. We have found that the superconducting-gap sizes of σ and surface bands are 6.5 ± 0.5 and 6.0 ± 0.5 meV, respectively, while that of the π band is much smaller (1.5 ± 0.5 meV). The present experimental result unambiguously demonstrates the validity of the two-band superconductivity in MgB 2.

  20. Direct observation of superconducting gaps in MgB2 by angle-resolved photoemission spectroscopy

    International Nuclear Information System (INIS)

    Souma, S.; Machida, Y.; Sato, T.; Takahashi, T.; Matsui, H.; Wang, S.-C.; Ding, H.; Kaminski, A.; Campuzano, J.C.; Sasaki, S.; Kadowaki, K.

    2004-01-01

    High-resolution angle-resolved photoemission spectroscopy has been carried out to clarify the anomalous superconductivity of MgB 2 . We observed three bands crossing the Fermi level, which are ascribed to B2p-σ, π and surface bands. We have succeeded for the first time in directly observing the superconducting gaps of these bands separately. We have found that the superconducting-gap sizes of σ and surface bands are 6.5 ± 0.5 and 6.0 ± 0.5 meV, respectively, while that of the π band is much smaller (1.5 ± 0.5 meV). The present experimental result unambiguously demonstrates the validity of the two-band superconductivity in MgB 2

  1. Tunable vacuum ultraviolet laser based spectrometer for angle resolved photoemission spectroscopy

    Energy Technology Data Exchange (ETDEWEB)

    Jiang, Rui; Mou, Daixiang; Wu, Yun; Huang, Lunan; Kaminski, Adam [Division of Materials Science and Engineering, Ames Laboratory, Ames, Iowa 50011 (United States); Department of Physics and Astronomy, Iowa State University, Ames, Iowa 50011 (United States); McMillen, Colin D.; Kolis, Joseph [Department of Chemistry, Clemson University, Clemson, South Carolina 29634 (United States); Giesber, Henry G.; Egan, John J. [Advanced Photonic Crystals LLC, Fort Mill, South Carolina 29708 (United States)

    2014-03-15

    We have developed an angle-resolved photoemission spectrometer with tunable vacuum ultraviolet laser as a photon source. The photon source is based on the fourth harmonic generation of a near IR beam from a Ti:sapphire laser pumped by a CW green laser and tunable between 5.3 eV and 7 eV. The most important part of the set-up is a compact, vacuum enclosed fourth harmonic generator based on potassium beryllium fluoroborate crystals, grown hydrothermally in the US. This source can deliver a photon flux of over 10{sup 14} photon/s. We demonstrate that this energy range is sufficient to measure the k{sub z} dispersion in an iron arsenic high temperature superconductor, which was previously only possible at synchrotron facilities.

  2. Angle-resolved and resonant photoemission spectroscopy of rare-earth and actinide intermetallics

    Science.gov (United States)

    Reihl, Bruno

    1985-07-01

    In this paper, some aspects of our angle-resolved and resonant photoemission work on rare-earth and actinide intermetallics will be summarized. The systems specifically mentioned are Gd(0001), UIr 3(100), UN(100), UO 2, α-γ- Ce 0.9Th 0.1, U xTh 1- xSb, USb xTe 1- x, UPd 3, UCu xNi 5- x, CeCu 2Si 2, UBe 13, U 2Zn 17 , SmAl 2, EuPd 13, YbBe 13, TmS, Yb xY 1- xAl 2, EuPd 2Si 2, TmSe, and UAs xSe 1- x.

  3. Gas-phase photoemission with soft x-rays: cross sections and angular distributions

    International Nuclear Information System (INIS)

    Shirley, D.A.; Kobrin, P.H.; Truesdale, C.M.; Lindle, D.W.; Ferrett, T.A.; Heimann, P.A.; Becker, U.; Kerkhoff, H.G.; Southworth, S.H.

    1983-09-01

    A summary is presented of typical gas-phase photoemission studies based on synchrotron radiation in the 50-5000 eV range, using beam lines at the Stanford Synchrotron Radiation Laboratory. Three topics are addressed: atomic inner-shell photoelectron cross sections and asymmetries, correlation peaks in rare gases, and core-level shape resonances in molecules

  4. Momentum-resolved electronic structure at a buried interface from soft X-ray standing-wave angle-resolved photoemission

    NARCIS (Netherlands)

    Gray, A.X.; Minar, J.; Plucinski, L.; Huijben, Mark; Bostwick, A.; Rotenberg, E.; Yang, S.-H.; Braun, J.; Winkelmann, A.; Conti, G.; Eiteneer, D.; Rattanachata, A.; Greer, A.A.; Ciston, J.; Ophus, C.; Rijnders, Augustinus J.H.M.; Blank, David H.A.; Doennig, D.; Pentcheva, R.; Kortright, J.B.; Schneider, C.M.; Ebert, H.; Fadley, C.S.

    2013-01-01

    Angle-resolved photoemission spectroscopy (ARPES) is a powerful technique for the study of electronic structure, but it lacks a direct ability to study buried interfaces between two materials. We address this limitation by combining ARPES with soft X-ray standing-wave (SW) excitation (SWARPES), in

  5. High-resolution angle-resolved photoemission investigation of potassium and phosphate tungsten bronzes

    International Nuclear Information System (INIS)

    Paul, Sanhita; Kumari, Spriha; Raj, Satyabrata

    2016-01-01

    Highlights: • Electronic structure of potassium and phosphate tungsten bronzes. • Origin of transport anomalies in bronzes. • Flat segments of Fermi surfaces are connected by a nesting vector, q. • Nesting driven charge-density wave is responsible for the anomalies. - Abstract: We have performed high-resolution angle-resolved photoemission spectroscopy (ARPES) and density functional ab initio theoretical calculation to study the electronic structure of potassium (K 0.25 WO 3 ) and phosphate (P 4 W 12 O 44 ) tungsten bronzes. We have experimentally determined the band dispersions and Fermi surface topology of these bronzes and compared with our theoretical calculations and a fair agreement has been seen between them. Our experimental as well as theoretical investigation elucidates the origin of transport anomalies in these bronzes. The Fermi surfaces of these bronzes consist of flat patches, which can be connected with each other by a constant nesting wave vector, q. The scattering wave vectors found from diffraction measurements match with these nesting vectors and the anomalies in the transport properties of these bronzes can be well explained by the evolution of charge-density wave with a partial nesting between the flat segments of the Fermi surfaces.

  6. Angle-resolved photoemission spectroscopy of rare earth LaSb{sub 2}

    Energy Technology Data Exchange (ETDEWEB)

    Michiardi, Matteo; Arnold, Fabian; Faerch Fisher, Karl Frederik; Svane, Axel; Bianchi, Marco; Brummerstedt Iversen, Bo; Hofmann, Philip [Aarhus University (Denmark); Shwetha, G.; Kanchana, V. [IIT-Hyderabad (India); Ganapathy, Vaitheeswaran [University of Hyderabad (India)

    2016-07-01

    Several rare earth diantimonides have been found to exhibit intriguing electronic properties such as anisotropic linear and non-saturating magnetoresistance. Among these materials, LaSb{sub 2} is not only considered for application in magnetoresistive devices but it is also found to be superconducting at low temperatures and it is investigated as candidate material to host charge density wave phases. Despite the several studies on its transport properties, the electronic structure of LaSb{sub 2} is still largely unknown. Here we present an angle-resolved photoemission spectroscopy and ab-initio calculation study of LaSb{sub 2}(001). The observed band structure is found to be in good agreement with theoretical predictions. Our results reveal that LaSb{sub 2} is a semimetal with a strongly nested two-dimensional Fermi surface. The low energy spectrum is characterized by four massive hole pockets and by four shallow, strongly directional, electron pockets that exhibit Dirac-like dispersion. We speculate on the possibility that this peculiar electronic structure drives the magnetoresistance to its quantum limit, explaining its unconventional behavior.

  7. Angle-resolved photoemission spectroscopy studies of metallic surface and interface states of oxide insulators

    Science.gov (United States)

    Plumb, Nicholas C.; Radović, Milan

    2017-11-01

    Over the last decade, conducting states embedded in insulating transition metal oxides (TMOs) have served as gateways to discovering and probing surprising phenomena that can emerge in complex oxides, while also opening opportunities for engineering advanced devices. These states are commonly realized at thin film interfaces, such as the well-known case of LaAlO3 (LAO) grown on SrTiO3 (STO). In recent years, the use of angle-resolved photoemission spectroscopy (ARPES) to investigate the k-space electronic structure of such materials led to the discovery that metallic states can also be formed on the bare surfaces of certain TMOs. In this topical review, we report on recent studies of low-dimensional metallic states confined at insulating oxide surfaces and interfaces as seen from the perspective of ARPES, which provides a direct view of the occupied band structure. While offering a fairly broad survey of progress in the field, we draw particular attention to STO, whose surface is so far the best-studied, and whose electronic structure is probably of the most immediate interest, given the ubiquitous use of STO substrates as the basis for conducting oxide interfaces. The ARPES studies provide crucial insights into the electronic band structure, orbital character, dimensionality/confinement, spin structure, and collective excitations in STO surfaces and related oxide surface/interface systems. The obtained knowledge increases our understanding of these complex materials and gives new perspectives on how to manipulate their properties.

  8. Electronic properties of novel topological quantum materials studied by angle-resolved photoemission spectroscopy (ARPES)

    Energy Technology Data Exchange (ETDEWEB)

    Wu, Yun [Iowa State Univ., Ames, IA (United States)

    2016-12-17

    The discovery of quantum Hall e ect has motivated the use of topology instead of broken symmetry to classify the states of matter. Quantum spin Hall e ect has been proposed to have a separation of spin currents as an analogue of the charge currents separation in quantum Hall e ect, leading us to the era of topological insulators. Three-dimensional analogue of the Dirac state in graphene has brought us the three-dimensional Dirac states. Materials with three-dimensional Dirac states could potentially be the parent compounds for Weyl semimetals and topological insulators when time-reversal or space inversion symmetry is broken. In addition to the single Dirac point linking the two dispersion cones in the Dirac/Weyl semimetals, Dirac points can form a line in the momentum space, resulting in a topological node line semimetal. These fascinating novel topological quantum materials could provide us platforms for studying the relativistic physics in condensed matter systems and potentially lead to design of new electronic devices that run faster and consume less power than traditional, silicon based transistors. In this thesis, we present the electronic properties of novel topological quantum materials studied by angle-resolved photoemission spectroscopy (ARPES).

  9. Structural studies of molecular and metallic overlayers using angle- resolved photoemission extended fine structure

    International Nuclear Information System (INIS)

    Huang, Z.

    1992-10-01

    Angle-resolved photoemission extended fine structure (ARPEFS) was used to study molecular and metallic overlayers on metal surfaces through analysis of p2mg(2x1)CO/Ni(110) and the p(2x2)K/Ni(111) adsorption. For the dense p2mg(2x1)CO/Ni(110) surface layer, photoemission intensities from C 1s level were measured in three directions at photoelectron kinetic energies 60-400 eV. Using multiple-scattering spherical-wave (MSSW) modeling, it was found that CO molecules are adsorbed on short-bridge sites, with adjacent CO along the [110] direction displaced alternatively in opposite directions towards the [001] azimuths to form a zigzag chain geometry. The tilt angle is 16±2 degree from the surface normal for the direction linking the C atom and the center of the Ni bridge. The carbon C-Ni interatomic distance was determined to be 1.94±0.02 Angstrom. The first- to second-layer spacing of Ni is 1.27±0.04 Angstrom, up from 1.10 Angstrom for the clean Ni(110) surface, but close to the 1.25 Angstrom Ni interlayer spacing in the bulk. The C-O bond length and tilt angle were varied within small ranges (1.10--1.20 Angstrom and 15--23 degrees) in our MSSW simulations. Best agreement between experiment and simulations was achieved at 1.16 Angstrom and 19 degrees. This yields an O-O distance of 2.95 Angstrom for the two nearest CO molecules, (van der Waals' radius ∼ 1.5 Angstrom for oxygen). Two different partial-wave phase-shifts were used in MSSW, and structural results from both are in very good agreement. For the p(2x2)K/Ni(111) overlayer, ARPEFS χ(k) curves from K 1s level measured along [111] and [771] at 130K showed that the K atoms are preferentially adsorbed on the atop sites, in agreement with a LEED study of the same system

  10. Method to map one-dimensional electronic wave function by using multiple Brillouin zone angle resolved photoemission

    Directory of Open Access Journals (Sweden)

    Dong-Wook Lee

    2010-10-01

    Full Text Available Angle resolved photoemission spectroscopy (ARPES is a powerful tool to investigate electronic structures in solids and has been widely used in studying various materials. The electronic structure information by ARPES is obtained in the momentum space. However, in the case of one-dimensional system, we here show that we extract the real space information from ARPES data taken over multiple Brillouin zones (BZs. Intensities in the multiple BZs are proportional to the photoemission matrix element which contains information on the coefficient of the Bloch wave function. It is shown that the Bloch wave function coefficients can be extracted from ARPES data, which allows us to construct the real space wave function. As a test, we use ARPES data from proto-typical one-dimensional system SrCuO2 and construct the real space wave function.

  11. Soft X-ray angle-resolved photoemission spectroscopy of heavily boron-doped superconducting diamond films

    Directory of Open Access Journals (Sweden)

    T. Yokoya, T. Nakamura, T. Matushita, T. Muro, H. Okazaki, M. Arita, K. Shimada, H. Namatame, M. Taniguchi, Y. Takano, M. Nagao, T. Takenouchi, H. Kawarada and T. Oguchi

    2006-01-01

    Full Text Available We have performed soft X-ray angle-resolved photoemission spectroscopy (SXARPES of microwave plasma-assisted chemical vapor deposition diamond films with different B concentrations in order to study the origin of the metallic behavior of superconducting diamond. SXARPES results clearly show valence band dispersions with a bandwidth of ~23 eV and with a top of the valence band at gamma point in the Brillouin zone, which are consistent with the calculated valence band dispersions of pure diamond. Boron concentration-dependent band dispersions near the Fermi level (EF exhibit a systematic shift of EF, indicating depopulation of electrons due to hole doping. These SXARPES results indicate that diamond bands retain for heavy boron doping and holes in the diamond band are responsible for the metallic states leading to superconductivity at low temperature. A high-resolution photoemission spectroscopy spectrum near EF of a heavily boron-doped diamond superconductor is also presented.

  12. Nano-Angle Resolved Photoemission Spectroscopy on Topological insulator Sb2Te3 nanowires responsible of quantum transport

    Science.gov (United States)

    Avila, José; Chen, Chaoyu; Arango, Yulieth C.; Huang, Liubing; Grützmacher, Detlev; Lüth, Hans; Lu, J. Grace; Schäpers, Thomas; Asensio, Maria C.

    2017-06-01

    Using high-resolution Nano-Angle Resolved Photoemission Spectroscopy (Nano-ARPES), we have determined the electronic structure of the surface and bulk states of topological insulator Sb2Te3 nanowires, which have been also characterized by magnetoresistance measurements. The observed Aharonov-Bohm-type oscillations could be unambiguously related to the transport by topological protected surface states directly recorded by photoemission. We have measured Nano-ARPES on individual nanowires of a few nanometers wide to provide direct evidence of the existence of the nontrivial topological surface states, as well as their doping. Our findings are consistent with theoretical predictions and confirm that the surface states of intrinsically doped unidimensional topological insulator nanowires are responsible for the quantum transport.

  13. Beamline for angle-resolved photoemission spectroscopy at low-temperature constructed at NTT Atsugi R and D Center

    International Nuclear Information System (INIS)

    Suzuki, Satoru; Yamamoto, Hideki; Maeda, Fumihiko; Watanabe, Yoshio; Yamada, Koji; Kiyokura, Takanori

    2005-01-01

    A vacuum ultra-violet beamline for in situ angle-resolved photoemission spectroscopy of MBE-grown high-T c superconductors at low temperature has been constructed at beamline ABL-6B of the normal-conducting ring in the synchrotron radiation facility of the NTT Atsugi R and D Center. The constant-deviation-angle varied-line-spacing plane grating monochromator covers the energy range of 20-200 eV by using two gratings. A photon flux of the order of 10 11 s -1 with a resolving power of 2000 or more was achieved in the whole energy range. The endstation is equipped with an angle-resolved photoelectron spectrometer, an rf-stimulated He discharge lamp, a custom-designed sample manipulator for low-temperature measurements and a loadlock system for in situ measurements. Total energy resolution of about 13 meV has been obtained for the photoemission spectrum of the Au Fermi edge, in spite of the bending-magnet light source of a second-generation synchrotron radiation ring

  14. Theory of angle-resolved photoemission experiments on a two-band model

    OpenAIRE

    De Cao, Tian

    2008-01-01

    Considering the electron states inside and outside the solid, we derive a formula of photoemission intensity. A general theoretical way to determine electronic structures of solids from ARPES experiments is outlined. It is shown that the spectral function inside the solids cannot be measured directly by ARPES, the effects of free electron states on the electronic structure observed by ARPES measurements must be considered, and the results from ARPES experiments cannot be understood until thes...

  15. Deflection gating for time-resolved x-ray magnetic circular dichroism-photoemission electron microscopy using synchrotron radiation

    Science.gov (United States)

    Wiemann, C.; Kaiser, A. M.; Cramm, S.; Schneider, C. M.

    2012-06-01

    In this paper, we present a newly developed gating technique for a time-resolving photoemission microscope. The technique makes use of an electrostatic deflector within the microscope's electron optical system for fast switching between two electron-optical paths, one of which is used for imaging, while the other is blocked by an aperture stop. The system can be operated with a switching time of 20 ns and shows superior dark current rejection. We report on the application of this new gating technique to exploit the time structure in the injection bunch pattern of the synchrotron radiation source BESSY II at Helmholtz-Zentrum Berlin for time-resolved measurements in the picosecond regime.

  16. Review of the theoretical description of time-resolved angle-resolved photoemission spectroscopy in electron-phonon mediated superconductors

    Energy Technology Data Exchange (ETDEWEB)

    Kemper, A.F. [Department of Physics, North Carolina State University, Raleigh, NC (United States); Sentef, M.A. [Max Planck Institute for the Structure and Dynamics of Matter, Center for Free Electron Laser Science, Hamburg (Germany); Moritz, B. [Stanford Institute for Materials and Energy Sciences (SIMES), SLAC National Accelerator Laboratory, Menlo Park, CA (United States); Devereaux, T.P. [Stanford Institute for Materials and Energy Sciences (SIMES), SLAC National Accelerator Laboratory, Menlo Park, CA (United States); Geballe Laboratory for Advanced Materials, Stanford University, Stanford, CA (United States); Freericks, J.K. [Department of Physics, Georgetown University, Washington, DC (United States)

    2017-09-15

    We review recent work on the theory for pump/probe photoemission spectroscopy of electron-phonon mediated superconductors in both the normal and the superconducting states. We describe the formal developments that allow one to solve the Migdal-Eliashberg theory in nonequilibrium for an ultrashort laser pumping field, and explore the solutions which illustrate the relaxation as energy is transferred from electrons to phonons. We focus on exact results emanating from sum rules and approximate numerical results which describe rules of thumb for relaxation processes. In addition, in the superconducting state, we describe how Anderson-Higgs oscillations can be excited due to the nonlinear coupling with the electric field and describe mechanisms where pumping the system enhances superconductivity. (copyright 2017 by WILEY-VCH Verlag GmbH and Co. KGaA, Weinheim)

  17. Angle-Resolved Photoemission Spectroscopy on Electronic Structure and Electron-Phonon Coupling in Cuprate Superconductors

    Energy Technology Data Exchange (ETDEWEB)

    Zhou, X.J.

    2010-04-30

    In addition to the record high superconducting transition temperature (T{sub c}), high temperature cuprate superconductors are characterized by their unusual superconducting properties below T{sub c}, and anomalous normal state properties above T{sub c}. In the superconducting state, although it has long been realized that superconductivity still involves Cooper pairs, as in the traditional BCS theory, the experimentally determined d-wave pairing is different from the usual s-wave pairing found in conventional superconductors. The identification of the pairing mechanism in cuprate superconductors remains an outstanding issue. The normal state properties, particularly in the underdoped region, have been found to be at odd with conventional metals which is usually described by Fermi liquid theory; instead, the normal state at optimal doping fits better with the marginal Fermi liquid phenomenology. Most notable is the observation of the pseudogap state in the underdoped region above T{sub c}. As in other strongly correlated electrons systems, these unusual properties stem from the interplay between electronic, magnetic, lattice and orbital degrees of freedom. Understanding the microscopic process involved in these materials and the interaction of electrons with other entities is essential to understand the mechanism of high temperature superconductivity. Since the discovery of high-T{sub c} superconductivity in cuprates, angle-resolved photoemission spectroscopy (ARPES) has provided key experimental insights in revealing the electronic structure of high temperature superconductors. These include, among others, the earliest identification of dispersion and a large Fermi surface, an anisotropic superconducting gap suggestive of a d-wave order parameter, and an observation of the pseudogap in underdoped samples. In the mean time, this technique itself has experienced a dramatic improvement in its energy and momentum resolutions, leading to a series of new discoveries not

  18. Direct observation of superconducting gaps in MgB{sub 2} by angle-resolved photoemission spectroscopy

    Energy Technology Data Exchange (ETDEWEB)

    Souma, S.; Machida, Y.; Sato, T.; Takahashi, T.; Matsui, H.; Wang, S.-C.; Ding, H.; Kaminski, A.; Campuzano, J.C.; Sasaki, S.; Kadowaki, K

    2004-08-01

    High-resolution angle-resolved photoemission spectroscopy has been carried out to clarify the anomalous superconductivity of MgB{sub 2}. We observed three bands crossing the Fermi level, which are ascribed to B2p-{sigma}, {pi} and surface bands. We have succeeded for the first time in directly observing the superconducting gaps of these bands separately. We have found that the superconducting-gap sizes of {sigma} and surface bands are 6.5 {+-} 0.5 and 6.0 {+-} 0.5 meV, respectively, while that of the {pi} band is much smaller (1.5 {+-} 0.5 meV). The present experimental result unambiguously demonstrates the validity of the two-band superconductivity in MgB{sub 2}.

  19. Electronic anisotropies revealed by detwinned angle-resolved photo-emission spectroscopy measurements of FeSe

    Science.gov (United States)

    Watson, Matthew D.; Haghighirad, Amir A.; Rhodes, Luke C.; Hoesch, Moritz; Kim, Timur K.

    2017-10-01

    We report high resolution angle-resolved photo-emission spectroscopy (ARPES) measurements of detwinned FeSe single crystals. The application of a mechanical strain is used to promote the volume fraction of one of the orthorhombic domains in the sample, which we estimate to be 80 % detwinned. While the full structure of the electron pockets consisting of two crossed ellipses may be observed in the tetragonal phase at temperatures above 90 K, we find that remarkably, only one peanut-shaped electron pocket oriented along the longer a axis contributes to the ARPES measurement at low temperatures in the nematic phase, with the expected pocket along b being not observed. Thus the low temperature Fermi surface of FeSe as experimentally determined by ARPES consists of one elliptical hole pocket and one orthogonally-oriented peanut-shaped electron pocket. Our measurements clarify the long-standing controversies over the interpretation of ARPES measurements of FeSe.

  20. Direct Observation of Localized Spin Antiferromagnetic Transition in PdCrO2 by Angle-Resolved Photoemission Spectroscopy

    Science.gov (United States)

    Noh, Han-Jin; Jeong, Jinwon; Chang, Bin; Jeong, Dahee; Moon, Hyun Sook; Cho, En-Jin; Ok, Jong Mok; Kim, Jun Sung; Kim, Kyoo; Min, B. I.; Lee, Han-Koo; Kim, Jae-Young; Park, Byeong-Gyu; Kim, Hyeong-Do; Lee, Seongsu

    2014-01-01

    We report the first case of the successful measurements of a localized spin antiferromagnetic transition in delafossite-type PdCrO2 by angle-resolved photoemission spectroscopy (ARPES). This demonstrates how to circumvent the shortcomings of ARPES for investigation of magnetism involved with localized spins in limited size of two-dimensional crystals or multi-layer thin films that neutron scattering can hardly study due to lack of bulk compared to surface. Also, our observations give direct evidence for the spin ordering pattern of Cr3+ ions in PdCrO2 suggested by neutron diffraction and quantum oscillation measurements, and provide a strong constraint that has to be satisfied by a microscopic mechanism for the unconventional anomalous Hall effect recently reported in this system. PMID:24419488

  1. Electronic structure of K0.5CoO2 studied by angle-resolved photoemission spectroscopy

    International Nuclear Information System (INIS)

    Usui, H.; Iwasawa, H.; Hirose, M.; Maeda, Y.; Saitoh, T.; Osada, H.; Kyomen, T.; Hanaya, M.; Aiura, Y.; Kotani, Y.; Kubota, M.; Ono, K.

    2010-01-01

    We have investigated the electronic structure of K 0.5 CoO 2 in the metallic phase by high-resolution angle-resolved photoemission spectroscopy at a low temperature. An observed Fermi surface of K 0.5 CoO 2 was a large hexagonal one around the Γ point only, with no hole pockets on the Γ-K lines which was typically predicted by band-structure calculations with local-density approximation (LDA). We also found that a modulation of the Fermi velocity, which was the largest at K point and the smallest at M point, was again opposite to the prediction by LDA band-theory. In spite of this conflicting with LDA band-theory, our results are both in agreement with what was observed in Na x CoO 2 .

  2. Dissimilarities between the electronic structure of chemically doped and chemically pressurized iron pnictides from an angle-resolved photoemission spectroscopy study

    NARCIS (Netherlands)

    Thirupathaiah, S.; Rienks, E.D.L.; Jeevan, H.S.; Ovsyannikov, R.; Slooten, E.; Kaas, J.; van Heumen, E.; de Jong, S.; Duerr, H.A.; Siemensmeyer, K.; Follath, R.; Gegenwart, P.; Golden, M.S.; Fink, J.

    2011-01-01

    We have studied the electronic structure of EuFe2As2-xPx using high-resolution angle-resolved photoemission spectroscopy. Upon substituting As with the isovalent P, which leads to chemical pressure and to superconductivity, we observe a nonrigid-band-like change of the electronic structure along the

  3. Dissimilarities between the electronic structure of chemically doped and chemically pressurized iron pnictides from an angle-resolved photoemission spectroscopy study

    NARCIS (Netherlands)

    Thirupathaiah, S.; Rienks, E.D.L.; Jeevan, H.S.; Ovsyannikov, R.; Slooten, E.; Kaas, J.; van Heumen, E.; de Jong, S.; Dürr, H.A.; Siemensmeyer, K.; Follath, R.; Gegenwart, P.; Golden, M.S.; Fink, J.

    2010-01-01

    We have studied the electronic structure of EuFe2As2-xPx using high resolution angle-resolved photoemission spectroscopy. Upon substituting As with the isovalent P, which leads to a chemical pressure and to superconductivity, we observe a non-rigid-band like change of the electronic structure along

  4. A high-efficiency spin-resolved photoemission spectrometer combining time-of-flight spectroscopy with exchange-scattering polarimetry

    Energy Technology Data Exchange (ETDEWEB)

    Jozwiak, Chris M.; Graff, Jeff; Lebedev, Gennadi; Andresen, Nord; Schmid, Andreas; Fedorov, Alexei; El Gabaly, Farid; Wan, Weishi; Lanzara, Alessandra; Hussain, Zahid

    2010-04-13

    We describe a spin-resolved electron spectrometer capable of uniquely efficient and high energy resolution measurements. Spin analysis is obtained through polarimetry based on low-energy exchange scattering from a ferromagnetic thin-film target. This approach can achieve a similar analyzing power (Sherman function) as state-of-the-art Mott scattering polarimeters, but with as much as 100 times improved efficiency due to increased reflectivity. Performance is further enhanced by integrating the polarimeter into a time-of-flight (TOF) based energy analysis scheme with a precise and flexible electrostatic lens system. The parallel acquisition of a range of electron kinetic energies afforded by the TOF approach results in an order of magnitude (or more) increase in efficiency compared to hemispherical analyzers. The lens system additionally features a 90 degrees bandpass filter, which by removing unwanted parts of the photoelectron distribution allows the TOF technique to be performed at low electron drift energy and high energy resolution within a wide range of experimental parameters. The spectrometer is ideally suited for high-resolution spin- and angle-resolved photoemission spectroscopy (spin-ARPES), and initial results are shown. The TOF approach makes the spectrometer especially ideal for time-resolved spin-ARPES experiments.

  5. An Angle Resolved Photoemission Study of a Mott Insulator and Its Evolution to a High Temperature Superconductor

    Energy Technology Data Exchange (ETDEWEB)

    Ronning, Filip

    2002-03-19

    One of the most remarkable facts about the high temperature superconductors is their close proximity to an antiferromagnetically ordered Mott insulating phase. This fact suggests that to understand superconductivity in the cuprates we must first understand the insulating regime. Due to material properties the technique of angle resolved photoemission is ideally suited to study the electronic structure in the cuprates. Thus, a natural starting place to unlocking the secrets of high Tc would appears to be with a photoemission investigation of insulating cuprates. This dissertation presents the results of precisely such a study. In particular, we have focused on the compound Ca{sub 2-x}Na{sub x}CuO{sub 2}Cl{sub 2}. With increasing Na content this system goes from an antiferromagnetic Mott insulator with a Neel transition of 256K to a superconductor with an optimal transition temperature of 28K. At half filling we have found an asymmetry in the integrated spectral weight, which can be related to the occupation probability, n(k). This has led us to identify a d-wave-like dispersion in the insulator, which in turn implies that the high energy pseudogap as seen by photoemission is a remnant property of the insulator. These results are robust features of the insulator which we found in many different compounds and experimental conditions. By adding Na we were able to study the evolution of the electronic structure across the insulator to metal transition. We found that the chemical potential shifts as holes are doped into the system. This picture is in sharp contrast to the case of La{sub 2-x}Sr{sub x}CuO{sub 4} where the chemical potential remains fixed and states are created inside the gap. Furthermore, the low energy excitations (ie the Fermi surface) in metallic Ca{sub 1.9}Na{sub 0.1}CuO{sub 2}Cl{sub 2} is most well described as a Fermi arc, although the high binding energy features reveal the presence of shadow bands. Thus, the results in this dissertation provide a

  6. Mass resolved angular distribution of fission products in 20Ne + 232Th reaction

    International Nuclear Information System (INIS)

    Tripathi, R.; Sodaye, S.; Sudarshan, K.; Kumar, Amit; Guin, R.

    2011-01-01

    Mass resolved angular distribution of fission products was measured in 20 Ne + 232 Th reaction at beam energy of 120 MeV. A preliminary analysis of the angular distribution data of fission products shows higher average anisotropy compared to that calculated using statistical theory. A signature of rise in anisotropy near symmetry, as reported in earlier studies in literature, is also seen. Further study is in progress to get more detailed information about the contribution from non-compound nucleus fission and dependence of angular anisotropy on asymmetry of mass division

  7. Resolving Two Dimensional Angular Velocity within a Rotary Tumbler

    Science.gov (United States)

    Helminiak, Nathaniel; Helminiak, David; Cariapa, Vikram; Borg, John

    2015-11-01

    In this study, a horizontally oriented cylindrical tumbler, filled at variable depth with cylindrical media, was rotated at various constant speeds. A monoplane layer of media was photographed with a high-speed camera and images were post processed with Particle Tracking Velocimetry (PTV) algorithms in order to resolve both the translational and rotational flow fields. Although the translational velocity fields have been well characterized, contemporary resources enabled the ability to expand upon and refine data regarding rotational characteristics of particles within a rotary tumbler. The results indicate that particles rotate according to intermittent no-slip interactions between the particles and solid body rotation. Particles within the bed, not confined to solid body rotation, exhibited behavior indicative of gearing between particles; each reacting to the tangential component of contact forming rotation chains. Furthermore, it was observed that solid body interactions corresponded to areas of confined motion, as areas of high interaction dissuaded no-slip rotation, while areas of developing flow tended towards no-slip rotation. Special thanks to: NASA Wisconsin Space Grant Consortium Program as well as Marquette University OPUS College of Engineering.

  8. Electronic band structure of epitaxial PbTe (111) thin films observed by angle-resolved photoemission spectroscopy

    Science.gov (United States)

    Ye, Zhenyu; Cui, Shengtao; Shu, Tianyu; Ma, Songsong; Liu, Yang; Sun, Zhe; Luo, Jun-Wei; Wu, Huizhen

    2017-04-01

    Using angle-resolved photoemission spectroscopy (ARPES), we studied bulk and surface electronic band structures of narrow-gap semiconductor lead telluride (PbTe) thin films grown by molecular beam epitaxy both perpendicular and parallel to the Γ -L direction. The comparison of ARPES data with the first-principles calculation reveals the details of band structures, orbital characters, spin-orbit splitting energies, and surface states. The photon-energy-dependent spectra show the bulk character. Both the L and Σ valence bands are observed and their energy difference is determined. The spin-orbit splitting energies at L and Γ points are 0.62 eV and 0.88 eV, respectively. The surface states below and close to the valence band maximum are identified. The valence bands are composed of a mixture of Pb 6 s and Te 5 pz orbitals with dominant in-plane even parity, which is attributed to the layered distortion in the vicinity of the PbTe (111) surface. These findings provide insights into PbTe fundamental properties and shall benefit relevant thermoelectric and optoelectronic applications.

  9. Evidence for Itinerant Carriers in an Anisotropic Narrow-Gap Semiconductor by Angle-Resolved Photoemission Spectroscopy.

    Science.gov (United States)

    Ju, Sailong; Bai, Wei; Wu, Liming; Lin, Hua; Xiao, Chong; Cui, Shengtao; Li, Zhou; Kong, Shuai; Liu, Yi; Liu, Dayong; Zhang, Guobin; Sun, Zhe; Xie, Yi

    2018-01-01

    The ability to accurately determine the electronic structure of solids has become a key prerequisite for modern functional materials. For example, the precise determination of the electronic structure helps to balance the three thermoelectric parameters, which is the biggest challenge to design high-performance thermoelectric materials. Herein, by high-resolution, angle-resolved photoemission spectroscopy (ARPES), the itinerant carriers in CsBi 4 Te 6 (CBT) are revealed for the first time. CBT is a typical anisotropic, narrow-gap semiconductor used as a practical candidate for low-temperature thermoelectric applications, and p-doped CBT series show superconductivity at relatively low carrier concentrations. The ARPES results show a significantly larger bandwidth near the Fermi surface than calculations, which means the carriers transport anisotropically and itinerantly in CBT. It is reasonable to believe that these newly discovered features of carriers in narrow-gap semiconductors are promising for designing optimal thermoelectric materials and superconductors. © 2017 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

  10. Anisotropic electronic band structure of intrinsic Si(110) studied by angle-resolved photoemission spectroscopy and first-principles calculations

    Science.gov (United States)

    Matsushita, Stephane Yu; Takayama, Akari; Kawamoto, Erina; Hu, Chunping; Hagiwara, Satoshi; Watanabe, Kazuyuki; Takahashi, Takashi; Suto, Shozo

    2017-09-01

    We have studied the electronic band structure of the hydrogen-terminated Si(110)-(1 ×1 ) [H:Si(110)-(1 ×1 )] surface using angle-resolved photoemission spectroscopy (ARPES) and first-principles calculations in the framework of density functional theory with local density approximation (LDA). The bulk-truncated H:Si(110)-(1 ×1 ) surface is a good template to investigate the electronic band structure of the intrinsic Si(110). In the ARPES spectra, seven bulk states and one surface state due to the H-H interaction are observed clearly. The four bulk states consisting of Si 3 px y orbitals exhibit anisotropic band dispersions along the high symmetric direction of Γ ¯-X ¯ and Γ ¯-X¯' directions, where one state shows one-dimensional character. The calculated band structures show a good agreement with the experimental results except the surface state. We discuss the exact nature of electronic band structures and the applicability of LDA. We have estimated the anisotropic effective masses of electrons and holes of Si(110) for device application.

  11. Photoemission with high-order harmonics: A tool for time-resolved core-level spectroscopy

    DEFF Research Database (Denmark)

    Christensen, Bjarke Holl; Raarup, Merete Krog; Balling, Peter

    2010-01-01

    A setup for femtosecond time-resolved photoelectron spectroscopy of solid surfaces is presented. The photon energies for core-level spectroscopy experiments are created by high-order harmonic generation from infrared 120-femtosecond laser pulses focused in a Ne gas jet. The present experimental r...... from the sample are collected by a large-solid-angle time-of-flight electron spectrometer based on a parabolic-grid reflector. Results from experiments probing the Bi 5d core-levels are presented, and the results of preliminary pump-probe experiments are described....

  12. Evidence for Anionic Excess Electrons in a Quasi-Two-Dimensional Ca2N Electride by Angle-Resolved Photoemission Spectroscopy.

    Science.gov (United States)

    Oh, Ji Seop; Kang, Chang-Jong; Kim, Ye Ji; Sinn, Soobin; Han, Moonsup; Chang, Young Jun; Park, Byeong-Gyu; Kim, Sung Wng; Min, Byung Il; Kim, Hyeong-Do; Noh, Tae Won

    2016-03-02

    Angle-resolved photoemission spectroscopy (ARPES) study of a layered electride Ca2N was carried out to reveal its quasi-two-dimensional electronic structure. The band dispersions and the Fermi-surface map are consistent with the density functional theory results except for a chemical potential shift that may originate from the high reactivity of surface excess electrons. Thus, the existence of anionic excess electrons in the interlayer region of Ca2N is strongly supported by ARPES.

  13. High Resolution Angle Resolved Photoemission Studies on Quasi-Particle Dynamics in Graphite

    Energy Technology Data Exchange (ETDEWEB)

    Leem, C.S.

    2010-06-02

    We obtained the spectral function of the graphite H point using high resolution angle resolved photoelectron spectroscopy (ARPES). The extracted width of the spectral function (inverse of the photo-hole lifetime) near the H point is approximately proportional to the energy as expected from the linearly increasing density of states (DOS) near the Fermi energy. This is well accounted by our electron-phonon coupling theory considering the peculiar electronic DOS near the Fermi level. And we also investigated the temperature dependence of the peak widths both experimentally and theoretically. The upper bound for the electron-phonon coupling parameter is 0.23, nearly the same value as previously reported at the K point. Our analysis of temperature dependent ARPES data at K shows that the energy of phonon mode of graphite has much higher energy scale than 125K which is dominant in electron-phonon coupling.

  14. Electronic structure of R Sb (R =Y , Ce, Gd, Dy, Ho, Tm, Lu) studied by angle-resolved photoemission spectroscopy

    Science.gov (United States)

    Wu, Yun; Lee, Yongbin; Kong, Tai; Mou, Daixiang; Jiang, Rui; Huang, Lunan; Bud'ko, S. L.; Canfield, P. C.; Kaminski, Adam

    2017-07-01

    We use high-resolution angle-resolved photoemission spectroscopy (ARPES) and electronic structure calculations to study the electronic properties of rare-earth monoantimonides RSb (R = Y, Ce, Gd, Dy, Ho, Tm, Lu). The experimentally measured Fermi surface (FS) of RSb consists of at least two concentric hole pockets at the Γ point and two intersecting electron pockets at the X point. These data agree relatively well with the electronic structure calculations. Detailed photon energy dependence measurements using both synchrotron and laser ARPES systems indicate that there is at least one Fermi surface sheet with strong three-dimensionality centered at the Γ point. Due to the "lanthanide contraction", the unit cell of different rare-earth monoantimonides shrinks when changing the rare-earth ion from CeSb to LuSb. This results in the differences in the chemical potentials in these compounds, which are demonstrated by both ARPES measurements and electronic structure calculations. Interestingly, in CeSb, the intersecting electron pockets at the X point seem to be touching the valence bands, forming a fourfold-degenerate Dirac-like feature. On the other hand, the remaining rare-earth monoantimonides show significant gaps between the upper and lower bands at the X point. Furthermore, similar to the previously reported results of LaBi, a Dirac-like structure was observed at the Γ point in YSb, CeSb, and GdSb, compounds showing relatively high magnetoresistance. This Dirac-like structure may contribute to the unusually large magnetoresistance in these compounds.

  15. Unusually large chemical potential shift in a degenerate semiconductor: Angle-resolved photoemission study of SnSe and Na-doped SnSe

    Science.gov (United States)

    Maeda, M.; Yamamoto, K.; Mizokawa, T.; Saini, N. L.; Arita, M.; Namatame, H.; Taniguchi, M.; Tan, G.; Zhao, L. D.; Kanatzidis, M. G.

    2018-03-01

    We have studied the electronic structure of SnSe and Na-doped SnSe by means of angle-resolved photoemission spectroscopy. The valence-band top reaches the Fermi level by the Na doping, indicating that Na-doped SnSe can be viewed as a degenerate semiconductor. However, in the Na-doped system, the chemical potential shift with temperature is unexpectedly large and is apparently inconsistent with the degenerate semiconductor picture. The large chemical potential shift and anomalous spectral shape are key ingredients for an understanding of the novel metallic state with the large thermoelectric performance in Na-doped SnSe.

  16. Time-resolved angular distributions of plume ions from silver at low and medium laser fluence

    DEFF Research Database (Denmark)

    Christensen, Bo Toftmann; Schou, Jørgen

    Even at moderate fluence (0.6 -2.4 J/cm2) laser impact on metals in the UV regime results in a significant number of ions emitted from the surface. The ablated particles are largely neutrals at the lowest fluence, but the fraction of ions increases strongly with fluence. We have irradiated silver...... in a vacuum chamber (~ 10-7 mbar) with a Nd:YAG laser at a wavelength of 355 nm and made detailed measurements of the time-resolved angular distribution. The ion flow in different directions has been measured with a hemispherical array of Langmuir probes, by which the time-of-flight spectra, as well...

  17. Angle-resolved photoemission studies of lattice polaron formation in the cuprate Ca2CuO2Cl2

    Energy Technology Data Exchange (ETDEWEB)

    Shen, K.M.

    2010-05-03

    To elucidate the nature of the single-particle excitations in the undoped parent cuprates, we have performed a detailed study of Ca{sub 2}CuO{sub 2}Cl{sub 2} using photoemission spectroscopy. The photoemission lineshapes of the lower Hubbard band are found to be well-described by a polaron model. By comparing the lineshape and temperature dependence of the lower Hubbard band with additional O 2p and Ca 3p states, we conclude that the dominant broadening mechanism arises from the interaction between the photohole and the lattice. The strength of this interaction was observed to be strongly anisotropic and may have important implications for the momentum dependence of the first doped hole states.

  18. Time resolved photoemission spectroscopy of electronic cooling and localization in CH$_3$NH$_3$PbI$_3$ crystals

    OpenAIRE

    Chen, Zhesheng; Lee, Min-i; Zhang, Zailan; Diab, Hiba; Garrot, Damien; Lédée, Ferdinand; Fertey, Pierre; Papalazarou, Evangelos; Marsi, Marino; Ponseca, Carlito; Deleporte, Emmanuelle; Tejeda, Antonio; Perfetti, Luca

    2017-01-01

    We measure the surface of CH$_3$NH$_3$PbI$_3$ single crystals by making use of two photon photoemission spectroscopy. Our method monitors the electronic distribution of photoexcited electrons, explicitly discriminating the initial thermalization from slower dynamical processes. The reported results disclose the fast dissipation channels of hot carriers (0.25 ps), set a upper bound to the surface induced recombination velocity ($

  19. Electronic structure studies of ferro-pnictide superconductors and their parent compounds using angle-resolved photoemission spectroscopy (ARPES)

    Energy Technology Data Exchange (ETDEWEB)

    Setti, Thirupathaiah

    2011-07-14

    The discovery of high temperature superconductivity in the iron pnictide compound LaO{sub 1-x}F{sub x}FeAs with T{sub c} = 26 K as created enormous interest in the high-T{sub c} superconductor community. So far, four prototypes of crystal structures have been found in the Fe-pnictide family. All four show a structural deformation followed or accompanied by a magnetic transition from a high temperature paramagnetic conductor to a low temperature antiferromagnetic metal whose transition temperature T{sub N} varies between the compounds. Charge carrier doping, isovalent substitution of the As atoms or the application of pressure suppresses the antiferromagnetic spin density wave (SDW) order and leads to a superconducting phase. More recently high Tc superconductivity has been also detected in iron chalchogenides with similar normal state properties. Since superconductivity is instability of the normal state, the study of normal state electronic structure in comparison with superconducting state could reveal important information on the pairing mechanism. Therefore, it is most important to study the electronic structure of these new superconductors, i.e., to determine Fermi surfaces and band dispersions near the Fermi level at the high symmetry points in order to obtain a microscopic understanding of the superconducting properties. Using the technique angle-resolved photoemission spectroscopy (ARPES) one measures the electrons ejected from a sample when photons impinge on it. In this way one can map the Fermi surface which provides useful information regarding the physics behind the Fermi surface topology of high T{sub c} superconductors. Furthermore, this technique provides information on the band dispersion, the orbital character of the bands, the effective mass, the coupling to bosonic excitations, and the superconducting gap. This emphasizes the importance of studying the electronic structure of the newly discovered Fe-pnictides using ARPES. In this work we have

  20. Angle-resolved photoemission spectroscopy with 9-eV photon-energy pulses generated in a gas-filled hollow-core photonic crystal fiber

    Energy Technology Data Exchange (ETDEWEB)

    Bromberger, H., E-mail: Hubertus.Bromberger@mpsd.mpg.de; Liu, H.; Chávez-Cervantes, M.; Gierz, I. [Max Planck Institute for the Structure and Dynamics of Matter, Luruper Chaussee 149, 22761 Hamburg (Germany); Ermolov, A.; Belli, F.; Abdolvand, A.; Russell, P. St. J.; Travers, J. C. [Max Planck Institute for the Science of Light, Günther-Scharowsky-Str. 1, 91058 Erlangen (Germany); Calegari, F. [Max Planck Institute for the Structure and Dynamics of Matter, Luruper Chaussee 149, 22761 Hamburg (Germany); Institute for Photonics and Nanotechnologies, IFN-CNR, Piazza Leonardo da Vinci 32, I-20133 Milano (Italy); Li, M. T.; Lin, C. T. [Max Planck Institute for Solid State Research, Heisenbergstr. 1, 70569 Stuttgart (Germany); Cavalleri, A. [Max Planck Institute for the Structure and Dynamics of Matter, Luruper Chaussee 149, 22761 Hamburg (Germany); Clarendon Laboratory, Department of Physics, University of Oxford, Parks Rd. Oxford OX1 3PU (United Kingdom)

    2015-08-31

    A recently developed source of ultraviolet radiation, based on optical soliton propagation in a gas-filled hollow-core photonic crystal fiber, is applied here to angle-resolved photoemission spectroscopy (ARPES). Near-infrared femtosecond pulses of only few μJ energy generate vacuum ultraviolet radiation between 5.5 and 9 eV inside the gas-filled fiber. These pulses are used to measure the band structure of the topological insulator Bi{sub 2}Se{sub 3} with a signal to noise ratio comparable to that obtained with high order harmonics from a gas jet. The two-order-of-magnitude gain in efficiency promises time-resolved ARPES measurements at repetition rates of hundreds of kHz or even MHz, with photon energies that cover the first Brillouin zone of most materials.

  1. Time-resolved photoemission spectroscopy of electronic cooling and localization in CH3NH3PbI3 crystals

    Science.gov (United States)

    Chen, Zhesheng; Lee, Min-i.; Zhang, Zailan; Diab, Hiba; Garrot, Damien; Lédée, Ferdinand; Fertey, Pierre; Papalazarou, Evangelos; Marsi, Marino; Ponseca, Carlito; Deleporte, Emmanuelle; Tejeda, Antonio; Perfetti, Luca

    2017-09-01

    We measure the surface of CH3NH3PbI3 single crystals by making use of two-photon photoemission spectroscopy. Our method monitors the electronic distribution of photoexcited electrons, explicitly discriminating the initial thermalization from slower dynamical processes. The reported results disclose the fast-dissipation channels of hot carriers (0.25 ps), set an upper bound to the surface-induced recombination velocity (PbI3 samples is consistent with the progressive reduction of photoconversion efficiency in operating devices. Minimizing the density of shallow traps and solving the aging problem may boost the macroscopic efficiency of solar cells to the theoretical limit.

  2. Time- and angle-resolved photoemission spectroscopy with optimized high-harmonic pulses using frequency-doubled Ti:Sapphire lasers

    International Nuclear Information System (INIS)

    Eich, S.; Stange, A.; Carr, A.V.; Urbancic, J.; Popmintchev, T.; Wiesenmayer, M.; Jansen, K.; Ruffing, A.; Jakobs, S.; Rohwer, T.; Hellmann, S.; Chen, C.; Matyba, P.; Kipp, L.; Rossnagel, K.; Bauer, M.; Murnane, M.M.; Kapteyn, H.C.; Mathias, S.; Aeschlimann, M.

    2014-01-01

    Highlights: • We present a scheme to generate high intensity XUV pulses from HHG with variable time-bandwidth product. • Shorter-wavelength driven high-harmonic XUV trARPES provides higher photon flux and increased energy resolution. • High-quality high-harmonic XUV trARPES data with sub 150 meV energy and sub 30 fs time resolution is presented. - Abstract: Time- and angle-resolved photoemission spectroscopy (trARPES) using femtosecond extreme ultraviolet high harmonics has recently emerged as a powerful tool for investigating ultrafast quasiparticle dynamics in correlated-electron materials. However, the full potential of this approach has not yet been achieved because, to date, high harmonics generated by 800 nm wavelength Ti:Sapphire lasers required a trade-off between photon flux, energy and time resolution. Photoemission spectroscopy requires a quasi-monochromatic output, but dispersive optical elements that select a single harmonic can significantly reduce the photon flux and time resolution. Here we show that 400 nm driven high harmonic extreme-ultraviolet trARPES is superior to using 800 nm laser drivers since it eliminates the need for any spectral selection, thereby increasing photon flux and energy resolution to <150 meV while preserving excellent time resolution of about 30 fs

  3. Identification of Ni2C electronic states in graphene-Ni(111) growth through resonant and dichroic angle-resolved photoemission at the C K -edge

    Science.gov (United States)

    Drera, G.; Cepek, C.; Patera, L. L.; Bondino, F.; Magnano, E.; Nappini, S.; Africh, C.; Lodi-Rizzini, A.; Joshi, N.; Ghosh, P.; Barla, A.; Mahatha, S. K.; Pagliara, S.; Giampietri, A.; Pintossi, C.; Sangaletti, L.

    2017-10-01

    The graphene-Ni(111) (GrNi) growth via chemical vapor deposition has been explored by resonant, angle-resolved, and dichroic photoemission spectroscopy (soft x-ray Res-ARPES) in order to identify the possible contributions to the electronic structure deriving from different phases that can coexist in this complex system. We provide evidences of electronic states so far unexplored at the Γ ¯ point of GrNi, appearing at the C K -edge resonance. These states show both circular dichroism (CD) and k dependence, suggesting a long-range orbital ordering, as well as a coherent matching with the underlying lattice. Through a comparison of core-level photoemission, valence band resonances, and constant initial-state spectroscopy, we demonstrate that these states are actually induced by a low residual component of nickel carbide (Ni2C ). These results also show that caution must be exercised while interpreting x-ray magnetic circular dichroism collected on C K -edge with Auger partial yield method, due to the presence of CD in photoelectron spectra unrelated to magnetic effects.

  4. Rapid high-resolution spin- and angle-resolved photoemission spectroscopy with pulsed laser source and time-of-flight spectrometer.

    Science.gov (United States)

    Gotlieb, K; Hussain, Z; Bostwick, A; Lanzara, A; Jozwiak, C

    2013-09-01

    A high-efficiency spin- and angle-resolved photoemission spectroscopy (spin-ARPES) spectrometer is coupled with a laboratory-based laser for rapid high-resolution measurements. The spectrometer combines time-of-flight (TOF) energy measurements with low-energy exchange scattering spin polarimetry for high detection efficiencies. Samples are irradiated with fourth harmonic photons generated from a cavity-dumped Ti:sapphire laser that provides high photon flux in a narrow bandwidth, with a pulse timing structure ideally matched to the needs of the TOF spectrometer. The overall efficiency of the combined system results in near-E(F) spin-resolved ARPES measurements with an unprecedented combination of energy resolution and acquisition speed. This allows high-resolution spin measurements with a large number of data points spanning multiple dimensions of interest (energy, momentum, photon polarization, etc.) and thus enables experiments not otherwise possible. The system is demonstrated with spin-resolved energy and momentum mapping of the L-gap Au(111) surface states, a prototypical Rashba system. The successful integration of the spectrometer with the pulsed laser system demonstrates its potential for simultaneous spin- and time-resolved ARPES with pump-probe based measurements.

  5. The application of angular resolved scatter to the documentation of damage to smooth mirrors

    International Nuclear Information System (INIS)

    Gillespie, C.H.; Edwards, D.F.; Stover, J.C.

    1986-01-01

    Mirrors designed to survive exposure to damaging radiation are being irradiated and then measured to determine the mechanisms of failure and to improve the ability of analysis codes to predict an exposure damage threshold. The differences between survival and catastrophic failure are easily recognized and recorded by macro photography. However, the coal of this project is to quantify the onset of mirror degradation utilizing non contact methods that have good measurement sensitivity to small changes in reflectivity (material properties) and light scatter (roughness). A new angular resolved scatterometer is described that has an extended dynamic range and integrated analysis capable of displaying the surface power spectral density (PSD) over large bandwidths of surface spatial frequencies. Graphical displays of the scattered light power before and after exposure to the radiation are compared and integrated over equivalent spatial bandwidths of sensitivity for other instruments to compare calculated RMS roughness values

  6. Angular and mass resolved energy distribution measurements with a gallium liquid metal ion source

    International Nuclear Information System (INIS)

    Marriott, Philip

    1987-06-01

    Ionisation and energy broadening mechanisms relevant to liquid metal ion sources are discussed. A review of experimental results giving a picture of source operation and a discussion of the emission mechanisms thought to occur for the ionic species and droplets emitted is presented. Further work is suggested by this review and an analysis system for angular and mass resolved energy distribution measurements of liquid metal ion source beams has been constructed. The energy analyser has been calibrated and a series of measurements, both on and off the beam axis, of 69 Ga + , Ga ++ and Ga 2 + ions emitted at various currents from a gallium source has been performed. A comparison is made between these results and published work where possible, and the results are discussed with the aim of determining the emission and energy spread mechanisms operating in the gallium liquid metal ion source. (author)

  7. Tuning across the BCS-BEC crossover in the multiband superconductor Fe1+ySe x Te1-x: An angle-resolved photoemission study.

    Science.gov (United States)

    Rinott, Shahar; Chashka, K B; Ribak, Amit; Rienks, Emile D L; Taleb-Ibrahimi, Amina; Le Fevre, Patrick; Bertran, François; Randeria, Mohit; Kanigel, Amit

    2017-04-01

    The crossover from Bardeen-Cooper-Schrieffer (BCS) superconductivity to Bose-Einstein condensation (BEC) is difficult to realize in quantum materials because, unlike in ultracold atoms, one cannot tune the pairing interaction. We realize the BCS-BEC crossover in a nearly compensated semimetal, Fe 1+ y Se x Te 1- x , by tuning the Fermi energy ε F via chemical doping, which permits us to systematically change Δ/ε F from 0.16 to 0.50, where Δ is the superconducting (SC) gap. We use angle-resolved photoemission spectroscopy to measure the Fermi energy, the SC gap, and characteristic changes in the SC state electronic dispersion as the system evolves from a BCS to a BEC regime. Our results raise important questions about the crossover in multiband superconductors, which go beyond those addressed in the context of cold atoms.

  8. Bulk electronic structure of superconducting LaRu2P2 single crystals measured by soft-X-ray angle-resolved photoemission spectroscopy.

    Science.gov (United States)

    Razzoli, E; Kobayashi, M; Strocov, V N; Delley, B; Bukowski, Z; Karpinski, J; Plumb, N C; Radovic, M; Chang, J; Schmitt, T; Patthey, L; Mesot, J; Shi, M

    2012-06-22

    We present a soft x-ray angle-resolved photoemission spectroscopy (SX-ARPES) study of the stoichiometric pnictide superconductor LaRu(2)P(2). The observed electronic structure is in good agreement with density functional theory (DFT) calculations. However, it is significantly different from its counterpart in high-temperature superconducting Fe pnictides. In particular, the bandwidth renormalization present in the Fe pnictides (~2-3) is negligible in LaRu(2)P(2) even though the mass enhancement is similar in both systems. Our results suggest that the superconductivity in LaRu(2) P(2) has a different origin with respect to the iron pnictides. Finally, we demonstrate that the increased probing depth of SX-ARPES, compared to the widely used ultraviolet ARPES, is essential in determining the bulk electronic structure in the experiment.

  9. Multiple Nodeless Superconducting Gaps in (Ba0.6K0.4)Fe2As2 Superconductor from Angle-Resolved Photoemission Spectroscopy

    International Nuclear Information System (INIS)

    Lin, Zhao; Hai-Yun, Liu; Wen-Tao, Zhang; Jian-Qiao, Meng; Xiao-Wen, Jia; Guo-Dong, Liu; Xiao-Li, Dong; Wei, Lu; Xing-Jiang, Zhou; Gen-Fu, Chen; Jian-Lin, Luo; Nan-Lin, Wang; Gui-Ling, Wang; Yong, Zhou; Zu-Yan, Xu; Yong, Zhu; Xiao-Yang, Wang; Chuang-Tian, Chen

    2008-01-01

    High resolution angle-resolved photoemission measurements have been carried out to study the superconducting gap in the (Ba 0.6 K 0.4 )Fe 2 As 2 superconductor with T e = 35 K. Two hole-like Fermi surface sheets around the I' point exhibit different superconducting gaps. The inner Fermi surface sheet shows larger (10 ∼ 12 meV) and slightly momentum-dependent gap while the outer one has smaller (7 ∼ 8meV) and nearly isotropic gap. The lack of gap node in both Fermi surface sheets favours s-wave superconducting gap symmetry. Superconducting gap opening is also observed at the M(π, π) point. The two Fermi surface spots near the M point are gapped below T e but the gap persists above T e. The rich and detailed superconducting gap information will provide key insights and constraints in understanding pairing mechanism in the iron-based superconductors

  10. Exploring the Electronic Structure and Chemical Homogeneity of Individual Bi2Te3 Nanowires by Nano-Angle-Resolved Photoemission Spectroscopy.

    Science.gov (United States)

    Krieg, Janina; Chen, Chaoyu; Avila, José; Zhang, Zeying; Sigle, Wilfried; Zhang, Hongbin; Trautmann, Christina; Asensio, Maria Carmen; Toimil-Molares, Maria Eugenia

    2016-07-13

    Due to their high surface-to-volume ratio, cylindrical Bi2Te3 nanowires are employed as model systems to investigate the chemistry and the unique conductive surface states of topological insulator nanomaterials. We report on nanoangle-resolved photoemission spectroscopy (nano-ARPES) characterization of individual cylindrical Bi2Te3 nanowires with a diameter of 100 nm. The nanowires are synthesized by electrochemical deposition inside channels of ion-track etched polymer membranes. Core level spectra recorded with submicron resolution indicate a homogeneous chemical composition along individual nanowires, while nano-ARPES intensity maps reveal the valence band structure at the single nanowire level. First-principles electronic structure calculations for chosen crystallographic orientations are in good agreement with those revealed by nano-ARPES. The successful application of nano-ARPES on single one-dimensional nanostructures constitutes a new avenue to achieve a better understanding of the electronic structure of topological insulator nanomaterials.

  11. Topological events in polarization resolved angular patterns of nematic liquid crystal cells at varying ellipticity of incident wave

    OpenAIRE

    Kiselev, Alexei D.; Vovk, Roman G.

    2008-01-01

    We study the angular structure of polarization of light transmitted through a nematic liquid crystal (NLC) cell by analyzing the polarization state as a function of the incidence angles and the polarization of the incident wave. The polarization resolved angular patterns emerging after the NLC cell illuminated by the convergent light beam are described in terms of the polarization singularities such as C-points (points of circular polarization) and L-lines (lines of linear polarization). For ...

  12. Photoemission and ferromagnetism

    International Nuclear Information System (INIS)

    Johnson, P.D.

    1994-01-01

    Photoemission is a well established technique for the study of the electronic structure of atoms and solids. In particular, angle-resolved photoemission has been used extensively to map the band structure of clean and adsorbate covered surfaces, both metal and semiconductor. Extending the technique by measuring the spin of the photoemitted electrons allows the possibility of examining the exchange split band structures characterizing ferromagnetic systems. Here the technique becomes particularly useful in the study of the magnetic properties of surfaces, thin films and associated interfaces

  13. Time- and energy resolved photoemission electron microscopy-imaging of photoelectron time-of-flight analysis by means of pulsed excitations

    International Nuclear Information System (INIS)

    Oelsner, Andreas; Rohmer, Martin; Schneider, Christian; Bayer, Daniela; Schoenhense, Gerd; Aeschlimann, Martin

    2010-01-01

    The present work enlightens the developments in time- and energy resolved photoemission electron microscopy over the past few years. We describe basic principles of the technique and demonstrate different applications. An energy- and time-filtering photoemission electron microscopy (PEEM) for real-time spectroscopic imaging can be realized either by a retarding field or hemispherical energy analyzer or by using time-of-flight optics with a delay line detector. The latter method has the advantage of no data loss at all as all randomly incoming particles are measured not only by position but also by time. This is of particular interest for pump-probe experiments in the femtosecond and attosecond time scale where space charge processes drastically limit the maximum number of photoemitted electrons per laser pulse. This work focuses particularly on time-of-flight analysis using a novel delay line detector. Time and energy resolved PEEM instruments with delay line detectors enable 4D imaging (x, y, Δt, E Kin ) on a true counting basis. This allows a broad range of applications from real-time observation of dynamic phenomena at surfaces to fs time-of-flight spectro-microscopy and even aberration correction. By now, these time-of-flight analysis instruments achieve intrinsic time resolutions of 108 ps absolute and 13.5 ps relative. Very high permanent measurement speeds of more than 4 million events per second in random detection regimes have been realized using a standard USB2.0 interface. By means of this performance, the time-resolved PEEM technique enables to display evolutions of spatially resolved (<25 nm) and temporal sliced images life on any modern computer. The method allows dynamics investigations of variable electrical, magnetic, and optical near fields at surfaces and great prospects in dynamical adaptive photoelectron optics. For dynamical processes in the ps time scale such as magnetic domain wall movements, the time resolution of the delay line detectors

  14. Multiple π-bands and Bernal stacking of multilayer graphene on C-face SiC, revealed by nano-Angle Resolved Photoemission.

    Science.gov (United States)

    Johansson, Leif I; Armiento, Rickard; Avila, Jose; Xia, Chao; Lorcy, Stephan; Abrikosov, Igor A; Asensio, Maria C; Virojanadara, Chariya

    2014-02-24

    Only a single linearly dispersing π-band cone, characteristic of monolayer graphene, has so far been observed in Angle Resolved Photoemission (ARPES) experiments on multilayer graphene grown on C-face SiC. A rotational disorder that effectively decouples adjacent layers has been suggested to explain this. However, the coexistence of μm-sized grains of single and multilayer graphene with different azimuthal orientations and no rotational disorder within the grains was recently revealed for C-face graphene, but conventional ARPES still resolved only a single π-band. Here we report detailed nano-ARPES band mappings of individual graphene grains that unambiguously show that multilayer C-face graphene exhibits multiple π-bands. The band dispersions obtained close to the K-point moreover clearly indicate, when compared to theoretical band dispersion calculated in the framework of the density functional method, Bernal (AB) stacking within the grains. Thus, contrary to earlier claims, our findings imply a similar interaction between graphene layers on C-face and Si-face SiC.

  15. Energy-resolved photoemission studies of Be-containing surfaces for fusion; Energievariierte Photoemissionsstudien an berylliumhaltigen Oberflaechen fuer die Fusion

    Energy Technology Data Exchange (ETDEWEB)

    Koeppen, Martin

    2013-02-04

    Fusion research aims at the exploitation of the deuterium-tritium reaction for energy production. Next step on the roadmap is the construction of the experimental reactor ITER. The three elements beryllium, carbon and tungsten are to be used as armour materials for the vacuum vessel. After erosion due to plasma processes, these materials are transported and redeposited together with plasma impurities like oxygen from surface oxides. This leads to the formation of compounds by chemical reactions and diffusive processes, induced both by elevated temperatures and implantation of energetic particles. Due to the complexity of the induced surface processes, a method is required which is capable of both qualitative and quantitative analysis of the involved chemical species. X-ray photoelectron spectroscopy (XPS) provides the chemical analysis. Since diffusive processes play an important role in solid-state reactions, a depth-resolved method is required. In this work, energy-resolved XPS using synchrotron radiation with variable photon energies is extended towards a quantitative depth-resolved analysis. For the quantitative analysis a new model is derived which calculates the depth-resolved composition and the respective composition-dependent electron inelastic mean free path in a self-consistent way. Input is the XPS data which is normalized with all parameters influencing the photoelectron intensities. This fully quantitative model is applied to describe the interaction of energetic oxygen ions with the beryllium-tungsten alloy Be{sub 2}W. Oxygen ions from the plasma are able to interact with plasma facing materials. Formation of Be{sub 2}W is to be expected at the first wall and in the divertor region of ITER. Irradiation of this alloy leads to its decompositions. After decomposition, formation of beryllium oxide BeO is preferred compared to formation of tungsten oxides. Heating to 600K leads to chemical reduction of tungsten oxides. Metallic Be acts as reduction agent

  16. Angle-resolved photoemission spectroscopy for VO{sub 2} thin films grown on TiO{sub 2} (0 0 1) substrates

    Energy Technology Data Exchange (ETDEWEB)

    Muraoka, Y., E-mail: ymuraoka@cc.okayama-u.ac.j [Graduate School of Natural Science and Technology, Okayama University, 3-1-1 Tsushima-naka, Kita-ku, Okayama 700-8530 (Japan); Faculty of Science, Research Laboratory for Surface Science, Okayama University, 3-1-1 Tsushima-naka, Kita-ku, Okayama 700-8530 (Japan); Saeki, K.; Yao, Y. [Graduate School of Natural Science and Technology, Okayama University, 3-1-1 Tsushima-naka, Kita-ku, Okayama 700-8530 (Japan); Wakita, T. [Faculty of Science, Research Laboratory for Surface Science, Okayama University, 3-1-1 Tsushima-naka, Kita-ku, Okayama 700-8530 (Japan); Hirai, M.; Yokoya, T. [Graduate School of Natural Science and Technology, Okayama University, 3-1-1 Tsushima-naka, Kita-ku, Okayama 700-8530 (Japan); Faculty of Science, Research Laboratory for Surface Science, Okayama University, 3-1-1 Tsushima-naka, Kita-ku, Okayama 700-8530 (Japan); Eguchi, R.; Shin, S. [RIKEN/SPring-8, 1-1-1 Kouto, Sayo, Hyogo 679-5148 (Japan)

    2010-08-15

    We present the results of angle-resolved photoemission spectroscopy (ARPES) measurements of metallic VO{sub 2} thin films. The VO{sub 2} thin films have been grown on TiO{sub 2} (0 0 1) single crystal substrates using pulsed laser deposition. The films exhibit a first-order metal-insulator transition (MIT) at 305 K. In the ARPES spectra of the metallic phase for the films, the O 2p band shows highly dispersive feature in the binding energy range of 3-8 eV along the {Gamma}-Z direction. The periodicity of the dispersive band is found to be 2.2 A{sup -1} which is almost identical with the periodicity expected from the c-axis length of the VO{sub 2} thin films. The overall feature of the experimental band structure is similar to the band structure calculations, supporting that we have succeeded in observing the dispersive band of the O 2p state in the metallic VO{sub 2} thin film. The present work indicates that the ARPES measurements using epitaxial thin films are promising for determining the band structure of VO{sub 2}.

  17. Si(111)-sq root 21 x sq root 21 -(Ag+Cs) surface studied by scanning tunneling microscopy and angle-resolved photoemission spectroscopy

    CERN Document Server

    Liu, C; Morikawa, H; Okino, H; Hasegawa, S; Okuda, T; Kinoshita, T

    2003-01-01

    Scanning tunneling microscopy (STM) and angle-resolved photoemission spectroscopy (ARPES) were used to study the atomic and electronic structures of the Si(111)-sq root 21 x sq root 21-(Ag + Cs) surface (sq root 21-Cs in short), which was induced by depositing caesium atoms on the Si(111)-sq root 3 x sq root 3-Ag surface at room temperature (RT). Compared with previously reported STM images of noble-metal induced sq root 21 x sq root 21 phases including the Si(111)-sq root 21 x sq root 21-(Ag+Ag) and Si(111)-sq root 21 x sq root 21-(Ag+Au) surfaces (sq root 21-Ag and sq root 21-Au, respectively), the sq root 21-Cs surface displayed quite different features in STM images. The ARPES data of the sq root 21-Cs surface revealed an intrinsic dispersive surface-state band, together with a non-dispersive one near the Fermi level, which was also different from those of the sq root 21-Ag and sq root 21-Au surfaces. These results strongly suggest different atomic arrangements between Cs- and noble-metal induced sq root ...

  18. High-resolution angle-resolved photoemission studies of high Tc superconductor Bi2Sr2CaCu2O8

    International Nuclear Information System (INIS)

    Liu, Rong.

    1990-01-01

    An angle-resolved photoemission study of the normal and superconducting states in Bi 2 Sr 2 CaCu 2 O 8 was performed. Measurements in the normal state show bands dispersing through the Fermi level from at least 350 meV below E F . The Fermi level crossings are consistant with local-density band calculation, including a point calculated to be of Bi-O character. Additional measurements were made where bands crossed the Fermi level between 100 and 250K, along with measurements on an adjacent Pt foil. The Fermi edges of both materials agree to within the noise. Below the Fermi level, the spectra show correlation effects on the form of an increased effective mass. The shape of the spectra can be explained by a lifetime-broadened photohole and secondary electrons. The effective inverse photohole lifetime is linear in energy. A superconducting gap has been measured at a number of points where there is density at the Fermi level in the normal state. By proper modeling, a gap of 24 meV was obtained for all these points, including points of Cu-O and Bi-O character respectively, according to band calculation. The lack of gap anisotropy in the basal plane suggests that pinning in this material is not d-wave pairing

  19. Electronic Structure of Epitaxial Thin Films of the Transparent Conducting Oxide La:BaSnO3 Measured By In-Situ Angle-Resolved Photoemission Spectroscopy

    Science.gov (United States)

    Lochocki, Edward; Paik, Hanjong; Uchida, Masaki; Schlom, Darrell; Shen, Kyle

    Lanthanum-doped barium stannate (La:BaSnO3) is a transparent conducting oxide where single crystals have exhibited unusually high mobility and oxygen stability. Here we present in-situ angle-resolved photoemission (ARPES) measurements of La:BaSnO3 epitaxial films that were co-deposited onto lattice-matched rare-earth scandate substrates by molecular-beam epitaxy (MBE). Density functional theory (DFT) calculations agree well with the observed valence bands and predict a parabolic conduction band. However, the features observed near the Fermi energy (EF) are non-dispersive yet localized in momentum space. This unusual appearance may be the result of quasi-localized charge carriers or out-of-plane momentum broadening. Over long measurement periods, we also observe changes to the valence band and near-EF feature that bear a strong resemblance to the beam-induced two-dimensional electron gases previously reported in SrTiO3 and KTaO3. The origin of these unexpected phenomena and their relationship to the structural and transport properties of these films will be discussed.

  20. Orbital character and electron correlation effects on two- and three-dimensional Fermi surfaces in KFe2As2 revealed by angle-resolved photoemission spectroscopy

    Directory of Open Access Journals (Sweden)

    Teppei eYoshida

    2014-04-01

    Full Text Available We have investigated orbital character and electron correlation effects on Fermi surfaces in the hole-overdoped iron pnictide superconductor KFe2As2, which shows a low Tc of ~4 K, by angle-resolved photoemission spectroscopy. From the polarization-dependence of the ARPES spectra, we have determined the orbital character of each Fermi surface. Electron mass renormalization of each band is quantitatively consistent with de Haas-van Alphen results. The outer beta and middle zeta Fermi surfaces show large renormalization factor of m*/mb ~6-7, while the inner Fermi surface has a smaller factor m*/mb ~2. Middle hole Fermi surface zeta has strong three-dimensionality compared to other Fermi surfaces, indicating the d3z2-r2 orbital character, which may be related to the octet-line nodes recently observed by laser ARPES. The observed orbital-dependent mass renormalization would give constraints on the pairing mechanism with line nodes of this system.

  1. Electronic structure and polar catastrophe at the surface of LixCoO2 studied by angle-resolved photoemission spectroscopy

    Science.gov (United States)

    Okamoto, Y.; Matsumoto, R.; Yagihara, T.; Iwai, C.; Miyoshi, K.; Takeuchi, J.; Horiba, K.; Kobayashi, M.; Ono, K.; Kumigashira, H.; Saini, N. L.; Mizokawa, T.

    2017-09-01

    We report an angle-resolved photoemission spectroscopy (ARPES) study of LixCoO2 single crystals which have a hole-doped CoO2 triangular lattice. Similar to NaxCoO2 , the Co 3 d a1 g band crosses the Fermi level with strongly renormalized band dispersion while the Co 3 d eg' bands are fully occupied in LixCoO2 (x =0.46 and 0.71). At x =0.46 , the Fermi surface area is consistent with the bulk hole concentration indicating that the ARPES result represents the bulk electronic structure. On the other hand, at x =0.71 , the Fermi surface area is larger than the expectation which can be associated with the inhomogeneous distribution of Li reported in the previous scanning tunneling microscopy study by Iwaya et al. [Phys. Rev. Lett. 111, 126104 (2013), 10.1103/PhysRevLett.111.126104]. However, the Co 3 d peak is systematically shifted towards the Fermi level with hole doping excluding phase separation between hole rich and hole poor regions in the bulk. Therefore, the deviation of the Fermi surface area at x =0.71 can be attributed to hole redistribution at the surface avoiding polar catastrophe. The bulk Fermi surface of Co 3 d a1 g is very robust around x =0.5 even in the topmost CoO2 layer due to the absence of the polar catastrophe.

  2. Site-specific intermolecular valence-band dispersion in α-phase crystalline films of cobalt phthalocyanine studied by angle-resolved photoemission spectroscopy.

    Science.gov (United States)

    Yamane, Hiroyuki; Kosugi, Nobuhiro

    2014-12-14

    The valence band structure of α-phase crystalline films of cobalt phthalocyanine (CoPc) grown on Au(111) is investigated by using angle-resolved photoemission spectroscopy (ARPES) with synchrotron radiation. The photo-induced change in the ARPES peaks is noticed in shape and energy of the highest occupied molecular orbital (HOMO, C 2p) and HOMO-1 (Co 3d) of CoPc, and is misleading the interpretation of the electronic properties of CoPc films. From the damage-free normal-emission ARPES measurement, the clear valence-band dispersion has been first observed, showing that orbital-specific behaviors are attributable to the interplay of the intermolecular π-π and π-d interactions. The HOMO band dispersion of 0.1 eV gives the lower limit of the hole mobility for α-CoPc of 28.9 cm(2) V(-1) s(-1) at 15 K. The non-dispersive character of the split HOMO-1 bands indicates that the localization of the spin state is a possible origin of the antiferromagnetism.

  3. Quantum Transport and Nano Angle-resolved Photoemission Spectroscopy on the Topological Surface States of Single Sb2Te3 Nanowires

    Science.gov (United States)

    Arango, Yulieth C.; Huang, Liubing; Chen, Chaoyu; Avila, Jose; Asensio, Maria C.; Grützmacher, Detlev; Lüth, Hans; Lu, Jia Grace; Schäpers, Thomas

    2016-01-01

    We report on low-temperature transport and electronic band structure of p-type Sb2Te3 nanowires, grown by chemical vapor deposition. Magnetoresistance measurements unravel quantum interference phenomena, which depend on the cross-sectional dimensions of the nanowires. The observation of periodic Aharonov-Bohm-type oscillations is attributed to transport in topologically protected surface states in the Sb2Te3 nanowires. The study of universal conductance fluctuations demonstrates coherent transport along the Aharonov-Bohm paths encircling the rectangular cross-section of the nanowires. We use nanoscale angle-resolved photoemission spectroscopy on single nanowires (nano-ARPES) to provide direct experimental evidence on the nontrivial topological character of those surface states. The compiled study of the bandstructure and the magnetotransport response unambiguosly points out the presence of topologically protected surface states in the nanowires and their substantial contribution to the quantum transport effects, as well as the hole doping and Fermi velocity among other key issues. The results are consistent with the theoretical description of quantum transport in intrinsically doped quasi-one-dimensional topological insulator nanowires. PMID:27581169

  4. Adsorption site and structure determination of c(2x2) N{sub 2}/Ni(100) using angle-resolved photoemission extended fine structure

    Energy Technology Data Exchange (ETDEWEB)

    Moler, E.J.; Kellar, S.A.; Huff, W.R.A. [Lawrence Berkeley National Lab., CA (United States)] [and others

    1997-04-01

    The authors have determined the atomic spatial structure of c(2x2) N2Ni(100) with Angle-Resolved Photoemission Extended Fine Structure (ARPEFS) from the nitrogen 1s core level using monochromatized x-rays from beamline 6.1 at SSRL and beamline 9.3.2 at the ALS. The chemically shifted N 1s peak intensities were summed together to obtain ARPEFS curves for both nitrogen atoms in the molecule. They used a new, highly-optimized program based on the Rehr-Albers scattering matrix formalism to find the adsorption site and to quantitatively determine the bond-lengths. The nitrogen molecule stands upright at an atop site, with a N-Ni bond length of 2.25(1) {angstrom}, a N-N bond length of 1.10(7) {angstrom}, and a first layer Ni-Ni spacing of 1.76(4) {angstrom}. The shake-up peak shows an identical ARPEFS diffraction pattern, confirming its intrinsic nature and supporting a previous use of this feature to decompose the peak into contributions from the chemically inequivalent nitrogen atoms. Comparison to a previously published theoretical treatment of N-N-Ni and experimental structures of analogous adsorbate systems demonstrates the importance of adsorbate-adsorbate interactions in weakly chemisorbed systems.

  5. Exploring electronic structure of one-atom thick polycrystalline graphene films: A nano angle resolved photoemission study

    Science.gov (United States)

    Avila, José; Razado, Ivy; Lorcy, Stéphane; Fleurier, Romain; Pichonat, Emmanuelle; Vignaud, Dominique; Wallart, Xavier; Asensio, María C.

    2013-01-01

    The ability to produce large, continuous and defect free films of graphene is presently a major challenge for multiple applications. Even though the scalability of graphene films is closely associated to a manifest polycrystalline character, only a few numbers of experiments have explored so far the electronic structure down to single graphene grains. Here we report a high resolution angle and lateral resolved photoelectron spectroscopy (nano-ARPES) study of one-atom thick graphene films on thin copper foils synthesized by chemical vapor deposition. Our results show the robustness of the Dirac relativistic-like electronic spectrum as a function of the size, shape and orientation of the single-crystal pristine grains in the graphene films investigated. Moreover, by mapping grain by grain the electronic dynamics of this unique Dirac system, we show that the single-grain gap-size is 80% smaller than the multi-grain gap recently reported by classical ARPES. PMID:23942471

  6. Characterization of the α-SN/CDTE(110) interface by angle-resolved X-ray photoemission

    International Nuclear Information System (INIS)

    Lin, T.S.; Partin, W.J.; Chung, Y.W.

    1987-01-01

    Stoichiometric and atomically clean CdTe(110) surfaces have been prepared by suitable chemical etching, followed by argon sputtering, and sample annealing in ultra-high vacuum. Cubic (α) -tin was grown on CdTe(110) by tin evaporation from a tungsten filament at a substrate temperature of 30 0 C. Angle-resolved X-ray photoelectron spectroscopy (ARXPS) was used to determine the α-Sn growth mechanism and the composition profile of this semiconductor heterostructure nondestructively. From their analyses, the authors conclude that α-Sn grows on CdTe(110) at 30 0 C by a layer by layer mechanism and forms an abrupt junction with CdTe(110)

  7. A study of angle-resolved photoemission extended fine structure as applied to the Ni 3p, Cu 3s, and Cu 3p core levels of the respective clean (111) surfaces

    Energy Technology Data Exchange (ETDEWEB)

    Huff, W.R.A.; Moler, E.J.; Kellar, S.A. [Lawrence Berkeley National Lab., CA (United States)] [and others

    1997-04-01

    The first non-s initial state angle-resolved photoemission extended fine structure (ARPEFS) study of clean surfaces for the purpose of further understanding the technique is reported. The surface structure sensitivity of ARPEFS applied to clean surfaces and to arbitrary initial states is studied using normal photoemission data taken from the Ni 3p core levels of a Ni(111) single crystal and the Cu 3s and the Cu 3p core-levels of a Cu(111) single crystal. The Fourier transforms of these clean surface data are dominated by backscattering. Unlike the s initial state data, the p initial state data show a peak in the Fourier transform corresponding to in-plane scattering from the six nearest-neighbors to the emitter. Evidence was seen for single-scattering events from in the same plane as the emitters and double-scattering events. Using a newly developed, multiple-scattering calculation program, ARPEFS data from clean surfaces and from p initial states can be modeled to high precision. Although there are many layers of emitters when measuring photoemission from a clean surface, test calculations show that the ARPEFS signal is dominated by photoemission from atoms in the first two crystal layers. Thus, ARPEFS applied to clean surfaces is sensitive to surface reconstruction. The known contraction of the first two Cu(111) layers is confirmed. The best-fit calculation for clean Ni(111) indicates an expansion of the first two layers. To better understand the ARPEFS technique, the authors studied s and non-s initial state photoemission from clean metal surfaces.

  8. Time-resolved two-photon photoemission at the Si(001)-surface. Hot electron dynamics and two-dimensional Fano resonance; Zeitaufgeloeste Zweiphotonen-Photoemission an der Si(001)-Oberflaeche. Dynamik heisser Elektronen und zweidimensionaler Fano-Effekt

    Energy Technology Data Exchange (ETDEWEB)

    Eickhoff, Christian

    2010-10-27

    By combining ultrafast laser excitation with energy-, angle- and time-resolved twophoton photoemission (2PPE), the electronic properties of bulk silicon and the Si(001) surface are investigated in this thesis. A custom-built laser- and UHV-systemequipped with a display type 2D-CCD-detector gives new insight into the relaxation dynamics of excited carriers on a femtosecond timescale. The bandgap between occupied valence bands and unoccupied conduction bands characteristically influences the dynamics of excited electrons in the bulk, as well as in surface states and resonances. For the electron-phonon interaction this leads to the formation of a bottleneck during the relaxation of hot electrons in the conduction band, which maintains the elevated electronic temperature for several picoseconds. During relaxation, excited electrons also scatter from the conduction band into the unoccupied dangling-bond surface state D{sub down}. Depending on the excitation density this surface recombination is dominated by electron-electron- or electron-phonon scattering. The relaxation of the carriers in the D{sub down}-band is again slowed down by the formation of a bottleneck in electron-phonon coupling. Furthermore, the new laser system has allowed detection of the Rydberg-like series of image-potential resonances on the Si(001)-surface. It is shown that the lifetime of these image-potential resonances in front of the semiconducting surface exhibits the same behavior as those in front of metallic surfaces. Moreover the electron-phonon coupling in the first image-potential resonance was investigated and compared to the D{sub down}-surface state. For the first time, Fano-type lineprofiles are demonstrated and analyzed in a 2PPEprocess on a surface. Tuning the photon energy of the pump-laser across the resonance between the occupied dangling-bond state D{sub up}, and the unoccupied image-potential resonance n=1, reveals a clear intensity variation that can be successfully described

  9. Polarization-resolved angular patterns of nematic liquid crystal cells: Topological events driven by incident light polarization

    Science.gov (United States)

    Kiselev, Alexei D.; Vovk, Roman G.; Egorov, Roman I.; Chigrinov, Vladimir G.

    2008-09-01

    We study the angular structure of polarization of light transmitted through a nematic liquid crystal (NLC) cell by analyzing the polarization state as a function of the incidence angles and the polarization of the incident wave. The polarization-resolved angular (conoscopic) patterns emerging after the NLC cell illuminated by the convergent light beam are described in terms of the polarization singularities such as C points (points of circular polarization) and L lines (lines of linear polarization). For the homeotropically aligned cell, the Stokes polarimetry technique is used to measure the polarization resolved conoscopic patterns at different values of the ellipticity of the incident light, γell(inc) , impinging onto the cell. Using the exact analytical expressions for the transfer matrix we show that variations of the ellipticity, γell(inc) , induce transformations of the angular pattern exhibiting the effect of avoided L -line crossings and characterized by topological events such as creation and annihilation of the C points. The predictions of the theory are found to be in good agreement with the experimental results.

  10. Angular resolved scattering by a nano-textured ZnO/silicon interface

    NARCIS (Netherlands)

    Schulte, M.; Bittkau, K.; Jäger, K.; Ermes, M.; Zeman, M.; Pieters, B.E.

    2011-01-01

    Textured interfaces in thin-film silicon solar cells improve the efficiency by light scattering. A technique to get experimental access to the angular intensity distribution (AID) at textured interfaces of the transparent conductive oxide (TCO) and silicon is introduced. Measurements are performed

  11. A scintillator-based online detector for the angularly resolved measurement of laser-accelerated proton spectra.

    Science.gov (United States)

    Metzkes, J; Karsch, L; Kraft, S D; Pawelke, J; Richter, C; Schürer, M; Sobiella, M; Stiller, N; Zeil, K; Schramm, U

    2012-12-01

    In recent years, a new generation of high repetition rate (~10 Hz), high power (~100 TW) laser systems has stimulated intense research on laser-driven sources for fast protons. Considering experimental instrumentation, this development requires online diagnostics for protons to be added to the established offline detection tools such as solid state track detectors or radiochromic films. In this article, we present the design and characterization of a scintillator-based online detector that gives access to the angularly resolved proton distribution along one spatial dimension and resolves 10 different proton energy ranges. Conceived as an online detector for key parameters in laser-proton acceleration, such as the maximum proton energy and the angular distribution, the detector features a spatial resolution of ~1.3 mm and a spectral resolution better than 1.5 MeV for a maximum proton energy above 12 MeV in the current design. Regarding its areas of application, we consider the detector a useful complement to radiochromic films and Thomson parabola spectrometers, capable to give immediate feedback on the experimental performance. The detector was characterized at an electrostatic Van de Graaff tandetron accelerator and tested in a laser-proton acceleration experiment, proving its suitability as a diagnostic device for laser-accelerated protons.

  12. Strong electron correlations in the normal state of the iron-based FeSe0.42Te0.58 superconductor observed by angle-resolved photoemission spectroscopy.

    Science.gov (United States)

    Tamai, A; Ganin, A Y; Rozbicki, E; Bacsa, J; Meevasana, W; King, P D C; Caffio, M; Schaub, R; Margadonna, S; Prassides, K; Rosseinsky, M J; Baumberger, F

    2010-03-05

    We investigate the normal state of the "11" iron-based superconductor FeSe0.42Te0.58 by angle-resolved photoemission. Our data reveal a highly renormalized quasiparticle dispersion characteristic of a strongly correlated metal. We find sheet dependent effective carrier masses between approximately 3 and 16m{e} corresponding to a mass enhancement over band structure values of m{*}/m{band} approximately 6-20. This is nearly an order of magnitude higher than the renormalization reported previously for iron-arsenide superconductors of the "1111" and "122" families but fully consistent with the bulk specific heat.

  13. Time-Resolved Photoelectron Angular Distributions from Strong-Field Ionization of Rotating Naphthalene Molecules

    DEFF Research Database (Denmark)

    Hansen, Jonas Lerche; Stapelfeldt, Henrik; Dimitrovski, Darko

    2011-01-01

    A nanosecond laser pulse confines the spatial orientation of naphthalene in 1D or 3D while a femtosecond kick pulse initiates rotation of the molecular plane around the fixed long axis. Time-dependent photoelectron angular distributions (PADs), resulting from ionization by an intense femtosecond...... probe pulse, exhibit pronounced changes as the molecular plane rotates. Enhanced 3D alignment, occurring shortly after the kick pulse, provides strongly improved contrast in molecular-frame PADs. Calculations in the strong-field approximation show that the striking structures observed in the PADs...

  14. Automated angle-scanning photoemission end-station with molecular beam epitaxy at KEK-PF BL-1C

    CERN Document Server

    Ono, K; Horiba, K; Oh, J H; Nakazono, S; Kihara, T; Nakamura, K; Mano, T; Mizuguchi, M; Oshima, M; Aiura, Y; Kakizaki, A

    2001-01-01

    In order to satisfy demands to study the electronic structure of quantum nanostructures, a VUV beamline and a high-resolution and high-throughput photoemission end-station combined with a molecular beam epitaxy (MBE) system have been constructed at the BL-1C of the Photon Factory. An angle-resolved photoemission spectrometer, having high energy- and angular-resolutions; VG Microtech ARUPS10, was installed. The total energy resolution of 31 meV at the 60 eV of photon energy is achieved. For the automated angle-scanning photoemission, the electron spectrometer mounted on a two-axis goniometer can be rotated in vacuum by the computer-controlled stepping motors. Another distinctive feature of this end-station is a connection to a MBE chamber in ultahigh vacuum (UHV). In this system, MBE-grown samples can be transferred into the photoemission chamber without breaking UHV. Photoemission spectra of MBE-grown GaAs(0 0 1) surfaces were measured with high-resolution and bulk and surface components are clearly resolved.

  15. Angle Resolved Photoemission Spectroscopy Studies of the Mott Insulator to Superconductor Evolution in Ca2-xNaxCuO2Cl2

    Energy Technology Data Exchange (ETDEWEB)

    Shen, Kyle Michael

    2005-09-02

    It is widely believed that many of the exotic physical properties of the high-T{sub c} cuprate superconductors arise from the proximity of these materials to the strongly correlated, antiferromagnetic Mott insulating state. Therefore, one of the fundamental questions in the field of high-temperature superconductivity is to understand the insulator-to-superconductor transition and precisely how the electronic structure of Mott insulator evolves as the first holes are doped into the system. This dissertation presents high-resolution, doping dependent angle-resolved photoemission (ARPES) studies of the cuprate superconductor Ca{sub 2-x}Na{sub x}CuO{sub 2}Cl{sub 2}, spanning from the undoped parent Mott insulator to a high-temperature superconductor with a T{sub c} of 22 K. A phenomenological model is proposed to explain how the spectral lineshape, the quasiparticle band dispersion, and the chemical potential all progress with doping in a logical and self-consistent framework. This model is based on Franck-Condon broadening observed in polaronic systems where strong electron-boson interactions cause the quasiparticle residue, Z, to be vanishingly small. Comparisons of the low-lying states to different electronic states in the valence band strongly suggest that the coupling of the photohole to the lattice (i.e. lattice polaron formation) is the dominant broadening mechanism for the lower Hubbard band states. Combining this polaronic framework with high-resolution ARPES measurements finally provides a resolution to the long-standing controversy over the behavior of the chemical potential in the high-T{sub c} cuprates. This scenario arises from replacing the conventional Fermi liquid quasiparticle interpretation of the features in the Mott insulator by a Franck-Condon model, allowing the reassignment of the position of the quasiparticle pole. As a function of hole doping, the chemical potential shifts smoothly into the valence band while spectral weight is transferred

  16. Spectrally and angularly resolved measurements of three-halves harmonic emission from laser-produced plasmas

    Science.gov (United States)

    Kang, N.; Liu, H.; Lin, Z.; Lei, A.; Zhou, S.; Fang, Z.; An, H.; Li, K.; Fan, W.

    2017-10-01

    Spectra of three-halves harmonic emissions (3{ω }0/2) from laser-produced plasmas were measured at different angles, including both forward and backward sides, from the direction of incident laser beams. The 3{ω }0/2 emitted from carbon-hydrogen (CH) targets was observed to be larger than that from aluminum (Al) targets with the same incident laser intensity, which supports the argument that the two-plasmon decay (TPD) instability could be inhibited by using medium-Z ablator instead of CH ablator in direct-drive inertial confinement fusion. Besides, the measured 3{ω }0/2-incident intensity curves for both materials suggest relatively lower threshold of TPD than the calculated values. In experiments with thin Al targets, the angular distribution of the blue- and red-shifted peaks of 3{ω }0/2 spectra were obtained, which shows that the most intense blue- and red-shifted peaks may not be produced in paired plasmons, but the spectra produced by their ‘twin’ plasmons were not observed. Because 3{ω }0/2 may have been influenced by other physical processes during their propagation from their birth places to the detectors, the mismatches on emission angle, wavelength shift, and threshold may be qualitatively explained through the assumption that small-scale light filaments widely existed in the corona of laser-produced plasmas.

  17. Magnetometry of buried layers—Linear magnetic dichroism and spin detection in angular resolved hard X-ray photoelectron spectroscopy

    International Nuclear Information System (INIS)

    Gloskovskii, Andrei; Stryganyuk, Gregory; Fecher, Gerhard H.; Felser, Claudia; Thiess, Sebastian; Schulz-Ritter, Heiko; Drube, Wolfgang; Berner, Götz; Sing, Michael; Claessen, Ralph; Yamamoto, Masafumi

    2012-01-01

    Highlights: ► Newly commissioned HAXPES instrument at P09 beamline of the PETRA III ring at DESY. ► We report HAXPES studies on buried magnetic nanolayers in a multi-layer sample. ► Linear magnetic dichroism of photoelectrons from buried CoFe–Ir 78 Mn 22 layers. ► Spin-resolved HAXPES measurements on buried magnetic multilayers using Mott detector. - Abstract: The electronic properties of buried magnetic nano-layers were studied using the linear magnetic dichroism in the angular distribution of photoemitted Fe, Co, and Mn 2p electrons from a CoFe–Ir 78 Mn 22 multi-layered sample. The buried layers were probed using hard X-ray photoelectron spectroscopy, HAXPES, at the undulator beamline P09 of the 3rd generation storage ring PETRA III. The results demonstrate that this magnetometry technique can be used as a sensitive element specific probe for magnetic properties suitable for application to buried ferromagnetic and antiferromagnetic magnetic materials and multilayered spintronics devices. Using the same instrument, spin-resolved Fe 2p HAXPES spectra were obtained from the buried layer with good signal quality.

  18. Angle-resolved photoemission spectroscopy of (Ca, Na) sub 2 CuO sub 2 Cl sub 2 crystals: Fingerprints of a magnetic insulator in a heavily underdoped superconductor

    CERN Document Server

    Kohsaka, Y; Ronning, F

    2003-01-01

    Electric evolution from an antiferromagnet to a high-T sub c superconductor is revealed by angle-resolved photoemission experiments on tetragonal Ca sub 1 sub . sub 9 Na sub 0 sub . sub 1 CuO sub 2 Cl sub 2 single crystals, which were successfully grown for the first time under high pressures. In this underdoped superconductor, we found clear fingerprints of the parent insulator: a shadow band and a large pseudogap. These observations are most likely described by a 'chemical potential shift', which contrasts clearly with the prevailing wisdom of the pinned chemical potential' learned from the prototype La sub 2 sub - sub x Sr sub x CuO sub 4 , demonstrating that the route to a high-T sub c superconductor is not unique. (author)

  19. Absence of a holelike fermi surface for the iron-based K0.8F1.7Se2 superconductor revealed by angle-resolved photoemission spectroscopy.

    Science.gov (United States)

    Qian, T; Wang, X-P; Jin, W-C; Zhang, P; Richard, P; Xu, G; Dai, X; Fang, Z; Guo, J-G; Chen, X-L; Ding, H

    2011-05-06

    We have performed an angle-resolved photoemission spectroscopy study of the new iron-based superconductor K(0.8)Fe(1.7)Se(2) (T(c)∼30 K). Clear band dispersion is observed with the overall bandwidth renormalized by a factor of 2.5 compared to our local density approximation calculations, indicating relatively strong correlation effects. Only an electronlike band crosses the Fermi energy, forming a nearly circular Fermi surface (FS) at M (π, 0). The holelike band at Γ sinks ∼90 meV below the Fermi energy, with an indirect band gap of 30 meV, to the bottom of the electronlike band. The observed FS topology in this superconductor favors (π, π) inter-FS scattering between the electronlike FSs at the M points, in sharp contrast to other iron-based superconductors which favor (π, 0) inter-FS scattering between holelike and electronlike FSs.

  20. Reaffirming the d(x2-y2) superconducting gap using the autocorrelation angle-resolved photoemission spectroscopy of Bi1.5Pb0.55Sr1.6La0.4CuO(6+δ).

    Science.gov (United States)

    Hashimoto, M; He, R-H; Testaud, J P; Meevasana, W; Moore, R G; Lu, D H; Yoshida, Y; Eisaki, H; Devereaux, T P; Hussain, Z; Shen, Z-X

    2011-04-22

    Knowledge of the gap function is important to understand the pairing mechanism for high-temperature (T(c)) superconductivity. However, Fourier transform scanning tunneling spectroscopy (FT STS) and angle-resolved photoemission spectroscopy (ARPES) in the cuprates have reported contradictory gap functions, with FT-STS results deviating strongly from a canonical d(x2-y2) form. By applying an "octet model" analysis to autocorrelation ARPES, we reveal that a contradiction occurs because the octet model does not consider the effects of matrix elements and the pseudogap. This reaffirms the canonical d(x2-y2) superconducting gap around the node, which can be directly determined from ARPES. Further, our study suggests that the FT-STS reported fluctuating superconductivity around the node at far above T(c) is not necessary to explain the existence of the quasiparticle interference at low energy.

  1. Optics of short-pitch deformed-helix ferroelectric liquid crystals: Symmetries, exceptional points, and polarization-resolved angular patterns

    Science.gov (United States)

    Kiselev, Alexei D.; Chigrinov, Vladimir G.

    2014-10-01

    In order to explore electric-field-induced transformations of polarization singularities in the polarization-resolved angular (conoscopic) patterns emerging after deformed-helix ferroelectric liquid crystal (DHFLC) cells with subwavelength helix pitch, we combine the transfer matrix formalism with the results for the effective dielectric tensor of biaxial FLCs evaluated using an improved technique of averaging over distorted helical structures. Within the framework of the transfer matrix method, we deduce a number of symmetry relations and show that the symmetry axis of L lines (curves of linear polarization) is directed along the major in-plane optical axis which rotates under the action of the electric field. When the angle between this axis and the polarization plane of incident linearly polarized light is above its critical value, the C points (points of circular polarization) appear in the form of symmetrically arranged chains of densely packed star-monstar pairs. We also emphasize the role of phase singularities of a different kind and discuss the enhanced electro-optic response of DHFLCs near the exceptional point where the condition of zero-field isotropy is fulfilled.

  2. Stable five axes cryogenic photoemission manipulator without a differentially pumped rotary feedthrough

    International Nuclear Information System (INIS)

    Kim, Bum Joon; Kim, Hyeong-Do; Cho, Deok-Yong; Kim, Myongjin; Oh, S.-J.; Kim, Changyoung

    2005-01-01

    We report on the design and construction of an ultrahigh vacuum compatible cryogenic manipulator for angle resolved photoemission spectroscopy. Unlike designs that have been used so far, our design allows five motions (three translational and two angular) without a differentially pumped rotary feedthrough. The design greatly reduces the sample motion upon rotation, which is crucial in automatic data acquisition over a large area in the momentum space. The constructed manipulator shows smooth motions in vacuum and the lowest temperature it could reach is about 8 K at the sample position. Angular reproducibilities are found to be about 0.02 deg. for both of the angular motions. The wobbling motion from the rotation around the vertical rotation axis is found to be virtually nonexistent (less than 0.1 mm)

  3. Inner-shell photoemission from atoms and molecules using synchrotron radiation

    International Nuclear Information System (INIS)

    Lindle, D.W.

    1983-12-01

    Photoelectron spectroscopy, in conjunction with synchrotron radiation, has been used to study inner-shell photoemission from atoms and molecules. The time structure of the synchrotron radiation permits the measurements of time-of-flight (TOF) spectra of Auger and photoelectrons, thereby increasing the electron collection efficiency. The double-angle TOF method yielded angle-resolved photoelectron intensities, which were used to determine photoionization cross sections and photoelectron angular distributions in several cases. Comparison to theoretical calculations has been made where possible to help explain observed phenomena in terms of the electronic structure and photoionization dynamics of the systems studied. 154 references, 23 figures, 7 tables

  4. Spatially and angularly resolved spectroscopy for in-situ estimation of concentration and particle size in colloidal suspensions.

    Science.gov (United States)

    Chen, Yi-Chieh; Foo, David; Dehanov, Nicolau; Thennadil, Suresh N

    2017-12-01

    Successful implementation of process analytical technology (PAT) hinges on the ability to make continuous or frequent measurements in-line or at-line of critical product attributes such as composition and particle size, the latter being an important parameter for particulate processes such as suspensions and emulsions. A novel probe-based spatially and angularly-resolved diffuse reflectance measurement (SAR-DRM) system is proposed. This instrument, along with appropriate calibration models, is designed for online monitoring of concentration of chemical species and particle size of the particulate species in process systems involving colloidal suspensions. This measurement system was investigated using polystyrene suspensions of various particle radius and concentration to evaluate its performance in terms of the information obtained from the novel configuration which allows the measurement of a combination of incident light at different angles and collection fibres at different distances from the source fibres. Different strategies of processing and combining the SAR-DRM measurements were considered in terms of the impact on partial least squares (PLS) model performance. The results were compared with those obtained using a bench-top instrument which was used as the reference (off-line) instrument for comparison purposes. The SAR-DRM system showed similar performance to the bench top reference instrument for estimation of particle radius, and outperforms the reference instrument in estimating particle concentration. The investigation shows that the improvement in PLS regression model performance using the SAR-DRM system is related to the extra information captured by the SAR-DRM configuration. The differences in SAR-DRM spectra collected by the different collection fibres from different angular source fibres are the dominant reason for the significant improvement in the model performance. The promising results from this study suggest the potential of the SAR

  5. Plasmon Enhanced Photoemission

    Energy Technology Data Exchange (ETDEWEB)

    Polyakov, Aleksandr [Univ. of California, Berkeley, CA (United States)

    2012-05-08

    this work, the structure consisted of rectangular nano-grooves (NGs) arranged in a subwavelength grating on a metal surface is presented that provides a dramatic increase in the metal’s absorption, field localization, and field enhancement. When light is polarized perpendicular to the orientation of the grooves a standing SPP wave is excited along the vertical walls in the NGs, that act as Fabry-Perot resonators. By adjusting the geometry of the NGs and the period of the subwavelength grating the resonance can be fine tuned to a desired position, for example, the laser fundamental wavelength, anywhere from the UV to the near infrared (NIR). Two types of gratings are presented: (a) a gold grating with period of 600 nm, and (b) an aluminum-gold grating with a period of 100 nm; both with resonance at 720 nm. In each case, strong on-resonance absorption was observed, with over 98% for grating (b). Unlike the grating-coupled SPP waves, where the angle is well defined by the momentum matching condition, the resonant NGs allow coupling to the standing modes at a range of angles of incidence, referred to as the angular bandwidth. A new model for the on-resonance absorption based on the ensamble action of the NGs is presented that serves as the basis for a design of an NG grating with an ultrawide spectral as well as angular bandwidth. For sample (b), the angular bandwidth is 80 degrees, corresponding to an opening angle of 160 degrees. The photoemission enhancement for such a grating was measured to be seven orders of magnitude for a four-photon photoemission. This is an incredible result demonstrating the power of the plasmonic grating presented, which is an efficient light trapper and field enhancer for a non-linear processes. These results demonstrate that the metal photocathode prepared with a NG grating on the metal surface will provide sufficient pulse charge driven by a 1 μJ 15fs pulsed laser at 800 nm for the optimum FEL operation.

  6. Insights from angle-resolved photoemission spectroscopy on the metallic states of YbB6(001): E(k) dispersion, temporal changes, and spatial variation

    NARCIS (Netherlands)

    Frantzeskakis, E.; de Jong, N.; Zhang, J.X.; Zhang, X.; Li, Z.; Liang, C.L.; Wang, Y.; Varykhalov, A.; Huang, Y.K.; Golden, M.S.

    2014-01-01

    We report high-resolution angle-resolved photoelectron spectroscopy (ARPES) results on the (001) cleavage surface of YbB6, a rare-earth compound that has been recently predicted to host surface electronic states with topological character. We observe two types of well-resolved metallic states, whose

  7. Quasiparticle dynamics across the full Brillouin zone of Bi2Sr2CaCu2O8+δ traced with ultrafast time and angle-resolved photoemission spectroscopy

    Directory of Open Access Journals (Sweden)

    Georgi L. Dakovski

    2015-09-01

    Full Text Available A hallmark in the cuprate family of high-temperature superconductors is the nodal-antinodal dichotomy. In this regard, angle-resolved photoemission spectroscopy (ARPES has proven especially powerful, providing band structure information directly in energy-momentum space. Time-resolved ARPES (trARPES holds great promise of adding ultrafast temporal information, in an attempt to identify different interaction channels in the time domain. Previous studies of the cuprates using trARPES were handicapped by the low probing energy, which significantly limits the accessible momentum space. Using 20.15 eV, 12 fs pulses, we show for the first time the evolution of quasiparticles in the antinodal region of Bi2Sr2CaCu2O8+δ and demonstrate that non-monotonic relaxation dynamics dominates above a certain fluence threshold. The dynamics is heavily influenced by transient modification of the electron-phonon interaction and phase space restrictions, in stark contrast to the monotonic relaxation in the nodal and off-nodal regions.

  8. Developments in inverse photoemission spectroscopy

    International Nuclear Information System (INIS)

    Sheils, W.; Leckey, R.C.G.; Riley, J.D.

    1996-01-01

    In the 1950's and 1960's, Photoemission Spectroscopy (PES) established itself as the major technique for the study of the occupied electronic energy levels of solids. During this period the field divided into two branches: X-ray Photoemission Spectroscopy (XPS) for photon energies greater than ∼l000eV, and Ultra-violet Photoemission Spectroscopy (UPS) for photon energies below ∼100eV. By the 1970's XPS and UPS had become mature techniques. Like XPS, BIS (at x-ray energies) does not have the momentum-resolving ability of UPS that has contributed much to the understanding of the occupied band structures of solids. BIS moved into a new energy regime in 1977 when Dose employed a Geiger-Mueller tube to obtain density of unoccupied states data from a tantalum sample at a photon energy of ∼9.7eV. At similar energies, the technique has since become known as Inverse Photoemission Spectroscopy (IPS), in acknowledgment of its complementary relationship to UPS and to distinguish it from the higher energy BIS. Drawing on decades of UPS expertise, IPS has quickly moved into areas of interest where UPS has been applied; metals, semiconductors, layer compounds, adsorbates, ferromagnets, and superconductors. At La Trobe University an IPS facility has been constructed. This presentation reports on developments in the experimental and analytical techniques of IPS that have been made there. The results of a study of the unoccupied bulk and surface bands of GaAs are presented

  9. Spatial structure determination of ({radical}3 x {radical}3)R30{degrees} and (1.5 x 1.5)R18{degrees}CO on Cu(111) using angle-resolved photoemission extended fine structure

    Energy Technology Data Exchange (ETDEWEB)

    Moler, E.J.; Kellar, S.A.; Huff, W.R.A. [Lawrence Berkeley National Lab., CA (United States)] [and others

    1997-04-01

    The authors report a study of the spatial structure of ({radical}3 x {radical}3)R30{degrees} (low coverage) and (1.5 x 1.5)R18{degrees} (intermediate coverage) CO adsorbed on Cu(111), using the Angle-Resolved Photoemission Extended Fine Structure (ARPEFS) technique at beamline 9.3.2 at the Advanced Light Source. The CO molecule adsorbs on an atop site for both adsorption phases. Full multiple-scattering spherical-wave (MSSW) calculations were used to extract the C-Cu. bond length and the first Cu-Cu layer spacing for each adsorption phase. The authors find that the C-Cu bond length remains unchanged with increasing coverage, but the 1st Cu-Cu layer spacing contracts at the intermediate coverage. They calculate the bending mode force constant in the (1.5 x 1.5)R18{degrees} phase to be K{sub {delta}} = 2.2 (1) x 10{sup {minus}12} dyne-cm/rad from their experimentally determined bond lengths combined with previously published infra-red absorption frequencies.

  10. A New Spin on Photoemission Spectroscopy

    Energy Technology Data Exchange (ETDEWEB)

    Jozwiak, Chris [Univ. of California, Berkeley, CA (United States)

    2008-12-01

    The electronic spin degree of freedom is of general fundamental importance to all matter. Understanding its complex roles and behavior in the solid state, particularly in highly correlated and magnetic materials, has grown increasingly desirable as technology demands advanced devices and materials based on ever stricter comprehension and control of the electron spin. However, direct and efficient spin dependent probes of electronic structure are currently lacking. Angle Resolved Photoemission Spectroscopy (ARPES) has become one of the most successful experimental tools for elucidating solid state electronic structures, bolstered by-continual breakthroughs in efficient instrumentation. In contrast, spin-resolved photoemission spectroscopy has lagged behind due to a lack of similar instrumental advances. The power of photoemission spectroscopy and the pertinence of electronic spin in the current research climate combine to make breakthroughs in Spin and Angle Resolved Photoemission Spectroscopy (SARPES) a high priority . This thesis details the development of a unique instrument for efficient SARPES and represents a radical departure from conventional methods. A custom designed spin polarimeter based on low energy exchange scattering is developed, with projected efficiency gains of two orders of magnitude over current state-of-the-art polarimeters. For energy analysis, the popular hemispherical analyzer is eschewed for a custom Time-of-Flight (TOF) analyzer offering an additional order of magnitude gain in efficiency. The combined instrument signifies the breakthrough needed to perform the high resolution SARPES experiments necessary for untangling the complex spin-dependent electronic structures central to today's condensed matter physics.

  11. Angle-Resolved Photoemission Study of the Evolution of Band Structure And Charge Density Wave Properties in Rte (3) (R=Y, La, Ce, Sm, Gd, Tb, And Dy)

    Energy Technology Data Exchange (ETDEWEB)

    Brouet, V.; Yang, W.L.; Zhou, X.J.; Hussain, Z.; Moore, R.G.; He, R.; Lu, D.H.; Shen, Z.X.; Laverock, J.; Dugdale, S.B.; Ru, N.; Fisher, I.R.

    2009-05-12

    We present a detailed angle-resolved photoemission spectroscopy (ARPES) investigation of the RTe{sub 3} family, which sets this system as an ideal 'textbook' example for the formation of a nesting driven charge density wave (CDW). This family indeed exhibits the full range of phenomena that can be associated to CDW instabilities, from the opening of large gaps on the best nested parts of Fermi surface (up to 0.4 eV), to the existence of residual metallic pockets. ARPES is the best suited technique to characterize these features, thanks to its unique ability to resolve the electronic structure in k space. An additional advantage of RTe{sub 3} is that the band structure can be very accurately described by a simple two dimensional tight-binding (TB) model, which allows one to understand and easily reproduce many characteristics of the CDW. In this paper, we first establish the main features of the electronic structure by comparing our ARPES measurements with the linear muffin-tin orbital band calculations. We use this to define the validity and limits of the TB model. We then present a complete description of the CDW properties and of their strong evolution as a function of R. Using simple models, we are able to reproduce perfectly the evolution of gaps in k space, the evolution of the CDW wave vector with R, and the shape of the residual metallic pockets. Finally, we give an estimation of the CDW interaction parameters and find that the change in the electronic density of states n(E{sub F}), due to lattice expansion when different R ions are inserted, has the correct order of magnitude to explain the evolution of the CDW properties.

  12. Time-resolved and integrated angular distributions of plume ions from silver at low and medium laser fluence

    DEFF Research Database (Denmark)

    Christensen, Bo Toftmann; Schou, Jørgen

    2013-01-01

    Laser impact on metals in the UV regime results in a significant number of ablated plume ions even at moderate fluence (0.7–2.4 J/cm2). The ablated particles are largely neutrals at the lowest fluence, but the fraction of ions increases strongly with fluence. The ion flow in different directions...... from a silver target irradiated by a laser beam at a wavelength of 355 nm in vacuum was measured with a hemispherical array of Langmuir probes. The time-of-flight spectra in all directions, as well as the total angular yield were determined. The angular distribution peaks strongly in forward direction...

  13. Frequency-resolved measurement of the orbital angular momentum spectrum of femtosecond ultra-broadband optical-vortex pulses based on field reconstruction

    International Nuclear Information System (INIS)

    Yamane, Keisaku; Yang, Zhili; Toda, Yasunori; Morita, Ryuji

    2014-01-01

    We propose a high-precision method for measuring the orbital angular momentum (OAM) spectrum of ultra-broadband optical-vortex (OV) pulses from fork-like interferograms between OV pulses and a reference plane-wave pulse. It is based on spatial reconstruction of the electric fields of the pulses to be measured from the frequency-resolved interference pattern. Our method is demonstrated experimentally by obtaining the OAM spectra for different spectral components of the OV pulses, enabling us to characterize the frequency dispersion of the topological charge of the OAM spectrum by a simple experimental setup. Retrieval is carried out in quasi-real time, allowing us to investigate OAM spectra dynamically. Furthermore, we determine the relative phases (including the sign) of the topological-charge-resolved electric-field amplitudes, which are significant for evaluating OVs or OV pulses with arbitrarily superposed modes. (paper)

  14. Angle-resolved photoemission study of the evolution of band structure and charge density wave properties in RTe3 (R= Y, La, Ce, Sm, Gd, Tb and Dy)

    Energy Technology Data Exchange (ETDEWEB)

    Brouet, V.; Yang, W.L.; Zhou, X.J.; Hussain, Z.; Moore, R.G.; He, R.; Lu, D.H.; Shen, Z.X.; Laverock, J.; Dugdale, S.; Ru, N.; Fisher, I.R.

    2010-02-15

    We present a detailed ARPES investigation of the RTe{sub 3} family, which sets this system as an ideal 'textbook' example for the formation of a nesting driven Charge Density Wave (CDW). This family indeed exhibits the full range of phenomena that can be associated to CDW instabilities, from the opening of large gaps on the best nested parts of Fermi Surface (FS) (up to 0.4eV), to the existence of residual metallic pockets. ARPES is the best suited technique to characterize these features, thanks to its unique ability to resolve the electronic structure in k-space. An additional advantage of RTe{sub 3} is that the band structure can be very accurately described by a simple 2D tight-binding (TB) model, which allows one to understand and easily reproduce many characteristics of the CDW. In this paper, we first establish the main features of the electronic structure, by comparing our ARPES measurements with Linear Muffin-Tin Orbital band calculations. We use this to define the validity and limits of the TB model. We then present a complete description of the CDW properties and, for the first time, of their strong evolution as a function of R. Using simple models, we are able to reproduce perfectly the evolution of gaps in k-space, the evolution of the CDW wave vector with R and the shape of the residual metallic pockets. Finally, we give an estimation of the CDW interaction parameters and find that the change in the electronic density of states n(Ef), due to lattice expansion when different R ions are inserted, has the correct order of magnitude to explain the evolution of the CDW properties.

  15. Future directions in standing-wave photoemission

    International Nuclear Information System (INIS)

    Gray, Alexander X.

    2014-01-01

    Highlights: • Probing magnetic properties at the buried interface with SW-MCD. • Probing electronic structure at the buried interface with resonant SW-XPS and SW-HAXPES. • Probing momentum-resolved electronic structure at a buried interface with SWARPES. • Adding depth resolution to photoemission microscopy with standing-wave excitation. • Standing-wave localization, total reflection and waveguide effects. - Abstract: Over the past decade, standing-wave photoemission (SW-XPS) has evolved into a powerful and versatile non-destructive technique for probing element-specific electronic, magnetic, and structural properties of buried layers and interfaces with sub-nanometer depth resolution. In this article, I will discuss several promising future directions in this emergent field stemming from experimental and theoretical studies wherein SW-XPS is combined with other X-ray techniques, such as magnetic circular dichroism (MCD), hard X-ray photoemission spectroscopy (HAXPES), angle-resolved photoemission (ARPES), and photoemission microscopy (PEEM), adding extra dimensions to the measurement and thus widening the scope of scientific and technological questions accessible via the use of standing waves. I will further discuss examples of recently developed methods for X-ray standing-wave data analysis, which yield layer-resolved matrix-element-weighted densities of states at interfaces as well as Ångstrom-level changes in periodicity of synthetic superlattices. Finally, I will explore the possibility of localizing the standing waves near the surface and within a buried layer by the use of aperiodic superlattices, total reflection, and X-ray waveguide effects

  16. Photoelectron spectroscopy at a free-electron laser. Investigation of space-charge effects in angle-resolved and core-level spectroscopy and realizaton of a time-resolved core-level photoemission experiment

    International Nuclear Information System (INIS)

    Marczynski-Buehlow, Martin

    2012-01-01

    The free-electron laser (FEL) in Hamburg (FLASH) is a very interesting light source with which to perform photoelectron spectroscopy (PES) experiments. Its special characteristics include highly intense photon pulses (up to 100 J/pulse), a photon energy range of 30 eV to 1500 eV, transverse coherence as well as pulse durations of some ten femtoseconds. Especially in terms of time-resolved PES (TRPES), the deeper lying core levels can be reached with photon energies up to 1500 eV with acceptable intensity now and, therefore, element-specific, time-resolved core-level PES (XPS) is feasible at FLASH. During the work of this thesis various experimental setups were constructed in order to realize angle-resolved (ARPES), core-level (XPS) as well as time-resolved PES experiments at the plane grating monochromator beamline PG2 at FLASH. Existing as well as newly developed systems for online monitoring of FEL pulse intensities and generating spatial and temporal overlap of FEL and optical laser pulses for time-resolved experiments are successfully integrated into the experimental setup for PES. In order to understand space-charge effects (SCEs) in PES and, therefore, being able to handle those effects in future experiments using highly intense and pulsed photon sources, the origin of energetic broadenings and shifts in photoelectron spectra are studied by means of a molecular dynamic N-body simulation using a modified Treecode Algorithm for sufficiently fast and accurate calculations. It turned out that the most influencing parameter is the ''linear electron density'' - the ratio of the number of photoelectrons to the diameter of the illuminated spot on the sample. Furthermore, the simulations could reproduce the observations described in the literature fairly well. Some rules of thumb for XPS and ARPES measurements could be deduced from the simulations. Experimentally, SCEs are investigated by means of ARPES as well as XPS measurements as a function of FEL pulse

  17. Photoelectron spectroscopy at a free-electron laser. Investigation of space-charge effects in angle-resolved and core-level spectroscopy and realizaton of a time-resolved core-level photoemission experiment

    Energy Technology Data Exchange (ETDEWEB)

    Marczynski-Buehlow, Martin

    2012-01-30

    The free-electron laser (FEL) in Hamburg (FLASH) is a very interesting light source with which to perform photoelectron spectroscopy (PES) experiments. Its special characteristics include highly intense photon pulses (up to 100 J/pulse), a photon energy range of 30 eV to 1500 eV, transverse coherence as well as pulse durations of some ten femtoseconds. Especially in terms of time-resolved PES (TRPES), the deeper lying core levels can be reached with photon energies up to 1500 eV with acceptable intensity now and, therefore, element-specific, time-resolved core-level PES (XPS) is feasible at FLASH. During the work of this thesis various experimental setups were constructed in order to realize angle-resolved (ARPES), core-level (XPS) as well as time-resolved PES experiments at the plane grating monochromator beamline PG2 at FLASH. Existing as well as newly developed systems for online monitoring of FEL pulse intensities and generating spatial and temporal overlap of FEL and optical laser pulses for time-resolved experiments are successfully integrated into the experimental setup for PES. In order to understand space-charge effects (SCEs) in PES and, therefore, being able to handle those effects in future experiments using highly intense and pulsed photon sources, the origin of energetic broadenings and shifts in photoelectron spectra are studied by means of a molecular dynamic N-body simulation using a modified Treecode Algorithm for sufficiently fast and accurate calculations. It turned out that the most influencing parameter is the ''linear electron density'' - the ratio of the number of photoelectrons to the diameter of the illuminated spot on the sample. Furthermore, the simulations could reproduce the observations described in the literature fairly well. Some rules of thumb for XPS and ARPES measurements could be deduced from the simulations. Experimentally, SCEs are investigated by means of ARPES as well as XPS measurements as a function of

  18. Direct angle resolved photoemission spectroscopy and ...

    Indian Academy of Sciences (India)

    [3] Karl Alex Mueller, personal communications (2006). In contrast, see P W Anderson, Nature Phys. 2, 626 (2006) or the whole issue Nature. Phys. - 20 years of HTSC (March 2006). [4] G Baskaran, personal communication, Kanpur (2006), also CM9910161v1. [5] T Timusk and B Statt, Rep. Prog. Phys. 62(1), 61 (1999).

  19. Direct angle resolved photoemission spectroscopy and ...

    Indian Academy of Sciences (India)

    We gratefully acknowledge financial support by the EPFL and the Swiss National. Fund for Scientific Research. This work is based upon research conducted at the. Synchrotron Radiation Center, University of Wisconsin-Madison, which is sup- ported by the NSF under Award No. DMR-0084402. DP gratefully acknowledges.

  20. Fourier Transform Photoemission Spectroscopy

    NARCIS (Netherlands)

    Meinders, M.B.J.; Drabe, K.E.; Jonkman, H.T.; Sawatzky, G.A.

    1996-01-01

    It is shown that photoemission spectra can be obtained by exciting the electrons with two phase-correlated wave trains. The phase-correlated wave trains are obtained by sending broad-band ultra-violet light, coming from a deuterium lamp, through a Michelson interferometer. It is possible to

  1. Fourier transform photoemission spectroscopy

    NARCIS (Netherlands)

    Meinders, M.B J; Drabe, K.E.; Jonkman, H.T.; Sawatzky, G.A

    It is shown that photoemission spectra can be obtained by exciting the electrons with two phase-correlated wave trains. The phase-correlated wave trains are obtained by sending broad-band ultra-violet light, coming from a deuterium lamp, through a Michelson interferometer. It is possible to

  2. State resolved rotational excitation in HD+D2 collisions. II. Angular dependence of 0→2 transitions

    International Nuclear Information System (INIS)

    Buck, U.; Huisken, F.; Maneke, G.; Schaefer, J.

    1983-01-01

    Time-of-flight spectra for the scattering of HD molecules from D 2 molecules have been measured at a collision energy of E = 70.3 meV over a range of center-of-mass scattering angles from 45 0 to 158 0 . The spectra reveal clearly resolved transitions at the energy loss ΔE = 33 meV which corresponds to 0→2 transitions of HD and the double transition 0→1 of HD and 0→2 of D 2 . The differential cross sections derived from these spectra increase with increasing scattering angle from 1.7% to 34.7% of the elastic cross section. The pure 0→2 transition of D 2 which only needs 22 meV to be induced could not be detected within our experimental sensitivity of 0.02 A 2 /sr. Closed coupled calculations based on the ab initio potential surface of Meyer and Schaefer show that this result can be explained by the different coupling terms which are responsible for these transitions. In contrast to the 0→1 transition the 0→2 transition of HD proved to be sensitive to the anisotropic part of the interaction potential for the homonuclear system. The comparison of experimental and calculated cross sections for the ab initio potential of Meyer and Schaefer reveals discrepancies for the 0→1 transition of HD, but shows agreement for the 0→2 transition of HD at intermediate angles

  3. Photoemission electronic states of epitaxially grown magnetite films

    International Nuclear Information System (INIS)

    Zalecki, R.; Kolodziejczyk, A.; Korecki, J.; Spiridis, N.; Zajac, M.; Kozlowski, A.; Kakol, Z.; Antolak, D.

    2007-01-01

    The valence band photoemission spectra of epitaxially grown 300 A single crystalline magnetite films were measured by the angle-resolved ultraviolet photoemission spectroscopy (ARUPS) at 300 K. The samples were grown either on MgO(0 0 1) (B termination) or on (0 0 1) Fe (iron-rich A termination), thus intentionally presenting different surface stoichiometry, i.e. also different surface electronic states. Four main features of the electron photoemission at about -1.0, -3.0, -5.5 and -10.0 eV below a chemical potential show systematic differences for two terminations; this difference depends on the electron outgoing angle. Our studies confirm sensitivity of angle resolved PES technique on subtleties of surface states

  4. General survey of recent development of photoemission spectroscopy

    International Nuclear Information System (INIS)

    Edamoto, Kazuyuki

    1994-01-01

    On the present state of the recent development of photoemission spectroscopy, by limiting the topics to the development of the spectroscopy proper and the development contributing to the progress of surface science, general explanation is made. As to the development that enabled to heighten spectrum resolution, surface core-level shift and the precise measurement of the Fermi surface of surface level are described, showing the example. Also a number of the developments which enabled the utilization of the light source, of which the wavelength is variable, and which was brought about by synchrotron radiation beam, were mentioned. Besides, spin polarized photoelectron spectroscopy, the development of photoelectron microscope and others are outlined. Photoemission spectroscopy is very useful for analyzing the electron condition of solid surfaces. There are two factors in heightening core level spectrum resolution, namely, heightening the resolution of an electron energy analyzer proper and the utilization of synchrotron radiation as a light source. High resolution core-level spectra, angle-resolved photoemission spectroscopy, and as the light source of which the wavelength is variable, resonance photoemission spectroscopy, constant initial state spectroscopy and soft X-ray photoemission spectroscopy, and as the recently developed spectroscopy, spin polarized photoemission spectroscopy, Auger photoelectron coincidence spectroscopy and photoelectron microscope are explained. (K.I.)

  5. Relaxation and cross section effects in valence band photoemission spectroscopy

    International Nuclear Information System (INIS)

    McFeely, F.R.

    1976-09-01

    Various problems relating to the interpretation of valence band x-ray photoemission (XPS) spectra of solids are discussed. The experiments and calculations reported herein deal with the following questions: (1) To what extent do many-body effects manifest themselves in an XPS valence band spectrum, and thus invalidate a direct comparison between the photoemission energy distribution, I(E), and the density of states, N(E), calculated on the basis of ground-state one-electron theory. (2) The effect of the binding-energy-dependent photoemission cross section on I(E) at XPS energies. (3) In favorable cases indicated by (1) and (2) we examine the effect of the interaction of the crystal field with the apparent spin-orbit splittings of core levels observed in XPS spectra. (4) The use of tight binding band structure calculations to parameterize the electronic band structure from XPS and other data is described. (5) The use of high energy angle-resolved photoemission on oriented single crystals to gain orbital symmetry information is discussed. (6) The evolution of the shape of the photoemission energy distribution (of polycrystalline Cu) as a function of photon energy from 50 less than or equal h ω less than or equal 175 is discussed

  6. Inverse photoemission of uranium oxides

    International Nuclear Information System (INIS)

    Roussel, P.; Morrall, P.; Tull, S.J.

    2009-01-01

    Understanding the itinerant-localised bonding role of the 5f electrons in the light actinides will afford an insight into their unusual physical and chemical properties. In recent years, the combination of core and valance band electron spectroscopies with theoretic modelling have already made significant progress in this area. However, information of the unoccupied density of states is still scarce. When compared to the forward photoemission techniques, measurements of the unoccupied states suffer from significantly less sensitivity and lower resolution. In this paper, we report on our experimental apparatus, which is designed to measure the inverse photoemission spectra of the light actinides. Inverse photoemission spectra of UO 2 and UO 2.2 along with the corresponding core and valance electron spectra are presented in this paper. UO 2 has been reported previously, although through its inclusion here it allows us to compare and contrast results from our experimental apparatus to the previous Bremsstrahlung Isochromat Spectroscopy and Inverse Photoemission Spectroscopy investigations

  7. Spin polarization and magnetic dichroism in core-level photoemission from ferromagnets

    Energy Technology Data Exchange (ETDEWEB)

    Menchero, Jose Gabriel [Univ. of California, Berkeley, CA (United States). Dept. of Physics

    1997-05-01

    In this thesis we present a theoretical investigation of angle- and spin-resolved core-level photoemission from ferromagnetic Fe and Ni. We also consider magneto-dichroic effects due to reversal of the photon helicity or reversal of the sample magnetization direction. In chapter 1, we provide a brief outline of the history of photoemission, and show how it has played an important role in the development of modern physics. We then review the basic elements of the theory of core-level photoemission, and discuss the validity of the some of the commonly-used approximations. In chapter 2, we present a one-electron theory to calculate spin- and angle-resolved photoemission spectra for an arbitrary photon polarization. The Hamiltonian includes both spin-orbit and exchange interactions. As test cases for the theory, we calculate the spin polarization and magnetic dichroism for the Fe 2p core level, and find that agreement with experiment is very good.

  8. Photoemission and the origin of high temperature superconductivity

    Energy Technology Data Exchange (ETDEWEB)

    Norman, M. R.; Randeria, M.; Janko, B.; Campuzano, J. C.

    2000-03-01

    The condensation energy can be shown to be a moment of the change in the occupied part of the spectral function when going from the normal to the superconducting state. As a consequence, there is a one to one correspondence between the energy gain associated with forming the superconducting ground state, and the dramatic changes seen in angle resolved photoemission spectra. Some implications this observation has are offered.

  9. Photoemission and the origin of high temperature superconductivity

    International Nuclear Information System (INIS)

    Norman, M. R.; Randeria, M.; Janko, B.; Campuzano, J. C.

    2000-01-01

    The condensation energy can be shown to be a moment of the change in the occupied part of the spectral function when going from the normal to the superconducting state. As a consequence, there is a one to one correspondence between the energy gain associated with forming the superconducting ground state, and the dramatic changes seen in angle resolved photoemission spectra. Some implications this observation has are offered

  10. Photoemission spectroscopy using synchrotron radiation

    International Nuclear Information System (INIS)

    Kobayashi, K.L.I.

    1980-01-01

    It is an epoch making event for photoemission spectroscopy that the light sources of continuous wavelength from vacuum ultra-violet to X-ray region have become available by the advent of synchrotron radiation. Specifically the progress after stable intense light has become obtainable from storage rings is very significant. One of the features of these synchrotron radiation is its extreme polarization of radiating pattern. Though the elementary processes of photoemission out of solids are the basic themes, phenomenalistic 3-stage model is usually applied to the analysis of experiments. In this model, the process of photoemission is considered by dividing into three stages, namely the generation of photoelectrons due to optical transition between electron status -- the transportation of photoelectrons to solid surfaces -- breaking away from the surfaces. The spectrometers, the energy analyzers of photoelectrons, and sample-preparing room used for photoemission spectroscopy are described. Next, energy distribution curves are explained. At the end, photoelectron yield spectroscopy, CFS (constant final energy spectroscopy) and CIS (constant initial energy spectroscopy), Auger yield and interatomic Auger yield, the determination of surface structure by normal emission CIS, and surface EXAFS (extended X-ray absorption fine structure) are described. As seen above, the application specifically to surface physics is promising in the future. (Wakatsuki, Y.)

  11. Vacuum scanning capillary photoemission microscopy

    DEFF Research Database (Denmark)

    Aseyev, S.A.; Cherkun, A P; Mironov, B N

    2017-01-01

    We demonstrate the use of a conical capillary in a scanning probe microscopy for surface analysis. The probe can measure photoemission from a substrate by transmitting photoelectrons along the capillary as a function of probe position. The technique is demonstrated on a model substrate consisting...

  12. Valence band photoemission studies of clean metals

    Energy Technology Data Exchange (ETDEWEB)

    Wehner, P.S.

    1978-04-01

    The application of Angle-Resolved Photoelectron Spectroscopy (ARPES) to crystalline solids and the utilization of such studies to illuminate several questions concerning the detailed electronic structure of such materials, are discussed. Specifically, by construction of a Direct Transition (DT) model and the utilization of energy-dependent angle-resolved normal photoemission in the photon energy range 32 eV < or = h..nu.. < or = 200 eV, the bulk band structure of copper is experimentally mapped out along three different directions in the Brillouin Zone; GAMMA to K, GAMMA to L, and GAMMA to X. In addition, various effects which influence the obtainable resolution in vector k-space, namely, thermal disorder, momentum broadening, and band mixing, are discussed and are shown to place severe limitations on the applicability of the DT model. Finally, a model for Angle-Resolved X-ray Photoelectron Spectroscopy (ARXPS) based on the symmetry of the initial-state wavefunctions is presented and compared to experimental results obtained from copper single crystals.

  13. Photoemission beyond the sudden approximation

    Science.gov (United States)

    Almbladh, Carl-Olof

    2006-04-01

    The many-body theory of photoemission in solids is reviewed with emphasis on methods based on response theory. The classification of diagrams into loss and no-loss diagrams is discussed and related to Keldysh path-ordering book-keeping. Some new results on energy losses in valence-electron photoemission from free-electron-like metal surfaces are presented. A way to group diagrams is presented in which spectral intensities acquire a Golden-Rule-like form which guarantees positiveness. This way of regrouping should be useful also in other problems involving spectral intensities, such as the problem of improving the one-electron spectral function away from the quasiparticle peak.

  14. New ambient pressure photoemission endstation at Advanced Light Source beamline 9.3.2

    KAUST Repository

    Grass, Michael E.

    2010-01-01

    During the past decade, the application of ambient pressure photoemission spectroscopy (APPES) has been recognized as an important in situ tool to study environmental and materials science, energy related science, and many other fields. Several APPES endstations are currently under planning or development at the USA and international light sources, which will lead to a rapid expansion of this technique. The present work describes the design and performance of a new APPES instrument at the Advanced Light Source beamline 9.3.2 at Lawrence Berkeley National Laboratory. This new instrument, Scienta R4000 HiPP, is a result of collaboration between Advanced Light Source and its industrial partner VG-Scienta. The R4000 HiPP provides superior electron transmission as well as spectromicroscopy modes with 16 μm spatial resolution in one dimension and angle-resolved modes with simulated 0.5° angular resolution at 24° acceptance. Under maximum transmission mode, the electron detection efficiency is more than an order of magnitude better than the previous endstation at beamline 9.3.2. Herein we describe the design and performance of the system, which has been utilized to record spectra above 2 mbar. © 2010 American Institute of Physics.

  15. Strong Linear Dichroism in Spin-Polarized Photoemission from Spin-Orbit-Coupled Surface States.

    Science.gov (United States)

    Bentmann, H; Maaß, H; Krasovskii, E E; Peixoto, T R F; Seibel, C; Leandersson, M; Balasubramanian, T; Reinert, F

    2017-09-08

    A comprehensive understanding of spin-polarized photoemission is crucial for accessing the electronic structure of spin-orbit coupled materials. Yet, the impact of the final state in the photoemission process on the photoelectron spin has been difficult to assess in these systems. We present experiments for the spin-orbit split states in a Bi-Ag surface alloy showing that the alteration of the final state with energy may cause a complete reversal of the photoelectron spin polarization. We explain the effect on the basis of ab initio one-step photoemission theory and describe how it originates from linear dichroism in the angular distribution of photoelectrons. Our analysis shows that the modulated photoelectron spin polarization reflects the intrinsic spin density of the surface state being sampled differently depending on the final state, and it indicates linear dichroism as a natural probe of spin-orbit coupling at surfaces.

  16. Chiral orbital-angular momentum in the surface states of Bi2Se3.

    Science.gov (United States)

    Park, Seung Ryong; Han, Jinhee; Kim, Chul; Koh, Yoon Young; Kim, Changyoung; Lee, Hyungjun; Choi, Hyoung Joon; Han, Jung Hoon; Lee, Kyung Dong; Hur, Nam Jung; Arita, Masashi; Shimada, Kenya; Namatame, Hirofumi; Taniguchi, Masaki

    2012-01-27

    We performed angle-resolved photoemission (ARPES) experiments with circularly polarized light and first-principles density functional calculation with spin-orbit coupling to study surface states of a topological insulator Bi2Se3. We observed circular dichroism (CD) as large as 30% in the ARPES data with upper and lower Dirac cones showing opposite signs in CD. The observed CD is attributed to the existence of local orbital-angular momentum (OAM). First-principles calculation shows that OAM in the surface states is significant and is locked to the electron momentum in the opposite direction to the spin, forming chiral OAM states. Our finding opens a new possibility for strong light-induced spin-polarized current in surface states. We also provide a proof for local OAM origin of the CD in ARPES.

  17. Determination of strain localization in aluminum alloys using photoemission measurements

    Science.gov (United States)

    Cai, Mingdong; Langford, Stephen; Levine, Lyle; Dickinson, Thomas

    2004-03-01

    We report photoemission measurements during uniaxial tensile deformation of aluminum (1200), Al-Mn (3003), Al-Mg (5052), and Al-Mg-Si (6061) alloys during exposure to pulsed excimer laser radiation (248-nm). Photostimulated electron emission increases with strain as slip exposes fresh metal to the vacuum; strain localization alters the production rate of slip bands and hence can be monitored by this technique. All samples were annealed at 300 °C for three hours immediately after polishing to produce a relatively thick (typically 40-nm) surface oxide. This oxide reduces photoemission from undeformed material. Time-resolved electron emission measurements after each laser pulse show two or more photoemission peaks. The intensity of the late (slow) peaks changes little during deformation and apparently reflects electron emission from oxidized, undeformed portions of the sample and other nearby surfaces. The intensity of the first (fast) electron peak reflects emission from fresh metal along slip lines/bands generated by deformation. As strain proceeds, the intensity of the fast peak shows three stages of growth: a gradually increasing, incipient growth during the onset of deformation, followed by two linear increasing stages. We provide evidence that the transition between the two linear stages corresponds to the onset of strain localization.

  18. 3d spin-orbit photoemission spectrum of nonferromagnetic materials : The test cases of CoO and Cu

    NARCIS (Netherlands)

    Ghiringhelli, G; Tjeng, LH; Tanaka, A; Tjernberg, O; Mizokawa, T; de Boer, JL; Brookes, NB

    2002-01-01

    The x-ray photoemission spectrum of the valence states of 3d transition-metal systems is spin polarized when using circularly polarized photons. The integral of the spin-orbit spectrum is proportional to the expectation value of the angular part of the 3d spin-orbit operator in the initial state. We

  19. Angular Momentum

    Science.gov (United States)

    Shakur, Asif; Sinatra, Taylor

    2013-01-01

    The gyroscope in a smartphone was employed in a physics laboratory setting to verify the conservation of angular momentum and the nonconservation of rotational kinetic energy. As is well-known, smartphones are ubiquitous on college campuses. These devices have a panoply of built-in sensors. This creates a unique opportunity for a new paradigm in…

  20. Hot Electron Photoemission from Plasmonic Nanostructures: The Role of Surface Photoemission and Transition Absorption

    DEFF Research Database (Denmark)

    Babicheva, Viktoriia; Zhukovsky, Sergei; Ikhsanov, Renat Sh

    2015-01-01

    We study mechanisms of photoemission of hot electrons from plasmonic nanoparticles. We analyze the contribution of "transition absorption", i.e., loss of energy of electrons passing through the boundary between different materials, to the surface mechanism of photoemission. We calculate photoemis......We study mechanisms of photoemission of hot electrons from plasmonic nanoparticles. We analyze the contribution of "transition absorption", i.e., loss of energy of electrons passing through the boundary between different materials, to the surface mechanism of photoemission. We calculate...... photoemission rate and transition absorption for nanoparticles surrounded by various media with a broad range of permittivities and show that photoemission rate and transition absorption follow the same dependence on the permittivity. Thus, we conclude that transition absorption is responsible...

  1. Widespread spin polarization effects in photoemission from topological insulators

    Energy Technology Data Exchange (ETDEWEB)

    Jozwiak, C.; Chen, Y. L.; Fedorov, A. V.; Analytis, J. G.; Rotundu, C. R.; Schmid, A. K.; Denlinger, J. D.; Chuang, Y.-D.; Lee, D.-H.; Fisher, I. R.; Birgeneau, R. J.; Shen, Z.-X.; Hussain, Z.; Lanzara, A.

    2011-06-22

    High-resolution spin- and angle-resolved photoemission spectroscopy (spin-ARPES) was performed on the three-dimensional topological insulator Bi{sub 2}Se{sub 3} using a recently developed high-efficiency spectrometer. The topological surface state's helical spin structure is observed, in agreement with theoretical prediction. Spin textures of both chiralities, at energies above and below the Dirac point, are observed, and the spin structure is found to persist at room temperature. The measurements reveal additional unexpected spin polarization effects, which also originate from the spin-orbit interaction, but are well differentiated from topological physics by contrasting momentum and photon energy and polarization dependencies. These observations demonstrate significant deviations of photoelectron and quasiparticle spin polarizations. Our findings illustrate the inherent complexity of spin-resolved ARPES and demonstrate key considerations for interpreting experimental results.

  2. Coherent and incoherent processes in resonant photoemission

    Energy Technology Data Exchange (ETDEWEB)

    Magnuson, M.; Karis, O.; Weinelt, M. [Uppsala Univ. (Sweden)] [and others

    1997-04-01

    In this contribution the authors present the distinction between coherent and incoherent processes in resonant photoemission. As a first step they determine whether an autoionization process is photoemission-like or Auger-like. The discussion is based on measurements for a weakly bonded adsorption system, Ar/Pt(111). This type of system is well adapted to investigate these effects since it yields distinctly shifted spectral features depending on the nature of the process. After this, the question of resonance photoemission in metallic systems is addressed. This is done in connection with measurements at the 2p edges for Ni metal. Ni has been one of the prototype systems for resonant photoemission. The resonances have been discussed in connection with the strong correlation and d-band localization effects in this system. Based on the results some general comments about the appearance of resonant effects in metallic systems are made.

  3. Angularly resolved electron wave packet interferences

    International Nuclear Information System (INIS)

    Varju, K; Johnsson, P; Mauritsson, J; Remetter, T; Ruchon, T; Ni, Y; Lepine, F; Kling, M; Khan, J; Schafer, K J; Vrakking, M J J; L'Huillier, A

    2006-01-01

    We study experimentally the ionization of argon atoms by a train of attosecond pulses in the presence of a strong infrared laser field, using a velocity map imaging technique. The recorded momentum distribution strongly depends on the delay between the attosecond pulses and the laser field. We interpret the interference patterns observed for different delays using numerical and analytical calculations within the strong field approximation

  4. Angularly resolved electron wave packet interferences

    Energy Technology Data Exchange (ETDEWEB)

    Varju, K [Department of Physics, Lund University, PO Box 118, SE-221 00 Lund (Sweden); Johnsson, P [Department of Physics, Lund University, PO Box 118, SE-221 00 Lund (Sweden); Mauritsson, J [Department of Physics, Lund University, PO Box 118, SE-221 00 Lund (Sweden); Remetter, T [Department of Physics, Lund University, PO Box 118, SE-221 00 Lund (Sweden); Ruchon, T [Department of Physics, Lund University, PO Box 118, SE-221 00 Lund (Sweden); Ni, Y [FOM-Institute AMOLF, Kruislaan 407, 1098 SJ Amsterdam (Netherlands); Lepine, F [FOM-Institute AMOLF, Kruislaan 407, 1098 SJ Amsterdam (Netherlands); Kling, M [FOM-Institute AMOLF, Kruislaan 407, 1098 SJ Amsterdam (Netherlands); Khan, J [FOM-Institute AMOLF, Kruislaan 407, 1098 SJ Amsterdam (Netherlands); Schafer, K J [Department of Physics and Astronomy, Louisiana State University, Baton Rouge, LA 70803-4001 (United States); Vrakking, M J J [FOM-Institute AMOLF, Kruislaan 407, 1098 SJ Amsterdam (Netherlands); L' Huillier, A [Department of Physics, Lund University, PO Box 118, SE-221 00 Lund (Sweden)

    2006-09-28

    We study experimentally the ionization of argon atoms by a train of attosecond pulses in the presence of a strong infrared laser field, using a velocity map imaging technique. The recorded momentum distribution strongly depends on the delay between the attosecond pulses and the laser field. We interpret the interference patterns observed for different delays using numerical and analytical calculations within the strong field approximation.

  5. Calculations of Photoemission from Rutile

    Science.gov (United States)

    Hjalmarson, Harold; Schultz, Peter; Moore, Chris

    2015-03-01

    Photoemission is a well-known mechanism for release of electrons from a surface during electrical breakdown of a gas such as air. During air breakdown, UV photons, which are emitted from the highly excited gas molecules, are absorbed in the surfaces such as the cathode and the anode. These absorbed photons create energetic electrons, and a small portion of these electrons reach the surface. Those that overcome the potential energy barrier at the surface tend to be emitted. In this talk, the Boltzmann equation that describes these phenomena is formulated. A Monte Carlo probabilistic method is used to obtain the rate of electron emission as a function of photon energy. The role of bandstructure effects will be discussed. This bandstructure information is obtained by using a density-functional theory (DFT) method. Sandia National Laboratories is a multi-program laboratory managed and operated by Sandia Corporation, a wholly owned subsidiary of Lockheed Martin Corporation, for the U.S. Department of Energy's National Nuclear Security Administration under contract DE-AC04-94AL85000.

  6. Direct observation of spin-resolved full and empty electron states in ferromagnetic surfaces

    Energy Technology Data Exchange (ETDEWEB)

    Berti, G., E-mail: giulia.berti@polimi.it; Calloni, A.; Brambilla, A.; Bussetti, G.; Duò, L.; Ciccacci, F. [Dipartimento di Fisica, Politecnico di Milano, Piazza Leonardo da Vinci 32, I-20133, Milano (Italy)

    2014-07-15

    We present a versatile apparatus for the study of ferromagnetic surfaces, which combines spin-polarized photoemission and inverse photoemission spectroscopies. Samples can be grown by molecular beam epitaxy and analyzed in situ. Spin-resolved photoemission spectroscopy analysis is done with a hemispherical electron analyzer coupled to a 25 kV-Mott detector. Inverse photoemission spectroscopy experiments are performed with GaAs crystals as spin-polarized electron sources and a UV bandpass photon detector. As an example, measurements on the oxygen passivated Fe(100)-p(1×1)O surface are presented.

  7. Bulk photoemission from metal films and nanoparticles

    Energy Technology Data Exchange (ETDEWEB)

    Ikhsanov, R Sh [Research Institute of Scientific Instruments, ' Rosatom' ' State Atomic Energy Corporation (Russian Federation); Babicheva, V E [Technical University of Denmark (Denmark); Protsenko, I E; Uskov, A V [P N Lebedev Physics Institute, Russian Academy of Sciences, Moscow (Russian Federation); Guzhva, M E [St. Petersburg State Politechnical University, St. Petersburg (Russian Federation)

    2015-01-31

    Internal emission of photoelectrons from metal films and nanoparticles (nanowires and nanospheres) into a semiconductor matrix is studied theoretically by taking into account the jump of the effective electron mass at the metal – semiconductor interface and the cooling effect of hot electrons due to electron – electron collisions in the metal. The internal quantum efficiency of photoemission for the film and nanoparticles of two types (nanospheres and nanowires) is calculated. It is shown that the reduction of the effective mass of the electron during its transition from metal to semiconductor may lead to a significant (orders of magnitude and higher) decrease in the internal quantum efficiency of bulk photoemission. (nanostructures)

  8. Multidimensional photoemission spectroscopy—the space-charge limit

    Science.gov (United States)

    Schönhense, B.; Medjanik, K.; Fedchenko, O.; Chernov, S.; Ellguth, M.; Vasilyev, D.; Oelsner, A.; Viefhaus, J.; Kutnyakhov, D.; Wurth, W.; Elmers, H. J.; Schönhense, G.

    2018-03-01

    Photoelectron spectroscopy, especially at pulsed sources, is ultimately limited by the Coulomb interaction in the electron cloud, changing energy and angular distribution of the photoelectrons. A detailed understanding of this phenomenon is crucial for future pump-probe photoemission studies at (x-ray) free electron lasers and high-harmonic photon sources. Measurements have been performed for Ir(111) at hν = 1000 eV with photon flux densities between ˜102 and 104 photons per pulse and μm2 (beamline P04/PETRA III, DESY Hamburg), revealing space-charge induced energy shifts of up to 10 eV. In order to correct the essential part of the energy shift and restore the electron distributions close to the Fermi energy, we developed a semi-analytical theory for the space-charge effect in cathode-lens instruments (momentum microscopes, photoemission electron microscopes). The theory predicts a Lorentzian profile of energy isosurfaces and allows us to quantify the charge cloud from measured energy profiles. The correction is essential for the determination of the Fermi surface, as we demonstrate by means of ‘k-space movies’ for the prototypical high-Z material tungsten. In an energy interval of about 1 eV below the Fermi edge, the bandstructure can be restored up to substantial shifts of ˜7 eV. Scattered photoelectrons strongly enhance the inelastic background in the region several eV below E F, proving that the majority of scattering events involves a slow electron. The correction yields a gain of two orders of magnitude in usable intensity compared with the uncorrected case (assuming a tolerable shift of 250 meV). The results are particularly important for future experiments at SASE-type free electron lasers, since the correction also works for strongly fluctuating (but known) pulse intensities.

  9. Photoemission from optoelectronic materials and their nanostructures

    CERN Document Server

    Ghatak, Kamakhya Prasad; Bhattacharya, Sitangshu

    2009-01-01

    This monograph investigates photoemission from optoelectronic materials and their nanostructures. It contains open-ended research problems which form an integral part of the text and are useful for graduate courses as well as aspiring Ph.D.'s and researchers..

  10. Femtosecond spectroscopic imaging by time-of-flight photoemission electron microscopy

    Science.gov (United States)

    Min, Chang-Ki; Kim, Jeong Won; Park, Yongsup

    2007-10-01

    Advances in electron optics and fast-pulsed light sources have enabled the imaging of nanoscale structures with simultaneous energy and time resolutions. We present the results obtained from a time-resolved time-of-flight photoemission electron microscopy (TR-TOF-PEEM) system. This system combined the spatial resolution of conventional PEEM with the time resolution of a femtosecond-pulsed laser and the energy resolution of a TOF energy analyzer. The TOF-PEEM system consists of three electrostatic lenses in front, a drift tube for the measurement of TOF, and a delay line detector (DLD) at the end of the optics. The excitation source is femtosecond pulses from a cavity-dumped Ti:sapphire oscillator that is frequency-doubled to 400 nm using a β-barium borate (BBO) crystal. Using a pump-probe two-photon photoemission technique, we demonstrate an example of sub-100 nm space-resolved ultrafast time evolution of the electron energy spectra for the plasmon resonance of an Ag-coated Si nanostructure, which exhibited unexpectedly intense high energy photoemission signals that show different time evolution between bright and dark regions in a PEEM image.

  11. Hard X-ray photoemission spectroscopy

    International Nuclear Information System (INIS)

    Kobayashi, Keisuke

    2009-01-01

    Except in the very early stage of the development of X-ray photoemission spectroscopy (XPS) by Kai Siegbahn and his coworkers, the excitation sources for XPS studies have predominantly been the Al Kα and Mg Kα emission lines. The advent of synchrotron radiation sources opened up the possibility of tuning the excitation photon energy with much higher throughputs for photoemission spectroscopy, however the excitation energy range was limited to the vacuum ultra violet and soft X-ray regions. Over the past 5-6 years, bulk-sensitive hard X-ray photoemission spectroscopy using high-brilliance high-flux X-rays from third generation synchrotron radiation facilities has been developed. This article reviews the history of HXPES covering the period from Kai Siegbahn and his coworkers' pioneering works to the present, and describes the fundamental aspects, instrumentation, applications to solid state physics, applied physics, materials science, and industrial applications of HXPES. Finally, several challenging new developments which have been conducted at SPring-8 by collaborations among several groups are introduced.

  12. Time-Resolved 2PPE and Time-Resolved PEEM as a Probe of LSP's in Silver Nanoparticles

    Directory of Open Access Journals (Sweden)

    D. Bayer

    2008-01-01

    Full Text Available The time-resolved two-photon photoemission technique (TR-2PPE has been applied to study static and dynamic properties of localized surface plasmons (LSP in silver nanoparticles. Laterally, integrated measurements show the difference between LSP excitation and nonresonant single electron-hole pair creation. Studies below the optical diffraction limit were performed with the detection method of time-resolved photoemission electron microscopy (TR-PEEM. This microscopy technique with a resolution down to 40 nm enables a systematic study of retardation effects across single nanoparticles. In addition, as will be shown in this paper, it is a highly sensitive sensor for coupling effects between nanoparticles.

  13. Photoemission starting of induction rf-driven multicusp ion sources

    International Nuclear Information System (INIS)

    Pickard, D.S.; Leung, K.N.; Perkins, L.T.; Ponce, D.M.; Young, A.T.

    1996-01-01

    It has been demonstrated that pulsed and continuous wave, rf-driven hydrogen discharges can be started with photoemission. The extracted H - current from a photoemission-started plasma has been investigated and does not differ significantly from that of a filament-started plasma. The minimum pressure for photoemissive starting was found to be higher than that of filament starting, 17 mTorr compared to 7 mTorr, respectively, in this particular configuration. copyright 1996 American Institute of Physics

  14. Increased electron photoemission from plasmonic nanoparticles and photoemission enhanced solar cells

    DEFF Research Database (Denmark)

    Novitsky, Andrey; Uskov, Alexander; Gritti, Claudia

    2011-01-01

    Numerical simulation shows possibility to enhance substantially (by one-two orders) the electron photoemission through surface of metal nanoparticles embedded into photovoltaic structures. This, in turn, can lead to increase of the solar cells efficiency due to efficient light-to-electricity tran......Numerical simulation shows possibility to enhance substantially (by one-two orders) the electron photoemission through surface of metal nanoparticles embedded into photovoltaic structures. This, in turn, can lead to increase of the solar cells efficiency due to efficient light...

  15. Band structure of Heusler compounds studied by photoemission and tunneling spectroscopy

    Energy Technology Data Exchange (ETDEWEB)

    Arbelo Jorge, Elena

    2011-07-01

    Heusler compounds are key materials for spintronic applications. They have attracted a lot of interest due to their half-metallic properties predicted by band structure calculations. The aim of this work is to evaluate experimentally the validity of the predictions of half metallicity by band structure calculations for two specific Heusler compounds, Co{sub 2}FeAl{sub 0.3}Si{sub 0.7} and Co{sub 2}MnGa. Two different spectroscopy methods for the analysis of the electronic properties were used: Angular Resolved Ultraviolet Photoemission Spectroscopy (ARUPS) and Tunneling Spectroscopy. Heusler compounds are prepared as thin films by RF-sputtering in an ultra high vacuum system. For the characterization of the samples, bulk and surface crystallographic and magnetic properties of Co{sub 2}FeAl{sub 0.3}Si{sub 0.7} and Co{sub 2}MnGa are studied. X-ray and electron diffraction reveal a bulk and surface crossover between two different types of sublattice order (from B2 to L2{sub 1}) with increasing annealing temperature. X-ray magnetic circular dichroism results show that the magnetic properties in the surface and bulk are identical, although the magnetic moments obtained are 5 % below from the theoretically predicted. By ARUPS evidence for the validity of the predicted total bulk density of states (DOS) was demonstrated for both Heusler compounds. Additional ARUPS intensity contributions close to the Fermi energy indicates the presence of a specific surface DOS. Moreover, it is demonstrated that the crystallographic order, controlled by annealing, plays an important role on broadening effects of DOS features. Improving order resulted in better defined ARUPS features. Tunneling magnetoresistance measurements of Co{sub 2}FeAl{sub 0.3}Si{sub 0.7} and Co{sub 2}MnGa based MTJ's result in a Co{sub 2}FeAl{sub 0.3}Si{sub 0.7} spin polarization of 44 %, which is the highest experimentally obtained value for this compound, although it is lower than the 100 % predicted. For Co

  16. UNCONTROLLED PHOTOMULTIPLIER CURRENT IN PHOTOEMISSION ANALYSIS

    Directory of Open Access Journals (Sweden)

    K. A. Viazava

    2016-01-01

    Full Text Available The dependence of photon energy from energy of photoelectron is base of photoemission radiation analysis. In such photoemission measurements except current of photocathode is always exist a reverse current from the collector of electrons to the photocathode in two-electrode sensors. There are various ways of reverse and uncontrolled current eliminating or reducing their influence. The constructive method is based on creating an electron-optical system of photoelectronic device, which would be a photoelectron energy analyzer. The second method – technological. However, it requires the manufacture of the photocathode and the dynode system in different vacuum chamber with subsequent connection to a single device in vacuum environment without exposure to the atmosphere. The purpose of this article is to determinate the effect of photoemission from photocathode chamber and the first dynode of photomultiplier on energy distribution of the photoelectrons from photocathode. To solve this problem authors obtained calibration curves for measuring pyrometer module ПИФ 4/2 with ФЭУ-114 as a sensor at supply voltage 1350 V and different decelerating voltages. The effect of illumination on the value of modulation coefficient on temperature k(T and wavelength k(λ is shown. In temperature measurements, this effect is evident in fact that at temperatures below 1400 K linear dependence ln k – T-1 is broken. Still this linear dependence is a necessary consequence of the fact that the measured temperature is color temperature. However, this calibration curve can be used to measure low temperature if the target measurements condition and calibration conditions are identical. In wavelength calibration, curve k(λ at λ > 760 nm is two-valued, that doesn’t allow to identify monochromatic radiation by this method and bring in errors in temperature measurements. 

  17. Scanning photoemission microscopy with synchrotron radiation

    Science.gov (United States)

    Ade, Harald W.

    1992-08-01

    Progress in photoemission spectro-microscopy at various synchrotron radiation facilities is reviewed. Microprobe devices such as MAXIMUM at the SRC in Wisconsin, the X1-SPEM at the NSLS at BNL, as well as the ellipsoidal ring mirror microscope at DESY in Hamburg, recorded first images during the last few years. The present status of these devices which achieve their lateral resolution by focusing X-rays to a small spot is the primary focus of this paper, but work representing other approaches to spectro-microscopy is also discussed.

  18. Angular Accelerating White Light

    CSIR Research Space (South Africa)

    Dudley, Angela L

    2015-08-01

    Full Text Available angular acceleration during propagation which is achieved by superpositions of Bessel beams with non-canonical phase functions. They demonstrate these angular accelerating fields by modulating the phase and amplitude of a supercontinuum source with the use...

  19. Electronic structure and photoemission spectra of thin (GaAs).sub.n./sub. (AlAs).sub.n./sub. superlattices

    Czech Academy of Sciences Publication Activity Database

    Bartoš, Igor; Strasser, T.; Schattke, W.

    507-510, - (2002), s. 160-164 ISSN 0039-6028 R&D Projects: GA AV ČR IAA1010108 Institutional research plan: CEZ:AV0Z1010914 Keywords : electron density * excitation spectra calculations * Green's function methods * angle resolved photoemission * photoelectron emission * Gallium arsenide * low index single crystal surfaces * superlattices Subject RIV: BM - Solid Matter Physics ; Magnetism Impact factor: 2.140, year: 2002

  20. Photoemission from alfa and beta phases of the GaAs(001)-c(4x4) surface

    Czech Academy of Sciences Publication Activity Database

    Jiříček, Petr; Cukr, Miroslav; Bartoš, Igor; Sadowski, J.

    2009-01-01

    Roč. 603, č. 20 (2009), s. 3088-3093 ISSN 0039-6028 R&D Projects: GA ČR GA202/07/0601; GA AV ČR IAA100100628 Institutional research plan: CEZ:AV0Z10100521 Keywords : gallium arsenide * angle resolved photoemission * synchrotron radiation photoelectron spectroscopy * molecular beam epitaxy * surface core level shift Subject RIV: BM - Solid Matter Physics ; Magnetism Impact factor: 1.798, year: 2009

  1. Photoemission perspective on pseudogap, superconducting fluctuations, and charge order: a review of recent progress.

    Science.gov (United States)

    Vishik, Inna

    2018-03-29

    In the course of seeking the microscopic mechanism of superconductivity in cuprate high temperature superconductors, the pseudogap phase\\textemdash the very abnormal 'normal' state on the hole-doped side\\textemdash has proven to be as big of a quandary as superconductivity itself. Angle-resolved photoemission spectroscopy (ARPES) is a powerful tool for assessing the momentum-dependent phenomenology of the pseudogap, and recent technological developments have permitted a more detailed understanding. This report reviews recent progress in understanding the relationship between superconductivity and the pseudogap, the Fermi arc phenomena, and the relationship between charge order and pseudogap from the perspective of ARPES measurements. © 2018 IOP Publishing Ltd.

  2. Photoemission and magnetic response in the bipolaronic superconductor

    CERN Document Server

    Dent, C

    2001-01-01

    in the cuprates is extended to explain the crossing point in the curves of induced magnetization divided by the square root of field against temperature in the less anisotropic cuprates. This model has already been shown to provide a parameter-free expression for T sub c in a wide range of cuprates. We compare our results with experiment in YBa sub 2 Cu sub 3 O sub 7 sub - subdelta. A theory of angle-resolved photoemission (ARPES) in doped charge-transfer Mott insulators is developed taking into account the realistic band structure, (bi)polaron formation due to the strong electron-phonon interaction, and a random field potential. We derive the coherent part of the ARPES spectra with the oxygen hole spectral function calculated in the non-crossing (ladder) approximation and with the exact spectral function of a one-dimensional hole in a random potential. On the basis of this theory, explanations are proposed for several features of the ARPES spectra taken from the cuprate superconductors. These include the pol...

  3. Theory of temperature dependent photoemission spectrum of heavy fermion semiconductors

    International Nuclear Information System (INIS)

    Riseborough, P.S.

    1998-01-01

    The heavy fermion semiconductors are a class of strongly correlated materials, that at high temperatures show properties similar to those of heavy fermion materials, but at low temperatures show a cross-over into a semi-conducting state. The low temperature insulating state is characterized by an anomalously small energy gap, varying between 10 and 100 K. The smallness of the gap is attributed to the result of a many-body renormalization, and is temperature dependent. The temperature dependence of the electronic spectral density of states is calculated, using the Anderson lattice model at half filling. The spectrum is calculated to second order in 1/N, where N is the degeneracy of the 'f' orbitals, using a slave boson technique. The system is an indirect gap semi-conductor, with an extremely temperature dependent electronic spectral density A(k, ω). The indirect gap is subject to a temperature dependent many-body renormalization, and leads to a sharp temperature dependent structure in the angle resolved photo-emission spectrum at the indirect threshold. The theoretical predictions are compared with experimental observations on FeSi. (Copyright (1998) World Scientific Publishing Co. Pte. Ltd)

  4. Professional AngularJS

    CERN Document Server

    Karpov, Valeri

    2015-01-01

    A comprehensive guide to AngularJS, Google's open-source client-side framework for app development. Most of the existing guides to AngularJS struggle to provide simple and understandable explanations for more advanced concepts. As a result, some developers who understand all the basic concepts of AngularJS struggle when it comes to building more complex real-world applications. Professional AngularJS provides a thorough understanding of AngularJS, covering everything from basic concepts, such as directives and data binding, to more advanced concepts like transclusion, build systems, and auto

  5. Molecular photoemission studies using synchrotron radiation

    International Nuclear Information System (INIS)

    Truesdale, C.M.

    1983-04-01

    The angular distributions of photoelectrons and Auger electrons were measured by electron spectroscopy using synchrotron radiation. The experimental results are compared with theoretical calculations to interpret the electronic behavior of photoionization for molecular systems

  6. High-energy photoemission studies of oxide interfaces

    Science.gov (United States)

    Claessen, Ralph

    2015-03-01

    The interfaces of complex oxide heterostructures can host novel quantum phases not existing in the bulk of the constituents, with the high-mobility 2D electron system (2DES) in LaAlO3/SrTiO3 (LAO/STO) representing a prominent example. Despite extensive research the origin of the 2DES and its unusual properties - including the supposed coexistence of superconductivity and ferromagnetism - are still a matter of intense debate. Photoelectron spectroscopy, recently extended into the soft (SX-ARPES) and hard (HAXPES) X-ray regime, is a powerful method to provide detailed insight into the electronic structure of these heterostructures and, in particular, of the buried interface. This includes the identification of the orbital character of the 2DES as well as the determination of vital band structure information, such as band alignment, band bending, and even k-resolved band dispersions and Fermi surface topology. Moreover, resonant photoemission at the Ti L-edge reveals the existence of two different species of Ti 3d states, localized and itinerant, which can be distinguished and identified by their different resonance behavior. The role of oxygen vacancies is studied by controlled in-situ oxidation, which allows us to vary the composition from fully stoichiometric to strongly O-deficient. By comparison to free STO surfaces we can thus demonstrate that the metallicity of the heteointerfaces is intrinsic, i . e . it persists even in the absence of O defects. I will discuss our photoemission results on LAO/STO heterostructures in both (100) and (111) orientation as well as on the related system γ-Al2O3/STO(100), which also hosts a 2DES with an even higher mobility. Work in collaboration with J. Mannhart (MPI-FKF, Stuttgart), N. Pryds (TU Denmark), G. Rijnders (U Twente), S. Suga (U Osaka), M. Giorgoi (BESSY, HZB), W. Drube (DESY Photon Science), V.N. Strocov (Swiss Light Source), J. Denlinger (Advanced Light Source, LBNL), and T.-L. Lee (Diamond Light Source). Support by

  7. Timing analysis of two-electron photoemission

    International Nuclear Information System (INIS)

    Kheifets, A S; Ivanov, I A; Bray, Igor

    2011-01-01

    We predict a significant delay of two-electron photoemission from the helium atom after absorption of an attosecond XUV pulse. We establish this delay by solving the time-dependent Schroedinger equation and by subsequently tracing the field-free evolution of the two-electron wave packet. This delay can also be related to the energy derivative of the phase of the complex double-photoionization (DPI) amplitude which we evaluate by using the convergent close-coupling method. Our observations indicate that future attosecond time delay measurements on DPI of He can provide information on the absolute quantum phase and elucidate various mechanisms of this strongly correlated ionization process. (fast track communication)

  8. Angular correlation methods

    International Nuclear Information System (INIS)

    Ferguson, A.J.

    1974-01-01

    An outline of the theory of angular correlations is presented, and the difference between the modern density matrix method and the traditional wave function method is stressed. Comments are offered on particular angular correlation theoretical techniques. A brief discussion is given of recent studies of gamma ray angular correlations of reaction products recoiling with high velocity into vacuum. Two methods for optimization to obtain the most accurate expansion coefficients of the correlation are discussed. (1 figure, 53 references) (U.S.)

  9. Final state selection in the 4p photoemission of Rb by combining laser spectroscopy with soft-x-ray photoionization

    International Nuclear Information System (INIS)

    Schulz, J.; Tchaplyguine, M.; Rander, T.; Bergersen, H.; Lindblad, A.; Oehrwall, G.; Svensson, S.; Heinaesmaeki, S.; Sankari, R.; Osmekhin, S.; Aksela, S.; Aksela, H.

    2005-01-01

    Fine structure resolved 4p photoemission studies have been performed on free rubidium atoms in the ground state and after excitation into the [Kr]5p 2 P 1/2 and 2 P 3/2 states. The 4p 5 5p final states have been excited in the 4p 6 5s→4p 5 5p conjugate shakeup process from ground state atoms as well as by direct photoemission from laser excited atoms. The relative intensities differ considerably in these three excitation schemes. The differences in the laser excited spectra could be described well using calculations based on the pure jK-coupling scheme. Thereby it was possible to specify the character of the various final states. Furthermore it has been possible to resolve two of the final states whose energy separation is smaller than the experimental resolution by selectively exciting them in a two step scheme, where the laser selects the spin-orbit coupling in the intermediate state and determines the final state coupling after x-ray photoemission

  10. Angular Acceleration without Torque?

    Science.gov (United States)

    Kaufman, Richard D.

    2012-01-01

    Hardly. Just as Robert Johns qualitatively describes angular acceleration by an internal force in his article "Acceleration Without Force?" here we will extend the discussion to consider angular acceleration by an internal torque. As we will see, this internal torque is due to an internal force acting at a distance from an instantaneous center.

  11. Rotations and angular momentum

    International Nuclear Information System (INIS)

    Nyborg, P.; Froyland, J.

    1979-01-01

    This paper is devoted to the analysis of rotational invariance and the properties of angular momentum in quantum mechanics. In particular, the problem of addition of angular momenta is treated in detail, and tables of Clebsch-Gordan coefficients are included

  12. Photoemission studies using laboratory and synchrotron sources

    International Nuclear Information System (INIS)

    Phase, D.M.

    2012-01-01

    Synchrotron radiation sources, providing intense, polarized and stable beams of ultra violet soft and hard X-ray photons, are having great impact on physics, chemistry, biology materials science and other areas research. In particular synchrotron radiation has revolutionized photoelectron spectroscopy by enhancing its capabilities for investigating the electronic properties of solids. The first Indian synchrotron storage ring, Indus- 1 is in operation at RRCAT, Indore. The UGC-DAE CSR with the help of university scientist had designed and developed an angle integrated photoelectron spectroscopy (PES) beamline on this 450 MeV storage ring. A storage ring of this kind is most suitable for investigation in the energy range from few electron volts to around five hundred electron volts. In this lecture we will describe the details of PES beamline and its experimental station. Till date the different university users carried out photoemission measurements on variety of samples. Some of the spectra recorded by users will be presented in order to show the capability of this beamline. In the later part we will report a review of our recent research work carried out on dilute magnetic thin films using this beamline. (author)

  13. Spectrally resolved longitudinal spatial coherence inteferometry

    Science.gov (United States)

    Woodard, Ethan R.; Kudenov, Michael W.

    2017-05-01

    We present an alternative imaging technique using spectrally resolved longitudinal spatial coherence interferometry to encode a scene's angular information onto the source's power spectrum. Fourier transformation of the spectrally resolved channeled spectrum output yields a measurement of the incident scene's angular spectrum. Theory for the spectrally resolved interferometric technique is detailed, demonstrating analogies to conventional Fourier transform spectroscopy. An experimental proof of concept system and results are presented using an angularly-dependent Fabry-Perot interferometer-based optical design for successful reconstruction of one-dimensional sinusoidal angular spectra. Discussion for a potential future application of the technique, in which polarization information is encoded onto the source's power spectrum is also given.

  14. Quark Orbital Angular Momentum

    Directory of Open Access Journals (Sweden)

    Burkardt Matthias

    2015-01-01

    Full Text Available Definitions of orbital angular momentum based on Wigner distributions are used as a framework to discuss the connection between the Ji definition of the quark orbital angular momentum and that of Jaffe and Manohar. We find that the difference between these two definitions can be interpreted as the change in the quark orbital angular momentum as it leaves the target in a DIS experiment. The mechanism responsible for that change is similar to the mechanism that causes transverse single-spin asymmetries in semi-inclusive deep-inelastic scattering.

  15. Optical Angular Momentum

    International Nuclear Information System (INIS)

    Arimondo, Ennio

    2004-01-01

    For many years the Institute of Physics has published books on hot topics based on a collection of reprints from different journals, including some remarks by the editors of each volume. The book on Optical Angular Momentum, edited by L Allen, S M Barnett and M J Padgett, is a recent addition to the series. It reproduces forty four papers originally published in different journals and in a few cases it provides direct access to works not easily accessible to a web navigator. The collection covers nearly a hundred years of progress in physics, starting from an historic 1909 paper by Poynting, and ending with a 2002 paper by Padgett, Barnett and coworkers on the measurement of the orbital angular momentum of a single photon. The field of optical angular momentum has expanded greatly, creating an interdisciplinary attraction for researchers operating in quantum optics, atomic physics, solid state physics, biophysics and quantum information theory. The development of laser optics, especially the control of single mode sources, has made possible the specific design of optical radiation modes with a high degree of control on the light angular momentum. The editors of this book are important figures in the field of angular momentum, having contributed to key progress in the area. L Allen published an historical paper in 1999, he and M J Padgett (together with M Babiker) produced few years ago a long review article which is today still the most complete basic introduction to the angular momentum of light, while S M Barnett has contributed several high quality papers to the progress of this area of physics. The editors' choice provides an excellent overview to all readers, with papers classified into eight different topics, covering the basic principles of the light and spin and orbital angular momentum, the laboratory tools for creating laser beams carrying orbital angular momentum, the optical forces and torques created by laser beams carrying angular momentum on

  16. Comparison between laser-induced photoemissions and phototransmission of hard tissues using fibre-coupled Nd:YAG and Er(3+)-doped fibre lasers.

    Science.gov (United States)

    El-Sherif, Ashraf Fathy

    2012-07-01

    During pulsed laser irradiation of dental enamel, laser-induced photoemissions result from the laser-tissue interaction through mechanisms including fluorescence and plasma formation. Fluorescence induced by non-ablative laser light interaction has been used in tissue diagnosis, but the photoemission signal accompanying higher power ablative processes may also be used to provide real-time monitoring of the laser-tissue interaction. The spectral characteristics of the photoemission signals from normal and carious tooth enamel induced by two different pulsed lasers were examined. The radiation sources compared were a high-power extra-long Q-switched Nd:YAG laser operating at a wavelength of 1,066 nm giving pulses (with pulse durations in the range 200-250 μs) in the near infrared and a free-running Er(3+)-doped ZBLAN fibre laser operating at a wavelength near 3 μm with similar pulse durations in the mid-infrared region. The photoemission spectra produced during pulsed laser irradiation of enamel samples were recorded using a high-resolution spectrometer with a CCD array detector that enabled an optical resolution as high as 0.02 nm (FWHM). The spectral and time-dependence of the laser-induced photoemission due to thermal emission and plasma formation were detected during pulsed laser irradiation of hard tissues and were used to distinguish between normal and carious teeth. The use of these effects to distinguish between hard and soft biological tissues during photothermal ablation with a pulsed Nd:YAG laser or an Er fibre laser appears feasible. The real-time spectrally resolved phototransmission spectrum produced during pulsed Nd:YAG laser irradiation of human tooth enamel samples was recorded, with a (normalized) relative transmission coefficient of 1 (100%) for normal teeth and 0.6 (60%) for the carious teeth. The photoemission signal accompanying ablative events may also be used to provide real-time monitoring of the laser-tissue interaction.

  17. DC photoemission electron guns as ERL sources

    International Nuclear Information System (INIS)

    Sinclair, Charles K.

    2006-01-01

    Very-high-voltage DC electron guns, delivering moderate duration bunches from photoemission cathodes, and followed by conventional drift bunching and acceleration, offer a practical solution for an ERL injector. In a variant of this scheme, a DC gun is placed in close proximity to a superconducting RF accelerator cavity, with few or no active elements between the gun and cavity. The principal technical challenge with such electron guns arises from field emission from the cathode electrode and its support structure. Field emission may result in voltage breakdown across the cathode-anode gap, or a punch-through failure of the insulator holding off the cathode potential, as well as lesser though still serious problems. Various means to mitigate these problems are described. The operational lifetime of high quantum efficiency photocathodes in these guns is determined by the vacuum conditions, through phenomena such as chemical poisoning and ion back-bombardment. Minimization of the field strength on electrode structures pushes high-voltage DC guns toward large dimensions and, correspondingly, large outgassing loads, but it is also true that these guns offer many opportunities for achieving excellent vacuum conditions. Good solutions to vacuum problems that had previously limited cathode lifetime have been demonstrated in recent years. Designs for DC guns presently in use and planned for the near future will be described. The parameters necessary for a 100 mA average current, very-high-voltage DC gun with a photocathode operational lifetime greater than 100 h appear to be within reach, but have yet to be demonstrated. A 1 A average current source with good cathode operational lifetime will require developments beyond the present state-of-the-art

  18. Spectroscopic imaging, diffraction, and holography with x-ray photoemission

    International Nuclear Information System (INIS)

    1992-02-01

    X-ray probes are capable of determining the spatial structure of an atom in a specific chemical state, over length scales from about a micron all the way down to atomic resolution. Examples of these probes include photoemission microscopy, energy-dependent photoemission diffraction, photoelectron holography, and X-ray absorption microspectroscopy. Although the method of image formation, chemical-state sensitivity, and length scales can be very different, these X-ray techniques share a common goal of combining a capability for structure determination with chemical-state specificity. This workshop will address recent advances in holographic, diffraction, and direct imaging techniques using X-ray photoemission on both theoretical and experimental fronts. A particular emphasis will be on novel structure determinations with atomic resolution using photoelectrons

  19. Spectroscopic imaging, diffraction, and holography with x-ray photoemission

    Energy Technology Data Exchange (ETDEWEB)

    1992-02-01

    X-ray probes are capable of determining the spatial structure of an atom in a specific chemical state, over length scales from about a micron all the way down to atomic resolution. Examples of these probes include photoemission microscopy, energy-dependent photoemission diffraction, photoelectron holography, and X-ray absorption microspectroscopy. Although the method of image formation, chemical-state sensitivity, and length scales can be very different, these X-ray techniques share a common goal of combining a capability for structure determination with chemical-state specificity. This workshop will address recent advances in holographic, diffraction, and direct imaging techniques using X-ray photoemission on both theoretical and experimental fronts. A particular emphasis will be on novel structure determinations with atomic resolution using photoelectrons.

  20. Simulation and characterization of the crystal growth by photoemission

    International Nuclear Information System (INIS)

    Fazouan, N.

    1994-01-01

    In this thesis, we argue in favour of photoemission as an in-situ characterization tool for the homo-epitaxial growth of GaAs. The first part, is concerned with the interpretation of the origin of the photoemission oscillations as first observed by J.N. Eckstein and al during MBE growth of GaAs. To study this effect, two approaches have been used. These approaches are based on reaction surface and roughness observations to study the growth mode. They associate the photoemission current with the presence of uncovered gallium adatoms, i.e. those which do not have an arsenic atom above them. The first approach is based on chemical rate theory, whereas the second is based on an atomistic simulation of GaAs homo-epitaxy. This last approach introduces the notion of interlayer migration processes and uses a Monte Carlo technique to look at the temporal evolution of the configuration and hence the morphology. It is shown with these two approaches that the photoemission current has similar characteristics as to those of RHEED, c.g.the same oscillation period. The results obtained have shown the relationship between the photoemission oscillations amplitude and the growth mode which are determined by the mechanisms of absorption and diffusion of gallium atoms and arsenic atoms of molecules. Finally, the study of the effect of the surface reactions shows the importance of these in the case where arsenic is supplied in molecular form (As 2 ). The last part concerns the experimental measurements at the threshold photoemission current during epitaxial growth of GaAs by metal-organic vapour phase epitaxy (MOVPE). The objective of this experimental study is to test the good running of the photo-assisted MOVPE low pressure system and to study the possibilities offered by this as an in-situ diagnostic tool for MOVPE. (author). 101 refs., 80 figs., 6 tabs

  1. High-Resolution Resonance Photoemission Study of CeNi

    International Nuclear Information System (INIS)

    Sekiyama, A.; Kadono, K.; Iwasaki, T.; Imada, S.; Kasai, S.; Suga, S.; Araki, S.; Onuki, Y.

    2003-01-01

    We have performed the high-resolution Ce 3d - 4f resonance photoemission study of a considerably hybridized CeNi with the Kondo temperature of ∼ 150 K. The tail of the Kondo-resonance peak is predominantly observed in the bulk Ce 4f photoemission spectra, where its spin-orbit partner is suppressed compared with the so far reported surface-sensitive Ce 4d-4f resonance spectrum. Our results show that the bulk 4f electronic states are essentially understood by the single impurity Anderson model. (author)

  2. Photoemission study of S adsorption on GaAs (0 0 1)

    International Nuclear Information System (INIS)

    Strasser, T; Kipp, L; Skibowski, M; Schattke, W

    2005-01-01

    Angle-resolved photoemission spectra have been calculated with the one-step model for S/GaAs(0 0 1) and compared with experimental distributions. The data are analysed in terms of the ideal 1 x 1 and, furthermore, of the reconstructed 2 x 6 surface which is assumed to be closest to the experimentally realized structure. Emissions are characterized by electronic structure terms such as energy bands and orbital composition, though partly also by geometric properties. In particular, the determination of the second layer as consisting of Ga atoms has been achieved because of the distinct differences in the theoretical spectra with S-Ga and those with S-As bonds

  3. Fission fragment angular momentum

    International Nuclear Information System (INIS)

    Frenne, D. De

    1991-01-01

    Most of the energy released in fission is converted into translational kinetic energy of the fragments. The remaining excitation energy will be distributed among neutrons and gammas. An important parameter characterizing the scission configuration is the primary angular momentum of the nascent fragments. Neutron emission is not expected to decrease the spin of the fragments by more than one unit of angular momentum and is as such of less importance in the determination of the initial fragment spins. Gamma emission is a suitable tool in studying initial fragment spins because the emission time, number, energy, and multipolarity of the gammas strongly depend on the value of the primary angular momentum. The main conclusions of experiments on gamma emission were that the initial angular momentum of the fragments is large compared to the ground state spin and oriented perpendicular to the fission axis. Most of the recent information concerning initial fragment spin distributions comes from the measurement of isomeric ratios for isomeric pairs produced in fission. Although in nearly every mass chain isomers are known, only a small number are suitable for initial fission fragment spin studies. Yield and half-life considerations strongly limit the number of candidates. This has the advantage that the behavior of a specific isomeric pair can be investigated for a number of fissioning systems at different excitation energies of the fragments and fissioning nuclei. Because most of the recent information on primary angular momenta comes from measurements of isomeric ratios, the global deexcitation process of the fragments and the calculation of the initial fragment spin distribution from measured isomeric ratios are discussed here. The most important results on primary angular momentum determinations are reviewed and some theoretical approaches are given. 45 refs., 7 figs., 2 tabs

  4. Photoelectron spectrometer for high-resolution angular resolved studies

    International Nuclear Information System (INIS)

    Parr, A.C.; Southworth, S.H.; Dehmer, J.L.; Holland, D.M.P.

    1982-01-01

    We report on a new electron spectrometer system designed for use on storage-ring light sources. The system features a large (76 cm dia. x 92 cm long) triply magnetically shielded vacuum chamber and two 10.2 cm mean radius hemispherical electron-energy analyzers. One of the analyzers is fixed and the other is rotatable through about 150 0 . The chamber is pumped by a cryopump and a turbomolecular pump combination so as to enable experiments with a variety of gases under different conditions. The light detection includes both a direct beam monitor and polarization analyzer. The electron detection is accomplished with either a continuous-channel electron multiplier or with multichannel arrays used as area detectors

  5. Electronic structure of elemental curium studied by photoemission

    Czech Academy of Sciences Publication Activity Database

    Gouder, T.; van der Laan, G.; Shick, Alexander; Haire, R.G.; Caciuffo, R.

    2011-01-01

    Roč. 83, č. 12 (2011), "125111-1"-"125111-6" ISSN 1098-0121 R&D Projects: GA ČR(CZ) GAP204/10/0330 Institutional research plan: CEZ:AV0Z10100520 Keywords : photoemission * actinides Subject RIV: BM - Solid Matter Physics ; Magnetism Impact factor: 3.691, year: 2011

  6. Directional uv photoemission from (100) and (110) molybdenum surfaces

    DEFF Research Database (Denmark)

    Cinti, R. C.; Khoury, E. Al; Chakraverty, B. K.

    1976-01-01

    A study of the (100) and (110) molybdenum surfaces by directional photoemission spectroscopy is presented. Energy distribution spectra formed by photoelectrons emitted normal to the surfaces have been measured for photon energies between 10.2 and 21.2 eV. The results are discussed in terms...

  7. CALCULATION OF CU 2P RESONANT PHOTOEMISSION SPECTRA IN CUO

    NARCIS (Netherlands)

    SEINO, Y; OGASAWARA, H; KOTANI, A; THOLE, BT; VANDERLAAN, G

    We investigated theoretically the Cu 2p resonance of 3d, 3p and 3s X-ray photoemission spectra (XPS) in CuO using a cluster model including multiplet coupling, crystal field and anisotropic hybridization. The spectra were calculated by taking into account the radiative transitions up to the first

  8. Time-resolved photoelectron nano-spectroscopy of individual silver particles: Perspectives and limitations

    DEFF Research Database (Denmark)

    Rohmer, Martin; Bauer, Michael; Leissner, Till

    2010-01-01

    Simultaneous time- and energy-resolved two-photon photoemission with nanometer resolution is demonstrated for the first time. We monitor the energy dependence of the decay dynamics of electron excitations in individual silver particles, which were deposited from a gas aggregation cluster source...

  9. Angular momentum projected semiclassics

    International Nuclear Information System (INIS)

    Hasse, R.W.

    1986-10-01

    By using angular momentum projected plane waves as wave functions, we derive semiclassical expressions for the single-particle propagator, the partition function, the nonlocal density matrix, the single-particle density and the one particle- one hole level density for fixed angular momentum and fixed z-component or summed over the z-components. Other quantities can be deduced from the propagator. In coordinate space (r, r') the relevant quantities depend on vertical stroker - r 3 vertical stroke instead of vertical stroker - r'vertical stroke and in Wigner space (R, P) they become proportional to the angular momentum constraints δ(vertical strokeRxPvertical stroke/ℎ - l) and δ((RxP) z /ℎ - m). As applications we calculate the single-particle and one particle- one hole level densities for harmonic oscillator and Hill-Wheeler box potentials and the imaginary part of the optical potential and its volume integral with an underlying harmonic oscillator potential and a zero range two-body interaction. (orig.)

  10. Angular Momentum in Fission

    Science.gov (United States)

    Gönnenwein, F.; Bunakov, V.; Dorvaux, O.; Gagarski, A.; Guseva, I.; Hanappe, F.; Kadmensky, S.; von Kalben, J.; Khlebnikov, S.; Kinnard, V.; Kopatch, Yu.; Mutterer, M.; Nesvizhevsky, V.; Petrov, G.; Prokhorova, E.; Rubchenya, V.; Sillanpää, M.; Simpson, G.; Sokolov, V.; Soldner, T.; Stuttgé, L.; Tiourine, G.; Trzaska, W.; Tsekhanovich, I.; Wagemans, C.; Wollersheim, H.-J.; Zavarukhina, T.; Zimmer, O.

    2008-04-01

    Three novel experiments in spontaneous and thermal neutron induced fission all with a bearing on angular momentum in fission are reviewed. In the first experiment it was observed that, in the reaction 235U(n, f) with incident polarized cold neutrons, the nucleus undergoing scission is rotating. This was inferred from the shift in angular distributions of ternary particles being dependent on the orientation of neutron spin. In the second study the properties of the angular momentum of spherical fission fragments was investigated. Current theories trace the spin of fragments to their deformations allowing for collective rotational vibrations at scission. However, in particular the spherical 132Te isotope exhibits a large spin at variance with theory. Exploiting the specific properties of cold deformed fission it could be proven that, for 132Te, single particle excitations instead of collective modes are responsible for the large spin observed. In a third project a pilot study was exploring the possibility to search for an evaporation of neutrons from fragments being anisotropic in their own cm-system. Due to fragment spin this anisotropy is claimed since decades to exist. It was so far never observed. A scheme has been devised and tested were triple coincidences between a fragment and two neutrons are evaluated in a way to bring the cm-anisotropy into the foreground while getting rid of the kinematical anisotropy in the lab-system due to evaporation from moving fragments. The test was run for spontaneous fission of 252Cf.

  11. Studies of Dirac and Weyl fermions by angle resolved photoemission spectroscopy

    Energy Technology Data Exchange (ETDEWEB)

    Huang, Lunan [Iowa State Univ., Ames, IA (United States)

    2016-01-01

    This dissertation consists of three parts. First, we study magnetic domains in Nd2Fe14B single crystals using high resolution magnetic force microscopy (MFM). In addition to the elongated, wavy nano-domains reported by a previous MFM study, we found that the micrometer size, star-shaped fractal pattern is constructed of an elongated network of nano-domains about 20 nm in width, with resolution-limited domain walls thinner than 2 nm. Second, we studied extra Dirac cones of multilayer graphene on SiC surface by ARPES and SPA-LEED. We discovered extra Dirac cones on Fermi surface due to SiC 6 x 6 and graphene 6√ 3 6√ 3 coincidence lattice on both single-layer and three-layer graphene sheets. We interpreted the position and intensity of the Dirac cone replicas, based on the scattering vectors from LEED patterns. We found the positions of replica Dirac cones are determined mostly by the 6 6 SiC superlattice even graphene layers grown thicker. Finally, we studied the electronic structure of MoTe2 by ARPES and experimentally con rmed the prediction of type II Weyl state in this material. By combining the result of Density Functional Theory calculations and Berry curvature calculations with out experimental data, we identi ed Fermi arcs, track states and Weyl points, all features predicted to exist in a type II Weyl semimetal. This material is an excellent playground for studies of exotic Fermions.

  12. Electronic structure of ion arsenic high temperature superconductors studied by angle resolved photoemission spectroscopy

    Energy Technology Data Exchange (ETDEWEB)

    Liu, Chang [Iowa State Univ., Ames, IA (United States)

    2011-01-01

    The main purpose of the present thesis is to present our ARPES results on the iron arsenic superconductors. As revealed by a series of ARPES measurements on both the AEFe2As2 and the RFeAs(O,F) families (parent compound and carrier-doped systems), the electronic structures of the pnictides are complicated, three dimensional, and closely linked to their superconducting behavior (13; 14; 15; 16; 17; 18; 19). Parent compounds of these materials exhibit the basic hole-electron pocket dual plus an apparent Fermi surface reconstruction caused by long range antiferromagnetism (13; 15). When carriers are introduced, the chemical potential shifts in accordance with the Luttinger theorem and the rigid band shifting picture (13). Importantly, both the appearance and disappearance of the superconducting dome at low and high doping levels have intimate relation with topological changes at the Fermi surfaces, resulting in a specific Fermi topology being favored by superconductivity (15; 16). On the low doping side, superconductivity emerges in the phase diagram once the antiferromagnetic reconstruction disappears below the Fermi level, returning the Fermi surface to its paramagnetic-like appearance. On the high doping side, superconductivity disappears around a doping level at which the central hole pocket vanishes due to increasing electron concentration. Such phenomena are evidence for the governing role the electronic structure plays in their superconducting behavior.

  13. Thermal and Field Enhanced Photoemission Comparison of Theory to Experiment

    CERN Document Server

    Lynn-Jensen, Kevin

    2004-01-01

    Photocathodes are a critical component of high-gain FEL’s and the analysis of their emission is complex. Relating their performance under laboratory conditions to conditions of an rf photoinjector is difficult. Useful models must account for cathode surface conditions and material properties, as well as drive laser parameters. We have developed a time-dependent model accounting for the effects of laser heating and thermal propagation on photoemission. It accounts for surface conditions (coating, field enhancement, reflectivity), laser parameters (duration, intensity, wavelength), and material characteristics (reflectivity, laser penetration depth, scattering rates) to predict current distribution and quantum efficiency. The applicatIon will focus on photoemission from metals and, in particular, dispenser photocathodes: the later introduces complications such as coverage non-uniformity and field enhancement. The performance of experimentally characterized photocathodes will be extrapolated to 0.1 - 1 nC bunch...

  14. Core-level photoemission revealing the Mott transition

    International Nuclear Information System (INIS)

    Kim, Hyeong-Do; Noh, Han-Jin; Kim, K.H.; Oh, S.-J.

    2005-01-01

    Ru 3d core-level X-ray photoemission spectra of various ruthenates are examined. They show in general two-peak structures, which can be assigned as the screened and unscreened peaks. The screened peak is absent in a Mott insulator, but develops into a main peak as the correlation strength becomes weak. This spectral behavior is well explained by the dynamical mean-field theory calculation for the single-band Hubbard model with the on-site core-hole potential using the exact diagonalization method. The new mechanism of the core-level photoemission satellite can be utilized to reveal the Mott transition phenomenon in various strongly correlated electron systems

  15. Optical angular momentum and atoms.

    Science.gov (United States)

    Franke-Arnold, Sonja

    2017-02-28

    Any coherent interaction of light and atoms needs to conserve energy, linear momentum and angular momentum. What happens to an atom's angular momentum if it encounters light that carries orbital angular momentum (OAM)? This is a particularly intriguing question as the angular momentum of atoms is quantized, incorporating the intrinsic spin angular momentum of the individual electrons as well as the OAM associated with their spatial distribution. In addition, a mechanical angular momentum can arise from the rotation of the entire atom, which for very cold atoms is also quantized. Atoms therefore allow us to probe and access the quantum properties of light's OAM, aiding our fundamental understanding of light-matter interactions, and moreover, allowing us to construct OAM-based applications, including quantum memories, frequency converters for shaped light and OAM-based sensors.This article is part of the themed issue 'Optical orbital angular momentum'. © 2017 The Author(s).

  16. AngularJS directives

    CERN Document Server

    Vanston, Alex

    2013-01-01

    This book uses a practical, step-by-step approach, starting with how to build directives from the ground up before moving on to creating web applications comprised of multiple modules all working together to provide the best user experience possible.This book is intended for intermediate JavaScript developers who are looking to enhance their understanding of single-page web application development with a focus on AngularJS and the JavaScript MVC frameworks.It is expected that readers will understand basic JavaScript patterns and idioms and can recognize JSON formatted data.

  17. Nanoscale spatial analysis of clay minerals containing cesium by synchrotron radiation photoemission electron microscopy

    Science.gov (United States)

    Yoshigoe, Akitaka; Shiwaku, Hideaki; Kobayashi, Toru; Shimoyama, Iwao; Matsumura, Daiju; Tsuji, Takuya; Nishihata, Yasuo; Kogure, Toshihiro; Ohkochi, Takuo; Yasui, Akira; Yaita, Tsuyoshi

    2018-01-01

    A synchrotron radiation photoemission electron microscope (SR-PEEM) was applied to demonstrate the pinpoint analysis of micrometer-sized weathered biotite clay particles with artificially adsorbed cesium (Cs) atoms. Despite the insulating properties of the clay, we observed the spatial distributions of constituent elements (Si, Al, Cs, Mg, and Fe) without charging issues and clarified reciprocal site-correlations among these elements with nanometer resolution. We found that Cs atoms were likely to be adsorbed evenly over the entire particle; however, we identified an occupational conflict between Cs and Mg atoms, implying that Cs sorption involves ion exchange processes. Spatially resolved X-ray absorption spectra (XAS) of the Cs4,5 M-edge region showed Cs to be present in a monocation state (Cs+) as typically observed for Cs compounds. Further pinpoint XAS measurements were also performed at the Fe L2,3-edge to determine the chemical valence of the Fe atoms. The shapes of the spectra were similar to those for Fe2O3, indicating that Fe in the clay was in a 3+ oxidation state. From these observations, we infer that charge compensation facilitates Cs adsorption in the vicinity of a substitution site where Si4+ ions are replaced by Fe3+ ions in SiO4 tetrahedral sheets. Our results demonstrate the utility of SR-PEEM as a tool for spatially resolved chemical analyses of various environmental substances, which is not limited by the poor conductivity of samples.

  18. Bulk sensitive hard x-ray photoemission electron microscopy.

    Science.gov (United States)

    Patt, M; Wiemann, C; Weber, N; Escher, M; Gloskovskii, A; Drube, W; Merkel, M; Schneider, C M

    2014-11-01

    Hard x-ray photoelectron spectroscopy (HAXPES) has now matured into a well-established technique as a bulk sensitive probe of the electronic structure due to the larger escape depth of the highly energetic electrons. In order to enable HAXPES studies with high lateral resolution, we have set up a dedicated energy-filtered hard x-ray photoemission electron microscope (HAXPEEM) working with electron kinetic energies up to 10 keV. It is based on the NanoESCA design and also preserves the performance of the instrument in the low and medium energy range. In this way, spectromicroscopy can be performed from threshold to hard x-ray photoemission. The high potential of the HAXPEEM approach for the investigation of buried layers and structures has been shown already on a layered and structured SrTiO3 sample. Here, we present results of experiments with test structures to elaborate the imaging and spectroscopic performance of the instrument and show the capabilities of the method to image bulk properties. Additionally, we introduce a method to determine the effective attenuation length of photoelectrons in a direct photoemission experiment.

  19. Angular Distribution of GRBs

    Directory of Open Access Journals (Sweden)

    L. G. Balázs

    2012-01-01

    Full Text Available We studied the complete randomness of the angular distribution of BATSE gamma-ray bursts (GRBs. Based on their durations and peak fluxes, we divided the BATSE sample into 5 subsamples (short1, short2, intermediate, long1, long2 and studied the angular distributions separately. We used three methods to search for non-randomness in the subsamples: Voronoi tesselation, minimal spanning tree, and multifractal spectra. To study any non-randomness in the subsamples we defined 13 test-variables (9 from Voronoi tesselation, 3 from the minimal spanning tree and one from the multifractal spectrum. We made Monte Carlo simulations taking into account the BATSE’s sky-exposure function. We tested therandomness by introducing squared Euclidean distances in the parameter space of the test-variables. We recognized that the short1, short2 groups deviate significantly (99.90%, 99.98% from the fully random case in the distribution of the squared Euclidean distances but this is not true for the long samples. In the intermediate group, the squared Euclidean distances also give significant deviation (98.51%.

  20. Time resolved techniques: An overview

    International Nuclear Information System (INIS)

    Larson, B.C.; Tischler, J.Z.

    1990-06-01

    Synchrotron sources provide exceptional opportunities for carrying out time-resolved x-ray diffraction investigations. The high intensity, high angular resolution, and continuously tunable energy spectrum of synchrotron x-ray beams lend themselves directly to carrying out sophisticated time-resolved x-ray scattering measurements on a wide range of materials and phenomena. When these attributes are coupled with the pulsed time-structure of synchrotron sources, entirely new time-resolved scattering possibilities are opened. Synchrotron beams typically consist of sub-nanosecond pulses of x-rays separated in time by a few tens of nanoseconds to a few hundred nanoseconds so that these beams appear as continuous x-ray sources for investigations of phenomena on time scales ranging from hours down to microseconds. Studies requiring time-resolution ranging from microseconds to fractions of a nanosecond can be carried out in a triggering mode by stimulating the phenomena under investigation in coincidence with the x-ray pulses. Time resolution on the picosecond scale can, in principle, be achieved through the use of streak camera techniques in which the time structure of the individual x-ray pulses are viewed as quasi-continuous sources with ∼100--200 picoseconds duration. Techniques for carrying out time-resolved scattering measurements on time scales varying from picoseconds to kiloseconds at present and proposed synchrotron sources are discussed and examples of time-resolved studies are cited. 17 refs., 8 figs

  1. Relaxation of strongly coupled electron and phonon fields after photoemission and high-energy part of ARPES spectra of cuprates

    Science.gov (United States)

    Myasnikova, A. E.; Zhileeva, E. A.; Moseykin, D. V.

    2018-03-01

    An approach to considering systems with a high concentration of correlated carriers and strong long-range electron–phonon interaction and to calculating the high-energy part of the angle-resolved photoemission spectroscopy (ARPES) spectra of such systems is suggested. Joint relaxation of strongly coupled fields—a field of correlated electrons and phonon field—after photoemission is studied to clarify the nature of characteristic features observed in the high-energy part of the ARPES spectra of cuprate superconductors. Such relaxation occurs in systems with strong predominantly long-range electron–phonon interaction at sufficiently high carrier concentration due to the coexistence of autolocalized and delocalized carriers. A simple method to calculate analytically a high-energy part of the ARPES spectrum arising is proposed. It takes advantage of using the coherent states basis for the phonon field in the polaron and bipolaron states. The approach suggested yields all the high-energy spectral features like broad Gaussian band and regions of ‘vertical dispersion’ being in good quantitative agreement with the experiments on cuprates at any doping with both types of carriers. Demonstrated coexistence of autolocalized and delocalized carriers in superconducting cuprates changes the idea about their ground state above the superconducting transition temperature that is important for understanding transport and magnetic properties. High density of large-radius autolocalized carriers revealed may be a key to the explanation of charge ordering in doped cuprates.

  2. Fermi surface and effective masses in photoemission response of the (Ba1-xKx)Fe2As2superconductor.

    Science.gov (United States)

    Derondeau, Gerald; Bisti, Federico; Kobayashi, Masaki; Braun, Jürgen; Ebert, Hubert; Rogalev, Victor A; Shi, Ming; Schmitt, Thorsten; Ma, Junzhang; Ding, Hong; Strocov, Vladimir N; Minár, Ján

    2017-08-18

    The angle-resolved photoemission spectra of the superconductor (Ba 1-x K x )Fe 2 As 2 have been investigated accounting coherently for spin-orbit coupling, disorder and electron correlation effects in the valence bands combined with final state, matrix element and surface effects. Our results explain the previously obscured origins of all salient features of the ARPES response of this paradigm pnictide compound and reveal the origin of the Lifshitz transition. Comparison of calculated ARPES spectra with the underlying DMFT band structure shows an important impact of final state effects, which result for three-dimensional states in a deviation of the ARPES spectra from the true spectral function. In particular, the apparent effective mass enhancement seen in the ARPES response is not an entirely intrinsic property of the quasiparticle valence bands but may have a significant extrinsic contribution from the photoemission process and thus differ from its true value. Because this effect is more pronounced for low photoexcitation energies, soft-X-ray ARPES delivers more accurate values of the mass enhancement due to a sharp definition of the 3D electron momentum. To demonstrate this effect in addition to the theoretical study, we show here new state of the art soft-X-ray and polarisation dependent ARPES measurments.

  3. First studies on pulsed photoemission with a power laser

    International Nuclear Information System (INIS)

    Bergeret, H.; Boussoukaya, M.; Chehab, R.; Leblond, B.

    1985-07-01

    In lasertron studies, the photocathode emission investigation represents an essential part. For that, in order to determine the photo-emissivity of different materials we studied the lanthanum hexaboride as a first step. Obtained results with a Nd.YAG laser with different wavelengthes from 1064 to 355 nm, concern emission densities from some mA/cm 2 to 7kA/cm 2 with quantum efficiencies from 2.10 -7 to 10 -3 . Some of that results are in good agreement with those obtained by J. Lafferty in 1950 [fr

  4. Reflection and photoemission studies of neutron-irradiated graphite

    International Nuclear Information System (INIS)

    Fukutani, Hirohito; Yamada, Akio; Yagi, Kazutoshi; Ooe, Satoshi; Higashiyama, Kazuyuki; Kato, Hiroo; Iwata, Tadao.

    1990-01-01

    Neutron-irradiated graphites were studied by reflectivity and photoemission (UPS, ARUPS, XPS) measurements. The π-band reflectivity peak of graphite, located at 5 eV, changed significantly and a small absorption band ascribed to vacancies produced by neutron bombardment was found to grow around 3 eV. Modification of the valence band by neutron irradiation was studied by ARUPS. The π-valence band shifts to lower binding energy towards the Fermi level and its band width becomes smaller. These results were also confirmed by the optical joint density of states obtained from K-K analysis of the reflectivity. (author)

  5. Angular integrals in d dimensions

    International Nuclear Information System (INIS)

    Somogyi, Gabor

    2011-01-01

    We discuss the evaluation of certain d dimensional angular integrals which arise in perturbative field theory calculations. We find that the angular integral with n denominators can be computed in terms of a certain special function, the so-called H-function of several variables. We also present several illustrative examples of the general result and briefly consider some applications. (orig.)

  6. Angular-domain scattering interferometry.

    Science.gov (United States)

    Shipp, Dustin W; Qian, Ruobing; Berger, Andrew J

    2013-11-15

    We present an angular-scattering optical method that is capable of measuring the mean size of scatterers in static ensembles within a field of view less than 20 μm in diameter. Using interferometry, the method overcomes the inability of intensity-based models to tolerate the large speckle grains associated with such small illumination areas. By first estimating each scatterer's location, the method can model between-scatterer interference as well as traditional single-particle Mie scattering. Direct angular-domain measurements provide finer angular resolution than digitally transformed image-plane recordings. This increases sensitivity to size-dependent scattering features, enabling more robust size estimates. The sensitivity of these angular-scattering measurements to various sizes of polystyrene beads is demonstrated. Interferometry also allows recovery of the full complex scattered field, including a size-dependent phase profile in the angular-scattering pattern.

  7. Extreme regimes of femtosecond photoemission from a copper cathode in a dc electron gun

    Directory of Open Access Journals (Sweden)

    P. L. E. M. Pasmans

    2016-10-01

    Full Text Available The femtosecond photoemission yield from a copper cathode and the emittance of the created electron beams has been studied in a 12  MeV/m, 100 keV dc electron gun over a wide range of laser fluence, from the linear photoemission regime until the onset of image charge limitations and cathode damaging. The measured photoemission curves can be described well with available theory which includes the Schottky effect, second-order photoemission, and image charge limitation. The second-order photoemission can be explained by thermally assisted one-photon photoemission (1PPE and by above-threshold two-photon photoemission (2PPE. Measurements with a fresh cathode suggest that the 2PPE process is dominant. The beam emittance has been measured for the entire range of initial surface charge densities as well. The emittance measurements of space-charge dominated beams can be described well by an envelope equation with generalized perveance. The dc gun produces 0.1 pC bunches with 25 nm rms normalized emittance, corresponding to a normalized brightness usually associated with rf photoguns. In this experimental study the limits of femtosecond photoemission from a copper cathode have been explored and analyzed in great detail, resulting in improved understanding of the underlying mechanisms.

  8. Giant Cu 2p Resonances in CuO Valence-Band Photoemission

    NARCIS (Netherlands)

    Tjeng, L.H.; Chen, C.T.; Ghijsen, J.; Rudolf, P.; Sette, F.

    1991-01-01

    We report the observation of a giant resonance in the Cu 2p resonant-photoemission spectra of CuO. The study allows the unambiguous identification of the local Cu 3d8 configuration in the valence-band photoemission spectrum, providing conclusive evidence for the charge-transfer nature of the

  9. Iron 1s X-ray photoemission of Fe2O3

    NARCIS (Netherlands)

    Miedema, P. S.; Borgatti, F.; Offi, F.; Panaccione, G.; de Groot, F. M. F.

    We present the Is X-ray photoemission spectrum of alpha-Fe2O3 in comparison with its 2p photoemission spectrum. We show that in case of transition metal oxides, because the 1s core hole is not affected by core hole spin-orbit coupling and almost not affected by core-valence multiplet effects, the Fe

  10. Synchronization and Characterization of an Ultra-Short Laser for Photoemission and Electron-Beam Diagnostics Studies at a Radio Frequency Photoinjector

    Energy Technology Data Exchange (ETDEWEB)

    Maxwell, Timothy; Ruan, Jinhao; Piot, Philippe; Lumpkin, Alex

    2012-03-01

    A commercially-available titanium-sapphire laser system has recently been installed at the Fermilab A0 photoinjector laboratory in support of photoemission and electron beam diagnostics studies. The laser system is synchronized to both the 1.3-GHz master oscillator and a 1-Hz signal use to trigger the radiofrequency system and instrumentation acquisition. The synchronization scheme and performance are detailed. Long-term temporal and intensity drifts are identified and actively suppressed to within 1 ps and 1.5%, respectively. Measurement and optimization of the laser's temporal profile are accomplished using frequency-resolved optical gating.

  11. Iron 1s X-ray photoemission of Fe2O3

    International Nuclear Information System (INIS)

    Miedema, P.S.; Borgatti, F.; Offi, F.; Panaccione, G.; Groot, F.M.F. de

    2015-01-01

    Highlights: • Three peaks of 1s XPS of Fe 2 O 3 means use of three configurations. • 1s XPS vs 2p XPS: advantage of 1s XPS for charge transfer parameter analysis. • Charge transfer multiplet analysis with same parameters for 1s and 2p XPS. - Abstract: We present the 1s X-ray photoemission spectrum of α-Fe 2 O 3 in comparison with its 2p photoemission spectrum. We show that in case of transition metal oxides, because the 1s core hole is not affected by core hole spin-orbit coupling and almost not affected by core-valence multiplet effects, the Fe 1s spectrum and the complementary charge transfer multiplet calculations allow for an accurate determination of the charge transfer parameters. The consistency of the obtained parameters for the 1s photoemission was confirmed with 2p photoemission calculations and compared to 2p experimental photoemission spectra

  12. Hard X-ray photoemission spectroscopy of transition-metal oxide thin films and interfaces

    International Nuclear Information System (INIS)

    Wadati, H.; Fujimori, A.

    2013-01-01

    Highlights: •Photoemission spectroscopy is a powerful technique to study the electronic structures of transition-metal oxides. •Hard X-ray photoemission spectroscopy (HXPES) is a new type of photoemission spectroscopy which can probe bulk states. •HXPES is very suitable for studying oxide thin films such as the composition dependence and the film thickness dependence. -- Abstract: Photoemission spectroscopy is a powerful experimental technique to study the electronic structures of solids, especially of transition-metal oxides. Recently, hard X-ray photoemission spectroscopy (HXPES) has emerged as a more relevant experimental technique to obtain clear information about bulk states. Here, we describe how HXPES can be conveniently applied to study the interesting subjects on oxide thin films such as the composition dependence and the film thickness dependence of the electronic structures and the interfacial electronic structure of multilayers

  13. Intact Dirac Cones at Broken Sublattice Symmetry: Photoemission Study of Graphene on Ni and Co

    Directory of Open Access Journals (Sweden)

    A. Varykhalov

    2012-12-01

    Full Text Available The appearance of massless Dirac fermions in graphene requires two equivalent carbon sublattices of trigonal shape. While the generation of an effective mass and a band gap at the Dirac point remains an unresolved problem for freestanding extended graphene, it is well established by breaking translational symmetry by confinement and by breaking sublattice symmetry by interaction with a substrate. One of the strongest sublattice-symmetry-breaking interactions with predicted and measured band gaps ranging from 400 meV to more than 3 eV has been attributed to the interfaces of graphene with Ni and Co, which are also promising spin-filter interfaces. Here, we apply angle-resolved photoemission to epitaxial graphene on Ni(111 and Co(0001 to show the presence of intact Dirac cones 2.8 eV below the Fermi level. Our results challenge the common belief that the breaking of sublattice symmetry by a substrate and the opening of the band gap at the Dirac energy are in a straightforward relation. A simple effective model of a biased bilayer structure composed of graphene and a sublattice-symmetry-broken layer, corroborated by density-functional-theory calculations, demonstrates the general validity of our conclusions.

  14. First results from the high energy resolution photoemission beam line at ELETTRA

    International Nuclear Information System (INIS)

    Quaresima, C.; Astaldi, C.; Zacchigna, M.; Romanzin, L.; Savoia, A.

    1995-01-01

    We report the first results obtained from the high energy resolution beam line at the storage ring ELETTRA of Trieste. The beam line has been designed to perform photoemission experiments in the vacuum ultraviolet (VUV) and soft X-ray (SXR) energy range. The radiation source is an undulator which consists of three sections, with 36 periods and a period length of 12.5 cm. It allows scanning of an energy range 17-900 eV using the 1st, 3rd and 5th harmonics. The monochromator is a spherical grating type and the resolving power at 400 eV, estimated from the K-shell photoabsorption of the N 2 molecule is well above 10 000. The spectra are better than any other spectra taken while operating with high flux, i.e. first order diffraction and grating not masked. Measurements taken at the oxygen and neon K-edges, the argon L 2,3 edges and of the helium double ionization spectra, indicate that the resolution is excellent from 65 to 870 eV. (orig.)

  15. Photon absorption and photocurrent in solar cells below semiconductor bandgap due to electron photoemission from plasmonic nanoantennas

    DEFF Research Database (Denmark)

    Novitsky, Andrey; Uskov, Alexander; Gritti, Claudia

    2014-01-01

    We model the electron photoemission frommetal nanoparticles into a semiconductor in a Schottky diode with a conductive oxide electrode hosting the nanoparticles. We show that plasmonic effects in the nanoparticles lead to a substantial enhancement in photoemission compared with devices with conti....... Such structure can form the dais of the development of plasmonic photoemission enhanced solar cells....

  16. Development of high energy resolution inverse photoemission technique

    International Nuclear Information System (INIS)

    Asakura, D.; Fujii, Y.; Mizokawa, T.

    2004-01-01

    Full text: It is highly important to study occupied and unoccupied electronic states in order to understand electronic properties of strongly correlated electron systems. Photoemission spectroscopy (PES) and inverse photoemission spectroscopy (IPES) are complementary to each other and very powerful experimental methods to study the electronic structure. While PES directly investigates the occupied states below the Fermi level, IPES observes the unoccupied states above it. Although the energy resolution of 2 meV has been achieved for PES, the energy resolution of IPES is still around 200 meV. The poor energy resolution of IPES considerably limits information of unoccupied states. In order to investigate unoccupied states of strongly correlated electron systems, we have designed and constructed a new IPES instrument based on two ideas: off-plane Eagle mounting of the optical system [1, 2] and dispersion matching between incoming electron and outgoing ultraviolet light. In the IPES system, a parallel plate electron analyzer is employed to give the energy dispersion to the incoming electron beam. The outgoing ultraviolet light is monochromatized by a concave grating. The sample, the grating, and the position sensitive detector are arranged in the off-plane Eagle mounting to achieve a good focusing of light. Ray-trace simulations have shown that the energy resolution of 20 meV is expected for the perfect dispersion matching. We will present the principle, mechanism, and current status of our IPES instrument

  17. Electronic Structures of Magnetic Iron and Cobalt Thin Films on TUNGSTEN(001): a Spin-Polarized Inverse Photoemission Study

    Science.gov (United States)

    Cai, Qing

    Electronic structure is a central question in metallic magnetism as well as in magnetic materials research. The electronic properties in a two-dimensional system such as thin films of a few atomic layers is an important issue in surface science. The epitaxial thin film preparation and morphology are of special technological interests. In this thesis, these questions are addressed. Spin-polarized inverse photoemission spectroscopy is used to study the unoccupied electron band states in magnetic thin film magnets of Fe and Co epitaxially grown on W(001) surface. The clean W(001) surface was studied by angle -resolved inverse photoemission spectroscopy and the bulk band dispersion was determined. Ultrathin Fe overlayers on W(001) show a square lateral crystal structure similar to the bcc-Fe(001) surface. The electronic structure develops into a structure that is close to that of bulk Fe at about four atomic layers. In the normal-incidence spin polarized inverse photoemission spectra, direct transitions to the majority and minority final states near the H^'_ {25} point are identified in good agreement with the theoretical calculations. One Fe monolayer, or multilayers less than four, showed behavior corresponding to a gradually reduced Curie temperature. When the film thickness is reduced, the spin-resolved spectral behavior show that the majority spin signal peak moves from near the Fermi energy to about 1.3 eV while the minority peak stays at about the same position near 1.3 eV. The results are used to examine the spatial correlation of the spin fluctuations in the system in comparison with a theoretical spectral calculation, and favors the disordered-local-moment picture in the contemporary theory of itinerant magnetism. The Co overlayer shows an overlayer structure that consists of equivalent, mutually rotated domains of distorted hexagonal lateral structure. For one atomic layer of Co in that structure, which has a nominal lateral atomic density twice that of the

  18. AngularJS testing cookbook

    CERN Document Server

    Bailey, Simon

    2015-01-01

    This book is intended for developers who have an understanding of the basic principles behind both AngularJS and test-driven development. You, as a developer, are interested in eliminating the fear related to either introducing tests to an existing codebase or starting out testing on a fresh AngularJS application. If you're a team leader or part of a QA team with the responsibility of ensuring full test coverage of an application, then this book is ideal for you to comprehend the full testing scope required by your developers. Whether you're new to or are well versed with AngularJS, this book

  19. Lidar Orbital Angular Momentum Sensor

    Data.gov (United States)

    National Aeronautics and Space Administration — The recognition in recent decades that electromagnetic fields have angular momentum (AM) in the form of not only polarization (or spin AM) but also orbital (OAM) has...

  20. Angular momentum from tidal torques

    International Nuclear Information System (INIS)

    Barnes, J.; Efstathiou, G.; Cambridge Univ., England)

    1987-01-01

    The origin of the angular momentum of bound objects in large N-body simulations is studied using three sets of models. One model with white-noise initial conditions is analyzed as well as two in which the initial conditions have more power on large scales, as predicted in models with cold dark matter. The growth and distribution of angular momentum in individual objects is studied and it is found that the specific angular momentum distribution of bound clumps increases in a near linear fashion with radius while the orientation of the angular momentum in the inner high-density regions is often poorly correlated with that of the outer parts. It is also found that the dimensionless spin parameter is insensitive to the initial perturbation spectrum and has a median value of about 0.05. 61 references

  1. Plasmons with orbital angular momentum

    International Nuclear Information System (INIS)

    Mendonca, J. T.; Ali, S.; Thide, B.

    2009-01-01

    Electron plasma waves carrying orbital angular momentum are investigated in an unmagnetized collisionless plasma composed of inertial electrons and static ions. For this purpose, the usual plasmon dispersion relation is employed to derive an approximate paraxial equation. The latter is analyzed with a Gaussian beam solution. For a finite angular momentum associated with the plasmon, Laguerre-Gaussian (LG) solutions are employed for solving the electrostatic potential problem which gives approximate solution and is valid for plasmon beams in the paraxial approximation. The LG potential determines the electric field components and energy flux of plasmons with finite angular momentum. Numerical illustrations show that the radial and angular mode numbers strongly modify the profiles of the LG potential.

  2. Rectilinear Graphs and Angular Resolution

    NARCIS (Netherlands)

    Bodlaender, H.L.; Tel, G.

    2003-01-01

    In this note we show that a planar graph with angular resolution at least π/2 can be drawn with all angles an integer multiple of π/2, that is, in a rectilinear manner. Moreover, we show that for d ≠ 4, d › 2, having an angular resolution of 2π/d does not imply that the graph can be drawn with all

  3. Time-resolved ARPES with sub-15 fs temporal and near Fourier-limited spectral resolution.

    Science.gov (United States)

    Rohde, G; Hendel, A; Stange, A; Hanff, K; Oloff, L-P; Yang, L X; Rossnagel, K; Bauer, M

    2016-10-01

    An experimental setup for time- and angle-resolved photoelectron spectroscopy with sub-15 fs temporal resolution is presented. A hollow-fiber compressor is used for the generation of 6.5 fs white light pump pulses, and a high-harmonic-generation source delivers 11 fs probe pulses at a photon energy of 22.1 eV. A value of 13 fs full width at half-maximum of the pump-probe cross correlation signal is determined by analyzing a photoemission intensity transient probing a near-infrared interband transition in 1T-TiSe 2 . Notably, the energy resolution of the setup conforms to typical values reported in conventional time-resolved photoemission studies using high harmonics, and an ultimate resolution of 170 meV is feasible.

  4. heterojunction interface investigated by X-ray photoemission spectroscopy

    Science.gov (United States)

    Lin, Lingyan; Yu, Jinling; Cheng, Shuying; Lu, Peimin; Lai, Yunfeng; Lin, Sile; Zhao, Pengyi

    2014-09-01

    The band alignment at the In2S3/Cu2ZnSnS4 heterojunction interface is investigated by X-ray photoemission spectroscopy. In2S3 is thermally evaporated onto the contamination-free polycrystalline Cu2ZnSnS4 surface prepared by magnetron sputtering. The valence band offset is measured to be 0.46 ± 0.1 eV, which matches well with the valance band offset value 0.49 eV calculated using "transitivity" method. The conduction band offset is determined to be 0.82 ± 0.1 eV, indicating a `type I' band alignment at the heterojunction interface.

  5. Photoemission of graded-doping GaN photocathode

    International Nuclear Information System (INIS)

    Fu Xiao-Qian; Chang Ben-Kang; Wang Xiao-Hui; Li Biao; Du Yu-Jie; Zhang Jun-Ju

    2011-01-01

    We study the photoemission process of graded-doping GaN photocathode and find that the built-in electric fields can increase the escape probability and the effective diffusion length of photo-generated electrons, which results in the enhancement of quantum efficiency. The intervalley scattering mechanism and the lattice scattering mechanism in high electric fields are also investigated. To prevent negative differential mobility from appearing, the surface doping concentration needs to be optimized, and it is calculated to be 3.19×10 17 cm −3 . The graded-doping GaN photocathode with higher performance can be realized by further optimizing the doping profile. (condensed matter: electronic structure, electrical, magnetic, and optical properties)

  6. Photoemission of graded-doping GaN photocathode

    Science.gov (United States)

    Fu, Xiao-Qian; Chang, Ben-Kang; Wang, Xiao-Hui; Li, Biao; Du, Yu-Jie; Zhang, Jun-Ju

    2011-03-01

    We study the photoemission process of graded-doping GaN photocathode and find that the built-in electric fields can increase the escape probability and the effective diffusion length of photo-generated electrons, which results in the enhancement of quantum efficiency. The intervalley scattering mechanism and the lattice scattering mechanism in high electric fields are also investigated. To prevent negative differential mobility from appearing, the surface doping concentration needs to be optimized, and it is calculated to be 3.19×1017 cm-3. The graded-doping GaN photocathode with higher performance can be realized by further optimizing the doping profile. Project supported by the National Natural Science Foundation of China (Grant No. 60871012) and the Research Fund of Nanjing University of Science and Technology (Grant No. 2010ZYTS032).

  7. Electric field stimulation setup for photoemission electron microscopes.

    Science.gov (United States)

    Buzzi, M; Vaz, C A F; Raabe, J; Nolting, F

    2015-08-01

    Manipulating magnetisation by the application of an electric field in magnetoelectric multiferroics represents a timely issue due to the potential applications in low power electronics and the novel physics involved. Thanks to its element sensitivity and high spatial resolution, X-ray photoemission electron microscopy is a uniquely suited technique for the investigation of magnetoelectric coupling in multiferroic materials. In this work, we present a setup that allows for the application of in situ electric and magnetic fields while the sample is analysed in the microscope. As an example of the performances of the setup, we present measurements on Ni/Pb(Mg(0.66)Nb(0.33))O3-PbTiO3 and La(0.7)Sr(0.3)MnO3/PMN-PT artificial multiferroic nanostructures.

  8. Microlens Array Laser Transverse Shaping Technique for Photoemission Electron Source

    Energy Technology Data Exchange (ETDEWEB)

    Halavanau, A. [Northern Illinois Univ., DeKalb, IL (United States); Fermi National Accelerator Lab. (FNAL), Batavia, IL (United States); Ha, G. [Argonne National Lab. (ANL), Argonne, IL (United States); Pohang Univ. of Science and Technology (POSTECH) (Korea, Republic of); Qiang, G. [Argonne National Lab. (ANL), Argonne, IL (United States); Tsinghua Univ., Beijing (China); Gai, W. [Argonne National Lab. (ANL), Argonne, IL (United States); Power, J. [Argonne National Lab. (ANL), Argonne, IL (United States); Piot, P. [Northern Illinois Univ., DeKalb, IL (United States); Fermi National Accelerator Lab. (FNAL), Batavia, IL (United States); Wisniewski, E. [Argonne National Lab. (ANL), Argonne, IL (United States); Edstrom, D. [Fermi National Accelerator Lab. (FNAL), Batavia, IL (United States); Ruan, J. [Fermi National Accelerator Lab. (FNAL), Batavia, IL (United States); Santucci, J. [Fermi National Accelerator Lab. (FNAL), Batavia, IL (United States)

    2016-09-06

    A common issue encountered in photoemission electron sources used in electron accelerators is distortion of the laser spot due to non ideal conditions at all stages of the amplification. Such a laser spot at the cathode may produce asymmetric charged beams that will result in degradation of the beam quality due to space charge at early stages of acceleration and fail to optimally utilize the cathode surface. In this note we study the possibility of using microlens arrays to dramatically improve the transverse uniformity of the drive laser pulse on UV photocathodes at both Fermilab Accelerator Science \\& Technology (FAST) facility and Argonne Wakefield Accelerator (AWA). In particular, we discuss the experimental characterization of the homogeneity and periodic patterned formation at the photocathode. Finally, we compare the experimental results with the paraxial analysis, ray tracing and wavefront propagation software.

  9. Measurement and analysis of thermal photoemission from a dispenser cathode

    Directory of Open Access Journals (Sweden)

    Kevin L. Jensen

    2003-08-01

    Full Text Available Photocathodes for free electron lasers (FELs are required to produce nano-Coulomb pulses in picosecond time scales with demonstrable reliability, lifetime, and efficiency. Dispenser cathodes, traditionally a rugged and long-lived thermionic source, are under investigation to determine their utility as a photocathode and have shown promise. The present study describes theoretical models under development to analyze experimental data from dispenser cathodes and to create predictive time-dependent models to predict their performance as an FEL source. Here, a steady-state model of a dispenser cathode with partial coverage of a low work function coating and surface nonuniformity is developed. Quantitative agreement is found for experimental data, especially with regard to temperature, field, laser intensity, and quantum efficiency versus laser wavelength dependence. In particular, for long wavelength incident lasers of sufficient intensity, the majority of the absorbed energy heats the electron gas and background lattice, and photoemission from the heated electron distribution constitutes the emitted current.

  10. Photoemission from Coated Surfaces A Comparison of Theory to Experiment

    CERN Document Server

    Jensen, K

    2005-01-01

    Photocathodes for FELs and accelerators will benefit from rugged and self-rejuvenating photocathodes with high QE at the longest possible wavelength. The needs of a high power FEL are not met at present by existing photocathode-drive laser combinations: requirements generally necessitate barrier-lowering coatings which are degraded by operation. We seek to develop a controlled porosity dispenser cathode, and shall report on our coordinated experimental and theoretical studies. Our models account for field, thermal, and surface effects of cesium monolayers on photoemission, and compare well with concurrent experiments examining the QE, patchiness, and evolution of the coatings. Field enhancement, thermal variation of specific heat and electron relaxation rates and their relation to high laser intensity and/or short pulse-to-pulse separation, variations in work function effects due to coating non-uniformity, and the dependence on the wavelength of the incident light are included. The status of methods by which ...

  11. Energy band dispersion in photoemission spectra of argon clusters

    International Nuclear Information System (INIS)

    Foerstel, Marko; Mucke, Melanie; Arion, Tiberiu; Lischke, Toralf; Barth, Silko; Ulrich, Volker; Ohrwall, Gunnar; Bjoerneholm, Olle; Hergenhahn, Uwe; Bradshaw, Alex M.

    2011-01-01

    Using photoemission we have investigated free argon clusters from a supersonic nozzle expansion in the photon energy range from threshold up to 28 eV. Measurements were performed both at high resolution with a hemispherical electrostatic energy analyser and at lower resolution with a magnetic bottle device. The latter experiments were performed for various mean cluster sizes. In addition to the ∼1.5 eV broad 3p-derived valence band seen in previous work, there is a sharper feature at ∼15 eV binding energy. Surprisingly for non-oriented clusters, this peak shifts smoothly in binding energy over the narrow photon energy range 15.5-17.7 eV, indicating energy band dispersion. The onset of this bulk band-like behaviour could be determined from the cluster size dependence.

  12. Uncertainty principle for angular position and angular momentum

    International Nuclear Information System (INIS)

    Franke-Arnold, Sonja; Barnett, Stephen M; Yao, Eric; Leach, Jonathan; Courtial, Johannes; Padgett, Miles

    2004-01-01

    The uncertainty principle places fundamental limits on the accuracy with which we are able to measure the values of different physical quantities (Heisenberg 1949 The Physical Principles of the Quantum Theory (New York: Dover); Robertson 1929 Phys. Rev. 34 127). This has profound effects not only on the microscopic but also on the macroscopic level of physical systems. The most familiar form of the uncertainty principle relates the uncertainties in position and linear momentum. Other manifestations include those relating uncertainty in energy to uncertainty in time duration, phase of an electromagnetic field to photon number and angular position to angular momentum (Vaccaro and Pegg 1990 J. Mod. Opt. 37 17; Barnett and Pegg 1990 Phys. Rev. A 41 3427). In this paper, we report the first observation of the last of these uncertainty relations and derive the associated states that satisfy the equality in the uncertainty relation. We confirm the form of these states by detailed measurement of the angular momentum of a light beam after passage through an appropriate angular aperture. The angular uncertainty principle applies to all physical systems and is particularly important for systems with cylindrical symmetry

  13. Synchrotron radiation photoemission studies of core level excitation effects

    International Nuclear Information System (INIS)

    Williams, G.P.; Lapeyre, G.J.; Anderson, J.; Cerrina, F.; Dietz, R.E.; Yafet, Y.

    1979-01-01

    The recent availability of intense polarized radiation tunable over the range 20-150 eV enables several core levels to be excited. Several remarkable effects have recently been reported when core excitation thresholds have been reached. For example, an increase in yield of 50% was observed in GaSe at the Se 3d threshold (h omega approx. = 57 eV). A considerable increase in photoemission intensity at 6 eV binding energy has been reported by Guillot et al. for Ni at the 3p threshold. A very careful study was made using the CIS, CFS, and EDC modes of photoemission spectroscopy of core threshold effects in Ni, Pt, and GaSe. A modulation of the Ni Fermi edge emission as a function of photon energy is found which is attributed to a configuration interaction between 3p 5 3d 10 4s and 3p 6 3d 8 4s epsilon f. Similar effects occur in Pt at the 4f threshold involving the configurations 4f 13 5d 10 6s and 4f 14 5d 8 6s. Further, the lineshapes of the Pt and Ni upper valence band CIS's resemble those obtained by electron energy loss (ELS) and photoabsorption, all of which can be fitted theoretically to a Fano model. Emission from levels lying well below the Fermi level often has superimposed contributions due to incoherent effects which complicate the interpretation. In cases in which core levels are excited well above threshold, the CIS technique may be used to examinefinal states. Of particular interest is the possible consequent determination of adsorbate site geometry. Data are presented for 2p emission from a c(2x2) Na overlayer on Ni

  14. Fingerprints of spin-orbital polarons and of their disorder in the photoemission spectra of doped Mott insulators with orbital degeneracy

    Science.gov (United States)

    Avella, Adolfo; Oleś, Andrzej M.; Horsch, Peter

    2018-04-01

    means of a complementary many-body polaron theory, which yields a similar robust spin and orbital order as the Hartree-Fock approximation. Using realistic parameters for the vanadium perovskite La1 -xCaxVO3 , we show that its soft gap is reproduced as well as the marginal doping dependence of the position of the chemical potential relative to the center of the lower Hubbard band. The present theory uncovers also the reasons why the d1→d0 satellite excitations, which directly probe the effect of the random defect fields on the polaron state, are not well resolved in the available experimental photoemission spectra for La1 -xCaxVO3 .

  15. Thermal Stability of Au/NbOx/Nb and Au/Nb2O5/W Model Catalysts Studied by Angle-resolved X-ray Photoelectron Spectroscopy

    Czech Academy of Sciences Publication Activity Database

    Lykhach, Yaroslava; Plšek, Jan; Spirovová, Ilona; Bastl, Zdeněk

    2003-01-01

    Roč. 68, č. 10 (2003), s. 1791-1804 ISSN 0010-0765 R&D Projects: GA ČR GA104/02/0664 Institutional research plan: CEZ:AV0Z4040901 Keywords : model metal catalysts * angle resolved photoemission * depth profiles Subject RIV: CF - Physical ; Theoretical Chemistry Impact factor: 1.041, year: 2003

  16. Instant AngularJS starter

    CERN Document Server

    Menard, Dan

    2013-01-01

    Get to grips with a new technology, understand what it is and what it can do for you, and then get to work with the most important features and tasks. This book is written in an easytoread style, with a strong emphasis on realworld, practical examples. Stepbystep explanations are provided for performing important tasks.This book is for web developers familiar with JavascriptIt doesn't cover the history of AngularJS, and it's not a pitch to convince you that AngularJS is the best framework on the entire web. It's a guide to help you learn everything you need to know about AngularJS in as few pa

  17. Development of high current electron source using photoemission from metals with ultrashort laser pulses

    International Nuclear Information System (INIS)

    Tsang, T.; Srinivasan-Rao, T.; Fischer, J.

    1990-10-01

    We summarize the studies of photoemission from metal photocathodes using picosecond pulses in the UV (4.66 eV) wavelength and femtosecond laser pulses in the visible (2 eV) wavelengths. To achieve high current density yield from metal photocathodes, multiphoton photoemission using femtosecond laser pulses are suggested. Electron yield improvement incorporating surface photoemission and surface plasmon resonance in metals and metal films are demonstrated. We examine the possibility of the nonlinear photoemission process overtaking the linear process, and identity some possible complexity. To extract the large amount of electrons free of space charge, a pulsed high voltage is designed; the results of the preliminary test are presented. Finally, for the first time, the width of the electron temporal profiles are measured, utilizing the nonlinear photoelectric effect, to below 100 fsec time regime. The results indicated that the electron pulse duration follows the laser pulses and are not limited by the material. 8 refs., 15 figs

  18. Automated Angular Momentum Recoupling Algebra

    Science.gov (United States)

    Williams, H. T.; Silbar, Richard R.

    1992-04-01

    We present a set of heuristic rules for algebraic solution of angular momentum recoupling problems. The general problem reduces to that of finding an optimal path from one binary tree (representing the angular momentum coupling scheme for the reduced matrix element) to another (representing the sub-integrals and spin sums to be done). The method lends itself to implementation on a microcomputer, and we have developed such an implementation using a dialect of LISP. We describe both how our code, called RACAH, works and how it appears to the user. We illustrate the use of RACAH for several transition and scattering amplitude matrix elements occurring in atomic, nuclear, and particle physics.

  19. Experiments recently carried out on the photoemission station at Beijing Synchrotron Radiation Facility

    International Nuclear Information System (INIS)

    Kurash Ibrahim; Wu Ziyu; Qian Haijie; Zhang Jing; Abbas, M.I.; Chen Zhigang; Su Run; Liu Fengqin

    2003-01-01

    With a sustained and steady operation of the photoemission station at Beijing Synchrotron Radiation Facility, users from different research fields have carried out their investigation on the electronic structure of metal surface-interface, metal doped fullerene as well as colossal magneto-resistance materials utilizing different experimental modes provided by the photoemission station. In this paper authors would present some representative experimental results obtained on the station

  20. Two-photon Photoemission of Organic Semiconductor Molecules on Ag(111)

    Energy Technology Data Exchange (ETDEWEB)

    Yang, Aram [Univ. of California, Berkeley, CA (United States)

    2008-05-01

    Angle- and time-resolved two-photon photoemission (2PPE) was used to study systems of organic semiconductors on Ag(111). The 2PPE studies focused on electronic behavior specific to interfaces and ultrathin films. Electron time dynamics and band dispersions were characterized for ultrathin films of a prototypical n-type planar aromatic hydrocarbon, PTCDA, and representatives from a family of p-type oligothiophenes.In PTCDA, electronic behavior was correlated with film morphology and growth modes. Within a fewmonolayers of the interface, image potential states and a LUMO+1 state were detected. The degree to which the LUMO+1 state exhibited a band mass less than a free electron mass depended on the crystallinity of the layer. Similarly, image potential states were measured to have free electron-like effective masses on ordered surfaces, and the effective masses increased with disorder within the thin film. Electron lifetimes were correlated with film growth modes, such that the lifetimes of electrons excited into systems created by layer-by-layer, amorphous film growth increased by orders of magnitude by only a few monolayers from the surface. Conversely, the decay dynamics of electrons in Stranski-Krastanov systems were limited by interaction with the exposed wetting layer, which limited the barrier to decay back into the metal.Oligothiophenes including monothiophene, quaterthiophene, and sexithiophene were deposited on Ag(111), and their electronic energy levels and effective masses were studied as a function of oligothiophene length. The energy gap between HOMO and LUMO decreased with increasing chain length, but effective mass was found to depend on domains from high- or low-temperature growth conditions rather than chain length. In addition, the geometry of the molecule on the surface, e.g., tilted or planar, substantially affected the electronic structure.

  1. Direct surface magnetometry with photoemission magnetic x-ray dichroism

    Energy Technology Data Exchange (ETDEWEB)

    Tobin, J.G.; Goodman, K.W. [Lawrence Berkeley National Lab., CA (United States); Schumann, F.O. [Pennsylvania State Univ., University Park, PA (United States)] [and others

    1997-04-01

    Element specific surface magnetometry remains a central goal of synchrotron radiation based studies of nanomagnetic structures. One appealing possibility is the combination of x-ray absorption dichroism measurements and the theoretical framework provided by the {open_quotes}sum rules.{close_quotes} Unfortunately, sum rule analysis are hampered by several limitations including delocalization of the final state, multi-electronic phenomena and the presence of surface dipoles. An alternative experiment, Magnetic X-Ray Dichroism in Photoelectron Spectroscopy, holds out promise based upon its elemental specificity, surface sensitivity and high resolution. Computational simulations by Tamura et al. demonstrated the relationship between exchange and spin orbit splittings and experimental data of linear and circular dichroisms. Now the authors have developed an analytical framework which allows for the direct extraction of core level exchange splittings from circular and linear dichroic photoemission data. By extending a model initially proposed by Venus, it is possible to show a linear relation between normalized dichroism peaks in the experimental data and the underlying exchange splitting. Since it is reasonable to expect that exchange splittings and magnetic moments track together, this measurement thus becomes a powerful new tool for direct surface magnetometry, without recourse to time consuming and difficult spectral simulations. The theoretical derivation will be supported by high resolution linear and circular dichroism data collected at the Spectromicroscopy Facility of the Advanced Light Source.

  2. Direct surface magnetometry with photoemission magnetic x-ray dichroism

    International Nuclear Information System (INIS)

    Tobin, J.G.; Goodman, K.W.; Schumann, F.O.

    1997-01-01

    Element specific surface magnetometry remains a central goal of synchrotron radiation based studies of nanomagnetic structures. One appealing possibility is the combination of x-ray absorption dichroism measurements and the theoretical framework provided by the open-quotes sum rules.close quotes Unfortunately, sum rule analysis are hampered by several limitations including delocalization of the final state, multi-electronic phenomena and the presence of surface dipoles. An alternative experiment, Magnetic X-Ray Dichroism in Photoelectron Spectroscopy, holds out promise based upon its elemental specificity, surface sensitivity and high resolution. Computational simulations by Tamura et al. demonstrated the relationship between exchange and spin orbit splittings and experimental data of linear and circular dichroisms. Now the authors have developed an analytical framework which allows for the direct extraction of core level exchange splittings from circular and linear dichroic photoemission data. By extending a model initially proposed by Venus, it is possible to show a linear relation between normalized dichroism peaks in the experimental data and the underlying exchange splitting. Since it is reasonable to expect that exchange splittings and magnetic moments track together, this measurement thus becomes a powerful new tool for direct surface magnetometry, without recourse to time consuming and difficult spectral simulations. The theoretical derivation will be supported by high resolution linear and circular dichroism data collected at the Spectromicroscopy Facility of the Advanced Light Source

  3. Einstein's photoemission emission from heavily-doped quantized structures

    CERN Document Server

    Ghatak, Kamakhya Prasad

    2015-01-01

    This monograph solely investigates the Einstein's Photoemission(EP) from Heavily Doped(HD) Quantized Structures on the basis of newly formulated electron dispersion laws. The materials considered are quantized structures of HD non-linear optical, III-V, II-VI, Ge, Te, Platinum Antimonide, stressed materials, GaP, Gallium Antimonide, II-V, Bismuth Telluride together with various types of HD superlattices and their Quantized counterparts respectively. The EP in HD opto-electronic materials and their nanostructures is studied in the presence of strong light waves and intense electric fields  that control the studies of such quantum effect devices. The suggestions for the experimental determinations of different important physical quantities in HD 2D and 3D materials  and the importance of measurement of band gap in HD optoelectronic materials under intense built-in electric field in nano devices and strong external photo excitation (for measuring   physical properties in the presence of intense light waves w...

  4. Photoemission Study of the Rare Earth Intermetallic Compounds: RNi2Ge2 (R=Eu, Gd)

    Energy Technology Data Exchange (ETDEWEB)

    Park, Jongik [Iowa State Univ., Ames, IA (United States)

    2004-01-01

    EuNi2Ge2 and GdNi2Ge2 are two members of the RT2X2 (R = rare earth, T = transition metal and X = Si, Ge) family of intermetallic compounds, which has been studied since the early 1980s. These ternary rare-earth intermetallic compounds with the tetragonal ThCr2Si2 structure are known for their wide variety of magnetic properties, Extensive studies of the RT2X2 series can be found in Refs [ 1,2,3]. The magnetic properties of the rare-earth nickel germanides RNi2Ge2 were recently studied in more detail [4]. The purpose of this dissertation is to investigate the electronic structure (both valence band and shallow core levels) of single crystals of EuNi2Ge2 and GdNi2Ge2 and to check the assumptions that the f electrons are non-interacting and, consequently, the rigid-band model for these crystals would work [11], using synchrotron radiation because, to the best of our knowledge, no photoemission measurements on those have been reported. Photoemission spectroscopy has been widely used to study the detailed electronic structure of metals and alloys, and especially angle-resolved photoemission spectroscopy (ARPES) has proven to be a powerful technique for investigating Fermi surfaces (FSs) of single-crystal compounds.

  5. Study of Si-N amorphous compounds combining XPS (X photoemission) and EELS (electron energy loss spectra) optical measurements. Internal levels photoemission. Pt. 2

    International Nuclear Information System (INIS)

    Guraya, M.M.; Acolani, H.; Zampieri, G.E.; Silva, J.H. Dias da; Cisneros, J.I.; Cantao, M.; Marques, F.C.

    1990-01-01

    A Si-N non-stoichiometric hydrogenated amorphous compounds study with different N- contents is presented. The shape and shifts of the photoemission peaks corresponding to the N - 1s and Si - 2p internal levels are analyzed. Based on the latter, the homogeneity of the samples and the Si - N bonds charge transfer is discussed. (Author) [es

  6. On Dunkl angular momenta algebra

    Energy Technology Data Exchange (ETDEWEB)

    Feigin, Misha [School of Mathematics and Statistics, University of Glasgow,15 University Gardens, Glasgow G12 8QW (United Kingdom); Hakobyan, Tigran [Yerevan State University,1 Alex Manoogian, 0025 Yerevan (Armenia); Tomsk Polytechnic University,Lenin Ave. 30, 634050 Tomsk (Russian Federation)

    2015-11-17

    We consider the quantum angular momentum generators, deformed by means of the Dunkl operators. Together with the reflection operators they generate a subalgebra in the rational Cherednik algebra associated with a finite real reflection group. We find all the defining relations of the algebra, which appear to be quadratic, and we show that the algebra is of Poincaré-Birkhoff-Witt (PBW) type. We show that this algebra contains the angular part of the Calogero-Moser Hamiltonian and that together with constants it generates the centre of the algebra. We also consider the gl(N) version of the subalgebra of the rational Cherednik algebra and show that it is a non-homogeneous quadratic algebra of PBW type as well. In this case the central generator can be identified with the usual Calogero-Moser Hamiltonian associated with the Coxeter group in the harmonic confinement.

  7. Phonons with orbital angular momentum

    International Nuclear Information System (INIS)

    Ayub, M. K.; Ali, S.; Mendonca, J. T.

    2011-01-01

    Ion accoustic waves or phonon modes are studied with orbital angular momentum (OAM) in an unmagnetized collissionless uniform plasma, whose constituents are the Boltzmann electrons and inertial ions. For this purpose, we have employed the fluid equations to obtain a paraxial equation in terms of ion density perturbations and discussed its Gaussian beam and Laguerre-Gauss (LG) beam solutions. Furthermore, an approximate solution for the electrostatic potential problem is presented, allowing to express the components of the electric field in terms of LG potential perturbations. The energy flux due to phonons is also calculated and the corresponding OAM is derived. Numerically, it is shown that the parameters such as azimuthal angle, radial and angular mode numbers, and beam waist, strongly modify the profiles of the phonon LG potential. The present results should be helpful in understanding the phonon mode excitations produced by Brillouin backscattering of laser beams in a uniform plasma.

  8. Angular momentum in QGP holography

    Directory of Open Access Journals (Sweden)

    Brett McInnes

    2014-10-01

    Full Text Available The quark chemical potential is one of the fundamental parameters describing the quark–gluon plasma produced by sufficiently energetic heavy-ion collisions. It is not large at the extremely high temperatures probed by the LHC, but it plays a key role in discussions of the beam energy scan programmes at the RHIC and other facilities. On the other hand, collisions at such energies typically (that is, in peripheral collisions give rise to very high values of the angular momentum density. Here we explain that holographic estimates of the quark chemical potential of a rotating sample of plasma can be very considerably improved by taking the angular momentum into account.

  9. AngularJS test-driven development

    CERN Document Server

    Chaplin, Tim

    2015-01-01

    This book is for developers who want to learn about AngularJS development by applying testing techniques. You are assumed to have a basic knowledge and understanding of HTML, JavaScript, and AngularJS.

  10. Angular Momentum of Topologically Structured Darkness.

    Science.gov (United States)

    Alperin, Samuel N; Siemens, Mark E

    2017-11-17

    We theoretically analyze and experimentally measure the extrinsic angular momentum contribution of topologically structured darkness found within fractional vortex beams, and show that this structured darkness can be explained by evanescent waves at phase discontinuities in the generating optic. We also demonstrate the first direct measurement of the intrinsic orbital angular momentum of light with both intrinsic and extrinsic angular momentum, and explain why the total orbital angular momenta of fractional vortices do not match the winding number of their generating phases.

  11. Simple theoretical analysis of the photoemission from quantum confined effective mass superlattices of optoelectronic materials

    Directory of Open Access Journals (Sweden)

    Debashis De

    2011-07-01

    Full Text Available The photoemission from quantum wires and dots of effective mass superlattices of optoelectronic materials was investigated on the basis of newly formulated electron energy spectra, in the presence of external light waves, which controls the transport properties of ultra-small electronic devices under intense radiation. The effect of magnetic quantization on the photoemission from the aforementioned superlattices, together with quantum well superlattices under magnetic quantization, has also been investigated in this regard. It appears, taking HgTe/Hg1−xCdxTe and InxGa1−xAs/InP effective mass superlattices, that the photoemission from these quantized structures is enhanced with increasing photon energy in quantized steps and shows oscillatory dependences with the increasing carrier concentration. In addition, the photoemission decreases with increasing light intensity and wavelength as well as with increasing thickness exhibiting oscillatory spikes. The strong dependence of the photoemission on the light intensity reflects the direct signature of light waves on the carrier energy spectra. The content of this paper finds six different applications in the fields of low dimensional systems in general.

  12. AngularJS web application development

    CERN Document Server

    Darwin, Peter Bacon

    2013-01-01

    The book will be a step-by-step guide showing the readers how to build a complete web app with AngularJSJavaScript developers who want to learn AngularJS for developing web apps. Knowledge of JavaScript and HTML is expected. No knowledge of AngularJS is required.

  13. Optical angular momentum in classical electrodynamics

    Science.gov (United States)

    Mansuripur, Masud

    2017-06-01

    Invoking Maxwell’s classical equations in conjunction with expressions for the electromagnetic (EM) energy, momentum, force, and torque, we use a few simple examples to demonstrate the nature of the EM angular momentum. The energy and the angular momentum of an EM field will be shown to have an intimate relationship; a source radiating EM angular momentum will, of necessity, pick up an equal but opposite amount of mechanical angular momentum; and the spin and orbital angular momenta of the EM field, when absorbed by a small particle, will be seen to elicit different responses from the particle.

  14. Dependency injection with AngularJS

    CERN Document Server

    Knol, Alex

    2013-01-01

    This book is a practical, hands-on approach to using dependency injection and implementing test-driven development using AngularJS. Dependency Injection with AngularJS is aimed at developers who are aware of AngularJS but need to get started with using it in real life applications. Also, developers who want to get into test-driven development with AngularJS can use this book as practical guide. Even if you know about dependency injection, it can serve as a good reference on how it is used within AngularJS. Readers are expected to have some experience with JavaScript.

  15. Synchrotron photoemission study of (Zn,Co)O films with uniform Co distribution

    DEFF Research Database (Denmark)

    Guziewicz, E.; Lukasiewicz, M. I.; Wachnicki, L.

    2011-01-01

    We present results of a resonant photoemission study of (Zn,Co)O films with Co content between 2% and 7%. The films were grown by Atomic Layer Deposition (ALD) at low temperature of 160°C, and show fully paramagnetic behavior. The Co ions are uniformly distributed in the ZnO matrix and are free...... of foreign phases and metal accumulations as indicated by TEM data. The electronic structure of (Zn,Co)O films was studied by Resonant Photoemission Spectroscopy across the Co3p–Co3d photoionization threshold. We have observed that the resonant enhancement of the photoemission intensity from the Co3d shell...... is not the same for samples with different cobalt content. We suggest that the Co3d contribution to the valence band depends on both Co and H content....

  16. PHOTOEMISSION METHOD OF TEMPERATURE MEASURING IN THE PROCESS OF SPARK PLASMA SINTERING POWDERS OF REFRACTORY METALS

    Directory of Open Access Journals (Sweden)

    D. V. Minko

    2012-01-01

    Full Text Available Construction and algorithm of the photoemission pyrometer based on a photomultiplier are outlined; the calibration procedure is set out. The application of the photoemission method in a rapidly changing temperature is showed. It is proved that during spark plasma sintering the maximal temperature is 5500– 7500 °C, while the speed of temperature increase to its maximum ~108–109 °C/s, and the rate of decrease to 2000–4000 °C may be 106–107 °C/sec. It is recommended to use photoemission method when developing technological conditions, adjustment and control of technological processes using modern high-energy equipment (plasma, laser, cathode-ray tube to produce new materials, coatings and products for mechanical engineering, electronic industry and medicine.

  17. Measurement of total angular momentum values of high-lying even ...

    Indian Academy of Sciences (India)

    Spectrally resolved laser-induced fluorescence technique was used to uniquely assign total angular momentum () values to high-lying even-parity energy levels of atomic samarium. Unique value assignment was done for seven energy levels in the energy region 34,800–36,200 cm-1 , recently observed and reported in ...

  18. Measurement of total angular momentum values of high-lying even ...

    Indian Academy of Sciences (India)

    Measurement of total angular momentum values of high-lying even-parity atomic states of samarium by spectrally resolved laser-induced fluorescence technique. A K PULHANI∗, M L SHAH, G P GUPTA and B M SURI. Laser and Plasma Technology Division, Bhabha Atomic Research Centre,. Mumbai 400 085, India.

  19. Angular structure of light polarization and singularities in transmittance of nematic liquid crystal cells

    Science.gov (United States)

    Kiselev, Alexei D.; Vovk, Roman G.; Buinyi, Igor O.; Soskin, Marat S.

    2007-06-01

    We study the angular structure of polarization of light transmitted through a nematic liquid crystal (NLC) cell by analyzing the polarization state as a function of the incidence angles. Our theoretical results are obtained by evaluating the Stokes parameters that characterize the polarization state of plane waves propagating through the NLC layer at varying direction of incidence. Using the Stokes polarimetry technique we carried out the measurements of the polarization resolved conoscopic patterns emerging after the homeotropically aligned NLC cell illuminated by the convergent light beam. The resulting polarization resolved angular patterns are described both theoretically and experimentally in terms of the polarization singularities such as C-points (points of circular polarization) and L-lines (lines of linear polarization). When the ellipticity of the incident light varies, the angular patterns are found to undergo transformations involving the processes of creation and annihilation of the C-points.

  20. Probing the switching state of a surface-mounted azobenzene derivative using femtosecond XUV photoemission

    Science.gov (United States)

    Grunau, Jan; Heinemann, Nils; Rohwer, Timm; Zargarani, Dordaneh; Kuhn, Sonja; Jung, Ullrich; Kipp, Lutz; Magnussen, Olaf; Herges, Rainer; Bauer, Michael

    2012-03-01

    Photoemission spectroscopy using femtosecond XUV light pulses is applied to probe the isomerization state of the molecular switch 3-(4-(4-hexyl-phenylazo)-phenoxy)-propane-1-thiol deposited by liquid phase self-assembly on Au(111). Spectral shifts of valence-electronic signatures that we associate with the carbon C2s orbital enable us to distinguish the trans and the cis isomerization state of the adsorbed molecules. These preliminary results envision the potential to probe reversible switching processes of surface-mounted molecules in real time by tracking the temporal evolution of the electronic and nuclear degrees of freedom in a femtosecond XUV photoemission experiment.

  1. Angle - resolved photoemission study of two phases of the GaAs(100)-c(4x4) surface

    Czech Academy of Sciences Publication Activity Database

    Cukr, Miroslav; Jiříček, Petr; Bartoš, Igor; Sadowski, J.

    2008-01-01

    Roč. 100, - (2008), 072017/1-072017/4 ISSN 1742-6588 R&D Projects: GA AV ČR IAA100100628; GA ČR GA202/07/0601 Institutional research plan: CEZ:AV0Z10100521 Keywords : gallium arsenide * molecular beam epitaxy * photoelectron spectroscopy * surface reconstruction * surface phases * electron states Subject RIV: BM - Solid Matter Physics ; Magnetism

  2. The electronic structure of clean and adsorbate-covered Bi2Se3: an angle-resolved photoemission study

    DEFF Research Database (Denmark)

    Bianchi, Marco; Hatch, Richard; Guan, Dandan

    2012-01-01

    , the Dirac point moves to higher binding energies, indicating an increasingly strong downward bending of the bands near the surface. This time-dependent band bending is related to a contamination of the surface and can be accelerated by intentionally exposing the surface to carbon monoxide and other species...

  3. Real-time monitoring of initial thermal oxidation on Si(001) surfaces by synchrotron radiation photoemission spectroscopy

    CERN Document Server

    Yoshigoe, A; Teraoka, Y

    2003-01-01

    The thermal oxidation of Si(001) surfaces at 860 K, 895 K, 945 K and 1000 K under the O sub 2 pressure of 1 x 10 sup - sup 4 Pa has been investigated by time-resolved photoemission measurements with synchrotron radiation. Based on time evolution analyses by reaction kinetics models, it was found that the oxidation at 860 K, 895 K and 945 K has progressed with the Langmuir adsorption type, whereas the oxidation at 1000 K has showed the character of the two-dimensional island growth involving SiO desorption. The oxidation rates increases with increasing surface temperature in the passive oxidation condition. The time evolution of each Si oxidation state (Si sup n sup + : n = 1, 2, 3, 4) derived from the Si-2p core-level shifts has also been analyzed. The results revealed that the thermal energy contribution to the migration process of the adsorbed oxygen and the emission of the bulk silicon atoms. Thus, the fraction of the Si sup 4 sup + bonding state, i.e. SiO sub 2 structure, was increased. (author)

  4. Photoemission of Bi_{2}Se_{3} with Circularly Polarized Light: Probe of Spin Polarization or Means for Spin Manipulation?

    Directory of Open Access Journals (Sweden)

    J. Sánchez-Barriga

    2014-03-01

    Full Text Available Topological insulators are characterized by Dirac-cone surface states with electron spins locked perpendicular to their linear momenta. Recent theoretical and experimental work implied that this specific spin texture should enable control of photoelectron spins by circularly polarized light. However, these reports questioned the so far accepted interpretation of spin-resolved photoelectron spectroscopy. We solve this puzzle and show that vacuum ultraviolet photons (50–70 eV with linear or circular polarization indeed probe the initial-state spin texture of Bi_{2}Se_{3} while circularly polarized 6-eV low-energy photons flip the electron spins out of plane and reverse their spin polarization, with its sign determined by the light helicity. Our photoemission calculations, taking into account the interplay between the varying probing depth, dipole-selection rules, and spin-dependent scattering effects involving initial and final states, explain these findings and reveal proper conditions for light-induced spin manipulation. Our results pave the way for future applications of topological insulators in optospintronic devices.

  5. Photoemission study of the electronic structure and charge density waves of Na2Ti2Sb2O.

    Science.gov (United States)

    Tan, S Y; Jiang, J; Ye, Z R; Niu, X H; Song, Y; Zhang, C L; Dai, P C; Xie, B P; Lai, X C; Feng, D L

    2015-04-30

    The electronic structure of Na2Ti2Sb2O single crystal is studied by photon energy and polarization dependent angle-resolved photoemission spectroscopy (ARPES). The obtained band structure and Fermi surface agree well with the band structure calculation of Na2Ti2Sb2O in the non-magnetic state, which indicates that there is no magnetic order in Na2Ti2Sb2O and the electronic correlation is weak. Polarization dependent ARPES results suggest the multi-band and multi-orbital nature of Na2Ti2Sb2O. Photon energy dependent ARPES results suggest that the electronic structure of Na2Ti2Sb2O is rather two-dimensional. Moreover, we find a density wave energy gap forms below the transition temperature and reaches 65 meV at 7 K, indicating that Na2Ti2Sb2O is likely a weakly correlated CDW material in the strong electron-phonon interaction regime.

  6. Dual electromagnetism: helicity, spin, momentum and angular momentum

    International Nuclear Information System (INIS)

    Bliokh, Konstantin Y; Nori, Franco; Bekshaev, Aleksandr Y

    2013-01-01

    The dual symmetry between electric and magnetic fields is an important intrinsic property of Maxwell equations in free space. This symmetry underlies the conservation of optical helicity and, as we show here, is closely related to the separation of spin and orbital degrees of freedom of light (the helicity flux coincides with the spin angular momentum). However, in the standard field-theory formulation of electromagnetism, the field Lagrangian is not dual symmetric. This leads to problematic dual-asymmetric forms of the canonical energy–momentum, spin and orbital angular-momentum tensors. Moreover, we show that the components of these tensors conflict with the helicity and energy conservation laws. To resolve this discrepancy between the symmetries of the Lagrangian and Maxwell equations, we put forward a dual-symmetric Lagrangian formulation of classical electromagnetism. This dual electromagnetism preserves the form of Maxwell equations, yields meaningful canonical energy–momentum and angular-momentum tensors, and ensures a self-consistent separation of the spin and orbital degrees of freedom. This provides a rigorous derivation of the results suggested in other recent approaches. We make the Noether analysis of the dual symmetry and all the Poincaré symmetries, examine both local and integral conserved quantities and show that only the dual electromagnetism naturally produces a complete self-consistent set of conservation laws. We also discuss the observability of physical quantities distinguishing the standard and dual theories, as well as relations to quantum weak measurements and various optical experiments. (paper)

  7. Internal photoemission for photovoltaic using p-type Schottky barrier: Band structure dependence and theoretical efficiency limits

    Science.gov (United States)

    Shih, Ko-Han; Chang, Yin-Jung

    2018-01-01

    Solar energy conversion via internal photoemission (IPE) across a planar p-type Schottky junction is quantified for aluminum (Al) and copper (Cu) in the framework of direct transitions with non-constant matrix elements. Transition probabilities and k-resolved group velocities are obtained based on pseudo-wavefunction expansions and realistic band structures using the pseudopotential method. The k-resolved number of direct transitions, hole photocurrent density, quantum yield (QY), and the power conversion efficiency (PCE) under AM1.5G solar irradiance are subsequently calculated and analyzed. For Al, the parabolic and "parallel-band" effect along the U-W-K path significantly enhances the transition rate with final energies of holes mainly within 1.41 eV below the Fermi energy. For Cu, d-state hot holes mostly generated near the upper edge of 3d bands dominate the hole photocurrent and are weekly (strongly) dependent on the barrier height (metal film thickness). Hot holes produced in the 4s band behave just oppositely to their d-state counterparts. Non-constant matrix elements are shown to be necessary for calculations of transitions due to time-harmonic perturbation in Cu. Compared with Cu, Al-based IPE in p-type Schottky shows the highest PCE (QY) up to about 0.2673% (5.2410%) at ΦB = 0.95 eV (0.5 eV) and a film thickness of 11 nm (20 nm). It is predicted that metals with relatively dispersionless d bands (such as Cu) in most cases do not outperform metals with photon-accessible parallel bands (such as Al) in photon energy conversion using a planar p-type Schottky junction.

  8. Angular Positioning Sensor for Space Mechanisms

    Science.gov (United States)

    Steiner, Nicolas; Chapuis, Dominique

    2013-09-01

    Angular position sensors are used on various rotating mechanisms such as solar array drive mechanisms, antenna pointing mechanisms, scientific instruments, motors or actuators.Now a days, potentiometers and encoders are mainly used for angular measurement purposes. Both of them have their own pros and cons.As alternative, Ruag Space Switzerland Nyon (RSSN) is developing and qualifying two innovative technologies of angular position sensors which offer easy implementation, medium to very high lifetime and high flexibility with regards to the output signal shape/type.The Brushed angular position sensor uses space qualified processes which are already flying on RSSN's sliprings for many years. A large variety of output signal shape can be implemented to fulfill customer requirements (digital, analog, customized, etc.).The contactless angular position sensor consists in a new radiation hard Application Specific Integrated Circuit (ASIC) based on the Hall effect and providing the angular position without complex processing algorithm.

  9. Oral candidiasis and angular cheilitis.

    Science.gov (United States)

    Sharon, Victoria; Fazel, Nasim

    2010-01-01

    Candidiasis, an often encountered oral disease, has been increasing in frequency. Most commonly caused by the overgrowth of Candida albicans, oral candidiasis can be divided into several categories including acute and chronic forms, and angular cheilitis. Risk factors for the development of oral candidiasis include immunosuppression, wearing of dentures, pharmacotherapeutics, smoking, infancy and old age, endocrine dysfunction, and decreased salivation. Oral candidiasis may be asymptomatic. More frequently, however, it is physically uncomfortable, and the patient may complain of burning mouth, dysgeusia, dysphagia, anorexia, and weight loss, leading to nutritional deficiency and impaired quality of life. A plethora of antifungal treatments are available. The overall prognosis of oral candidiasis is good, and rarely is the condition life threatening with invasive or recalcitrant disease.

  10. Management of angular cheilitis for children

    Directory of Open Access Journals (Sweden)

    Fajriani Fajriani

    2016-06-01

    Full Text Available Angular cheilitis is one type of oral soft tissue disease that can occur in both children and adults, the condition is characterized by cracks and inflammation in both corners of the mouth. Although this disease does not cause severe disruption but quite disturbing activity and also one's physical appearance. Angular cheilitis light will disappear on their own over time.Severe conditions that can cause pain and bleading. aims to give feedback on peers about managment angular cheilitis in children.

  11. Aberration-corrected multipole Wien filter for energy-filtered x-ray photoemission electron microscopy

    OpenAIRE

    Niimi, Hironobu; Chun, Wang-Jae; Suzuki, Shushi; Asakura, Kiyotaka; Kato, Makoto

    2007-01-01

    The aberration of a multipole Wien filter for energy-filtered x-ray photoemission electron microscopy was analyzed and the optimized Fourier components of the electric and magnetic fields for the third-order aperture aberration corrections were obtained. It was found that the third-order aperture aberration correction requires 12 electrodes and magnetic poles. ©2007 American Institute of Physics

  12. Aberration-corrected multipole Wien filter for energy-filtered x-ray photoemission electron microscopy

    Science.gov (United States)

    Niimi, Hironobu; Chun, Wang-Jae; Suzuki, Shushi; Asakura, Kiyotaka; Kato, Makoto

    2007-06-01

    The aberration of a multipole Wien filter for energy-filtered x-ray photoemission electron microscopy was analyzed and the optimized Fourier components of the electric and magnetic fields for the third-order aperture aberration corrections were obtained. It was found that the third-order aperture aberration correction requires 12 electrodes and magnetic poles.

  13. A vacuum photoemission detector for X-ray tomography on the ITER facility

    NARCIS (Netherlands)

    Barykov, IA; Gott, YV; Stepanenko, MM

    2004-01-01

    A vacuum photoemission detector designed for plasma tornography in X rays on the ITER facility is described. Such detectors allow X rays to be detected in the presence of intense neutron and gamma-photon fluxes. The results of tests of a prototype of this detector on a Co-60 source of gamma rays,

  14. Correlation versus surface effects in photoemission of quasi-1D organic conductors

    DEFF Research Database (Denmark)

    Claessen, R.; Schwingenschlogl, U.; Sing, M.

    2002-01-01

    The absence of spectral weight at the Fermi level in photoemission spectra of quasi-1D organic conductors has been interpreted as possible evidence for an unusual many-body state. We demonstrate that great care must be exercised to draw this conclusion exclusively on the basis of a pseudogap. A d...

  15. Absorption enhancement in metal nanoparticles for photoemission current for solar cells

    DEFF Research Database (Denmark)

    Gritti, Claudia; Novitsky, Andrey; Malureanu, Radu

    2012-01-01

    In order to improve the photoconversion efficiency, we consider the possibility of increasing the photocurrent in solar cells exploiting the electron photoemission from small metal nanoparticles into a semiconductor. The effect is caused by the absorption of photons and generation of local surfac...

  16. Attosecond-controlled photoemission from metal nanowire tips in the few-electron regime

    Directory of Open Access Journals (Sweden)

    B. Ahn

    2017-03-01

    Full Text Available Metal nanotip photoemitters have proven to be versatile in fundamental nanoplasmonics research and applications, including, e.g., the generation of ultrafast electron pulses, the adiabatic focusing of plasmons, and as light-triggered electron sources for microscopy. Here, we report the generation of high energy photoelectrons (up to 160 eV in photoemission from single-crystalline nanowire tips in few-cycle, 750-nm laser fields at peak intensities of (2-7.3 × 1012 W/cm2. Recording the carrier-envelope phase (CEP-dependent photoemission from the nanowire tips allows us to identify rescattering contributions and also permits us to determine the high-energy cutoff of the electron spectra as a function of laser intensity. So far these types of experiments from metal nanotips have been limited to an emission regime with less than one electron per pulse. We detect up to 13 e/shot and given the limited detection efficiency, we expect up to a few ten times more electrons being emitted from the nanowire. Within the investigated intensity range, we find linear scaling of cutoff energies. The nonlinear scaling of electron count rates is consistent with tunneling photoemission occurring in the absence of significant charge interaction. The high electron energy gain is attributed to field-induced rescattering in the enhanced nanolocalized fields at the wires apex, where a strong CEP-modulation is indicative of the attosecond control of photoemission.

  17. Effect of wave-function localization on the time delay in photoemission from surfaces

    International Nuclear Information System (INIS)

    Zhang, C.-H.; Thumm, U.

    2011-01-01

    We investigate streaking time delays in the photoemission from a solid model surface as a function of the degree of localization of the initial-state wave functions. We consider a one-dimensional slab with lattice constant a latt of attractive Gaussian-shaped core potentials of width σ. The parameter σ/a latt thus controls the overlap between adjacent core potentials and localization of the electronic eigenfunctions on the lattice points. Small values of σ/a latt latt > or approx 0.4. By numerically solving the time-dependent Schroedinger equation, we calculate photoemission spectra from which we deduce a characteristic bimodal shape of the band-averaged photoemission time delay: as the slab eigenfunctions become increasingly delocalized, the time delay quickly decreases near σ/a latt =0.3 from relatively large values below σ/a latt ∼0.2 to much smaller delays above σ/a latt ∼0.4. This change in wave-function localization facilitates the interpretation of a recently measured apparent relative time delay between the photoemission from core and conduction-band levels of a tungsten surface.

  18. Enhanced photoemission from laser-excited plasmonic nano-objects in periodic arrays

    Czech Academy of Sciences Publication Activity Database

    Fedorov, N.; Geoffroy, G.; Duchateau, G.; Štolcová, L.; Proška, J.; Novotný, F.; Domonkos, Mária; Jouin, H.; Martin, P.; Raynaud, M.

    2016-01-01

    Roč. 28, č. 31 (2016), s. 1-15, č. článku 315301. ISSN 0953-8984 R&D Projects: GA ČR(CZ) GBP108/12/G108 Institutional support: RVO:68378271 Keywords : photoemission * laser excitation * surface plasmon * plasmonics Subject RIV: BH - Optics, Masers, Lasers Impact factor: 2.649, year: 2016

  19. Attosecond-controlled photoemission from metal nanowire tips in the few-electron regime

    KAUST Repository

    Ahn, B.

    2017-02-07

    Metal nanotip photoemitters have proven to be versatile in fundamental nanoplasmonics research and applications, including, e.g., the generation of ultrafast electron pulses, the adiabatic focusing of plasmons, and as light-triggered electron sources for microscopy. Here, we report the generation of high energy photoelectrons (up to 160 eV) in photoemission from single-crystalline nanowire tips in few-cycle, 750-nm laser fields at peak intensities of (2-7.3) × 1012 W/cm2. Recording the carrier-envelope phase (CEP)-dependent photoemission from the nanowire tips allows us to identify rescattering contributions and also permits us to determine the high-energy cutoff of the electron spectra as a function of laser intensity. So far these types of experiments from metal nanotips have been limited to an emission regime with less than one electron per pulse. We detect up to 13 e/shot and given the limited detection efficiency, we expect up to a few ten times more electrons being emitted from the nanowire. Within the investigated intensity range, we find linear scaling of cutoff energies. The nonlinear scaling of electron count rates is consistent with tunneling photoemission occurring in the absence of significant charge interaction. The high electron energy gain is attributed to field-induced rescattering in the enhanced nanolocalized fields at the wires apex, where a strong CEP-modulation is indicative of the attosecond control of photoemission.

  20. Transverse and longitudinal angular momenta of light

    Energy Technology Data Exchange (ETDEWEB)

    Bliokh, Konstantin Y., E-mail: k.bliokh@gmail.com [Center for Emergent Matter Science, RIKEN, Wako-shi, Saitama 351-0198 (Japan); Nonlinear Physics Centre, RSPhysE, The Australian National University, Canberra, ACT 0200 (Australia); Nori, Franco [Center for Emergent Matter Science, RIKEN, Wako-shi, Saitama 351-0198 (Japan); Physics Department, University of Michigan, Ann Arbor, MI 48109-1040 (United States)

    2015-08-26

    We review basic physics and novel types of optical angular momentum. We start with a theoretical overview of momentum and angular momentum properties of generic optical fields, and discuss methods for their experimental measurements. In particular, we describe the well-known longitudinal (i.e., aligned with the mean momentum) spin and orbital angular momenta in polarized vortex beams. Then, we focus on the transverse (i.e., orthogonal to the mean momentum) spin and orbital angular momenta, which were recently actively discussed in theory and observed in experiments. First, the recently-discovered transverse spin  angular momenta appear in various structured fields: evanescent waves, interference fields, and focused beams. We show that there are several kinds of transverse spin angular momentum, which differ strongly in their origins and physical properties. We describe extraordinary features of the transverse optical spins and overview recent experiments. In particular, the helicity-independent transverse spin inherent in edge evanescent waves offers robust spin–direction coupling at optical interfaces (the quantum spin Hall effect of light). Second, we overview the transverse orbital angular momenta of light, which can be both extrinsic and intrinsic. These two types of the transverse orbital angular momentum are produced by spatial shifts of the optical beams (e.g., in the spin Hall effect of light) and their Lorentz boosts, respectively. Our review is underpinned by a unified theory of the angular momentum of light based on the canonical momentum and spin densities, which avoids complications associated with the separation of spin and orbital angular momenta in the Poynting picture. It allows us to construct a comprehensive classification of all known optical angular momenta based on their key parameters and main physical properties.

  1. Linear and circular dichroism in angle resolved Fe 3p photomission. Revision 1

    International Nuclear Information System (INIS)

    Tamura, E.; Waddill, G.D.; Tobin, J.G.; Sterne, P.A.

    1994-01-01

    Using a recently developed spin-polarized, fully relativistic, multiple scattering approach based on the layer KKR Green function method, we have reproduced the Fe 3p angle-resolved soft x-ray photoemission spectra and analyzed the associated large magnetic dichroism effects for excitation with both linearly and circularly polarized light. Comparison between theory and experiment yields a spin-orbit splitting of 1.0--1.2 eV and an exchange splitting of 0.9-- 1.0 eV for Fe 3p. These values are 50--100% larger than those hitherto obtained experimentally

  2. Final state effects in photoemission studies of Fermi surfaces

    International Nuclear Information System (INIS)

    Kurtz, Richard L; Browne, Dana A; Mankey, Gary J

    2007-01-01

    Photoelectron spectroscopy is one of the most important methods for extracting information about the Fermi surface (FS) of materials. An electron photoexcited from the FS is emitted from the crystal conserving the parallel momentum, k parallel , while the perpendicular momentum k perpendicular is reduced due to the surface potential barrier. A simple interpretation of the process assumes the final state is free-electron-like allowing one to 'map' the detected photoelectron back to its initial k momentum. There are multiple final state effects that can complicate the interpretation of photoelectron data and these effects are reviewed here. These can involve both energy and k broadening, which can give rise to shadow or ghost FS contours, scattering and final state diffraction effects that modify intensities, and matrix element effects which reflect the symmetries of the states involved and can be highly dependent on photon polarization. These matrix elements result in contours of photoelectron intensity that follow the dispersion in k-space of the initial state, the FS, and the final state. Locations where intensities go to zero due to matrix element and symmetry effects can result in gaps where FS contours 'disappear'. Recognition that these effects can play a significant role in determining the measured angular distributions is crucial in developing an informed model of where the FS contours actually lie in relation to measured intensity contours

  3. Angular momentum transfer in incomplete fusion

    Indian Academy of Sciences (India)

    fusion reactions. The angular momentum of the intermediate nucleus formed in incomplete fusion was deduced from the isomeric cross-section ratio by considering the statistical de- excitation of the incompletely fused composite nucleus. The data show that incomplete fusion is associated with angular momenta slightly ...

  4. Responsive web design with AngularJS

    CERN Document Server

    Patel, Sandeep Kumar

    2014-01-01

    If you are an AngularJS developer who wants to learn about responsive web application development, this book is ideal for you. Responsive Web Design with AngularJS is intended for web developers or designers with a basic knowledge of HTML, CSS, and JavaScript.

  5. Angular momentum transfer in incomplete fusion

    Indian Academy of Sciences (India)

    The angular momentum of the intermediate nucleus formed in incomplete fusion was deduced from the isomeric cross-section ratio by considering the statistical de-excitation of the incompletely fused composite nucleus. The data show that incomplete fusion is associated with angular momenta slightly smaller than critical ...

  6. Accelerated rotation with orbital angular momentum modes

    CSIR Research Space (South Africa)

    Schulze, C

    2015-04-01

    Full Text Available A 91, 043821 (2015) Accelerated rotation with orbital angular momentum modes Christian Schulze, Filippus S. Roux, Angela Dudley, Ronald Rop, Michael Duparr´e, and Andrew Forbes Abstract: We introduce a class of light field that angularly...

  7. Dijet angular distributions at D0

    International Nuclear Information System (INIS)

    Fatyga, M.K.

    1996-09-01

    Measurements of the dijet angular distributions are relatively insensitive to parton distribution functions and thus offer an excellent method of testing the LO and NLO predictions of perturbative QCD. The authors present measurements of the dijet angular distributions for |η| < 3.0 in p anti p collisions at √s = 1.8 TeV

  8. Experimental determination of high angular momentum states

    International Nuclear Information System (INIS)

    Barreto, J.L.V.

    1985-01-01

    The current knowledge of the atomic nucleus structure is summarized. A short abstract of the nuclear properties at high angular momentum and a more detailed description of the experimental methods used in the study of high angular momenta is made. (L.C.) [pt

  9. Concepts of radial and angular kinetic energies

    DEFF Research Database (Denmark)

    Dahl, Jens Peder; Schleich, W.P.

    2002-01-01

    We consider a general central-field system in D dimensions and show that the division of the kinetic energy into radial and angular parts proceeds differently in the wave-function picture and the Weyl-Wigner phase-space picture, Thus, the radial and angular kinetic energies are different quantities...

  10. Perturbed angular correlations and distributions

    International Nuclear Information System (INIS)

    Makaryunas, K.

    1976-01-01

    The present index comprises original works and review papers on the perturbed angular correlations (PAC) and distributions (PAD). The articles published in the Soviet and foreign journals as well as the materials of conferences, monographs and collections published in the USSR and abroad, the preprints produced by various institutes and abstracts of disertations are included from 1948 up to 1973. The whole material compiled in this index is divided into three parts. Part one is a bibliographic index. All papers in this part are divided into three sections. Section one comprises the papers devoted to the theoretical works on PAC, review papers, monographs, materials of conferences. Section two deals with the works of methodical character where correlation spectrometers as well as the treatment of experimental data are described. In section three experimental works with concrete nuclei are compiled. Part two gives the characteristic of works performed with concrete nuclei. This part is presented in the form of the table in which the works are systematized according to the chemical elements and isotopes. The table shows the characteristics of the nuclear levels used in the investigations by PAC as well as brief characteristics of experiments and results obtained. Part three - appendix contains alphabetic index of the authors, the list of the used editions with the abbreviations of the titles of these editions. The lists indicating the dynamic of the quantity of works on PAC and the distribution according to the literature sources are also given

  11. Observation of two-photon photoemission from cesium telluride photocathodes excited by a near-infrared laser

    Science.gov (United States)

    Panuganti, H.; Piot, P.

    2017-02-01

    We explore the nonlinear photoemission in cesium telluride (Cs2Te) photocathodes where an ultrashort (˜100 fs full width at half max) 800-nm infrared laser is used as the drive-laser in lieu of the typical ˜266-nm ultraviolet laser. An important figure of merit for photocathodes, the quantum efficiency, we define here for nonlinear photoemission processes in order to compare with linear photoemission. The charge against drive-laser (infrared) energy is studied for different laser energy and intensity values and cross-compared with previously performed similar studies on copper [P. Musumeci et al., Phys. Rev. Lett. 104, 084801 (2010)], a metallic photocathode. We particularly observe two-photon photoemission in Cs2Te using the infrared laser in contrast to the anticipated three-photon process as observed for metallic photocathodes.

  12. Angle-resolved ion TOF spectrometer with a position sensitive detector

    Energy Technology Data Exchange (ETDEWEB)

    Saito, Norio [Electrotechnical Lab., Tsukuba, Ibaraki (Japan); Heiser, F.; Wieliczec, K.; Becker, U.

    1996-07-01

    A angle-resolved ion time-of-flight mass spectrometer with a position sensitive anode has been investigated. Performance of this spectrometer has been demonstrated by measuring an angular distribution of a fragment ion pair, C{sup +} + O{sup +}, from CO at the photon energy of 287.4 eV. The obtained angular distribution is very close to the theoretically expected one. (author)

  13. Resonant photoemission of La and Yb at the 3d absorption edge

    CERN Document Server

    Lagarde, P; Ogasawara, H; Kotani, A

    2003-01-01

    Resonant photoemission and resonant Auger experiments at the 3d threshold are presented for La and Yb over a binding energy domain which extends up to the 4p levels. These experimental results are well explained by calculations in the framework of full-multiplet Hartree-Fock theory with an atomic model. Strong participator and spectator Auger transitions are observed without ordinary Auger transition, indicating that the 4f wavefunction is well localized in the intermediate state even in the case of La. The 4d sub 3 sub / sub 2 and 4d sub 5 sub / sub 2 branching ratio of the 4d resonant photoemission of La at the M sub 4 and M sub 5 edges is observed experimentally and analyzed theoretically. The difference in the resonant processes behavior for La and Yb is discussed based upon the different 4f occupation number.

  14. Recent Developments at the High-Charge PHIN Photoinjector and the CERN Photoemission Laboratory

    CERN Document Server

    Hessler, C; Doebert, S; Fedosseev, V; Martini, I; Martyanov, M; Perillo Marcone, A; Sroka, S

    2014-01-01

    The high-charge PHIN photoinjector has originally been developed to study the feasibility of a photoinjector option for the drive beam of the CLIC Test Facility 3 (CTF3) at CERN and is now being used to inevestigate the feasibility of a drive beam photoinjector for CLIC. In this paper recent R&D efforts to improve the parameters of the existing system towards CLIC requirements will be discussed. This includes studies of a feedback loop for intensity stabilization, the upgrade of the PHIN vacuum system and the planned upgrade of the driving laser system. For photocathode production and R&D a dedicated photoemission laboratory is available at CERN. To increase the production rate of photocathodes and the availability of the photoemission lab for other studies, an upgrade of the photocathode preparation system with a load-lock system is under study and will also be presented.

  15. DC High Voltage Conditioning of Photoemission Guns at Jefferson Lab FEL

    International Nuclear Information System (INIS)

    DC high voltage photoemission electron guns with GaAs photocathodes have been used to produce polarized electron beams for nuclear physics experiments for about 3 decades with great success. In the late 1990s, Jefferson Lab adopted this gun technology for a free electron laser (FEL), but to assist with high bunch charge operation, considerably higher bias voltage is required compared to the photoguns used at the Jefferson Lab Continuous Electron Beam Accelerator Facility. The FEL gun has been conditioned above 400 kV several times, albeit encountering non-trivial challenges with ceramic insulators and field emission from electrodes. Recently, high voltage processing with krypton gas was employed to process very stubborn field emitters. This work presents a summary of the high voltage techniques used to high voltage condition the Jefferson Lab FEL photoemission gun.

  16. Volume and surface photoemission from tungsten. I. Calculation of band structure and emission spectra

    DEFF Research Database (Denmark)

    Christensen, N. Egede; Feuerbacher, B.

    1974-01-01

    of photoemission spectra from W single crystals. The nondirect as well as the direct models for bulk photoemission processes are investigated. The emission from the three low-index surfaces (100), (110), and (111) exhibits strong dependence on direction and acceptance cone. According to the present band model...... there should essentially be no emission normal to the (110) face for photon energies between 9.4 and 10.6 eV. Experimental observation of emission in this gap, however, implies effects not included in the simple bulk models. In particular, effects arising from surface emission have been considered, i.......e., emission of those electrons which are excited in a single-step process from initial states near the surface to final states outside the crystal. The electrons that are emitted from the surface in directions perpendicular to the crystal planes carry information on the one-dimensional surface density...

  17. Coherent Peaks and Minimal Probing Depth in Photoemission Spectroscopy of Mott-Hubbard Systems

    Science.gov (United States)

    Panaccione, G.; Altarelli, M.; Fondacaro, A.; Georges, A.; Huotari, S.; Lacovig, P.; Lichtenstein, A.; Metcalf, P.; Monaco, G.; Offi, F.; Paolasini, L.; Poteryaev, A.; Tjernberg, O.; Sacchi, M.

    2006-09-01

    We have measured hard x-ray photoemission spectra of pure vanadium sesquioxide (V2O3) across its metal-insulator transition. We show that, in the metallic phase, a clear correlation exists between the shakedown satellites observed in the vanadium 2p and 3p core-level spectra and the coherent peak measured at the Fermi level. Comparing experimental results and dynamical mean-field theory calculations, we estimate the Hubbard energy U in V2O3 (4.20±0.05eV). From our bulk-sensitive photoemission spectra we infer the existence of a critical probing depth for investigating electronic properties in strongly correlated solids.

  18. Photoemission from Low Work Function Coated Metal Surfaces A Comparison of Theory to Experiment

    CERN Document Server

    Jensen, Kevin; Moody, Nathan A

    2005-01-01

    The development of rugged and/or self rejuvenating photocathodes with high quantum efficiency (QE) using the longest wavelength drive laser is of paramount importance for RF photo-injectors for high power FELs and accelerators. We report on our program to develop advanced photocathodes and to develop and validate models of photoemission from coated metals to analyze experimental data,* provide emission models usable by beam simulation codes,** and project performance. The model accounts for the effects of laser heating, thermal evolution, surface conditions, laser parameters, and material characteristics, and predicts current distribution and QE. The photoemission and QE from metals and dispenser photocathodes is evaluated: the later introduces complications such as coverage non-uniformity and field enhancement. The performance of the models is compared to our experimental results for dispenser photocathodes and cesiated surfaces (e.g., tungsten, silver, etc.) in which the time-dependent models are shown to a...

  19. Introduction of spectroscopic photoemission and low energy electron microscope in SPring-8

    International Nuclear Information System (INIS)

    Guo, FangZhun; Kobayashi, Keisuke; Kinoshita, Toyohiko

    2005-01-01

    An upright configuration SPELEEM (Spectroscopic PhotoEmission and Low Energy Electron Microscope) has been introduced in SPring-8 in the framework of the nanotechnology support project of Ministry of Education, Culture, Sport, Science and Technology (MEXT), Japan. SPELEEM combines microscopy, spectroscopy and diffraction in one system, which allows a comprehensive characterization of the specimen. The combination of SPELEEM and polarized (circularly or linearly) soft X-rays in SPring-8 is expected to realize the highest performance. The characteristics of SPELEEM and typical results, for example nano-XANES (X-ray absorption near edge structure) of Fe oxide on Fe(100) surface, nano-XPS (X-ray photoemission spectroscopy) of indium (In) on Si(111) and antiferro-magnetic domain structure images of NiO(001) single crystal, are reported. (author)

  20. Electron attachment rate constant measurement by photoemission electron attachment ion mobility spectrometry (PE-EA-IMS)

    International Nuclear Information System (INIS)

    Su, Desheng; Niu, Wenqi; Liu, Sheng; Shen, Chengyin; Huang, Chaoqun; Wang, Hongmei; Jiang, Haihe; Chu, Yannan

    2012-01-01

    Photoemission electron attachment ion mobility spectrometry (PE-EA-IMS), with a source of photoelectrons induced by vacuum ultraviolet radiation on a metal surface, has been developed to study electron attachment reaction at atmospheric pressure using nitrogen as the buffer gas. Based on the negative ion mobility spectra, the rate constants for electron attachment to tetrachloromethane and chloroform were measured at ambient temperature as a function of the average electron energy in the range from 0.29 to 0.96 eV. The experimental results are in good agreement with the data reported in the literature. - Highlights: ► Photoemission electron attachment ion mobility spectrometry (PE-EA-IMS) was developed to study electron attachment reaction. ► The rate constants of electron attachment to CCl 4 and CHCl 3 were determined. ► The present experimental results are in good agreement with the previously reported data.

  1. Plasmonic silicon Schottky photodetectors: The physics behind graphene enhanced internal photoemission

    Directory of Open Access Journals (Sweden)

    Uriel Levy

    2017-02-01

    Full Text Available Recent experiments have shown that the plasmonic assisted internal photoemission from a metal to silicon can be significantly enhanced by introducing a monolayer of graphene between the two media. This is despite the limited absorption in a monolayer of undoped graphene ( ∼ π α = 2.3 % . Here we propose a physical model where surface plasmon polaritons enhance the absorption in a single-layer graphene by enhancing the field along the interface. The relatively long relaxation time in graphene allows for multiple attempts for the carrier to overcome the Schottky barrier and penetrate into the semiconductor. Interface disorder is crucial to overcome the momentum mismatch in the internal photoemission process. Our results show that quantum efficiencies in the range of few tens of percent are obtainable under reasonable experimental assumptions. This insight may pave the way for the implementation of compact, high efficiency silicon based detectors for the telecom range and beyond.

  2. Core and valence level photoemission and photoabsorption study of icosahedral Al-Pd-Mn quasicrystals

    International Nuclear Information System (INIS)

    Horn, K; Theis, W; Paggel, J J; Barman, S R; Rotenberg, E; Ebert, Ph; Urban, K

    2006-01-01

    The electronic structure of quasicrystalline Al-Pd-Mn is investigated by means of valence and core level photoelectron spectroscopy. Variations of the photoionization cross section in the constituents' valence electronic levels as a function of photon energy are used to identify contributions from the different atomic species, in particular near the Pd 4d Cooper minimum. Resonant photoemission at the Mn 2p absorption edge shows the contribution of the Mn 3d states to the density of states in a region near the Fermi level. The asymmetry of Pd 3d and Mn 2p core level photoemission lines, and its difference for emission from metallic and quasicrystalline phases, are utilized to infer the contributions of the different constituents to the density of states at the Fermi level

  3. Photoemission in the Anderson model for rare earth compounds with floating valences

    International Nuclear Information System (INIS)

    Frota, H.O. da.

    1985-01-01

    X-ray photoemission spectra (XPS) are calculated for the spin-degenerate Anderson model of valence fluctuation compounds. Based on the renormalization group technique originally introduced by Wilson to calculate the magnetic susceptibility for the Kondo model, the numerical calculation has uniform accuracy over the entire parameter space of the Anderson model; at any given photoelectron energy, a maximum error of 4% is estimated for the calculated photoemission current. The calculated spectra display two peaks associated with the two possible x-ray induced transitions between the n f = 0,1 or 2 occupations of the f-orbital: a first ionization peak corresponding to the n f = 2 → n f = 1 transition and a second ionization peak due to the n f 1 → n f = 0 transition. (author)

  4. Dilution effect on the U 5f states in Au matrix: a photoemission spectroscopy study

    Czech Academy of Sciences Publication Activity Database

    Eloirdi, R.; Gouder, T.; Wastin, F.; Huber, F.; Shick, Alexander; Kolorenč, Jindřich

    2011-01-01

    Roč. 84, č. 23 (2011), 235143/1-235143/7 ISSN 1098-0121 R&D Projects: GA ČR(CZ) GAP204/10/0330; GA AV ČR IAA100100912 Institutional research plan: CEZ:AV0Z10100520 Keywords : x-ray photoemission * electronic-structure * photoelectron-spectroscopy * fermion systems Subject RIV: BM - Solid Matter Physics ; Magnetism Impact factor: 3.691, year: 2011

  5. Hot Electron Photoemission from Plasmonic Nanoparticles: Role of Transient Absorption in Surface Mechanism

    DEFF Research Database (Denmark)

    Uskov, Alexander V.; Protsenko, Igor E.; Ikhsanov, Renat S.

    2014-01-01

    We analyze and compare surface- and vol ume-based internal photoelectric effects from spherical nanoparticles, obtaining analytical expression s for the photoemission rate in both cases. Similar to results for a flat metal surface, one can show that the surface mechanism preva ils, since it is un...... it is unaffected by detrimental hot electron collisions. Transient ab sorption results from dielectric permittivity discontinuity at the nanoparticle boundary and leads to a substantial (by ~5 times) increase of the photoelectron emission rate....

  6. Photoemission study of 5f localization in UPd3 - x(Pt,Rh)x

    Science.gov (United States)

    Arko, A. J.; Koelling, D. D.; Dunlap, B. D.; Mitchell, A. W.; Capasso, C.; del Giudice, M.

    1988-04-01

    Photoemission measurements in the two systems UPd3-x(Pt,Rh)x show that the 5f spectra are consistent with localized 5f electrons (peak in spectral weight is below EF for all x within the double hexagonal DO24 phase) while at both phase transitions the 5f peaks lock in at EF consistent with intinerancy. A satellite 5f peak which we attribute to d screening is observed in both localized and itinerant systems.

  7. Angular distribution of ions and extreme ultraviolet emission in laser-produced tin droplet plasma

    Science.gov (United States)

    Chen, Hong; Wang, Xinbing; Duan, Lian; Lan, Hui; Chen, Ziqi; Zuo, Duluo; Lu, Peixiang

    2015-05-01

    Angular-resolved ion time-of-flight spectra as well as extreme ultraviolet radiation in laser-produced tin droplet plasma are investigated experimentally and theoretically. Tin droplets with a diameter of 150 μm are irradiated by a pulsed Nd:YAG laser. The ion time-of-flight spectra measured from the plasma formed by laser irradiation of the tin droplets are interpreted in terms of a theoretical elliptical Druyvesteyn distribution to deduce ion density distributions including kinetic temperatures of the plasma. The opacity of the plasma for extreme ultraviolet radiation is calculated based on the deduced ion densities and temperatures, and the angular distribution of extreme ultraviolet radiation is expressed as a function of the opacity using the Beer-Lambert law. Our results show that the calculated angular distribution of extreme ultraviolet radiation is in satisfactory agreement with the experimental data.

  8. Angular cheilitis as the initial sign of Crohn’s disease in children

    Directory of Open Access Journals (Sweden)

    Nuzul Rezki Ramadhani

    2016-06-01

    Full Text Available Crohn’s disease (CD is a chronic inflammatory process of gastrointestinal tract and originally described as a disorder of the smallest intestine caused by an inappropiate mucosal inflammatory response to intestinal bacteria in genetically predisposed host. Oral manifestation are important clinical finding in Crohn’s disease especially in a pediatric patient. This review highlight oral manifestation of gastrointestinal disorder with angular cheilitis as the initial sign of CD in children. Angular cheilitis are considered to be an important extraintestinal manifestation an presenting as the initial sign of Crohn’s disease in children, although uncommon but can be an important clue in the diagnosis of CD before the development of gastrointestinal symptoms. Angular cheilitis may occasionally occur before the onset of gastrointestinal  disease be present during the disease process or persist even even after the disease has resolved.

  9. Watching Electrons Transfer from Metals to Insulators using Two Photon Photoemission

    Energy Technology Data Exchange (ETDEWEB)

    Johns, James E. [Univ. of California, Berkeley, CA (United States)

    2010-05-01

    Ultrafast angle-resolved two photon photoemission was used to study the dynamics and interfacial band structure of ultrathin films adsorbed onto Ag(111). Studies focused on the image potential state (IPS) in each system as a probe for measuring changes in electronic behavior in differing environments. The energetics and dynamics of the IPS at the toluene/Ag(111) interface are strongly dependent upon coverage. For a single monolayer, the first IPS is bound by 0.81 eV below the vacuum level and has a lifetime of 50 femtoseconds (fs). Further adsorption of toluene creates islands of toluene with an exposed wetting layer underneath. The IPS is then split into two peaks, one corresponding to the islands and one corresponding to the monolayer. The wetting layer IPS shows the same dynamics as the monolayer, while the lifetime of the islands increases exponentially with increasing thickness. Furthermore, the island IPS transitions from delocalized to localized within 500 fs, and electrons with larger parallel momenta decay much faster. Attempts were made using a stochastic model to extract the rates of localization and intraband cooling at differing momenta. In sexithiophene (6T) and dihexyl-sexithiophene (DH6T), the IPS was used as a probe to see if the nuclear motion of spectating side chains can interfere with molecular conduction. The energy and band mass of the IPS was measured for 6T and two geometries of DH6T on Ag(111). Electrons injected into the thicker coverages of DH6T grew exponentially heavier until they were completely localized by 230 fs, while those injected into 6T remained nearly free electron like. Based off of lifetime arguments and the density of defects, the most likely cause for the mass enhancement of the IPS in this system is small polaron formation caused by coupling of the electron to vibrations of the alkyl substituents. The energetic relaxation of the molecular adsorbate was also measured to be 20 meV/100 fs for the DH6T, and 0 meV/100 fs for

  10. Auger and x-ray photoemission spectroscopy study on Cs2Te photocathodes

    Science.gov (United States)

    di Bona, A.; Sabary, F.; Valeri, S.; Michelato, P.; Sertore, D.; Suberlucq, G.

    1996-09-01

    Thin films of Cs2Te have been produced and analyzed by Auger depth profiling and x-ray photoemission spectroscopy (XPS). The formation of the photoemissive material passes through different phases, each of them has been characterized by XPS and by its total yield in the spectral region 3.5-5 eV. Copper and molybdenum substrates have been considered. While Mo behaves to all practical purposes like an ideal support for Cs2Te, strong diffusion from the substrate material into the photoemissive film has been observed on photocathodes fabricated on Cu. The ruggedness of the photocathodes has been tested by exposing them to a few hundred Langmuirs of different gases, namely O2, CO2, CO, N2, and CH4. The last three have no effect on the photocathode lifetime, while a substantial reduction of the quantum efficiency has been observed after the exposure to oxygen. The main reason for this is the formation of a thick cesium oxide layer at the surface of the photocathode. However, the oxygen pollution can be partially recovered by the combined effect of heating the photocathode at 230 °C and illuminating the poisoned material with the 4.9 eV radiation. No rejuvenation has been observed under the effect of the temperature or the radiation alone.

  11. Integrated spectral study of small angular diameter galactic open clusters

    Science.gov (United States)

    Clariá, J. J.; Ahumada, A. V.; Bica, E.; Pavani, D. B.; Parisi, M. C.

    2017-10-01

    This paper presents flux-calibrated integrated spectra obtained at Complejo Astronómico El Leoncito (CASLEO, Argentina) for a sample of 9 Galactic open clusters of small angular diameter. The spectra cover the optical range (3800-6800 Å), with a resolution of ˜14 Å. With one exception (Ruprecht 158), the selected clusters are projected into the fourth Galactic quadrant (282o evaluate their membership status. The current cluster sample complements that of 46 open clusters previously studied by our group in an effort to gather a spectral library with several clusters per age bin. The cluster spectral library that we have been building is an important tool to tie studies of resolved and unresolved stellar content.

  12. Optical communication beyond orbital angular momentum

    CSIR Research Space (South Africa)

    Trichili, A

    2016-06-01

    Full Text Available Mode division multiplexing (MDM) is mooted as a technology to address future bandwidth issues, and has been successfully demonstrated in free space using spatial modes with orbital angular momentum (OAM). To further increase the data transmission...

  13. Dynamical Model of Fission Fragment Angular Distribution

    Science.gov (United States)

    Drozdov, V. A.; Eremenko, D. O.; Fotina, O. V.; Platonov, S. Yu.; Yuminov, O. A.; Giardina, G.; Taccone, A.

    2002-01-01

    A dynamical model of fission fragment angular distributions is suggested. The model allows one to calculate fission fragment angular distributions, prescission light particle multyplicities, evaporation residue cross sections etc. for the cases of decay of hot and rotating heavy nuclei. The experimental data on angular anisotropies of fission fragments and prescission neutron multiplicities are analyzed for the 16O + 208Pb, 232Th, 248Cm and 238U reactions at the energies of the incident 16O ions ranging from 90 to 160 MeV. This analysis allows us to extract both the nuclear friction coefficient value and the relaxation time for the tilting mode. It is also demonstrated that the angular distributions are sensitive to the deformation dependence of the nuclear friction.

  14. Amplitude damping channel for orbital angular momentum

    CSIR Research Space (South Africa)

    Dudley, Angela L

    2010-03-01

    Full Text Available Since the pioneering work on the entanglement of the orbital angular momentum (OAM) states of light, much attention has been devoted to the subject, with particular attention into the quantum aspects of information processing using OAM. Furthermore...

  15. Revolution evolution: tracing angular momentum during star and planetary system formation

    Science.gov (United States)

    Davies, Claire Louise

    2015-04-01

    disc to expand. I used spatially resolved submillimetre detections of the dust and gas components of protoplanetary discs, gathered from the literature, to measure the radial extent of discs around low-mass pre-main sequence stars of ∼ 1-10 Myr and probe their viscous evolution. I find no clear observational evidence for the radial expansion of the dust component. However, I find tentative evidence for the expansion ofthe gas component. This suggests that the evolution of the gas and dust components of protoplanetary discs are likely governed by different astrophysical processes. Observations of jets and outflows emanating from protostars and pre-main sequence stars highlight that it may also be possible to remove angular momentum from the circumstellar material. Using the sample of spatially resolved protoplanetary discs, I find no evidence for angular momentum removal during disc evolution. I also use the spatially resolved debris discs from the Submillimetre Common-User Bolometer Array-2 Observations of Nearby Stars survey to constrain the amount of angular momentum retained within planetary systems. This sample is compared to the protoplanetary disc angular momenta and to the angular momentum contained within pre-stellar cores. I find that significant quantities of angular momentum must be removed during disc formation and disc dispersal. This likely occurs via magnetic braking during the formation of the disc, via the launching of a disc or photo-evaporative wind, and/or via ejection of planetary material following dynamical interactions.

  16. Mastering AngularJD for .NET developers

    CERN Document Server

    Majid, Mohammad Wadood

    2015-01-01

    This book is envisioned for traditional developers and programmers who want to develop client-side applications using the AngularJS framework and ASP.NET Web API 2 with Visual Studio. .NET developers who have already built web applications or web services and who have a fundamental knowledge of HTML, JavaScript, and CSS and want to explore single-page applications will also find this guide useful. Basic knowledge of AngularJS would be helpful.

  17. Partial angular coherence and the angular Schmidt spectrum of entangled two-photon fields

    Energy Technology Data Exchange (ETDEWEB)

    Jha, Anand Kumar; Boyd, Robert W. [Institute of Optics, University of Rochester, Rochester, New York 14627 (United States); Agarwal, Girish S. [Department of Physics, Oklahoma State University, Stillwater, Oklahoma 74078 (United States)

    2011-12-15

    We study partially coherent fields that have a coherent-mode representation in the orbital-angular-momentum-mode basis. For such fields, we introduce the concepts of the angular coherence function and the coherence angle. Such fields are naturally produced by the process of parametric down-conversion--a second-order nonlinear optical process in which a pump photon breaks up into two entangled photons, known as the signal and idler photons. We show that the angular coherence functions of the signal and idler fields are directly related to the angular Schmidt (spiral) spectrum of the down-converted two-photon field and thus that the angular Schmidt spectrum can be measured directly by measuring the angular coherence function of either the signal or the idler field, without requiring coincidence detection.

  18. Communication: angular momentum alignment and fluorescence polarization of alkali atoms photodetached from helium nanodroplets.

    Science.gov (United States)

    Hernando, Alberto; Beswick, J Alberto; Halberstadt, Nadine

    2013-12-14

    The theory of photofragments angular momentum polarization is applied to the photodetachment of an electronically excited alkali atom from a helium nanocluster (N = 200). The alignment of the electronic angular momentum of the bare excited alkali atoms produced is calculated quantum mechanically by solving the excited states coupled equations with potentials determined by density functional theory (DFT). Pronounced oscillations as a function of excitation energy are predicted for the case of Na@(He)200, in marked contrast with the absorption cross-section and angular distribution of the ejected atoms which are smooth functions of the energy. These oscillations are due to quantum interference between different coherently excited photodetachment pathways. Experimentally, these oscillations should be reflected in the fluorescence polarization and polarization-resolved photoelectron yield of the ejected atoms, which are proportional to the electronic angular momentum alignment. In addition, this result is much more general than the test case of NaHe200 studied here. It should be observable for larger droplets, for higher excited electronic states, and for other alkali as well as for alkali-earth atoms. Detection of these oscillations would show that the widely used pseudo-diatomic model can be valid beyond the prediction of absorption spectra and could help in interpreting parts of the dynamics, as already hinted by some experimental results on angular anisotropy of bare alkali fragments.

  19. Time-resolved ARPES at LACUS: Band Structure and Ultrafast Electron Dynamics of Solids.

    Science.gov (United States)

    Crepaldi, Alberto; Roth, Silvan; Gatti, Gianmarco; Arrell, Christopher A; Ojeda, José; van Mourik, Frank; Bugnon, Philippe; Magrez, Arnaud; Berger, Helmuth; Chergui, Majed; Grioni, Marco

    2017-05-31

    The manipulation of the electronic properties of solids by light is an exciting goal, which requires knowledge of the electronic structure with energy, momentum and temporal resolution. Time- and angle-resolved photoemission spectroscopy (tr-ARPES) is the most direct probe of the effects of an optical excitation on the band structure of a material. In particular, tr-ARPES in the extreme ultraviolet (VUV) range gives access to the ultrafast dynamics over the entire Brillouin zone. VUV tr-ARPES experiments can now be performed at the ASTRA (ARPES Spectrometer for Time-Resolved Applications) end station of Harmonium, at LACUS. Its capabilities are illustrated by measurements of the ultrafast electronic response of ZrSiTe, a novel topological semimetal characterized by linearly dispersing states located at the Brillouin zone boundary.

  20. Angular-resolved elastic peak electron spectroscopy: experiment and Monte Carlo calculations

    Czech Academy of Sciences Publication Activity Database

    Zemek, Josef; Jiříček, Petr; Werner, W. S. M.; Lesiak, B.; Jablonski, A.

    2006-01-01

    Roč. 38, - (2006), s. 615-619 ISSN 0142-2421 Grant - others:FWF(AT) P15938-N02; EU-SURPHARE(XE) GMA1-2002-72057 Institutional research plan: CEZ:AV0Z10100521 Keywords : elastic peak electron spectroscopy * EPES * inelestic mean free path * IMFP * surface excitations Subject RIV: BM - Solid Matter Physics ; Magnetism Impact factor: 1.427, year: 2006

  1. Highly efficient angularly resolving x-ray spectrometer optimized for absorption measurements with collimated sources

    Czech Academy of Sciences Publication Activity Database

    Šmíd, Michal; Gonzalez, I.G.; Ekerfelt, H.; Svensson, J.B.; Hansson, M.; Wood, I. C.; Persson, A.; Mangles, S.P.D.; Lundh, O.; Falk, Kateřina

    2017-01-01

    Roč. 88, č. 6 (2017), s. 1-8, č. článku 063102. ISSN 0034-6748 R&D Projects: GA MŠk EF15_008/0000162; GA MŠk LQ1606 EU Projects: European Commission(XE) 654148 - LASERLAB-EUROPE Grant - others:ELI Beamlines(XE) CZ.02.1.01/0.0/0.0/15_008/0000162 Institutional support: RVO:68378271 Keywords : acceleration * measurments * x ray * high energy Subject RIV: BL - Plasma and Gas Discharge Physics OBOR OECD: Fluids and plasma physics (including surface physics) Impact factor: 1.515, year: 2016

  2. Transverse angular momentum in topological photonic crystals

    Science.gov (United States)

    Deng, Wei-Min; Chen, Xiao-Dong; Zhao, Fu-Li; Dong, Jian-Wen

    2018-01-01

    Engineering local angular momentum of structured light fields in real space enables applications in many fields, in particular, the realization of unidirectional robust transport in topological photonic crystals with a non-trivial Berry vortex in momentum space. Here, we show transverse angular momentum modes in silicon topological photonic crystals when considering transverse electric polarization. Excited by a chiral external source with either transverse spin angular momentum or transverse phase vortex, robust light flow propagating along opposite directions is observed in several kinds of sharp-turn interfaces between two topologically-distinct silicon photonic crystals. A transverse orbital angular momentum mode with alternating phase vortex exists at the boundary of two such photonic crystals. In addition, unidirectional transport is robust to the working frequency even when the ring size or location of the pseudo-spin source varies in a certain range, leading to the superiority of the broadband photonic device. These findings enable one to make use of transverse angular momentum, a kind of degree of freedom, to achieve unidirectional robust transport in the telecom region and other potential applications in integrated photonic circuits, such as on-chip robust delay lines.

  3. Angular distribution of oriented nucleus fission neutrons

    International Nuclear Information System (INIS)

    Barabanov, A.L.; Grechukhin, D.P.

    1982-01-01

    Calculations of anisotropy of angular distribution of oriented 235 U nuclei thermal fission neutrons have been carried out. the neutrons were assumed to evaporate isotropically by completely accelerated fragements in the fragment system with only its small part, i. e. fission-producing neutrons, emitted at the moment of neck break. It has been found out that at low energies of neutrons Esub(n)=1-2 MeV the sensitivity of the angular distribution anisotropy to variations of spectrum of neutron evaporation from fragments and the magnitude of a share of fission-producing neutrons reaches approximately 100%, which at high energies, Esub(n) > 5 MeV it does not exceed approximately 20%. Therefore the angular distribution of fast neutrons to a greater degree of confidence may be used for restoring the angular distribution anisotropy of fragments while the angular distribution of low energy neutrons may be used for deriving information on the fission process, but only in case 6f the experiment accuracy is better than approximately 3%

  4. Angular Spectral Analysis and Lowpass Filtering of Aeromagnetic ...

    African Journals Online (AJOL)

    Total-field aeromagnetic data over the western half of the Bornu basin and its surrounding areas were analyzed using angular spectral analysis, upward continuation and lowpass filtering techniques. Results revealed several angular spectral peaks at various angular orientations. The angular orientations correlated with the ...

  5. Data-oriented development with AngularJS

    CERN Document Server

    Waikar, Manoj

    2015-01-01

    This book helps beginner-level AngularJS developers organize AngularJS applications by discussing important AngularJS concepts and best practices. If you are an experienced AngularJS developer but haven't written directives or haven't created custom HTML controls before, then this book is ideal for you.

  6. Angular correlations and high energy evolution

    International Nuclear Information System (INIS)

    Kovner, Alex; Lublinsky, Michael

    2011-01-01

    We address the question of to what extent JIMWLK evolution is capable of taking into account angular correlations in a high energy hadronic wave function. Our conclusion is that angular (and indeed other) correlations in the wave function cannot be reliably calculated without taking into account Pomeron loops in the evolution. As an example we study numerically the energy evolution of angular correlations between dipole scattering amplitudes in the framework of the large N c approximation to JIMWLK evolution (the 'projectile dipole model'). Target correlations are introduced via averaging over an (isotropic) ensemble of anisotropic initial conditions. We find that correlations disappear very quickly with rapidity even inside the saturation radius. This is in accordance with our physical picture of JIMWLK evolution. The actual correlations inside the saturation radius in the target QCD wave function, on the other hand, should remain sizable at any rapidity.

  7. Electron attachment rate constant measurement by photoemission electron attachment ion mobility spectrometry (PE-EA-IMS)

    Science.gov (United States)

    Su, Desheng; Niu, Wenqi; Liu, Sheng; Shen, Chengyin; Huang, Chaoqun; Wang, Hongmei; Jiang, Haihe; Chu, Yannan

    2012-12-01

    Photoemission electron attachment ion mobility spectrometry (PE-EA-IMS), with a source of photoelectrons induced by vacuum ultraviolet radiation on a metal surface, has been developed to study electron attachment reaction at atmospheric pressure using nitrogen as the buffer gas. Based on the negative ion mobility spectra, the rate constants for electron attachment to tetrachloromethane and chloroform were measured at ambient temperature as a function of the average electron energy in the range from 0.29 to 0.96 eV. The experimental results are in good agreement with the data reported in the literature.

  8. Physical origin of satellites in photoemission of doped graphene: an ab initio GW plus cumulant study.

    Science.gov (United States)

    Lischner, Johannes; Vigil-Fowler, Derek; Louie, Steven G

    2013-04-05

    We calculate the photoemission spectra of suspended and epitaxial doped graphene using an ab initio cumulant expansion of the Green's function based on the GW self-energy. Our results are compared to experiment and to standard GW calculations. For doped graphene on a silicon carbide substrate, we find, in contrast to earlier calculations, that the spectral function from GW only does not reproduce experimental satellite properties. However, ab initio GW plus cumulant theory combined with an accurate description of the substrate screening results in good agreement with experiment, but gives no plasmaron (i.e., no extra well-defined excitation satisfying Dyson's equation).

  9. Vacancy formation in MoO3: hybrid density functional theory and photoemission experiments

    KAUST Repository

    Salawu, Omotayo Akande

    2016-09-29

    Molybdenum oxide (MoO3) is an important material that is being considered for numerous technological applications, including catalysis and electrochromism. In the present study, we apply hybrid density functional theory to investigate O and Mo vacancies in the orthorhombic phase. We determine the vacancy formation energies of different defect sites as functions of the electron chemical potential, addressing different charge states. In addition, we investigate the consequences of defects for the material properties. Ultraviolet photoemission spectroscopy is employed to study the valence band of stoichiometric and O defective MoO3. We show that O vacancies result in occupied in-gap states.

  10. Laser-excited photoemission spectroscopy study of superconducting boron-doped diamond

    Directory of Open Access Journals (Sweden)

    K. Ishizaka, R. Eguchi, S. Tsuda, T. Kiss, T. Shimojima, T. Yokoya, S. Shin, T. Togashi, S. Watanabe, C.-T. Chen, C.Q. Zhang, Y. Takano, M. Nagao, I. Sakaguchi, T. Takenouchi and H. Kawarada

    2006-01-01

    Full Text Available We have investigated the low-energy electronic state of boron-doped diamond thin film by the laser-excited photoemission spectroscopy. A clear Fermi-edge is observed for samples doped above the semiconductor–metal boundary, together with the characteristic structures at 150×n meV possibly due to the strong electron–lattice coupling effect. In addition, for the superconducting sample, we observed a shift of the leading edge below Tc indicative of a superconducting gap opening. We discuss the electron–lattice coupling and the superconductivity in doped diamond.

  11. Internal photoemission from plasmonic nanoparticles: comparison between surface and volume photoelectric effects

    DEFF Research Database (Denmark)

    Uskov, Alexander; Protsenko, Igor E.; Ikhsanov, Renat S.

    2014-01-01

    emission rate from a nanoparticle. Calculations have been carried out for a step potential at the surface of a spherical nanoparticle, and a simple model for the hot electron cooling has been used. We highlight the effect of the discontinuity of the dielectric permittivity at the nanoparticle boundary...... through the effect of the discontinuity of the dielectric permittivity at the nanoparticle boundary. The latter is stronger at relatively lower photon energies and correspondingly is more substantial for internal photoemission than for an external one. We show that in the general case, it is essential...

  12. Athermal electron distribution probed by femtosecond multiphoton photoemission from image potential states

    International Nuclear Information System (INIS)

    Ferrini, Gabriele; Giannetti, Claudio; Pagliara, Stefania; Banfi, Francesco; Galimberti, Gianluca; Parmigiani, Fulvio

    2005-01-01

    Image potential states are populated through indirect, scattering-mediated multiphoton absorption induced by femtosecond laser pulses and revealed by single-photon photoemission. The measured effective mass is significantly different from that obtained with direct, resonant population. These features reveal a strong coupling of the electrons residing in the image potential state, outside the solid, with the underlying hot electron population created by the laser pulse. The coupling is mediated by a many-body scattering interaction between the image potential state electrons and bulk electrons in highly excited states

  13. CONTUR: A program for X-ray photoemission spectroscopic personal computer-based data analysis

    Science.gov (United States)

    Contini, G.; Turchini, S.

    1996-03-01

    CONTUR, a computer program for photoemission data analysis written in QuickBasic that operates using an IBM personal computer (PC) or compatible, is described. It includes the following functions: plotting of up to four files, files saving, spectra comparison (including addition, subtraction and division) smoothing and median filtering, data marking, differentiating, resizing of X and Y scales, transforming binding into kinetic energy and vice versa, X axis cutting, showing X and Y values of the files, spikes removing, linear and Shirley background subtraction, calculating the area of the peaks, determination of maxima of the file, DOS shell. A brief description of the program and its capabilities is given.

  14. Observation of injection and pinning of domain walls in magneticnanowires using photoemission electron microscopy

    Energy Technology Data Exchange (ETDEWEB)

    Thomas, Luc; Rettner, Charles; Hayashi, Masamitsu; Samant, MaheshG.; Parkin Stuart S.P.; Doran, Andrew; Scholl, Andreas

    2005-12-19

    Photoemission electron microscopy is used to explore the injection and pinning of magnetic domain walls in 250-nm-wide, 20-nm-thick Permalloy nanowires. Domain walls are injected from a micron-sized elliptical nucleation pad at one end of the nanowire. A vortex-like structure is readily nucleated in this pad at low magnetic fields 15 Oe, whereas injection of a domain wall into the nanowire requires significantly larger fields 60 Oe. Domain walls are pinned in the nanowire at notches patterned along the wires edges. The domain walls are observed to have vortex-like structures with chiralities that vary in successive experiments.

  15. Observation of injection and pinning of domain walls in magnetic nanowires using photoemission electron microscopy

    Science.gov (United States)

    Thomas, Luc; Rettner, Charles; Hayashi, Masamitsu; Samant, Mahesh G.; Parkin, Stuart S. P.; Doran, Andrew; Scholl, Andreas

    2005-12-01

    Photoemission electron microscopy is used to explore the injection and pinning of magnetic domain walls in 250-nm-wide, 20-nm-thick Permalloy nanowires. Domain walls are injected from a micron-sized elliptical nucleation pad at one end of the nanowire. A vortex-like structure is readily nucleated in this pad at low magnetic fields (<15Oe), whereas injection of a domain wall into the nanowire requires significantly larger fields (˜60Oe). Domain walls are pinned in the nanowire at notches patterned along the wire's edges. The domain walls are observed to have vortex-like structures with chiralities that vary in successive experiments.

  16. High resolution hard X-ray photoemission using synchrotron radiation as an essential tool for characterization of thin solid films

    International Nuclear Information System (INIS)

    Kim, J.J.; Ikenaga, E.; Kobata, M.; Takeuchi, A.; Awaji, M.; Makino, H.; Chen, P.P.; Yamamoto, A.; Matsuoka, T.; Miwa, D.; Nishino, Y.; Yamamoto, T.; Yao, T.; Kobayashi, K.

    2006-01-01

    Recently, we have shown that hard X-ray photoemission spectroscopy using undulator X-rays at SPring-8 is quite feasible with both high resolution and high throughput. Here we report an application of hard X-ray photoemission spectroscopy to the characterization of electronic and chemical states of thin solid films, for which conventional PES is not applicable. As a typical example, we focus on the problem of the scatter in the reported band-gap values for InN. We show that oxygen incorporation into the InN film strongly modifies the valence and plays a crucial role in the band gap problem. The present results demonstrate the powerful applicability of high resolution photoemission spectroscopy with hard X-rays from a synchrotron source

  17. Probing long-range structural order in SnPc/Ag(111) by umklapp process assisted low-energy angle-resolved photoelectron spectroscopy

    Science.gov (United States)

    Jauernik, Stephan; Hein, Petra; Gurgel, Max; Falke, Julian; Bauer, Michael

    2018-03-01

    Laser-based angle-resolved photoelectron spectroscopy is performed on tin-phthalocyanine (SnPc) adsorbed on silver Ag(111). Upon adsorption of SnPc, strongly dispersing bands are observed which are identified as secondary Mahan cones formed by surface umklapp processes acting on photoelectrons from the silver substrate as they transit through the ordered adsorbate layer. We show that the photoemission data carry quantitative structural information on the adsorbate layer similar to what can be obtained from a conventional low-energy electron diffraction (LEED) study. More specifically, we compare photoemission data and LEED data probing an incommensurate-to-commensurate structural phase transition of the adsorbate layer. Based on our results we propose that Mahan-cone spectroscopy operated in a pump-probe configuration can be used in the future to probe structural dynamics at surfaces with a temporal resolution in the sub-100-fs regime.

  18. Angular and linear momentum of excited ferromagnets

    NARCIS (Netherlands)

    Yan, P.; Kamra, A.; Cao, Y.; Bauer, G.E.W.

    2013-01-01

    The angular momentum vector of a Heisenberg ferromagnet with isotropic exchange interaction is conserved, while under uniaxial crystalline anisotropy the projection of the total spin along the easy axis is a constant of motion. Using Noether's theorem, we prove that these conservation laws persist

  19. Angular distribution in ternary cold fission

    International Nuclear Information System (INIS)

    Delion, D.S.; J.W. Goethe Univ., Frankfurt; Sandulescu, A.; J.W. Goethe Univ., Frankfurt; Greiner, W.

    2003-01-01

    We describe the spontaneous ternary cold fission of 252 Cf, accompanied by 4 He, 10 Be and 14 C. The light cluster decays from the first resonant eigenstate in the Coulomb potential plus a harmonic oscillator potential. We have shown that the angular distribution of the emitted light particle is strongly connected with its deformation and the equatorial distance. (author)

  20. Probabilistic calculation for angular dependence collision

    International Nuclear Information System (INIS)

    Villarino, E.A.

    1990-01-01

    This collision probabilistic method is broadly used in cylindrical geometry (in one- or two-dimensions). It constitutes a powerful tool for the heterogeneous Response Method where, the coupling current is of the cosine type, that is, without angular dependence at azimuthal angle θ and proportional to μ (cosine of the θ polar angle). (Author) [es

  1. Heteromodal conceptual processing in the angular gyrus.

    Science.gov (United States)

    Bonner, Michael F; Peelle, Jonathan E; Cook, Philip A; Grossman, Murray

    2013-05-01

    Concepts bind together the features commonly associated with objects and events to form networks in long-term semantic memory. These conceptual networks are the basis of human knowledge and underlie perception, imagination, and the ability to communicate about experiences and the contents of the environment. Although it is often assumed that this distributed semantic information is integrated in higher-level heteromodal association cortices, open questions remain about the role and anatomic basis of heteromodal representations in semantic memory. Here we used combined neuroimaging evidence from functional magnetic resonance imaging (fMRI) and diffusion tensor imaging (DTI) to characterize the cortical networks underlying concept representation. Using a lexical decision task, we examined the processing of concepts in four semantic categories that varied on their sensory-motor feature associations (sight, sound, manipulation, and abstract). We found that the angular gyrus was activated across all categories regardless of their modality-specific feature associations, consistent with a heteromodal account for the angular gyrus. Exploratory analyses suggested that categories with weighted sensory-motor features additionally recruited modality-specific association cortices. Furthermore, DTI tractography identified white matter tracts connecting these regions of modality-specific functional activation with the angular gyrus. These findings are consistent with a distributed semantic network that includes a heteromodal, integrative component in the angular gyrus in combination with sensory-motor feature representations in modality-specific association cortices. Copyright © 2013 Elsevier Inc. All rights reserved.

  2. INVESTIGATION OF ANGULAR BALL BEARING WEAR

    Directory of Open Access Journals (Sweden)

    A. L. Savchenko

    2006-01-01

    Full Text Available Wearing process of balls in an angular ball bearing has been investigated in the paper. Force affecting a separator from the side of balls is determined theoretically. Wear rate may be calculated with a formula for abrasive wear while substituting numerical parameter values of the investigated ball bearing for formula symbols.

  3. Canonical three-body angular basis

    International Nuclear Information System (INIS)

    Matveenko, A.V.

    2001-01-01

    Three-body problems are basic for the quantum mechanics of molecular, atomic, or nuclear systems. We demonstrate that their variational solution for rotational states can be greatly simplified. A special choice of coordinates (hyperspherical) and of the kinematics (body-fixed coordinate frame) allows one to choose basis functions in a form that makes the angular coupling trivial. (author)

  4. Temperature and angular momentum dependence of the ...

    Indian Academy of Sciences (India)

    Temperature and angular momentum dependence of the quadrupole deformation is studied in the middle of the sd-shell for 28Si and 27Si isotopes using the spherical shell model approach. The shell model calculations have been performed using the standard universal sd-shell (USD) interaction and the canonical ...

  5. Angular momentum gated neutron evaporation studies

    International Nuclear Information System (INIS)

    Banerjee, K.; Kundu, S.; Rana, T.K.; Bhattacharya, C.; Mukherjee, G.; Gohil, M.; Meena, J.K.; Pandey, R.; Pai, H.; Dey, A.; Biswas, M.; Mukhopadhyay, S.; Pandit, D.; Pal, S.; Banerjee, S.R.; Bhattacharya, S.; Bandhopadhyay, T.

    2010-01-01

    The inverse level density parameter k (k = A/a, where A is the mass number of the compound nucleus)is investigated as a function of angular momentum by measuring γ-ray fold gated neutron evaporation spectrum in 4 He + 115 In fusion reaction using 35 MeV 4 He ion beam from VECC K130 cyclotron

  6. Angular-momentum-bearing modes in fission

    International Nuclear Information System (INIS)

    Moretto, L.G.; Peaslee, G.F.; Wozniak, G.J.

    1989-03-01

    The angular-momentum-bearing degrees of freedom involved in the fission process are identified and their influence on experimental observables is discussed. The excitation of these modes is treated in the ''thermal'' limit, and the resulting distributions of observables are calculated. Experiments demonstrating the role of these modes are presented and discussed. 61 refs., 12 figs

  7. Angular Intermittency and Analytical QCD Predictions

    CERN Document Server

    Chekanov, S.V.

    1997-01-01

    We present a comparison of local multiplicity fluctuations in angular phase-space intervals with first-order QCD predictions. The data are based on 810k hadronic events at 91.2 GeV collected with the L3 detector at LEP during 1994.

  8. Angular momentum transfer in incomplete fusion

    Indian Academy of Sciences (India)

    Keywords. Heavy-ion reactions; incomplete fusion; isomeric cross-section ratio; 12C, 16O beams; 93Nb; 89Y targets; angular momentum. ... R Tripathi1 A Goswami1. Radiochemistry Division, Bhabha Atomic Research Centre, Mumbai 400 085, India; School of Studies in Physics, Vikram University, Ujjain 456 010, India ...

  9. Temperature and angular momentum dependence of the ...

    Indian Academy of Sciences (India)

    Abstract. Temperature and angular momentum dependence of the quadrupole deformation is studied in the middle of the sd-shell for 28Si and 27Si isotopes using the spherical shell model ... Department of Physics, University of Kashmir, Srinagar 190 006, India; Inter-University Accelerator Centre, New Delhi 110 067, India ...

  10. On the angular momentum in star formation

    International Nuclear Information System (INIS)

    Horedt, G.P.

    1978-01-01

    The author discusses the rotation of interstellar clouds which are in a stage immediately before star formation. Cloud collisions seem to be the principal cause of the observed rotation of interstellar clouds. The rotational motion of the clouds is strongly influenced by turbulence. Theories dealing with the resolution of the angular momentum problem in star formation are classified into five major groups. The old idea that the angular momentum of an interstellar cloud passes during star formation into the angular momentum of double star systems and/or circumstellar clouds, is developed. It is suggested that a rotating gas cloud contracts into a ring-like structure which fragments into self-gravitating subcondensations. By collisions and gas accretion these subcondensations accrete into binary systems surrounded by circumstellar clouds. Using some rough approximations the authors find analytical expressions for the semi-major axis of the binary system and for the density of the circumstellar clouds as a function of the initial density and of the initial angular velocity of an interstellar cloud. The obtained values are well within the observational limits. (Auth.)

  11. A Novel Permanent Magnetic Angular Acceleration Sensor

    Directory of Open Access Journals (Sweden)

    Hao Zhao

    2015-07-01

    Full Text Available Angular acceleration is an important parameter for status monitoring and fault diagnosis of rotary machinery. Therefore, we developed a novel permanent magnetic angular acceleration sensor, which is without rotation angle limitations and could directly measure the instantaneous angular acceleration of the rotating system. The sensor rotor only needs to be coaxially connected with the rotating system, which enables convenient sensor installation. For the cup structure of the sensor rotor, it has a relatively small rotational inertia. Due to the unique mechanical structure of the sensor, the output signal of the sensor can be directed without a slip ring, which avoids signal weakening effect. In this paper, the operating principle of the sensor is described, and simulated using finite element method. The sensitivity of the sensor is calibrated by torsional pendulum and angle sensor, yielding an experimental result of about 0.88 mV/(rad·s−2. Finally, the angular acceleration of the actual rotating system has been tested, using both a single-phase asynchronous motor and a step motor. Experimental result confirms the operating principle of the sensor and indicates that the sensor has good practicability.

  12. Variation in angular velocity and angular acceleration of a particle in rectilinear motion

    International Nuclear Information System (INIS)

    Mashood, K K; Singh, V A

    2012-01-01

    We discuss the angular velocity and angular acceleration associated with a particle in rectilinear motion with constant acceleration. The discussion was motivated by an observation that students and even teachers have difficulty in ascribing rotational motion concepts to a particle when the trajectory is a straight line. We present some details of our observations. A formal derivation of ω and α is presented which reveals ‘surprising’ and non-intuitive aspects, namely non-monotonic behaviour with an associated extremum. The special case of constant velocity is studied and we find that angular acceleration associated with it also has an extremum. We discuss a plausible source of difficulty. (paper)

  13. ZnO nanocrystals on SiO2/Si surfaces thermally cleaned in ultrahigh vacuum and characterized using spectroscopic photoemission and low energy electron microscopy

    International Nuclear Information System (INIS)

    Ericsson, Leif K. E.; Magnusson, Kjell O.; Zakharov, Alexei A.

    2010-01-01

    Thermal cleaning in ultrahigh vacuum of ZnO nanocrystals distributed on SiO 2 /Si surfaces has been studied using spectroscopic photoemission and low energy electron microscopy (SPELEEM). This study thus concern weakly bound ZnO nanocrystals covering only 5%-10% of the substrate. Chemical properties, crystallinity, and distribution of nanocrystals are used to correlate images acquired with the different techniques showing excellent correspondence. The nanocrystals are shown to be clean enough after thermal cleaning at 650 deg. C to be imaged by LEEM and x-ray PEEM as well as chemically analyzed by site selective x-ray photoelectron spectroscopy (μ-XPS). μ-XPS shows a sharp Zn 3d peak and resolve differences in O 1s states in oxides. The strong LEEM reflections together with the obtained chemical information indicates that the ZnO nanocrystals were thermally cleaned, but do not indicate any decomposition of the nanocrystals. μ-XPS was also used to determine the thickness of SiO 2 on Si. This article is the first to our knowledge where the versatile technique SPELEEM has been used to characterize ZnO nanocrystals.

  14. Study of photoemission mechanism for varied doping GaN photocathode

    Science.gov (United States)

    Qiao, Jianliang; Xu, Yuan; Niu, Jun; Gao, Youtang; Chang, Benkang

    2015-10-01

    Negative electron affinity (NEA) GaN photocathode has many virtues, such as high quantum efficiency, low dark current, concentrated electrons energy distribution and angle distribution, adjustive threshold and so on. The quantum efficiency is an important parameter for the preparation and evaluation of NEA GaN photocathode. The varied doping GaN photocathode has the directional inside electric field within the material, so the higher quantum efficiency can be obtained. The varied doping NEA GaN photocathode has better photoemission performance. According to the photoemission theory of NEA GaN photocathode, the quantum efficiency formulas for uniform doping and varied doping NEA GaN photocathodes were given. In the certain condition, the quantum efficiency formula for varied doping GaN photocathode consists with the uniform doping. The activation experiment was finished for varied doping GaN photocathode. The cleaning method and technics for varied doping GaN photocathode were given in detail. To get an atom clean surface, the heat cleaning must be done after the chemical cleaning. Using the activation and evaluation system for NEA photocathode, the varied doping GaN photocathode was activated with Cs and O, and the photocurrent curve for varied doping GaN photocathode was gotten.

  15. Study on photoemission surface of varied doping GaN photocathode

    Science.gov (United States)

    Qiao, Jianliang; Du, Ruijuan; Ding, Huan; Gao, Youtang; Chang, Benkang

    2014-09-01

    For varied doping GaN photocathode, from bulk to surface the doping concentrations are distributed from high to low. The varied doping GaN photocathode may produce directional inside electric field within the material, so the higher quantum efficiency can be obtained. The photoemission surface of varied doping GaN photocathode is very important to the high quantum efficiency, but the forming process of the surface state after Cs activation or Cs/O activation has been not known completely. Encircling the photoemission mechanism of varied GaN photocathode, considering the experiment phenomena during the activation and the successful activation results, the varied GaN photocathode surface model [GaN(Mg):Cs]:O-Cs after activation with cesium and oxygen was given. According to GaN photocathode activation process and the change of electronic affinity, the comparatively ideal NEA property can be achieved by Cs or Cs/O activation, and higher quantum efficiency can be obtained. The results show: The effective NEA characteristic of GaN can be gotten only by Cs. [GaN(Mg):Cs] dipoles form the first dipole layer, the positive end is toward the vacuum side. In the activation processing with Cs/O, the second dipole layer is formed by O-Cs dipoles, A O-Cs dipole includes one oxygen atom and two Cs atoms, and the positive end is also toward the vacuum side thus the escape of electrons can be promoted.

  16. Highly resolving computerized tomography

    International Nuclear Information System (INIS)

    Kurtz, B.; Petersen, D.; Walter, E.

    1984-01-01

    With the development of highly-resolving devices for computerized tomography, CT diagnosis of the lumbar vertebral column has gained increasing importance. As an ambulatory, non-invasive method it has proved in comparative studies to be at least equivalent to myelography in the detection of dislocations of inter-vertebral disks (4,6,7,15). Because with modern devices not alone the bones, but especially the spinal soft part structures are clearly and precisely presented with a resolution of distinctly below 1 mm, a further improvement of the results is expected as experience will increase. The authors report on the diagnosis of the lumbar vertebral column with the aid of a modern device for computerized tomography and wish to draw particular attention to the possibility of doing this investigation as a routine, and to the diagnostic value of secondary reconstructions. (BWU) [de

  17. Vibrational excitation and vibrationally resolved electronic excitation cross sections of positron-H2 scattering

    Science.gov (United States)

    Zammit, Mark; Fursa, Dmitry; Savage, Jeremy; Bray, Igor

    2016-09-01

    Vibrational excitation and vibrationally resolved electronic excitation cross sections of positron-H2 scattering have been calculated using the single-centre molecular convergent close-coupling (CCC) method. The adiabatic-nuclei approximation was utilized to model the above scattering processes and obtain the vibrationally resolved positron-H2 scattering length. As previously demonstrated, the CCC results are converged and accurately account for virtual and physical positronium formation by coupling basis functions with large orbital angular momentum. Here vibrationally resolved integrated and differential cross sections are presented over a wide energy range and compared with previous calculations and available experiments. Los Alamos National Laboratory and Curtin University.

  18. Development of Angular Motion, Angular Momentum, and Torque Knowledge Bases for an Intelligent Physics Tutoring System

    National Research Council Canada - National Science Library

    Eason, Michael

    1998-01-01

    .... The knowledge base developed in this project provides the physics backbone for the rest of the tutoring system by generating the necessary equations and solution graphs to solve selected angular motion...

  19. Valence and inner-valence shell dissociative photoionization of CO in the 26-33 eV range. II. Molecular-frame and recoil-frame photoelectron angular distributions

    DEFF Research Database (Denmark)

    Lebech, M.; Houver, J.C.; Raseev, G.

    2012-01-01

    Experimental and theoretical results for molecular-frame photoemission are presented for inner-valence shell photoionization of the CO molecule induced by linearly and circularly polarized light. The experimental recoil frame photoelectron angular distributions (RFPADs) obtained from dissociative...... for the case of general elliptically polarized light, to obtain the RFPAD rather than the molecular frame photoelectron angular distribution (MFPAD), which would be obtained with the assumption of instantaneous dissociation. We have considered photoionization of CO for the photon energies of 26.0 eV, 29.5 e......V, and 32.5 eV. A comparison of experimental and theoretical RFPADs allows us to identify the ionic states detected in the experimental studies. In addition to previously identified states, we found evidence for the 2 (2)Delta state with an ionization potential of 25.3 eV and (2)Sigma(+) states...

  20. Inverse photoemission

    International Nuclear Information System (INIS)

    Namatame, Hirofumi; Taniguchi, Masaki

    1994-01-01

    Photoelectron spectroscopy is regarded as the most powerful means since it can measure almost perfectly the occupied electron state. On the other hand, inverse photoelectron spectroscopy is the technique for measuring unoccupied electron state by using the inverse process of photoelectron spectroscopy, and in principle, the similar experiment to photoelectron spectroscopy becomes feasible. The development of the experimental technology for inverse photoelectron spectroscopy has been carried out energetically by many research groups so far. At present, the heightening of resolution of inverse photoelectron spectroscopy, the development of inverse photoelectron spectroscope in which light energy is variable and so on are carried out. But the inverse photoelectron spectroscope for vacuum ultraviolet region is not on the market. In this report, the principle of inverse photoelectron spectroscopy and the present state of the spectroscope are described, and the direction of the development hereafter is groped. As the experimental equipment, electron guns, light detectors and so on are explained. As the examples of the experiment, the inverse photoelectron spectroscopy of semimagnetic semiconductors and resonance inverse photoelectron spectroscopy are reported. (K.I.)

  1. Multichannel system for angular distribution measurements

    International Nuclear Information System (INIS)

    Burjan, V.; Kroha, V.; Putz, K.

    A description is given of the individual blocks of the spectrometric apparatus used for measuring the angular distribution of particle spectra and excitation functions of (d,p) reactions at an electrostatic accelerator and the U-120 M cyclotron, both operating at the Nuclear Physics Institute of the Czechoslovak Academy of Sciences at Rez. Main attention was devoted to attaining maximum energy resolution at a high measurement efficiency, this by installing 8 independent spectrometric chains allowing simultaneous measurement of angular distribution in 8 points of the beam. The semiconductor detectors were cooled to -40 degC to -60 degC, which significantly reduced the level of inherent detector noise. An energy resolution of 13 keV was attained using Tesla detectors at a particle energy of 11 MeV. A brief review of data processing and software is given. (B.S.)

  2. A theoretical investigation of photoemission spectra from (GaAs).sub.2./sub. (AlAs).sub.2./sub. superlattices

    Czech Academy of Sciences Publication Activity Database

    Strasser, T.; Solterbeck, C.; Schattke, W.; Bartoš, Igor; Cukr, Miroslav; Jiříček, Petr; Fadley, C. S.; Van Hove, M. A.

    114-116, - (2001), s. 1127-1132 ISSN 0368-2048 Institutional research plan: CEZ:A02/98:Z1-010-914 Keywords : superlattices * III/V semiconductors * photoemission * one-step model Subject RIV: BM - Solid Matter Physics ; Magnetism Impact factor: 1.259, year: 2001

  3. On the excess photon noise in single-beam measurements with photo-emissive and photo-conductive cells

    NARCIS (Netherlands)

    Alkemade, C.T.J.

    In this paper the so-called excess photon noise is theoretically considered with regard to noise power measurements with a single, illumined photo-emissive or photo-conductive cell. Starting from a modification of Mandel's stochastic association of the emission of photo-electrons with wave

  4. The multiplicity of massive stars: A high angular resolution survey with the HST fine guidance sensor

    International Nuclear Information System (INIS)

    Aldoretta, E. J.; Gies, D. R.; Henry, T. J.; Jao, W.-C.; Norris, R. P.

    2015-01-01

    We present the results of an all-sky survey made with the Fine Guidance Sensor on the Hubble Space Telescope to search for angularly resolved binary systems among massive stars. The sample of 224 stars is comprised mainly of Galactic O- and B-type stars and luminous blue variables, plus a few luminous stars in the Large Magellanic Cloud. The FGS TRANS mode observations are sensitive to the detection of companions with an angular separation between 0.″01 and 1.″0 and brighter than △m=5. The FGS observations resolved 52 binary and 6 triple star systems and detected partially resolved binaries in 7 additional targets (43 of these are new detections). These numbers yield a companion detection frequency of 29% for the FGS survey. We also gathered literature results on the numbers of close spectroscopic binaries and wider astrometric binaries among the sample, and we present estimates of the frequency of multiple systems and the companion frequency for subsets of stars residing in clusters and associations, field stars, and runaway stars. These results confirm the high multiplicity fraction, especially among massive stars in clusters and associations. We show that the period distribution is approximately flat in increments of logP. We identify a number of systems of potential interest for long-term orbital determinations, and we note the importance of some of these companions for the interpretation of the radial velocities and light curves of close binaries that have third companions.

  5. Coherent Control of Photoelectron Wavepacket Angular Interferograms

    OpenAIRE

    Hockett, Paul; Wollenhaupt, Matthias; Baumert, Thomas

    2015-01-01

    Coherent control over photoelectron wavepackets, via the use of polarization-shaped laser pulses, can be understood as a time and polarization-multiplexed process. In this work, we investigate this multiplexing via computation of the observable photoelectron angular interferograms resulting from multi-photon atomic ionization with polarization-shaped laser pulses. We consider the polarization sensitivity of both the instantaneous and cumulative continuum wavefunction; the nature of the cohere...

  6. Angular distribution of laser ablation plasma

    International Nuclear Information System (INIS)

    Kondo, K.; Kanesue, T.; Dabrowski, R.; Okamura, M.

    2010-01-01

    An expansion of a laser induced plasma is fundamental and important phenomena in a laser ion source. To understand the expanding direction, an array of Langmuir probes were employed. The chosen ion for the experiment was Ag 1+ which was created by a second harmonics of a Nd-YAG laser. The obtained angular distribution was about ±10 degree. This result also indicates a proper positioning of a solenoid magnet which enhances ion beam current.

  7. Continuum angular distributions in the transition regions

    International Nuclear Information System (INIS)

    Kalbach, C.

    1993-01-01

    One of the open questions from the 1988 published systematics of continuum angular distributions in light particle reactions is addressed. Evidence for a smooth transition in the systematics at incident energies of ∼125 MeV is summarized, and appropriate revisions to the global parameterization are proposed. Applying similar changes to the second-order term helps to remove problems noted in the literature with low-energy (N,α) reactions

  8. Coincident-inclusive electrofission angular correlations

    International Nuclear Information System (INIS)

    Arruda Neto, J.D.T.

    1983-08-01

    A method for the joint analysis of coincident and inclusive electrofission data, in order to minimize effects of the model dependence of data interpretation, is developed. Explicit calculations of the (e,e'f) angular correlations are presented. The potentialities of the method to the study of sub- and near-barrier properties of the fission process, and to the study of the giant resonances fission mode, are discussed. (Author) [pt

  9. Spatial angular compounding of photoacoustic images

    OpenAIRE

    Kang, Hyun Jae; Bell, Muyinatu A Lediju; Guo, Xiaoyu; Boctor, Emad M.

    2016-01-01

    Photoacoustic (PA) images utilize pulsed lasers and ultrasound transducers to visualize targets with higher optical absorption than the surrounding medium. However, they are susceptible to acoustic clutter and background noise artifacts that obfuscate biomedical structures of interest. We investigated three spatial-angular compounding methods to improve PA image quality for biomedical applications, implemented by combining multiple images acquired as an ultrasound probe was rotated about the ...

  10. Orbital angular momentum light in microscopy.

    Science.gov (United States)

    Ritsch-Marte, Monika

    2017-02-28

    Light with a helical phase has had an impact on optical imaging, pushing the limits of resolution or sensitivity. Here, special emphasis will be given to classical light microscopy of phase samples and to Fourier filtering techniques with a helical phase profile, such as the spiral phase contrast technique in its many variants and areas of application.This article is part of the themed issue 'Optical orbital angular momentum'. © 2017 The Author(s).

  11. Resolving inventory differences

    International Nuclear Information System (INIS)

    Weber, J.H.; Clark, J.P.

    1991-01-01

    Determining the cause of an inventory difference (ID) that exceeds warning or alarm limits should not only involve investigation into measurement methods and reexamination of the model assumptions used in the calculation of the limits, but also result in corrective actions that improve the quality of the accountability measurements. An example illustrating methods used by Savannah River Site (SRS) personnel to resolve an ID is presented that may be useful to other facilities faced with a similar problem. After first determining that no theft or diversion of material occurred and correcting any accountability calculation errors, investigation into the IDs focused on volume and analytical measurements, limit of error of inventory difference (LEID) modeling assumptions, and changes in the measurement procedures and methods prior to the alarm. There had been a gradual gain trend in IDs prior to the alarm which was reversed by the alarm inventory. The majority of the NM in the facility was stored in four large tanks which helped identify causes for the alarm. The investigation, while indicating no diversion or theft, resulted in changes in the analytical method and in improvements in the measurement and accountability that produced a 67% improvement in the LEID

  12. Continuous particle spectra and their angular distributions

    International Nuclear Information System (INIS)

    Sastry, Ch.V.; Jain, R.K.; Rama Rao, J.; Ernst, J.; Machner, H.

    1996-01-01

    The angular distribution of continuous particle spectra in pre-equilibrium reactions is still an unsolved problem, particularly so at forward angles. In the present work, the angular distributions of alpha particles emitted in (α, α',x) reactions in the target elements gold and rhodium have been studied in detail. Alpha particle beams of energy 60 MeV from the Variable Energy Cyclotron of Calcutta were used in these experiments. The theoretical calculations were done using an extended exciton model of Kalbach incorporated into the Computer Code PRECO-D2. The formalism used in the exciton model was modified to include division of pre equilibrium cross section into multi-step direct (MSD) and multi-step compound (MSC) components. These MSD and MSC cross sections were used to calculate the angular distributions in terms of Legendre polynomials whose coefficients are given by simple phenomenological relations. Even with a reasonable set of parameters, the agreement between theory and experiment was far from satisfactory at forward angles. Similar conclusion was also drawn in the case of continuous particle spectra of deuterons in (d, d'x) reactions at 25 MeV in various targets. (author). 10 refs., 2 figs

  13. The Cosmology Large Angular Scale Surveyor

    Science.gov (United States)

    Harrington, Kathleen; Marriage, Tobias; Ali, Aamir; Appel, John; Bennett, Charles; Boone, Fletcher; Brewer, Michael; Chan, Manwei; Chuss, David T.; Colazo, Felipe; hide

    2016-01-01

    The Cosmology Large Angular Scale Surveyor (CLASS) is a four telescope array designed to characterize relic primordial gravitational waves from inflation and the optical depth to reionization through a measurement of the polarized cosmic microwave background (CMB) on the largest angular scales. The frequencies of the four CLASS telescopes, one at 38 GHz, two at 93 GHz, and one dichroic system at 145217 GHz, are chosen to avoid spectral regions of high atmospheric emission and span the minimum of the polarized Galactic foregrounds: synchrotron emission at lower frequencies and dust emission at higher frequencies. Low-noise transition edge sensor detectors and a rapid front-end polarization modulator provide a unique combination of high sensitivity, stability, and control of systematics. The CLASS site, at 5200 m in the Chilean Atacama desert, allows for daily mapping of up to 70% of the sky and enables the characterization of CMB polarization at the largest angular scales. Using this combination of a broad frequency range, large sky coverage, control over systematics, and high sensitivity, CLASS will observe the reionization and recombination peaks of the CMB E- and B-mode power spectra. CLASS will make a cosmic variance limited measurement of the optical depth to reionization and will measure or place upper limits on the tensor-to-scalar ratio, r, down to a level of 0.01 (95% C.L.).

  14. The Cosmology Large Angular Scale Surveyor (CLASS)

    Science.gov (United States)

    Harrington, Kathleen; Marriange, Tobias; Aamir, Ali; Appel, John W.; Bennett, Charles L.; Boone, Fletcher; Brewer, Michael; Chan, Manwei; Chuss, David T.; Colazo, Felipe; hide

    2016-01-01

    The Cosmology Large Angular Scale Surveyor (CLASS) is a four telescope array designed to characterize relic primordial gravitational waves from in ation and the optical depth to reionization through a measurement of the polarized cosmic microwave background (CMB) on the largest angular scales. The frequencies of the four CLASS telescopes, one at 38 GHz, two at 93 GHz, and one dichroic system at 145/217 GHz, are chosen to avoid spectral regions of high atmospheric emission and span the minimum of the polarized Galactic foregrounds: synchrotron emission at lower frequencies and dust emission at higher frequencies. Low-noise transition edge sensor detectors and a rapid front-end polarization modulator provide a unique combination of high sensitivity, stability, and control of systematics. The CLASS site, at 5200 m in the Chilean Atacama desert, allows for daily mapping of up to 70% of the sky and enables the characterization of CMB polarization at the largest angular scales. Using this combination of a broad frequency range, large sky coverage, control over systematics, and high sensitivity, CLASS will observe the reionization and recombination peaks of the CMB E- and B-mode power spectra. CLASS will make a cosmic variance limited measurement of the optical depth to reionization and will measure or place upper limits on the tensor-to-scalar ratio, r, down to a level of 0.01 (95% C.L.).

  15. Verification of angular dependence in MOSFET detector

    International Nuclear Information System (INIS)

    Souza, Clayton H.; Shorto, Julian M.B.; Siqueira, Paulo T.D.; Nunes, Maíra G.; Silva Junior, Iremar A.; Yoriyaz, Hélio

    2017-01-01

    In vivo dosimetry is an essential tool for quality assurance programs, being a procedure commonly performed with thermoluminescent dosimeters (TLDs) or diodes. However, a type of dosimeter that has increasing popularity in recent years is the metal-oxide-semiconductor field effect transistor (MOSFET) detector. MOSFET dosimeters fulfill all the necessary characteristics to realize in vivo dosimetry since it has a small size, good precision and feasibility of measurement, as well as easy handling. Nevertheless, its true differential is to allow reading of the dose in real time, enabling immediate intervention in the correction of physical parameters deviations and anticipation of small anatomical changes in a patient during treatment. In order for MOSFET dosimeter to be better accepted in clinical routine, information reporting performance should be available frequently. For this reason, this work proposes to verify reproducibility and angular dependence of a standard sensitivity MOSFET dosimeter (TN-502RD-H) for Cs-137 and Co-60 sources. Experimental data were satisfactory and MOSFET dosimeter presented a reproducibility of 3.3% and 2.7% (1 SD) for Cs-137 and Co-60 sources, respectively. In addition, an angular dependence of up to 6.1% and 16.3% for both radioactive sources, respectively. It is conclusive that MOSFET dosimeter TN-502RD-H has satisfactory reproducibility and a considerable angular dependence, mainly for the Co-60 source. This means that although precise measurements, special attention must be taken for applications in certain anatomical regions in a patient. (author)

  16. Angular craniometry in craniocervical junction malformation.

    Science.gov (United States)

    Botelho, Ricardo Vieira; Ferreira, Edson Dener Zandonadi

    2013-10-01

    The craniometric linear dimensions of the posterior fossa have been relatively well studied, but angular craniometry has been poorly studied and may reveal differences in the several types of craniocervical junction malformation. The objectives of this study were to evaluate craniometric angles compared with normal subjects and elucidate the main angular differences among the types of craniocervical junction malformation and the correlation between craniocervical and cervical angles. Angular craniometries were studied using primary cranial angles (basal and Boogard's) and secondary craniocervical angles (clivus canal and cervical spine lordosis). Patients with basilar invagination had significantly wider basal angles, sharper clivus canal angles, larger Boogard's angles, and greater cervical lordosis than the Chiari malformation and control groups. The Chiari malformation group does not show significant differences when compared with normal controls. Platybasia occurred only in basilar invagination and is suggested to be more prevalent in type II than in type I. Platybasic patients have a more acute clivus canal angle and show greater cervical lordosis than non-platybasics. The Chiari group does not show significant differences when compared with the control, but the basilar invagination groups had craniometric variables significantly different from normal controls. Hyperlordosis observed in the basilar inavagination group was associated with craniocervical kyphosis conditioned by acute clivus canal angles.

  17. Verification of angular dependence in MOSFET detector

    Energy Technology Data Exchange (ETDEWEB)

    Souza, Clayton H.; Shorto, Julian M.B.; Siqueira, Paulo T.D.; Nunes, Maíra G.; Silva Junior, Iremar A.; Yoriyaz, Hélio, E-mail: chsouza@usp.br [Instituto de Pesquisas Energeticas e Nucleares (IPEN/CNEN-SP), Sao Paulo, SP (Brazil)

    2017-07-01

    In vivo dosimetry is an essential tool for quality assurance programs, being a procedure commonly performed with thermoluminescent dosimeters (TLDs) or diodes. However, a type of dosimeter that has increasing popularity in recent years is the metal-oxide-semiconductor field effect transistor (MOSFET) detector. MOSFET dosimeters fulfill all the necessary characteristics to realize in vivo dosimetry since it has a small size, good precision and feasibility of measurement, as well as easy handling. Nevertheless, its true differential is to allow reading of the dose in real time, enabling immediate intervention in the correction of physical parameters deviations and anticipation of small anatomical changes in a patient during treatment. In order for MOSFET dosimeter to be better accepted in clinical routine, information reporting performance should be available frequently. For this reason, this work proposes to verify reproducibility and angular dependence of a standard sensitivity MOSFET dosimeter (TN-502RD-H) for Cs-137 and Co-60 sources. Experimental data were satisfactory and MOSFET dosimeter presented a reproducibility of 3.3% and 2.7% (1 SD) for Cs-137 and Co-60 sources, respectively. In addition, an angular dependence of up to 6.1% and 16.3% for both radioactive sources, respectively. It is conclusive that MOSFET dosimeter TN-502RD-H has satisfactory reproducibility and a considerable angular dependence, mainly for the Co-60 source. This means that although precise measurements, special attention must be taken for applications in certain anatomical regions in a patient. (author)

  18. Recent trends in spin-resolved photoelectron spectroscopy

    Science.gov (United States)

    Okuda, Taichi

    2017-12-01

    Since the discovery of the Rashba effect on crystal surfaces and also the discovery of topological insulators, spin- and angle-resolved photoelectron spectroscopy (SARPES) has become more and more important, as the technique can measure directly the electronic band structure of materials with spin resolution. In the same way that the discovery of high-Tc superconductors promoted the development of high-resolution angle-resolved photoelectron spectroscopy, the discovery of this new class of materials has stimulated the development of new SARPES apparatus with new functions and higher resolution, such as spin vector analysis, ten times higher energy and angular resolution than conventional SARPES, multichannel spin detection, and so on. In addition, the utilization of vacuum ultra violet lasers also opens a pathway to the realization of novel SARPES measurements. In this review, such recent trends in SARPES techniques and measurements will be overviewed.

  19. Time-resolved studies

    International Nuclear Information System (INIS)

    Mills, D.M.

    1992-01-01

    When new or more powerful probes become available that offer both shorter data-collection times and the opportunity to apply innovative approaches to established techniques, it is natural that investigators consider the feasibility of exploring the kinetics of time-evolving systems. This stimulating area of research not only can lead to insights into the metastable or excited states that a system may populate on its way to a ground state, but can also lead to a better understanding of that final state. Synchrotron radiation, with its unique properties, offers just such a tool to extend X-ray measurements from the static to the time-resolved regime. The most straight-forward application of synchrotron radiation to the study of transient phenomena is directly through the possibility of decreased data-collection times via the enormous increase in flux over that of a laboratory X-ray system. Even further increases in intensity can be obtained through the use of novel X-ray optical devices. Widebandpass monochromators, e.g., that utilize the continuous spectral distribution of synchrotron radiation, can increase flux on the sample several orders of magnitude over conventional X-ray optical systems thereby allowing a further shortening of the data-collection time. Another approach that uses the continuous spectral nature of synchrotron radiation to decrease data-collection times is the open-quote parallel data collectionclose quotes method. Using this technique, intensities as a function of X-ray energy are recorded simultaneously for all energies rather than sequentially recording data at each energy, allowing for a dramatic decrease in the data-collection time

  20. Aberration correction in photoemission microscopy and applications in photonics and plasmonics

    Energy Technology Data Exchange (ETDEWEB)

    Koenenkamp, Rolf [Portland State Univ., Portland, OR (United States)

    2017-09-28

    We report on the design, assembly, operation and application of an aberration-corrected photoemission electron microscope. The instrument used novel hyperbolic mirror-correctors with two and three electrodes that allowed simultaneous correction of spherical and chromatic aberrations. A spatial resolution of 5.4nm was obtained with this instrument in 2009, and 4.7nm in subsequent years. New imaging methodology was introduced involving interferometric imaging of light diffraction. This methodology was applied in nano-photonics and in the characterization of surface-plasmon polaritons. Photonic crystals and waveguides, optical antennas and new plasmonic devices such as routers, localizers and filters were designed and demonstrated using the new capabilities offered by the microscope.

  1. Magnetic x-ray linear dichroism in resonant and non-resonant Gd 4f photoemission

    Energy Technology Data Exchange (ETDEWEB)

    Mishra, S.; Gammon, W.J.; Pappas, D.P. [Virginia Commonwealth Univ., Richmond, VA (United States)] [and others

    1997-04-01

    The enhancement of the magnetic linear dichroism in resonant 4f photoemission (MLDRPE) is studied from a 50 monolayer film of Gd/Y(0001). The ALS at beamline 7.0.1 provided the source of linearly polarized x-rays used in this study. The polarized light was incident at an angle of 30 degrees relative to the film plane, and the sample magnetization was perpendicular to the photon polarization. The linear dichroism of the 4f core levels is measured as the photon energy is tuned through the 4d-4f resonance. The authors find that the MLDRPE asymmetry is strongest at the resonance. Near the threshold the asymmetry has several features which are out of phase with the fine structure of the total yield.

  2. Influence of Al fraction on photoemission performance of AlGaN photocathode.

    Science.gov (United States)

    Hao, Guanghui; Chang, Benkang; Shi, Feng; Zhang, Junju; Zhang, Yijun; Chen, Xinlong; Jin, Muchun

    2014-06-10

    To research the photoemission performance of a transmission-mode Al(1-x)Ga(x)N photocathode, Al0.24Ga0.76N and GaN photocathodes with the same structure were activated, their spectral responses were measured using a multi-information measurement system at room temperature, and the photocathode parameters were obtained by fitting quantum efficiency curves. The results showed that both the reflective-mode and transmission-mode spectral responses of the AlGaN photocathode were lower than those of the GaN photocathode. Compared with the GaN photocathode, the short-wavelength spectral response of the Al0.24Ga0.76N photocathode was less seriously affected by lattice defects between the buffer and emission layers. The Al atom at the AlGaN photocathode surface could affect the optimal Cs adsorption position, which mainly affects the surface electron escape probability of the photocathode.

  3. Study of adsorption states for lubricant molecule using hard X-ray photoemission spectroscopy

    International Nuclear Information System (INIS)

    Ikenaga, E.; Kobata, M.; Kim, J.J.; Wakabayashi, A.; Nishino, Y.; Tamasaku, K.; Sakane, Y.; Ishikawa, T.; Komiya, S.; Kobayashi, K.

    2007-01-01

    The adsorption states for lubricant molecules have been investigated using hard X-ray (hν = 7.95 keV) photoemission spectroscopy (HX-PES). This method has the advantage for the organic molecules to be able to measure damage few. Being aware of the fact that P atoms exist only in cyclotriphosphazene base, we measured the take-off angle dependence of the P1s spectra. Each spectrum consists from two peaks, that is, substrate NiP peak and cyclotriphosphazene P peak. The cyclotriphosphazene P peak rapidly disappears with increasing take-off angle. We have also measured C1s spectra. Combining these experimental results, we have found that the adsorption state of cyclotriphosphazene end group is undergoing

  4. A new aberration correction method for photoemission electron microscopy by means of moving focus

    International Nuclear Information System (INIS)

    Koshikawa, T; Shimizu, H; Amakawa, R; Ikuta, T; Yasue, T; Bauer, E

    2005-01-01

    A new aberration correction method has been developed for photoemission electron microscopy (PEEM). In order to correct the spherical and chromatic aberrations, a moving focus method was adopted. Several experimental limitations to achieving optimal resolution have also been overcome. A high brightness Hg lamp system has been developed to overcome the insufficient brightness of the conventional Hg lamp. An improvement of brightness by over 100 times as compared with the conventional lamp was achieved. Image blur was also found due to a weak environmental AC magnetic field caused by essential microscope components, i.e., the power transformer and CCD camera. After implementing the high brightness lamp and eliminating stray magnetic field by proper shielding, preliminary experiments demonstrate that aberration correction by moving focus can improve the PEEM image resolution

  5. Common Features in Electronic Structure of the Oxypnictide Superconductors from Photoemission Spectroscopy

    International Nuclear Information System (INIS)

    Xiao-Wen, Jia; Hai-Yun, Liu; Wen-Tao, Zhang; Lin, Zhao; Jian-Qiao, Meng; Guo-Dong, Liu; Xiao-Li, Dong; Zhi-An, Ren; Wei, Yi; Guang-Can, Che; Zhong-Xian, Zhao; Gang, Wu; Rong-Hua, Liu; Xian-Hui, Chen; Gen-Fu, Chen; Nan-Lin, Wang; Yong, Zhu; Xiao-Yang, Wang; Gui-Ling, Wang; Yong, Zhou

    2008-01-01

    High resolution photoemission measurements are carried out on non-superconducting LaFeAsO parent compound and various superconducting RFeAs(O 1-x F x ) (R=La, Ce and Pr) compounds. It is found that the parent LaFeAsO compound shows a metallic character. By extensive measurements, several common features are identified in the electronic structure of these Fe-based compounds: (1) 0.2 eV feature in the valence band, (2) a universal 13-16 meV feature, (3) near Ef spectral weight suppression with decreasing temperature. These universal features can provide important information about band structure, superconducting gap and pseudogap in these Fe-based materials

  6. Hard X-ray PhotoEmission Spectroscopy of strongly correlated systems

    Science.gov (United States)

    Panaccione, Giancarlo; Offi, Francesco; Sacchi, Maurizio; Torelli, Piero

    2008-06-01

    Hard X-ray PhotoEmission Spectroscopy (HAXPES) is a new tool for the study of bulk electronic properties of solids using synchrotron radiation. We review recent achievements of HAXPES, with particular reference to the VOLPE project, showing that high energy resolution and bulk sensitivity can be obtained at kinetic energies of 6-8 keV. We present also the results of recent studies on strongly correlated materials, such as vanadium sesquioxide and bilayered manganites, revealing the presence of different screening properties in the bulk with respect to the surface. We discuss the relevant experimental features of the metal-insulator transition in these materials. To cite this article: G. Panaccione et al., C. R. Physique 9 (2008).

  7. Retention Characteristics of CBTi144 Thin Films Explained by Means of X-Ray Photoemission Spectroscopy

    Directory of Open Access Journals (Sweden)

    G. Biasotto

    2010-01-01

    Full Text Available CaBi4Ti4O15 (CBTi144 thin films were grown on Pt/Ti/SiO2/Si substrates using a soft chemical solution and spin-coating method. Structure and morphology of the films were characterized by the X-ray Diffraction (XRD, Fourier-transform infrared spectroscopy (FT-IR, Raman analysis, X-ray photoemission spectroscopy (XPS, and transmission electron microscopy (TEM. The films present a single phase of layered-structured perovskite with polar axis orient. The a/b-axis orientation of the ferroelectric film is considered to be associated with the preferred orientation of the Pt bottom electrode. XPS measurements were employed to understand the nature of defects on the retention behavior of CBTi144 films. We have observed that the main source of retention-free characteristic of the capacitors is the oxygen environment in the CBTi144 lattice.

  8. Absence of U 5f band states in resonant photoemission spectra of UPd2Al3

    Science.gov (United States)

    Fujimori, Shin-Ichi; Saito, Yasuharu; Seki, Masaharu; Tamura, Koji; Mizuta, Munenori; Yamaki, Ken-Ichiro; Sato, Ken; Tanaka, Akinori; Sato, Noriaki; Suzuki, Shoji; Sato, Shigeru; Okane, Tetsuo; Komatsubara, Takemi; Tezuka, Yasuhisa; Shin, Shik; Ishii, Takehiko

    1999-04-01

    The U 5f spectral weight of UxLa1-xPd2Al3 (x=0.1, 0.25, 0.6, and 1.0) is obtained by the resonant photoemission spectroscopy (RPES), and is compared with the results of the band-structure calculations. We have found that the spectrum of UPd2Al3 (x=1) could not be reproduced by the calculated U 5f density of states in shape and position, even if the contribution from U 6d states is considered. Moreover, the essential spectral shape did not change until x=0.1, where most of the uranium atoms are substituted with lanthanum atoms. All these results indicate that the U 5f band states are not observed in the RPES spectrum of UPd2Al3, and the single site effects govern it.

  9. The interaction of oxygen with TiC(001): Photoemission and first-principles studies

    International Nuclear Information System (INIS)

    Rodriguez, J.A.; Liu, P.; Dvorak, J.; Jirsak, T.; Gomes, J.; Takahashi, Y.; Nakamura, K.

    2004-01-01

    High-resolution photoemission and first-principles density-functional slab calculations were used to study the interaction of oxygen with a TiC(001) surface. Atomic oxygen is present on the TiC(001) substrate after small doses of O 2 at room temperature. A big positive shift (1.5-1.8 eV) was detected for the C 1s core level. These photoemission studies suggest the existence of strong O↔C interactions. A phenomenon corroborated by the results of first-principles calculations, which show a CTiTi hollow as the most stable site for the adsorption of O. Ti and C atoms are involved in the adsorption and dissociation of the O 2 molecule. In general, the bond between O and the TiC(001) surface contains a large degree of ionic character. The carbide→O charge transfer is substantial even at high coverages (>0.5 ML) of oxygen. At 500 K and large doses of O 2 , oxidation of the carbide surface occurs with the removal of C and formation of titanium oxides. There is an activation barrier for the exchange of Ti-C and Ti-O bonds which is overcome only by the formation of C-C or C-O bonds on the surface. The mechanism for the removal of a C atom as CO gas involves a minimum of two O adatoms, and three O adatoms are required for the formation of CO 2 gas. Due to the high stability of TiC, an O adatom alone cannot induce the generation of a C vacancy in a flat TiC(001) surface

  10. Progresses in low energy electron microscopy and photoemission electron microscopy studies (LEEM and PEEM)

    International Nuclear Information System (INIS)

    Koshikawa, Takanori; Yasue, Tsuneo; Kobayashi, Keisuke; Kinoshita, Toyohiko; Ono, Kanta

    2008-02-01

    Photon factory workshop on low energy electron microscopy (LEEM) and photoemission electron microscopy (PEEM) studies was held on October 12-13, 2005. The workshop had 18 presentations and 8 contributions to the poster session with 62 attendees. The workshop started with an invitation presentation about nano-imaging and nano-spectroscopy by photoemission electron microscope using synchrotron radiation x-rays. Next two reports were about antiferromagnetic domain structure observations of a NiO(100) surface using a combined method of PEEM and soft x-ray linear dichroism. Recent development of spin SEM (scanning electron microscope) and the observation of magnetic domains of La 1.36 Sr 1.64 Mn 2 O 7 were reported. A new method for observing magnetic domain structures with SEM was developed in which the image is the result of spin polarization of secondary electrons. This method is called spin SEM. A lecture about observation of ultra-high speed phenomena by PEEM and the invitation presentation about spin dynamics in nano-scale magnetic materials attracted much attention. Structural studies of surfaces by LEEM and PEEM were actively discussed. Summaries about the measurements of Au-Si alloy island at atomic steps on Si(111), fabrication of Ga nano-dots in SiO 2 , growth of pentacene films on thin bismuth film and graphite, the surface phase transition on metal surfaces of In/Cu(001) and Sn/Cu(001), and Cu thin film growth on W(110) were also compiled in this report. Many contributions in this report were resulted from the experiments by LEEM and PEEM using SPring-8 synchrotron radiations. (Y.K.)

  11. Magnetic dichroism in photoemission: a new element-specific magnetometer with atomic-layer resolution

    International Nuclear Information System (INIS)

    Starke, K.; Arenholz, E.; Kaindl, G.

    1998-01-01

    Full text: Magnetic coupling in layered metallic structures has become a key issue in thin-film magnetism since the observation of oscillatory exchange coupling across non-ferromagnetic spacer layers. Although this phenomenon was discovered in rare earths (RE) superlattices, mostly transition-metal systems have been studied and are now applied in data-storage industry. An understanding of the coupling mechanisms has been reached after a fabrication of high-quality interfaces became possible. It allowed, in particular, the experimental finding of induced ferromagnetic order in 'nonmagnetic' atomic layers near an interface, using element-specific probes such as magnetic circular dichroism in x-ray absorption. - In layered RE systems, by contrast, the well known intermiscibility has prevented a preparation of atomically sharp interfaces, and all RE superlattices studied so far showed interdiffusion zones of several atomic layers. In the present overview, we report the first fabrication of atomically flat heteromagnetic RE interfaces, their structural characterization and their magnetic analysis using magnetic dichroism in photoemission (MDPE). This new tool gives access to the magnetization of individual atomic layers near interfaces in favourite cases. Merits of MDPE as a magnetometer are demonstrated at the example of Eu/Gd(0001), where chemical shifts of core-level photoemission lines allow to spectroscopically separate up to four different atomic layers. The high surface sensitivity of MDPE, together with the well known dependence of the core-level binding energies on the coordination number of the photo emitting atom, opens the door to future site-specific studies of magnetism in sub-monolayer systems such as 'nanowires'

  12. Characterizing the effects of regolith surface roughness on photoemission from surfaces in space

    Science.gov (United States)

    Dove, A.; Horanyi, M.; Wang, X.

    2017-12-01

    Surfaces of airless bodies and spacecraft in space are exposed to a variety of charging environments. A balance of currents due to plasma bombardment, photoemission, electron and ion emission and collection, and secondary electron emission determines the surface's charge. Photoelectron emission is the dominant charging process on sunlit surfaces in the inner solar system due to the intense solar UV radiation. This can result in a net positive surface potential, with a cloud of photoelectrons immediately above the surface, called the photoelectron sheath. Conversely, the unlit side of the body will charge negatively due the collection of the fast-moving solar wind electrons. The interaction of charged dust grains with these positively and negatively charged surfaces, and within the photoelectron and plasma sheaths may explain the occurrence of dust lofting, levitation and transport above the lunar surface. The surface potential of exposed objects is also dependent on the material properties of their surfaces. Composition and particle size primarily affect the quantum efficiency of photoelectron generation; however, surface roughness can also control the charging process. In order to characterize these effects, we have conducted laboratory experiments to examine the role of surface roughness in generating photoelectrons in dedicated laboratory experiments using solid and dusty surfaces of the same composition (CeO2), and initial comparisons with JSC-1 lunar simulant. Using Langmuir probe measurements, we explore the measured potentials above insulating surfaces exposed to UV and an electric field, and we show that the photoemission current from a dusty surface is largely reduced due to its higher surface roughness, which causes a significant fraction of the emitted photoelectrons to be re-absorbed within the surface. We will discuss these results in context of similar situations on planetary surfaces.

  13. Empirical relationship between x-ray photoemission spectra and electrical conductivity in a colossal magnetoresistive manganite La_{1-x}Sr_{x}MnO_{3}

    OpenAIRE

    Hishida, T.; Ohbayashi, K.; Kobata, M.; Ikenaga, E.; Sugiyama, T.; Kobayashi, K.; Okawa, M.; Saitoh, T.

    2013-01-01

    By using laboratory x-ray photoemission spectroscopy (XPS) and hard x-ray photoemission spectroscopy (HX-PES) at a synchrotron facility, we report an empirical semi-quantitative relationship between the valence/core-level x-ray photoemission spectral weight and electrical conductivity in La_{1-x}Sr_{x}MnO_{3} as a function of x. In the Mn 2p_{3/2} HX-PES spectra, we observed the shoulder structure due to the Mn^{3+} well-screened state. However, the intensity at x=0.8 was too small to explain...

  14. Spatially resolved investigation of all optical magnetization switching in TbFe alloys.

    Science.gov (United States)

    Arora, Ashima; Mawass, Mohamad-Assaad; Sandig, Oliver; Luo, Chen; Ünal, Ahmet A; Radu, Florin; Valencia, Sergio; Kronast, Florian

    2017-08-25

    Optical control of magnetization using femtosecond laser without applying any external magnetic field offers the advantage of switching magnetic states at ultrashort time scales. Recently, all-optical helicity-dependent switching (AO-HDS) has drawn a significant attention for potential information and data storage device applications. In this work, we employ element and magnetization sensitive photoemission electron microscopy (PEEM) to investigate the role of heating in AO-HDS for thin films of the rare-earth transition-metal alloy TbFe. Spatially resolved measurements in a 3-5 μm sized stationary laser spot demonstrate that AO-HDS is a local phenomenon in the vicinity of thermal demagnetization in a 'ring' shaped region. The efficiency of AO-HDS further depends on a local temperature profile around the demagnetized region and thermally activated domain wall motion. We also demonstrate that the thickness of the film determines the preferential switching direction for a particular helicity.

  15. Circularly polarized light interaction in topological insulators investigated by time-resolved ARPES

    Science.gov (United States)

    Bugini, D.; Hedayat, H.; Boschini, F.; Yi, H.; Chen, C.; Zhou, X.; Manzoni, C.; Dallera, C.; Cerullo, G.; Carpene, E.

    2017-10-01

    Topological Insulators (TI) represent a hot-topic for both basic physics and promising applications because of the in-plane spin-polarized surface states (TSS) arising within the bulk insulating energy gap. The backscattering protection and the control of the spin polarization using ultrashort light pulses open new scenarios in the use of this class of materials for future opto-spintronic devices. Using time- and angle-resolved photoemission spectroscopy on Sb x Bi(2‑x )Se y Te(3‑y ) class we studied the response of spin-polarized electrons to ultrashort circularly-polarized pulses. Here, we report for the first time the experimental evidence of a direct coupling between light and empty topological surface states (ESS) and the establishment of a flow of spin-polarized electrons in k-space i.e. a photon-induced spin-current.

  16. Angular-Momentum Evolution in Laser-Plasma Accelerators

    CERN Document Server

    Thaury, Cédric; Corde, Sébastien; Lehe, Rémi; Le Bouteiller, Madeleine; Ta Phuoc, Kim; Davoine, Xavier; Rax, J. M.; Rousse, Antoine; Malka, Victor

    2013-01-01

    The transverse properties of an electron beam are characterized by two quantities, the emittance which indicates the electron beam extent in the phase space and the angular momentum which allows for non-planar electron trajectories. Whereas the emittance of electron beams produced in laserplasma accelerator has been measured in several experiments, their angular momentum has been scarcely studied. It was demonstrated that electrons in laser-plasma accelerator carry some angular momentum, but its origin was not established. Here we identify one source of angular momentum growth and we present experimental results showing that the angular momentum content evolves during the acceleration.

  17. Isotopically resolved photoelectron imaging unravels complex atomic autoionization dynamics by two-color resonant ionization.

    Science.gov (United States)

    O'Keeffe, P; Gryzlova, E V; Cubaynes, D; Garcia, G A; Nahon, L; Grum-Grzhimailo, A N; Meyer, M

    2013-12-13

    Angle-resolved electron spectroscopy in coincidence with high-resolution mass spectroscopy has been applied to study two-color resonant photoionization in atomic xenon. Separation of different isotopes enabled us to extract results for the electronic dynamics free from depolarization effects, which are generally introduced by the coupling of the electronic and nuclear angular momenta. The concerted experimental and theoretical analysis of the photoelectron angular distributions in the region of an autoionizing resonance emphasizes the strong sensitivity of the observed structures to the fine details of the treatment of the underlying dynamics.

  18. ANGULAR MOMENTUM AND GALAXY FORMATION REVISITED

    International Nuclear Information System (INIS)

    Romanowsky, Aaron J.; Fall, S. Michael

    2012-01-01

    Motivated by a new wave of kinematical tracers in the outer regions of early-type galaxies (ellipticals and lenticulars), we re-examine the role of angular momentum in galaxies of all types. We present new methods for quantifying the specific angular momentum j, focusing mainly on the more challenging case of early-type galaxies, in order to derive firm empirical relations between stellar j * and mass M * (thus extending earlier work by Fall). We carry out detailed analyses of eight galaxies with kinematical data extending as far out as 10 effective radii, and find that data at two effective radii are generally sufficient to estimate total j * reliably. Our results contravene suggestions that ellipticals could harbor large reservoirs of hidden j * in their outer regions owing to angular momentum transport in major mergers. We then carry out a comprehensive analysis of extended kinematic data from the literature for a sample of ∼100 nearby bright galaxies of all types, placing them on a diagram of j * versus M * . The ellipticals and spirals form two parallel j * -M * tracks, with log-slopes of ∼0.6, which for the spirals are closely related to the Tully-Fisher relation, but for the ellipticals derives from a remarkable conspiracy between masses, sizes, and rotation velocities. The ellipticals contain less angular momentum on average than spirals of equal mass, with the quantitative disparity depending on the adopted K-band stellar mass-to-light ratios of the galaxies: it is a factor of ∼3-4 if mass-to-light ratio variations are neglected for simplicity, and ∼7 if they are included. We decompose the spirals into disks and bulges and find that these subcomponents follow j * -M * trends similar to the overall ones for spirals and ellipticals. The lenticulars have an intermediate trend, and we propose that the morphological types of galaxies reflect disk and bulge subcomponents that follow separate, fundamental j * -M * scaling relations. This provides a

  19. ANGULAR MOMENTUM AND GALAXY FORMATION REVISITED

    Energy Technology Data Exchange (ETDEWEB)

    Romanowsky, Aaron J. [University of California Observatories, 1156 High Street, Santa Cruz, CA 95064 (United States); Fall, S. Michael [Space Telescope Science Institute, 3700 San Martin Drive, Baltimore, MD 21218 (United States)

    2012-12-15

    Motivated by a new wave of kinematical tracers in the outer regions of early-type galaxies (ellipticals and lenticulars), we re-examine the role of angular momentum in galaxies of all types. We present new methods for quantifying the specific angular momentum j, focusing mainly on the more challenging case of early-type galaxies, in order to derive firm empirical relations between stellar j{sub *} and mass M{sub *} (thus extending earlier work by Fall). We carry out detailed analyses of eight galaxies with kinematical data extending as far out as 10 effective radii, and find that data at two effective radii are generally sufficient to estimate total j{sub *} reliably. Our results contravene suggestions that ellipticals could harbor large reservoirs of hidden j{sub *} in their outer regions owing to angular momentum transport in major mergers. We then carry out a comprehensive analysis of extended kinematic data from the literature for a sample of {approx}100 nearby bright galaxies of all types, placing them on a diagram of j{sub *} versus M{sub *}. The ellipticals and spirals form two parallel j{sub *}-M{sub *} tracks, with log-slopes of {approx}0.6, which for the spirals are closely related to the Tully-Fisher relation, but for the ellipticals derives from a remarkable conspiracy between masses, sizes, and rotation velocities. The ellipticals contain less angular momentum on average than spirals of equal mass, with the quantitative disparity depending on the adopted K-band stellar mass-to-light ratios of the galaxies: it is a factor of {approx}3-4 if mass-to-light ratio variations are neglected for simplicity, and {approx}7 if they are included. We decompose the spirals into disks and bulges and find that these subcomponents follow j{sub *}-M{sub *} trends similar to the overall ones for spirals and ellipticals. The lenticulars have an intermediate trend, and we propose that the morphological types of galaxies reflect disk and bulge subcomponents that follow

  20. Research on static angular stiffness measurement of flexible joint

    Directory of Open Access Journals (Sweden)

    Yongchao HUANG

    2016-10-01

    Full Text Available Measurement accuracy of the angular stiffness of flexible joint is directly related to the control accuracy and sensitivity of gyro, but the traditional measurement methods have many problems. According to the principle of angular stiffness measurement of flexible joint, two static measurement methods of angular stiffness are proposed based on different loading ways, namely mechanical loading angular stiffness measurement and piezoelectric loading angular stiffness measurement. The mechanical loading angular stiffness measurement system is built by using a motor driven indexing feeding tilting table, the measure experiment if the angular stiffness of flexible joint is conducted, and the angular stiffness of flexible joint is measured. For the excessive fluctuation problem of the measure result in mechanical load test, a piezoelectric loading structure is designed and a measurement method employing piezoelectric actuator is proposed for angular stiffness measurement of flexible joint. Based on ANSYS Workbench, the displacement output of the piezoelectric loading structure is analyzed by simulations. The simulation results illustrate that the displacement output meets the requirement of static loading angular stiffness measurement of flexible joint, and the theoretical feasibility of piezoelectric loading angular stiffness measurement method is validated.

  1. Angular Rate Estimation Using a Distributed Set of Accelerometers

    Directory of Open Access Journals (Sweden)

    Sung Kyung Hong

    2011-11-01

    Full Text Available A distributed set of accelerometers based on the minimum number of 12 accelerometers allows for computation of the magnitude of angular rate without using the integration operation. However, it is not easy to extract the magnitude of angular rate in the presence of the accelerometer noises, and even worse, it is difficult to determine the direction of a rotation because the angular rate is present in its quadratic form within the inertial measurement system equations. In this paper, an extended Kalman filter scheme to correctly estimate both the direction and magnitude of the angular rate through fusion of the angular acceleration and quadratic form of the angular rate is proposed. We also provide observability analysis for the general distributed accelerometers-based inertial measurement unit, and show that the angular rate can be correctly estimated by general nonlinear state estimators such as an extended Kalman filter, except under certain extreme conditions.

  2. Angular Position Tracking Control of a Quadcopter

    OpenAIRE

    T. V. Glazkov; A. E. Golubev

    2017-01-01

    The paper dwells on tracking the quad-copter angular position with desired quality parameters of transient processes. The aerial vehicle is considered as a rigid body with six degrees of freedom.  A full rigid body quad-copter mathematical model is considered without the assumption of smallness of the Euler angles.Among the most well known methods of non-linear stabilization are feedback linearization and backstepping. The backstepping approach allows us to have an effective solution of the s...

  3. Angular Momentum Sensitive Two-Center Interference

    Science.gov (United States)

    Ilchen, M.; Glaser, L.; Scholz, F.; Walter, P.; Deinert, S.; Rothkirch, A.; Seltmann, J.; Viefhaus, J.; Decleva, P.; Langer, B.; Knie, A.; Ehresmann, A.; Al-Dossary, O. M.; Braune, M.; Hartmann, G.; Meissner, A.; Tribedi, L. C.; AlKhaldi, M.; Becker, U.

    2014-01-01

    In quantum mechanics the Young-type double-slit experiment can be performed with electrons either traveling through a double slit or being coherently emitted from two inversion symmetric molecular sites. In the latter one the valence photoionization cross sections of homonuclear diatomic molecules were predicted to oscillate over kinetic energy almost 50 years ago. Beyond the direct proof of the oscillatory behavior of these photoionization cross sections σ, we show that the angular distribution of the emitted electrons reveals hitherto unexplored information on the relative phase shift between the corresponding partial waves through two-center interference patterns.

  4. Projection of angular momentum via linear algebra

    Science.gov (United States)

    Johnson, Calvin W.; O'Mara, Kevin D.

    2017-12-01

    Projection of many-body states with good angular momentum from an initial state is usually accomplished by a three-dimensional integral. We show how projection can instead be done by solving a straightforward system of linear equations. We demonstrate the method and give sample applications to 48Cr and 60Fe in the p f shell. This new projection scheme, which is competitive against the standard numerical quadrature, should also be applicable to other quantum numbers such as isospin and particle number.

  5. The angular momentum of isolated white dwarfs

    Directory of Open Access Journals (Sweden)

    Brassard P.

    2013-03-01

    Full Text Available This is a very brief report on an ongoing program aimed at mapping the internal rotation profiles of stars through asteroseismology. Three years ago, we developed and applied successfully a new technique to the pulsating GW Vir white dwarf PG 1159−035, and were able to infer that it rotates very slowly and rigidly over some 99% of its mass. We applied the same approach to the three other GW Vir pulsators with available rotational splitting data, and found similar results. We discuss the implications of these findings on the question of the angular momentum of white dwarfs resulting from single star evolution.

  6. Models and theory for precompound angular distributions

    Energy Technology Data Exchange (ETDEWEB)

    Blann, M.; Pohl, B.A.; Remington, B.A. (Lawrence Livermore National Lab., CA (USA)); Scobel, W.; Trabandt, M. (Hamburg Univ. (Germany, F.R.). 1. Inst. fuer Experimentalphysik); Byrd, R.C. (Los Alamos National Lab., NM (USA)); Foster, C.C. (Indiana Univ. Cyclotron Facility, Bloomington, IN (USA)); Bonetti, R.; Chiesa, C. (Milan Univ. (Italy). Ist. di Fisica Generale Applicata); Grimes, S.M. (Ohio Univ

    1990-06-06

    We compare angular distributions calculated by folding nucleon- nucleon scattering kernels, using the theory of Feshbach, Kerman and Koonin, and the systematics of Kalbach, with a wide range of data. The data range from (n,xn) at 14 MeV incident energy to (p,xn) at 160 MeV incident energy. The FKK theory works well with one adjustable parameter, the depth of the nucleon-nucleon interaction potential. The systematics work well when normalized to the hybrid model single differential cross section prediction. The nucleon- nucleon scattering approach seems inadequate. 9 refs., 10 figs.

  7. A proposed measurement of optical orbital and spin angular momentum and its implications for photon angular momentum

    Science.gov (United States)

    Leader, Elliot

    2018-04-01

    The expression for the total angular momentum carried by a laser optical vortex beam, splits, in the paraxial approximation, into two terms which seem to represent orbital and spin angular momentum respectively. There are, however, two very different competing versions of the formula for the spin angular momentum, one based on the use of the Poynting vector, as in classical electrodynamics, the other related to the canonical expression for the angular momentum which occurs in Quantum Electrodynamics. I analyze the possibility that a sufficiently sensitive optical measurement could decide which of these corresponds to the actual physical angular momentum carried by the beam.

  8. An angular-selective electron source for the KATRIN experiment

    Czech Academy of Sciences Publication Activity Database

    Beck, M.; Bokeloh, K.; Hein, H.; Bauer, S.; Baumeister, H.; Bonn, J.; Ortjohann, H.W.; Ostrick, B.; Rosendahl, S.; Streubel, S.; Valerius, K.; Zbořil, Miroslav; Weinheimer, C.

    2014-01-01

    Roč. 9, č. 11 (2014), č. článku 11020. ISSN 1748-0221 R&D Projects: GA ČR(CZ) GAP203/12/1896 Institutional support: RVO:61389005 Keywords : spectrometers * photoemission * detector alignment and calibration methods Subject RIV: BF - Elementary Particles and High Energy Physics OBOR OECD: Particles and field physics Impact factor: 1.399, year: 2014

  9. The Cosmology Large Angular Scale Surveyor (CLASS)

    Science.gov (United States)

    Cleary, Joseph

    2018-01-01

    The Cosmology Large Angular Scale Surveyor (CLASS) is an array of four telescopes designed to measure the polarization of the Cosmic Microwave Background. CLASS aims to detect the B-mode polarization from primordial gravitational waves predicted by cosmic inflation theory, as well as the imprint left by reionization upon the CMB E-mode polarization. This will be achieved through a combination of observing strategy and state-of-the-art instrumentation. CLASS is observing 70% of the sky to characterize the CMB at large angular scales, which will measure the entire CMB power spectrum from the reionization peak to the recombination peak. The four telescopes operate at frequencies of 38, 93, 145, and 217 GHz, in order to estimate Galactic synchrotron and dust foregrounds while avoiding atmospheric absorption. CLASS employs rapid polarization modulation to overcome atmospheric and instrumental noise. Polarization sensitive cryogenic detectors with low noise levels provide CLASS the sensitivity required to constrain the tensor-to-scalar ratio down to levels of r ~ 0.01 while also measuring the optical depth the reionization to sample-variance levels. These improved constraints on the optical depth to reionization are required to pin down the mass of neutrinos from complementary cosmological data. CLASS has completed a year of observations at 38 GHz and is in the process of deploying the rest of the telescope array. This poster provides an overview and update on the CLASS science, hardware and survey operations.

  10. Electromagnetic angular positioner based on DC micromotor

    Directory of Open Access Journals (Sweden)

    Bodnicki Maciej

    2018-01-01

    Full Text Available The presented works concerned launching of an angular positioner powered by an electromagnetic actuator, designed for performing angular micromovements within a range of few microradians. The principle of operation is based on balancing the electromagnetic torque of the motor with a torque that is twisting a compliant element. As electrodynamic actuators have no distinguished controlled positions, therefore in typical positioning systems desired positions are obtained applying a closed-loop position control. Usually, such systems employ also a feedback (dumping related to velocity of the moving elements, what simplifies forming of dynamics of the system. The design of the physical model employs a DC micromotor, whose rotor is coupled with a torsional torquemeter. A feedback signal is generated by resistive strain gauges. The paper presents a mathematical model of the positioning system, results of simulation study as well as results of experimental study. The simulation study indicates that it is possible to select such design features and such type of the micoromotor that a high dynamics of positioning is ensured.

  11. Practical scaling law for photoelectron angular distributions

    International Nuclear Information System (INIS)

    Guo Dongsheng; Zhang Jingtao; Xu Zhizhan; Li Xiaofeng; Fu Panming; Freeman, R.R.

    2003-01-01

    A practical scaling law that predicts photoelectron angular distributions (PADs) is derived using angular distribution formulas which explicitly contain spontaneous emission. The scaling law is used to analyze recent PAD measurements in above-threshold ionization, and to predict results of future experiments. Our theoretical and numerical studies show that, in the non-relativistic regime and long-wavelength approximation, the shapes of PADs are determined by only three dimensionless numbers: (1) u p ≡U p /(ℎ/2π)ω, the ponderomotive number (ponderomotive energy in units of laser photon energy); (2) ε b ≡E b /(ℎ/2π)ω, the binding number (atomic binding energy in units of the laser photon energy); (3) j, the absorbed-photon number. The scaling law is shown to be useful in predictions of results from strong-field Kapitza-Dirac effect measurements; specifically, the application of this scaling law to recently reported Kapitza-Dirac diffraction is discussed. Possible experimental tests to verify the scaling law are suggested

  12. Orbital angular momentum of general astigmatic modes

    International Nuclear Information System (INIS)

    Visser, Jorrit; Nienhuis, Gerard

    2004-01-01

    We present an operator method to obtain complete sets of astigmatic Gaussian solutions of the paraxial wave equation. In case of general astigmatism, the astigmatic intensity and phase distribution of the fundamental mode differ in orientation. As a consequence, the fundamental mode has a nonzero orbital angular momentum, which is not due to phase singularities. Analogous to the operator method for the quantum harmonic oscillator, the corresponding astigmatic higher-order modes are obtained by repeated application of raising operators on the fundamental mode. The nature of the higher-order modes is characterized by a point on a sphere, in analogy with the representation of polarization on the Poincare sphere. The north and south poles represent astigmatic Laguerre-Gaussian modes, similar to circular polarization on the Poincare sphere, while astigmatic Hermite-Gaussian modes are associated with points on the equator, analogous to linear polarization. We discuss the propagation properties of the modes and their orbital angular momentum, which depends on the degree of astigmatism and on the location of the point on the sphere

  13. [Sensitivity of four representative angular cephalometric measures].

    Science.gov (United States)

    Xü, T; Ahn, J; Baumrind, S

    2000-05-01

    Examined the sensitivity of four representative cephalometric angles to the detection of different vectors of craniofacial growth. Landmark coordinate data from a stratified random sample of 48 adolescent subjects were used to calculate conventional values for changes between the pretreatment and end-of-treatment lateral cephalograms. By modifying the end-of-treatment coordinate values appropriately, the angular changes could be recalculated reflecting three hypothetical situations: Case 1. What if there were no downward landmark displacement between timepoints? Case 2. What if there were no forward landmark displacement between timepoints? Case 3. What if there were no Nasion change? These questions were asked for four representative cephalometric angles: SNA, ANB, NAPg and UI-SN. For Case 1, the associations (r) between the baseline and the modified measure for the three angles were very highly significant (P < 0.001) with r2 values no lower than 0.94! For Case 2, however, the associations were much weaker and no r value reached significance. These angular measurements are less sensitive for measuring downward landmark displacement than they are for measuring forward landmark displacement.

  14. Critique of the angular momentum sum rules and a new angular momentum sum rule

    NARCIS (Netherlands)

    Bakker, B.L.G.; Leader, E.; Trueman, T. L.

    2004-01-01

    We present a study of the tensorial structure of the hadronic matrix elements of the angular momentum operators J. Well known results in the literature are shown to be incorrect, and we have taken pains to derive the correct expressions in three different ways, two involving explicit physical wave

  15. Inefficient Angular Momentum Transport in Accretion Disk Boundary Layers: Angular Momentum Belt in the Boundary Layer

    Science.gov (United States)

    Belyaev, Mikhail A.; Quataert, Eliot

    2018-04-01

    We present unstratified 3D MHD simulations of an accretion disk with a boundary layer (BL) that have a duration ˜1000 orbital periods at the inner radius of the accretion disk. We find the surprising result that angular momentum piles up in the boundary layer, which results in a rapidly rotating belt of accreted material at the surface of the star. The angular momentum stored in this belt increases monotonically in time, which implies that angular momentum transport mechanisms in the BL are inefficient and do not couple the accretion disk to the star. This is in spite of the fact that magnetic fields are advected into the BL from the disk and supersonic shear instabilities in the BL excite acoustic waves. In our simulations, these waves only carry a small fraction (˜10%) of the angular momentum required for steady state accretion. Using analytical theory and 2D viscous simulations in the R - ϕ plane, we derive an analytical criterion for belt formation to occur in the BL in terms of the ratio of the viscosity in the accretion disk to the viscosity in the BL. Our MHD simulations have a dimensionless viscosity (α) in the BL that is at least a factor of ˜100 smaller than that in the disk. We discuss the implications of these results for BL dynamics and emission.

  16. Photoemission spectroscopy of the charge-ordering transition in Pr0.5Sr0.5MnO3

    International Nuclear Information System (INIS)

    Chainani, A.; Kumigashira, H.; Takahashi, T.; Tomioka, Y.; Kuwahara, H.; Tokura, Y.

    1996-01-01

    In this paper, the electronic structure of the magnetite Pr 0.5 Sr 0.5 MnO 3 across the charge ordering transition is studied using temperature-dependent photoemission spectroscopy. Ultra-violet photoemission spectroscopy have been performed as a function of temperature (25-300K) to investigate the changes in the single-particle density of states across the metal-nonmetal and the para-ferro transitions

  17. An EM Induction Hi-Speed Rotation Angular Rate Sensor.

    Science.gov (United States)

    Li, Kai; Li, Yuan; Han, Yan

    2017-03-17

    A hi-speed rotation angular rate sensor based on an electromagnetic induction signal is proposed to provide a possibility of wide range measurement of high angular rates. An angular rate sensor is designed that works on the principle of electromagnetism (EM) induction. In addition to a zero-phase detection technique, this sensor uses the feedback principle of magnetic induction coils in response to a rotating magnetic field. It solves the challenge of designing an angular rate sensor that is suitable for both low and high rotating rates. The sensor was examined for angular rate measurement accuracy in simulation tests using a rotary table. The results show that it is capable of measuring angular rates ranging from 1 rps to 100 rps, with an error within 1.8‰ of the full scale (FS). The proposed sensor is suitable to measurement applications where the rotation angular rate is widely varied, and it contributes to design technology advancements of real-time sensors measuring angular acceleration, angular rate, and angular displacement of hi-speed rotary objects.

  18. An EM Induction Hi-Speed Rotation Angular Rate Sensor

    Directory of Open Access Journals (Sweden)

    Kai Li

    2017-03-01

    Full Text Available A hi-speed rotation angular rate sensor based on an electromagnetic induction signal is proposed to provide a possibility of wide range measurement of high angular rates. An angular rate sensor is designed that works on the principle of electromagnetism (EM induction. In addition to a zero-phase detection technique, this sensor uses the feedback principle of magnetic induction coils in response to a rotating magnetic field. It solves the challenge of designing an angular rate sensor that is suitable for both low and high rotating rates. The sensor was examined for angular rate measurement accuracy in simulation tests using a rotary table. The results show that it is capable of measuring angular rates ranging from 1 rps to 100 rps, with an error within 1.8‰ of the full scale (FS. The proposed sensor is suitable to measurement applications where the rotation angular rate is widely varied, and it contributes to design technology advancements of real-time sensors measuring angular acceleration, angular rate, and angular displacement of hi-speed rotary objects.

  19. Electronic states of solids probed by bulk-sensitive high-resolution soft X-ray photoemission spectroscopy

    CERN Document Server

    Sekiyama, A

    2003-01-01

    High-energy and high-resolution soft x-ray photoemission studies have been performed on strongly correlated Ce compounds and vanadium oxides at BL25SU of SPring-8. The bulk spectra of CeRu sub 2 are explained by a band-structure calculation (itinerant model) whereas the other Ce 4f spectra are well reproduced by calculations based on the single impurity Anderson model (model from a localized limit). In a strong contrast to so far reported results, the bulk spectral functions are revealed to be insensitive to x for Sr sub 1 sub - sub x Ca sub x VO sub 3. Our study has demonstrated the importance of high-energy and high-resolution photoemission spectroscopy for revealing detailed bulk electronic states of strongly correlated systems. (author)

  20. Calculation of fluctuations and photoemission properties in a tetrahedral-cluster model for an intermediate-valence system

    International Nuclear Information System (INIS)

    Reich, A.; Falicov, L.M.

    1986-01-01

    An exact solution of a four-site tetrahedral-crystal model, the smallest face-centered-cubic crystal, is presented in the case of an intermediate-valence system. The model consists of the following: (a) one extended orbital and one localized orbital per atom, (b) an interatomic transfer term between extended orbitals, (c) an interatomic hybridization between the localized and extended orbitals, (d) strong intra-atomic Coulomb repulsion between opposite-spin localized states, and (e) intermediate-strength intra-atomic Coulomb repulsion between the localized and extended states. These competing effects are examined as they manifest themselves in the intermediate-valence, photoemission, inverse-photoemission, and thermodynamic properties

  1. A hard x-ray spectrometer for high angular resolution observations of cosmic sources

    International Nuclear Information System (INIS)

    Hailey, C.J.; Ziock, K.P.; Harrison, F.; Kahn, S.M.; Liedahl, D.; Lubin, P.M.; Seiffert, M.

    1988-01-01

    LAXRIS (large area x-ray imaging spectrometer) is an experimental, balloon-borne, hard x-ray telescope that consists of a coaligned array of x-ray imaging spectrometer modules capable of obtaining high angular resolution (1--3 arcminutes) with moderate energy resolution in the 20- to 300-keV region. Each spectrometer module consists of a CsI(Na) crystal coupled to a position-sensitive phototube with a crossed-wire, resistive readout. Imaging is provided by a coded aperture mask with a 4-m focal length. The high angular resolution is coupled with rather large area (/approximately/800 cm 2 ) to provide good sensitivity. Results are presented on performance and overall design. Sensitivity estimates are derived from a Monte-Carlo code developed to model the LAXRIS response to background encountered at balloon altitudes. We discuss a variety of observations made feasible by high angular resolution. For instance, spatially resolving the nonthermal x-ray emission from clusters of galaxies is suggested as an ideal program for LAXRIS. 15 refs., 5 figs

  2. High angular resolution observations of star-forming regions with BETTII and SOFIA

    Science.gov (United States)

    Rizzo, Maxime; Rinehart, Stephen; Mundy, Lee G.; Benford, Dominic J.; Dhabal, Arnab; Fixsen, Dale J.; Leisawitz, David; Maher, Stephen F.; Mentzell, Eric; Silverberg, Robert F.; Staguhn, Johannes; Veach, Todd; Cardiff BETTII Team

    2016-01-01

    High angular resolution observations in the far-infrared are important to understand the star formation process in embedded star clusters where extinction is large and stars form in close proximity. The material taking part in the star forming process is heated by the young stars and emits primarily in the far-IR; hence observations of the far-IR dust emission yields vital information about the gravitational potential, the mass and energy distribution, and core/star formation process. Previous observatories, such as Herschel, Spitzer and WISE lack the angular resolution required to study these dense star forming cores and are further limited by saturation in bright cores.The Balloon Experimental Twin Telescope for Infrared Interferometry (BETTII) is pioneering the path to sub-arcsecond resolution at far-IR wavelengths. This thesis talk discusses the instrumental challenges in building BETTII, as well as results from our SOFIA survey to illustrate the potential of higher-angular resolution observations. The 8m-long two element interferometer is being tested at NASA GSFC and is scheduled for first flight in fall 2016. BETTII will provide 0.5 to 1 arcsecond spatial resolution and spectral resolving power of 10 to 100 between 30 and 90 microns, where most of the dust continuum emission peaks in local star forming regions. It will achieve spatially-resolved spectroscopy of bright, dense cores with unprecedented high definition. This talk focuses on the main challenges and solutions associated with building BETTII: thermal stability, attitude/pointing control, and path length stabilization. In each of these areas we look at the trade-off between design, control, and knowledge in order to achieve the best-possible instrumental capability and sensitivity.As a first step towards resolving cluster cores, we surveyed 10 nearby star-forming clusters with SOFIA FORCAST at 11, 19, 31 and 37 microns. The FORCAST instrument has the highest angular resolution currently available in

  3. Femto-second dynamics probed by resonant photoemission and coincidence techniques

    International Nuclear Information System (INIS)

    Miron, C.; Ceolin, D.; Morin, P.

    2004-01-01

    Full text: It is well known nowadays that inner-shell excitation induces very rich dynamics where nuclear motion and electronic decay compete on a very short time scale, like in the case of ultra-fast molecular dissociation. Since the st experimental evidence was given by P. Morin and I. Nenner in 1986 for HBr and until now, it was shown that it acted as a general phenomenon taking place in a large variety of molecular systems. A nice consequence of such a process was shown by Prof. Svensson's group in Sweden by resonant photoemission measurements of the decay of the O 1s → σ * core-excited state in O 2 : the Auger-Doppler effect. More recently, a Japanese group demonstrated that the Auger-Doppler effect may be employed as a probe of the Auger emission anisotropy. The present talk will mainly deal with the mechanisms of intra-molecular ultra-fast chemical reaction pathways induced by inner-shell excitation and probed by energy selected resonant Auger electron-ion coincidences (ES-RAEPICO) and resonant photoemission measurements. Such a reactive pathway could be revealed through the appearance of rearrangement products. The dynamics of such ultra-fast chemical reactions, if they occur, will be entirely governed by the competition between the nuclear motion in the core-excited state and electronic decay (Auger decay). Since the chemical reaction is able to occur only during the lifetime of the core-excited state, the Auger decay may be seen in this context as a chemical reaction inhibitor, which leads the excited system towards a different relaxation pathway. The measurement in coincidence of the kinetic energy of the ejected Auger electrons and of fragment ions is able to reveal in such a case the energetics and kinematics of the possible decay mechanisms. Moreover, the photon energy detuning with respect to the nominal core-excitation energy allows changing the energy of the reactants and influence the chemical dynamics on a femtosecond time scale

  4. Direct comparison of photoemission spectroscopy and in situ Kelvin probe work function measurements on indium tin oxide films

    International Nuclear Information System (INIS)

    Beerbom, M.M.; Laegel, B.; Cascio, A.J.; Doran, B.V.; Schlaf, R.

    2006-01-01

    The work function of commercially available indium tin oxide (ITO) films on glass substrates was measured using photoemission spectroscopy (PES) and ultra-high vacuum (UHV) Kelvin probe in direct comparison. Absolute Kelvin probe work function values were determined via calibration of the measured contact potential difference (CPD) using an in situ sputtered Au reference sample. The Kelvin probe data confirmed that ultraviolet photoemission spectroscopy (UPS) measurements change the work function of ITO surfaces previously exposed to ambient environment, when measured without in situ surface cleaning procedures. The results also demonstrate that both Kelvin probe and PES yield virtually identical work function values, as long as the Kelvin probe data are calibrated against a known standard. As a consequence, previously reported higher work function values determined with Kelvin probe as compared to values obtained with UPS on similar samples are likely related to a photochemically generated surface dipole during UPS measurements. Comparison between Kelvin probe and low intensity X-ray photoemission spectroscopy (LIXPS) work function measurements demonstrated that accurate work function measurements on ITO previously exposed to the ambient are possible with PES

  5. Inhomogeneous Broadening in Perturbed Angular Correlation Spectroscopy

    Science.gov (United States)

    Bunker, Austin; Adams, Mike; Hodges, Jeffery; Park, Tyler; Stufflebeam, Michael; Evenson, William; Matheson, Phil; Zacate, Matthew

    2009-10-01

    Our research concerns the effect of a static distribution of defects on the net electric field gradient (EFG) within crystal structures. Defects and vacancies perturb the distribution of gamma rays emitted from radioactive probe nuclei within the crystal. These defects and vacancies produce a net EFG at the site of the probe which causes the magnetic quadrupole moment of the nucleus of the probe to precess about the EFG. The net EFG, which is strongly dependent upon the defect concentration, perturbs the angular correlation (PAC) of the gamma rays, and is seen in the damping of the perturbation function, G2(t), in time and broadening of the spectral peaks in the Fourier transform. We have used computer simulations to study the probability distribution of EFG tensor components in order to uncover the concentration dependence of G2(t). This in turn can be used to analyze experimental PAC data and quantitatively describe properties of the crystal.

  6. Topological photonic orbital-angular-momentum switch

    Science.gov (United States)

    Luo, Xi-Wang; Zhang, Chuanwei; Guo, Guang-Can; Zhou, Zheng-Wei

    2018-04-01

    The large number of available orbital-angular-momentum (OAM) states of photons provides a unique resource for many important applications in quantum information and optical communications. However, conventional OAM switching devices usually rely on precise parameter control and are limited by slow switching rate and low efficiency. Here we propose a robust, fast, and efficient photonic OAM switch device based on a topological process, where photons are adiabatically pumped to a target OAM state on demand. Such topological OAM pumping can be realized through manipulating photons in a few degenerate main cavities and involves only a limited number of optical elements. A large change of OAM at ˜10q can be realized with only q degenerate main cavities and at most 5 q pumping cycles. The topological photonic OAM switch may become a powerful device for broad applications in many different fields and motivate a topological design of conventional optical devices.

  7. Coherent control of photoelectron wavepacket angular interferograms

    International Nuclear Information System (INIS)

    Hockett, P; Wollenhaupt, M; Baumert, T

    2015-01-01

    Coherent control over photoelectron wavepackets, via the use of polarization-shaped laser pulses, can be understood as a time and polarization-multiplexed process, where the final (time-integrated) observable coherently samples all instantaneous states of the light–matter interaction. In this work, we investigate this multiplexing via computation of the observable photoelectron angular interferograms resulting from multi-photon atomic ionization with polarization-shaped laser pulses. We consider the polarization sensitivity of both the instantaneous and cumulative continuum wavefunction; the nature of the coherent control over the resultant photoelectron interferogram is thus explored in detail. Based on this understanding, the use of coherent control with polarization-shaped pulses as a methodology for a highly multiplexed coherent quantum metrology is also investigated, and defined in terms of the information content of the observable. (paper)

  8. Coherent control of photoelectron wavepacket angular interferograms

    Science.gov (United States)

    Hockett, P.; Wollenhaupt, M.; Baumert, T.

    2015-11-01

    Coherent control over photoelectron wavepackets, via the use of polarization-shaped laser pulses, can be understood as a time and polarization-multiplexed process, where the final (time-integrated) observable coherently samples all instantaneous states of the light-matter interaction. In this work, we investigate this multiplexing via computation of the observable photoelectron angular interferograms resulting from multi-photon atomic ionization with polarization-shaped laser pulses. We consider the polarization sensitivity of both the instantaneous and cumulative continuum wavefunction; the nature of the coherent control over the resultant photoelectron interferogram is thus explored in detail. Based on this understanding, the use of coherent control with polarization-shaped pulses as a methodology for a highly multiplexed coherent quantum metrology is also investigated, and defined in terms of the information content of the observable.

  9. Angular filter refractometry analysis using simulated annealing.

    Science.gov (United States)

    Angland, P; Haberberger, D; Ivancic, S T; Froula, D H

    2017-10-01

    Angular filter refractometry (AFR) is a novel technique used to characterize the density profiles of laser-produced, long-scale-length plasmas [Haberberger et al., Phys. Plasmas 21, 056304 (2014)]. A new method of analysis for AFR images was developed using an annealing algorithm to iteratively converge upon a solution. A synthetic AFR image is constructed by a user-defined density profile described by eight parameters, and the algorithm systematically alters the parameters until the comparison is optimized. The optimization and statistical uncertainty calculation is based on the minimization of the χ 2 test statistic. The algorithm was successfully applied to experimental data of plasma expanding from a flat, laser-irradiated target, resulting in an average uncertainty in the density profile of 5%-20% in the region of interest.

  10. Nuclear scissors modes and hidden angular momenta

    Energy Technology Data Exchange (ETDEWEB)

    Balbutsev, E. B., E-mail: balbuts@theor.jinr.ru; Molodtsova, I. V. [Joint Institute for Nuclear Research (Russian Federation); Schuck, P. [Université Paris-Sud, Institut de Physique Nucléaire, IN2P3–CNRS (France)

    2017-01-15

    The coupled dynamics of low-lying modes and various giant resonances are studied with the help of the Wigner Function Moments method generalized to take into account spin degrees of freedom and pair correlations simultaneously. The method is based on Time-Dependent Hartree–Fock–Bogoliubov equations. The model of the harmonic oscillator including spin–orbit potential plus quadrupole–quadrupole and spin–spin interactions is considered. New low-lying spin-dependent modes are analyzed. Special attention is paid to the scissors modes. A new source of nuclear magnetism, connected with counter-rotation of spins up and down around the symmetry axis (hidden angular momenta), is discovered. Its inclusion into the theory allows one to improve substantially the agreement with experimental data in the description of energies and transition probabilities of scissors modes.

  11. Angular reduction in multiparticle matrix elements

    International Nuclear Information System (INIS)

    Lehman, D.R.; Parke, W.C.

    1989-01-01

    A general method for reduction of coupled spherical harmonic products is presented. When the total angular coupling is zero, the reduction leads to an explicitly real expression in the scalar products of the unit vector arguments of the spherical harmonics. For nonscalar couplings, the reduction gives Cartesian tensor forms for the spherical harmonic products; tensors built from the physical vectors in the original expression. The reduction for arbitrary couplings is given in closed form, making it amenable to symbolic manipulation on a computer. The final expressions do not depend on a special choice of coordinate axes, nor do they contain azimuthal quantum number summations, or do they have complex tensor terms for couplings to a scalar; consequently, they are easily interpretable from the properties of the physical vectors they contain

  12. Chiral symmetries associated with angular momentum

    International Nuclear Information System (INIS)

    Bhattacharya, M; Kleinert, M

    2014-01-01

    In quantum mechanics courses, symmetries of a physical system are usually introduced as operators which commute with the Hamiltonian. In this paper we will consider chiral symmetries which anticommute with the Hamiltonian. Typically, introductory courses at the (under)graduate level do not discuss these simple, useful and beautiful symmetries at all. The first time a student encounters them is when the Dirac equation is discussed in a course on relativistic quantum mechanics, or when particle–hole symmetry is studied in the context of superconductivity. In this paper, we will show how chiral symmetries can be simply elucidated using the theory of angular momentum, which is taught in virtually all introductory quantum mechanics courses. (paper)

  13. Cierre angular primario: opciones quirúrgicas

    Directory of Open Access Journals (Sweden)

    Henry Pérez-González

    2014-10-01

    Full Text Available Se realizó una revisión bibliográfica con el objetivo de exponer las principales opciones quirúrgicas en el tratamiento del cierre angular primario efectuando una búsqueda de los principales artículos científicos de los últimos años, así como de la literatura impresa que incluye el tema, siendo seleccionados los contenidos más relevantes para la confección del informe final. Las opciones de tratamiento incluyen la cirugía láser (iridotomía, iridoplastia y la cirugía incisional (filtrante, extracción del cristalino, dependiendo de los factores fisiopatológicos involucrados y la forma clínica en el momento del diagnóstico.

  14. Untangling Galaxy Components - The Angular Momentum Parameter

    Science.gov (United States)

    Tabor, Martha; Merrifield, Michael; Aragon-Salamanca, Alfonso

    2017-06-01

    We have developed a new technique to decompose Integral Field spectral data cubes into separate bulge and disk components, allowing us to study the kinematic and stellar population properties of the individual components and how they vary with position. We present here the application of this method to a sample of fast rotator early type galaxies from the MaNGA integral field survey, and demonstrate how it can be used to explore key properties of the individual components. By extracting ages, metallicities and the angular momentum parameter lambda of the bulges and disks, we show how this method can give us new insights into the underlying structure of the galaxies and discuss what this can tell us about their evolution history.

  15. Angular biasing in implicit Monte-Carlo

    International Nuclear Information System (INIS)

    Zimmerman, G.B.

    1994-01-01

    Calculations of indirect drive Inertial Confinement Fusion target experiments require an integrated approach in which laser irradiation and radiation transport in the hohlraum are solved simultaneously with the symmetry, implosion and burn of the fuel capsule. The Implicit Monte Carlo method has proved to be a valuable tool for the two dimensional radiation transport within the hohlraum, but the impact of statistical noise on the symmetric implosion of the small fuel capsule is difficult to overcome. We present an angular biasing technique in which an increased number of low weight photons are directed at the imploding capsule. For typical parameters this reduces the required computer time for an integrated calculation by a factor of 10. An additional factor of 5 can also be achieved by directing even smaller weight photons at the polar regions of the capsule where small mass zones are most sensitive to statistical noise

  16. Angular Position Tracking Control of a Quadcopter

    Directory of Open Access Journals (Sweden)

    T. V. Glazkov

    2017-01-01

    Full Text Available The paper dwells on tracking the quad-copter angular position with desired quality parameters of transient processes. The aerial vehicle is considered as a rigid body with six degrees of freedom.  A full rigid body quad-copter mathematical model is considered without the assumption of smallness of the Euler angles.Among the most well known methods of non-linear stabilization are feedback linearization and backstepping. The backstepping approach allows us to have an effective solution of the stabilization problems with uncertainties available in the system. However, in synthesis of the feedback through backstepping, there is still an urgent issue: how to ensure desirable quality of transients in the closed-loop system. The paper presents a solution of this problem using as an example the tracking a given (programmed change of the angular position of a quad-copter.The control algorithms obtained in this paper are implemented using the Rolling Spider MATLAB Toolbox (ROSMAT tool package on the Parrot Rolling Spider quad-copter. A numerical simulation and experiments have shown the efficiency of obtained control laws, with the transient processes taking into account the desired quality indicators. However, the experiments showed that lack of terms in the mathematical model to describe the aerodynamic effects, resulted in the instability of the quad-copter flight near the obstacle (the effect of the reflected airflow.Further research can be aimed at solving the control problem in question using a mathematical model of the quad-copter motion that takes into account various aerodynamic effects.One of the potential application areas for the theoretical results, obtained in the paper, is to solve the problems of automatic control of unmanned aerial vehicles.

  17. SiO mass spectrometry and Si-2p photoemission spectroscopy for the study of oxidation reaction dynamics of Si(001) surface by supersonic O sub 2 molecular beams under 1000K

    CERN Document Server

    Teraoka, Y; Moritani, K

    2003-01-01

    The Si sup 1 sup 8 O desorption yield was measured in the Si(001) surface temperature region from 900K to 1300K at the sup 1 sup 8 O sub 2 incident energies of 0.7eV, 2.2eV and 3.3eV. The Si sup 1 sup 8 O desorption yield in a surface temperature region higher than 1000K increased with increasing incident energy, indicating the incident-energy-induced oxidation and the variation of angular distribution of Si sup 1 sup 8 O desorption. Inversely, the Si sup 1 sup 8 O desorption yield decreased with increasing incident energy in the region from 900K to 1000K, indicating the coexistence of the passive and the active oxidation. In order to clarify the reaction mechanisms of the later phenomenon, real-time in-situ Si-2p photoemission spectroscopy has been performed. The obtained Si-2p spectra showed the variation of the oxide-nuclei quality from the sub-oxide-rich structure to the SiO sub 2 -rich structure. The formation of the SiO sub 2 structure suppresses the SiO desorption due to the enhanced O sub 2 sticking a...

  18. Tuning the electronic structure of bulk FeSe with chemical pressure using quantum oscillations and angle resolved photoemission spectroscopy (ARPES)

    Science.gov (United States)

    Coldea, Amalia

    FeSe is a unique and intriguing superconductor which can be tuned into a high temperature superconducting state using applied pressure, chemical intercalation and surface doping. In the absence of magnetism, the structural transition in FeSe is believed to be electronically driven, with the orbital degrees of freedom playing an important part. This scenario supports the stabilization of a nematic state in FeSe, which manifests as a Fermi surface deformation in the presence of strong interactions, as detected by ARPES. Another manifestation of the nematicity is the enhanced nematic susceptibility determined from elastoresistance measurements under applied strain. Isovalent Sulphur substitution onto the Selenium site constitutes a chemical pressure, which subtly modifies the electronic structure of FeSe, suppressing the structural transition without inducing high temperature superconductivity. I will present the evolution of the electronic structure with chemical pressure in FeSe, as determined from quantum oscillations and ARPES studies and I will discuss the suppression of the nematic electronic state and the role of electronic correlations. Experiments were performed at high magnetic field facilities in Tallahassee, Nijmegen and Toulouse and Diamond Light Source, UK. This work is mainly supported by EPSRC, UK (EP/I004475/1, EP/I017836/1) and I acknowledge my collaborators from Refs. .

  19. Time-resolved imaging of purely valence-electron dynamics during a chemical reaction

    DEFF Research Database (Denmark)

    Hockett, Paul; Bisgaard, Christer Z.; Clarkin, Owen J.

    2011-01-01

    Chemical reactions are manifestations of the dynamics of molecular valence electrons and their couplings to atomic motions. Emerging methods in attosecond science can probe purely electronic dynamics in atomic and molecular systems(1-6). By contrast, time-resolved structural-dynamics methods......,17): in both cases, this sensitivity derives from the ionization-matrix element(18,19). Here we demonstrate a time-resolved molecular-frame photoelectron-angular-distribution (TRMFPAD) method for imaging the purely valence-electron dynamics during a chemical reaction. Specifically, the TRMFPADs measured during...

  20. A study of Al/Si interface by photoemission, Auger electron yield and Auger electron spectroscopies

    International Nuclear Information System (INIS)

    Kobayashi, K.L.I.; Barth, J.; Gerken, F.; Kunz, C.; Deutsches Elektronen-Synchrotron

    1980-06-01

    Photoemission, Auger electron yield and Auger electron spectra were observed for Al/Si(111) interfaces with various Al coverage prepared by successive deposition using a molecular beam source. The Al 3p derived states are introduced at around the top of the valence band by the Al coverage of less than one monolayer. The Al surface layer behaves as a 'metal' and the Fermi level is stabilized in the Al 3p derived states at about 0.3 eV above the top of the valence band of Si. The Schottky barrier height in this stage is about 0.8 eV and further increase in Al coverage does not change the barrier height. A covalent bonding model of the Al/Si interface based on the experimental results is proposed. The present result favors the on-top geometry of Al atoms on Si(111) surface among the geometries used in the pseudopotential calculation by Zhang and Schlueter. (orig.)

  1. Surface photovoltage investigation of gold chains on Si(111) by two-photon photoemission

    Energy Technology Data Exchange (ETDEWEB)

    Otto, Sebastian; Biedermann, Kerstin; Fauster, Thomas [Lehrstuhl fuer Festkoerperphysik, Universitaet Erlangen-Nuernberg, Staudtstr. 7, D-91058 Erlangen (Germany)

    2011-07-01

    We present surface photovoltage measurements on Si(111)-(7 x 7) with monoatomic gold chains. The gold coverage was varied between zero and 0.6 ML, where the Si(111)-(5 x 2)-Au reconstruction covers the surface completely. During the two-photon photoemission experiments the p- or n-doped samples were illuminated by infrared (IR, E{sub IR}=1.55 eV) and ultraviolet (UV, E{sub UV}=4.65 eV) laser pulses. For all coverages the photovoltage was determined for sample temperatures of 90 K and 300 K by variation of the IR and UV laser power. P-doped as well as n-doped Si(111) wafers show a linear dependence of the photovoltage on gold coverage. This stands in contrast to scanning tunneling spectroscopy measurements, which show a coverage-independent photovoltage over a wide coverage range for n-doped wafers. While for p-doped wafers our experimentally determined photovoltage is in agreement with previous reports, for n-doped wafers the observed values are lower than expected.

  2. Metal-organic semiconductor interfacial barrier height determination from internal photoemission signal in spectral response measurements

    Science.gov (United States)

    Kumar, Sandeep; Iyer, S. Sundar Kumar

    2017-04-01

    Accurate and convenient evaluation methods of the interfacial barrier ϕb for charge carriers in metal semiconductor (MS) junctions are important for designing and building better opto-electronic devices. This becomes more critical for organic semiconductor devices where a plethora of molecules are in use and standardised models applicable to myriads of material combinations for the different devices may have limited applicability. In this paper, internal photoemission (IPE) from spectral response (SR) in the ultra-violet to near infra-red range of different MS junctions of metal-organic semiconductor-metal (MSM) test structures is used to determine more realistic MS ϕb values. The representative organic semiconductor considered is [6, 6]-phenyl C61 butyric acid methyl ester, and the metals considered are Al and Au. The IPE signals in the SR measurement of the MSM device are identified and separated before it is analysed to estimate ϕb for the MS junction. The analysis of IPE signals under different bias conditions allows the evaluation of ϕb for both the front and back junctions, as well as for symmetric MSM devices.

  3. X-ray photoemission electron microscopy for the study of semiconductor materials

    International Nuclear Information System (INIS)

    Anders, Simone; Stammler, Thomas; Padmore, Howard A.; Terminello, Louis J.; Jankowski, Alan F.; Stoehr, Joachim; Diaz, Javier; Cossy-Favre, Aline; Singh, Sangeet

    1998-01-01

    Photoemission Electron Microscopy using X-rays (X-PEEM) is a novel combination of two established materials analysis techniques--PEEM using UV light, and Near Edge X-ray Absorption Fine Structure (NEXAFS) spectroscopy. This combination allows the study of elemental composition and bonding structure of the sample by NEXAFS spectroscopy with a high spatial resolution given by the microscope. A simple, two lens, 10 kV operation voltage PEEM has been used at the Stanford Synchrotron Radiation Laboratory and at the Advanced Light Source (ALS) in Berkeley to study various problems including materials of interest for the semiconductor industry. In the present paper we give a short overview over the method and the instrument which was used, and describe in detail a number of applications. These applications include the study of the different phases of titanium disilicide, various phases of boron nitride, and the analysis of small particles. A brief outlook is given on possible new fields of application of the PEEM technique, and the development of new PEEM instruments

  4. X-ray photoemission electron microscopy for the study of semiconductor materials

    Energy Technology Data Exchange (ETDEWEB)

    Anders, S.; Stammler, T.; Padmore, H. [Lawrence Berkeley National Lab., CA (United States). Advanced Light Source Div.; Terminello, L.J.; Jankowski, A.F. [Lawrence Livermore National Lab., CA (United States); Stohr, J. [IBM Almaden Research Center, San Jose, CA (United States); Diaz, J. [Univ. de Oviedo (Spain). Dept. de Fisica; Cossy-Gantner, A. [EMPA, Duebendorf (Germany)

    1998-03-01

    Photoemission Electron Microscopy (PEEM) using X-rays is a novel combination of two established materials analysis techniques--PEEM using UV light, and Near Edge X-ray Absorption Fine Structure (NEXAFS) spectroscopy. This combination allows the study of elemental composition and bonding structure of the sample by NEXAFS spectroscopy with a high spatial resolution given by the microscope. A simple, two lens, 10 kV operation voltage PEEM has been used at the Stanford Synchrotron Radiation Laboratory and at the Advanced Light Source (ALS) in Berkeley to study various problems including materials of interest for the semiconductor industry. In the present paper the authors give a short overview over the method and the instrument which was used, and describe in detail a number of applications. These applications include the study of the different phases of titanium disilicide, various phases of boron nitride, and the analysis of small particles. A brief outlook is given on possible new fields of application of the PEEM technique, and the development of new PEEM instruments.

  5. X-ray photoemission electron microscopy for the study of semiconductor materials

    Energy Technology Data Exchange (ETDEWEB)

    Anders, S.; Stammler, T.; Padmore, H.A. [Lawrence Berkeley National Laboratory, 1 Cyclotron Road, Berkeley, California 94720 (United States); Terminello, L.J.; Jankowski, A.F. [Lawrence Livermore National Laboratory, 7000 East Ave., Livermore, California 94550 (United States); Stoehr, J. [IBM Almaden Research Center, 650 Harry Road, San Jose, California 95120 (United States); Diaz, J. [Departamento de Fisic, Facultad de Ciencias, Universidad de Oviedo, Avda. Calvo Sotelo s/n, Oviedo, 33007 (Spain); Cossy-Favre, A. [EMPA, Duebendorf, Ueberlandstrasse 129, 8600 Duebendorf (Switzerland); Singh, S. [Center for X-ray Lithography, University of Wisconsin-Madison, Stoughton, Wisconsin 53589 (United States)

    1998-11-01

    Photoemission Electron Microscopy using X-rays (X-PEEM) is a novel combination of two established materials analysis techniques{emdash}PEEM using UV light, and Near Edge X-ray Absorption Fine Structure (NEXAFS) spectroscopy. This combination allows the study of elemental composition and bonding structure of the sample by NEXAFS spectroscopy with a high spatial resolution given by the microscope. A simple, two lens, 10 kV operation voltage PEEM has been used at the Stanford Synchrotron Radiation Laboratory and at the Advanced Light Source (ALS) in Berkeley to study various problems including materials of interest for the semiconductor industry. In the present paper we give a short overview over the method and the instrument which was used, and describe in detail a number of applications. These applications include the study of the different phases of titanium disilicide, various phases of boron nitride, and the analysis of small particles. A brief outlook is given on possible new fields of application of the PEEM technique, and the development of new PEEM instruments. {copyright} {ital 1998 American Institute of Physics.}

  6. Oxide effects on photoemission from high current GaAs photocathodes

    International Nuclear Information System (INIS)

    Garwin, E.L.; Kirby, R.E.; Sinclair, C.K.; Roder, A.

    1981-03-01

    During four years of on line operation of the SLAC polarized electron gun (PEGGY) and polarized LEED (PLEED) system, we have observed and characterized the failure modes of the GaAs (100) photocathodes (PC's) used in these systems. Several modes are observed. Gradual decreases in electron polarization and intensity are attributed to the physisorption of CO 2 on the PC's during running at LN 2 temperatures. Such PC's can be rejuvenated by warming to 90K, i.e., above the CO 2 desorption temperature. These PC's recover 90% of their original intensity. A second well-characterized failure mode results from overheating the PC during in-situ heat cleaning prior to activation. In this mode, As is preferentially evaporated from the GaAs, leaving a Ga 2 O 3 layer on the surface. This effect has been studied by AES sputter profiling which indicates that the substantial thickness of the oxide layer blocks photoemission. These PC's may only be recovered by chemically removing the oxide layer. A third mode which is not as well characterized appears for thin Ga oxide layers. Properties of these PC's include reduced emission and the presence of a cutoff bias level. Such PC's are also not recoverable in-situ

  7. Spectral phase shift and residual angular dispersion of an accousto-optic programme dispersive filter

    International Nuclear Information System (INIS)

    Boerzsoenyi, A.; Meroe, M.

    2010-01-01

    Complete text of publication follows. There is an increasing demand for active and precise dispersion control of ultrashort laser pulses. In chirped pulse amplification (CPA) laser systems, the dispersion of the optical elements of the laser has to be compensated at least to the fourth order to obtain high temporal contrast compressed pulses. Nowadays the most convenient device for active and programmable control of spectral phase and amplitude of broadband laser pulses is the acousto-optic programmable dispersive filter (AOPDF), claimed to be able to adjust the spectral phase up to the fourth order. Although it has been widely used, surprisingly enough there has been only a single, low resolution measurement reported on the accuracy of the induced spectral phase shift of the device. In our paper we report on the first systematic experiment aiming at the precise characterization of an AOPDF device. In the experiment the spectral phase shift of the AOPDF device was measured by spectrally and spatially resolved interferometry, which is especially powerful tool to determine small dispersion values with high accuracy. Besides the spectral phase dispersion, we measured both the propagation direction angular dispersion (PDAD) and the phase front angular dispersion (PhFAD). Although the two quantities are equal for plane waves, there may be noticeable difference for Gaussian pulses. PDAD was determined simply by focusing the beam on the slit of an imaging spectrograph, while PhFAD was measured by the use of an inverted Mach-Zehnder interferometer and an imaging spectrograph. In the measurements, the spectral phase shift and both types of angular dispersion have been recorded upon the systematic change of all the accessible functions of the acousto-optic programmable dispersive filter. The measured values of group delay dispersion (GDD) and third order dispersion (TOD) have been found to agree with the preset values within the error of the measurement (1 fs 2 and 10 fs 3

  8. Mapping unoccupied electronic states of freestanding graphene by angle-resolved low-energy electron transmission

    OpenAIRE

    Wicki Flavio; Longchamp Jean-Nicolas; Latychevskaia Tatiana; Escher Conrad; Fink Hans-Werner

    2016-01-01

    We report angle-resolved electron transmission measurements through freestanding graphene sheets in the energy range of 18 to 30 eV above the Fermi level. The measurements are carried out in a low-energy electron point source microscope, which allows simultaneously probing the transmission for a large angular range. The characteristics of low-energy electron transmission through graphene depend on its electronic structure above the vacuum level. The experimental technique described here allow...

  9. Super-resolved refocusing with a plenoptic camera

    Science.gov (United States)

    Zhou, Zhiliang; Yuan, Yan; Bin, Xiangli; Qian, Lulu

    2011-03-01

    This paper presents an approach to enhance the resolution of refocused images by super resolution methods. In plenoptic imaging, we demonstrate that the raw sensor image can be divided to a number of low-resolution angular images with sub-pixel shifts between each other. The sub-pixel shift, which defines the super-resolving ability, is mathematically derived by considering the plenoptic camera as equivalent camera arrays. We implement simulation to demonstrate the imaging process of a plenoptic camera. A high-resolution image is then reconstructed using maximum a posteriori (MAP) super resolution algorithms. Without other degradation effects in simulation, the super resolved image achieves a resolution as high as predicted by the proposed model. We also build an experimental setup to acquire light fields. With traditional refocusing methods, the image is rendered at a rather low resolution. In contrast, we implement the super-resolved refocusing methods and recover an image with more spatial details. To evaluate the performance of the proposed method, we finally compare the reconstructed images using image quality metrics like peak signal to noise ratio (PSNR).

  10. Angular correlations between recoil velocity and angular momentum vectors in molecular photodissociation

    Science.gov (United States)

    Hall, G. E.; Sivakumar, N.; Chawla, D.; Houston, P. L.; Burak, I.

    1988-03-01

    A technique has been developed for determining the angular correlation between a photofragment's angular momentum vector J, its recoil velocity vector v, and the transition dipole moment of the parent molecule μp . Doppler profile spectroscopy used in conjunction with laser-induced fluorescence probing by polarized light can be used to determine the correlations. The pairwise correlations between these vectors as well as their triple correlation are discussed for limiting cases using a classical approach as well as for the general case using a quantum approach based on density matrices. The current formulations differ in two ways from the recent approach of Dixon, who used a bipolar expansion of the correlated velocity and angular momentum distributions. The physical basis for the influence of the vector correlations on the Doppler profile is somewhat more transparent in the current formulations, and the direct connection between the measured correlations and the t-matrix elements occurring in the theory of Balint-Kurti and Shapiro for the photodissociation of a triatomic molecule is also demonstrated.

  11. Multichannel spin polarimeter for energy- and angle-dispersive photoemission measurements; Vielkanal-Spinpolarimeter fuer energie- und winkeldispersive Photoemissionsmessungen

    Energy Technology Data Exchange (ETDEWEB)

    Kolbe, Michaela

    2011-09-09

    Spin polarization measurements of free electrons remain challenging since their first realization by Mott. The relevant quantity of a spin polarimeter is its figure of merit, FoM=S{sup 2}I/I{sub 0}, with the asymmetry function S and the ratio between scattered and primary intensity I/I{sub 0}. State-of-the-art devices are based on single-channel scattering (spin-orbit or exchange interaction) which is characterized by FoM {approx_equal}10{sup -4}. On the other hand, modern hemispherical analyzers feature an efficient multichannel detection of spin-integral intensity with more than 10{sup 4} data points simultaneously. In comparison between spin-resolved and spin-integral electron spectroscopy we are thus faced with a difference in counting efficiency by 8 orders of magnitude. The present work concentrates on the development and investigation of a novel technique for increasing the efficiency in spin-resolved electron spectroscopy by multichannel detection. The spin detector was integrated in a {mu}-metal shielded UHV-chamber and mounted behind a conventional hemispherical analyzer. The electrostatic lens system's geometry was determined by electron-optical simulations. The basic concept is the k {sub parallel} -conserving elastic scattering of the (0,0)-beam on a W(100) scattering crystal under 45 impact angle. It could be demonstrated that app. 960 data points (15 energy and 64 angular points) could be displayed simultaneously on a delayline detector in an energy interval of {approx_equal}3 eV. This leads to a two-dimensional figure of merit of FoM{sub 2D}=1.7. Compared to conventional spin detectors, the new type is thus characterized by a gain in efficiency of 4 orders of magnitude. The operational reliability of the new spin polarimeter could be proven by measurements with a Fe/MgO(100) and O p(1 x 1)/Fe(100)-sample, where results from the literature were reproduced with strongly decreased measuring time. Due to the high intensity it becomes possible, to

  12. Resolved Hapke parameter maps of the Moon

    Science.gov (United States)

    Sato, H.; Robinson, M. S.; Hapke, B.; Denevi, B. W.; Boyd, A. K.

    2014-08-01

    We derived spatially resolved near-global Hapke photometric parameter maps of the Moon from 21 months of Lunar Reconnaissance Orbiter Camera (LROC) Wide Angle Camera (WAC) multispectral observations using a novel "tile-by-tile method" (1° latitude by 1° longitude bins). The derived six parameters (w,b,c,BS0,hS, andθ¯p) for each tile were used to normalize the observed reflectance (standard angles i = g = 60°, e = 0° instead of the traditional angles i = g = 30°, e = 0°) within each tile, resulting in accurate normalization optimized for the local photometric response. Each pixel in the seven-color near-global mosaic (70°S to 70°N and 0°E to 360°E) was computed by the median of normalized reflectance from large numbers of repeated observations (UV: ˜50 and visible: ˜126 on average). The derived mosaic exhibits no significant artifacts with latitude or along the tile boundaries, demonstrating the quality of the normalization procedure. The derived Hapke parameter maps reveal regional photometric response variations across the lunar surface. The b, c (Henyey-Greenstein double-lobed phase function parameters) maps demonstrate decreased backscattering in the maria relative to the highlands (except 321 nm band), probably due to the higher content of both SMFe (submicron iron) and ilmenite in the interiors of back scattering agglutinates in the maria. The hS (angular width of shadow hiding opposition effect) map exhibits relatively lower values in the maria than the highlands and slightly higher values for immature highland crater ejecta, possibly related to the variation in a grain size distribution of regolith.

  13. Enforcement actions: Significant actions resolved

    International Nuclear Information System (INIS)

    1989-06-01

    This compilation summarizes significant enforcement actions that have been resolved during one quarterly period (January--March 1989) and includes copies of letters, Notices, and Orders sent by the Nuclear Regulatory Commission to licensees with respect to these enforcement actions. Also included are a number of enforcement actions that had been previously resolved but not published in this NUREG. It is anticipated that the information in this publication will be widely disseminated to managers and employees engaged in activities licensed by the NRC, so that actions can be taken to improve safety by avoiding future violations similar to those described in this publication

  14. Enforcement actions: Significant actions resolved

    International Nuclear Information System (INIS)

    1990-05-01

    This compilation summarizes significant enforcement actions that have been resolved during one quarterly period (January--March 1990) and includes copies of letters, Notices, and Orders sent by the Nuclear Regulatory Commission to licensees with respect to these enforcement actions. Also included are a number of enforcement actions that had been previously resolved but not published in this NUREG. It is anticipated that the information in this publication will be widely disseminated to managers and employees engaged in activities licensed by the NRC, so that actions can be taken to improve safety by avoiding future violations similar to those described in this publication

  15. Direct observation of temperature-driven magnetic symmetry transitions by vectorial resolved MOKE magnetometry.

    Science.gov (United States)

    Luis F Cuñado, Jose; Pedrosa, Javier; Ajejas, Fernando; Perna, Paolo; Miranda, Rodolfo; Camarero, Julio

    2017-10-11

    Angle- and temperature-dependent vectorial magnetometry measurements are necessary to disentangle the effective magnetic symmetry in magnetic nanostructures. Here we present a detailed study on an Fe(1 0 0) thin film system with competing collinear biaxial (four-fold symmetry) and uniaxial (two-fold) magnetic anisotropies, carried out with our recently developed full angular/broad temperature range/vectorial-resolved magneto-optical Kerr effect magnetometer, named TRISTAN. The data give direct views on the angular and temperature dependence of the magnetization reversal pathways, from which characteristic axes, remanences, critical fields, domain wall types, and effective magnetic symmetry are obtained. In particular, although the remanence shows four-fold angular symmetry for all investigated temperatures (15 K-400 K), the critical fields show strong temperature and angular dependencies and the reversal mechanism changes for specific angles at a given (angle-dependent) critical temperature, showing signatures of an additional collinear two-fold symmetry. This symmetry-breaking is more relevant as temperature increases to room temperature. It originates from the competition between two anisotropy contributions with different symmetry and temperature evolution. The results highlight the importance of combining temperature and angular studies, and the need to look at different magnetic parameters to unravel the underlying magnetic symmetries and temperature evolutions of the symmetry-breaking effects in magnetic nanostructures.

  16. Inheritance of resistance to angular leaf spot in yellow beans ...

    African Journals Online (AJOL)

    Angular leaf spot (Phaeoisariopsis griseola (Sacc) is an important disease of common bean (Phaseolus vulgaris L.) in most parts of Africa, causing yield losses of 40-80%. This study was carried out to determine the inheritance of resistance to angular leaf spot in yellow beans. Biparental crosses were done between ...

  17. Prospects of Measuring the Angular Power Spectrum of the Diffuse ...

    Indian Academy of Sciences (India)

    Review. J. Astrophys. Astr. (2016) 37: 35. DOI: 10.1007/s12036-016-9413-x. Prospects of Measuring the Angular Power Spectrum of the Diffuse. Galactic .... In this section we briefly review the Tapered Gridded Estimator (TGE), the details ... of the product of the primary beam pattern A(θ) and δI(θ) the angular fluctuation.

  18. Measuring Average Angular Velocity with a Smartphone Magnetic Field Sensor

    Science.gov (United States)

    Pili, Unofre; Violanda, Renante

    2018-01-01

    The angular velocity of a spinning object is, by standard, measured using a device called a tachometer. However, by directly using it in a classroom setting, the activity is likely to appear as less instructive and less engaging. Indeed, some alternative classroom-suitable methods for measuring angular velocity have been presented. In this paper,…

  19. A kinematic model for calculating the magnitude of angular ...

    African Journals Online (AJOL)

    Keplerian velocity laws imply the existence of velocity shear and shear viscosity within an accretion disk. Due to this viscosity, angular momentum is transferred from the faster moving inner regions to the slower-moving outer regions of the disk. Here we have formulated a model for calculating the magnitude of angular ...

  20. Learning web development with Bootstrap and AngularJS

    CERN Document Server

    Radford, Stephen

    2015-01-01

    Whether you know a little about Bootstrap or AngularJS, or you're a complete beginner, this book will enhance your capabilities in both frameworks and you'll build a fully functional web app. A working knowledge of HTML, CSS, and JavaScript is required to fully get to grips with Bootstrap and AngularJS.

  1. 3D printed bio-inspired angular acceleration sensor

    NARCIS (Netherlands)

    van Tiem, Joël; Groenesteijn, Jarno; Sanders, Remco G.P.; Krijnen, Gijsbertus J.M.

    2015-01-01

    Abstract—We present a biomimetic angular acceleration sensor inspired by the vestibular system, as found e.g. in mammals and fish. The sensor consist of a fluid filled circular channel. When exposed to angular accelerations the fluid flows relative to the channel. Read-out is based on

  2. inheritance of resistance to angular leaf spot in yellow beans ...

    African Journals Online (AJOL)

    Prof. Adipala Ekwamu

    Susceptible. II -indeterminate erect; III -indeterminate semi-prostate; ALS = Angular leaf spot. Isolation of Phaeoisariopsis griseola and plant inoculation. Isolation of angular leaf spot was made from lesions of naturally infected bean leaves showing fungal sporulation. In the case of non-sporulating lesions, the fungus was.

  3. Angular sensitivity of blowfly photoreceptors : broadening by artificial electrical coupling

    NARCIS (Netherlands)

    Smakman, J.G.J.; Stavenga, D.G.

    1987-01-01

    1. Electrical coupling between R1-6 photoreceptors was investigated by measuring angular sensitivities and quantum bumps. 2. Recordings were made from two extreme types of cells: Type a: cells with a diffraction-like angular sensitivity profile. Only large bumps could be obtained from these cells.

  4. Epidemiology Of Angular Deformities Of The Knee In Children In ...

    African Journals Online (AJOL)

    Background: Bony problems such as angular deformities and metabolic bone disease are of high frequency in Nigeria. Objective: The aim of this study was to define the pattern of presentation in children with angular deformities of the knee. Methodology: It was an 18-month prospective study involving children aged ...

  5. Fundamental methods to measure the orbital angular momentum of light

    NARCIS (Netherlands)

    Berkhout, Gregorius Cornelis Gerardus (Joris)

    2011-01-01

    Light is a ubiquitous carrier of information. This information can be encoded in the intensity, direction, frequency and polarisation of the light and, which was described more recently, in its orbital angular momentum. Although creating light beams with orbital angular momentum is relatively easy,

  6. Resolving Ethical Issues at School

    Science.gov (United States)

    Benninga, Jacques S.

    2013-01-01

    Although ethical dilemmas are a constant in teachers' lives, the profession has offered little in the way of training to help teachers address such issues. This paper presents a framework, based on developmental theory, for resolving professional ethical dilemmas. The Four-Component Model of Moral Maturity, when used in conjunction with a…

  7. Time-resolved quantitative phosphoproteomics

    DEFF Research Database (Denmark)

    Verano-Braga, Thiago; Schwämmle, Veit; Sylvester, Marc

    2012-01-01

    proteins involved in the Ang-(1-7) signaling, we performed a mass spectrometry-based time-resolved quantitative phosphoproteome study of human aortic endothelial cells (HAEC) treated with Ang-(1-7). We identified 1288 unique phosphosites on 699 different proteins with 99% certainty of correct peptide...

  8. Time-resolved vibrational spectroscopy

    Energy Technology Data Exchange (ETDEWEB)

    Tokmakoff, Andrei [Massachusetts Inst. of Technology (MIT), Cambridge, MA (United States); Champion, Paul [Northeastern Univ., Boston, MA (United States); Heilweil, Edwin J. [National Inst. of Standards and Technology (NIST), Boulder, CO (United States); Nelson, Keith A. [Massachusetts Inst. of Technology (MIT), Cambridge, MA (United States); Ziegler, Larry [Boston Univ., MA (United States)

    2009-05-14

    This document contains the Proceedings from the 14th International Conference on Time-Resolved Vibrational Spectroscopy, which was held in Meredith, NH from May 9-14, 2009. The study of molecular dynamics in chemical reaction and biological processes using time-resolved spectroscopy plays an important role in our understanding of energy conversion, storage, and utilization problems. Fundamental studies of chemical reactivity, molecular rearrangements, and charge transport are broadly supported by the DOE's Office of Science because of their role in the development of alternative energy sources, the understanding of biological energy conversion processes, the efficient utilization of existing energy resources, and the mitigation of reactive intermediates in radiation chemistry. In addition, time-resolved spectroscopy is central to all fiveof DOE's grand challenges for fundamental energy science. The Time-Resolved Vibrational Spectroscopy conference is organized biennially to bring the leaders in this field from around the globe together with young scientists to discuss the most recent scientific and technological advances. The latest technology in ultrafast infrared, Raman, and terahertz spectroscopy and the scientific advances that these methods enable were covered. Particular emphasis was placed on new experimental methods used to probe molecular dynamics in liquids, solids, interfaces, nanostructured materials, and biomolecules.

  9. Optical communications beyond orbital angular momentum

    Science.gov (United States)

    Rosales-Guzmán, Carmelo; Trichili, Abderrahmen; Dudley, Angela; Ndagano, Bienvenu; Ben Salem, Amine; Zghal, Mourad; Forbes, Andrew

    2016-09-01

    Current optical communication technologies are predicted to face a bandwidth capacity limit in the near future. The nature of the limitation is fundamental rather than technological and is set by nonlinearities in optical fibers. One solution, suggested over 30 years ago, comprises the use of spatial modes of light as information carriers. Along this direction, light beams endowed with orbital angular momentum (OAM) have been demonstrated as potential information carriers in both, free space and fibres. However, recent studies suggest that purely OAM modes does not increase the bandwidth of optical communication systems. In fact, in all work to date, only the azimuthal component of transverse spatial modes has been used. Crucially, all transverse spatial modes require two degrees of freedom to be described; in the context of Laguerre-Gaussian (LGp`) beams these are azimuthal (l) and radial (p), the former responsible for OAM. Here, we demonstrate a technique where both degrees of freedom of LG modes are used as information carrier over free space. We transfer images encoded using 100 spatial modes in three wavelengths as our basis, and employ a spatial demultiplexing scheme that detects all 100 modes simultaneously. Our scheme is a hybrid of MIMO and SMM, and serves as a proof-of-principle demonstration. The cross-talk between the modes is small and independent of whether OAM modes are used or not.

  10. CLASS: The Cosmology Large Angular Scale Surveyor

    Science.gov (United States)

    Essinger-Hileman, Thomas; Ali, Aamir; Amiri, Mandana; Appel, John W.; Araujo, Derek; Bennett, Charles L.; Boone, Fletcher; Chan, Manwei; Cho, Hsiao-Mei; Chuss, David T.; hide

    2014-01-01

    The Cosmology Large Angular Scale Surveyor (CLASS) is an experiment to measure the signature of a gravitational wave background from inflation in the polarization of the cosmic microwave background (CMB). CLASS is a multi-frequency array of four telescopes operating from a high-altitude site in the Atacama Desert in Chile. CLASS will survey 70% of the sky in four frequency bands centered at 38, 93, 148, and 217 GHz, which are chosen to straddle the Galactic-foreground minimum while avoiding strong atmospheric emission lines. This broad frequency coverage ensures that CLASS can distinguish Galactic emission from the CMB. The sky fraction of the CLASS survey will allow the full shape of the primordial B-mode power spectrum to be characterized, including the signal from reionization at low-length. Its unique combination of large sky coverage, control of systematic errors, and high sensitivity will allow CLASS to measure or place upper limits on the tensor-to-scalar ratio at a level of r = 0:01 and make a cosmic-variance-limited measurement of the optical depth to the surface of last scattering, tau. (c) (2014) COPYRIGHT Society of Photo-Optical Instrumentation Engineers (SPIE). Downloading of the abstract is permitted for personal use only.

  11. Angular distributions of sputtered particles from NiTi alloy

    International Nuclear Information System (INIS)

    Neshev, I.; Hamishkeev, V.; Chernysh, V.S.; Postnikov, S.; Mamaev, B.

    1993-01-01

    The angular distributions of sputtered Ni and Ti from a polycrystalline NiTi (50-50%) alloy are investigated by Auger electron spectroscopy and Rutherford backscattering spectroscopy. A difference in the angular distributions is observed with Ni being sputtered preferentially near the surface normal. A computer program for the calculation of the angular distributions of constituents sputtered from binary targets is created and used. The mechanisms responsible for the observed differences in the angular distributions are discussed. It is found that the collisional cascade theory is not directly applicable to the results of the constituents' angular distributions obtained in the presence of oxygen. The fitted coefficients of bombardment-induced segregation are found to be greater than the experimentally obtained ones. (author)

  12. Transition from the adiabatic to the sudden limit in core-electron photoemission

    Science.gov (United States)

    Hedin, Lars; Michiels, John; Inglesfield, John

    1998-12-01

    Experimental results for core-electron photoemission Jk(ω) are often compared with the one-electron spectral function Ac(ɛk-ω), where ω is the photon energy, ɛk is the photoelectron energy, and the optical transition matrix elements are taken as constant. Since Jk(ω) is nonzero only for ɛk>0, we must actually compare it with Ac(ɛk-ω)θ(ɛk). For metals Ac(ω) is known to have a quasiparticle (QP) peak with an asymmetric power-law [theories of Mahan, Nozières, de Dominicis, Langreth, and others (MND)] singularity due to low-energy particle-hole excitations. The QP peak starts at the core-electron energy ɛc, and is followed by an extended satellite (shakeup) structure at smaller ω. For photon energies ω just above threshold, ωth=-ɛc, Ac(ɛk-ω)θ(ɛk) as a function of ɛk (ω constant) is cut just behind the quasiparticle peak, and neither the tail of the MND line nor the plasmon satellites are present. The sudden (high-energy) limit is given by a convolution of Ac(ω) and a loss function, i.e., by the Berglund-Spicer two-step expression. Thus Ac(ω) alone does not give the correct photoelectron spectrum, neither at low nor at high energies. We present an extension of the quantum-mechanical (QM) models developed earlier by Inglesfield, and by Bardyszewski and Hedin to calculate Jk(ω). It includes recoil and damping, as well as shakeup effects and extrinsic losses, is exact in the high-energy limit, and allows calculations of Jk(ω) including the MND line and multiple plasmon losses. The model, which involves electrons coupled to quasibosons, is motivated by detailed arguments. As an illustration we have made quantitative calculations for a semi-infinite jellium with the density of aluminum metal and an embedded atom. The coupling functions (fluctuation potentials) between the electron and the quasibosons are related to the random-phase-approximation dielectric function, and different levels of approximations are evaluated numerically. The differences

  13. The slope-background for the near-peak regimen of photoemission spectra

    Energy Technology Data Exchange (ETDEWEB)

    Herrera-Gomez, A., E-mail: aherrera@qro.cinvestav.mx [CINVESTAV-Unidad Queretaro, Queretaro 76230 (Mexico); Bravo-Sanchez, M. [CINVESTAV-Unidad Queretaro, Queretaro 76230 (Mexico); Aguirre-Tostado, F.S. [Centro de Investigación en Materiales Avanzados, Chihuahua, Chihuahua 31109 (Mexico); Vazquez-Lepe, M.O. [Departamento de Ingeniería de Proyectos, Universidad de Guadalajara, Jalisco 44430 (Mexico)

    2013-08-15

    Highlights: •We propose a method that accounts for the change in the background slope of XPS data. •The slope-background can be derived from Tougaard–Sigmund's transport theory. •The total background is composed by Shirley–Sherwood and Tougaard type backgrounds. •The slope-background employs one parameter that can be related to REELS spectra. •The slope, in conjunction with the Shirley–Sherwood background, provides better fits. -- Abstract: Photoemission data typically exhibits a change on the intensity of the background between the two sides of the peaks. This step is usually very well reproduced by the Shirley–Sherwood background. Yet, the change on the slope of the background in the near-peak regime, although usually present, is not always as obvious to the eye. However, the intensity of the background signal associated with the evolution of its slope can be appreciable. The slope-background is designed to empirically reproduce the change on the slope. Resembling the non-iterative Shirley method, the proposed functional form relates the slope of the background to the integrated signal at higher electron kinetic energies. This form can be predicted under Tougaard–Sigmund's electron transport theory in the near-peak regime. To reproduce both the step and slope changes on the background, it is necessary to employ the slope-background in conjunction with the Shirley–Sherwood background under the active-background method. As it is shown for a series of materials, the application of the slope-background provides excellent fits, is transparent to the operator, and is much more independent of the fitting range than other background methods. The total area assessed through the combination of the slope and the Shirley–Sherwood backgrounds is larger than when only the Shirley–Sherwood background is employed, and smaller than when the Tougaard background is employed.

  14. Chemical bonding in Tl cuprates studied by x-ray photoemission

    International Nuclear Information System (INIS)

    Vasquez, R.P.; Siegal, M.P.; Overmyer, D.L.; Ren, Z.F.; Lao, J.Y.; Wang, J.H.

    1999-01-01

    Epitaxial thin films of the Tl cuprate superconductors Tl 2 Ba 2 CaCu 2 O 8 , Tl 2 Ba 2 Ca 2 Cu 3 O 10 , and Tl 0.78 Bi 0.22 Ba 0.4 Sr 1.6 Ca 2 Cu 3 O 9-δ are studied with x-ray photoemission spectroscopy. These data, together with previous measurements in this lab of Tl 2 Ba 2 CuO 6+δ and TlBa 2 CaCu 2 O 7-δ , comprise a comprehensive data set for a comparative study of Tl cuprates with a range of chemical and electronic properties. In the Cu 2p spectra, a larger energy separation between the satellite and main peaks (E s -E m ) and a lower intensity ratio (I s /I m ) are found to correlate with higher values of T c . Analysis of these spectra within a simple configuration interaction model suggests that higher values of T c are related to low values of the O 2p→Cu 3d charge transfer energy. In the O 1s region, a smaller bond length between Ba and Cu-O planar oxygen is found to correlate with a lower binding energy for the signal associated with Cu-O bonding, most likely resulting from the increased polarization screening by Ba 2+ ions. For samples near optimum doping, maximum T c is observed to occur when the Tl 4f 7/2 binding energy is near 117.9 eV, which is near the middle of the range of values observed for Tl cuprates. Higher Tl 4f 7/2 binding energies, corresponding to formal oxidation states nearer Tl 1+ , are also found to correlate with longer bond lengths between Ba and Tl-O planar oxygen, and with higher binding energies of the O 1s signal associated with Tl-O bonding. copyright 1999 The American Physical Society

  15. Efficiency Limits of Solar Energy Harvesting via Internal Photoemission in Carbon Materials

    Directory of Open Access Journals (Sweden)

    Svetlana V. Boriskina

    2018-02-01

    Full Text Available We describe strategies to estimate the upper limits of the efficiency of photon energy harvesting via hot electron extraction from gapless absorbers. Gapless materials such as noble metals can be used for harvesting the whole solar spectrum, including visible and near-infrared light. The energy of photo-generated non-equilibrium or ‘hot’ charge carriers can be harvested before they thermalize with the crystal lattice via the process of their internal photo-emission (IPE through the rectifying Schottky junction with a semiconductor. However, the low efficiency and the high cost of noble metals necessitates the search for cheaper abundant alternative materials, and we show here that carbon can serve as a promising IPE material candidate. We compare the upper limits of performance of IPE photon energy-harvesting platforms, which incorporate either gold or carbon as the photoactive material where hot electrons are generated. Through a combination of density functional theory, joint electron density of states calculations, and Schottky diode efficiency modeling, we show that the material electron band structure imposes a strict upper limit on the achievable efficiency of the IPE devices. Our calculations reveal that graphite is a good material candidate for the IPE absorber for harvesting visible and near-infrared photons. Graphite electron density of states yields a sizeable population of hot electrons with energies high enough to be collected across the potential barrier. We also discuss the mechanisms that prevent the IPE device efficiency from reaching the upper limits imposed by their material electron band structures. The proposed approach is general and allows for efficient pre-screening of materials for their potential use in IPE energy converters and photodetectors within application-specific spectral windows.

  16. A photoemission study of Mn grown on GaAs(100)

    International Nuclear Information System (INIS)

    James, D.; Riley, J.; Leckey, R.; Usher, B.; Sieber, N.; Seyller, Th.; Ley, L.

    2002-01-01

    Full text: Metal contacts on semiconductors have been an important area for device manufacture. The possibility of lattice matched growth of magnetic metals on semiconductors was once thought to be a unobtainable goal. More recently it has been found that transition metals can react with the semiconductor substrates, forming another lattice with a more comparable lattice constant, from which epitaxial growth can then proceed. Al grows epitaxially on GaN even with a lattice mismatch greater than 10%. In this instance, Al displaces Ga being driven by a larger heat of formation to produce an AlN buffer layer, on which Al can then grow. This paper investigates the room temperature deposition of Mn onto GaAs(100) at room temperature. The Photoemission study was carried out at the UEL56/2 PGM2 beam line at BESSY II in Berlin, Germany. Synchrotron radiation was used to observe the surface as thin layers of Mn were deposited. The interaction of manganese with the substrate tends to donate electron density to neighbouring atoms, decreasing binding energy. No further segregation of substitutional or interstitial Mn and Ga can be seen from angle dependence data at this temperature, with metallic manganese eventually attenuating the bulk Ga signal to the point where it is indistinguishable from the background. It is concluded that there the metal reacts with the semiconductor surface with some indiffusion as confirmed using SIMS. Previously, the reaction was only thought to have taken place above room temperature. The resulting structure consists of a Ga-As-Mn buffer layer as with the higher temperature depositions

  17. Photoemission intensity oscillations in the valence bands of C70 film

    International Nuclear Information System (INIS)

    Li Yanjun; Wang Peng; Ni Jingfu; Meng Liang; Wang Xiaobo; Sheng Chunqi; Li Hongnian; Zhang Wenhua; Xu Yang; Xu Faqiang; Zhu Junfa

    2011-01-01

    Highlights: → The article develops a procedure for obtaining the accurate spectral intensities in the studies of the photoionization cross-section oscillation of C 70 . → The article fulfills the observation of all oscillating periods of the cross-section oscillation of C 70 . → The article reports the oscillating data for more molecular orbitals (feature C in the article) as compared with the published works. → The article reveals that some simple theoretical models based on the spherical symmetric approximation survive for the ellipsoidally shaped C 70 . - Abstract: We have measured and analyzed the photoemission spectra (PES) of a C 70 film in the photon energy region from 13.4 eV to 98.4 eV. The photoelectron intensities of two C 2p π-derived features (denoted by A and B) oscillate regularly in the whole energy region with some fine structures below ∼30 eV. To obtain the detailed information of the oscillations, we have developed a sophisticated but practical procedure for intensity calculation. The procedure consists of two core concepts. The first is ascribing the PES features to their corresponding molecular orbitals with the help of density functional calculations. The second is a background subtraction algorithm. With this procedure, we obtained the oscillating behavior for individual features (A and B), which is by and large consistent with the predictions based on the spherical symmetric approximation although C 70 has the ellipsoidal shape. Owing to the solid state effect, the oscillating amplitudes of the A/B intensity ratios are smaller than those of gas phase C 70 , but an orbital shift reported recently was not observed on our sample. The oscillating curve of a deeper feature, which consists of both σ and π states, are also reported.

  18. Internal photoemission from plasmonic nanoparticles: comparison between surface and volume photoelectric effects.

    Science.gov (United States)

    Uskov, Alexander V; Protsenko, Igor E; Ikhsanov, Renat S; Babicheva, Viktoriia E; Zhukovsky, Sergei V; Lavrinenko, Andrei V; O'Reilly, Eoin P; Xu, Hongxing

    2014-05-07

    We study the emission of photoelectrons from plasmonic nanoparticles into a surrounding matrix. We consider two mechanisms of electron emission from the nanoparticles--surface and volume ones--and use models for these two mechanisms which allow us to obtain analytical results for the photoelectron emission rate from a nanoparticle. Calculations have been carried out for a step potential at the surface of a spherical nanoparticle, and a simple model for the hot electron cooling has been used. We highlight the effect of the discontinuity of the dielectric permittivity at the nanoparticle boundary in the surface mechanism, which leads to a substantial (by ∼5 times) increase of the internal photoelectron emission rate from a nanoparticle compared to the case when such a discontinuity is absent. For a plasmonic nanoparticle, a comparison of the two photoeffect mechanisms was undertaken for the first time which showed that the surface photoeffect can in the general case be larger than the volume one, which agrees with the results obtained for a flat metal surface first formulated by Tamm and Schubin in their pioneering development of a quantum-mechanical theory of photoeffect in 1931. In accordance with our calculations, this possible predominance of the surface effect is based on two factors: (i) effective cooling of hot carriers during their propagation from the volume of the nanoparticle to its surface in the scenario of the volume mechanism and (ii) strengthening of the surface mechanism through the effect of the discontinuity of the dielectric permittivity at the nanoparticle boundary. The latter is stronger at relatively lower photon energies and correspondingly is more substantial for internal photoemission than for an external one. We show that in the general case, it is essential to take both mechanisms into account in the development of devices based on the photoelectric effect and when considering hot electron emission from a plasmonic nanoantenna.

  19. Lateral light propagation and angular variation of the reflectance of paper

    Science.gov (United States)

    Coppel, Ludovic G.

    2014-02-01

    The appearance of translucent materials is strongly affected by bulk (or sub surface) scattering. For paper and carton board, lateral light propagation and angle-resolved reflection have been studied extensively but treated separately. The present work aims at modelling the BSSRDF of turbid media in order to study the angular variation of the reflectance as function of the lateral propagation within the medium. Monte Carlo simulations of the spatial- and angle resolved reflectance of turbid media are performed for different scattering and absorption coefficients, phase functions and surface topographies representative for uncoated paper grades. The angle-resolved radiance factor of turbid media is found to be function of the lateral light propagation within the substrate and both the reflected radiance factor and the fluorescence emission are found to be clearly non- Lambertian, although the latter clearly depends on the light absorption at the excitation wavelength. It is also suggested that the modelling of uncoated paper should not include surface scattering. The findings impact on the appearance of turbid media at different angles and make measurements of the lateral light propagation dependent on the instrument geometry.

  20. Attosecond-Resolved Electron Dynamics in Many-Electron Atoms: Quantitative Theory and Comparison with Measurements

    Directory of Open Access Journals (Sweden)

    Cleanthes Anthony Nicolaides

    2018-03-01

    Full Text Available A variety of processes originating from the interaction of atomic or molecular N-electron states with strong and/or hypershort radiation pulses can be understood quantitatively only by first determining with good accuracy the solutions of the many-electron time-dependent Schrödinger equation (METDSE that describe the corresponding physics. The METDSE is solvable nonperturbatively via the state-specific expansion approach (SSEA. SSEA solutions have been used, or can be used, for quantitative explanation and numerically reliable predictions of quantities that have been measured or are measurable in modern laser-driven experiments that can track, with hypershort (attosecond time resolution, the effects of electron rearrangements in atoms and molecules. The calculations take into account in a transparent way the interplay between the phenomena and the electronic structures of the physically significant states in discrete and multichannel continuous spectra, including multiply- and inner-hole–excited resonance states. The discussion focuses on novel topics of time-resolved many-electron physics and includes a comparison of our predictions to recent quantitative measurements of attosecond-resolved generation of the profile of the doubly excited resonance state of helium during photoionization and of the relative time delay in photoemission of the (2s,2p electrons of neon.