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Sample records for angle-resolved electron energy

  1. Materials characterisation by angle-resolved scanning transmission electron microscopy

    Science.gov (United States)

    Müller-Caspary, Knut; Oppermann, Oliver; Grieb, Tim; Krause, Florian F.; Rosenauer, Andreas; Schowalter, Marco; Mehrtens, Thorsten; Beyer, Andreas; Volz, Kerstin; Potapov, Pavel

    2016-11-01

    Solid-state properties such as strain or chemical composition often leave characteristic fingerprints in the angular dependence of electron scattering. Scanning transmission electron microscopy (STEM) is dedicated to probe scattered intensity with atomic resolution, but it drastically lacks angular resolution. Here we report both a setup to exploit the explicit angular dependence of scattered intensity and applications of angle-resolved STEM to semiconductor nanostructures. Our method is applied to measure nitrogen content and specimen thickness in a GaNxAs1‑x layer independently at atomic resolution by evaluating two dedicated angular intervals. We demonstrate contrast formation due to strain and composition in a Si- based metal-oxide semiconductor field effect transistor (MOSFET) with GexSi1‑x stressors as a function of the angles used for imaging. To shed light on the validity of current theoretical approaches this data is compared with theory, namely the Rutherford approach and contemporary multislice simulations. Inconsistency is found for the Rutherford model in the whole angular range of 16–255 mrad. Contrary, the multislice simulations are applicable for angles larger than 35 mrad whereas a significant mismatch is observed at lower angles. This limitation of established simulations is discussed particularly on the basis of inelastic scattering.

  2. Angle-Resolved Photoemission of Solvated Electrons in Sodium-Doped Clusters

    CERN Document Server

    West, Adam H C; Luckhaus, David; Saak, Clara-Magdalena; Doppelbauer, Maximilian; Signorell, Ruth

    2015-01-01

    Angle-resolved photoelectron spectroscopy of the unpaired electron in sodium-doped water, methanol, ammonia, and dimethyl ether clusters is presented. The experimental observations and the complementary calculations are consistent with surface electrons for the cluster size range studied. Evidence against internally solvated electrons is provided by the photoelectron angular distribution. The trends in the ionization energies seem mainly determined by the degree of hydrogen bonding in the solvent and the solvation of the ion core. The onset ionization energies of water and methanol clusters do not level off at small cluster sizes, but decrease slightly with increasing cluster size.

  3. Momentum-Dependent Charge Transfer Excitations in Sr{sub {bold 2}}CuO {sub {bold 2}}Cl{sub {bold 2}} Angle-Resolved Electron Energy Loss Spectroscopy

    Energy Technology Data Exchange (ETDEWEB)

    Wang, Y.Y.; Zhang, F.C.; Dravid, V.P.; Ng, K.K.; Klein, M.V.; Schnatterly, S.E.; Miller, L.L. [Department of Materials Science and Engineering, Northwestern University, Evanston, Illinois 60208 (United States)]|[Science and Technology Center for Superconductivity, Northwestern University, Evanston, Illinois 60208 (United States)]|[Department of Physics, University of Cincinnati, Cincinnati, Ohio 45221 (United States)]|[Department of Physics, Hong Kong University of Science and Technology, Clear Water Bay, Kowloon (Hong Kong)]|[Department of Physics, Science and Technology Center for Superconductivity, University of Illinois, Urbana, Illinois 61801 (United States)]|[Department of Physics, University of Virginia, Charlottesville, Virginia 22901 (United States)]|[Ames Laboratory, Iowa State University, Ames, Iowa 50011 (United States)

    1996-08-01

    Electron-hole pair excitations in the insulating cuprates Sr{sub 2}CuO{sub 2}Cl{sub 2} were investigated by angle-resolved electron energy loss spectroscopy. The optically allowed and optically forbidden transitions were observed to be strongly anisotropic in Cu-O{sub 2} plane. The former show a large energy dispersion {approximately}1.5 eV along [110], and the latter appear at a higher energy position ({approximately}4.5 eV) only along [100], but not along [110]. We interpret these results as transitions involving excitons. A small exciton model is examined to explain both the observed features. {copyright} {ital 1996 The American Physical Society.}

  4. Note: A new angle-resolved proton energy spectrometer

    Energy Technology Data Exchange (ETDEWEB)

    Zheng, Y.; Su, L. N.; Liu, M.; Liu, B. C.; Shen, Z. W.; Fan, H. T.; Li, Y. T.; Chen, L. M.; Lu, X.; Ma, J. L.; Wang, W. M.; Wang, Z. H.; Wei, Z. Y. [Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences, Beijing 100190 (China); Zhang, J. [Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences, Beijing 100190 (China); Key Laboratory for Laser Plasmas (MoE) and Department of Physics, Shanghai Jiao Tong University, Shanghai 200240 (China)

    2013-09-15

    In typical laser-driven proton acceleration experiments Thomson parabola proton spectrometers are used to measure the proton spectra with very small acceptance angle in specific directions. Stacks composed of CR-39 nuclear track detectors, imaging plates, or radiochromic films are used to measure the angular distributions of the proton beams, respectively. In this paper, a new proton spectrometer, which can measure the spectra and angular distributions simultaneously, has been designed. Proton acceleration experiments performed on the Xtreme light III laser system demonstrates that the spectrometer can give angle-resolved spectra with a large acceptance angle. This will be conductive to revealing the acceleration mechanisms, optimization, and applications of laser-driven proton beams.

  5. Electronic structure of MgB2 from angle-resolved photoemission spectroscopy.

    Science.gov (United States)

    Uchiyama, H; Shen, K M; Lee, S; Damascelli, A; Lu, D H; Feng, D L; Shen, Z-X; Tajima, S

    2002-04-15

    The first angle-resolved photoemission spectroscopy results from MgB2 single crystals are reported. Along the GammaK and GammaM directions, we observed three distinct dispersive features approaching the Fermi energy. These can be assigned to the theoretically predicted sigma (B 2p(x,y)) and pi (B 2p(z)) bands. In addition, a small parabolic-like band is detected around the Gamma point, which can be attributed to a surface-derived state. The overall agreement between our results and the band calculations suggests that the electronic structure of MgB2 is of a conventional nature, thus implying that electron correlations are weak and may be of little importance to superconductivity in this system.

  6. Surface and subsurface oxidation of Mo2C/Mo(100): low-energy ion-scattering, auger electron, angle-resolved X-ray photoelectron, and mass spectroscopy studies.

    Science.gov (United States)

    Ovári, László; Kiss, János; Farkas, Arnold P; Solymosi, Frigyes

    2005-03-17

    The interaction of oxygen with a carburized Mo(100) surface was investigated at different temperatures (300-1000 K). The different information depths of low-energy ion-scattering (LEIS) spectroscopy, with topmost layer sensitivity, Auger electron spectroscopy (AES), and angle-resolved X-ray photoelectron spectroscopy (ARXPS) allowed us to discriminate between reactions on the topmost layer and subsurface transformations. According to ARXPS measurements, a carbide overlayer was prepared by the high-temperature decomposition of C(2)H(4) on Mo(100), and the carbon distribution proved to be homogeneous with a Mo(2)C stoichiometry down to the information depth of XPS. O(2) adsorbs dissociatively on the carbide layer at room temperature. One part of the chemisorbed oxygen is bound to both C and Mo sites, indicated by LEIS. Another fraction of oxygen atoms probably resides in the hollow sites not occupied by C. The removal of C from the outermost layer by O(2), in the form of CO, detected by mass spectroscopy (MS), was observed at 500-600 K. The carbon-depleted first layer is able to adsorb more oxygen compared to the Mo(2)C/Mo(100) surface. Applying higher doses of O(2) at 800 K results in the inward diffusion of O and the partial oxidation of Mo atoms. This process, however, is not accompanied by the removal of C from subsurface sites. The depletion of C from the bulk starts only at 900 K (as shown by MS, AES, and XPS), very probably by the diffusion of C to the surface followed by its reaction with oxygen. At T(ads) = 1000 K, the carbon content of the sample, down to the information depth of XPS, decreased further, accompanied by the attenuation of the C concentration gradient and a substantially decreased amount of oxygen.

  7. Photon energy dependence of angle-resolved photoemission spectroscopy in graphene

    Science.gov (United States)

    Ayria, Pourya; Nugraha, Ahmad R. T.; Hasdeo, Eddwi H.; Czank, Thomas R.; Tanaka, Shin-ichiro; Saito, Riichiro

    2015-11-01

    The photon energy dependence of angle-resolved photoemission spectroscopy (ARPES) in graphene is investigated experimentally and theoretically. By applying light with energy of around 46 eV , we found an unexpected increase in the ARPES relative intensity of graphene for the p branch (ARPES spectra brightened by the p -polarized light) with respect to the s branch (those brightened by the s -polarized light). The origin of the enhanced p -branch intensity is explained by first-principles calculations, in which we show (1) the optical dipole vector as a function of final-state energies of the excited electron, (2) the absorption intensity as a function of the incident light angle, and (3) the symmetry of the initial and the final states. The calculated results imply that the dipole vector of the excited electron near 46 eV has an exceptionally large component in the normal direction of the graphene surface compared to that within the graphene plane, which could be the main reason for the enhancement of the p -branch intensity.

  8. Quantifying electronic band interactions in van der Waals materials using angle-resolved reflected-electron spectroscopy

    Science.gov (United States)

    Jobst, Johannes; van der Torren, Alexander J. H.; Krasovskii, Eugene E.; Balgley, Jesse; Dean, Cory R.; Tromp, Rudolf M.; van der Molen, Sense Jan

    2016-11-01

    High electron mobility is one of graphene's key properties, exploited for applications and fundamental research alike. Highest mobility values are found in heterostructures of graphene and hexagonal boron nitride, which consequently are widely used. However, surprisingly little is known about the interaction between the electronic states of these layered systems. Rather pragmatically, it is assumed that these do not couple significantly. Here we study the unoccupied band structure of graphite, boron nitride and their heterostructures using angle-resolved reflected-electron spectroscopy. We demonstrate that graphene and boron nitride bands do not interact over a wide energy range, despite their very similar dispersions. The method we use can be generally applied to study interactions in van der Waals systems, that is, artificial stacks of layered materials. With this we can quantitatively understand the `chemistry of layers' by which novel materials are created via electronic coupling between the layers they are composed of.

  9. Angle-Resolved Photoemission Spectroscopy on Electronic Structure and Electron-Phonon Coupling in Cuprate Superconductors

    Energy Technology Data Exchange (ETDEWEB)

    Zhou, X.J.

    2010-04-30

    In addition to the record high superconducting transition temperature (T{sub c}), high temperature cuprate superconductors are characterized by their unusual superconducting properties below T{sub c}, and anomalous normal state properties above T{sub c}. In the superconducting state, although it has long been realized that superconductivity still involves Cooper pairs, as in the traditional BCS theory, the experimentally determined d-wave pairing is different from the usual s-wave pairing found in conventional superconductors. The identification of the pairing mechanism in cuprate superconductors remains an outstanding issue. The normal state properties, particularly in the underdoped region, have been found to be at odd with conventional metals which is usually described by Fermi liquid theory; instead, the normal state at optimal doping fits better with the marginal Fermi liquid phenomenology. Most notable is the observation of the pseudogap state in the underdoped region above T{sub c}. As in other strongly correlated electrons systems, these unusual properties stem from the interplay between electronic, magnetic, lattice and orbital degrees of freedom. Understanding the microscopic process involved in these materials and the interaction of electrons with other entities is essential to understand the mechanism of high temperature superconductivity. Since the discovery of high-T{sub c} superconductivity in cuprates, angle-resolved photoemission spectroscopy (ARPES) has provided key experimental insights in revealing the electronic structure of high temperature superconductors. These include, among others, the earliest identification of dispersion and a large Fermi surface, an anisotropic superconducting gap suggestive of a d-wave order parameter, and an observation of the pseudogap in underdoped samples. In the mean time, this technique itself has experienced a dramatic improvement in its energy and momentum resolutions, leading to a series of new discoveries not

  10. Valence Electronic Structure of Oxygen-Modified α-Mo2C(0001) Surface:. Angle-Resolved Photoemission Study

    Science.gov (United States)

    Kato, M.; Ozawa, K.; Sato, T.; Edamoto, K.

    Adsorption of oxygen on α-Mo2C(0001) is investigated with Auger electron spectroscopy (AES), low-energy electron diffraction (LEED) and angle-resolved photoemission spectroscopy (ARPES) utilizing synchrotron radiation. It is found that C KLL Auger peak intensity does not change during O2 exposure, indicating that the depletion of C atoms does not proceed. It is deduced from ARPES and LEED results that adsorbed oxygen atoms from a well-ordered (1 × 1) lattice on the α-Mo2C(0001) surface. The ARPES study shows that oxygen adsorption induces a peculiar state around Fermi level (EF). Off-normal-emission measurements prove that the state is a half-filled metallic state.

  11. Experimental electronic structure and Fermi-surface instability of the correlated 3d sulphide BaVS3 : High-resolution angle-resolved photoemission spectroscopy

    Science.gov (United States)

    Mitrovic, S.; Fazekas, P.; Søndergaard, C.; Ariosa, D.; Barišić, N.; Berger, H.; Cloëtta, D.; Forró, L.; Höchst, H.; Kupčić, I.; Pavuna, D.; Margaritondo, G.

    2007-04-01

    The correlated 3d sulphide BaVS3 exhibits an interesting coexistence of one-dimensional and three-dimensional properties. Our experiments determine the electronic band structure and shed light on this puzzle. High-resolution angle-resolved photoemission measurements in a 4-eV -wide range below the Fermi energy level uncover and investigate the coexistence of a1g wide-band and eg narrow-band d electrons, which lead to the complicated electronic properties of this material. We explore the effects of strong correlations and the Fermi surface instability associated with the metal-insulator transition.

  12. Electronic states localized at surface defects on Cu(755) studied by angle-resolved ultraviolet photoelectron spectroscopy using synchrotron radiation

    CERN Document Server

    Ogawa, K; Namba, H

    2003-01-01

    'Regularly stepped' and 'defective' surfaces of Cu(755) were prepared by low- and high-temperature annealing, respectively, of a clean specimen. Electronic states on both surfaces were studied by angle-resolved ultraviolet photoelectron spectroscopy using synchrotron radiation. On the defective Cu(755), we found a new photoelectron peak due to surface defects just below the Fermi level. The dispersion profile of the defect state is derived to be almost flat, which demonstrates the localized nature of the defects. High activity to oxygen adsorption of the defect state was revealed. (author)

  13. Electronic structure studies of ferro-pnictide superconductors and their parent compounds using angle-resolved photoemission spectroscopy (ARPES)

    Energy Technology Data Exchange (ETDEWEB)

    Setti, Thirupathaiah

    2011-07-14

    The discovery of high temperature superconductivity in the iron pnictide compound LaO{sub 1-x}F{sub x}FeAs with T{sub c} = 26 K as created enormous interest in the high-T{sub c} superconductor community. So far, four prototypes of crystal structures have been found in the Fe-pnictide family. All four show a structural deformation followed or accompanied by a magnetic transition from a high temperature paramagnetic conductor to a low temperature antiferromagnetic metal whose transition temperature T{sub N} varies between the compounds. Charge carrier doping, isovalent substitution of the As atoms or the application of pressure suppresses the antiferromagnetic spin density wave (SDW) order and leads to a superconducting phase. More recently high Tc superconductivity has been also detected in iron chalchogenides with similar normal state properties. Since superconductivity is instability of the normal state, the study of normal state electronic structure in comparison with superconducting state could reveal important information on the pairing mechanism. Therefore, it is most important to study the electronic structure of these new superconductors, i.e., to determine Fermi surfaces and band dispersions near the Fermi level at the high symmetry points in order to obtain a microscopic understanding of the superconducting properties. Using the technique angle-resolved photoemission spectroscopy (ARPES) one measures the electrons ejected from a sample when photons impinge on it. In this way one can map the Fermi surface which provides useful information regarding the physics behind the Fermi surface topology of high T{sub c} superconductors. Furthermore, this technique provides information on the band dispersion, the orbital character of the bands, the effective mass, the coupling to bosonic excitations, and the superconducting gap. This emphasizes the importance of studying the electronic structure of the newly discovered Fe-pnictides using ARPES. In this work we have

  14. Method to map one-dimensional electronic wave function by using multiple Brillouin zone angle resolved photoemission

    Directory of Open Access Journals (Sweden)

    Dong-Wook Lee

    2010-10-01

    Full Text Available Angle resolved photoemission spectroscopy (ARPES is a powerful tool to investigate electronic structures in solids and has been widely used in studying various materials. The electronic structure information by ARPES is obtained in the momentum space. However, in the case of one-dimensional system, we here show that we extract the real space information from ARPES data taken over multiple Brillouin zones (BZs. Intensities in the multiple BZs are proportional to the photoemission matrix element which contains information on the coefficient of the Bloch wave function. It is shown that the Bloch wave function coefficients can be extracted from ARPES data, which allows us to construct the real space wave function. As a test, we use ARPES data from proto-typical one-dimensional system SrCuO2 and construct the real space wave function.

  15. Electronic structure of the iron chalcogenide KFeAgTe2 revealed by angle-resolved photoemission spectroscopy

    Science.gov (United States)

    Ang, R.; Nakayama, K.; Yin, W.-G.; Sato, T.; Lei, Hechang; Petrovic, C.; Takahashi, T.

    2013-10-01

    We have performed angle-resolved photoemission spectroscopy (ARPES) of KFeAgTe2, and revealed the absence of band crossing at the Fermi level (EF) indicative of the unconventional insulating nature of this material. Comparison of the ARPES-derived band dispersions with the first-principles calculations based on local density approximation and the inclusion of electron correlation U demonstrated that the ground state of KFeAgTe2 is not a simple band insulator. And also, our fitting result on the ARPES experimental density of states near EF plausibly excludes the possibility of Anderson insulator. We suggest that KFeAgTe2 is most likely a Mott insulator or a Hund insulator, providing a deep insight into the insulating ground state.

  16. Attosecond electronic and nuclear quantum photodynamics of ozone monitored with time and angle resolved photoelectron spectra

    CERN Document Server

    Decleva, P; Perveaux, A; Lauvergnat, D; Gatti, F; Lasorne, B; Halász, G J; Vibók, Á

    2016-01-01

    Recently we reported a series of numerical simulations proving that it is possible in principle to create an electronic wave packet and subsequent electronic motion in a neutral molecule photoexcited by a UV pump pulse within a few femtoseconds. We considered the ozone molecule: for this system the electronic wave packet leads to a dissociation process. In the present work, we investigate more specifically the time-resolved photoelectron angular distribution of the ozone molecule that provides a much more detailed description of the evolution of the electronic wave packet. We thus show that this experimental technique should be able to give access to observing in real time the creation of an electronic wave packet in a neutral molecule and its impact on a chemical process.

  17. Attosecond electronic and nuclear quantum photodynamics of ozone monitored with time and angle resolved photoelectron spectra

    Science.gov (United States)

    Decleva, Piero; Quadri, Nicola; Perveaux, Aurelie; Lauvergnat, David; Gatti, Fabien; Lasorne, Benjamin; Halász, Gábor J.; Vibók, Ágnes

    2016-11-01

    Recently we reported a series of numerical simulations proving that it is possible in principle to create an electronic wave packet and subsequent electronic motion in a neutral molecule photoexcited by a UV pump pulse within a few femtoseconds. We considered the ozone molecule: for this system the electronic wave packet leads to a dissociation process. In the present work, we investigate more specifically the time-resolved photoelectron angular distribution of the ozone molecule that provides a much more detailed description of the evolution of the electronic wave packet. We thus show that this experimental technique should be able to give access to observing in real time the creation of an electronic wave packet in a neutral molecule and its impact on a chemical process.

  18. Electronic structure of ion arsenic high temperature superconductors studied by angle resolved photoemission spectroscopy

    Energy Technology Data Exchange (ETDEWEB)

    Liu, Chang [Iowa State Univ., Ames, IA (United States)

    2011-01-01

    The main purpose of the present thesis is to present our ARPES results on the iron arsenic superconductors. As revealed by a series of ARPES measurements on both the AEFe2As2 and the RFeAs(O,F) families (parent compound and carrier-doped systems), the electronic structures of the pnictides are complicated, three dimensional, and closely linked to their superconducting behavior (13; 14; 15; 16; 17; 18; 19). Parent compounds of these materials exhibit the basic hole-electron pocket dual plus an apparent Fermi surface reconstruction caused by long range antiferromagnetism (13; 15). When carriers are introduced, the chemical potential shifts in accordance with the Luttinger theorem and the rigid band shifting picture (13). Importantly, both the appearance and disappearance of the superconducting dome at low and high doping levels have intimate relation with topological changes at the Fermi surfaces, resulting in a specific Fermi topology being favored by superconductivity (15; 16). On the low doping side, superconductivity emerges in the phase diagram once the antiferromagnetic reconstruction disappears below the Fermi level, returning the Fermi surface to its paramagnetic-like appearance. On the high doping side, superconductivity disappears around a doping level at which the central hole pocket vanishes due to increasing electron concentration. Such phenomena are evidence for the governing role the electronic structure plays in their superconducting behavior.

  19. Electronic structure studies of YBa[sub 2]Cu[sub 3]O[sub x](6. 2 [le] x [le] 6. 9) using angle resolved photoemission

    Energy Technology Data Exchange (ETDEWEB)

    Veal, B.W.; Liu, Rong; Paulikas, A.P.; Koelling, D.D.; Downey, J.W. (Argonne National Lab., IL (United States)); Shi, Hao (Argonne National Lab., IL (United States) Missouri Univ., Kansas City, MO (United States). Dept. of Physics); Olson, C.G. (Ames Lab., IA (United States)); Arko, A.J.; Joyce, J.J.; Blythe, R. (Los Alamos National Lab., NM (United States))

    1992-11-01

    Using high resolution angle resolved photoemission, the electronic structure of YBa[sub 2]Cu[sub 3]O[sub x] is examined when oxygen stoichiometries are varied in the range 6.2 [le] [times] [le] 6.9. Detailed measurements of the Fermi surface for YBa[sub 2]Cu[sub 3]O[sub 6.9] are presented and are compared with predictions of band theory. In the metallic region of the phase diagram, changes in the Fermi surfaces are measured as a function of oxygen stoichiometry. The electronic structure is monitored as the oxide changes from a metal to a semiconductor with additional oxygen depletion. For intermediate stoichiometries, effects of oxygen vacancy ordering are considered. Unusual resonant effects observed at several photon energies are examined as oxygen content is varied.

  20. Electronic structure studies of YBa[sub 2]Cu[sub 3]O[sub x] (6. 2[<=]x[<=]6. 9) using angle-resolved photoemission

    Energy Technology Data Exchange (ETDEWEB)

    Veal, B.W.; Liu, Rong; Paulikas, A.P.; Koelling, D.D.; Shi, Hao; Downey, J.W. (Materials Science Division and Science and Technology Center for Superconductivity, Argonne National Laboratory, Argonne, IL (United States)); Olson, C.G. (Ames Laboratory and Department of Physics, Iowa State University, Ames, IA (United States)); Arko, A.J.; Joyce, J.J.; Blythe, R. (Los Alamos National Laboratory, Los Alamos, NM (United States))

    1993-12-01

    Using high-resolution angle-resolved photoemission, the electronic structure of YBa[sub 2]Cu[sub 3]O[sub x] is examined when oxygen stoichiometries are varied in the range 6.2[<=]x[<=]6.9. Detailed measurements of the Fermi surface for YBa[sub 2]Cu[sub 3]O[sub 6.9] are presented and are compared with predictions of band theory. In the metallic region of the phase diagram, changes in the Fermi surfaces are measured as a function of oxygen stoichiometry. The electronic structure is monitored as the oxide changes from a metal to a semiconductor with additional oxygen depletion. For intermediate stoichiometries, effects of oxygen-vacancy ordering are considered. Unusual resonant effects observed at several photon energies are examined as the oxygen content is varied.

  1. Angle-resolved energy distributions of laser ablated silver ions in vacuum

    DEFF Research Database (Denmark)

    Hansen, T.N.; Schou, Jørgen; Lunney, J.G.

    1998-01-01

    The energy distributions of ions ablated from silver in vacuum have been measured in situ for pulsed laser irradiation at 355 nm. We have determined the energy spectra for directions ranging from 5 degrees to 75 degrees with respect to the normal in the intensity range from 100 to 400 MW/cm(2...

  2. Angle-resolved photoemission spectroscopy study of adsorption process and electronic structure of silver on ZnO(1010).

    Science.gov (United States)

    Ozawa, K; Sato, T; Kato, M; Edamoto, K; Aiura, Y

    2005-08-01

    The adsorption process and valence band structure of Ag on ZnO(1010) have been investigated by angle-resolved photoelectron spectroscopy utilizing synchrotron radiation. The coverage-dependent measurements of the Ag 4d band structure reveal that the Ag bands with a dispersing feature are formed even at low coverages and that the basic structure of the bands is essentially the same throughout the submonolayer region. These results indicate that the Ag atoms aggregate to form islands with an atomically ordered structure from the low coverages. Upon annealing the Ag-covered surface at 900 K, the Ag 4d band undergoes only a minor change, suggesting that the ordered structure within the Ag islands is persistent against mild annealing. From the dispersive feature of the Ag 4d states, we propose that the atomic structure has locally rectangular symmetry with a good lattice matching with the ZnO(1010) surface.

  3. Exploring the Limits of the Dipole Approximation with Angle-Resolved Electron Time-of-Flight Spectrometry

    Energy Technology Data Exchange (ETDEWEB)

    Laidman, S.; Pangilinan, J.; Guillemin, R.; Yu, S.U.; Ohrwall, G.; Lindle, D.; Hemmers, O.

    2002-01-01

    Understanding the electronic structure of atoms and molecules is fundamental in determining their basic properties as well as the interactions that occur with different particles such as light. One such interaction is single photoionization; a process in which a photon collides with an atom or molecule and an electron with a certain kinetic energy is emitted, leaving behind a residual ion. Theoretical models of electronic structures use the dipole approximation to simplify x-ray interactions by assuming that the electromagnetic field of the radiation, expressed as a Taylor-series expansion, can be simplified by using only the first term. It has been known for some time that the dipole approximation becomes inaccurate at high photon energies, but the threshold at which this discrepancy begins is ambiguous. In order to enhance our understanding of these limitations, we measured the electron emissions of nitrogen. Beamline 8.0.1 at the Advanced Light Source was used with an electron Time-of-Flight (TOF) end station, which measures the time required for electrons emitted to travel a fixed distance. Data were collected over a broad range of photon energies (413 - 664 eV) using five analyzers rotated to 15 chamber angles. Preliminary analysis indicates that these results confirm the breakdown of the dipole approximation at photon energies well below 1 keV and that this breakdown is greatly enhanced in molecules just above the core-level ionization threshold. As a result, new theoretical models must be made that use higher order terms that were previously truncated.

  4. A spin- and angle-resolving photoelectron spectrometer

    CERN Document Server

    Berntsen, M H; Leandersson, M; Hahlin, A; hlund, J \\AA; Wannberg, B; nsson, M M\\aa; Tjernberg, O

    2010-01-01

    A new type of hemispherical electron energy analyzer that permits angle and spin resolved photoelectron spectroscopy has been developed. The analyzer permits standard angle resolved spectra to be recorded with a two-dimensional detector in parallel with spin detection using a mini-Mott polarimeter. General design considerations as well as technical solutions are discussed and test results from the Au(111) surface state are presented.

  5. Angle-resolved photoemission spectroscopy with 9-eV photon-energy pulses generated in a gas-filled hollow-core photonic crystal fiber

    Energy Technology Data Exchange (ETDEWEB)

    Bromberger, H., E-mail: Hubertus.Bromberger@mpsd.mpg.de; Liu, H.; Chávez-Cervantes, M.; Gierz, I. [Max Planck Institute for the Structure and Dynamics of Matter, Luruper Chaussee 149, 22761 Hamburg (Germany); Ermolov, A.; Belli, F.; Abdolvand, A.; Russell, P. St. J.; Travers, J. C. [Max Planck Institute for the Science of Light, Günther-Scharowsky-Str. 1, 91058 Erlangen (Germany); Calegari, F. [Max Planck Institute for the Structure and Dynamics of Matter, Luruper Chaussee 149, 22761 Hamburg (Germany); Institute for Photonics and Nanotechnologies, IFN-CNR, Piazza Leonardo da Vinci 32, I-20133 Milano (Italy); Li, M. T.; Lin, C. T. [Max Planck Institute for Solid State Research, Heisenbergstr. 1, 70569 Stuttgart (Germany); Cavalleri, A. [Max Planck Institute for the Structure and Dynamics of Matter, Luruper Chaussee 149, 22761 Hamburg (Germany); Clarendon Laboratory, Department of Physics, University of Oxford, Parks Rd. Oxford OX1 3PU (United Kingdom)

    2015-08-31

    A recently developed source of ultraviolet radiation, based on optical soliton propagation in a gas-filled hollow-core photonic crystal fiber, is applied here to angle-resolved photoemission spectroscopy (ARPES). Near-infrared femtosecond pulses of only few μJ energy generate vacuum ultraviolet radiation between 5.5 and 9 eV inside the gas-filled fiber. These pulses are used to measure the band structure of the topological insulator Bi{sub 2}Se{sub 3} with a signal to noise ratio comparable to that obtained with high order harmonics from a gas jet. The two-order-of-magnitude gain in efficiency promises time-resolved ARPES measurements at repetition rates of hundreds of kHz or even MHz, with photon energies that cover the first Brillouin zone of most materials.

  6. Exploring electronic structure of one-atom thick polycrystalline graphene films: A nano angle resolved photoemission study

    Science.gov (United States)

    Avila, José; Razado, Ivy; Lorcy, Stéphane; Fleurier, Romain; Pichonat, Emmanuelle; Vignaud, Dominique; Wallart, Xavier; Asensio, María C.

    2013-01-01

    The ability to produce large, continuous and defect free films of graphene is presently a major challenge for multiple applications. Even though the scalability of graphene films is closely associated to a manifest polycrystalline character, only a few numbers of experiments have explored so far the electronic structure down to single graphene grains. Here we report a high resolution angle and lateral resolved photoelectron spectroscopy (nano-ARPES) study of one-atom thick graphene films on thin copper foils synthesized by chemical vapor deposition. Our results show the robustness of the Dirac relativistic-like electronic spectrum as a function of the size, shape and orientation of the single-crystal pristine grains in the graphene films investigated. Moreover, by mapping grain by grain the electronic dynamics of this unique Dirac system, we show that the single-grain gap-size is 80% smaller than the multi-grain gap recently reported by classical ARPES. PMID:23942471

  7. Angle resolved photoemission spectroscopy and surface states

    Science.gov (United States)

    Kar, Nikhiles

    2016-10-01

    Angle Resolved Photo Emission Spectroscopy (ARPES) has been a very effective tool to study the electronic states of solids, from simple metals to complex systems like cuprate superconductors. For photon energy in the range of 10 - 100 eV, it is a surface sensitive process as the free path of the photo emitted electrons is of the order of a few lattice parameters. However to interpret the experimental data one needs to have a theoretical foundation for the photoemission process. From the theory of photoemission it may be seen that one can get information about the state from which the electron has been excited. As the translational periodicity is broken normal to the surface, a new type of electron state in the forbidden energy gap can exist localized in the surface region. ARPES can reveal the existence and the property of such surface states. We shall also discuss briefly how the electromagnetic field of the photons are influenced by the presence of the surface and how one can try to take that into account in photoemission theory.

  8. Electronic structure studies of YBa{sub 2}Cu{sub 3}O{sub x}(6.2 {le} x {le} 6.9) using angle resolved photoemission

    Energy Technology Data Exchange (ETDEWEB)

    Veal, B.W.; Liu, Rong; Paulikas, A.P.; Koelling, D.D.; Downey, J.W. [Argonne National Lab., IL (United States); Shi, Hao [Argonne National Lab., IL (United States)]|[Missouri Univ., Kansas City, MO (United States). Dept. of Physics; Olson, C.G. [Ames Lab., IA (United States); Arko, A.J.; Joyce, J.J.; Blythe, R. [Los Alamos National Lab., NM (United States)

    1992-11-01

    Using high resolution angle resolved photoemission, the electronic structure of YBa{sub 2}Cu{sub 3}O{sub x} is examined when oxygen stoichiometries are varied in the range 6.2 {le} {times} {le} 6.9. Detailed measurements of the Fermi surface for YBa{sub 2}Cu{sub 3}O{sub 6.9} are presented and are compared with predictions of band theory. In the metallic region of the phase diagram, changes in the Fermi surfaces are measured as a function of oxygen stoichiometry. The electronic structure is monitored as the oxide changes from a metal to a semiconductor with additional oxygen depletion. For intermediate stoichiometries, effects of oxygen vacancy ordering are considered. Unusual resonant effects observed at several photon energies are examined as oxygen content is varied.

  9. The electronic structure of clean and adsorbate-covered Bi2Se3: an angle-resolved photoemission study

    DEFF Research Database (Denmark)

    Bianchi, Marco; Hatch, Richard; Guan, Dandan;

    2012-01-01

    , the Dirac point moves to higher binding energies, indicating an increasingly strong downward bending of the bands near the surface. This time-dependent band bending is related to a contamination of the surface and can be accelerated by intentionally exposing the surface to carbon monoxide and other species...

  10. High-resolution angle-resolved photoemission study of the Fermi surface and the normal-state electronic structure of Bi sub 2 Sr sub 2 CaCu sub 2 O sub 8

    Energy Technology Data Exchange (ETDEWEB)

    Olson, C.G.; Liu, R.; Lynch, D.W. (Ames Laboratory, Ames, IA (USA) Physics Department, Iowa State University, Ames, IA (USA)); List, R.S.; Arko, A.J. (Los Alamos National Laboratory, Los Alamos, NM (USA)); Veal, B.W.; Chang, Y.C.; Jiang, P.Z.; Paulikas, A.P. (Argonne National Laboratory, Argonne, IL (USA))

    1990-07-01

    High-resolution angle-resolved photoelectron spectroscopic measurements were made of the Fermi edge of a single crystal of Bi{sub 2}Sr{sub 2}CaCu{sub 2}O{sub 8} at 90 K along several directions in the Brillouin zone. The resultant Fermi-level crossings are consistent with local-density band calculations, including a point calculated to be of Bi-O character. Additional measurements were made where bands crossed the Fermi level between 100 and 250 K, along with measurements on an adjacent Pt foil. The Fermi edges of both materials agree to within the noise. Below the Fermi level the spectra show correlation effects in the form of an increased effective mass, but the essence of the single-particle band structure is retained. The shape of the spectra can be explained by a lifetime-broadened photohole and secondary electrons. The effective inverse photohole lifetime is linear in energy.

  11. Spin-dependent surface electronic structure of Gd(0001) near the Fermi-level: An angle-resolved (I)PE study

    Energy Technology Data Exchange (ETDEWEB)

    Budke, Michael; Wittkowski, Alexander; Correa, Juliet; Donath, Markus [Physikalisches Institut, WWU Muenster, Wilhelm-Klemm-Str. 10, 48149 Muenster (Germany)

    2008-07-01

    A widely accepted picture for the surface electronic structure of Gd(0001) comprises a spin-split surface state (SS) with its majority part 0.2 eV below E{sub F} and its minority part 0.5 eV above E{sub F} with a finite exchange splitting of 0.4 eV at T{sub C}. The discussion about this SS remains controversially because spin-resolved inverse photoemission identified a SS with both minority and majority components above E{sub F}. The reason for these conflicting results might be found in different sample conditions since the Gd films are usually grown on W(110), a material with considerably different lattice constant than Gd. To overcome this suspicion, we performed both, spin- and angle-resolved direct (PE) and inverse photoemission (IPE) on the same sample preparation of a 30 ML Gd film grown on Y(0001). We were able to identify two SSs with their minority and majority components well separated from E{sub F}. While the occupied SS shows spin-mixing behaviour as observed in other PE experiments, the unoccupied SS exhibits an exchange splitting of 250 meV that vanishes at T{sub C}. To identify the nature of the unexpected SS, we performed angular-resolved IPE measurements that support the interpretation as d-like SS above E{sub F} and reveal a variety of additional spectral features.

  12. Level sequence and splitting identification of closely-spaced energy levels by angle-resolved analysis of the fluorescence light

    CERN Document Server

    Wu, Z W; Surzhykov, A; Dong, C Z; Fritzsche, S

    2016-01-01

    The angular distribution and linear polarization of the fluorescence light following the resonant photoexcitation is investigated within the framework of the density matrix and second-order perturbation theory. Emphasis has been placed on "signatures" for determining the level sequence and splitting of intermediate (partially) overlapping resonances, if analyzed as a function of the photon energy of the incident light. Detailed computations within the multiconfiguration Dirac-Fock method have been performed especially for the $1s^{2}2s^{2}2p^{6}3s\\;\\, J_{i}=1/2 \\,+\\, \\gamma_{1} \\:\\rightarrow\\: (1s^{2}2s2p^{6}3s)_{1}3p_{3/2}\\;\\, J=1/2, \\, 3/2 \\:\\rightarrow\\: 1s^{2}2s^{2}2p^{6}3s\\;\\, J_{f}=1/2 \\,+\\, \\gamma_{2}$ photoexcitation and subsequent fluorescence emission of atomic sodium. A remarkably strong dependence of the angular distribution and linear polarization of the $\\gamma_{2}$ fluorescence emission is found upon the level sequence and splitting of the intermediate $(1s^{2}2s2p^{6}3s)_{1}3p_{3/2}\\;\\, J=1/2,...

  13. Electronic structure, Dirac points and Fermi arc surface states in three-dimensional Dirac semimetal Na3Bi from angle-resolved photoemission spectroscopy

    Institute of Scientific and Technical Information of China (English)

    梁爱基; 彭莹莹; 刘艳; 刘德发; 胡成; 赵林; 刘国东; 董晓莉; 张君; M Nakatake; H Iwasawa; 陈朝宇; K Shimada; M Arita; H Namatame; M Taniguchi; 许祖彦; 陈创天; 翁红明; 戴希; 方忠; 周兴江; 王志俊; 石友国; 冯娅; 伊合绵; 谢卓晋; 何少龙; 何俊峰

    2016-01-01

    The three-dimensional (3D) Dirac semimetals have linearly dispersive 3D Dirac nodes where the conduction band and valence band are connected. They have isolated 3D Dirac nodes in the whole Brillouin zone and can be viewed as a 3D counterpart of graphene. Recent theoretical calculations and experimental results indicate that the 3D Dirac semimetal state can be realized in a simple stoichiometric compound A3Bi (A=Na, K, Rb). Here we report comprehensive high-resolution angle-resolved photoemission (ARPES) measurements on the two cleaved surfaces, (001) and (100), of Na3Bi. On the (001) surface, by comparison with theoretical calculations, we provide a proper assignment of the observed bands, and in particular, pinpoint the band that is responsible for the formation of the three-dimensional Dirac cones. We observe clear evidence of 3D Dirac cones in the three-dimensional momentum space by directly measuring on the kx–ky plane and by varying the photon energy to get access to different out-of-plane kzs. In addition, we reveal new features around the Brillouin zone corners that may be related with surface reconstruction. On the (100) surface, our ARPES measurements over a large momentum space raise an issue on the selection of the basic Brillouin zone in the (100) plane. We directly observe two isolated 3D Dirac nodes on the (100) surface. We observe the signature of the Fermi-arc surface states connecting the two 3D Dirac nodes that extend to a binding energy of∼150 meV before merging into the bulk band. Our observations constitute strong evidence on the existence of the Dirac semimetal state in Na3Bi that are consistent with previous theoretical and experimental work. In addition, our results provide new information to clarify on the nature of the band that forms the 3D Dirac cones, on the possible formation of surface reconstruction of the (001) surface, and on the issue of basic Brillouin zone selection for the (100) surface.

  14. Observation by resonant angle-resolved photoemission of a critical thickness for 2-dimensional electron gas formation in SrTiO{sub 3} embedded in GdTiO{sub 3}

    Energy Technology Data Exchange (ETDEWEB)

    Nemšák, S. [Department of Physics, University of California, 1 Shields Ave, Davis, California 95616 (United States); Materials Sciences Division, Lawrence Berkeley National Laboratory, 1 Cyclotron Rd., Berkeley, California 94720 (United States); Peter-Grünberg-Institut PGI-6, Forschungszentrum Jülich, 52425 Jülich (Germany); Conti, G.; Palsson, G. K.; Conlon, C.; Fadley, C. S. [Department of Physics, University of California, 1 Shields Ave, Davis, California 95616 (United States); Materials Sciences Division, Lawrence Berkeley National Laboratory, 1 Cyclotron Rd., Berkeley, California 94720 (United States); Cho, S.; Rault, J. E.; Avila, J.; Asensio, M.-C. [Synchrotron SOLEIL, L' Orme des Merisiers, Saint-Aubin, 91192 Gif sur Yvette Cedex (France); Jackson, C. A.; Moetakef, P.; Janotti, A.; Bjaalie, L.; Himmetoglu, B.; Van de Walle, C. G.; Stemmer, S. [Materials Department, University of California, Santa Barbara, California 93106-5050 (United States); Balents, L. [Department of Physics, University of California, Santa Barbara, California 93106-9530 (United States); Schneider, C. M. [Peter-Grünberg-Institut PGI-6, Forschungszentrum Jülich, 52425 Jülich (Germany)

    2015-12-07

    For certain conditions of layer thickness, the interface between GdTiO{sub 3} (GTO) and SrTiO{sub 3} (STO) in multilayer samples has been found to form a two-dimensional electron gas (2DEG) with very interesting properties including high mobilities and ferromagnetism. We have here studied two trilayer samples of the form [2 nm GTO/1.0 or 1.5 unit cells STO/10 nm GTO] as grown on (001) (LaAlO{sub 3}){sub 0.3}(Sr{sub 2}AlTaO{sub 6}){sub 0.7}, with the STO layer thicknesses being at what has been suggested is the critical thickness for 2DEG formation. We have studied these with Ti-resonant angle-resolved and angle-integrated photoemission and find that the spectral feature in the spectra associated with the 2DEG is present in the 1.5 unit cell sample, but not in the 1.0 unit cell sample. We also observe through core-level spectra additional states in Ti and Sr, with the strength of a low-binding-energy state for Sr being associated with the appearance of the 2DEG, and we suggest it to have an origin in final-state core-hole screening.

  15. Angle-resolved photoemission study of the electronic structures of AuAl{sub 2} and PtGa{sub 2}

    Energy Technology Data Exchange (ETDEWEB)

    Hsu, L.S. [National Chang-Hua Univ. of Education (Taiwan, Province of China). Dept. of Physics; Denlinger, J.D.; Allen, J.W. [Univ. of Michigan, Ann Arbor, MI (United States). Randall Lab.

    1998-12-31

    Synchrotron-radiation-excited angle-resolved photoemission spectra of AuAl{sub 2} and PtGa{sub 2} are presented. Experimental dispersion relations from normal emission spectra are compared to semi-relativistic augmented-plane-wave band-structure calculations. For PtGa{sub 2}, the Pt 5d bands show good agreement within a few tenths of an eV, while for AuAl{sub 2}, the experimental Au 5d band width is {approx} 0.5 eV greater than theory. In addition, polar-angle spectra and Fermi-edge intensity mapping allow the band dispersions of weak s-p bands to be revealed, and a hole pocket centered on the L-point is observed.

  16. Angle-Resolved Light-Matter Interaction in Anisotropic Layered Black Phosphorus

    Science.gov (United States)

    Huang, Shengxi; Ling, Xi; Hasdeo, Eddwi; Liang, Liangbo; Parkin, William; Tatsumi, Yuki; Nugraha, Ahmad; Puretzky, Alexander; Das, Paul; Sumpter, Bobby; Geohegan, David; Kong, Jing; Saito, Riichiro; Drndic, Marija; Meunier, Vincent; Dresselhaus, Mildred

    Orthorhombic black phosphorus (BP) and other layered materials, such as gallium telluride and tin selenide, stand out among two-dimensional (2D) materials owing to their anisotropic in-plane structure. This anisotropy adds a new dimension to the properties of 2D materials and stimulates the development of angle-resolved photonics and electronics. However, understanding the effect of anisotropy has remained unsatisfactory to-date, as shown by a number of inconsistencies in the recent literature. We use angle-resolved absorption and Raman spectroscopies to investigate the role of anisotropy on the electron-photon and electron-phonon interactions in BP. We highlight, both experimentally and theoretically, a non-trivial dependence between anisotropies and flake thickness, photon and phonon energies. We show that the anisotropic optical absorption is a reliable and simple way to identify the crystalline orientation of BP, which cannot be determined from Raman spectroscopy without the explicit consideration of excitation wavelength and flake thickness.

  17. Angle resolved photoemission in semiconductors

    Energy Technology Data Exchange (ETDEWEB)

    Petroff, Y.

    1983-02-01

    Bases of angular resolved photoemission: determination of the electronic band structure of solids (bulk), measurements of life-time and mean free path, determination of surfaces states (valence and core) and their relationship with surface reconstruction are described.

  18. Angle-resolved photoelectron spectroscopy studies of the many-body effects in the electronic structure of high-T{sub c} cuprates

    Energy Technology Data Exchange (ETDEWEB)

    Inosov, Dmytro S.

    2008-06-18

    In the present work some steps are done towards understanding the anomalous effects observed in the single-particle excitation spectra of cuprates. First, the electronic properties of BSCCO are considered. The main result of this part of the work is a model of the Green's function that is later used for calculating the two-particle excitation spectrum. Then, the matrix element effects in the photoemission spectra of cuprates are discussed. After a general introduction to the problem, the thesis focuses on the recently discovered anomalous behavior of the ARPES spectra that partially originates from the momentum-dependent photoemission matrix element. The momentum- and excitation energy dependence of the anomalous high-energy dispersion, termed ''waterfalls'', is covered in full detail. Understanding the role of the matrix element effects in this phenomenon proves crucial, as they obstruct the view of the underlying excitation spectrum that is of indisputable interest. For the optimally doped bilayer Bi-based cuprate, the renormalized two-particle correlation function in the superconducting state is calculated from ARPES data within an itinerant model based on the random phase approximation (RPA). (orig.)

  19. Photoelectron spectroscopy at a free-electron laser. Investigation of space-charge effects in angle-resolved and core-level spectroscopy and realizaton of a time-resolved core-level photoemission experiment

    Energy Technology Data Exchange (ETDEWEB)

    Marczynski-Buehlow, Martin

    2012-01-30

    The free-electron laser (FEL) in Hamburg (FLASH) is a very interesting light source with which to perform photoelectron spectroscopy (PES) experiments. Its special characteristics include highly intense photon pulses (up to 100 J/pulse), a photon energy range of 30 eV to 1500 eV, transverse coherence as well as pulse durations of some ten femtoseconds. Especially in terms of time-resolved PES (TRPES), the deeper lying core levels can be reached with photon energies up to 1500 eV with acceptable intensity now and, therefore, element-specific, time-resolved core-level PES (XPS) is feasible at FLASH. During the work of this thesis various experimental setups were constructed in order to realize angle-resolved (ARPES), core-level (XPS) as well as time-resolved PES experiments at the plane grating monochromator beamline PG2 at FLASH. Existing as well as newly developed systems for online monitoring of FEL pulse intensities and generating spatial and temporal overlap of FEL and optical laser pulses for time-resolved experiments are successfully integrated into the experimental setup for PES. In order to understand space-charge effects (SCEs) in PES and, therefore, being able to handle those effects in future experiments using highly intense and pulsed photon sources, the origin of energetic broadenings and shifts in photoelectron spectra are studied by means of a molecular dynamic N-body simulation using a modified Treecode Algorithm for sufficiently fast and accurate calculations. It turned out that the most influencing parameter is the ''linear electron density'' - the ratio of the number of photoelectrons to the diameter of the illuminated spot on the sample. Furthermore, the simulations could reproduce the observations described in the literature fairly well. Some rules of thumb for XPS and ARPES measurements could be deduced from the simulations. Experimentally, SCEs are investigated by means of ARPES as well as XPS measurements as a function of

  20. Angle-Resolved Spectroscopy of Parametric Fluorescence

    CERN Document Server

    Hsu, Feng-kuo

    2013-01-01

    The parametric fluorescence from a nonlinear crystal forms a conical radiation pattern. We measure the angular and spectral distributions of parametric fluorescence in a beta-barium borate crystal pumped by a 405-nm diode laser employing angle-resolved imaging spectroscopy. The experimental angle-resolved spectra and the generation efficiency of parametric down conversion are compared with a plane-wave theoretical analysis. The parametric fluorescence is used as a broadband light source for the calibration of the instrument spectral response function in the wavelength range from 450 to 1000 nm.

  1. Tuning the electronic structure of bulk FeSe with chemical pressure using quantum oscillations and angle resolved photoemission spectroscopy (ARPES)

    Science.gov (United States)

    Coldea, Amalia

    FeSe is a unique and intriguing superconductor which can be tuned into a high temperature superconducting state using applied pressure, chemical intercalation and surface doping. In the absence of magnetism, the structural transition in FeSe is believed to be electronically driven, with the orbital degrees of freedom playing an important part. This scenario supports the stabilization of a nematic state in FeSe, which manifests as a Fermi surface deformation in the presence of strong interactions, as detected by ARPES. Another manifestation of the nematicity is the enhanced nematic susceptibility determined from elastoresistance measurements under applied strain. Isovalent Sulphur substitution onto the Selenium site constitutes a chemical pressure, which subtly modifies the electronic structure of FeSe, suppressing the structural transition without inducing high temperature superconductivity. I will present the evolution of the electronic structure with chemical pressure in FeSe, as determined from quantum oscillations and ARPES studies and I will discuss the suppression of the nematic electronic state and the role of electronic correlations. Experiments were performed at high magnetic field facilities in Tallahassee, Nijmegen and Toulouse and Diamond Light Source, UK. This work is mainly supported by EPSRC, UK (EP/I004475/1, EP/I017836/1) and I acknowledge my collaborators from Refs. .

  2. High Resolution Angle Resolved Photoemission Studies on Quasi-Particle Dynamics in Graphite

    Energy Technology Data Exchange (ETDEWEB)

    Leem, C.S.

    2010-06-02

    We obtained the spectral function of the graphite H point using high resolution angle resolved photoelectron spectroscopy (ARPES). The extracted width of the spectral function (inverse of the photo-hole lifetime) near the H point is approximately proportional to the energy as expected from the linearly increasing density of states (DOS) near the Fermi energy. This is well accounted by our electron-phonon coupling theory considering the peculiar electronic DOS near the Fermi level. And we also investigated the temperature dependence of the peak widths both experimentally and theoretically. The upper bound for the electron-phonon coupling parameter is 0.23, nearly the same value as previously reported at the K point. Our analysis of temperature dependent ARPES data at K shows that the energy of phonon mode of graphite has much higher energy scale than 125K which is dominant in electron-phonon coupling.

  3. Differential reflectivity and angle-resolved photoemission of PbS(1 0 0)

    Science.gov (United States)

    Cricenti, A.; Tallarida, M.; Ottaviani, C.; Kowalski, B.; Gutievitz, E.; Szczerbakow, A.; Orlowski, B. A.

    2001-06-01

    The surface electronic structure of a PbS sample, cleaved in ultra-high-vacuum environment, has been studied with surface differential reflectivity (SDR) and angle-resolved photoelectron spectroscopy (ARUPS). The ARUPS spectra show the presence of two surface (resonance) states along the two angular directions [0 0 1] and [0 1 1]. SDR shows the existence of a gap of approximately 2.1 eV and two more optical transitions at energies of 2.7 and 3.1 eV. These transitions have been, tentatively, assigned to different points in the surface Brillouin zone.

  4. Direct observation of the mass renormalization in SrVO3 by angle resolved photoemission spectroscopy

    Energy Technology Data Exchange (ETDEWEB)

    Yoshida, t.

    2010-05-03

    We have performed an angle-resolved photoemission study of the three-dimensional perovskite-type SrVO{sub 3}. Observed spectral weight distribution of the coherent part in the momentum space shows cylindrical Fermi surfaces consisting of the V 3d t{sub 2g} orbitals as predicted by local-density approximation (LDA) band-structure calculation. The observed energy dispersion shows a moderately enhanced effective mass compared to the LDA results, corresponding to the effective mass enhancement seen in the thermodynamic properties. Contributions from the bulk and surface electronic structures to the observed spectra are discussed based on model calculations.

  5. Angle-resolved photoemission study of Ag(1 1 1)

    Science.gov (United States)

    Edamoto, K.; Miyazaki, E.; Shimokoshi, K.; Kato, H.

    1990-01-01

    The (1 1 1) face of Ag has been studied by angle-resolved photoemission spectroscopy utilizing synchrotron radiation as the excitation source (25 FIRO method. The peak positions thus determined are used to map the dispersion curves along the lang1 1 1rang (Γ-L) direction. The results show general agreement with calculated band structure, so far as the energy levels and symmetries are concerned. However, it is found that the density of state effect is dominant in the spectra obtained in the present photon energy region. The emission from the Ag 5s, p bands is observed to be broadened due to the indirect transition process.

  6. Development of a high resolution laser based angle-resolving time-of-flight photoelectron spectrometer

    CERN Document Server

    Berntsen, M H; Tjernberg, O

    2011-01-01

    We present the design and performance of a novel Laser-based Angle-Resolving Time-of-Flight (LARTOF) system for photoemission from solids in the vacuum ultraviolet (VUV) energy range. A pulsed laser provides photons which through a third harmonic generation (THG) process performed in a xenon filled gas cell generates VUV photons of energy 10.5 eV. The time-of-flight analyzer is able to collect all electrons that are emitted from the sample within a circular cone of up to +/-15 degrees. By simultaneously measuring the energy and emission angle along two spatial directions for the electrons the analyzer provides three-dimensional detection capability. Data from a test measurement performed on the Au(111) surface state is presented along with some more advanced measurements of the Fermi surface of the high-temperature superconductor Bi2212.

  7. Angle resolved photoemission spectroscopy reveals spin charge separation in metallic MoSe2 grain boundary

    Science.gov (United States)

    Ma, Yujing; Diaz, Horacio Coy; Avila, José; Chen, Chaoyu; Kalappattil, Vijaysankar; Das, Raja; Phan, Manh-Huong; Čadež, Tilen; Carmelo, José M. P.; Asensio, Maria C.; Batzill, Matthias

    2017-02-01

    Material line defects are one-dimensional structures but the search and proof of electron behaviour consistent with the reduced dimension of such defects has been so far unsuccessful. Here we show using angle resolved photoemission spectroscopy that twin-grain boundaries in the layered semiconductor MoSe2 exhibit parabolic metallic bands. The one-dimensional nature is evident from a charge density wave transition, whose periodicity is given by kF/π, consistent with scanning tunnelling microscopy and angle resolved photoemission measurements. Most importantly, we provide evidence for spin- and charge-separation, the hallmark of one-dimensional quantum liquids. Our studies show that the spectral line splits into distinctive spinon and holon excitations whose dispersions exactly follow the energy-momentum dependence calculated by a Hubbard model with suitable finite-range interactions. Our results also imply that quantum wires and junctions can be isolated in line defects of other transition metal dichalcogenides, which may enable quantum transport measurements and devices.

  8. Angle-resolved photoemission study of quasi one-dimensional TlInSe{sub 2}

    Energy Technology Data Exchange (ETDEWEB)

    Mimura, Kojiro [Department of Mathematical Sciences, Graduate School of Engineering, Osaka Prefecture University, Sakai 599-8531 (Japan)], E-mail: mimura@ms.osakafu-u.ac.jp; Wakita, Kazuki [Department of Physics and Electronics, Graduate School of Engineering, Osaka Prefecture University, Sakai 599-8531 (Japan); Arita, Masashi [Hiroshima Synchrotron Radiation Center, Hiroshima University, Higashi-Hiroshima 739-0046 (Japan); Mamedov, Nazim; Orudzhev, Guseyn [Institute of Physics, Azerbaijan National Academy of Science, Baku, AZ-1143 (Azerbaijan); Taguchi, Yukihiro; Ichikawa, Kouichi [Department of Mathematical Sciences, Graduate School of Engineering, Osaka Prefecture University, Sakai 599-8531 (Japan); Namatame, Hirofumi; Taniguchi, Masaki [Hiroshima Synchrotron Radiation Center, Hiroshima University, Higashi-Hiroshima 739-0046 (Japan)

    2007-05-15

    TlInSe{sub 2} with a quasi one-dimensional chain structure and a giant Seebeck coefficient of more than 10{sup 6} {mu}V/K below 140 {sup o}C has been investigated by means of angle-resolved photoemission spectroscopy at 50 K and 280 K. The obtained energy bands favorably agree with the calculated band structure and show quite noticeable dispersion in the direction normal to the chains. A rigid shift toward lower binding energies, a splitting and the formation of the mini-gap-like structures are clearly observed in the experimental electronic bands with the temperature reduced to 50 K. These features are indicative of an incommensurate superlattice phase emerging in TlInSe{sub 2} with temperature, and causing the record-breaking values of Seebeck coefficient.

  9. Highly Angle-Resolved X-Ray Photoelectron Diffraction from Solid Surfaces

    Science.gov (United States)

    Tamura, K.; Shiraki, S.; Ishii, H.; Owari, M.; Nihei, Y.

    We have carried out the highly angle-resolved X-ray photoelectron diffraction (XPED) measurements by using the input-lens system for restriction of the detection angle. In the input-lens system, high angular resolution and high throughput are accomplished by placing an aperture not on the image plane but on the diffraction plane of electron optics. The aperture sizes (ϕ 4 mm, ϕ 2 mm, ϕ 0.5 mm, ϕ 0.25 mm) correspond to the angular resolutions (± 0.6°, ± 0.3°, ± 0.08°, ± 0.04°) respectively. Highly angle-resolved Ge3d XPED patterns from Ge(111) obtained by the angle-resolving system contain fine structure such as Kikuchi patterns. The fine structure was reproduced by multiple scattering cluster calculations.

  10. Precision angle-resolved autoionization resonances in Ar and Ne

    Energy Technology Data Exchange (ETDEWEB)

    Berrah, N.; Langer, B.; Gorczyca, T.W. [Western Michigan Univ., Kalamazoo, MI (United States)] [and others

    1997-04-01

    Theoretical work has shown that the electron angular distribution and the shape of the autoionization resonances are crucial to the understanding of certain types of electron-electron correlation. Autoionization resonances in Ne (Ar) result from the decay of the excited discrete state Ne{sup *} 2s2p{sup 6} np (Ar{sup *} 3s3p{sup 6} np) into the continuum state Ne{sup +} 2s{sup 2}2p{sup 5} + e{sup {minus}} (ks,kd) (Ar{sup +} 3s{sup 2}3p{sup 5} + e{sup {minus}} (ks,kd)). Since the continuum can also be reached by direct photoionization, both paths add coherently, giving rise to interferences that produce the characteristic Beutler-Fano line shape. In this work, the authors report on quantitative angle-resolved electron spectrometry studies of (a) the Ne 2s{sup 2}2p{sup 6} {r_arrow} 2s2p{sup 6} np (n=3-5) autoionizing resonances and the 2s{sup 2}2p{sup 6} {r_arrow} 2p{sup 4}3s3p doubly excited resonance, (b) the Ar 3s{sup 2}3p{sup 6} {r_arrow} 3s3p{sup 6} np (n=4-9) autoionization resonances and extended R-matrix calculations of the angular-distribution parameters for both Ne and Ar measurements. Their results are compared with previous theoretical work by Taylor.

  11. Phonon-assisted indirect transitions in angle-resolved photoemission spectra of graphite and graphene

    Science.gov (United States)

    Ayria, Pourya; Tanaka, Shin-ichiro; Nugraha, Ahmad R. T.; Dresselhaus, Mildred S.; Saito, Riichiro

    2016-08-01

    Indirect transitions of electrons in graphene and graphite are investigated by means of angle-resolved photoemission spectroscopy (ARPES) with several different incident photon energies and light polarizations. The theoretical calculations of the indirect transition for graphene and for a single crystal of graphite are compared with the experimental measurements for highly-oriented pyrolytic graphite and a single crystal of graphite. The dispersion relations for the transverse optical (TO) and the out-of-plane longitudinal acoustic (ZA) phonon modes of graphite and the TO phonon mode of graphene can be extracted from the inelastic ARPES intensity. We find that the TO phonon mode for k points along the Γ -K and K -M -K' directions in the Brillouin zone can be observed in the ARPES spectra of graphite and graphene by using a photon energy ≈11.1 eV. The relevant mechanism in the ARPES process for this case is the resonant indirect transition. On the other hand, the ZA phonon mode of graphite can be observed by using a photon energy ≈6.3 eV through a nonresonant indirect transition, while the ZA phonon mode of graphene within the same mechanism should not be observed.

  12. Invited Article: High resolution angle resolved photoemission with tabletop 11 eV laser

    Energy Technology Data Exchange (ETDEWEB)

    He, Yu; Vishik, Inna M.; Yi, Ming; Yang, Shuolong; Lee, James J.; Chen, Sudi; Rebec, Slavko N.; Leuenberger, Dominik; Shen, Zhi-Xun [SIMES, SLAC National Accelerator Laboratory, Menlo Park, California 94025 (United States); Department of Applied Physics, Stanford University, Stanford, California 94305 (United States); Liu, Zhongkai [SIMES, SLAC National Accelerator Laboratory, Menlo Park, California 94025 (United States); Department of Physics, Stanford University, Stanford, California 94305 (United States); Zong, Alfred [Department of Physics, Stanford University, Stanford, California 94305 (United States); Jefferson, C. Michael; Merriam, Andrew J. [Lumeras LLC, 207 McPherson St, Santa Cruz, California 95060 (United States); Moore, Robert G.; Kirchmann, Patrick S. [SIMES, SLAC National Accelerator Laboratory, Menlo Park, California 94025 (United States)

    2016-01-15

    We developed a table-top vacuum ultraviolet (VUV) laser with 113.778 nm wavelength (10.897 eV) and demonstrated its viability as a photon source for high resolution angle-resolved photoemission spectroscopy (ARPES). This sub-nanosecond pulsed VUV laser operates at a repetition rate of 10 MHz, provides a flux of 2 × 10{sup 12} photons/s, and enables photoemission with energy and momentum resolutions better than 2 meV and 0.012 Å{sup −1}, respectively. Space-charge induced energy shifts and spectral broadenings can be reduced below 2 meV. The setup reaches electron momenta up to 1.2 Å{sup −1}, granting full access to the first Brillouin zone of most materials. Control over the linear polarization, repetition rate, and photon flux of the VUV source facilitates ARPES investigations of a broad range of quantum materials, bridging the application gap between contemporary low energy laser-based ARPES and synchrotron-based ARPES. We describe the principles and operational characteristics of this source and showcase its performance for rare earth metal tritellurides, high temperature cuprate superconductors, and iron-based superconductors.

  13. High Resolution Angle Resolved Photoemission with Tabletop 11eV Laser

    CERN Document Server

    He, Yu; Yi, Ming; Yang, Shuolong; Liu, Zhongkai; Lee, James; Chen, Sudi; Rebec, Slavko; Leuenberger, Dominik; Zong, Alfred; Jefferson, Michael; Moore, Robert; Kirchmann, Patrick; Merriam, Andrew; Shen, Zhixun

    2015-01-01

    We developed a table-top vacuum ultraviolet (VUV) laser with $113.778$nm wavelength (10.897eV) and demonstrated its viability as a photon source for high resolution angle-resolved photoemission spectroscopy (ARPES). This sub-nanosecond pulsed VUV laser operates at a repetition rate of 10MHz, provides a flux of 2$\\times$10$^{12}$ photons/second, and enables photoemission with energy and momentum resolutions better than 2meV and 0.012\\AA$^{-1}$, respectively. Space-charge induced energy shifts and spectral broadenings can be reduced below 2meV. The setup reaches electron momenta up to 1.2\\AA$^{-1}$, granting full access to the first Brillouin zone of most materials. Control over the linear polarization, repetition rate, and photon flux of the VUV source facilitates ARPES investigations of a broad range of quantum materials, bridging the application gap between contemporary low energy laser-based ARPES and synchrotron-based ARPES. We describe the principles and operational characteristics of this source, and sho...

  14. Angle-resolved ion TOF spectrometer with a position sensitive detector

    Energy Technology Data Exchange (ETDEWEB)

    Saito, Norio [Electrotechnical Lab., Tsukuba, Ibaraki (Japan); Heiser, F.; Wieliczec, K.; Becker, U.

    1996-07-01

    A angle-resolved ion time-of-flight mass spectrometer with a position sensitive anode has been investigated. Performance of this spectrometer has been demonstrated by measuring an angular distribution of a fragment ion pair, C{sup +} + O{sup +}, from CO at the photon energy of 287.4 eV. The obtained angular distribution is very close to the theoretically expected one. (author)

  15. Fermi surfaces of YBa sub 2 Cu sub 3 O sub 6. 9 as seen by angle-resolved photoemission

    Energy Technology Data Exchange (ETDEWEB)

    Campuzano, J.C.; Jennings, G.; Faiz, M.; Beaulaigue, L.; Veal, B.W.; Liu, J.Z.; Paulikas, A.P.; Vandervoort, K.; Claus, H. (Argonne National Laboratory, 9700 South Cass Avenue, Argonne, IL (USA) University of Illinois at Chicago, Chicago, IL (USA)); List, R.S.; Arko, A.J.; Bartlett, R.J. (Los Alamos National Laboratory, Los Alamos, NM (USA))

    1990-05-07

    We have carried out angle-resolved photoemission spectroscopy on single crystals of YBa{sub 2}Cu{sub 3}O{sub 6.9}. The crystals were cleaved {ital in} {ital situ}, under ultrahigh vacuum while the sample stage was cooled to 8 K. By observing the dispersion of the electron energy bands as they cross the Fermi energy, we have mapped the Fermi surfaces. There is reasonable agreement between the experimental results and the predictions of band-structure calculations using the local-density approximation, as well as with positron annihilation experiments. Rather than {delta} holes, these results indicate that the Fermi surface of YBa{sub 2}Cu{sub 3}O{sub 6.9} encloses 1+{delta} holes, where {delta} is the doping level.

  16. Angle-resolved diffraction grating biosensor based on porous silicon

    Science.gov (United States)

    Lv, Changwu; Jia, Zhenhong; Liu, Yajun; Mo, Jiaqing; Li, Peng; Lv, Xiaoyi

    2016-03-01

    In this study, an optical biosensor based on a porous silicon composite structure was fabricated using a simple method. This structure consists of a thin, porous silicon surface diffraction grating and a one-dimensional porous silicon photonic crystal. An angle-resolved diffraction efficiency spectrum was obtained by measuring the diffraction efficiency at a range of incident angles. The angle-resolved diffraction efficiency of the 2nd and 3rd orders was studied experimentally and theoretically. The device was sensitive to the change of refractive index in the presence of a biomolecule indicated by the shift of the diffraction efficiency spectrum. The sensitivity of this sensor was investigated through use of an 8 base pair antifreeze protein DNA hybridization. The shifts of the angle-resolved diffraction efficiency spectrum showed a relationship with the change of the refractive index, and the detection limit of the biosensor reached 41.7 nM. This optical device is highly sensitive, inexpensive, and simple to fabricate. Using shifts in diffraction efficiency spectrum to detect biological molecules has not yet been explored, so this study establishes a foundation for future work.

  17. Band structures of 4f and 5f materials studied by angle-resolved photoelectron spectroscopy

    Science.gov (United States)

    Fujimori, Shin-ichi

    2016-04-01

    Recent remarkable progress in angle-resolved photoelectron spectroscopy (ARPES) has enabled the direct observation of the band structures of 4f and 5f materials. In particular, ARPES with various light sources such as lasers (hν ∼ 7~\\text{eV} ) or high-energy synchrotron radiations (hν ≳ 400~\\text{eV} ) has shed light on the bulk band structures of strongly correlated materials with energy scales of a few millielectronvolts to several electronvolts. The purpose of this paper is to summarize the behaviors of 4f and 5f band structures of various rare-earth and actinide materials observed by modern ARPES techniques, and understand how they can be described using various theoretical frameworks. For 4f-electron materials, ARPES studies of \\text{Ce}M\\text{I}{{\\text{n}}5} (M=\\text{Rh} , \\text{Ir} , and \\text{Co} ) and \\text{YbR}{{\\text{h}}2}\\text{S}{{\\text{i}}2} with various incident photon energies are summarized. We demonstrate that their 4f electronic structures are essentially described within the framework of the periodic Anderson model, and that the band-structure calculation based on the local density approximation cannot explain their low-energy electronic structures. Meanwhile, electronic structures of 5f materials exhibit wide varieties ranging from itinerant to localized states. For itinerant \\text{U}~5f compounds such as \\text{UFeG}{{\\text{a}}5} , their electronic structures can be well-described by the band-structure calculation assuming that all \\text{U}~5f electrons are itinerant. In contrast, the band structures of localized \\text{U}~5f compounds such as \\text{UP}{{\\text{d}}3} and \\text{U}{{\\text{O}}2} are essentially explained by the localized model that treats \\text{U}~5f electrons as localized core states. In regards to heavy fermion \\text{U} -based compounds such as the hidden-order compound \\text{UR}{{\\text{u}}2}\\text{S}{{\\text{i}}2} , their electronic structures exhibit complex behaviors. Their overall band structures

  18. Direct angle resolved photoemission spectroscopy and superconductivity of strained high-c films

    Indian Academy of Sciences (India)

    Davor Pavuna; Daniel Ariosa; Dominique Cloetta; Claudia Cancellieri; Mike Abrecht

    2008-02-01

    Since 1997 we systematically perform direct angle resolved photoemission spectroscopy (ARPES) on in-situ grown thin (< 30 nm) cuprate films. Specifically, we probe low-energy electronic structure and properties of high-c superconductors (HTSC) under different degrees of epitaxial (compressive vs. tensile) strain. In overdoped and underdoped in-plane compressed (the strain is induced by the choice of substrate) ≃ 15 nm thin La2-SrCuO4 (LSCO) films we almost double c to 40 K, from 20 K and 24 K, respectively. Yet the Fermi surface (FS) remains essentially two-dimensional. In contrast, ARPES data under tensile strain exhibit the dispersion that is three-dimensional, yet c drastically decreases. It seems that the in-plane compressive strain tends to push the apical oxygen far away from the CuO2 plane, enhances the two-dimensional character of the dispersion and increases c, while the tensile strain acts in the opposite direction and the resulting dispersion is three-dimensional. We have established the shape of the FS for both cases, and all our data are consistent with other ongoing studies, like EXAFS. As the actual lattice of cuprates is like a `Napoleon-cake', i.e. rigid CuO2 planes alternating with softer `reservoir', that distort differently under strain, our data rule out all oversimplified two-dimensional (rigid lattice) mean field models. The work is still in progress on optimized La-doped Bi-2201 films with enhanced c.

  19. Depth-Resolved Composition and Electronic Structure of Buried Layers and Interfaces in a LaNiO{sub 3}/SrTiO{sub 3} Superlattice from Soft- and Hard- X-ray Standing-Wave Angle-Resolved Photoemission

    Energy Technology Data Exchange (ETDEWEB)

    Eiteneer, D. [Department of Physics, University of California, Davis, California 95616 (United States); Materials Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, California 94720 (United States); Pálsson, G.K., E-mail: gunnar.palsson@physics.uu.se [Department of Physics, University of California, Davis, California 95616 (United States); Materials Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, California 94720 (United States); Nemšák, S. [Department of Physics, University of California, Davis, California 95616 (United States); Materials Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, California 94720 (United States); Peter-Grünberg-Institut PGI-6, Forschungszentrum Julich, 52425 Julich (Germany); Gray, A.X. [Department of Physics, University of California, Davis, California 95616 (United States); Materials Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, California 94720 (United States); Stanford Institute for Materials and Energy Sciences, SLAC National Accelerator Laboratory, Menlo Park, California 94025 (United States); Kaiser, A.M. [Department of Physics, University of California, Davis, California 95616 (United States); Materials Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, California 94720 (United States); Son, J.; LeBeau, J. [Materials Department, University of California, Santa Barbara, California 93106 (United States); Conti, G. [Department of Physics, University of California, Davis, California 95616 (United States); Materials Sciences Division, Lawrence Berkeley National Laboratory, Berkeley, California 94720 (United States); and others

    2016-08-15

    Highlights: • Depth resolved electronic structure of LaNiO{sub 3}/SrTiO{sub 3} superlattices is measured. • The structure is determined by x-ray standing wave angle-resolved photoemission. • Similarity to the electronic structure of La{sub 0.7}Sr{sub 0.3}MnO{sub 3}/SrTiO{sub 3} is discussed. - Abstract: LaNiO{sub 3} (LNO) is an intriguing member of the rare-earth nickelates in exhibiting a metal-insulator transition for a critical film thickness of about 4 unit cells [Son et al., Appl. Phys. Lett. 96, 062114 (2010)]; however, such thin films also show a transition to a metallic state in superlattices with SrTiO{sub 3} (STO) [Son et al., Appl. Phys. Lett. 97, 202109 (2010)]. In order to better understand this transition, we have studied a strained LNO/STO superlattice with 10 repeats of [4 unit-cell LNO/3 unit-cell STO] grown on an (LaAlO{sub 3}){sub 0.3}(Sr{sub 2}AlTaO{sub 6}){sub 0.7} substrate using soft x-ray standing-wave-excited angle-resolved photoemission (SWARPES), together with soft- and hard- x-ray photoemission measurements of core levels and densities-of-states valence spectra. The experimental results are compared with state-of-the-art density functional theory (DFT) calculations of band structures and densities of states. Using core-level rocking curves and x-ray optical modeling to assess the position of the standing wave, SWARPES measurements are carried out for various incidence angles and used to determine interface-specific changes in momentum-resolved electronic structure. We further show that the momentum-resolved behavior of the Ni 3d e{sub g} and t{sub 2g} states near the Fermi level, as well as those at the bottom of the valence bands, is very similar to recently published SWARPES results for a related La{sub 0.7}Sr{sub 0.3}MnO{sub 3}/SrTiO{sub 3} superlattice that was studied using the same technique (Gray et al., Europhysics Letters 104, 17004 (2013)), which further validates this experimental approach and our conclusions. Our

  20. Tetragonal and collapsed-tetragonal phases of CaFe2As2 : A view from angle-resolved photoemission and dynamical mean-field theory

    Science.gov (United States)

    van Roekeghem, Ambroise; Richard, Pierre; Shi, Xun; Wu, Shangfei; Zeng, Lingkun; Saparov, Bayrammurad; Ohtsubo, Yoshiyuki; Qian, Tian; Sefat, Athena S.; Biermann, Silke; Ding, Hong

    2016-06-01

    We present a study of the tetragonal to collapsed-tetragonal transition of CaFe2As2 using angle-resolved photoemission spectroscopy and dynamical mean field theory-based electronic structure calculations. We observe that the collapsed-tetragonal phase exhibits reduced correlations and a higher coherence temperature due to the stronger Fe-As hybridization. Furthermore, a comparison of measured photoemission spectra and theoretical spectral functions shows that momentum-dependent corrections to the density functional band structure are essential for the description of low-energy quasiparticle dispersions. We introduce those using the recently proposed combined "screened exchange + dynamical mean field theory" scheme.

  1. The electronic structure of La{sub 0.66}Ca{sub 0.33}MnO{sub 3} and La{sub 1.2}Sr{sub 1.8}Mn{sub 2}O{sub 7} studied by angle resolved photoemission

    Energy Technology Data Exchange (ETDEWEB)

    Liu, Rong [Department of Physics, Michigan State University, East Lansing, Michigan 48824 (United States); Tonjes, W. C. [Department of Physics, Michigan State University, East Lansing, Michigan 48824 (United States); Olson, C. G. [Ames Laboratory, Ames, Iowa 50011 (United States); Joyce, J. J. [Los Alamos National Laboratory, Los Alamos, New Mexico 87545 (United States); Arko, A. J. [Los Alamos National Laboratory, Los Alamos, New Mexico 87545 (United States); Neumeier, J. J. [Los Alamos National Laboratory, Los Alamos, New Mexico 87545 (United States); Mitchell, J. F. [Materials Science Division, Argonne National Laboratory, Argonne, Illinois 60439 (United States); Zheng, H. [Materials Science Division, Argonne National Laboratory, Argonne, Illinois 60439 (United States)

    2000-07-15

    We report angle resolved photoemission studies of La{sub 0.66}Ca{sub 0.33}MnO{sub 3} and La{sub 1.2}Sr{sub 1.8}Mn{sub 2}O{sub 7} using single crystal samples. The Mn 3p-3d resonance photoemission data of La{sub 0.66}Ca{sub 0.33}MnO{sub 3} show that the states at 2.5 eV binding energy have predominantly Mn 3d character, qualitatively consistent with the predictions of local spin density approximation calculations except for a 1 eV shift toward higher binding energy. Band dispersions are observed in the normal emission data. The spectra of La{sub 1.2}Sr{sub 1.8}Mn{sub 2}O{sub 7} show well defined features and strong matrix element effects, indicating excellent surface quality. (c) 2000 American Institute of Physics.

  2. Angle-resolved effective potentials for disk-shaped molecules

    Energy Technology Data Exchange (ETDEWEB)

    Heinemann, Thomas, E-mail: thomas.heinemann@tu-berlin.de; Klapp, Sabine H. L., E-mail: klapp@physik.tu-berlin.de [Institut für Theoretische Physik, Technische Universität Berlin, Hardenbergstr. 36, 10623 Berlin (Germany); Palczynski, Karol, E-mail: karol.palczynski@helmholtz-berlin.de; Dzubiella, Joachim, E-mail: joachim.dzubiella@helmholtz-berlin.de [Institut für Physik, Humboldt Universität zu Berlin, Newtonstraße 15, 12489 Berlin (Germany); Helmholtz Zentrum Berlin (HZB), Institute of Soft Matter and Functional Materials, Hahn-Meitner Platz 1, 14109 Berlin (Germany)

    2014-12-07

    We present an approach for calculating coarse-grained angle-resolved effective pair potentials for uniaxial molecules. For integrating out the intramolecular degrees of freedom we apply umbrella sampling and steered dynamics techniques in atomistically-resolved molecular dynamics (MD) computer simulations. Throughout this study we focus on disk-like molecules such as coronene. To develop the methods we focus on integrating out the van der Waals and intramolecular interactions, while electrostatic charge contributions are neglected. The resulting coarse-grained pair potential reveals a strong temperature and angle dependence. In the next step we fit the numerical data with various Gay-Berne-like potentials to be used in more efficient simulations on larger scales. The quality of the resulting coarse-grained results is evaluated by comparing their pair and many-body structure as well as some thermodynamic quantities self-consistently to the outcome of atomistic MD simulations of many-particle systems. We find that angle-resolved potentials are essential not only to accurately describe crystal structures but also for fluid systems where simple isotropic potentials start to fail already for low to moderate packing fractions. Further, in describing these states it is crucial to take into account the pronounced temperature dependence arising in selected pair configurations due to bending fluctuations.

  3. Angle-resolved effective potentials for disk-shaped molecules.

    Science.gov (United States)

    Heinemann, Thomas; Palczynski, Karol; Dzubiella, Joachim; Klapp, Sabine H L

    2014-12-07

    We present an approach for calculating coarse-grained angle-resolved effective pair potentials for uniaxial molecules. For integrating out the intramolecular degrees of freedom we apply umbrella sampling and steered dynamics techniques in atomistically-resolved molecular dynamics (MD) computer simulations. Throughout this study we focus on disk-like molecules such as coronene. To develop the methods we focus on integrating out the van der Waals and intramolecular interactions, while electrostatic charge contributions are neglected. The resulting coarse-grained pair potential reveals a strong temperature and angle dependence. In the next step we fit the numerical data with various Gay-Berne-like potentials to be used in more efficient simulations on larger scales. The quality of the resulting coarse-grained results is evaluated by comparing their pair and many-body structure as well as some thermodynamic quantities self-consistently to the outcome of atomistic MD simulations of many-particle systems. We find that angle-resolved potentials are essential not only to accurately describe crystal structures but also for fluid systems where simple isotropic potentials start to fail already for low to moderate packing fractions. Further, in describing these states it is crucial to take into account the pronounced temperature dependence arising in selected pair configurations due to bending fluctuations.

  4. Nodal Quasiparticle Meltdown in Ultra-High Resolution Pump-Probe Angle-Resolved Photoemission

    Energy Technology Data Exchange (ETDEWEB)

    Graf, Jeff; Jozwiak, Chris; Smallwood, Chris L.; Eisaki, H.; Kaindl, Robert A.; Lee, Dung-Hai; Lanzara, Alessandra

    2011-06-03

    High-T{sub c} cuprate superconductors are characterized by a strong momentum-dependent anisotropy between the low energy excitations along the Brillouin zone diagonal (nodal direction) and those along the Brillouin zone face (antinodal direction). Most obvious is the d-wave superconducting gap, with the largest magnitude found in the antinodal direction and no gap in the nodal direction. Additionally, while antin- odal quasiparticle excitations appear only below T{sub c}, superconductivity is thought to be indifferent to nodal excitations as they are regarded robust and insensitive to T{sub c}. Here we reveal an unexpected tie between nodal quasiparticles and superconductivity using high resolution time- and angle-resolved photoemission on optimally doped Bi{sub 2}Sr{sub 2}CaCu{sub 2}O{sub 8+{delta}} . We observe a suppression of the nodal quasiparticle spectral weight following pump laser excitation and measure its recovery dynamics. This suppression is dramatically enhanced in the superconducting state. These results reduce the nodal-antinodal dichotomy and challenge the conventional view of nodal excitation neutrality in superconductivity. The electronic structures of high-Tc cuprates are strongly momentum-dependent. This is one reason why the momentum-resolved technique of angle-resolved photoemission spectroscopy (ARPES) has been a central tool in the field of high-temperature superconductivity. For example, coherent low energy excitations with momenta near the Brillouin zone face, or antinodal quasiparticles (QPs), are only observed below T{sub c} and have been linked to superfluid density. They have therefore been the primary focus of ARPES studies. In contrast, nodal QPs, with momenta along the Brillouin zone diagonal, have received less attention and are usually regarded as largely immune to the superconducting transition because they seem insensitive to perturbations such as disorder, doping, isotope exchange, charge ordering, and temperature. Clearly

  5. Application of a time-of-flight spectrometer with delay-line detector for time- and angle-resolved two-photon photoemission

    Energy Technology Data Exchange (ETDEWEB)

    Damm, A. [Fachbereich Physik und Zentrum für Materialwissenschaften, Philipps-Universität, D-35032 Marburg (Germany); Güdde, J., E-mail: Jens.Guedde@physik.uni-marburg.de [Fachbereich Physik und Zentrum für Materialwissenschaften, Philipps-Universität, D-35032 Marburg (Germany); Feulner, P. [Physikdepartment E20, Technische Universität München, 85747 Garching (Germany); Czasch, A.; Jagutzki, O.; Schmidt-Böcking, H. [Institut für Kernphysik, Goethe-Universität, D-60438 Frankfurt am Main (Germany); RoentDek Handels GmbH, D-65779 Kelkheim (Germany); Höfer, U. [Fachbereich Physik und Zentrum für Materialwissenschaften, Philipps-Universität, D-35032 Marburg (Germany)

    2015-07-15

    Highlights: • The performance of a 2D time-of-flight electron spectrometer is demonstrated. • We discuss its application for time- and angle-resolved two-photon photoemission. • The decay dynamics of the first image-potential state on Cu(1 0 0) is investigated. • We find an azimuthal anisotropy of the decay rate with one-fold symmetry. • The anisotropy is attributed to residual steps on the nominal flat surface. - Abstract: We describe the design and operation of a time-of-flight electron spectrometer which is capable of simultaneously acquiring the energy and momentum distribution of low-energy photoelectrons in two dimensions parallel to the surface. We discuss its capabilities and limitations in particular for time- and angle-resolved two-photon photoemission (2PPE) with pulsed lasers. The performance of the spectrometer is demonstrated by presenting 2PPE data on the momentum-dependent electron dynamics of the first (n = 1) image-potential state on Cu(0 0 1). The data reveal a weak but systematic dependence of the decay dynamics on sample azimuth with one-fold symmetry which we attribute to a small residual step density on the nominal flat surface.

  6. Direct angle resolved photoemission spectroscopy and superconductivity of strained high-Tc films

    Science.gov (United States)

    Pavuna, Davor; Ariosa, Daniel; Cloetta, Dominique; Cancellieri, Claudia; Abrecht, Mike

    2008-02-01

    Since 1997 we systematically perform direct angle resolved photoemission spectroscopy (ARPES) on in-situ grown thin (<30 nm) cuprate films. Specifically, we probe low-energy electronic structure and properties of high-T_{c} superconductors (HTSC) under different degrees of epitaxial ({compressive vs. tensile}) strain. In overdoped and underdoped in-plane compressed (the strain is induced by the choice of substrate) ≈15 nm thin La_{2-x}Sr_{x}CuO_{4} (LSCO) films we almost double T_{c} to 40 K, from 20 K and 24 K, respectively. Yet the Fermi surface (FS) remains essentially two-dimensional. In contrast, ARPES data under {tensile} strain exhibit the dispersion that is three-dimensional, yet T_{c} drastically decreases. It seems that the in-plane compressive strain tends to push the apical oxygen far away from the CuO_{2} plane, enhances the two-dimensional character of the dispersion and increases T_{c}, while the tensile strain acts in the opposite direction and the resulting dispersion is three-dimensional. We have established the shape of the FS for both cases, and all our data are consistent with other ongoing studies, like EXAFS. As the actual lattice of cuprates is like a `Napoleon-cake', i.e. rigid CuO_{2 } planes alternating with softer `reservoir', that distort differently under strain, our data rule out all oversimplified two-dimensional (rigid lattice) mean field models. The work is still in progress on optimized La-doped Bi-2201 films with enhanced T_{c}.

  7. Angle-Resolved Plasmonic Properties of Single Gold Nanorod Dimers

    Institute of Scientific and Technical Information of China (English)

    Jian Wu; Xuxing Lu; Qiannan Zhu; Junwei Zhao; Qishun Shen; Li Zhan; Weihai Ni

    2014-01-01

    Through wet-chemical assembly methods, gold nanorods were placed close to each other and formed a dimer with a gap distance*1 nm, and hence degenerated plasmonic dipole modes of individual nanorods coupled together to produce hybridized bonding and antibonding resonance modes. Previous studies using a condenser for illumination result in averaged signals over all excitation angles. By exciting an individual dimer obliquely at different angles, we demonstrate that these two new resonance modes are highly tunable and sensitive to the angle between the excitation polarization and the dimer orientation, which follows cos2u dependence. Moreover, for dimer structures with various structure angles, the resonance wavelengths as well as the refractive index sensitivities were found independent of the structure angle. Cal-culated angle-resolved plasmonic properties are in good agreement with the measurements. The assembled nanostructures investigated here are important for fundamental researches as well as potential applications when they are used as building blocks in plasmon-based optical and optoelectronic devices.

  8. First-principles approach to excitons in time-resolved and angle-resolved photoemission spectra

    Science.gov (United States)

    Perfetto, E.; Sangalli, D.; Marini, A.; Stefanucci, G.

    2016-12-01

    In this work we put forward a first-principles approach and propose an accurate diagrammatic approximation to calculate the time-resolved (TR) and angle-resolved photoemission spectrum of systems with excitons. We also derive an alternative formula to the TR photocurrent which involves a single time-integral of the lesser Green's function. The diagrammatic approximation applies to the relaxed regime characterized by the presence of quasistationary excitons and vanishing polarization. The nonequilibrium self-energy diagrams are evaluated using excited Green's functions; since this is not standard, the analytic derivation is presented in detail. The final result is an expression for the lesser Green's function in terms of quantities that can all be calculated in a first-principles manner. The validity of the proposed theory is illustrated in a one-dimensional model system with a direct gap. We discuss possible scenarios and highlight some universal features of the exciton peaks. Our results indicate that the exciton dispersion can be observed in TR and angle-resolved photoemission.

  9. Angle-resolved multioctave supercontinua from mid-infrared laser filaments.

    Science.gov (United States)

    Mitrofanov, A V; Voronin, A A; Sidorov-Biryukov, D A; Mitryukovsky, S I; Rozhko, M V; Pugžlys, A; Fedotov, A B; Panchenko, V Ya; Baltuška, A; Zheltikov, A M

    2016-08-01

    Angle-resolved spectral analysis of a multioctave high-energy supercontinuum output of mid-infrared laser filaments is shown to provide a powerful tool for understanding intricate physical scenarios behind laser-induced filamentation in the mid-infrared. The ellipticity of the mid-infrared driver beam breaks the axial symmetry of filamentation dynamics, offering a probe for a truly (3+1)-dimensional spatiotemporal evolution of mid-IR pulses in the filamentation regime. With optical harmonics up to the 15th order contributing to supercontinuum generation in such filaments alongside Kerr-type and ionization-induced nonlinearities, the output supercontinuum spectra span over five octaves from the mid-ultraviolet deep into the mid-infrared. Full (3+1)-dimensional field evolution analysis is needed for an adequate understanding of this regime of laser filamentation. Supercomputer simulations implementing such analysis articulate the critical importance of angle-resolved measurements for both descriptive and predictive power of filamentation modeling. Strong enhancement of ionization-induced blueshift is shown to offer new approaches in filamentation-assisted pulse compression, enabling the generation of high-power few- and single-cycle pulses in the mid-infrared.

  10. Modeling angle-resolved photoemission of graphene and black phosphorus nano structures.

    Science.gov (United States)

    Park, Sang Han; Kwon, Soonnam

    2016-05-10

    Angle-resolved photoemission spectroscopy (ARPES) data on electronic structure are difficult to interpret, because various factors such as atomic structure and experimental setup influence the quantum mechanical effects during the measurement. Therefore, we simulated ARPES of nano-sized molecules to corroborate the interpretation of experimental results. Applying the independent atomic-center approximation, we used density functional theory calculations and custom-made simulation code to compute photoelectron intensity in given experimental setups for every atomic orbital in poly-aromatic hydrocarbons of various size, and in a molecule of black phosphorus. The simulation results were validated by comparing them to experimental ARPES for highly-oriented pyrolytic graphite. This database provides the calculation method and every file used during the work flow.

  11. Angle-resolved photoemission spectroscopy (ARPES) studies of cuprate superconductors

    Energy Technology Data Exchange (ETDEWEB)

    Palczewski, Ari Deibert [Iowa State Univ., Ames, IA (United States)

    2010-01-01

    This dissertation is comprised of three different angle-resolved photoemission spectroscopy (ARPES) studies on cuprate superconductors. The first study compares the band structure from two different single layer cuprates Tl2Ba2CuO6+δ (Tl2201) Tc, max ≈ 95 K and (Bi 1.35Pb0.85)(Sr1.47La0.38)CuO6+δ (Bi2201) Tc, max ≈ 35 K. The aim of the study was to provide some insight into the reasons why single layer cuprate's maximum transition temperatures are so different. The study found two major differences in the band structure. First, the Fermi surface segments close to (π,0) are more parallel in Tl2201 than in Bi2201. Second, the shadow band usually related to crystal structure is only present in Bi2201, but absent in higher Tc Tl2201. The second study looks at the different ways of doping Bi2Sr2CaCu2O8+δ (Bi2212) in-situ by only changing the post bake-out vacuum conditions and temperature. The aim of the study is to systematically look into the generally overlooked experimental conditions that change the doping of a cleaved sample in ultra high vacuum (UHV) experiments. The study found two major experimental facts. First, in inadequate UHV conditions the carrier concentration of Bi2212 increases with time, due to the absorption of oxygen from CO2/CO molecules, prime contaminants present in UHV systems. Second, in a very clean UHV system at elevated temperatures (above about 200 K), the carrier concentration decreases due to the loss of oxygen atoms from the Bi-O layer. The final study probed the particle-hole symmetry of the pseudogap phase in high temperature superconducting cuprates by looking at the thermally excited bands above the Fermi level. The data showed a particle-hole symmetric pseudogap which symmetrically closes away from the nested FS before the node. The data is

  12. Tunable VUV laser based spectrometer for Angle Resolved Photoemission Spectroscopy (ARPES)

    CERN Document Server

    Jiang, Rui; Wu, Yun; Huang, Lunan; McMillen, Colin D; Kolis, Joseph; Giesber, Henry G; Egan, John J; Kaminski, Adam

    2014-01-01

    We have developed an angle-resolved photoemission spectrometer with tunable VUV laser as a photon source. The photon source is based on the fourth harmonic generation of a near IR beam from a Ti:sapphire laser pumped by a CW green laser and tunable between 5.3eV and 7eV. The most important part of the set-up is a compact, vacuum enclosed fourth harmonic generator based on KBBF crystals, grown hydrothermally in the US. This source can deliver a photon flux of over 10^14 photons/s. We demonstrate that this energy range is sufficient to measure the kz dispersion in an iron arsenic high temperature superconductor, which was previously only possible at synchrotron facilities.

  13. Angle-resolved photoemission studies of the superconducting gap symmetry in Fe-based superconductors

    Directory of Open Access Journals (Sweden)

    Y.-B. Huang

    2012-12-01

    Full Text Available The superconducting gap is the fundamental parameter that characterizes the superconducting state, and its symmetry is a direct consequence of the mechanism responsible for Cooper pairing. Here we discuss about angle-resolved photoemission spectroscopy measurements of the superconducting gap in the Fe-based high-temperature superconductors. We show that the superconducting gap is Fermi surface dependent and nodeless with small anisotropy, or more precisely, a function of the momentum location in the Brillouin zone. We show that while this observation seems inconsistent with weak coupling approaches for superconductivity in these materials, it is well supported by strong coupling models and global superconducting gaps. We also suggest that a smaller lifetime of the superconducting Cooper pairs induced by the momentum dependent interband scattering inherent to these materials could affect the residual density of states at low energies, which is critical for a proper evaluation of the superconducting gap.

  14. Anomalous asymmetry in the Fermi surface of the high-temperature superconductor YBa2Cu4O8 revealed by angle-resolved photoemission spectroscopy

    Energy Technology Data Exchange (ETDEWEB)

    Kondo, Takeshi; Khasanov, R.; Sassa, Y.; Bendounan, A.; Paihes, S.; Chang, J.; Mesot, J.; Keller, H.; Zhigadlo, N.D.; Shi, M.; Bukowski, Z.; Karpinski, J.; Kaminski, A.

    2009-09-15

    We use microprobe angle-resolved photoemission spectroscopy to study the Fermi surface and band dispersion of the CuO{sub 2} planes in the high-temperature superconductor, YBa{sub 2}Cu{sub 4}O{sub 8}. We find a strong in-plane asymmetry of the electronic structure between directions along a and b axes. The saddle point of the antibonding band lies at a significantly higher energy in the a direction ({pi},0) than the b direction (0,{pi}), whereas the bonding band displays the opposite behavior. We demonstrate that the abnormal band shape is due to a strong asymmetry of the bilayer band splitting, likely caused by a nontrivial hybridization between the planes and chains. This asymmetry has an important implication for interpreting key properties of the Y-Ba-Cu-O family, especially the superconducting gap, transport, and results of inelastic neutron scattering.

  15. Angle resolved x-ray photoelectron spectroscopy (ARXPS) analysis of lanthanum oxide for micro-flexography printing

    Energy Technology Data Exchange (ETDEWEB)

    Hassan, S., E-mail: suhaimihas@uthm.edu.my; Yusof, M. S., E-mail: mdsalleh@uthm.edu.my; Maksud, M. I., E-mail: midris1973@gmail.com [Faculty of Mechanical and Manufacturing Engineering, Universiti Tun Hussein Onn Malaysia, 86400 Batu Pahat, Johor (Malaysia); Embong, Z., E-mail: zaidi@uthm.edu.my [Faculty of Science, Technology and Human Development, Universiti Tun Hussein Onn Malaysia, 86400 Batu Pahat, Johor (Malaysia)

    2016-01-22

    Micro-flexography printing was developed in patterning technique from micron to nano scale range to be used for graphic, electronic and bio-medical device on variable substrates. In this work, lanthanum oxide (La{sub 2}O{sub 3}) has been used as a rare earth metal candidate as depositing agent. This metal deposit was embedded on Carbon (C) and Silica (Si) wafer substrate using Magnetron Sputtering technique. The choose of Lanthanum as a target is due to its wide application in producing electronic devices such as thin film battery and printed circuit board. The La{sub 2}O{sub 3} deposited on the surface of Si wafer substrate was then analyzed using Angle Resolve X-Ray Photoelectron Spectroscopy (ARXPS). The position for each synthetic component in the narrow scan of Lanthanum (La) 3d and O 1s are referred to the electron binding energy (eV). The La 3d narrow scan revealed that the oxide species of this particular metal is mainly contributed by La{sub 2}O{sub 3} and La(OH){sub 3}. The information of oxygen species, O{sup 2-} component from O 1s narrow scan indicated that there are four types of species which are contributed from the bulk (O{sup 2−}), two chemisorb component (La{sub 2}O{sub 3}) and La(OH){sub 3} and physisorp component (OH). Here, it is proposed that from the adhesive and surface chemical properties of La, it is suitable as an alternative medium for micro-flexography printing technique in printing multiple fine solid lines at nano scale. Hence, this paper will describe the capability of this particular metal as rare earth metal for use in of micro-flexography printing practice. The review of other parameters contributing to print fine lines will also be described later.

  16. Angle-resolved X-ray photoelectron spectroscopy (ARXPS) and a modified Levenberg-Marquardt fit procedure: a new combination for modeling thin layers

    NARCIS (Netherlands)

    Aarnink, W.A.M.; Weishaupt, A.; Silfhout, van A.

    1990-01-01

    The combination of angle-resolved X-ray photoelectron spectroscopy (ARXPS) and a modified Levenberg-Marquardt (LM) fit procedure has been used to study a native oxide layer on a clean Si(100) substrate. Numerical calculations show that with an aperture of 3° or 9° of the electron analyser, the photo

  17. Insights from angle-resolved photoemission spectroscopy on the metallic states of YbB6(001): E(k) dispersion, temporal changes, and spatial variation

    NARCIS (Netherlands)

    Frantzeskakis, E.; de Jong, N.; Zhang, J.X.; Zhang, X.; Li, Z.; Liang, C.L.; Wang, Y.; Varykhalov, A.; Huang, Y.K.; Golden, M.S.

    2014-01-01

    We report high-resolution angle-resolved photoelectron spectroscopy (ARPES) results on the (001) cleavage surface of YbB6, a rare-earth compound that has been recently predicted to host surface electronic states with topological character. We observe two types of well-resolved metallic states, whose

  18. High-resolution angle-resolved photoemission investigation of potassium and phosphate tungsten bronzes

    Energy Technology Data Exchange (ETDEWEB)

    Paul, Sanhita; Kumari, Spriha; Raj, Satyabrata, E-mail: raj@iiserkol.ac.in

    2016-04-15

    Highlights: • Electronic structure of potassium and phosphate tungsten bronzes. • Origin of transport anomalies in bronzes. • Flat segments of Fermi surfaces are connected by a nesting vector, q. • Nesting driven charge-density wave is responsible for the anomalies. - Abstract: We have performed high-resolution angle-resolved photoemission spectroscopy (ARPES) and density functional ab initio theoretical calculation to study the electronic structure of potassium (K{sub 0.25}WO{sub 3}) and phosphate (P{sub 4}W{sub 12}O{sub 44}) tungsten bronzes. We have experimentally determined the band dispersions and Fermi surface topology of these bronzes and compared with our theoretical calculations and a fair agreement has been seen between them. Our experimental as well as theoretical investigation elucidates the origin of transport anomalies in these bronzes. The Fermi surfaces of these bronzes consist of flat patches, which can be connected with each other by a constant nesting wave vector, q. The scattering wave vectors found from diffraction measurements match with these nesting vectors and the anomalies in the transport properties of these bronzes can be well explained by the evolution of charge-density wave with a partial nesting between the flat segments of the Fermi surfaces.

  19. Spin- and angle-resolved photoemission spectroscopy study of the Au(1 1 1) Shockley surface state

    Energy Technology Data Exchange (ETDEWEB)

    Muntwiler, Matthias E-mail: m.muntwiler@physik.unizh.ch; Hoesch, Moritz; Petrov, Vladimir N.; Hengsberger, Matthias; Patthey, Luc; Shi Ming; Falub, Mihaela; Greber, Thomas; Osterwalder, Juerg

    2004-07-01

    The spin character of the splitting of the Shockley surface state on Au(111) is directly verified by measurements of the in-plane and out-of-plane spin polarizations in angle-resolved photoemission spectra. The two parabolic sub-bands that are momentum-shifted with respect to each other, reveal a distinct, opposite spin polarization that within the errors lies in the surface plane. The measured in-plane orientation of the spin vectors is consistent with the simple spin structure expected from a nearly-free-electron model, where the polarization axis is tangential to the Fermi surface of the surface state.

  20. Angle Resolved Performance Measurements on PV Glass and Modules

    DEFF Research Database (Denmark)

    Juutilainen, Line Tollund; Thorsteinsson, Sune; Poulsen, Peter Behrensdorff

    2016-01-01

    The angular response of PV-modules has significant impact on the energy production. This is especially pronounced in BIPV where installation angles often are far from optimal. Nevertheless, a gain in energy yield may be obtained by choosing a proper glass as superstrate. In this work we present...... the concept of PV balconies as cost efficient and easy way of integrating PV into buildings. The experimental work consists of the fabrication of single cell mini modules with different glass covering, and characterizing their angular response in a custom made setup, where only the direct sunlight is used...

  1. Angle-resolved neutralization-reionization mass spectrometry.

    Science.gov (United States)

    Fura, A; Turecek, F; McLafferty, F W

    1991-12-01

    Neutralization -reionization mass spectra of 2-propenal, isomeric butenes, and isomeric n-hexenes have been found to depend significantly on the z-axis scattering angle of the neutralization event. As shown by Cooks for ion dissociations, increasing scattering angles generally favor products of higher activation-energy reactions. For isomeric butenes and n-hexenes, these reactions provide more definitive information for isomeric characterization.

  2. Angle-Resolved Auger Spectroscopy as a Sensitive Access to Vibronic Coupling

    Science.gov (United States)

    Knie, A.; Patanen, M.; Hans, A.; Petrov, I. D.; Bozek, J. D.; Ehresmann, A.; Demekhin, Ph. V.

    2016-05-01

    In the angle-averaged excitation and decay spectra of molecules, vibronic coupling may induce the usually weak dipole-forbidden transitions by the excitation intensity borrowing mechanism. The present complementary theoretical and experimental study of the resonant Auger decay of core-to-Rydberg excited CH4 and Ne demonstrates that vibronic coupling plays a decisive role in the formation of the angle-resolved spectra by additionally involving the decay rate borrowing mechanism. Thereby, we propose that the angle-resolved Auger spectroscopy can in general provide very insightful information on the strength of the vibronic coupling.

  3. Fringing field correction of the second-order angular aberration in sector field electron energy analyzers

    Energy Technology Data Exchange (ETDEWEB)

    Yavor, M.I. [Institute for Analytical Instrumentation RAS, 190103 St. Petersburg (Russian Federation)], E-mail: mikhail.yavor@gmail.com; Belov, V.D.; Pomozov, T.V. [Institute for Analytical Instrumentation RAS, 190103 St. Petersburg (Russian Federation)

    2008-12-15

    A new way of correcting the second-order angular aberration in sector field and polar-toroidal electron energy analyzers with object and image located outside the field is proposed. Correction is performed by biasing the optic axis electrostatic potential inside the analyzer with respect to the potential of surrounding field-free space. The strength of the correcting aberration concentrated in the fringing field regions of the analyzer is calculated with the aid of the fringing field integral method. The described correction allows achieving second-order focusing and thus increasing the energy resolving power in sector field analyzers, in particular used for angle resolved energy measurements.

  4. Gantry-angle resolved VMAT pretreatment verification using EPID image prediction

    Energy Technology Data Exchange (ETDEWEB)

    Woodruff, Henry C.; Rowshanfarzad, Pejman [School of Mathematical and Physical Sciences, The University of Newcastle, NSW 2308 (Australia); Fuangrod, Todsaporn [School of Electrical Engineering and Computer Science, The University of Newcastle, NSW 2308 (Australia); McCurdy, Boyd M. C. [Division of Medical Physics, CancerCare Manitoba, 675 McDermot Avenue, Winnipeg, Manitoba R3E 0V9 (Canada); Department of Physics and Astronomy, University of Manitoba, Winnipeg, Manitoba R3T 2N2 (Canada); Department of Radiology, University of Manitoba, Winnipeg, Manitoba R3T 2N2 (Canada); Greer, Peter B. [School of Mathematical and Physical Sciences, The University of Newcastle, NSW 2308, Australia and Department of Radiation Oncology, Calvary Mater Newcastle Hospital, Locked Bag 7, Hunter region Mail Centre, Newcastle, NSW 2310 (Australia)

    2013-08-15

    Purpose: Pretreatment verification of volumetric modulated arc therapy (VMAT) dose delivery with electronic portal imaging device (EPID) uses images integrated over the entire delivery or over large subarcs. This work aims to develop a new method for gantry-angle-resolved verification of VMAT dose delivery using EPID.Methods: An EPID dose prediction model was used to calculate EPID images as a function of gantry angle for eight prostate patient deliveries. EPID image frames at 7.5 frames per second were acquired during delivery via a frame-grabber system. The gantry angle for each image was encoded in kV frames which were synchronized to the MV frames. Gamma analysis results as a function of gantry angle were assessed by integrating the frames over 2° subarcs with an angle-to-agreement tolerance of 0.5° about the measured image angle.Results: The model agreed with EPID images integrated over the entire delivery with average Gamma pass-rates at 2%, 2 mm of 99.7% (10% threshold). The accuracy of the kV derived gantry angle for each image was found to be 0.1° (1 SD) using a phantom test. For the gantry-resolved analysis all Gamma pass-rates were greater than 90% at 3%, 3 mm criteria (with only two exceptions), and more than 90% had a 95% pass-rate, with an average of 97.3%. The measured gantry angle lagged behind the predicted angle by a mean of 0.3°± 0.3°, with a maximum lag of 1.3°.Conclusions: The method provides a comprehensive and highly efficient pretreatment verification of VMAT delivery using EPID. Dose delivery accuracy is assessed as a function of gantry angle to ensure accurate treatment.

  5. Angle-resolved photoemission observation of Mn-pnictide hybridization and negligible band structure renormalization in BaMn2As2 and BaMn2Sb2

    Science.gov (United States)

    Zhang, W.-L.; Richard, P.; van Roekeghem, A.; Nie, S.-M.; Xu, N.; Zhang, P.; Miao, H.; Wu, S.-F.; Yin, J.-X.; Fu, B. B.; Kong, L.-Y.; Qian, T.; Wang, Z.-J.; Fang, Z.; Sefat, A. S.; Biermann, S.; Ding, H.

    2016-10-01

    We performed an angle-resolved photoemission spectroscopy study of BaMn2As2 and BaMn2Sb2 , which are isostructural to the parent compound BaFe2As2 of the 122 family of ferropnictide superconductors. We show the existence of a strongly kz-dependent band gap with a minimum at the Brillouin zone center, in agreement with their semiconducting properties. Despite the half filling of the electronic 3 d shell, we show that the band structure in these materials is almost not renormalized from the Kohn-Sham bands of density functional theory. Our photon-energy-dependent study provides evidence for Mn-pnictide hybridization, which may play a role in tuning the electronic correlations in these compounds.

  6. Angle-resolved soft X-ray magnetic circular dichroism in a monatomic Fe layer facing an MgO(0 0 1) tunnel barrier

    Energy Technology Data Exchange (ETDEWEB)

    Mamiya, K. [Photon Factory, Institute of Materials Structure Science (IMSS), High Energy Accelerator Research Organization, 1-1 Oho, Tsukuba, Ibaraki 305-0801 (Japan); Koide, T. [Photon Factory, Institute of Materials Structure Science (IMSS), High Energy Accelerator Research Organization, 1-1 Oho, Tsukuba, Ibaraki 305-0801 (Japan)]. E-mail: tsuneharu.koide@kek.jp; Ishida, Y. [Department of Complexity Science and Engineering, University of Tokyo, 5-1-5 Kashiwanoha, Kashiwa, Chiba 277-8561 (Japan); Osafune, Y. [Department of Complexity Science and Engineering, University of Tokyo, 5-1-5 Kashiwanoha, Kashiwa, Chiba 277-8561 (Japan); Fujimori, A. [Department of Complexity Science and Engineering, University of Tokyo, 5-1-5 Kashiwanoha, Kashiwa, Chiba 277-8561 (Japan); Suzuki, Y. [Graduate School of Engineering Science, Osaka University, 1-3 Toyonaka, Osaka 560-8531 (Japan); NanoElectronics Research Institute, National Institute of Advanced Industrial Science and Technology (AIST), Tsukuba, Ibaraki 305-8568 (Japan); Katayama, T. [NanoElectronics Research Institute, National Institute of Advanced Industrial Science and Technology (AIST), Tsukuba, Ibaraki 305-8568 (Japan); Yuasa, S. [NanoElectronics Research Institute, National Institute of Advanced Industrial Science and Technology (AIST), Tsukuba, Ibaraki 305-8568 (Japan)

    2006-11-15

    The electronic and magnetic states of a monatomic Fe(0 0 1) layer directly facing an MgO(0 0 1) tunnel barrier were studied by angle-resolved X-ray magnetic circular dichroism (XMCD) at the Fe L {sub 2,3} edges in the longitudinal (L) and transverse (T) arrangements. A strong XMCD reveals no oxidation of the 1-ML Fe, showing its crucial role in giant tunnel magnetoresistance effects in Fe/MgO/Fe magnetic tunnel junctions. Sum-rule analyses of the angle-resolved XMCD give values of a spin moment, in-plane and out-of-plane orbital and magnetic dipole moments. Argument is given on their physical implication.

  7. Gauge invariance in the theoretical description of time-resolved angle-resolved pump/probe photoemission spectroscopy

    Energy Technology Data Exchange (ETDEWEB)

    Freericks, J. K.; Krishnamurthy, H. R.; Sentef, M. A.; Devereaux, T. P.

    2015-10-01

    Nonequilibrium calculations in the presence of an electric field are usually performed in a gauge, and need to be transformed to reveal the gauge-invariant observables. In this work, we discuss the issue of gauge invariance in the context of time-resolved angle-resolved pump/probe photoemission. If the probe is applied while the pump is still on, one must ensure that the calculations of the observed photocurrent are gauge invariant. We also discuss the requirement of the photoemission signal to be positive and the relationship of this constraint to gauge invariance. We end by discussing some technical details related to the perturbative derivation of the photoemission spectra, which involve processes where the pump pulse photoexcites electrons due to nonequilibrium effects.

  8. Soft X-ray angle-resolved photoemission spectroscopy of heavily boron-doped superconducting diamond films

    Directory of Open Access Journals (Sweden)

    T. Yokoya, T. Nakamura, T. Matushita, T. Muro, H. Okazaki, M. Arita, K. Shimada, H. Namatame, M. Taniguchi, Y. Takano, M. Nagao, T. Takenouchi, H. Kawarada and T. Oguchi

    2006-01-01

    Full Text Available We have performed soft X-ray angle-resolved photoemission spectroscopy (SXARPES of microwave plasma-assisted chemical vapor deposition diamond films with different B concentrations in order to study the origin of the metallic behavior of superconducting diamond. SXARPES results clearly show valence band dispersions with a bandwidth of ~23 eV and with a top of the valence band at gamma point in the Brillouin zone, which are consistent with the calculated valence band dispersions of pure diamond. Boron concentration-dependent band dispersions near the Fermi level (EF exhibit a systematic shift of EF, indicating depopulation of electrons due to hole doping. These SXARPES results indicate that diamond bands retain for heavy boron doping and holes in the diamond band are responsible for the metallic states leading to superconductivity at low temperature. A high-resolution photoemission spectroscopy spectrum near EF of a heavily boron-doped diamond superconductor is also presented.

  9. Angle resolved characterization of nanostructured and conventionally textured silicon solar cells

    DEFF Research Database (Denmark)

    Davidsen, Rasmus Schmidt; Ormstrup, Jeppe; Ommen, Martin Lind;

    2015-01-01

    We report angle resolved characterization of nanostructured and conventionally textured silicon solar cells. The nanostructured solar cells are realized through a single step, mask-less, scalable reactive ion etching (RIE) texturing of the surface. Photovoltaic properties including short circuit...... current, open circuit voltage, fill factor (FF) and power conversion efficiency are each measured as function of the relative incident angle between the solar cell and the light source. The relative incident angle is varied from 0° to 90° in steps of 10° in orthogonal axes, such that each solar cell...... is characterized at 100 different angle combinations. The angle resolved photovoltaic properties are summarized in terms of the average, angle-dependent electrical power output normalized to the power output at normal incidence and differently textured cells on different silicon substrates are compared in terms...

  10. Spectral data of specular reflectance, narrow-angle transmittance and angle-resolved surface scattering of materials for solar concentrators.

    Science.gov (United States)

    Good, Philipp; Cooper, Thomas; Querci, Marco; Wiik, Nicolay; Ambrosetti, Gianluca; Steinfeld, Aldo

    2016-03-01

    The spectral specular reflectance of conventional and novel reflective materials for solar concentrators is measured with an acceptance angle of 17.5 mrad over the wavelength range 300-2500 nm at incidence angles 15-60° using a spectroscopic goniometry system. The same experimental setup is used to determine the spectral narrow-angle transmittance of semi-transparent materials for solar collector covers at incidence angles 0-60°. In addition, the angle-resolved surface scattering of reflective materials is recorded by an area-scan CCD detector over the spectral range 350-1050 nm. A comprehensive summary, discussion, and interpretation of the results are included in the associated research article "Spectral reflectance, transmittance, and angular scattering of materials for solar concentrators" in Solar Energy Materials and Solar Cells.

  11. High energy electron cooling

    Energy Technology Data Exchange (ETDEWEB)

    Parkhomchuk, V. [Budker Institute of Nuclear Physics, Novosibirsk (Russian Federation)

    1997-09-01

    High energy electron cooling requires a very cold electron beam. The questions of using electron cooling with and without a magnetic field are presented for discussion at this workshop. The electron cooling method was suggested by G. Budker in the middle sixties. The original idea of the electron cooling was published in 1966. The design activities for the NAP-M project was started in November 1971 and the first run using a proton beam occurred in September 1973. The first experiment with both electron and proton beams was started in May 1974. In this experiment good result was achieved very close to theoretical prediction for a usual two component plasma heat exchange.

  12. High-resolution angle-resolved photoemission studies of high Tc superconductor Bi sub 2 Sr sub 2 CaCu sub 2 O sub 8

    Energy Technology Data Exchange (ETDEWEB)

    Liu, Rong.

    1990-09-21

    An angle-resolved photoemission study of the normal and superconducting states in Bi{sub 2}Sr{sub 2}CaCu{sub 2}O{sub 8} was performed. Measurements in the normal state show bands dispersing through the Fermi level from at least 350 meV below E{sub F}. The Fermi level crossings are consistant with local-density band calculation, including a point calculated to be of Bi-O character. Additional measurements were made where bands crossed the Fermi level between 100 and 250K, along with measurements on an adjacent Pt foil. The Fermi edges of both materials agree to within the noise. Below the Fermi level, the spectra show correlation effects on the form of an increased effective mass. The shape of the spectra can be explained by a lifetime-broadened photohole and secondary electrons. The effective inverse photohole lifetime is linear in energy. A superconducting gap has been measured at a number of points where there is density at the Fermi level in the normal state. By proper modeling, a gap of 24 meV was obtained for all these points, including points of Cu-O and Bi-O character respectively, according to band calculation. The lack of gap anisotropy in the basal plane suggests that pinning in this material is not d-wave pairing.

  13. Structural studies of molecular and metallic overlayers using angle- resolved photoemission extended fine structure

    Energy Technology Data Exchange (ETDEWEB)

    Huang, Z.

    1992-10-01

    Angle-resolved photoemission extended fine structure (ARPEFS) was used to study molecular and metallic overlayers on metal surfaces through analysis of p2mg(2[times]1)CO/Ni(110) and the p(2[times]2)K/Ni(111) adsorption. For the dense p2mg(2[times]1)CO/Ni(110) surface layer, photoemission intensities from C 1s level were measured in three directions at photoelectron kinetic energies 60-400 eV. Using multiple-scattering spherical-wave (MSSW) modeling, it was found that CO molecules are adsorbed on short-bridge sites, with adjacent CO along the [110] direction displaced alternatively in opposite directions towards the [001] azimuths to form a zigzag chain geometry. The tilt angle is 16[plus minus]2[degree] from the surface normal for the direction linking the C atom and the center of the Ni bridge. The carbon C-Ni interatomic distance was determined to be 1.94[plus minus]0.02[Angstrom]. The first- to second-layer spacing of Ni is 1.27[plus minus]0.04[Angstrom], up from 1.10[Angstrom] for the clean Ni(110) surface, but close to the 1.25[Angstrom] Ni interlayer spacing in the bulk. The C-O bond length and tilt angle were varied within small ranges (1.10--1.20[Angstrom] and 15--23[degrees]) in our MSSW simulations. Best agreement between experiment and simulations was achieved at 1.16[Angstrom] and 19[degrees]. This yields an O-O distance of 2.95[Angstrom] for the two nearest CO molecules, (van der Waals' radius [approximately] 1.5 [Angstrom] for oxygen). Two different partial-wave phase-shifts were used in MSSW, and structural results from both are in very good agreement. For the p(2[times]2)K/Ni(111) overlayer, ARPEFS [chi](k) curves from K 1s level measured along [111] and [771] at 130K showed that the K atoms are preferentially adsorbed on the atop sites, in agreement with a LEED study of the same system.

  14. Structural studies of molecular and metallic overlayers using angle- resolved photoemission extended fine structure

    Energy Technology Data Exchange (ETDEWEB)

    Huang, Z.

    1992-10-01

    Angle-resolved photoemission extended fine structure (ARPEFS) was used to study molecular and metallic overlayers on metal surfaces through analysis of p2mg(2{times}1)CO/Ni(110) and the p(2{times}2)K/Ni(111) adsorption. For the dense p2mg(2{times}1)CO/Ni(110) surface layer, photoemission intensities from C 1s level were measured in three directions at photoelectron kinetic energies 60-400 eV. Using multiple-scattering spherical-wave (MSSW) modeling, it was found that CO molecules are adsorbed on short-bridge sites, with adjacent CO along the [110] direction displaced alternatively in opposite directions towards the [001] azimuths to form a zigzag chain geometry. The tilt angle is 16{plus_minus}2{degree} from the surface normal for the direction linking the C atom and the center of the Ni bridge. The carbon C-Ni interatomic distance was determined to be 1.94{plus_minus}0.02{Angstrom}. The first- to second-layer spacing of Ni is 1.27{plus_minus}0.04{Angstrom}, up from 1.10{Angstrom} for the clean Ni(110) surface, but close to the 1.25{Angstrom} Ni interlayer spacing in the bulk. The C-O bond length and tilt angle were varied within small ranges (1.10--1.20{Angstrom} and 15--23{degrees}) in our MSSW simulations. Best agreement between experiment and simulations was achieved at 1.16{Angstrom} and 19{degrees}. This yields an O-O distance of 2.95{Angstrom} for the two nearest CO molecules, (van der Waals` radius {approximately} 1.5 {Angstrom} for oxygen). Two different partial-wave phase-shifts were used in MSSW, and structural results from both are in very good agreement. For the p(2{times}2)K/Ni(111) overlayer, ARPEFS {chi}(k) curves from K 1s level measured along [111] and [771] at 130K showed that the K atoms are preferentially adsorbed on the atop sites, in agreement with a LEED study of the same system.

  15. Laser angle-resolved photoemission as a probe of initial state kz dispersion, final-state band gaps, and spin texture of Dirac states in the Bi2Te3 topological insulator

    Science.gov (United States)

    Ä; rrälä, Minna; Hafiz, Hasnain; Mou, Daixiang; Wu, Yun; Jiang, Rui; Riedemann, Trevor; Lograsso, Thomas A.; Barbiellini, Bernardo; Kaminski, Adam; Bansil, Arun; Lindroos, Matti

    2016-10-01

    We have obtained angle-resolved photoemission spectroscopy (ARPES) spectra from single crystals of the topological insulator material Bi2Te3 using a tunable laser spectrometer. The spectra were collected for 11 different photon energies ranging from 5.57 to 6.70 eV for incident light polarized linearly along two different in-plane directions. Parallel first-principles, fully relativistic computations of photointensities were carried out using the experimental geometry within the framework of the one-step model of photoemission. A reasonable overall accord between theory and experiment is used to gain insight into how properties of the initial- and final-state band structures as well as those of the topological surface states and their spin textures are reflected in the laser-ARPES spectra. Our analysis reveals that laser-ARPES is sensitive to both the initial-state kz dispersion and the presence of delicate gaps in the final-state electronic spectrum.

  16. Simple surface structure determination from Fourier transforms of angle-resolved photoemission extended fine structure

    Energy Technology Data Exchange (ETDEWEB)

    Zheng, Y. [Pennsylvania State Univ., University Park, PA (United States)]|[Lawrence Berkeley Lab., CA (United States); Shirley, D.A. [Pennsylvania State Univ., University Park, PA (United States)

    1995-02-01

    The authors show by Fourier analyses of experimental data, with no further treatment, that the positions of all the strong peaks in Fourier transforms of angle-resolved photoemission extended fine structure (ARPEFS) from adsorbed surfaces can be explicitly predicted from a trial structure with an accuracy of about {+-} 0.3 {angstrom} based on a single-scattering cluster model together with the concept of a strong backscattering cone, and without any additional analysis. This characteristic of ARPEFS Fourier transforms can be developed as a simple method for determining the structures of adsorbed surfaces to an accuracy of about {+-} 0.1 {angstrom}.

  17. Angle-Resolved Scatter Measurements of Laser Damaged DKDP Crystals Using a Bi-Directional Scatter Diagnostics

    Energy Technology Data Exchange (ETDEWEB)

    Fluck, R; Wegner, P; Sheehan, L; Hackel, L A

    2000-12-22

    We built a bi-directional scatter diagnostics to measure and quantify losses due to scattering and absorption of harmonic conversion crystals (DKDP) for the National Ignition Facility (NIF). The main issues to be addressed are (1) amount of total energy reaching the target if the target hole was {+-}200 {micro}rad in size, (2) distribution of energy inside the target hole, (3) collateral damage of other optics by scattered light. The scatter diagnostics enables angle-resolved measurements at 351 nm, and is capable of both near specular transmission and large angle scatter measurements. In the near specular setup, the transmission can be measured within {+-}65 {micro}rad up to {+-}60 mrad acceptance angle. A silicon photo detector and a scientific-grade CCD camera provide total energy and energy distribution. A linear swing arm detection system enables large angle scatter measurements of 360{sup o}, in principal, with step sizes as small as 0.01{sup o} and different collection angle ranging between 1 and 20 mad. In this paper, scatter effects from laser damage and final finishing process of DKDP are discussed.

  18. Is the Separable Propagator Perturbation Approach Accurate in Calculating Angle Resolved Photoelectron Diffraction Spectra?

    Science.gov (United States)

    Ng, C. N.; Chu, T. P.; Wu, Huasheng; Tong, S. Y.; Huang, Hong

    1997-03-01

    We compare multiple scattering results of angle-resolved photoelectron diffraction spectra between the exact slab method and the separable propagator perturbation method. In the slab method,footnote C.H. Li, A.R. Lubinsky and S.Y. Tong, Phys. Rev. B17, 3128 (1978). the source wave and multiple scattering within the strong scattering atomic layers are expanded in spherical waves while interlayer scattering is expressed in plane waves. The transformation between spherical waves and plane waves is done exactly. The plane waves are then matched across the solid-vacuum interface to a single outgoing plane wave in the detector's direction. The separable propagator perturbation approach uses two approximations: (i) A separable representation of the Green's function propagator and (ii) A perturbation expansion of multiple scattering terms. Results of c(2x2) S-Ni(001) show that this approximate method fails to converge due to the very slow convergence of the separable representation for scattering angles less than 90^circ. However, this method is accurate in the backscattering regime and may be applied to XAFS calculations.(J.J. Rehr and R.C. Albers, Phys. Rev. B41, 8139 (1990).) The use of this method for angle-resolved photoelectron diffraction spectra is substantially less reliable.

  19. Angle - resolved - photoemission study of Bi sub 2 Sr sub 2 CaCu sub 2 O sub 8+. delta. : Metallicity of the Bi-O plane

    Energy Technology Data Exchange (ETDEWEB)

    Wells, B.O.; Shen, Z.; Dessau, D.S.; Spicer, W.E.; Olson, C.G.; Mitzi, D.B.; Kapitulnik, A.; List, R.S.; Arko, A. (Stanford Electronics Laboratories, Stanford University, Stanford, CA (USA) Ames Laboratory, Iowa State University, Ames, IA Department of Applied Physics, Stanford University, Stanford, CA (USA) Los Alamos National Laboratory, Los Alamos, NM (USA))

    1990-12-10

    We have performed high-resolution angle-resolved-photoemission experiments on Bi{sub 2}Sr{sub 2}CaCu{sub 2}O{sub 8+{delta}} single crystals with different annealing histories. By depositing a small amount of Au on the surface, we were able to distinguish electronic states associated with the Bi-O surface layer. We found that the Bi-O atomic surface layer is metallic and superconducting for samples that were high-temperature annealed in oxygen but not for as-grown samples. The Cu-O plane is found to be superconducting in all samples.

  20. Quantitative angle-resolved small-spot reflectance measurements on plasmonic perfect absorbers: impedance matching and disorder effects.

    Science.gov (United States)

    Tittl, Andreas; Harats, Moshe G; Walter, Ramon; Yin, Xinghui; Schäferling, Martin; Liu, Na; Rapaport, Ronen; Giessen, Harald

    2014-10-28

    Plasmonic devices with absorbance close to unity have emerged as essential building blocks for a multitude of technological applications ranging from trace gas detection to infrared imaging. A crucial requirement for such elements is the angle independence of the absorptive performance. In this work, we develop theoretically and verify experimentally a quantitative model for the angular behavior of plasmonic perfect absorber structures based on an optical impedance matching picture. To achieve this, we utilize a simple and elegant k-space measurement technique to record quantitative angle-resolved reflectance measurements on various perfect absorber structures. Particularly, this method allows quantitative reflectance measurements on samples where only small areas have been nanostructured, for example, by electron-beam lithography. Combining these results with extensive numerical modeling, we find that matching of both the real and imaginary parts of the optical impedance is crucial to obtain perfect absorption over a large angular range. Furthermore, we successfully apply our model to the angular dispersion of perfect absorber geometries with disordered plasmonic elements as a favorable alternative to current array-based designs.

  1. Intermolecular band dispersion of quasi-single crystalline organic semiconductor monolayer measured by angle-resolved photoemission spectroscopy

    Science.gov (United States)

    Ohtomo, Manabu; Shimada, Toshihiro; Hasegawa, Tetsuya

    2010-03-01

    Band structure of organic semiconductors is important knowledge to improve the molecular design. Angle-Resolved Photoemission Spectroscopy (ARPES) studies using highly conductive single domain samples grown in-situ is the most direct technique. In this study, we developed a novel method to grow quasi-single crystalline monolayer on conductive substrate and electronic structure was investigated. As a template for orientation control, we used a step-bunched Si(111) substrate with dangling bond termination. In case of pentacene, it was confirmed that the crystal is quasi-single crystal with 2.2^o rotated twins. The band dispersion was identical to that of thin-film phase. The effective mass and transfer integrals are evaluated using two-dimensional tight binding fit and compared with band calculations [1]. We also report the growth of 2,7-Dipheny[1]benzothieno[3,2-b]benzothiophene (DPh-BTBT) [2] on Bi-Si substrate and compare discuss its band structure. [4pt] [1] M.Ohtomo et al., APL 95, 123308 (2009).[0pt] [2] K.Takimiya, JACS 128, 3044 (2006).

  2. Angle-resolved spin wave band diagrams of square antidot lattices studied by Brillouin light scattering

    Energy Technology Data Exchange (ETDEWEB)

    Gubbiotti, G.; Tacchi, S. [Istituto Officina dei Materiali del Consiglio Nazionale delle Ricerche (IOM-CNR), Sede di Perugia, c/o Dipartimento di Fisica e Geologia, Via A. Pascoli, I-06123 Perugia (Italy); Montoncello, F.; Giovannini, L. [Dipartimento di Fisica e Scienze della Terra, Università di Ferrara, Via G. Saragat 1, I-44122 Ferrara (Italy); Madami, M.; Carlotti, G. [Dipartimento di Fisica e Geologia, Università di Perugia, Via A. Pascoli, I-06123 Perugia (Italy); Ding, J.; Adeyeye, A. O. [Information Storage Materials Laboratory, Department of Electrical and Computer Engineering, National University of Singapore, Singapore 117576 (Singapore)

    2015-06-29

    The Brillouin light scattering technique has been exploited to study the angle-resolved spin wave band diagrams of squared Permalloy antidot lattice. Frequency dispersion of spin waves has been measured for a set of fixed wave vector magnitudes, while varying the wave vector in-plane orientation with respect to the applied magnetic field. The magnonic band gap between the two most dispersive modes exhibits a minimum value at an angular position, which exclusively depends on the product between the selected wave vector magnitude and the lattice constant of the array. The experimental data are in very good agreement with predictions obtained by dynamical matrix method calculations. The presented results are relevant for magnonic devices where the antidot lattice, acting as a diffraction grating, is exploited to achieve multidirectional spin wave emission.

  3. Multiple Bosonic Mode Coupling in Electron Self-Energy of (La_2-xSr_x)CuO_4

    Energy Technology Data Exchange (ETDEWEB)

    Zhou, X.J.

    2010-06-02

    High resolution angle-resolved photoemission spectroscopy data with significantly improved statistics reveal tne structure in the electron self-energy of the underdoped (La{sub 2-x}Sr{sub x}) CuO{sub 4} (x=0.03, 0.036 and 0.07) samples in the normal state. Four fine structure have been identified near 27, 45, 61 and 75 meV. These features show good correspondence to the structure in the phonon density of states as measured from neutron scattering.

  4. Diversification of nanostructure morphology by modifying angle-resolved heterogeneous shadow mask.

    Science.gov (United States)

    Wang, Chaoguang; Wu, Xuezhong; Dong, Peitao; Wang, Junfeng; Di, Di; Chen, Jian; Wang, Haoxu

    2013-12-01

    This article presents a facile and generally applicable methodology for the morphology diversification of two-dimensional (2D) nanostructure arrays by modifying angle-resolved heterogeneous shadow mask (AR-HSM). Colloid spheres are used to prepare scalable well-organized monolayer film by self-assembly method and then etched in oxygen plasma to reduce size. Subsequently, the heterogeneous layer is generated by tilted metal deposition technique, then utilized as shadow mask in the substrate etching process, and finally removed by wet etching technique. As a result, the controllable fabrication of a series of complex morphologies, ranging from the crescent structure to the hoof-like structure and the stripes with apexes, is realized. The morphology of the nanostructure array is depend on the profile of the heterogeneous shadow mask (HSM) which is correlated to the incidence angle of the metal vapor. Therefore, a theoretical model is built for the prediction and design of the nanostructure morphology. This AR-HSM aided approach provides a novel and accessible route for the diversification of nanostructure morphology; and can be readily extended to other functional substrates which may be applied in photovoltaic devices or bio-chemical sensors.

  5. Comparison of models and measurements of angle-resolved scatter from irregular aerosols

    Science.gov (United States)

    Milstein, Adam B.; Richardson, Jonathan M.

    2015-01-01

    We have developed and validated a method for modeling the elastic scattering properties of biological and inert aerosols of irregular shape at near- and mid-wave infrared wavelengths. The method, based on Gaussian random particles, calculates the ensemble-average optical cross section and Mueller scattering matrix, using the measured aerodynamic size distribution and previously-reported refractive index as inputs. The utility of the Gaussian particle model is that it is controlled by only two parameters (σ and Γ) which we have optimized such that the model best reproduces the full angle-resolved Mueller scattering matrices measured at λ=1.55 μm in the Standoff Aerosol Active Signature Testbed (SAAST). The method has been applied to wet-generated singlet biological spore samples, dry-generated biological spore clusters, and kaolin. The scattering computation is performed using the Discrete Dipole Approximation (DDA), which requires significant computational resources, and is thus implemented on LLGrid, a large parallel grid computer. For the cases presented, the best fit Gaussian particle model is in good qualitative correspondence with microscopy images of the corresponding class of particles. The measured and computed cross sections agree well within a factor of two overall, with certain cases bearing closer correspondence. In particular, the DDA reproduces the shape of the measured scatter function more accurately than Mie predictions. The DDA-computed depolarization factors are also in good agreement with measurement.

  6. Dirac cones, Floquet side bands, and theory of time-resolved angle-resolved photoemission

    Science.gov (United States)

    Farrell, Aaron; Arsenault, A.; Pereg-Barnea, T.

    2016-10-01

    Pump-probe techniques with high temporal resolution allow one to drive a system of interest out of equilibrium and at the same time probe its properties. Recent advances in these techniques open the door to studying new, nonequilibrium phenomena such as Floquet topological insulators and superconductors. These advances also necessitate the development of theoretical tools for understanding the experimental findings and predicting new ones. In the present paper, we provide a theoretical foundation to understand the nonequilibrium behavior of a Dirac system. We present detailed numerical calculations and simple analytic results for the time evolution of a Dirac system irradiated by light. These results are framed by appealing to the recently revitalized notion of side bands [A. Farrell and T. Pereg-Barnea, Phys. Rev. Lett. 115, 106403 (2015), 10.1103/PhysRevLett.115.106403; Phys. Rev. B 93, 045121 (2016), 10.1103/PhysRevB.93.045121], extended to the case of nonperiodic drive where the fast oscillations are modified by an envelope function. We apply this formalism to the case of photocurrent generated by a second probe pulse. We find that, under the application of circularly polarized light, a Dirac point only ever splits into two copies of side bands. Meanwhile, the application of linearly polarized light leaves the Dirac point intact while producing side bands. In both cases the population of the side bands are time dependent through their nonlinear dependence on the envelope of the pump pulse. Our immediate interest in this work is in connection to time- and angle-resolved photoemission experiments, where we find excellent qualitative agreement between our results and those in the literature [Wang et al., Science 342, 453 (2013), 10.1126/science.1239834]. However, our results are general and may prove useful beyond this particular application and should be relevant to other pump-probe experiments.

  7. Quasiparticle dynamics across the full Brillouin zone of Bi2Sr2CaCu2O8+δ traced with ultrafast time and angle-resolved photoemission spectroscopy

    Directory of Open Access Journals (Sweden)

    Georgi L. Dakovski

    2015-09-01

    Full Text Available A hallmark in the cuprate family of high-temperature superconductors is the nodal-antinodal dichotomy. In this regard, angle-resolved photoemission spectroscopy (ARPES has proven especially powerful, providing band structure information directly in energy-momentum space. Time-resolved ARPES (trARPES holds great promise of adding ultrafast temporal information, in an attempt to identify different interaction channels in the time domain. Previous studies of the cuprates using trARPES were handicapped by the low probing energy, which significantly limits the accessible momentum space. Using 20.15 eV, 12 fs pulses, we show for the first time the evolution of quasiparticles in the antinodal region of Bi2Sr2CaCu2O8+δ and demonstrate that non-monotonic relaxation dynamics dominates above a certain fluence threshold. The dynamics is heavily influenced by transient modification of the electron-phonon interaction and phase space restrictions, in stark contrast to the monotonic relaxation in the nodal and off-nodal regions.

  8. A flat band at the chemical potential of a Fe1.03Te0.94S0.06 superconductor observed by angle-resolved photoemission spectroscopy.

    Science.gov (United States)

    Starowicz, P; Schwab, H; Goraus, J; Zajdel, P; Forster, F; Rak, J R; Green, M A; Vobornik, I; Reinert, F

    2013-05-15

    The electronic structure of superconducting Fe1.03Te0.94S0.06 has been studied by angle-resolved photoemission spectroscopy (ARPES). Experimental band topography is compared to the calculations using the methods of Korringa-Kohn-Rostoker (KKR) with the coherent potential approximation (CPA) and the linearized augmented plane wave with local orbitals (LAPW+LO) method. The region of the Γ point exhibits two hole pockets and a quasiparticle peak close to the chemical potential (μ) with undetectable dispersion. This flat band with mainly d(z)(2) orbital character is most likely formed by the top of the outer hole pocket or is evidence of a third hole band. It may cover up to 3% of the Brillouin zone volume and should give rise to a Van Hove singularity. Studies performed for various photon energies indicate that at least one of the hole pockets has a two-dimensional character. The apparently nondispersing peak at μ is clearly visible for 40 eV and higher photon energies, due to an effect of the photoionization cross-section rather than band dimensionality. Orbital characters calculated by LAPW+LO for stoichiometric FeTe do not reveal the flat dz(2) band but are in agreement with the experiment for the other dispersions around Γ in Fe1.03Te0.94S0.06.

  9. Angle Resolved Photoemission Spectroscopy Studies of the Mott Insulator to Superconductor Evolution in Ca2-xNaxCuO2Cl2

    Energy Technology Data Exchange (ETDEWEB)

    Shen, Kyle Michael

    2005-09-02

    It is widely believed that many of the exotic physical properties of the high-T{sub c} cuprate superconductors arise from the proximity of these materials to the strongly correlated, antiferromagnetic Mott insulating state. Therefore, one of the fundamental questions in the field of high-temperature superconductivity is to understand the insulator-to-superconductor transition and precisely how the electronic structure of Mott insulator evolves as the first holes are doped into the system. This dissertation presents high-resolution, doping dependent angle-resolved photoemission (ARPES) studies of the cuprate superconductor Ca{sub 2-x}Na{sub x}CuO{sub 2}Cl{sub 2}, spanning from the undoped parent Mott insulator to a high-temperature superconductor with a T{sub c} of 22 K. A phenomenological model is proposed to explain how the spectral lineshape, the quasiparticle band dispersion, and the chemical potential all progress with doping in a logical and self-consistent framework. This model is based on Franck-Condon broadening observed in polaronic systems where strong electron-boson interactions cause the quasiparticle residue, Z, to be vanishingly small. Comparisons of the low-lying states to different electronic states in the valence band strongly suggest that the coupling of the photohole to the lattice (i.e. lattice polaron formation) is the dominant broadening mechanism for the lower Hubbard band states. Combining this polaronic framework with high-resolution ARPES measurements finally provides a resolution to the long-standing controversy over the behavior of the chemical potential in the high-T{sub c} cuprates. This scenario arises from replacing the conventional Fermi liquid quasiparticle interpretation of the features in the Mott insulator by a Franck-Condon model, allowing the reassignment of the position of the quasiparticle pole. As a function of hole doping, the chemical potential shifts smoothly into the valence band while spectral weight is transferred

  10. Nanofocusing, shadowing, and electron mean free path in the photoemission from aerosol droplets

    CERN Document Server

    Signorell, Ruth; Yoder, Bruce L; Bodi, Andras; Chasovskikh, Egor; Lang, Lukas; Luckhaus, David

    2016-01-01

    Angle-resolved photoelectron spectroscopy of aerosol droplets is a promising method for the determination of electron mean free paths in liquids. It is particularly attractive for volatile liquids, such as water. Here we report the first angle-resolved photoelectron images of droplets with defined sizes, viz. of water, glycerol, and dioctyl phthalate droplets. We present an approach that allows one to gradually vary the conditions from dominant shadowing to dominant nanofocusing to optimize the information content contained in the photoelectron images. Example simulations of water droplet photoelectron images and preliminary data for electron mean free paths for liquid water at low kinetic energy (<3eV) are provided.

  11. Photodetachment studies on few-electron atomic negative ions. [[approx] 2 eV

    Energy Technology Data Exchange (ETDEWEB)

    Pegg, D.J.

    1992-01-01

    A crossed laser-negative ion beams apparatus, situated at Oak Ridge National Laboratory has been used for energy and angle-resolved photoelectron spectroscopic measurements following photodetachment. In the current grant period measurements of the cross sections for photodetaching an electron from the Li[sup [minus

  12. Origin of robust nanoscale ferromagnetism in Fe-doped Ge revealed by angle-resolved photoemission spectroscopy and first-principles calculation

    Science.gov (United States)

    Sakamoto, S.; Wakabayashi, Y. K.; Takeda, Y.; Fujimori, S.-i.; Suzuki, H.; Ban, Y.; Yamagami, H.; Tanaka, M.; Ohya, S.; Fujimori, A.

    2017-02-01

    Ge1 -xFex (Ge:Fe) shows ferromagnetic behavior up to a relatively high temperature of 210 K and hence is a promising material for spintronic applications compatible with Si technology. Unlike the prototypical system (Ga,Mn)As where itinerant holes induce long-range ferromagnetic order of the Mn spins, however, its ferromagnetism evolves from robust nanoscale ferromagnetic domains formed in Fe-rich regions. We have studied its underlying electronic structure by soft x-ray angle-resolved photoemission spectroscopy measurements and first-principles supercell calculation. We observed finite Fe 3 d components in the states at the Fermi level (EF) in a wide region of momentum space, and the EF was located ˜0.35 eV above the valence-band maximum of the host Ge. Our calculation indicates that the EF is also within the deep acceptor-level impurity band induced by the strong p -d (t2) hybridization. We conclude that the additional minority-spin d (e ) electron characteristic of the Fe2 + state is responsible for the short-range ferromagnetic coupling between Fe atoms, making the magnetism markedly different from that of (Ga,Mn)As.

  13. Extracting the temperature of hot carriers in time- and angle-resolved photoemission

    DEFF Research Database (Denmark)

    Ulstrup, Søren; Johannsen, Jens Christian; Grioni, Marco;

    2014-01-01

    The interaction of light with a material’s electronic system creates an out-of-equilibrium (nonthermal) distribution of optically excited electrons. Non-equilibrium dynamics relaxes this distribution on an ultrafast timescale to a hot Fermi-Dirac distribution with a well-defined temperature. The ......, we introduce a method that circumvents these difficulties and accurately extracts both the temperature and the position of the Fermi level for a hot carrier distribution by tracking the occupation statistics of the carriers measured in a TR-ARPES experiment...

  14. High resolution-angle resolved photoemission studies of high temperature superconductors

    Energy Technology Data Exchange (ETDEWEB)

    Olson, C.G.; Liu, R.; Lynch, D.W. (Ames Lab. and Dept. of Physics, Iowa State Univ. (USA)); Veal, B.W.; Chang, Y.C.; Jiang, P.Z.; Liu, J.Z.; Paulikas, A.P. (Argonne National Lab., IL (USA)); Arko, A.J.; List, R.S. (Los Alamos National Lab., NM (USA))

    1989-12-01

    Recent photoemission studies of Y 123 and Bi 2212 performed with high energy and angular resolution have provided detailed information on the nature of the states near the Fermi level. Measurements of the superconducting gap, band dispersion, and the density of states near the Fermi level in the normal state all support a Fermi liquid description of these materials. (orig.).

  15. High resolution-angle resolved photoemission studies of high temperature superconductors

    Energy Technology Data Exchange (ETDEWEB)

    Olson, C.G.; Liu, R.; Lynch, D.W.; Veal, B.W.; Chang, Y.C.; Jiang, P.Z.; Liu, J.Z.; Paulikas, A.P.; Arko, A.J.; List, R.S. (Ames Lab., IA (USA); Argonne National Lab., IL (USA); Los Alamos National Lab., NM (USA))

    1989-08-01

    Recent photoemission studies of Y 123 and Bi 2212 performed with high energy and angular resolution have provided detailed information on the nature of the states near the Fermi level. Measurements of the superconducting gap, band dispersion, and the density of states near the Fermi level in the normal state all support a Fermi liquid description of these materials. 5 refs., 4 figs.

  16. Angle resolved photoelectron distribution of the 1{pi} resonance of CO/Pt(111)

    Energy Technology Data Exchange (ETDEWEB)

    Haarlammert, Thorben; Wegner, Sebastian; Tsilimis, Grigorius; Zacharias, Helmut [Physikalisches Institut, Westfaelische Wilhelms Universitaet, Muenster (Germany); Golovin, Alexander [Institute of Physics, St. Petersburg State University (Russian Federation)

    2009-07-01

    The CO 1{pi} level of a c(4 x 2)-2CO/Pt(111) reconstruction shows a significant resonance when varying the photon energy between h{nu}=23 eV and h{nu}=48 e V. This resonance has not been observed in gas phase measurements or on the Pt(1 10) surface. To investigate the photoelectron distribution of the 1{pi} level high harmonic radiaton has been used. By conversion in rare gases like argon, neon, or helium photon energies of up to 100 eV have been generated at repetition r ates of up to 10 kHz. The single harmonics have been separated and focused by a toroidal grating and directed to the sample surface. A time-of-flight detector with multiple anodes registers the kinetic energies of the emitted photoelectrons and enables the simultaneous detection of multiple emission angles. The angular distributions of photoelectrons emitted from the CO 1{pi} level have been measured for a variety of initial photon energies. Further the angular distributions of the CO 1{pi} level photoelectrons emitted from a CO-Pt{sub 7} cluster have been calculated using the MSX{alpha}-Method which shows good agreement with the ex perimental data.

  17. Quantum Transport and Nano Angle-resolved Photoemission Spectroscopy on the Topological Surface States of Single Sb2Te3 Nanowires

    Science.gov (United States)

    Arango, Yulieth C.; Huang, Liubing; Chen, Chaoyu; Avila, Jose; Asensio, Maria C.; Grützmacher, Detlev; Lüth, Hans; Lu, Jia Grace; Schäpers, Thomas

    2016-09-01

    We report on low-temperature transport and electronic band structure of p-type Sb2Te3 nanowires, grown by chemical vapor deposition. Magnetoresistance measurements unravel quantum interference phenomena, which depend on the cross-sectional dimensions of the nanowires. The observation of periodic Aharonov-Bohm-type oscillations is attributed to transport in topologically protected surface states in the Sb2Te3 nanowires. The study of universal conductance fluctuations demonstrates coherent transport along the Aharonov-Bohm paths encircling the rectangular cross-section of the nanowires. We use nanoscale angle-resolved photoemission spectroscopy on single nanowires (nano-ARPES) to provide direct experimental evidence on the nontrivial topological character of those surface states. The compiled study of the bandstructure and the magnetotransport response unambiguosly points out the presence of topologically protected surface states in the nanowires and their substantial contribution to the quantum transport effects, as well as the hole doping and Fermi velocity among other key issues. The results are consistent with the theoretical description of quantum transport in intrinsically doped quasi-one-dimensional topological insulator nanowires.

  18. Si(111)-sq root 21 x sq root 21 -(Ag+Cs) surface studied by scanning tunneling microscopy and angle-resolved photoemission spectroscopy

    CERN Document Server

    Liu, C; Morikawa, H; Okino, H; Hasegawa, S; Okuda, T; Kinoshita, T

    2003-01-01

    Scanning tunneling microscopy (STM) and angle-resolved photoemission spectroscopy (ARPES) were used to study the atomic and electronic structures of the Si(111)-sq root 21 x sq root 21-(Ag + Cs) surface (sq root 21-Cs in short), which was induced by depositing caesium atoms on the Si(111)-sq root 3 x sq root 3-Ag surface at room temperature (RT). Compared with previously reported STM images of noble-metal induced sq root 21 x sq root 21 phases including the Si(111)-sq root 21 x sq root 21-(Ag+Ag) and Si(111)-sq root 21 x sq root 21-(Ag+Au) surfaces (sq root 21-Ag and sq root 21-Au, respectively), the sq root 21-Cs surface displayed quite different features in STM images. The ARPES data of the sq root 21-Cs surface revealed an intrinsic dispersive surface-state band, together with a non-dispersive one near the Fermi level, which was also different from those of the sq root 21-Ag and sq root 21-Au surfaces. These results strongly suggest different atomic arrangements between Cs- and noble-metal induced sq root ...

  19. Evidence of the nature of core-level photoemission satellites using angle-resolved photoemission extended fine structure

    Energy Technology Data Exchange (ETDEWEB)

    Moler, E.J.; Kellar, S.A.; Huff, W.R.A. [Lawrence Berkeley National Lab., CA (United States)] [and others

    1997-04-01

    The authors present a unique method of experimentally determining the angular momentum and intrinsic/extrinsic origin of core-level photoemission satellites by examining the satellite diffraction pattern in the Angle Resolved Photoemission Extended Fine Structure (ARPEFS) mode. They show for the first time that satellite peaks not associated with chemically differentiated atomic species display an ARPEFS intensity oscillation. They present ARPEFS data for the carbon 1s from ({radical}3x{radical}3)R30 CO/Cu(111) and p2mg(2xl)CO/Ni(110), nitrogen 1s from c(2x2) N{sub 2}/Ni(100), cobalt 1s from p(1x1)Co/Cu(100), and nickel 3p from clean nickel (111). The satellite peaks and tails of the Doniach-Sunjic line shapes in all cases exhibit ARPEFS curves which indicate an angular momentum identical to the main peak and are of an intrinsic nature.

  20. Anomalous High-Energy Waterfall-Like Electronic Structure in 5 d Transition Metal Oxide Sr2IrO4 with a Strong Spin-Orbit Coupling.

    Science.gov (United States)

    Liu, Yan; Yu, Li; Jia, Xiaowen; Zhao, Jianzhou; Weng, Hongming; Peng, Yingying; Chen, Chaoyu; Xie, Zhuojin; Mou, Daixiang; He, Junfeng; Liu, Xu; Feng, Ya; Yi, Hemian; Zhao, Lin; Liu, Guodong; He, Shaolong; Dong, Xiaoli; Zhang, Jun; Xu, Zuyan; Chen, Chuangtian; Cao, Gang; Dai, Xi; Fang, Zhong; Zhou, X J

    2015-08-12

    The low energy electronic structure of Sr2IrO4 has been well studied and understood in terms of an effective Jeff = 1/2 Mott insulator model. However, little work has been done in studying its high energy electronic behaviors. Here we report a new observation of the anomalous high energy electronic structure in Sr2IrO4. By taking high-resolution angle-resolved photoemission measurements on Sr2IrO4 over a wide energy range, we have revealed for the first time that the high energy electronic structures show unusual nearly-vertical bands that extend over a large energy range. Such anomalous high energy behaviors resemble the high energy waterfall features observed in the cuprate superconductors. While strong electron correlation plays an important role in producing high energy waterfall features in the cuprate superconductors, the revelation of the high energy anomalies in Sr2IrO4, which exhibits strong spin-orbit coupling and a moderate electron correlation, points to an unknown and novel route in generating exotic electronic excitations.

  1. The band structure of VO2 measured by angle-resolved photoemission

    Science.gov (United States)

    Moreschini, Luca; Chang, Young Jun; Innocenti, Davide; Walter, Andrew L.; Kim, Young Su; Gaines, Geoffrey; Bostwick, Aaron; Denlinger, Jonathan; Rotenberg, Eli

    2011-03-01

    The origin of the 340K metal-insulator transition (MIT) in VO2 is still under debate. the main reason is that no direct experimental verifications of the electronic structure of VO2 exist up to this point. The quality of the available single crystals is not sufficient for ARPES measurements, so that photoemission is limited to angle-integrated mode. New opportunities are offered by oxide films, on which data of equal or even higher quality have been reported (Saeki et al., PRB 2009). WIth the in situ pulsed-laser-deposition (PLD) system available on beamline 7.0.1 at the Advanced Light Source we have grown VO2(001) films on a TiO2 substrate and measured the Fermi surface of the metallic phase. These results will permit a direct comparison with the existing band calculations and open the way to the study of the MIT as a function, e.g., of film thickness or electron doping with Cr. Work supported by U.S. DOE (DE-AC02-05CH11231 for ALS), the Max Planck Society, and the Swiss National Science Foundation (PBELP2-125484).

  2. Thermo electronic laser energy conversion

    Science.gov (United States)

    Hansen, L. K.; Rasor, N. S.

    1976-01-01

    The thermo electronic laser energy converter (TELEC) is described and compared to the Waymouth converter and the conventional thermionic converter. The electrical output characteristics and efficiency of TELEC operation are calculated for a variety of design variables. Calculations and results are briefly outlined. It is shown that the TELEC concept can potentially convert 25 to 50 percent of incident laser radiation into electric power at high power densities and high waste heat rejection temperatures.

  3. Crank angle resolved flow field characterization of a heavy-duty one-cylinder optical engine

    Energy Technology Data Exchange (ETDEWEB)

    Van der Meyden, T.J.

    2009-03-15

    Soot and nitric oxide (NOx) production are the main negative aspects of Diesel combustion. This is why new combustion strategies are being investigated, such as Premixed Charge Compression Ignition (PCCI). PCCI is one of the most promising combustion strategies for internal combustion engines in the future, since PCCI combustion is able to realize very low soot and nitric oxide emissions. PCCI combines the efficiency of a diesel and the low particulate emission of an Otto engine. To achieve PCCI combustion with limited heat release rates, the influence of charge stratification on combustion should be investigated. In this work, the first steps to achieve that goal are made. The first step is to determine in-cylinder velocities by measuring flow fields using Particle Image Velocimetry (PIV). The test setup consists of a one-cylinder optically accessible heavy duty engine driven by an electrical motor. The upper part of the liner and piston bottom are both made of sapphire. For PIV measurements a 10 Hz Nd:YAG Continuum Surelite laser is used with pulse energies of 140 mJ. The used camera is a Kodak Megaplus ES 1.0 CCD with 1008 x 1018 pixels. The seeding particles are produced from silicon oil using Laskin nozzles and have a diameter of about 0.7 im. Pre- and post- processing and the evaluation of the recorded PIV images is done using the commercially available software program PIVview (Pivtec). The velocity analysis is done using the commercial software program Tecplot. More knowledge is gathered on the in-cylinder velocities, aimed at a future detailed study on the effect of charge stratification in PCCI combustion. Ensemble averaged velocities, vorticities and strain rates, turbulence intensities and turbulent kinetic energies as a function of the crank angle, engine speed, measurement height and compression ratio have been investigated. Velocity and turbulence appear to be proportional to the engine speed. The position of the ensemble averaged swirl center as a

  4. Nodal gap detection through polar angle-resolved density of states measurements in uniaxial superconductors

    Science.gov (United States)

    Tsutsumi, Yasumasa; Nomoto, Takuya; Ikeda, Hiroaki; Machida, Kazushige

    2016-12-01

    We propose a spectroscopic method to identify the nodal gap structure in unconventional superconductors. This method is best suited for locating the horizontal line node and for pinpointing the isolated point nodes by measuring polar angle (θ ) resolved zero-energy density of states N (θ ) . This is measured by specific heat or thermal conductivity at low temperatures under a magnetic field. We examine a variety of uniaxially symmetric nodal structures, including point and/or line nodes with linear and quadratic dispersions, by solving the Eilenberger equation in vortex states. It is found that (a) the maxima of N (θ ) continuously shift from the antinodal to the nodal direction (θn) as a field increases accompanying the oscillation pattern reversal at low and high fields. Furthermore, (b) local minima emerge next to θn on both sides, except for the case of the linear point node. These features are robust and detectable experimentally. Experimental results of N (θ ) performed on several superconductors, UPd2Al3,URu2Si2,CuxBi2Se3 , and UPt3, are examined and commented on in light of the present theory.

  5. High-resolution soft X-ray beamline ADRESS at the Swiss Light Source for resonant inelastic X-ray scattering and angle-resolved photoelectron spectroscopies

    Energy Technology Data Exchange (ETDEWEB)

    Strocov, V. N., E-mail: vladimir.strocov@psi.ch; Schmitt, T.; Flechsig, U.; Schmidt, T.; Imhof, A.; Chen, Q.; Raabe, J. [Swiss Light Source, Paul Scherrer Institut, CH-5232 Villigen-PSI (Switzerland); Betemps, R.; Zimoch, D.; Krempasky, J. [Paul Scherrer Institut, CH-5232 Villigen-PSI (Switzerland); Wang, X. [Swiss Light Source, Paul Scherrer Institut, CH-5232 Villigen-PSI (Switzerland); Institut de Physique de la Matiére Condensé, Ecole Polytechnique Fédéderale de Lausanne (Switzerland); Grioni, M. [Institut de Physique de la Matiére Condensé, Ecole Polytechnique Fédéderale de Lausanne (Switzerland); Piazzalunga, A. [Swiss Light Source, Paul Scherrer Institut, CH-5232 Villigen-PSI (Switzerland); Dipartimento di Fisica, Politecnico di Milano, Piazza Leonardo da Vinci 32, I-20133 Milano (Italy); Patthey, L. [Swiss Light Source, Paul Scherrer Institut, CH-5232 Villigen-PSI (Switzerland)

    2010-09-01

    Concepts and technical realization of the high-resolution soft X-ray beamline ADRESS at the Swiss Light Source are described. Optimization of the optical scheme for high resolution and photon flux as well as diagnostics tools and alignment strategies are discussed. The concepts and technical realisation of the high-resolution soft X-ray beamline ADRESS operating in the energy range from 300 to 1600 eV and intended for resonant inelastic X-ray scattering (RIXS) and angle-resolved photoelectron spectroscopy (ARPES) are described. The photon source is an undulator of novel fixed-gap design where longitudinal movement of permanent magnetic arrays controls not only the light polarization (including circular and 0–180° rotatable linear polarizations) but also the energy without changing the gap. The beamline optics is based on the well established scheme of plane-grating monochromator operating in collimated light. The ultimate resolving power E/ΔE is above 33000 at 1 keV photon energy. The choice of blazed versus lamellar gratings and optimization of their profile parameters is described. Owing to glancing angles on the mirrors as well as optimized groove densities and profiles of the gratings, the beamline is capable of delivering high photon flux up to 1 × 10{sup 13} photons s{sup −1} (0.01% BW){sup −1} at 1 keV. Ellipsoidal refocusing optics used for the RIXS endstation demagnifies the vertical spot size down to 4 µm, which allows slitless operation and thus maximal transmission of the high-resolution RIXS spectrometer delivering E/ΔE > 11000 at 1 keV photon energy. Apart from the beamline optics, an overview of the control system is given, the diagnostics and software tools are described, and strategies used for the optical alignment are discussed. An introduction to the concepts and instrumental realisation of the ARPES and RIXS endstations is given.

  6. d0 Perovskite-Semiconductor Electronic Structure

    OpenAIRE

    Bistritzer, R.; Khalsa, G.; MacDonald, A. H.

    2010-01-01

    We address the low-energy effective Hamiltonian of electron doped d0 perovskite semiconductors in cubic and tetragonal phases using the k*p method. The Hamiltonian depends on the spin-orbit interaction strength, on the temperature-dependent tetragonal distortion, and on a set of effective-mass parameters whose number is determined by the symmetry of the crystal. We explain how these parameters can be extracted from angle resolved photo-emission, Raman spectroscopy, and magneto-transport measu...

  7. Pump laser-induced space-charge effects in HHG-driven time- and angle-resolved photoelectron spectroscopy

    Science.gov (United States)

    Oloff, L.-P.; Hanff, K.; Stange, A.; Rohde, G.; Diekmann, F.; Bauer, M.; Rossnagel, K.

    2016-06-01

    With the advent of ultrashort-pulsed extreme ultraviolet sources, such as free-electron lasers or high-harmonic-generation (HHG) sources, a new research field for photoelectron spectroscopy has opened up in terms of femtosecond time-resolved pump-probe experiments. The impact of the high peak brilliance of these novel sources on photoemission spectra, so-called vacuum space-charge effects caused by the Coulomb interaction among the photoemitted probe electrons, has been studied extensively. However, possible distortions of the energy and momentum distributions of the probe photoelectrons caused by the low photon energy pump pulse due to the nonlinear emission of electrons have not been studied in detail yet. Here, we systematically investigate these pump laser-induced space-charge effects in a HHG-based experiment for the test case of highly oriented pyrolytic graphite. Specifically, we determine how the key parameters of the pump pulse—the excitation density, wavelength, spot size, and emitted electron energy distribution—affect the measured time-dependent energy and momentum distributions of the probe photoelectrons. The results are well reproduced by a simple mean-field model, which could open a path for the correction of pump laser-induced space-charge effects and thus toward probing ultrafast electron dynamics in strongly excited materials.

  8. Optically Forbidden Excitations of 2s Electron of Neon Studied by Fast Electron Impact

    Institute of Scientific and Technical Information of China (English)

    GE Min; ZHU Lin-Fan; LIU Cun-Ding; XU Ke-Zun

    2008-01-01

    The electron energy loss spectrum in the energy region of 42-48.5 eV of neon is measured with an angle-resolved fast-electron energy-loss spectrometer at an incident electron energy of 2500eV. Besides the dipole-allowed autoionization transitions of 2s-1np (n = 3, 4) and 2p-23s3p, the dipole-forbidden ones of 2s-1ns (n = 3 - 6) and 2s-13d are observed. The line profile parameters, i.e. ET, F and q for these transitions, are determined, and the momentum transfer dependence behaviour is discussed.

  9. Energy Efficient Electronics Cooling Project

    Energy Technology Data Exchange (ETDEWEB)

    Steve O' Shaughnessey; Tim Louvar; Mike Trumbower; Jessica Hunnicutt; Neil Myers

    2012-02-17

    Parker Precision Cooling Business Unit was awarded a Department of Energy grant (DE-EE0000412) to support the DOE-ITP goal of reducing industrial energy intensity and GHG emissions. The project proposed by Precision Cooling was to accelerate the development of a cooling technology for high heat generating electronics components. These components are specifically related to power electronics found in power drives focused on the inverter, converter and transformer modules. The proposed cooling system was expected to simultaneously remove heat from all three of the major modules listed above, while remaining dielectric under all operating conditions. Development of the cooling system to meet specific customer's requirements and constraints not only required a robust system design, but also new components to support long system functionality. Components requiring further development and testing during this project included pumps, fluid couplings, cold plates and condensers. All four of these major categories of components are required in every Precision Cooling system. Not only was design a key area of focus, but the process for manufacturing these components had to be determined and proven through the system development.

  10. Power Electronics, Energy Harvesting and Renewable Energies Laboratory

    Data.gov (United States)

    Federal Laboratory Consortium — The research in the Power Electronics, Energy Harvesting and Renewable Energies Laboratory (PEHREL) is mainly focused on investigation, modeling, simulation, design,...

  11. Doping Dependence of the $(\\pi,\\pi)$ Shadow Band in La-Based Cuprates Studied by Angle-Resolved Photoemission Spectroscopy

    Energy Technology Data Exchange (ETDEWEB)

    Shen, Z. X.

    2011-08-15

    The ({pi},{pi}) shadow band (SB) in La-based cuprate family (La214) was studied by angle-resolved photoemission spectroscopy (ARPES) over a wide doping range from x = 0.01 to x = 0.25. Unlike the well-studied case of the Bi-based cuprate family, an overall strong, monotonic doping dependence of the SB intensity at the Fermi level (E{sub F}) was observed. In contrast to a previous report for the presence of the SB only close to x = 1/8, we found it exists in a wide doping range, associated with a doping-independent ({pi},{pi}) wave vector but strongly doping-dependent intensity: It is the strongest at x {approx} 0.03 and systematically diminishes as the doping increases until it becomes negligible in the overdoped regime. This SB with the observed doping dependence of intensity can in principle be caused by the antiferromagnetic fluctuations or a particular form of low-temperature orthorhombic lattice distortion known to persist up to x {approx} 0.21 in the system, with both being weakened with increasing doping. However, a detailed binding energy dependent analysis of the SB at x = 0.07 does not appear to support the former interpretation, leaving the latter as a more plausible candidate, despite a challenge in quantitatively linking the doping dependences of the SB intensity and the magnitude of the lattice distortion. Our finding highlights the necessity of a careful and global consideration of the inherent structural complications for correctly understanding the cuprate Fermiology and its microscopic implication.

  12. High-energy electron diffraction and microscopy

    CERN Document Server

    Peng, L M; Whelan, M J

    2011-01-01

    This book provides a comprehensive introduction to high energy electron diffraction and elastic and inelastic scattering of high energy electrons, with particular emphasis on applications to modern electron microscopy. Starting from a survey of fundamental phenomena, the authors introduce the most important concepts underlying modern understanding of high energy electron diffraction. Dynamical diffraction in transmission (THEED) and reflection (RHEED) geometries is treated using ageneral matrix theory, where computer programs and worked examples are provided to illustrate the concepts and to f

  13. Power electronics for renewable energy systems

    DEFF Research Database (Denmark)

    Iov, Florin; Blaabjerg, Frede

    2009-01-01

    sources from the conventional, fossil (and short term) based energy sources to renewable energy resources. Another is to use high efficient power electronics in power generation, power transmission/distribution and end-user application. This paper discuss some of the most emerging renewable energy sources......, wind energy and photovoltaics, which by means of power electronics are changing from being minor energy sources to be acting as important power sources in the energy system....

  14. Electron energy loss and diffraction of backscattered electrons from silicon

    Science.gov (United States)

    Winkelmann, Aimo; Aizel, Koceila; Vos, Maarten

    2010-05-01

    Electrons backscattered from crystals can show Kikuchi patterns: variations in intensity for different outgoing directions due to diffraction by the lattice. Here, we measure these effects as a function of their energy loss for 30 keV electrons backscattered from silicon. The change in diffraction contrast with energy loss depends strongly on the scattering geometry. At steep incidence on the sample, diffraction contrast in the observed Kikuchi bands decreases rapidly with energy loss. For an energy loss larger than about 150 eV the contrast is more than 5 times less than the contrast due to electrons near zero energy loss. However, for grazing incidence angles, maximum Kikuchi band contrast is observed for electrons with an energy loss near 60 eV, where the contrast is more than 2.5× larger than near zero energy loss. In addition, in this grazing incidence geometry, the Kikuchi diffraction effects stay significant even for electrons that have lost hundreds of electron volts. For the maximum measured energy loss of 440 eV, the electrons still show a contrast that is 1.5 × larger than that of the electrons near zero energy loss. These geometry-dependent observations of Kikuchi band diffraction contrast are interpreted based on the elastic and inelastic scattering properties of electrons and dynamical diffraction simulations.

  15. Protein coverage on silicon surfaces modified with amino-organic films: a study by AFM and angle-resolved XPS.

    Science.gov (United States)

    Awsiuk, K; Bernasik, A; Kitsara, M; Budkowski, A; Rysz, J; Haberko, J; Petrou, P; Beltsios, K; Raczkowska, J

    2010-10-01

    An approach to determine structural features, such as surface fractional coverage F and thickness d of protein layers immobilized on silicon substrates coated with amino-organic films is presented. To demonstrate the proposed approach rabbit gamma globulins (RgG) are adsorbed from a 0.66muM solution onto SiO(2) and Si(3)N(4) modified with (3-aminopropyl)triethoxysilane (APTES). Atomic force microscopy data are analyzed by applying an integral geometry approach to yield average coverage values for silanized Si(3)N(4) and SiO(2) coated with RgG, F=0.99+/-0.01 and 0.76+/-0.08, respectively. To determine the RgG thickness d from angle-resolved X-ray photoelectron spectroscopy (ARXPS), a model of amino-organic bilayer with non-homogeneous top lamellae is introduced. For an APTES layer thickness of 1.0+/-0.1nm, calculated from independent ARXPS measurements, and for fractional surface RgG coverage determined from AFM analysis, this model yields d=1.0+/-0.2nm for the proteins on both silanized substrates. This value, confirmed by an evaluation (1.0+/-0.2nm) from integral geometry analysis of AFM images, is lower than the RgG thickness expected for monomolecular film ( approximately 4nm). Structures visible in phase contrast AFM micrographs support the suggested sparse molecular packing in the studied RgG layers. XPS data, compared for bulk and adsorbed RgG, suggest preferential localization of oxygen- and nitrogen-containing carbon groups at silanized silicon substrates. These results demonstrate the potential of the developed AFM/ARXPS approach as a method for the evaluation of surface-protein coverage homogeneity and estimation of adsorbed proteins conformation on silane-modified silicon substrates used in bioanalytical applications.

  16. Fast Electronics in High-Energy Physics

    Energy Technology Data Exchange (ETDEWEB)

    Weigand, Clyde

    1958-08-08

    A brief review of fast electronics is given, leading up to the present state of the art. Cherenkov counters in high-energy physics are discussed, including an example of a velocity-selecting Cherenkov counter. An electronic device to aid in aligning external beams from high-energy accelerators is described. A scintillation-counter matrix to identify bubble chamber tracks is discussed. Some remarks on the future development of electronics in high-energy physics experiments are included.

  17. Spin orbit splitting in the valence bands of ZrS{sub x}Se{sub 2−x}: Angle resolved photoemission and density functional theory

    Energy Technology Data Exchange (ETDEWEB)

    Moustafa, Mohamed, E-mail: moustafa@physik.hu-berlin.de [Institut für Physik, Humboldt Universität zu Berlin, Newtonstr. 15, D-12489 Berlin (Germany); Faculty of Engineering, Pharos University in Alexandria, Canal El Mahmoudia Str., Alexandria (Egypt); Ghafari, Aliakbar; Paulheim, Alexander; Janowitz, Christoph; Manzke, Recardo [Institut für Physik, Humboldt Universität zu Berlin, Newtonstr. 15, D-12489 Berlin (Germany)

    2013-08-15

    Highlights: ► We performed high resolution ARPES on 1T–ZrS{sub x}Se{sub 2−x}. ► A characteristic splitting of the chalcogen p-derived VB along high symmetry directions was observed. ► The splitting size at the A point of the BZ is found to increase from 0.06 to 0.31 eV from ZrS{sub 2} towards ZrSe{sub 2}. ► Electronic structure calculations based on the DFT were performed using the model of TB–MBJ. ► The calculations show that the splitting is due to SO coupling of the valence bands. -- Abstract: Angle-resolved photoelectron spectroscopy using synchrotron radiation has been performed on 1T–ZrS{sub x}Se{sub 2−x}, where x varies from 0 to 2, in order to study the influence of the spin-orbit interaction in the valence bands. The crystals were grown by chemical vapour transport technique using Iodine as transport agent. A characteristic splitting of the chalcogen p-derived valence bands along high symmetry directions has been observed experimentally. The size of the splitting increases with the increase of the atomic number of the chalcogenide, e.g. at the A point of the Brillouin zone from 0.06 eV to 0.31 eV with an almost linear dependence with x, as progressing from ZrS{sub 2} towards ZrSe{sub 2}, respectively. Electronic structure calculations based on the density functional theory have been performed using the model of Tran–Blaha [1] and the modified version of the exchange potential proposed by Becke and Johnson [2] (TB–MBJ) both with and without spin-orbit (SO) coupling. The calculations show that the splitting is mainly due to spin-orbit coupling and the degeneracy of the valance bands is lifted.

  18. Single track nanodosimetry of low energy electrons

    Energy Technology Data Exchange (ETDEWEB)

    Bantsar, A. [Soltan Institute for Nuclear Studies, 05-400 Otwock-Swierk (Poland); Grosswendt, B. [Physikalisch-Technische Bundesanstalt, 38116 Braunschweig (Germany); Pszona, S. [Soltan Institute for Nuclear Studies, 05-400 Otwock-Swierk (Poland)], E-mail: pszona@ipj.gov; Kula, J. [Soltan Institute for Nuclear Studies, 05-400 Otwock-Swierk (Poland)

    2009-02-11

    Auger-electron-emitting radionuclides (for instance, {sup 125}I) with a predominant energy spectrum below 3 keV are an active area of research towards the clinical application of radiopharmaceuticals. Hence, the necessity for an adequate description of the effects of radiation by low-energy electrons on nanometric biological targets seems to be unquestionable. Experimental nanodosimetry for low-energy electrons has been accomplished with a device named JET COUNTER. The present paper describes, for the first time, nanodosimetric experiments in nanometer-sized cavities of nitrogen using low energy electrons ranging from 100 eV to 2 keV.

  19. Single track nanodosimetry of low energy electrons

    Science.gov (United States)

    Bantsar, A.; Grosswendt, B.; Pszona, S.; Kula, J.

    2009-02-01

    Auger-electron-emitting radionuclides (for instance, 125I) with a predominant energy spectrum below 3 keV are an active area of research towards the clinical application of radiopharmaceuticals. Hence, the necessity for an adequate description of the effects of radiation by low-energy electrons on nanometric biological targets seems to be unquestionable. Experimental nanodosimetry for low-energy electrons has been accomplished with a device named JET COUNTER. The present paper describes, for the first time, nanodosimetric experiments in nanometer-sized cavities of nitrogen using low energy electrons ranging from 100 eV to 2 keV.

  20. Power Electronics for Renewable Energy Systems

    DEFF Research Database (Denmark)

    Choi, U. M.; Lee, K. B.; Blaabjerg, Frede

    2012-01-01

    The use of renewable energy sources are increased because of the depletion of natural resources and the increasing pollution level from energy production. The wind energy and the solar energy are most widely used among the renewable energy sources. Power electronics is needed in almost all kinds...... of renewable energy system. It controls the renewable source and interfaces with the load effectively, which can be grid-connected or van work in stand-alone mode. In this presentation, overview of wind and photovoltaic energy systems are introduced. Next, the power electronic circuits behind the most common...

  1. The mapping of electronic energy distributions using experimental electron density.

    Science.gov (United States)

    Tsirelson, Vladimir G

    2002-08-01

    It is demonstrated that the approximate kinetic energy density calculated using the second-order gradient expansion with parameters of the multipole model fitted to experimental structure factors reproduces the main features of this quantity in a molecular or crystal position space. The use of the local virial theorem provides an appropriate derivation of approximate potential energy density and electronic energy density from the experimental (model) electron density and its derivatives. Consideration of these functions is not restricted by the critical points in the electron density and provides a comprehensive characterization of bonding in molecules and crystals.

  2. Attainment of Electron Beam Suitable for Medium Energy Electron Cooling

    Energy Technology Data Exchange (ETDEWEB)

    Seletskiy, Sergei M. [Univ. of Rochester, NY (United States)

    2005-01-01

    Electron cooling of charged particle beams is a well-established technique at electron energies of up to 300 keV. However, up to the present time the advance of electron cooling to the MeV-range energies has remained a purely theoretical possibility. The electron cooling project at Fermilab has recently demonstrated the ¯rst cooling of 8.9 GeV/c antiprotons in the Recycler ring, and therefore, has proved the validity of the idea of relativistic electron cool- ing. The Recycler Electron Cooler (REC) is the key component of the Teva- tron Run II luminosity upgrade project. Its performance depends critically on the quality of electron beam. A stable electron beam of 4.3 MeV car- rying 0.5 A of DC current is required. The beam suitable for the Recycler Electron Cooler must have an angular spread not exceeding 200 ¹rad. The full-scale prototype of the REC was designed, built and tested at Fermilab in the Wideband laboratory to study the feasibility of attaining the high-quality electron beam. In this thesis I describe various aspects of development of the Fermilab electron cooling system, and the techniques used to obtain the electron beam suitable for the cooling process. In particular I emphasize those aspects of the work for which I was principally responsible.

  3. Energy spectra in relativistic electron precipitation events.

    Science.gov (United States)

    Rosenberg, T. J.; Lanzerotti, L. J.; Bailey, D. K.; Pierson, J. D.

    1972-01-01

    Two events in August 1967, categorized as relativistic electron precipitation (REP) events by their effect on VHF transmissions propagated via the forward-scatter mode, have been examined with regard to the energy spectra of trapped and precipitated electrons. These two substorm-associated events August 11 and August 25 differ with respect to the relativistic, trapped electron population at synchronous altitude; in the August 25 event there was a nonadiabatic enhancement of relativistic (greater than 400 keV) electrons, while in the August 11 event no relativistic electrons were produced. In both events electron spectra deduced from bremsstrahlung measurements (made on a field line close to that of the satellite) had approximately the same e-folding energies as the trapped electron enhancements. However, the spectrum of electrons in the August 25 event was significantly harder than the spectrum in the event of August 11.

  4. Direct angle resolved photoelectron spectroscopy (DARPES) on high-Tc films: doping, strains, Fermi surface topology and superconductivity

    Science.gov (United States)

    Pavuna, D.; Ariosa, D.; Cancellieri, C.; Cloetta, D.; Abrecht, M.

    2008-03-01

    Since 1997 we systematically perform Direct ARPES ( = DARPES) on in-situ grown, non-cleaved, ultra-thin (<25nm) cuprate films. Specifically, we probe low energy electronic structure and properties of high-Tc films under different degree of epitaxial (compressive vs tensile) strain. In overdoped in-plane compressed La2-xSrxCuO4 (LSCO) thin films we double Tc from 20K to 40K, yet the Fermi surface (FS) remains essentially 2-dimensional (2D). In contrast, tensile strained films show 3-dimensional (3D) dispersion, while Tc is drastically reduced. It seems that the in-plane compressive strain tends to push the apical oxygen far away from the CuO2 plane, enhances the 2D character of the dispersion and increases Tc, while the tensile strain seems to act exactly in the opposite direction and the resulting dispersion is 3D. We have the FS topology for both cases. As the actual lattice of cuprates is 'Napoleon-cake' -like i.e. rigid CuO2 planes alternate with softer 'reservoir' (that strains distort differently) our results tend to rule out 2D rigid lattice mean field models. Finally, we briefly discuss recent successful determination of the FS topology from the observed wavevector quantization by DARPES in cuprate films thinner than 18 units cells (<24nm). Such an approach is of broader interest as it can be extended to other similar confined (ultra-thin) functional oxide systems.

  5. Comparative angle-resolved photoemission spectroscopy study of CaRuO3 and SrRuO3 thin films: Pronounced spectral weight transfer and possible precursor of lower Hubbard band

    Science.gov (United States)

    Yang, H. F.; Fan, C. C.; Liu, Z. T.; Yao, Q.; Li, M. Y.; Liu, J. S.; Jiang, M. H.; Shen, D. W.

    2016-09-01

    In the prototypical 4 d system (Sr ,Ca ) RuO3 , the degree and origin of electron correlations, and how they correlate with physical properties, still remain elusive, though extensive studies have been performed. In this work we present a comparative electronic structure study of high-quality epitaxial CaRuO3 and SrRuO3 thin films, by means of reactive molecular beam epitaxy and in situ angle-resolved photoemission spectroscopy. We found that while SrRuO3 possesses sharp features signaling the Fermi liquid state, the isostructural CaRuO3 exhibits broad features and its spectral weight is markedly transferred from the Fermi level to -1.2 eV forming a "hump" structure which resembles the Mott-Hubbard system (Sr ,Ca ) VO3 . We suggest that this hump is the precursor of the lower Hubbard band, and the U /W (U and W represent the on-site Coulomb interactions and bandwidth, respectively) of our CaRuO3 thin film is much larger than that of SrRuO3. In addition, we discuss the origin of electron correlations as well as the ferromagnetism in SrRuO3 which is absent in CaRuO3. Our findings put constraints on future studies, and also show that perovskite ruthenates are indeed an experimentally tunable system for the study of electron correlations.

  6. Direct angle resolved photoelectron spectroscopy (DARPES) on high-T{sub c} films: doping, strains, Fermi surface topology and superconductivity

    Energy Technology Data Exchange (ETDEWEB)

    Pavuna, D; Ariosa, D; Cancellieri, C; Cloetta, D; Abrecht, M [Institute of Physics of Complex Matter, FSB, Ecole Polytechnique Federale de Lausanne (EPFL), CH-1015 Lausanne (Switzerland)], E-mail: davor.pavuna@epfl.ch

    2008-03-15

    Since 1997 we systematically perform Direct ARPES ( = DARPES) on in-situ grown, non-cleaved, ultra-thin (<25nm) cuprate films. Specifically, we probe low energy electronic structure and properties of high-T{sub c} films under different degree of epitaxial (compressive vs tensile) strain. In overdoped in-plane compressed La{sub 2-x}Sr{sub x}CuO{sub 4} (LSCO) thin films we double T{sub c} from 20K to 40K, yet the Fermi surface (FS) remains essentially 2-dimensional (2D). In contrast, tensile strained films show 3-dimensional (3D) dispersion, while T{sub c} is drastically reduced. It seems that the in-plane compressive strain tends to push the apical oxygen far away from the CuO{sub 2} plane, enhances the 2D character of the dispersion and increases T{sub c}, while the tensile strain seems to act exactly in the opposite direction and the resulting dispersion is 3D. We have the FS topology for both cases. As the actual lattice of cuprates is 'Napoleon-cake' -like i.e. rigid CuO{sub 2} planes alternate with softer 'reservoir' (that strains distort differently) our results tend to rule out 2D rigid lattice mean field models. Finally, we briefly discuss recent successful determination of the FS topology from the observed wavevector quantization by DARPES in cuprate films thinner than 18 units cells (<24nm). Such an approach is of broader interest as it can be extended to other similar confined (ultra-thin) functional oxide systems.

  7. Electron energy and angular distributions in radiotherapy

    Energy Technology Data Exchange (ETDEWEB)

    Deasy, J.O.

    1992-01-01

    Electron energy and angular distributions and associated effects for radiotherapy accelerators and beta-ray ophthalmic applicators have been measured and modeled. Ophthalmic applicator extrapolation chamber calibration geometries were studied using Monte Carlo calculations and analytic methods. A large interface effect increases the surface dose by a factor of about 1.5 and makes very small gap width measurements necessary (0.1--0.2 mm). Dose deposition in tissue near the surface was simulated using the Monte Carlo technique. Charge collection in the extrapolation chamber was analytically modeled on the basis of ionized free electrons back-diffusing into the cathode, while taking into account attachment to O[sub 2] ions. Two small, portable, magnetic spectrometers for the measurement of clinical radiotherapy electron beams were constructed. One employs film as a spectrograph and is suitable for routine measurements; the second is a 90[degree] single-focusing spectrometer and uses fast pulse counting electrons and pulse-height analysis. Spectra were measured for the University of Louisville's Theratronics T20 and Philips SL25 linear accelerators. The T20 spectra were all Gaussian with energy widths of about 5%. The SL25 energy spectra were of varied shapes, with energy widths of 10--20%. Evidence of 3--7% shifts in the average energy of the SL25 beams was observed. Angular measurements were made which showed the Gaussian angular spread of the incident beam. The Monte Carlo code CYLTRAN and measured spectra were used to reconstruct depth dose curves. The peak energy structure only marginally affects the shape of the depth-dose curve, and some features of the depth-dose curves must be affected by incident straggled or widely-scattered electrons. In the absence of lower energy straggled electrons, the range parameters and the maximum dose gradient depend on the mean energy of the peak electrons.

  8. Momentum-resolved electron-phonon coupling and self-energy effects in YBa{sub 2}Cu{sub 3}O{sub 7}: an LDA study

    Energy Technology Data Exchange (ETDEWEB)

    Heid, Rolf; Bohnen, Klaus-Peter [Forschungszentrum Karlsruhe, Institut fuer Festkoerperphysik (Germany); Zeyher, Roland; Manske, Dirk [Max-Planck-Institut fuer Festkoerperforschung, Stuttgart (Germany)

    2008-07-01

    The observation of kinks in the electronic dispersion of high-T{sub c} cuprates by angle resolved photoemission experiments has revived the discussion about the importance of electron-phonon interaction in the cuprates. Here we determine the effect of the electron-phonon coupling on the electronic self-energy in the normal state within the local-density approximation. Using a realistic phonon spectrum we determine the momentum and frequency dependence of {alpha}{sup 2}F(k,{omega}) in YBa{sub 2}Cu{sub 3}O{sub 7} for the bonding, antibonding, and chain band. We find that the maximum in the real part of the self-energy at low frequencies is about a factor 5 too small compared to the experiment. The renormalization factor Z(k,{omega}), which determines the change in the slope of the electronic dispersion due to the interaction, varies smoothly as a function of frequency and momentum. These findings show that, at least within the LDA, phonons cannot produce well-pronounced kinks in YBa{sub 2}Cu{sub 3}O{sub 7}.

  9. Angle-resolved photoemission spectroscopy on high-temperature superconductors. Studies of Bi2212 and single-layer FeSe film grown on SrTiO{sub 3} substrate

    Energy Technology Data Exchange (ETDEWEB)

    He, Junfeng [Chinese Academy of Sciences, Beijing (China). Inst. of Physics

    2016-07-01

    This book mainly focuses on the study of the high-temperature superconductor Bi{sub 2}Sr{sub 2}CaCu{sub 2}O{sub 8+δ} (Bi2212) and single-layer FeSe film grown on SrTiO{sub 3} (STO) substrate by means of angle-resolved photoemission spectroscopy (ARPES). It provides the first electronic evidence for the origin of the anomalous high-temperature superconductivity in single-layer FeSe grown on SrTiO{sub 3} substrate. Two coexisted sharp-mode couplings have been identified in superconducting Bi2212. The first ARPES study on single-layer FeSe/STO films has provided key insights into the electronic origin of superconductivity in this system. A phase diagram and electronic indication of high T{sub c} and insulator to superconductor crossover have been established in the single-layer FeSe/STO films. Readers will find essential information on the techniques used and interesting physical phenomena observed by ARPES.

  10. Low energy electron scattering from fuels

    Energy Technology Data Exchange (ETDEWEB)

    Lopes, M. Cristina A.; Silva, Daniel G.M.; Coelho, Rafael F.; Duque, Humberto V.; Santos, Rodrigo R. dos; Ribeiro, Thiago M. [Universidade Federal de Juiz de Fora (UFJF), MG (Brazil). Dept. de Fisica; Yates, Brent; Hong, Ling; Khakoo, Murtadha A. [California State University at Fullerton, CA (US). Physics Department; Bettega, Marcio H.F. [Universidade Federal do Parana (UFPR), Curitiba, PR (Brazil). Dept. de Fisica; Costa, Romarly F. da [Universidade Federal do ABC (UFABC), Santo Andre, SP (Brazil). Centro de Ciencias Naturais e Humanas; Lima, Marco A.P. [Laboratorio Nacional de Ciencia e Tecnologia do Bioetanol (CTBE/CNPEM), Campinas, SP (Brazil)

    2011-07-01

    Full text. Accurate and precise values of absolute total cross section (TCS) represent important information in many scientific and technological applications. In our case, for example, we are motivated to provide such information for electron-fuel collision processes which are specifically relevant to modeling spark ignition in alcohol-fuelled internal combustion engines. Many electron scattering TCS measurements are presently available for a diverse range of atomic and molecular targets. However, lack of data for important bio-molecular targets still remains. Disagreements between the available TCS data for the alcohols have prompted several studies of electron scattering collision of slow electrons with these molecules which are currently important in applications as bio- fuels. This relevance, which has attracted much attention, has been one of the subjects of a recent collaboration between experimental and theoretical groups in the USA and Brazil. Recently this collaboration reported first measurements and calculations of differential cross sections for elastic low-energy (rotationally unresolved) electron scattering by several primary alcohols. In this work we address methanol and ethanol TCSs at low energy range and report additional studies of resonant structure in ethanol using the detection of metastable states produced by electron impact excitation with high energy resolution. We have recently constructed a TCS apparatus in our laboratory at Universidade Federal de Juiz de Fora, Brazil, based on the well-known linear transmission technique. The experimental setup is based on the measurement of the attenuation of a collimated electron beam through a gas cell containing the atoms or molecules to be studied at a given pressure. It consists essentially of an electron gun, a gas cell and an electron energy analyzer composed of an array of decelerating electrostatic lenses, a cylindrical dispersive 127o analyzer and a Faraday cup. To our knowledge, there exist

  11. Electron Energy and Angular Distributions in Radiotherapy.

    Science.gov (United States)

    Deasy, Joseph Owen

    1992-01-01

    Electron energy and angular distributions and associated effects for radiotherapy accelerators and beta -ray ophthalmic applicators have been measured and modeled. Ophthalmic applicator extrapolation chamber calibration geometries were studied using Monte Carlo calculations and analytic methods. A large interface effect increases the surface dose by a factor of about 1.5 and makes very small gap width measurements necessary (0.1-0.2 mm). Dose deposition in tissue near the surface was simulated using the Monte Carlo technique. Charge collection in the extrapolation chamber was analytically modeled on the basis of ionized free electrons back-diffusing into the cathode, while taking into account attachment to O_2 ions. Previous models underpredict the charge loss, mainly because they assume that all the charge carriers are ions. Two small, portable, magnetic spectrometers for the measurement of clinical radiotherapy electron beams were constructed. One employs film as a spectrograph and is suitable for routine measurements; the second is a 90^circ single-focusing spectrometer and uses fast pulse counting electronics and pulse-height analysis. Tests with monoenergetic electron beams at the National Research Council of Canada's electron linear accelerator showed that the system is free from spectral distortion and verified the spectrometers' energy calibrations. Spectra were measured for the University of Louisville's Theratronics T20 and Philips SL25 linear accelerators. The T20 spectra were all nearly Gaussian in shape with energy widths of about 5%. The SL25 energy spectra were of varied shapes, with energy widths of 10-20%. Evidence of 3-7% shifts in the average energy of the SL25 beams was observed. Angular measurements were made which showed the Gaussian angular spread of the incident beam. The Monte Carlo code CYLTRAN and measured spectra were used to reconstruct depth dose curves. Comparisons with measured depth dose curves show that the peak energy structure

  12. Stability of electron energy in the Fermilab electron cooler

    Energy Technology Data Exchange (ETDEWEB)

    Shemyakin, A.; Carlson, K.; Prost, L.R.; Saewert, G.; /Fermilab

    2009-02-01

    A powerful electron beam (4.3 MeV, 0.1 A DC) generated by an electrostatic accelerator has been used at Fermilab for three years to cool antiprotons in the Recycler ring. For electron cooling to be effective, the electron energy should not deviate from its optimum value by more than 500V. The main tool for studying the energy stability is the electron beam position in a high-dispersion area. The energy ripple (frequencies above 0.2 Hz) was found to be less than 150 eV rms; the main cause of the ripple is the fluctuations of the chain current. In addition, the energy can drift to up to several keV that is traced to two main sources. One of them is a drift of the charging current, and another is a temperature dependence of generating voltmeter readings. The paper describes the efforts to reach the required level of stability as well as the setup, diagnostics, results of measurements, and operational experience.

  13. Local operator partitioning of electronic energy for electronic energy transfer: An efficient algorithm

    CERN Document Server

    Nagesh, Jayashree; Brumer, Paul

    2013-01-01

    An efficient computational algorithm to implement a local operator approach to partitioning electronic energy in general molecular systems is presented. This approach, which rigorously defines the electronic energy on any subsystem within a molecule, gives a precise meaning to the subsystem ground and excited electronic energies, which is crucial for investigating electronic energy transfer from first principles. We apply the technique to the $9-$(($1-$naphthyl)$-$methyl)-anthracene (A1N) molecule by partitioning A1N into anthracenyl and CH$_2-$naphthyl groups as subsystems, and examine their electronic energies and populations for several excited states using Configuration Interaction Singles method. The implemented approach shows a wide variety of different behaviors amongst these excited electronic states.

  14. On Puthoff's Semiclassical Electron and Vacuum Energy

    Science.gov (United States)

    Pereira, N. R.

    2016-09-01

    A possible connection between a point electron and vacuum energy was recently claimed by Puthoff (Int. J. Theor. Phys. 46, 3005 (2007)). He envisions a point electron as an ideally conducting spherical shell with a distributed charge on the surface, in equilibrium with the radiation pressure from electromagnetic vacuum fluctuations on the outside, and claims that his analysis demonstrates the reality of high-energy-density vacuum fluctuation fields. The present paper finds, instead, that the analysis is meaningless without specific knowledge on the cutoff frequency that is a free parameter in the model.

  15. Powering the Digital: From Energy Ecologies to Electronic Environmentalism

    OpenAIRE

    Gabrys, Jennifer

    2014-01-01

    Electronics and all that they plug into are energy intensive. Energy is another form of waste, like electronic waste that contributes to the material footprint of electronic technologies. This chapter examines the particular ways in which electronics use energy, from manufacture to powering devices to running cloud servers. While electronics consume energy, they are also used to manage energy consumption with the hope of achieving greater sustainability. By developing the concept of “electron...

  16. Applications for Energy Recovering Free Electron Lasers

    Energy Technology Data Exchange (ETDEWEB)

    George Neil

    2007-08-01

    The availability of high-power, high-brilliance sources of tunable photons from energy-recovered Free Electron Lasers is opening up whole new fields of application of accelerators in industry. This talk will review some of the ideas that are already being put into production, and some of the newer ideas that are still under development.

  17. Electronic Energy Transfer in Polarizable Heterogeneous Environments

    DEFF Research Database (Denmark)

    Svendsen, Casper Steinmann; Kongsted, Jacob

    2015-01-01

    Theoretical prediction of transport and optical properties of protein-pigment complexes is of significant importance when aiming at understanding the structure versus function relationship in such systems. Electronic energy transfer (EET) couplings represent a key property in this respect since...

  18. Electronic excitation of molecular hydrogen by low-energy electrons

    Science.gov (United States)

    Hargreaves, Leigh

    2016-09-01

    Molecular hydrogen is the most abundant element in the universe, particularly in interstellar plasmas such as atmospheres of gas giant planets and stars. Electron collision data for hydrogen is critical to interpreting the spectroscopy of interstellar objects, as well as being of applied value for modelling technological plasmas. Hydrogen is also fundamentally interesting, as while highly accurate wave functions for this simple molecule are available, providing an accurate, ab initio, treatment the collision dynamics has proven challenging, on account of the need to have a complete description of channel coupling and polarization effects. To date, no single theoretical approach has been able to replicate experimental results across all transitions and incident energies, while the experimental database that is available is far from complete and not all available measurements are in satisfactory agreement. In this talk, we present differential and integral cross section measurements for electronic excitation cross sections for molecular hydrogen by low-energy electron impact. The data were measured at incident energies below 20eV, using a well-tested crossed beam apparatus and employing a moveable gas source approach to ensure that background contributions to the scattering are accurately accounted for. These measurements are compared with new theoretical results employing the convergent close coupling approach.

  19. Electron clouds in high energy hadron accelerators

    Energy Technology Data Exchange (ETDEWEB)

    Petrov, Fedor

    2013-08-29

    The formation of electron clouds in accelerators operating with positrons and positively charge ions is a well-known problem. Depending on the parameters of the beam the electron cloud manifests itself differently. In this thesis the electron cloud phenomenon is studied for the CERN Super Proton Synchrotron (SPS) and Large Hadron Collider (LHC) conditions, and for the heavy-ion synchrotron SIS-100 as a part of the FAIR complex in Darmstadt, Germany. Under the FAIR conditions the extensive use of slow extraction will be made. After the acceleration the beam will be debunched and continuously extracted to the experimental area. During this process, residual gas electrons can accumulate in the electric field of the beam. If this accumulation is not prevented, then at some point the beam can become unstable. Under the SPS and LHC conditions the beam is always bunched. The accumulation of electron cloud happens due to secondary electron emission. At the time when this thesis was being written the electron cloud was known to limit the maximum intensity of the two machines. During the operation with 25 ns bunch spacing, the electron cloud was causing significant beam quality deterioration. At moderate intensities below the instability threshold the electron cloud was responsible for the bunch energy loss. In the framework of this thesis it was found that the instability thresholds of the coasting beams with similar space charge tune shifts, emittances and energies are identical. First of their kind simulations of the effect of Coulomb collisions on electron cloud density in coasting beams were performed. It was found that for any hadron coasting beam one can choose vacuum conditions that will limit the accumulation of the electron cloud below the instability threshold. We call such conditions the ''good'' vacuum regime. In application to SIS-100 the design pressure 10{sup -12} mbar corresponds to the good vacuum regime. The transition to the bad vacuum

  20. Gas Electron multipliers for low energy beams

    CERN Document Server

    Arnold, F; Ropelewski, L; Spanggaard, J; Tranquille, G

    2010-01-01

    Gas Electron Multipliers (GEM) find their way to more and more applications in beam instrumentation. Gas Electron Multiplication uses a very similar physical phenomenon to that of Multi Wire Proportional Chambers (MWPC) but for small profile monitors they are much more cost efficient both to produce and to maintain. This paper presents the new GEM profile monitors intended to replace the MWPCs currently used at CERN’s low energy Antiproton Decelerator (AD). It will be shown how GEMs overcome the documented problems of profile measurements with MWPCs for low energy beams, where the interaction of the beam with the detector has a large influence on the measured profile. Results will be shown of profile measurements performed at 5 MeV using four different GEM prototypes, with discussion on the possible use of GEMs at even lower energies needed at the AD in 2013.

  1. Low-temperature (1 K) angle-resolved photoemission investigation of the predicted topological Kondo insulator behavior of SmB6

    Science.gov (United States)

    Rader, Oliver; Hlawenka, Peter; Rienks, Emile; Siemensmeyer, Konrad; Weschke, Eugen; Varykhalov, Andrei; Shitsevalova, Natalya; Gabani, Slavomir; Flachbart, Karol

    2015-03-01

    The system SmB6 is known for its unusual resistivity which increases exponentially with decreasing temperature and saturates below 3 K. This has recently been attributed to topological-Kondo-insulator behavior where a topological surface state is created by Sm 4 f - 5 d hybridization and is responsible for the transport. Local-density-approximation + Gutzwiller calculations of the (100) surface predict the appearance of three Dirac cones in the surface Brillouin zone. We perform angle-resolved photoemission at temperatures below 1 K and reveal surface states at Γ and X . Bulk conduction band states near X appear at higher temperature. These findings will be discussed in detail vis-á-vis the theoretical and experimental literature.

  2. Superconducting gap in Bi-Sr-Ca-Cu-O by high-resolution angle-resolved photoelectron spectroscopy

    Energy Technology Data Exchange (ETDEWEB)

    Olson, C.G.; Liu, R.; Yang, A.B.; Lynch, D.W. (Iowa State Univ., Ames (USA)); Arko, A.J.; List, R.S. (Los Alamos National Lab., NM (USA)); Veal, B.W.; Chang, Y.C.; Jiang, P.Z.; Paulikas, A.P. (Argonne National Lab., IL (USA))

    1989-08-18

    Detailed studies indicate a superconducting gap in the high-temperature superconductor Bi{sub 2}Sr{sub 2}CaCu{sub 2}O{sub 8}. Photoemission measurements with high energy and angle resolution isolate the behavior of a single band as it crosses the Fermi level in both the normal and superconducting states, giving support to the Fermi liquid picture. The magnitude of the gap is 24 millielectron volts. 18 refs., 3 figs.

  3. Electronic and structural characterizations of unreconstructed {l_brace}0001{r_brace} surfaces and the growth of graphene overlayers

    Energy Technology Data Exchange (ETDEWEB)

    Emtsev, Konstantin

    2009-06-03

    The present work is focused on the characterization of the clean unreconstructed SiC{l_brace}0001{r_brace} surfaces and the growth of graphene overlayers thereon. Electronic properties of SiC surfaces and their interfaces with graphene and few layer graphene films were investigated by means of angle resolved photoelectron spectroscopy, X-ray photoelectron spectroscopy and low energy electron diffraction. Structural characterizations of the epitaxial graphene films grown on SiC were carried out by atomic force microscopy and low energy electron microscopy. Supplementary data was obtained by scanning tunneling microscopy. (orig.)

  4. Energy Transformation in Molecular Electronic Systems

    Energy Technology Data Exchange (ETDEWEB)

    Kasha, Michael

    1999-05-17

    This laboratory has developed many new ideas and methods in the electronic spectroscopy of molecules. This report covers the contract period 1993-1995. A number of the projects were completed in 1996, and those papers are included in the report. The DOE contract was terminated at the end of 1995 owing to a reorganizational change eliminating nationally the projects under the Office of Health and Environmental Research, U. S. Department of Energy.

  5. Low-energy electron scattering from cyanamide

    Science.gov (United States)

    Wang, Kedong; Guo, Shuangcheng; Meng, Ju; Huang, Xiaotian; Wang, Yongfeng

    2016-09-01

    The low-energy electron collisions with cyanamide molecule are investigated by using the UK molecular R -matrix codes for electron energies ranging from 0.01 eV to 10 eV. Three models including static-exchange, static-exchange plus polarization, and close-coupling (CC) approximations are employed to reveal the dynamic interaction. Elastic (integrated and differential), momentum-transfer, and excitation cross sections from the ground state to the three low-lying electron excited states have been presented. Two shape resonances, two core-excited resonances, and two Feshbach resonances are detected in the CC approximation. The role of active space in the target and scattering problem including the resonances is discussed. The precise resonance parameters are found to be sensitive to the treatment of polarization effects employed. These resonances may be responsible for the fragments observed in a recent experiment of the dissociative electron attachments to cyanamide. Since the cyanamide molecule has a large permanent dipole moment, a Born closure procedure is used to account for the contribution of partial waves higher than l =4 to obtain converged cross sections.

  6. Isotope Effect on Electron-Phonon Coupling in Multiband Superconductor MgB2

    Science.gov (United States)

    Mou, Daixiang; Taufour, Valentin; Wu, Yun; Huang, Lunan; Bud'Ko, Serguei; Canfield, Paul; Kaminski, Adam

    We systematically investigate the isotope effect of electron-phonon coupling in multi-band superconductor MgB2 by laser based Angle Resolved Photoemission Spectroscopy. The kink structure around 70 meV on two σ bands, which is caused by electron coupling to E2 g phonon mode, is shifted to higher binding energy in Mg10B2 than that in Mg11B2. The measured shifting energy of 3.5 meV is consistent with theoretical calculation based on harmonic phonon in MgB2. Our temperature dependent measurement also indicates the isotope effect of kink structure is not dependent on superconducting transition.

  7. Electron-electron correlations in square-well quantum dots: direct energy minimization approach.

    Science.gov (United States)

    Goto, Hidekazu; Hirose, Kikuji

    2011-04-01

    Electron-electron correlations in two-dimensional square-well quantum dots are investigated using the direct energy minimization scheme. Searches for groundstate charges and spin configurations are performed with varying the sizes of dots and the number of electrons. For a two-electron system, a standout difference between the configurations with and without counting correlation energy is demonstrated. The emergence and melting of Wigner-molecule-like structures arising from the interplay between the kinetic energy and Coulombic interaction energy are described. Electron-electron correlation energies and addition energy spectra are calculated, and special electron numbers related to peculiar effects of the square well are extracted.

  8. Design and validation of an angle-resolved low-coherence interferometry fiber probe for in vivo clinical measurements of depth-resolved nuclear morphology

    Science.gov (United States)

    Zhu, Yizheng; Terry, Neil G.; Woosley, John T.; Shaheen, Nicholas J.; Wax, Adam

    2011-01-01

    We present a novel Fourier-domain angle-resolved low-coherence interferometry (a /LCI) fiber probe designed for in vivo clinical application in gastrointestinal endoscopy. The a/LCI technique measures the depth-resolved angular scattering distribution to determine the size distribution and optical density of cell nuclei for assessing the health of epithelial tissues. Clinical application is enabled by an endoscopic fiber-optic probe that employs a 2.3-m-long coherent fiber bundle and is compatible with the standard 2.8-mm-diam biopsy channel of a gastroscope. The probe allows for real-time data acquisition by collecting the scattering from multiple angles in parallel, enabled by the Fourier domain approach. The performance of the probe is characterized through measurement of critical parameters. The depth-resolved sizing capability of the system is demonstrated using single- and double-layer microsphere phantoms with subwavelength sizing precision and accuracy achieved. Initial results from a clinical feasibility test are also presented to show in vivo application in the human esophagus.

  9. Influence of surface hydroxylation on 3-aminopropyltriethoxysilane growth mode during chemical functionalization of GaN Surfaces: an angle-resolved X-ray photoelectron spectroscopy Study.

    Science.gov (United States)

    Arranz, A; Palacio, C; García-Fresnadillo, D; Orellana, G; Navarro, A; Muñoz, E

    2008-08-19

    A comparative study of the chemical functionalization of undoped, n- and p-type GaN layers grown on sapphire substrates by metal-organic chemical vapor deposition was carried out. Both types of samples were chemically functionalized with 3-aminopropyltriethoxysilane (APTES) using a well-established silane-based approach for functionalizing hydroxylated surfaces. The untreated surfaces as well as those modified by hydroxylation and APTES deposition were analyzed using angle-resolved X-ray photoelectron spectroscopy. Strong differences were found between the APTES growth modes on n- and p-GaN surfaces that can be associated with the number of available hydroxyl groups on the GaN surface of each sample. Depending on the density of surface hydroxyl groups, different mechanisms of APTES attachment to the GaN surface take place in such a way that the APTES growth mode changes from a monolayer to a multilayer growth mode when the number of surface hydroxyl groups is decreased. Specifically, a monolayer growth mode with a surface coverage of approximately 78% was found on p-GaN, whereas the formation of a dense film, approximately 3 monolayers thick, was observed on n-GaN.

  10. Cation profiling of passive films on stainless steel formed in sulphuric and acetic acid by deconvolution of angle-resolved X-ray photoelectron spectra

    Energy Technology Data Exchange (ETDEWEB)

    Högström, Jonas, E-mail: jhogstrom@gmail.com; Fredriksson, Wendy, E-mail: wendy.fredriksson@kemi.uu.se; Edstrom, Kristina, E-mail: kristina.edstrom@kemi.uu.se; Björefors, Fredrik, E-mail: fredrik.bjorefors@kemi.uu.se; Nyholm, Leif, E-mail: leif.nyholm@kemi.uu.se; Olsson, Claes-Olof A., E-mail: drclabbe@kth.se

    2013-11-01

    An approach for determining depth gradients of metal-ion concentrations in passive films on stainless steel using angle-resolved X-ray photoelectron spectroscopy (ARXPS) is described. The iterative method, which is based on analyses of the oxidised metal peaks, provides increased precision and hence allows faster ARXPS measurements to be carried out. The method was used to determine the concentration depth profiles for molybdenum, iron and chromium in passive films on 316L/EN 1.4432 stainless steel samples oxidised in 0.5 M H{sub 2}SO{sub 4} and acetic acid diluted with 0.02 M Na{sub 2}B{sub 4}O{sub 7} · 10H{sub 2}O and 1 M H{sub 2}O, respectively. The molybdenum concentration in the film is pin-pointed to the oxide/metal interface and the films also contained an iron-ion-enriched surface layer and a chromium-ion-dominated middle layer. Although films of similar composition and thickness (i.e., about 2 nm) were formed in the two electrolytes, the corrosion currents were found to be three orders of magnitude larger in the acetic acid solution. The differences in the layer composition, found for the two electrolytes as well as different oxidation conditions, can be explained based on the oxidation potentials of the metals and the dissolution rates of the different metal ions.

  11. Adsorption site and structure determination of c(2x2) N{sub 2}/Ni(100) using angle-resolved photoemission extended fine structure

    Energy Technology Data Exchange (ETDEWEB)

    Moler, E.J.; Kellar, S.A.; Huff, W.R.A. [Lawrence Berkeley National Lab., CA (United States)] [and others

    1997-04-01

    The authors have determined the atomic spatial structure of c(2x2) N2Ni(100) with Angle-Resolved Photoemission Extended Fine Structure (ARPEFS) from the nitrogen 1s core level using monochromatized x-rays from beamline 6.1 at SSRL and beamline 9.3.2 at the ALS. The chemically shifted N 1s peak intensities were summed together to obtain ARPEFS curves for both nitrogen atoms in the molecule. They used a new, highly-optimized program based on the Rehr-Albers scattering matrix formalism to find the adsorption site and to quantitatively determine the bond-lengths. The nitrogen molecule stands upright at an atop site, with a N-Ni bond length of 2.25(1) {angstrom}, a N-N bond length of 1.10(7) {angstrom}, and a first layer Ni-Ni spacing of 1.76(4) {angstrom}. The shake-up peak shows an identical ARPEFS diffraction pattern, confirming its intrinsic nature and supporting a previous use of this feature to decompose the peak into contributions from the chemically inequivalent nitrogen atoms. Comparison to a previously published theoretical treatment of N-N-Ni and experimental structures of analogous adsorbate systems demonstrates the importance of adsorbate-adsorbate interactions in weakly chemisorbed systems.

  12. High energy electron beams for ceramic joining

    Energy Technology Data Exchange (ETDEWEB)

    Turman, B.N.; Glass, S.J.; Halbleib, J.A.; Helmich, D.R.; Loehman, R.E. [Sandia National Labs., Albuquerque, NM (United States); Clifford, J.R. [Titan Corp., Albuquerque, NM (United States)

    1994-12-31

    Joining of structural ceramics is possible using high melting point metals such as Mo and Pt that are heated with a high energy electron beam, with the potential for high temperature joining. A 10 MeV electron beam can penetrate through 1 cm of ceramic, offering the possibility of buried interface joining. Because of transient heating and the lower heat capacity of the metal relative to the ceramic, a pulsed high power beam has the potential for melting the metal without decomposing or melting the ceramic. We have demonstrated the feasibility of the process with a series of 10 MeV, 1 kW electron beam experiments. Shear strengths up to 28 MPa have been measured. This strength is comparable to that reported in the literature for bonding silicon nitride to molybdenum with copper-silver-titanium braze, but weaker than that reported for Si{sub 3}N{sub 4}-Si{sub 3}N{sub 4} with gold-nickel braze. The bonding mechanism appears to be a thin silicide layer.

  13. Electron-beam induced disorder effects in optimally doped Bi2Sr2CaCu2O8+x single crystal samples

    Science.gov (United States)

    Vobornik, I.; Berger, H.; Pavuna, D.; Margaritondo, G.; Forro, L.; Grioni, M.; Rullier-Albenque, F.; Onellion, M.; EPFL Collaboration; Laboratoire Des Solides Irradiés Collaboration

    2000-03-01

    We report on the effects of electron-beam induced disorder in optimally doped Bi2Sr2CaCu2O8+x single crystal samples, measured with angle-resolved photoemission. In the superconducting state, the disorder fills in the gap, without changing the binding energy or the width of the narrow coherent feature.[1] In the normal state, disorder leads to an anisotropic pseudogap in angle-resolved photoemission, with the largest pseudogap near the (0,p) point and no pseudogap in the direction.[2,3] We discuss implications of these data. 1. I. Vobornik et.al., Phys. Rev. Lett. 82 , 3128 (1999). 2. I. Vobornik, Ph.D. thesis, EPFL, Lausanne, Switzerland, October, 1999. 3. I. Vobornik et.al., unpublished.

  14. Femtosecond spectroscopy of electron-electron and electron-phonon energy relaxation in Ag and Au

    Science.gov (United States)

    Groeneveld, Rogier H. M.; Sprik, Rudolf; Lagendijk, Ad

    1995-05-01

    We show experimentally that the electron distribution of a laser-heated metal is a nonthermal distribution on the time scale of the electron-phonon (e-ph) energy relaxation time τE. We measured τE in 45-nm Ag and 30-nm Au thin films as a function of lattice temperature (Ti=10-300 K) and laser-energy density (Ul=0.3-1.3 J cm-3), combining femtosecond optical transient-reflection techniques with the surface-plasmon polariton resonance. The experimental effective e-ph energy relaxation time decreased from 710-530 fs and 830-530 fs for Ag and Au, respectively, when temperature is lowered from 300 to 10 K. At various temperatures we varied Ul between 0.3-1.3 J cm-3 and observed that τE is independent from Ul within the given range. The results were first compared to theoretical predictions of the two-temperature model (TTM). The TTM is the generally accepted model for e-ph energy relaxation and is based on the assumption that electrons and lattice can be described by two different time-dependent temperatures Te and Ti, implying that the two subsystems each have a thermal distribution. The TTM predicts a quasiproportional relation between τE and Ti in the perturbative regime where τE is not affected by Ul. Hence, it is shown that the measured dependencies of τE on lattice temperature and energy density are incompatible with the TTM. It is proven that the TTM assumption of a thermal electron distribution does not hold especially under our experimental conditions of low laser power and lattice temperature. The electron distribution is a nonthermal distribution on the picosecond time scale of e-ph energy relaxation. We developed a new model, the nonthermal electron model (NEM), in which we account for the (finite) electron-electron (e-e) and electron-phonon dynamics simultaneously. It is demonstrated that incomplete electron thermalization yields a slower e-ph energy relaxation in comparison to the thermalized limit. With the NEM we are able to give a consistent

  15. Trapping Surface Electrons on Graphene Layers and Islands

    OpenAIRE

    Niesner, D.; Fauster, Th.; Dadap, J. I.; Zaki, N.; Knox, K. R.; Yeh, P. -C.; Bhandari, R.; Osgood, R. M.; Petrović, M; Kralj, M.

    2011-01-01

    We report the use of time- and angle-resolved two-photon photoemission to map the bound, unoccupied electronic structure of the weakly coupled graphene/Ir(111) system. The energy, dispersion, and lifetime of the lowest three image-potential states are measured. In addition, the weak interaction between Ir and graphene permits observation of resonant transitions from an unquenched Shockley-type surface state of the Ir substrate to graphene/Ir image-potential states. The image-potential-state l...

  16. Power Electronics Control of Wind Energy in Distributed Power System

    DEFF Research Database (Denmark)

    Iov, Florin; Ciobotaru, Mihai; Blaabjerg, Frede

    2008-01-01

    emerging renewable energy sources, wind energy, which by means of power electronics are changing from being a minor energy source to be acting as an important power source in the energy system. Power electronics is the enabling technology and the presentation will cover the development in wind turbine...

  17. Isotope effect on electron-phonon interaction in the multiband superconductor MgB2

    Science.gov (United States)

    Mou, Daixiang; Manni, Soham; Taufour, Valentin; Wu, Yun; Huang, Lunan; Bud'ko, S. L.; Canfield, P. C.; Kaminski, Adam

    2016-04-01

    We investigate the effect of isotope substitution on the electron-phonon interaction in the multiband superconductor MgB2 using tunable laser-based angle-resolved photoemission spectroscopy. The kink structure around 70 meV in the σ band, which is caused by electron coupling to the E2 g phonon mode, is shifted to higher binding energy by ˜3.5 meV in Mg 10B2 and the shift is not affected by superconducting transition. These results serve as the benchmark for investigations of isotope effects in known, unconventional superconductors and newly discovered superconductors where the origin of pairing is unknown.

  18. Automated classification of single airborne particles from two-dimensional angle-resolved optical scattering (TAOS) patterns by non-linear filtering

    Science.gov (United States)

    Crosta, Giovanni Franco; Pan, Yong-Le; Aptowicz, Kevin B.; Casati, Caterina; Pinnick, Ronald G.; Chang, Richard K.; Videen, Gorden W.

    2013-12-01

    Measurement of two-dimensional angle-resolved optical scattering (TAOS) patterns is an attractive technique for detecting and characterizing micron-sized airborne particles. In general, the interpretation of these patterns and the retrieval of the particle refractive index, shape or size alone, are difficult problems. By reformulating the problem in statistical learning terms, a solution is proposed herewith: rather than identifying airborne particles from their scattering patterns, TAOS patterns themselves are classified through a learning machine, where feature extraction interacts with multivariate statistical analysis. Feature extraction relies on spectrum enhancement, which includes the discrete cosine FOURIER transform and non-linear operations. Multivariate statistical analysis includes computation of the principal components and supervised training, based on the maximization of a suitable figure of merit. All algorithms have been combined together to analyze TAOS patterns, organize feature vectors, design classification experiments, carry out supervised training, assign unknown patterns to classes, and fuse information from different training and recognition experiments. The algorithms have been tested on a data set with more than 3000 TAOS patterns. The parameters that control the algorithms at different stages have been allowed to vary within suitable bounds and are optimized to some extent. Classification has been targeted at discriminating aerosolized Bacillus subtilis particles, a simulant of anthrax, from atmospheric aerosol particles and interfering particles, like diesel soot. By assuming that all training and recognition patterns come from the respective reference materials only, the most satisfactory classification result corresponds to 20% false negatives from B. subtilis particles and classification method may be adapted into a real-time operation technique, capable of detecting and characterizing micron-sized airborne particles.

  19. Triple Hybrid Energy Harvesting Interface Electronics

    Science.gov (United States)

    Uluşan, H.; Chamanian, S.; Pathirana, W. M. P. R.; Zorlu, Ö.; Muhtaroğlu, A.; Külah, H.

    2016-11-01

    This study presents a novel triple hybrid system that combines simultaneously generated power from thermoelectric (TE), vibration-based electromagnetic (EM) and piezoelectric (PZT) harvesters for a relatively high power supply capability. In the proposed solution each harvesting source utilizes a distinct power management circuit that generates a DC voltage suitable for combining the three parallel supplies. The circuits are designed and implemented in 180 nm standard CMOS technology, and are terminated with a schottky diode to avoid reverse current flow. The harvested AC signal from the EM harvester is rectified with a self-powered AC-DC doubler, which utilizes active diode structures to minimize the forward- bias voltage drop. The PZT interface electronics utilizes a negative voltage converter as the first stage, followed by synchronous power extraction and DC-to-DC conversion through internal switches, and an external inductor. The ultra-low voltage DC power harvested by the TE generator is stepped up through a charge-pump driven by an LC oscillator with fully- integrated center-tapped differential inductors. Test results indicate that hybrid energy harvesting circuit provides more than 1 V output for load resistances higher than 100 kΩ (10 μW) where the stand-alone harvesting circuits are not able to reach 1 V output. This is the first hybrid harvester circuit that simultaneously extracts energy from three independent sources, and delivers a single DC output.

  20. Observation of the weak electronic correlations in KFeCoAs2 (3d 6): an isoelectronic to the parent compounds of 122 series of iron pnictides BaFe2As2

    Science.gov (United States)

    Liu, Z. H.; Yaresko, A. N.; Li, Y.; Dai, P. C.; Zhang, H.; Büchner, B.; Lin, C. T.; Borisenko, S. V.

    2017-03-01

    Using the angle-resolved photoemission spectroscopy and band structure calculations we study the electronic structure of KFeCoAs2, which is isoelectronic to the parent material of 122 series of iron-based superconductors BaFe2As2. Although band structure calculations predict nearly identical dispersions of the electronic states in both compounds, experiment reveals drastic differences in both the global renormalization and Fermi surfaces. On the basis of the comparison of electronic structures of these two isoelectronic compounds, we demonstrate local magnetic correlations as a vital role for the peculiar low-energy electron dynamics of iron-based superconductors.

  1. Energy-filtered electron-diffracted beam holography

    Energy Technology Data Exchange (ETDEWEB)

    Herring, R.A. [Center for Advanced Materials and Related Technology, Department of Mechanical Engineering, University of Victoria, P.O. Box. 3055, STN CSC, Victoria, BC, V8N 4T6 (Canada)]. E-mail: rherring@uvic.ca

    2005-10-15

    A method of energy-filtered electron holography is described where any two electron-diffracted beams can be interfered using an electron biprism. A Gatan image filter is used to select the energy loss of the electrons produced in the holograms. Gallium arsenide is used as the TEM specimen. This method of microscopy confirms that fringes extending beyond a limiting aperture were due to inelastically scattered electrons and specifically electrons scattered from the bulk plasmon. The degree of coherence of the zero-loss and energy-loss electrons were high and measured to be {approx}0.3, which was maintained even for the high energy-loss electrons up to 100 eV. Future systematic studies using this method should help understand the Stobbs factor and contribute to the development of quantitative high-resolution electron microscopy.

  2. Energy-filtered electron-diffracted beam holography.

    Science.gov (United States)

    Herring, R A

    2005-10-01

    A method of energy-filtered electron holography is described where any two electron-diffracted beams can be interfered using an electron biprism. A Gatan image filter is used to select the energy loss of the electrons produced in the holograms. Gallium arsenide is used as the TEM specimen. This method of microscopy confirms that fringes extending beyond a limiting aperture were due to inelastically scattered electrons and specifically electrons scattered from the bulk plasmon. The degree of coherence of the zero-loss and energy-loss electrons were high and measured to be approximately 0.3, which was maintained even for the high energy-loss electrons up to 100 eV. Future systematic studies using this method should help understand the Stobbs factor and contribute to the development of quantitative high-resolution electron microscopy.

  3. Optimal Electron Energies for Driving Chromospheric Evaporation in Solar Flares

    CERN Document Server

    Reep, Jeffrey; Alexander, David

    2015-01-01

    In the standard model of solar flares, energy deposition by a beam of electrons drives strong chromospheric evaporation leading to a significantly denser corona and much brighter emission across the spectrum. Chromospheric evaporation was examined in great detail by Fisher, Canfield, & McClymont (1985a,b,c), who described a distinction between two different regimes, termed explosive and gentle evaporation. In this work, we examine the importance of electron energy and stopping depths on the two regimes and on the atmospheric response. We find that with explosive evaporation, the atmospheric response does not depend strongly on electron energy. In the case of gentle evaporation, lower energy electrons are significantly more efficient at heating the atmosphere and driving up-flows sooner than higher energy electrons. We also find that the threshold between explosive and gentle evaporation is not fixed at a given beam energy flux, but also depends strongly on the electron energy and duration of heating. Furt...

  4. On electron-proton energy exchange in strong magnetic field

    Science.gov (United States)

    Zelener, B. B.; Zelener, B. V.; Manykin, E. A.; Bronin, S. Y.; Bobrov, A. A.

    2016-11-01

    Heating of protons in cold electron gas in strong magnetic field is studied. Calculations of heating process are preformed using molecular dynamics method. Estimations of heating rate depending on initial proton energies and electron gas temperatures are made.

  5. Ionization By Impact Electrons in Solids: Electron Mean Free Path Fitted Over A Wide Energy Range

    Energy Technology Data Exchange (ETDEWEB)

    Ziaja, B; London, R A; Hajdu, J

    2005-06-09

    We propose a simple formula for fitting the electron mean free paths in solids both at high and at low electron energies. The free-electron-gas approximation used for predicting electron mean free paths is no longer valid at low energies (E < 50 eV), as the band structure effects become significant at those energies. Therefore we include the results of the band structure calculations in our fit. Finally, we apply the fit to 9 elements and 2 compounds.

  6. Manifestation of nonlocal electron-electron interaction in graphene

    Science.gov (United States)

    Ulstrup, Søren; Schüler, Malte; Bianchi, Marco; Fromm, Felix; Raidel, Christian; Seyller, Thomas; Wehling, Tim; Hofmann, Philip

    2016-08-01

    Graphene is an ideal platform to study many-body effects due to its semimetallic character and the possibility to dope it over a wide range. Here we study the width of graphene's occupied π band as a function of doping using angle-resolved photoemission. Upon increasing electron doping, we observe the expected shift of the band to higher binding energies. However, this shift is not rigid and the bottom of the band moves less than the Dirac point. We show that the observed shift cannot be accounted for by single-particle effects and local self-energies alone, but that nonlocal many-body effects, in particular exchange interactions, must be taken into account.

  7. Kramer-Pesch Approximation for Analyzing Field-Angle-Resolved Measurements Made in Unconventional Superconductors: A Calculation of the Zero-Energy Density of States

    Science.gov (United States)

    Nagai, Yuki; Hayashi, Nobuhiko

    2008-08-01

    By measuring the angular-oscillations behavior of the heat capacity with respect to the applied field direction, one can detect the details of the gap structure. We introduce the Kramer-Pesch approximation as a new method to analyze the field-angle-dependent experiments, which improves the previous Doppler-shift technique. We show that the Fermi-surface anisotropy is an indispensable factor for identifying the superconducting gap symmetry.

  8. Energy distribution asymmetry of electron precipitation signatures at Mars

    Science.gov (United States)

    Soobiah, Y. I. J.; Barabash, S.; Nilsson, H.; Stenberg, G.; Lundin, R.; Coates, A. J.; Winningham, J. D.; Frahm, R. A.

    2013-02-01

    The different types of asymmetry observed in the energy distributions of electrons and heavy-ions (M/Q=16-44) during signatures of electron precipitation in the Martian ionosphere have been classified. This has been achieved using the space plasma instrumentation of MEX ASPERA-3 from peri-centre altitude to 2200 km. ASPERA-3 ELS observes signatures of electron precipitation on 43.0% of MEX orbits. Unaccelerated electrons in the form of sudden electron flux enhancements are the most common type of electron precipitation signature at Mars and account for ∼70% of the events observed in this study. Electrons that form unaccelerated electron precipitation signatures are either local ionospheric electrons with enhanced density, or electrons transported from another region of ionosphere, solar wind or tail, or a combination of local and transported electrons. The heating of electrons has a strong influence on the shape of most electron energy spectra from accelerated precipitation signatures. On most occasions the general flow of heavy-ions away from Mars is unchanged during the precipitation of electrons, which is thought to be the result of the finite gyroradius effect of the heavy-ions on crustal magnetic field lines. Only ∼17% of events show some form of heavy-ion acceleration that is either concurrent or at the periphery of an electron precipitation signature. The most common combination of electron and heavy-ion energy distributions for signatures of electron precipitation involves electrons that visually have very little asymmetry or are isotropic and heavy-ions that have a upward net flux, and suggest the upward current associated with aurora. Due to a lack of reliable measurements of electrons travelling towards Mars, it is likely we miss further evidence of upward currents. The second most common combination of electron and heavy-ion energy distributions for signatures of electron precipitation, are those distributions of electrons that are asymmetric and

  9. Electronic structure of NiO: Correlation and band effects

    Energy Technology Data Exchange (ETDEWEB)

    Shen, Z. (Stanford Electronics Laboratory, Stanford University, Stanford, California (USA)); List, R.S. (Los Alamos National Laboratory, Los Alamos, New Mexico (USA)); Dessau, D.S.; Wells, B.O. (Stanford Electronics Laboratory, Stanford University, Stanford, California (USA)); Jepsen, O. (Max-Planck-Institute for Solid State Research, D-7000 Stuttgart 80 (Federal Republic of Germany)); Arko, A.J.; Barttlet, R. (Los Alamos National Laboratory, Los Alamos, New Mexico (USA)); Shih, C.K. (Department of Physics, University of Texas, Austin, Texas (USA)); Parmigiani, F. (IBM Research Division, Almaden Research Center, 650 Harry Road, San Jose, California (USA)); Huang, J.C.; Lindberg, P.A.P. (Stanford Electronics Laboratory, Stanford University, Stanford, California (USA))

    1991-08-15

    We have performed angle-resolved-photoemission experiments and local-density-functional (LDA) band calculations on NiO to study correlation and band effects of this conceptually important compound. Our experimental result suggests a dual nature of the electronic structure of NiO. On the one hand, the LDA band calculation has some relevance to the electronic structure of NiO, and the inclusion of the antiferromagnetic order is essential. For the lower O 2{ital p} bands, the LDA calculation agrees almost perfectly with experimental energy positions and dispersion relations. On the other hand, discrepancies between the experiment and the LDA calculation do exist, especially for the Ni 3{ital d} bands and the O 2{ital p} bands that are heavily mixed with the Ni 3{ital d} bands. It appears that the main discrepancies between the experimental results and the LDA calculation are concentrated in the regions of the insulating gap and the valence-band satellite. In addition to these results, we also report the interesting angle and photon-energy dependence of the satellite emission. The above results show that the angle-resolved-photoemission studies can provide much additional information about the electronic structure of correlated materials like NiO.

  10. Sterilization of foods with low-energy electrons (``soft-electrons'')

    Science.gov (United States)

    Hayashi, Toru; Takahashi, Yoko; Todoriki, Setsuko

    1998-06-01

    Electrons with an energy of 300 keV or lower were defined as "Soft-electrons", which showed several advantages over conventional irradiation with gamma-rays or high-energy electrons in decontamination of grains and spices. Energies of electrons necessary to reduce microbial loads to levels lower than 10 CFU/g were 60 keV for brown rice, 75 keV for wheat, 100 keV for white pepper, coriander and basil, 130 keV for buckwheat, 160 keV for rough rice, and 210 keV for black pepper. Electrons with such energies did not significantly influence the quality.

  11. Sterilization of foods with low-energy electrons ('soft-electrons')

    Energy Technology Data Exchange (ETDEWEB)

    Hayashi, Toru; Takahashi, Yoko; Todoriki, Setsuko

    1998-06-01

    Electrons with an energy of 300 keV or lower were defined as 'Soft-electrons', which showed several advantages over conventional irradiation with gamma-rays or high-energy electrons in decontamination of grains and spices. Energies of electrons necessary to reduce microbial loads to levels lower than 10 CFU/g were 60 keV for brown rice, 75 keV for wheat, 100 keV for white pepper, coriander and basil, 130 keV for buckwheat, 160 keV for rough rice, and 210 keV for black pepper. Electrons with such energies did not significantly influence the quality.

  12. Power electronic converter systems for direct drive renewable energy applications

    DEFF Research Database (Denmark)

    Chen, Zhe

    2013-01-01

    This chapter presents power electronic conversion systems for wind and marine energy generation applications, in particular, direct drive generator energy conversion systems. Various topologies are presented and system design optimization and reliability are briefly discussed....

  13. Low-energy electron beams through ultra-thin foils, applications for electron microscopy

    NARCIS (Netherlands)

    Van Aken, R.H.

    2005-01-01

    This thesis has discussed two electron microscopy applications that make use of ultra-thin foils: the tunnel junction emitter and the low-energy foil corrector. Both applications have in common that the electron beam is sent through the thin foil at low energy. Part of the electrons will scatter in

  14. Is the electron radiation length constant at high energies?

    Science.gov (United States)

    Hansen, H D; Uggerhøj, U I; Biino, C; Ballestrero, S; Mangiarotti, A; Sona, P; Ketel, T J; Vilakazi, Z Z

    2003-07-04

    Experimental results for the radiative energy loss of 149, 207, and 287 GeV electrons in a thin Ir target are presented. From the data we conclude that at high energies the radiation length increases in accordance with the Landau-Pomeranchuk-Migdal (LPM) theory and thus electrons become more penetrating the higher the energy. The increase of the radiation length as a result of the LPM effect has a significant impact on the behavior of high-energy electromagnetic showers.

  15. ELEC-2005: Electronics in High Energy Physics

    CERN Multimedia

    Monique Duval

    2004-01-01

    ELEC-2005 is a new course series on modern electronics, given by CERN physicists and engineers in the format of the successful ELEC-2002 course series, and within the framework of the 2005 Technical Training Programme. This comprehensive course series is designed for people who are not electronics specialists, for example physicists, engineers and technicians working at or visiting the laboratory, who use or will use electronics in their present or future activities, in particular in the context of the LHC accelerator and experiments. ELEC-2005 will composed of four Terms throughout the year: Winter Term: Introduction to electronics in HEP (January-February, 6 lectures) Spring Term: Integrated circuits and VLSI technology for physics (March, 6 lectures) Summer Term: System electronics for physics: Issues (May, 7 lectures) Winter Term: Electronics applications in HEP experiments (November-December, 10 lectures) Lectures within each Term will take place on Tuesdays and Thursdays, from 10:00 to 12:30. The...

  16. Electrospun Fibers for Energy, Electronic, & Environmental Applications

    Science.gov (United States)

    Bedford, Nicholas M.

    Electrospinning is an established method for creating polymer and bio-polymer fibers of dimensions ranging from ˜10 nanometers to microns. The process typically involves applying a high voltage between a solution source (usually at the end of a capillary or syringe) and a substrate on which the nanofibers are deposited. The high electric field distorts the shape of the liquid droplet, creating a Taylor cone. Additional applied voltage ejects a liquid jet of the polymer solution in the Taylor cone toward the counter electrode. The formation of fibers is generated by the rapid electrostatic elongation and solvent evaporation of this viscoelastic jet, which typically generates an entangled non-woven mesh of fibers with a high surface area to volume ratio. Electrospinning is an attractive alternative to other processes for creating nano-scale fibers and high surface area to volume ratio surfaces due to its low start up cost, overall simplicity, wide range of processable materials, and the ability to generate a moderate amount of fibers in one step. It has also been demonstrated that coaxial electrospinning is possible, wherein the nanofiber has two distinct phases, one being the core and another being the sheath. This method is advantageous because properties of two materials can be combined into one fiber, while maintaining two distinct material phases. Materials that are inherently electrospinable could be made into fibers using this technique as well. The most common applications areas for electrospun fibers are in filtration and biomedical areas, with a comparatively small amount of work done in energy, environmental, and sensor applications. Furthermore, the use of biologically materials in electrospun fibers is an avenue of research that needs more exploration, given the unique properties these materials can exhibit. The research aim of this thesis is to explore the use of electrospun fibers for energy, electrical and environmental applications. For energy

  17. Influence of binding energies of electrons on nuclear mass predictions

    Science.gov (United States)

    Tang, Jing; Niu, Zhong-Ming; Guo, Jian-You

    2016-07-01

    Nuclear mass contains a wealth of nuclear structure information, and has been widely employed to extract the nuclear effective interactions. The known nuclear mass is usually extracted from the experimental atomic mass by subtracting the masses of electrons and adding the binding energy of electrons in the atom. However, the binding energies of electrons are sometimes neglected in extracting the known nuclear masses. The influence of binding energies of electrons on nuclear mass predictions are carefully investigated in this work. If the binding energies of electrons are directly subtracted from the theoretical mass predictions, the rms deviations of nuclear mass predictions with respect to the known data are increased by about 200 keV for nuclei with Z, N ⩾ 8. Furthermore, by using the Coulomb energies between protons to absorb the binding energies of electrons, their influence on the rms deviations is significantly reduced to only about 10 keV for nuclei with Z, N ⩾ 8. However, the binding energies of electrons are still important for the heavy nuclei, about 150 keV for nuclei around Z = 100 and up to about 500 keV for nuclei around Z = 120. Therefore, it is necessary to consider the binding energies of electrons to reliably predict the masses of heavy nuclei at an accuracy of hundreds of keV. Supported by National Natural Science Foundation of China (11205004)

  18. An extension of the Eisberg-Resnick treatment for electron energies in many-electron atoms

    Science.gov (United States)

    Whitaker, M. A. B.; Bennett, I.

    1989-03-01

    Eisberg and Resnick present a simple argument for the energy of an electron in a multielectron atom using the concept of shielding from electrons in inner shells. The results of such a treatment are unfortunately confined so as to be out of range of experimental values. Here, the effect of electrons in outer shells is included, and, in the nonrelativistic region, energies are obtained for electrons in the first and second shells in reasonable agreement with experiment.

  19. Effects, determination, and correction of count rate nonlinearity in multi-channel analog electron detectors

    Energy Technology Data Exchange (ETDEWEB)

    Reber, T. J.; Plumb, N. C.; Waugh, J. A.; Dessau, D. S. [Department of Physics, University of Colorado, Boulder, Colorado 80309-0390 (United States)

    2014-04-15

    Detector counting rate nonlinearity, though a known problem, is commonly ignored in the analysis of angle resolved photoemission spectroscopy where modern multichannel electron detection schemes using analog intensity scales are used. We focus on a nearly ubiquitous “inverse saturation” nonlinearity that makes the spectra falsely sharp and beautiful. These artificially enhanced spectra limit accurate quantitative analysis of the data, leading to mistaken spectral weights, Fermi energies, and peak widths. We present a method to rapidly detect and correct for this nonlinearity. This algorithm could be applicable for a wide range of nonlinear systems, beyond photoemission spectroscopy.

  20. The source of multi spectral energy of solar energetic electron

    Energy Technology Data Exchange (ETDEWEB)

    Herdiwijaya, Dhani [Astronomy Division and Bosscha Observatory, Faculty Mathematics and Natural Sciences, Intitute Technology of Bandung, Ganesha 10, Bandung, Indonesia 40132 dhani@as.itb.ac.id (Indonesia)

    2015-04-16

    We study the solar energetic electron distribution obtained from ACE and GOES satellites which have different altitudes and electron spectral energy during the year 1997 to 2011. The electron spectral energies were 0.038–0.315 MeV from EPAM instrument onboard ACE satellite and >2 MeV from GOES satellite. We found that the low electron energy has no correlation with high energy. In spite of we have corrected to the altitude differences. It implied that they originated from time dependent events with different sources and physical processes at the solar atmosphere. The sources of multi spectral energetic electron were related to flare and CME phenomena. However, we also found that high energetic electron comes from coronal hole.

  1. Spectral shape variation of interstellar electrons at high energies

    Science.gov (United States)

    Tan, L. C.

    1985-01-01

    The high energy electron spectrum analysis has shown that the electron intensity inside the H2 cloud region, or in a spiral arm, should be much lower than that outside it and the observed electron energy spectrum should flatten again at about 1 TeV. In the framework of the leady box model the recently established rigidity dependence of the escape pathlength of cosmic rays would predict a high energy electron spectrum which is flatter than the observed one. This divergence is explained by assuming that the leaky box model can only apply to cosmic ray heavy nuclei, and light nuclei and electrons in cosmic rays may have different behaviors in the interstellar propagation. Therefore, the measured data on high energy electrons should be analyzed based on the proposed nonuniform galactic disk (NUGD) mode.

  2. Clinical implementation of electron energy changes of varian linear accelerators.

    Science.gov (United States)

    Zhang, Sean; Liengsawangwong, Praimakorn; Lindsay, Patricia; Prado, Karl; Sun, Tzouh-Liang; Steadham, Roy; Wang, Xiaochun; Salehpour, Mohammad; Gillin, Michael

    2009-10-27

    Modern dual photon energy linear accelerators often come with a few megavoltage electron beams. The megavoltage electron beam has limited range and relative sharp distal falloff in its depth dose curve compared to that of megavoltage photon beam. Its radiation dose is often delivered appositionally to cover the target volume to its distal 90% depth dose (d90), while avoiding the normal--sometimes critical--structure immediately distal to the target. Varian linear accelerators currently offer selected electron beams of 4, 6, 9, 12, 16 and 20 MeV electron beam energies. However, intermediate electron energy is often needed for optimal dose distribution. In this study we investigated electron beam characteristics and implemented two intermediate 7 and 11 MeV electron beams on Varian linear accelerators. Comprehensive tests and measurements indicated the new electron beams met all dosimetry parameter criteria and operational safety standards. Between the two new electron beams and the existing electron beams we were able to provide a choice of electron beams of 4, 6, 7, 9, 11, 12, 16 and 20 MeV electron energies, which had d90 depth between 1.5 cm and 6.0 cm (from 1.5 cm to 4.0 cm in 0.5 cm increments) to meet our clinical needs.

  3. Low energy electron microscopy imaging using Medipix2 detector

    NARCIS (Netherlands)

    Sikharulidze, I.; Gastel, van R.; Schramm, S.; Abrahams, J.P.; Poelsema, B.; Tromp, R.M.; Molen, van der S.J.

    2011-01-01

    Low Energy Electron Microscopy (LEEM) and Photo-Emission Electron Microscopy (PEEM) predominantly use a combination of microchannel plate (MCP), phosphor screen and optical camera to record images formed by 10–20 keV electrons. We have tested the performance of a LEEM/PEEM instrument with a Medipix2

  4. Electron-helium and electron-neon scattering cross sections at low electron energies using a photoelectron source

    Science.gov (United States)

    Kumar, Vijay; Subramanian, K. P.; Krishnakumar, E.

    1987-01-01

    Absolute electron-helium and electron-neon scattering cross sections have been measured at low electron energies using the powerful technique of photoelectron spectroscopy. The measurements have been carried out at 17 electron energies varying from 0.7 to 10 eV with an accuracy of + or - 2.7 percent. The results obtained in the present work have been compared with other recent measurement and calculations.

  5. Simple simulation for electron energy levels in geometrical potential wells

    CERN Document Server

    Pengpan, Teparksorn

    2008-01-01

    An octopus program is demonstrated to generate electron energy levels in three-dimensional geometrical potential wells. The wells are modeled to have shapes similar to cone, pyramid and truncated-pyramid. To simulate the electron energy levels in quantum mechanical scheme like the ones in parabolic band approximation scheme, the program is run initially to find a suitable electron mass fraction that can produce ground-state energies in the wells as close to those in quantum dots as possible and further to simulate excited-state energies. The programs also produce wavefunctions for exploring and determining their degeneracies and vibrational normal modes.

  6. Power electronics - The key technology for Renewable Energy Systems

    DEFF Research Database (Denmark)

    Blaabjerg, Frede; Ma, Ke; Yang, Yongheng

    2014-01-01

    and effectively, energy conversion systems, currently based on power electronics technology, will again play an essential role in this energy paradigm shift. Using highly efficient power electronics in power generation, power transmission/distribution and end-user application, together with advanced control...... solutions, can pave the way for renewable energies. In light of this, some of the most emerging renewable energies, e.g. wind energy and photovoltaic, which by means of power electronics are changing character as a major part in the electricity generation, are explored in this paper. Issues like technology...... development, implementation, power converter technologies, control of the systems, and synchronization are addressed. Special focuses are paid on the future trends in power electronics for those systems like how to lower the cost of energy and to develop emerging power devices and better reliability tool....

  7. Electronically droplet energy harvesting using piezoelectric cantilevers

    KAUST Repository

    Al Ahmad, Mahmoud Al

    2012-01-01

    A report is presented on free falling droplet energy harvesting using piezoelectric cantilevers. The harvester incorporates a multimorph clamped-free cantilever which is composed of five layers of lead zirconate titanate piezoelectric thick films. During the impact, the droplet kinetic energy is transferred into the form of mechanical stress forcing the piezoelectric structure to vibrate. Experimental results show energy of 0.3 μJ per droplet. The scenario of moderate falling drop intensity, i.e. 230 drops per second, yields a total energy of 400 μJ. © 2012 The Institution of Engineering and Technology.

  8. Detecting electron beam energy shifts with a commercially available energy monitor.

    Science.gov (United States)

    Evans, M D; Moftah, B A; Olivares, M; Podgorsak, E B

    2000-07-01

    Routine electron beam quality assurance requires an accurate, yet practical, method of energy characterization. Subtle shifts in beam energy may be produced by the linac bending magnet assembly, and the sensitivity of a commercially available electron beam energy-monitoring device for monitoring these small energy drifts has been evaluated. The device shows an 11% change in signal for a 2 mm change in the I50 energy parameter for low energy electron beams (in the vicinity of 6 MeV) and a 2.5% change in signal for a 2 mm change in the I50 energy parameter for high energy electron beams (in the vicinity of 22 MeV). Thus the device is capable of detecting small energy shifts resulting from bending magnet drift for all clinically relevant electron beams.

  9. Energy-filtered Electron Transport Structures for Low-power Low-noise 2-D Electronics.

    Science.gov (United States)

    Pan, Xuan; Qiu, Wanzhi; Skafidas, Efstratios

    2016-10-31

    In addition to cryogenic techniques, energy filtering has the potential to achieve high-performance low-noise 2-D electronic systems. Assemblies based on graphene quantum dots (GQDs) have been demonstrated to exhibit interesting transport properties, including resonant tunnelling. In this paper, we investigate GQDs based structures with the goal of producing energy filters for next generation lower-power lower-noise 2-D electronic systems. We evaluate the electron transport properties of the proposed GQD device structures to demonstrate electron energy filtering and the ability to control the position and magnitude of the energy passband by appropriate device dimensioning. We also show that the signal-to-thermal noise ratio performance of the proposed nanoscale device can be modified according to device geometry. The tunability of two-dimensional GQD structures indicates a promising route for the design of electron energy filters to produce low-power and low-noise electronics.

  10. The electron energy loss rate due to radiative recombination

    Science.gov (United States)

    Mao, Junjie; Kaastra, Jelle; Badnell, N. R.

    2017-02-01

    Context. For photoionized plasmas, electron energy loss rates due to radiative recombination (RR) are required for thermal equilibrium calculations, which assume a local balance between the energy gain and loss. While many calculations of total and/or partial RR rates are available from the literature, specific calculations of associated RR electron energy loss rates are lacking. Aims: Here we focus on electron energy loss rates due to radiative recombination of H-like to Ne-like ions for all the elements up to and including zinc (Z = 30), over a wide temperature range. Methods: We used the AUTOSTRUCTURE code to calculate the level-resolved photoionization cross section and modify the ADASRR code so that we can simultaneously obtain level-resolved RR rate coefficients and associated RR electron energy loss rate coefficients. We compared the total RR rates and electron energy loss rates of H i and He i with those found in the literature. Furthermore, we utilized and parameterized the weighted electron energy loss factors (dimensionless) to characterize total electron energy loss rates due to RR. Results: The RR electron energy loss data are archived according to the Atomic Data and Analysis Structure (ADAS) data class adf48. The RR electron energy loss data are also incorporated into the SPEX code for detailed modeling of photoionized plamsas. Full Tables 1 and 2 are available at the CDS via anonymous ftp to http://cdsarc.u-strasbg.fr (http://130.79.128.5) or via http://cdsarc.u-strasbg.fr/viz-bin/qcat?J/A+A/599/A10

  11. Power Electronics and Control of Renewable Energy Systems

    DEFF Research Database (Denmark)

    Iov, Florin; Ciobotaru, Mihai; Sera, Dezso

    2007-01-01

    sources from the conventional, fossil (and short term) based energy sources to renewable energy resources. Another is to use high efficient power electronics in power generation, power transmission/distribution and end-user application. This paper discuss some of the most emerging renewable energy sources......, wind energy and photovoltaics, which by means of power electronics are changing from being minor energy sources to be acting as important power sources in the energy system.......The global electrical energy consumption is still rising and there is a demand to double the power capacity within 20 years. The production, distribution and use of energy should be as technological efficient as possible and incentives to save energy at the end-user should also be set up...

  12. Plasma expansion into vacuum assuming a steplike electron energy distribution.

    Science.gov (United States)

    Kiefer, Thomas; Schlegel, Theodor; Kaluza, Malte C

    2013-04-01

    The expansion of a semi-infinite plasma slab into vacuum is analyzed with a hydrodynamic model implying a steplike electron energy distribution function. Analytic expressions for the maximum ion energy and the related ion distribution function are derived and compared with one-dimensional numerical simulations. The choice of the specific non-Maxwellian initial electron energy distribution automatically ensures the conservation of the total energy of the system. The estimated ion energies may differ by an order of magnitude from the values obtained with an adiabatic expansion model supposing a Maxwellian electron distribution. Furthermore, good agreement with data from experiments using laser pulses of ultrashort durations τ(L)Maxwellian electron distribution is assumed.

  13. Energy Spread Reduction of Electron Beams Produced via Laser Wake

    Energy Technology Data Exchange (ETDEWEB)

    Pollock, Bradley Bolt [Univ. of California, San Diego, CA (United States)

    2012-01-01

    Laser wakefield acceleration of electrons holds great promise for producing ultra-compact stages of GeV scale, high quality electron beams for applications such as x-ray free electron lasers and high energy colliders. Ultra-high intensity laser pulses can be self-guided by relativistic plasma waves over tens of vacuum diffraction lengths, to give >1 GeV energy in cm-scale low density plasma using ionization-induced injection to inject charge into the wake at low densities. This thesis describes a series of experiments which investigates the physics of LWFA in the self-guided blowout regime. Beginning with high density gas jet experiments the scaling of the LWFA-produced electron beam energy with plasma electron density is found to be in excellent agreement with both phenomenological theory and with 3-D PIC simulations. It is also determined that self-trapping of background electrons into the wake exhibits a threshold as a function of the electron density, and at the densities required to produce electron beams with energies exceeding 1 GeV a different mechanism is required to trap charge into low density wakes. By introducing small concentrations of high-Z gas to the nominal He background the ionization-induced injection mechanism is enabled. Electron trapping is observed at densities as low as 1.3 x 1018 cm-3 in a gas cell target, and 1.45 GeV electrons are demonstrated for the first time from LWFA. This is currently the highest electron energy ever produced from LWFA. The ionization-induced trapping mechanism is also shown to generate quasi-continuous electron beam energies, which is undesirable for accelerator applications. By limiting the region over which ionization-induced trapping occurs, the energy spread of the electron beams can be controlled. The development of a novel two-stage gas cell target provides the capability to tailor the gas composition in the longitudinal direction, and confine the trapping process to occur only in a

  14. Microbunched electron cooling for high-energy hadron beams.

    Science.gov (United States)

    Ratner, D

    2013-08-23

    Electron and stochastic cooling are proven methods for cooling low-energy hadron beams, but at present there is no way of cooling hadrons as they near the TeV scale. In the 1980s, Derbenev suggested that electron instabilities, such as free-electron lasers, could create collective space charge fields strong enough to correct the hadron energies. This Letter presents a variation on Derbenev's electron cooling scheme using the microbunching instability as the amplifier. The large bandwidth of the instability allows for faster cooling of high-density beams. A simple analytical model illustrates the cooling mechanism, and simulations show cooling rates for realistic parameters of the Large Hadron Collider.

  15. High-Current Energy-Recovering Electron Linacs

    Energy Technology Data Exchange (ETDEWEB)

    Nikolitsa Merminga; David Douglas; Geoffrey Krafft

    2003-12-01

    The use of energy recovery provides a potentially powerful new paradigm for generation of the charged particle beams used in synchrotron radiation sources, high-energy electron cooling devices, electron-ion colliders, and other applications in photon science and nuclear and high-energy physics. Energy-recovering electron linear accelerators (called energy-recovering linacs, or ERLs) share many characteristics with ordinary linacs, as their six-dimensional beam phase space is largely determined by electron source properties. However, in common with classic storage rings, ERLs possess a high average-current-carrying capability enabled by the energy recovery process, and thus promise similar efficiencies. The authors discuss the concept of energy recovery and its technical challenges and describe the Jefferson Lab (JLab) Infrared Demonstration Free-Electron Laser (IR Demo FEL), originally driven by a 3548-MeV, 5-mA superconducting radiofrequency (srf) ERL, which provided the most substantial demonstration of energy recovery to date: a beam of 250 kW average power. They present an overview of envisioned ERL applications and a development path to achieving the required performance. They use experimental data obtained at the JLab IR Demo FEL and recent experimental results from CEBAF-ERL GeV-scale, comparatively low-current energy-recovery demonstration at JLab to evaluate the feasibility of the new applications of high-current ERLs, as well as ERLs' limitations and ultimate performance.

  16. HIGH-ENERGY ELECTRON COOLING BASED ON REALISTIC SIX-DIMENSIONAL DISTRIBUTION OF ELECTRONS

    Energy Technology Data Exchange (ETDEWEB)

    FEDOTOV,A.; BEN-ZVI, I.; ET AL.

    2007-06-25

    The high-energy electron cooling system for RHIC-II is unique compared to standard coolers. It requires bunched electron beam. Electron bunches are produced by an Energy Recovery Linac (ERL), and cooling is planned without longitudinal magnetic field. To address unique features of the RHIC cooler, a generalized treatment of cooling force was introduced in BETACOOE code which allows us to calculate friction force for an arbitrary distribution of electrons. Simulations for RHIC cooler based on electron distribution from ERL are presented.

  17. Theoretical Study of Lithium Ionic Conductors by Electronic Stress Tensor Density and Electronic Kinetic Energy Density

    CERN Document Server

    Nozaki, Hiroo; Ichikawa, Kazuhide; Watanabe, Taku; Aihara, Yuichi; Tachibana, Akitomo

    2016-01-01

    We analyze the electronic structure of lithium ionic conductors, ${\\rm Li_3PO_4}$ and ${\\rm Li_3PS_4}$, using the electronic stress tensor density and kinetic energy density with special focus on the ionic bonds among them. We find that, as long as we examine the pattern of the eigenvalues of the electronic stress tensor density, we cannot distinguish between the ionic bonds and bonds among metalloid atoms. We then show that they can be distinguished by looking at the morphology of the electronic interface, the zero surface of the electronic kinetic energy density.

  18. Electron tunneling in single layer graphene with an energy gap

    Institute of Scientific and Technical Information of China (English)

    Xu Xu-Guang; Zhang Chao; Xu Gong-Jie; Cao Jun-Cheng

    2011-01-01

    When a single layer graphene is epitaxially grown on silicon carbide, it will exhibit a finite energy gap like a conventional semiconductor, and its energy dispersion is no longer linear in momentum in the low energy regime. In this paper, we have investigated the tunneling characteristics through a two-dimensional barrier in a single layer graphene with an energy gap. It is found that when the electron is at a zero angle of incidence, the transmission probability as a function of incidence energy has a gap. Away from the gap the transmission coefficient oscillates with incidence energy which is analogous to that of a conventional semiconductor. The conductance under zero temperature has a gap. The properties of electron transmission may be useful for developing graphene-based nano-electronics.

  19. Modified Fermi energy of electrons in a superhigh magnetic field

    Science.gov (United States)

    Zhu, Cui; Gao, Zhi Fu; Li, Xiang Dong; Wang, Na; Yuan, Jian Ping; Peng, Qiu He

    2016-04-01

    In this paper, we investigate the electron Landau level stability and its influence on the electron Fermi energy, EF(e), in the circumstance of magnetars, which are powered by magnetic field energy. In a magnetar, the Landau levels of degenerate and relativistic electrons are strongly quantized. A new quantity gn, the electron Landau level stability coefficient is introduced. According to the requirement that gn decreases with increasing the magnetic field intensity B, the magnetic field index β in the expression of EF(e) must be positive. By introducing the Dirac-δ function, we deduce a general formulae for the Fermi energy of degenerate and relativistic electrons, and obtain a particular solution to EF(e) in a superhigh magnetic field (SMF). This solution has a low magnetic field index of β = 1/6, compared with the previous one, and works when ρ ≥ 107g cm-3 and Bcr ≪ B ≤ 1017 Gauss. By modifying the phase space of relativistic electrons, a SMF can enhance the electron number density ne, and decrease the maximum of electron Landau level number, which results in a redistribution of electrons. According to Pauli exclusion principle, the degenerate electrons will fill quantum states from the lowest Landau level to the highest Landau level. As B increases, more and more electrons will occupy higher Landau levels, though gn decreases with the Landau level number n. The enhanced ne in a SMF means an increase in the electron Fermi energy and an increase in the electron degeneracy pressure. The results are expected to facilitate the study of the weak-interaction processes inside neutron stars and the magnetic-thermal evolution mechanism for magnetars.

  20. Polarization of high-energy electrons traversing a laser beam

    CERN Document Server

    Kotkin, G L; Serbo, V G

    1998-01-01

    When polarized electrons traverse a region where the laser light is focused their polarization varies even if their energy and direction of motion are not changed. This effect is due to interference of the incoming electron wave and an electron wave scattered at zero angle. Equations are obtained which determine the variation of the electron density matrix, and their solutions are given. The change in the electron polarization depends not only on the Compton cross section but on the real part of the forward Compton amplitude as well. It should be taken into account, for example, in simulations of the $e \\to \\gamma$ conversion for future $\\gamma \\gamma$ colliders.

  1. Electron, photons, and molecules: Storing energy from light

    Energy Technology Data Exchange (ETDEWEB)

    Miller, J.R. [Argonne National Laboratory, IL (United States)

    1996-09-01

    Molecular charge separation has important potential for photochemical energy storage. Its efficiency can be enhanced by principals which maximize the rates of the electron transfer steps which separate charge and minimize those which recombine high-energy charge pairs to lose stored energy. Dramatic scientific progress in understanding these principals has occurred since the founding of DOE and its predecessor agency ERDA. While additional knowledge in needed in broad areas of molecular electron transfer, some key areas of knowledge hold particular promise for the possibility of moving this area from science toward technology capable of contributing to the nation`s energy economy.

  2. Simulations and measurements in scanning electron microscopes at low electron energy.

    Science.gov (United States)

    Walker, Christopher G H; Frank, Luděk; Müllerová, Ilona

    2016-11-01

    The advent of new imaging technologies in Scanning Electron Microscopy (SEM) using low energy (0-2 keV) electrons has brought about new ways to study materials at the nanoscale. It also brings new challenges in terms of understanding electron transport at these energies. In addition, reduction in energy has brought new contrast mechanisms producing images that are sometimes difficult to interpret. This is increasing the push for simulation tools, in particular for low impact energies of electrons. The use of Monte Carlo calculations to simulate the transport of electrons in materials has been undertaken by many authors for several decades. However, inaccuracies associated with the Monte Carlo technique start to grow as the energy is reduced. This is not simply associated with inaccuracies in the knowledge of the scattering cross-sections, but is fundamental to the Monte Carlo technique itself. This is because effects due to the wave nature of the electron and the energy band structure of the target above the vacuum energy level become important and these are properties which are difficult to handle using the Monte Carlo method. In this review we briefly describe the new techniques of scanning low energy electron microscopy and then outline the problems and challenges of trying to understand and quantify the signals that are obtained. The effects of charging and spin polarised measurement are also briefly explored. SCANNING 38:802-818, 2016. © 2016 Wiley Periodicals, Inc.

  3. In Situ Electron Energy Loss Spectroscopy in Liquids

    CERN Document Server

    Holtz, Megan E; Gao, Jie; Abruña, Héctor D; Muller, David A

    2012-01-01

    In situ scanning transmission electron microscopy (STEM) through liquids is a promising approach for exploring biological and materials processes. However, options for in situ chemical identification are limited: X-ray analysis is precluded because the holder shadows the detector, and electron energy loss spectroscopy (EELS) is degraded by multiple scattering events in thick layers. Here, we explore the limits of EELS for studying chemical reactions in their native environments in real time and on the nanometer scale. The determination of the local electron density, optical gap and thickness of the liquid layer by valence EELS is demonstrated for liquids. By comparing theoretical and experimental plasmon energies, we find that liquids appear to follow the free-electron model that has been previously established for solids. Signals at energies below the optical gap and plasmon energy of the liquid provide a high signal-to-background ratio as demonstrated for LiFePO4 in aqueous solution. The potential for using...

  4. Electron energy spectrum in core-shell elliptic quantum wire

    Directory of Open Access Journals (Sweden)

    V.Holovatsky

    2007-01-01

    Full Text Available The electron energy spectrum in core-shell elliptic quantum wire and elliptic semiconductor nanotubes are investigated within the effective mass approximation. The solution of Schrodinger equation based on the Mathieu functions is obtained in elliptic coordinates. The dependencies of the electron size quantization spectrum on the size and shape of the core-shell nanowire and nanotube are calculated. It is shown that the ellipticity of a quantum wire leads to break of degeneration of quasiparticle energy spectrum. The dependences of the energy of odd and even electron states on the ratio between semiaxes are of a nonmonotonous character. The anticrosing effects are observed at the dependencies of electron energy spectrum on the transversal size of the core-shell nanowire.

  5. Treatment of foods with 'soft-electrons' (low-energy electrons)

    Energy Technology Data Exchange (ETDEWEB)

    Hayashi, Toru [Japan International Research Center for Agricultural Sciences (JIRCAS), Tsukuba, Ibaraki (Japan); Todoriki, Setsuko [National Food Research Institute (NFRI), Tsukuba, Ibaraki (Japan)

    2003-02-01

    Electrons with energies of 300 keV or lower were defined as soft-electrons'. Soft-electrons can eradicate microorganisms residing on the surface of grains, pulses, spices, dehydrated vegetables, tea leaves and seeds, and reduce their microbial loads to levels lower than 10 CFU/g with little quality deterioration. Soft-electrons can inactivate insect pests infesting grains and pulses and inhibit sprouting of potatoes. (author)

  6. Radial Distribution of Electron Spectra from High-Energy Ions

    Science.gov (United States)

    Cucinotta, Francis A.; Katz, Robert; Wilson, John W.

    1998-01-01

    The average track model describes the response of physical and biological systems using radial dose distribution as the key physical descriptor. We report on an extension of this model to describe the average distribution of electron spectra as a function of radial distance from an ion. We present calculations of these spectra for ions of identical linear energy transfer (LET), but dissimilar charge and velocity to evaluate the differences in electron spectra from these ions. To illustrate the usefulness of the radial electron spectra for describing effects that are not described by electron dose, we consider the evaluation of the indirect events in microdosimetric distributions for ions. We show that folding our average electron spectra model with experimentally determined frequency distributions for photons or electrons provides a good representation of radial event spectra from high-energy ions in 0.5-2 micrometer sites.

  7. International Conference on Power Electronics and Renewable Energy Systems

    CERN Document Server

    Suresh, L; Dash, Subhransu; Panigrahi, Bijaya

    2015-01-01

    The book is a collection of high-quality peer-reviewed research papers presented in Proceedings of International Conference on Power Electronics and Renewable Energy Systems (ICPERES 2014) held at Rajalakshmi Engineering College, Chennai, India. These research papers provide the latest developments in the broad area of Power Electronics and Renewable Energy. The book discusses wide variety of industrial, engineering and scientific applications of the emerging techniques. It presents invited papers from the inventors/originators of new applications and advanced technologies.

  8. A digital energy control system for the LEAR electron cooler

    CERN Document Server

    Caspers, Fritz; Molinari, G; Ramos, U

    1993-01-01

    A feedback control system has been developed to correct any energy errors that may occur when operating the electron cooler on LEAR. Drifts and, above all, the space charge effects are the main sources of error. Error cancellation must be compatible with the pulsed mode of operation of the electron cooler so that the beam must be stabilized at the right energy before the end of the corresponding flat top is reached.

  9. Evaluation of Miscellaneous and Electronic Device Energy Use in Hospitals

    Energy Technology Data Exchange (ETDEWEB)

    Black, Douglas R.; Lanzisera, Steven M.; Lai, Judy; Brown, Richard E.; Singer, Brett C.

    2012-09-01

    Miscellaneous and electronic loads (MELs) consume about one-thirdof the primary energy used in US buildings, and their energy use is increasing faster than other end-uses. In healthcare facilities, 30percent of the annual electricity was used by MELs in 2008. This paper presents methods and challenges for estimating medical MELs energy consumption along with estimates of energy use in a hospital by combining device-level metered data with inventories and usage information. An important finding is that common, small devices consume large amounts of energy in aggregate and should not be ignored when trying to address hospital energy use.

  10. High energy electron-positron physics

    CERN Document Server

    Ali, Ahmed

    1988-01-01

    With the termination of the physics program at PETRA, and with the start of TRISTAN and the SLC and later LEP, an era of e+e- physics has come to an end and a new one begins. The field is changing from a field of few specialists, to becoming one of the mainstream efforts of the high energy community. It seems appropriate at this moment to summarize what has been learned over the past years, in a way most useful to any high energy physicists, in particular to newcomers in the e+e- field. This is the purpose of the book. This book should be used as a reference for future workers in the field of

  11. Catalogue of Radionuclide Low-Energy Electron Spectra (LEES)

    CERN Document Server

    Vylov, T D; Kovalik, A; Yakushev, E A; Mahmoud, M; Novgorodov, A F; Lebedev, N A; Filossofov, D V; Briançon, C; Walen, R J; Coursol, N F; Minkova, A; Petev, P; Dragoun, O; Brabec, V; Inoyatov, A

    2003-01-01

    More than 100 of apparatus low-energy electron spectra from radionuclides with Z=24-95 are collected in the presented LEES Catalogue. These spectra have been recorded in systematical investigations of Auger and internal conversion electrons with the ESA-50 electrostatic spectrometer during past 20 years.

  12. Utilization of low-energy electron accelerators in Korea

    Energy Technology Data Exchange (ETDEWEB)

    Lee, Byung Cheol [Korea Atomic Energy Research Institute, Taejon (Korea, Republic of)

    2003-02-01

    There are more than 20 electron accelerators in Korea. Most of those are installed in factories for heat-resistant cables, heat-shrinkable cables, radial tires, foams, tube/ films, curing, etc. Four low-energy electron accelerators are in operation for research purposes such as polymer modification, purification of flue gas, waste water treatment, modification of semiconductor characteristics, etc. (author)

  13. Characteristic energy losses of electrons in organic NTCDA-films

    CERN Document Server

    Komolov, S A; Sidorenko, A G; Alyaev, Y G; Novolodskij, V A

    2001-01-01

    The studies on the characteristic energy losses of slow electrons in the NTCDA thin film on the ZnO (0001) surface are presented. It is shown, that the spectrum of the energy losses (E sub p =4.0; 5.6; 12.5 and 14.5 eV) in the area of low energies (< 60 eV) reflects the structure of transitions between the valency zone and the conductivity zone. The energy losses on the plasma oscillations excitation the excitation of pi-plasmon with the energy of 6.5 eV and excitation of the pi-sigma plasmon with the energy of 25 eV become prevailing with the growth of the initial electrons energy

  14. Electron energy loss spectroscopy with parallel readout of energy and momentum

    CERN Document Server

    Ibach, Harald; Sforzini, Jessica; Soubatch, Serguei; Tautz, F Stefan

    2016-01-01

    We introduce a high energy resolution electron source that matches the requirements for parallel readout of energy and momentum of modern hemispherical electron energy analyzers. The system is designed as an add-on device to typical photoemission chambers. Due to the multiplex gain, a complete phonon dispersion of a Cu(111) surface was measured in seven minutes with 4 meV energy resolution.

  15. Continuous Electron--Energy Variation of the Eindhoven Racetrack Microtron.

    Science.gov (United States)

    Theuws, W. H. C.; Botman, J. I. M.; Hagedoorn, H. L.

    1997-05-01

    Energy variation of the Eindhoven racetrack microtron, which has been designed as a fixed--energy electron accelerator at 75 MeV, is considered in this paper. By taking the orbit pattern in the RTM as constant and varying certain parameters continuous energy variation can be obtained. The microtron injector is a linac producing electrons between 6 and 12 MeV. The microtron cavity potential and the magnetic guide fields must be adapted to the injection energy in order to fulfil the synchronism condition. The transverse and longitudinal acceptance of the RTM are effected by deviations of the electron velocity from the speed of light, which are different for each parameter setting. An account of these effects is presented together with the energy--setting measurements by using one of the microtron magnets as a spectrometer.

  16. Modelling low energy electron interactions for biomedical uses of radiation

    Energy Technology Data Exchange (ETDEWEB)

    Fuss, M; Garcia, G [Instituto de Fisica Fundamental, Consejo Superior de Investigaciones CientIficas (CSIC), Serrano 113-bis, 28006 Madrid (Spain); Munoz, A; Oller, J C [Centro de Investigaciones Energeticas, Medioambientales y Tecnologicas (CIEMAT), Avenida Complutense 22, 28040 Madrid (Spain); Blanco, F [Departamento de Fisica Atomica, Molecular y Nuclear, Universidad Complutense de Madrid, Avenida Complutense s.n., 28040 Madrid (Spain); Limao-Vieira, P [Departamento de Fisica, Universidade Nova de Lisboa, 2829-516 Caparica (Portugal); Huerga, C; Tellez, M [Hospital Universitario La Paz, paseo de la Castellana 261, 28046 Madrid (Spain); Hubin-Fraskin, M J [Department of Chemistry, University of Liege, 4000 Liege 1 (Belgium); Nixon, K; Brunger, M, E-mail: g.garcia@imaff.cfmac.csic.e [School of Chemistry, Physics and Earth Sciences, Flinders University, GPO Box 2100, Adelaide, SA 5001 (Australia)

    2009-11-15

    Current radiation based medical applications in the field of radiotherapy, radio-diagnostic and radiation protection require modelling single particle interactions at the molecular level. Due to their relevance in radiation damage to biological systems, special attention should be paid to include the effect of low energy secondary electrons. In this study we present a single track simulation procedure for photons and electrons which is based on reliable experimental and theoretical cross section data and the energy loss distribution functions derived from our experiments. The effect of including secondary electron interactions in this model will be discussed.

  17. A molecularly based theory for electron transfer reorganization energy

    Energy Technology Data Exchange (ETDEWEB)

    Zhuang, Bilin; Wang, Zhen-Gang, E-mail: zgw@cheme.caltech.edu [Division of Chemistry and Chemical Engineering, California Institute of Technology, Pasadena, California 91125 (United States)

    2015-12-14

    Using field-theoretic techniques, we develop a molecularly based dipolar self-consistent-field theory (DSCFT) for charge solvation in pure solvents under equilibrium and nonequilibrium conditions and apply it to the reorganization energy of electron transfer reactions. The DSCFT uses a set of molecular parameters, such as the solvent molecule’s permanent dipole moment and polarizability, thus avoiding approximations that are inherent in treating the solvent as a linear dielectric medium. A simple, analytical expression for the free energy is obtained in terms of the equilibrium and nonequilibrium electrostatic potential profiles and electric susceptibilities, which are obtained by solving a set of self-consistent equations. With no adjustable parameters, the DSCFT predicts activation energies and reorganization energies in good agreement with previous experiments and calculations for the electron transfer between metallic ions. Because the DSCFT is able to describe the properties of the solvent in the immediate vicinity of the charges, it is unnecessary to distinguish between the inner-sphere and outer-sphere solvent molecules in the calculation of the reorganization energy as in previous work. Furthermore, examining the nonequilibrium free energy surfaces of electron transfer, we find that the nonequilibrium free energy is well approximated by a double parabola for self-exchange reactions, but the curvature of the nonequilibrium free energy surface depends on the charges of the electron-transferring species, contrary to the prediction by the linear dielectric theory.

  18. Electron energy can oscillate near a crystal dislocation

    Science.gov (United States)

    Li, Mingda; Cui, Wenping; Dresselhaus, Mildred S.; Chen, Gang

    2017-01-01

    Crystal dislocations govern the plastic mechanical properties of materials but also affect the electrical and optical properties. However, a fundamental and quantitative quantum field theory of a dislocation has remained undiscovered for decades. Here we present an exactly-solvable one-dimensional quantum field theory of a dislocation, for both edge and screw dislocations in an isotropic medium, by introducing a new quasiparticle which we have called the ‘dislon’. The electron-dislocation relaxation time can then be studied directly from the electron self-energy calculation, which is reducible to classical results. In addition, we predict that the electron energy will experience an oscillation pattern near a dislocation. Compared with the electron density’s Friedel oscillation, such an oscillation is intrinsically different since it exists even with only single electron is present. With our approach, the effect of dislocations on materials’ non-mechanical properties can be studied at a full quantum field theoretical level.

  19. Renewable Energy Systems in the Power Electronics Curriculum

    DEFF Research Database (Denmark)

    Blaabjerg, Frede; Chen, Zhe; Teodorescu, Remus

    2005-01-01

    Power Electronics is still an emerging technology and its applications are increasing. The primary function is to convert electrical energy from one stage to another and it is used in many different applications. The power electronics curriculum is multidisciplinary covering fields like devices......, magnetics, electrical machines, power systems, analogue and digital control, materials, power converters, electronics, materials, thermal design and EMC. However, those fields may not be enough in order to give the students enough skills. It is also necessary to learn about systems and for the moment one...... of the most important area is renewable energy systems. This paper will discuss the basic courses for the power electronics curriculum. It will also discuss how to teach power electronic systems efficiently through a projectoriented and problem-based learning approach with Aalborg University in Denmark...

  20. Electron and photon energy measurement calibration with the ATLAS detector

    CERN Document Server

    Manzoni, Stefano; The ATLAS collaboration

    2016-01-01

    An accurate calibration of the energy measurement of electron and photon is paramount for many ATLAS physics analysis. The calibration of the energy measurement is performed in-situ using a large statistics of Z->ee events. The results obtained with the pp collisions data recorded in 2015 and 2016 at sqrt(s)= 13 TeV, corresponding to an integrated luminosity of 3.2 fb-1 and 2.7 fb-1 respectively , as well as the corresponding uncertainties on the electron and photon energy scales, are presented.

  1. Electron and photon energy measurement calibration with the ATLAS detector

    CERN Document Server

    Manzoni, Stefano; The ATLAS collaboration

    2016-01-01

    An accurate calibration of the energy measurement of electrons and photons is paramount for many ATLAS physics analyses. The calibration of the energy measurement is performed $in$-$situ$ using a large statistics of $Z \\rightarrow ee$ events. The results obtained with the $pp$ collisions data recorded in 2015 and 2016 at $\\sqrt{s}=13$ TeV, corresponding to an integrated luminosity of 3.2 fb$^{-1}$ and 2.7 fb$^{-1}$ respectively, as well as the corresponding uncertainties on the electron and photon energy scales, are presented

  2. GEANT4 simulation of electron energy deposition in extended media

    CERN Document Server

    Kadri, O; Gharbi, F; Trabelsi, A

    2007-01-01

    The present work demonstrates that GEANT4 yields a consistent description of electron transport processes in semi-infinite homogeneous and heterogeneous extended media. This comparison covers the e− energy deposition profiles in a range of elements from aluminum to tantalum through molybdenum at source energies from 0.3 to 1.0 MeV and at incident angles from 0° to 60°. The good agreement between simulation results and data confirms that the Monte Carlo used code is capable of accurate electron beam energy deposition calculation even under such conditions.

  3. Separated high-energy electron beams using synchrotron radiation

    CERN Document Server

    Farley, F J M; Picasso, Emilio

    1972-01-01

    Electrons with kinetic energy in the 100 GeV range may be separated from other particles by using their energy-loss due to synchrotron radiation in a high-field magnet. In this paper the associated fluctuations in energy and angle are shown to be small enough for the method to be useful. Detailed design formulae are presented for several magnet configurations. (7 refs).

  4. Time Evolution of the Electron Swarm Energy Distribution Function

    Science.gov (United States)

    1989-06-28

    25 Characteristic energy c and mobility g in a pulsed electric field in air lasting 25 ns ....... ............................... 55 26...Characteristic energy E and mobility tz in a pulsed electric field in air lasting 100 ns ........ ............................... 56 27 Electron energy...originally thermal swarm in a rapidly varying pulsed electric field . We do so in air in spite of the fact that it stresses the Fokker-Planck

  5. Photodetachment studies on few-electron atomic negative ions

    Energy Technology Data Exchange (ETDEWEB)

    Pegg, D.J.

    1992-12-31

    A crossed laser-negative ion beams apparatus, situated at Oak Ridge National Laboratory has been used for energy and angle-resolved photoelectron spectroscopic measurements following photodetachment. In the current grant period measurements of the cross sections for photodetaching an electron from the Li{sup {minus}} ion were finished. Measurements of the {sigma}(B{sup {minus}})/{sigma}(Li{sup {minus}}) ratio, with a goal of determining photodetachment cross section for B{sup {minus}}, were started. An investigation of the photodetachment of the metastable ion Be{sup {minus}} also began. Preliminary data on the electron affinity, asymmetry parameter and cross section associated with the photodetachment of Be{sup {minus}} at a photon energy of 2.076 eV is reported.

  6. Power electronics for renewable energy systems, transportation and industrial applications

    CERN Document Server

    Malinowski, Mariusz; Al-Haddad, Kamal

    2014-01-01

    Power Electronics for Renewable Energy, Transportation, and Industrial Applications combines state-of-the-art global expertise to present the latest research on power electronics and its application in transportation, renewable energy, and different industrial applications. This timely book aims to facilitate the implementation of cutting-edge techniques to design problems offering innovative solutions to the growing power demands in small- and large-size industries. Application areas in the book range from smart homes and electric and plug-in hybrid electrical vehicles (PHEVs), to smart distribution and intelligence operation centers where significant energy efficiency improvements can be achieved through the appropriate use and design of power electronics and energy storage devices.

  7. Power electronics - key technology for renewable energy systems

    DEFF Research Database (Denmark)

    Blaabjerg, Frede; Iov, Florin; Kerekes, Tamas

    2011-01-01

    sources to renewable energy sources. Another is to use high efficient power electronics in power generation, power transmission/distribution and end-user application. This paper discuss trends of the most emerging renewable energy sources, wind energy and photovoltaics, which by means of power electronics...... are changing and challenging the future electrical infrastructure but also contributes steadily more to non-carbon based electricity production. Most focus in the paper is on the power electronics technologies used. In the case of photovoltaics transformer-less systems are discussed as they have the potential...... as efficient as possible. Further, the emerging climate changes is arguing to find sustainable future solutions. Of many options, two major technologies will play important roles to solve parts of those future problems. One is to change the electrical power production from conventional, fossil based energy...

  8. Trends in Power Electronics and Control of Renewable Energy Systems

    DEFF Research Database (Denmark)

    Blaabjerg, Frede; Iov, Florin; Kerekes, Tamas

    2010-01-01

    term) based energy sources to renewable energy sources. Another is to use high efficient power electronics in power generation, power transmission/distribution and end-user application. This paper discuss trends of the most emerging renewable energy sources, wind energy and photovoltaics, which...... by means of power electronics are changing the future electrical infrastructure but also contributes steadily more to non-carbon based electricity production. Most focus is on the power electronics technologies used. In the case of photovoltaics transformer-less systems are discussed as they have...... are done as efficient as possible. Further, emerging climate changes argues to find future solutions which also are sustainable. Two major technologies will play important roles to solve parts of those future problems. One is the change the electrical power production from conventional, fossil (and short...

  9. Modeling power electronics and interfacing energy conversion systems

    CERN Document Server

    Simões, Marcelo Godoy

    2017-01-01

    Discusses the application of mathematical and engineering tools for modeling, simulation and control oriented for energy systems, power electronics and renewable energy. This book builds on the background knowledge of electrical circuits, control of dc/dc converters and inverters, energy conversion and power electronics. The book shows readers how to apply computational methods for multi-domain simulation of energy systems and power electronics engineering problems. Each chapter has a brief introduction on the theoretical background, a description of the problems to be solved, and objectives to be achieved. Block diagrams, electrical circuits, mathematical analysis or computer code are covered. Each chapter concludes with discussions on what should be learned, suggestions for further studies and even some experimental work.

  10. Studies on electronic structure of GaN(0001) surface

    CERN Document Server

    Xie Chang Kun; Xu Fa Qiang; Deng Rui; Liu Feng; Yibulaxin, K

    2002-01-01

    An electronic structure investigation on GaN(0001) is reported. The authors employ a full-potential linearized augmented plane-wave (FPLAPW) approach to calculate the partial density of state, which is in agreement with previous experimental results. The effects of the Ga3d semi-core levels on the electronic structure of GaN are discussed. The valence-electronic structure of the wurtzite GaN(0001) surface is investigated using synchrotron radiation excited angle-resolved photoemission spectroscopy. The bulk bands dispersion along GAMMA A direction in the Brillouin zones is measured using normal-emission spectra by changing photon-energy. The band structure derived from authors' experimental data is compared well with the results of authors' FPLAPW calculation. Furthermore, off-normal emission spectra are also measured along the GAMMA K and GAMMA M directions. Two surface states are identified, and their dispersions are characterized

  11. Position and size of the electron beam in the high-energy electron beam ion trap

    CERN Document Server

    Utter, S B; López-Urrutia, J R C; Widmann, K

    1999-01-01

    In the last decade, many spectroscopic studies have been performed using the electron beam ion trap. Often these measurements rely on the electron beam as an effective slit, yet until now, no systematic study of the position and size of the electron beam under various operating conditions has been made. Here, we present a thorough study of the electron beam's position and size (and thus the electron density) as affected by various operating parameters, and give optimal parameter ranges for operating the device as a spectroscopic source. It is shown that the diameter is constant as the energy is varied, which is important for accurate cross-section measurements.

  12. Calculation of Electron Beam Potential Energy from RF Photocathode Gun

    CERN Document Server

    Liu Wan Ming; Power, John G; Wang, Haitao

    2005-01-01

    In this paper, we consider the contribution of potential energy to beam dynamics as simulated by PARMELA at low energies (10 - 30MeV). We have developed a routine to calculate the potential energy of the relativistic electron beam using the static coulomb potential in the rest frame (first order approximation as in PARMELA). We found that the potential energy contribution to the beam dynamics could be very significant, particularly with high charge beams generated by an RF photocathode gun. Our results show that when the potential energy is counted correctly and added to the kinetic energy from PARMELA, the total energy is conserved. Simulation results of potential and kinetic energies for short beams (~1 mm) at various charges (1 - 100 nC) generated by a high current RF photocathode gun are presented.

  13. Study of energy delivery and mean free path of low energy electrons in EUV resists

    Science.gov (United States)

    Bhattarai, Suchit; Neureuther, Andrew R.; Naulleau, Patrick P.

    2016-03-01

    The relative importance of secondary electrons in delivering energy in photoresist films was assessed by performing large area exposures and by quantifying the inelastic mean free path of electrons in a leading chemically amplified positive tone EUV resist. A low energy electron microscope was used to directly pattern large (~15μm x 20μm) features with 15-80 eV electrons followed by analyzing the resulting dissolution rate contrast curve data. In the 40 to 80 eV regime the energy delivery was found to scale roughly proportionally with electron energy. In 15 to 30 eV regime however, this energy scaling did not explain the resist thickness loss data. The dose required to lower the resist thickness down to 20 nm was found to be 2-5X larger for 15 eV electrons than for 20, 25 and 30 eV electrons. Using scattering models from the literature including phonon scattering and optical data deduced electron energy loss spectroscopy and optical reflectometry, the inelastic mean free path values at energies between 10 eV and 92 eV range between about 2.8 and 0.6 nm respectively.

  14. Communication: Investigation of the electron momentum density distribution of nanodiamonds by electron energy-loss spectroscopy

    Energy Technology Data Exchange (ETDEWEB)

    Feng, Zhenbao; Yang, Bing; Lin, Yangming; Su, Dangsheng, E-mail: dssu@imr.ac.cn [Shenyang National Laboratory of Materials Science, Institute of Metal Research, Chinese Academy of Sciences, Wenhua Road 72, Shenyang 110016 (China)

    2015-12-07

    The electron momentum distribution of detonation nanodiamonds (DND) was investigated by recording electron energy-loss spectra at large momentum transfer in the transmission electron microscope (TEM), which is known as electron Compton scattering from solid (ECOSS). Compton profile of diamond film obtained by ECOSS was found in good agreement with prior photon experimental measurement and theoretical calculation that for bulk diamond. Compared to the diamond film, the valence Compton profile of DND was found to be narrower, which indicates a more delocalization of the ground-state charge density for the latter. Combining with other TEM characterizations such as high-resolution transmission electron spectroscopy, diffraction, and energy dispersive X-ray spectroscopy measurements, ECOSS was shown to be a great potential technique to study ground-state electronic properties of nanomaterials.

  15. Design for Reliability of Power Electronics in Renewable Energy Systems

    DEFF Research Database (Denmark)

    Ma, Ke; Yang, Yongheng; Wang, Huai

    2014-01-01

    Power electronics is the enabling technology for maximizing the power captured from renewable electrical generation, e.g., the wind and solar technology, and also for an efficient integration into the grid. Therefore, it is important that the power electronics are reliable and do not have too many...... electronics technology as well as to know how the power electronics technology is loaded in terms of temperature and other stressors relevant, to reliability. Hence, this chapter will show the basics of power electronics technology for renewable energy systems, describe the mission profile of the technology...... failures during operation which otherwise will increase cost for operation, maintenance and reputation. Typically, power electronics in renewable electrical generation has to be designed for 20–30 years of operation, and in order to do that, it is crucial to know about the mission profile of the power...

  16. Technical Training: ELEC-2005: Electronics in High Energy Physics

    CERN Multimedia

    Monique Duval

    2005-01-01

    CERN Technical Training 2005: Learning for the LHC! ELEC-2005: Electronics in High Energy Physics - Spring Term ELEC-2005 is a new course series on modern electronics, given by CERN physicists and engineers within the framework of the 2005 Technical Training Programme, in an extended format of the successful ELEC-2002 course series. This comprehensive course series is designed for people who are not electronics specialists, for example physicists, engineers and technicians working at or visiting the laboratory, who use or will use electronics in their present or future activities, in particular in the context of the LHC accelerator and experiments. ELEC-2005 is composed of four Terms: the Winter Term, Introduction to electronics in HEP, already took place; the next three Terms will run throughout the year: Spring Term: Integrated circuits and VLSI technology for physics (March, 6 lectures) - now open for registration Summer Term: System electronics for physics: Issues (May, 7 lectures) Autumn Term: Ele...

  17. Energy Filtering and Coaxial Detection of the Backscattered Electrons in Scanning Electron Microscope

    Institute of Scientific and Technical Information of China (English)

    JIANG Chang-Zhong; P. Morin; N. Rosenberg

    2000-01-01

    A new detection system in scanning electron microscope, which filters in energy and detects the backscattered electrons close to the microscope axis, is described. This technique ameliorates the dependence of the back. scat tering coefficient on atomic number, and suppresses effectively the relief contrast at the same time. Therefore this new method is very suitable to the composition analysis.

  18. Detectors for low energy electron cooling in RHIC

    Energy Technology Data Exchange (ETDEWEB)

    Carlier, F. S. [Brookhaven National Lab. (BNL), Upton, NY (United States)

    2016-02-15

    Low energy operation of RHIC is of particular interest to study the location of a possible critical point in the QCD phase diagram. The performance of RHIC at energies equal to or lower than 10 GV/nucleon is limited by nonlinearities, Intra-BeamScattering (IBS) processes and space-charge effects. To successfully address the luminosity and ion store lifetime limitations imposed by IBS the method of electron cooling has been envisaged. During electron cooling processes electrons are injected along with the ion beam at the nominal ion bunch velocities. The velocity spread of the ion beam is reduced in all planes through Coulomb interactions between the cold electron beam and the ion beam. The electron cooling system proposed for RHIC will be the first of its kind to use bunched beams for the delivery of the electron bunches, and will therefore be accompanied by the necessary challenges. The designed electron cooler will be located in IP2. The electron bunches will be accelerated by a linac before being injected along side the ion beams. Thirty consecutive electron bunches will be injected to overlap with a single ion bunch. They will first cool the yellow beam before being extracted turned by 180-degrees and reinjected into the blue beam for cooling. As such, both the yellow and blue beams will be cooled by the same ion bunches. This will pose considerable challenges to ensure proper electron beam quality to cool the second ion beam. Furthermore, no ondulator will be used in the electron cooler so radiative recombination between the ions and the electrons will occur.

  19. Sustainably powering wearable electronics solely by biomechanical energy

    Science.gov (United States)

    Wang, Jie; Li, Shengming; Yi, Fang; Zi, Yunlong; Lin, Jun; Wang, Xiaofeng; Xu, Youlong; Wang, Zhong Lin

    2016-09-01

    Harvesting biomechanical energy is an important route for providing electricity to sustainably drive wearable electronics, which currently still use batteries and therefore need to be charged or replaced/disposed frequently. Here we report an approach that can continuously power wearable electronics only by human motion, realized through a triboelectric nanogenerator (TENG) with optimized materials and structural design. Fabricated by elastomeric materials and a helix inner electrode sticking on a tube with the dielectric layer and outer electrode, the TENG has desirable features including flexibility, stretchability, isotropy, weavability, water-resistance and a high surface charge density of 250 μC m-2. With only the energy extracted from walking or jogging by the TENG that is built in outsoles, wearable electronics such as an electronic watch and fitness tracker can be immediately and continuously powered.

  20. Power Electronics and Reliability in Renewable Energy Systems

    DEFF Research Database (Denmark)

    Blaabjerg, Frede; Ma, Ke; Zhou, Dao

    2012-01-01

    Power Electronics are needed in almost all kind of renewable energy systems. It is used both for controlling the renewable source and also for interfacing to the load, which can be grid-connected or working in stand-alone mode. More and more efforts are put into making renewable energy systems...... better in terms of reliability in order to ensure a high availability of the power sources, in this case the knowledge of mission profile of a certain application is crucial for the reliability evaluation/design of power electronics. In this paper an overview on the power electronic circuits behind...... the most common converter configurations for wind turbine and photovoltaic is done. Next different aspects of improving the system reliability are mapped. Further on examples of how to control the chip temperature in different power electronic configurations as well as operation modes for wind power...

  1. Sustainably powering wearable electronics solely by biomechanical energy.

    Science.gov (United States)

    Wang, Jie; Li, Shengming; Yi, Fang; Zi, Yunlong; Lin, Jun; Wang, Xiaofeng; Xu, Youlong; Wang, Zhong Lin

    2016-09-28

    Harvesting biomechanical energy is an important route for providing electricity to sustainably drive wearable electronics, which currently still use batteries and therefore need to be charged or replaced/disposed frequently. Here we report an approach that can continuously power wearable electronics only by human motion, realized through a triboelectric nanogenerator (TENG) with optimized materials and structural design. Fabricated by elastomeric materials and a helix inner electrode sticking on a tube with the dielectric layer and outer electrode, the TENG has desirable features including flexibility, stretchability, isotropy, weavability, water-resistance and a high surface charge density of 250 μC m(-2). With only the energy extracted from walking or jogging by the TENG that is built in outsoles, wearable electronics such as an electronic watch and fitness tracker can be immediately and continuously powered.

  2. Sustainably powering wearable electronics solely by biomechanical energy

    Science.gov (United States)

    Wang, Jie; Li, Shengming; Yi, Fang; Zi, Yunlong; Lin, Jun; Wang, Xiaofeng; Xu, Youlong; Wang, Zhong Lin

    2016-01-01

    Harvesting biomechanical energy is an important route for providing electricity to sustainably drive wearable electronics, which currently still use batteries and therefore need to be charged or replaced/disposed frequently. Here we report an approach that can continuously power wearable electronics only by human motion, realized through a triboelectric nanogenerator (TENG) with optimized materials and structural design. Fabricated by elastomeric materials and a helix inner electrode sticking on a tube with the dielectric layer and outer electrode, the TENG has desirable features including flexibility, stretchability, isotropy, weavability, water-resistance and a high surface charge density of 250 μC m−2. With only the energy extracted from walking or jogging by the TENG that is built in outsoles, wearable electronics such as an electronic watch and fitness tracker can be immediately and continuously powered. PMID:27677971

  3. Power Electronics as Efficient Interface of Renewable Energy Sources

    DEFF Research Database (Denmark)

    Blaabjerg, Frede; Chen, Zhe; Kjær, Søren Bækhøj

    2004-01-01

    renewable energy conversion system, will play an important part in our future energy supply. But other sources like microturbines, photovoltaics and fuel cell systems may also be serious contributor to the power supply. Characteristically, power electronics will be an efficient and important interface......The global electrical energy consumption is steadily rising and consequently there is a demand to increase the power generation capacity. A significant percentage of the required capacity increase can be based on renewable energy sources. Wind turbine technology, as the most cost effective...

  4. Flexible Nanogenerators for Energy Harvesting and Self-Powered Electronics.

    Science.gov (United States)

    Fan, Feng Ru; Tang, Wei; Wang, Zhong Lin

    2016-06-01

    Flexible nanogenerators that efficiently convert mechanical energy into electrical energy have been extensively studied because of their great potential for driving low-power personal electronics and self-powered sensors. Integration of flexibility and stretchability to nanogenerator has important research significance that enables applications in flexible/stretchable electronics, organic optoelectronics, and wearable electronics. Progress in nanogenerators for mechanical energy harvesting is reviewed, mainly including two key technologies: flexible piezoelectric nanogenerators (PENGs) and flexible triboelectric nanogenerators (TENGs). By means of material classification, various approaches of PENGs based on ZnO nanowires, lead zirconate titanate (PZT), poly(vinylidene fluoride) (PVDF), 2D materials, and composite materials are introduced. For flexible TENG, its structural designs and factors determining its output performance are discussed, as well as its integration, fabrication and applications. The latest representative achievements regarding the hybrid nanogenerator are also summarized. Finally, some perspectives and challenges in this field are discussed.

  5. Data Acquisition System for Electron Energy Loss Coincident Spectrometers

    Institute of Scientific and Technical Information of China (English)

    Zhang Chi; Yu Xiaoqi; Yang Tao

    2005-01-01

    A Data Acquisition System (DAQ) for electron energy loss coincident spectrometers (EELCS) has been developed. The system is composed of a Multiplex Time-Digital Converter (TDC) that measures the flying time of positive and negative ions and a one-dimension positionsensitive detector that records the energy loss of scattering electrons. The experimental data are buffered in a first-in-first-out(FIFO) memory module, then transferred from the FIFO memory to PC by the USB interface. The DAQ system can record the flying time of several ions in one collision, and allows of different data collection modes. The system has been demonstrated at the Electron Energy Loss Coincident Spectrometers at the Laboratory of Atomic and Molecular Physics, USTC. A detail description of the whole system is given and experimental results shown.

  6. Soft electron (low energy electron) processing of foods for microbial control

    Energy Technology Data Exchange (ETDEWEB)

    Todoriki, Setsuko E-mail: setsuko@nfri.affrc.go.jp; Kikuchi, Olivia Kimiko; Nakaoka, Motoko; Miike, Mika; Hayashi, Toru

    2002-03-01

    'Soft-electron' is a new term we have created referring to electrons with energies of 300 kV or lower. Homogenous irradiation of surfaces with soft electrons can decontaminate dry food ingredients such as gains, pulses, spices, dehydrated vegetables and tealeaves without detrimental effects. Treatment of soybeans with electrons of acceleration voltages at 170 kV reduced their microbial count to an undetectable level. Pre-treatment of soybeans with soft electrons enabled the extension of soymilk without sterilization process at a high temperature (120 deg. C). The gelatinized property of soymilk from soft electron-treated beans was better than that of high-temperature sterilized soymilks. These results indicate that soft-electron sterilization improved the quality of soybeans for the processing of soymilk and Tofu(soymilk curd)

  7. Proposal to detect an emission of unusual super-high energy electrons in electron storage rings

    Directory of Open Access Journals (Sweden)

    Da-peng Qian

    2014-01-01

    Full Text Available According to an extended Lorentz–Einstein mass formula taken into the uncertainty principle, it is predicted that the electron beams passing accelerating electric field should with a small probability generate abnormal super-high energy electrons which are much higher than the beam energy. Author’s preliminary experiment result at electron storage ring has hinted these signs, so suggests to more strictly detect this unusual phenomenon, and thus to test the extended mass formula as well as a more perfect special relativity.

  8. Fe/GaAs(001) and MgO/Fe/GaAs(001) epitaxial systems: A spin- and angle-resolved photoemission study

    Energy Technology Data Exchange (ETDEWEB)

    Gottlob, Daniel [Forschungszentrum Juelich GmbH (Germany); Technische Universitaet Dortmund (Germany); Plucinski, Lukasz; Schneider, Claus M. [Forschungszentrum Juelich GmbH (Germany); Westphal, Carsten [Technische Universitaet Dortmund (Germany)

    2011-07-01

    Spintronics is an important field of current Solid State Research and memory units based on Magnetic Tunnel Junctions (MTJs) are now within reach. In MTJ's the nature of the electronic structure at the interface determines the spin-selectivity of the tunneling process, and thereby the magnetorestive potential of the MTJ. Electronic interface states can influence the tunneling process in epitaxial MTJs especially for thinner tunnel barriers. The research that has been done at Beamline 5, DELTA, Dortmund in the context of a Diploma thesis focussed on the electronic structure of Fe/GaAs(001) and MgO/Fe/GaAs(001) and a surface/interface state of these systems. The samples have been prepared in situ by molecular beam epitaxy and characterized by LEED and Auger spectroscopy. The electronic structure was probed in two different regions of the Brillouin zone, which have been chosen for reference (normal emission, {gamma} point) and the expectation of the surface state (21 off normal) that has been seen on Fe/W(001) in a previous study. Measurements on the MgO capped iron sample have been conducted to confirm whether the surface state does transform into an interface state.

  9. Transfer of chirality from adsorbed chiral molecules to the substrates highlighted by circular dichroism in angle-resolved valence photoelectron spectroscopy

    DEFF Research Database (Denmark)

    Contini, G.; Turchini, S.; Sanna, Simone

    2012-01-01

    Studies of self-assembled chiral molecules on achiral metallic surfaces have mostly focused on the determination of the geometry of adsorbates and their electronic structure. The aim of this paper is to provide direct information on the chirality character of the system and on the chirality trans...

  10. Superconductor digital electronics: Scalability and energy efficiency issues (Review Article)

    Science.gov (United States)

    Tolpygo, Sergey K.

    2016-05-01

    Superconductor digital electronics using Josephson junctions as ultrafast switches and magnetic-flux encoding of information was proposed over 30 years ago as a sub-terahertz clock frequency alternative to semiconductor electronics based on complementary metal-oxide-semiconductor (CMOS) transistors. Recently, interest in developing superconductor electronics has been renewed due to a search for energy saving solutions in applications related to high-performance computing. The current state of superconductor electronics and fabrication processes are reviewed in order to evaluate whether this electronics is scalable to a very large scale integration (VLSI) required to achieve computation complexities comparable to CMOS processors. A fully planarized process at MIT Lincoln Laboratory, perhaps the most advanced process developed so far for superconductor electronics, is used as an example. The process has nine superconducting layers: eight Nb wiring layers with the minimum feature size of 350 nm, and a thin superconducting layer for making compact high-kinetic-inductance bias inductors. All circuit layers are fully planarized using chemical mechanical planarization (CMP) of SiO2 interlayer dielectric. The physical limitations imposed on the circuit density by Josephson junctions, circuit inductors, shunt and bias resistors, etc., are discussed. Energy dissipation in superconducting circuits is also reviewed in order to estimate whether this technology, which requires cryogenic refrigeration, can be energy efficient. Fabrication process development required for increasing the density of superconductor digital circuits by a factor of ten and achieving densities above 107 Josephson junctions per cm2 is described.

  11. Energy limitation of laser-plasma electron accelerators

    CERN Document Server

    Cardenas, D E; Xu, J; Hofmann, L; Buck, A; Schmid, K; Sears, C M S; Rivas, D E; Shen, B; Veisz, L

    2015-01-01

    We report on systematic and high-precision measurements of dephasing, an effect that fundamentally limits the performance of laser wakefield accelerators. Utilizing shock-front injection, a technique providing stable, tunable and high-quality electron bunches, acceleration and deceleration of few-MeV quasi-monoenergetic beams were measured with sub-5-fs and 8-fs laser pulses. Typical density dependent electron energy evolution with 65-300 micrometers dephasing length and 6-20 MeV peak energy was observed and is well described with a simple model.

  12. Mercuric iodide dosimeter response to high energy electron beams

    Energy Technology Data Exchange (ETDEWEB)

    Loewinger, E.; Nissenbaum, J.; Schieber, M.M.

    1988-01-01

    Mercuric iodide solid state dosimeter response to high energy electron beams of up to 35 MeV is reported. High sensitivity of up to 1.5 V/cGy was observed with a 200 V external bias, as well as several mV/cGy, with no external bias for small volume (approx. 10 mm/sup 3/) detectors. The physical characteristics of the detector response are discussed, showing the feasibility of mercuric iodide as a reliable dosimeter for high energy electron beams.

  13. Double aberration correction in a low-energy electron microscope

    Energy Technology Data Exchange (ETDEWEB)

    Schmidt, Th., E-mail: schmidtt@fhi-berlin.mpg.de [Fritz-Haber-Institut der Max-Planck-Gesellschaft, Faradayweg 6-8, D-14195 Berlin (Germany); Universitaet Wuerzburg, Experimentelle Physik II, Am Hubland, D-97074 Wuerzburg (Germany); Marchetto, H.; Levesque, P.L. [Fritz-Haber-Institut der Max-Planck-Gesellschaft, Faradayweg 6-8, D-14195 Berlin (Germany); Groh, U.; Maier, F. [Universitaet Wuerzburg, Experimentelle Physik II, Am Hubland, D-97074 Wuerzburg (Germany); Preikszas, D. [Technische Universitaet Darmstadt, Angewandte Physik, Hochschulstrasse 6, D-64289 Darmstadt (Germany); Carl Zeiss NTS GmbH, Carl-Zeiss-Strasse 56, D-73447 Oberkochen (Germany); Hartel, P.; Spehr, R. [Technische Universitaet Darmstadt, Angewandte Physik, Hochschulstrasse 6, D-64289 Darmstadt (Germany); Lilienkamp, G. [Technische Universitaet Clausthal, Physikalisches Institut, Leibnizstrasse 4, D-38678 (Germany); Engel, W. [Fritz-Haber-Institut der Max-Planck-Gesellschaft, Faradayweg 6-8, D-14195 Berlin (Germany); Fink, R. [Universitaet Erlangen-Nuernberg, Physikalische Chemie II, Egerlandstrasse 3, D-91058 Erlangen (Germany); Bauer, E. [Technische Universitaet Clausthal, Physikalisches Institut, Leibnizstrasse 4, D-38678 (Germany); Arizona State University, Department of Physics, Tempe, AZ 85287 (United States); Rose, H. [Technische Universitaet Darmstadt, Angewandte Physik, Hochschulstrasse 6, D-64289 Darmstadt (Germany); Umbach, E. [Universitaet Wuerzburg, Experimentelle Physik II, Am Hubland, D-97074 Wuerzburg (Germany); Freund, H.-J. [Fritz-Haber-Institut der Max-Planck-Gesellschaft, Faradayweg 6-8, D-14195 Berlin (Germany)

    2010-10-15

    The lateral resolution of a surface sensitive low-energy electron microscope (LEEM) has been improved below 4 nm for the first time. This breakthrough has only been possible by simultaneously correcting the unavoidable spherical and chromatic aberrations of the lens system. We present an experimental criterion to quantify the aberration correction and to optimize the electron optical system. The obtained lateral resolution of 2.6 nm in LEEM enables the first surface sensitive, electron microscopic observation of the herringbone reconstruction on the Au(1 1 1) surface.

  14. Free electron lasers for transmission of energy in space

    Science.gov (United States)

    Segall, S. B.; Hiddleston, H. R.; Catella, G. C.

    1981-01-01

    A one-dimensional resonant-particle model of a free electron laser (FEL) is used to calculate laser gain and conversion efficiency of electron energy to photon energy. The optical beam profile for a resonant optical cavity is included in the model as an axial variation of laser intensity. The electron beam profile is matched to the optical beam profile and modeled as an axial variation of current density. Effective energy spread due to beam emittance is included. Accelerators appropriate for a space-based FEL oscillator are reviewed. Constraints on the concentric optical resonator and on systems required for space operation are described. An example is given of a space-based FEL that would produce 1.7 MW of average output power at 0.5 micrometer wavelength with over 50% conversion efficiency of electrical energy to laser energy. It would utilize a 10 m-long amplifier centered in a 200 m-long optical cavity. A 3-amp, 65 meV electrostatic accelerator would provide the electron beam and recover the beam after it passes through the amplifier. Three to five shuttle flights would be needed to place the laser in orbit.

  15. Low energy electron interactions with complex biological targets

    Science.gov (United States)

    Orlando, Thomas

    2012-10-01

    The low energy (1-25 eV) electron-induced damage of DNA oligomers have been examined both theoretically and experimentally. Specifically, elastic scattering of 5-30 eV electrons within B-DNA 5'-CCGGCGCCGG-3' and A-DNA 5'-CGCGAATTCGCG-3' sequences has been calculated using the separable representation of a free-space electron propagator and a curved wave multiple scattering formalism. The disorder brought about by the surrounding water and helical base stacking leads to featureless amplitude build-up of elastically scattered electrons on the sugars and phosphate groups for all energies between 5-30 eV. However, some constructive interference features arising from diffraction were revealed when examining the structural waters within the major groove. We correlated these scattering features with measured DNA single and double strand breaks. Compound resonance states involving interfacial water and excitation energies > 5 eV seem to be required for lethal double strand breaks. We have recently extended this work to excitation energies below 5 eV by examining the damage using Raman-microscopy and scanning electrostatic force microscopy. Very efficient damage via single strand breaks is observed below 5 eV excitation energies. This involves π* negative ion resonances that are initially localized on the bases but transferred to the σ* states of the sugar-phosphate bond. The efficacies of these channels depend upon the base-pair sequences as well as the presence of water.

  16. Polarization of high-energy electrons traversing a laser beam

    Energy Technology Data Exchange (ETDEWEB)

    Kotkin, G.L.; Serbo, V.G. [Novosibirsk State Univ. (Russian Federation). Phys. Dept.; Perlt, H. [Institut fuer Theoretische Physik, Leipzig University, 04109, Leipzig, BRD (Germany)

    1998-02-21

    When polarized electrons traverse a region where the laser light is focused their polarization varies even if their energy and direction of motion are not changed. This effect is due to interference of the incoming electron wave and an electron wave scattered at zero angle. Equations are obtained which determine the variation of the electron-density matrix, and their solutions are given. The change in the electron polarization depends not only on the Compton cross section but on the real part of the forward Compton amplitude as well. It should be taken into account, for example, in simulations of the e{yields}{gamma} conversion for future {gamma}{gamma} colliders. (orig.). 16 refs.

  17. Bremsstrahlung Energy Losses for Cosmic Ray Electrons and Positrons

    CERN Document Server

    Widom, A; Srivastava, R

    2015-01-01

    Recently cosmic ray electrons and positrons, i.e. cosmic ray charged leptons, have been observed. To understand the distances from our solar system to the sources of such lepton cosmic rays, it is important to understand energy losses from cosmic electrodynamic fields. Energy losses for ultra-relativistic electrons and/or positrons due to classical electrodynamic bremsstrahlung are computed. The energy losses considered are (i) due to Thompson scattering from fluctuating electromagnetic fields in the background cosmic thermal black body radiation and (ii) due to the synchrotron radiation losses from quasi-static domains of cosmic magnetic fields. For distances to sources of galactic length proportions, the lepton cosmic ray energy must be lass than about a TeV.

  18. Electron mean free path from angle-dependent photoelectron spectroscopy of aerosol particles

    CERN Document Server

    Goldmann, Maximilian; West, Adam H C; Yoder, Bruce L; Signorell, Ruth

    2015-01-01

    We propose angle-resolved photoelectron spectroscopy of aerosol particles as an alternative way to determine the electron mean free path of low energy electrons in solid and liquid materials. The mean free path is obtained from fits of simulated photoemission images to experimental ones over a broad range of different aerosol particle sizes. The principal advantage of the aerosol approach is twofold. Firstly, aerosol photoemission studies can be performed for many different materials, including liquids. Secondly, the size-dependent anisotropy of the photoelectrons can be exploited in addition to size-dependent changes in their kinetic energy. These finite size effects depend in different ways on the mean free path and thus provide more information on the mean free path than corresponding liquid jet, thin film, or bulk data. The present contribution is a proof of principle employing a simple model for the photoemission of electrons and preliminary experimental data for potassium chloride aerosol particles.

  19. Electronic transport of molecular nanowires by considering of electron hopping energy between the second neighbors

    Directory of Open Access Journals (Sweden)

    H Rabani

    2015-07-01

    Full Text Available In this paper, we study the electronic conductance of molecular nanowires by considering the electron hopping between the first and second neighbors with the help Green’s function method at the tight-binding approach. We investigate three types of structures including linear uniform and periodic chains as well as poly(p-phenylene molecule which are embedded between two semi-infinite metallic leads. The results show that in the second neighbor approximation, the resonance, anti-resonance and Fano phenomena occur in the conductance spectra of these structures. Moreover, a new gap is observed at edge of the lead energy band wich its width depends on the value of the electron hopping energy between the second neighbors. In the systems including intrinsic gap, this hopping energy shifts the gap in the energy spectra.

  20. Electron attachment to oxygen clusters studied with high energy resolution

    Science.gov (United States)

    Matejcik, S.; Stampfli, P.; Stamatovic, A.; Scheier, P.; Märk, T. D.

    1999-08-01

    Highly monochromatized electrons (with energy distributions of less than 30 meV FWHM) are used in a crossed beam experiments to investigate electron attachment to oxygen clusters (O2)n at electron energies from approximately zero eV up to several eV. At energies close to zero the attachment cross section for the reaction (O2)n+e→(O2)m- (for m=1, 2, and 3) rises strongly with decreasing electron energy compatible with s-wave electron capture to (O2)n. Peaks in the oxygen attachment cross sections present at higher energies (≈80 meV, 193 meV, 302 meV) can be ascribed to vibrational levels of the anion populated by attachment of an electron to a single oxygen molecule within the target cluster via a direct Franck-Condon transition from the ground vibrational state v=0 to a vibrational excited state v'=7,8,9,… of the anion produced. The vibrational structures observed here for the first time can be quantitatively accounted for by model calculations using a microscopic model to examine the attachment of an electron to an oxygen molecule inside a cluster. This involves (i) molecular dynamics simulations to calculate the structure of neutral clusters prior to the attachment process and (ii) calculation of the solvation energy of an oxygen anion in the cluster from the electrostatic polarization of the molecules of the cluster. The occurrence of this polarization energy at the surface of larger clusters explains the appearance of an s-wave capturing cross section at 0 eV and the slightly smaller spacings (compared to the monomer case) between the peaks at finite energy, as observed experimentally. The relative transition probabilities from the ground state of the neutral oxygen molecule to the different vibrational levels of the anion are obtained by calculating the corresponding Franck-Condon factors thereby resulting in a reasonable theoretical fit to the observed yields of negatively charged oxygen molecules and clusters.

  1. Towards understanding the influence of electron-gas interactions on imaging in an environmental TEM

    DEFF Research Database (Denmark)

    Wagner, Jakob Birkedal; Boothroyd, Chris; Beleggia, Marco

    2011-01-01

    The latest generation of environmental transmission electron microscopes (ETEMs) incorporates aberration correction and monochromation, allowing studies of chemical reactions and growth processes with improved spatial and spectral resolution. These additions to the columns of commercial ETEMs have...... be used. In the differential pumping approach, the gas is confined to the region around the specimen only by pressure-limiting apertures. In order to retain flexibility in the sample region, the pole piece gap and the highest pressure part of the column are relatively large (~7mm). As a result, electron...... by scattering from gas molecules. Furthermore, the electrons lose energy when they are scattered by gas molecules leading to a less isochromatic incident electron beam. Figure 2 shows a preliminary result of angle-resolved low-loss EELS acquired in the presence of 980 Pa of O2 in the absence of a specimen. Our...

  2. From electron energy-loss spectroscopy to multi-dimensional and multi-signal electron microscopy.

    Science.gov (United States)

    Colliex, Christian

    2011-01-01

    This review intends to illustrate how electron energy-loss spectroscopy (EELS) techniques in the electron microscope column have evolved over the past 60 years. Beginning as a physicist tool to measure basic excitations in solid thin foils, EELS techniques have gradually become essential for analytical purposes, nowadays pushed to the identification of individual atoms and their bonding states. The intimate combination of highly performing techniques with quite efficient computational tools for data processing and ab initio modeling has opened the way to a broad range of novel imaging modes with potential impact on many different fields. The combination of Angström-level spatial resolution with an energy resolution down to a few tenths of an electron volt in the core-loss spectral domain has paved the way to atomic-resolved elemental and bonding maps across interfaces and nanostructures. In the low-energy range, improved energy resolution has been quite efficient in recording surface plasmon maps and from them electromagnetic maps across the visible electron microscopy (EM) domain, thus bringing a new view to nanophotonics studies. Recently, spectrum imaging of the emitted photons under the primary electron beam and the spectacular introduction of time-resolved techniques down to the femtosecond time domain, have become innovative keys for the development and use of a brand new multi-dimensional and multi-signal electron microscopy.

  3. Energy Conversion Mechanism for Electron Perpendicular Energy in High Guide-Field Reconnection

    Science.gov (United States)

    Guo, Xuehan; Horiuchi, Ritoku; Kaminou, Yasuhiro; Cheng, Frank; Ono, Yasushi

    2016-10-01

    The energy conversion mechanism for electron perpendicular energy, both the thermal and the kinetic energy, is investigated by means of two-dimensional, full-particle simulations in an open system. It is shown that electron perpendicular heating is mainly due to the breaking of magnetic moment conservation in separatrix region because the charge separation generates intense variation of electric field within the electron Larmor radius. Meanwhile, electron perpendicular acceleration takes place manly due to the polarization drift term as well as the curvature drift term of E . u⊥ in the downstream near the X-point. The enhanced electric field due to the charge separation there results in a significant effect of the polarization drift term on the dissipation of magnetic energy within the ion inertia length in the downstream. Japan Society for the Promotion of Science (JSPS) Fellows 15J03758.

  4. High-power, narrow-band, high-repetition-rate, 5.9 eV coherent light source using passive optical cavity for laser-based angle-resolved photoelectron spectroscopy.

    Science.gov (United States)

    Omachi, J; Yoshioka, K; Kuwata-Gonokami, M

    2012-10-08

    We demonstrate a scheme for efficient generation of a 5.9 eV coherent light source with an average power of 23 mW, 0.34 meV linewidth, and 73 MHz repetition rate from a Ti: sapphire picosecond mode-locked laser with an output power of 1 W. Second-harmonic light is generated in a passive optical cavity by a BiB(3)O(6) crystal with a conversion efficiency as high as 67%. By focusing the second-harmonic light transmitted from the cavity into a β-BaB(2)O(4) crystal, we obtain fourth-harmonic light at 5.9 eV. This light source offers stable operation for at least a week. We discuss the suitability of the laser light source for high-resolution angle-resolved photoelectron spectroscopy by comparing it with other sources (synchrotron radiation facilities and gas discharge lamp).

  5. Metal-insulator transition and tunable Dirac-cone surface state in the topological insulator TlBi1 -xSbxTe2 studied by angle-resolved photoemission

    Science.gov (United States)

    Trang, Chi Xuan; Wang, Zhiwei; Yamada, Keiko; Souma, Seigo; Sato, Takafumi; Takahashi, Takashi; Segawa, Kouji; Ando, Yoichi

    2016-04-01

    We report a systematic angle-resolved photoemission spectroscopy on topological insulator (TI) TlBi1 -xSbxTe2 which is bulk insulating at 0.5 ≲x ≲0.9 and undergoes a metal-insulator-metal transition with the Sb content x . We found that this transition is characterized by a systematic hole doping with increasing x , which results in the Fermi-level crossings of the bulk conduction and valence bands at x ˜0 and x ˜1 , respectively. The Dirac point of the topological surface state is gradually isolated from the valence-band edge, accompanied by a sign reversal of Dirac carriers. We also found that the Dirac velocity is the largest among known solid-solution TI systems. The TlBi1 -xSbxTe2 system thus provides an excellent platform for Dirac-cone engineering and device applications of TIs.

  6. Modified Fermi Energy of Electrons in a Superhigh Magnetic Field

    CERN Document Server

    Zhu, C; Li, X D; Wang, N; Yuan, J P; Peng, Q H

    2016-01-01

    In this paper, we investigate the electron Landau-level stability and its influence on the electron Fermi energy, $E_{\\rm F}(e)$, in the circumstance of magnetars, which are powered by magnetic field energy. In a magnetar, the Landau levels of degenerate and relativistic electrons are strongly quantized. A new quantity $g_{n}$, the electron Landau-level stability coefficient is introduced. According to the requirement that $g_{n}$ decreases with increasing the magnetic field intensity $B$, the magnetic-field index $\\beta$ in the expression of $E_{\\rm F}(e)$ must be positive. By introducing the Dirac$-\\delta$ function, we deduce a general formulae for the Fermi energy of degenerate and relativistic electrons, and obtain a particular solution to $E_{\\rm F}(e)$ in a superhigh magnetic field. This solution has a low magnetic-field index of $\\beta=1/6$, compared with the previous one, and works when $\\rho\\geq 10^{7}$~g cm$^{-3}$ and $B_{\\rm cr}\\ll B\\leq 10^{17}$~Gauss. By modifying the phase space of relativistic ...

  7. Angle-resolved photoemission study of the evolution of band structure and charge density wave properties in RTe3 (R= Y, La, Ce, Sm, Gd, Tb and Dy)

    Energy Technology Data Exchange (ETDEWEB)

    Brouet, V.; Yang, W.L.; Zhou, X.J.; Hussain, Z.; Moore, R.G.; He, R.; Lu, D.H.; Shen, Z.X.; Laverock, J.; Dugdale, S.; Ru, N.; Fisher, I.R.

    2010-02-15

    We present a detailed ARPES investigation of the RTe{sub 3} family, which sets this system as an ideal 'textbook' example for the formation of a nesting driven Charge Density Wave (CDW). This family indeed exhibits the full range of phenomena that can be associated to CDW instabilities, from the opening of large gaps on the best nested parts of Fermi Surface (FS) (up to 0.4eV), to the existence of residual metallic pockets. ARPES is the best suited technique to characterize these features, thanks to its unique ability to resolve the electronic structure in k-space. An additional advantage of RTe{sub 3} is that the band structure can be very accurately described by a simple 2D tight-binding (TB) model, which allows one to understand and easily reproduce many characteristics of the CDW. In this paper, we first establish the main features of the electronic structure, by comparing our ARPES measurements with Linear Muffin-Tin Orbital band calculations. We use this to define the validity and limits of the TB model. We then present a complete description of the CDW properties and, for the first time, of their strong evolution as a function of R. Using simple models, we are able to reproduce perfectly the evolution of gaps in k-space, the evolution of the CDW wave vector with R and the shape of the residual metallic pockets. Finally, we give an estimation of the CDW interaction parameters and find that the change in the electronic density of states n(Ef), due to lattice expansion when different R ions are inserted, has the correct order of magnitude to explain the evolution of the CDW properties.

  8. Control System for Multi-energy Electron Irradiation Accelerator

    Institute of Scientific and Technical Information of China (English)

    ZHANG; Li-feng; LIU; Bao-jie

    2012-01-01

    <正>Multi-energy electron irradiation accelerator has a wide range of applications in areas such as industrial irradiation. Accelerator is operated under control system with accelerator subsystems, in which new technologies are involved, such as fiber-based network communication technology and PLC technology. The control system integrates pulse modulator systems,

  9. Electron Energy Level Statistics in Graphene Quantum Dots

    NARCIS (Netherlands)

    De Raedt, H.; Katsnellson, M. I.; Katsnelson, M.I.

    2008-01-01

    Motivated by recent experimental observations of size quantization of electron energy levels in graphene quantum dots [7] we investigate the level statistics in the simplest tight-binding model for different dot shapes by computer simulation. The results are in a reasonable agreement with the experi

  10. Probing Plasmonic Nanostructures with Electron Energy - Loss Spectroscopy

    DEFF Research Database (Denmark)

    Raza, Søren

    for nonlocal response. The experimental work comprises the use of electron energy-loss spectroscopy (EELS) to excite and study both localized and propagating surface plasmons in metal structures. Following a short introduction, we present the theoretical foundation to describe nonlocal response in Maxwell...

  11. An Energy Recovery Electron Linac On Ring Collider

    Energy Technology Data Exchange (ETDEWEB)

    Nikolitsa Merminga; Geoffrey Krafft; Valeri Lebedev; Ilan Ben-Zvi

    2001-09-01

    Electron-proton/ion colliders with center of mass energies between 14 GeV and 100 GeV (protons) or 63 GeV/A (ions) and luminosities at the 10{sup 33} (per nucleon) level have been proposed recently as a means for studying hadronic structure. Electron beam polarization appears to be crucial for many of the experiments. Two accelerator design scenarios have been examined in detail: colliding rings and recirculating linac-on-ring. Although the linac-on-ring scenario is not as well developed as the ring-ring scenario, comparable luminosities appear feasible. The linac-on-ring option presents significant advantages with respect to: (1) spin manipulations; (2) reduction of the synchrotron radiation load in the detectors; (3) a wide range of continuous energy variability. Rf power and beam dump considerations require that the electron linac recover the beam energy. This technology has been demonstrated at Jefferson Lab's IR FEL with cw current up to 5 mA and beam energy up to 50 MeV. Based on extrapolations from actual measurements and calculations, energy recovery is expected to be feasible at higher currents (a few hundred mA) and higher energies (a few GeV) as well. The report begins with a brief overview of Jefferson Lab's experience with energy recovery and summarize its benefits. Luminosity projections for the linac-ring scenario based on fundamental limitations are presented next. The feasibility of an energy recovery electron linac-on-proton ring collider is investigated and four conceptual point designs are shown corresponding to electron to proton energies of: 3 GeV on 15 GeV, 5 GeV on 50 GeV and 10 GeV on 250 GeV, and for gold ions with 100 GeV/A. The last two designs assume that the protons or ions are stored in the existing RHIC accelerator. Accelerator physics issues relevant to proton rings and energy recovery linacs are discussed next and a list of required R and D for the realization of such a design is presented.

  12. Preliminary investigations on high energy electron beam tomography

    Energy Technology Data Exchange (ETDEWEB)

    Baertling, Yves; Hoppe, Dietrich; Hampel, Uwe

    2010-12-15

    In computed tomography (CT) cross-sectional images of the attenuation distribution within a slice are created by scanning radiographic projections of an object with a rotating X-ray source detector compound and subsequent reconstruction of the images from these projection data on a computer. CT can be made very fast by employing a scanned electron beam instead of a mechanically moving X-ray source. Now this principle was extended towards high-energy electron beam tomography with an electrostatic accelerator. Therefore a dedicated experimental campaign was planned and carried out at the Budker Institute of Nuclear Physics (BINP), Novosibirsk. There we investigated the capabilities of BINP's accelerators as an electron beam generating and scanning unit of a potential high-energy electron beam tomography device. The setup based on a 1 MeV ELV-6 (BINP) electron accelerator and a single detector. Besides tomographic measurements with different phantoms, further experiments were carried out concerning the focal spot size and repeat accuracy of the electron beam as well as the detector's response time and signal to noise ratio. (orig.)

  13. Ultra High Energy Electrons Powered by Pulsar Rotation

    CERN Document Server

    Mahajan, Swadesh; Osmanov, Zaza; Chkheidze, Nino

    2013-01-01

    A new mechanism of particle acceleration to ultra high energies, driven by the rotational slow down of a pulsar (Crab pulsar, for example), is explored. The rotation, through the time dependent centrifugal force, can very efficiently excite unstable Langmuir waves in the e-p plasma of the star magnetosphere via a parametric process. These waves, then, Landau damp on electrons accelerating them in the process. The net transfer of energy is optimal when the wave growth and the Landau damping times are comparable and are both very short compared to the star rotation time. We show, by detailed calculations, that these are precisely the conditions for the parameters of the Crab pulsar. This highly efficient route for energy transfer allows the electrons in the primary beam to be catapulted to multiple TeV ($\\sim 100$ TeV) and even PeV energy domain. It is expected that the proposed mechanism may, partially, unravel the puzzle of the origin of ultra high energy cosmic ray electrons.

  14. Power Electronics for Renewable Energy Systems - Status and Trends

    DEFF Research Database (Denmark)

    Blaabjerg, Frede; Ma, Ke; Yang, Yongheng

    2014-01-01

    electronics in generation, transmission/distribution and end-user application, together with advanced controls, can pave the way for renewable energy resources. In view of this, some of the most promising renewable candidates like wind power and photovoltaic, which are becoming a significant part...... in the electricity production, are explored in this paper. Issues like technology demands, power converter topologies, and control structures are addressed. Some special focuses are also paid on the emerging trends in power electronics development for those systems....... and use of the energy to be as technological efficient as possible, and incentives to save energy at the end-user should also be strengthened. In order to realize the transition smoothly and effectively, power conversion systems will continue to play an essential role. Using highly efficient power...

  15. Controlled cooling of an electronic system for reduced energy consumption

    Science.gov (United States)

    David, Milnes P.; Iyengar, Madhusudan K.; Schmidt, Roger R.

    2016-08-09

    Energy efficient control of a cooling system cooling an electronic system is provided. The control includes automatically determining at least one adjusted control setting for at least one adjustable cooling component of a cooling system cooling the electronic system. The automatically determining is based, at least in part, on power being consumed by the cooling system and temperature of a heat sink to which heat extracted by the cooling system is rejected. The automatically determining operates to reduce power consumption of the cooling system and/or the electronic system while ensuring that at least one targeted temperature associated with the cooling system or the electronic system is within a desired range. The automatically determining may be based, at least in part, on one or more experimentally obtained models relating the targeted temperature and power consumption of the one or more adjustable cooling components of the cooling system.

  16. Numerically fitting the electron Fermi energy and the electron fraction in a neutron star

    Science.gov (United States)

    Li, Xing Hu; Gao, Zhi Fu; Li, Xiang Dong; Xu, Yan; Wang, Pei; Wang, Na; Peng, Qiu He

    2016-10-01

    Based on the basic definition of the Fermi energy of degenerate and relativistic electrons, we obtain a special solution to the electron Fermi energy, EF(e), and express EF(e) as a function of the electron fraction, Ye, and matter density, ρ. We obtain several useful analytical formula for Ye and ρ within classical models and the work of Dutra et al. (2014) (Type-2) in relativistic mean-field theory are obtained using numerically fitting. When describing the mean-field Lagrangian, density, we adopt the TMA parameter set, which is remarkably consistent with the updated astrophysical observations of neutron stars (NSs). Due to the importance of the density dependence of the symmetry energy, J, in nuclear astrophysics, a brief discussion on J and its slop is presented. Combining these fitting formula with boundary conditions for different density regions, we can evaluate the value of EF(e) in any given matter density, and obtain a schematic diagram of EF(e) as a continuous function of ρ. Compared with previous studies on the electron Fermi energy in other studies models, our methods of calculating EF(e) are more simple and convenient, and can be universally suitable for the relativistic electron regions in the circumstances of common neutron stars. We have deduced a general expression of EF(e) and ne, which could be used to indirectly test whether one equation of state of a NS is correct in our future studies on neutron star matter properties. Since URCA reactions are expected in the center of a massive star due to high-value electron Fermi energy and electron fraction, this study could be useful in the future studies on the NS thermal evolution.

  17. High energy electron processing of icy regoliths on Saturn's moons

    Science.gov (United States)

    Schaible, Micah; Johnson, Robert E.

    2015-11-01

    A unique space weathering phenomenon has been identified on several icy Saturnian moons. Cassini revealed anomalous lens shaped regions in both optical and thermal wavelengths, colloquially known as the 'PacMan' feature, which are centered on the leading hemispheres and approximately symmetric about the equators. In particular, the Cassini InfraRed Spectrometer (CIRS) measurements of thermal emission in the mid-IR showed that surface temperature variations during a diurnal cycle were smaller inside the anomalous regions. The locations of the anomalies were shown to closely match the expected deposition profile of high energy (~ MeV) electrons moving counter rotational to the moons, suggesting an energetic source to drive their formation. However, the mechanisms by which thermal conductivity enhancement occur lack quantitative comparison with theoretical and experimental results.Electron interactions with the grains can excite molecules, which, if near enough to an intergrain contact, can cause atoms or molecules to migrate into the contact region, thus increasing the contact volume or 'sintering' the grains. Sintering improves the thermal contact between grains, leading to increased effective thermal conductivity of the regolith. Equations previously developed to describe material behavior in nuclear reactor were used to estimate the timescale for the energetic electrons to increase the contact volume sufficiently to describe the enhanced thermal conductivity of the anomalous regions. In order to properly constrain the sintering calculations, the unique electron energy distribution measured in the vicinity of each of the moons was used in the calculations, and molecular dynamics simulations of excited electrons in water ice were carried out to determine the length scale for an average electron excitation or ionization event. This length scale determines the distance from the primary reaction at which electrons can still be mobilized to move into the contact region

  18. Energy transfer from lower energy to higher-energy electrons mediated by whistler waves in the radiation belts

    Science.gov (United States)

    Shklyar, D. R.

    2017-01-01

    We study the problem of energy exchange between waves and particles, which leads to energization of the latter, in an unstable plasma typical of the radiation belts. The ongoing Van Allen Probes space mission brought this problem among the most discussed in space physics. A free energy which is present in an unstable plasma provides the indispensable condition for energy transfer from lower energy particles to higher-energy particles via resonant wave-particle interaction. This process is studied in detail by the example of electron interactions with whistler mode wave packets originated from lightning-induced emission. We emphasize that in an unstable plasma, the energy source for electron energization is the energy of other particles, rather than the wave energy as is often assumed. The way by which the energy is transferred from lower energy to higher-energy particles includes two processes that operate concurrently, in the same space-time domain, or sequentially, in different space-time domains, in which a given wave packet is located. In the first process, one group of resonant particles gives the energy to the wave. The second process consists in wave absorption by another group of resonant particles, whose energy therefore increases. We argue that this mechanism represents an efficient means of electron energization in the radiation belts.

  19. Asymmetric electron energy sharing in electron-impact double ionization of helium

    Science.gov (United States)

    Silenou Mengoue, M.; Tetchou Nganso, H. M.

    2016-12-01

    We present the fully fivefold differential cross sections (FDCSs) for (e ,3 e ) processes in helium within the first Born approximation. The calculation is performed for a coplanar geometry in which the incident electron is fast (˜6 keV), the momentum transfer is small (0.24 a.u.), and for an asymmetric energy sharing between both slow ejected electrons at excess energy of 20 eV. Two cases have been considered: E1=15 eV, E2=5 eV and E1=8 eV, E2=12 eV. While waiting for new theoretical and experimental results for confrontations, in particular for asymmetric energy sharing, our results clearly demonstrate that, for the same incident energy, the same momentum transfer and the same excess energy, the (e ,3 e ) process in helium with asymmetric energy sharing between ejected electrons is more likely than the case with symmetric energy sharing. The two- and three-dimensional representation of the FDCSs covering all possible values of the angle of ejections are presented and discussed. The theoretical cross sections are calculated by using a compact-kernel-integral-equation approach associated with the Jacobi matrix method to calculate a three-body wave function and which leads to a full convergence in terms of the basis size.

  20. Detailed Monte Carlo Simulation of electron transport and electron energy loss spectra.

    Science.gov (United States)

    Attarian Shandiz, M; Salvat, F; Gauvin, R

    2016-11-01

    A computer program for detailed Monte Carlo simulation of the transport of electrons with kinetic energies in the range between about 0.1 and about 500 keV in bulk materials and in thin solid films is presented. Elastic scattering is described from differential cross sections calculated by the relativistic (Dirac) partial-wave expansion method with different models of the scattering potential. Inelastic interactions are simulated from an optical-data model based on an empirical optical oscillator strength that combines optical functions of the solid with atomic photoelectric data. The generalized oscillator strength is built from the adopted optical oscillator strength by using an extension algorithm derived from Lindhard's dielectric function for a free-electron gas. It is shown that simulated backscattering fractions of electron beams from bulk (semi-infinite) specimens are in good agreement with experimental data for beam energies from 0.1 keV up to about 100 keV. Simulations also yield transmitted and backscattered fractions of electron beams on thin solid films that agree closely with measurements for different film thicknesses and incidence angles. Simulated most probable deflection angles and depth-dose distributions also agree satisfactorily with measurements. Finally, electron energy loss spectra of several elemental solids are simulated and the effects of the beam energy and the foil thickness on the signal to background and signal to noise ratios are investigated. SCANNING 38:475-491, 2016. © 2015 Wiley Periodicals, Inc.

  1. Whole body irradiation by high energy electron for mycosis fungoides

    Energy Technology Data Exchange (ETDEWEB)

    Koga, Kenji; Nishikawa, Kiyoshi; Wakuta, Yuhji; Asada, Keiko; Murai, Nobuko; Watanabe, Katsushi; Takada, Takuo

    1985-02-01

    Five patients with mycosis fungoides were treated with whole body irradiation by high energy electron. They were irradiated by a linear accelerator (ML-15MIII, Mitsubishi Company) with the electron of 8 MeV, using the acrylics decelerator at the window to reduce the electron energy. Source skin distance was 150 cm and three beams with a separation of 60 cm were used. The dose distribution at the skin surface was within homogeneity of +-7.5%. The 2 patients have been alive without evidence of disease for 2 years, and 1 year and half after the treatment, respectively. Three patients were dead; two of the dead were associated with pancytopenia, one irradiated 6 times for 2 years and 4 months and the other 3 times for 2 years. The remaining one patient developed the brain metastasis without skin lesions 6 months later. Our results suggest that mycosis fungoides is curable in infiltrative stage, but not in tumorous stage. Some discussion on the problem of this treatment technique and haematological changes caused by the contaminated X-ray as well as high energy electron were made, reviewing the pertinent literatures on the device to reduce the contaminated X-ray. (author).

  2. Low-Energy Electron Scattering by Sugarcane Lignocellulosic Biomass Molecules

    Science.gov (United States)

    Oliveira, Eliane; Sanchez, Sergio; Bettega, Marcio; Lima, Marco; Varella, Marcio

    2012-06-01

    The use of second generation (SG) bioethanol instead of fossil fuels could be a good strategy to reduce greenhouse gas emissions. However, the efficient production of SG bioethanol has being a challenge to researchers around the world. The main barrier one must overcome is the pretreatment, a very important step in SG bioethanol aimed at breaking down the biomass and facilitates the extraction of sugars from the biomass. Plasma-based treatment, which can generate reactive species, could be an interesting possibility since involves low-cost atmospheric-pressure plasma. In order to offer theoretical support to this technique, the interaction of low-energy electrons from the plasma with biomass is investigated. This study was motived by several works developed by Sanche et al., in which they understood that DNA damage arises from dissociative electron attachment, a mechanism in which electrons are resonantly trapped by DNA subunits. We will present elastic cross sections for low-energy electron scattering by sugarcane biomass molecules, obtained with the Schwinger multichannel method. Our calculations indicate the formation of π* shape resonances in the lignin subunits, while a series of broad and overlapping σ* resonances are found in cellulose and hemicellulose subunits. The presence of π* and σ* resonances could give rise to direct and indirect dissociation pathways in biomass. Then, theoretical resonance energies can be useful to guide the plasma-based pretreatment to break down specific linkages of interest in biomass.

  3. Energy Dependence of SEP Electron and Proton Onset Times

    CERN Document Server

    Xie, Hong; Gopalswamy, Nat; Cyr, Orville St

    2016-01-01

    We study the large solar energetic particle (SEP) events that were detected by GOES in the $>$ 10 MeV energy channel during December 2006 to March 2014. We derive and compare solar particle release (SPR) times for the 0.25--10.4 MeV electrons and 10--100 MeV protons for the 28 SEP events. In the study, the electron SPR times are derived with the time-shifting analysis (TSA) and the proton SPR times are derived using both the TSA and the velocity dispersion analysis (VDA). Electron anisotropies are computed to evaluate the amount of scattering for the events under study. Our main results include: 1)near-relativistic electrons and high-energy protons are released at the same time within 8 min for most (16 of 23) SEP events. 2)There exists a good correlation between electron and proton acceleration, peak intensity and intensity time profiles. 3) The TSA SPR times for 90.5 MeV and 57.4 MeV protons have maximum errors of 6 min and 10 min compared to the proton VDA release times, respectively, while the maximum err...

  4. Chiral asymmetry in the angle-resolved O and C 1s-1 core photoemissions of the R enantiomer of glycidol

    Science.gov (United States)

    Powis, Ivan; Harding, Chris J.; Barth, Silko; Joshi, Sanjeev; Ulrich, Volker; Hergenhahn, Uwe

    2008-11-01

    We present measurements of a photoelectron circular dichroism in photoionization from O and C 1s core levels, of the R enantiomer of glycidol (C3H6O2) in the gas phase. This dichroism emerges from a forward-backward asymmetry in the angular distribution of electrons created on ionization with circularly polarized synchrotron radiation and is already fully present in the pure electric dipole approximation. Asymmetry factors obtained for the core levels in this study range up to a few percent, but it is likely that these values are limited by a failure to resolve photoemission from individual atomic sites. Theoretical modeling is provided to examine possible differences between these alternative atomic photoemission sites, and between different conformational structures of glycidol. The calculated chiral angular distribution parameters that support the circular dichroism display a much enhanced sensitivity to the molecular conformation compared to the conventional photoionization cross section and the β parameter. Likely conformer structures can be suggested after comparison with the experiment.

  5. Very Low Energy Electron Scattering from Ozone and Chlorine Dioxide

    Science.gov (United States)

    Gulley, R. J.; Field, T. A.; Steer, W. A.; Mason, N. J.; Ziesel, J. P.; Lunt, S. L.; Field, D.

    1998-10-01

    Total cross-sections are reported for the scattering of electrons from ozone (O_3) and chlorine dioxide (OClO) for energies in the range of 9 meV to 10 eV. The measurements were made in transmission experiments using a synchrotron photoionization apparatus with an energy resolution in the incident electron beam of ~ 3.5 meV (FWHM). The cross section for O3 shows strong rotational scattering at low energy, through the presence of the permanent dipole moment of O_3. Superposed on this strong scattering signal, there is evidence of a weak structure around 50 meV associated with dissociative attachment. A shape resonance, known from earlier work at ~ 4 meV, is also observed. Electron scattering from OClO is dominated by rotationally inelastic scattering decreasing from a peak at essentially zero eV to an energy of 40 meV, where p-wave attachment becomes more important, peaking at 50--60 meV and extending to several hundred meV.

  6. Low-energy electron scattering from molecules, biomolecules and surfaces

    CERN Document Server

    Carsky, Petr

    2011-01-01

    Since the turn of the 21st century, the field of electron molecule collisions has undergone a renaissance. The importance of such collisions in applications from radiation chemistry to astrochemistry has flowered, and their role in industrial processes such as plasma technology and lighting are vital to the advancement of next generation devices. Furthermore, the development of the scanning tunneling microscope highlights the role of such collisions in the condensed phase, in surface processing, and in the development of nanotechnology.Low-Energy Electron Scattering from Molecules, Biomolecule

  7. Probing Battery Chemistry with Liquid Cell Electron Energy Loss Spectroscopy

    Energy Technology Data Exchange (ETDEWEB)

    Unocic, Raymond R.; Baggetto, Loic; Veith, Gabriel M.; Aguiar, Jeffery A.; Unocic, Kinga A.; Sacci, Robert L.; Dudney, Nancy J.; More, Karren L.

    2015-11-25

    We demonstrate the ability to apply electron energy loss spectroscopy (EELS) to follow the chemistry and oxidation states of LiMn2O4 and Li4Ti5O12 battery electrodes within a battery solvent. The use and importance of in situ electrochemical cells coupled with a scanning/transmission electron microscope (S/TEM) has expanded and been applied to follow changes in battery chemistry during electrochemical cycling. Furthermore, we discuss experimental parameters that influence measurement sensitivity and provide a framework to apply this important analytical method to future in situ electrochemical studies.

  8. Weissenberg reflection high-energy electron diffraction for surface crystallography.

    Science.gov (United States)

    Abukawa, Tadashi; Yamazaki, Tomoyuki; Yajima, Kentaro; Yoshimura, Koji

    2006-12-15

    The principle of a Weissenberg camera is applied to surface crystallographic analysis by reflection high-energy electron diffraction. By removing inelastic electrons and measuring hundreds of patterns as a function of sample rotation angle phi, kinematical analysis can be performed over a large volume of reciprocal space. The data set is equivalent to a three-dimensional stack of Weissenberg photographs. The method is applied to analysis of an Si(111)-square root of 3 x square root of 3-Ag surface, and the structural data obtained are in excellent agreement with the known atomic structure.

  9. Electron energy-loss spectroscopy study of hydrogenated amorphous silicon

    Energy Technology Data Exchange (ETDEWEB)

    Burnham, N.A.; Fisher, R.F.; Asher, S.E.; Kazmerski, L.L.

    1987-07-01

    Electron energy-loss spectroscopy is used to study hydrogenated amorphous silicon (a-Si:H). Core-level and plasma excitations were examined as a function of hydrogen content. This technique and its interpretation reveals a consistent picture of the electron excitations within this important material. The a-Si:H thin films were fabricated by rf sputtering. Their hydrogen concentrations ranged from 0% to 15%. Hydrogen content was determined by infrared spectroscopy and secondary ion mass spectroscopy. X-ray photoelectron spectroscopy and inspection of the silicon Auger-KLL peak confirmed the silicon core levels.

  10. Electron thermal self-energy in a magnetic field

    CERN Document Server

    Persson, D

    1995-01-01

    Using the general form of the static energy solutions to the Dirac equation with a magnetic field, we calculate a general self-energy matrix in the Furry-picture. In the limit of high temperatures, but even higher magnetic fields, a self-consistent dispersion relation is solved. In contrast to the high temperature limit, this merely results in a small mass shift. The electron anomalous magnetic moment is calculated. The contribution from thermal fermions is found to be different from the corresponding contribution using perturbation theory and plane-wave external states. In the low temperature limit the self-energy is shown to exhibit de Haas--van Alphen oscillations. In the limit of low temperatures and high densities, the self-energy becomes very large.

  11. Electron energy-loss spectroscopy of coupled plasmonic systems: beyond the standard electron perspective

    Science.gov (United States)

    Bernasconi, G. D.; Flauraud, V.; Alexander, D. T. L.; Brugger, J.; Martin, O. J. F.; Butet, J.

    2016-09-01

    Electron energy-loss spectroscopy (EELS) has become an experimental method of choice for the investigation of localized surface plasmon resonances, allowing the simultaneous mapping of the associated field distributions and their resonant energies with a nanoscale spatial resolution. The experimental observations have been well-supported by numerical models based on the computation of the Lorentz force acting on the impinging electrons by the scattered field. However, in this framework, the influence of the intrinsic properties of the plasmonic nanostructures studied with the electron energy-loss (EEL) measurements is somehow hidden in the global response. To overcome this limitation, we propose to go beyond this standard, and well-established, electron perspective and instead to interpret the EELS data using directly the intrinsic properties of the nanostructures, without regard to the force acting on the electron. The proposed method is particularly well-suited for the description of coupled plasmonic systems, because the role played by each individual nanoparticle in the observed EEL spectrum can be clearly disentangled, enabling a more subtle understanding of the underlying physical processes. As examples, we consider different plasmonic geometries in order to emphasize the benefits of this new conceptual approach for interpreting experimental EELS data. In particular, we use it to describe results from samples made by traditional thin film patterning and by arranging colloidal nanostructures.

  12. LDRD project 151362 : low energy electron-photon transport.

    Energy Technology Data Exchange (ETDEWEB)

    Kensek, Ronald Patrick; Hjalmarson, Harold Paul; Magyar, Rudolph J.; Bondi, Robert James; Crawford, Martin James

    2013-09-01

    At sufficiently high energies, the wavelengths of electrons and photons are short enough to only interact with one atom at time, leading to the popular %E2%80%9Cindependent-atom approximation%E2%80%9D. We attempted to incorporate atomic structure in the generation of cross sections (which embody the modeled physics) to improve transport at lower energies. We document our successes and failures. This was a three-year LDRD project. The core team consisted of a radiation-transport expert, a solid-state physicist, and two DFT experts.

  13. Narrow beam dosimetry for high-energy hadrons and electrons

    CERN Document Server

    Pelliccioni, M; Ulrici, Luisa

    2001-01-01

    Organ doses and effective dose were calculated with the latest version of the Monte Carlo transport code FLUKA in the case of an anthropomorphic mathematical model exposed to monoenergetic narrow beams of protons, pions and electrons in the energy range 10°— 400 GeV. The target organs considered were right eye, thyroid, thymus, lung and breast. Simple scaling laws to the calculated values are given. The present data and formula should prove useful for dosimetric estimations in case of accidental exposures to high-energy beams.

  14. Narrow beam dosimetry for high energy hadrons and electrons.

    Science.gov (United States)

    Pelliccioni, M; Silari, M; Ulrici, L

    2001-01-01

    Organ doses and effective dose were calculated with the latest version of the Monte Carlo transport code FLUKA in the case of an anthropomorphic mathematical model exposed to monoenergetic narrow beams of protons, pions and electrons in the energy range 10-400 GeV. The target organs considered were right eye, thyroid, thymus, lung and breast. Simple scaling laws to the calculated values are given. The present data and formulae should prove useful for dosimetric estimations in the case of accidental exposures to high energy beams.

  15. Low-Energy Electron Beam Direct Writing Equipment

    Science.gov (United States)

    Fuse, Takashi; Ando, Atsushi; Kotsugi, Tadashi; Kinoshita, Hidetoshi; Sugihara, Kazuyoshi

    2007-09-01

    We proposed an electron beam direct writing (EBDW) system capable of high throughput and maskless operation based on a novel concept of using both low-energy electron beam (EB) and character projection (CP) system. We fabricated an EB optical column of low-energy EBDW equipment and obtained a resist pattern. We also investigated the beam blur and line width roughness (LWR) of lines and spaces (L/S) formed on a resist to change various EB current densities and convergence half angles. The obtained results show that a Coulomb interaction effect markedly affects the beam blur in our EB optical column. Thus, we reduce the number of sources caused by LWR and developed photoresists to obtain small LWR L/S patterns for achieving a high throughput.

  16. National energy use of consumer electronics in 1999

    Energy Technology Data Exchange (ETDEWEB)

    Rosen, Karen; Meier, Alan; Zandelin, Stefan

    2000-02-15

    The major consumer electronics in U.S. homes accounted for nearly 7 percent of U.S. residential electricity consumption in 1999. We attribute more than half of this figure (3.6 percent) to televisions, videocassette recorders, and DVD players, and nearly one-third (1.8 percent) to audio products. Set-top boxes currently account for a relatively small fraction of residential electricity use (0.7 percent), but we expect this end-use to grow quickly with the proliferation of digital set-top boxes, which currently use 40 percent more energy per unit than the average TV set. In all, these consumer electronics plus telephone products consumed 75 TWh in the U.S. in 1999, half of which was consumed while the products were not in use. This energy use is expected to grow as products with new or advanced functionality hit the market.

  17. Excitation of the lowest electronic transitions in ethanol by low-energy electrons

    Science.gov (United States)

    Hargreaves, L. R.; Khakoo, M. A.; Winstead, C.; McKoy, V.

    2016-09-01

    We report absolute differential and integral cross sections for electronic excitation of ethanol, by low-energy electron impact. Cross sections for low-lying excited states were measured at incident electron energies from 9 to 20 eV and at scattering angles from {5}\\circ through {130}\\circ . Our results include cross sections for excitation of the 1{}3A\\prime \\prime and 1{}1A\\prime \\prime states as well as for the 2{}3A\\prime \\prime + 1{}3A\\prime and 2{}1A\\prime \\prime + 2{}1A\\prime cross section sums. Corresponding calculations were also performed using the Schwinger multichannel method, within an 11-channel close-coupling scheme.

  18. New stopping power formula for intermediate energy electrons.

    Science.gov (United States)

    Gümüş, Hasan

    2008-12-01

    This study presents a new stopping power (SP) formula for electrons. In the modified Bethe-Bloch SP expression, analytical expressions for the effective charge and effective mean excitation energies (EMEE) of target atoms are used, while for the effective charge of incoming electrons, Sugiyama's semiempirical formula from Peterson and Green is used. An analytical expression for practical SP calculations is obtained using the Bethe approximation and a Thomas-Fermi model of the atom. The calculated results of the SP for electrons in some materials, such as H(2)O, H(2), CO(2), N(2), and O(2), are compared with experimental data, together with Penelope code results and a number of other semiempirical and analytical calculations.

  19. Electron energy-loss spectroscopy of branched gap plasmon resonators

    Science.gov (United States)

    Raza, Søren; Esfandyarpour, Majid; Koh, Ai Leen; Mortensen, N. Asger; Brongersma, Mark L.; Bozhevolnyi, Sergey I.

    2016-12-01

    The miniaturization of integrated optical circuits below the diffraction limit for high-speed manipulation of information is one of the cornerstones in plasmonics research. By coupling to surface plasmons supported on nanostructured metallic surfaces, light can be confined to the nanoscale, enabling the potential interface to electronic circuits. In particular, gap surface plasmons propagating in an air gap sandwiched between metal layers have shown extraordinary mode confinement with significant propagation length. In this work, we unveil the optical properties of gap surface plasmons in silver nanoslot structures with widths of only 25 nm. We fabricate linear, branched and cross-shaped nanoslot waveguide components, which all support resonances due to interference of counter-propagating gap plasmons. By exploiting the superior spatial resolution of a scanning transmission electron microscope combined with electron energy-loss spectroscopy, we experimentally show the propagation, bending and splitting of slot gap plasmons.

  20. Electron Beam Energy Compensation by Controlling RF Pulse Shape

    CERN Document Server

    Kii, T; Kusukame, K; Masuda, K; Nakai, Y; Ohgaki, H; Yamazaki, T; Yoshikawa, K; Zen, H

    2005-01-01

    We have studied on improvement of electron beam macropulse properties from a thermionic RF gun. Though a thermionic RF gun has many salient features, there is a serious problem that back-bombardment effect worsens quality of the beam. To reduce beam energy degradation by this effect, we tried to feed non-flat RF power into the gun. As a result, we successfully obtained about 1.5 times longer macropulse and two times larger total charge per macropulse. On the other hand, we calculated transient evolution of RF power considering non-constant beam loading. The beam loading is evaluated from time evolution of cathode temperature, by use of one dimensional heat conduction model and electron trajectories' calculations by a particle simulation code. Then we found good agreement between the experimental and calculation results. Furthermore, with the same way, we studied the electron beam output dependence on the cathode radius.

  1. Parity nonconservation in polarized electron scattering at high energies

    Energy Technology Data Exchange (ETDEWEB)

    Prescott, C.Y.

    1979-10-01

    Recent observations of parity violation in inelastic scattering of electrons at high energy is discussed with reference to the process e(polarized) + D(unpolarized) ..-->.. e + X. The kinetics of this process, the idealized case of scattering from free quark targets, experimental techniques and results, and relations to atomic physics of parity violation in bismuth and thallium atoms with a model independent analysis. 17 references. (JFP)

  2. Nanobiotechnology in energy, environment and electronics methods and applications

    CERN Document Server

    Nicolini, Claudio

    2015-01-01

    Introduction: Present Challenges and Future Solutions via Nanotechnology for Electronics, Environment and Energy; Claudio NicoliniPart A: MethodsInfluence of Chromosome Translocation on Yeast Life Span: Implications for Long-Term Industrial Biofermentation; Jason Sims, Dmitri Nikitin, and Carlo V. BruschiPulsed Power Nanotechnologies for Disintegration and Breaking Up of Refractory Precious Metals Ores; Valentin A. Chanturiya and Igor Zh. BuninModeling of Software Sensors in Bioprocess; Luca Belmonte and Claudio NicoliniN

  3. Nanocellulose as Material Building Block for Energy and Flexible Electronics

    Science.gov (United States)

    Hu, Liangbing

    2014-03-01

    In this talk, I will discuss the fabrications, properties and device applications of functional nanostructured paper based on nanocellulose. Nanostructures with tunable optical, electrical, ionic and mechanical properties will be discussed. Lab-scale demonstration devices, including low-cost Na-ion batteries, microbial fuel cells, solar cells, transparent transistors, actuators and touch screens will be briefly mentioned. These studies show that nanocellulose is a promising green material for electronics and energy devices.

  4. Structural and electronic properties of V2O3 ultrathin film on Ag(001): LEED and photoemission study

    Science.gov (United States)

    Kundu, Asish K.; Menon, Krishnakumar S. R.

    2016-05-01

    V2O3 ultrathin films were grown on Ag(001) substrate by reactive evaporation of vanadium (V) metal in presence of oxygen and their structural and electronic properties were studied by Low Energy Electron Diffraction (LEED), X-ray Photo Electron Spectroscopy (XPS) and Angle Resolved Photoemission Spectroscopic (ARPES) techniques, respectively. On top of square symmetry substrate Ag(001), hexagonal surface of V2O3 (0001) is stabilized in the form of two domain structure, rotated by 30°(or 90°)to each other, has been observed by LEED. Rather than epitaxial flat monolayer, formation of well-ordered V2O3 (0001) island has been confirmed from the LEED and the Photoemission Spectroscopic (PES) study. Stoichiometry of the grown film was confirmed by the XPS study. Evolution of valance band electronic structure of V2O3 (0001) surface has been studied as a function of film thickness by ARPES.

  5. Electronic and optical properties of Fe, Pd, and Ti studied by reflection electron energy loss spectroscopy

    Energy Technology Data Exchange (ETDEWEB)

    Tahir, Dahlang [Department of Physics, Hasanuddin University, Makassar 90245 (Indonesia); Kraaer, Jens; Tougaard, Sven [Department of Physics, Chemistry, and Pharmacy, University of Southern Denmark, DK-5230 Odense M (Denmark)

    2014-06-28

    We have studied the electronic and optical properties of Fe, Pd, and Ti by reflection electron energy-loss spectroscopy (REELS). REELS spectra recorded for primary energies in the range from 300 eV to 10 keV were corrected for multiple inelastically scattered electrons to determine the effective inelastic-scattering cross section. The dielectric functions and optical properties were determined by comparing the experimental inelastic-electron scattering cross section with a simulated cross section calculated within the semi-classical dielectric response model in which the only input is Im(−1/ε) by using the QUEELS-ε(k,ω)-REELS software package. The complex dielectric functions ε(k,ω), in the 0–100 eV energy range, for Fe, Pd, and Ti were determined from the derived Im(−1/ε) by Kramers-Kronig transformation and then the refractive index n and extinction coefficient k. The validity of the applied model was previously tested and found to give consistent results when applied to REELS spectra at energies between 300 and 1000 eV taken at widely different experimental geometries. In the present paper, we provide, for the first time, a further test on its validity and find that the model also gives consistent results when applied to REELS spectra in the full range of primary electron energies from 300 eV to 10000 eV. This gives confidence in the validity of the applied method.

  6. Simulating electron energy loss spectroscopy with the MNPBEM toolbox

    Science.gov (United States)

    Hohenester, Ulrich

    2014-03-01

    Within the MNPBEM toolbox, we show how to simulate electron energy loss spectroscopy (EELS) of plasmonic nanoparticles using a boundary element method approach. The methodology underlying our approach closely follows the concepts developed by García de Abajo and coworkers (Garcia de Abajo, 2010). We introduce two classes eelsret and eelsstat that allow in combination with our recently developed MNPBEM toolbox for a simple, robust, and efficient computation of EEL spectra and maps. The classes are accompanied by a number of demo programs for EELS simulation of metallic nanospheres, nanodisks, and nanotriangles, and for electron trajectories passing by or penetrating through the metallic nanoparticles. We also discuss how to compute electric fields induced by the electron beam and cathodoluminescence. Catalogue identifier: AEKJ_v2_0 Program summary URL:http://cpc.cs.qub.ac.uk/summaries/AEKJ_v2_0.html Program obtainable from: CPC Program Library, Queen’s University, Belfast, N. Ireland Licensing provisions: Standard CPC licence, http://cpc.cs.qub.ac.uk/licence/licence.html No. of lines in distributed program, including test data, etc.: 38886 No. of bytes in distributed program, including test data, etc.: 1222650 Distribution format: tar.gz Programming language: Matlab 7.11.0 (R2010b). Computer: Any which supports Matlab 7.11.0 (R2010b). Operating system: Any which supports Matlab 7.11.0 (R2010b). RAM:≥1 GB Classification: 18. Catalogue identifier of previous version: AEKJ_v1_0 Journal reference of previous version: Comput. Phys. Comm. 183 (2012) 370 External routines: MESH2D available at www.mathworks.com Does the new version supersede the previous version?: Yes Nature of problem: Simulation of electron energy loss spectroscopy (EELS) for plasmonic nanoparticles. Solution method: Boundary element method using electromagnetic potentials. Reasons for new version: The new version of the toolbox includes two additional classes for the simulation of electron energy

  7. Vibrational and Electronic Energy Transfer and Dissociation of Diatomic Molecules by Electron Collisions

    Science.gov (United States)

    Huo, Winifred M.; Langhoff, Stephen R. (Technical Monitor)

    1995-01-01

    At high altitudes and velocities equal to or greater than the geosynchronous return velocity (10 kilometers per second), the shock layer of a hypersonic flight will be in thermochemical nonequilibrium and partially ionized. The amount of ionization is determined by the velocity. For a trans atmospheric flight of 10 kilometers per second and at an altitude of 80 kilometers, a maximum of 1% ionization is expected. At a velocity of 12 - 17 kilometer per second, such as a Mars return mission, up to 30% of the atoms and molecules in the flow field will be ionized. Under those circumstances, electrons play an important role in determining the internal states of atoms and molecules in the flow field and hence the amount of radiative heat load and the distance it takes for the flow field to re-establish equilibrium. Electron collisions provide an effective means of transferring energy even when the electron number density is as low as 1%. Because the mass of an electron is 12,760 times smaller than the reduced mass of N2, its average speed, and hence its average collision frequency, is more than 100 times larger. Even in the slightly ionized regime with only 1% electrons, the frequency of electron-molecule collisions is equal to or larger than that of molecule-molecule collisions, an important consideration in the low density part of the atmosphere. Three electron-molecule collision processes relevant to hypersonic flows will be considered: (1) vibrational excitation/de-excitation of a diatomic molecule by electron impact, (2) electronic excitation/de-excitation, and (3) dissociative recombination in electron-diatomic ion collisions. A review of available data, both theory and experiment, will be given. Particular attention will be paid to tailoring the molecular physics to the condition of hypersonic flows. For example, the high rotational temperatures in a hypersonic flow field means that most experimental data carried out under room temperatures are not applicable. Also

  8. Influence of Heat-radiating on Multi-photon Compton Scattering High-energy Electron

    Institute of Scientific and Technical Information of China (English)

    HAO Dong-shan; WANG Xin-min

    2007-01-01

    Using the model of the inverse Compton scattering between high-energy electrons and heat-radiation photons, the influence of heat-radiating photons on multi-photon Compton scattering high-energy electrons is studied . The results show that the energy loss, power loss, light resistance and light pressure of the high-energy electron formed by heat radiating are all proportional to the temperature T4 of the vacuum cavity of the electron,the Lorentz factor γ2 of the high-energy electrons, the scattering section of the electron and the number of photons acting at the same time with high-energy electrons. A good method for lessening the energy loss of the high-energy electron by using the one-photon Compton scattering between high-energy electrons and heat radiation photons is proposed.

  9. Reduced density matrix hybrid approach: application to electronic energy transfer.

    Science.gov (United States)

    Berkelbach, Timothy C; Markland, Thomas E; Reichman, David R

    2012-02-28

    Electronic energy transfer in the condensed phase, such as that occurring in photosynthetic complexes, frequently occurs in regimes where the energy scales of the system and environment are similar. This situation provides a challenge to theoretical investigation since most approaches are accurate only when a certain energetic parameter is small compared to others in the problem. Here we show that in these difficult regimes, the Ehrenfest approach provides a good starting point for a dynamical description of the energy transfer process due to its ability to accurately treat coupling to slow environmental modes. To further improve on the accuracy of the Ehrenfest approach, we use our reduced density matrix hybrid framework to treat the faster environmental modes quantum mechanically, at the level of a perturbative master equation. This combined approach is shown to provide an efficient and quantitative description of electronic energy transfer in a model dimer and the Fenna-Matthews-Olson complex and is used to investigate the effect of environmental preparation on the resulting dynamics.

  10. Measuring the electron beam energy in a magnetic bunch compressor

    Energy Technology Data Exchange (ETDEWEB)

    Hacker, Kirsten

    2010-09-15

    Within this thesis, work was carried out in and around the first bunch compressor chicane of the FLASH (Free-electron LASer in Hamburg) linear accelerator in which two distinct systems were developed for the measurement of an electron beams' position with sub-5 {mu}m precision over a 10 cm range. One of these two systems utilized RF techniques to measure the difference between the arrival-times of two broadband electrical pulses generated by the passage of the electron beam adjacent to a pickup antenna. The other system measured the arrival-times of the pulses from the pickup with an optical technique dependent on the delivery of laser pulses which are synchronized to the RF reference of the machine. The relative advantages and disadvantages of these two techniques are explored and compared to other available approaches to measure the same beam property, including a time-of-flight measurement with two beam arrival-time monitors and a synchrotron light monitor with two photomultiplier tubes. The electron beam position measurement is required as part of a measurement of the electron beam energy and could be used in an intra-bunch-train beam-based feedback system that would stabilize the amplitude of the accelerating field. By stabilizing the accelerating field amplitude, the arrival-time of the electron beam can be made more stable. By stabilizing the electron beam arrival-time relative to a stable reference, diagnostic, seeding, and beam-manipulation lasers can be synchronized to the beam. (orig.)

  11. Low Energy Electrons as Probing Tool for Astrochemical Reaction Mechanisms

    Science.gov (United States)

    Hendrik Bredehöft, Jan; Swiderek, Petra; Hamann, Thorben

    The complexity of molecules found in space varies widely. On one end of the scale of molecular complexity is the hydrogen molecule H2 . Its formation from H atoms is if not understood than at least thoroughly investigated[1]. On the other side of said spectrum the precursors to biopolymers can be found, such as amino acids[2,3], sugars[4], lipids, cofactors[5], etc, and the kerogen-like organic polymer material in carbonaceous meteorites called "black stuff" [6]. These have also received broad attention in the last decades. Sitting in the middle between these two extremes are simple molecules that are observed by radio astronomy throughout the Universe. These are molecules like methane (CH4 ), methanol (CH3 OH), formaldehyde (CH2 O), hydrogen cyanide (HCN), and many many others. So far more than 40 such species have been identified.[7] They are often used in laboratory experiments to create larger complex molecules on the surface of simulated interstellar dust grains.[2,8] The mechanisms of formation of these observed starting materials for prebiotic chemistry is however not always clear. Also the exact mechanisms of formation of larger molecules in photochemical experiments are largely unclear. This is mostly due to the very complex chemistry going on which involves many different radicals and ions. The creation of radicals and ions can be studied in detail in laboratory simulations. They can be created in a setup mimicking interstellar grain chemistry using slow electrons. There is no free electron radiation in space. What can be found though is a lot of radiation of different sorts. There is electromagnetic radiation (UV light, X-Rays, rays, etc.) and there is particulate radiation as well in the form of high energy ions. This radiation can provide energy that drives chemical reactions in the ice mantles of interstellar dust grains. And while the multitude of different kinds of radiation might be a little confusing, they all have one thing in common: Upon

  12. Electron Thermionic Emission from Graphene and a Thermionic Energy Converter

    Science.gov (United States)

    Liang, Shi-Jun; Ang, L. K.

    2015-01-01

    In this paper, we propose a model to investigate the electron thermionic emission from single-layer graphene (ignoring the effects of the substrate) and to explore its application as the emitter of a thermionic energy converter (TIC). An analytical formula is derived, which is a function of the temperature, work function, and Fermi energy level. The formula is significantly different from the traditional Richardson-Dushman (RD) law for which it is independent of mass to account for the supply function of the electrons in the graphene behaving like massless fermion quasiparticles. By comparing with a recent experiment [K. Jiang et al., Nano Res. 7, 553 (2014)] measuring electron thermionic emission from suspended single-layer graphene, our model predicts that the intrinsic work function of single-layer graphene is about 4.514 eV with a Fermi energy level of 0.083 eV. For a given work function, a scaling of T3 is predicted, which is different from the traditional RD scaling of T2. If the work function of the graphene is lowered to 2.5-3 eV and the Fermi energy level is increased to 0.8-0.9 eV, it is possible to design a graphene-cathode-based TIC operating at around 900 K or lower, as compared with the metal-based cathode TIC (operating at about 1500 K). With a graphene-based cathode (work function=4.514 eV ) at 900 K and a metallic-based anode (work function=2.5 eV ) like LaB6 at 425 K, the efficiency of our proposed TIC is about 45%.

  13. Power electronics for renewable and distributed energy systems a sourcebook of topologies, control and integration

    CERN Document Server

    Chakraborty, Sudipta; Kramer, William E

    2013-01-01

    While most books approach power electronics and renewable energy as two separate subjects, Power Electronics for Renewable and Distributed Energy Systems takes an integrative approach; discussing power electronic converters topologies, controls and integration that are specific to the renewable and distributed energy system applications. An overview of power electronic technologies is followed by the introduction of various renewable and distributed energy resources that includes photovoltaics, wind, small hydroelectric, fuel cells, microturbines and variable speed generation. Energy storage s

  14. Emission of Low-Energy Photons by Electrons at Electron-Positron and Electron-Ion Colliders with Dense Bunches

    CERN Document Server

    Jentschura, U D; Serbo, V G; 10.1103/PhysRevSTAB.12.011003

    2009-01-01

    Usually, the emission of low-energy photons in electron-positron (or electron-ion) bunch collisions is calculated with the same approach as for synchrotron radiation (beamstrahlung). However, for soft photons (E_gamma < E_c where E_c is a critical photon energy), when the coherence length of the radiation becomes comparable to the bunch length, the beamstrahlung approximation becomes invalid. In this paper, we present results of our calculation for this region based on approximation of classical currents. We consider several colliders with dense bunches. The number of low-energy photons dN_gamma emitted by N_e electrons per bunch crossing in the energy interval dE_gamma is dN_gamma = alpha g N_e dE_gamma/E_gamma, where alpha is the fine-structure constant, and the function g, which depends on the bunch parameters, typically is of order unity for modern colliders. In particular, for the ILC, we find that E_c = 83 keV and g=5.5 at a vanishing beam axis displacement, and g=0.88, E_c=0.24 keV for KEKB. We also...

  15. Angle-resolved cathodoluminescence imaging polarimetry

    CERN Document Server

    Osorio, Clara I; Brenny, Benjamin; Polman, Albert; Koenderink, A Femius

    2015-01-01

    Cathodoluminescence spectroscopy (CL) allows characterizing light emission in bulk and nanostructured materials and is a key tool in fields ranging from materials science to nanophotonics. Previously, CL measurements focused on the spectral content and angular distribution of emission, while the polarization was not fully determined. Here we demonstrate a technique to access the full polarization state of the cathodoluminescence emission, that is the Stokes parameters as a function of the emission angle. Using this technique, we measure the emission of metallic bullseye nanostructures and show that the handedness of the structure as well as nanoscale changes in excitation position induce large changes in polarization ellipticity and helicity. Furthermore, by exploiting the ability of polarimetry to distinguish polarized from unpolarized light, we quantify the contributions of different types of coherent and incoherent radiation to the emission of a gold surface, silicon and gallium arsenide bulk semiconductor...

  16. Angle-resolved catholdoluminescence imaging polarimetry

    NARCIS (Netherlands)

    Osorio, C.I.; Coenen, T.; Brenny, B.J.M.; Polman, A.; Koenderink, A.F.

    2015-01-01

    Cathodoluminescence spectroscopy (CL) allows characterizing light emission in bulk and nanostructured materials and is a key tool in fields ranging from materials science to nanophotonics. Previously, CL measurements focused on the spectral content and angular distribution of emission, while the pol

  17. Angle-resolved time delay in photoemission

    CERN Document Server

    Wätzel, Jonas; Pavlyukh, Yaroslav; Berakdar, Jamal

    2014-01-01

    We investigate theoretically the relative time delay of photoelectrons originating from different atomic subshells of noble gases. This quantity was measured via attosecond streaking and studied theoretically by Schultze et al. [Science 328, 1658 (2010)] for neon. A substantial discrepancy was found between the measured and the calculated values of the relative time delay. Several theoretical studies were put forward to resolve this issue, e.g., by including correlation effects. In the present paper we explore a further aspect, namely the directional dependence of time delay. In contrast to neon, for argon target a strong angular dependence of time delay is found near a Cooper minimum.

  18. An experimental study of secondary electron emission in the limit of low electron energy

    Science.gov (United States)

    Demidov, V. I.; Kaganovich, I. D.; Koepke, M. E.

    2013-09-01

    Study of secondary electron emission (SEE) from solid surfaces is important for many areas of science and technology, including but not limited to the formation of electron clouds in particle accelerators, plasma measurements by electrostatic probes and operation of Hall plasma thrusters. The measurements at low incident electron energy below 2eV are very challenging. The goal of this work is to measure SEE coefficient for molybdenum surface in contact with plasmas. In this study nearly mono-energetic electrons arising in plasma-chemical reactions like pair collisions of metastable atoms have been used for the measurements. Variation of the target voltage and measurement of the corresponding electron current from the mono-energetic electrons allows us to obtain the SEE coefficient. It is experimentally demonstrated that the coefficient is close to zero (less than 0.1) for clean targets and may have much higher value for contaminated targets with some absorbed gas on the surface. This work has been supported by DoE contract No. DE-SC0001939 and SPbGU.

  19. Energy distribution of elastically scattered electrons from double layer samples

    Science.gov (United States)

    Tőkési, K.; Varga, D.

    2016-02-01

    We present a theoretical description of the spectra of electrons elastically scattered from thin double layered Au-C samples. The analysis is based on the Monte Carlo simulation of the recoil and Doppler effects in reflection and transmission geometries of the scattering at a fixed angle of 44.3 ° and a primary energy of 40 keV. The relativistic correction is taken into account. Besides the experimentally measurable energy distributions the simulations give many partial distributions separately, depending on the number of elastic scatterings (single, and multiple scatterings of different types). Furthermore, we present detailed analytical calculations for the main parameters of the single scattering, taking into account both the ideal scattering geometry, i.e. infinitesimally small angular range, and the effect of the real, finite angular range used in the measurements. We show our results for intensity ratios, peak shifts and broadenings for four cases of measurement geometries and layer thicknesses. While in the peak intensity ratios of gold and carbon for transmission geometries were found to be in good agreement with the results of the single scattering model, especially large deviations were obtained in reflection geometries. The separation of the peaks, depending on the geometry and the thickness, generally smaller, and the peak width generally larger than it can be expected from the nominal values of the primary energy, scattering angle, and mean kinetic energy of the atoms. We also show that the peaks are asymmetric even for the case of the single scattering due to the finite solid angle. Finally, we present a qualitative comparison with the experimental data. We find our resulting energy distribution of elastically scattered electrons to be in good agreement with recent measurements.

  20. DFT calculation of core-electron binding energies

    Energy Technology Data Exchange (ETDEWEB)

    Takahata, Yuji; Chong, Delano P. E-mail: chong@chem.ubc.ca

    2003-11-01

    A total of 59 core-electron binding energies (CEBEs) were studied with the Amsterdam Density Functional Program (ADF) program and compared with the observed values. The results indicate that a polarized triple-zeta basis set of Slater-type orbitals is adequate for routine assessment of the performance of each method of computation. With such a basis set, seven density functionals were tested. In addition, the performance of 21 energy density functionals were computed from the density calculated with the statistical average of orbital potentials (SAOP). Among all the choices tested, the best density functional for core-electron binding energies of C to F turns out to be the combination of Perdew-Wang (1986) functional for exchange and the Perdew-Wang (1991) functional for correlation, confirming earlier studies based on contracted Gaussian-type orbitals. For this best functional, five Slater-type orbital basis sets were examined, ranging from polarized double-zeta quality to the largest set available in the ADF package. For the best functional with the best basis set, the average absolute deviation (AAD) of the calculated value from experiment is only 0.16 eV.

  1. Measurement of Low Energy Electronic Recoil Response and Electronic/Nuclear Recoils Discrimination in XENON100

    Science.gov (United States)

    Ye, Jingqiang; Xenon Collaboration

    2017-01-01

    The XENON100 detector uses liquid xenon time projection chamber to search for nuclear recoils(NR) caused by hypothetical Weakly Interacting Massive Particles (WIMPs). The backgrounds are mostly electronic recoils(ER), thus it's crucial to distinguish NR from ER. Using high statistical calibration data from tritiated methane, AmBe and other sources in XENON100, the ER/NR discrimination under different electric fields are measured. The Photon yield and recombination fluctuation of low energy electronic recoils under different fields will also be presented and compared to results from NEST and other experiments, which is crucial to understanding the response of liquid xenon detectors in the energy regime of searching dark matter.

  2. Electron scattering by O2 at intermediate and high energies

    Institute of Scientific and Technical Information of China (English)

    Deheng Shi; Jinfeng Sun; Xiangdong Yang; Zunlue Zhu; Yufang Liu

    2005-01-01

    @@ A complex optical model potential correlated by the concept of bonded atoms, which considers the overlapping effect of electron clouds between two atoms in a molecule, is firstly employed to calculate the absolute differential cross sections, the integrated and momentum transfer cross sections for electrons scattered by O2 at intermediate and high energies by using additivity rule model at Hartree-Fock level. In the study,the complex optical model potential is composed of static, exchange, correlation polarization plus absorption contributions. The quantitative absolute differential cross sections, the integrated and momentum transfer cross sections are obtained. Compared with available experimental data, this approach presents good results. It is shown that the additivity rule model together with the complex optical model potential correlated by the concept of bonded atoms is completely suitable for the calculations of the absolute differential cross sections, the integrated and momentum transfer cross sections.

  3. Spatial structure determination of ({radical}3 x {radical}3)R30{degrees} and (1.5 x 1.5)R18{degrees}CO on Cu(111) using angle-resolved photoemission extended fine structure

    Energy Technology Data Exchange (ETDEWEB)

    Moler, E.J.; Kellar, S.A.; Huff, W.R.A. [Lawrence Berkeley National Lab., CA (United States)] [and others

    1997-04-01

    The authors report a study of the spatial structure of ({radical}3 x {radical}3)R30{degrees} (low coverage) and (1.5 x 1.5)R18{degrees} (intermediate coverage) CO adsorbed on Cu(111), using the Angle-Resolved Photoemission Extended Fine Structure (ARPEFS) technique at beamline 9.3.2 at the Advanced Light Source. The CO molecule adsorbs on an atop site for both adsorption phases. Full multiple-scattering spherical-wave (MSSW) calculations were used to extract the C-Cu. bond length and the first Cu-Cu layer spacing for each adsorption phase. The authors find that the C-Cu bond length remains unchanged with increasing coverage, but the 1st Cu-Cu layer spacing contracts at the intermediate coverage. They calculate the bending mode force constant in the (1.5 x 1.5)R18{degrees} phase to be K{sub {delta}} = 2.2 (1) x 10{sup {minus}12} dyne-cm/rad from their experimentally determined bond lengths combined with previously published infra-red absorption frequencies.

  4. Direct Measurements of the Electron Energy Flux versus Electron Temperature Gradient in Tokamak Discharges

    Institute of Scientific and Technical Information of China (English)

    K.W. Gentle; M.E. Austin; P.E. Phillips

    2004-01-01

    Electron thermal transport is one of the most complex processes in fusion plasmas. It is generally described by a simple thermal diffusivity in transport analyses of discharges, but there is evidence of critical gradient effects with moderate stiffness. By analyzing periodic perturbations to an equilibrium, one can measure the variations in electron energy flux and electron temperature gradient over the perturbation cycle, obtaining the flux as a function of gradient over the range of parameters generated by the perturbation. Although time-dependent transport analysis is very sensitive to noise in the input data, averaging over many cycles of a periodic perturbation can provide data of sufficient quality. The analyses presented here are based on the ECE temperature data with high spatial and temporal resolution and full profile coverage on DIII-D for sawteeth and modulated ECH heating.

  5. Laser acceleration of electrons to giga-electron-volt energies using highly charged ions.

    Science.gov (United States)

    Hu, S X; Starace, Anthony F

    2006-06-01

    The recent proposal to use highly charged ions as sources of electrons for laser acceleration [S. X. Hu and A. F. Starace, Phys. Rev. Lett. 88, 245003 (2002)] is investigated here in detail by means of three-dimensional, relativistic Monte Carlo simulations for a variety of system parameters, such as laser pulse duration, ionic charge state, and laser focusing spot size. Realistic laser focusing effects--e.g., the existence of longitudinal laser field components-are taken into account. Results of spatial averaging over the laser focus are also presented. These numerical simulations show that the proposed scheme for laser acceleration of electrons from highly charged ions is feasible with current or near-future experimental conditions and that electrons with GeV energies can be obtained in such experiments.

  6. Microwave beatwave excitation of electron plasma wave and high energy electron production

    Energy Technology Data Exchange (ETDEWEB)

    Yatsuzuka, M.; Obata, K.; Nobuhara, S. [Himeji Inst. of Tech., Hyogo (Japan)

    1997-12-31

    Two X-band microwave beams with a slightly different frequency and the maximum output power of 50 kW are injected into a target plasma antiparallel to each other through a standard horn. The resonant excitation of an electron plasma wave is observed when the difference in frequency between counterstreaming microwaves is equal to the electron plasma frequency. The excited wave propagates in the same direction as the higher-frequency microwave with a wave length which satisfies the resonance condition of wave number. The wave amplitude grows with an increase in incident microwave power, and reaches the density perturbation {delta}n/n{sub 0} of approximately 3.2 % at the incident microwave power of 40 kW and beat frequency of 600 MHz. A small amount of high-energy electrons with the speed of 27 eV are observed in the high-power region of incident microwave. (author)

  7. High energy electron beam joining of ceramic components

    Energy Technology Data Exchange (ETDEWEB)

    Turman, B.N.; Glass, S.J.; Halbleib, J.A. [and others

    1997-07-01

    High strength, hermetic braze joints between ceramic components have been produced using high energy electron beams. With a penetration depth into a typical ceramic of {approximately}1 cm for a 10 MeV electron beam, this method provides the capability for rapid, transient brazing operations where temperature control of critical components is essential. The method deposits energy directly into a buried joint, allowing otherwise inaccessible interfaces to be brazed. Because of transient heating, higher thermal conductivity, lower heat capacity, and lower melting temperature of braze metals relative to the ceramic materials, a pulsed high power beam can melt a braze metal without producing excessive ceramic temperatures. We have demonstrated the feasibility of this process related to ceramic coupons as well as ceramic and glass tubes. The transient thermal response was predicted, using as input the energy absorption predicted from the coupled electron-photon transport analysis. The joining experiments were conducted with an RF Linac accelerator at 10-13 MV. The repetition rate of the pulsed beam was varied between 8 and 120 Hz, the average beam current was varied between 8 and 120 microamps, and the power was varied up to 1.5 kW. These beam parameters gave a beam power density between 0.2 to 2 kW/cm{sup 2}. The duration of the joining runs varied from 5 to 600 sec. Joining experiments have provided high strength between alumina - alumina and alumina - cermet joints in cylindrical geometry. These joints provided good hermetic seals. A series of tests was conducted to determine the minimum beam power and exposure time for producing, a hermetic seal.

  8. Electronic structure and electron energy-loss spectroscopy of ZrO2 zirconia

    Science.gov (United States)

    Dash, L. K.; Vast, Nathalie; Baranek, Philippe; Cheynet, Marie-Claude; Reining, Lucia

    2004-12-01

    The atomic and electronic structures of zirconia are calculated within density functional theory, and their evolution is analyzed as the crystal-field symmetry changes from tetrahedral [cubic (c-ZrO2) and tetragonal (t-ZrO2) phases] to octahedral (hypothetical rutile ZrO2 ), to a mixing of these symmetries (monoclinic phase, m-ZrO2 ). We find that the theoretical bulk modulus in c-ZrO2 is 30% larger than the experimental value, showing that the introduction of yttria in zirconia has a significant effect. Electronic structure fingerprints which characterize each phase from their electronic spectra are identified. We have carried out electron energy-loss spectroscopy experiments at low momentum transfer and compared these results to the theoretical spectra calculated within the random phase approximation. We show a dependence of the valence and 4p ( N2,3 edge) plasmons on the crystal structure, the dependence of the latter being brought into the spectra by local-field effects. Last, we attribute low energy excitations observed in EELS of m-ZrO2 to defect states 2eV above the top of the intrinsic valence band, and the EELS fundamental band gap value is reconciled with the 5.2 or 5.8eV gaps determined by vacuum ultraviolet spectroscopy.

  9. High-temperature behavior of supported graphene: Electron-phonon coupling and substrate-induced doping

    DEFF Research Database (Denmark)

    Ulstrup, Søren; Bianchi, Marco; Guan, Dandan

    2012-01-01

    The temperature-dependent electronic structure and electron-phonon coupling of weakly doped supported graphene is studied by angle-resolved photoemission spectroscopy and ab initio molecular dynamics simulations. The electron-phonon coupling is found to be extremely weak, reaching the lowest value...

  10. Numerically Fitting The Electron Fermi Energy and The Electron Fraction in A Neutron Star

    CERN Document Server

    Li, Xing Hu; Li, Xiang Dong; Xu, Yan; Wang, Pei; Wang, Na; Yuan, Jianping

    2016-01-01

    Based on the basic definition of Fermi energy of degenerate and relativistic electrons, we obtain a special solution to electron Fermi energy, $E_{\\rm F}(e)$, and express $E_{\\rm F}(e)$ as a function of electron fraction, $Y_{e}$, and matter density, $\\rho$. Several useful analytical formulae for $Y_{e}$ and $\\rho$ within classical models and the work of Dutra et al. 2014 (Type-2) in relativistic mean field theory are obtained using numerically fitting. When describing the mean-field Lagrangian, density, we adopt the TMA parameter set, which is remarkably consistent with with the updated astrophysical observations of neutron stars. Due to the importance of the density dependence of the symmetry energy, $S$, in nuclear astrophysics, a brief discussion on the symmetry parameters $S_v$ and $L$ (the slope of $S$) is presented. Combining these fit formulae with boundary conditions for different density regions, we can evaluate the value of $E_{\\rm F}(e)$ in any given matter density, and obtain a schematic diagram ...

  11. Quantitative measurements of Kikuchi bands in diffraction patterns of backscattered electrons using an electrostatic analyzer.

    Science.gov (United States)

    Went, M R; Winkelmann, A; Vos, M

    2009-09-01

    Diffraction patterns of backscattered electrons can provide important crystallographic information with high spatial resolution. Recently, the dynamical theory of electron diffraction was applied to reproduce in great detail backscattering patterns observed in the scanning electron microscope (SEM). However, a fully quantitative comparison of theory and experiment requires angle-resolved measurements of the intensity and the energy of the backscattered electrons, which is difficult to realize in an SEM. This paper determines diffraction patterns of backscattered electrons using an electrostatic analyzer, operating at energies up to 40 keV with sub-eV energy resolution. Measurements are done for different measurement geometries and incoming energies. Generally a good agreement is found between theory and experiment. This spectrometer also allows us to test the influence of the energy loss of the detected electron on the backscattered electron diffraction pattern. It is found that the amplitude of the intensity variation decreases only slowly with increasing energy loss from 0 to 60 eV.

  12. Diffraction and electron energy loss to plasmons in silicon slabs

    Science.gov (United States)

    Levine, Zachary H.

    2008-03-01

    Dynamical diffraction patterns were calculated for 25nm slabs of silicon with [001], [111], and [110] faces for a 120keV electron beam. The calculation used the mixed dynamical form factor in the dielectric formulation. Dielectric matrices with wave vector and frequency dependence were calculated within the local density approximation using the random phase approximation. The energy losses, 10-25eV , span the plasmon peak. Near the zone axes, the results show the preservation of elastic contrast and both excess and deficit Kikuchi lines.

  13. An Emphasis of Electron Energy Calculation in Quantum Wells

    Institute of Scientific and Technical Information of China (English)

    GAOShao-Wen; CAOJun-Cheng; FENGSong-Lin

    2004-01-01

    We investigate various methods for the calculation of the electron energy in semiconductor quantum wells and focus on a matrix algorithm method. The results show better fitness of the factor -h2/2 э/эz 1/m*(z) э/эz than that of -h2/2 1/m*(z) э2/эz2 in the first part of the Schroedinger equation. The effect of nonparabolicity in the conduction band is also discussed.

  14. Control and power electronics technology in renewable energy

    Institute of Scientific and Technical Information of China (English)

    2008-01-01

    As the cut-in point of research on control and power electronics technology used in renewable energy, this paper does not aim to analyze particular theories or tech-nologies in this field, but, instead, is to go back to the fountainhead of the issue to illustrate the essential concepts in this field, which are usually neglected and may become bottle-neck of the research. Research experiences have shown that con-fusion and trouble may be created if researchers do not understand these essential concepts well.

  15. Measurement of the Electron Structure Function at LEP energies

    CERN Document Server

    Abdallah, J; Adam, W; Adzic, P; Albrecht, T; Alemany-Fernandez, R; Allmendinger, T; Allport, P P; Amaldi, U; Amapane, N; Amato, S; Anashkin, E; Andreazza, A; Andringa, S; Anjos, N; Antilogus, P; Apel, W-D; Arnoud, Y; Ask, S; Asman, B; Augustin, J E; Augustinus, A; Baillon, P; Ballestrero, A; Bambade, P; Barbier, R; Bardin, D; Barker, G J; Baroncelli, A; Battaglia, M; Baubillier, M; Becks, K-H; Begalli, M; Behrmann, A; Ben-Haim, E; Benekos, N; Benvenuti, A; Berat, C; Berggren, M; Bertrand, D; Besancon, M; Besson, N; Bloch, D; Blom, M; Bluj, M; Bonesini, M; Boonekamp, M; Booth, P S L; Borisov, G; Botner, O; Bouquet, B; Bowcock, T J V; Boyko, I; Bracko, M; Brenner, R; Brodet, E; Bruckman, P; Brunet, J M; Buschbeck, B; Buschmann, P; Calvi, M; Camporesi, T; Canale, V; Carena, F; Castro, N; Cavallo, F; Chapkin, M; Charpentier, Ph; Checchia, P; Chierici, R; Chliapnikov, P; Chudoba, J; Chung, S U; Cieslik, K; Collins, P; Contri, R; Cosme, G; Cossutti, F; Costa, M J; Crennell, D; Cuevas, J; D'Hondt, J; da Silva, T; Da Silva, W; Della Ricca, G; De Angelis, A; De Boer, W; De Clercq, C; De Lotto, B; De Maria, N; De Min, A; de Paula, L; Di Ciaccio, L; Di Simone, A; Doroba, K; Drees, J; Eigen, G; Ekelof, T; Ellert, M; Elsing, M; Espirito Santo, M C; Fanourakis, G; Fassouliotis, D; Feindt, M; Fernandez, J; Ferrer, A; Ferro, F; Flagmeyer, U; Foeth, H; Fokitis, E; Fulda-Quenzer, F; Fuster, J; Gandelman, M; Garcia, C; Gavillet, Ph; Gazis, E; Gokieli, R; Golob, B; Gomez-Ceballos, G; Goncalves, P; Graziani, E; Grosdidier, G; Grzelak, K; Guy, J; Haag, C; Hallgren, A; Hamacher, K; Hamilton, K; Haug, S; Hauler, F; Hedberg, V; Hennecke, M; Hoffman, J; Holmgren, S-O; Holt, P J; Houlden, M A; Jackson, J N; Jarlskog, G; Jarry, P; Jeans, D; Johansson, E K; Jonsson, P; Joram, C; Jungermann, L; Kapusta, F; Katsanevas, S; Katsoufis, E; Kernel, G; Kersevan, B P; Kerzel, U; King, B T; Kjaer, N J; Kluit, P; Kokkinias, P; Kourkoumelis, C; Kouznetsov, O; Krumstein, Z; Kucharczyk, M; Lamsa, J; Leder, G; Ledroit, F; Leinonen, L; Leitner, R; Lemonne, J; Lepeltier, V; Lesiak, T; Liebig, W; Liko, D; Lipniacka, A; Lopes, J H; Lopez, J M; Loukas, D; Lutz, P; Lyons, L; MacNaughton, J; Malek, A; Maltezos, S; Mandl, F; Marco, J; Marco, R; Marechal, B; Margoni, M; Marin, J-C; Mariotti, C; Markou, A; Martinez-Rivero, C; Masik, J; Mastroyiannopoulos, N; Matorras, F; Matteuzzi, C; Mazzucato, F; Mazzucato, M; Mc Nulty, R; Meroni, C; Migliore, E; Mitaroff, W; Mjoernmark, U; Moa, T; Moch, M; Moenig, K; Monge, R; Montenegro, J; Moraes, D; Moreno, S; Morettini, P; Mueller, U; Muenich, K; Mulders, M; Mundim, L; Murray, W; Muryn, B; Myatt, G; Myklebust, T; Nassiakou, M; Navarria, F; Nawrocki, K; Nemecek, S; Nicolaidou, R; Nikolenko, M; Oblakowska-Mucha, A; Obraztsov, V; Olshevski, A; Onofre, A; Orava, R; Osterberg, K; Ouraou, A; Oyanguren, A; Paganoni, M; Paiano, S; Palacios, J P; Palka, H; Papadopoulou, Th D; Pape, L; Parkes, C; Parodi, F; Parzefall, U; Passeri, A; Passon, O; Peralta, L; Perepelitsa, V; Perrotta, A; Petrolini, A; Piedra, J; Pieri, L; Pierre, F; Pimenta, M; Piotto, E; Podobnik, T; Poireau, V; Pol, M E; Polok, G; Pozdniakov, V; Pukhaeva, N; Pullia, A; Radojicic, D; Rebecchi, P; Rehn, J; Reid, D; Reinhardt, R; Renton, P; Richard, F; Ridky, J; Rivero, M; Rodriguez, D; Romero, A; Ronchese, P; Roudeau, P; Rovelli, T; Ruhlmann-Kleider, V; Ryabtchikov, D; Sadovsky, A; Salmi, L; Salt, J; Sander, C; Savoy-Navarro, A; Schwickerath, U; Sekulin, R; Siebel, M; Sisakian, A; Slominski, W; Smadja, G; Smirnova, O; Sokolov, A; Sopczak, A; Sosnowski, R; Spassov, T; Stanitzki, M; Stocchi, A; Strauss, J; Stugu, B; Szczekowski, M; Szeptycka, M; Szumlak, T; Szwed, J; Tabarelli, T; Tegenfeldt, F; Timmermans, J; Tkatchev, L; Tobin, M; Todorovova, S; Tome, B; Tonazzo, A; Tortosa, P; Travnicek, P; Treille, D; Tristram, G; Trochimczuk, M; Troncon, C; Turluer, M L; Tyapkin, I A; Tyapkin, P; Tzamarias, S; Uvarov, V; Valenti, G; Van Dam, P; Van Eldik, J; van Remortel, N; Van Vulpen, I; Vegni, G; Veloso, F; Venus, W; Verdier, P; Verzi, V; Vilanova, D; Vitale, L; Vrba, V; Wahlen, H; Washbrook, A J; Weiser, C; Wicke, D; Wickens, J; Wilkinson, G; Winter, M; Witek, M; Yushchenko, O; Zalewska, A; Zalewski, P; Zavrtanik, D; Zhuravlov, V; Zimin, N I; Zintchenko, A; Zupan, M

    2010-01-01

    The hadronic part of the Electron Structure Function (ESF) has been measured for the first time, using e+e- data collected by the DELPHI experiment at LEP, at centre-of-mass energies sqrt(s) = 91.2-209.5 GeV. The data analysis is simpler than that of the measurement of the photon structure function. The ESF data are compared to predictions of phenomenological models based on the photon structure function. It is shown that the quasi-real photon virtuality contribution is significant. The presented data can serve as a cross-check of the photon structure function analyses and help in refining existing parametrizations.

  16. Radiation processing of liquid with low energy electron accelerator

    Energy Technology Data Exchange (ETDEWEB)

    Makuuchi, Keizo [Japan Atomic Energy Research Inst., Takasaki, Gunma (Japan). Takasaki Radiation Chemistry Research Establishment

    2003-02-01

    Radiation induced emulsion polymerization, radiation vulcanization of NR latex (RVNRL) and radiation degradation of natural polymers were selected and reviewed as the radiation processing of liquid. The characteristic of high dose rate emulsion polymerization is the occurrence of cationic polymerization. Thus, it can be used for the production of new materials that cannot be obtained by radical polymerization. A potential application will be production of polymer emulsion that can be used as water-borne UV/EB curing resins. The technology of RVNRL by {gamma}-ray has been commercialized. RVNRL with low energy electron accelerator is under development for further vulcanization cost reduction. Vessel type irradiator will be favorable for industrial application. Radiation degradation of polysaccharides is an emerging and promising area of radiation processing. However, strict cost comparison between liquid irradiation with low energy EB and state irradiation with {gamma}-ray should be carried out. (author)

  17. An electronic structure perspective of graphene interfaces

    Science.gov (United States)

    Schultz, Brian J.; Dennis, Robert V.; Lee, Vincent; Banerjee, Sarbajit

    2014-03-01

    The unusual electronic structure of graphene characterized by linear energy dispersion of bands adjacent to the Fermi level underpins its remarkable transport properties. However, for practical device integration, graphene will need to be interfaced with other materials: 2D layered structures, metals (as ad-atoms, nanoparticles, extended surfaces, and patterned metamaterial geometries), dielectrics, organics, or hybrid structures that in turn are constituted from various inorganic or organic components. The structural complexity at these nanoscale interfaces holds much promise for manifestation of novel emergent phenomena and provides a means to modulate the electronic structure of graphene. In this feature article, we review the modifications to the electronic structure of graphene induced upon interfacing with disparate types of materials with an emphasis on iterative learnings from theoretical calculations and electronic spectroscopy (X-ray absorption fine structure (XAFS) spectroscopy, scanning transmission X-ray microscopy (STXM), angle-resolved photoemission spectroscopy (ARPES), and X-ray magnetic circular dichroism (XMCD)). We discuss approaches for engineering and modulating a bandgap in graphene through interfacial hybridization, outline experimental methods for examining electronic structure at interfaces, and overview device implications of engineered interfaces. A unified view of how geometric and electronic structure are correlated at interfaces will provide a rational means for designing heterostructures exhibiting emergent physical phenomena with implications for plasmonics, photonics, spintronics, and engineered polymer and metal matrix composites.

  18. Low-energy electron elastic scattering from Os atom: New electron affinity

    Science.gov (United States)

    Felfli, Z.; Kiros, F.; Msezane, A. Z.

    2013-05-01

    Bilodeau and Haugan measured the binding energies (BEs) of the ground state and the excited state of the Os- ion to be 1.07780(12) eV and 0.553(3) eV, respectively. These values are consistent with those calculated in. Here our investigation, using the recent complex angular momentum methodology wherein is embedded the crucial electron-electron correlations and the vital core polarization interaction, has found that the near threshold electron-Os elastic scattering total cross section (TCS) is characterized by three stable bound states of the Os- ion formed as resonances during the slow electron collision, with BEs of 1.910 eV, 1.230 eV and 0.224 eV. The new extracted electron affinity (EA) value from the TCS of 1.910 eV for the Os atom is significantly different from that measured in. Our calculated elastic differential cross sections (DCSs) also yield the relevant BEs for the ground and the two excited states of the Os- ion. The complex characteristic resonance structure in the TCS for the Os atom is ideal for catalysis, but makes it difficult to execute the Wigner threshold law in describing the threshold detachment behavior of complex atoms and extracting the reliable attendant EAs. Supported by U.S. DOE, AFOSR and CAU CFNM, NSF-CREST Program.

  19. Advanced Power Electronics Interfaces for Distributed Energy Workshop Summary: August 24, 2006, Sacramento, California

    Energy Technology Data Exchange (ETDEWEB)

    Treanton, B.; Palomo, J.; Kroposki, B.; Thomas, H.

    2006-10-01

    The Advanced Power Electronics Interfaces for Distributed Energy Workshop, sponsored by the California Energy Commission Public Interest Energy Research program and organized by the National Renewable Energy Laboratory, was held Aug. 24, 2006, in Sacramento, Calif. The workshop provided a forum for industry stakeholders to share their knowledge and experience about technologies, manufacturing approaches, markets, and issues in power electronics for a range of distributed energy resources. It focused on the development of advanced power electronic interfaces for distributed energy applications and included discussions of modular power electronics, component manufacturing, and power electronic applications.

  20. Strongly anisotropic spin-orbit splitting in a two-dimensional electron gas

    DEFF Research Database (Denmark)

    Michiardi, Matteo; Bianchi, Marco; Dendzik, Maciej

    2015-01-01

    Near-surface two-dimensional electron gases on the topological insulator Bi$_2$Te$_2$Se are induced by electron doping and studied by angle-resolved photoemission spectroscopy. A pronounced spin-orbit splitting is observed for these states. The $k$-dependent splitting is strongly anisotropic...... Rashba Hamiltonian. However, a $\\mathbf{k} \\cdot \\mathbf{p}$ model that includes the possibility of band structure anisotropy as well as both isotropic and anisotropic third order Rashba splitting can explain the results. The isotropic third order contribution to the Rashba Hamiltonian is found...... to be negative, reducing the energy splitting at high $k$. The interplay of band structure, higher order Rashba effect and tuneable doping offers the opportunity to engineer not only the size of the spin-orbit splitting but also its direction....

  1. Low energy electron point source microscopy: beyond imaging.

    Science.gov (United States)

    Beyer, André; Gölzhäuser, Armin

    2010-09-01

    Low energy electron point source (LEEPS) microscopy has the capability to record in-line holograms at very high magnifications with a fairly simple set-up. After the holograms are numerically reconstructed, structural features with the size of about 2 nm can be resolved. The achievement of an even higher resolution has been predicted. However, a number of obstacles are known to impede the realization of this goal, for example the presence of electric fields around the imaged object, electrostatic charging or radiation induced processes. This topical review gives an overview of the achievements as well as the difficulties in the efforts to shift the resolution limit of LEEPS microscopy towards the atomic level. A special emphasis is laid on the high sensitivity of low energy electrons to electrical fields, which limits the structural determination of the imaged objects. On the other hand, the investigation of the electrical field around objects of known structure is very useful for other tasks and LEEPS microscopy can be extended beyond the task of imaging. The determination of the electrical resistance of individual nanowires can be achieved by a proper analysis of the corresponding LEEPS micrographs. This conductivity imaging may be a very useful application for LEEPS microscopes.

  2. Electronic Structure and Maximum Energy Product of MnBi

    Directory of Open Access Journals (Sweden)

    Jihoon Park

    2014-08-01

    Full Text Available We have performed first-principles calculations to obtain magnetic moment, magnetocrystalline anisotropy energy (MAE, i.e., the magnetic crystalline anisotropy constant (K, and the Curie temperature (Tc of low temperature phase (LTP MnBi and also estimated the maximum energy product (BHmax at elevated temperatures. The full-potential linearized augmented plane wave (FPLAPW method, based on density functional theory (DFT within the local spin density approximation (LSDA, was used to calculate the electronic structure of LPM MnBi. The Tc was calculated by the mean field theory. The calculated magnetic moment, MAE, and Tc are 3.63 μB/f.u. (formula unit (79 emu/g or 714 emu/cm3, −0.163 meV/u.c. (or K = −0.275 × 106 J/m3 and 711 K, respectively. The (BHmax at the elevated temperatures was estimated by combining experimental coercivity (Hci and the temperature dependence of magnetization (Ms(T. The (BHmax is 17.7 MGOe at 300 K, which is in good agreement with the experimental result for directionally-solidified LTP MnBi (17 MGOe. In addition, a study of electron density maps and the lattice constant c/a ratio dependence of the magnetic moment suggested that doping of a third element into interstitial sites of LTP MnBi can increase the Ms.

  3. Feasibility of ceramic joining with high energy electron beams

    Energy Technology Data Exchange (ETDEWEB)

    Turman, B.N.; Glass, S.J.; Halbleib, J.A.; Helmich, D.R.; Loehman, R.E. [Sandia National Labs., Albuquerque, NM (United States); Clifford, J.R. [Titan Corp., Albuquerque, NM (United States)

    1995-01-01

    Joining structural ceramics is possible using high melting point metals such as Mo and Pt that are heated with a high energy electron beam, with the potential for producing joints with high temperature capability. A 10 MeV electron beam can penetrate through 1 cm of ceramic, offering the possibility of buried interface joining. Because of transient heating and the lower heat capacity of the metal relative to the ceramic, a pulsed high power beam has the potential for melting the metal without decomposing or melting the adjacent ceramic. The authors have demonstrated the feasibility of the process with a series of 10 MeV, 1 kW electron beam experiments. Shear strengths up to 28 NTa have been measured for Si{sub 3}N{sub 4}-Mo-Si{sub 3}N{sub 4}. These modest strengths are due to beam non-uniformity and the limited area of bonding. The bonding mechanism appears to be a thin silicide reaction layer. Si{sub 3}N{sub 4}-Si{sub 3}N{sub 4} joints with no metal layer were also produced, apparently bonded an yttrium apatite grain boundary phase.

  4. TCO/metal/TCO structures for energy and flexible electronics

    Energy Technology Data Exchange (ETDEWEB)

    Guillen, C., E-mail: c.guillen@ciemat.es; Herrero, J.

    2011-10-31

    There is increasing attention paid to improving transparent conductive electrodes for applications in large area photovoltaic devices and displays that are being developed for energy and electronics. To date, transparent and conductive oxides (TCO) based on In{sub 2}O{sub 3}, ZnO, or SnO{sub 2} are commonly used, but advanced devices require new electrodes with lower resistivities than previously achieved and with optical properties superior to those of the present generation. TCO/metal/TCO multilayer structures have emerged as an interesting alternative because they provide optical and electrical characteristics globally superior to those attainable with a single-layer TCO or metal electrode and can be deposited at low temperatures onto inexpensive plastic substrates. Indeed, the fabrication of thin film devices on flexible substrates has substantial interest for application to lightweight products and implementation of roll-to-roll deposition processes that can significantly reduce production costs. In this sense, organic electronics that require low deposition temperatures have the best chance to be the first transferred from conventional glass to inexpensive plastic substrates. The present critical review summarizes current TCO/metal/TCO research results, first analyzed for materials and thickness selection as a function of the optical transmittance and electrical resistance parameters, and then analyzed according to other important properties such as mechanical reliability and thermal and humidity stability. The review concludes with a brief discussion of the results obtained for TCO/metal/TCO structures applied as electrodes in several organic electronic devices.

  5. Energy Quantization and Probability Density of Electron in Intense-Field-Atom Interactions

    Institute of Scientific and Technical Information of China (English)

    敖淑艳; 程太旺; 李晓峰; 吴令安; 付盘铭

    2003-01-01

    We find that, due to the quantum correlation between the electron and the field, the electronic energy becomes quantized also, manifesting the particle aspect of light in the electron-light interaction. The probability amplitude of finding electron with a given energy is given by a generalized Bessel function, which can be represented as a coherent superposition of contributions from a few electronic quantum trajectories. This concept is illustrated by comparing the spectral density of the electron with the laser assisted recombination spectrum.

  6. DZ-12/4 Multi-energy Electron Linear Accelerator Acceptance Test

    Institute of Scientific and Technical Information of China (English)

    XIA; Wen; YE; Hong-sheng; ZHANG; Wei-dong; CHEN; Yi-zhen; LIN; Min; XU; Li-jun; CHEN; Ke-sheng; LI; Ming

    2015-01-01

    DZ-12/4multi-energy electron linear accelerator device established by China Institute of Atomic Energy can provide 6 MeV,8 MeV,10MeV,12MeV electron energy beam,mainly used to establish electron beam reference radiation fields of radiation processing dose level,and

  7. Practical spatial resolution of electron energy loss spectroscopy in aberration corrected scanning transmission electron microscopy.

    Science.gov (United States)

    Shah, A B; Ramasse, Q M; Wen, J G; Bhattacharya, A; Zuo, J M

    2011-08-01

    The resolution of electron energy loss spectroscopy (EELS) is limited by delocalization of inelastic electron scattering rather than probe size in an aberration corrected scanning transmission electron microscope (STEM). In this study, we present an experimental quantification of EELS spatial resolution using chemically modulated 2×(LaMnO(3))/2×(SrTiO(3)) and 2×(SrVO(3))/2×(SrTiO(3)) superlattices by measuring the full width at half maxima (FWHM) of integrated Ti M(2,3), Ti L(2,3), V L(2,3), Mn L(2,3), La N(4,5), La N(2,3) La M(4,5) and Sr L(3) edges over the superlattices. The EELS signals recorded using large collection angles are peaked at atomic columns. The FWHM of the EELS profile, obtained by curve-fitting, reveals a systematic trend with the energy loss for the Ti, V, and Mn edges. However, the experimental FWHM of the Sr and La edges deviates significantly from the observed experimental tendency.

  8. Strongly correlated electron systems: Photoemission and the single-impurity model

    Energy Technology Data Exchange (ETDEWEB)

    Arko, A.J.; Joyce, J.J.; Andrews, A.B.; Thompson, J.D.; Smith, J.L.; Mandrus, D.; Hundley, M.F.; Cornelius, A.L. [Los Alamos National Laboratories, Los Alamos, New Mexico 87545 (United States); Moshopoulou, E.; Fisk, Z. [NHMFL, Florida State University, Tallahassee, Florida 32306-4005 (United States); Canfield, P.C. [Iowa State University/Ames Laboratory, Ames, Iowa 50011 (United States); Menovsky, A. [Natuurkundig Laboratorium, University of Amsterdam, Amsterdam (The Netherlands)

    1997-09-01

    We present high-resolution, angle-resolved photoemission spectra for Ce-based and U-based strongly correlated electron systems. The experimental results are irreconcilable with the long-accepted single-impurity model, which predicts a narrow singlet state, in close proximity to the Fermi energy, whose linewidth and binding energy are a constant determined by a characteristic temperature T{sub K} for the material. We report that both 4f and 5f photoemission features disperse with crystal momentum at temperatures both above and below T{sub K}; these are characteristics consistent with narrow bands but not with the single-impurity model. Inclusion of the lattice must be considered at all temperatures. Variants of the periodic Anderson model are consistent with this approach. {copyright} {ital 1997} {ital The American Physical Society}

  9. A Flexible Power Electronics Configuration for Coupling Renewable Energy Sources

    Directory of Open Access Journals (Sweden)

    Mattia Filippini

    2015-05-01

    Full Text Available A combination of series, parallel and multilevel power electronics has been investigated as a potential interface for two different types of renewable energy sources and in order to reach higher power levels. Renewable energy sources are typically dispersed in a territory, and sources, like wind and solar, allow small to medium-scale generation of electricity. The configuration investigated in this article aims at adapting the coupling solution to the specific generation characteristics of the renewable energy source to make it fit the electrical network. The configuration consists of a combination of three-phase multilevel converters and single-phase inverters, which are designed to provide flexibility, high power quality and high efficiency. A detailed analysis and simulation is performed to identify the properties in conjunction with the electrical grid requirements and the potential challenges encountered during operation. An optimized operation example of wind generation combined with solar PV generation is presented to exemplify the flexibility and benefits of the proposed configuration.

  10. Electron to Muon Conversion in Low-Energy Electron-Nucleus Scattering

    CERN Document Server

    Diener, Kai-Peer O

    2004-01-01

    We present an estimate of the electron to muon conversion cross section in fixed-target elastic electron scattering. The matrix element $$ is calculated analytically in two scenarios introducing suitable approximations. We consider on the one hand side the case of three light Dirac neutrinos with CKM-type leptonic mixing and on the other hand a typical see-saw scenario. We evaluate the coulombic contribution to the scattering cross section in the limit of vanishing energy transfer to the nucleus and, thus, obtain a realistic estimate for the total conversion cross section. Although we find that in the see-saw scenario the cross section can be enhanced by as much as twenty orders of magnitude in comparison to the Dirac case, it is still not experimentally accessible.

  11. Low-energy electron transmission through high aspect ratio Al O nanocapillaries

    DEFF Research Database (Denmark)

    Milosavljević, A.R.; Jureta, J.; Víkor, G.;

    2009-01-01

    Electron transmission through insulating AlO nanocapillaries of different diameters (40 and 270 nm) and 15 μm length has been investigated for low-energy electrons (2-120 V). The total intensity of transmitted current weakly depends on the incident electron energy and tilt angle defined with resp......Electron transmission through insulating AlO nanocapillaries of different diameters (40 and 270 nm) and 15 μm length has been investigated for low-energy electrons (2-120 V). The total intensity of transmitted current weakly depends on the incident electron energy and tilt angle defined...

  12. A study of angle-resolved photoemission extended fine structure as applied to the Ni 3p, Cu 3s, and Cu 3p core levels of the respective clean (111) surfaces

    Energy Technology Data Exchange (ETDEWEB)

    Huff, W.R.A.; Moler, E.J.; Kellar, S.A. [Lawrence Berkeley National Lab., CA (United States)] [and others

    1997-04-01

    The first non-s initial state angle-resolved photoemission extended fine structure (ARPEFS) study of clean surfaces for the purpose of further understanding the technique is reported. The surface structure sensitivity of ARPEFS applied to clean surfaces and to arbitrary initial states is studied using normal photoemission data taken from the Ni 3p core levels of a Ni(111) single crystal and the Cu 3s and the Cu 3p core-levels of a Cu(111) single crystal. The Fourier transforms of these clean surface data are dominated by backscattering. Unlike the s initial state data, the p initial state data show a peak in the Fourier transform corresponding to in-plane scattering from the six nearest-neighbors to the emitter. Evidence was seen for single-scattering events from in the same plane as the emitters and double-scattering events. Using a newly developed, multiple-scattering calculation program, ARPEFS data from clean surfaces and from p initial states can be modeled to high precision. Although there are many layers of emitters when measuring photoemission from a clean surface, test calculations show that the ARPEFS signal is dominated by photoemission from atoms in the first two crystal layers. Thus, ARPEFS applied to clean surfaces is sensitive to surface reconstruction. The known contraction of the first two Cu(111) layers is confirmed. The best-fit calculation for clean Ni(111) indicates an expansion of the first two layers. To better understand the ARPEFS technique, the authors studied s and non-s initial state photoemission from clean metal surfaces.

  13. Electron-nuclear energy sharing in above-threshold multiphoton dissociative ionization of H2.

    Science.gov (United States)

    Wu, J; Kunitski, M; Pitzer, M; Trinter, F; Schmidt, L Ph H; Jahnke, T; Magrakvelidze, M; Madsen, C B; Madsen, L B; Thumm, U; Dörner, R

    2013-07-12

    We report experimental observation of the energy sharing between electron and nuclei in above-threshold multiphoton dissociative ionization of H2 by strong laser fields. The absorbed photon energy is shared between the ejected electron and nuclei in a correlated fashion, resulting in multiple diagonal lines in their joint energy spectrum governed by the energy conservation of all fragment particles.

  14. Electron-Nuclear Energy Sharing in Above-Threshold Multiphoton Dissociative Ionization of H2

    DEFF Research Database (Denmark)

    Wu, J.; Kunitski, M.; Pitzer, M.

    2013-01-01

    We report experimental observation of the energy sharing between electron and nuclei in above-threshold multiphoton dissociative ionization of H2 by strong laser fields. The absorbed photon energy is shared between the ejected electron and nuclei in a correlated fashion, resulting in multiple...... diagonal lines in their joint energy spectrum governed by the energy conservation of all fragment particles....

  15. Simulations and Measurement of Electron Energy and Effective Electron Temperature of Nanosecond Pulsed Argon Plasma%Simulations and Measurement of Electron Energy and Effective Electron Temperature of Nanosecond Pulsed Argon Plasma

    Institute of Scientific and Technical Information of China (English)

    闻雪晴; 信裕; 冯春雷; 丁洪斌

    2012-01-01

    The behavior of argon plasma driven by nanosecond pulsed plasma in a low-pressure plasma reactor is investigated using a global model, and the results are compared with the experimental measurements. The time evolution of plasma density and the electron energy probability function are calculated by solving the energy balance and Boltzmann equations. During and shortly after the discharge pulse, the electron energy probability function can be represented by a bi-Maxwellian distribution, indicating two energy groups of electrons. According to the effective electron temperature calculation, we find that there are more high-energy electrons that play an important role in the excitation and ionization processes than low-energy electrons. The effective electron temperature is also measured via optical emission spectroscopy to evaluate the simulation model. In the comparison, the simulation results are found to be in agreement with the measure- ments. Furthermore, variations of the effective electron temperature are presented versus other discharge parameters, such as pulse width time, pulse rise time and gas pressure.

  16. Graphene for energy harvesting/storage devices and printed electronics

    Institute of Scientific and Technical Information of China (English)

    Lorenzo Grande; Vishnu Teja Chundi; Di Wei; Chris Bower; Piers Andrew; Tapani Ryh(a)nen

    2012-01-01

    Graphene-based materials are intriguing from the perspective of fundamental science and technology because they are non-toxic,chemically and thermally tolerant,and mechanically robust.Graphene exhibits superior electrical conductivity,high surface area and a broad electrochemical window that may be particularly advantageous for their applications in energy storage devices.In addition,graphene can be prepared in the form of a colloidal suspension with adjustable solubility and thus is suitable for printing applications and offers both transparency and good conductivity at the same time.In this review,applications of graphene in solar cells,batteries,supercapacitors and fuel cells are summarized with the latest developments.Furthermore,graphene as a conductive ink for printed electronics is also discussed.

  17. Design Considerations for High Energy Electron -- Positron Storage Rings

    Science.gov (United States)

    Richter, B.

    1966-11-01

    High energy electron-positron storage rings give a way of making a new attack on the most important problems of elementary particle physics. All of us who have worked in the storage ring field designing, building, or using storage rings know this. The importance of that part of storage ring work concerning tests of quantum electrodynamics and mu meson physics is also generally appreciated by the larger physics community. However, I do not think that most of the physicists working tin the elementary particle physics field realize the importance of the contribution that storage ring experiments can make to our understanding of the strongly interacting particles. I would therefore like to spend the next few minutes discussing the sort of things that one can do with storage rings in the strongly interacting particle field.

  18. Accurate studies on the full vibrational energy spectra and molecular dissociation energies for some electronic states of N2 molecule

    Institute of Scientific and Technical Information of China (English)

    REN; Weiyi; SUN; Weiguo; HOU; Shilin; FENG; Hao

    2005-01-01

    It is usually very difficult to directly obtain molecular dissociation energy De and all accurate high-lying vibrational energies for most diatomic electronic states using modern experimental techniques or quantum theories, and it is also very difficult to give accurate analytical expression for diatomic molecular dissociation energy. This study proposes a new analytical formula for obtaining accurate molecular dissociation energy based on the LeRoy and Bernstein's energy expression in dissociation limit. A set of full vibrational energy spectra for some electronic states of N2 molecule are studied using the algebraic method (AM) suggested recently, and the corresponding accurate molecular dissociation energies are evaluated using the proposed new formula and high-lying AM vibrational energies. The results show that the AM spectra and the new theoretical dissociation energies agree excellently with experimental data, and thereby providing a new physical approach to generating accurate dissociation energies for electronic states of diatomic molecules.

  19. Energy dissipation from a correlated system driven out of equilibrium

    Science.gov (United States)

    Rameau, J. D.; Freutel, S.; Kemper, A. F.; Sentef, M. A.; Freericks, J. K.; Avigo, I.; Ligges, M.; Rettig, L.; Yoshida, Y.; Eisaki, H.; Schneeloch, J.; Zhong, R. D.; Xu, Z. J.; Gu, G. D.; Johnson, P. D.; Bovensiepen, U.

    2016-12-01

    In complex materials various interactions have important roles in determining electronic properties. Angle-resolved photoelectron spectroscopy (ARPES) is used to study these processes by resolving the complex single-particle self-energy and quantifying how quantum interactions modify bare electronic states. However, ambiguities in the measurement of the real part of the self-energy and an intrinsic inability to disentangle various contributions to the imaginary part of the self-energy can leave the implications of such measurements open to debate. Here we employ a combined theoretical and experimental treatment of femtosecond time-resolved ARPES (tr-ARPES) show how population dynamics measured using tr-ARPES can be used to separate electron-boson interactions from electron-electron interactions. We demonstrate a quantitative analysis of a well-defined electron-boson interaction in the unoccupied spectrum of the cuprate Bi2Sr2CaCu2O8+x characterized by an excited population decay time that maps directly to a discrete component of the equilibrium self-energy not readily isolated by static ARPES experiments.

  20. High energy electron generation by the 15 mJ ultrashort pulse laser

    Energy Technology Data Exchange (ETDEWEB)

    Takano, K; Hotta, E; Nemoto, K [Department of Energy Sciences Tokyo Institute of Technology 4259 Nagatsuta-cho Midori-ku Yokohama 226-8502 (Japan); Nayuki, T; Oishi, Y; Fujii, T; Zhidkov, A [Central Research Institute of Electric Power Industry 2-6-1 Nagasaka, Yokosuka, Kanagawa, 240-0196 (Japan); Todoriki, M; Hasegawa, S [University of Tokyo 7-3-1 Hongo Bunkyo-ku Tokyo 113-8654 (Japan)], E-mail: k-tn@plasma.es.titech.ac.jp

    2008-05-01

    We propose a small size high energy X-ray source utilizing ultrashort pulse lasers, and a new scheme for generating quasi-monoenergetic electrons. In this paper, we developed a compact laser electron generator and performed experiment that generated energetic electrons over 1 MeV electrons with only 15 mJ laser energy. The temperatures of emitted electrons were measured to be 0.2 MeV and 0.25 MeV without and with prepulse, respectively.

  1. Formation of Hubbard-like bands as a fingerprint of strong electron-electron interactions in FeSe

    Science.gov (United States)

    Watson, Matthew D.; Backes, Steffen; Haghighirad, Amir A.; Hoesch, Moritz; Kim, Timur K.; Coldea, Amalia I.; Valentí, Roser

    2017-02-01

    We use angle-resolved photoemission spectroscopy (ARPES) to explore the electronic structure of single crystals of FeSe over a wide range of binding energies and study the effects of strong electron-electron correlations. We provide evidence for the existence of "Hubbard-like bands" at high binding energies consisting of incoherent many-body excitations originating from Fe 3 d states in addition to the renormalized quasiparticle bands near the Fermi level. Many high-energy features of the observed ARPES data can be accounted for when incorporating the effects of strong local Coulomb interactions in calculations of the spectral function via dynamical mean-field theory, including the formation of a Hubbard-like band. This shows that over the energy scale of several eV, local correlations arising from the on-site Coulomb repulsion and Hund's coupling are essential for a proper understanding of the electronic structure of FeSe and other related iron-based superconductors.

  2. Conductive Elastomers for Stretchable Electronics, Sensors and Energy Harvesters

    Directory of Open Access Journals (Sweden)

    Jin-Seo Noh

    2016-04-01

    Full Text Available There have been a wide variety of efforts to develop conductive elastomers that satisfy both mechanical stretchability and electrical conductivity, as a response to growing demands on stretchable and wearable devices. This article reviews the important progress in conductive elastomers made in three application fields of stretchable technology: stretchable electronics, stretchable sensors, and stretchable energy harvesters. Diverse combinations of insulating elastomers and non-stretchable conductive materials have been studied to realize optimal conductive elastomers. It is noted that similar material combinations and similar structures have often been employed in different fields of application. In terms of stretchability, cyclic operation, and overall performance, fields such as stretchable conductors and stretchable strain/pressure sensors have achieved great advancement, whereas other fields like stretchable memories and stretchable thermoelectric energy harvesting are in their infancy. It is worth mentioning that there are still obstacles to overcome for the further progress of stretchable technology in the respective fields, which include the simplification of material combination and device structure, securement of reproducibility and reliability, and the establishment of easy fabrication techniques. Through this review article, both the progress and obstacles associated with the respective stretchable technologies will be understood more clearly.

  3. Electronics in cars: consequences for the energy-supply system

    Science.gov (United States)

    Beil, Falk

    The amount of electronics in cars is constantly increasing. Thus, the question arises, whether the current wiring designs will continue to be able to meet the required output related to this increase in the future. Which consequences result, then, for the design of the wiring system and its components? An examination of the electrical consumers currently installed in motor vehicles, and of those planned for future use, shows that the wiring system load during driving will increase to as much as 2000 W. Many new devices, such as the telephone, will also enjoy increasing use while the vehicle is at a standstill, which will result in the type of wiring system load changing in the future. In addition to this, loading will increase due to greater traffic density; the vehicle will be operated more often at idling speed, leading to a reduction in the available current. Thus, a balanced current supply can no longer be ensured with present designs. That means new energy supply concepts are required, e.g. the 24 V wiring system and energy management. In addition, the wiring system components must be optimized. This particularly applies to the battery, which must be further developed in order to obtain increased cell strength, a longer service life and improved temperature stability.

  4. High-Resolution Measurements of Low-Energy Conversion Electrons

    CERN Multimedia

    Gizon, A; Putaux, J

    2002-01-01

    Measurements of low-energy internal conversion electrons have been performed with high energy resolution in some N = 105 odd and odd-odd nuclei using a semi-circular spectrograph associated to a specific tape transport system. These experiments aimed to answer the following questions~: \\begin{itemize} \\item Do M3 isomeric transitions exist in $^{183}$Pt and $^{181}$Os, isotones of $^{184}$Au~? \\item Are the neutron configurations proposed to describe the isomeric and ground states of $^{184}$Au right or wrong~? \\item Does it exist an isomeric state in $^{182}$Ir, isotone of $^{181}$Os, $^{183}$Pt and $^{184}$Au~? \\item What are the spin and parity values of the excited states of $^{182}$Ir~? \\end{itemize} In $^{183}$Pt, the 35.0 keV M3 isomeric transition has been clearly observed and the reduced transition probability has been determined. The deduced hindrance factor is close to that observed in the neighbouring odd-odd $^{184}$Au nucleus. This confirms the neutron configurations previously proposed for the ...

  5. DFPT approach to the temperature dependence of electronic band energies

    Science.gov (United States)

    Boulanger, Paul; Cote, Michel; Gonze, Xavier

    2010-03-01

    The energy bands of semiconductors exhibit significant shifts and broadening with temperature at constant volume. This is an effect of the direct renormalization of band energies due to electron-phonon interactions. In search of an efficient linear response DFT approach to this effect, beyond semi-empirical approximation or frozen- phonon DFT, we have implemented formulas derived by Allen and Heine [J. Phys. C 9, 2305 (1976)] inside the ABINIT package. We have found that such formulas need a great number of bands, O(1000), to properly converge the thermal corrections of deep potential well atoms, i.e. elements of the first row. This leads to heavy computational costs even for simple systems like diamond. The DFPT formalism can be used to circumvent entirely the need for conduction bands by computing the first-order wave-functions using the self-consistent Sternheimer equation. We will compare the results of both formalism demonstrating that the DFPT approach reproduces the correct converged results of the formulas of Allen and Heine.

  6. Energy-filtered real- and k-space secondary and energy-loss electron imaging with Dual Emission Electron spectro-Microscope: Cs/Mo(110)

    Energy Technology Data Exchange (ETDEWEB)

    Grzelakowski, Krzysztof P., E-mail: k.grzelakowski@opticon-nanotechnology.com

    2016-05-15

    Since its introduction the importance of complementary k{sub ||}-space (LEED) and real space (LEEM) information in the investigation of surface science phenomena has been widely demonstrated over the last five decades. In this paper we report the application of a novel kind of electron spectromicroscope Dual Emission Electron spectroMicroscope (DEEM) with two independent electron optical channels for reciprocal and real space quasi-simultaneous imaging in investigation of a Cs covered Mo(110) single crystal by using the 800 eV electron beam from an “in-lens” electron gun system developed for the sample illumination. With the DEEM spectromicroscope it is possible to observe dynamic, irreversible processes at surfaces in the energy-filtered real space and in the corresponding energy-filtered k{sub ǁ}-space quasi-simultaneously in two independent imaging columns. The novel concept of the high energy electron beam sample illumination in the cathode lens based microscopes allows chemically selective imaging and analysis under laboratory conditions. - Highlights: • A novel concept of the electron sample illumination with “in-lens” e- gun is realized. • Quasi-simultaneous energy selective observation of the real- and k-space in EELS mode. • Observation of the energy filtered Auger electron diffraction at Cs atoms on Mo(110). • Energy-loss, Auger and secondary electron momentum microscopy is realized.

  7. Photoelectron spectroscopy bulk and surface electronic structures

    CERN Document Server

    Suga, Shigemasa

    2014-01-01

    Photoelectron spectroscopy is now becoming more and more required to investigate electronic structures of various solid materials in the bulk, on surfaces as well as at buried interfaces. The energy resolution was much improved in the last decade down to 1 meV in the low photon energy region. Now this technique is available from a few eV up to 10 keV by use of lasers, electron cyclotron resonance lamps in addition to synchrotron radiation and X-ray tubes. High resolution angle resolved photoelectron spectroscopy (ARPES) is now widely applied to band mapping of materials. It attracts a wide attention from both fundamental science and material engineering. Studies of the dynamics of excited states are feasible by time of flight spectroscopy with fully utilizing the pulse structures of synchrotron radiation as well as lasers including the free electron lasers (FEL). Spin resolved studies also made dramatic progress by using higher efficiency spin detectors and two dimensional spin detectors. Polarization depend...

  8. Energy shift of H-atom electrons due to Gibbons-Hawking thermal bath

    CERN Document Server

    Pardy, Miroslav

    2016-01-01

    The electromagnetic shift of energy levels of H-atom electrons is determined by calculating an electron coupling to the Gibbons-Hawking electromagnetic field thermal bath. Energy shift of electrons in H-atom is determined in the framework of the non-relativistic quantum mechanics.

  9. Mechanism and Experimental Observability of Global Switching Between Reactive and Nonreactive Coordinates at High Total Energies

    Science.gov (United States)

    Teramoto, Hiroshi; Toda, Mikito; Takahashi, Masahiko; Kono, Hirohiko; Komatsuzaki, Tamiki

    2015-08-01

    We present a mechanism of global reaction coordinate switching, namely, a phenomenon in which the reaction coordinate dynamically switches to another coordinate as the total energy of the system increases. The mechanism is based on global changes in the underlying phase space geometry caused by a switching of dominant unstable modes from the original reactive mode to another nonreactive mode in systems with more than 2 degrees of freedom. We demonstrate an experimental observability to detect a reaction coordinate switching in an ionization reaction of a hydrogen atom in crossed electric and magnetic fields. For this reaction, the reaction coordinate is a coordinate along which electrons escape and its switching changes the escaping direction from the direction of the electric field to that of the magnetic field and, thus, the switching can be detected experimentally by measuring the angle-resolved momentum distribution of escaping electrons.

  10. Introduction to electronics and applications in high energy physics

    CERN Document Server

    CERN. Geneva

    2004-01-01

    Electronics in HEP experiments: specificities and evolution The Art of Electronics: is there something beyond Ohm's law? Basic building blocks of Analog electronics: quickly understanding a schematic Charge preamps, current preamps and future preamps, shaping and the rest Electronics noise: fundamental and practical Evolution of technology: ASICs, FPGAs...

  11. A New Method of Measuring Electron Emission Induced by Low Energy Ions from Solids

    Institute of Scientific and Technical Information of China (English)

    ZHANG Heng-Da; A. Breskin; R. Chechik; S. Shckemelinin; E. Cheifetz

    2005-01-01

    @@ A new mathematical method of measuring electron emission induced by low energy ions from solids is described and used to calculate secondary electron emission according to the recorded pulse-height spectra of ions and ultraviolet (UV) photons. Using the UV single secondary electron spectra, we predict the shape of many secondary electron distributions under consideration of detection efficiency of MCP detector. These calculated distributions allow us to characterize the secondary electrons yield, and to give a secondary electron distribution for measured data. It seems rather feasible to determine secondary electron yield emitted by low energy ions at very low ion fluxes.

  12. Multi-port power electronic interface for renewable energy sources

    Science.gov (United States)

    Jiang, Wei

    Energy intensive products and services are penetrating people's daily life as well as different sectors of industry during recent decades. Further effort to improve efficiency, reduce green house gas and hazardous particle emission lead to the emergence of the "more electric" concept in several industries including transportation. This trend, however, burdens the aging power system and existing local power networks. To offer a remedy to the problem and a smooth transition to a more reliable, more diverse, and more efficient power grid of the future, the concept of Multi-port Power Electronic Interface (MPEI) for localized power processing is introduced in this dissertation, which interfaces and manages various sources, loads and storages. Different means of integrating multiple sources and storages into the existing power system are studied and evaluated; the six phase-leg structure is chosen to interface five sources/loads: fuel cell, wind turbine, solar cell, battery and utility grid. Partitioning of source-interface and load-interface on a system level as well as analysis and modeling on small signal level are performed. A novel control structure for source-interface is proposed in the design, which forms Controlled Quasi Current Source (CQCS) during the load sharing operation and offers several salient advantages: • Inherent average current-mode control. • Easy share of steady state current/power. • Share of load dynamics for better source protection. Local control loops for various input ports are designed based on linearized system model; controller performance is tuned to accommodate the characteristics of different sources. To maintain a sustainable operation, different modes of operation are defined for MPEI; detailed state-transition with associated events are also defined in each operation mode. Prototype of MPEI is built and control system is implemented digitally in a digital signal processor; steady state and transient performance of MPEI is

  13. Electronic structure of a superconducting topological insulator Sr-doped Bi{sub 2}Se{sub 3}

    Energy Technology Data Exchange (ETDEWEB)

    Han, C. Q.; Chen, W. J.; Zhu, Fengfeng; Yao, Meng-Yu [Key Laboratory of Artificial Structures and Quantum Control (Ministry of Education), Department of Physics and Astronomy, Shanghai Jiao Tong University, Shanghai 200240 (China); Li, H.; Li, Z. J.; Wang, M.; Gao, Bo F., E-mail: bo-f-gao@mail.sim.ac.cn [Shanghai Institute of Microsystem and Information Technology, Chinese Academy of Science, Shanghai 200050 (China); Guan, D. D.; Liu, Canhua; Qian, Dong, E-mail: dqian@sjtu.edu.cn; Jia, Jin-Feng [Key Laboratory of Artificial Structures and Quantum Control (Ministry of Education), Department of Physics and Astronomy, Shanghai Jiao Tong University, Shanghai 200240 (China); Collaborative Innovation Center of Advanced Microstructures, Nanjing 210093 (China); Gao, C. L. [Key Laboratory of Artificial Structures and Quantum Control (Ministry of Education), Department of Physics and Astronomy, Shanghai Jiao Tong University, Shanghai 200240 (China); Collaborative Innovation Center of Advanced Microstructures, Nanjing 210093 (China); Department of Physics, Fudan University, Shanghai 200433 (China)

    2015-10-26

    Using high-resolution angle-resolved photoemission spectroscopy and scanning tunneling microscopy/spectroscopy, the atomic and low energy electronic structure of the Sr-doped superconducting topological insulators (Sr{sub x}Bi{sub 2}Se{sub 3}) was studied. Scanning tunneling microscopy shows that most of the Sr atoms are not in the van der Waals gap. After Sr doping, the Fermi level was found to move further upwards when compared with the parent compound Bi{sub 2}Se{sub 3}, which is consistent with the low carrier density in this system. The topological surface state was clearly observed, and the position of the Dirac point was determined in all doped samples. The surface state is well separated from the bulk conduction bands in the momentum space. The persistence of separated topological surface state combined with small Fermi energy makes this superconducting material a very promising candidate for the time reversal invariant topological superconductor.

  14. Electronic structure of reconstructed InAs(001) surfaces - identification of bulk and surface bands based on their symmetries

    Science.gov (United States)

    Olszowska, Natalia; Kolodziej, Jacek J.

    2016-02-01

    Using angle-resolved photoelectron spectroscopy (ARPES) band structures of indium- and arsenic-terminated InAs(001) surfaces are investigated. These surfaces are highly reconstructed, elementary cells of their lattices contain many atoms in different chemical configurations, and moreover, they are composed of domains having related but different reconstructions. These domain-type surface reconstructions result in the reciprocal spaces containing regions with well-defined k→∥-vector and regions with not-well-defined one. In the ARPES spectra most of the surface related features appear as straight lines in the indeterminate k→∥-vector space. It is shown that, thanks to differences in crystal and surface symmetries, the single photon energy ARPES may be successfully used for classification of surface and bulk bands of electronic states on complex, highly reconstructed surfaces instead of the most often used variable photon energy studies.

  15. A facility for the analysis of the electronic structures of solids and their surfaces by synchrotron radiation photoelectron spectroscopy.

    Science.gov (United States)

    Hoesch, M; Kim, T K; Dudin, P; Wang, H; Scott, S; Harris, P; Patel, S; Matthews, M; Hawkins, D; Alcock, S G; Richter, T; Mudd, J J; Basham, M; Pratt, L; Leicester, P; Longhi, E C; Tamai, A; Baumberger, F

    2017-01-01

    A synchrotron radiation beamline in the photon energy range of 18-240 eV and an electron spectroscopy end station have been constructed at the 3 GeV Diamond Light Source storage ring. The instrument features a variable polarisation undulator, a high resolution monochromator, a re-focussing system to form a beam spot of 50 × 50 μm(2), and an end station for angle-resolved photoelectron spectroscopy (ARPES) including a 6-degrees-of-freedom cryogenic sample manipulator. The beamline design and its performance allow for a highly productive and precise use of the ARPES technique at an energy resolution of 10-15 meV for fast k-space mapping studies with a photon flux up to 2 ⋅ 10(13) ph/s and well below 3 meV for high resolution spectra.

  16. A facility for the analysis of the electronic structures of solids and their surfaces by synchrotron radiation photoelectron spectroscopy

    Science.gov (United States)

    Hoesch, M.; Kim, T. K.; Dudin, P.; Wang, H.; Scott, S.; Harris, P.; Patel, S.; Matthews, M.; Hawkins, D.; Alcock, S. G.; Richter, T.; Mudd, J. J.; Basham, M.; Pratt, L.; Leicester, P.; Longhi, E. C.; Tamai, A.; Baumberger, F.

    2017-01-01

    A synchrotron radiation beamline in the photon energy range of 18-240 eV and an electron spectroscopy end station have been constructed at the 3 GeV Diamond Light Source storage ring. The instrument features a variable polarisation undulator, a high resolution monochromator, a re-focussing system to form a beam spot of 50 × 50 μm2, and an end station for angle-resolved photoelectron spectroscopy (ARPES) including a 6-degrees-of-freedom cryogenic sample manipulator. The beamline design and its performance allow for a highly productive and precise use of the ARPES technique at an energy resolution of 10-15 meV for fast k-space mapping studies with a photon flux up to 2 ṡ 1013 ph/s and well below 3 meV for high resolution spectra.

  17. Development of a high-resolution soft x-ray (30--1500 eV) beamline at the Advanced Light Source and its use for the study of angle-resolved photoemission extended fine structure

    Energy Technology Data Exchange (ETDEWEB)

    Huff, W R.A. [California Univ., Berkeley, CA (United States). Dept. of Chemistry

    1996-02-01

    ALS Bending magnet beamline 9.3.2 is for high resolution spectroscopy, with circularly polarized light. Fixed included-angle SGM uses three gratings for 30--1500 eV photons; circular polarization is produced by an aperture for selecting the beam above or below the horizontal plane. Photocurrent from upper and lower jaws of entrance slit sets a piezoelectric drive feedback loop on the vertically deflecting mirror for stable beam. End station has a movable platform. With photomeission data from Stanford, structure of c(2{times}2)P/Fe(100) was determined using angle-resolved photoemission extended fine structure (ARPEFS). Multiple-scattering spherical-wave (MSSW) calculations indicate that P atoms adsorb in fourfold hollow sites 1.02A above the first Fe layer. Self-consistent-field X{alpha} scattered wave calculation confirm that the Fe{sub 1}-Fe{sub 2} space is contracted for S/Fe but not for P/Fe; comparison is made to atomic N and O on Fe(100). Final-state effects on ARPEFS curves used literature data from the S 1s and 2p core levels of c(2{times}2)S/Ni(001); a generalized Ramsauer-Townsend splitting is present in the 1s but not 2p data. An approximate method for analyzing ARPEFS data from a non-s initial state using only the higher-{ell} partial wave was tested successfully. ARPEFS data from clean surfaces were collected normal to Ni(111) (3p core levels) and 5{degree} off-normal from Cu(111)(3s, 3p). Fourier transforms (FT) resemble adsorbate systems, showing backscattering signals from atoms up to 4 layers below emitters. 3p FTs show scattering from 6 nearest neighbors in the same crystal layer as the emitters. MSSW calulation indicate that Cu 3p photoemission is mostly d-wave. FTs also indicate double-scattering and single-scattering from laterally distant atoms; calculations indicate that the signal is dominated by photoemission from the first 2 crystal layers.

  18. Applications of CCTO supercapacitor in energy storage and electronics

    Directory of Open Access Journals (Sweden)

    R. K. Pandey

    2013-06-01

    Full Text Available Since the discovery of colossal dielectric constant in CCTO supercapacitor in 2000, development of its practical application to energy storage has been of great interest. In spite of intensive efforts, there has been thus far, no report of proven application. The object of this research is to understand the reason for this lack of success and to find ways to overcome this limitation. Reported herein is the synthesis of our research in ceramic processing of this material and its characterization, particularly with the objective of identifying potential applications. Experimental results have shown that CCTO's permittivity and loss tangent, the two most essential dielectric parameters of fundamental importance for the efficiency of a capacitor device, are intrinsically coupled. They increase or decrease in tandem. Therefore, efforts to simultaneously retain the high permittivity while minimizing the loss tangent of CCTO might not succeed unless an entirely non-typical approach is taken for processing this material. Based on the experimental results and their analysis, it has been identified that it is possible to produce CCTO bulk ceramics with conventional processes having properties that can be exploited for fabricating an efficient energy storage device (EDS. We have additionally identified that CCTO can be used for the development of efficient solid state capacitors of Class II type comparable to the widely used barium titanate (BT capacitors. Based on high temperature studies of the resistivity and the Seebeck coefficient it is found that CCTO is a wide bandgap n-type semiconductor material which could be used for high temperature electronics. The temperature dependence of the linear thermal expansion of CCTO shows the presence of possible phase changes at 220 and 770 °C the origin of which remains unexplained.

  19. Modeling the high-energy electronic state manifold of adenine: Calibration for nonlinear electronic spectroscopy

    Energy Technology Data Exchange (ETDEWEB)

    Nenov, Artur, E-mail: Artur.Nenov@unibo.it; Giussani, Angelo; Segarra-Martí, Javier; Jaiswal, Vishal K. [Dipartimento di Chimica “G. Ciamician,” Università di Bologna, Via Selmi 2, IT-40126 Bologna (Italy); Rivalta, Ivan [Université de Lyon, CNRS, Institut de Chimie de Lyon, École Normale Supérieure de Lyon, 46 Allée d’Italie, F-69364 Lyon Cedex 07 (France); Cerullo, Giulio [Dipartimento di Fisica, Politecnico di Milano, IFN-CNR, Piazza Leonardo Da Vinci 32, IT-20133 Milano (Italy); Mukamel, Shaul [Department of Chemistry, University of California, Irvine, California 92697-2025 (United States); Garavelli, Marco, E-mail: marco.garavelli@unibo.it, E-mail: marco.garavelli@ens-lyon.fr [Dipartimento di Chimica “G. Ciamician,” Università di Bologna, Via Selmi 2, IT-40126 Bologna (Italy); Université de Lyon, CNRS, Institut de Chimie de Lyon, École Normale Supérieure de Lyon, 46 Allée d’Italie, F-69364 Lyon Cedex 07 (France)

    2015-06-07

    Pump-probe electronic spectroscopy using femtosecond laser pulses has evolved into a standard tool for tracking ultrafast excited state dynamics. Its two-dimensional (2D) counterpart is becoming an increasingly available and promising technique for resolving many of the limitations of pump-probe caused by spectral congestion. The ability to simulate pump-probe and 2D spectra from ab initio computations would allow one to link mechanistic observables like molecular motions and the making/breaking of chemical bonds to experimental observables like excited state lifetimes and quantum yields. From a theoretical standpoint, the characterization of the electronic transitions in the visible (Vis)/ultraviolet (UV), which are excited via the interaction of a molecular system with the incoming pump/probe pulses, translates into the determination of a computationally challenging number of excited states (going over 100) even for small/medium sized systems. A protocol is therefore required to evaluate the fluctuations of spectral properties like transition energies and dipole moments as a function of the computational parameters and to estimate the effect of these fluctuations on the transient spectral appearance. In the present contribution such a protocol is presented within the framework of complete and restricted active space self-consistent field theory and its second-order perturbation theory extensions. The electronic excited states of adenine have been carefully characterized through a previously presented computational recipe [Nenov et al., Comput. Theor. Chem. 1040–1041, 295-303 (2014)]. A wise reduction of the level of theory has then been performed in order to obtain a computationally less demanding approach that is still able to reproduce the characteristic features of the reference data. Foreseeing the potentiality of 2D electronic spectroscopy to track polynucleotide ground and excited state dynamics, and in particular its expected ability to provide

  20. The role of low-energy (≤ 20 eV) electrons in astrochemistry

    Science.gov (United States)

    Boyer, Michael C.; Rivas, Nathalie; Tran, Audrey A.; Verish, Clarissa A.; Arumainayagam, Christopher R.

    2016-10-01

    UV photon-driven condensed phase cosmic ice reactions have been the main focus in understanding the extraterrestrial synthesis of complex organic molecules. Low-energy (≤ 20 eV) electron-induced reactions, on the other hand, have been largely ignored. In this article, we review studies employing surface science techniques to study low-energy electron-induced condensed phase reactions relevant to astrochemistry. In particular, we show that low-energy electron irradiation of methanol ices leads to the synthesis of many of the same complex molecules formed through UV irradiation. Moreover, our results are qualitatively consistent with the hypothesis that high-energy condensed phase radiolysis is mediated by low-energy electron-induced reactions. In addition, due to the numbers of available low-energy secondary electrons resulting from the interaction of high-energy radiation with matter as well as differences between electron- and photon-induced processes, low-energy electron-induced reactions are perhaps as, or even more, effective than photon-induced reactions in initiating condensed-phase chemical reactions in the interstellar medium. Consequently, we illustrate a need for astrochemical models to include the details of electron-induced reactions in addition to those driven by UV photons. Finally, we show that low-energy electron-induced reactions may lead to the production of unique molecular species that could serve as tracer molecules for electron-induced condensed phase reactions in the interstellar medium.

  1. The mass angular scattering power method for determining the kinetic energies of clinical electron beams

    Energy Technology Data Exchange (ETDEWEB)

    Blais, N.; Podgorsak, E.B. (Montreal General Hospital, PQ (Canada). Dept. of Medical Physics)

    1992-10-01

    A method for determining the kinetic energy of clinical electron beams is described, based on the measurement in air of the spatial spread of a pencil electron beam which is produced from the broad clinical electron beam. As predicted by the Fermi-Eyges theory, the dose distribution measured in air on a plane, perpendicular to the incident direction of the initial pencil electron beam, is Gaussian. The square of its spatial spread is related to the mass angular scattering power which in turn is related to the kinetic energy of the electron beam. The measured spatial spread may thus be used to determine the mass angular scattering power, which is then used to determine the kinetic energy of the electron beam from the known relationship between mass angular scattering power and kinetic energy. Energies obtained with the mass angular scattering power method agree with those obtained with the electron range method. (author).

  2. The applications of in situ electron energy loss spectroscopy to the study of electron beam nanofabrication.

    Science.gov (United States)

    Chen, Shiahn J; Howitt, David G; Gierhart, Brian C; Smith, Rosemary L; Collins, Scott D

    2009-06-01

    An in situ electron energy loss spectroscopy (EELS) technique has been developed to investigate the dynamic processes associated with electron-beam nanofabrication on thin membranes. In this article, practical applications germane to e-beam nanofabrication are illustrated with a case study of the drilling of nanometer-sized pores in silicon nitride membranes. This technique involves successive acquisitions of the plasmon-loss and the core-level ionization-loss spectra in real time, both of which provide the information regarding the hole-drilling kinetics, including two respective rates for total mass loss, individual nitrogen and silicon element depletion, and the change of the atomic bonding environment. In addition, the in situ EELS also provides an alternative method for endpoint detection with a potentially higher time resolution than by imaging. On the basis of the time evolution of in situ EELS spectra, a qualitative working model combining knock-on sputtering, irradiation-induced mass transport, and phase separation can be proposed.

  3. High-Energy Electron Confinement in a Magnetic Cusp Configuration

    Science.gov (United States)

    Park, Jaeyoung; Krall, Nicholas A.; Sieck, Paul E.; Offermann, Dustin T.; Skillicorn, Michael; Sanchez, Andrew; Davis, Kevin; Alderson, Eric; Lapenta, Giovanni

    2015-04-01

    We report experimental results validating the concept that plasma confinement is enhanced in a magnetic cusp configuration when β (plasma pressure/magnetic field pressure) is of order unity. This enhancement is required for a fusion power reactor based on cusp confinement to be feasible. The magnetic cusp configuration possesses a critical advantage: the plasma is stable to large scale perturbations. However, early work indicated that plasma loss rates in a reactor based on a cusp configuration were too large for net power production. Grad and others theorized that at high β a sharp boundary would form between the plasma and the magnetic field, leading to substantially smaller loss rates. While not able to confirm the details of Grad's work, the current experiment does validate, for the first time, the conjecture that confinement is substantially improved at high β . This represents critical progress toward an understanding of the plasma dynamics in a high-β cusp system. We hope that these results will stimulate a renewed interest in the cusp configuration as a fusion confinement candidate. In addition, the enhanced high-energy electron confinement resolves a key impediment to progress of the Polywell fusion concept, which combines a high-β cusp configuration with electrostatic fusion for a compact, power-producing nuclear fusion reactor.

  4. Simulation of the secondary electrons energy deposition produced by proton beams in PMMA: influence of the target electronic excitation description

    Science.gov (United States)

    Dapor, Maurizio; Abril, Isabel; de Vera, Pablo; Garcia-Molina, Rafael

    2015-06-01

    We have studied the radial dependence of the energy deposition of the secondary electron generated by swift proton beams incident with energies T = 50 keV-5 MeV on poly(methylmethacrylate) (PMMA). Two different approaches have been used to model the electronic excitation spectrum of PMMA through its energy loss function (ELF), namely the extended-Drude ELF and the Mermin ELF. The singly differential cross section and the total cross section for ionization, as well as the average energy of the generated secondary electrons, show sizeable differences at T ⩽ 0.1 MeV when evaluated with these two ELF models. In order to know the radial distribution around the proton track of the energy deposited by the cascade of secondary electrons, a simulation has been performed that follows the motion of the electrons through the target taking into account both the inelastic interactions (via electronic ionizations and excitations as well as electron-phonon and electron trapping by polaron creation) and the elastic interactions. The radial distribution of the energy deposited by the secondary electrons around the proton track shows notable differences between the simulations performed with the extended-Drude ELF or the Mermin ELF, being the former more spread out (and, therefore, less peaked) than the latter. The highest intensity and sharpness of the deposited energy distributions takes place for proton beams incident with T ~ 0.1-1 MeV. We have also studied the influence in the radial distribution of deposited energy of using a full energy distribution of secondary electrons generated by proton impact or using a single value (namely, the average value of the distribution); our results show that differences between both simulations become important for proton energies larger than ~0.1 MeV. The results presented in this work have potential applications in materials science, as well as hadron therapy (due to the use of PMMA as a tissue phantom) in order to properly consider the

  5. Momentum-resolved electronic structure of the superconductor parent compound BaBiO3

    Science.gov (United States)

    Plumb, N. C.; Ristic, Z.; Park, J.; Wang, Z.; Matt, C. E.; Xu, N.; Lv, B. Q.; Gawryluk, D.; Pomjakushina, E.; Conder, K.; Wang, Y.; Johnston, S.; Mesot, J.; Shi, M.; Radovic, M.

    We use in situ angle-resolved photoemission to study thin films of BaBiO3, a parent compound of bismuthate superconductors with Tc up to 30 K. By simple electron counting, BaBiO3 should be metallic. However, in analogy with many unconventional and high-Tc superconductor families, it is instead insulating, and superconductivity emerges with doping. Our experiments reveal a folded band structure consistent with known BiO6 breathing distortions. However, charge ordering often thought to accompany the distortions is virtually nonexistent. The data combined with DFT calculations indicate that states near EF are primarily oxygen-derived. Hence BaBiO3 appears to be characterized by negative charge transfer energy. This can account for the seeming discrepancy between the atomic structure and ''missing'' charge order. It should also be relevant for understanding the doping evolution and superconductivity in bismuthates.

  6. Ultrafast Spin Density Wave Transition in Chromium Governed by Thermalized Electron Gas

    Science.gov (United States)

    Nicholson, C. W.; Monney, C.; Carley, R.; Frietsch, B.; Bowlan, J.; Weinelt, M.; Wolf, M.

    2016-09-01

    The energy and momentum selectivity of time- and angle-resolved photoemission spectroscopy is exploited to address the ultrafast dynamics of the antiferromagnetic spin density wave (SDW) transition photoexcited in epitaxial thin films of chromium. We are able to quantitatively extract the evolution of the SDW order parameter Δ through the ultrafast phase transition and show that Δ is governed by the transient temperature of the thermalized electron gas, in a mean field description. The complete destruction of SDW order on a sub-100 fs time scale is observed, much faster than for conventional charge density wave materials. Our results reveal that equilibrium concepts for phase transitions such as the order parameter may be utilized even in the strongly nonadiabatic regime of ultrafast photoexcitation.

  7. Ab initio electronic band structure study of III-VI layered semiconductors

    Science.gov (United States)

    Olguín, Daniel; Rubio-Ponce, Alberto; Cantarero, Andrés

    2013-08-01

    We present a total energy study of the electronic properties of the rhombohedral γ-InSe, hexagonal ɛ-GaSe, and monoclinic GaTe layered compounds. The calculations have been done using the full potential linear augmented plane wave method, including spin-orbit interaction. The calculated valence bands of the three compounds compare well with angle resolved photoemission measurements and a discussion of the small discrepancies found has been given. The present calculations are also compared with recent and previous band structure calculations available in the literature for the three compounds. Finally, in order to improve the calculated band gap value we have used the recently proposed modified Becke-Johnson correction for the exchange-correlation potential.

  8. Determining the band gap and mean kinetic energy of atoms from reflection electron energy loss spectra

    Energy Technology Data Exchange (ETDEWEB)

    Vos, M. [Atomic and Molecular Physics Laboratories, Research School of Physics and Engineering, Australian National University, Canberra ACT (Australia); Marmitt, G. G. [Atomic and Molecular Physics Laboratories, Research School of Physics and Engineering, Australian National University, Canberra ACT (Australia); Instituto de Fisica da Universidade Federal do Rio Grande do Sul, Avenida Bento Goncalves 9500, 91501-970 Porto Alegre, RS (Brazil); Finkelstein, Y. [Nuclear Research Center — Negev, Beer-Sheva 84190 (Israel); Moreh, R. [Physics Department, Ben-Gurion University of the Negev, Beer-Sheva 84105 (Israel)

    2015-09-14

    Reflection electron energy loss spectra from some insulating materials (CaCO{sub 3}, Li{sub 2}CO{sub 3}, and SiO{sub 2}) taken at relatively high incoming electron energies (5–40 keV) are analyzed. Here, one is bulk sensitive and a well-defined onset of inelastic excitations is observed from which one can infer the value of the band gap. An estimate of the band gap was obtained by fitting the spectra with a procedure that includes the recoil shift and recoil broadening affecting these measurements. The width of the elastic peak is directly connected to the mean kinetic energy of the atom in the material (Doppler broadening). The experimentally obtained mean kinetic energies of the O, C, Li, Ca, and Si atoms are compared with the calculated ones, and good agreement is found, especially if the effect of multiple scattering is taken into account. It is demonstrated experimentally that the onset of the inelastic excitation is also affected by Doppler broadening. Aided by this understanding, we can obtain a good fit of the elastic peak and the onset of inelastic excitations. For SiO{sub 2}, good agreement is obtained with the well-established value of the band gap (8.9 eV) only if it is assumed that the intensity near the edge scales as (E − E{sub gap}){sup 1.5}. For CaCO{sub 3}, the band gap obtained here (7 eV) is about 1 eV larger than the previous experimental value, whereas the value for Li{sub 2}CO{sub 3} (7.5 eV) is the first experimental estimate.

  9. Development of Grid Control Electron Gun for Multi-energy Irradiation Accelerator

    Institute of Scientific and Technical Information of China (English)

    HAN; Guang-wen; ZHU; Zhi-bin; WANG; Shu-xian

    2012-01-01

    <正>In the project of multi-energy electron irradiation accelerator, It is necessary to adjust the electron beam pulse inject to the accelerating tube. Under the same conditions of the injection energy, the grid controlled electron gun was used in the accelerator. Using cathode-grid assembly, after the simulation of electron optics program design, we manufactured focus electrode, the anode, and built an experiment

  10. Calculations of energies and absolute intensities of Auger electrons and X-rays arising from electron capture decay

    Institute of Scientific and Technical Information of China (English)

    ZHOU Chun-Mei; WU Zhen-Dong; HUANG Xiao-Long

    2005-01-01

    Calculations of energies and absolute intensities of Auger electron and X-ray arising from electron capture are introduced briefly. The calculation codes and main process are also presented. The application is also given by taking 55Fe ε decay as an example.

  11. Non-local electron energy probability function in a plasma expanding along a magnetic nozzle.

    Directory of Open Access Journals (Sweden)

    Roderick William Boswell

    2015-03-01

    Full Text Available Electron energy probability functions (eepfs have been measured along the axis of low pressure plasma expanding in a magnetic nozzle. The eepf at the maximum magnetic field of the nozzle shows a depleted tail commencing at an energy corresponding to the measured potential drop in the magnetic nozzle. The eepfs measured along the axis demonstrate that the potential and kinetic energies of the electrons are conserved and confirm the non-local collisionless kinetics of the electron dynamics.

  12. Correlation effects on the energy spectra of quantum dot electrons with harmonic model interactions

    Institute of Scientific and Technical Information of China (English)

    2000-01-01

    The low-lying excitation energy spectra of two, three and five quantum dot electrons with harmonic model interactions in a large magnetic field are calculated by the Hartree-Fock(HF) methods. Correlation effects on the energy level structures are investigated by comparing the HF results with the exact ones. It is found that the pure collective excitations(center-of-mass mode quanta) existing in the exact energy spectra do not appear in the HF energy spectra. The degeneracies of energy levels are also related to the correlation interactions, especially in the energy spectrum of two electrons. In the cases of more than two electrons, as the electron-electron interaction strength is increased the HF energy levels exhibit more complex crossings than the exact ones.

  13. Theoretical study of atoms by the electronic kinetic energy density and stress tensor density

    CERN Document Server

    Nozaki, Hiroo; Tachibana, Akitomo

    2016-01-01

    We analyze the electronic structure of atoms in the first, second and third periods using the electronic kinetic energy density and stress tensor density, which are local quantities motivated by quantum field theoretic consideration, specifically the rigged quantum electrodynamics. We compute the zero surfaces of the electronic kinetic energy density, which we call the electronic interfaces, of the atoms. We find that their sizes exhibit clear periodicity and are comparable to the conventional atomic and ionic radii. We also compute the electronic stress tensor density and its divergence, tension density, of the atoms, and discuss how their electronic structures are characterized by them.

  14. Electronic stopping power of hydrogen in KCl at the stopping maximum and at very low energies

    Science.gov (United States)

    Primetzhofer, D.; Markin, S. N.; Bauer, P.

    2011-10-01

    The electronic energy loss of hydrogen ions in KCl was investigated in a wide energy range. Thin films of KCl were evaporated on an Au/Si substrate. Rutherford Backscattering Spectrometry (RBS) was performed with protons and deuterons at energies from 30 to 400 keV/nucleon. At lower energies experiments were performed by Time-Of-Flight Low energy ion scattering (TOF-LEIS) again with proton and deuteron projectiles. Experimental results are compared to calculated/tabulated values for the electronic energy loss. Whereas at energies beyond the stopping maximum very good agreement is found, at lower ion energies discrepancies between experiment and calculations increase. At very low ion velocities the extrapolated stopping cross section ɛ predicts vanishing electronic energy loss at energies below 100 eV/nucleon.

  15. A DSP based power electronics interface for alternative /renewable energy system.

    Energy Technology Data Exchange (ETDEWEB)

    NONE

    1999-09-28

    This report is an update on the research project involving the implementation of a DSP-based power electronics interface for alternate/renewable energy systems, that was funded by the Department of Energy under the Inventions and Innovations program.

  16. Tailoring electron energy distribution functions through energy confinement in dual radio-frequency driven atmospheric pressure plasmas

    Energy Technology Data Exchange (ETDEWEB)

    O' Neill, C.; Waskoenig, J. [Centre for Plasma Physics, School of Maths and Physics, Queen' s University Belfast, Belfast BT7 1NN (United Kingdom); Gans, T. [Centre for Plasma Physics, School of Maths and Physics, Queen' s University Belfast, Belfast BT7 1NN (United Kingdom); York Plasma Institute, Department of Physics, University of York, York YO10 5DD (United Kingdom)

    2012-10-08

    A multi-scale numerical model based on hydrodynamic equations with semi-kinetic treatment of electrons is used to investigate the influence of dual frequency excitation on the effective electron energy distribution function (EEDF) in a radio-frequency driven atmospheric pressure plasma. It is found that variations of power density, voltage ratio, and phase relationship provide separate control over the electron density and the mean electron energy. This is exploited to directly influence both the phase dependent and time averaged effective EEDF. This enables tailoring the EEDF for enhanced control of non-equilibrium plasma chemical kinetics at ambient pressure and temperature.

  17. Energy modulation of nonrelativistic electrons in an optical near field on a metal microslit

    Science.gov (United States)

    Ishikawa, R.; Bae, J.; Mizuno, K.

    2001-04-01

    Energy modulation of nonrelativistic electrons with a laser beam using a metal microslit as an interaction circuit has been investigated. An optical near field is induced in the proximity of the microslit by illumination of the laser beam. The electrons passing close to the slit are accelerated or decelerated by an evanescent wave contained in the near field whose phase velocity is equal to the velocity of the electrons. The electron-evanescent wave interaction in the microslit has been analyzed theoretically and experimentally. The theory has predicted that electron energy can be modulated at optical frequencies. Experiments performed in the infrared region have verified theoretical predictions. The electron-energy changes of more than ±5 eV with a 10 kW CO2 laser pulse at the wavelength of 10.6 μm has been successfully observed for an electron beam with an energy of less than 80 keV.

  18. Low energy electron loss peaks of CuInTe/sub 2/

    Energy Technology Data Exchange (ETDEWEB)

    Kleint, C. (Karl-Marx-Universitaet, Leipzig (German Democratic Republic). Sektion Physik); Schulze, S. (Technische Hochschule, Karl-Marx-Stadt (German Democratic Republic). Sektion Physik/Elektronische Bauelemente); Tomlinson, R.D. (Salford Univ. (UK). Dept. of Electrical Engineering)

    1982-09-01

    Reflection low energy electron loss spectra were observed from CuInTe/sub 2/ monocrystals. The spectra were taken with a LEED system to obtain the first derivative of the scattered electron energy distribution using primary energies of 50, 90, and 190 eV. The second derivative and the loss maxima energies have been determined after a smoothing procedure. The loss peaks are coordinated to plasmon features, surfaces states, and interband transitions.

  19. Two-photon photoemission study of the coverage-dependent electronic structure of chemisorbed alkali atoms on a Ag(111) surface.

    Science.gov (United States)

    Wang, Lei-Ming; Sametoglu, Vahit; Winkelmann, Aimo; Zhao, Jin; Petek, Hrvoje

    2011-09-01

    We report a systematic investigation of the electronic structure of chemisorbed alkali atoms (Li-Cs) on a Ag(111) surface by two-photon photoemission spectroscopy. Angle-resolved two-photon photoemission spectra are obtained for 0-0.1 monolayer coverage of alkali atoms. The interfacial electronic structure as a function of periodic properties and the coverage of alkali atoms is observed and interpreted assuming ionic adsorbate/substrate interaction. The energy of the alkali atom σ-resonance at the limit of zero coverage is primarily determined by the image charge interaction, whereas at finite alkali atom coverages, it follows the formation of a dipolar surface field. The coverage- and angle-dependent two-photon photoemission spectra provide information on the photoinduced charge-transfer excitation of adsorbates on metal surfaces. This work complements the previous work on alkali/Cu(111) chemisorption [Phys. Rev. B 2008, 78, 085419].

  20. Low energy electron generator design and depth dose prediction for micro-superficies tumors treatment purposes

    Science.gov (United States)

    Khorshidi, Abdollah; Rajaee, Azimeh; Ahmadinejad, Marjan; Ghoranneviss, Mahmood; Ettelaee, Mehdi

    2014-09-01

    We investigate deposited energy and linear energy transfer (LET) of low energy ejection electrons in air and water layers of a generator design via a plasma source. A structured model of a concave cold cathode electron generator was designed and simulated by using Monte Carlo n-particle version X 2.7.0 (MCNPX) code. A negative dc high voltage was applied to a concave cathode up to -12 kV to determine electron energy activity. Results determined that the geometric dimensions of field size toward the anode increased in relation to the angle of the conic beam, widening the accumulated bulks. The increased field size increased the anode current, which also resulted in an increase of electron energy, a reduction in LET, a stretched build-up area and a dose curve that shifted to a higher depth. The biological effect of low energy electron radiation can be increased with an increase of LET; as the depth dose decreased, the electron energy increased at the same time. The study of electron irradiation as a conic beam from an electron generator may provide an accurate investigation of the indirect effect of low energy electrons on bystander cells.

  1. Technical Training: ELEC-2005 - Electronics in High Energy Physics

    CERN Multimedia

    Monique Duval

    2005-01-01

    Learning for the LHC! ELEC-2005 is a new course series on modern electronics, given by CERN physicists and engineers within the framework of the 2005 Technical Training Programme, in an extended format of the successful ELEC-2002 course series. This comprehensive course series is designed for people who are not electronics specialists, for example physicists, engineers and technicians working at or visiting the laboratory, who use or will use electronics in their present or future activities, in particular in the context of the LHC accelerator and experiments. ELEC-2005 is composed of four Terms that will run throughout the year: Winter Term: Introduction to electronics in HEP (January-February, 6 lectures) Spring Term: Integrated circuits and VLSI technology for physics (March, 6 lectures) Summer Term: System electronics for physics: Issues (May, 7 lectures) Autumn Term: Electronics applications in HEP experiments (November-December, 10 lectures) Lectures within each Term will take place on Tuesdays an...

  2. Suprathermal plasma analyzer for the measurement of low-energy electron distribution in the ionosphere.

    Science.gov (United States)

    Shimoyama, M; Oyama, K-I; Abe, T; Yau, A W

    2011-07-01

    It is commonly believed that an energy transfer from thermal to suprathermal electrons (thermal to suprathermal energy continuously with high-energy resolution of about 0.15 eV. The measurement principle is based on the combination of a retarding potential analyzer with a channel electron multiplier (CEM) and the Druyvesteyn method, which derives energy distribution from the current-voltage characteristics. The capability of detecting plasma space potential enables absolute calibration of electron energy. The instrument with a small vacuum pump, which is required for the CEM to work in low-vacuum region, was first successfully tested by a sounding rocket S-310-37 in the ionospheric E region. The instrument is expected to provide new opportunities to measure energy distribution of thermal and non-thermal electrons in low-density plasma, where a Langmuir probe cannot measure electron temperature because of low plasma density.

  3. A new semiclassical decoupling scheme for electronic transitions in molecular collisions - Application to vibrational-to-electronic energy transfer

    Science.gov (United States)

    Lee, H.-W.; Lam, K. S.; Devries, P. L.; George, T. F.

    1980-01-01

    A new semiclassical decoupling scheme (the trajectory-based decoupling scheme) is introduced in a computational study of vibrational-to-electronic energy transfer for a simple model system that simulates collinear atom-diatom collisions. The probability of energy transfer (P) is calculated quasiclassically using the new scheme as well as quantum mechanically as a function of the atomic electronic-energy separation (lambda), with overall good agreement between the two sets of results. Classical mechanics with the new decoupling scheme is found to be capable of predicting resonance behavior whereas an earlier decoupling scheme (the coordinate-based decoupling scheme) failed. Interference effects are not exhibited in P vs lambda results.

  4. New Free Electron Wire for Loss Free Utilization of Electrical Energy and Highly Energy Efficient Electrical Appliances

    Directory of Open Access Journals (Sweden)

    Sabyasachi Haldar

    2014-07-01

    Full Text Available New Free Electrons Wire will enable the use of electrical energy and also energy in various other forms, in a loss free way, at room temperature. Free Electrons confined in vacuum at the order of 10-4 torr or more, at the core of the wire, can move a distance as long as about, to a few kilometers without any collision. The vacuum is maintained in a tube made up of alternate layers of Teflon and Silicon Oxynitride. The columbic repulsion between these free electrons will actually conduct energy without any loss. The free electrons trapped in vacuum tube, should be at a particular density of around 2.02 x 108 electrons per unit area. A metal encapsulation(s over the wire is there to keep the electromagnetic field remain confined within the free electron wire, to make it harmless to the health of living creatures. Apart from loss free energy transportation, the free electron wire is also capable of generating very high electromagnetic field due to the free electrons, simply by removing the metal encapsulation(s, which can be used for various purposes. The materials and techniques adopted will make New Free Electron Wire producible commercially, at the cost of general copper wires.

  5. Energy dispersive X-ray analysis in the electron microscope

    CERN Document Server

    Bell, DC

    2003-01-01

    This book provides an in-depth description of x-ray microanalysis in the electron microscope. It is sufficiently detailed to ensure that novices will understand the nuances of high-quality EDX analysis. Includes information about hardware design as well as the physics of x-ray generation, absorption and detection, and most post-detection data processing. Details on electron optics and electron probe formation allow the novice to make sensible adjustments to the electron microscope in order to set up a system which optimises analysis. It also helps the reader determine which microanalytical me

  6. High energy gain of trapped electrons in a tapered, diffraction-dominated inverse-free-electron laser.

    Science.gov (United States)

    Musumeci, P; Tochitsky, S Ya; Boucher, S; Clayton, C E; Doyuran, A; England, R J; Joshi, C; Pellegrini, C; Ralph, J E; Rosenzweig, J B; Sung, C; Tolmachev, S; Travish, G; Varfolomeev, A A; Varfolomeev, A A; Yarovoi, T; Yoder, R B

    2005-04-22

    Energy gain of trapped electrons in excess of 20 MeV has been demonstrated in an inverse-free-electron-laser (IFEL) accelerator experiment. A 14.5 MeV electron beam is copropagated with a 400 GW CO2 laser beam in a 50 cm long undulator strongly tapered in period and field amplitude. The Rayleigh range of the laser, approximately 1.8 cm, is much shorter than the undulator length yielding a diffraction-dominated interaction. Experimental results on the dependence of the acceleration on injection energy, laser focus position, and laser power are discussed. Simulations, in good agreement with the experimental data, show that most of the energy gain occurs in the first half of the undulator at a gradient of 70 MeV/m and that the structure in the measured energy spectrum arises because of higher harmonic IFEL interaction in the second half of the undulator.

  7. Expeditious Stochastic Calculation of Random-Phase Approximation Energies for Thousands of Electrons in Three Dimensions.

    Science.gov (United States)

    Neuhauser, Daniel; Rabani, Eran; Baer, Roi

    2013-04-04

    A fast method is developed for calculating the random phase approximation (RPA) correlation energy for density functional theory. The correlation energy is given by a trace over a projected RPA response matrix, and the trace is taken by a stochastic approach using random perturbation vectors. For a fixed statistical error in the total energy per electron, the method scales, at most, quadratically with the system size; however, in practice, due to self-averaging, it requires less statistical sampling as the system grows, and the performance is close to linear scaling. We demonstrate the method by calculating the RPA correlation energy for cadmium selenide and silicon nanocrystals with over 1500 electrons. We find that the RPA correlation energies per electron are largely independent of the nanocrystal size. In addition, we show that a correlated sampling technique enables calculation of the energy difference between two slightly distorted configurations with scaling and a statistical error similar to that of the total energy per electron.

  8. Low Energy X-Ray and Electron Interactions within Matter.

    Science.gov (United States)

    1980-03-01

    Microscopy at Pomona College," Norelco Reporter, VII, 137 (1960). b."Isolation of Selected Elements with an Electron Microscope ," Norelco Reporter...38. "Measurement of Primary Electron Interaction Coefficients (500 to 1500 eV Region," Colloque International du C.N.R.S., Processus Electroniques

  9. Simulation of energy-dependent electron diffusion processes in the Earth's outer radiation belt

    Science.gov (United States)

    Ma, Q.; Li, W.; Thorne, R. M.; Nishimura, Y.; Zhang, X.-J.; Reeves, G. D.; Kletzing, C. A.; Kurth, W. S.; Hospodarsky, G. B.; Henderson, M. G.; Spence, H. E.; Baker, D. N.; Blake, J. B.; Fennell, J. F.; Angelopoulos, V.

    2016-05-01

    The radial and local diffusion processes induced by various plasma waves govern the highly energetic electron dynamics in the Earth's radiation belts, causing distinct characteristics in electron distributions at various energies. In this study, we present our simulation results of the energetic electron evolution during a geomagnetic storm using the University of California, Los Angeles 3-D diffusion code. Following the plasma sheet electron injections, the electrons at different energy bands detected by the Magnetic Electron Ion Spectrometer (MagEIS) and Relativistic Electron Proton Telescope (REPT) instruments on board the Van Allen Probes exhibit a rapid enhancement followed by a slow diffusive movement in differential energy fluxes, and the radial extent to which electrons can penetrate into depends on energy with closer penetration toward the Earth at lower energies than higher energies. We incorporate radial diffusion, local acceleration, and loss processes due to whistler mode wave observations to perform a 3-D diffusion simulation. Our simulation results demonstrate that chorus waves cause electron flux increase by more than 1 order of magnitude during the first 18 h, and the subsequent radial extents of the energetic electrons during the storm recovery phase are determined by the coupled radial diffusion and the pitch angle scattering by EMIC waves and plasmaspheric hiss. The radial diffusion caused by ULF waves and local plasma wave scattering are energy dependent, which lead to the observed electron flux variations with energy dependences. This study suggests that plasma wave distributions in the inner magnetosphere are crucial for the energy-dependent intrusions of several hundred keV to several MeV electrons.

  10. Velocity Dispersion of Correlated Energy Spread Electron Beams in the Free Electron Laser

    CERN Document Server

    Campbell, L T

    2016-01-01

    The effects of a correlated linear energy/velocity chirp in the electron beam in the FEL, and how to compensate for its effects by using an appropriate taper (or reverse-taper) of the undulator magnetic field, is well known. The theory, as described thus far, ignores velocity dispersion from the chirp in the undulator, taking the limit of a `small' chirp. In the following, the physics of compensating for chirp in the beam is revisited, including the effects of velocity dispersion, or beam compression or decompression, in the undulator. It is found that the limit of negligible velocity dispersion in the undulator is different from that previously identified as the small chirp limit, and is more significant than previously considered. The velocity dispersion requires a taper which is non-linear to properly compensate for the effects of the detuning, and also results in a varying peak current (end thus a varying gain length) over the length of the undulator. The results may be especially significant for plasma d...

  11. eV-TEM: Transmission electron microscopy in a low energy cathode lens instrument

    Energy Technology Data Exchange (ETDEWEB)

    Geelen, Daniël, E-mail: geelen@physics.leidenuniv.nl [Huygens-Kamerlingh Onnes Laboratory, Leiden Institute of Physics, Leiden University, P.O. Box 9504, 2300 RA Leiden (Netherlands); Thete, Aniket [Huygens-Kamerlingh Onnes Laboratory, Leiden Institute of Physics, Leiden University, P.O. Box 9504, 2300 RA Leiden (Netherlands); Schaff, Oliver; Kaiser, Alexander [SPECS GmbH, Voltastrasse 5, D-13355 Berlin (Germany); Molen, Sense Jan van der [Huygens-Kamerlingh Onnes Laboratory, Leiden Institute of Physics, Leiden University, P.O. Box 9504, 2300 RA Leiden (Netherlands); Tromp, Rudolf [IBM T.J. Watson Research Center, 1101 Kitchawan Road, P.O. Box 218, Yorktown Heights, NY 10598 (United States)

    2015-12-15

    We are developing a transmission electron microscope that operates at extremely low electron energies, 0–40 eV. We call this technique eV-TEM. Its feasibility is based on the fact that at very low electron energies the number of energy loss pathways decreases. Hence, the electron inelastic mean free path increases dramatically. eV-TEM will enable us to study elastic and inelastic interactions of electrons with thin samples. With the recent development of aberration correction in cathode lens instruments, a spatial resolution of a few nm appears within range, even for these very low electron energies. Such resolution will be highly relevant to study biological samples such as proteins and cell membranes. The low electron energies minimize adverse effects due to radiation damage. - Highlights: • We present a new way of performing low energy transmission electron microscopy in an aberration corrected LEEM/PEEM instrument. • We show a proof of principle where we measure transmitted electrons through a suspended graphene monolayer with a preliminary setup. • We present an improved setup design that provides better control of the incident electron beam.

  12. Treatment of Electronic Energy Level Transition and Ionization Following the Particle-Based Chemistry Model

    Science.gov (United States)

    Liechty, Derek S.; Lewis, Mark

    2010-01-01

    A new method of treating electronic energy level transitions as well as linking ionization to electronic energy levels is proposed following the particle-based chemistry model of Bird. Although the use of electronic energy levels and ionization reactions in DSMC are not new ideas, the current method of selecting what level to transition to, how to reproduce transition rates, and the linking of the electronic energy levels to ionization are, to the author s knowledge, novel concepts. The resulting equilibrium temperatures are shown to remain constant, and the electronic energy level distributions are shown to reproduce the Boltzmann distribution. The electronic energy level transition rates and ionization rates due to electron impacts are shown to reproduce theoretical and measured rates. The rates due to heavy particle impacts, while not as favorable as the electron impact rates, compare favorably to values from the literature. Thus, these new extensions to the particle-based chemistry model of Bird provide an accurate method for predicting electronic energy level transition and ionization rates in gases.

  13. Determining binding energies of valence-band electrons in insulators and semiconductors via lanthanide spectroscopy

    NARCIS (Netherlands)

    Dorenbos, P.

    2013-01-01

    Models and methods to determine the absolute binding energy of 4f-shell electrons in lanthanide dopants will be combined with data on the energy of electron transfer from the valence band to a lanthanide dopant. This work will show that it provides a powerful tool to determine the absolute binding e

  14. 77 FR 13109 - Petition for Waiver of Samsung Electronics America, Inc. From the Department of Energy...

    Science.gov (United States)

    2012-03-05

    ... of Energy Efficiency and Renewable Energy Petition for Waiver of Samsung Electronics America, Inc.... SUMMARY: This notice announces receipt of and publishes the Samsung Electronics America, Inc. (Samsung...-freezers. In its petition, Samsung provides an alternate test procedure that is the same as the...

  15. Dynamic Behavior and Quasi-energy Spectrum of Multiband Superlattice Bloch Electrons in Quantum Kicked Potential

    Institute of Scientific and Technical Information of China (English)

    OUYANG BiYao; ZHAO XianGeng; CHEN ShiGang; LIU Jie

    2001-01-01

    In this paper, we study the dynamic behavior and quasi-energy spectrum of multiband superlattice Bloch electrons in quantum kicked potential. We show analytically and numerically the avoided crossing and band suppression about the quasi-energy spectrum, the dynamic nonlocalization, and the electron oscillation behavior between two bands.

  16. D-mu-A new concept in industrial low-energy electron dosimetry

    DEFF Research Database (Denmark)

    Helt-Hansen, Jakob; Miller, Arne; Sharpe, Peter;

    2010-01-01

    Irradiation with low-energy electrons (100–300 keV) results in dose gradients across the thickness of the dosimeters that are typically used for dose measurement at these energies. This leads to different doses being measured with different thickness dosimeters irradiated at the same electron bea...

  17. A magnetic-free high-resolution parabolic mirror time-of-flight electron energy spectrometer

    Institute of Scientific and Technical Information of China (English)

    张戈; 沈鸿元; 曾瑞荣; 黄呈辉; 林文雄; 黄见洪

    2001-01-01

    The principle and structure of a magnetic-free high-resolution high-efficiency parabolic mirror time-offligght electron energy spectrometer are presented. The electron energy spectrum of Nz in a flight tube is measured using a 105 fs Ti:sappbire laser under different gas pressures.

  18. Solar energy absorption in norbornadiene-quadricyclane system through electron donating or withdrawing substituents1

    Science.gov (United States)

    Edjlali, L.; Vessally, E.; Abbasian, M.

    2011-05-01

    An attempt is made to maximize the solar energy absorption in norbornadiene ( 1)-quadricyclane ( 2) system, through direct attachment of substituents at C1, C2, or C7 atoms of 1; calculating the corresponding energies at B3LYP/6-311++G** level of theory. The electron donating and electron withdrawing substituents of 1 n-X, attached at C2, were suitable for both solar absorption bands and solar energy storage. DFT calculations indicate that the solar absorption bands of 12-X were shifted to the visible spectrum region through the electron withdrawing substituents more than through electron donating substituents.

  19. Differential cross sections for electron-impact vibrational-excitation of tetrahydrofuran at intermediate impact energies

    Energy Technology Data Exchange (ETDEWEB)

    Do, T. P. T. [School of Chemical and Physical Sciences, Flinders University, GPO Box 2100, Adelaide, South Australia 5001 (Australia); School of Education, Can Tho University, Campus II, 3/2 Street, Xuan Khanh, Ninh Kieu, Can Tho City (Viet Nam); Duque, H. V. [School of Chemical and Physical Sciences, Flinders University, GPO Box 2100, Adelaide, South Australia 5001 (Australia); Departamento de Física, Universidade Federal de Juiz de Fora, 36036-330 Juiz de Fora, Minas Gerais (Brazil); Lopes, M. C. A. [Departamento de Física, Universidade Federal de Juiz de Fora, 36036-330 Juiz de Fora, Minas Gerais (Brazil); Konovalov, D. A.; White, R. D. [College of Science, Technology and Engineering, James Cook University, Townsville (Australia); Brunger, M. J., E-mail: michael.brunger@flinders.edu.au, E-mail: darryl.jones@flinders.edu.au [School of Chemical and Physical Sciences, Flinders University, GPO Box 2100, Adelaide, South Australia 5001 (Australia); Institute of Mathematical Sciences, University of Malaya, 50603 Kuala Lumpur (Malaysia); Jones, D. B., E-mail: michael.brunger@flinders.edu.au, E-mail: darryl.jones@flinders.edu.au [School of Chemical and Physical Sciences, Flinders University, GPO Box 2100, Adelaide, South Australia 5001 (Australia)

    2015-03-28

    We report differential cross sections (DCSs) for electron-impact vibrational-excitation of tetrahydrofuran, at intermediate incident electron energies (15-50 eV) and over the 10°-90° scattered electron angular range. These measurements extend the available DCS data for vibrational excitation for this species, which have previously been obtained at lower incident electron energies (≤20 eV). Where possible, our data are compared to the earlier measurements in the overlapping energy ranges. Here, quite good agreement was generally observed where the measurements overlapped.

  20. An efficient implementation of the localized operator partitioning method for electronic energy transfer

    CERN Document Server

    Nagesh, Jayashree; Brumer, Paul

    2014-01-01

    The localized operator partitioning method [Y. Khan and P. Brumer, J. Chem. Phys. 137, 194112 (2012)] rigorously defines the electronic energy on any subsystem within a molecule and gives a precise meaning to the subsystem ground and excited electronic energies, which is crucial for investigating electronic energy transfer from first principles. However, an efficient implementation of this approach has been hindered by complicated one- and two-electron integrals arising in its formulation. Using a resolution of the identity in the definition of partitioning we reformulate the method in a computationally e?cient manner that involves standard one- and two-electron integrals. We apply the developed algorithm to the 9-((1-naphthyl)-methyl)-anthracene (A1N) molecule by partitioning A1N into anthracenyl and CH2-naphthyl groups as subsystems, and examine their electronic energies and populations for several excited states using Configuration Interaction Singles method. The implemented approach shows a wide variety o...

  1. Electromagnetic cascade in high energy electron, positron, and photon interactions with intense laser pulses

    CERN Document Server

    Bulanov, S S; Esarey, E; Leemans, W P

    2013-01-01

    The interaction of high energy electrons, positrons, and photons with intense laser pulses is studied in head-on collision geometry. It is shown that electrons and/or positrons undergo a cascade-type process involving multiple emissions of photons. These photons can consequently convert into electron-positron pairs. As a result charged particles quickly lose their energy developing an exponentially decaying energy distribution, which suppresses the emission of high energy photons, thus reducing the number of electron-positron pairs being generated. Therefore, this type of interaction suppresses the development of the electromagnetic avalanche-type discharge, i.e., the exponential growth of the number of electrons, positrons, and photons does not occur in the course of interaction. The suppression will occur when 3D effects can be neglected in the transverse particle orbits, i.e., for sufficiently broad laser pulses with intensities that are not too extreme. The final distributions of electrons, positrons, and...

  2. Energy Levels in Helium and Neon Atoms by an Electron-Impact Method.

    Science.gov (United States)

    Taylor, N.; And Others

    1981-01-01

    Electronic energy levels in noble gas atoms may be determined with a simple teaching apparatus incorporating a resonance potentials tube in which the electron beam intensity is held constant. The resulting spectra are little inferior to those obtained by more elaborate electron-impact methods and complement optical emission spectra. (Author/SK)

  3. Low-energy electron microscopy on two-dimensional systems : : growth, potentiometry and band structure mapping

    NARCIS (Netherlands)

    Kautz, Jaap

    2015-01-01

    Low Energy Electron Microscopy (LEEM) is a microscopy technique typically used to study surface processes. The sample is illuminated with a parallel beam of electrons under normal incidence and the reflected electrons are projected onto a pixelated detector, where an image is formed. In the first

  4. A Low-Energy-Spread Rf Accelerator for a Far-Infrared Free-Electron Laser

    NARCIS (Netherlands)

    van der Geer, C. A. J.; Bakker, R. J.; van der Meer, A. F. G.; van Amersfoort, P. W.; Gillespie, W. A.; Saxon, G.; Poole, M. W.

    1993-01-01

    A high electron current and a small energy spread are essential for the operation of a free electron laser (FEL). In this paper we discuss the design and performance of the accelerator for FELIX, the free electron laser for infrared experiments. The system consists of a thermionic gun, a prebuncher,

  5. Comparative analysis of characteristic electron energy loss spectra and inelastic scattering cross-section spectra of Fe

    Science.gov (United States)

    Parshin, A. S.; Igumenov, A. Yu.; Mikhlin, Yu. L.; Pchelyakov, O. P.; Zhigalov, V. S.

    2016-05-01

    The inelastic electron scattering cross section spectra of Fe have been calculated based on experimental spectra of characteristic reflection electron energy loss as dependences of the product of the inelastic mean free path by the differential inelastic electron scattering cross section on the electron energy loss. It has been shown that the inelastic electron scattering cross-section spectra have certain advantages over the electron energy loss spectra in the analysis of the interaction of electrons with substance. The peaks of energy loss in the spectra of characteristic electron energy loss and inelastic electron scattering cross sections have been determined from the integral and differential spectra. It has been shown that the energy of the bulk plasmon is practically independent of the energy of primary electrons in the characteristic electron energy loss spectra and monotonically increases with increasing energy of primary electrons in the inelastic electron scattering cross-section spectra. The variation in the maximum energy of the inelastic electron scattering cross-section spectra is caused by the redistribution of intensities over the peaks of losses due to various excitations. The inelastic electron scattering cross-section spectra have been analyzed using the decomposition of the spectra into peaks of the energy loss. This method has been used for the quantitative estimation of the contributions from different energy loss processes to the inelastic electron scattering cross-section spectra of Fe and for the determination of the nature of the energy loss peaks.

  6. Electronic structure studies of topological materials

    Science.gov (United States)

    Zhou, Shuyun

    Three-dimensional (3D) Dirac fermions are a new class of topological quantum materials. In 3D Dirac semimetals, the conduction and valence bands touch each other at discrete points in the momentum space and show linear dispersions along all momentum directions, forming 3D Dirac cones which are protected by the crystal symmetry. Here I will present our recent studies of the electronic structures of novel materials which host 3D Dirac fermions by using angle-resolved photoemission spectroscopy.

  7. Momentum-Resolved Electronic Structure of the High-T_{c} Superconductor Parent Compound BaBiO_{3}.

    Science.gov (United States)

    Plumb, N C; Gawryluk, D J; Wang, Y; Ristić, Z; Park, J; Lv, B Q; Wang, Z; Matt, C E; Xu, N; Shang, T; Conder, K; Mesot, J; Johnston, S; Shi, M; Radović, M

    2016-07-15

    We investigate the band structure of BaBiO_{3}, an insulating parent compound of doped high-T_{c} superconductors, using in situ angle-resolved photoemission spectroscopy on thin films. The data compare favorably overall with density functional theory calculations within the local density approximation, demonstrating that electron correlations are weak. The bands exhibit Brillouin zone folding consistent with known BiO_{6} breathing distortions. Though the distortions are often thought to coincide with Bi^{3+}/Bi^{5+} charge ordering, core level spectra show that bismuth is monovalent. We further demonstrate that the bands closest to the Fermi level are primarily oxygen derived, while the bismuth 6s states mostly contribute to dispersive bands at deeper binding energy. The results support a model of Bi-O charge transfer in which hole pairs are localized on combinations of the O 2p orbitals.

  8. Direct observation of electron-to-hole energy transfer in CdSe quantum dots.

    Science.gov (United States)

    Hendry, E; Koeberg, M; Wang, F; Zhang, H; de Mello Donegá, C; Vanmaekelbergh, D; Bonn, M

    2006-02-10

    We independently determine the subpicosecond cooling rates for holes and electrons in CdSe quantum dots. Time-resolved luminescence and terahertz spectroscopy reveal that the rate of hole cooling, following photoexcitation of the quantum dots, depends critically on the electron excess energy. This constitutes the first direct, quantitative measurement of electron-to-hole energy transfer, the hypothesis behind the Auger cooling mechanism proposed in quantum dots, which is found to occur on a 1 +/- 0.15 ps time scale.

  9. Imaging the potential distribution of charged adsorbates on graphene by low-energy electron holography

    CERN Document Server

    Latychevskaia, Tatiana; Escher, Conrad; Fink, Hans-Werner

    2016-01-01

    While imaging individual atoms can routinely be achieved in high resolution transmission electron microscopy, visualizing the potential distribution of individually charged adsorbates leading to a phase shift of the probing electron wave is still a challenging task. Since low-energy electrons are sensitive to localized potential gradients, we employed this tool in the 30 eV kinetic energy range to visualize the potential distribution of localized charged adsorbates present on free-standing graphene.

  10. Stopping power for electrons in pyrimidine in the energy range 20-3000 eV.

    Science.gov (United States)

    Colmenares, R; Sanz, A G; Fuss, M C; Blanco, F; García, G

    2014-01-01

    In this work, we present new experimental electron energy loss distribution functions for pyrimidine (C4H4N2) measured for the incident energy range 30-2000 eV. Theoretical total and elastic cross sections for electron scattering from pyrimidine were calculated using the screening-corrected additivity rule (IAM-SCAR) method. Based on the mean energy loss observed in the experiment and the theoretical integral inelastic cross section, the stopping power for electrons in pyrimidine is calculated in the energy range 20-3000 eV.

  11. Direct Measurement of the Band Structure of a Buried Two-Dimensional Electron Gas

    DEFF Research Database (Denmark)

    Miwa, Jill; Hofmann, Philip; Simmons, Michelle Y.;

    2013-01-01

    We directly measure the band structure of a buried two dimensional electron gas (2DEG) using angle resolved photoemission spectroscopy. The buried 2DEG forms 2 nm beneath the surface of p-type silicon, because of a dense delta-type layer of phosphorus n-type dopants which have been placed there. ...

  12. Electronic structure of the quasi-one-dimensional organic conductor TTF-TCNQ

    DEFF Research Database (Denmark)

    Sing, M.; Schwingenschlögl, U.; Claessen, R.;

    2003-01-01

    We study the electronic structure of the quasi-one-dimensional organic conductor TTF-TCNQ by means of density-functional band theory, Hubbard model calculations, and angle-resolved photoelectron spectroscopy (ARPES). The experimental spectra reveal significant quantitative and qualitative...

  13. Clocked, fast electronics trigger for high energy physics

    Energy Technology Data Exchange (ETDEWEB)

    Gray, R.; Rutherfoord, J.P.

    1986-04-01

    For a Fermilab experiment we have designed and built gated-pulse-stretcher modules which allow us to clock all of the fast electronics with the accelerator rf, thus simplifying the trigger design. (orig.).

  14. A Low-Cost Electronic Solar Energy Control

    Science.gov (United States)

    Blade, Richard A.; Small, Charles T.

    1978-01-01

    Describes the design of a low-cost electronic circuit to serve as a differential thermostat, to control the operation of a solar heating system. It uses inexpensive diodes for sensoring temperature, and a mechanical relay for a switch. (GA)

  15. Correlation between energy deposition and molecular damage from Auger electrons: A case study of ultra-low energy (5–18 eV) electron interactions with DNA

    Energy Technology Data Exchange (ETDEWEB)

    Rezaee, Mohammad, E-mail: Mohammad.Rezaee@USherbrooke.ca; Hunting, Darel J.; Sanche, Léon [Groupe en Sciences des Radiations, Département de Médecine Nucléaire et Radiobiologie, Faculté de Médecine et des Sciences de la Santé, Université de Sherbrooke, Sherbrooke, Québec J1H 5N4 (Canada)

    2014-07-15

    Purpose: The present study introduces a new method to establish a direct correlation between biologically related physical parameters (i.e., stopping and damaging cross sections, respectively) for an Auger-electron emitting radionuclide decaying within a target molecule (e.g., DNA), so as to evaluate the efficacy of the radionuclide at the molecular level. These parameters can be applied to the dosimetry of Auger electrons and the quantification of their biological effects, which are the main criteria to assess the therapeutic efficacy of Auger-electron emitting radionuclides. Methods: Absorbed dose and stopping cross section for the Auger electrons of 5–18 eV emitted by{sup 125}I within DNA were determined by developing a nanodosimetric model. The molecular damages induced by these Auger electrons were investigated by measuring damaging cross section, including that for the formation of DNA single- and double-strand breaks. Nanoscale films of pure plasmid DNA were prepared via the freeze-drying technique and subsequently irradiated with low-energy electrons at various fluences. The damaging cross sections were determined by employing a molecular survival model to the measured exposure–response curves for induction of DNA strand breaks. Results: For a single decay of{sup 125}I within DNA, the Auger electrons of 5–18 eV deposit the energies of 12.1 and 9.1 eV within a 4.2-nm{sup 3} volume of a hydrated or dry DNA, which results in the absorbed doses of 270 and 210 kGy, respectively. DNA bases have a major contribution to the deposited energies. Ten-electronvolt and high linear energy transfer 100-eV electrons have a similar cross section for the formation of DNA double-strand break, while 100-eV electrons are twice as efficient as 10 eV in the induction of single-strand break. Conclusions: Ultra-low-energy electrons (<18 eV) substantially contribute to the absorbed dose and to the molecular damage from Auger-electron emitting radionuclides; hence, they should

  16. Power Electronics – The Key Technology for Renewable Energy System Integration

    DEFF Research Database (Denmark)

    Blaabjerg, Frede; Yang, Yongheng; Ma, Ke

    2015-01-01

    and effectively, energy conversion systems, currently based on power electronics technology, will again play an essential role in this energy paradigm shift. Using highly efficient power electronics in power generation, power transmission/distribution and end-user application, together with advanced control...... solutions makes the way for renewable energies. In light of this, some of the most emerging renewable energies, e.g. wind energy and photovoltaic, which by means of power electronics are changing character as a major part in the electricity generation, are explored in this presentation. Issues like...... technology development, implementation, power converter technologies, control of the systems, and synchronization are addressed. Special focuses are paid on the future trends in power electronics for those systems like how to lower the cost of energy and to develop emerging power devices and better...

  17. Energy dissipation of energetic electrons in the inhomogeneous intergalactic medium during the epoch of reionization

    CERN Document Server

    Kaurov, Alexander A

    2015-01-01

    We explore a time-dependent energy dissipation of the energetic electrons in the inhomogeneous intergalactic medium (IGM) during the epoch of cosmic reionization. In addition to the atomic processes we take into account the Inverse Compton (IC) scattering of the electrons on the comic microwave background (CMB) photons, which is the dominant channel of energy loss for the electrons with energies above a few MeV. We show that: (1) the effect on the IGM has both local (atomic processes) and non-local (IC radiation) components; (2) the energy distribution between Hydrogen and Helium ionizations depends on the initial electron energy; (3) the local baryon overdensity significantly affects the fractions of energy distributed in each channel; and (4) the relativistic effect of atomic cross section become important during the epoch of cosmic reionization. We release our code as open source for further modification by the community.

  18. Contribution from individual nearby sources to the spectrum of high-energy cosmic-ray electrons

    Energy Technology Data Exchange (ETDEWEB)

    Sedrati, R., E-mail: rafik.sedrati@univ-annaba.org; Attallah, R.

    2014-04-01

    In the last few years, very important data on high-energy cosmic-ray electrons and positrons from high-precision space-born and ground-based experiments have attracted a great deal of interest. These particles represent a unique probe for studying local comic-ray accelerators because they lose energy very rapidly. These energy losses reduce the lifetime so drastically that high-energy cosmic-ray electrons can attain the Earth only from rather local astrophysical sources. This work aims at calculating, by means of Monte Carlo simulation, the contribution from some known nearby astrophysical sources to the cosmic-ray electron/positron spectra at high energy (≥10GeV). The background to the electron energy spectrum from distant sources is determined with the help of the GALPROP code. The obtained numerical results are compared with a set of experimental data.

  19. Ultrafast quenching of electron-boson interaction and superconducting gap in a cuprate superconductor.

    Science.gov (United States)

    Zhang, Wentao; Hwang, Choongyu; Smallwood, Christopher L; Miller, Tristan L; Affeldt, Gregory; Kurashima, Koshi; Jozwiak, Chris; Eisaki, Hiroshi; Adachi, Tadashi; Koike, Yoji; Lee, Dung-Hai; Lanzara, Alessandra

    2014-01-01

    Ultrafast spectroscopy is an emerging technique with great promise in the study of quantum materials, as it makes it possible to track similarities and correlations that are not evident near equilibrium. Thus far, however, the way in which these processes modify the electron self-energy--a fundamental quantity describing many-body interactions in a material--has been little discussed. Here we use time- and angle-resolved photoemission to directly measure the ultrafast response of self-energy to near-infrared photoexcitation in high-temperature cuprate superconductor. Below the critical temperature of the superconductor, ultrafast excitations trigger a synchronous decrease of electron self-energy and superconducting gap, culminating in a saturation in the weakening of electron-boson coupling when the superconducting gap is fully quenched. In contrast, electron-boson coupling is unresponsive to ultrafast excitations above the critical temperature of the superconductor and in the metallic state of a related material. These findings open a new pathway for studying transient self-energy and correlation effects in solids.

  20. Determination of electronic properties of nanostructures using reflection electron energy loss spectroscopy: Nano-metalized polymer as case study

    Energy Technology Data Exchange (ETDEWEB)

    Deris, Jamileh [Department of Physics, Yasouj University, Yasouj 75918-74831 (Iran, Islamic Republic of); Hajati, Shaaker, E-mail: Hajati@mail.yu.ac.ir [Department of Physics, Yasouj University, Yasouj 75918-74831 (Iran, Islamic Republic of); Tougaard, Sven [Department of Physics, Chemistry and Pharmacy, University of Southern Denmark, 5230 Odense M (Denmark); Zaporojtchenko, Vladimir [Lehrstuhl fur Materialverbunde, Technische Fakultat der CAU, Kaiserstr 2, D-24143 Kiel (Germany)

    2016-07-30

    Highlights: • Application of reflection electron energy loss spectroscopy. • Determination of electron inelastic cross section of Nano-metalized Polymer. • Determination of energy loss function of Nano-metalized Polymer. • Determination of electron inelastic mean free path of Nano-metalized Polymer. • Determination of surface excitation parameters of Nano-metalized Polymer. - Abstract: In this work, Au was deposited with nominal effective thickness of 0.8 nm on polystyrene (PS) at room temperature. According to previous study, using XPS peak shape analysis [S. Hajati, V. Zaporojtchenko, F. Faupel, S. Tougaard, Surf. Sci. 601 (2007) 3261–3267], Au nanoparticles (Au-NPs) of sizes 5.5 nm were formed corresponding to such effective thickness (0.8 nm). Then the sample was annealed to 200 °C, which is far above the glass transition of PS. At this temperature, the Au-NPs were diffused within the depth 0.5 nm–6.5 nm as found using nondestructive XPS peak shape analysis. Electrons with primary energy 500 eV were used because the electronic properties will then be probed in utmost surface (∼1 IMFP range of depths that is 1.8 nm for PS). By using QUEELS software, theoretical and experimental electron inelastic cross section, energy loss function, electron inelastic mean free path and surface excitation parameters were obtained for the sample. The information obtained here, does not rely on any previously known information on the sample. This means that the method, applied here, is suitable for the determination of the electronic properties of new and unknown composite nanostructures.

  1. A study of energy gap, refractive index and electronic polarizability of ternary chalcopyrite semiconductors

    Directory of Open Access Journals (Sweden)

    A Ahmad

    2014-12-01

    Full Text Available A simple relation between the optical electronegativity, energy gap, refractive index and electronic polarizability is given for ternary chalcopyrite semiconductors. Energy gap has been evaluated from the optical electronegativity whereas refractive index and electronic polarizability values have been evaluated from the energy gap by proposing a linear relation between them. The calculated values are in fair agreement with the experimental values and earlier researchers. This work highlights the significance of interrelation between these parameters.

  2. Design, Synthesis, and Characterization of High Performance Polymer Electrolytes for Printed Electronics and Energy Storage

    Science.gov (United States)

    2016-03-31

    AFRL-AFOSR-VA-TR-2016-0168 Design, Synthesis, and Characterization of High Performance Polymer Electrolytes for Printed Electronics and Energy ...Sep 2015 4. TITLE AND SUBTITLE Design, Synthesis, and Characterization of High Performance Polymer Electrolytes for Printed Electronics and Energy ... energy storage. This project produced 11 peer reviewed papers and results in the training of 3 graduate students and two postdoctoral fellows. The

  3. Coherent diffraction and holographic imaging of individual biomolecules using low-energy electrons

    CERN Document Server

    Latychevskaia, Tatiana; Escher, Conrad; Fink, Hans-Werner

    2013-01-01

    Modern microscopy techniques are aimed at imaging an individual molecule at atomic resolution. Here we show that low-energy electrons with kinetic energies of 50-250 eV offer a possibility of overcome the problem of radiation damage, and obtaining images of individual biomolecules. Two experimental schemes for obtaining images of individual molecules, holography and coherent diffraction imaging, are discussed and compared. Images of individual molecules obtained by both techniques, using low-energy electrons, are shown.

  4. Computation of energy states of hydrogenic quantum dot with two-electrons

    Science.gov (United States)

    Yakar, Y.; Özmen, A.; ćakır, B.

    2016-03-01

    In this study we have investigated the electronic structure of the hydrogenic quantum dot with two electrons inside an impenetrable potential surface. The energy eigenvalues and wavefunctions of the ground and excited states of spherical quantum dot have been calculated by using the Quantum Genetic Algorithm (QGA) and Hartree-Fock Roothaan (HFR) method, and the energies are investigated as a function of dot radius. The results show that as dot radius increases, the energy of quantum dot decreases.

  5. Reexamination of the Electronic Structure of Bi{sub 2}Sr{sub 2}CaCu{sub 2}O{sub 8 +{delta}} and Bi{sub 2}Sr{sub 2}Cu{sub 1}O{sub 6+{delta}} : Electronlike Portions of the Fermi Surface and Depletion of Spectral Weight near {bar M}

    Energy Technology Data Exchange (ETDEWEB)

    Chuang, Y.; Gromko, A.D.; Dessau, D.S. [Department of Physics, University of Colorado, Boulder, Colorado 80309-0390 (United States); Aiura, Y.; Yamaguchi, Y.; Oka, K. [Electrotechnical Laboratory (ETL), 1-1-4 Umezono, Tsukuba, Ibaraki 305 (Japan); Arko, A.J.; Joyce, J. [Los Alamos National Laboratory, Los Alamos, New Mexico 87545 (United States); Eisaki, H.; Uchida, S.I. [Department of Superconductivity, University of Tokyo, 7-3-1 Hongo, Bunkyo-ku, Tokyo 113 (Japan); Nakamura, K.; Ando, Y. [Central Research Institute of Electric Power Industry (CRIEPI), 2-11-1 Iwato-Kita, Komae, Tokyo 201-8511 (Japan)

    1999-11-01

    We present a reexamination of the electronic structure and Fermi surface (FS) topology of Bi-Sr-Ca-Cu-O (BSCCO) as obtained from angle-resolved photoemission experiments. By applying a stricter set of FS crossing criteria as well as by varying the incident photon energy outside the usual range, we have found very different behavior from that previously observed. In particular, we have found a FS that is centered around the {Gamma} point and contains electronlike portions, and we observe a depletion of spectral weight around {bar M} . The flat bands observed at other photon energies may indicate the presence of two electronic components in the cuprates. {copyright} {ital 1999} {ital The American Physical Society }

  6. Noninvasive measurement of micron electron beam size of high energy using diffraction radiation

    CERN Document Server

    Naumenko, G A

    2003-01-01

    Treatments of the usage of diffraction radiation from the relativistic electrons moving though a conductive slit for the transverse beam size measurement encounter hard limitation of the method sensitivity for the electron energy larger than 1 GeV. We consider in this article a possibility of application of the artificial phase shift, which can take place when transverse electron position varies. This allows us to realize the measurements of transverse size of supper-relativistic electron beams with the small emittance.

  7. Two-Electron Energy Spectrum in a Parabolic Quantum Dot Under a Magnetic Field

    Institute of Scientific and Technical Information of China (English)

    XIE Wen-Fang

    2003-01-01

    Two interacting electrons in a harmonic oscillator potential under the influence of a perpendicular homo-geneous magnetic field are considered. The energies of two-electron quantum dots with the electron-LO-phonon couplingas a function of magnetic field are calculated. Calculations are made by using the method of few-body physics withinthe effective-mass approximation. Our results show that the electron-LO-phonon coupling effect is very important insemiconductor quantum dots.

  8. High-Brightness High-Energy Electron Beams from a Laser Wakefield Accelerator via Energy Chirp Control

    Science.gov (United States)

    Wang, W. T.; Li, W. T.; Liu, J. S.; Zhang, Z. J.; Qi, R.; Yu, C. H.; Liu, J. Q.; Fang, M.; Qin, Z. Y.; Wang, C.; Xu, Y.; Wu, F. X.; Leng, Y. X.; Li, R. X.; Xu, Z. Z.

    2016-09-01

    By designing a structured gas density profile between the dual-stage gas jets to manipulate electron seeding and energy chirp reversal for compressing the energy spread, we have experimentally produced high-brightness high-energy electron beams from a cascaded laser wakefield accelerator with peak energies in the range of 200-600 MeV, 0.4%-1.2% rms energy spread, 10-80 pC charge, and ˜0.2 mrad rms divergence. The maximum six-dimensional brightness B6 D ,n is estimated as ˜6.5 ×1 015 A /m2/0.1 % , which is very close to the typical brightness of e beams from state-of-the-art linac drivers. These high-brightness high-energy e beams may lead to the realization of compact monoenergetic gamma-ray and intense coherent x-ray radiation sources.

  9. An energy recovery electron accelerator for DIS at the LHC

    CERN Document Server

    Schulte, Daniel; Jensen, Erk; Valloni, Alessandra; Zimmermann, Frank; Klein, Max

    2014-01-01

    The Large Hadron Electron Collider (LHeC) is a proposed faci lity which will exploit the LHC beams for electron–proton/nucleus scattering, using a new 60 GeV electron accelerator. Following the release of its detailed conceptual design report last ye ar, the configuration of a linac with racetrack shape has been chosen for its default design. Furt her work has been pursued in order to adapt the electron and high luminosity beam optics, to desig n an LHeC Test Facility at CERN and to maximise the ep luminosity to achieve values close to 10 34 cm − 2 s − 1 as is desirable for precision Higgs physics with the LHeC. The talk presents an overview on the design, recent activities and an outlook for further developments

  10. Trend of Energy Saving in Electronic Devices for Research and Development

    Directory of Open Access Journals (Sweden)

    Rahmayanti R.

    2016-01-01

    Full Text Available In electronic industry, energy saving is one of the performance indicators of competitiveness beside price, speed, bandwidth and reliability. This affects research and development (R&D activity in mechatronic systems which uses electronic components and electronic systems. A review of trend of electronic devices technology development has been conducted with focus on energy saving. This review includes electronic devices, semiconductor, and nanotechnology. It can be concluded that the trend in electronic devices is mainly dictated by semiconductor technology development. The trend can be concluded as smaller size, lower voltage leading to energy saving, less heat, higher speed, more reliable, and cheaper. In accordance to such technology development, R&D activities in mechatronics especially in Indonesia is being pushed to make proper alignment.Some of such alignment actions are surface mount technology (SMT for installing surface mount devices components (SMD, design layout and SMD troubleshooting tools as well as human resources training and development.

  11. The negative energy density for a three-single-electron state in the Dirac field

    Institute of Scientific and Technical Information of China (English)

    Shu Wei-Xing; Yu Hong-Wei; Wu Pu-Xun

    2004-01-01

    We examine the energy density produced by a state vector which is the superposition of three single electron states in the Dirac field in the four-dimensional Minkowski spacetime. We derive the conditions on which the energy density can be negative. We then show that the energy density satisfies two quantum inequalities in the ultrarelativistic limit.

  12. An electron/ion spectrometer with the ability of low energy electron measurement for fast ignition experiments

    Energy Technology Data Exchange (ETDEWEB)

    Ozaki, T.; Sakagami, H. [National Institute for Fusion Science, 322-6, Oroshi, Toki, Gifu 509-5292 (Japan); Kojima, S.; Arikawa, Y.; Shiraga, H.; Fujioka, S. [Institute of Laser Engineering, Osaka University, 2-6, Yamada-oka, Suita, Osaka 565-0871 (Japan); Kato, R., E-mail: ozaki@nifs.ac.jp [Institute of Scientific and Industrial Research, Osaka University, 8-1, Mihogaoka, Ibaraki, Osaka 567-0047 (Japan)

    2014-11-15

    An electron energy spectrometer (ESM) is one of the most fundamental diagnostics in the fast ignition experiment. It is necessary to observe the spectra down to a low energy range in order to obtain the accurate deposition efficiency toward the core. Here, we realize the suitable ESM by using a ferrite magnet with a moderate magnetic field of 0.3 T and a rectangular magnetic circuit covered with a steel plate in the inlet side.

  13. [Excitation energy and frequency of transition spectral line of electron in an asymmetry quantum dot].

    Science.gov (United States)

    Xiao, Jing-Lin

    2009-03-01

    In an asymmetry quantum dot, the properties of the electron, which is strongly coupled with phonon, were investigated. The variational relations of the first internal excited state energy, the excitation energy and the frequency of transition spectral line between the first internal excited state and the ground state of the electron which is strongly coupled with phonon in an asymmetry quantum dot with the transverse and longituainal effective confinement length of quantum dot and the electron-phonon coupling strength were studied by using a linear combination operator and the unitary transformation methods. Numerical calculations for the variational relations of the first internal excited state energy, the excitation energy and the frequency of transition spectral line between the first internal excited state and the ground state of the electron which is strongly coupled with phonon in an asymmetry quantum dot with the transverse and longituainal effective confinement length of quantum dot and the electron-phonon coupling strength were performed and the results show that the first internal excited state energy, the excitation energy and the frequency of transition spectral line between the first internal excited state and the ground state of the electron which is strongly coupled with phonon in an asymmetry quantum dot will strongly increase with decreasing the transverse and longitudinal effective confinement length. The first internal excited state energy of the electron which is strongly coupled with phonon in an asymmetry quantum dot will decrease with increasing the electron-phonon coupling strength. The excitation energy and the frequency of transition spectral line between the first internal excited state and the ground state of the electron which is strongly coupled with phonon in an asymmetry quantum dot will increase with increasing the electron-phonon coupling strength.

  14. Realization and Comparison of Several Regression Algorithms for Electron Energy Spectrum Reconstruction

    Institute of Scientific and Technical Information of China (English)

    LI Gui; LIN Hui; WU Ai-Dong; SONG Gang; WU Yi-Can

    2008-01-01

    To determine the electron energy spectra for medical accelerator effectively, we investigate a nonlinear programming model with several nonlinear regression algorithms, including Levenberg-Marquardt, Quasi-Newton, Gradient, Conjugate Gradient, Newton, Principal-Axis and NMinimize algorithms. The local relaxation-bound method is also developed to increase the calculation accuracy. The testing results demonstrate that the above methods could reconstruct the electron energy spectra effectively. Especially, further with the local relaxationbound method the Levenberg Marquardt, Newton and N Minimize algorithms could precisely obtain both the electron energy spectra and the photon contamination. Further study shows that ignoring about 4% photon contamination would increase error greatly, and it also inaccurately makes the electron energy spectra 'drift' to the low energy.

  15. Towards Novel Energy Solutions - an Electronic/Atomistic Simulation Approach

    Science.gov (United States)

    Dong, Rui

    This thesis focuses on computer modeling and multi-scale simulations of new materials that can potentially be used in novel energy applications, i.e., the dye molecules in dye-sensitizedsolar- cells and polymers for the capacitive energy storage. The aim is to understand physical properties of existing materials and then to find ways to improve them. (Abstract shortened by ProQuest.).

  16. High Energy Electron Reconstruction in the BeamCal

    CERN Document Server

    Sailer, Andre

    2016-01-01

    This note discusses methods of particle reconstruction in the forward region detectors of future e+ e− linear colliders such as ILC or CLIC. At the nominal luminosity the innermost electromagnetic calorimeters undergo high particle fluxes from the beam-induced background. In this prospect, different methods of the background simulation and signal electron reconstruction are described.

  17. Ion and Electron Interactions at Thermal and Suprathermal Energies

    Science.gov (United States)

    1989-09-30

    halide ions with both esters occur so rapidly indicates that they are exothermic. If a thermody- namic cycle is constructed the enthalpy change, .H, for...efficiently neutralised to give products. Any OH X2H(v"-O) resulting from the dissociative recombination reactions of H30+, HCO 2+ and N20H+ with electrons

  18. Revealing the Mechanism of Low-Energy Electron Yield Enhancement from Sensitizing Nanoparticles

    CERN Document Server

    Verkhovtsev, Alexey V; Solov'yov, Andrey V

    2014-01-01

    We provide a physical explanation for enhancement of the low-energy electron production by sensitizing nanoparticles due to irradiation by fast ions. It is demonstrated that a significant increase in the number of emitted electrons arises from the collective electron excitations in the nanoparticle. We predict a new mechanism of the yield enhancement due to the plasmon excitations and quantitatively estimate its contribution to the electron production. Revealing the nanoscale mechanism of the electron yield enhancement, we provide an efficient tool for evaluating the yield of emitted electron from various sensitizers. It is shown that the number of low-energy electrons generated by the gold and platinum nanoparticles of a given size exceeds that produced by the equivalent volume of water and by other metallic (e.g., gadolinium) nanoparticles by an order of magnitude. This observation emphasizes the sensitization effect of the noble metal nanoparticles and endorses their application in novel technologies of ca...

  19. Syntrophic growth with direct interspecies electron transfer as the primary mechanism for energy exchange

    DEFF Research Database (Denmark)

    Shrestha, Pravin Malla; Rotaru, Amelia-Elena; Aklujkar, Muktak

    2013-01-01

    Direct interspecies electron transfer (DIET) through biological electrical connections is an alternative to interspecies H2 transfer as a mechanism for electron exchange in syntrophic cultures. However, it has not previously been determined whether electrons received via DIET yield energy...... dehydrogenase, the pilus-associated c-type cytochrome OmcS and pili consistent with electron transfer via DIET. These results suggest that electrons transferred via DIET can serve as the sole energy source to support anaerobic respiration....... to support cell growth. In order to investigate this, co-cultures of Geobacter metallireducens, which can transfer electrons to wild-type G. sulfurreducens via DIET, were established with a citrate synthase-deficient G. sulfurreducens strain that can receive electrons for respiration through DIET only...

  20. On the possibility of kinetic energy density evaluation from the experimental electron-density distribution

    Energy Technology Data Exchange (ETDEWEB)

    Abramov, Yu.A. [National Inst. for Research in Inorganic Materials, Tsukuba, Ibaraki (Japan)

    1997-05-01

    A simple new approach for the evaluation of the electronic kinetic energy density, G(r), from the experimental (multipole-fitted) electron density is proposed. It allows a quantitative and semi-quantitative description of the G(r) behavior at the bond critical points of compounds with closed-shell and shared interactions, respectively. This can provide information on the values of the kinetic electron energy densities at the bond critical points, which appears to be useful for quantum-topological studies of chemical interactions using experimental electron densities. (orig.).

  1. Measurements of the runaway electron energy during disruptions in the tokamak TEXTOR

    Science.gov (United States)

    Forster, M.; Finken, K. H.; Lehnen, M.; Willi, O.; Xu, Y.; the TEXTOR Team

    2012-05-01

    Calorimetric measurements of the total runaway electron energy are carried out using a reciprocating probe during induced TEXTOR disruptions. A comparison with the energy inferred from runaway energy spectra, which are measured with a scintillator probe, is used as an independent check of the results. A typical runaway current of 100 kA at TEXTOR contains 30 to 35 kJ of runaway energy. The dependencies of the runaway energy on the runaway current, the radial probe position, the toroidal magnetic field and the predisruptive plasma current are studied. The conversion efficiency of the magnetic plasma energy into runaway energy is calculated to be up to 26%.

  2. Transparency of graphene for low-energy electrons measured in a vacuum-triode setup

    Directory of Open Access Journals (Sweden)

    G. Hassink

    2015-07-01

    Full Text Available Graphene, being an atomically thin conducting sheet, is a candidate material for gate electrodes in vacuum electronic devices, as it may be traversed by low-energy electrons. The transparency of graphene to electrons with energies between 2 and 40 eV has been measured by using an optimized vacuum-triode setup. The measured graphene transparency equals ∼60% in most of this energy range. Based on these results, nano-patterned sheets of graphene or of related two-dimensional materials are proposed as gate electrodes for ambipolar vacuum devices.

  3. Electrochemical Electron Transfer and Proton-Coupled Electron Transfer: Effects of Double Layer and Ionic Environment on Solvent Reorganization Energies

    Energy Technology Data Exchange (ETDEWEB)

    Ghosh, Soumya; Soudackov, Alexander; Hammes-Schiffer, Sharon

    2016-06-14

    Electron transfer and proton coupled electron transfer (PCET) reactions at electrochemical interfaces play an essential role in a broad range of energy conversion processes. The reorganization energy, which is a measure of the free energy change associated with solute and solvent rearrangements, is a key quantity for calculating rate constants for these reactions. We present a computational method for including the effects of the double layer and ionic environment of the diffuse layer in calculations of electrochemical solvent reorganization energies. This approach incorporates an accurate electronic charge distribution of the solute within a molecular-shaped cavity in conjunction with a dielectric continuum treatment of the solvent, ions, and electrode using the integral equations formalism polarizable continuum model. The molecule-solvent boundary is treated explicitly, but the effects of the electrode-double layer and double layer-diffuse layer boundaries, as well as the effects of the ionic strength of the solvent, are included through an external Green’s function. The calculated total reorganization energies agree well with experimentally measured values for a series of electrochemical systems, and the effects of including both the double layer and ionic environment are found to be very small. This general approach was also extended to electrochemical PCET and produced total reorganization energies in close agreement with experimental values for two experimentally studied PCET systems. This research was supported as part of the Center for Molecular Electrocatalysis, an Energy Frontier Research Center, funded by the U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences.

  4. Functional zinc oxide nanostructures for electronic and energy applications

    Science.gov (United States)

    Prasad, Abhishek

    ZnO has proven to be a multifunctional material with important nanotechnological applications. ZnO nanostructures can be grown in various forms such as nanowires, nanorods, nanobelts, nanocombs etc. In this work, ZnO nanostructures are grown in a double quartz tube configuration thermal Chemical Vapor Deposition (CVD) system. We focus on functionalized ZnO Nanostructures by controlling their structures and tuning their properties for various applications. The following topics have been investigated: (1) We have fabricated various ZnO nanostructures using a thermal CVD technique. The growth parameters were optimized and studied for different nanostructures. (2) We have studied the application of ZnO nanowires (ZnONWs) for field effect transistors (FETs). Unintentional n-type conductivity was observed in our FETs based on as-grown ZnO NWs. We have then shown for the first time that controlled incorporation of hydrogen into ZnO NWs can introduce p-type characters to the nanowires. We further found that the n-type behaviors remained, leading to the ambipolar behaviors of hydrogen incorporated ZnO NWs. Importantly, the detected p- and n- type behaviors are stable for longer than two years when devices were kept in ambient conditions. All these can be explained by an ab initio model of Zn vacancy-Hydrogen complexes, which can serve as the donor, acceptors, or green photoluminescence quencher, depend on the number of hydrogen atoms involved. (3) Next ZnONWs were tested for electron field emission. We focus on reducing the threshold field (Eth) of field emission from non-aligned ZnO NWs. As encouraged by our results on enhancing the conductivity of ZnO NWs by hydrogen annealing described in Chapter 3, we have studied the effect of hydrogen annealing for improving field emission behavior of our ZnO NWs. We found that optimally annealed ZnO NWs offered much lower threshold electric field and improved emission stability. We also studied field emission from ZnO NWs at moderate

  5. Power Electronics – Key Technology for Renewable Energy Systems – Status and Future

    DEFF Research Database (Denmark)

    Blaabjerg, Frede; Yang, Yongheng; Ma, Ke

    2013-01-01

    , distribution and use of the energy should be as technological efficient as possible and incentives to save energy at the end-user should also be streng-thened. In order to realize the transition smoothly and effectively, energy conversion systems, currently based on power electronics technology, will again...... play an essential role. Using highly efficient power electronics in power generation, power transmission/ distribution and end-user application, together with advanced control solutions, can pave the way for renewable energies. In view of this, some of the most emerging renewable energies, e.g. wind...... energy and photovoltaic, which by means of power electronics are changing character as a major part in the electricity generation, are explored in this paper. Issues like technology development, implementation, power converter technologies, control of the systems, and synchronization are addressed...

  6. Analyzer of high-load electron beams with resolution in two energy components, space and time

    Directory of Open Access Journals (Sweden)

    Alexander V. Arkhipov

    2015-03-01

    Full Text Available The new apparatus is developed for experimental determination of electron energy and spatial distributions in dense medium-energy long-pulsed magnetically confined beams – typically, 10 A/cm2, 60 keV, 100 µs, 0.1 T. To provide most detailed and unambiguous information, direct electrostatic cut-off method is used for electron energy analysis. In combination with variation of the magnetic field in the analysis area, this method allows to determine both (axial and transverse components of electron energy. Test experiments confirmed ∼1% energy resolution being predicted from calculations, accounting for electrode shapes, space-charge effects and non-adiabatic energy transfer effects in varied magnetic field. Space and time resolution of the apparatus are determined by the input aperture size (∼1 mm and cut-off electric field pulse-length (∼5–10 µs respectively.

  7. Secondary-electron-emission spectroscopy of tungsten: Angular dependence and phenomenology

    DEFF Research Database (Denmark)

    Willis, Roy F.; Christensen, Niels Egede

    1978-01-01

    spectra from (100), (110), and (111) tungsten surfaces has been studied as a function of polar angle 0°≲Θ≲70° along azimuthal directions φ such that the energy- and angle-resolved SEE current jSEE (E, Ω) effectively scans states throughout the 1 / 48th irreducible body-centered-cubic zone. Calculations...

  8. Using a CCD for the direct detection of electrons in a low energy space plasma spectrometer

    Science.gov (United States)

    Bedington, R.; Kataria, D.; Walton, D.

    2012-01-01

    An E2V CCD64 back-illuminated, ion-implanted CCD (charge-coupled device) has been used as a direct electron imaging detector with CATS (Conceptual And Tiny Spectrometer), a highly miniaturised prototype plasma analyser head. This is in place of an MCP (microchannel plate) with a position sensing anode which would more conventionally be used as a detector in traditional low energy space plasma analyser instruments. The small size of CATS however makes it well matched to the size of the CCD, and the ion implants reduce the depth of the CCD backside electron potential well making it more sensitive to lower energy electrons than standard untreated silicon. Despite ionisation damage from prolonged exposure to excessively energetic electrons, the CCD has been able to detect electrons with energies above 500eV, at temperatures around room temperature. Using both a long integration 'current measuring' mode and a short integration `electron counting' mode it has been used to image the low energy electrons exiting the analyser, enhancing our understanding of the CATS electrostatic optics. The CCD has been selected as the detector for use with CATS for an instrument on a low-altitude student sounding rocket flight. Although it cannot detect the lowest energy electrons that an MCP can detect, and it is more sensitive to stray light, the low voltages required, the lack of vacuum requirements and its novelty and availability made it the most attractive candidate detector.

  9. Hot-electron-based solar energy conversion with metal-semiconductor nanodiodes.

    Science.gov (United States)

    Lee, Young Keun; Lee, Hyosun; Lee, Changhwan; Hwang, Euyheon; Park, Jeong Young

    2016-06-29

    Energy dissipation at metal surfaces or interfaces between a metal and a dielectric generally results from elementary excitations, including phonons and electronic excitation, once external energy is deposited to the surface/interface during exothermic chemical processes or an electromagnetic wave incident. In this paper, we outline recent research activities to develop energy conversion devices based on hot electrons. We found that photon energy can be directly converted to hot electrons and that hot electrons flow through the interface of metal-semiconductor nanodiodes where a Schottky barrier is formed and the energy barrier is much lower than the work function of the metal. The detection of hot electron flow can be successfully measured using the photocurrent; we measured the photoyield of photoemission with incident photons-to-current conversion efficiency (IPCE). We also show that surface plasmons (i.e. the collective oscillation of conduction band electrons induced by interaction with an electromagnetic field) are excited on a rough metal surface and subsequently decay into secondary electrons, which gives rise to enhancement of the IPCE. Furthermore, the unique optical behavior of surface plasmons can be coupled with dye molecules, suggesting the possibility for producing additional channels for hot electron generation.

  10. Measurements of the energy spectrum of electrons emanating from solid materials irradiated by a picosecond laser

    Energy Technology Data Exchange (ETDEWEB)

    Di Stefano, C. A., E-mail: carlosds@umich.edu; Kuranz, C. C.; Thomas, A. G. R.; Drake, R. P.; Keiter, P. A.; Rasmus, A. M.; Wan, W. C.; Joglekar, A. S.; McKelvey, A.; Zhao, Z.; Klein, S. R. [University of Michigan, Ann Arbor, Michigan 48109 (United States); Seely, J. F. [Artep, Inc., Ellicott City, Mary land 21042 (United States); Williams, G. J.; Park, J.; Chen, H.; Kemp, G. E. [Lawrence Livermore National Laboratory, Livermore, California 94551 (United States); MacDonald, M. J. [University of Michigan, Ann Arbor, Michigan 48109 (United States); SLAC National Accelerator Laboratory, Menlo Park, California 94025 (United States); Pereira, N. R. [Ecopulse, Inc., Springfield, Virginia 22150 (United States); Jarrott, L. C.; Peebles, J. [University of California, San Diego, Energy Research Center, La Jolla, California 92093 (United States); and others

    2015-04-15

    In this work, we present the results of experiments observing the properties of the electron stream generated laterally when a laser irradiates a metal. We find that the directionality of the electrons is dependent upon their energies, with the higher-energy tail of the spectrum (∼1 MeV and higher) being more narrowly focused. This behavior is likely due to the coupling of the electrons to the electric field of the laser. The experiments are performed by using the Titan laser to irradiate a metal wire, creating the electron stream of interest. These electrons propagate to nearby spectator wires of differing metals, causing them to fluoresce at their characteristic K-shell energies. This fluorescence is recorded by a crystal spectrometer. By varying the distances between the wires, we are able to probe the divergence of the electron stream, while by varying the medium through which the electrons propagate (and hence the energy-dependence of electron attenuation), we are able to probe the energy spectrum of the stream.

  11. Enzymology of Electron Transport: Energy Generation with Geochemical Consequences

    Energy Technology Data Exchange (ETDEWEB)

    Dichristina, Thomas J.; Fredrickson, Jim K.; Zachara, John M.

    2005-12-20

    Dissimilatory metal-reducing bacteria (DMRB) are important components of the microbial community residing in redox-stratified freshwater and marine environments. DMRB occupy a central position in the biogeochemical cycles of metals, metalloids and radionuclides, and serve as catalysts for a variety of other environmentally important processes including biomineralization, biocorrosion, bioremediation and mediators of ground water quality. DMRB are presented, however, with a unique physiological challenge: they are required to respire anaerobically on terminal electron acceptors which are either highly insoluble (e.g., Fe(III)- and Mn(IV)-oxides) and reduced to soluble end-products or highly soluble (e.g., U(VI) and Tc(VII)) and reduced to insoluble end-products. To overcome physiological problems associated with metal and radionuclide solubility, DMRB are postulated to employ a variety of novel respiratory strategies not found in other gram-negative bacteria which respire on soluble electron acceptors such as O2, NO3- and SO42-. The novel respiratory strategies include (1) direct enzymatic reduction at the outer membrane, (2) electron shuttling pathways and (3) metal solubilization by exogenous or bacterially-produced organic ligands followed by reduction of soluble organic-metal compounds. The first section of this chapter highlights the latest findings on the enzymatic mechanisms of metal and radionuclide reduction by two of the most extensively studied DMRB (Geobacter and Shewanella), with particular emphasis on electron transport chain enzymology. The second section emphasizes the geochemical consequences of DMRB activity, including the direct and indirect effects on metal solubility, the reductive transformation of Fe- and Mn-containing minerals, and the biogeochemical cycling of metals at redox interfaces in chemically stratified environments.

  12. Energy deposition of quasi-two temperature relativistic electrons in fast-shock ignition scenario

    Science.gov (United States)

    Ghasemi, Seyed Abolfazl; Farahbod, Amir Hossein

    2016-10-01

    Previous calculations from Solodov et al. (2008) indicate that classical stopping and scattering dominate electrons energy deposition and transport when the electrons reach the dense plasma in FSI inertial confinement fusion concept [1]. Our calculations show that, by using quasi- two temperature electrons energy distribution function [2] in comparison with exponential [3] or monoenergetic distribution function and also increasing fast electrons energy to about 7 MeV, the ratio of beam blooming to straggling definitely decreases. Our analytical analysis shows that for fuel mass more than 1 mg and for fast ignitor wavelength λif > 0.53 μ m, straggling and beam blooming increases. Meanwhile, by reducing fast ignitor wavelength from 0.53 to 0.35 micron, and for fuel mass about 2 mg, electron penetration into the dense fuel slightly increases. Therefore, reduction of scattering (blooming and straggling) of electrons and enhancement of electron penetration into the dense fuel, can be obtained in relativistic regime with high energy fast electrons of the order of 5 Mev and more. Such derivations can be used in theoretical studies of the ignition conditions and PIC simulations of the electron transport in fast ignition scenario.

  13. The effects of local correlations on the electronic structure of FeSe

    Science.gov (United States)

    Watson, Matthew; Kim, Timur; Haghighirad, Amir; Coldea, Amalia

    FeSe is structurally the simplest of Fe-based superconductors, but its complex and unique properties pose important theoretical questions. One important aspect of the physics of FeSe is the understanding of the strength and effects of electronic correlations. In order to explore this, we have performed angle-resolved photo-emission spectroscopy (ARPES) measurements on high quality bulk single crystals of FeSe over a wide range of binding energies, in different scattering geometries and with varying incident photon energies, analysing the quasiparticle renormalisations, scattering rates and degree of coherence. We find that FeSe exhibits moderately strong, orbital-dependent correlation effects which are understood to arise primarily due to local electron-electron interactions on the Fe sites. We conclude that electronic correlations constitute a key ingredient in understanding the electronic structure of FeSe. Part of this work was supported by EPSRC, UK (EP/I004475/1, EP/I017836/1). We thank Diamond Light Source for access to Beamline I05.

  14. Energy saving estimation on radiation process. Electron beam curing of paint

    Energy Technology Data Exchange (ETDEWEB)

    Kaneko, Hideaki (Nihon Parkerizing Co., Ltd., Tokyo); Maekawa, H.; Ito, Y.; Nishikawa, I.; Fujii, H.; Murata, K.

    1982-01-01

    When the quantity of paint used for industrial coating is assumed to be 420,000 tons, it is estimated that the area being coated is 2.8 billion m/sup 2/, the petroleum required for pretreatment steam, drying and baking is 1.68 million tons, and the required amount of energy saving is 120,000 tons per year in terms of petroleum. The authors examined how the adoption of electron beam curing for surface coating contributes to the energy saving. So far, it has been said that electron beam curing is more efficient than thermal or light curing in energy consumption, but the premise condition was not clear. The theoretical energy requirement for thermal curing, light curing and electron beam curing was calculated and compared. The comparison of the measured values was also performed. The amount of energy required for thermal curing, UV light curing and electron beam curing was roughly 100:10:1, and the cost of energy for them was 50:5:1. In spite of the large merit of electron beam curing, it has not spread as expected, because of the repayment cost of the facility and the cost of inert gas required for the process. Energy saving is brought about by electron beam curing, but the overall cost must be examined case by case.

  15. Theorectical Studies of Excitation in Low-Energy Electron-Polyatomic Molecule Collisions

    Energy Technology Data Exchange (ETDEWEB)

    Rescigno, T N; McCurdy, C W; Isaacs, W A; Orel, A E; Meyer, H D

    2001-08-13

    This paper focuses on the channeling of energy from electronic to nuclear degrees of freedom in electron-polyatomic molecule collisions. We examine the feasibility of attacking the full scattering problem, both the fixed-nuclei electronic problem and the post-collision nuclear dynamics, entirely from first principles. The electron-CO{sub 2} system is presented as an example. We study resonant vibrational excitation, showing how a6 initio, fixed-nuclei electronic cross sections can provide the necessary input for a multi-dimensional treatment of the nuclear vibrational dynamics.

  16. Non-equilibrium vibrational and electron energy distribution functions in mtorr, high-electron-density nitrogen discharges and afterglows

    Science.gov (United States)

    Capitelli, M.; Colonna, G.; D’Ammando, G.; Laricchiuta, A.; Pietanza, L. D.

    2017-03-01

    Non-equilibrium vibrational distributions (vdf) and non-equilibrium electron energy distribution functions (eedf) in a nitrogen plasma at low pressure (mtorr) have been calculated by using a time-dependent plasma physics model coupled to the Boltzmann equation and heavy particle kinetics. Different case studies have been selected showing the non-equilibrium character of both vdf and eedf under discharge and post-discharge conditions in the presence of large concentrations of electrons. Particular attention is devoted to the electron-molecule resonant vibrational excitation cross sections acting in the whole vibrational ladder. The results in the post-discharge conditions show the interplay of superelastic vibrational and electronic collisions in forming structures in the eedf. The link between the present results in the mtorr afterglow regime with the existing eedf in the torr and atmospheric regimes is discussed.

  17. Low-Energy Plasma Focus Device as an Electron Beam Source

    Directory of Open Access Journals (Sweden)

    Muhammad Zubair Khan

    2014-01-01

    Full Text Available A low-energy plasma focus device was used as an electron beam source. A technique was developed to simultaneously measure the electron beam intensity and energy. The system was operated in Argon filling at an optimum pressure of 1.7 mbar. A Faraday cup was used together with an array of filtered PIN diodes. The beam-target X-rays were registered through X-ray spectrometry. Copper and lead line radiations were registered upon usage as targets. The maximum electron beam charge and density were estimated to be 0.31 μC and 13.5×1016/m3, respectively. The average energy of the electron beam was 500 keV. The high flux of the electron beam can be potentially applicable in material sciences.

  18. Total and elastic electron scattering cross sections from Xe at intermediate and high energies

    Energy Technology Data Exchange (ETDEWEB)

    Garcia, G [Instituto de Matematicas y Fisica Fundamental, CSIC, Serrano 123, 28006 Madrid (Spain); Pablos, J L de [Departamento de Fusion y Particulas Elementales, CIEMAT, Avenida Complutense 22, 28040 Madrid (Spain); Blanco, F [Departamento de Fisica Atomica Molecular y Nuclear, Universidad Complutense de Madrid, 28040 Madrid (Spain); Williart, A [Departamento de Fisica de los Materiales, UNED, Senda del Rey 9, 28040 Madrid (Spain)

    2002-11-28

    Experimental total electron scattering cross sections from Xe in the energy range 300-5000 eV have been obtained with experimental errors of about 3%. The method was based on the measurement of the attenuation of a linear electron beam through a Xe gas cell in combination with an electron spectroscopy technique to analyse the energy of the transmitted electrons. Differential and integral elastic cross sections have been calculated using a scattering potential method which includes relativistic effects. The consistency of our theoretical and experimental results is also discussed in the paper. Finally, analytical formulae depending on two parameters, namely the number of target electrons and the atomic polarizability, are given to reproduce the experimental data for Ne, Ar, Kr and Xe in the energy range 500-10 000 eV.

  19. Double-electron capture by highly-ionized atoms isolated at very low energy

    Science.gov (United States)

    Fogwell Hoogerheide, Shannon; Dreiling, Joan M.; Sahiner, Arda; Tan, Joseph N.

    2016-05-01

    Charge exchange with background gases, also known as electron capture processes, is important in the study of comets, controlled fusion energy, anti-matter atoms, and proposed one-electron ions in Rydberg states. However, there are few experiments in the very low energy regime that could be useful for further theoretical development. At NIST, highly-charged ions extracted from an electron-beam ion trap can be isolated with energy state. Analysis using a system of rate equations yields information about the ion cloud expansion and single-electron capture rates. A substantial amount of double-electron capture is also observed. We present the relative rates and discuss the error budget. SFH and JMD were funded by National Research Council Research Associateship Awards during some of this work.

  20. XPS STUDY ON DNA DAMAGE BY LOW-ENERGY ELECTRON IRRADIATION

    Energy Technology Data Exchange (ETDEWEB)

    Noh, Hyung Ah; Cho, Hyuck [Chungnam National University, Physics Department, Daejeon (Korea, Republic of)

    2011-12-15

    After the first report that electrons with sub-ionization energy of DNA could cause single strand breaks or double strand breaks to DNA, there have been various studies to investigate the mechanisms of DNA damage by low-energy electrons. In this paper, we examined the possibility of using X-ray photoelectron spectroscopy (XPS) to analyze the dissociation patterns of the molecular bonds by electron irradiation on DNA thin films and tried to establish the method as a general tool for studying the radiation damage of biomolecules by low energy electrons. For the experiment, pBR322 plasmid DNA solution was formed into the films on tantalum plates by lyophilization and was irradiated by 5-eV electrons. Un-irradiated and irradiated DNA films were compared and analyzed using the XPS technique.