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Sample records for 6li 7li 9be

  1. $\\Sigma^- p$ emission rates in $K^-$ absorptions at rest on $^6$Li, $^7$Li, $^{9}$Be, $^{13}$C and $^{16}$O

    CERN Document Server

    Agnello, M; Bertani, M; Bonomi, G; Botta, E; Bregant, M; Bressani, T; Bufalino, S; Busso, L; Calvo, D; Camerini, P; Dalena, B; De Mori, F; D'Erasmo, G; Feliciello, A; Filippi, A; Fiore, E M; Fontana, A; Fujioka, H; Genova, P; Gianotti, P; Grion, N; Lucherini, V; Marcello, S; Morra, O; Nagae, T; Outa, H; Pantaleo, A; Paticchio, V; Piano, S; Rui, R; Simonetti, G; Wheadon, R; Zenoni, A

    2015-01-01

    An experimental study of the $K^-_{stop}A\\rightarrow \\Sigma^- p A'$ reaction on $A=^6$Li, $^7$Li, $^9$Be, $^{13}$C and $^{16}$O $p$-shell nuclei is presented. The data were collected by the FINUDA spectrometer operating at the DA$\\Phi$NE $\\phi$-factory (LNF-INFN, Italy). Emission rates for the reaction in the mentioned nuclei are measured and compared with the few existing data. The spectra of several observables are discussed; indications of Quasi-Free absorptions by a $(np)$ pair embedded in the $A$ nucleus can be obtained from the study of the missing mass distributions.

  2. 6Li/7Li estimates for metal-poor stars

    CERN Document Server

    Perez, A E Garcia; Inoue, S; Ryan, S G; Suzuki, T K; Chiba, M

    2009-01-01

    The presence of the lithium-6 isotope in some metal-poor stars is a matter of surprise because of the high values observed. Non-standard models of Big Bang nucleosynthesis and pre-Galactic cosmic ray fusion and spallation have been proposed to explain these values. However, the observations of this light isotope are challenging which may make some detections disputable. The goal was to determine 6Li/7Li for a sample of metal-poor stars; three of them have been previously studied and the remaining two are new for this type of study. The purpose was to increase, if possible, the number of lithium-6 detections and to confirm previously published results. Spectra of the resonance doublet line of neutral lithium Li I 670.78nm were taken with the High Dispersion Spectrograph at the Subaru 8.2m-telescope for a sample of five metal-poor stars (-3.12 < [Fe/H] < -2.19). The contribution of lithium-6 to the total observed line profile was estimated from the 1D-LTE analysis of the line asymmetry. Observed asymmetri...

  3. Hyperfine structure in photoassociative spectra of 6Li2 and 7Li2

    NARCIS (Netherlands)

    Abraham, E.R.I.; McAlexander, W.I.; Stoof, H.T.C.; Hulet, R.G.

    1996-01-01

    We present spectra of hyperfine resolved vibrational levels of the A1Σu+and 1 3Σg+ states of 6Li2 and 7Li2 obtained via photoassociation of colliding ultracold atoms in a magneto-optical trap. A simple first-order perturbation theory analysis accurately accounts for the frequency splittings and rela

  4. Theory of laser enhancement and suppression of cold reactions: the fermion-boson 6Li+7Li2(variant Planck's over 2pi omega0) 6Li7Li+7Li radiative collision.

    Science.gov (United States)

    Li, Xuan; Parker, Gregory A; Brumer, Paul; Thanopulos, Ioannis; Shapiro, Moshe

    2008-03-28

    We present a nonperturbative time-dependent quantum mechanical theory of the laser catalysis and control of a bifurcating A+BC(variant Planck's over 2pi omega(0))ABC*(v)(variant Planck's over 2pi omega(0) )AB+C reaction, with ABC*(v) denoting an intermediate, electronically excited, complex of ABC in the vth vibrational state. We apply this theory to the low collision energy fermion-boson light-induced exchange reaction, (6)Li((2)S)+(7)Li(2)((3)Sigma(u)(+))(variant Planck's over 2pi omega(0))((6)Li(7)Li(7)Li)*(variant Planck's over 2pi omega(0))(6)Li(7)Li((3)Sigma(+))+(7)Li((2)S). We show that at very low collision energies and energetically narrow (approximately 0.01 cm(-1)) initial reactant wave packets, it is possible to tune the yield of the exchange reaction from 0 to near-unity (yield >or=99%) values. Controllability is somewhat reduced at collisions involving energetically wider (approximately 1 cm(-1)) initial reactant wave packets. At these energetic bandwidths, the radiative reactive control, although still impressive, is limited to the 0%-76% reactive-probabilities range.

  5. Systematics of the breakup probability function for {sup 6}Li and {sup 7}Li projectiles

    Energy Technology Data Exchange (ETDEWEB)

    Capurro, O.A., E-mail: capurro@tandar.cnea.gov.ar [Laboratorio TANDAR, Comisión Nacional de Energía Atómica, Av. General Paz 1499, B1650KNA San Martín, Buenos Aires (Argentina); Pacheco, A.J.; Arazi, A. [Laboratorio TANDAR, Comisión Nacional de Energía Atómica, Av. General Paz 1499, B1650KNA San Martín, Buenos Aires (Argentina); CONICET, Av. Rivadavia 1917, C1033AAJ Buenos Aires (Argentina); Carnelli, P.F.F. [CONICET, Av. Rivadavia 1917, C1033AAJ Buenos Aires (Argentina); Instituto de Investigación e Ingeniería Ambiental, Universidad Nacional de San Martín, 25 de Mayo y Francia, B1650BWA San Martín, Buenos Aires (Argentina); Fernández Niello, J.O. [Laboratorio TANDAR, Comisión Nacional de Energía Atómica, Av. General Paz 1499, B1650KNA San Martín, Buenos Aires (Argentina); CONICET, Av. Rivadavia 1917, C1033AAJ Buenos Aires (Argentina); Instituto de Investigación e Ingeniería Ambiental, Universidad Nacional de San Martín, 25 de Mayo y Francia, B1650BWA San Martín, Buenos Aires (Argentina); and others

    2016-01-15

    Experimental non-capture breakup cross sections can be used to determine the probability of projectile and ejectile fragmentation in nuclear reactions involving weakly bound nuclei. Recently, the probability of both type of dissociations has been analyzed in nuclear reactions involving {sup 9}Be projectiles onto various heavy targets at sub-barrier energies. In the present work we extend this kind of systematic analysis to the case of {sup 6}Li and {sup 7}Li projectiles with the purpose of investigating general features of projectile-like breakup probabilities for reactions induced by stable weakly bound nuclei. For that purpose we have obtained the probabilities of projectile and ejectile breakup for a large number of systems, starting from a compilation of the corresponding reported non-capture breakup cross sections. We parametrize the results in accordance with the previous studies for the case of beryllium projectiles, and we discuss their systematic behavior as a function of the projectile, the target mass and the reaction Q-value.

  6. Line shift, line asymmetry, and the 6Li/7Li isotopic ratio determination

    CERN Document Server

    Cayrel, Roger; Chand, Hum; Bonifacio, Piercarlo; Spite, Monique; Spite, François; Petitjean, Patrick; Ludwig, Hans-Günter; Caffau, Elisabetta

    2007-01-01

    Context: Line asymmetries are generated by convective Doppler shifts in stellar atmospheres, especially in metal-poor stars, where convective motions penetrate to higher atmospheric levels. Such asymmetries are usually neglected in abundance analyses. The determination of the 6Li/7Li isotopic ratio is prone to suffering from such asymmetries, as the contribution of 6Li is a slight blending reinforcement of the red wing of each component of the corresponding 7Li line, with respect to its blue wing. Aims: The present paper studies the halo star HD 74000 and estimates the impact of convection-related asymmetries on the Li isotopic ratio determination. Method: Two methods are used to meet this aim. The first, which is purely empirical, consists in deriving a template profile from another element that can be assumed to originate in the same stellar atmospheric layers as Li I, producing absorption lines of approximately the same equivalent width as individual components of the 7Li I resonance line. The second metho...

  7. Elastic and inelastic scattering of {sup 6}Li + {sup 18}O versus {sup 7}Li + {sup 18}O and {sup 6}Li + {sup 16}O

    Energy Technology Data Exchange (ETDEWEB)

    Rudchik, Adam T., E-mail: rudchik@kinr.kiev.ua [Institute for Nuclear Research, Ukrainian Academy of Sciences, Prospect Nauki 47, 03680 Kyiv (Ukraine); Kliczewski, Stanislaw [H. Niewodniczański Institute of Nuclear Physics, Polish Academy of Sciences, ul. Radzikowskiego 152, PL-31-342 Cracow (Poland); Chercas, Kostyantyn A. [Institute for Nuclear Research, Ukrainian Academy of Sciences, Prospect Nauki 47, 03680 Kyiv (Ukraine); Kemper, Kirby W. [Physics Department, Florida State University, Tallahassee, FL 32306-4350 (United States); Koshchy, Evgeniy I. [Kharkiv National University, pl. Svobody 4, 61077 Kharkiv (Ukraine); Rusek, Krzysztof [National Centre for Nuclear Research, ul. Hoża 69, PL-00-681 Warsaw (Poland); Heavy Ion Laboratory of Warsaw University, ul. L. Pasteura 5A, PL-02-093 Warsaw (Poland); Rudchik, Andryi A.; Mezhevych, Sergyi Yu.; Pirnak, Valeryi M. [Institute for Nuclear Research, Ukrainian Academy of Sciences, Prospect Nauki 47, 03680 Kyiv (Ukraine); Plujko, Volodymyr A. [Taras Shevchenko Kyiv National University, vul. Volodymyrs' ka 64, 01033 Kyiv (Ukraine); Ponkratenko, Oleg A. [Institute for Nuclear Research, Ukrainian Academy of Sciences, Prospect Nauki 47, 03680 Kyiv (Ukraine); Choiński, Jaroslaw [Heavy Ion Laboratory of Warsaw University, ul. L. Pasteura 5A, PL-02-093 Warsaw (Poland); Czech, Bronislaw; Siudak, Regina; Szczurek, Antoni [H. Niewodniczański Institute of Nuclear Physics, Polish Academy of Sciences, ul. Radzikowskiego 152, PL-31-342 Cracow (Poland); Stolarz, Anna [Heavy Ion Laboratory of Warsaw University, ul. L. Pasteura 5A, PL-02-093 Warsaw (Poland); Zelinskyi, Ruslan M. [Institute for Nuclear Research, Ukrainian Academy of Sciences, Prospect Nauki 47, 03680 Kyiv (Ukraine)

    2014-02-15

    Inverse kinematics scattering of {sup 18}O on {sup 6}Li at E{sub lab}({sup 18}O) = 114 MeV was measured to obtain elastic and inelastic scattering cross sections. In this way cross sections for excited states in {sup 6}Li and {sup 18}O were determined. The data were analyzed within the optical model and coupled reaction channel method. The {sup 6}Li + {sup 18}O optical potential as well as the {sup 6}Li and {sup 18}O deformation parameters were deduced. Contributions of different nuclear processes to the {sup 6}Li + {sup 18}O elastic and inelastic scattering were explored. The isotopic differences between the {sup 6,7}Li + {sup 18}O and {sup 6}Li + {sup 16,18}O potential parameters were determined.

  8. Fast neutron measurements with {sup 7}Li and {sup 6}Li enriched CLYC scintillators

    Energy Technology Data Exchange (ETDEWEB)

    Giaz, A., E-mail: agnese.giaz@mi.infn.it [INFN Milano, Via Celoria 16, 20133 Milano (Italy); Blasi, N.; Boiano, C.; Brambilla, S. [INFN Milano, Via Celoria 16, 20133 Milano (Italy); Camera, F. [INFN Milano, Via Celoria 16, 20133 Milano (Italy); Università degli Studi di Milano, Physics Department, Via Celoria 16, 20133 Milano (Italy); Cattadori, C. [INFN sezione di Milano Bicocca, Piazza della Scienza 3, 20125 Milano (Italy); Ceruti, S. [INFN Milano, Via Celoria 16, 20133 Milano (Italy); Università degli Studi di Milano, Physics Department, Via Celoria 16, 20133 Milano (Italy); Gramegna, F.; Marchi, T. [INFN Laboratori Nazionali di Legnaro, Viale dell’Università, 2, 35020 Legnaro, PD (Italy); Mattei, I. [INFN Milano, Via Celoria 16, 20133 Milano (Italy); Mentana, A. [INFN Milano, Via Celoria 16, 20133 Milano (Italy); Università degli Studi di Milano, Physics Department, Via Celoria 16, 20133 Milano (Italy); Million, B.; Pellegri, L. [INFN Milano, Via Celoria 16, 20133 Milano (Italy); Rebai, M. [Università degli Studi di Milano Bicocca, Physics Department, Piazza della Scienza 3, 20126 Milano (Italy); Riboldi, S. [INFN Milano, Via Celoria 16, 20133 Milano (Italy); Università degli Studi di Milano, Physics Department, Via Celoria 16, 20133 Milano (Italy); Salamida, F. [INFN sezione di Milano Bicocca, Piazza della Scienza 3, 20125 Milano (Italy); Tardocchi, M. [Istituto di Fisica del Plasma, Associazione EURATOM-ENEA-CNR, Via R. Cozzi 53, 2015 Milano (Italy)

    2016-07-21

    The recently developed Cs{sub 2}LiYCl{sub 6}:Ce (CLYC) crystals are interesting scintillation detectors not only for their gamma energy resolution (<5% at 662 keV) but also for their capability to identify and measure the energy of both gamma rays and fast/thermal neutrons. The thermal neutrons were detected by the {sup 6}Li(n,α)t reaction while for the fast neutrons the {sup 35}Cl(n,p){sup 35}S and {sup 35}Cl(n,α){sup 32}P neutron-capture reactions were exploited. The energy of the outgoing proton or α particle scales linearly with the incident neutron energy. The kinetic energy of the fast neutrons can be measured using both the Time Of Flight (TOF) technique and using the CLYC energy signal. In this work, the response to monochromatic fast neutrons (1.9–3.8 MeV) of two CLYC 1″×1″ crystals was measured using both the TOF and the energy signal. The observables were combined to identify fast neutrons, to subtract the thermal neutron background and to identify different fast neutron-capture reactions on {sup 35}Cl, in other words to understand if the detected particle is an α or a proton. We performed a dedicated measurement at the CN accelerator facility of the INFN Legnaro National Laboratories (Italy), where the fast neutrons were produced by impinging a proton beam (4.5, 5.0 and 5.5 MeV) on a {sup 7}LiF target. We tested a CLYC detector {sup 6}Li-enriched at about 95%, which is ideal for thermal neutron measurements, in parallel with another CLYC detector {sup 7}Li-enriched at more than 99%, which is suitable for fast neutron measurements.

  9. Fast neutron measurements with 7Li and 6Li enriched CLYC scintillators

    Science.gov (United States)

    Giaz, A.; Blasi, N.; Boiano, C.; Brambilla, S.; Camera, F.; Cattadori, C.; Ceruti, S.; Gramegna, F.; Marchi, T.; Mattei, I.; Mentana, A.; Million, B.; Pellegri, L.; Rebai, M.; Riboldi, S.; Salamida, F.; Tardocchi, M.

    2016-07-01

    The recently developed Cs2LiYCl6:Ce (CLYC) crystals are interesting scintillation detectors not only for their gamma energy resolution (<5% at 662 keV) but also for their capability to identify and measure the energy of both gamma rays and fast/thermal neutrons. The thermal neutrons were detected by the 6Li(n,α)t reaction while for the fast neutrons the 35Cl(n,p)35S and 35Cl(n,α)32P neutron-capture reactions were exploited. The energy of the outgoing proton or α particle scales linearly with the incident neutron energy. The kinetic energy of the fast neutrons can be measured using both the Time Of Flight (TOF) technique and using the CLYC energy signal. In this work, the response to monochromatic fast neutrons (1.9-3.8 MeV) of two CLYC 1″×1″ crystals was measured using both the TOF and the energy signal. The observables were combined to identify fast neutrons, to subtract the thermal neutron background and to identify different fast neutron-capture reactions on 35Cl, in other words to understand if the detected particle is an α or a proton. We performed a dedicated measurement at the CN accelerator facility of the INFN Legnaro National Laboratories (Italy), where the fast neutrons were produced by impinging a proton beam (4.5, 5.0 and 5.5 MeV) on a 7LiF target. We tested a CLYC detector 6Li-enriched at about 95%, which is ideal for thermal neutron measurements, in parallel with another CLYC detector 7Li-enriched at more than 99%, which is suitable for fast neutron measurements.

  10. Gamow shell model description of radiative capture reactions $^6$Li$(p,\\gamma)$$^7$Be and $^6$Li$(n,\\gamma)$$^7$Li

    CERN Document Server

    Dong, G X; Fossez, K; Płoszajczak, M; Jaganathen, Y; Betan, R M Id

    2016-01-01

    According to standard stellar evolution, lithium abundance is believed to be a useful indicator of the stellar age. However, many evolved stars like red giants show huge fluctuations around expected theoretical abundances that are not yet fully understood. The better knowledge of nuclear reactions that contribute to the creation and destruction of lithium can help to solve this puzzle. In this work we apply the Gamow shell model (GSM) formulated in the coupled-channel representation (GSM-CC) to investigate the mirror radiative capture reactions $^6$Li$(p,\\gamma)$$^7$Be and $^6$Li$(n,\\gamma)$$^7$Li. The cross-sections are calculated using a translationally invariant Hamiltonian with the finite-range interaction which is adjusted to reproduce spectra, binding energies and one-nucleon separation energies in $^{6-7}$Li, $^7$Be. All relevant $E1$, $M1$, and $E2$ transitions from the initial continuum states to the final bound states $J={3/2}_1^-$ and $J={1/2}^-$ of $^7$Li and $^7$Be are included. We demonstrate th...

  11. (p,px) reaction on /sup 6/Li and /sup 7/Li nuclei at incident proton energy of 70 MeV

    Energy Technology Data Exchange (ETDEWEB)

    Gorpinich, O.K.; Kadkin, E.P.; Kondrat' ev, S.N.; Lobach, Yu.M.; Pasechnik, M.V.; Saltykov, L.S.; Tokarevskij, V.V. (AN Ukrainskoj SSR, Kiev. Inst. Yadernykh Issledovanij)

    1983-01-01

    Measurements of two-dimensional coincidence spectra of charged particles from the /sup 6/Li(p, 2p)/sup 5/He, /sup 6/Li(p, p..cap alpha..)/sup 2/H, /sup 7/Li(p, pt)/sup 4/He, /sup 7/Li(p, p..cap alpha..)/sup 3/H reactions has been carried out using the equipment for simultaneous investigation of correlation of charged particles of different types. The /sup 6/Li(p, pd) reaction probability reaches the maximum value when the residual nucleus momentum is close to zero. This fact may confirm an existance of strong /sup 6/Li ..cap alpha..d-clusterization. The /sup 7/Li(p, pt) reaction occurs with the minimum probability in a quasi-free region that confirms /sup 7/Li ..cap alpha..t-structure. A direct comparison of particle two-dimensional spectra projections of (p, px) type reactions reveals that a probability of quasi-free scattering of proton on deuteron (triton) /sup 6/Li(/sup 7/Li) cluster is higher than quasi-free scattering on intranuclear protons. This fact is also confirmed by an assumption on ..cap alpha..d(..cap alpha..t)-cluster /sup 6/Li(/sup 7/Li) nucleus structure.

  12. Role of neutron transfer processes on the 6Li+120Sn and 7Li+119Sn fusion reactions

    Directory of Open Access Journals (Sweden)

    Fisichella M.

    2015-01-01

    Full Text Available The results concerning the study of 6Li+120Sn and 7Li+119Sn systems are presented. These two sistems are characterised by very similar structures of the interacting nuclei and by different Q-value for one-and two- neutron transfer. Our aim is to disentangle the possible effects due to the different n-transfer Q-values, at sub-barriers energies, by comparing the two fusion excitation function. In these experiments the fusion cross section has been measured by using a stack activation technique. No particular differences in the two fusion excitation functions have been observed.

  13. Threshold behavior of interaction potential for the system 7Li + 64Ni: Comparison with 6Li + 64Ni

    Science.gov (United States)

    Shaikh, Md. Moin; Das, Mili; Roy, Subinit; Sinha, M.; Pradhan, M. K.; Basu, P.; Datta, U.; Ramachandran, K.; Shrivastava, A.

    2016-09-01

    The elastic scattering angular distributions for the system 7Li + 64Ni were measured in the bombarding energy range of 12 MeV ≤Elab ≤ 26.4 MeV. A phenomenological optical model analysis was performed for the measured data. The strengths of the fitted potential components at the surface were estimated to extract their variation with energy. Further analyses of the measured angular distributions were performed with a hybrid potential composed of a renormalized folded real and a phenomenological imaginary potential. Both the model potentials predict similar energy dependent behavior for the effective interaction potential around the barrier. Unlike the heavy targets, 7Li + 64Ni does not show a normal threshold behavior. It also does not clearly exhibit a behavior similar to 6Li + 64Ni. The real potential for 7Li + 64Ni does not exhibit any significant energy dependence and the imaginary potential strength remains almost independent of energy above the Coulomb barrier (∼ 14 MeV). However, at energies below the barrier, a sudden drop in the imaginary potential strength is observed.

  14. 同位素7Li和6Li的性质殊异%The diverse of isotopes 7 Li and 6 Li

    Institute of Scientific and Technical Information of China (English)

    朱正和; 宋江锋; 罗德礼

    2014-01-01

    本文研究了同位素7 Li和6 Li在几个方面的性质差异.用相对论量子力学计算指出,6 Li的电子能级比7 Li的能级低,同时,对电偶极E (1)和磁偶极M (1)的能级跃迁波长,6 Li的跃迁波长都要比7 Li的长.由于7 Li和6 Li的核自旋的大小不同,可以看出在磁场2万高斯和温度100-20 K之间,7 Li的磁极化比6 Li的约大13倍.7 Li和6 Li的磁极化这种差异,也是一种可能的同位素7 Li/6 Li的分离方法.%The diverse of isotopes 7 Li and 6 Li was examined on the several respects.The calculations of relativistic quantum mechanics shows that the energy levels of 6 Li are lower than that of 7 Li, and therefore the transitional wave length of E(1) and M(1) for 6 Li are longer than that of 7 Li.The variation of couple constant due to the different nu-clear spin of 7 Li and 6 Li could be as a basis for the isotope separation between 7 Li and 6 Li.Ratio of the molar intensi-ty of magnetization of 7 Li to 6 Li is about 13 under 100-20 K and 20, 000 gauss, which is favorable to separate out 6 Li.

  15. {sup 6}Li({sup 18}O, {sup 17}O){sup 7}Li reaction and comparison of {sup 6, 7}Li + {sup 16, 17, 18}O potentials

    Energy Technology Data Exchange (ETDEWEB)

    Rudchik, A.T., E-mail: rudchik@kinr.kiev.ua [Institute for Nuclear Research, Ukrainian Academy of Sciences, Prospect Nauki 47, 03680 Kyiv (Ukraine); Chercas, K.A. [Institute for Nuclear Research, Ukrainian Academy of Sciences, Prospect Nauki 47, 03680 Kyiv (Ukraine); Kemper, K.W. [Physics Department, Florida State University, Tallahassee, FL 32306-4350 (United States); Rudchik, A.A. [Institute for Nuclear Research, Ukrainian Academy of Sciences, Prospect Nauki 47, 03680 Kyiv (Ukraine); Kliczewski, S. [H. Niewodniczański Institute of Nuclear Physics, Polish Academy of Sciences, ul. Radzikowskiego 152, PL-31-342 Cracow (Poland); Koshchy, E.I. [Kharkiv National University, pl. Svobody 4, 61077 Kharkiv (Ukraine); Rusek, K. [National Center for Nuclear Reseaches, ul. Hoża 69, PL-00-681 Warsaw (Poland); Heavy Ion Laboratory of Warsaw University, ul. L. Pasteura 5A, PL-02-093 Warsaw (Poland); Mezhevych, S.Yu.; Ponkratenko, O.A.; Pirnak, Val.M. [Institute for Nuclear Research, Ukrainian Academy of Sciences, Prospect Nauki 47, 03680 Kyiv (Ukraine); Plujko, V.A. [Taras Shevchenko National University, ul. Volodymyrska 64, 01033 Kyiv (Ukraine); Choiński, J. [Heavy Ion Laboratory of Warsaw University, ul. L. Pasteura 5A, PL-02-093 Warsaw (Poland); Czech, B.; Siudak, R.; Szczurek, A. [H. Niewodniczański Institute of Nuclear Physics, Polish Academy of Sciences, ul. Radzikowskiego 152, PL-31-342 Cracow (Poland)

    2014-07-15

    Angular distributions of the {sup 6}Li({sup 18}O, {sup 17}O){sup 7}Li reaction were measured at E{sub lab}({sup 18}O)=114 MeV for ground and excited states of the exit channel nuclei for the first time. The data were analyzed within the coupled-reaction-channels method (CRC). The {sup 6}Li + {sup 18}O elastic and inelastic scattering channels as well as simplest one- and two-step reactions were included in the coupled-reaction-channels scheme. The {sup 7}Li + {sup 17}O potential was deduced by fitting CRC calculations to the reaction data. The spectroscopic amplitudes for single nucleon and nuclear cluster configurations were calculated within the translationally invariant shell model. Isotopic differences of the {sup 7}Li + {sup 16, 17, 18}O and {sup 7, 8}Li + {sup 17}O potentials and the reaction mechanisms were studied.

  16. Measurements of double-differential neutron emission cross sections of {sup 6}Li and {sup 7}Li for 18 MeV neutrons

    Energy Technology Data Exchange (ETDEWEB)

    Ibaraki, Masanobu; Baba, Mamoru; Matsuyama, Shigeo; Sanami, Toshiya; Win, T.; Miura, Takako; Hirakawa, Naohiro [Tohoku Univ., Sendai (Japan). Faculty of Engineering

    1997-03-01

    Double-differential neutron emission cross sections of {sup 6}Li and {sup 7}Li were measured for 18 MeV neutrons at Tohoku University 4.5 MV Dynamitron facility. Neutron emission spectra were obtained down to 1 MeV at 13 angles with energy resolution good enough to separate discrete levels. A care was taken to eliminate the sample-dependent background due to parasitic neutrons. Experimental results were in fair agreement with the JENDL-3.2 data and a simple model considering a three-body breakup process and discrete level excitations. (author)

  17. All-optical production of dual Bose-Einstein condensates of paired fermions and bosons with 6Li and 7Li

    Science.gov (United States)

    Ikemachi, Takuya; Ito, Aki; Aratake, Yukihito; Chen, Yiping; Koashi, Masato; Kuwata-Gonokami, Makoto; Horikoshi, Munekazu

    2017-01-01

    We report the first all-optical production of dual Bose-Einstein condensates (BECs) of paired 6Li (fermion) and one spin state of 7Li (boson) at the magnetic field where the s-wave interactions between fermions are resonant. Fermions are cooled efficiently by evaporative cooling and they serve as coolant for bosons. As a result, the dual condensates can be achieved by using a simple experimental apparatus and procedures, as in the case of the all-optical production of a single BEC. We show that the all-optical method enables us to realize variety of ultracold Bose-Fermi mixtures.

  18. Interaction of loosely bound radioactive {sup 7}Be and stable {sup 7}Li with {sup 9}Be

    Energy Technology Data Exchange (ETDEWEB)

    Verma, S.; Mandal, S.; Ranjit,; Datta, S.K.; Singh, R. [University of Delhi, Department of Physics and Astrophysics, Delhi (India); Das, J.J.; Jhingan, A.; Golda, K.S.; Madhavan, N.; Sugathan, P.; Nath, S.; Varughese, T.; Gehlot, J. [Inter University Accelerator Centre, New Delhi (India); Kalita, K.; Barua, S. [Gauhati University, Department of Physics, Guwahati (India); Sahu, P.K.; John, B.; Nayak, B.K.; Jha, V.; Saxena, A. [Bhabha Atomic Research Centre, Nuclear Physics Division, Mumbai (India)

    2010-06-15

    Quasielastic scattering angular distributions have been measured for the {sup 7}Be+{sup 9}Be system at E{sub lab} = 17, 19 and 21MeV in the angular range {theta}{sub cm}=24 - 57 . An optical model (OM) analysis of these data has been carried out in order to extract optical potential parameters and reaction cross-sections. One-proton stripping cross-sections were also measured for this system at E{sub lab} = 19 and 21MeV. These transfer angular-distribution data were compared with the finite-range distorted-wave Born approximation (FRDWBA) calculations. For the {sup 7}Li+{sup 9}Be system quasielastic scattering angular distributions were measured and emitted light charged particles were detected at E{sub lab} = 15.75, 24.00 and 30.00MeV in the angular range {theta}{sub cm} = 7 - 70 . Fusion cross-sections were obtained by reproducing the measured {alpha} -evaporation spectra from the compound nucleus at backward angles with the statistical model calculations. The ratios of the experimental fusion cross-sections to the total reaction cross-sections (obtained from OM analysis) were found to be small. This result suggests that the break-up process has a strong influence on the fusion process leading to a reduction in the fusion cross-section. (orig.)

  19. Parsec-scale Variations in the 7Li i/6Li i Isotope Ratio Toward IC 348 and the Perseus OB 2 Association

    Science.gov (United States)

    Knauth, D. C.; Taylor, C. J.; Ritchey, A. M.; Federman, S. R.; Lambert, D. L.

    2017-01-01

    Measurements of the lithium isotopic ratio in the diffuse interstellar medium from high-resolution spectra of the Li i λ6708 resonance doublet have now been reported for a number of lines of sight. The majority of the results for the 7Li/6Li ratio are similar to the solar system ratio of 12.2, but the line of sight toward o Per, a star near the star-forming region IC 348, gave a ratio of about two, the expected value for gas exposed to spallation and fusion reactions driven by cosmic rays. To examine the association of IC 348 with cosmic rays more closely, we measured the lithium isotopic ratio for lines of sight to three stars within a few parsecs of o Per. One star, HD 281159, has 7Li/6Li ≃ 2 confirming production by cosmic rays. The lithium isotopic ratio toward o Per and HD 281159 together with published analyses of the chemistry of interstellar diatomic molecules suggest that the superbubble surrounding IC 348 is the source of the cosmic rays. Based on observations obtained with the Hobby-Eberly Telescope, which is a joint project of the University of Texas at Austin, the Pennsylvania State University, Ludwig-Maximilians-Universität München, and Georg-August-Universität Göttingen.

  20. The study of 12C(α,γ astrophysical reaction using 12C(6Li,d and 12C(7Li,t reaction at 20 MeV and in the framework of the potential model

    Directory of Open Access Journals (Sweden)

    Adhikari S.

    2015-01-01

    Full Text Available The triton angular distribution in the 12C(7Li,t16O reaction has been measured at 20 MeV incident energy. Comparison of the data with Finite Range DWBA and CDCC-CRC calculations show that breakup coupling effects are prominent in the transfer to the ground state. This observation is similar to that in the 12C(6Li,d reaction at the same incident energy. The alpha spectroscopic factor of the 16O ground state is determined (Sα=0.25 from a comparison of the measured angular distribution with respect to the CDCC-CRC calculations. The E2 S-factor of the 12C(α,γ reaction at 300 keV in the framework of a potential model is determined to be about 118 keV-barn.

  1. The use of enriched 6Li and 7Li Lif:Mg,Cu,P glass-rod thermoluminescent dosemeters for linear accelerator out-of-field radiation dose measurements.

    Science.gov (United States)

    Takam, R; Bezak, E; Liu, G; Marcu, L

    2012-06-01

    (6)LiF:Mg,Cu,P and (7)LiF:Mg,Cu,P glass-rod thermoluminescent dosemeters (TLDs) were used for measurements of out-of-field photon and neutron doses produced by Varian iX linear accelerator. Both TLDs were calibrated using 18-MV X-ray beam to investigate their dose-response sensitivity and linearity. CR-39 etch-track detectors (Luxel+, Landauer) were employed to provide neutron dose data to calibrate (6)LiF:Mg,Cu,P TLDs at various distances from the isocentre. With cadmium filters employed, slow neutrons (neutrons. The average in-air photon dose equivalents per monitor unit (MU) ranged from 1.5±0.4 to 215.5±94.6 μSv at 100 and 15 cm from the isocentre, respectively. Based on the cross-calibration factors obtained with CR-39 etch-track detectors, the average in-air fast neutron dose equivalents per MU range from 10.6±3.8 to 59.1±49.9 μSv at 100 and 15 cm from the isocentre, respectively. Contribution of thermal neutrons to total neutron dose equivalent was small: 3.1±7.2 μSv per MU at 15 cm from the isocentre.

  2. Evidence of Cluster Structure of $^9$Be from $^3$He+$^9$Be Reaction

    CERN Document Server

    Lukyanov, S M; Naumenko, M A; Xu, Yi; Trzaska, W H; Burjan, V; Kroha, V; Mrazek, J; Glagolev, V; Piskoř, Š; Voskoboynik, E I; Khlebnikov, S V; Penionzhkevich, Yu E; Skobelev, N K; Sobolev, Yu G; Tyurin, G P; Kuterbekov, K; Tuleushev, Yu

    2015-01-01

    The study of inelastic scattering and multi-nucleon transfer reactions was performed by bombarding a $^{9}$Be target with a $^3$He beam at an incident energy of 30 MeV. Angular distributions for $^9$Be($^3$He,$^3$He)$^{9}$Be, $^9$Be($^3$He,$^4$He)$^{8}$Be, $^9$Be($^3$He,$^5$He)$^{7}$Be, $^9$Be($^3$He,$^6$Li)$^6$Li and $^9$Be($^3$He,$^5$Li)$^7$Li reaction channels were measured. Experimental angular distributions for the corresponding ground states (g.s.) were analysed within the framework of the optical model, the coupled-channel approach and the distorted-wave Born approximation. Cross sections for channels leading to unbound $^5$He$_{g.s.}$, $^5$Li$_{g.s.}$ and $^8$Be systems were obtained from singles measurements where the relationship between the energy and the scattering angle of the observed stable ejectile is constrained by two-body kinematics. Information on the cluster structure of $^{9}$Be was obtained from the transfer channels. It was concluded that cluster transfer is an important mechanism in t...

  3. 6^Li in the atmosphere of GJ 117

    CERN Document Server

    Christian, D J; Jevremovic, D; Hauschildt, P H; Baron, E

    2005-01-01

    We present high resolution VLT UVES observations of the active K dwarf GJ 117. 6^Li enhancement has been shown for energetic solar events, one chromospherically active binary, and several dwarf halo stars. Our analysis reveals the detection of 6^Li on this source with 6^Li/7^Li = 0.030+/-0.010. We found no significant contribution from other lines, including Ti I, in the Li profile of GJ 117 and a template star of similar spectral type and metallicity. We discuss the possibility for 6^Li production by spallation and find it to be consistent with the activity levels of the object.

  4. Big Bang 6Li nucleosynthesis studied deep underground (LUNA collaboration)

    Science.gov (United States)

    Trezzi, D.; Anders, M.; Aliotta, M.; Bellini, A.; Bemmerer, D.; Boeltzig, A.; Broggini, C.; Bruno, C. G.; Caciolli, A.; Cavanna, F.; Corvisiero, P.; Costantini, H.; Davinson, T.; Depalo, R.; Elekes, Z.; Erhard, M.; Ferraro, F.; Formicola, A.; Fülop, Zs.; Gervino, G.; Guglielmetti, A.; Gustavino, C.; Gyürky, Gy.; Junker, M.; Lemut, A.; Marta, M.; Mazzocchi, C.; Menegazzo, R.; Mossa, V.; Pantaleo, F.; Prati, P.; Rossi Alvarez, C.; Scott, D. A.; Somorjai, E.; Straniero, O.; Szücs, T.; Takacs, M.

    2017-03-01

    The correct prediction of the abundances of the light nuclides produced during the epoch of Big Bang Nucleosynthesis (BBN) is one of the main topics of modern cosmology. For many of the nuclear reactions that are relevant for this epoch, direct experimental cross section data are available, ushering the so-called "age of precision". The present work addresses an exception to this current status: the 2H(α,γ)6Li reaction that controls 6Li production in the Big Bang. Recent controversial observations of 6Li in metal-poor stars have heightened the interest in understanding primordial 6Li production. If confirmed, these observations would lead to a second cosmological lithium problem, in addition to the well-known 7Li problem. In the present work, the direct experimental cross section data on 2H(α,γ)6Li in the BBN energy range are reported. The measurement has been performed deep underground at the LUNA (Laboratory for Underground Nuclear Astrophysics) 400 kV accelerator in the Laboratori Nazionali del Gran Sasso, Italy. The cross section has been directly measured at the energies of interest for Big Bang Nucleosynthesis for the first time, at Ecm = 80, 93, 120, and 133 keV. Based on the new data, the 2H(α,γ)6Li thermonuclear reaction rate has been derived. Our rate is even lower than previously reported, thus increasing the discrepancy between predicted Big Bang 6Li abundance and the amount of primordial 6Li inferred from observations.

  5. THE 2H(alpha, gamma6LI REACTION AT LUNA AND BIG BANG NUCLEOSYNTHETIS

    Directory of Open Access Journals (Sweden)

    Carlo Gustavino

    2013-12-01

    Full Text Available The 2H(α, γ6Li reaction is the leading process for the production of 6Li in standard Big Bang Nucleosynthesis. Recent observations of lithium abundance in metal-poor halo stars suggest that there might be a 6Li plateau, similar to the well-known Spite plateau of 7Li. This calls for a re-investigation of the standard production channel for 6Li. As the 2H(α, γ6Li cross section drops steeply at low energy, it has never before been studied directly at Big Bang energies. For the first time the reaction has been studied directly at Big Bang energies at the LUNA accelerator. The preliminary data and their implications for Big Bang nucleosynthesis and the purported 6Li problem will be shown.

  6. Electric dipolarizability of 7Li

    Indian Academy of Sciences (India)

    Sudhir R Jain; Arun K Jain; S Kailas

    2008-12-01

    We calculate the electric dipolarizability of 7Li nucleus within the cluster model and estimate a value of about 0.0188 fm3. We also discuss the possibility of observing this in the scattering of 7Li from a 208Pb target at energies about 30 MeV.

  7. Lamb shifts and hyperfine structure in 6Li+ and 7Li+: Theory and experiment

    DEFF Research Database (Denmark)

    Riis, E.; Sinclair, A. G.; Poulsen, Ove;

    1994-01-01

    High-precision laser-resonance measurements accurate to +/-0.5 MHz, or better are reported for transitions among the 1s2s S-3(1)-1s2p P-3(J) hyperfine manifolds for each of J = 0, 1, and 2 in both Li-6(+) and Li-7(+). A detailed analysis of hyperfine structure is performed for both the S and P...... states, using newly calculated values for the magnetic dipole and electric quadrupole coupling constants, and the hyperfine shifts subtracted from the measurements. The resulting transition frequencies are then analysed on three different levels. First, the isotope shifts in the fine-structure splittings....... The accuracy of 11 parts per million is the best two-electron Lamb shift measurement in the literature, and is comparable to the accuracies achieved in hydrogen. Theoretical contributions to the two-electron Lamb shift are discussed, including terms of order (alpha Z)(4) recently obtained by Chen, Cheng...

  8. Neutron Transfer reactions induced by 8Li on 9Be

    CERN Document Server

    Guimarães, V; Amro, H; Assunção, M; Barioni, A; Becchetti, F D; Carmargo, O; Garcia, H; Jiang, H; Kolata, J J; Lichtenthäler, R; Lizcano, D; Martines-Quiroz, E; Jiang, Hao

    2007-01-01

    Angular distributions for the elastic scattering of 8Li on 9Be and the neutron transfer reactions 9Be(8Li,7Li)10Be and 9Be(8Li,9Li)8Be have been measured with a 27 MeV 8Li radioactive nuclear beam. Spectroscopic factors for 8Li|n=9Li and 7Li|n=8Li bound systems were obtained from the comparison between the experimental differential cross section and finite-range DWBA calculations with the code FRESCO. The spectroscopic factors obtained are compared to shell model calculations and to other experimental values from (d,p) reactions. Using the present values for the spectroscopic factor, cross sections for the direct neutron-capture reactions 7Li(n,g)8Li and 8Li(n,g)9Li were calculated in the framework of a potential model.

  9. /sup 7/Li production in Nova explosions

    Energy Technology Data Exchange (ETDEWEB)

    Starrfield, S.; Truran, J.W.; Sparks, W.M.; Arnould, M.

    1978-06-01

    Calculations of /sup 7/Li production occurring as a concomitant of thermonuclear runaways in hydrogen envelopes of white dwarfs are reported. It is found that sufficient /sup 7/Li can be produced in models displaying fast--nova-like features to suggest that the corresponding objects represent significant contributors to the /sup 7/Li enrichment of galactic matter. The sensitivities of these results to various assumptions and uncertainties are discussed.

  10. Exploring contributions from incomplete fusion in $^{6,7}$Li+$^{209}$Bi and $^{6,7}$Li+$^{198}$Pt reactions

    CERN Document Server

    Parkar, V V; Kailas, S

    2016-01-01

    We use the breakup absorption model to simultaneously describe the measured cross-sections of the Complete fusion (CF), Incomplete fusion (ICF), and Total fusion (TF) in nuclear reactions induced by weakly bound nuclei $^{6,7}$Li on $^{209}$Bi and $^{198}$Pt targets. The absorption cross-sections are calculated using the Continuum Discretized Coupled Channels (CDCC) method with different choices of short range imaginary potentials to get the ICF, CF and TF cross-sections. It is observed that the cross-sections for deuteron-ICF/deuteron-capture are of similar magnitude as the $\\alpha$-ICF/$\\alpha$-capture, in case of $^{6}$Li projectile, while the cross-sections for triton-ICF/triton-capture is more dominant than $\\alpha$-ICF/$\\alpha$-capture in case of $^{7}$Li projectile. Both these observations are also corroborated by the experimental data. The ratio of ICF to TF cross-sections, which defines the value of fusion suppression factor is found to be in agreement with the data available from the literature. The...

  11. First direct measurement of the 2H(α,γ)6Li cross section at big bang energies and the primordial lithium problem.

    Science.gov (United States)

    Anders, M; Trezzi, D; Menegazzo, R; Aliotta, M; Bellini, A; Bemmerer, D; Broggini, C; Caciolli, A; Corvisiero, P; Costantini, H; Davinson, T; Elekes, Z; Erhard, M; Formicola, A; Fülöp, Zs; Gervino, G; Guglielmetti, A; Gustavino, C; Gyürky, Gy; Junker, M; Lemut, A; Marta, M; Mazzocchi, C; Prati, P; Rossi Alvarez, C; Scott, D A; Somorjai, E; Straniero, O; Szücs, T

    2014-07-25

    Recent observations of (6)Li in metal poor stars suggest a large production of this isotope during big bang nucleosynthesis (BBN). In standard BBN calculations, the (2)H(α,γ)(6)Li reaction dominates (6)Li production. This reaction has never been measured inside the BBN energy region because its cross section drops exponentially at low energy and because the electric dipole transition is strongly suppressed for the isoscalar particles (2)H and α at energies below the Coulomb barrier. Indirect measurements using the Coulomb dissociation of (6)Li only give upper limits owing to the dominance of nuclear breakup processes. Here, we report on the results of the first measurement of the (2)H(α,γ)(6)Li cross section at big bang energies. The experiment was performed deep underground at the LUNA 400 kV accelerator in Gran Sasso, Italy. The primordial (6)Li/(7)Li isotopic abundance ratio has been determined to be (1.5 ± 0.3) × 10(-5), from our experimental data and standard BBN theory. The much higher (6)Li/(7)Li values reported for halo stars will likely require a nonstandard physics explanation, as discussed in the literature.

  12. Tritium production in a sphere of /sup 6/LiD irradiated by 14-MeV neutrons

    Energy Technology Data Exchange (ETDEWEB)

    Hemmendinger, A.; Ragan, C.E.; Shunk, E.R.; Ellis, A.N.; Anaya, J.M.; Wallace, J.M.

    1978-10-01

    The specific production of tritium in samples of /sup 6/LiH and /sup 7/LiH embedded in a 600-mm-diam sphere of /sup 6/LiD irradiated by a central source of 14-MeV neutrons was determined by measuring the activity of the hydrogen evolved from the samples of each isotope at each of five different radii in the /sup 6/LiD assembly. The entire process of decomposing the LiH, transferring the evolved gas into counters, and determining the decay rate was standardized by processing LiH samples irradiated by thermal neutrons for which the /sup 6/Li(n,..cap alpha..) cross section is well known. The specific production of tritium in /sup 6/LiH and /sup 7/LiH (embedded samples) and the activation of radiochemical detector foils of /sup 45/Sc, /sup 89/Y, /sup 90/Zr, /sup 169/Tm, /sup 191/Ir /sub 373/, /sup 193/Ir /sub 627/, /sup 197/Au, /sup 235/U, and /sup 238/U placed at various positions in the /sup 6/LiD sphere were calculated and compared with the experimental data. One- and three-dimensional Monte Carlo and S/sub n/ neutron-transport calculations were performed. The most reliable (three-dimensional Monte Carlo) calculation is in reasonable agreement with both the tritium-production and the radiochemical-activation data. The existing discrepancies between calculation and experiment appear largely attributable to uncertainties in some tritium-production and radiochemical-activation cross sections. 15 references.

  13. 6Li foil thermal neutron detector

    Energy Technology Data Exchange (ETDEWEB)

    Ianakiev, Kiril D [Los Alamos National Laboratory; Swinhoe, Martyn T [Los Alamos National Laboratory; Favalli, Andrea [Los Alamos National Laboratory; Chung, Kiwhan [Los Alamos National Laboratory; Macarthur, Duncan W [Los Alamos National Laboratory

    2010-01-01

    In this paper we report on the design of a multilayer thermal neutron detector based on {sup 6}Li reactive foil and thin film plastic scintillators. The {sup 6}Li foils have about twice the intrinsic efficiency of {sup 10}B films and about four times higher light output due to a unique combination of high energy of reaction particles, low self absorption, and low ionization density of tritons. The design configuration provides for double sided readout of the lithium foil resulting in a doubling of the efficiency relative to a classical reactive film detector and generating a pulse height distribution with a valley between neutron and gamma signals similar to {sup 3}He tubes. The tens of microns thickness of plastic scintillator limits the energy deposited by gamma rays, which provides the necessary neutron/gamma discrimination. We used MCNPX to model a multilayer Li foil detector design and compared it with the standard HLNCC-II (18 {sup 3}He tubes operated at 4 atm). The preliminary results of the {sup 6}Li configuration show higher efficiency and one third of the die-away time. These properties, combined with the very short dead time of the plastic scintillator, offer the potential of a very high performance detector.

  14. Lattice dynamics in Bosonic 7 Li

    Science.gov (United States)

    Chen, Huiyao Y.; Jung, Minwoo; Rabinowitz, Jacob; Madjarov, Ivaylo S.; Cheung, Hil F. H.; Patil, Yogesh Sharad; Vengalattore, Mukund

    2016-05-01

    The light mass and strong spin-dependent interactions in 7 Li make it an attractive candidate to study Bosonic quantum magnetism and lattice dynamics in regimes where rapid dynamics is favored, e.g. percolative transport and entropy segregation. Such studies require large ensembles of quantum degenerate 7 Li atoms which has proved to be a technical challenge. We describe our ongoing efforts to overcome this challenge using Raman sideband cooling (RSC). In addition to enabling the rapid production of large degenerate gases, RSC is also a very powerful means of local control of lattice gas dynamics. Extending this to a spinful 7 Li Bose gas will also enable studies of transport and defect dynamics in F=1 lattice gases. This work is supported by the ARO MURI on non-equilibrium dynamics.

  15. Elastic and inelastic scattering of {sup 14}N ions by {sup 7}Li at 80 MeV (c.m. 26.7 MeV)

    Energy Technology Data Exchange (ETDEWEB)

    Rudchik, A.T.; Herashchenko, O.V.; Rudchik, A.A.; Mezhevych, S.Yu.; Mokhnach, A.V.; Pirnak, V.M.; Ponkratenko, O.A.; Ilyin, A.P.; Uleshchenko, V.V. [Institute for Nuclear Research, Kyiv (Ukraine); Kemper, K.W. [Florida State University, Physics Department, Tallahassee, Florida (United States); Rusek, K. [National Institute for Nuclear Research, Warsaw (Poland); Heavy Ion Laboratory of Warsaw University, Warsaw (Poland); Koshchy, E.I. [Kharkiv National University, Kharkiv (Ukraine); Kliczewski, S.; Siudak, R.; Szczurek, A. [H. Niewodniczanski Institute of Nuclear Physics, Cracow (Poland); Plujko, V.A. [Taras Shevchenko Kyiv National University, Kyiv (Ukraine); Choinski, J. [Heavy Ion Laboratory of Warsaw University, Warsaw (Poland); Stolarz, A. [National Institute for Nuclear Research, Warsaw (Poland)

    2014-10-15

    New angular distribution data for {sup 7}Li + {sup 14}N elastic and inelastic scattering at the energy E{sub lab} ({sup 14}N) = 80 MeV (c.m. 26.7MeV) are presented. The data were analyzed within the optical model and the coupled-reaction-channels method using a channels-coupling scheme that included the {sup 7}Li and {sup 14}N inelastic scattering channels, spin reorientations of {sup 7}Li and {sup 14}N as well as most important transfer reactions. The low-energy excited states of {sup 7}Li and {sup 14}N were assumed to be collective in nature. The {sup 7}Li + {sup 14}N potential parameters as well as deformation parameters of {sup 7}Li and {sup 14}N were deduced. The {sup 7}Li + {sup 14}N potential and the data were compared with those of {sup 6}Li + {sup 14}N to observe isotopic differences. The enhanced large-angle elastic and inelastic scattering data are shown to have a large contribution from the ground-state reorientation of {sup 7}Li. (orig.)

  16. Reaction mechanism study of 7Li(7Li, 6He) reaction at above Coulomb barrier energies

    Indian Academy of Sciences (India)

    V V Parkar; V Jha; S Santra; B J Roy; K Ramachandran; A Shrivastava; K Mahata; A Chatterjee; S Kailas

    2009-02-01

    The elastic scattering and the 6He angular distributions were measured in 7Li + 7Li reaction at two energies, lab = 20 and 25 MeV. FRDWBA calculations have been performed to explain the measured 6He data. The calculations were very sensitive to the choice of the optical model potentials in entrance and exit channels. The one-step proton transfer was found to be the dominant reaction mechanism in 6He production.

  17. Relation between (e, e') sum rules in {sup 6,7}Li and {sup 4}He nuclei: Experiment and cluster model

    Energy Technology Data Exchange (ETDEWEB)

    Efros, V.D. [National Research Center ' ' Kurchatov Institute' ' , Moscow (Russian Federation); National Research Nuclear University MEPhI (Moscow Engineering Physics Institute), Moscow (Russian Federation); Timchenko, I.S.; Buki, A.Yu. [National Science Center ' ' Kharkov Institute of Physics and Technology' ' , Kharkov (Ukraine)

    2016-09-15

    The sums over (e, e') spectra of {sup 6}Li and {sup 7}Li nuclei which correspond to the longitudinal sum rule are studied. It is suggested that due to the cluster structure of the lithium isotopes these sums may approximately be expressed in terms of such a sum pertaining to the α-particle. Calculation of these sums is performed in the framework of cluster models with antisymmetrization done with respect to all the nucleons. At momentum transfers higher than 0.8 fm{sup -1} the relations expressing the A = 6 or 7 sum in terms of the A = 4 sum prove to be valid with rather high accuracy. In the region of momentum transfers around 1 fm{sup -1} the longitudinal correlation functions of {sup 6}Li and {sup 7}Li nuclei are found to be close to that of the α-particle. Basing on this, the difference between the q values at which the high-q limit of the inelastic sum rule is reached in the {sup 6,7}Li cases and the {sup 4}He case is explained. The experimental longitudinal sums in the range between 0.450 and 1.625 fm{sup -1} are employed to perform comparison with the theoretical sum rule calculated in the framework of cluster models. Out of the experimental sums, those in the range between 0.750 and 1.000 fm{sup -1} in the {sup 6}Li case and between 0.750 and 1.125 fm{sup -1} in the {sup 7}Li case are obtained in the present work. In the {sup 6}Li case a complete agreement between experiment and the calculated sum rule is found while in the {sup 7}Li case an agreement only at a qualitative level is observed. (orig.)

  18. Triple α resonances in the 6Li + 6Li → 3α reaction at low energy

    Directory of Open Access Journals (Sweden)

    A. Tumino

    2015-11-01

    Full Text Available The 6Li + 6Li → 3α reaction has been measured in a kinematically complete experiment at 3.1 MeV of beam energy. The reaction mainly proceeds via intermediate 8Be states. The interaction between any two of the three α particles provides events with one, two or three 8Be interfering levels, with strong enhancement in the α–α coincidence yield. Evidence of three 8Be levels within the same 3α event suggests that one α particle is exchanged between the other two. This is a condition for Efimov states to occur in nuclei, for which no observation exists yet. The hyperspherical formalism for the low-energy three-body problem has been applied to point out the 3α particle correlation.

  19. Diffusion of $^{6}$Li in Ta and W

    CERN Document Server

    Vacik, J

    2006-01-01

    The objective of this work was the study of 6Li diffusion in the Ta and W refractory metals. The samples were prepared by ion implantation of 380 keV 6Li+ ions into W and Ta thin foils (up to the fluence of 1016 ions/cm2) and annealed up to the temperature 1940 °C. The depth profiles of 6Li were determined using the Thermal Neutron Depth Profiling (TNDP) technique. The results showed that diffusion of 6Li in both W and Ta foils is very complex and cannot be described by simple Fick’s laws. Trapping centers (in the subsurface layers of both W and Ta metals) were supposed in a trial to explain the 6Li diffusion behaviour. However, the 6Li depth profiles were only partly explained. Other aspects are necessary to take into account for more proper quantification; such as spatially dependent diffusion coefficients, etc.

  20. Compounds of 6Li and natural Li for EPR dosimetry in photon/neutron mixed radiation fields.

    Science.gov (United States)

    Lund, E; Gustafsson, H; Danilczuk, M; Sastry, M D; Lund, A

    2004-05-01

    Formates and dithionates of 6Li, enriched and 7Li in natural composition of Li offer a possibility to measure the absorbed dose from photons and thermal neutrons in a mixed radiation field for instance at a boron neutron capture therapy (BNCT) facility. Tests with formates and dithionates of enriched 6Li and lithium compounds with natural composition have been performed at the BNCT facility at Studsvik, Sweden. Irradiations have been performed at 3 cm depth in a Perspex phantom in a fluence rate of thermal neutrons 1.8 x 10(9) n cm(-2) s(-1). The compounds were also irradiated in a pure X-ray field from a 4MV linear accelerator at 5 cm depth in a phantom with accurately determined absorbed doses. The signal intensity and shape was investigated within 3 h after the irradiation. A single line spectrum attributed to the CO2- radical was observed after irradiation of lithium formate. An increase in line width occurring after neutron irradiation in comparison with photon irradiation of the 6Li sample was attributed to dipolar broadening between CO2- radicals trapped in the tracks of the alpha particles. A spectrum due to the SO3- radical anion was observed after irradiation of lithium dithionate. The signal amplitude increased using the 6Li in place of the Li with natural composition of isotopes, in studies with low energy X-ray irradiation. Due to the decreased line width, caused by the difference in g(N) and I between the isotopes, the sensitivity with 6Li dithionate may be enhanced by an order of magnitude compared to alanine dosimetry. After comprehensive examination of the different combinations of compounds with different amounts of 6Li and 7Li regarding dosimetry, radiation chemistry and EPR properties these dosimeter material might be used for dose determinations at BNCT treatments and for biomedical experiments. Interesting properties of the radical formation might be visible due to the large difference in ionization density of neutrons compared to photons.

  1. A method for investigation of the D({sup 4}He, γ){sup 6}Li reaction in the Ultralow energy region under a high background

    Energy Technology Data Exchange (ETDEWEB)

    Bystritsky, V.M. [Joint Institute for Nuclear Research, Dubna (Russian Federation); Dudkin, G.N. [National Research Tomsk Polytechnic University, Tomsk (Russian Federation); Krylov, A.R. [Joint Institute for Nuclear Research, Dubna (Russian Federation); Gazi, S.; Huran, J. [Institute of Electrical Engineering, Slovak Academy of Sciences, Bratislava (Slovakia); Nechaev, B.A.; Padalko, V.N. [National Research Tomsk Polytechnic University, Tomsk (Russian Federation); Sadovsky, A.B. [Joint Institute for Nuclear Research, Dubna (Russian Federation); Tuleushev, Yu.Zh. [Institute of Nuclear Physics, Ministry of Power Engineering, Almaty (Kazakhstan); Filipowicz, M. [Faculty of Energy and Fuels, University of Science and Technologies, Krakow (Poland); Philippov, A.V. [Joint Institute for Nuclear Research, Dubna (Russian Federation)

    2016-07-21

    The cosmological lithium problem, that is, a noticeable discrepancy between the predicted and observed abundances of lithium, is in conflict with the Standard Big Bang Nucleosynthesis model. For example, the abundance of {sup 7}Li is 2–4 times smaller than predicted by the Standard Big Bang Nucleosynthesis. As to the abundance of {sup 6}Li, recent more accurate optical investigations have yielded only the upper limit on the {sup 6}Li/{sup 7}Li ratio, which makes the problem of {sup 6}Li abundance and accordingly of disagreement with the Standard Big Bang Nucleosynthesis predictions less acute. However, experimental study of the D({sup 4}He, γ){sup 6}Li reaction cross section is still of current importance because there is a theoretical approach predicting its anomalously large value in the region of energies below the Standard Big Bang Nucleosynthesis energy. The work is dedicated to the measurement of the cross section for the D({sup 4}He, γ){sup 6}Li reaction proceeding in zirconium deuteride at the incident {sup 4}He{sup +}ion energy of 36 keV. The experiment is performed at a pulsed Hall plasma accelerator with an energy spread of 20% FWHM. A method for direct measurement of the background from the reaction chain D({sup 4}He, {sup 4}He)D→D(D, n){sup 3}He→(n, γ) and/or (n, n′γ) ending with activation of the surrounding material by neutrons is proposed and implemented in the work. An upper limit on the D({sup 4}He, γ){sup 6}Li reaction cross section σ≤7·10{sup −36} cm{sup 2} at the 90% confidence level is obtained.

  2. A method for investigation of the D(4He, γ)6Li reaction in the Ultralow energy region under a high background

    Science.gov (United States)

    Bystritsky, V. M.; Dudkin, G. N.; Krylov, A. R.; Gazi, S.; Huran, J.; Nechaev, B. A.; Padalko, V. N.; Sadovsky, A. B.; Tuleushev, Yu. Zh.; Filipowicz, M.; Philippov, A. V.

    2016-07-01

    The cosmological lithium problem, that is, a noticeable discrepancy between the predicted and observed abundances of lithium, is in conflict with the Standard Big Bang Nucleosynthesis model. For example, the abundance of 7Li is 2-4 times smaller than predicted by the Standard Big Bang Nucleosynthesis. As to the abundance of 6Li, recent more accurate optical investigations have yielded only the upper limit on the 6Li/7Li ratio, which makes the problem of 6Li abundance and accordingly of disagreement with the Standard Big Bang Nucleosynthesis predictions less acute. However, experimental study of the D(4He, γ)6Li reaction cross section is still of current importance because there is a theoretical approach predicting its anomalously large value in the region of energies below the Standard Big Bang Nucleosynthesis energy. The work is dedicated to the measurement of the cross section for the D(4He, γ)6Li reaction proceeding in zirconium deuteride at the incident 4He+ion energy of 36 keV. The experiment is performed at a pulsed Hall plasma accelerator with an energy spread of 20% FWHM. A method for direct measurement of the background from the reaction chain D(4He, 4He)D→D(D, n)3He→(n, γ) and/or (n, n‧γ) ending with activation of the surrounding material by neutrons is proposed and implemented in the work. An upper limit on the D(4He, γ)6Li reaction cross section σ≤7·10-36 cm2 at the 90% confidence level is obtained.

  3. Four-body dynamics in 6Li elastic scattering

    CERN Document Server

    Watanabe, Shin; Ogata, Kazuyuki; Yahiro, Masanobu

    2015-01-01

    We analyze 6Li elastic scattering in a wide range of incident energies (Ein), assuming the n + p + alpha + target four-body model and solving the dynamics with the four-body version of the continuum-discretized coupled-channels method (CDCC). Four-body CDCC well reproduces the experimental data with no adjustable parameter for 6Li + 209Bi scattering at Ein = 24-50 MeV and 6Li + 208Pb scattering at Ein = 29-210 MeV. In the wide Ein range, 6Li breakup is significant and provides repulsive corrections to the folding potential. As an interesting property, d breakup is strongly suppressed in 6Li-breakup processes independently of Ein. We investigate what causes the d-breakup suppression.

  4. Prospective conceptual qualification of hybrid centrifugation/distillatory for {sup 6}LI nuclear fusion technology scaled supply demands; Calificacion conceptual prospectiva de centrifugador/destilador hibrido para produccion de {sup 6}Li a demanda de la tecnologia Nuclear Fusion

    Energy Technology Data Exchange (ETDEWEB)

    Sedano, L.; Herranz, J. L.; Casado, J. L.; Castro, P.; Xiberta, J.

    2013-07-01

    The change in the demand for exploitation of lithium as a resource appears during the last decade, related to the development of the ion-Li batteries market and with the requirements of Nuclear Fusion fuels (deuterium and lithium) as coming energy option. A prospective analysis of synergistic demands of both markets, in its technical and in its economic aspects appears of prospective interest. The civil market {sup 6}Li/{sup 7}Li enrichment demand is analyzed. Specific technological developments permitting on-line production according to demand is discussed. A [centrifugation /thermal diffusion / combined distillation] technique is selected and qualified as technologically viable option for scaled production of litiated-forms. A conceptual design of a production plant is finally proposed according to the new technical capability.

  5. Fusion around the barrier for 7Li + 12C

    Indian Academy of Sciences (India)

    A Mukherjee; M Dasgupta; D J Hinde; C R Morton; A C Berriman; R D Butt; J O Newton; H Timmers

    2001-07-01

    Fusion cross-sections for the 7Li + 12C reaction have been measured at energies above the Coulomb barrier by the direct detection of evaporation residues. The heavy evaporation residues with energies below 3 MeV could not be separated out from the -particles in the spectrum and hence their contribution was estimated using statistical model calculations. The present work indicates that suppression of fusion cross-sections due to the breakup of 7Li may not be significant for 7Li + 12C reaction at energies around the barrier.

  6. Buffer-gas-assisted polarization spectroscopy of 6Li.

    Science.gov (United States)

    Ohtsubo, Nozomi; Aoki, Takatoshi; Torii, Yoshio

    2012-07-15

    We report on the demonstration of Doppler-free polarization spectroscopy of the D2 line of (6)Li atoms. Counterintuitively, the presence of an Ar buffer gas, in a certain pressure range, causes a drastic enhancement of the polarization rotation signal. The observed dependence of the signal amplitude on the Ar buffer pressure and the pump laser power is reproduced by calculations based on simple rate equations. We performed stable laser frequency locking using a dispersion signal obtained by polarization spectroscopy for laser cooling of (6)Li atoms.

  7. Reaction mechanisms in the 6Li+ 52Cr system

    Directory of Open Access Journals (Sweden)

    Pandey Bhawna

    2015-01-01

    Full Text Available Reactions induced by the weakly bound 6Li projectile interacting with the intermediate mass target 52Cr are investigated. The choice of this particular reaction in our study is because it is proposed as a surrogate reaction [6Li(52Cr, d56Fe*] for the measurement of 55Fe(n,p reaction cross-section, which has been found to be very important in fusion reactor studies. All the conditions which have to be satisfied for using the surrogate method have been checked. The energy of 6Li beam is selected in a way so as to get equivalent neutron energy in the region of 9-14 MeV, which is of primary interest in fusion reactor application. In the present work, statistical model calculations PACE (Projection-Angular-Momentum-Coupled-Evaporation, ALICE and Continuum-Discretized–Coupled-Channel (CDCC: FRESCO have been used to provide information for the 6Li + 52Cr system and the respective contributions of different reaction mechanisms. The present theoretical work is an important step in the direction towards studying the cross-section of the 55Fe(n, p55Mn reaction by surrogate method.

  8. Unusual Threshold Anomaly in the 6Li+208Pb System

    Institute of Scientific and Technical Information of China (English)

    ZHANG Chun-Lei; JIA Hui-Ming; WU Zhen-Dong; XU Xin-Xing; BAI Chun-Lin; ZHANG Huan-Qiao; LIN Cheng-Jian; RUAN Ming; LIU Zu-Hua; YANG Feng; WU Xiu-Kun; ZHOU Ping; AN Guang-Peng

    2006-01-01

    @@ The angular distributions of elastic scattering for the 6Li +208Pb system have been measured at several energies around the Coulomb barrier. The parameters of optical potential are extracted by means of a phenomenological optical model analysis. It is found that the real and imaginal potentials show a pronounced energy dependence.The behaviour of the potential at the nearly especially sub-barrier energies in the 6Li+208Pb system is quite different from the results of some previous reports observed in other systems, such as 19 F +208 Pb and 16 O+208 Pb.This unusual threshold phenomenon indicates that breakup channel is strongly coupled with the elastic channel and has obvious effects on optical potential.

  9. Triple α resonances in the {sup 6}Li + {sup 6}Li → 3α reaction at low energy

    Energy Technology Data Exchange (ETDEWEB)

    Tumino, A., E-mail: tumino@lns.infn.it [Facoltà di Ingegneria e Architettura, Università degli Studi di Enna “Kore”, Enna (Italy); INFN, Laboratori Nazionali del Sud, Catania (Italy); Bonasera, A.; Giuliani, G. [INFN, Laboratori Nazionali del Sud, Catania (Italy); Cyclotron Laboratory, Texas A& M University, College Station, TX (United States); Lattuada, M. [INFN, Laboratori Nazionali del Sud, Catania (Italy); Dipartimento di Fisica e Astronomia, Università di Catania, Catania (Italy); Milin, M. [Faculty of Science, University of Zagreb, Zagreb (Croatia); Pizzone, R.G. [INFN, Laboratori Nazionali del Sud, Catania (Italy); Spitaleri, C. [INFN, Laboratori Nazionali del Sud, Catania (Italy); Dipartimento di Fisica e Astronomia, Università di Catania, Catania (Italy); Tudisco, S. [INFN, Laboratori Nazionali del Sud, Catania (Italy)

    2015-11-12

    The {sup 6}Li + {sup 6}Li → 3α reaction has been measured in a kinematically complete experiment at 3.1 MeV of beam energy. The reaction mainly proceeds via intermediate {sup 8}Be states. The interaction between any two of the three α particles provides events with one, two or three {sup 8}Be interfering levels, with strong enhancement in the α–α coincidence yield. Evidence of three {sup 8}Be levels within the same 3α event suggests that one α particle is exchanged between the other two. This is a condition for Efimov states to occur in nuclei, for which no observation exists yet. The hyperspherical formalism for the low-energy three-body problem has been applied to point out the 3α particle correlation.

  10. Coulomb Breakup of Nucleus 6 Li on Ion 208Pb

    OpenAIRE

    Irgaziev, B. F.; ERGASHBAEV, H. T.

    1998-01-01

    In the framework of the three-body approach the A(a,bc)A Coulomb breakup has been investigated. The three-body Coulomb dynamic is taken into account to derive the expression for the reaction matrix element. The mechanism of the breakup includes the direct process and the excitation of resonance state of the particle a. The calculation of the triple differential cross section of the 208Pb(6Li, a d)208Pb Coulomb dissociation have been performed in the energy region Ea d < 1MeV. Cal...

  11. Investigation of α-cluster states in 13C via the (6Li,d) reaction

    CERN Document Server

    Rodrigues, M R D; Horodynski-Matsushigue, L B; Cunsolo, A; Cappuzzello, F; Duarte, J L M; Rodrigues, C L; Ukita, G M; Souza, M A; Miyake, H

    2010-01-01

    The 9Be(6Li,d)13C reaction was used to investigate possible α-cluster states in 13C. The reaction was measured at 25.5 MeV incident energy, employing the São Paulo Pelletron-Enge-Spectrograph facility and the nuclear emulsion detection technique. Ten out of sixteen known levels of 13C, up to 11 MeV of excitation, were observed and, due to the much improved energy resolution of 50 keV, at least three doublets could be resolved. This work presents a preliminary analysis of five of the most intensely populated states, also in comparison with the results of former transfer studies.

  12. The 9Be(d,n) 10B-reaction as intense neutron source with continuous energy spectrum

    Science.gov (United States)

    Baumann, F. M.; Domogala, G.; Freiesleben, H.; Paul, H. J.; Puhlvers, S.; Sohlbach, H.

    1986-06-01

    Neutron energy spectra produced by deuterons of 3 to 8 MeV in a thick 9Be-target were measured at various scattering angles. Significant angle dependences were observed. Angular distributions of the most energetic neutrons produced in thin 9Be targets can be described quantitatively in DWBA, which is an indication for a direct reaction mechanism. As a consequence all but 0°-neutrons are polarized to a certain extent. Also presented is the neutron energy spectrum of 7Li(d,n) 8Be at 0° produced in a thick 7Li-target. The potential of these intense 0°-neutron beams with continuous energy distributions is demonstrated by a measurement of the neutron absorption cross section of natural carbon.

  13. Three-body parameter for Efimov states in 6Li

    Science.gov (United States)

    Huang, Bo; O'Hara, Kenneth M.; Grimm, Rudolf; Hutson, Jeremy M.; Petrov, Dmitry S.

    2014-10-01

    We present a state-of-the-art reanalysis of experimental results on Efimov resonances in the three-fermion system of 6Li. We discuss different definitions of the three-body parameter (3BP) for Efimov states and adopt a definition that excludes effects due to deviations from universal scaling for low-lying states. We develop a finite-temperature model for the case of three distinguishable fermions and apply it to the excited-state Efimov resonance to obtain the most accurate determination to date of the 3BP in an atomic three-body system. Our analysis of ground-state Efimov resonances in the same system yields values for the three-body parameter that are consistent with the excited-state result. Recent work has suggested that the reduced 3BP for atomic systems is a near-universal quantity, almost independent of the particular atom involved. However, the value of the 3BP obtained for 6Li is significantly (˜20 % ) different from that previously obtained from the excited-state resonance in Cs. The difference between these values poses a challenge for theory.

  14. Photoassociative creation of ultracold heteronuclear 6Li40K* molecules

    CERN Document Server

    Ridinger, Armin; Salez, Thomas; Fernandes, Diogo Rio; Bouloufa, Nadia; Dulieu, Olivier; Salomon, Christophe; Chevy, Frederic

    2011-01-01

    We investigate the formation of weakly bound, electronically excited, heteronuclear 6Li40K* molecules by single-photon photoassociation in a magneto-optical trap. We performed trap loss spectroscopy within a range of 325 GHz below the Li(2S_(1/2))+K(4P_(3/2)) and Li(2S_(1/2))+K(4P_(1/2)) asymptotic states and observed more than 60 resonances, which we identify as rovibrational levels of 7 of 8 attractive long-range molecular potentials. The long-range dispersion coefficients and rotational constants are derived. We find large molecule formation rates of up to ~3.5x10^7s^(-1), which are shown to be comparable to those for homonuclear 40K_2*. Using a theoretical model we infer decay rates to the deeply bound electronic ground-state vibrational level X^1\\Sigma^+(v'=3) of ~5x10^4s^(-1). Our results pave the way for the production of ultracold bosonic ground-state 6Li40K molecules which exhibit a large intrinsic permanent electric dipole moment.

  15. Ab initio no-core solutions for $^6$Li

    CERN Document Server

    Shin, Ik Jae; Maris, Pieter; Vary, James P; Forssén, Christian; Rotureau, Jimmy; Michel, Nicolas

    2016-01-01

    We solve for properties of $^6$Li in the ab initio No-Core Full Configuration approach and we separately solve for its ground state and $J^{\\pi}=2_{2}^{+}$ resonance with the Gamow Shell Model in the Berggren basis. We employ both the JISP16 and chiral NNLO$_{opt}$ realistic nucleon-nucleon interactions and investigate the ground state energy, excitation energies, point proton root-mean-square radius and a suite of electroweak observables. We also extend and test methods to extrapolate the ground state energy, point proton root-mean-square radius, and electric quadrupole moment. We attain improved estimates of these observables in the No-Core Full Configuration approach by using basis spaces up through N$_{max}$=18 that enable more definitive comparisons with experiment. Using the Density Matrix Renormalization Group approach with the JISP16 interaction, we find that we can significantly improve the convergence of the Gamow Shell Model treatment of the $^6$Li ground state and $J^{\\pi}=2_{2}^{+}$ resonance by ...

  16. Study of the {sup 6}He+{sup 9}Be elastic scattering at low energies

    Energy Technology Data Exchange (ETDEWEB)

    Pires, K.C.C.; Lichtenthaeler, R.; Lepine-Szily, A.; Guimaraes, V.; Faria, P.N.; Crema, E.; Barioni, A.; Mendes Junior, V.; Morcelle, V.; Morais, M.C.; Pampa Condori, R.; Huiza, J.F.P. [Universidade de Sao Paulo (IF/USP), SP (Brazil). lnst. de Fisica. Dept. de Fisica Nuclear; Moro, A.M.; Rodriguez-Gallardo, M. [University of Seville (Sri Lanka). Dept. of Atomic, Molecular and Nuclear Physics; Assuncao, M. [Universidade Federal de Sao Paulo (UNIFESP), SP (Brazil); Shorto, J.M.B. [Instituto de Pesquisas Energeticas e Nucleares (IPEN/CNEN-SP) Sao Paulo, SP (Brazil); Mukherjee, S. [University of Baroda, Vadodara (India). Faculty of Science. Dept. of Physics

    2011-07-01

    New data of the {sup 6}He+{sup 9}Be elastic scattering at E{sub lab}=16.2MeV and 21.3MeV have been measured. A very large reaction cross section has been previously observed in the collision of {sup 6}He with medium and heavy mass targets, which has been attributed to high 6He breakup probability in the strong Coulomb + nuclear interaction. More recently the importance of neutron transfer reactions between projectile and target has been pointed out. The main goal of the present experiment is to investigate the halo nature of the {sup 6}He nucleus by its interaction with a light target. The experiment has been performed at the Pelletron Laboratory of the Institute of Physics of the University of Sao Paulo, Brazil, using the RIBRAS facility. The RIBRAS system consists of two superconducting solenoids used to focus and select the radioactive secondary beam. The {sup 6}He secondary beam was produced by the {sup 9}Be({sup 7}Li,{sup 6}He) reaction with a {sup 7}Li primary beam of 200nA. The detection system consisted of four {Delta}E-E Silicon telescopes, with 20{mu}m and 1000{mu}m thickness respectively, which allow to separate the {sup 6}He particles from the {sup 7}Li, {sup 4}He, and light particles contaminants. The {sup 6}He+{sup 9}Be angular distributions have been analyzed with optical model, Coupled Channels (CC) and Continuum Discretized Coupled Channels (CDCC) calculations. The comparison between the experimental data and the CDCC calculations allow us to conclude that the breakup of the projectile via the coupling to the {sup 6}He 2{sup +} resonance is very important to reproduce the data. In addition, we studied the effect of excitation of the {sup 9}Be target explicitly by a CC calculation, using a collective model to describe the excitation of the first low lying states of {sup 9}Be. We found that the coupling to these states significantly affects the elastic scattering. From this analysis it was possible to obtain the total reaction cross section which was

  17. Measurement of multinucleon transfer cross-sections in 58Ni,56Fe(12C, ); : 13,11C, 11,10B, 10,9,7Be, 8Be.s. and 7,6Li at (12C) = 60 MeV

    Indian Academy of Sciences (India)

    B J Roy; A Parmar; T Nandi; Biraja Mohanty; M Oswal; Sunil Kumar; A Jhingan; V Jha; D C Biswas

    2016-01-01

    Cross-sections for one- and multinucleon transfer reactions, namely, 58Ni(12C, 13C), 58Ni(12C, 11C), 58Ni(12C, 11B), 58Ni(12C, 10B), 58Ni(12C, 10Be), 58Ni(12C, 9Be), 58Ni(12C, 8Be.s.), 58Ni(12C, 7Be), 58Ni(12C, 7Li) and 58Ni(12C, 6Li) have been measured at an incident energy of 60 MeV. The reaction cross-section for the corresponding transfer channels in the system 12C+56Fe have also been measured under the same kinematical conditions. Angular distribution of the elastic scattering cross-section is measured at 60 MeV. The measured elastic scattering angular distributions for these two systems have been analysed using the optical model search code SFRESCO and the potential parameters are extracted. The multinucleon transfer data are analysed to obtain cross-section dependence on the number of nucleons transferred and on the ground state -values. The transfer probabilities for multinucleon stripping are extracted. A detailed comparison in the multiparticle stripping and elastic scattering cross-sections between these two systems are made to understand the mechanism of multinucleon transfer and possible role of two extra protons in 58Ni target nucleus as compared to the 56Fe core.

  18. Efimov Physics in a 6Li-133Cs Atomic Mixture

    Science.gov (United States)

    Johansen, Jacob; Feng, Lei; Parker, Colin; Chin, Cheng; Wang, Yujun

    2015-05-01

    We investigate Efimov physics based on three-body recombination in an atomic mixture of 6Li and 133Cs in the vicinity of interspecies Feshbach resonances at 843 and 889 G. This allows us to compare the loss spectra near different resonances and test the universality of Efimov states. Theoretically the Efimov spectrum near 889 G is expected to be similar to that near 843 G, except that the first resonance is absent near the former Feshbach resonance. This is due to the difference in the Cs-Cs scattering length near the two resonances: At 843 G it is negative, whereas at 889 G it is positive. Although it is primarily the Li-Cs interactions that lead to Efimov resonances, the Cs-Cs scattering length is expected to influence the spectrum. This work is supported by NSF and Chicago MRSEC.

  19. High-energy break-up of 6Li as a tool to study the Big-Bang nucleosynthesis reaction 2H(alpha,gamma)6Li

    CERN Document Server

    Hammache, F; Typel, S; Galaviz, D; Sümmerer, K; Coc, A; Uhlig, F; Attallah, F; Caamano, M; Cortina, D; Geissel, H; Hellström, M; Iwasa, N; Kiener, J; Koczon, P; Kohlmeyer, B; Mohr, P; Schwab, E; Schwarz, K; Schümann, F; Senger, P; Sorlin, O; Tatischeff, V; Thibaud, J P; Vangioni, E; Wagner, A; Walus, W

    2010-01-01

    The recently claimed observations of non-negligible amounts of 6Li in old halo stars have renewed interest in the Big-Bang Nucleosynthesis (BBN) of 6Li. One important ingredient in the predicted BBN abundance of 6Li is the low-energy 2H(alpha,gamma)6Li cross section. Up to now, the only available experimental result for this cross section showed an almost constant astrophysical S-factor below 400 keV, contrary to theoretical expectations. We report on a new measurement of the 2H(alpha,gamma)6Li reaction using the break-up of 6Li at 150 A MeV. Even though we cannot separate experimentally the Coulomb contribution from the nuclear one, we find clear evidence for Coulomb-nuclear interference by analyzing the scattering-angular distributions. This is in-line with our theoretical description which indicates a drop of the S_24-factor at low energies as predicted also by most other models. Consequently, we find even lower upper limits for the calculated primordial 6Li abundance than before.

  20. Microscopic Model Analysis of the $^{6}He,^{6}Li$ + $^{28}Si$ Total Reaction Cross Sections at the Energy Range 5-50 a Mev

    CERN Document Server

    Lukyanov, K V; Lukyanov, V K; Penionzhkevich, Yu E; Sobolev, Y G; Zemlyanaya, E V; Penionzhkevich, Yu.E.; Sobolev, Yu.G.

    2007-01-01

    The existing and some preliminary experimental data on the total cross sections of the $^{4,6}$He, $^{6,7}$Li +$^{28}$Si reactions at energies E=5-50 A MeV are demonstrated. The data on $^{6}$Li,$^{6}$He+$^{28}$Si are analyzed in the framework of the microscopic optical potential with real and imaginary parts obtained with a help of the double-folding procedure and by using the current models of densities of the projectile nuclei. Besides, the microscopic double-folding Coulomb potential is calculated and its effect on cross sections is compared with that when one applies the traditional Coulomb potential of the uniform charge distribution. The semi-microscopic potentials are constructed from both the renormalized microscopic potentials and their derivatives to take into account collective motion effect and to improve an agreement with experimental data.

  1. All-optical production of 6Li quantum gases

    Science.gov (United States)

    Burchianti, A.; Seman, J. A.; Valtolina, G.; Morales, A.; Inguscio, M.; Zaccanti, M.; Roati, G.

    2015-03-01

    We report efficient production of quantum gases of 6Li using a sub-Doppler cooling scheme based on the D1 transition. After loading in a standard magneto-optical trap, an atomic sample of 109 atoms is cooled at a temperature of 40 μK by a bichromatic D1 gray-molasses. More than 2×107 atoms are then transferred into a high-intensity optical dipole trap, where a two-spin state mixture is evaporatively cooled down to quantum degeneracy. We observe that D1 cooling remains effective in the deep trapping potential, allowing an effective increase of the atomic phase-space density before starting the evaporation. In a total experimental cycle of 11 s, we produce weakly-interacting degenerate Fermi gases of 7×105 atoms at T/TF molecules. We further describe a simple and compact optical system both for high-resolution imaging and for imprinting a thin optical barrier on the atomic cloud; this represents a first step towards the study of quantum tunneling in strongly interacting superfluid Fermi gases.

  2. (9)Be(d,n)(10)B-based neutron sources for BNCT.

    Science.gov (United States)

    Capoulat, M E; Herrera, M S; Minsky, D M; González, S J; Kreiner, A J

    2014-06-01

    In the frame of accelerator-based BNCT, the (9)Be(d,n)(10)B reaction was investigated as a possible source of epithermal neutrons. In order to determine the configuration in terms of bombarding energy, target thickness and Beam Shaping Assembly (BSA) design that results in the best possible beam quality, a systematic optimization study was carried out. From this study, the optimal configuration resulted in tumor doses ≥40Gy-Eq, with a maximum value of 51Gy-Eq at a depth of about 2.7cm, in a 60min treatment. The optimal configuration was considered for the treatment planning assessment of a real Glioblastoma Multiforme case. From this, the resulted dose performances were comparable to those obtained with an optimized (7)Li(p,n)-based neutron source, under identical conditions and subjected to the same clinical protocol.

  3. Thin target sup 7 Li(p, p'gamma) sup 7 Li inelastic gamma-ray yield measurements

    CERN Document Server

    Aslam; McNeill, F E

    2002-01-01

    Thin target angular distributions of inelastic gamma-ray yields resulting from sup 7 Li(p, p'gamma) sup 7 Li interaction have been measured for incident proton energies between 1.0 and 1.8 MeV. McMaster 3 MV KN Van de Graaff accelerator facility primarily dedicated to in-vivo neutron activation measurements has been used to perform experiments using a thin lithium metal target and 7.62 cm x 7.62 cm, 12.7 cm x 12.7 cm NaI(Tl) scintillation detectors and HPGe detectors. The uncertainty in the relative yield determination is based on the statistics of the data, uncertainty in the 478 keV peak area determination due to other interfering reactions, and the uncertainty in the recording of the proton charge. The results for the angular distribution provide an evidence for anisotropic nature of the radiation as compared to the presumed isotropic nature. The total relative yield was determined from the angular distributions and then compared with the published total cross sections for the reaction. Thick target yields...

  4. Search for the Halo Effect in the ~1H(~6He, ~6Li)n Reaction

    Institute of Scientific and Technical Information of China (English)

    2001-01-01

    The experiment is carried out using the secondary beam facility of the HI-13 tandem accelerator at China Institute of Atomic Energy, Beijing. The experimental setup is similar to the previously illustrated. A 7Li beam with energy of 44 MeV from the tandem impinged on a D2 gas cell at pressure of 1.5×105 Pa, in which 6He ions are produced via 2H(7Li, 6He)3He reaction. The front and rear

  5. Magnetic signature of charge ordering in Li[Mn sub 1 sub . sub 9 sub 6 Li sub 0 sub . sub 0 sub 4]O sub 4 and Li sub 0 sub . sub 2 [Mn sub 1 sub . sub 9 sub 6 Li sub 0 sub . sub 0 sub 4]O sub 4

    CERN Document Server

    Verhoeven, V W J; Mulder, F M

    2002-01-01

    The stoichiometric compound LiMn sub 2 O sub 4 is known to show charge ordering with well-defined Mn sup 3 sup + and Mn sup 4 sup + sites just below room temperature (RT). Above RT the electrons are hopping rapidly between sites. For lithium-ion batteries the material Li[Mn sub 1 sub . sub 9 sub 6 Li sub 0 sub . sub 0 sub 4]O sub 4 is technologically relevant. Due to the small amount of Li on the Mn site, the low-T regular ordering of the Mn charge appears to be destroyed completely, as is evidenced by neutron diffraction in the magnetically ordered state. However, the charges are still fixed in an irregular fashion, as can also be deduced from sup 7 Li nuclear magnetic resonance measurements. In the lithium-extracted compound Li sub 0 sub . sub 2 [Mn sub 1 sub . sub 9 sub 6 Li sub 0 sub . sub 0 sub 4]O sub 4 , predominantly Mn sup 4 sup + is present. Neutron diffraction in the magnetically ordered state shows a well-defined antiferromagnetic ordering, with doubling of the unit cell in three directions. Clear...

  6. Characterization of {sup 6}LiF:Mg,Cu,P (TLD-600 H) estimate of E, b and s parameters

    Energy Technology Data Exchange (ETDEWEB)

    Andres, P. A., E-mail: andresp@cab.cnea.gov.ar [Centro Atomico Bariloche, Division Proteccion Radiologica / CNEA, Av. E. Bustillo Km 9.5, R8402AGP San Carlos de Bariloche (Argentina)

    2015-10-15

    LiF:Mg,Cu,P dosemeters are useful for low-dose measurements because of its high sensitivity compared to the LiF:Mg,Ti dosemeters. {sup 7}LiF:Mg,Cu,P have been used for environmental dosimetry in Bariloche Atomic Centre for almost a decade. Since {sup 6}LiF:Mg,Cu,P dosemeters were intended to be used for X ray diagnosis dosimetry in neonatology, they had to be characterized first. The main goal of measuring and analyzing Tl glow curves is the extraction of some parameters that can be used to describe the Tl process in the material. This job focused on the estimation of the activation energy E for the Tl traps, the frequency factor s and the order of kinetics b of the Tl process. Furthermore, the most appropriate time-temperature profile (Ttp) was determined as well as the annealing temperature and time, which resulted being 240 degrees C for 10 minutes. The Ttp used was 140 degrees C for 10 seconds, a heating rate of 20/s until 240 degrees C, remaining at this temperature for 20 seconds, and then an exponential cooling until 50 degrees C. After applying the whole glow-peak method for different orders of kinetic, and the Kitis equation assuming a first order kinetics, the values obtained were: E = (1.066 ± 0.025) eV, as a weighted average of both methods, and a frequency factor s = (3.57 ± 1.56) E-10 s{sup -1} again as a weighted average of both methods. In both cases a first order kinetics (b = 1) was assumed. The dosemeters were irradiated with a calibrated {sup 137}Cs source and read with a Harshaw TLD{sup TM} Model 3500 reader resulting in a minimum detectable dose of about 20 μGy. (Author)

  7. Studies of the Efimov Effect in 7 Li

    Science.gov (United States)

    Luo, D.; Nguyen, J. H. V.; Hulet, R. G.

    2016-05-01

    Ultracold atomic gases provide an ideal environment to study few body physics in the universal regime. Passive techniques, such as monitoring loss of the atomic sample while varying the hold time allows us to explore properties such as the scaling behavior of Efimov trimers. In our experiment, we explore how the Efimov states are affected by non-zero temperature. We measure the three-body loss rate for a 7 Li atom gas at different scattering lengths and extract the location and width of an Efimov recombination minimum for various temperatures. Alternatively, we may perform more active experiments such as creating dimers using RF-field modulation as a probe of molecular binding energies. We use RF-association to form Feshbach dimers and Efimov trimers, and find a strong enhancement of the dimer formation rate at the atom-dimer resonance, which could be explained by an avalanche mechanism. In the past the enhancement in the three-body recombination rate at the same location had also been observed, and attributed to the avalanche. We explore the link between these findings with a side-by-side comparison of the dimer-formation rate and the three-body loss rate. Work supported by the NSF, an ARO MURI Grant, and the Welch Foundation.

  8. Non-Gaussian error distribution of 7Li abundance measurements

    Science.gov (United States)

    Crandall, Sara; Houston, Stephen; Ratra, Bharat

    2015-07-01

    We construct the error distribution of 7Li abundance measurements for 66 observations (with error bars) used by Spite et al. (2012) that give A(Li) = 2.21 ± 0.065 (median and 1σ symmetrized error). This error distribution is somewhat non-Gaussian, with larger probability in the tails than is predicted by a Gaussian distribution. The 95.4% confidence limits are 3.0σ in terms of the quoted errors. We fit the data to four commonly used distributions: Gaussian, Cauchy, Student’s t and double exponential with the center of the distribution found with both weighted mean and median statistics. It is reasonably well described by a widened n = 8 Student’s t distribution. Assuming Gaussianity, the observed A(Li) is 6.5σ away from that expected from standard Big Bang Nucleosynthesis (BBN) given the Planck observations. Accounting for the non-Gaussianity of the observed A(Li) error distribution reduces the discrepancy to 4.9σ, which is still significant.

  9. Study of the {sup 6}He+{sup 9}Be reaction at low energies

    Energy Technology Data Exchange (ETDEWEB)

    Pires, K.C.C.; Lichtenthaeler, R.; Lepine-Szily, A. [Universidade de Sao Paulo (IF/USP), SP (Brazil). Inst. de Fisica. Dept. de Fisica Nuclear

    2010-07-01

    Full text: Elastic scattering measurements of the exotic {sup 6}He nuclei on heavy and medium mass targets (eg. {sup 6}He+{sup 208}Pb, {sup 6}He+{sup 64}Zn) show large values of the reaction cross section compared with reactions induced by stable weakly bound projectiles. This phenomenon could be a consequence of the halo nature of the {sup 6}He, which can easily breakup in the Coulomb and nuclear fields of the target. In this work we present new scattering data of the light system {sup 6}He+{sup 9}Be at E{sub lab} = 16:2 MeV and E{sub lab} = 21:3 MeV. For this light system the Coulomb interaction is small compared to the nuclear and the Coulomb breakup of the projectile is expected to have little influence. The measurements have been performed at the Pelletron Laboratory of the Institute of Physics of the University of Sao Paulo, Brazil, using the RIBRAS facility. The RIBRAS system consists of two superconducting solenoids used to focalize and select the radioactive secondary beam. The {sup 6}He beam was produced using the {sup 9}Be({sup 7}Li,{sup 6}He) production reaction. The detection system consisted of four {Delta}E-E Silicon telescopes, with 20{mu}m and 1000{mu}m thickness respectively which allow to separate the {sup 6}He particles from the {sup 7}Li beam contaminant and light particles. We performed optical model, coupled channels and CDCC calculations. In the last one, the continuum spectrum was discretized in energy bins. The comparison between the experimental data and the optical model and CDCC calculations allow us to conclude that even for these light targets the breakup of the projectile and the coupling to the 2{sup +} resonance of {sup 6}He nucleus is very important. Furthermore, using the coupled channels method, we studied the effect of excitation of the target explicitly, using a collective model for describe the coupling to the first states of {sup 9}Be nucleus. We found that the coupling to these states also affects the elastic scattering

  10. Search for the Halo Effect in the 1H(6He, 6Li)n Peaction

    Institute of Scientific and Technical Information of China (English)

    李志宏; 柳卫平; 白希祥; 王友宝; 连钢; 李志常; 申庆彪; 林承键; 曾晟; 符长波

    2002-01-01

    The angular distributions of the charge exchange reaction 1 H(6He, 6Li)n were measured in reverse kinematics with a secondary 6He beam at the energy of4.17 AMeV. The data were analysed in the context ora microscopic calculation. It is shown that both the ground state of6He and the second excited state of6Li (3.563 MeV, 0+) have a halo structure.

  11. 6LiF oleic acid capped nanoparticles entrapment in siloxanes for thermal neutron detection

    Science.gov (United States)

    Carturan, S.; Maggioni, G.; Marchi, T.; Gramegna, F.; Cinausero, M.; Quaranta, A.; Palma, M. Dalla

    2016-07-01

    The good light output of siloxane based scintillators as displayed under γ-rays and α particles has been exploited here to obtain clear and reliable response toward thermal neutrons. Sensitization towards thermal neutrons has been pursued by adding 6LiF, in form of nanoparticles. Aiming at the enhancement of compatibility between the inorganic nanoparticles and the low polarity, siloxane based surrounding medium, oleic acid-capped 6LiF nanoparticles have been synthesized by thermal decomposition of Li trifluoroacetate. Thin pellets siloxane scintillator maintained their optical transmittance up to weight load of 2% of 6Li. Thin samples with increasing 6Li concentration and thicker ones with fixed 6Li amount have been prepared and tested with several sources (α, γ-rays, moderated neutrons). Light output as high as 80% of EJ212 under α irradiation was measured with thin samples, and negligible changes have been observed as a result of 6LiF addition. In case of thick samples, severe light loss has been observed, as induced by opacity. Nevertheless, thermal neutrons detection has been assessed and the data have been compared with GS20, based on Li glass, taken as a reference material.

  12. Determining the 6Li Doped Side of a Glass Scintillator for Ultra Cold Neutrons

    CERN Document Server

    Jamieson, Blair

    2015-01-01

    Ultracold neutron (UCN) detectors using two visually very similar, to the microscopic level, pieces of optically contacted Cerium doped lithium glasses have been proposed for high rate UCN experiments. The chief difference between the two glass scintillators is that one side is 6Li depleted and the other side Li doped. This note outlines a method to determine which side of the glass stack is doped with 6Li using AmBe and 252Cf neutron sources, and a Si surface barrier detector. The method sees an excess of events around the alpha and triton energies of neutron capture on 6Li when the enriched side is facing the Si surface barrier detector.

  13. Properties of 4He and 6Li with improved chiral EFT interactions

    Science.gov (United States)

    Maris, P.; Binder, S.; Calci, A.; Epelbaum, E.; Furnstahl, R. J.; Golak, J.; Hebeler, K.; Kamada, H.; Krebs, H.; Langhammer, J.; Liebig, S.; Meißner, U.-G.; Minossi, D.; Nogga, A.; Potter, H.; Roth, R.; Skibiński, R.; Topolnicki, K.; Vary, J. P.; Witala, H.

    2016-03-01

    We present recent results for 4He and 6Li obtained with improved NN interactions derived from chiral effective field theory up to N4LO. The many-body calculations are performed order-by-order in the chiral expansion. At N3LO and N4LO additional renormalization using the Similarity Renormalization Group is adopted to improve numerical convergence of the many-body calculations. We discuss results for the ground state energies, as well as the magnetic moment and the low-lying spectrum of 6Li.

  14. Properties of 4He and 6Li with improved chiral EFT interactions

    Directory of Open Access Journals (Sweden)

    Maris P.

    2016-01-01

    Full Text Available We present recent results for 4He and 6Li obtained with improved NN interactions derived from chiral effective field theory up to N4LO. The many-body calculations are performed order-by-order in the chiral expansion. At N3LO and N4LO additional renormalization using the Similarity Renormalization Group is adopted to improve numerical convergence of the many-body calculations. We discuss results for the ground state energies, as well as the magnetic moment and the low-lying spectrum of 6Li.

  15. Cosmic Ray Production of $^6$Li by Structure Formation Shocks in the Early Galaxy

    CERN Document Server

    Inoue, S; Inoue, Susumu; Suzuki, Takeru Ken

    2003-01-01

    We discuss the production of the element $^6$Li in the early Galaxy by cosmic rays accelerated at structure formation shocks, driven by the hierarchical merging of sub-Galactic halos during Galaxy formation. The salient features of this scenario are discussed and compared with observations of $^6$Li in metal-poor halo stars, including a recent Subaru HDS result on the star HD140283. Some unique predictions of the model are clearly testable by future observations and may also provide important insight into how the Galaxy formed.

  16. Study of reactions induced by 6He on 9Be

    Directory of Open Access Journals (Sweden)

    Pires K.C.C.

    2014-03-01

    Full Text Available We present the results of experiments using a 6He beam on a 9Be target at energies 7 − 9 times the Coulomb barrier. Angular distributions of the elastic, inelastic scattering (target breakup and the a-particle production in the 6He+9Be collision have been analysed. Total reaction cross sections were obtained from the elastic scatteringanalyses and a considerable enhancement has been observed by comparing to stable systems.

  17. Basic technology for {sup 6}Li enrichment using an ionic-liquid impregnated organic membrane

    Energy Technology Data Exchange (ETDEWEB)

    Hoshino, Tsuyoshi, E-mail: hoshino.tsuyoshi@jaea.go.jp [Blanket Irradiation and Analysis Group, Fusion Research and Development Directorate, Japan Atomic Energy Agency, 4002, Narita-cho, Oarai-machi, Higashi Ibaraki-gun, Ibaraki 311-1393 (Japan); Terai, Takayuki [The Institute of Engineering Innovation and Department of Nuclear Engineering and Management School of Engineering, The University of Tokyo, 2-11-16 Yayoi, Bunkyo-ku, Tokyo 113-8656 (Japan)

    2011-10-01

    The tritium needed as a fuel for fusion reactors is produced by the neutron capture reaction of lithium-6 ({sup 6}Li) in tritium breeding materials. However, natural Li contains only about 7.6 at.% {sup 6}Li. In this paper, a new lithium isotope separation technique using an ionic-liquid impregnated organic membrane is proposed. In order to separate and concentrate lithium isotopes, only lithium ions are able to move through the membrane by electrodialysis between the cathode and the anode in lithium solutions. Preliminary experiments of lithium isotope separation were conducted using this phenomenon. Organic membranes impregnated with TMPA-TFSI and PP13-TFSI as ionic liquids were prepared, and the relationship between the {sup 6}Li separation coefficient and the applied electrodialytic conditions was evaluated using them. The results showed that the {sup 6}Li isotope separation coefficient in this method (about 1.1-1.4) was larger than that in the mercury amalgam method (about 1.06).

  18. Resonant, direct, and transfer breakup of 6Li by 112Sn

    Science.gov (United States)

    Chattopadhyay, D.; Santra, S.; Pal, A.; Kundu, A.; Ramachandran, K.; Tripathi, R.; Sarkar, D.; Sodaye, S.; Nayak, B. K.; Saxena, A.; Kailas, S.

    2016-12-01

    Projectile breakup cross sections in the 6Li+112Sn reaction have been measured at two beam energies, 30 and 22 MeV. Cross sections for sequential breakup of 6Li into α +d via its resonant state of 1+ (5.65 MeV) in the continuum have been measured for the first time along with two other dominant resonant states of 3+ (2.18 MeV) and 2+ (4.31 MeV) at Ebeam=30 MeV. However, at 22 MeV, the α +d breakup is found to be only due to direct breakup process. Cross sections measured for sequential breakup via two transfer channels, (6Li,5Li ) and (6Li,8Be ), into α +p and α +α , respectively, and the above α +d breakup channels compared with the results of coupled-channels calculations unravel the reaction mechanisms involving a weakly bound projectile and different processes leading to large inclusive α -particle production.

  19. Nuclear reactions of the system {sup 6} Li on {sup 58} Ni near the Coulomb barrier; Reacciones nucleares del sistema {sup 6} Li sobre {sup 58} Ni cerca de la barrera de Coulomb

    Energy Technology Data Exchange (ETDEWEB)

    Lizcano, D.; Aguilera, E.F.; Garcia M, H.; Martinez Q, E. [ININ, 52045 Ocoyoacac, Estado de Mexico (Mexico)

    2004-07-01

    Protons, alpha particles and deuterons coming from the reactions {sup 6} Li + {sup 58} Ni are detected to three different energy around the Coulomb barrier. The possible effects of the weakly bound character of the projectile are studied and the results are compared with previous data for the system {sup 6} Li + {sup 59} Co. (Author)

  20. Breakup mechanisms for 7Li + 197Au, 204Pb systems at sub-barrier energies

    Directory of Open Access Journals (Sweden)

    Luong D.H.

    2013-12-01

    Full Text Available Coincidence measurements of breakup fragments were carried out for the 7Li + 197Au and 204Pb systems at sub-barrier energies. The mechanisms triggering breakup, and time-scales of each process, were identified through the reaction Q-values and the relative energy of the breakup fragments. Binary breakup of 7Li were found to be predominantly triggered by nucleon transfer, with p-pickup leading to 8Be → α + α decay being the preferred breakup mode. From the time-scales of each process, the coincidence yields were separated into prompt and delayed components, allowing the identification of breakup process important in the suppression of complete fusion of 7Li at above-barrier energies.

  1. Radioactive contamination of {sup 7}LiI(Eu) crystal scintillators

    Energy Technology Data Exchange (ETDEWEB)

    Belli, P. [INFN sezione Roma “Tor Vergata”, I-00133 Rome (Italy); Dipartimento di Fisica, Università di Roma “Tor Vergata”, I-00133 Rome (Italy); Bernabei, R., E-mail: rita.bernabei@roma2.infn.it [INFN sezione Roma “Tor Vergata”, I-00133 Rome (Italy); Dipartimento di Fisica, Università di Roma “Tor Vergata”, I-00133 Rome (Italy); Budakovsky, S.V. [Institute for Scintillation Materials, 61001 Kharkiv (Ukraine); Cappella, F. [INFN sezione Roma “La Sapienza”, I-00185 Rome (Italy); Dipartimento di Fisica, Università di Roma “La Sapienza”, I-00185 Rome (Italy); Cerulli, R. [INFN, Laboratori Nazionali del Gran Sasso, I-67100 Assergi (AQ) (Italy); Danevich, F.A. [Institute for Nuclear Research, MSP 03680 Kyiv (Ukraine); D' Angelo, S. [INFN sezione Roma “Tor Vergata”, I-00133 Rome (Italy); Dipartimento di Fisica, Università di Roma “Tor Vergata”, I-00133 Rome (Italy); Incicchitti, A. [INFN sezione Roma “La Sapienza”, I-00185 Rome (Italy); Dipartimento di Fisica, Università di Roma “La Sapienza”, I-00185 Rome (Italy); Laubenstein, M. [INFN, Laboratori Nazionali del Gran Sasso, I-67100 Assergi (AQ) (Italy); Poda, D.V. [Institute for Nuclear Research, MSP 03680 Kyiv (Ukraine); and others

    2013-03-11

    The radioactive contamination of two 26 g samples of low background lithium iodide crystal scintillators doped by europium and enriched in {sup 7}Li to 99.9% ({sup 7}LiI(Eu)) has been investigated by scintillation method at the sea level, and by ultra-low background HPGe γ spectrometry deep underground. No radioactive contamination was detected. In particular, the contamination of the crystal scintillators by {sup 226}Ra and {sup 228}Th does not exceed 1 mBq/kg, and the activity of {sup 40}K is less than 0.5 Bq/kg.

  2. Report for in-situ 7Li NMR experiment in PNNL Phase -1

    Energy Technology Data Exchange (ETDEWEB)

    Hu, Jian Zhi [Pacific Northwest National Laboratory

    2014-08-19

    To understand the detailed local structural evolution, an in-situ 7Li NMR study was performed. An operando identification of the lithium germanide phases under various cycling regimens permitted understanding of the kinetics of phase transition between different structural phases, including the amorphous phases, and how these correlated with capacity retention. Combining data from TEM and in-situ 7Li NMR, we discovered that the phase inter-conversion during cycling was mediated by co-existing amorphous and crystalline phases, and that the high capacity observed was correlated with an over-lithiated lithium germanide phase.

  3. Search for higher excited states of $^{8}$Be* to study the cosmological $^{7}$Li problem

    CERN Multimedia

    We would like to study the unresolved $^{7}$Li abundance anomaly by carrying out experiments that destroy the rare isotope $^{7}$Be, the main source of $^{7}$Li. Utilizing a 35 MeV $^{7}$Be beam from HIE-ISOLDE, we would like to measure the (d,p) and (d,d) reactions with T-REX. The higher beam energy, for the first time, would allow us to measure higher excitation energies in $^{8}$Be up to about 20 MeV. With a wider angular coverage, we can make improved average cross-section measurement without assuming isotropy done in earlier works.

  4. Inelastic p{sup 9}Be scattering and halo-structure of excited states of {sup 9}Be

    Energy Technology Data Exchange (ETDEWEB)

    Ibraeva, E.T., E-mail: ibraeva.elena@gmail.com [Institute of Nuclear Physics RK, 050032, str. Ibragimova 1, Almaty (Kazakhstan); Zhusupov, M.A. [Al-Farabi Kazakh National University, 050040, av. Al-Farabi 71, Almaty (Kazakhstan); Dzhazairov-Kakhramanov, A.V., E-mail: albert-j@yandex.ru [Institute of Nuclear Physics RK, 050032, str. Ibragimova 1, Almaty (Kazakhstan); V.G. Fessenkov Astrophysical Institute “NCSRT” NSA RK, 050020, Observatory 23, Kamenskoe plato, Almaty (Kazakhstan); Krassovitskiy, P.M. [Institute of Nuclear Physics RK, 050032, str. Ibragimova 1, Almaty (Kazakhstan)

    2015-01-15

    The calculation of the differential cross-section of inelastic p{sup 9}Be scattering (to the levels J{sup π}=1/2{sup +}, 3/2{sup +}) was made in the framework of the Glauber diffraction theory. We have used the wave function of {sup 9}Be in the ground and excited states in the three-body 2αn model. Expansion in series by gaussoids of the wave function of {sup 9}Be and presentation of the Glauber's operator Ω in the form, conjugated with three-body wave function make it possible for us to analytically calculate the matrix elements of inelastic scattering, taking into account all of the multiplicities of scattering and rescattering on clusters and nucleons, which are components of {sup 9}Be. The drawn-up profiles of probability densities of excited state functions allow us to form conclusions on their extended neutron distribution. The differential cross-section with the wave function in model 1 (with the αα-Ali–Bodmer potential) is in good agreement with available experimental data at E=180 MeV.

  5. Faddeev calculations for the Λ9Be spectrum

    Directory of Open Access Journals (Sweden)

    Vlahovic B.

    2010-04-01

    Full Text Available An α-cluster model is applied to study low-lying spectrum of the Λ9Be hypernicleus. The ααΛ three-body problem is numerically solved by the Faddeev equations in configuration space using phenomenological pair potentials. Found is a set of the potentials that reproduces experimental data for the ground state (1+/2 binding energy and excitation energy of the 5+/2 and 3+/2 states, simultaneously. This set includes the Ali-Bodmer potential of version “e” for αα and modified Tang-Herndon potential for αΛ interactions. The spin-orbit αΛ interaction is given by modified Scheerbaum potential. Low-lying energy levels are evaluated applying a variant of the analytical continuation method in coupling constant, and the experimental data for excitation energies are well reproduced by our calculations. This result improves previous α-cluster calculations. It is shown that the spectral properties of Λ9Be can be classified as an analog of 9Be spectrum with the exception of several “genuine hypernuclear states”, which agrees qualitatively with previous studies. The energy splitting of spin-flip doublet (9+/2 , 7+/2 is predicted.

  6. Importance of $1n$-stripping process in the $^{6}$Li+$^{159}$Tb reaction

    CERN Document Server

    Pradhan, M K; Roy, Subinit; Basu, P; Goswami, A; Kshetri, R; Palit, R; Parkar, V V; Ray, M; Sarkar, M Saha; Santra, S

    2013-01-01

    The inclusive cross sections of the $\\alpha$-particles produced in the reaction $^{6}$Li+$^{159}$Tb have been measured at energies around the Coulomb barrier. The measured cross sections are found to be orders of magnitude larger than the calculated cross sections of $^{6}$Li breaking into $\\alpha$ and $d$ fragments, thus indicating contributions from other processes. The experimental cross sections of $1n$-stripping and $1n$-pickup processes have been determined from an entirely different measurement, reported earlier. Apart from incomplete fusion and/ $d$-transfer processes, the $1n$-stripping process is found to be a significant contributor to the inclusive $\\alpha$-particle cross sections in this reaction.

  7. Narrow-linewidth cooling of $^{6}$Li atoms using the 2S-3P transition

    CERN Document Server

    Chen, Hao-Ze; Wu, Yu-Ping; Liu, Xiang-Pei; Wang, Xiao-Qiong; Chen, Yu-Ao; Pan, Jian-Wei

    2016-01-01

    We report on a narrow-linewidth cooling of $^{6}$Li atoms using the $2S_{1/2}\\to 3P_{3/2}$ transition in the ultraviolet (UV) wavelength regime. By combining the traditional red magneto-optical trap (MOT) at 671 nm and the UV MOT at 323 nm, we obtain a cold sample of $1.3\\times10^9$ atoms with a temperature of 58 $\\mu$K. Furthermore, we demonstrate a high efficiency magnetic transport for $^{6}$Li atoms with the help of the UV MOT. Finally, we obtain $8.1\\times10^8$ atoms with a temperature of 296 $\\mu$K at a magnetic gradient of 198 G/cm in the science chamber with a good vacuum environment and large optical access.

  8. Formation of eta'(958) Meson Bound States by the 6Li(gamma,d) reaction

    CERN Document Server

    Miyatani, M; Nagahiro, H; Hirenzaki, S

    2016-01-01

    We have investigated the 6Li(gamma,d) reaction theoretically for the formation of the eta'(958) mesic nucleus close to the recoilless kinematics. We have developed the theoretical formula and reported the quantitative results of the formation spectra for various cases in this article. We have found that the formation cross sections are reduced by the effects of the fragile deuteron form factor.

  9. Autler-Townes splitting in two-color photoassociation of 6Li

    CERN Document Server

    Schloeder, U; Silber, C; Zimmermann, C; Schloeder, Ulrike; Deuschle, Thomas; Silber, Christian; Zimmermann, Claus

    2003-01-01

    We report on high-resolution two-color photoassociation spectroscopy in the triplet system of magneto-optically trapped 6Li. The absolute transition frequencies have been measured. Strong optical coupling of the bound molecular states has been observed as Autler-Townes splitting in the photoassociation signal. The spontaneous bound-bound transition rate is determined and the molecule formation rate is estimated. The observed lineshapes are in good agreement with the theoretical model.

  10. Refractive effects in 9Be scattering and nuclear rainbow ghosts

    Science.gov (United States)

    Satchler, G. R.; Fulmer, C. B.; Auble, R. L.; Ball, J. B.; Bertrand, F. E.; Erb, K. A.; Gross, E. E.; Hensley, D. C.

    1983-08-01

    Data for the elastic scattering of 9Be on 12C and 16O at 158 MeV provide evidence of refractive effects that allow the optical potentials to be determined with little ambiguity. The real potentials are deep. Large angle data indicate dominance of negative-angle scattering from the far side of the target nucleus. The analysis also implies a residual rainbow phenomenon, contrary to what has been seen previously in heavy-ion scattering. We suggest this be called a rainbow ghost. Operated by Union Carbide Corporation under contract W-7405-eng-26 with the US Department of Energy.

  11. Optimization of {sup 6}LiF:ZnS(Ag) Scintillator Light Yield Using Geant4

    Energy Technology Data Exchange (ETDEWEB)

    Yehuda-Zada, Y. [Nuclear Research Center Negev, Beer-Sheva (Israel); Ben-Gurion University (Israel); Pritchard, K.; Ziegler, J.B.; Cooksey, C.; Siebein, K. [National Institute of Standards and Technology, Gaithersburg, Maryland (United States); Jackson, M.; Hurlbut, C. [Eljen Technology, Sweetwater Texas (United States); Kadmon, Y.; Cohen, Y.; Maliszewskyj, N.C. [Nuclear Research Center Negev, Beer-Sheva (Israel); Ibberson, R.M.; Majkrzak, C.F. [National Institute of Standards and Technology, Gaithersburg, Maryland (United States); Orion, Y. [Ben-Gurion University (Israel); Osovizky, A. [National Institute of Standards and Technology, Gaithersburg, Maryland (United States); Rotem Industries Ltd, Rotem Industrial Park (Israel); University of Maryland (United States)

    2015-07-01

    Neutrons provide an effective tool to probe materials structure. Neutron diffraction is a method to determine the atomic and magnetic structure of a material based on neutron scattering. By this method a collimated incident beam of thermal neutrons heat the examined sample and based on the obtained diffraction pattern information on the structure of the material is provided. Research for developing a novel cold neutron detector for Chromatic Analysis Neutron Diffractometer Or Reflectometer (CANDOR) is underway at the NIST center for neutron research. The system unique design is aimed to provide over ten times fold faster analysis of materials than conventional system. In order to achieve the fast analysis a large number of neutron detectors is required. A key design constraint for this detector is the thickness of the neutron sensitive element. This is met using {sup 6}LiF:ZnS(Ag) scintillation material with embedded wavelength shifting (WLS) fibers conducting scintillation light to silicon photomultiplier photo-sensors. The detector sensitivity is determined by both the neutron capture probability ({sup 6}Li density) and the detectable light output produced by the ZnS(Ag) ionization, the latter of which is hindered by the fluorescence absorption of the scintillation light by the ZnS. Tradeoffs between the neutron capture probability, stimulated light production and light attenuation for determining the optimal stoichiometry of the {sup 6}LiF and ZnS(Ag) as well as the volume ratio of scintillator and fiber. Simulations performed using the GEANT4 Monte Carlo package were made in order to optimize the detector design. GEANT4 enables the investigation of the neutron interaction with the detector, the ionization process and the light transfer process following the nuclear process. The series of conversions required for this detector were modelled: - A cold neutron enters the sensor and is captured by {sup 6}Li in the scintillator mixture ({sup 6}Li (n,α) {sup 3}H

  12. Astrophysical S factor for the radiative-capture reaction p{sup 6}Li {yields} {sup 7}Be{gamma}

    Energy Technology Data Exchange (ETDEWEB)

    Dubovichenko, S. B., E-mail: sergey@dubovichenko.ru [National Space Agency of the Republic of Kazakhstan, Fessenkov Astrophysical Institute, National Center of Space Research and Technology (Kazakhstan); Burtebaev, N., E-mail: burteb@inp.kz; Zazulin, D. M.; Kerimkulov, Zh. K. [National Nuclear Center of Republic of Kazakhstan, Institute of Nuclear Physics (Kazakhstan); Amar, A. S. A. [Al-Farabi Kazakh National University (Kazakhstan)

    2011-07-15

    A new measurement of differential cross sections for elastic p{sup 6}Li scattering in the energy range 0.35-1.2 MeV was performed. A partial-wave analysis of the data obtained in this way was carried out, and potentials simulating the p{sup 6}Li interaction were constructed. Various experiments devoted to studying elastic p{sup 6}Li scattering over the broad energy range of 0.5-50 MeV were analyzed on the basis of the optical model. By using the potentials obtained from the partial-wave analysis, the possibility of describing the astrophysical S factor for radiative proton capture on {sup 6}Li at low energies was considered within the potential cluster model involving forbidden states.

  13. Model Calculation of n + 6Li Reactions Below 20 MeV

    Institute of Scientific and Technical Information of China (English)

    ZHANG Jing-Shang; HAN Yin-Lu

    2001-01-01

    Based on the unified Hauser-Feshbach and exciton model for light nuclei, the calculations of reaction cross sections and the double-differential cross sections for n + 6Li are performed. Since all of the first-particle emissions are from the compound nucleus to the discrete levels, the angular momentum coupling effect in pre-equilibrium mechanism must be taken into account. The fitting of the measured data indicates that the three-body break-up process needs to be involved, and the pre-equilibrium reaction mechanism dominates the reaction processes. In light nucleus reactions the recoil effect must be taken into account.``

  14. Comparative analysis of pulse shape discrimination methods in a {sup 6}Li loaded plastic scintillator

    Energy Technology Data Exchange (ETDEWEB)

    Balmer, Matthew J.I., E-mail: m.balmer@lancaster.ac.uk [Department of Engineering, Lancaster University, LA1 4YR (United Kingdom); Gamage, Kelum A.A. [Department of Engineering, Lancaster University, LA1 4YR (United Kingdom); Taylor, Graeme C. [Neutron Metrology Group, National Physical Laboratory, Teddington, TW11 0LW (United Kingdom)

    2015-07-11

    Three algorithms for discriminating between fast neutrons, thermal neutrons and gamma rays in a {sup 6}Li loaded plastic scintillator have been compared. Following a literature review of existing pulse shape discrimination techniques, the performance of the charge comparison method, triangular filtering and frequency gradient analysis were investigated in this work. The scintillator was exposed to three different mixed gamma/neutron radiation fields. The figure of merit of neutron/gamma separation was investigated over a broad energy range, as well as for the neutron capture energy region. After optimisation, all three methods were found to perform similarly in terms of neutron/gamma separation.

  15. {sup 6}Li breakup and suppression of complete fusion above the Coulomb barrier

    Energy Technology Data Exchange (ETDEWEB)

    Elmahdy, N.A. [Modern Academy for Engineering and Technology, Cairo (Egypt); Denikin, A.S. [Dubna International University, Dubna (Russian Federation); JINR, Flerov Laboratory of Nuclear Reactions, Dubna (Russian Federation); Ismail, M.; Ellithi, A.Y. [Cairo University, Cairo (Egypt)

    2015-05-15

    We study the role of the projectile breakup in the fusion process by example of the {sup 6}Li reactions with the {sup 59}Co, {sup 144}Sm and {sup 209}Bi targets in vicinity of the Coulomb barrier. The coupled channel and distorted wave approaches are employed in order to calculate the complete fusion and the breakup cross sections, respectively. The partial cross sections in both the channels are compared in order to estimate the breakup fraction responsible for the suppression of complete fusion. The calculations are compared with available experimental data. The conclusions and recommendations are made. (orig.)

  16. Characterization of the silicon+6LiF thermal neutron detection technique

    Science.gov (United States)

    Pappalardo, A.; Barbagallo, M.; Cosentino, L.; Marchetta, C.; Musumarra, A.; Scirè, C.; Scirè, S.; Vecchio, G.; Finocchiaro, P.

    2016-02-01

    The worldwide need to replace 3He for neutron detection has triggered research and development on new technologies and methods. A promising one is based on commercial solid state silicon detectors coupled with thin neutron converter layers containing 6Li. After proving the feasibility of this technique, we characterized the behavior of such a detector with different converter layer thicknesses. In this paper we also disentangle other contributions to the overall spectrum shape observed with this kind of detector, proving that its detection efficiency can be made reasonably high and that the gamma/neutron discrimination capability is comparable to that of 3He tubes.

  17. Characterization of the silicon+6LiF thermal neutron detection technique

    CERN Document Server

    Pappalardo, A; Cosentino, L; Marchetta, C; Musumarra, A; Scirè, C; Scirè, S; Vecchio, G; Finocchiaro, P

    2015-01-01

    The worldwide need to replace 3He for the neutron detection has triggered R&D on new technologies and methods. A promising one is based on commercial solid state silicon detectors coupled with thin neutron converter layers containing 6Li. After proving the feasibility of this technique, we characterized the behavior of such a detector with different converter layer thicknesses. In this paper we also disentangle other contributions to the overall spectrum shape observed with this kind of detector, proving that its detection efficiency can be made reasonably high and that the gamma/neutron discrimination capability is comparable to the one of 3He tubes.

  18. Characterization of the silicon+{sup 6}LiF thermal neutron detection technique

    Energy Technology Data Exchange (ETDEWEB)

    Pappalardo, A. [INFN Laboratori Nazionali del Sud, Catania (Italy); Barbagallo, M. [INFN Sezione di Bari (Italy); Cosentino, L.; Marchetta, C. [INFN Laboratori Nazionali del Sud, Catania (Italy); Musumarra, A. [INFN Laboratori Nazionali del Sud, Catania (Italy); Università di Catania (Italy); Scirè, C.; Scirè, S.; Vecchio, G.; Finocchiaro, P. [INFN Laboratori Nazionali del Sud, Catania (Italy)

    2016-02-21

    The worldwide need to replace {sup 3}He for neutron detection has triggered research and development on new technologies and methods. A promising one is based on commercial solid state silicon detectors coupled with thin neutron converter layers containing {sup 6}Li. After proving the feasibility of this technique, we characterized the behavior of such a detector with different converter layer thicknesses. In this paper we also disentangle other contributions to the overall spectrum shape observed with this kind of detector, proving that its detection efficiency can be made reasonably high and that the gamma/neutron discrimination capability is comparable to that of {sup 3}He tubes.

  19. Pulse-Shape Analysis of Neutron-Induced Scintillation Light in Ni-doped 6LiF/ZnS

    Energy Technology Data Exchange (ETDEWEB)

    Cowles, Christian C.; Behling, Richard S.; Imel, G. R.; Kouzes, Richard T.; Lintereur, Azaree; Robinson, Sean M.; Stave, Sean C.; Siciliano, Edward R.; Wang, Zheming

    2016-10-06

    Abstract–Alternatives to 3He are being investigated for gamma-ray insensitive neutron detection applications, including plutonium assay. One promising material is lithium-6 fluoride with silver activated zinc sulfide 6LiF/ZnS(Ag) in conjunction with a wavelength shifting plastic. Doping the 6LiF/ZnS(Ag) with nickel (Ni) has been proposed as a means of reducing the decay time of neutron signal pulses. This research performed a pulse shape comparison between Ni-doped and non-doped 6LiF/ZnS(Ag) neutron pulses. The Ni-doped 6LiF/ZnS(Ag) had a 32.7% ± 0.3 increase in neutron pulse height and a 32.4% ± 0.3 decrease in neutron pulse time compared to the non-doped 6LiF/ZnS(Ag). Doping 6LiF/ZnS(Ag) with nickel may allow neutron detector operation with improved signal to noise ratios, and reduced pulse pileup affects, increasing the accuracy and range of source activities with which such a detector could operate.

  20. Role of the cluster structure of {sup 7}Li in the dynamics of fragment capture

    Energy Technology Data Exchange (ETDEWEB)

    Shrivastava, A., E-mail: aradhana@barc.gov.in [Nuclear Physics Division, Bhabha Atomic Research Centre, Mumbai 400085 (India); Navin, A. [GANIL, CEA/DSM - CNRS/IN2P3, Bd Henri Becquerel, BP 55027, F-14076 Caen Cedex 5 (France); Diaz-Torres, A. [ECT, Villa Tambosi, I-38123 Villazzano, Trento (Italy); Nanal, V. [DNAP, Tata Institute of Fundamental Research, Mumbai 400005 (India); Ramachandran, K. [Nuclear Physics Division, Bhabha Atomic Research Centre, Mumbai 400085 (India); Rejmund, M. [GANIL, CEA/DSM - CNRS/IN2P3, Bd Henri Becquerel, BP 55027, F-14076 Caen Cedex 5 (France); Bhattacharyya, S. [Variable Energy Cyclotron Centre, 1/AF Bidhan Nagar, Kolkata 700064 (India); Chatterjee, A.; Kailas, S. [Nuclear Physics Division, Bhabha Atomic Research Centre, Mumbai 400085 (India); Lemasson, A. [GANIL, CEA/DSM - CNRS/IN2P3, Bd Henri Becquerel, BP 55027, F-14076 Caen Cedex 5 (France); Palit, R. [DNAP, Tata Institute of Fundamental Research, Mumbai 400005 (India); Parkar, V.V. [Nuclear Physics Division, Bhabha Atomic Research Centre, Mumbai 400085 (India); Pillay, R.G. [DNAP, Tata Institute of Fundamental Research, Mumbai 400005 (India); Rout, P.C. [Nuclear Physics Division, Bhabha Atomic Research Centre, Mumbai 400085 (India); Sawant, Y. [DNAP, Tata Institute of Fundamental Research, Mumbai 400005 (India)

    2013-01-08

    Exclusive measurements of prompt {gamma}-rays from the heavy-residues with various light charged particles in the {sup 7}Li + {sup 198}Pt system, at an energy near the Coulomb barrier (E/V{sub b}{approx}1.6) are reported. Recent dynamic classical trajectory calculations, constrained by the measured fusion, {alpha}- and t-capture cross-sections have been used to explain the excitation energy dependence of the residue cross-sections. These calculations distinctly illustrate a two-step process, breakup followed by fusion, in case of the capture of t and {alpha} clusters; whereas for {sup 6}He+p and {sup 5}He+d configurations, massive transfer is inferred to be the dominant mechanism. The present work clearly demonstrates the role played by the cluster structures of {sup 7}Li in understanding the reaction dynamics at energies around the Coulomb barrier.

  1. Role of the cluster structure of $^7$Li in the dynamics of fragment capture

    CERN Document Server

    Shrivastava, A; Diaz-Torres, A; Nanal, V; Ramachandran, K; Rejmund, M; Bhattacharyya, S; Chatterjee, A; Kailas, S; Lemasson, A; Palit, R; Parkar, V V; Pillay, R G; Rout, P C; Sawant, Y

    2012-01-01

    Exclusive measurements of prompt $\\gamma$-rays from the heavy-residues with various light charged particles in the $^7$Li + $^{198}$Pt system, at an energy near the Coulomb barrier (E/$V_b$ $\\sim$ 1.6) are reported. Recent dynamic classical trajectory calculations, constrained by the measured fusion, $\\alpha$ and $t$ capture cross-sections have been used to explain the excitation energy dependence of the residue cross-sections. These calculations distinctly illustrate a two step process, breakup followed by fusion in case of the capture of $t$ and $\\alpha$ clusters; whereas for $^{6}$He + $p$ and $^{5}$He + $d$ configurations, massive transfer is inferred to be the dominant mechanism. The present work clearly demonstrates the role played by the cluster structures of $^7$Li in understanding the reaction dynamics at energies around the Coulomb barrier.

  2. Probing transfer to unbound states of the ejectile with weakly bound 7Li on 93Nb

    CERN Document Server

    Pandit, S K; Mahata, K; Keeley, N; Parkar, V V; Rout, P C; Martel, I; Palshetkar, C S; Kumar, A; Ramachandran, K; Patale, P; Chatterjee, A; Kailas, S

    2016-01-01

    The two-step process of transfer followed by breakup is explored by measuring a rather complete set of exclusive data for reaction channels populating states in the ejectile continua of the $^7$Li+$^{93}$Nb system at energies close to the Coulomb barrier. The cross sections for $\\alpha+\\alpha$ events from one proton pickup were found to be smaller than those for $\\alpha+d$ events from one neutron stripping and $\\alpha+t$ events from direct breakup of $^7$Li. Coupled channels Born approximation and continuum discretized coupled channels calculations describe the data well and support the conclusion that the $\\alpha+d$ and $\\alpha+\\alpha$ events are produced by direct transfer to unbound states of the ejectile.

  3. Scintillation properties of semiconducting {sup 6}LiInSe{sub 2} crystals to ionizing radiation

    Energy Technology Data Exchange (ETDEWEB)

    Wiggins, Brenden [Y-12 National Security Complex, Oak Ridge, TN (United States); Vanderbilt University, Nashville, TN (United States); Groza, Michael; Tupitsyn, Eugene [Fisk University, Nashville, TN (United States); Lukosi, Eric [University of Tennessee, Knoxville, TN (United States); Stassun, Keivan; Burger, Arnold [Vanderbilt University, Nashville, TN (United States); Fisk University, Nashville, TN (United States); Stowe, Ashley [Y-12 National Security Complex, Oak Ridge, TN (United States); Vanderbilt University, Nashville, TN (United States); University of Tennessee, Knoxville, TN (United States)

    2015-11-21

    {sup 6}LiInSe{sub 2} has gained attention recently as a semiconducting thermal neutron detector. As presented herein, the chalcogenide compound semiconductor also detects incident neutrons via scintillation, making {sup 6}LiInSe{sub 2} the only lithium containing semiconductor to respond to neutrons via both detection mechanisms. Both yellow and red crystals, which appear in the literature, were investigated. Only the yellow crystal responded favorably to ionizing radiation, similar to the semiconducting operation utilizing electrodes. The obtained light yield for yellow crystals is 4400 photons/MeV, referenced to Bi{sub 4}Ge{sub 3}O{sub 12} (BGO).The estimated thermal neutron light yield was 21,000 photons/thermal neutron. The two measured decay time components were found to be 31±1 ns (49%) and 143±9 ns (51%).This crystal provides efficient, robust detection of neutrons via scintillation with respectable light yield and rapid response, enabling its use for a broad array of neutron detection applications.

  4. On the nuclear $(n;t)-$reaction in the three-electron ${}^{6}$Li atom

    CERN Document Server

    Frolov, Alexei M

    2012-01-01

    The nuclear $(n;t)-$reaction of the three-electron ${}^{6}$Li atom with thermal/slow neutrons is considered. An effective method has been developed for determining the probabilities of formation of various atoms and ions in different bound states. We discuss a number of fundamental questions directly related to numerical computations of the final state atomic probabilities. A few appropriate variational expansions for atomic wave functions of the incident lithium atom and final helium atom and/or tritium negatively charged ion are discussed. It appears that the final ${}^4$He atom arising during the nuclear $(n,{}^{6}$Li; ${}^4$He$,t)$-reaction in the three-electron Li atom can also be created in its triplet states. The formation of the quasi-stable three-electron $e^{-}_3$ during the nuclear $(n; t)-$reaction at the Li atom is briefly discussed. Bremsstrahlung emitted by atomic electrons accelerated by the rapidly moving fragments from this reaction is analyzed. The frequency spectrum of the emitted radiatio...

  5. New measurement of the 10B(n,α)7 Li through the Trojan Horse Method

    Science.gov (United States)

    Spartá, Roberta

    2016-04-01

    B(n,α) Li reaction cross section has been measured using the Trojan Horse method, with the specific aim to separate the α1 contribution (coming from the first Li excited level) by the αo (related to the Li ground state), using a very thin target. Preliminary results are shown of the three-body B(d,α7 Li)H cross section.

  6. In-beam PET measurement of $^{7}Li^{3+}$ irradiation induced $\\beta^+}$-activity

    CERN Document Server

    Priegnitz, M; Parodi, K; Sommerer, F; Fiedler, F; Enghardt, W

    2008-01-01

    At present positron emission tomography (PET) is the only feasible method of an in situ and non-invasive monitoring of patient irradiation with ions. At the experimental carbon ion treatment facility of the Gesellschaft für Schwerionenforschung (GSI) Darmstadt an in-beam PET scanner has been integrated into the treatment site and lead to a considerable quality improvement of the therapy. Since ions other than carbon are expected to come into operation in future patient treatment facilities, it is highly desirable to extend in-beam PET also to other therapeutic relevant ions, e.g. 7Li. Therefore, by means of the in-beam PET scanner at GSI the β+-activity induced by 7Li3+ ions has been investigated for the first time. Targets of PMMA, water, graphite and polyethylene were irradiated with monoenergetic, pencil-like beams of 7Li3+ with energies between 129.1 A MeV and 205.3 A MeV and intensities ranging from 3.0 × 107 to 1.9 × 108 ions s−1. This paper presents the measured β+-activity profiles as well as d...

  7. MeV Neutron Production from Thermal Neutron Capture in 6Li Simulated With Geant4

    Science.gov (United States)

    Santoro, Valentina; DiJulio, Douglas D.; Bentley, Phillip M.

    2016-09-01

    Various Li compounds are commonly used at neutron facilities as neutron absorbers. These compounds provide one of the highest ratios of neutron attenuation to y- ray production. Unfortunately, the usage of these compounds can also give rise to fast neutron emission with energies up to almost 16 MeV. Historically, some details in this fast neutron production mechanism can be absent from some modeling packages under some optimization scenarios. In this work, we tested Geant4 to assess the performance of this simulation toolkit for the fast neutron generation mechanism. We compare the results of simulations performed with Geant4 to available measurements. The outcome of our study shows that results of the Geant4 simulations are in good agreement with the available measurements for 6 Li fast neutron production, and suitable for neutron instrument background evaluation at spallation neutron sources.

  8. Time-of-flight calibration of a 6Li glass epithermal neutron detector

    Science.gov (United States)

    Livingston; Saleh; Block; Brand

    2000-10-01

    The curing of Portland cement concrete involves the conversion of water from a free to a bound state. The process can be monitored nondestructively by measuring the shift in the neutron energy spectrum in the epithermal range (0.025-1 eV). A tuned array of 6Li glass detectors has been constructed with varying efficiencies over the epithermal energy range. To determine the efficiency of each detector as a function of neutron energy, it is necessary to calibrate it against a reference neutron spectrum. This was accomplished using a time-of-flight approach with a pulsed neutron beam produced at the Gaerttner LINAC Laboratory at Rensselaer Polytechnic Institute. With a neutron flight path of 25 m it was possible to determine the neutron detector efficiencies to an energy resolution of 11 microeV. The data showed good agreement with the detector design calculations.

  9. Observation of repulsive Fermi polarons in a resonant mixture of ultracold ${}^6$Li atoms

    CERN Document Server

    Scazza, F; Massignan, P; Recati, A; Amico, A; Burchianti, A; Fort, C; Inguscio, M; Zaccanti, M; Roati, G

    2016-01-01

    We employ radio-frequency spectroscopy to investigate a polarized spin-mixture of ultracold ${}^6$Li atoms close to a broad Feshbach scattering resonance. Focusing on the regime of strong repulsive interactions, we observe well-defined coherent quasiparticles even for unitarity-limited interactions. We characterize the many-body system by extracting the key properties of repulsive Fermi polarons: the energy $E_+$, the effective mass $m^*$, the residue $Z$ and the decay rate $\\Gamma$. Above a critical interaction, $E_+$ is found to exceed the Fermi energy of the bath while $m^*$ diverges and even turns negative. Such findings reveal that the paramagnetic Fermi liquid state becomes thermodynamically unstable towards an energetically favored ferromagnetic phase.

  10. MeV Neutron Production from Thermal Neutron Capture in {6}^Li Simulated with Geant4

    CERN Document Server

    Santoro, Valentina; Bentley, Phillip M

    2015-01-01

    Various Li compounds are commonly used at neutron facilities as neutron absorbers. These compounds provide one of the highest ratios of neutron attenuation to $\\gamma$-ray production. Unfortunately, the usage of these compounds can also give rise to fast neutron emission with energies up to almost 16 MeV. Historically, some details in this fast neutron production mechanism can be absent from some modeling packages under some optimization scenarios. In this work, we tested Geant4 to assess the performance of this simulation toolkit for the fast neutron generation mechanism. We compare the results of simulations performed with Geant4 to available measurements. The outcome of our study shows that results of the Geant4 simulations are in good agreement with the available measurements for $^6$Li fast neutron production, and suitable for neutron instrument background evaluation at spallation neutron sources.

  11. Fusion excitation function measurement for 6Li+64Ni at near-barrier energies

    Directory of Open Access Journals (Sweden)

    Shaikh Md. Moin

    2015-01-01

    Full Text Available Total fusion excitation function has been measured for the reaction of weakly bound 6Li projectile on medium mass 64Ni target at energies near the Coulomb barrier of the system. Online characteristic γ-ray detection method has been used to identify and determine the cross sections of the residues. No suppression of total fusion cross section (σTF is observed at above barrier energies. But enhancement of measured cross section with respect to the one-dimensional barrier penetration model (1-DBPM calculation is observed at below barrier energies. The enhancement can not be explained by coupled channels calculation with dominant projectile and target excitations as well as one-neutron stripping reaction.

  12. Thermal neutron detection by entrapping 6LiF nanocrystals in siloxane scintillators

    Science.gov (United States)

    Carturan, S. M.; Marchi, T.; Maggioni, G.; Gramegna, F.; Degerlier, M.; Cinausero, M.; Dalla Palma, M.; Quaranta, A.

    2015-06-01

    Exploiting the long experience in design and production of scintillating mixtures based on siloxane matrices with combinations of primary dye and waveshifter, a first set of 6LiF loaded scintillator disks has been produced. The synthesis is herein described and reported, as well as preliminary results on their light response towards thermal neutrons. The preservation of transparency and mechanical integrity of the scintillator material is challenging when introducing the inorganic salt LiF which is a "foreign body" to the organic polysiloxane host matrix Different strategies such as synthesis of nanoparticles and surface functionalization have been pursued to succeed in the entrapment of the neutron converter whilst maintaining moderate light output, optical transparency and flexibility of the base scintillator.

  13. Reaction mechanisms in the {sup 6}Li + {sup 59}Co system

    Energy Technology Data Exchange (ETDEWEB)

    Souza, F.A. [Instituto de Fisica - Universidade de Sao Paulo, Departamento de Fisica Nuclear, C.P. 66318, 05315-970 Sao Paulo, SP (Brazil)], E-mail: fsouza@dfn.if.usp.br; Beck, C. [Institut Pluridisciplinaire Hubert Curien, UMR 7178, CNRS-IN2P3 et Universite Louis Pasteur, Boite Postale 28, F-67037 Strasbourg, Cedex 2 (France); Carlin, N. [Instituto de Fisica - Universidade de Sao Paulo, Departamento de Fisica Nuclear, C.P. 66318, 05315-970 Sao Paulo, SP (Brazil); Keeley, N. [CEA-Saclay DSM/IRFU/SPhN, F-91191 Gif sur Yvette Cedex (France); Neto, R. Liguori; Moura, M.M. de; Munhoz, M.G.; Del Santo, M.G.; Suaide, A.A.P.; Szanto, E.M.; Szanto de Toledo, A. [Instituto de Fisica - Universidade de Sao Paulo, Departamento de Fisica Nuclear, C.P. 66318, 05315-970 Sao Paulo, SP (Brazil)

    2009-04-15

    The reactions induced by the weakly bound {sup 6}Li projectile interacting with the intermediate mass target {sup 59}Co were investigated. Light charged particles singles and {alpha}-d coincidence measurements were performed at the near barrier energies E{sub lab}=17.4, 21.5, 25.5 and 29.6 MeV. The main contributions of the different competing mechanisms are discussed. A statistical model analysis, Continuum-Discretized Coupled-Channels (CDCC) calculations and two-body kinematics were used as tools to provide information to disentangle the main components of these mechanisms. A significant contribution of the direct breakup was observed through the difference between the experimental sequential breakup cross section and the CDCC prediction for the non-capture breakup cross section.

  14. Alpha cluster states in light nuclei populated through the (6Li,d) reaction

    Energy Technology Data Exchange (ETDEWEB)

    Borello-Lewin, Thereza; Rodrigues, M.R.D.; Horodynski-Matsushigue, L.B.; Duarte, J.L.M.; Rodrigues, C.L.; Souza, M.A. [Universidade de Sao Paulo (IF/USP), SP (Brazil). Inst. de Fisica; Cunsolo, A.; Cappuzzello, F. [Universita di Catania (Italy). Istituto Nazionale di Fisica Nucleare. Lab. Nazionali del Sud; Ukita, Gilberto Mitsuo [Universidade de Santo Amaro (UNISA), Sao Paulo, SP (Brazil). Fac. de Psicologia

    2011-07-01

    Full text: The alpha cluster correlation is an important concept in the nuclear physics of light nuclei. The main purpose of the research program in progress is the investigation of the alpha clustering phenomenon in (x{alpha}) and(x{alpha}+{nu}) nuclei through the ({sup 6}Li,d) alpha transfer reaction. In fact, there is scarce experimental information on the subject, in particular associated with resonant states predicted near (x{alpha}) and (x{alpha}+{nu}) thresholds. Measurements of the {sup 12},{sup 13}C({sup 6}Li,d) {sup 16},{sup 17}O reactions, at an incident energy of 25.5 MeV, have been performed employing the Sao Paulo Pelletron-Enge Split-Pole facility and the nuclear emulsion detection technique. The work is under way and an experimental energy resolution of 30 keV was obtained. Near the (4{alpha}) breakup threshold in {sup 16}O, three narrow alpha resonances, not previously measured, were detected, revealing important {alpha} + {sup 12}C(G.S.) components. One of these resonances corresponds to the known 0{sup +} state at 15.1 MeV[5] of excitation that has probably, according to Funaki et al., the gas like configuration of the 4{alpha} condensate state, with a very dilute density and a large component of {alpha} + {sup 12}C(Hoyle) configuration. As was already mentioned, our experimental information points to the necessity of including the {alpha} + {sup 12}C(G.S.) component in the wave function. (author)

  15. Photoassociation spectroscopy of long-range molecular states below the 2s + 3p 6Li2 asymptote

    Science.gov (United States)

    Gross, Christian; Chaudhuri, Saptarishi; Gan, Jaren; Dieckmann, Kai

    2015-05-01

    We present photoassociation spectra of high-lying vibrational states of the interatomic potentials correlating to the 2s + 3p asymptote of 6Li2 . Starting from an atomic cloud in a magneto-optical trap we first drive a free-to-bound transition into a molecular bound state using a tunable ultra-violet laser. Thereafter we ionize these long-range molecules using a 532 nm laser and detect the resulting ions with a channeltron. We determine the absolute positions of the transitions with MHz precision utilizing a frequency comb based calibration. Lithium dimers are extensively studied theoretically using various models and methods. Spectroscopic measurements are crucial to test and benchmark these methods and are available for various electronic states and inter-nuclear distances of 6Li2 molecule. Our study provides the first experimental observation of long-range states of the 2s + 3p asymptote of 6Li2 .

  16. The Astrophysical S-factor for the 2H(, )6Li Nuclear Reaction at Low-Energies

    Indian Academy of Sciences (India)

    H. Sadeghi; A. Moghadasi; M. Ghamary

    2014-12-01

    The alpha radiative capture reactions are the key to understand about primordial nucleosynthesis and the observed abundance of light nucleus in stars. The astrophysical S-factor for the process 2H(, )6Li has been calculated at the low-energies relevant to big-bang nucleosynthesis and in comparison with laboratory data. On the basis of the model, the alpha radiative capture process is studied by using the two-and three-body electromagnetic currents. The bound and resonance states of 6Li are calculated via an inverse process, deuteron- photodisintegration of a 6Li nucleus. In comparison with other theoretical approaches and available laboratory data, excellent agreement is achieved for the astrophysical S-factor of this process.

  17. Angular Distribution of the 12C(6He, 7Li)11B Reaction

    Institute of Scientific and Technical Information of China (English)

    LI Er-Tao; LI Zhi-Hong; LI Yun-Ju; YAN Sheng-Quan; BAI Xi-Xiang; GUO Bing; SU Jun; WANG You-Bao; WANG Bao-Xiang; LIAN Gang; ZENG Sheng; FANG Xiao; ZHAO Wei-Juan; LIU Wei-Ping

    2009-01-01

    Angular distribution of the 12C(6He, 7Li)11B transfer reaction is measured with a secondary 6He beam of 36.4 Me V for the first time. The experimental angular distribution is well reproduced by the distorted-wave Born approxima-tion (DWBA) calculation. The success of the present experiment shows that it is feasible to measure one-nucleon transfer reaction on a light nucleus target with the secondary beam facility of the HI-13 tandem accelerator at China Institute of Atomic Energy (CIAE), Beifing.

  18. Corrosion barriers processed by Al electroplating and their resistance against flowing Pb–15.7Li

    Energy Technology Data Exchange (ETDEWEB)

    Krauss, Wolfgang, E-mail: wolfgang.krauss@kit.edu; Konys, Jürgen; Wulf, Sven-Erik

    2014-12-15

    In the HCLL blanket design, ferritic–martensitic steels are in direct contact with the flowing liquid breeder Pb–15.7Li and have to withstand severe corrosion attack. Beyond corrosion, T-permeation from the breeder into the RAFM-steels is also an important issue and has to be reduced significantly. Earlier work showed that Al-based coatings can act as barriers for both, however, applied processes e.g. HDA or VPS exhibited strong drawbacks in the past. Meanwhile new industrial relevant coating processes, using electroplating technology are under development and called ECA (electrochemical aluminization) and ECX (electrochemical deposition from ionic liquids) process. In this study electrochemically Al-coated and heat-treated Eurofer samples were tested in PICOLO loop for exposure times up to 12,000 h (ECA) and 2000 h (first results ECX) respectively to determine corrosion properties in flowing Pb–15.7Li (550 °C, 0.1 m/s). Cross section analysis afterward corrosion testing proved the ability of thin Al-based barriers made by electrochemical techniques to protect the bare Eurofer from corrosion attack even at exposure times of 12,000 h. Determined radial corrosion rates lay between 10 and 20 μm/a. First results for ECX coated samples (2000 h) revealed more homogeneous corrosion behavior of the barrier layer itself compared to ECA.

  19. 6LiF Semiconductor Sandwich Spectrometer for Fast Neutron Spectrum Measurement%用于快中子能谱测量的6LiF夹心半导体谱仪

    Institute of Scientific and Technical Information of China (English)

    蒋勇; 李俊杰; 张涛; 范晓强; 郑春

    2012-01-01

    A detector of 6LiF semiconductor sandwich spectrometer was designed and manufactured. Characteristics of the spectrometer were tested in the fast neutron critical assembly. Measurement principle, configuration of detector and electronic circuit were introduced. Fast neutron spectrum was measured using the 6LiF semiconductor sandwich spectrometer. When the detector's 6 LiF mass thickness is 186 μg/cm2, the spectrometer's energy resolution is 363 keV in the thermal neutron field. For this spectrometer, the optimal fathomable neutron energy range is 0. 3-7. 5 MeV, and the background counts only take possession of 1 % in this area.%本文介绍了6 LiF夹心谱仪的测量原理、自行设计研制的6LiF夹心半导体谱仪探头结构及电子学系统组成等.在热中子场中测试了夹心谱仪的性能,获得了α粒子峰、T粒子峰及“和”峰在多道上的位置与能量分辨率,并用T粒子与“和”峰两个能量点的峰位对谱仪系统进行了能量刻度.分别用效应探头和本底探头测量了临界装置表面的效应谱和本底谱,当效应探头采用的6 LiF镀层质量厚度为186 μg/cm2时,6 LiF夹心谱仪对热中子的能量分辨率为363 keY,测量中子最佳能区为0.3~7.5 MeV,在该能区内,本底谱约占1%.

  20. A study of the proton spectra following the capture of $K^-$ in $^6$Li and $^{12}$C with FINUDA

    CERN Document Server

    Agnello, M; Benussi, L; Bertani, M; Bhang, H C; Bianco, S; Bonomi, G; Botta, E; Bregant, M; Bressani, Tullio; Bufalino, S; Busso, L; Calvo, D; Camerini, P; Cerello, P; Dalena, B; Mori, F D; D'Erasmo, G; Santo, D D; Elia, D; Fabbri, F L; Faso, D; Feliciello, A; Filippi, A; Filippini, V; Fini, R A; Fiore, E M; Fujioka, H; Gianotti, P; Grion, N; Hartmann, O; Krasnoperov, A V; Lenti, V; Lucherini, V; Manzari, V; Marcello, S; Maruta, T; Mirfakhraee, N; Morra, O; Nagae, T; Olin, A; Outa, H; Pace, E; Pallotta, M; Palomba, M; Pantaleo, A; Panzarasa, A; Paticchio, V; Piano, S; Pompili, F; Rui, R; Simonetti, G; Tereshchenko, V V; Tomassini, S; Toyoda, A; Wheadon, R; Zenoni, A

    2006-01-01

    Momenta spectra of protons emitted following the capture of $K^-$ in $^6$Li and $^{12}$C have been measured with 1% resolution. The $^{12}$C spectrum is smooth whereas for $^6$Li a well defined peak appears at about 500 MeV/$c$. The first observation of a structure in this region was identified as a strange tribaryon or, possibly, a $\\bar K$-nuclear state. The peak is correlated with a $\\pi^-$ coming from $\\Sigma^-$ decay in flight, selected by setting momenta larger than 275 MeV/$c$. The $\\Sigma^-$ could be produced, together with a 500 MeV/$c$ proton, by the capture of a $K^-$ in a deuteron-cluster substructure of the $^6$Li nucleus. The capture rate for such a reaction is $(1.62\\pm 0.23_{stat} ^{+0.71}_{-0.44}(sys))%/K^-_{stop}$, in agreement with the existing observations on $^4$He targets and with the hypothesis that the $^6$Li nucleus can be interpreted as a $(d+\\alpha)$ cluster.

  1. Development of a 6LiF/ZnS-based Neutron Multiplicity Counter

    Energy Technology Data Exchange (ETDEWEB)

    Stave, Sean C.; Behling, Richard S.; Bernacki, Bruce E.; Bliss, Mary; Cowles, Christian C.; Kouzes, Richard T.; Lintereur, Azaree; Robinson, Sean M.; Siciliano, Edward R.

    2016-10-06

    Abstract–Neutron multiplicity counters are used in safeguards to provide rapid assay of samples which contain an unknown amount of plutonium in a potentially unknown configuration. A project at PNNL is using regular and nickel-quenched 6LiF/ZnS neutron-scintillator sheets and wavelength shifting plastic for light pipes in place of 3He. A combination of laboratory and modeling work predicts a LiF/ZnS-based system to be able to match or exceed the performance of the best 3He-based systems available. Also, the Ni-quenched material is expected to allow for improved neutron/gamma-ray discrimination at twice the event rate relative to the non-Ni-quenched LiF/ZnS. A new system based on the LiF/ZnS material is under construction and components are being used to optimize the detection efficiency and neutron/gamma-ray discrimination properties. Components of the new system are partially constructed and undergoing performance testing utilizing high-speed digitizers with field programmable gate arrays to perform the neutron/gamma-ray discrimination. The expected performance of the full-scale system is expected to be nearly the same as for 3He-based systems and is due for completion in 2016.

  2. Dynamics of fragment capture for cluster structures of weakly bound 7Li

    Directory of Open Access Journals (Sweden)

    Shrivastava A.

    2013-12-01

    Full Text Available Role of cluster structures of 7Li on reaction dynamics have been studied by performing exclusive measurements of prompt-γ rays from residues with scattered particles at energy, E/Vb = 1.6, with 198Pt target. Yields of the residues resulting after capture of t and 4,5,6He, corresponding to different excitation energies of the composite system were estimated. The results were compared with three body classical-dynamical model for breakup fusion, constrained by the measured fusion, α and t capture cross-sections. The cross-section of residues from capture of α and t agreed well with the prediction of the model showing dominance of the two step process - breakup fusion, while those from tightly bound 6He showed massive transfer to be the dominant mechanism.

  3. Towards {sup 6}Li-{sup 40}K ground state molecules

    Energy Technology Data Exchange (ETDEWEB)

    Brachmann, Johannes Felix Simon

    2013-02-08

    The production of a quantum gas with strong long - range dipolar interactions is a major scientific goal in the research field of ultracold gases. In their ro - vibrational ground state Li-K dimers possess a large permanent dipole moment, which could possibly be exploited for the realization of such a quantum gas. A production of these molecules can be achieved by the association of Li and K at a Feshbach resonance, followed by a coherent state transfer. In this thesis, detailed theoretical an experimental preparations to achieve state transfer by means of Stimulated Raman Adiabatic Passage (STIRAP) are described. The theoretical preparations focus on the selection of an electronically excited molecular state that is suitable for STIRAP transfer. In this context, molecular transition dipole moments for both transitions involved in STIRAP transfer are predicted for the first time. This is achieved by the calculation of Franck-Condon factors and a determination of the state in which the {sup 6}Li-{sup 40}K Feshbach molecules are produced. The calculations show that state transfer by use of a single STIRAP sequence is experimentally very well feasible. Further, the optical wavelengths that are needed to address the selected states are calculated. The high accuracy of the data will allow to carry out the molecular spectroscopy in a fast and efficient manner. Further, only a comparatively narrow wavelength tuneability of the spectroscopy lasers is needed. The most suitable Feshbach resonance for the production of {sup 6}Li-{sup 40}K molecules at experimentally manageable magnetic field strengths is occurring at 155 G. Experimentally, this resonance is investigated by means of cross-dimensional relaxation. The application of the technique at various magnetic field strengths in the vicinity of the 155 G Feshbach resonance allows a determination of the resonance position and width with so far unreached precision. This reveals the production of molecules on the atomic side

  4. Low-energy photodisintegration of {sup 9}Be and {alpha}+{alpha}+n<->{sup 9}Be+{gamma} reactions at astrophysical conditions

    Energy Technology Data Exchange (ETDEWEB)

    Efros, V.D. [Rossijskij Nauchnyj Tsentr ``Kurchatovskij Inst.``, Moscow (Russian Federation); Oberhummer, H. [Institut fuer Kernphysik, Wiedner Hauptstrasse 8--10, TU Wien, A--1040, Vienna (Austria); Pushkin, A. [Department of Mathematical Physics, Lund Institute of Technology, P.O. Box, 118 S--221 00 Lund (Sweden); Thompson, I.J. [Department of Physics, University of Surrey, Guildford GU2 5XH (United Kingdom)

    1998-04-01

    A semi-microscopic model for the low-energy photodisintegration of the {sup 9}Be nucleus is constructed, and the experimental data are analyzed with its help. The older radioactive isotope data are supported by this analysis. The theoretical photodisintegration cross section is derived. The astrophysical rates for the reaction {alpha}+{alpha}+n{yields}{sup 9}Be +{gamma} and the reverse photodisintegration of {sup 9}Be are calculated. The new reaction rate for {alpha}+{alpha}+n{yields}{sup 9}Be +{gamma} is compared with previous estimations. (orig.) With 3 figs., 1 tab., 30 refs.

  5. Integration of a $^6$LiInSe$_2$ Thermal Neutron Detector into a CubeSat Instrument

    CERN Document Server

    Egner, Joanna C; Burger, Arnold; Stassun, Keivan G; Buliga, Vladimir; Matei, Liviu; Bodnarik, Julia G; Stowe, Ashley C; Prettyman, Thomas H

    2016-01-01

    We present a preliminary design for a novel neutron detection system that is compact, lightweight, and low power consuming, utilizing the CubeSat platform making it suitable for space-based applications. This is made possible using the scintillating crystal lithium indium diselenide ($^6$LiInSe$_2$), the first crystal to include $^6$Li in the crystalline structure, and a silicon avalanche photodiode (Si-APD). The schematics of this instrument are presented as well as the response of the instrument to initial testing under alpha radiation. A principal aim of this work is to demonstrate the feasibility of such a neutron detection system within a CubeSat platform. The entire end-to-end system presented here is 10 cm x 10 cm x 15 cm, weighs 670 grams and requires 5 Volts direct current at 3 Watts.

  6. Astrophysical S-factor for $^6$Li$(p,\\gamma)$$^7$Be in the coupled-channel Gamow shell model

    CERN Document Server

    Dong, G X; Michel, N; Płoszajczak, M

    2015-01-01

    We have applied the Gamow shell model (GSM) in the coupled-channel representation to study the astrophysical $S$-factor for the proton radiative capture reaction of $^6$Li. Reaction channels are built by coupling the proton wave function expanded in different partial waves with the GSM wave functions of the ground state ($1^+$) and the excited states ($3^+_1$, $0^+_1$ and $2^+_1$) of $^6$Li. All relevant $E1$, $M1$, and $E2$ transitions from the initial continuum states in $^7$Be to the final bound states (${3/2}^-_1$ and ${1/2}^-_1$) states are included. It is found that the calculated total astrophysical $S$ factor for this reaction agrees well with the experimental data.

  7. Projectile breakup dynamics for {sup 6}Li+{sup 59}Co: Kinematical analysis of {alpha}-d coincidences

    Energy Technology Data Exchange (ETDEWEB)

    Souza, F.A.; Carlin, N.; Liguori Neto, R.; Siqueira-Mello, C.; Moura, M.M. de; Munhoz, M.G.; Oliveira, R.A.N.; Santo, M.G. del; Suaide, A.A.P.; Szanto, E.M.; Szanto de Toledo, A. [Instituto de Fisica - Universidade de Sao Paulo, Departamento de Fisica Nuclear, Sao Paulo, SP (Brazil); Beck, C. [CNRS-IN2P3 and Universite Louis Pasteur, Institut Pluridisciplinaire Hubert Curien, UMR 7178, Strasbourg (France); Keeley, N. [The Andrzej Soltan Institute for Nuclear Studies, Department of Nuclear Reactions, Warsaw (Poland); Diaz-Torres, A. [University of Surrey, Department of Physics, Faculty of Engineering and Physical Sciences, Guildford (United Kingdom)

    2010-05-15

    A study of the kinematics of the {alpha} -d coincidences in the {sup 6}Li+{sup 59}Co system at a bombarding energy of E{sub lab}=29.6 MeV is presented. With exclusive measurements performed over different angular intervals it is possible to identify the respective contributions of the sequential and direct projectile breakup components. The angular distributions of both breakup components are fairly well described by the Continuum-Discretized Coupled-Channels framework (CDCC). Furthermore, a careful analysis of these processes using a semiclassical approach provides information on both their lifetime and their distance of occurrence with respect to the target. Breakup to the low-lying (near-threshold) continuum is delayed, and happens at large internuclear distances. This suggests that the influence of the projectile breakup on the complete fusion process can be related essentially to the direct breakup to the {sup 6}Li high-lying continuum spectrum. (orig.)

  8. Formation of η{sup '} (958) meson bound states by the {sup 6}Li(γ,d) reaction

    Energy Technology Data Exchange (ETDEWEB)

    Miyatani, M.; Nagahiro, H.; Hirenzaki, S. [Nara Women' s University, Department of Physics, Nara (Japan); Ikeno, N. [Tottori University, Department of Regional Environment, Tottori (Japan)

    2016-07-15

    We have investigated the {sup 6}Li(γ,d) reaction theoretically for the formation of the η{sup '}(958) mesic nucleus close to the recoilless kinematics. We have developed the theoretical formula and reported the quantitative results of the formation spectra for various cases in this article. We have found that the formation cross sections are reduced by the effects of the fragile deuteron form factor. (orig.)

  9. Theoretical study of the α +d →6Li +γ astrophysical capture process in a three-body model

    Science.gov (United States)

    Tursunov, E. M.; Kadyrov, A. S.; Turakulov, S. A.; Bray, I.

    2016-07-01

    The astrophysical capture process α +d →6Li is studied in a three-body model. The initial state is factorized into the deuteron bound state and the (α +d )-scattering state. The final nucleus 6Li (1+) is described as a three-body bound state α +n +p in the hyperspherical Lagrange-mesh method. The contribution of the E 1 -transition operator from the initial isosinglet states to the isotriplet components of the final state is estimated to be negligible. An estimation of the forbidden E 1 transition to the isosinglet components of the final state is comparable with the corresponding results of the two-body model. However, the contribution of the E 2 -transition operator is found to be much smaller than the corresponding estimations of the two-body model. The three-body model perfectly matches the new experimental data of the LUNA Collaboration with the spectroscopic factor of 2.586 estimated from the bound-state wave functions of 6Li and a deuteron.

  10. Unified description of $^6$Li structure and deuterium-$^4$He dynamics with chiral two- and three-nucleon forces

    CERN Document Server

    Hupin, Guillaume; Navrátil, Petr

    2014-01-01

    Prototype for the study of weakly bound projectiles colliding on stable targets, the scattering of deuterium ($d$) on $^4$He ($\\alpha$) is an important milestone in the search for a fundamental understanding of low-energy reactions. At the same time, it is also important for its role in the Big-bang nucleosynthesis of $^6$Li and applications in the characterization of deuterium impurities in materials. We present the first unified {\\em ab initio} study of the $^6$Li ground state and $d$-$^4$He elastic scattering using two- and three-nucleon forces derived within the framework of chiral effective field theory. The six-nucleon bound-state and scattering observables are calculated by means of the no-core shell model with continuum. %and are compared to available experimental data. We analyze the influence of the dynamic polarization of the deuterium and of the chiral three-nucleon force, and examine the role of the continuum degrees of freedom in shaping the low-lying spectrum of $^6$Li. We find that the adopted...

  11. Elastic scattering and fusion cross-sections in 7Li + 27Al reaction

    Indian Academy of Sciences (India)

    D Patel; S Santra; S Mukherjee; B K Nayak; P K Rath; V V Parkar; R K Choudhury

    2013-10-01

    With an aim to understand the effects of breakup and transfer channels on elastic scattering and fusion cross-sections in the 7Li + 27Al reaction, simultaneous measurement of elastic scattering angular distributions and fusion cross-sections have been carried out at various energies (lab = 8.0–16.0 MeV) around the Coulomb barrier. Optical model (OM) analysis of the elastic scattering data does not show any threshold anomaly or breakup threshold anomaly behaviour in the energy dependence of the real and imaginary parts of the OM potential. Fusion cross-section at each bombarding energy is extracted from the measured -particle evaporation energy spectra at backward angles by comparing with the statistical model prediction. Results on fusion cross-sections from the present measurements along with data from the literature have been compared with the coupled-channels predictions. Detailed coupled-channels calculations have been carried out to study the effect of coupling of breakup, inelastic and transfer, channels on elastic scattering and fusion. The effect of 1-stripping transfer coupling was found to be significant compared to that of the projectile breakup couplings in the present system.

  12. {sup 16}O resonances near 4α threshold through {sup 12}C({sup 6}Li,d) reaction

    Energy Technology Data Exchange (ETDEWEB)

    Rodrigues, M. R. D.; Borello-Lewin, T.; Miyake, H.; Horodynski-Matsushigue, L. B.; Duarte, J. L. M.; Rodrigues, C. L.; Faria, P. Neto de [Instituto de Física, Universidade de São Paulo, Caixa Postal 66318, CEP 05314-970, São Paulo, SP (Brazil); Cunsolo, A.; Cappuzzello, F.; Foti, A.; Agodi, C.; Cavallaro, M. [INFN - Laboratori Nazionali del Sud, Via S. Sofia 62, 95125 Catania (Italy); Napoli, M. di; Ukita, G. M. [Faculdade de Psicologia, Universidade de Santo Amaro, R. Prof. Eneas da Siqueira Neto, 340, CEP 04829-300, São Paulo, SP (Brazil)

    2014-11-11

    Several narrow alpha resonant {sup 16}O states were detected through the {sup 12}C({sup 6}Li,d) reaction, in the range of 13.5 to 17.5 MeV of excitation energy. The reaction was measured at a bombarding energy of 25.5 MeV employing the São Paulo Pelletron-Enge-Spectrograph facility and the nuclear emulsion technique. Experimental angular distributions associated with natural parity quasi-bound states around the 4α threshold are presented and compared to DWBA predictions. The upper limit for the resonance widths obtained is near the energy resolution (15 keV)

  13. Study of Two-Step Mechanisms in Pion Absorption on $^{6}Li$, $^{12}C$ via Deuteron Emission

    CERN Document Server

    Huber, G M; Papandreou, Z; Hovdebo, J; Naqvi, S I H; Ottewell, D F; Walden, P L; Jones, G; Aslanoglou, X

    2000-01-01

    The (pi+,pd), and (pi+,dd) reactions were investigated with pions of 100 and 165 MeV kinetic energy on 6Li and 12C targets. In comparison with previously published (pi+,pp) data on the same targets and at the same beam energies, kinematic regions were identified in which the neutron pickup process n+p->d dominated the observed deuteron yield. The importance of this mechanism increases with energy, contributing half of the observed cross section at 165 MeV. The contribution of direct quasi-triton absorption is significant only at 100 MeV.

  14. $^{7}Li(p,n)$ Nuclear Data Library for Incident Proton Energies to 150 MeV

    CERN Document Server

    Mashnik, S G; Hughes, H G; Little, R C; MacFarlane, R E; Waters, L S; Young, P G

    2000-01-01

    We describe evaluation methods that make use of experimental data, and nuclear model calculations, to develop an ENDF-formatted data library for the reaction p + Li7 for incident protons with energies up to 150 MeV. The important 7-Li(p,n_0) and 7-Li(p,n_1) reactions are evaluated from the experimental data, with their angular distributions represented using Lengendre polynomial expansions. The decay of the remaining reaction flux is estimated from GNASH nuclear model calculations. The evaluated ENDF-data are described in detail, and illustrated in numerous figures. We also illustrate the use of these data in a representative application by a radiation transport simulation with the code MCNPX.

  15. AB-BNCT beam shaping assembly based on {sup 7}Li(p,n){sup 7}Be reaction optimization

    Energy Technology Data Exchange (ETDEWEB)

    Minsky, D.M., E-mail: minsky@tandar.cnea.gov.ar [Gerencia de Investigacion y Aplicaciones, CNEA, Av. Gral Paz 1499 (B1650KNA), San Martin, Buenos Aires (Argentina)] [Escuela de Ciencia y Tecnologia, UNSAM, M. de Irigoyen 3100 (1650), San Martin (Argentina)] [CONICET, Av. Rivadavia 1917 (C1033AAJ), Buenos Aires (Argentina); Kreiner, A.J. [Gerencia de Investigacion y Aplicaciones, CNEA, Av. Gral Paz 1499 (B1650KNA), San Martin, Buenos Aires (Argentina)] [Escuela de Ciencia y Tecnologia, UNSAM, M. de Irigoyen 3100 (1650), San Martin (Argentina)] [CONICET, Av. Rivadavia 1917 (C1033AAJ), Buenos Aires (Argentina); Valda, A.A. [Gerencia de Investigacion y Aplicaciones, CNEA, Av. Gral Paz 1499 (B1650KNA), San Martin, Buenos Aires (Argentina)] [Escuela de Ciencia y Tecnologia, UNSAM, M. de Irigoyen 3100 (1650), San Martin (Argentina)

    2011-12-15

    A numerical optimization of a Beam Shaping Assembly (BSA) for Accelerator Based-Boron Neutron Capture Therapy (AB-BNCT) has been performed. The reaction {sup 7}Li(p,n){sup 7}Be has been considered using a proton beam on a lithium fluoride target. Proton energy and the dimensions of a simple BSA geometry have been varied to obtain a set of different configurations. The optimal configuration of this set is shown.

  16. Experimental probe for the production of 97Ru from the 7Li+93Nb reaction: A study of precompound emissions

    Science.gov (United States)

    Kumar, Deepak; Maiti, Moumita; Lahiri, Susanta

    2016-10-01

    Background: Interaction of weakly bound heavy ions with an intermediate or heavy target is not yet understood completely due to the scarcity of experimental data. In order to develop a clear understanding of breakup fusion or preequilibrium emission even in the low energy range, 3-10 MeV/nucleon, more experimental investigations are necessary. Purpose: We aim to study the reaction mechanisms involved in the weakly bound heavy-ion induced reaction 7Li+93Nb at low energies by measuring the production cross sections of the residual radionuclides. Method: Natural niobium (93Nb) foil, backed by an aluminum (Al) catcher, arranged in a stack was bombarded by 7Li ions of 20-45 MeV energy. Activity of the residues produced in each 93Nb target was measured by off line γ -ray spectrometry after the end of bombardment (EOB) and cross sections were calculated. Experimental cross sections were compared with those computed using compound and precompound models. Results: In general, measured excitation functions of all residues produced in the 7Li+93Nb reaction showed good agreement with the model calculations based on the Hauser-Feshbach formalism and the exciton model for compound and precompound processes, respectively. Significant preequilibrium emission of neutrons was observed at the relatively high energy tail of the excitation function of 97Ru. Conclusions: Preequilibrium processes played an important role in the enhancement of the cross section in the x n reaction channel over the compound reaction mechanism at higher energies for the 7Li+93Nb reaction. Additionally, indirect evidence of incomplete or breakup fusion was also perceived.

  17. Preliminary study of the 19F(7Li,7Be)19O reaction at 52 MeV with MAGNEX

    CERN Document Server

    Cavallaro, M; Cappuzzello, F; Carbone, D; Foti, A; Orrigo, S E A; Rodrigues, M R D; Schillaci, M; Borello-Lewin, T; Petrascu, H

    2010-01-01

    The 19F(7Li,7Be)19O charge-exchange reaction at 52 MeV incident energy has been performed at INFN-LNS in Catania using the MAGNEX spectrometer. The use of an algebraic ray-reconstruction technique has allowed to extract the 19O excitation energy spectrum and the experimental angular distributions obtained with a single angular setting of the spectrometer.

  18. Prediction of a weakly bound excited state of Efimov character in a 7LiHe42 system

    Science.gov (United States)

    Wu, Meng-Shan; Han, Hui-Li; Li, Cheng-Bin; Shi, Ting-Yun

    2014-12-01

    We carry out calculations on the van der Waals trimer 7LiHe42 using the mapping method within the frame of hyperspherical coordinates, which allows us to give accurate binding energies and wave functions for both the ground and excited state of the system. When the realistic two-body potentials are adopted, the system presents an excited state which shows Efimov character. We study the range of the interaction strength in which the excited state could exist and find that the state persists within the experiment error band for binding energy of LiHe molecule. We also study the three-body parameter (3BP) of 7LiHe42 system and its relationship with the background scattering length aHeHe. Our calculations demonstrate that the 3BP of 7LiHe42 system is dependent on the value of the scattering length aHeHe, independent of the short-range details of the He-He interaction. The results confirm the prediction of Wang et al. [Phys. Rev. Lett. 109, 243201 (2012), 10.1103/PhysRevLett.109.243201] that the 3BP for a heteronuclear atomic system is universally determined from the van der Waals lengths and the homonuclear scattering length.

  19. Interspecies collision-induced losses in a dual species 7Li-85Rb magneto-optical trap

    Science.gov (United States)

    Dutta, Sourav; Altaf, Adeel; Lorenz, John; Elliott, D. S.; Chen, Yong P.

    2014-05-01

    In this article, we report the measurement of collision-induced loss rate coefficients βLi, Rb and βRb, Li, and also discuss means to significantly suppress such collision-induced losses. We first describe our dual-species magneto-optical trap (MOT) that allows us to simultaneously trap ≥5 × 108 7Li atoms loaded from a Zeeman slower and ≥2 × 108 85Rb atoms loaded from a dispenser. We observe strong interspecies collision-induced losses in the MOTs which dramatically reduce the maximum atom number achievable in the MOTs. We measure the trap loss rate coefficients βLi, Rb and βRb, Li, and, from a study of their dependence on the MOT parameters, determine the cause for the losses observed. Our results provide valuable insights into ultracold collisions between 7Li and 85Rb, guide our efforts to suppress collision-induced losses, and also pave the way for the production of ultracold 7Li85Rb molecules.

  20. Interspecies collision-induced losses in a dual species 7Li-85Rb magneto-optical trap

    CERN Document Server

    Dutta, Sourav; Lorenz, John; Elliott, D S; Chen, Yong P

    2013-01-01

    In this article, we report the measurement of collision-induced loss coefficients \\beta_{Li,Rb} and \\beta_{Rb,Li}, and also discuss means to significantly suppress such collision induced losses. We first describe our dual-species magneto-optical trap (MOT) that allows us to simultaneously trap > 5x10^8 7Li atoms loaded from a Zeeman slower and > 2x10^8 85Rb atoms loaded from a dispenser. We observe strong interspecies collision-induced losses in the MOTs which dramatically reduce the maximum atom number achievable in the MOTs. We measure the trap loss rate coefficients \\beta_{Li,Rb} and \\beta_{Rb,Li}, and, from a study of their dependence on the MOT parameters, determine the cause for the losses observed. Our results provide valuable insights into ultracold collisions between 7Li and 85Rb, guide our efforts to suppress collision induced losses, and also pave the way for the production of ultracold 7Li85Rb molecules.

  1. Theoretical study of the $\\alpha+d$ $\\rightarrow$ $^6$Li + $\\gamma $ astrophysical capture process in a three-body model

    CERN Document Server

    Tursunov, E M; Turakulov, S A; Bray, I

    2016-01-01

    The astrophysical capture process $\\alpha+d$ $\\rightarrow$ $^6$Li + $\\gamma$ is studied in a three-body model. The initial state is factorized into the deuteron bound state and the $\\alpha+d$ scattering state. The final nucleus $^6$Li(1+) is described as a three-body bound state $\\alpha+n+p$ in the hyperspherical Lagrange-mesh method. The contribution of the E1 transition operator from the initial isosinglet states to the isotriplet components of the final state is estimated to be negligible. An estimation of the forbidden E1 transition to the isosinglet components of the final state is comparable with the corresponding results of the two-body model. However, the contribution of the E2 transition operator is found to be much smaller than the corresponding estimations of the two-body model. The three-body model perfectly matches the new experimental data of the LUNA collaboration with the help of the spectroscopic factor 2.586, very consistent with the three-body structure of the final state.

  2. Analysis of the normal optical, Michel and molecular potentials on the $^{40}$Ca($^6$Li, d)$^{44}$ Ti reaction

    Indian Academy of Sciences (India)

    MAZUMDER UTTAM K; SOMADDER ANOCK; HOQUE ENAMUL; HAQUE YASMEEN; DAS SUSANTA K; SEN GUPTA H M

    2016-06-01

    Full finite-range (FFR) distorted-wave Born approximation (DWBA) method has been applied to analyse the angular distributions of cross-sections of the $^{40}$Ca($^{6}$Li, d)$^{44}$Ti reaction at 28 MeV incident energy for the 22 transitions involving both the bound and unbound states of $^{44}$Ti byusing the normal optical, Michel and molecular potentials. The extracted spectroscopic factors for the three optical potentials are compared with those of some previous studies of zero-range (ZR) calculations of the$^{40}$Ca($^{6}$Li, d)$^{44}$Ti reaction using the normal optical potential. The $\\chi^{2}$ values of all the levels are obtained for the three optical potentials to estimate the quality of the fits. Molecular and Michel potentials have been used for the first time to analyse the four-nucleon transfer reaction and it seems that the molecular potential fits the experimental data more satisfactorily for some of the states than the normal optical and Michel potentials.

  3. Low energy R-matrix fits for the 6Li(d,a)4He S factor

    CERN Document Server

    Grineviciute, J; Lamia, L; Spitaleri, C; La Cognata, M

    2014-01-01

    Background: The information about the 6Li(d,a)4He reaction rates of the astrophysical interest can be obtained by extrapolating direct data to the lower energies, or by indirect methods. The indirect Trojan Horse method, as well as various R-matrix and polynomial fits to direct data, estimate the electron screening energies much larger than the adiabatic limit. Calculations that include the subthreshold resonance estimate smaller screening energies. Purpose: Obtain the 6Li(d,a)4He reaction R-matrix parameters and the astrophysical S factor for the energies relevant to the stellar plasmas by fitting the R-matrix formulas for the subthreshold resonances to the S factor data above 60 keV. Methods: The bare S factor is calculated using the single and the two-level R-matrix formulas for the closest to the threshold 0+ and 2+ subthreshold states at 22.2, 20.2 and 20.1 MeV. The electron screening potential Ue is then obtained by fitting it as a single parameter to the low energy data. Results: The low energy S facto...

  4. Resonance and non-resonance effect of continuum states of 6Li on elastic scattering angular distributions

    Science.gov (United States)

    Gómez Camacho, A.

    2016-07-01

    CDCC calculations of elastic scattering angular distributions for reactions of the weakly bound projectile 6Li with targets 28Si and 58Ni at energies around the Coulomb barrier are presented. Special emphasis is given to account for the effect of couplings from 6Li resonance states l = 2, J π = 3+, 2+, 1+. Similarly, the effect produced by non-resonant state couplings is studied. The convergent calculations are carried out with global α-target and d-target interactions. The calculated elastic scattering angular distributions are in general in good agreement with the measurements for the systems considered in this work. It is found that the calculations with only resonance states are very similar to that with all couplings (resonance+non-resonance). So, the absence of these states have a strong effect on elastic scattering (non-resonance states calculation). It is shown that the effects increase as the collision energy increases. An interpretation of the strength of the different effects is given in terms of the polarization potentials that emerge from the different couplings.

  5. Inelastic p{sup 9}Be scattering and halo structure of the J{sup π} = 1/2{sup +} excited state of the {sup 9}Be nucleus

    Energy Technology Data Exchange (ETDEWEB)

    Zhusupov, M. A. [Al-Farabi Kazakh National University (Kazakhstan); Ibraeva, E. T., E-mail: ibr@inp.kz; Krassovitskiy, P. M. [National Nuclear Center of Republic of Kazakhstan, Institute of Nuclear Physics (Kazakhstan)

    2015-01-15

    Differential cross sections for inelastic p{sup 9}Be scattering (to the J{sup α} = 1/2{sup +} level) were calculated on the basis of Glauber’s diffraction theory. The wave function for the {sup 9}Be nucleus in the three-particle 2αn model was used in this calculation. An expansion of this wave function in a series in Gaussian functions and the representation of the Glauber operator Ω in the form conjugate to the three-particle wave function make it possible to calculate analytically inelastic-scattering matrix elements. The differential cross section calculated by using the 2αn wave functions agrees well with available experimental data at E = 180 MeV.

  6. Ghost anomaly and first excited state of sup 8 Be in the sup 9 Be(d,t. alpha. ) sup 4 He reaction at 7 MeV

    Energy Technology Data Exchange (ETDEWEB)

    Szczurek, A.; Bodek, K. (Uniwersytet Jagiellonski, Krakow (Poland). Inst. Fizyki Bochum Univ. (Germany). Inst. fuer Experimentalphysik 1); Jarczyk, L.; Kamys, B.; Strzalkowski, A. (Uniwersytet Jagiellonski, Krakow (Poland). Inst. Fizyki); Krug, J.; Luebcke, W.; Ruehl, H.; Seinke, M.; Stephan, M.; Kamke, D. (Bochum Univ. (Germany). Inst. fuer Experimentalphysik 1)

    1991-08-26

    The three-body reaction {sup 9}Be + d {yields} t + {alpha} + {alpha} has been investigated in kinematically complete experiments at E{sub d} = 7.0 MeV for {theta}{sub t} 100{sup 0}, {theta}{sub {alpha}} = -40{sup 0} and for {theta}{sub t} = 40{sup 0}, {theta}{sub {alpha}} = 72.5{sup 0} to -162.5{sup 0}. The experimental spectra are dominated by sequential processes via intermediate excited states of {sup 8}Be and {sup 7}Li. R-matrix theory was employed to describe the line shape of the first excited state and the ghost anomaly of the ground state of {sup 8}Be. Use was made of the {alpha}{alpha} phase shifts. The best fits were obtained assuming a channel radius of a{sub {alpha}{alpha}} = 4.5 fm. The average intensity of the ghost anomaly for E{sub {alpha}{alpha}} = 0.35-1.0 MeV is 4.3%/MeV ({theta}{sub t} = 40{sup 0}) and 8%/MeV ({theta}{sub t} = 100{sup 0}). For the first excited state of {sup 8}Be we find E{sub x} = 3.00 MeV and {Gamma}{sub x} = 1.23 MeV(FWHM). (orig.).

  7. River fluxes to the sea from the ocean's 10Be/9Be ratio

    Science.gov (United States)

    von Blanckenburg, F.; Bouchez, J.

    2013-12-01

    The ratio of the meteoric cosmogenic radionuclide 10Be to the stable isotope 9Be is proposed here to be a flux proxy of terrigenous input into the oceans. The ocean's dissolved 10Be/9Be is set by (1) the flux of meteoric 10Be produced in the atmosphere; (2) the denudational flux of the rivers discharging into a given ocean basin; (3) the fraction of 9Be that is released from primary minerals during weathering (meaning the 9Be transported by rivers in either the dissolved form or adsorbed onto sedimentary particles and incorporated into secondary oxides); and (4) the fraction of riverine 10Be and 9Be actually released into seawater. Using published 10Be/9Be data of rivers for which independent denudation rate estimates exist we first find that the global average fraction of 9Be released during weathering into river waters and their particulate load is 20% and does not depend on denudation rate. We then evaluate this quantitative denudation rate proxy by using published dissolved seawater Be isotope data and a compilation of global river loads (15Gt/yr). We find that the measured global average oceanic dissolved 10Be/9Be ratio of about 0.9E-7 is satisfied by the mass balance if only 6.5% of the dissolved and reactive riverine Be is eventually released to the open ocean by boundary exchange. Except for the South Atlantic and the South Pacific, in which the 10Be/9Be ratio is dominated by Be advected through ocean circulation, good agreement results between 10Be/9Be ratios predicted by denudation rates and measured ocean 10Be/9Be ratios when we establish this mass balance for individual ocean basins. As the seawater 10Be/9Be ratio is faithfully recorded in marine chemical precipitates the 10Be/9Be ratio extracted from authigenic sediments can now serve to estimate relative changes in terrigenous input into the oceans back through time on a global and on a basin scale.

  8. River fluxes to the sea from the oceanʼs 10Be/9Be ratio

    Science.gov (United States)

    von Blanckenburg, Friedhelm; Bouchez, Julien

    2014-02-01

    The ratio of the meteoric cosmogenic radionuclide 10Be to the stable isotope 9Be is proposed here to be a flux proxy of terrigenous input into the oceans. The ocean's dissolved 10Be/9Be is set by (1) the flux of meteoric 10Be produced in the atmosphere; (2) the denudational flux of the rivers discharging into a given ocean basin; (3) the fraction of 9Be that is released from primary minerals during weathering (meaning the 9Be transported by rivers in either the dissolved form or adsorbed onto sedimentary particles and incorporated into secondary oxides); and (4) the fraction of riverine 10Be and 9Be actually released into seawater. Using published 10Be/9Be data of rivers for which independent denudation rate estimates exist we first find that the global average fraction of 9Be released during weathering into river waters and their particulate load is 20% and does not depend on denudation rate. We then evaluate this quantitative proxy for terrigenous inputs by using published dissolved seawater Be isotope data and a compilation of global river loads. We find that the measured global average oceanic dissolved 10Be/9Be ratio of about 0.9×10-7 is satisfied by the mass balance if only about 6% of the dissolved and adsorbed riverine Be is eventually released to the open ocean after escaping the coastal zone. When we establish this mass balance for individual ocean basins good agreement results between 10Be/9Be ratios predicted from known river basin denudation rates and measured ocean 10Be/9Be ratios. Only in the South Atlantic and the South Pacific the 10Be/9Be ratio is dominated by advected Be and in these basins the ratio is a proxy for ocean circulation. As the seawater 10Be/9Be ratio is faithfully recorded in marine chemical precipitates the 10Be/9Be ratio extracted from authigenic sediments can now serve to estimate relative changes in terrigenous input into the oceans back through time on a global and on an ocean basin scale.

  9. Magnetic control of ultra-cold $^6$Li and $^{174}$Yb($^3P_2$) atom mixtures with Feshbach resonances

    CERN Document Server

    Petrov, Alexander; Kotochigova, Svetlana

    2015-01-01

    We theoretically evaluate the feasibility to form magnetically-tunable Feshbach molecules in collisions between fermionic $^6$Li atoms and bosonic metastable $^{174}$Yb($^3$P$_2$) atoms. In contrast to the well-studied alkali-metal atom collisions, collisions with meta-stable atoms are highly anisotropic. Our first-principle coupled-channel calculation of these collisions reveals the existence of broad Feshbach resonances due to the combined effect of anisotropic-molecular and atomic-hyperfine interactions. In order to fit our predictions to the specific positions of experimentally-observed broad resonance structures \\cite{Deep2015} we optimized the shape of the short-range potentials by direct least-square fitting. This allowed us to identify the dominant resonance by its leading angular momentum quantum numbers and describe the role of collisional anisotropy in the creation and broadening of this and other resonances.

  10. Characterization of charge-exchange collisions between ultracold $\\rm{^6Li}$ atoms and $\\rm{^{40}Ca^+}$ ions

    CERN Document Server

    Saito, R; Sasakawa, M; Nakai, R; Raoult, M; Silva, H Da; Dulieu, O; Mukaiyama, T

    2016-01-01

    We investigate the energy dependence and the internal-state dependence of the charge-exchange collision cross sections in a mixture of $^6$Li atoms and $^{40}$Ca$^+$ ions in the collision energy range from 0.2 mK to 1 K. Deliberately excited ion micromotion is used to control the collision energy of atoms and ions. The energy dependence of the charge-exchange collision cross section obeys the Langevin model in the temperature range of the current experiment, and the measured magnitude of the cross section is correlated to the internal state of the $^{40}$Ca$^+$ ions. Revealing the relationship between the charge-exchange collision cross sections and the interaction potentials is an important step toward the realization of the full quantum control of the chemical reactions at an ultralow temperature regime.

  11. Hypernuclear spectroscopy of products from 6Li projectiles on a carbon target at 2 AGeV

    CERN Document Server

    Rappold, C; Nakajima, D; Saito, T R; Bertini, O; Bianchin, S; Bozkurt, V; Kavatsyuk, M; Ma, Y; Maas, F; Minami, S; Özel-Tashenov, B; Yoshida, K; Achenbach, P; Ajimura, S; Aumann, T; Gayoso, C Ayerbe; Bhang, H C; Caesar, C; Erturk, S; Fukuda, T; Göküzüm, B; Guliev, E; Hiraiwa, T; Hoffmann, J; Ickert, G; Ketenci, Z S; Khaneft, D; Kim, M; Kim, S; Koch, K; Kurz, N; Fèvre, A Le; Mizoi, Y; Moritsu, M; Nagae, T; Nungesser, L; Okamura, A; Ott, W; Pochodzalla, J; Sakaguchi, A; Sako, M; Schmidt, C J; Sekimoto, M; Simon, H; Sugimura, H; Takahashi, T; Tambave, G J; Tamura, H; Trautmann, W; Voltz, S; Yokota, N; Yoon, C J

    2013-01-01

    A novel experiment, aiming at demonstrating the feasibility of hypernuclear spectroscopy with heavy-ion beams, was conducted. Using the invariant mass method, the spectroscopy of hypernuclear products of 6Li projectiles on a carbon target at 2 AGeV was performed. Signals of the \\Lambda-hyperon and 3\\Lambda H and 4\\Lambda H hypernuclei were observed for final states of p+\\pi^-, 3He+\\pi^- and 4He+\\pi^-, respectively, with significance values of 6.7, 4.7 and 4.9\\sigma. By analyzing the proper decay time from secondary vertex distribution with the unbinned maximum likelihood fitting method, their lifetime values were deduced to be $262 ^{+56}_{-43} \\pm 45$ ps for \\Lambda, $183 ^{+42}_{-32} \\pm 37$ ps for 3\\Lambda H, and $140 ^{+48}_{-33}\\pm 35 $ ps for 4\\Lambda H.

  12. Nuclear structure with accurate chiral perturbation theory nucleon-nucleon potential: Application to 6Li and 10B

    Energy Technology Data Exchange (ETDEWEB)

    Navratil, P; Caurier, E

    2003-10-14

    The authors calculate properties of A = 6 system using the accurate charge-dependent nucleon-nucleon (NN) potential at fourth order of chiral perturbation theory. By application of the ab initio no-core shell model (NCSM) and a variational calculation in the harmonic oscillator basis with basis size up to 16 {h_bar}{Omega} they obtain the {sup 6}Li binding energy of 28.5(5) MeV and a converged excitation spectrum. Also, they calculate properties of {sup 10}B using the same NN potential in a basis space of up to 8 {h_bar}{Omega}. The results are consistent with results obtained by standard accurate NN potentials and demonstrate a deficiency of Hamiltonians consisting of only two-body terms. At this order of chiral perturbation theory three-body terms appear. It is expected that inclusion of such terms in the Hamiltonian will improve agreement with experiment.

  13. The Benchmark Testing of ~9Be of CENDL-3.0

    Institute of Scientific and Technical Information of China (English)

    2002-01-01

    The 9Be data of CENDL-3.0 were updated again recently by Prof.Zhang Jing-shang et al. by using anew approach. In order to test the reliability of 9Be data of CENDL-3.0, some benchmarks were used. Inaddition to the values of Keff, the leakage spectrum of Be sphere was calculated. The data processing wascarried out by using the NJOY nuclear data processing code system. The calculations and analyses of

  14. Elastic forward analysis using sup 7 Li ions A useful tool for H and light elements determination

    CERN Document Server

    Romero, S; Murillo, G; Berdejo, H M

    2002-01-01

    Films of CN sub x /Si, TiN sub x /AISI 304 and AlO sub x /Si were analyzed with sup 7 Li ions from 4.0 to 4.5 MeV and an experimental arrangement that, through detection of scattered projectiles and recoils by a single detector, allows quantification of H, light elements and heavier ones. A discussion is presented of the capabilities of Rutherford backscattering spectrometry (RBS) and conventional elastic recoil detection analysis (ERDA) compared to elastic forward analysis.

  15. Ab initio no-core properties of 7Li and 7Be with JISP16 and NNLO_opt interactions

    CERN Document Server

    Heng, Taihua; Maris, Pieter

    2016-01-01

    We investigate the properties of 7Li with the JISP16 and chiral NNLO_opt nucleon-nucleon interactions and 7Be with the JISP16 interaction in the ab initio no-core full configuration (NCFC) approach. We calculate selected observables that include energy spectra, point proton root-mean-square radii, electromagnetic moments and transitions. We compare our results with experimental results, where available, as well as with results obtained using nucleon-nucleon plus three-nucleon interactions. We obtain reasonable agreement between theory and experiment for low-lying states that are dominated by p-shell configurations.

  16. Calculation of Double-Differential Cross Sections of n+7Li Reactions Below 20 MeV

    Institute of Scientific and Technical Information of China (English)

    ZHANG Jing-Shang; HAN Ying-Lu

    2002-01-01

    A new reaction model for light nuclei is proposed to analyze the measured data,especially for analysis of the double-differential cross sections of the outgoing particles.Many channels arc opened in the n + 7Li reaction below En< 20 MeV.The reaction mechanism is very complex,beside the sequential emissions there are also three-body breakup processes.Because of a strong recoil effect of light nucleus reactions,the energy balance is strictly taken into account.The comparisons of the calculated results with the double-differential measurements indicate that the model calculations are successful for the total outgoing neutrons.

  17. A TPD and AR based comparison of accelerator neutron irradiation fields between (7)Li and W targets for BNCT.

    Science.gov (United States)

    Tanaka, Kenichi; Endo, Satoru; Yonai, Shunsuke; Baba, Mamoru; Hoshi, Masaharu

    2014-06-01

    The characteristics of moderator assembly dimension was investigated for the usage of (7)Li(p,n) neutrons by 2.3-2.8MeV protons and W(p,n) neutrons by 50MeV protons. The indexes were the treatable protocol depth (TPD) and advantage depth (AD). Consequently, a configuration for W target with the Fe filter, Fluental moderator, Pb reflector showed the TPD of 5.8cm and AD of 9.3cm. Comparable indexes were found for the Li target in a geometry with the MgF2 moderator and Teflon reflector.

  18. Breakup Coupling Effects on Near-Barrier {sup 6}Li, {sup 7}Be and {sup 8}B + {sup 58}Ni Elastic Scattering Compared

    Energy Technology Data Exchange (ETDEWEB)

    Keeley, N. [Department of Nuclear Reactions, Andrzej Soltan Institute for Nuclear Studies, ul. Hoza 69, 00-681 Warsaw (Poland); Mackintosh, R.S. [Department of Physics and Astronomy, Open University, Milton Keynes, MK7 6AA (United Kingdom); Beck, C. [Institut Pluridisciplinaire Hubert Curien et Universite Louis Pasteur, Boite Postale 28, F-67037 Strasbourg Cedex 2 (France)

    2010-03-01

    New data for near-barrier {sup 6}Li, {sup 7}Be and {sup 8}B + {sup 58}Ni elastic scattering enable a comparison of breakup coupling effects for these loosely-bound projectiles. Coupled Discretised Continuum Channels (CDCC) calculations suggest that the large total reaction cross sections for {sup 8}B + {sup 58}Ni are dominated by breakup at near-barrier energies, unlike {sup 6}Li and {sup 7}Be where breakup makes a small contribution. In spite of this, the CDCC calculations show a small coupling influence due to breakup for {sup 8}B, in contrast to the situation for {sup 6}Li and {sup 7}Be. An examination of the S matrices gives a clue to this counter-intuitive behaviour.

  19. Elastic scattering and cluster-transfer reactions of 98Rb on 7Li at REX-ISOLDE

    CERN Document Server

    Bouma, Jake

    Exotic nuclei are nuclei with unusual proton to neutron ratios that exist far away from stability. Due to their instability, these nuclei are only available for nuclear reactions as radioactive ion beams. Experiments must therefore be performed in inverse kinematics at advanced radioactive isotope separation and acceleration facilities. REX-ISOLDE at CERN is one such facility, capable of producing post-accelerated radioactive ion beams with energies up to 2.85 MeV/u. Cluster-transfer reactions in inverse kinematics with a $^{7}$Li target are proposed as a tool for the study of exotic nuclei at REX-ISOLDE. In these reactions, either the $\\alpha$ or triton clusters that make up the weakly bound $^{7}$Li nucleus can be transfered to the beam nucleus. The remaining cluster that is not transferred can be detected, and identifies the particular transfer channel. Through this mechanism it is possible to populate states of very high spin, which is useful for $\\gamma$-spectroscopy in poorly known exotic regions. Speci...

  20. The 7Be(d,p)2alpha cross section at Big Bang energies and the primordial 7Li abundance

    CERN Document Server

    Angulo, C; Couder, M; Demaret, P; Leleux, P; Vanderbist, F; Coc, A; Kiener, J; Tatischeff, V; Davinson, T; Murphy, A S; Achouri, N L; Orr, N A; Cortina-Gil, D; Figuera, P; Fulton, B R; Mukha, I; Vangioni, E

    2005-01-01

    The WMAP satellite, devoted to the observations of the anisotropies of the Cosmic Microwave Background (CMB) radiation, has recently provided a determination of the baryonic density of the Universe with unprecedented precision. Using this, Big Bang Nucleosynthesis (BBN) calculations predict a primordial 7Li abundance which is a factor 2-3 higher than that observed in galactic halo dwarf stars. It has been argued that this discrepancy could be resolved if the 7Be(d,p)2alpha reaction rate is around a factor of 100 larger than has previously been considered. We have now studied this reaction, for the first time at energies appropriate to the Big Bang environment, at the CYCLONE radioactive beam facility at Louvain-la-Neuve. The cross section was found to be a factor of 10 smaller than derived from earlier measurements. It is concluded therefore that nuclear uncertainties cannot explain the discrepancy between observed and predicted primordial 7Li abundances, and an alternative astrophysical solution must be inve...

  1. Quasi-bound alpha resonant states populated by the {sup 12}C({sup 6}Li, d) reaction

    Energy Technology Data Exchange (ETDEWEB)

    Rodrigues, M.R.D.; Borello-Lewin, T.; Miyake, H.; Horodynski-Matsushigue, L.B.; Duarte, J.L.M.; Rodrigues, C.L.; Souza, M.A. [Universidade de Sao Paulo (IF/USP), SP (Brazil). Inst. de Fisica; Cunsolo, A.; Cappuzzello, F.; Foti, A.; Agodi, C.; Cavallaro, M. [Istituto Nazionale di Fisica Nucleare (LNS/INFN), Catania (Italy). Lab. Nazionali del Sud; Ukita, G.M. [Universidade de Santo Amaro (UNISA), Sao Paulo, SP (Brazil). Faculdade de Psicologia

    2012-07-01

    Full text: The alpha cluster phenomenon in the light nuclei structure has been the subject of a long time investigation since the proposal of the Ikeda diagrams [1]. The main purpose of the research program in progress is the investigation of this phenomenon in (x{alpha}) and (x{alpha}+n) nuclei through the ({sup 6}Li, d) alpha transfer reaction [2-4]. Alpha resonant states around the (4{alpha}) threshold in the nucleus {sup 16}O are the focus of the present contribution. In fact, the importance of these resonances at the elements production in stars is recognized, as primarily pointed out by Hoyle in {sup 12}C [6]. The existence of a rotational band with the {alpha} +{sup 12} C (Hoyle) cluster state structure was recently demonstrated by Ohkubo and Hirabayashi [6]. In order to explore this region of interest, measurements of the {sup 12}C({sup 6}Li, d){sup 16}O reaction up to 17 MeV of excitation at an incident energy of 25.5 MeV, have been performed employing the Sao Paulo Pelletron-Enge Split-Pole facility and the nuclear emulsion detection technique (plates Fuji G6B, 50 {mu}m thick). Spectra associated with six scattering angles, from 5 deg to 29 deg in the laboratory frame, each one 50 cm along the focal surface, were measured. Several narrow resonances with a quasi-bound behavior embedded in the continuum were detected and the resolution of 25 keV allowed for the separation of doublets not resolved before [7,8]. The absolute cross sections and the respective deuteron angular distributions were determined and the analysis is in progress. [1] K. Ikeda et al., Prog. Theor. Phys. Suppl. E 68, 464 (1968); H. Horiuchi, K. Ikeda, and Y. Suzuki, ibid. 44, 225 (1978). [2] M.R.D.Rodrigues et al., in12th International Conference on Nuclear Reaction Mechanism, Varenna, Italy, edited by F. Cerutti and A. Ferrari , CERN Proceedings, 2010-2, pp. 331- 335. [3] T. Borello-Lewin et al., Proceedings of SOTANCP2, Brussels, Belgium 2010, edited by P. Descouvemount et al., Int. J

  2. Earth surface erosion and weathering from the 10Be (meteoric)/9Be ratio

    Science.gov (United States)

    von Blanckenburg, F.; Bouchez, J.; Wittmann, H.; Dannhaus, N.

    2012-12-01

    A perfect clock of the stability of the Earth surface is one that combines a first isotope the flux of which depends on the release rate during erosion, and a second isotope produced at constant rate. The ratio of the meteoric cosmogenic nuclide 10Be to stable 9Be is such a system. We provide a quantitative framework for its use. In a weathering zone some of the 9Be, present typically in 2.5ppm concentrations in silicate minerals, is released and partitioned between a reactive phase (adsorbed to clay and hydroxide surfaces, given the high partition coefficients at intermediate pH), and into the dissolved phase. The combined mass flux of both phases is defined by the soil formation rate and a mineral dissolution rate - and is hence proportional to the chemical weathering rate and the denudation rate. At the same time, the surface of the weathering zone is continuously exposed to fallout of meteoric 10Be. This 10Be percolates into the weathering zone where it mixes with dissolved 9Be. Both isotopes may exchange with the adsorbed Be, given that equilibration rate of Be is fast relative to soil residence times. Hence a 10Be/9Be(reactive) ratio results in soils from which the total denudation rate can be calculated. A prerequisite is that the flux of meteoric 10Be is known from field experiments or from global production models [1], that the 9Be concentration in bedrock (mostly 2.5ppm) is known [2], and that the reactive Be can be chemically extracted from soil or sediment [3]. In rivers, when reactive Be and dissolved Be equilibrate, a catchment-wide denudation rate can be determined from both sediment and a sample of filtered river water, where the sediment 10Be/9Be ratio is independent of grain size. We have tested this approach in sediment-bound Be and dissolved Be in water of the Amazon and Orinoco basin. The reactive Be was extracted from sediment by combined hydroxylamine and HCl leaches [2]. In the Amazon trunk stream, the Orinoco, Apure, and La Tigra river 10Be

  3. Using the Doppler broadened γ line of the 10B(n,αγ)7Li reaction for thermal neutron detection

    Science.gov (United States)

    Ben-Galim, Y.; Wengrowicz, U.; Moreh, R.; Orion, I.; Raveh, A.

    2016-02-01

    When a thermal neutron is absorbed by 10B in the 10B(n,α)7Li reaction, there is a chance of 94% that a 478 keV photon be emitted by an excited 7Li nucleus. This reaction is exothermic with a Q-value of 2.31 MeV and the nuclei are emitted with kinetic energies of E(α)=1.47 MeV and E(7Li*)=0.84 MeV. This implies that the 478 keV γ line is emitted by a moving 7Li nucleus and hence is expected to be Doppler broadened. In the present work we suggest to use this broadening of the γ line as a fingerprint for the detection of thermal neutrons using a high resolution gamma spectrometer. We thus developed a Monte Carlo program using a MATLAB code based on a High Purity Germanium (HPGe) detector coupled with a Boron Carbide (B4C) sheet to calculate the γ line broadening. Our simulation shows that the FWHM width of the resulting γ line is 12.6 keV, in good agreement with our measurement. Hence the broadened γ line emitted by the 10B(n,αγ)7Li reaction and detected by a HPGe detector shows that this method is an effective tool for neutron detection while maintaining good gamma discrimination.

  4. Effects of t- and α-transfer on the spectroscopic information from the {sup 6}Li({sup 3}He,d){sup 7}Be reaction

    Energy Technology Data Exchange (ETDEWEB)

    Burtebayev, N., E-mail: nburtebayev@yandex.ru [Institute of Nuclear Physics of National Nuclear Center, 480082, Almaty, Ibragimova str. 1 (Kazakhstan); Burtebayeva, J.T.; Glushchenko, N.V.; Kerimkulov, Zh.K. [Institute of Nuclear Physics of National Nuclear Center, 480082, Almaty, Ibragimova str. 1 (Kazakhstan); Amar, A. [Al-Farabi Kazakh National University, 480078, Almaty, al-Farabi ave. 71 (Kazakhstan); Tanta University, Faculty of Science, Physics Department, Tanta (Egypt); Nassurlla, M. [Al-Farabi Kazakh National University, 480078, Almaty, al-Farabi ave. 71 (Kazakhstan); Sakuta, S.B. [National Research Center “Kurchatov Institute”, Kurchatov Sq. 1, 123182 Moscow (Russian Federation); Artemov, S.V.; Igamov, S.B.; Karakhodzhaev, A.A. [Institute of Nuclear Physics, Tashkent, Avliyo Ota str. 61 (Uzbekistan); Rusek, K. [Heavy Ion Laboratory of Warsaw University, ul. L. Pasteura 5A, PL-02-093 Warsaw (Poland); Kliczewski, S. [H. Niewodniczański Institute of Nuclear Physics, Polish Academy of Sciences, ul. Radzikowskiego 152, PL-31-342 Cracow (Poland)

    2013-07-01

    Angular distributions of differential cross sections have been measured for elastic, inelastic scattering and the ({sup 3}He,d) reaction on {sup 6}Li nuclei at the E{sub lab}({sup 3}He)=34 MeV energy. The new and early obtained elastic scattering data at 34, 50, 60 and 72 MeV have been analyzed with Coupled Reaction Channels Method (CRC) taking into account triton transfer mechanism. The spectroscopic factors for t+{sup 3}He configuration of {sup 6}Li were extracted. Parameters for real part of potential have been also calculated microscopically with double folding model. The differential cross sections for proton stripping to the {sup 7}Be ground and first excited states have been analyzed by modified DWBA and CRC methods at 34 MeV. The effect of triton and α exchange on proton transfer reaction {sup 6}Li({sup 3}He,d){sup 7}Be for both ground and excited state is discussed. Spectroscopic factors and asymptotical normalization coefficients for p+{sup 6}Li configuration of {sup 7}Be have been obtained from the experimental data.

  5. Spectroscopic strengths for /sup 6/Li-induced alpha-particle transfers on /sup 18/O at 72 MeV

    Energy Technology Data Exchange (ETDEWEB)

    Tanabe, T.; Ogino, K.; Kadota, Y.; Haga, K.; Kitahara, T.; Shiba, T.

    1982-08-01

    The /sup 18/O(/sup 6/Li,d)/sup 22/Ne reaction has been studied at 72-MeV bombarding energy. The angular distributions for transitions to low-lying states in /sup 22/Ne are fitted by exact finite-range distorted-wave Born approximation calculations and yield relative spectroscopic factors in good agreement with theoretical predictions.

  6. Multi-elemental characterization of organic liquid samples by use of a 13 MeV {sup 6}Li{sup 3+} beam

    Energy Technology Data Exchange (ETDEWEB)

    Liendo, J.A., E-mail: jliendo@usb.v [Department of Physics, Simon Bolivar University, PO Box 89000, Caracas 1080-A (Venezuela, Bolivarian Republic of); Bernal, M.A., E-mail: mbernal@usb.v [Department of Physics, Simon Bolivar University, PO Box 89000, Caracas 1080-A (Venezuela, Bolivarian Republic of); Gonzalez, A.C. [Centro de Fisica, Instituto Venezolano de Investigaciones Cientificas, Caracas (Venezuela, Bolivarian Republic of); Caussyn, D.D.; Fletcher, N.R.; Momotyuk, O.A. [Department of Physics, Florida State University, Tallahassee (United States); Muruganathan, R.M. [Department of Chemistry, Florida State University, Tallahassee (United States); Roeder, B.T.; Wiedenhoever, I. [Department of Physics, Florida State University, Tallahassee (United States); Fischer, T. [Department of Chemistry, Florida State University, Tallahassee (United States); Kemper, K.W.; Barber, P. [Department of Physics, Florida State University, Tallahassee (United States); Sajo-Bohus, L. [Department of Physics, Simon Bolivar University, PO Box 89000, Caracas 1080-A (Venezuela, Bolivarian Republic of)

    2009-10-15

    Evaporated amniotic fluid (AF) targets have been bombarded with a 13 MeV {sup 6}Li{sup 3+} beam. Forward angle data have served to identify the {sup 1}H({sup 6}Li,{sup 1}H){sup 6}Li reaction as an alternative for hydrogen characterization of such organic samples. Detected {sup 6}Li ions elastically scattered from C, N, O, Na and Cl can also be used to determine the concentrations of these elements in AF. The analyzed AF samples have been diluted with distilled water. The effect of sample dilution on the improvement of spectrum energy resolution has been observed, confirming previous reports. The hydrogen concentration determined in the studied AF targets is shown to vary linearly with sample dilution. Two detector arrangements have been used to find out which detection scheme is the most convenient. The combination of a counter telescope and a single detector, set up at the same polar angle on the opposite side of the beam, seems to be the best choice to have a reliable particle identification and an adequate energy resolution simultaneously.

  7. (/sup 6/Li,d) reactions on /sup 24/Mg and /sup 26/Mg at 73 MeV

    Energy Technology Data Exchange (ETDEWEB)

    Tanabe, T.; Haga, K.; Yasue, M.; Sato, K. (Tokyo Univ., Tanashi (Japan). Inst. for Nuclear Study); Ogino, K.; Kadota, Y.; Tochi, M.; Makino, K. (Kyoto Univ. (Japan). Faculty of Engineering); Kitahara, T. (Yamanashi Medical Coll. (Japan)); Shiba, T. (Kyoto Univ. (Japan). Lab. of Nuclear Reaction)

    1983-05-09

    The sup(24,26)Mg(/sup 6/Li, d)sup(28,30)Si reactions have been studied at 73 MeV bombarding energy. The angular distributions were analyzed with exact finite-range distorted wave Born approximation calculations assuming a direct ..cap alpha..-cluster transfer. Extracted spectroscopic strengths leading to low-lying levels of /sup 28/Si and relative spectroscopic strengths between transitions to /sup 28/Si and /sup 30/Si ground states are consistent with those previously obtained by several ..cap alpha..-transfer reactions. Many strongly populated levels have been observed at Esub(x)> or approx.10 MeV for /sup 28/Si. A marked similarity was found between the deuteron spectrum and the /sup 24/Mg(..cap alpha.., ..cap alpha..)/sup 24/Mg excitation function in this excitation energy region. A brief comparison of the present ..cap alpha..-transfer results with previous two-nucleon transfer data leading to sup(28,30)Si is also presented.

  8. Hypernuclear production cross section in the reaction of 6Li + 12C at 2A GeV

    Directory of Open Access Journals (Sweden)

    C. Rappold

    2015-07-01

    Full Text Available Hypernuclear production cross sections have been deduced for the first time with induced reaction of heavy ion beam on fixed target and by means of the invariant mass method by the HypHI Collaboration exploiting the reaction of 6Li + 12C at 2A GeV or sNN=2.70 GeV. A production cross section of 3.9±1.4 μb for 3ΛH and of 3.1±1.0 μb for 4ΛH respectively in the projectile rapidity region was inferred as well as the total production cross section of the Λ hyperon was measured and found to be equal to 1.7±0.8 mb. A global fit based on a Bayesian approach was performed in order to include and propagate statistical and systematic uncertainties. Production ratios of 3ΛH/4ΛH, 3ΛH/Λ and 4ΛH/Λ were included in the inference procedure. The strangeness population factors S3 and S4 of 3ΛH and 4ΛH respectively were extracted. In addition, the multiplicities of the Λ hyperon, 3ΛH, and 4ΛH together with the rapidity and transversal momentum density distributions of the observed hypernuclei were extracted and reported.

  9. Development of neutron-monitor detector using liquid organic scintillator coupled with 6Li + ZnS(Ag) Sheet.

    Science.gov (United States)

    Sato, Tatsuhiko; Endo, Akira; Yamaguchi, Yasuhiro; Takahashi, Fumiaki

    2004-01-01

    A phoswitch-type detector has been developed for monitoring neutron doses in high-energy accelerator facilities. The detector is composed of a liquid organic scintillator (BC501A) coupled with ZnS(Ag) sheets doped with 6Li. The dose from neutrons with energies above 1 MeV is evaluated from the light output spectrum of the BC501A by applying the G-function, which relates the spectrum to the neutron dose directly. The dose from lower energy neutrons, on the other hand, is estimated from the number of scintillations emitted from the ZnS(Ag) sheets. Characteristics of the phoswitch-type detector were studied experimentally in some neutron fields. It was found from the experiments that the detector has an excellent property of pulse-shape discrimination between the scintillations of BC501A and the ZnS(Ag) sheets. The experimental results also indicate that the detector is capable of reproducing doses from thermal neutrons as well as neutrons with energies from one to several tens of megaelectronvolts (MeV).

  10. Improved neutron-gamma discrimination for a 6Li-glass neutron detector using digital signal analysis methods

    Science.gov (United States)

    Wang, C. L.; Riedel, R. A.

    2016-01-01

    A 6Li-glass scintillator (GS20) based neutron Anger camera was developed for time-of-flight single-crystal diffraction instruments at Spallation Neutron Source. Traditional Pulse-Height Analysis (PHA) for Neutron-Gamma Discrimination (NGD) resulted in the neutron-gamma efficiency ratio (defined as NGD ratio) on the order of 104. The NGD ratios of Anger cameras need to be improved for broader applications including neutron reflectometers. For this purpose, six digital signal analysis methods of individual waveforms acquired from photomultiplier tubes were proposed using (i) charge integration, (ii) pulse-amplitude histograms, (iii) power spectrum analysis combined with the maximum pulse-amplitude, (iv) two event parameters (a1, b0) obtained from a Wiener filter, (v) an effective amplitude (m) obtained from an adaptive least-mean-square filter, and (vi) a cross-correlation coefficient between individual and reference waveforms. The NGD ratios are about 70 times those from the traditional PHA method. Our results indicate the NGD capabilities of neutron Anger cameras based on GS20 scintillators can be significantly improved with digital signal analysis methods.

  11. Hypernuclear spectroscopy of products from {sup 6}Li projectiles on a carbon target at 2A GeV

    Energy Technology Data Exchange (ETDEWEB)

    Rappold, C., E-mail: c.rappold@gsi.de [Justus-Liebig-Universität Giessen, Heinrich-Buff-Ring 16, 35392 Giessen (Germany); GSI Helmholtz Centre for Heavy Ion Research, Planckstrasse 1, 64291 Darmstadt (Germany); Kim, E. [GSI Helmholtz Centre for Heavy Ion Research, Planckstrasse 1, 64291 Darmstadt (Germany); Seoul National University, Gwanakro Sillim-dong, Gwanak-gu, Seoul 151-747 (Korea, Republic of); Nakajima, D. [GSI Helmholtz Centre for Heavy Ion Research, Planckstrasse 1, 64291 Darmstadt (Germany); The University of Tokyo, 7-3-1 Hongo, Bunkyo-ku, Tokyo 113-0033 (Japan); Saito, T.R., E-mail: t.saito@gsi.de [GSI Helmholtz Centre for Heavy Ion Research, Planckstrasse 1, 64291 Darmstadt (Germany); Johannes Gutenberg-Universität Mainz, J.J. Becherweg 40, 55099 Mainz (Germany); The Helmholtz Institute Mainz (HIM), J.J. Becherweg 40, 55099 Mainz (Germany); Bertini, O. [GSI Helmholtz Centre for Heavy Ion Research, Planckstrasse 1, 64291 Darmstadt (Germany); Johannes Gutenberg-Universität Mainz, J.J. Becherweg 40, 55099 Mainz (Germany); Bianchin, S. [GSI Helmholtz Centre for Heavy Ion Research, Planckstrasse 1, 64291 Darmstadt (Germany); Bozkurt, V. [GSI Helmholtz Centre for Heavy Ion Research, Planckstrasse 1, 64291 Darmstadt (Germany); Nigde University, 51100 Nigde (Turkey); Kavatsyuk, M. [KVI, University of Groningen, Zernikelaan 25, NL-9747 AA Groningen (Netherlands); Ma, Y. [GSI Helmholtz Centre for Heavy Ion Research, Planckstrasse 1, 64291 Darmstadt (Germany); Johannes Gutenberg-Universität Mainz, J.J. Becherweg 40, 55099 Mainz (Germany); Maas, F. [GSI Helmholtz Centre for Heavy Ion Research, Planckstrasse 1, 64291 Darmstadt (Germany); Johannes Gutenberg-Universität Mainz, J.J. Becherweg 40, 55099 Mainz (Germany); The Helmholtz Institute Mainz (HIM), J.J. Becherweg 40, 55099 Mainz (Germany); and others

    2013-09-02

    A novel experiment, aiming at demonstrating the feasibility of hypernuclear spectroscopy with heavy ion beams, was conducted. Using the invariant mass method, the spectroscopy of hypernuclear products of {sup 6}Li projectiles on a carbon target at 2A GeV was performed. Signals of the Λ-hyperon and {sup 3}{sub Λ}H and {sup 4}{sub Λ}H hypernuclei were observed for final states of p+π{sup −}, {sup 3}He+π{sup −} and {sup 4}He+π{sup −}, respectively, with significance values of 6.7, 4.7 and 4.9σ. By analyzing the proper decay time from secondary vertex distribution with the unbinned maximum likelihood fitting method, their lifetime values were deduced to be 262{sub −43}{sup +56}±45 ps for Λ, 183{sub −32}{sup +42}±37 ps for {sup 3}{sub Λ}H, and 140{sub −33}{sup +48}±35 ps for {sup 4}{sub Λ}H.

  12. Improved neutron-gamma discrimination for a {sup 6}Li-glass neutron detector using digital signal analysis methods

    Energy Technology Data Exchange (ETDEWEB)

    Wang, C. L., E-mail: wangc@ornl.gov; Riedel, R. A. [Instrument and Source Division, Neutron Sciences Directorate, Oak Ridge National Laboratory, Oak Ridge, Tennessee 37831 (United States)

    2016-01-15

    A {sup 6}Li-glass scintillator (GS20) based neutron Anger camera was developed for time-of-flight single-crystal diffraction instruments at Spallation Neutron Source. Traditional Pulse-Height Analysis (PHA) for Neutron-Gamma Discrimination (NGD) resulted in the neutron-gamma efficiency ratio (defined as NGD ratio) on the order of 10{sup 4}. The NGD ratios of Anger cameras need to be improved for broader applications including neutron reflectometers. For this purpose, six digital signal analysis methods of individual waveforms acquired from photomultiplier tubes were proposed using (i) charge integration, (ii) pulse-amplitude histograms, (iii) power spectrum analysis combined with the maximum pulse-amplitude, (iv) two event parameters (a{sub 1}, b{sub 0}) obtained from a Wiener filter, (v) an effective amplitude (m) obtained from an adaptive least-mean-square filter, and (vi) a cross-correlation coefficient between individual and reference waveforms. The NGD ratios are about 70 times those from the traditional PHA method. Our results indicate the NGD capabilities of neutron Anger cameras based on GS20 scintillators can be significantly improved with digital signal analysis methods.

  13. Reactive and dissolved meteoric 10Be/9Be ratios in the Amazon basin

    Science.gov (United States)

    Wittmann, Hella; Dannhaus, Nadine; von Blanckenburg, Friedhelm; Bouchez, Julien; Suessenberger, Annette; Guyot, Jean-Loup; Maurice, Laurence; Filizola, Naziano; Gaillardet, Jerome; Christl, Marcus

    2014-05-01

    Recently, the ratio of the meteoric cosmogenic nuclide 10Be to stable 9Be has been established as a weathering and erosion proxy where meteoric 10Be/9Be ratios in reactive phases of secondary weathering products leached from detrital Amazonian river sediment were measured[1]. For this dataset, we derived a new 10Be-based mass balance, which compares the fluxes exported during erosion and weathering, Fout, calculated by the sum of [10Be]reac multiplied by gauging-derived sediment discharge and [10Be]dissmultiplied by water discharge, to the meteoric depositional flux Fin. This assessment allows evaluating the weathering state of the Amazon basin. Further, in order to assess equilibration of reactive phases in the water column, we measured (10Be/9Be)reac ratios leached from suspended sediments for two depth profiles of the Amazon (55m depth) and Madeira (12m depth) Rivers, their corresponding surface dissolved 10Be/9Be ratios, as well as dissolved ratios of smaller Amazon tributaries (Beni, Madre de Dios) to compare with published reactive ratios[1]. In these rivers, modest pH and salinity fluctuations help to constrain a 'simple' system that might however still be affected by seasonally changing isotopic compositions between water and suspended sediment[2] and seasonal fluctuations of TSS and TDS[3]. The 10Be-based mass balance shows that in Andean source areas Fout/Fin ≡1, indicating a balance between ingoing and exported flux, whereas in the Shield headwaters, Fout/Fin=0.3, indicating a combination of decay of 10Be during storage and little export of 10Be associated with particulate and dissolved loads. In central Amazonia, the export of 10Be decreases slightly relative to its atmospheric flux as evidenced by Fout/Fin=0.8 for the Amazon and Madeira Rivers. This value is interpreted as being close to steady state, but its modification could be due to additions of Shield-derived sediment to sediment carried in the main river[4]. Regarding the depth profiles, our

  14. Functions of MgH2 in hydrogen storage reactions of the 6LiBH4-CaH2 reactive hydride composite.

    Science.gov (United States)

    Zhou, Yifan; Liu, Yongfeng; Zhang, Yu; Gao, Mingxia; Pan, Hongge

    2012-08-28

    A significant improvement of hydrogen storage properties was achieved by introducing MgH(2) into the 6LiBH(4)-CaH(2) system. It was found that ~8.0 wt% of hydrogen could be reversibly stored in a 6LiBH(4)-CaH(2)-3MgH(2) composite below 400 °C and 100 bar of hydrogen pressure with a stepwise reaction, which is superior to the pristine 6LiBH(4)-CaH(2) and LiBH(4) samples. Upon dehydriding, MgH(2) first decomposed to convert to Mg and liberate hydrogen with an on-set temperature of ~290 °C. Subsequently, LiBH(4) reacted with CaH(2) to form CaB(6) and LiH in addition to further hydrogen release. Hydrogen desorption from the 6LiBH(4)-CaH(2)-3MgH(2) composite finished at ~430 °C in non-isothermal model, a 160 °C reduction relative to the 6LiBH(4)-CaH(2) sample. JMA analyses revealed that hydrogen desorption was a diffusion-controlled reaction rather than an interface reaction-controlled process. The newly produced Mg of the first-step dehydrogenation possibly acts as the heterogeneous nucleation center of the resultant products of the second-step dehydrogenation, which diminishes the energy barrier and facilitates nucleation and growth, consequently reducing the operating temperature and improving the kinetics of hydrogen storage.

  15. Differences Between a Single- and a Double-Folding Nucleus-^{9}Be Optical Potential

    Science.gov (United States)

    Bonaccorso, A.; Carstoiu, F.; Charity, R. J.; Kumar, R.; Salvioni, G.

    2016-05-01

    We have recently constructed two very successful n-^9Be optical potentials (Bonaccorso and Charity in Phys Rev C89:024619, 2014). One by the Dispersive Optical Model (DOM) method and the other (AB) fully phenomenological. The two potentials have strong surface terms in common for both the real and the imaginary parts. This feature makes them particularly suitable to build a single-folded (light-) nucleus-^9Be optical potential by using ab-initio projectile densities such as those obtained with the VMC method (Wiringa http://www.phy.anl.gov/theory/research/density/). On the other hand, a VMC density together with experimental nucleon-nucleon cross-sections can be used also to obtain a neutron and/or proton-^9Be imaginary folding potential. We will use here an ab-initio VMC density (Wiringa http://www.phy.anl.gov/theory/research/density/) to obtain both a n-^9Be single-folded potential and a nucleus-nucleus double-folded potential. In this work we report on the cases of ^8B, ^8Li and ^8C projectiles. Our approach could be the basis for a systematic study of optical potentials for light exotic nuclei scattering on such light targets. Some of the projectiles studied are cores of other exotic nuclei for which neutron knockout has been used to extract spectroscopic information. For those cases, our study will serve to make a quantitative assessment of the core-target part of the reaction description, in particular its localization.

  16. New method to evaluate the {sup 7}Li(p, n){sup 7}Be reaction near threshold

    Energy Technology Data Exchange (ETDEWEB)

    Herrera, María S., E-mail: herrera@tandar.cnea.gov.ar [Comisión Nacional de Energía Atómica, Av. Gral. Paz 1499, Buenos Aires B1650KNA (Argentina); Consejo Nacional de Investigaciones Científicas y Técnicas, Av. Rivadavia 1917, Ciudad Autónoma de Buenos Aires C1033AAJ (Argentina); Escuela de Ciencia y Tecnología, UNSAM, 25 de Mayo y Francia, Buenos Aires B1650KNA (Argentina); Moreno, Gustavo A. [YPF Tecnología, Baradero S/N, Buenos Aires 1925 (Argentina); Departamento de Física J. J. Giambiagi, Facultad de Ciencias Exactas y Naturales, UBA, Ciudad Universitaria, Ciudad Autónoma de Buenos Aires 1428 (Argentina); Kreiner, Andrés J. [Comisión Nacional de Energía Atómica, Av. Gral. Paz 1499, Buenos Aires B1650KNA (Argentina); Consejo Nacional de Investigaciones Científicas y Técnicas, Av. Rivadavia 1917, Ciudad Autónoma de Buenos Aires C1033AAJ (Argentina); Escuela de Ciencia y Tecnología, UNSAM, 25 de Mayo y Francia, Buenos Aires B1650KNA (Argentina)

    2015-04-15

    In this work a complete description of the {sup 7}Li(p, n){sup 7}Be reaction near threshold is given using center-of-mass and relative coordinates. It is shown that this standard approach, not used before in this context, leads to a simple mathematical representation which gives easy access to all relevant quantities in the reaction and allows a precise numerical implementation. It also allows in a simple way to include proton beam-energy spread affects. The method, implemented as a C++ code, was validated both with numerical and experimental data finding a good agreement. This tool is also used here to analyze scattered published measurements such as (p, n) cross sections, differential and total neutron yields for thick targets. Using these data we derive a consistent set of parameters to evaluate neutron production near threshold. Sensitivity of the results to data uncertainty and the possibility of incorporating new measurements are also discussed.

  17. Analysis of length distribution of short DNA fragments induced by 7Li ions using the random-breakage model

    Institute of Scientific and Technical Information of China (English)

    KONG Fuquan; ZHAO Kui; ZHAN Yong; CAO Tianguang; NI Meinan; SUI Li; CAI Minghui; ZHUO Yizhong

    2005-01-01

    Deoxyribonucleic acid (DNA) is an important bio-macromolecule. DNA double strand breaks (DSBs) are considered to be the most important initial damage responsible for all biological effects induced by ionizing radiation. In this paper the length distribution of DNA fragments induced by 7Li ionizing radiation is fitted with the random breakage model. In this model, the parameter u is the average number of DSBs on every DNA molecule induced by ionizing radiation. The fitting result shows that the random breakage model cannot describe the distribution of DNA fragments in lower doses, while the random breakage model is in better accordance with the experimental data in higher doses. It is shown that the length distribution of DNA fragments has random statistical feature in higher doses. In this situation, the random breakage model looks like a model without any parameter since the u has specific physical meaning and can directly be obtained from experimental data.

  18. Helium Bubbles Cavitation Phenomena in Pb-15.7Li and Potential Impact on Tritium Transport Behaviour in HCLL Breeding Channels

    Energy Technology Data Exchange (ETDEWEB)

    Sedano, L. A.

    2007-09-27

    COMPU task is devoted to develop a Process Flow Diagram (PFD) modelling tool for DEMO tritium cycle for HCLL and HCPB blanket lines for DEMO. At the actual stage of definition of HCLL blanket design line this global objective requires to progress specifically on the physical reliability of tritium transport assessments at blanket design level. A rough reliability assessment with the identify cation of physical phenomena determining permeation rates into the coolant was tentatively advanced in COMPU Task Deliverable 1. In HCLL design, the tritium diffusion in the alloy under the flow conditions and radiation effects in Pb15.7Li can be theoretically justifies ed as the rate limiting processes for tritium transfer into the coolant. This Deliverable 2 focuses on the analysis of a specific radiation effect: the potential role of helium bubbles in Pb15.7Li, the discussion of its implications on tritium assessment for HCLL design and consequently the analysis of its quantitative impact (as cycle input) on HCLL PFD tritium cycle design. Thus, the contents of this report investigate: (1) the rationality of the consideration on HCLL design of helium bubble cavitation phenomena in irradiated Pb15.7Li channels on the base of fundamental analysis (He solution states in Pb15.7Li) from empirical clues provided by Pb15.7Li irradiation tests, (2) a preliminary rough He-bubble cavitation design assessment and bases for a more precise FEM calculation for helium bubble cavitation phenomena in HCLL blanket channels, (3) the analysis of direct experimental data and numerical developments needed for a precise cavitation assessment and (4) a proposal of the lay-out and general specifications of an integral proof-of-principle Cavitation Experiment (Cevitex) of Helium in Pb15.7Li. (Author) 40 refs.

  19. Using the Doppler broadened γ line of the {sup 10}B(n,αγ){sup 7}Li reaction for thermal neutron detection

    Energy Technology Data Exchange (ETDEWEB)

    Ben-Galim, Y., E-mail: ybgx3@walla.com [Department of Nuclear Engineering, Ben Gurion University (BGU) of the Negev (Israel); Wengrowicz, U. [Department of Nuclear Engineering, Ben Gurion University (BGU) of the Negev (Israel); NRC-Negev, P.O. Box 9001, Beer-Sheva 84190 (Israel); Moreh, R. [Physics Department, Ben Gurion University (BGU) of the Negev, Beer-Sheva 84105 (Israel); Orion, I. [Department of Nuclear Engineering, Ben Gurion University (BGU) of the Negev (Israel); Raveh, A. [Advanced Coatings Center at Rotem Industries Ltd., MishorYamin D.N. Arava 86800 (Israel)

    2016-02-21

    When a thermal neutron is absorbed by {sup 10}B in the {sup 10}B(n,α){sup 7}Li reaction, there is a chance of 94% that a 478 keV photon be emitted by an excited {sup 7}Li nucleus. This reaction is exothermic with a Q-value of 2.31 MeV and the nuclei are emitted with kinetic energies of E(α)=1.47 MeV and E({sup 7}Li*)=0.84 MeV. This implies that the 478 keV γ line is emitted by a moving {sup 7}Li nucleus and hence is expected to be Doppler broadened. In the present work we suggest to use this broadening of the γ line as a fingerprint for the detection of thermal neutrons using a high resolution gamma spectrometer. We thus developed a Monte Carlo program using a MATLAB code based on a High Purity Germanium (HPGe) detector coupled with a Boron Carbide (B{sub 4}C) sheet to calculate the γ line broadening. Our simulation shows that the FWHM width of the resulting γ line is 12.6 keV, in good agreement with our measurement. Hence the broadened γ line emitted by the {sup 10}B(n,αγ){sup 7}Li reaction and detected by a HPGe detector shows that this method is an effective tool for neutron detection while maintaining good gamma discrimination. - Highlights: • Thermal neutron detection by measuring the Doppler broadened 478 keV γ line from the {sup 10}B(n,αγ){sup 7}Li interaction. • Natural Boron Carbide coupled with a HPGe detector were used in this study. • A mathematical Monte-Carlo model for the suggested detector was introduced. • A calibration tool for the suggested detector is introduced. • Experimental results show that the suggested method can be used for neutron detection.

  20. The knockout reaction of 15C on a 9Be target at intermediate energies

    Science.gov (United States)

    Sadeghi, H.; Fereidonnejad, R.; Ghambari, M.

    2016-05-01

    In this work, neutron knockout reactions of 15C on a 9Be target at energy 103 and 250 MeV/nucleon are studied. Using the Eikonal approximation of the Glauber model, total neutron removal cross sections, the stripping and diffractive cross sections as well as 14C longitudinal momentum distributions are determined in both 15C ground state and exited states of the wave function. We compared the results of our calculations with the available experimental data obtained recently. The calculated cross sections of 15C and 14C reactions, as well as the momentum distribution are in relatively good agreement with available data.

  1. Isovector and isoscalar dipole excitations in $^{9}$Be and $^{10}$Be studied with antisymmetrized molecular dynamics

    CERN Document Server

    Kanada-En'yo, Yoshik

    2015-01-01

    Isovector and isoscalar dipole excitations in $^9$Be and $^{10}$Be are investigated in the framework of antisymmetrized molecular dynamics, in which angular-momentum and parity projections are performed. In the present method, 1p-1h excitations on the ground state and large amplitude $\\alpha$-cluster mode are incorporated. The isovector giant dipole resonance (GDR) in $E>20$ MeV shows the two peak structure which is understood by the dipole excitation in the 2$\\alpha$ core part with the prolate deformation. Because of valence neutron modes against the $2\\alpha$ core, low-energy E1 resonances appear in $E20$ MeV.

  2. Breakup of 33.4 MeV/u 17N on a 9Be Target

    Institute of Scientific and Technical Information of China (English)

    HUA Hui; GUO Zhong-Yan; LI Zu-Yu; WANG Hong-Wei; WANG Su-Fang; JIANG Dong-Xing; LI Xiang-Qing; QIAN Tao; WU He-Yu; JIN Gen-Ming; ZHAN Wen-Long; DUAN Li-Min; XIAO Zhi-Guang

    2000-01-01

    Correlation measurements of neutrons and fragments have been performed in a reaction of 33.4 MeV/u 17 N on a 9Be target. Energy spectra of n and nitrogen fragments were obtained at different angles. Based on the nuclear diffraction dissociation model, the measured energy spectra and the neutron angular distributions werereproduced quite well assuming that 1 7 N was composed of 16 N and n or 15 N and 2n interacting with the nonlocal separable potential. The satisfactory agreement between the heoretical calculations and the experimental data shows that the contribution of Coulomb dissociation is negligible in the reaction concerned.

  3. Comparison of the effects of couplings to breakup channels in reactions induced by {sup 6}Li and {sup 6}He on the same {sup 64}Zn target

    Energy Technology Data Exchange (ETDEWEB)

    Fernández-García, J. P., E-mail: fernandez@lns.infn.it; Di Pietro, A.; Figuera, P.; Fisichella, M. [INFN, Laboratori Nazionali del Sud, via S. Sofia 62, 1-95123 Catania (Italy); Lattuada, M.; Musumarra, A.; Pellegriti, M. G.; Scuderi, V.; Torresi, D. [INFN, Laboratori Nazionali del Sud, via S. Sofia 62, 1-95123 Catania (Italy); Dipartamento di Fisica e Astronomia, via S. Sofia 64, I-95123 Catania (Italy); Moro, A. M. [Departamento de FAMN, Universidad de Sevilla, Apartado 1065, E-41080 Seville (Spain); Zadro, M. [Ruder Bošković Institute, Bijenička cesta 54, HR-10000 Zagreb (Croatia)

    2015-10-15

    The experimental elastic scattering angular distributions for the weakly bound nuclei {sup 6,7}Li and for the halo nucleus {sup 6}He on the same {sup 64}Zn target at several energies around the Coulomb barrier were measured at the Laboratori Nazionali del Sud (LNS, Italy) and at the Cyclotron Research Center, Louvain La Neuve (Belgium), respectively. The measured elastic scattering angular distributions of these three systems at the same center of mass energy have been compared. The experimental data of the {sup 6,7}Li+ {sup 64}Zn systems have been analyzed within the CDCC method, while the {sup 6}He+{sup 64}Zn data have been compared with both both CDCC and CRC calculations.

  4. A High-Precision Determination of the Astrophysical Rate for Production of ^9Be

    Science.gov (United States)

    Arnold, C. W.; Clegg, T. B.; Karwowski, H. J.; Rich, G. C.; Tompkins, J. R.; Howell, C. R.

    2010-11-01

    New cross section measurements of the astrophysically important ^9Be(γ,n) reaction have been made from 1.5 to 5.18 MeV. The measurements were made using the nearly monoenergetic circularly polarized γ-ray beam at Triangle Universities Nuclear Laboratory's High Intensity γ-ray Source. Measurements over narrow resonances employed beams with energy spread dE/E <= 1%. The energy-dependent absolute efficiency of the neutron counter used in this work was measured to ± 3% accuracy. New resonance parameters for the 4 lowest lying states in ^9Be were determined. A new reaction rate for α+ α+ n has been determined to better than ± 5%. The present rate is ˜ 25% larger than two widely accepted rates [1-2] in the temperature range important for r-process nucleosynthesis. The implications of this new rate on r-process and nuclear abundance predictions will be discussed.[4pt] [1] C. Angulo et al. Nuc. Phys. A 656 (1999) 3-183. [0pt] [2] K. Sumiyoshi et al. Nuc. Phys A 709 (2002) 467-486.

  5. The quadruple deformation effects of 9Be in heavy-ion reactions

    Science.gov (United States)

    Seyyedi, S. A.

    2016-11-01

    The effects of the projectile deformation and orientation on the total potential characteristic have been studied for the reactions between weakly bound nucleus, 9Be, as the projectile and different targets. In this paper, the double-folding model is used to calculate the nuclear potentials and deformation of projectile included. It is shown that applying the deformation effects can modify the potential barrier height and depth in the interior regions of the potential. It is also shown that the gradient variation of the potential barrier height is linearly increased when the angle between the projectile and the target nuclei increases. The rate of the variation is constant in different reactions with 9Be. In order to study the possible effect of these deformation dependent potentials, application is made in the calculation of cross-sections of the different reactions. It is observed that the deformation and orientation are of important role in the dynamics of such reactions and improve the agreement with the experimental results.

  6. Spectroscopy of high lying resonances in 9Be produced with radioactive 8Li beams

    Directory of Open Access Journals (Sweden)

    Lépine-Szily A.

    2014-04-01

    Full Text Available We present the results of the 8Li(p,α5He and 8Li(p,p8Li reactions measured at the RIBRAS (Radioactive Ion Beams in Brazil system. The experiment was realized in inverse kinematics using a thick [CH2]n polyethylene target and an incident 8Li beam, produced by RIBRAS. Using the thick target method, the complete excitation function could be measured between Ecm = 0.2 − 2.1 MeV, which includes the Gamow peak energy region. The excitation function of the 8Li(p,α5He reaction, populating resonances between 16.888 and 19.0 MeV in 9Be, was obtained[1] and the resonances were fitted using R-matrix calculations. This study shed light on spins, parities, partial widths and isospin values of high lying resonances in 9Be. The measurement of the resonant elastic scattering 8Li(p,p8Li populating resonances in the same energy region can constrain the resonance parameters. Preliminary results of the elastic scattering are also presented.

  7. Spectroscopy of high lying resonances in {sup 9}Be produced with radioactive {sup 8}Li beams

    Energy Technology Data Exchange (ETDEWEB)

    Lepini-Szily, A.; Leistenschneider, E.; Lichtenthäler, R.; Guimaraes, V.; Condori, R. Pampa; Scarduelli, V.; Rossi, E.; Zagatto, V.A.; Aguiar, V.A.P.; Duarte, J., E-mail: alinka@if.usp.br [Universidade de Sao Paulo (USP), Sao Paulo, SP (Brazil). Instituto de Fisica; Mendes Junior, D.R.; Faria, P.N. de; Santos, H. [Universidade Federal Fluminense (UFF), Niteroi, RJ (Brazil). Instituto de Fisica; Descouvemont, P. [Physique Nucleaire Theorique et Physique Mathematique, Universite Libre de Bruxelles (ULB), Brussels (Belgium); Barioni, A. [Universidade Federal da Bahia (UFBA), Salvador, BA (Brazil); Pires, K.C.C. [Universidade Tecnologica Federal do Parana (UFTPR), Cornelio Procopio, PR (Brazil); Morcelle, V. [Universidade Federal de Itajuba (UNIFEI), Itabira, MG (Brazil); Moraes, M.C. [Centro Brasileiro de Pesquisas Fisicas (CBPF), Rio de Janeiro, RJ (Brazil); Britos, T.; Assuncao, M. [Universidade Federal de Sao Paulo (UNIFESP), Diadema, SP (Brazil); Zamora, J.C. [Technische Universität Darmstadt, (Germany); Shorto, J.M.B. [Instituto de Pesquisas Energeticas e Nucleares (IPEN/CNEN-SP), Sao Paulo, SP (Brazil)

    2014-07-01

    We present the results of the {sup 8}Li(p,α){sup 5}He and {sup 8}Li(p,p){sup 8}Li reactions measured at the RIBRAS (Radioactive Ion Beams in Brazil) system. The experiment was realized in inverse kinematics using a thick [CH{sub 2}]{sub n} polyethylene target and an incident {sup 8}Li beam, produced by RIBRAS. Using the thick target method, the complete excitation function could be measured between E{sub cm} = 0.2 - 2.1 MeV, which includes the Gamow peak energy region. The excitation function of the {sup 8}Li(p,α){sup 5}He reaction, populating resonances between 16.888 and 19.0 MeV in {sup 9}Be, was obtained[1] and the resonances were fitted using R-matrix calculations. This study shed light on spins, parities, partial widths and isospin values of high lying resonances in {sup 9}Be. The measurement of the resonant elastic scattering {sup 8}Li(p,p){sup 8}Li populating resonances in the same energy region can constrain the resonance parameters. Preliminary results of the elastic scattering are also presented. (author)

  8. Viabilidad técnica para la explotación y separación isotópica de Li y prospectiva en el mercado de baterías de ION-7Li y de 6Li como material base de diseño en reactores de fusión nuclear

    OpenAIRE

    Herranz García, José Luis

    2013-01-01

    En claro alineamiento con estrategias de sostenibilidad en el uso de recursos naturales en un escenario constante de aumento de la demanda energética mundial, el desarrollo de la tecnología energética en la Historia de la Especie Humana muestra un vector de evolución permanente desde su origen en el sentido del desarrollo y uso de nuevas fuentes energéticas con la explotación de recursos naturales de manera más eficiente: soluciones energéticas con aumento de la densidad energética (exoenergí...

  9. Structural investigation of aryllithium clusters in solution. I. A 13C and 7Li NMR studyof phenyllithium and some methyl-substituted phenyllithium derivatives

    NARCIS (Netherlands)

    Koten, G. van; Wehman, E.; Jastrzebski, J.T.B.H.; Ernsting, J.M.; Grove, D.M.

    1988-01-01

    }1{}3{C and }7{Li NMR spectra of phenyllithium and several methyl subsituted phenyllithium derivatives have been recorded in the presence of known amounts of coordinating solvents such as monodentate diethyl ether and THF and the potentially bidentate TMEDA (tetramethylethylenediamine). The relative

  10. Breakup of 42 MeV 7Li projectiles in the fields of 12C and 197Au nuclei

    Indian Academy of Sciences (India)

    Dhruba Gupta; C Samanta; R Kanungo; P Basu; Subinit Roy; S Kailas; A Chatterjee; B J Roy; K Mahata; A Samant; A Shrivastava

    2001-07-01

    Inclusive cross sections of particles and tritons from the breakup of 42 MeV 7Li by 12C and 197Au targets are presented and analysed in the framework of the Serber model. Spectral distortions due to the targets and relevant reaction mechanisms are discussed.

  11. Experimental apparatus for quantum simulation with two-dimensional 9Be + Coulomb crystals

    Science.gov (United States)

    Pyka, Karsten; Ball, Harrison; McRae, Terry; Edmunds, Claire; Lee, Michael W.; Henderson, Samuel; Biercuk, Michael J.; Quantum Control Lab Team

    2015-03-01

    We report on the development of a new experimental setup designed for Quantum Simulation studies at a computationally relevant scale using laser-cooled 9Be + ion-crystals in a Penning trap. The trap geometry is optimized using numerical calculations for trapping large ion crystals with enhanced optical access and reduced anharmonic perturbations. Separate loading and spectroscopy zones prevent long term drifts of the trapping parameters due to contamination of the trap electrodes with Be deposits. Our customized superconducting magnet provides a homogenous (dB/B telecom wavelength fiber laser systems in the IR via nonlinear conversion. Our new approach employs high-efficiency telecom modulators and mode-selecting cavities to generate multiple beamlines from a single Sum-frequency-Generation step. Ultimately, this newly developed setup will allow for studies of many-body spin systems with tuneable interaction strength from infinite-range to nearest-neighbour type interaction.

  12. Isovector and isoscalar dipole excitations in 9Be and 10Be studied with antisymmetrized molecular dynamics

    Science.gov (United States)

    Kanada-En'yo, Yoshiko

    2016-02-01

    Isovector and isoscalar dipole excitations in 9Be and 10Be are investigated in the framework of antisymmetrized molecular dynamics, in which angular-momentum and parity projections are performed. In the present method, 1p-1h excitation modes built on the ground state and a large amplitude α -cluster mode are taken into account. The isovector giant dipole resonance (GDR) in E >20 MeV shows the two-peak structure, which is understood from the dipole excitation in the 2 α core part with the prolate deformation. Because of valence neutron modes against the 2 α core, low-energy E 1 resonances appear in E Thomas-Reiche-Kuhn sum rule and 10 % of the calculated energy-weighted sum. The dipole resonance at E ˜15 MeV in 10Be can be interpreted as the parity partner of the ground state having a 6He+α structure and has remarkable E 1 strength because of the coherent contribution of two valence neutrons. The isoscalar dipole strength for some low-energy resonances is significantly enhanced by the coupling with the α -cluster mode. For the E 1 strength of 9Be, the calculation overestimates the energy-weighted sum (EWS) in the low-energy (E <20 MeV) and GDR (20

  13. Upgrade of the POLDI diffractometer with a ZnS(Ag)/6LiF scintillation detector read out with WLS fibers coupled to SiPMs

    OpenAIRE

    Mosset, J. -B.; Stoykov, A.; Davydov, V.; Hildebrandt, M.; Van Swygenhoven, H.; W. Wagner

    2013-01-01

    A thermal neutron detector based on ZnS(Ag)/6LiF scintillator, wavelength-shifting fibers (WLS) and silicon photomultipliers (SiPM) is under development at the Paul Scherrer Institute (PSI) for upgrading the POLDI instrument, a pulse-overlap diffractometer. The design of the detector is outlined, and the measurements performed on a single channel prototype are presented. An innovative signal processing system based on a photon counting approach is under development. Its principle of operation...

  14. Characteristics of a thermal neutrons scintillation detector with the [ZnS(Ag)+$^6$LiF] at different conditions of measurements

    OpenAIRE

    Alekseenko, V. V.; Barabanov, I. R.; Etezov, R. A.; Gavrilyuk, Yu. M.; Gangapshev, A. M.; Gezhaev, A. M.; Kazalov, V. V.; Khokonov, A. Kh.; V.V. Kuzminov; Panasenko, S. I.; Ratkevich, S. S.

    2015-01-01

    A construction of a thermal neutron testing detector with a thin [ZnS(Ag)+$^6$LiF] scintillator is described. Results of an investigation of sources of the detector pulse origin and the pulse features in a ground and underground conditions are presented. Measurements of the scintillator own background, registration efficiency and a neutron flux at different objects of the BNO INR RAS were performed. The results are compared with the ones measured by the $^3$He proportional counter.

  15. Ultracold neutron detection with {sup 6}Li-doped glass scintillators. NANOSC: A fast ultracold neutron detector for the nEDM experiment at the Paul Scherrer Institute

    Energy Technology Data Exchange (ETDEWEB)

    Ban, G.; Lefort, T.; Lemiere, Y.; Naviliat-Cuncic, O.; Pierre, E.; Quemener, G.; Rogel, G. [Normandie Univ, ENSICAEN, UNICAEN, CNRS/IN2P3, LPC Caen, Caen (France); Bison, G.; Chowdhuri, Z.; Henneck, R.; Lauss, B.; Mtchedlishvili, A.; Schmidt-Wellenburg, P.; Zsigmond, G. [Paul Scherrer Institute, Villigen-PSI (Switzerland); Bodek, K.; Zejma, J. [Jagiellonian University, Marian Smoluchowski Institute of Physics, Cracow (Poland); Geltenbort, P. [Institut Laue-Langevin, Grenoble (France); Griffith, W.C.; Musgrave, M. [University of Sussex, Falmer, Department of Physics and Astronomy, Brighton (United Kingdom); Helaine, V. [Normandie Univ, ENSICAEN, UNICAEN, CNRS/IN2P3, LPC Caen, Caen (France); Paul Scherrer Institute, Villigen-PSI (Switzerland); Kasprzak, M.; Koss, P.A.; Severijns, N.; Wursten, E. [Katholieke Universiteit Leuven, Instituut voor Kernen Stralingsfysica, Leuven (Belgium); Kermaidic, Y.; Pignol, G.; Rebreyend, D. [LPSC, Universite Grenoble Alpes, CNRS/IN2P3, Grenoble (France); Kirch, K.; Komposch, S.; Krempel, J.; Ries, D. [Paul Scherrer Institute, Villigen-PSI (Switzerland); Institute for Particle Physics, ETH Zuerich, Zuerich (Switzerland); Kozela, A. [Henryk Niedwodniczanski Institute for Nuclear Physics, Cracow (Poland); Piegsa, F.M.; Rawlik, M. [Institute for Particle Physics, ETH Zuerich, Zuerich (Switzerland); Roccia, S. [CSNSM, Universite Paris Sud, CNRS/IN2P3, Orsay (France)

    2016-10-15

    This paper summarizes the results from measurements aiming to characterize ultracold neutron detection with {sup 6}Li-doped glass scintillators. Single GS10 or GS20 scintillators, with a thickness of 100-200μm, fulfill the ultracold neutron detection requirements with an acceptable neutron-gamma discrimination. This discrimination is clearly improved with a stack of two scintillators: a {sup 6}Li-depleted glass bonded to a {sup 6}Li-enriched glass. The technique of optical contact bonding is used between the two glasses in order to eliminate the need for optical glue or grease between them. Relative to a {sup 3}He Strelkov gas detector, the scintillator's detection efficiency is lower for UCN energies close to the scintillator's Fermi potential (85-100 neV), but becomes larger at higher UCN energies. Coupled to a digital data acquisition system, counting rates up to a few 10{sup 5} counts/s can be handled. A detector based on such a scintillator stack arrangement was built and has been used in the neutron electric dipole moment experiment at the Paul Scherrer Institute since 2010. Its response for routine runs of the neutron electric dipole moment experiment is presented. (orig.)

  16. Ultracold neutron detection with 6Li-doped glass scintillators, NANOSC: a fast ultracold neutron detector for the nEDM experiment at the Paul Scherrer Institute

    CERN Document Server

    Ban, G; Bodek, K; Chowdhuri, Z; Geltenbort, P; Griffith, W C; Hélaine, V; Henneck, R; Kasprzak, M; Kermaidic, Y; Kirch, K; Komposch, S; Koss, P A; Kozela, A; Krempel, J; Lauss, B; Lefort, T; Lemière, Y; Mtchedlishvili, A; Musgrave, M; Naviliat-Cuncic, O; Piegsa, F M; Pierre, E; Pignol, G; Quéméner, G; Rawlik, M; Ries, D; Rebreyend, D; Roccia, S; Rogel, G; Schmidt-Wellenburg, P; Severijns, N; Wursten, E; Zejma, J; Zsigmond, G

    2016-01-01

    This paper summarizes the results from measurements aiming to characterize ultracold neutron detection with 6Li-doped glass scintillators. Single GS10 or GS20 scintillators, with a thickness of 100-200 micrometer, fulfill the ultracold neutron detection requirements with an acceptable neutron-gamma discrimination. This discrimination is clearly improved with a stack of two scintillators: a 6Li-depleted glass bonded to a 6Li-enriched glass. The optical contact bonding is used between the scintillators in order to obtain a perfect optical contact. The scintillator's detection efficiency is similar to that of a 3He Strelkov gas detector. Coupled to a digital data acquisition system, counting rates up to a few 10^5 counts/s can be handled. A detector based on such a scintillator stack arrangement was built and has been used in the neutron electric dipole moment experiment at the Paul Scherrer Institute since 2010. Its response for the regular runs of the neutron electric dipole moment experiment is presented.

  17. Ultracold neutron detection with 6Li-doped glass scintillators. NANOSC: A fast ultracold neutron detector for the nEDM experiment at the Paul Scherrer Institute

    Science.gov (United States)

    Ban, G.; Bison, G.; Bodek, K.; Chowdhuri, Z.; Geltenbort, P.; Griffith, W. C.; Hélaine, V.; Henneck, R.; Kasprzak, M.; Kermaidic, Y.; Kirch, K.; Komposch, S.; Koss, P. A.; Kozela, A.; Krempel, J.; Lauss, B.; Lefort, T.; Lemière, Y.; Mtchedlishvili, A.; Musgrave, M.; Naviliat-Cuncic, O.; Piegsa, F. M.; Pierre, E.; Pignol, G.; Quéméner, G.; Rawlik, M.; Ries, D.; Rebreyend, D.; Roccia, S.; Rogel, G.; Schmidt-Wellenburg, P.; Severijns, N.; Wursten, E.; Zejma, J.; Zsigmond, G.

    2016-10-01

    This paper summarizes the results from measurements aiming to characterize ultracold neutron detection with 6Li-doped glass scintillators. Single GS10 or GS20 scintillators, with a thickness of 100-200μm, fulfill the ultracold neutron detection requirements with an acceptable neutron-gamma discrimination. This discrimination is clearly improved with a stack of two scintillators: a 6Li-depleted glass bonded to a 6Li-enriched glass. The technique of optical contact bonding is used between the two glasses in order to eliminate the need for optical glue or grease between them. Relative to a 3He Strelkov gas detector, the scintillator's detection efficiency is lower for UCN energies close to the scintillator's Fermi potential (85-100 neV), but becomes larger at higher UCN energies. Coupled to a digital data acquisition system, counting rates up to a few 105 counts/s can be handled. A detector based on such a scintillator stack arrangement was built and has been used in the neutron electric dipole moment experiment at the Paul Scherrer Institute since 2010. Its response for routine runs of the neutron electric dipole moment experiment is presented.

  18. Excitation function shape and neutron spectrum of the 7Li(p ,n )7Be reaction near threshold

    Science.gov (United States)

    Martín-Hernández, Guido; Mastinu, Pierfrancesco; Maggiore, Mario; Pranovi, Lorenzo; Prete, Gianfranco; Praena, Javier; Capote-Noy, Roberto; Gramegna, Fabiana; Lombardi, Augusto; Maran, Luca; Scian, Carlo; Munaron, Enrico

    2016-09-01

    The forward-emitted low energy tail of the neutron spectrum generated by the 7Li(p ,n )7Be reaction on a thick target at a proton energy of 1893.6 keV was measured by time-of-flight spectroscopy. The measurement was performed at BELINA (Beam Line for Nuclear Astrophysics) of the Laboratori Nazionali di Legnaro. Using the reaction kinematics and the proton on lithium stopping power the shape of the excitation function is calculated from the measured neutron spectrum. Good agreement with two reported measurements was found. Our data, along with the previous measurements, are well reproduced by the Breit-Wigner single-resonance formula for s -wave particles. The differential yield of the reaction is calculated and the widely used neutron spectrum at a proton energy of 1912 keV was reproduced. Possible causes regarding part of the 6.5% discrepancy between the 197Au(n ,γ ) cross section measured at this energy by Ratynski and Kappeler [Phys. Rev. C 37, 595 (1988), 10.1103/PhysRevC.37.595] and the one obtained using the Evaluated Nuclear Data File version B-VII.1 are given.

  19. Dynamical 3-Space Predicts Hotter Early Universe: Resolves CMB-BBN 7-Li and 4-He Abundance Anomalies

    Directory of Open Access Journals (Sweden)

    Cahill R. T.

    2010-01-01

    Full Text Available The observed abundances of 7-Li and 4-He are significantly inconsistent with the predictions from Big Bang Nucleosynthesis (BBN when using the $Lambda$CDM cosmological model together with the value for $Omega_B h^2 = 0.0224pm0.0009$ from WMAP CMB fluctuations, with the value from BBN required to fit observed abundances being $0.009 < Omega_B h^2 < 0.013$. The dynamical 3-space theory is shown to predict a 20% hotter universe in the radiation-dominated epoch, which then results in a remarkable parameter-free agreement between the BBN and the WMAP value for $Omega_B h^2$. The dynamical 3-space also gives a parameter-free fit to the supernova redshift data, and predicts that the flawed $Lambda$CDM model would require $Omega_Lambda = 0.73$ and $Omega_M = 0.27$ to fit the 3-space dynamics Hubble expansion, and independently of the supernova data. These results amount to the discovery of new physics for the early universe that is matched by numerous other successful observational and experimental tests.

  20. Dynamical 3-Space Predicts Hotter Early Universe: Resolves CMB-BBN 7-Li and 4-He Abundance Anomalies

    Directory of Open Access Journals (Sweden)

    Cahill R. T.

    2010-01-01

    Full Text Available The observed abundances of 7 Li and 4 He are significantly inconsistent with the pre- dictions from Big Bang Nucleosynthesis (BBN when using the CDM cosmolog- ical model together with the value for B h 2 = 0 : 0224 0 : 0009 from WMAP CMB fluctuations, with the value from BBN required to fit observed abundances being 0 : 009 < B h 2 < 0 : 013. The dynamical 3-space theory is shown to predict a 20% hot- ter universe in the radiation-dominated epoch, which then results in a remarkable parameter-free agreement between the BBN and the WMAP value for B h 2 . The dy- namical 3-space also gives a parameter-free fit to the supernova redshift data, and pre- dicts that the flawed CDM model would require = 0 : 73 and M = 0 : 27 to fit the 3-space dynamics Hubble expansion, and independently of the supernova data. These results amount to the discovery of new physics for the early universe that is matched by numerous other successful observational and experimental tests.

  1. Measurement of Nuclear Reaction Q-values with High Accuracy: 7Li(p, n)7Be

    Science.gov (United States)

    White, R. E.; Barker, P. H.; Lovelock, D. M. J.

    1985-01-01

    A technique is described for the measurement of nuclear reaction Q-values with an accuracy of a few parts in 105, in which the ultimate reference is a one-volt standard. As a test of the technique the accurately known threshold energy of the 7Li(p, n)7Be reaction, 1880.51 +/- 0.08 keV, has been remeasured. The value found using the present technique is 1880.443 +/- 0.020 keV, in good agreement with previous values. An attempt to see evidence for atomic excitation effects in the 27A1(p,n)27Si reaction is also discussed. This yielded a new value of 5803.73 +/- 0.12 keV for the threshold of this reaction, again in a good agreement with, but more accurate than, previous values. Further test measurements are summarized. The main application of the technique, in measurements related to the theory of weak interactions, is discussed briefly and the results obtained to date are presented.

  2. Study of 11Be on 9Be one neutron transfer reactions at TRIUMF ISAC-II

    Science.gov (United States)

    Braid, Ryan; (Pcb)2 Collaboration; Tigress Collaboration

    2016-09-01

    The structure of neutron-rich Beryllium isotopes displays interesting properties arising from the interplay of alpha clustering and valence neutrons, leading in some cases to halo nuclei. In this presentation, preliminary results of the 11Be on 9Be reaction at 55 MeV and 30.14 MeV leading to two interesting exit channels will be shown, the first one enabling the study of 12Be and the second the study of 10Be. This reaction has advantages over the traditional (d,p) or (d,t) methods, since the reactants are equal in mass they both scatter in a detectable angular range. Additionally, TIGRESS allows precise γ-tagging for the excited states. Some challenges in analysis include the 10Be degeneracy, a large n breakup signature, and multiple particle excitation. The data and ongoing analysis will be presented. This work is partially supported by the US Department of Energy through Grant/Contract No. DE-FG03- 93ER40789 (Colorado School of Mines).

  3. Accurate Analytic Potential Energy Function and Spectroscopic Study for G1 ∏g State of Dimer 7Li2

    Institute of Scientific and Technical Information of China (English)

    SHI De-Heng; MA Heng; SUN Jin-Feng; ZHU Zun-Lue

    2007-01-01

    The reasonable dissociation limit for the G1∏g state of dimer 7Li2 is determined. The equilibrium internuclear distance, dissociation energy, harmonic frequency, vibrational zero energy, and adiabatic excitation energy are calculated using a symmetry-adapted-cluster configuration-interaction method in complete active space in Gaussian03 program package at such numerous basis sets as 6-311++G, 6-311++G(2df, 2pd), 6-311++G(2df, p), cc-PVTZ, 6-311++G(3df, 3pd), CEP-121G, 6-311++G(2df, pd), 6-311++G(d,p),6-311G(3df,3pd), D95(3df,3pd), 6-311++G(3df, 2p),6-311++G(2df), 6-311++G(df, pd) D95V++, and DGDZVP. The complete potential energy curves are obtained at these sets over a wide internuclear distance range and have least squares fitted to Murrell-Sorbie function. The conclusion shows that the basis set 6-311++G(2df, p) is a most suitable one for the G1∏g state. At this basis set, the calculated spectroscopic constants Te, De, Eo, Re, ωe, ωeXe, αe, and Be are of 3.9523 eV, 0.813 06 eV, 113.56 cm-1, 0.320 15 nm,227.96 cm-1, 1.6928 cm-1, 0.004 436 cm-1, and 0.4689 cm-1, respectively, which are in good agreement with measurements whenever available. The total 50 vibrational levels and corresponding inertial rotation constants are for the first time calculated and compared with available RKR data. And good agreement with measurements is obtained.

  4. Neutron beam optimization based on a 7Li(p,n)7Be reaction for treatment of deep-seated brain tumors by BNCT

    Science.gov (United States)

    Zahra Ahmadi, Ganjeh; S. Farhad, Masoudi

    2014-10-01

    Neutron beam optimization for accelerator-based Boron Neutron Capture Therapy (BNCT) is investigated using a 7Li(p,n)7Be reaction. Design and optimization have been carried out for the target, cooling system, moderator, filter, reflector, and collimator to achieve a high flux of epithermal neutron and satisfy the IAEA criteria. Also, the performance of the designed beam in tissue is assessed by using a simulated Snyder head phantom. The results show that the optimization of the collimator and reflector is critical to finding the best neutron beam based on the 7Li(p,n)7Be reaction. Our designed beam has 2.49×109n/cm2s epithermal neutron flux and is suitable for BNCT of deep-seated brain tumors.

  5. Charge transfer in Li/CFx-silver vanadium oxide hybrid cathode batteries revealed by solid state 7Li and 19F nuclear magnetic resonance spectroscopy

    Science.gov (United States)

    Sideris, Paul J.; Yew, Rowena; Nieves, Ian; Chen, Kaimin; Jain, Gaurav; Schmidt, Craig L.; Greenbaum, Steve G.

    2014-05-01

    Solid state 7Li and 19F magic angle spinning nuclear magnetic resonance (MAS NMR) experiments are conducted on several cathodes containing CFx-Silver vanadium oxide (CFx-Ag2V4O11) hybrid cathodes discharged to 50% depth of discharge (DoD) and stored at their open-circuit voltage for a period of one and three months. Three carbonaceous sources for the CFx phase are investigated: petroleum coke-based, fibrous, and mixed fibrous. For each hybrid cathode, a measurable increase in the relative amount of lithium fluoride is observed after a three month resting period in both the 7Li and 19F NMR spectra. These changes are attributed to lithium ion migration from the silver vanadium oxide to the CFx phase during the resting period, and help clarify the mechanism behind high power handling capability of this cathode.

  6. Indirect determination of Li via 74Ge(n,γ)75mGe activation reaction induced by neutrons from 7Li(p,n)7Be reaction

    Science.gov (United States)

    Kumar, Sanjiv; Reddy, G. L. N.; Rao, Pritty; Verma, Rakesh; Ramana, J. V.; Vikramkumar, S.; Raju, V. S.

    2012-03-01

    An indirect method to determine Li by 74Ge(n,γ)75mGe activation reaction induced in a high purity Ge (detector) crystal by neutrons from the 7Li(p,n)7Be reaction in a typical particle-induced γ-ray emission (PIGE) spectroscopy experimental set-up is described. Performed with proton beams of energies in excess of 1.88 MeV, the threshold energy (Eth) of the 7Li(p,n)7Be reaction, the determination involves the activity measurement of 75mGe isotope that has a half-life of 47.7 s and decays with the emission of 139 keV γ-rays. Rapidity, selectivity and sensitivity down to ppm levels are the attractive features of the method. It is a suitable alternative to 7Li(p,p'γ)7Li reaction based PIGE technique in the analyses of matrices that contain light elements such as Be, B, F, Na and Al in significant proportions. Interferences can arise from elements, for example V and Ti, that have Eth ⩽ 1.88 MeV for (p,n) reaction. In the case of elements such as Cu, Mo which have with Eth > 1.88 MeV, the incident proton beam energy can be judiciously selected to avoid or minimize an interference. The method, under optimized irradiation conditions, does not entail a risk of neutron stimulated degradation of the performance of the detector. Besides analytical purposes, the measurement of the 75mGe activity can serve as a powerful tool to monitor even low (˜25 n/cm2 s) thermal neutron fluxes.

  7. Synthesis and optical characterization of LiKB4O7, Li2B6O10, and LiCsB6O10 glasses

    Energy Technology Data Exchange (ETDEWEB)

    Adamiv, V.; Teslyuk, I.; Dyachok, Ya.; Romanyuk, G.; Krupych, O.; Mys, O.; Martynyuk-Lototska, I.; Burak, Ya.; Vlokh, R.

    2010-10-01

    In the current work we report on the synthesis of LiKB4O7, Li2B6O10, and LiCsB6O10 borate glasses. The results for their piezo-optic, acousto-optic, acoustic, elastic, refractive, optical transmission, and optical resistance properties are also presented. It is shown that some of these glasses represent efficient acousto-optic materials that are transparent down to the vacuum ultraviolet range and highly resistant to laser radiation.

  8. Synthesis and optical characterization of LiKB4O7, Li2B6O10, and LiCsB6O10 glasses.

    Science.gov (United States)

    Adamiv, V; Teslyuk, I; Dyachok, Ya; Romanyuk, G; Krupych, O; Mys, O; Martynyuk-Lototska, I; Burak, Ya; Vlokh, R

    2010-10-01

    In the current work we report on the synthesis of LiKB(4)O(7), Li(2)B(6)O(10), and LiCsB(6)O(10) borate glasses. The results for their piezo-optic, acousto-optic, acoustic, elastic, refractive, optical transmission, and optical resistance properties are also presented. It is shown that some of these glasses represent efficient acousto-optic materials that are transparent down to the vacuum ultraviolet range and highly resistant to laser radiation.

  9. Optical Potential Parameters for Halo Nucleus System 6He+12C from Transfer Reaction11B (7Li, 6He) 12C

    Institute of Scientific and Technical Information of China (English)

    WU Zhen-Dong; XU Xin-Xing; BAI Chun-Lin; YU Ning; JIA Fei; LIN Cheng-Jian; ZHANG Huan-Qiao; LIU Zu-Hua; YANG Feng; AN Guang-Peng; ZHANG Chun-Lei; ZHANG Gao-Long; JIA Hui-Ming

    2009-01-01

    The optical potential parameters for the halo nucleus system 6He+12 C are extracted from fits to the measured angular distributions of 11B(7 Li, 6He)12C reaction at energies of 18.3 and 28.3 MeV with distorted-wave Born approximation analysis. The characters of the obtained optical potential parameters are basically consistent with the results extracted from the fits to the elastic-scattering angular distributions in the literature.

  10. Effects of first-order correction to eikonal approximation in the analysis of {sup 9}Be({sup 15}C,{sup 14}C + n){sup 9}Be stripping reaction

    Energy Technology Data Exchange (ETDEWEB)

    Singh, M. [TERII, Department of Applied Sciences (India); Kharab, R., E-mail: kharabrajesh@rediffmail.com [Kurukshetra University, Department of Physics (India); Singh, R. M. [Ch. Devi Lal University, Department of Physics (India)

    2015-09-15

    We have studied the effects of the first-order correction to the eikonal approximation for {sup 9}Be({sup 15}C,{sup 14}C + n){sup 9}Be stripping reactions at 54A MeV incident energy and have found that the correction term slightly changes the tail of the longitudinal momentum distribution of the core fragment.

  11. Cross-section measurements for {sup 239}Pu(n,f) and {sup 6}Li(n,{alpha}) with a lead slowing-down spectrometer

    Energy Technology Data Exchange (ETDEWEB)

    Rochman, D. [National Nuclear Data Center, Brookhaven National Laboratory, Upton, NY 11973-5000 (United States)]. E-mail: drochman@bnl.gov; Haight, R.C. [Los Alamos National Laboratory, Los Alamos, NM 87545 (United States)]. E-mail: haight@lanl.gov; O' Donnell, J.M. [Los Alamos National Laboratory, Los Alamos, NM 87545 (United States)]. E-mail: odonnell@lanl.gov; Wender, S.A. [Los Alamos National Laboratory, Los Alamos, NM 87545 (United States)]. E-mail: wender@lanl.gov; Vieira, D.J. [Los Alamos National Laboratory, Los Alamos, NM 87545 (United States)]. E-mail: vieira@lanl.gov; Bond, E.M. [Los Alamos National Laboratory, Los Alamos, NM 87545 (United States)]. E-mail: bond@lanl.gov; Bredeweg, T.A. [Los Alamos National Laboratory, Los Alamos, NM 87545 (United States)]. E-mail: toddb@lanl.gov; Wilhelmy, J.B. [Los Alamos National Laboratory, Los Alamos, NM 87545 (United States)]. E-mail: j_wilhelmy@lanl.gov; Granier, T. [Commissariat a l' Energie Atomique, 91680 Bruyeres-le-Chatel (France)]. E-mail: granier@cea.fr; Ethvignot, T. [Commissariat a l' Energie Atomique, 91680 Bruyeres-le-Chatel (France)]. E-mail: ethvignot@cea.fr; Petit, M. [Commissariat a l' Energie Atomique, 91680 Bruyeres-le-Chatel (France)]. E-mail: petit@cea.fr; Danon, Y. [Rensselaer Polytechnic Institute, Troy, NY 12180 (United States)]. E-mail: danony@rpi.edu; Romano, C. [Rensselaer Polytechnic Institute, Troy, NY 12180 (United States)]. E-mail: romanc2@rpi.edu

    2006-08-01

    We present fission cross-section measurements with {approx}10ng of {sup 239}Pu performed using the LANSCE Lead Slowing-Down Spectrometer. Results of Li6(n,{alpha}) measurements with a sample size of 760ng of {sup 6}Li are also reported. This technical achievement demonstrates the feasibility of measuring neutron-induced fission cross-section on samples with 10ng of fissile actinides that are available on ultra-small quantities. Furthermore, results on neutron-induced alpha emission show that measurements for astrophysics purposes are feasible with the LSDS.

  12. Cross-section measurements for 239Pu(n,f) and 6Li(n, α) with a lead slowing-down spectrometer

    Science.gov (United States)

    Rochman, D.; Haight, R. C.; O'Donnell, J. M.; Wender, S. A.; Vieira, D. J.; Bond, E. M.; Bredeweg, T. A.; Wilhelmy, J. B.; Granier, T.; Ethvignot, T.; Petit, M.; Danon, Y.; Romano, C.

    2006-08-01

    We present fission cross-section measurements with ˜10 ng of 239Pu performed using the LANSCE Lead Slowing-Down Spectrometer. Results of Li6(n,α) measurements with a sample size of 760 ng of 6Li are also reported. This technical achievement demonstrates the feasibility of measuring neutron-induced fission cross-section on samples with 10 ng of fissile actinides that are available on ultra-small quantities. Furthermore, results on neutron-induced alpha emission show that measurements for astrophysics purposes are feasible with the LSDS.

  13. Digital signal processing for a thermal neutron detector using ZnS(Ag):6LiF scintillating layers read out with WLS fibers and SiPMs

    OpenAIRE

    Mosset, J. -B.; Stoykov, A.; Greuter, U.; Hildebrandt, M.; Schlumpf, N.

    2015-01-01

    We present a digital signal processing system based on a photon counting approach which we developed for a thermal neutron detector consisting of ZnS(Ag):6LiF scintillating layers read out with WLS fibers and SiPMs. Three digital filters have been evaluated: a moving sum, a moving sum after differentiation and a digital CR-RC^4 filter. The performances of the detector with these filters are presented. A full analog signal processing using a CR-RC^4 filter has been emulated digitally. The dete...

  14. Search for $^6_\\Lambda$H hypernucleus by the $^6$Li$(\\pi^-,K^+)$ reaction at $p_{\\pi^-}$ = 1.2 GeV/$c$

    CERN Document Server

    Sugimura, H; Ahn, J K; Ajimura, S; Akazawa, Y; Amano, N; Aoki, K; Bhang, H C; Chiga, N; Endo, M; Evtoukhovitch, P; Feliciello, A; Fujioka, H; Fukuda, T; Hasegawa, S; Hayakawa, S; Honda, R; Hosomi, K; Hwang, S H; Ichikawa, Y; Igarashi, Y; Imai, K; Ishibashi, N; Iwasaki, R; Joo, C W; Kiuchi, R; Lee, J K; Lee, J Y; Matsuda, K; Matsumoto, Y; Matsuoka, K; Miwa, K; Mizoi, Y; Moritsu, M; Nagae, T; Nagamiya, S; Nakagawa, M; Naruki, M; Noumi, H; Ota, R; Roy, B J; Saha, P K; Sakaguchi, A; Sako, H; Samanta, C; Samoilov, V; Sasaki, Y; Sato, S; Sekimoto, M; Shimizu, Y; Shiozaki, T; Shirotori, K; Soyama, T; Takahashi, T; Takahashi, T N; Tamura, H; Tanabe, K; Tanaka, T; Tanida, K; Tokiyasu, A O; Tsamalaidze, Z; Ukai, M; Yamamoto, T O; Yamamoto, Y; Yang, S B; Yoshida, K

    2014-01-01

    We have carried out an experiment to search for a neutron-rich hypernucleus, $^6_{\\Lambda}$H, by the $^6$Li($\\pi^-,K^+$) reaction at $p_{\\pi^-}$ =1.2 GeV/$c$. The obtained missing mass spectrum with an estimated energy resolution of 3.2 MeV (FWHM) showed no peak structure corresponding to the $^6_{\\Lambda}$H hypernucleus neither below nor above the $^4_{\\Lambda}$H$+2n$ particle decay threshold. An upper limit of the production cross section for the bound $^6_{\\Lambda}$H hypernucleus was estimated to be 1.2 nb/sr at 90% confidence level.

  15. Breakup coupling effects on near-barrier inelastic scattering of the weakly bound {sup 6}Li projectile on a {sup 144}Sm target

    Energy Technology Data Exchange (ETDEWEB)

    Woodard, A.E., E-mail: awoodard@nd.edu [Laboratorio Tandar, Comision Nacional de Energia Atomica, B1650KNA San Martin, Buenos Aires (Argentina); Figueira, J.M. [Laboratorio Tandar, Comision Nacional de Energia Atomica, B1650KNA San Martin, Buenos Aires (Argentina); Consejo Nacional de Investigaciones Cientificas y Tecnicas, C1033AAJ Ciudad de Buenos Aires (Argentina); Otomar, D.R. [Instituto de Fisica, Universidade Federal Fluminense, Gragoata, Niteroi, R. J., 24210-340 (Brazil); Fernandez Niello, J.O. [Laboratorio Tandar, Comision Nacional de Energia Atomica, B1650KNA San Martin, Buenos Aires (Argentina); Consejo Nacional de Investigaciones Cientificas y Tecnicas, C1033AAJ Ciudad de Buenos Aires (Argentina); Escuela de Ciencia y Tecnologia, Universidad de San Martin, B1650BWA San Martin, Buenos Aires (Argentina); Lubian, J. [Instituto de Fisica, Universidade Federal Fluminense, Gragoata, Niteroi, R. J., 24210-340 (Brazil)

    2012-01-01

    Angular distributions for the inelastic scattering of the weakly bound {sup 6}Li nucleus from a {sup 144}Sm target (associated with the contributions of both the 2{sub 1}{sup +} and 3{sub 1}{sup -144}Sm excited states together) were measured at bombarding energies close to the Coulomb barrier. The experimental data were compared with expected results based on continuum discretized coupled-channel (CDCC) calculations. The results confirm that it is essential to include continuum-continuum couplings to reproduce the experimental data. The analysis demonstrates that inelastic scattering data can be a critical tool in testing full CDCC calculations involving weakly bound nuclei.

  16. Digital signal processing for a thermal neutron detector using ZnS(Ag):6LiF scintillating layers read out with WLS fibers and SiPMs

    Science.gov (United States)

    Mosset, J.-B.; Stoykov, A.; Greuter, U.; Hildebrandt, M.; Schlumpf, N.

    2016-07-01

    We present a digital signal processing system based on a photon counting approach which we developed for a thermal neutron detector consisting of ZnS(Ag):6LiF scintillating layers read out with WLS fibers and SiPMs. Three digital filters have been evaluated: a moving sum, a moving sum after differentiation and a digital CR-RC4 filter. The performances of the detector with these filters are presented. A full analog signal processing using a CR-RC4 filter has been emulated digitally. The detector performance obtained with this analog approach is compared with the one obtained with the best performing digital approach.

  17. Digital signal processing for a thermal neutron detector using ZnS(Ag):6LiF scintillating layers read out with WLS fibers and SiPMs

    CERN Document Server

    Mosset, J -B; Greuter, U; Hildebrandt, M; Schlumpf, N

    2015-01-01

    We present a digital signal processing system based on a photon counting approach which we developed for a thermal neutron detector consisting of ZnS(Ag):6LiF scintillating layers read out with WLS fibers and SiPMs. Three digital filters have been evaluated: a moving sum, a moving sum after differentiation and a digital CR-RC^4 filter. The performances of the detector with these filters are presented. A full analog signal processing using a CR-RC^4 filter has been emulated digitally. The detector performance obtained with this analog approach is compared with the one obtained with the best performing digital approach.

  18. Test of special relativity theory by means of laser spectroscopy on relativistic {sup 7}Li{sup +} ions in the ESR; Test der Speziellen Relativitaetstheorie mittels Laserspektroskopie an relativistischen {sup 7}Li{sup +}-Ionen am ESR

    Energy Technology Data Exchange (ETDEWEB)

    Botermann, Benjamin

    2012-10-31

    The invariance under Lorentz transformation of the laws of physics is a fundamental postulate of modern physics and all theories of the fundamental interactions have been stated in a covariant form. Although the theory of Special Relativity (SR) has been tested and confirmed with high accuracy in a large number of experiments, improved tests are of fundamental interest due to the far-reaching relevance of this postulate. Additionally modern attempts of a unified description of the four fundamental interactions point to possible violations of Lorentz invariance. In this context experiments of the Ives-Stilwell type for a test of time dilation play an important role. High resolution laser spectroscopy is applied on relativistic particle beams to investigate the validity of the relativistic Doppler formula - and therefore of the time dilation factor γ. In the course of this thesis an Ives-Stilwell experiment was performed with {sup 7}Li{sup +} ions at a velocity of 34 % of the speed of light, which were stored at the experimental storage ring (ESR) of the GSI Helmholtzzentrum fuer Schwerionenforschung. The techniques of Λ- as well as saturation spectroscopy were employed on the 1s2s{sup 3}S{sub 1}→1s2p{sup 3}P{sub 2} transition. By a computer based analysis of the fluorescence detection system and utilization of appropriate edge filters the signal to noise ratio was decisively improved and the application of an additional pump laser allowed for the observation of a saturation signal for the first time. The frequency stability of both laser systems was specified by means of a frequency comb to obtain the highest possible accuracy. The data from the beam times were analyzed in the frameworks of the Robertson-Mansouri-Sexl test theory (RMS) and the Standard Model Extension (SME) and the corresponding upper limits of the relevant test parameters of the assigned theories were calculated. The upper limit of the parameter α was improved by a factor of 4 compared to

  19. Evidence for a dynamically refracted primary bow in weakly bound $^9$Be rainbow scattering from $^{16}$O

    CERN Document Server

    Ohkubo, S

    2016-01-01

    We present for the first time evidence for the existence of a dynamically refracted primary bow for $^{9}$Be+$^{16}$O scattering. This is demonstrated through the use of coupled channel calculations with an extended double folding potential derived from the density-dependent effective two-body force and precise microscopic cluster wave functions for $^{9}$Be. The calculations reproduce the experimental Airy structure in $^{9}$Be+$^{16}$O scattering well.It is found that coupling of a weakly bound $^{9}$Be nucleus to excited states plays the role of a booster lens, dynamically enhancing the refraction over the {\\it static} refraction due to the Luneburg lens mean field potential between the ground states of $^{9}$Be and $^{16}$O.

  20. Measurement of differential cross sections and cross sections of the 6Li(n, t)4He reaction in the 1-2MeV energy range%1-2 MeV能区6Li(n,t)4He反应微分截面与截面的实验测量

    Institute of Scientific and Technical Information of China (English)

    张国辉; 陈金象; 唐国有; Gledenov Yu M; Sedysheva M; Khuukhenkhuu G

    2006-01-01

    利用屏栅电离室对1.05、1.54及2.25 MeV中子6Li(n,t)4He反应的微分截面与截面进行了实验测量.采用氚固体靶的T(p,n)3He反应产生准单能中子,用相对效率已知的BF3长中子管和238U裂变片相结合来测定绝对中子通量.将测量结果与已有数据进行了比较,1-2 MeV能区6Li(n,t)4He反应截面的分歧在一定程度上得到了澄清.

  1. Natural Abundance 17O, 6Li NMR and Molecular Modeling Studies of the Solvation Structures of Lithium bis(fluorosulfonyl)imide/1,2-dimethoxyethane Liquid Electrolytes

    Energy Technology Data Exchange (ETDEWEB)

    Wan, Chuan; Hu, Mary Y.; Borodin, Oleg; Qian, Jiangfeng; Qin, Zhaohai; Zhang, Jiguang; Hu, Jian Z.

    2016-03-01

    Natural abundance 17O and 6Li NMR experiments, quantum chemistry and molecular dynamics studies were employed to investigate the solvation structures of Li+ at various concentrations of LiFSI in DME electrolytes in an effort to solve this puzzle. It was found that the chemical shifts of both 17O and 6Li changed with the concentration of LiFSI, indicating the changes of solvation structures with concentration. For the quantum chemistry calculations, the coordinated cluster LiFSI(DME)2 forms at first, and its relative ratio increases with increasing LiFSI concentration to 1 M. Then the solvation structure LiFSI(DME) become the dominant component. As a result, the coordination of forming contact ion pairs between Li+ and FSI- ion increases, but the association between Li+ and DME molecule decreases. Furthermore, at LiFSI concentration of 4 M the solvation structures associated with Li+(FSI-)2(DME), Li+2(FSI-)(DME)4 and (LiFSI)2(DME)3 become the dominant components. For the molecular dynamics simulation, with increasing concentration, the association between DME and Li+ decreases, and the coordinated number of FSI- increases, which is in perfect accord with the DFT results. These results provide more insight on the fundamental mechanism on the very high CE of Li deposition in these electrolytes, especially at high current density conditions.

  2. Simultaneous sub-Doppler laser cooling of fermionic $^6$Li and $^{40}$K on the D$_1$ line: Theory and Experiment

    CERN Document Server

    Sievers, Franz; Kretzschmar, Norman; Fernandes, Diogo Rio; Suchet, Daniel; Rabinovic, Michael; Parker, Colin V; Khaykovich, Lev; Salomon, Christophe; Chevy, Frédéric

    2014-01-01

    We report on simultaneous sub-Doppler laser cooling of fermionic $^6$Li and $^{40}$K using the D$_1$ optical transitions. We compare experimental results to a numerical simulation of the cooling process applying a semi-classical Monte Carlo wavefunction method. The simulation takes into account the three dimensional optical molasses setup and the dipole interaction between atoms and the bichromatic light field driving the D$_1$ transitions. We discuss the physical mechanisms at play, we identify the important role of coherences between the ground state hyperfine levels and compare D$_1$ and D$_2$ sub-Doppler cooling. In 5 ms, the D$_1$ molasses phase largely reduces the temperature for both $^6$Li and $^{40}$K at the same time, with a final temperature of 44 $\\mu$K and 11 $\\mu$K, respectively. For both species this leads to a phase-space density close to $10^{-4}$. These conditions are well suited to directly load an optical or magnetic trap for efficient evaporative cooling to quantum degeneracy.

  3. Ab initio calculations on the a3∑+u state properties of dimer 7Li2

    Institute of Scientific and Technical Information of China (English)

    Shi De-Heng; Sun Jin-Feng; Zhu Zun-Lue; Liu Yu-Fang

    2007-01-01

    The comparison between single-point energy scanning (SPES) and geometry optimization (OPT) in determining the equilibrium geometry of the a3∑u+ state for 7Li2 is made at numerous basis sets such as 6-311++G(2df), cc-PVTZ,6-311++G(2df, p), 6-311G(3df,3pd), 6-311++G(2df,2pd), D95(3df, 3pd), 6-311++G, DGDZVP, 6-311++G(3df,2pd),6-311G(2df,2pd), D95V++, CEP-121G, 6-311++G(d,p), 6-311++G(2df, pd) and 6-311++G(3df,3pd) in full active space using a symmetry-adapted-cluster/ symmetry-adapted-cluster configuration-interaction (SAC/SAC-CI) method presented in Gaussian03 program package. The difference of the equilibrium geometries obtained by SPES and by OPT is reported. Analyses show that the results obtained by SPES are more reasonable than those obtained by OPT. We have calculated the complete potential energy curves at these sets over a wide internuclear distance range from about 3.0a0to 37.0a0, and the conclusion is that the basis set cc-PVTZ is the most suitable one. With the potential obtained at cc-PVTZ, the spectroscopic data (Te, De, Do, ωe, ωeχe, αe and Be) are computed and they are 1.006 eV, 338.71 cm-1,307.12 cm-1, 64.88 cm-1, 3.41 cm-1, 0.0187 cm-1 and 0.279 cm-1, respectively, which are in good agreement with recent measurements. The total 11 vibrational states are found at J=0. Their corresponding vibrational levels and classical turning points are computed and compared with available RKR data, and good agreement is found. One inertial rotation constant (By) and six centrifugal distortion constants (Dy Hv, Lv, My, Nv and Ov) are calculated.The scattering length is calculated to be -27.138a0, which is in good accord with the experimental data.

  4. Simultaneous measurement of angular distribution of elastic scattering for {sup 6}Li, {sup 7}Be, and {sup 8}B in {sup 58}Ni; Medida simultanea de Distribuciones Angulares de Dispersion Elastica para {sup 6}Li, {sup 7}Be, y {sup 8}B en {sup 58}Ni

    Energy Technology Data Exchange (ETDEWEB)

    Ruiz S, A. [Facultad de Ciencias, UAEM, Toluca, Estado de Mexico (Mexico); Martinez Q, E.; Aguilera R, E.F.; Murillo O, G.; Lizcano C, D.; Gomez C, A. [Departamento de Aceleradores, ININ, 52750 La Marquesa, Estado de Mexico (Mexico)

    2007-07-01

    The experimental angular distributions of elastic scattering for the projectiles {sup 6}Li, {sup 7}Be, {sup 8}B in {sup 58}Ni were obtained. Using the Optical model with a Woods-Saxon potential form, as much for the real part as for the imaginary one, an adjustment to the experimental data varying only the depth of the imaginary part of the potential is made. A comparison of the results obtained for each projectile is made. (Author)

  5. Elastic and inelastic scattering of {sup 15}N ions by {sup 9}Be at 84 MeV

    Energy Technology Data Exchange (ETDEWEB)

    Rudchik, A.T., E-mail: rudchik@kinr.kiev.ua [Institute for Nuclear Research, Ukrainian Academy of Sciences, Prospect Nauki 47, 03680 Kyiv (Ukraine); Chercas, K.A. [Institute for Nuclear Research, Ukrainian Academy of Sciences, Prospect Nauki 47, 03680 Kyiv (Ukraine); Kemper, K.W. [Physics Department, Florida State University, Tallahassee, FL 32306-4350 (United States); Rusek, K. [Heavy Ion Laboratory of Warsaw University, ul. L. Pasteura 5A, PL-02-093 Warsaw (Poland); Rudchik, A.A.; Herashchenko, O.V. [Institute for Nuclear Research, Ukrainian Academy of Sciences, Prospect Nauki 47, 03680 Kyiv (Ukraine); Koshchy, E.I. [Kharkiv National University, pl. Svobody 4, 61077 Kharkiv (Ukraine); Pirnak, Val.M. [Institute for Nuclear Research, Ukrainian Academy of Sciences, Prospect Nauki 47, 03680 Kyiv (Ukraine); Piasecki, E.; Trzcińska, A. [Heavy Ion Laboratory of Warsaw University, ul. L. Pasteura 5A, PL-02-093 Warsaw (Poland); Sakuta, S.B. [Russian Research Center “Kurchatov Institute”, Kurchatov Sq. 1, 123182 Moscow (Russian Federation); Siudak, R. [H. Niewodniczański Institute of Nuclear Physics, Polish Academy of Sciences, ul. Radzikowskiego 152, PL-31-342 Cracow (Poland); Strojek, I. [National Center for Nuclear Researches, ul. Hoża 69, PL-00-681 Warsaw (Poland); Stolarz, A. [Heavy Ion Laboratory of Warsaw University, ul. L. Pasteura 5A, PL-02-093 Warsaw (Poland); Ilyin, A.P.; Ponkratenko, O.A.; Stepanenko, Yu.M.; Shyrma, Yu.O. [Institute for Nuclear Research, Ukrainian Academy of Sciences, Prospect Nauki 47, 03680 Kyiv (Ukraine); Szczurek, A. [H. Niewodniczański Institute of Nuclear Physics, Polish Academy of Sciences, ul. Radzikowskiego 152, PL-31-342 Cracow (Poland); Uleshchenko, V.V. [Institute for Nuclear Research, Ukrainian Academy of Sciences, Prospect Nauki 47, 03680 Kyiv (Ukraine)

    2016-03-15

    Angular distributions of the {sup 9}Be + {sup 15}N elastic and inelastic scattering were measured at E{sub lab}({sup 15}N) = 84 MeV (E{sub c.m.} = 31.5 MeV) for the 0–6.76 MeV states of {sup 9}Be and 0–6.32 MeV states of {sup 15}N. The data were analyzed within the optical model and coupled-reaction-channels method. The elastic and inelastic scattering, spin reorientations of {sup 9}Be in ground and excited states and {sup 15}N in excited states as well as the most important one- and two-step transfer reactions were included in the channels-coupling scheme. The parameters of the {sup 9}Be + {sup 15}N optical potential of Woods–Saxon form as well as deformation parameters of these nuclei were deduced. The analysis showed that the {sup 9}Be + {sup 15}N pure potential elastic scattering dominates at the forward angles whereas the ground state spin reorientation of {sup 9}Be gives a major contribution to the elastic scattering cross sections at the large angles. Contributions from particle transfers are found to be negligible for the present scattering system.

  6. Two-stage magneto-optical trapping and narrow-line cooling of $^6$Li atoms to high phase-space density

    CERN Document Server

    Sebastian, Jimmy; Li, Ke; Gan, Huat Chai Jaren; Li, Wenhui; Dieckmann, Kai

    2014-01-01

    We report an experimental study of peak and phase-space density of a two-stage magneto-optical trap (MOT) of 6-Li atoms, which exploits the narrower $2S_{1/2}\\rightarrow 3P_{3/2}$ ultra-violet (UV) transition at 323 nm following trapping and cooling on the more common D2 transition at 671 nm. The UV MOT is loaded from a red MOT and is compressed to give a high phase-space density up to $3\\times 10^{-4}$. Temperatures as low as 33 $\\mu$K are achieved on the UV transition. We study the density limiting factors and in particular find a value for the light-assisted collisional loss coefficient of $1.3 \\pm0.4\\times10^{-10}\\,\\textrm{cm}^3/\\textrm{s}$ for low repumping intensity.

  7. Angular Distribution and Cross Section Measurement of the 6Li(3He,n8B Reaction at 5.8 MeV

    Directory of Open Access Journals (Sweden)

    Cinausero M.

    2014-03-01

    Full Text Available The reaction 6Li(3He,n8B was studied at Laboratori Nazionali di Legnaro in the framework of the EUROnu Design Study for a Beta Beam facility at CERN. The 8B production cross section was determined through neutron angular distribution by using the time-of-flight technique. Thanks to the high statistics achieved, the neutron angular distribution for the population of the 8B first excited state has been measured for the first time. Discrepancies with other available data sets for 8B ground state population are discussed and interpreted in the framework of DWBA calculations. Further measurements at beam energies above 10 MeV are needed to clarify the behaviour of the angular distribution

  8. A reanalysis of radioisotope measurements of the $^9$Be$(\\gamma,n)^8$Be cross-section

    CERN Document Server

    Robinson, Alan E

    2016-01-01

    The $^9$Be$(\\gamma,n)^8$Be reaction is enhanced by a near threshold $1/2^+$ state. Contradictions between existing measurements of this reaction cross-section affect calculations of astrophysical r-process yields, dark matter detector calibrations, and the theory of the nuclear structure of $^9$Be. Select well-documented radioisotope $^9$Be$(\\gamma,n)$ source yield measurements have been reanalyzed, providing a set of high-accuracy independently measured cross sections. A Breit-Wigner fit of these corrected measurements yields $E_R=1738.8^{+5.0}_{-4.2}$~keV, $\\Gamma_\\gamma=0.771^{+0.055}_{-0.044}$~eV, and $\\Gamma_n=268^{+40}_{-33}$~keV for the $1/2^+$ state. The fit favors a resonant $1/2^+$ state, but a virtual state is not excluded.

  9. Lithium ion micrometer diffusion in a garnet-type cubic Li7La3Zr2O12 (LLZO) studied using 7Li NMR spectroscopy

    Science.gov (United States)

    Hayamizu, Kikuko; Seki, Shiro; Haishi, Tomoyuki

    2017-01-01

    Mobile lithium ions in a cubic garnet Li7La3Zr2O12 (Al-stabilized) were studied using 7Li NMR spectroscopy for membrane and powder samples, the latter of which was ground from the membrane. Lithium diffusion in a micrometer space was measured using the pulsed-gradient spin-echo 7Li NMR method between 70 and 130 °C. When the observation time (Δ ) was shorter than 20 ms, the echo attenuation showed diffusive diffraction patterns, indicating that the Li+ diffusing space is not free but restricted. For longer Δ, the values of apparent diffusion constant (Dapparent) became gradually smaller to approach an equilibrated value (close to a tracer diffusion constant). In addition, the Dapparent depends on the pulse field gradient strength (g) and became smaller as g became larger. These experimental results suggest that the lithium ions diffuse through Li+ pathways surrounded by stationary anions and lithium ions, and are affected by collisions and diffractions. One-dimensional profiles of the membrane sample of thickness 0.5 mm were observed from 65 to 110 °C and the area intensity, as well as the lithium occurrence near the surface, increased with the increase in temperature. The temperature-dependent area intensity showed a correspondence to the number of Li+ carrier ions estimated from the ionic conductivity and the equilibrated diffusion constant through the Nernst-Einstein relationship.

  10. The 181Ta(7Li,5n)183Os reaction: Measurement and analysis of the excitation function and isomeric cross-section ratios

    Science.gov (United States)

    Ismail, M.; Sharma, R. P.; Rashid, M. H.

    1998-03-01

    Excitation function and isomeric cross-section ratios for the production of 183Osm,g by 7Li-induced reactions on 181Ta are obtained from the measurements of the residual activities by the conventional stacked-foils technique from threshold to 50 MeV. The excitation function and isomeric cross-section ratios for nuclear reaction 181Ta(7Li,5n)183Osm,g are compared with the theoretical statistical model calculation by using the ALICE/91, STAPRE, and CASCADE codes. In the energy range of the present measurement the excitation functions are fitted fairly well by both the geometry dependent hybrid (GDH) model and the hybrid model of Blann with initial exciton number n0=7 (nn=4, np=3, nh=0) using the ALICE/91 code. The experimental isomeric cross-section ratios are also reproduced fairly well by the calculation using the STAPRE code. However, the CASCADE code calculations slightly underpredict the cross section but reproduce the shape. In general, the statistical model under a suitable set of global assumptions, can reproduce the excitation function as well as isomeric cross-section ratios.

  11. $\\gamma$ -spectroscopy of n-rich $^{95,96}$Rb nuclei by the incomplete fusion reaction of $^{94}$Kr on $^{7}$Li

    CERN Multimedia

    We propose an experiment with MINIBALL coupled to T-REX to investigate n-rich $^{95,96}$Rb nuclei by the incomplete fusion reaction of $^{94}$Kr on $^{7}$Li. The nuclei of interest will be populated by transfer of a triton into $^{94}$Kr, forming the excited $^{97}$Rb nucleus, followed by the emission of an alpha particle, which will be detected in the Si telescopes of T-REX. The $^{97}$Rb product will evaporate 1 or 2 (with the highest probability) neutrons leading to $^{96}$Rb or $^{95}$Rb, respectively. The aim of the experiment is twofold: \\\\ i) to perform a $\\gamma$- spectroscopy study of $^{95,96}$Rb nuclei with N=58,59, the structure of which is of particular interest in investigating the transition towards stable deformation at N=60, \\\\ ii) to acquire experience in using incomplete fusion reactions with the weakly bound $^{7}$Li target, in order to perform, at a later stage with HIE-ISOLDE, similar measurements induced by n-rich radioactive beams of Sn and Hg, for which at least 5 MeV/nucleon are need...

  12. Experimental studies on the neutron emission spectrum and induced radioactivity of the sup 7 Li(d,n) reaction in the 20-40 MeV region

    CERN Document Server

    Baba, M; Hagiwara, M; Sugimoto, M; Miura, T; Kawata, N; Yamadera, A; Orihara, H

    2002-01-01

    To improve the data accuracy of the neutron emission spectrum of the sup 7 Li(d,n) reaction and the radioactivity ( sup 7 Be, sup 3 H, etc.) accumulated in the sup 7 Li target in IFMIF, we have measured the neutron emission spectrum and the radioactivity of sup 7 Be induced in the lithium target for 25 MeV deuterons at the Tohoku University AVF cyclotron (K=110) facility. Neutron spectra were measured with the time-of-flight (TOF) method at four laboratory angles by using a beam swinger system and a well collimated TOF channel. Induced radioactivity was measured by detecting the gamma-rays from sup 7 Be with a pure Ge detector. Experimental results are compared with other experimental data. The present result of neutron emission spectra are in qualitative agreement with other experimental data but that of sup 7 Be production was much larger than expected by the recent codes. Measurement will be extended to several incident energies up to 40 MeV.

  13. Experimental studies on the neutron emission spectrum and induced radioactivity of the {sup 7}Li(d,n) reaction in the 20-40 MeV region

    Energy Technology Data Exchange (ETDEWEB)

    Baba, M. E-mail: babam@cyric.tohoku.ac.jp; Aoki, T.; Hagiwara, M.; Sugimoto, M.; Miura, T.; Kawata, N.; Yamadera, A.; Orihara, H

    2002-12-01

    To improve the data accuracy of the neutron emission spectrum of the {sup 7}Li(d,n) reaction and the radioactivity ({sup 7}Be, {sup 3}H, etc.) accumulated in the {sup 7}Li target in IFMIF, we have measured the neutron emission spectrum and the radioactivity of {sup 7}Be induced in the lithium target for 25 MeV deuterons at the Tohoku University AVF cyclotron (K=110) facility. Neutron spectra were measured with the time-of-flight (TOF) method at four laboratory angles by using a beam swinger system and a well collimated TOF channel. Induced radioactivity was measured by detecting the gamma-rays from {sup 7}Be with a pure Ge detector. Experimental results are compared with other experimental data. The present result of neutron emission spectra are in qualitative agreement with other experimental data but that of {sup 7}Be production was much larger than expected by the recent codes. Measurement will be extended to several incident energies up to 40 MeV.

  14. Formation of ultracold 7Li85Rb molecules in the lowest triplet electronic state by photoassociation and their detection by ionization spectroscopy

    Science.gov (United States)

    Altaf, Adeel; Dutta, Sourav; Lorenz, John; Pérez-Ríos, Jesús; Chen, Yong P.; Elliott, D. S.

    2015-03-01

    We report the formation of ultracold 7Li85Rb molecules in the a3Σ+ electronic state by photoassociation (PA) and their detection via resonantly enhanced multiphoton ionization (REMPI). With our dual-species Li and Rb magneto-optical trap apparatus, we detect PA resonances with binding energies up to ˜62 cm-1 below the 7Li 2s 2S1/2 + 85Rb 5p 2P1/2 asymptote. In addition, we use REMPI spectroscopy to probe the a3Σ+ state and excited electronic 33Π and 43Σ+ states and identify a3Σ+ (v″ = 7-13), 33Π (vΠ' = 0-10), and 43Σ+ (vΣ' = 0-5) vibrational levels. Our line assignments agree well with ab initio calculations. These preliminary spectroscopic studies on previously unobserved electronic states are crucial to discovering transition pathways for transferring ultracold LiRb molecules created via PA to deeply bound rovibrational levels of the electronic ground state.

  15. Corrosion resistance of Al-based coatings in flowing Pb–15.7Li produced by aluminum electrodeposition from ionic liquids

    Directory of Open Access Journals (Sweden)

    Sven-Erik Wulf

    2016-12-01

    Full Text Available Reduced activation ferritic–martensitic steels are intended to serve as structural materials in different blanket designs, e.g. HCLL, DCLL and WCLL. In these designs the material is supposed to be in direct contact with the flowing liquid breeder material Pb–15.7Li at an operating temperature of up to 550°C. These conditions will lead to severe corrosion attack of the steel and high corrosion rates of up to 400µm per year are reported in the literature. To avoid or reduce corrosion Al-based corrosion barriers were developed in the last years by using electrochemical techniques to deposit aluminum. Until now two processes have been developed. The first one, so called ECA process, is based on volatile toluene electrolytes. Long-term corrosion experiments on these coatings indicated reduced corrosion rates compared to bare Eurofer steel in flowing Pb–15.7Li. However, these Fe–Al scales showed inhomogeneous corrosion attack of the corrosion barrier itself. In this study the improved ECX process was applied to produce Al-based coatings. The short-term corrosion behavior of such barrier coatings was analyzed for up to 4000h by diameter measurements and metallographic examinations. The investigation revealed uniform corrosion in comparison to inhomogeneous attack in case of ECA coated samples and reduced corrosion rates of around 20µm/a even for low exposure times of 4000h.

  16. Measurement of $^{7}$Be(n,$\\alpha$)$^{4}$He and $^{7}$Be(n,p)$^{7}$Li cross-sections for the Cosmological Lithium Problem

    CERN Multimedia

    We propose to measure in the second experimental area of n TOF the $^{7}$Be(n,$\\alpha$)$^{4}$He and $^{7}$Be(n,p)$^{7}$Li reaction in a wide energy range. Both reactions are of interest for the long- standing "Cosmological $^{7}$Li problem" in Big Bang Nucleosynthesis (BBN). The very high specific activity of $^{7}$Be, and the low cross section of the (n,$\\alpha$) reaction make this measurement extremely dicult. As afirst step, we request some beam time for detector tests at EAR2. For the $^{7}$Be(n,p) reaction, previously measured up to 13 keV, the diculty is mostly associated withthe availability of a high-purity $^{7}$Be sample. To this purpose we ask for three shifts of offline ISOLDE mass separation for the preparation of the sample to be used at n TOF. To this end, a prior endorsement by INTC of the scientific validity and feasibility of the proposed measurement is requested, to start activity on the sample production. The present proposal is part of a wider collaborative effort aimed at measuring neutr...

  17. Production of {sup 6}He and {sup 9}Be by radiative capture and four-body recombination

    Energy Technology Data Exchange (ETDEWEB)

    Diego, R. de [Universidade de Lisboa, Centro de Fisica Nuclear, Lisboa (Portugal); Garrido, E. [CSIC, Instituto de Estructura de la Materia, Madrid (Spain); Fedorov, D.V.; Jensen, A.S. [Aarhus University, Department of Physics and Astronomy, Aarhus (Denmark)

    2014-06-15

    In this work we estimate the production rates for the three-body radiative capture processes α + n + n → {sup 6}He + γ and α + α + n → {sup 9}Be + γ, as well as the four-body recombination reactions α + α + n + n → {sup 6}He + α, α + n + n + n → {sup 6}He + n, α + α + n + n → {sup 9}Be + n and α + α + α + n → {sup 9}Be + α. These processes compete as a source of {sup 6}He and {sup 9}Be. The hyperspherical adiabatic expansion method is used. With this method no assumption is made about the capture mechanism. Both sequential and direct capture are included. The production rates for the radiative and the four-body recombination processes are found to be comparable for a mass density of about 10{sup 7}g/cm{sup 3} (∝ 10{sup 30} neutrons/cm{sup 3}) and temperatures of a few GK. (orig.)

  18. Ca(AlH4)2, CaAlH5, and CaH2+6LiBH4: Calculated dehydrogenation enthalpy, including zero point energy, and the structure of the phonon spectra

    NARCIS (Netherlands)

    Marashdeh, A.; Frankcombe, T.J.

    2008-01-01

    The dehydrogenation enthalpies of Ca(AlH4)2, CaAlH5, and CaH2+6LiBH4 have been calculated using density functional theory calculations at the generalized gradient approximation level. Harmonic phonon zero point energy (ZPE) corrections have been included using Parlinski’s direct method. The dehydrog

  19. Lithium diffusion in a new cathode material Li0.8[Ni0.6Sb0.4]O2 studied by 7Li NMR

    Directory of Open Access Journals (Sweden)

    Salikhov T., Klysheva E., Zvereva E., Nalbandyan V., Shukaev I., Medvedev B., Vavilova E.

    2016-12-01

    Full Text Available A rhombohedral layered α-NaFeO2-type compound, Lix[Ni(1+x/3Sb(2-x/3]O2 (x=0.8 has been prepared from the sodium analogue by ion exchange at 570 K. In contrast to the stoichiometric composition Li3Ni2SbO6, it shows considerable Li/Ni inversion and no long-range Ni/Sb ordering. The temperature dependence of the 7Li NMR spin-lattice relaxation rate and linewidth data measured at temperature range from 30-450 K show the sharp increase of lithium ions mobility comparing to the stoichiometric compound Li3Ni2SbO6. From the NMR data the activation energy was estimated by different methods.

  20. In situ7Li and 133Cs nuclear magnetic resonance investigations on the role of Cs+ additive in lithium-metal deposition process

    Science.gov (United States)

    Hu, Jian Zhi; Zhao, Zhenchao; Hu, Mary Y.; Feng, Ju; Deng, Xuchu; Chen, Xilin; Xu, Wu; Liu, Jun; Zhang, Ji-Guang

    2016-02-01

    Cesium ion (Cs+) has been reported to be an effective electrolyte additive to suppress Li dendrite growth which prevents the application of lithium (Li) metal as an anode for rechargeable Li batteries. In this work, we investigated the effect of Cs+ additive on Li depositions using quantitative in situ7Li and 133Cs nuclear magnetic resonance (NMR) with planar symmetric Li cells. It's found that the addition of Cs+ can significantly enhance both the formation of well aligned Li nanorods and reversibility of the Li electrode. In situ133Cs NMR directly confirms that Cs+ migrates to Li electrode to form a positively charged electrostatic shield during the charging process. Much more electrochemical "active" Li was found in Li films deposited with Cs+ additive, while more electrochemical "dead" and thicker Li rods were identified in Li films deposited without Cs+. Combining the in situ and the previous ex-situ results, a Li deposition model has been proposed to explain these observations.

  1. Ab initio calculations of accurate dissociation energy and analytic potential energy function for the second excited state B1П of 7LiH

    Institute of Scientific and Technical Information of China (English)

    Shi De-Heng; Liu Yu-Fang; Sun Jin-Feng; Zhu Zun-Lùe; Yang Xiang-Dong

    2006-01-01

    The reasonable dissociation limit of the second excited singlet state B1П of 7LiH molecule is obtained. The obtained over the internuclear distance ranging from about 0.10 nm to 0.54 nm, and has a least-square fit to the analytic compared with previous theoretical results. The equilibrium internuclear distance obtained by geometry optimization is found to be quite different from that obtained by single-point energy scanning under the same calculation condition.comparison of the theoretical calculations of dissociation energies, equilibrium interatomic distances and the analytic potential energy function with those obtained by previous theoretical results clearly shows that the present work is more theories.

  2. A Comprehensive Theoretical Analysis of 6,7Li + 64Zn Elastic Scattering in a Wide Angular Range Around the Coulomb Barrier

    Science.gov (United States)

    Ibraheem, Awad A.; Aygun, M.

    2016-08-01

    In this paper, the elastic scattering angular distributions of 6,7Li on 64Zn have been investigated by using various nuclear potentials. For this, we use the phenomenological Woods-Saxon potential, the real double folding potential with the density-independent M3Y effective interaction supplemented with an imaginary part in Woods-Saxon form and the double folding potentials multiplied with a normalization factor of the real and imaginary parts via the density-independent and CDM3Y6 density-dependent versions of the M3Y effective interaction have been used. The results have been compared with each other as well as with the experimental data. It has been observed that the agreement between the theoretical results and earlier reported data is perfect. Finally, the change of the total reaction cross sections with energy has been investigated.

  3. Measurements of neutron energy spectra from 7Li(p,n)7Be reaction with Bonner sphere spectrometer, Nested Neutron Spectrometer and ROSPEC.

    Science.gov (United States)

    Atanackovic, J; Matysiak, W; Witharana, S; Dubeau, J; Waker, A J

    2014-10-01

    Neutron spectrometry measurements were carried out at the McMaster Accelerator Laboratory (MAL), which is equipped with a 3-MV Van de Graaff-type accelerator. Protons were accelerated onto a thick natural lithium target inducing the (7)Li(p,n)(7)Be threshold reaction. Depending on the proton energy, slightly different poly-energetic neutron fields were produced. Neutron spectra were measured at two incident proton energies: 2.15 and 2.24 MeV, which produced poly-energetic neutrons with maximum kinetic energies of 401 and 511 keV, respectively. Measurements were performed at a distance of 1.5 m from the target in the forward direction with three different instruments: Bonner sphere spectrometer, Nested Neutron Spectrometer and ROtational proton recoil SPECtrometer.

  4. Fuskite® preliminary experimental tests based on permeation against vacuum for hydrogen recovery as a potential application in Pb15.7Li loop systems.

    Energy Technology Data Exchange (ETDEWEB)

    Sacristán, R., E-mail: mrosa.sacristan@sener.es [SENER Ingeniería y Sistemas, C/ Provença 392, 5a, 08025 Barcelona (Spain); Veredas, G. [EURATOM-CIEMAT Fusion Assoc., Fusion Technology Division, Av. Complutense 40, 28040 Madrid (Spain); Bonjoch, I. [SENER Ingeniería y Sistemas, C/ Provença 392, 5a, 08025 Barcelona (Spain); Peñalva, I. [UPV/EHU, Departamento de Ingeniería Nuclear y Mecánica de Fluidos, Alameda de Urquijo s/n, 48013 Bilbao (Spain); Calderón, E. [SENER Ingeniería y Sistemas, C/ Provença 392, 5a, 08025 Barcelona (Spain); Alberro, G. [UPV/EHU, Departamento de Ingeniería Nuclear y Mecánica de Fluidos, Alameda de Urquijo s/n, 48013 Bilbao (Spain); Balart, D. [SENER Ingeniería y Sistemas, Avda. Zugazarte 56, 48930 Las Arenas, Vizcaya (Spain); Sarrionandia-Ibarra, A. [UPV/EHU, Departamento de Ingeniería Nuclear y Mecánica de Fluidos, Alameda de Urquijo s/n, 48013 Bilbao (Spain); Pérez, V. [SENER Ingeniería y Sistemas, Avda. Zugazarte 56, 48930 Las Arenas, Vizcaya (Spain); Ibarra, A. [EURATOM-CIEMAT Fusion Assoc., Fusion Technology Division, Av. Complutense 40, 28040 Madrid (Spain); Legarda, F. [UPV/EHU, Departamento de Ingeniería Nuclear y Mecánica de Fluidos, Alameda de Urquijo s/n, 48013 Bilbao (Spain)

    2014-10-15

    Highlights: • Full material characterization as far as hydrogen transport properties are concern. • Quantification of permeator leaks and material degasification. • Analysis of H{sub 2} recovered by means of permeation against vacuum in different conditions. • Hydrogen recovery efficiencies determination. - Abstract: Tritium recovery in fusion reactors is one of the main goals in R and D, as a limited inventory is available and its uneconomic production. That is the reason why efficient technologies are indispensable to be developed in order to achieve fast tritium recovery and its subsequent reuse in the system for increasing its self-sufficiency. In this work a flexible tritium recovery demonstrator prototype based on permeation against vacuum concept has been designed and manufactured, as well as all necessary equipment for a Pb15.7Li loop implementation in order to test and demonstrate that an in-pipe integrated solution is possible, and at the same time, to validate the manufacturing process. Thus, efficient rates for more optimized future models could be then extrapolated. The aim of this paper is to show the different testing results that have been carried out in this research project. These results include permeation properties of the material considered for the permeator, as long as it has been manufactured with a novel technique, Selective Laser Melting. They also include vacuum tests on the permeator to quantify possible leakages and to set up and analyze the capability to generate vacuum inside the permeator, and finally, permeation tests with the prototype, in a first stage with a gas mixture of hydrogen and argon inside the loop instead of Pb15.7Li.

  5. Cell killing, nuclear damage and apoptosis in Chinese hamster V79 cells after irradiation with heavy-ion beams of (16)O, (12)C and (7)Li.

    Science.gov (United States)

    Pathak, Rupak; Dey, Subrata Kumar; Sarma, Asiti; Khuda-Bukhsh, Anisur Rahman

    2007-08-15

    Chinese hamster V79 cells were exposed to high LET (linear energy transfer) (16)O-beam (625keV/mum) radiation in the dose range of 0-9.83Gy. Cell survival, micronuclei (MN), chromosomal aberrations (CA) and induction of apoptosis were studied as a follow up of our earlier study on high LET radiations ((7)Li-beam of 60keV/mum and (12)C-beam of 295keV/mum) as well as (60)Co gamma-rays. Dose dependent decline in surviving fraction was noticed along with the increase of MN frequency, CA frequency as well as percentage of apoptosis as detected by nuclear fragmentation assay. The relative intensity of DNA ladder, which is a useful marker for the determination of the extent of apoptosis induction, was also increased in a dose dependent manner. Additionally, expression of tyrosine kinase lck-1 gene, which plays an important role in response to ionizing radiation induced apoptosis, was increased with the increase of radiation doses and also with incubation time. The present study showed that all the high LET radiations were generally more effective in cell killing and inflicting other cytogenetic damages than that of low LET gamma-rays. The dose response curves revealed that (7)Li-beam was most effective in cell killing as well as inducing other nuclear damages followed by (12)C, (16)O and (60)Co gamma-rays, in that order. The result of this study may have some application in biological dosimetry for assessment of genotoxicity in heavy ion exposed subjects and in determining suitable doses for radiotherapy in cancer patients where various species of heavy ions are now being generally used.

  6. In situ 7Li and 133Cs nuclear magnetic resonance investigations on the role of Cs+ additive in lithium-metal deposition process

    Energy Technology Data Exchange (ETDEWEB)

    Hu, Jian Zhi; Zhao, Zhenchao; Hu, Mary Y.; Feng, Ju; Deng, Xuchu; Chen, Xilin; Xu, Wu; Liu, Jun; Zhang, Ji-Guang

    2016-02-01

    Application of Li metal electrode in rechargeable lithium battery is hindered by safety concerns due to dendritic growth on the electrode over several charge-discharge cycles. We have found previously that adding low concentration Cs+ in electrolytes can promote smooth deposition of lithium onto metal electrode during repeated charge-discharge cycling using idea Li|Cu battery without the using of a separator. In this work, quantitative in situ 7Li and 133Cs NMR investigations using real planar symmetric lithium battery cells with and without Cs+ additives were carried out. It is found that the deposited lithium atoms on electrodes are highly porous. Detailed analysis of the data were carried out by separating the 7Li signal from deposited lithium that was oriented parallel to the electrode surface with the signal from the Li-metal nanorodes oriented perpendicular or nearly perpendicular to the electrode surface. The results demonstrate that addition of Cs+ can significantly enhance both the formation of uniform Li nanorods, and the reversibility of electrode. In situ 133Cs NMR directly confirms that Cs+ migrates to the electrode to form a positively charged electrostatic shield during cycling process. Combining the quantitative analysis of the orientation dependent signals of deposited metal Li and previous ex-situ results, different Li deposition models are proposed. During cycling process, more “active” lithium participates in the Li transfer between the electrode and nanorods for the battery with Cs+, while for the battery without Cs+ more dead and thinker lithium rods are formed and Li transfer between dendrites from different electrodes dominates.

  7. Treatment of the Mirror 3H(α, γ) 7Li and 3He(α, γ) 7Be Reactions in the Algebraic Version of the Resonating Group Model

    Science.gov (United States)

    Solovyev, A. S.; Igashov, S. Yu; Tchuvil'sky, Yu M.

    2014-12-01

    A unified microscopic approach based on the algebraic version of the resonating group model has been realized for description of the radiative capture reactions 3H(α, γ)7Li and 3He(α, γ)7Be, which play an important role for modern nuclear astrophysics. The astrophysical S-factors of the reactions and branching ratios between capture to the ground and first excited states of the 7Li and 7Be nuclei have been calculated. The comparison with the most recent experimental data demonstrates a good agreement.

  8. Measurement of the Breakup Cross Sections in 6He+9Be Reaction at 25 MeV/Nucleon

    Institute of Scientific and Technical Information of China (English)

    WANG Jia; HU Qing-Yuan; WU Cui-E; A. Ozawa; Y. Yamaguchi; R. Kanungo; D. Fang; I. Tanihata; YE Yan-Lin; JIANG Dong-Xing; ZHANG Gao-Long; PANG Dan-Yang; LI Zhi-Huan; ZHENG Tao; LI Xiang-Qing; WANG Quan-Jin

    2005-01-01

    @@ The breakup reaction cross sections were measured for the reaction of 6He at 25 MeV/nucleon from 9Be target with intensity of 105 pps. By fitting the energy spectra of breakup α particles with Gaussian functions, the angular distribution of differential cross sections in the laboratory system has been extracted and compared with the Serber model calculations. The good agreement between the calculation and the experimental data favours a dominant configuration of the 4He core plus valence neutrons for the structure of 6He.

  9. Isotopic Distributions of the l8N Fragmentation Products in Coincidence with Neutrons on Targets 197Au and 9Be

    Institute of Scientific and Technical Information of China (English)

    李湘庆; 江栋兴; 叶沿林; 华辉; 陈陶; 李智焕; 葛愉成; 王全进; 吴和宇; 靳根明; 段利敏; 肖志刚; 王宏伟; 李祖玉; 王素芳

    2002-01-01

    We present the experimental isotopic distributions of the 18 N projectile fragmentation products Li, Be,B and Cin coincidence with neutrons, as well as the inclusive ones on 197 Au and 9Be targets. In the framework of theabrasion-ablation model, these distributions are calculated for various nucleon density distributions of the projec-tile. The comparison with experimental isotopic distributions of the projectile-like fragments in coincidence withneutrons shows that the information on the nucleon density distribution of the 18N projectile can be extracted.

  10. Computing the Vibrational and Vibrational-rotational Energy Eigenvalues of 7Li2 by the Symplectic Scheme-matrix Algorithm%计算7Li2振动能级煌振动-转动能级的辛格式矩阵法

    Institute of Scientific and Technical Information of China (English)

    何建锋; 刘学深; 丁培柱

    2004-01-01

    利用辛格式矩阵法计算了双原子分子7Li2在A1∑+u态的振动能级和振动-转动能级,并与Ley-Koo等的计算结果作了比较.结果显示,辛格式矩阵法是收敛的和可靠的,是计算双原子分子的振动能级和振动-转动能级的合理的数值方法.

  11. Optimization of a neutron production target and a beam shaping assembly based on the 7Li( p, n) 7Be reaction for BNCT

    Science.gov (United States)

    Burlon, A. A.; Kreiner, A. J.; Valda, A. A.; Minsky, D. M.; Somacal, H. R.; Debray, M. E.; Stoliar, P.

    2005-02-01

    In this work a thick LiF target was studied through the 7Li( p, n) 7Be reaction as a neutron source for Accelerator-Based Boron Neutron Capture Therapy (AB-BNCT) to provide a testing ground for numerical simulations aimed at producing an optimized neutron production target and beam shaping assembly design. Proton beams in the 1.88-2.0 MeV energy range were produced with the tandem accelerator TANDAR ( TANDem ARgentino) at the Comisión Nacional de Energía Atómica (CNEA) in Buenos Aires, Argentina. A cylindrical water-filled head-phantom, containing a boric acid sample, was irradiated to study the resulting neutron flux. The dose deposited in the boric acid sample was inferred through the Compton-suppressed detection of the gamma radiation produced from the 10B( n, αγ) 7Li capture reaction. The thermal neutron flux was evaluated using bare and Cd-covered activation gold foils. In all cases, Monte Carlo simulations have been done showing good agreement with the experimental results. Extensive MCNP simulation trials have then been performed after the preliminary calculation tool validation in order to optimize a neutron beam shaping assembly. These simulations include a thick Li metal target (instead of LiF), a whole-body phantom, two different moderator-reflector assemblies (Al/AlF 3/LiF, Fluental ®, as moderator and lead as reflector and a combination of Al, PTFE (polytetrafluoroethylene) and LiF as moderator and lead as reflector) and the treatment room. The doses were evaluated for proton bombarding energies of 1.92 MeV (near to the threshold of the reaction), 2.0 MeV, 2.3 MeV (near the reaction resonance) and 2.5 MeV, and for three Fluental ® and Al/PTFE/LiF moderator thicknesses (18, 26 and 34 cm). In a later instance, the effect of the specific skin radiosensitivity (an RBE of 2.5 for the 10B( n, α) 7Li reaction) and a 10B uptake 50% greater than the healthy tissue one, was considered for the scalp. To evaluate the doses in the phantom, a comparison of

  12. Authigenic 10Be/9Be ratio signature of the Matuyama-Brunhes boundary in the Montalbano Jonico marine succession

    Science.gov (United States)

    Simon, Quentin; Bourlès, Didier L.; Bassinot, Franck; Nomade, Sébastien; Marino, Maria; Ciaranfi, Neri; Girone, Angela; Maiorano, Patrizia; Thouveny, Nicolas; Choy, Sandrine; Dewilde, Fabien; Scao, Vincent; Isguder, Gulay; Blamart, Dominique

    2017-02-01

    Geomagnetic dipole moment (GDM) lows associated with polarity reversals or geomagnetic excursions induce significant modulation of the cosmogenic nuclide Beryllium-10 (10Be) production. Hence, the reconstruction of atmospheric 10Be production rates from natural archives such as marine sedimentary sequences or ice cores constitutes a complementary approach, independent from paleomagnetic measurements, to decipher past GDM fluctuations. This is particularly important in the Montalbano Jonico succession (South Italy) since it is candidate to host the Global Stratotype Section and Point of the Middle Pleistocene Stage but where the magnetostratigraphic positioning of the Matuyama-Brunhes boundary (MBB) has not been available up to now. This study presents (1) original authigenic 10Be cosmogenic nuclide and 9Be stable isotope results, and (2) new high-resolution benthic oxygen isotope record covering termination IX and Marine Isotope Stage (MIS) 19. A robust chronological framework is established on the basis of (i) our oxygen isotope stratigraphy, using the strong analogies between MIS 1 and MIS 19c in terms of orbital forcing and CO2 level, and (ii) one precise 40Ar/39Ar date obtained in the tephra layer V4. The authigenic 10Be/9Be ratio record marks the atmospheric 10Be overproduction linked to the dipole low accompanying the MBB transition, with a characteristic twofold increase of the 10Be production at the end of MIS 19c and early MIS 19b. This signature is similar to those described in both marine and ice core records. The detailed chronostratigraphy constrained by a radiometrically-dated tephra layer (773.9 ± 1.3 ka) within the MBB interval, makes it possible to discuss the structure and to assess the timing of the 10Be-production changes, and thus the MBB geomagnetic variations, with an unprecedented accuracy for a marine archive (sedimentation rates ∼80 cm/ka). These new cosmogenic nuclide production signatures provide the only missing constraint required

  13. Digital signal processing for a thermal neutron detector using ZnS(Ag):{sup 6}LiF scintillating layers read out with WLS fibers and SiPMs

    Energy Technology Data Exchange (ETDEWEB)

    Mosset, J.-B., E-mail: jean-baptiste.mosset@psi.ch; Stoykov, A.; Greuter, U.; Hildebrandt, M.; Schlumpf, N.

    2016-07-11

    We present a digital signal processing system based on a photon counting approach which we developed for a thermal neutron detector consisting of ZnS(Ag):{sup 6}LiF scintillating layers read out with WLS fibers and SiPMs. Three digital filters have been evaluated: a moving sum, a moving sum after differentiation and a digital CR-RC{sup 4} filter. The performances of the detector with these filters are presented. A full analog signal processing using a CR-RC{sup 4} filter has been emulated digitally. The detector performance obtained with this analog approach is compared with the one obtained with the best performing digital approach. - Highlights: • Application of digital signal processing for a SiPM-based ZnS:6LiF neutron detector. • Optimisation of detector performances with 3 different digital filters. • Comparison with detector performances with a full analog signal processing.

  14. Study of 12Be using the 11Be(9Be,8Be) transfer reaction at TRIUMF ISAC-II

    Science.gov (United States)

    Braid, Ryan; Sarazin, Fred; TIGRESS Collaboration; (PCB)2 Collaboration

    2015-10-01

    Recent results at TRIUMF and NSCL have called into question the structure of 12Be, therefore another look at this nucleus is desirable. The structure is important information for theoretical models, since it constrains the mechanism that produces parity inversion in 11Be. The 12Be structure was probed in July 2014 using the (PCB)2 array (Printed Circuit Board Based Charged Particle) inside TIGRESS (TRIUMF - ISAC Gamma Ray Escape Suppressed Spectrometer) at TRIUMF using the 11Be(9Be,8Be)12Be reaction at 55 MeV in inverse kinematics. A second set of data at 30 MeV was collected. This reaction has numerous advantages over the traditional (d,p) method, foremost of which is the 8Be --> 2 α breakup since it allows for very clean identification and tagging. Additionally, TIGRESS will allow precise γ-tagging for the excited states. The initial data and analysis will be presented in this talk. This work is partially supported by the US Department of Energy through Grant/Contract No. DE-FG03-93ER40789 (Colorado School of Mines).

  15. Observation of breakup transfer process for the bound states of {sup 16}O populated from {sup 12}C({sup 6}Li,d) reaction at 20 MeV

    Energy Technology Data Exchange (ETDEWEB)

    Adhikari, S.; Basu, C.; Thompson, I. J.; Sugathan, P.; Jhinghan, A.; Golda, K. S.; Babu, A.; Singh, D.; Ray, S.; Mitra, A. K. [Nuclear Physics Division, Saha Institute of Nuclear Physics, Kolkata-700064 (India); Lawrence Livermore National Laboratory, L-414, Livermore CA 94551 (United States); Inter University Accelerator Centre, New Delhi 110067 (India); Physics Department, Ramkrishna Vivekananda University, Belur, Howrah (India); Nuclear Physics Division, Saha Institute of Nuclear Physics, Kolkata-700064 (India)

    2012-10-20

    The deuteron angular distribution for the {sup 12}C({sup 6}Li,d){sup 16}O* has been measured at 20 MeV populating bound and unbound states of {sup 16}O. Analysis shows a dominance of breakup induced alpha transfer in comparison to a direct alpha transfer process for the bound states. The effect increases as the excitation energy of {sup 16}O decreases, maximizing at the ground state.

  16. {sup 7}Li NMR spectroscopy and ion conduction mechanism of composite gel polymer electrolyte: A comparative study with variation of salt and plasticizer with filler

    Energy Technology Data Exchange (ETDEWEB)

    Saikia, D. [Department of Chemistry, Center for Nanotechnology and R and D Center for Membrane Technology, Chung Yuan Christian University, Chung Li 32023, Taiwan (China); Chen-Yang, Y.W. [Department of Chemistry, Center for Nanotechnology and R and D Center for Membrane Technology, Chung Yuan Christian University, Chung Li 32023, Taiwan (China)], E-mail: yuiwhei@cycu.edu.tw; Chen, Y.T.; Li, Y.K.; Lin, S.I. [Department of Chemistry, Center for Nanotechnology and R and D Center for Membrane Technology, Chung Yuan Christian University, Chung Li 32023, Taiwan (China)

    2009-01-30

    Microporous composite gel polymer electrolyte (CGPE) has been prepared by incorporating the home-made silica aerogel (SAG) particles into the poly(vinylidene fluoride-co-hexafluoropropylene) (PVdF-HFP) copolymer/LiClO{sub 4} matrix. The ionic transport behavior of the electrolyte is studied with various experimental techniques such as AC impedance, X-ray diffraction (XRD), infrared (IR) spectra, nuclear magnetic resonance (NMR), scanning electron microscopy (SEM), differential scanning calorimetry (DSC) and thermogravimetric analyzer (TGA), etc. The results reveal that the SAG particles are well dispersed in the electrolytes and incorporate with the other components of the CGPEs. The solid-state {sup 7}Li NMR study has confirmed the interactions of lithium ion with SAG, polymer and plasticizers, causing to form the microporous structure and reduce the glass transition temperature and crystallinity, resulting in an increase in ionic conductivity of the CGPE. The best ionic conductivity (1.04 x 10{sup -2} S/cm at room temperature) is obtained from the composite polymer electrolyte containing 4 wt% of SAG, which is approximately four times higher than the ionic conductivity of the electrolyte without the filler.

  17. What is the best proton energy for accelerator-based BNCT using the 7Li(p,n)7Be reaction?

    Science.gov (United States)

    Allen, D A; Beynon, T D

    2000-05-01

    With a growing interest in the use of accelerator-based epithermal neutron sources for BNCT programs, in particular those based upon the 7Li(p,n)7Be reaction, there is a need to address the question of "what is the best proton energy to use?" This paper considers this question by using radiation transport calculations to investigate a range of proton energies from 2.15 to 3.5 MeV and a range of moderator sizes. This study has moved away completely from the use of empty therapy beam parameters and instead defines the beam quality and optimizes the moderator design using widely accepted in-phantom treatment planning figures of merit. It is concluded that up to a proton energy of about 2.8 MeV there is no observed variation in the achievable therapy beam quality, but a price is paid in terms of treatment time for not choosing the upper limit of this range. For higher proton energies, the beam quality falls, but with no improvement in treatment time for optimum configurations.

  18. Quasi-monoenergetic neutron energy spectra for 246 and 389 MeV (7)Li(p,n) reactions at angles from 0 degrees to 300 degrees

    CERN Document Server

    Iwamoto, Y; Nakamura, T; Nakashima, H; Mares, V; Itoga, T; Matsumoto, T; Nakane, Y; Feldbaumer, E; Jaegerhofer, L; Pioch, C; Tamii, A; Satoh, D; Masuda, A; Sato, T; Iwase, H; Yashima, H; Nishiyama, J; Hagiwara, M; Hatanaka, K; Sakamoto, Y

    2011-01-01

    The authors measured the neutron energy spectra of a quasi-monoenergetic (7)Li(p,n) neutron source with 246 and 389 MeV protons set at seven angles (0 degrees, 2.5 degrees, 5 degrees, 10 degrees, 15 degrees, 20 degrees and 30 degrees), using a time-of-flight (TOF) method employing organic scintillators NE213 at the Research Center for Nuclear Physics (RCNP) of Osaka University. The energy spectra of the source neutrons were precisely deduced down to 2 MeV at 0 degrees and 10 MeV at other angles. The cross-sections of the peak neutron production reaction at 0 degrees were on the 35-40 mb line of other experimental data, and the peak neutron angular distribution agreed well with the Taddeucci formula. Neutron energy spectra below 100 MeV at all angles were comparable, but the shapes of the continuum above 150 MeV changed considerably with the angle. In order to consider the correction required to derive the response in the peak region from the measured total response for high-energy neutron monitors such as DAR...

  19. Spectroscopy of particle-phonon coupled states in $^{133}$Sb by the cluster transfer reaction of $^{132}$Sn on $^{7}$Li

    CERN Multimedia

    We propose to investigate, with MINIBALL coupled to T-REX, the one-valence-proton $^{133}$Sb nucleus by the cluster transfer reaction of $^{132}$Sn on $^{7}$Li. The excited $^{133}$Sb will be populated by transfer of a triton into $^{132}$Sn, followed by the emission of an $\\alpha$-particle (detected in T-REX) and 2 neutrons. The aim of the experiment is to locate states arising from the coupling of the valence proton of $^{133}$Sb to the collective low-lying phonon excitations of $^{132}$Sn (in particular the 3$^−$). According to calculations in the weak-coupling approach, these states lie in the 4$\\, - \\,$5 MeV excitation energy region and in the spin interval 1/2$\\, - \\,$ 19/2, i.e., in the region populated by the cluster transfer reaction. The results will be used to perform advanced tests of different types of nuclear interactions, usually employed in the description of particle-phonon coupled excitations. States arising from couplings of the proton with simpler core excitations, involving few nucleons...

  20. Mechanical Property and Intergranular Corrosion Sensitivity of Zn-Free and Zn-Microalloyed Al-2.7Cu-1.7Li-0.3Mg Alloys

    Science.gov (United States)

    Li, Jin-feng; Xu, Long; Cai, Chao; Chen, Yong-lai; Zhang, Xu-hu; Zheng, Zi-qiao

    2014-11-01

    The influence of 0.72 pct Zn addition on the tensile properties of Al-2.7Cu-1.7Li-0.3Mg alloys was investigated. Their intergranular corrosion (IGC) dependence on aging [T6 type at 423 K (150 °C) and 448 K (175 °C) and T8 type at 423 K (150 °C)] time was studied. An IGC diagram associated with aging process was established. The addition of 0.72 pct Zn enhanced the strength of the Al-Li alloy with T6 type aging at 448 K (175 °C). With aging process, the corrosion mode of the T6-aged Al-Li alloys was changed in the following order: pitting and local IGC (initial aging stage), general IGC (underaging stage), local IGC (near peak-aging stage), and pitting (overaging stage) again. The IGC depth was increased first and then decreased with aging time extension. The corrosion potential change of grains and the microstructure variation were used to explain the IGC sensitivity of the Al-Li alloy with different tempers. Meanwhile, 0.72 pct Zn addition decreased the IGC sensitivity of the Al-Li alloy, especially the T6-aged Al-Li alloy.

  1. A microdosimetric study of {sup 10}B(n,{alpha}){sup 7}Li and {sup 157}Gd(n,{gamma}) reactions for neutron capture therapy

    Energy Technology Data Exchange (ETDEWEB)

    Wang, C.K.C.; Sutton, M.; Evans, T.M. [Georgia Inst. of Tech., Atlanta, GA (United States); Laster, B.H. [Brookhaven National Lab., Upton, NY (United States). Medical Dept.

    1999-01-01

    This paper presents the microdosimetric analysis for the most interesting cell survival experiment recently performed at the Brookhaven National Laboratory (BNL). In this experiment, the cells were first treated with a gadolinium (Gd) labeled tumor-seeking boronated porphyrin (Gd-BOPP) or with BOPP alone, and then irradiated with thermal neutrons. The resulting cell-survival curves indicate that the {sup 157}Gd(n,{gamma}) reactions are very effective in cell killing. The death of a cell treated with Gd-BOPP was attributed to either the {sup 10}B(n,{alpha}){sup 7}Li reactions or the {sup 157}Gd(n,{gamma}) reactions (or both). However, the quantitative relationship between the two types of reaction and the cell-survival fraction was not clear. This paper presents the microdosimetric analysis for the BNL experiment based on the measured experimental parameters, and the results clearly suggest a quantitative relationship between the two types of reaction and the cell survival fraction. The results also suggest new research in gadolinium neutron capture therapy (GdNCT) which may lead to a more practical modality than the boron neutron capture therapy (BNCT) for treating cancers.

  2. Measurement of neutron energy spectra and neutron dose rates from {sup 7}Li(p,n){sup 7}Be reaction induced on thin LiF target

    Energy Technology Data Exchange (ETDEWEB)

    Atanackovic, Jovica, E-mail: atanacjz@gmail.com [Ontario Power Generation, Whitby, ON, Canada L1N 9E3 (Canada); Atomic Energy of Canada Limited, Chalk River Laboratories, Chalk River, Canada K0J 1J0 (Canada); Matysiak, Witold [University of Florida Proton Therapy Institute, Jacksonville, FL 32206 (United States); Dubeau, Jacques; Witharana, Sampath [DETEC, Gatineau, QC, Canada J8T 4J1 (Canada); Waker, Anthony [University of Ontario Institute of Technology, Oshawa, ON, Canada L1H 7K4 (Canada)

    2015-02-21

    The measurements of neutron energy spectra and neutron dose rates were performed using the KN Van de Graaff accelerator, located at the McMaster University Accelerator Laboratory (MAL). Protons were accelerated on the thin lithium fluoride (LiF) target and produced mono-energetic neutrons which were measured using three different spectrometers: Bonner Sphere Spectrometer (BSS), Nested Neutron Spectrometer (NNS), and Rotational Proton Recoil Spectrometer (ROSPEC). The purpose of this work is (1) measurement and quantification of low energy accelerator neutron fields in terms of neutron fluence and dose, (2) comparison of results obtained by three different instruments, (3) comparison of measurements with Monte Carlo simulations based on theoretical neutron yields from {sup 7}Li(p,n){sup 7}Be nuclear reaction, and (4) comparison of results obtained using different neutron spectral unfolding methods. The nominal thickness of the LiF target used in the experiment was 50μg/cm{sup 2}, which corresponds to the linear thickness of 0.19μm and results in approximately 6 keV energy loss for the proton energies used in the experiment (2.2, 2.3, 2.4 and 2.5 MeV). For each of the proton energies, neutron fluence per incident proton charge was measured and several dosimetric quantities of interest in radiation protection were derived. In addition, theoretical neutron yield calculations together with the results of Monte Carlo (MCNP) modeling of the neutron spectra are reported. Consistent neutron fluence spectra were obtained with three detectors and good agreement was observed between theoretically calculated and measured neutron fluences and derived dosimetric quantities for investigated proton energies at 2.3, 2.4 and 2.5 MeV. In the case of 2.2 MeV, some plausibly explainable discrepancies were observed.

  3. Optimization of the proton chopper for {sup 7}Li(p,n) neutron spectrometry using a {sup 3}He ionization chamber

    Energy Technology Data Exchange (ETDEWEB)

    Matysiak, W., E-mail: matysiw@mcmaster.c [Department of Medical Physics and Applied Radiation Sciences, McMaster University, Hamilton, ON, L8S 4K1 (Canada); Chettle, D.R.; Prestwich, W.V.; Byun, S.H. [Department of Medical Physics and Applied Radiation Sciences, McMaster University, Hamilton, ON, L8S 4K1 (Canada)

    2011-02-11

    Thick target {sup 7}Li(p,n) neutron spectra were measured with a {sup 3}He ion chamber in the proton energy region between 1.95 and 2.3 MeV using the McMaster pulsed accelerator neutron source. The pulsed neutron beam was produced by an electrostatic proton chopper to reject the slow neutron detection events, which seriously limit the fast neutron counting rate of the {sup 3}He ion chamber. To collect both arrival time and energy information of {sup 3}He detection events, a custom two-dimensional time-energy analyzer was built using a time scaler and a successive approximation peak-sensing ADC. At each proton energy, the optimum chopper operation was determined by taking into account the two competing requirements: high fast-to-slow neutron ratio and reasonable fast neutron counting rate. The proton pulse widths used were 10 {mu}s for 1.95 and 2.1 MeV proton energies, whereas a shorter, 5 {mu}s proton pulse was used for 2.3 MeV acquisition. The raw data were analyzed using three spectral unfolding methods: a simple division by detection efficiency, an iterative algorithm, and a regularized constrained inversion method. The three methods gave consistent neutron fluence spectra within 20% above 30 keV. Thanks to the enhanced fast-to-slow neutron ratio of the pulsed beam, the full detector response function could be employed in unfolding, which led to an extension of the dynamic energy range as well as a better stability of unfolding process in the low energy region.

  4. Ab initio calculations on the spectroscopic constants,vibrational levels and classical turning points for the 21Πu state of dimer 7Li2

    Institute of Scientific and Technical Information of China (English)

    Liu Yu-Fang; Sun Jin-Feng; Ma Heng; Zhu Zun-Lue

    2007-01-01

    The accurate dissociation energy and harmonic frequency for the highly excited 21 Πu state of dimer 7Li2 have been calculated using a symmetry-adapted-cluster configuration-interaction method in complete active space.The calculated results are in excellent agreement with experimental measurements.The potential energy curves at numerous basis sets for this state are obtained over a wide internuclear separation range from about 2.4ao to 37.0ao.And the conclusion is gained that the basis set 6-311++G(d,p) is a most suitable one.The calculated spectroscopic constants De,Re,ωe,ωeχe,αe and Be at 6-311++G(d,p) are 0.9670 eV,0.3125 nm,238.6 cm-1,1.3705cm-1,0.0039 cm-1 and 0.4921 cm-1.respectively.The vibrational levels are calculated by solving the radial Schr(o)dinger equation of nuclear motion.A total of 53 vibrational levels are found and reported for the first time.The classical turning points have been computed.Comparing with the measurements,in which only the first nine vibrational levels have been obtained so far,the present calculations are very encouraging.A careful comparison of the present results of the parameters De and ωe with those obtained from previous theories clearly shows that the present calculations are much closer to the measurements than previous theoretical results,thus representing an improvement on the accuracy of the ab initio calculations of the potentials for this state.

  5. Ab initio calculation of accurate dissociation energy,potential energy curve and dipole moment function for the A1∑+ state 7LiH molecule

    Institute of Scientific and Technical Information of China (English)

    Shi De-Heng; Liu Yu-Fang; Sun Jin-Feng; Yang Xiang-Dong; Zhu Zun-Lue

    2006-01-01

    The reasonable dissociation limit of the A1∑+ state 7LiH molecule is obtained. The accurate dissociation energy and the equilibrium geometry of this state are calculated using a symmetry-adapted-cluster configuration-interaction method in complete active space for the first time. The whole potential energy curve and the dipole moment function for the A1∑+ state are calculated over a wide internuclear separation range from about 0.1 to 1.4 nm. The calculated equilibrium geometry and dissociation energy of this potential energy curve are of Re=0.2487 nm and De=1.064 eV,respectively. The unusual negative values of the anharmonicity constant and the vibration-rotational coupling constant are of wexe=-4.7158cm-1 and αe=-0.08649cm-1, respectively. The vertical excitation energy from the ground to the A1∑+ state is calculated and the value is of 3.613eV at 0.15875nm (the equilibrium position of the ground state).The highly anomalous shape of this potential energy curve, which is exceptionally flat over a wide radial range around the equilibrium position, is discussed in detail. The harmonic frequency value of 502.47cm-1 about this state is approximately estimated. Careful comparison of the theoretical determinations with those obtained by previous theories about the A1∑+ state dissociation energy clearly shows that the present calculations are much closer to the experiments than previous theories, thus represents an improvement.

  6. The cross-section data from neutron activation experiments on niobium in the NPI p-7Li quasi-monoenergetic neutron field

    Directory of Open Access Journals (Sweden)

    Simakov S.P.

    2010-10-01

    Full Text Available The reaction of protons on 7Li target produces the high-energy quasi- monoenergetic neutron spectrum with the tail to lower energies. Proton energies of 19.8, 25.1, 27.6, 30.1, 32.6, 35.0 and 37.4 MeV were used to obtain quasi-monoenergetic neutrons with energies of 18, 21.6, 24.8, 27.6, 30.3, 32.9 and 35.6 MeV, respectively. Nb cross-section data for neutron energies higher than 22.5 MeV do not exist in the literature. Nb is the important material for fusion applications (IFMIF as well. The variable-energy proton beam of NPI cyclotron is utilized for the production of neutron field using thin lithium target. The carbon backing serves as the beam stopper. The system permits to produce neutron flux density about 109  n/cm2/s in peak at 30 MeV neutron energy. The niobium foils of 15 mm in diameter and approx. 0.75 g weight were activated. The nuclear spectroscopy methods with HPGe detector technique were used to obtain the activities of produced isotopes. The large set of neutron energies used in the experiment allows us to make the complex study of the cross-section values. The reactions (n,2n, (n,3n, (n,4n, (n,He3, (n,α and (n,2nα are studied. The cross-sections data of the (n,4n and (n,2nα are obtained for the first time. The cross-sections of (n,2n and (n,α reactions for higher neutron energies are strongly influenced by low energy tail of neutron spectra. This effect is discussed. The results are compared with the EAF-2007 library.

  7. Indirect determination of Li via {sup 74}Ge(n,{gamma}){sup 75m}Ge activation reaction induced by neutrons from {sup 7}Li(p,n){sup 7}Be reaction

    Energy Technology Data Exchange (ETDEWEB)

    Kumar, Sanjiv, E-mail: sanjucccm@rediffmail.com [National Centre for Compositional Characterization of Materials, BARC, ECIL Post, Hyderabad 500062 (India); Reddy, G.L.N.; Rao, Pritty [National Centre for Compositional Characterization of Materials, BARC, ECIL Post, Hyderabad 500062 (India); Verma, Rakesh [Analytical Chemistry Division, BARC, Mumbai 400085 (India); Ramana, J.V.; Vikramkumar, S.; Raju, V.S. [National Centre for Compositional Characterization of Materials, BARC, ECIL Post, Hyderabad 500062 (India)

    2012-03-01

    An indirect method to determine Li by {sup 74}Ge(n,{gamma}){sup 75m}Ge activation reaction induced in a high purity Ge (detector) crystal by neutrons from the {sup 7}Li(p,n){sup 7}Be reaction in a typical particle-induced {gamma}-ray emission (PIGE) spectroscopy experimental set-up is described. Performed with proton beams of energies in excess of 1.88 MeV, the threshold energy (E{sub th}) of the {sup 7}Li(p,n){sup 7}Be reaction, the determination involves the activity measurement of {sup 75m}Ge isotope that has a half-life of 47.7 s and decays with the emission of 139 keV {gamma}-rays. Rapidity, selectivity and sensitivity down to ppm levels are the attractive features of the method. It is a suitable alternative to {sup 7}Li(p,p Prime {gamma}){sup 7}Li reaction based PIGE technique in the analyses of matrices that contain light elements such as Be, B, F, Na and Al in significant proportions. Interferences can arise from elements, for example V and Ti, that have E{sub th} Less-Than-Or-Slanted-Equal-To 1.88 MeV for (p,n) reaction. In the case of elements such as Cu, Mo which have with E{sub th} > 1.88 MeV, the incident proton beam energy can be judiciously selected to avoid or minimize an interference. The method, under optimized irradiation conditions, does not entail a risk of neutron stimulated degradation of the performance of the detector. Besides analytical purposes, the measurement of the {sup 75m}Ge activity can serve as a powerful tool to monitor even low ({approx}25 n/cm{sup 2} s) thermal neutron fluxes.

  8. Study of the {sup 7}Be(p,{gamma}){sup 8}B and {sup 7}Li(n,{gamma}){sup 8}Li capture reactions using the shell model embedded in the continuum

    Energy Technology Data Exchange (ETDEWEB)

    Bennaceur, K.; Ploszajczak, M. [Grand Accelerateur National d`Ions Lourds (GANIL), 14 - Caen (France); Nowacki, F. [Grand Accelerateur National d`Ions Lourds (GANIL), 14 - Caen (France)]|[Strasbourg-1 Univ., 67 (France). Lab. de Physique Theorique; Okolowicz, J. [Grand Accelerateur National d`Ions Lourds (GANIL), 14 - Caen (France)]|[Institute of Nuclear Physics, Krakow (Poland)

    1999-02-01

    The realistic shell model which includes the coupling between many-particle (quasi-)bound states and the continuum of one-particle scattering states is applied to the spectroscopy of mirror nuclei: {sup 8}B and {sup 8}Li, as well as to the description of low energy cross sections (the astrophysical S factors) in the capture reactions: {sup 7}Be(p,{gamma}){sup 8}B and {sup 7}Li(n,{gamma}){sup 8}Li. (author) 49 refs.

  9. Fast Li ion dynamics in the solid electrolyte Li7 P3 S11 as probed by (6,7) Li NMR spin-lattice relaxation.

    Science.gov (United States)

    Wohlmuth, Dominik; Epp, Viktor; Wilkening, Martin

    2015-08-24

    The development of safe and long-lasting all-solid-state batteries with high energy density requires a thorough characterization of ion dynamics in solid electrolytes. Commonly, conductivity spectroscopy is used to study ion transport; much less frequently, however, atomic-scale methods such as nuclear magnetic resonance (NMR) are employed. Here, we studied long-range as well as short-range Li ion dynamics in the glass-ceramic Li7 P3 S11 . Li(+) diffusivity was probed by using a combination of different NMR techniques; the results are compared with those obtained from electrical conductivity measurements. Our NMR relaxometry data clearly reveal a very high Li(+) diffusivity, which is reflected in a so-called diffusion-induced (6) Li NMR spin-lattice relaxation peak showing up at temperatures as low as 313 K. At this temperature, the mean residence time between two successful Li jumps is in the order of 3×10(8) s(-1) , which corresponds to a Li(+) ion conductivity in the order of 10(-4) to 10(-3) S cm(-1) . Such a value is in perfect agreement with expectations for the crystalline but metastable glass ceramic Li7 P3 S11 . In contrast to conductivity measurements, NMR analysis reveals a range of activation energies with values ranging from 0.17 to 0.26 eV, characterizing Li diffusivity in the bulk. In our case, through-going Li ion transport, when probed by using macroscopic conductivity spectroscopy, however, seems to be influenced by blocking grain boundaries including, for example, amorphous regions surrounding the Li7 P3 S11 crystallites. As a result of this, long-range ion transport as seen by impedance spectroscopy is governed by an activation energy of approximately 0.38 eV. The findings emphasize how surface and grain boundary effects can drastically affect long-range ionic conduction. If we are to succeed in solid-state battery technology, such effects have to be brought under control by, for example, sophisticated densification or through the preparation

  10. Ca(AlH4)2, CaAlH5, and CaH2+6LiBH4: Calculated dehydrogenation enthalpy, including zero point energy, and the structure of the phonon spectra.

    Science.gov (United States)

    Marashdeh, Ali; Frankcombe, Terry J

    2008-06-21

    The dehydrogenation enthalpies of Ca(AlH(4))(2), CaAlH(5), and CaH(2)+6LiBH(4) have been calculated using density functional theory calculations at the generalized gradient approximation level. Harmonic phonon zero point energy (ZPE) corrections have been included using Parlinski's direct method. The dehydrogenation of Ca(AlH(4))(2) is exothermic, indicating a metastable hydride. Calculations for CaAlH(5) including ZPE effects indicate that it is not stable enough for a hydrogen storage system operating near ambient conditions. The destabilized combination of LiBH(4) with CaH(2) is a promising system after ZPE-corrected enthalpy calculations. The calculations confirm that including ZPE effects in the harmonic approximation for the dehydrogenation of Ca(AlH(4))(2), CaAlH(5), and CaH(2)+6LiBH(4) has a significant effect on the calculated reaction enthalpy. The contribution of ZPE to the dehydrogenation enthalpies of Ca(AlH(4))(2) and CaAlH(5) calculated by the direct method phonon analysis was compared to that calculated by the frozen-phonon method. The crystal structure of CaAlH(5) is presented in the more useful standard setting of P2(1)c symmetry and the phonon density of states of CaAlH(5), significantly different to other common complex metal hydrides, is rationalized.

  11. 基于6LiF/ZnS(Ag)闪烁体波移光纤读出中子探测器模拟研究%The Monte-Carlo Simulation on Neutron Detector of 6LiF/ZnS(Ag)Scintillator Using Wavelength-Shifting Readout Fibers

    Institute of Scientific and Technical Information of China (English)

    吴冲; 张强; 张鹏; 孙志嘉; 唐彬; 王拓

    2012-01-01

    利用GEANT4构建二维位置灵敏型闪烁体中子探测器模型,并对探测器的关键性能进行了系统的模拟研究.计算结果表明,采用双层闪烁屏与波移光纤作为夹层的“三明治”式结构探测器,其热中子探测效率可以达到49.1%.模拟和实验均表明:探测器具有较好的n/γ抑制能力.γ灵敏度小于10-5;中子位置分辨率随着光纤芯间距和光纤与闪烁屏距离的减小呈现减小趋势,本征空间分辨率最好可以达到X轴0.08 mm,Y轴0.12 mm;光纤与闪烁屏之间采用空气耦合位置分辨率好于硅油耦合.模拟结果与部分实验结果的对比验证显示,探测器具有较好的二维成像能力.%A prototype of position sensitive neutron detector based on 6LiF/ZnS(Ag) scintillator was constructed by GEANT 4 package, and its key properties were studied. The simulation result shows that the thermal neutron detection efficiency could reach 49.1% when the "sandwich structure" of detector was set. Both simulation and experimental result plot its good ability of n/y rejection ration,and the gamma sensitive is less than 10-5. The influences of the coupled material and space between wavelength shift fibers and scintillator,as well as the space between two fibers are considered. The intrinsic spatial resolution is 0. 08 mm for X-axis and 0.12 mm for Y-axis,and the detector has a good 2D imaging capability. The simulation results are compared with that of parts experimental results.

  12. First application of the n - 9Be optical potential to the study of the 10Be continuum via the (18O,17O ) neutron-transfer reaction

    Science.gov (United States)

    Carbone, D.; Bondı, M.; Bonaccorso, A.; Agodi, C.; Cappuzzello, F.; Cavallaro, M.; Charity, R. J.; Cunsolo, A.; De Napoli, M.; Foti, A.

    2014-12-01

    The 9Be(18O,17O ) 10Be reaction has been studied at an incident energy of 84 MeV, and the ejectiles have been detected at forward angles. The 10Be excitation energy spectrum has been obtained up to about 18 MeV, and several known bound and resonant states of 10Be have been identified. Calculations that describe the interaction of the neutron removed from the 18O projectile with the 9Be target by means of an optical potential with a semiclassical approximation for the relative motion account for a significant part of the 10Be continuum. Two parametrizations of the optical-model potential for the system n - 9Be have been used and compared.

  13. Applicability of the {sup 9}Be(d,n){sup 10}B reaction to AB-BNCT skin and deep tumor treatment

    Energy Technology Data Exchange (ETDEWEB)

    Capoulat, M.E., E-mail: capoulat@tandar.cnea.gov.ar [Gerencia de Investigacion y Aplicaciones, CNEA. Av. Gral. Paz 1499 (B1650KNA), San Martin, Buenos Aires (Argentina)] [Escuela de Ciencia y Tecnologia, Universidad Nacional de San Martin, M. de Irigoyen 3100 (1650), San Martin, Buenos Aires (Argentina)] [CONICET, Avenida Rivadavia 1917 (C1033AAJ), Buenos Aires (Argentina); Minsky, D.M.; Kreiner, A.J. [Gerencia de Investigacion y Aplicaciones, CNEA. Av. Gral. Paz 1499 (B1650KNA), San Martin, Buenos Aires (Argentina)] [Escuela de Ciencia y Tecnologia, Universidad Nacional de San Martin, M. de Irigoyen 3100 (1650), San Martin, Buenos Aires (Argentina)] [CONICET, Avenida Rivadavia 1917 (C1033AAJ), Buenos Aires (Argentina)

    2011-12-15

    In the range of low bombarding energies (less than about 1.5 MeV) the {sup 9}Be(d,n){sup 10}B reaction produces neutron spectra that can be moderated depending on the choice of the target thickness and the deuteron bombarding energy. In this work, a Monte Carlo simulation study to determine the capability of this reaction to deliver enough dose to efficiently control both skin and deep seated tumors has been performed by means of MCNP calculations using eight optimized {sup 9}Be targets.

  14. Quasi-elastic scattering of a secondary sup 6 He beam on a sup 9 Be target at 25 MeV/nucleon

    CERN Document Server

    Chen Tao; Li Zhi Huan; Jiang Dong Xing; Hua Hui; Li Xiang Qing; Wang Quan Jin; Ge Yuch Eng; Pang Dan Yang; Di Zhenyu; Jin Ge; Xiao Guo Qing; Guo Zhong Yan; Xiao Zhi Gang; Wang Hong Wei; Zhang Bao Guo; Wu He Yu; Li Jia Xing; Sun Zhi Yu; Zhan Wen Long

    2002-01-01

    The quasi-elastic scattering of a secondary sup 6 He beam (25 MeV/n) on a sup 9 Be target has been measured for the first time with the application of a sophisticated tracking detector system. The angular distribution is reported. A phenomenological optical potential is obtained by fitting the experimental data, which encourages more accurate experimental measurements

  15. Quasi-elastic Scattering of a Secondary 6He Beam on a 9Be Target at 25MeV/Nucleon

    Institute of Scientific and Technical Information of China (English)

    陈陶; 叶沿林; 李智焕; 江栋兴; 华辉; 李湘庆; 王全进; 葛榆成; 庞丹阳; 狄振宇; 靳根明; 肖国青; 郭忠言; 肖志刚; 王宏伟; 张保国; 吴和宇; 李家兴; 孙志宇; 詹文龙

    2002-01-01

    The quasi-elastic scattering of a secondary 6He beam (25 MeV/n) on a 9Be target has been measured for the firsttime with the application of a sophisticated tracking detector system. The angular distribution is reported. Aphenomenological optical potential is obtained by fitting the experimental data, which encourages more accurateexperimental measurements.

  16. Dose distributions in a human head phantom for neutron capture therapy using moderated neutrons from the 2.5 MeV proton-7Li reaction or from fission of 235U

    Science.gov (United States)

    Tanaka, Kenichi; Kobayashi, Tooru; Sakurai, Yoshinori; Nakagawa, Yoshinobu; Endo, Satoru; Hoshi, Masaharu

    2001-10-01

    The feasibility of neutron capture therapy (NCT) using an accelerator-based neutron source of the 7Li(p,n) reaction produced by 2.5 MeV protons was investigated by comparing the neutron beam tailored by both the Hiroshima University radiological research accelerator (HIRRAC) and the heavy water neutron irradiation facility in the Kyoto University reactor (KUR-HWNIF) from the viewpoint of the contamination dose ratios of the fast neutrons and the gamma rays. These contamination ratios to the boron dose were estimated in a water phantom of 20 cm diameter and 20 cm length to simulate a human head, with experiments by the same techniques for NCT in KUR-HWNIF and/or the simulation calculations by the Monte Carlo N-particle transport code system version 4B (MCNP-4B). It was found that the 7Li(p,n) neutrons produced by 2.5 MeV protons combined with 20, 25 or 30 cm thick D2O moderators of 20 cm diameter could make irradiation fields for NCT with depth-dose characteristics similar to those from the epithermal neutron beam at the KUR-HWNIF.

  17. 7Li NMR chemical shift titration and theoretical DFT calculation studies: solvent and anion effects on second-order complexation of 12-crown-4 and 1-aza-12-crown-4 with lithium cation in several aprotic solvents.

    Science.gov (United States)

    Masiker, Marilyn C; Mayne, Charles L; Boone, Brian J; Orendt, Anita M; Eyring, Edward M

    2010-02-01

    (7)Li NMR titration was used to determine stepwise complexation constants for the second-order complexation of lithium cation with 12-crown-4 in acetonitrile, propylene carbonate and a binary mixture of propylene carbonate and dimethyl carbonate. The anions used were perchlorate, hexaflurophosphate and trifluromethanesulfonate. A second ligand 1-aza-12-crown-4 was similarly investigated. The exchange between the free and complexed cation in these reactions is fast on an NMR timescale resulting in a single lithium peak which is a concentration-weighted average of the free and bound species. Solvent effects show that the 1:1 complex is much more stable in acetonitrile than in propylene carbonate or in the propylene carbonate dimethyl carbonate mixture. Anion effects for a given solvent were small. Optimized geometries of the free ligands and the 1:1 and 1:2 (sandwich) metal-ligand complexes were predicted by hybrid-density functional theory using the Gaussian 03 software package. Results were compared to literature values for 1:1 stability constants found by microcalorimetry for several of these systems and are found to be in good agreement. Although microcalorimetry only considered the formation of 1:1 complexes, (7)Li NMR shows evidence that both 1:1 and 1:2 complexes should be considered.

  18. Study of the reduction in detection limits of track detectors used for {sup 10}B(n,α){sup 7}Li reaction rate measure through annealing and chemical etching experiments; Estudo da reducao nos limites de deteccao de detectores de tracos utilizados na medida de taxa de reacao {sup 10}B(n, α){sup 7}Li atraves de experimentos de annealing e ataque quimico

    Energy Technology Data Exchange (ETDEWEB)

    Vasconcellos, Herminiane L.; Smilgys, Barbara; Guedes, Sandro, E-mail: hluizav@ifi.unicamp.br [Universidade Estadual de Campinas (UNICAMP), SP (Brazil). Instituto de Fisica Gleb Wataghin; Castro, Vinicius A. [Instituto de Pesquisas Energeticas e Nucleares (IPEN/CNEN-SP), Sao Paulo, SP (Brazil). Centro de Engenharia Nuclear

    2013-08-15

    The Boron Neutron Capture Therapy (BNCT) is an experimental radiotherapy for cancer treatment. It is based on {sup 10}B(n, α){sup 7}Li reaction, which can be measured by track detectors capable of recording events that strike them. With this recording, it is possible to determine the number of alpha particles and recoiling Lithium-7 nucleus, reaction products, and from this information, which amount of radiation dose a patient is exposed to. In this work, PADC detectors were characterized, irradiated at the IEA-R1 IPEN/CNEN reactor to assess the contribution of the{sup 10}B(n, α){sup 7}Li reaction and protons from fast neutron scattering with the elements that compounds the tissue. With the aim of reducing the proton background, the detectors were subjected to heating experiments at 80°C for periods in the range 0-100 hours. This was done in order to restore partially modified structure of the detector, causing a reduction in the size and density of tracks. This effect is known as annealing. For the visualization of tracks at microscope, detectors were made three chemical attacks with sodium hydroxide (NaOH) for 30, 60 and 90 minutes at 70°C. It was observed a reduction in the track density achieving a plateau heating time of 50 hours. For detectors that have not undergone annealing and were etched with another etchant, PEW solution, a reduction of 87% in track density was obtained. (author)

  19. Challenges in describing nuclear reactions outcomes at near-barrier energies

    Science.gov (United States)

    Dasgupta, M.; Simpson, E. C.; Kalkal, S.; Cook, K. J.; Carter, I. P.; Hinde, D. J.; Luong, D. H.

    2017-01-01

    The properties of light nuclei such as 6Li, 7Li, 9Be and 12C, and their reaction outcomes are known to be strongly influenced by their underlying α-cluster structure. Reaction models do not yet exist to allow accurate predictions of outcomes following a collision of these nuclei with another nucleus. As a result, reaction models within GEANT, and nuclear fusion models do not accurately describe measured products or cross sections. Recent measurements at the Australian National University have shown new reaction modes that lead to breakup of 6Li, 7Li into lighter clusters, again presenting a further challenge to current models. The new observations and subsequent model developments will impact on accurate predictions of reaction outcomes of 12C - a three α-cluster nucleus – that is used in heavy ion therapy.

  20. Mechanism of reactions induced by 7 MeV deuterons on /sup 9/Be ((d,p), (d,d), (d,t), (d,/sup 4/He))

    Energy Technology Data Exchange (ETDEWEB)

    Szczurek, A.; Bodek, K.; Krug, J.; Luebcke, W.; Ruehl, H.; Steinke, M.; Stephan, M.; Kamke, D.; Hajdas, W.; Jarczyk, L.

    1989-07-01

    Angular distributions of protons, deuterons, tritons and alpha-particles emitted from the reactions in the d+/sup 9/Be-system at E/sub d/=7 MeV as well as excitation functions at selected angles in the energy range E/sub d/=6.5-7.5 MeV (LAB) were measured. The potential part of the elastic scattering is described by the phenomenological optical model. The compound nucleus contribution to all exit channels is determined using the Hauser-Feshbach model. The collective excitation of the 2.43 MeV excited state of /sup 9/Be and transfer processes are analysed within the DWBA formalism. The analyses suggest a significant contribution of five-nucleon transfer to the (d, /sup 4/He) channel.

  1. Drivers of foraminiferal and bulk-sedimentary 10Be/9Be ratios in a marine sediment record offshore of sub-tropical Australia

    Science.gov (United States)

    Davies, M. H.; Abrajevitch, A.; Srncik, M.; Fifield, L. K.; De Deckker, P.; Heslop, D.; Roberts, A. P.

    2013-12-01

    Meteoric 10Be (half-life of ~1.5 My) is produced in the atmosphere via cosmic ray spallation of 16O, following which it is quickly transported to Earth's surface by precipitation. This process concentrates 10Be in the ocean, where it is thought to remain with a residence time of ~500-1000 years prior to export to the marine sedimentary record largely associated with sorption to the surface of settling clay particles. The bulk beryllium isotopic composition of marine clays hence reflects the convoluted factors of 10Be production and varying scavenging efficiency/terrigenous input. However, measurements of meteoric 10Be/9Be incorporated in the calcium carbonate tests of foraminifera (and hence presumably isolated from the dilution effects of sediment-bound terrigenous 9Be) may have the potential to provide useful chronological control for marine sediment records. Here we present 10Be/9Be results from a ~42 m-long sediment core collected off the NW coast of Australia (MD00-2361: 113°28.63‧E, 22°04.92‧S, 1805 m water depth). Measurements of δ18O on Globigerinoides ruber, supported by magnetostratigraphy, indicate that the record extends back >1.2 Ma. This independent chronology, in conjunction with excellent carbonate preservation at this site, allows preliminary evaluation of foraminiferal 10Be as a chronometer. We also evaluate the relationship between sedimentary 10Be/9Be ratios, regional surface ocean conditions as inferred from the δ18O stratigraphy and low-resolution Globigerinoides ruber Mg/Ca ratios, as well as large-scale changes in regional fluvial input as reconstructed from high-resolution XRF scanning profiles.

  2. The measurement of KNN,KLLINpd -->nX and p9Be-->nX at 800 MeV

    Science.gov (United States)

    Riley, P. J.; Hollas, C. L.; Newsom, C. R.; Ransome, R. D.; Bonner, B. E.; Simmons, J. E.; Bhatia, T. S.; Glass, G.; Hiebert, J. C.; Northcliffe, L. C.; Tippens, W. B.

    1981-07-01

    The polarization transfer parameters,KNN and KLL, have been measured in pd-->nX and p9Be-->nX at 0° and 800 MeV. The quasifree pd-->nX values for KNN and KLL are close to the free n-p measured values. The rather large values of KLL demonstrate that this transfer mechanism will provide a useful source of polarized neutrons at medium energies.

  3. Measurement of Cross Sections for the 10B(n,α)'7Li Reaction at 4.0 and 5.0 MeV Using an Asymmetrical Twin Gridded Ionization Chamber

    Institute of Scientific and Technical Information of China (English)

    ZHANG Guo-Hui; LIU Xiang; LIU Jia-Ming; XUE Zhi-Hua; WU Hao; CHEN Jin-Xiang

    2011-01-01

    @@ Cross sections of the 10B(n, α) 7Li reaction (including the total, the "leaking" alpha, forward alpha and backward alpha parts) at En=4.0 and 5.OMcV were measured using an asymmetrical twin gridded ionization chamber and two back-to-back 10B samples.Measurements were performed at the 4.5MV Van de Graaff accelerator of Peking University.Monoenergetic neutrons were produced through the 2H(d, n)3 He reaction with a deuterium gas target.Absolute neutron flux was determined by a 238 U sample set inside the gridded ionization chamber and a BF3 long counter was employed as a neutron flux monitor and for normalization.The present results are compared with previous measurements and evaluations.

  4. Authigenic (10)Be/(9)Be ratio signatures of the cosmogenic nuclide production linked to geomagnetic dipole moment variation since the Brunhes/Matuyama boundary.

    Science.gov (United States)

    Simon, Quentin; Thouveny, Nicolas; Bourlès, Didier L; Valet, Jean-Pierre; Bassinot, Franck; Ménabréaz, Lucie; Guillou, Valéry; Choy, Sandrine; Beaufort, Luc

    2016-11-01

    Geomagnetic dipole moment variations associated with polarity reversals and excursions are expressed by large changes of the cosmogenic nuclide beryllium-10 ((10)Be) production rates. Authigenic (10)Be/(9)Be ratios (proxy of atmospheric (10)Be production) from oceanic cores therefore complete the classical information derived from relative paleointensity (RPI) records. This study presents new authigenic (10)Be/(9)Be ratio results obtained from cores MD05-2920 and MD05-2930 collected in the west equatorial Pacific Ocean. Be ratios from cores MD05-2920, MD05-2930 and MD90-0961 have been stacked and averaged. Variations of the authigenic (10)Be/(9)Be ratio are analyzed and compared with the geomagnetic dipole low series reported from global RPI stacks. The largest (10)Be overproduction episodes are related to dipole field collapses (below a threshold of 2 × 10(22) Am(2)) associated with the Brunhes/Matuyama reversal, the Laschamp (41 ka) excursion, and the Iceland Basin event (190 ka). Other significant (10)Be production peaks are correlated to geomagnetic excursions reported in literature. The record was then calibrated by using absolute dipole moment values drawn from the Geomagia and Pint paleointensity value databases. The (10)Be-derived geomagnetic dipole moment record, independent from sedimentary paleomagnetic data, covers the Brunhes-Matuyama transition and the whole Brunhes Chron. It provides new and complementary data on the amplitude and timing of millennial-scale geomagnetic dipole moment variations and particularly on dipole moment collapses triggering polarity instabilities.

  5. Authigenic 10Be/9Be ratio signatures of the cosmogenic nuclide production linked to geomagnetic dipole moment variation since the Brunhes/Matuyama boundary

    Science.gov (United States)

    Thouveny, Nicolas; Bourlès, Didier L.; Valet, Jean‐Pierre; Bassinot, Franck; Ménabréaz, Lucie; Guillou, Valéry; Choy, Sandrine; Beaufort, Luc

    2016-01-01

    Abstract Geomagnetic dipole moment variations associated with polarity reversals and excursions are expressed by large changes of the cosmogenic nuclide beryllium‐10 (10Be) production rates. Authigenic 10Be/9Be ratios (proxy of atmospheric 10Be production) from oceanic cores therefore complete the classical information derived from relative paleointensity (RPI) records. This study presents new authigenic 10Be/9Be ratio results obtained from cores MD05‐2920 and MD05‐2930 collected in the west equatorial Pacific Ocean. Be ratios from cores MD05‐2920, MD05‐2930 and MD90‐0961 have been stacked and averaged. Variations of the authigenic 10Be/9Be ratio are analyzed and compared with the geomagnetic dipole low series reported from global RPI stacks. The largest 10Be overproduction episodes are related to dipole field collapses (below a threshold of 2 × 1022 Am2) associated with the Brunhes/Matuyama reversal, the Laschamp (41 ka) excursion, and the Iceland Basin event (190 ka). Other significant 10Be production peaks are correlated to geomagnetic excursions reported in literature. The record was then calibrated by using absolute dipole moment values drawn from the Geomagia and Pint paleointensity value databases. The 10Be‐derived geomagnetic dipole moment record, independent from sedimentary paleomagnetic data, covers the Brunhes‐Matuyama transition and the whole Brunhes Chron. It provides new and complementary data on the amplitude and timing of millennial‐scale geomagnetic dipole moment variations and particularly on dipole moment collapses triggering polarity instabilities. PMID:28163989

  6. One-neutron knockout in the vicinity of the N=32 sub-shell closure: 9Be(57Cr,56Cr+ gamma)X

    CERN Document Server

    Gade, A; Brown, B A; Campbell, C M; Carpenter, M P; Cook, J M; Deacon, A N; Dinca, D C; Freeman, S J; Glasmacher, T; Horoi, M; Janssens, R V F; Kay, B P; Mantica, P F; Müller, W F; Terry, J R; Tostevin, J A

    2006-01-01

    The one-neutron knockout reaction 9Be(57Cr,56Cr + gamma)X has been measured in inverse kinematics with an intermediate-energy beam. Cross sections to individual states in 56Cr were partially untangled through the detection of the characteristic gamma-ray transitions in coincidence with the reaction residues. The experimental inclusive longitudinal momentum distribution and the yields to individual states are compared to calculations that combine spectroscopic factors from the full fp shell model and nucleon-removal cross sections computed in a few-body eikonal approach.

  7. Isotopic distributions of the sup 1 sup 8 N fragmentation products in coincidence with neutrons on targets sup 1 sup 9 sup 7 Au and sup 9 Be

    CERN Document Server

    Li Xiang Qing; Ye Yan Lin; Hua Hui; Chen Tao; Li Zhi Huan; Ge Yuch Eng; Wang Quan Jin; Wu He Yu; Jin Ge; Duan Li Min; Xiao Zhi Gang; Wang Hong Wei; Li Zhu Yu; Wang Su Fang

    2002-01-01

    The authors present the experimental isotopic distributions of the sup 1 sup 8 N projectile fragmentation products Li, Be, B and C in coincidence with neutrons, as well as the inclusive ones on sup 1 sup 9 sup 7 Au and sup 9 Be targets. In the framework of the abrasion-ablation model, these distributions are calculated for various nucleon density distributions of the projectile. The comparison with experimental isotopic distributions of the projectile-like fragments in coincidence with neutrons shows that the information on the nucleon density distribution of the sup 1 sup 8 N projectile can be extracted

  8. Authigenic 10Be/9Be ratios and 10Be-fluxes (230Thxs-normalized) in central Baffin Bay sediments during the last glacial cycle: Paleoenvironmental implications

    Science.gov (United States)

    Simon, Quentin; Thouveny, Nicolas; Bourlès, Didier L.; Nuttin, Laurence; Hillaire-Marcel, Claude; St-Onge, Guillaume

    2016-05-01

    Authigenic 10Be/9Be ratios and 10Be-fluxes reconstructed using the 230Thxs normalization, proxies of the cosmogenic radionuclide 10Be production rate in the atmosphere, have been measured in a sedimentary core from Baffin Bay (North Atlantic) spanning the last 136 ka BP. The normalization applied on the exchangeable (authigenic) 10Be concentrations using the authigenic 9Be isotope and 230Thxs methods yield equivalent results strongly correlated with sedimentological parameters (grain-size and mineralogy). Lower authigenic beryllium (Be) concentrations and 10Be/9Be ratios are associated with coarse-grained carbonate-rich layers, while higher authigenic Be values are related to fine-grained felspar-rich sediments. This variability is due to: i) sediment composition control over beryllium-scavenging efficiency and, ii) glacial history that contributed to modify the 10Be concentration in Baffin Bay by input and boundary scavenging condition changes. Most paleo-denudation rates inferred from the 10Be/9Be ratio vary weakly around 220 ± 76 tons.km-2.yr-1 (0.09 ± 0.03 mm.yr-1) corresponding to relatively steady weathering fluxes over the last glacial cycle except for six brief intervals characterized by sharp increases of the denudation rate. These intervals are related to ice-surging episodes coeval with Heinrich events and the last deglaciation period. An average freshwater flux of 180.6 km3.yr-1 (0.006 Sv), consistent with recent models, has been calculated in order to sustain glacially-derived 10Be inputs into Baffin Bay. It is concluded that in such environments, the authigenic 10Be measured mainly depends on climatic effects related to the glacial dynamics, which masks the 10Be production variation modulated by geomagnetic field changes. Altogether, these results challenge the simple interpretation of 10Be-concentration variation as a proxy of Interglacial/Glacial (interstadial/stadial) cycles in Arctic and sub-Arctic regions. They rather suggest the effect of

  9. High-power electron beam tests of a liquid-lithium target and characterization study of (7)Li(p,n) near-threshold neutrons for accelerator-based boron neutron capture therapy.

    Science.gov (United States)

    Halfon, S; Paul, M; Arenshtam, A; Berkovits, D; Cohen, D; Eliyahu, I; Kijel, D; Mardor, I; Silverman, I

    2014-06-01

    A compact Liquid-Lithium Target (LiLiT) was built and tested with a high-power electron gun at Soreq Nuclear Research Center (SNRC). The target is intended to demonstrate liquid-lithium target capabilities to constitute an accelerator-based intense neutron source for Boron Neutron Capture Therapy (BNCT) in hospitals. The lithium target will produce neutrons through the (7)Li(p,n)(7)Be reaction and it will overcome the major problem of removing the thermal power >5kW generated by high-intensity proton beams, necessary for sufficient therapeutic neutron flux. In preliminary experiments liquid lithium was flown through the target loop and generated a stable jet on the concave supporting wall. Electron beam irradiation demonstrated that the liquid-lithium target can dissipate electron power densities of more than 4kW/cm(2) and volumetric power density around 2MW/cm(3) at a lithium flow of ~4m/s, while maintaining stable temperature and vacuum conditions. These power densities correspond to a narrow (σ=~2mm) 1.91MeV, 3mA proton beam. A high-intensity proton beam irradiation (1.91-2.5MeV, 2mA) is being commissioned at the SARAF (Soreq Applied Research Accelerator Facility) superconducting linear accelerator. In order to determine the conditions of LiLiT proton irradiation for BNCT and to tailor the neutron energy spectrum, a characterization of near threshold (~1.91MeV) (7)Li(p,n) neutrons is in progress based on Monte-Carlo (MCNP and Geant4) simulation and on low-intensity experiments with solid LiF targets. In-phantom dosimetry measurements are performed using special designed dosimeters based on CR-39 track detectors.

  10. Electrochemical performance and 7Li NMR studies on an inverse spinel LiNi 1/3Co 1/3Mn 1/3VO 4 for Li-ion batteries

    Science.gov (United States)

    Fey, George Ting-Kuo; Muralidharan, P.; Cho, Yung-Da; Chang, Pai-Ching; Kao, Hsien-Ming

    A new inverse spinel LiNi 1/3Co 1/3Mn 1/3VO 4 cathode material was synthesized through a citric acid assisted polyethylene glycol (CA:PEG; 3:1, 3:0.5 and 3:0) polymeric method, followed by calcination at 723 K for 5 h in air. The synthesized compound was characterized by TG/DTGA, XRD, FTIR, TEM, and 7Li NMR techniques. TG/DTGA curves showed that the formation of LiNi 1/3Co 1/3Mn 1/3VO 4 occurred between 523 and 673 K and the phase pure crystalline formed at 723 K, as also confirmed by XRD analysis which showed that the crystalline phase peaks formed when heated at 723 K for 5 h in air. TEM images revealed that nanosized particles ranged ∼170-190 nm. FTIR spectra showed that all organic residues were removed and LiNi 1/3Co 1/3Mn 1/3VO 4 formed. The 7Li MAS NMR spectrum of the LiNi 1/3Co 1/3Mn 1/3VO 4 sample revealed that the paramagnetic effect is small and small side band manifolds were observed. The galvanostatic cycling study suggests that the cycle stability and capacity retention were enhanced for LiNi 1/3Co 1/3Mn 1/3VO 4 prepared with a CA:PEG molar ratio of 3:1 when it was cycled between 2.8 and 4.9 V (versus Li) at a 0.15 C rate. The electrochemical impedance behavior suggested that a passive layer was formed on the surface of the cathode materials during continuous cycling.

  11. Lithium Ion Mobility in Lithium Phosphidosilicates: Crystal Structure, (7) Li, (29) Si, and (31) P MAS NMR Spectroscopy, and Impedance Spectroscopy of Li8 SiP4 and Li2 SiP2.

    Science.gov (United States)

    Toffoletti, Lorenzo; Kirchhain, Holger; Landesfeind, Johannes; Klein, Wilhelm; van Wüllen, Leo; Gasteiger, Hubert A; Fässler, Thomas F

    2016-12-05

    The need to improve electrodes and Li-ion conducting materials for rechargeable all-solid-state batteries has drawn enhanced attention to the investigation of lithium-rich compounds. The study of the ternary system Li-Si-P revealed a series of new compounds, two of which, Li8 SiP4 and Li2 SiP2 , are presented. Both phases represent members of a new family of Li ion conductors that display Li ion conductivity in the range from 1.15(7)×10(-6) Scm(-1) at 0 °C to 1.2(2)×10(-4) Scm(-1) at 75 °C (Li8 SiP4 ) and from 6.1(7)×10(-8) Scm(-1) at 0 °C to 6(1)×10(-6) Scm(-1) at 75 °C (Li2 SiP2 ), as determined by impedance measurements. Temperature-dependent solid-state (7) Li NMR spectroscopy revealed low activation energies of about 36 kJ mol(-1) for Li8 SiP4 and about 47 kJ mol(-1) for Li2 SiP2 . Both compounds were structurally characterized by X-ray diffraction analysis (single crystal and powder methods) and by (7) Li, (29) Si, and (31) P MAS NMR spectroscopy. Both phases consist of tetrahedral SiP4 anions and Li counterions. Li8 SiP4 contains isolated SiP4 units surrounded by Li atoms, while Li2 SiP2 comprises a three-dimensional network based on corner-sharing SiP4 tetrahedra, with the Li ions located in cavities and channels.

  12. Measurement of the $^{7}Be + ^{9}Be$ cross section at beam momenta of 13A, 20A and 30A GeV/c

    CERN Document Server

    Weimer, Ilona

    The NA61/SHINE experiment located at the SPS at CERN covers many purposes in various elds. It is a xed target experiment, which operates with di erent targets and beams. In 2012 and 2013 data was taken at di erent beam momenta with a 7 Be beam and a 9 Be target. Within this Bachelor work the data of NA61/SHINE was analyzed and the rst results on the 7 Be + 9 Be cross section at beam momenta of 13 A , 20 A and 30 A GeV/c are presented. In chapter 1 a de nition of the cross section is given and its approximation for the case of nucleus-nucleus collisions using the geometrical model is de ned and calcu- lated. The NA61/SHINE experiment and its detectors are described in chapter 2. The procedure which is used for the evaluation of the cross section and the interac- tion probability is presented and explained in chapter 3. It also includes information about the analyzed runs and the used event cuts. Further the interaction probability is calculated for all data sets with the standard cuts. The in uence of ...

  13. Evaluation of two thermal neutron detection units consisting of ZnS/${}^6$LiF scintillating layers with embedded WLS fibers read out with a SiPM

    CERN Document Server

    Mosset, J -B; Greuter, U; Hildebrandt, M; Schlumpf, N; Van Swygenhoven, H

    2014-01-01

    Two single channel detection units for thermal neutron detection are investigated in a neutron beam. They consist of two ZnS/${}^6$LiF scintillating layers sandwiching an array of WLS fibers. The pattern of this units can be repeated laterally and vertically in order to build up a one dimensional position sensitive multi-channel detector with the needed sensitive surface and with the required neutron absorption probability. The originality of this work arises from the fact that the WLS fibers are read out with SiPMs instead of the traditionally used PMTs or MaPMTs. The signal processing system is based on a photon counting approach. For SiPMs with a dark count rate as high as 0.7 MHz, a trigger efficiency of 80% is achieved together with a system background rate lower than ${10}^{-3}$ Hz and a dead time of 30 $\\mu$s. No change of performance is observed for neutron count rates of up to 3.6 kHz.

  14. Neutron-induced background by an alpha-beam incident on a deuterium gas target and its implications for the study of the 2H(alpha,gamma)6Li reaction at LUNA

    CERN Document Server

    Anders, M; Bellini, A; Aliotta, M; Bemmerer, D; Broggini, C; Caciolli, A; Costantini, H; Corvisiero, P; Davinson, T; Elekes, Z; Erhard, M; Formicola, A; Fülöp, Zs; Gervino, G; Guglielmetti, A; Gustavino, C; Gyürky, Gy; Junker, M; Lemut, A; Marta, M; Mazzocchi, C; Menegazzo, R; Prati, P; Alvarez, C Rossi; Scott, D; Somorjai, E; Straniero, O; Szücs, T

    2013-01-01

    The production of the stable isotope Li-6 in standard Big Bang nucleosynthesis has recently attracted much interest. Recent observations in metal-poor stars suggest that a cosmological Li-6 plateau may exist. If true, this plateau would come in addition to the well-known Spite plateau of Li-7 abundances and would point to a predominantly primordial origin of Li-6, contrary to the results of standard Big Bang nucleosynthesis calculations. Therefore, the nuclear physics underlying Big Bang Li-6 production must be revisited. The main production channel for Li-6 in the Big Bang is the 2H(alpha,gamma)6Li reaction. The present work reports on neutron-induced effects in a high-purity germanium detector that were encountered in a new study of this reaction. In the experiment, an {\\alpha}-beam from the underground accelerator LUNA in Gran Sasso, Italy, and a windowless deuterium gas target are used. A low neutron flux is induced by energetic deuterons from elastic scattering and, subsequently, the 2H(d,n)3He reaction....

  15. Theoretical model analysis of (d ,x n ) reactions on 9Be and 12C at incident energies up to 50 MeV

    Science.gov (United States)

    Nakayama, Shinsuke; Kouno, Hiroshi; Watanabe, Yukinobu; Iwamoto, Osamu; Ogata, Kazuyuki

    2016-07-01

    Background: In the design of deuteron accelerator neutron sources, accurate nuclear data of deuteron-induced reactions are indispensable over a wide range of incident energy. Reliable model calculations play an important role in completing the necessary nuclear data since currently available experimental data are insufficient. We have been developing a code system dedicated for the deuteron-induced reactions, called deuteron-induced reaction analysis code system (DEURACS). It was applied successfully to (d ,x p ) reactions at 56 and 100 MeV. Purpose: The purpose of the present work is to investigate the applicability of DEURACS to (d ,x n ) reactions on 9Be and 12C for incident energies below 50 MeV and to clarify neutron production mechanism. Methods: Double-differential thick target neutron yields (TTNYs) from deuteron bombardment on thick Be and C targets are analyzed. The TTNYs are derived using the double differential (d ,x n ) cross sections calculated by DEURACS and the stopping power of deuteron in the target. The calculated TTNYs are decomposed into individual components corresponding to elastic breakup, proton stripping, and statistical decay reactions. Results: The calculated TTNYs reproduced the experimental data quantitatively well in the incident energy range up to 50 MeV. From the analysis, it was found that the proton stripping reaction makes the most dominant contribution to neutron production. Conclusions: DEURACS is applicable to (d ,x n ) reactions on 9Be and 12C for incident energies below 50 MeV. Modeling of the stripping reaction is essential to predict neutron production yields accurately in the design of deuteron accelerator neutron sources.

  16. $\\gamma$- spectroscopy of n-rich $^{95,96}$Rb nuclei by the incomplete fusion reaction of $^{94}$Kr on $^{7}$Li: Introduction to HIE-ISOLDE studies of n-rich Sb and Tl isotopes with Sn and Hg radioactive beams.

    CERN Document Server

    Fornal, B; Bednarczyk, P; Cieplicka, N; Krolas, W; Maj, A; Leoni, S; Benzoni, G; Blasi, N; Bottoni, S; Bracco, A; Camera, F; Crespi, F; Million, B; Morales, A; Wieland, O; Rusek, K; Lunardi, S; Mengoni, D; Recchia, F; Ur, CA; Valiente-Dobon, J; de France, G; Clement, E; Elseviers, J; Flavigny, F; Huyse, M; Raabe, R; Sambi, S; Van Duppen, P; Sferrazza, M; Simpson, G; Georgiev, G; Sotty, C; Blazhev, A; German, R; Siebeck, B; Seidlitz, M; Reiter, P; Warr, N; Boenig, S; Ilieva, S; Kroell, T; Scheck, M; Thurauf, M; Gernhaeuser, R; Mucher, D; Janssens, R; Carpenter, MP; Zhu, S; Marginean, NM; Balabanski, D; Kowalska, M

    2012-01-01

    $\\gamma$- spectroscopy of n-rich $^{95,96}$Rb nuclei by the incomplete fusion reaction of $^{94}$Kr on $^{7}$Li: Introduction to HIE-ISOLDE studies of n-rich Sb and Tl isotopes with Sn and Hg radioactive beams.

  17. Isobaric yield ratio difference between the 140 $A$ MeV $^{58, 64}$Ni + $^{9}$Be reactions studied by antisymmetric molecular dynamics model

    CERN Document Server

    Qiao, C Y; Ma, C W; Zhang, Y L; Wang, S S

    2015-01-01

    \\item[Background] The isobaric yield ratio difference (IBD) method is found to be sensitive to the density difference of neutron-rich nucleus induced reaction around the Fermi energy. \\item[Purpose] An investigation is performed to study the IBD results in the transport model. \\item[Methods] The antisymmetric molecular dynamics (AMD) model plus the sequential decay model GEMINI are adopted to simulate the 140$A$ MeV $^{58, 64}$Ni + $^{9}$Be reactions. A relative small coalescence radius R$_c =$ 2.5 fm is used for the phase space at $t =$ 500 fm/c to form the hot fragment. Two limitations on the impact parameter ($b1 = 0 - 2$ fm and $b2 = 0 - 9$ fm) are used to study the effect of central collisions in IBD. \\item[Results] The isobaric yield ratios (IYRs) for the large--$A$ fragments are found to be suppressed in the symmetric reaction. The IBD results for fragments with neutron-excess $I = $ 0 and 1 are obtained. A small difference is found in the IBDs with the $b1$ and $b2$ limitations in the AMD simulated re...

  18. Development of a quasi-monoenergetic neutron field using the 7Li(p,n)7Be reaction in the energy range from 250 to 390 MeV at RCNP.

    Science.gov (United States)

    Taniguchi, S; Nakao, N; Nakamura, T; Yashima, H; Iwamoto, Y; Satoh, D; Nakane, Y; Nakashima, H; Itoga, T; Tamii, A; Hatanaka, K

    2007-01-01

    A quasi-monoenergetic neutron field using the (7)Li(p,n)(7)Be reaction has been developed at the ring cyclotron facility at the Research Center for Nuclear Physics (RCNP), Osaka University. Neutrons were generated from a 10-mm-thick Li target injected by 250, 350 and 392 MeV protons and neutrons produced at 0 degrees were extracted into the time-of-flight (TOF) room of 100-m length through the concrete collimator of 10 x 12 cm aperture and 150 cm thickness. The neutron energy spectra were measured by a 12.7-cm diam x 12.7-cm long NE213 organic liquid scintillator using the TOF method. The peak neutron fluence was 1.94 x 10(10), 1.07 x 10(10) and 1.50 x 10(10) n sr(-1) per muC of 250, 350 and 392 MeV protons, respectively. The neutron spectra generated from various thick (stopping length) targets of carbon, aluminium, iron and lead, bombarded by 250 and 350 MeV protons, were also measured with the TOF method. Although these measurements were performed to obtain thick target neutron yields, they are also used as a continuous energy neutron field. These neutron fields are very useful for characterising neutron detectors, measuring neutron cross sections, testing irradiation effects for various materials and performing neutron shielding experiments.

  19. Search for the p{sub 1/2{sup -}} resonance in {sup 7}He with the {sup 7}Li(d,{sup 2}He) reaction and measurement of the deuteron electrodisintegration under 180 at the S-DALINAC

    Energy Technology Data Exchange (ETDEWEB)

    Ryezayeva, N.

    2006-07-15

    The present work contains two parts, both devoted to the investigation of light nuclei. In the first part of the thesis the structure of the exotic {sup 7}He nucleus is studied. The disappearance of the usual magic numbers in extremely neutron-rich nuclei implies a considerable modification in the spin-orbit interaction. Recent experiments yield contradictory results about a possible existence of the p{sub 1/2{sup -}} spin-orbit partner of the {sup 7}He ground state with a dominant p{sub 3/2{sup -}} single-particle character. In order to clarify this question a study of the {sup 7}Li(d,{sup 2}He){sup 7}He reaction has been performed using a 171 MeV deuteron beam provided by the cyclotron at Kernfysisch Versneller Insituut (KVI) in Groningen. The experiment was carried out in April 2003. The setup at KVI offers a resolution {delta}E {approx} 150 keV (FWHM) in the measured spectra, better than the line width of the ground state of {sup 7}He. The unbound {sup 2}He system was identified by detecting coincidences between two protons with small relative energy. The data were taken over the angular range {theta}{sub cm}=0 -11.3 . A possible resonance at an excitation energy E{sub x}=(1.45{sub -0.5}{sup +0.7}) MeV with a width {gamma}=(2.0{sub -1.1}{sup +1.0}) MeV is suggested by a decomposition of the spectrum using known resonances, the breakup behaviour of {sup 7}He and quasifree charge-exchange contributions, taking into account the cluster structure of {sup 7}Li. Gamow-Teller strengths for transitions to the lowest states in {sup 7}He are in remarkable agreement with results from ab initio Quantum Monte Carlo calculations. The neutron spectroscopic factor S{sub n}=0.64{+-}0.09 of the {sup 7}He ground state ({sup 7}He={sup 6}He x n) is extracted by an R-matrix analysis. In the second part of the thesis the deuteron breakup has been studied in the {sup 2}H(e,e{sup '}) reaction at {theta}=180 . The present measurements were performed in March and April 2006 at the

  20. Characterization of high-energy quasi-monoenergetic neutron energy spectra and ambient dose equivalents of 80-389 MeV 7Li(p,n) reactions using a time-of-flight method

    Science.gov (United States)

    Iwamoto, Yosuke; Hagiwara, Masayuki; Satoh, Daiki; Araki, Shouhei; Yashima, Hiroshi; Sato, Tatsuhiko; Masuda, Akihiko; Matsumoto, Tetsuro; Nakao, Noriaki; Shima, Tatsushi; Kin, Tadahiro; Watanabe, Yukinobu; Iwase, Hiroshi; Nakamura, Takashi

    2015-12-01

    We completed a series of measurements on mono-energetic neutron energy spectra of the 7Li(p,n) reaction with 80-389-MeV protons in the 100-m time-of-flight (TOF) tunnel at the Research Center for Nuclear Physics cyclotron facility. For that purpose, we measured neutron energy spectra of the 80-, 100- and 296-MeV proton incident reactions, which had not been investigated in our previous studies. The neutron peak intensity was 0.9-1.1×1010 neutrons/sr/μC in the incident proton energy region of 80-389 MeV, and it was almost independent of the incident proton energy. The contribution of peak intensity of the spectrum to the total intensity integrated with energies above 3 MeV varied between 0.38 and 0.48 in the incident proton energy range of 80-389 MeV. To consider the correction required to derive a response in the peak region from the measured total responses of neutron monitors in the 100-m TOF tunnel, we proposed the subtraction method using energy spectra between 0° and 25°. The normalizing factor k against 25° neutron fluence to equalize it to 0° neutron fluence in the continuum region ranges from 0.74 to 1.02 depending on the incident proton energy and angle measured. Even without the TOF method, the subtraction method with the k factor almost decreases the response in the continuum region of a neutron spectrum against the total response of neutron monitors.

  1. Ab initio calculation on accurate analytic potential energy functions and harmonic frequencies of c3∑+g and B1∏u states of dimer 7Li2

    Institute of Scientific and Technical Information of China (English)

    Yu Ben-Hai; Shi De-Heng; Sun Jin-Feng; Zhu Zun-Lue; Liu Yu-Fang; Yang Xiang-Dong

    2007-01-01

    The comparison between single-point energy scanning (SPES) and geometry optimization (OPT) in determining the equilibrium geometries of c3∑+g and B1∏u states of dimer 7Li2 is made at numerous basis sets by using a symmetryadapted-cluster configuration-interaction (SAC-CI) method in the Gaussian 03 program package. In this paper the difference of the equilibrium geometries obtained by SPES and by OPT is reported. The results obtained by SPES are found to be more reasonable than those obtained by OPT in full active space at the present SAC-CI level of theory. And the conclusion is attained that the cc-PVTZ is a most suitable basis set for these states. The calculated dissociation energies and equilibrium geometries are 0.8818 eV and 0.3090 nm for c3∑+g state, and 0.3668 eV and 0.2932 nm for B1∏u state respectively. The potential energy curves are calculated over a wide internuclear distance range from about 2.5a0 to 37a0 and have a least-squares fit into the Murrell-Sorbie function. According to the calculated analytic potential energy functions, the harmonic frequencies (ωe) and other spectroscopic data (ωeχe, Be and αe) are calculated. Comparison of the theoretical determinations at present work with the experiments and other theories clearly shows that the present work is the most complete effort and thus represents an improvement over previous theoretical results.

  2. Impact of heat treatment on surface chemistry of Al-coated Eurofer for application as anti-corrosion and T-permeation barriers in a flowing Pb-15.7Li environment

    Energy Technology Data Exchange (ETDEWEB)

    Konys, J., E-mail: juergen.konys@kit.edu [Karlsruhe Institute of Technology, Hermann-von-Helmholtz-Platz 1 76344 Eggenstein-Leopoldshafen (Germany); Krauss, W.; Holstein, N.; Lorenz, J.; Wulf, S. [Karlsruhe Institute of Technology, Hermann-von-Helmholtz-Platz 1 76344 Eggenstein-Leopoldshafen (Germany); Bhanumurthy, K. [Scientific Information Resource Division, Bhabha Atomic Research Centre, Mumbai 400 085 (India)

    2012-08-15

    Highlights: Black-Right-Pointing-Pointer Electro-chemical Al deposition is industrially relevant for barrier formation. Black-Right-Pointing-Pointer Al scales have to be converted into protective layers by heat treatments. Black-Right-Pointing-Pointer Morphology of scales depend on deposition parameters. Black-Right-Pointing-Pointer Solid state diffusion step at 640 Degree-Sign C avoids critical Al melting and activates steel surface. Black-Right-Pointing-Pointer Al{sub 2}O{sub 3} protective scales detected. - Abstract: The compatibility testing of Eurofer steel in flowing Pb-15.7Li has shown that corrosion attack is a serious concern at least under view of precipitate formation from dissolved steel components in cooler system sections, leading to a high risk of tube blockages. Additionally, the T-permeation from the liquid breeder through the steel structure into the He-cooling system is an important safety issue. Both topics may be reduced by the application of barriers. Hot dip aluminization (HDA) showed that Al scales exhibit such ability but claimed also the development of improved coating technologies. Thus, two electro-chemically-based deposition processes, which exhibit industrial relevance and adjustable layer thickness of deposited Al, were developed, tested and characterized. Both are working with water-free electrolytes of toluene or ionic liquid (IL) base near room temperature (RT). The successfully deposited homogeneous layers need a heat treatment to establish the required protective/functional properties. During this stage, the Al reacts with the steel and forms an Al-enriched zone with a thin protective Al{sub 2}O{sub 3} surface scale. However, the topology is rough and pores are visible. Thus, for optimization of surface structure and scale quality, investigations concerning the required heat treatment were performed including effects coming from the applied coating technology.

  3. Photoneutron cross sections measurements in {sup 9}Be, {sup 13}C e {sup 17}O with thermal neutron capture gamma-rays; Medidas das secoes de choque de fotoneutrons do {sup 9}Be, {sup 13}C e {sup 17}O com radiacao gama de captura de neutrons termicos

    Energy Technology Data Exchange (ETDEWEB)

    Semmler, Renato

    2006-07-01

    Photoneutron cross sections measurements of {sup 9}Be, {sup 13}C and {sup 17}O have been obtained in the energy interval between 1,6 and 10,8 MeV, using neutron capture gamma-rays with high resolution in energy (3 a 21 eV), produced by 21 target materials, placed inside a tangential beam port, near the core of the IPEN/CNEN-SP IEA-R1 (5 MW) research reactor. The samples have been irradiated inside a 4{pi} geometry neutron detector system 'Long Counter', 520,5 cm away from the capture target. The capture gamma-ray flux was determined by means of the analysis of the gamma spectrum obtained by using a Ge(Li) solid-state detector (EG and G ORTEC, 25 cm{sup 3}, 5%), previously calibrated with capture gamma-rays from a standard target of Nitrogen (Melamine). The neutron photoproduction cross section has been measured for each target capture gamma-ray spectrum (compound cross section). A inversion matrix methodology to solve inversion problems for unfolding the set of experimental compound cross sections, was used in order to obtain the cross sections at specific excitation energy values (principal gamma line energies of the capture targets). The cross sections obtained at the energy values of the principal gamma lines were compared with experimental data reported by other authors, with have employed different gamma-ray sources. A good agreement was observed among the experimental data in this work with reported in the literature. (author)

  4. Isotopic Composition of Light Nuclei in Cosmic Rays: Results from AMS-01

    OpenAIRE

    Aguilar, M.; Alcaraz, J.; Allaby, J.; Alpat, B.; Ambrosi, G.; Anderhub, H.; Ao, L.; Arefiev, A.; Arruda, L.; P. Azzarello(c); Basile, M.; Barao, F.; G. Barreira(LIP Lisboa); Bartoloni, A; Battiston, R.

    2011-01-01

    The variety of isotopes in cosmic rays allows us to study different aspects of the processes that cosmic rays undergo between the time they are produced and the time of their arrival in the heliosphere. In this paper, we present measurements of the isotopic ratios 2H/4He, 3He/4He, 6Li/7Li, 7Be/(9Be+10Be), and 10B/11B in the range 0.2–1.4 GeV of kinetic energy per nucleon. The measurements are based on the data collected by the Alpha Magnetic Spectrometer, AMS-01, during the STS-91...

  5. Isotopic Composition of Light Nuclei in Cosmic Rays: Results from AMS-01

    Science.gov (United States)

    Aguilar, M.; Alcaraz, J.; Allaby, J.; Alpat, B.; Ambrosi, G.; Anderhub, H.; Ao, L.; Arefiev, A.; Arruda, L.; Azzarello, P.; Basile, M.; Barao, F.; Barreira, G.; Bartoloni, A.; Battiston, R.; Becker, R.; Becker, U.; Bellagamba, L.; Berdugo, J.; Berges, P.; Bertucci, B.; Biland, A.; Bindi, V.; Boella, G.; Boschini, M.; Bourquin, M.; Bruni, G.; Buénerd, M.; Burger, J. D.; Burger, W. J.; Cai, X. D.; Cannarsa, P.; Capell, M.; Casadei, D.; Casaus, J.; Castellini, G.; Cernuda, I.; Chang, Y. H.; Chen, H. F.; Chen, H. S.; Chen, Z. G.; Chernoplekov, N. A.; Chiueh, T. H.; Choi, Y. Y.; Cindolo, F.; Commichau, V.; Contin, A.; Cortina-Gil, E.; Crespo, D.; Cristinziani, M.; Dai, T. S.; dela Guia, C.; Delgado, C.; Di Falco, S.; Djambazov, L.; D'Antone, I.; Dong, Z. R.; Duranti, M.; Engelberg, J.; Eppling, F. J.; Eronen, T.; Extermann, P.; Favier, J.; Fiandrini, E.; Fisher, P. H.; Flügge, G.; Fouque, N.; Galaktionov, Y.; Gervasi, M.; Giovacchini, F.; Giusti, P.; Grandi, D.; Grimm, O.; Gu, W. Q.; Haino, S.; Hangarter, K.; Hasan, A.; Hermel, V.; Hofer, H.; Hungerford, W.; Ionica, M.; Jongmanns, M.; Karlamaa, K.; Karpinski, W.; Kenney, G.; Kim, D. H.; Kim, G. N.; Kim, K. S.; Kirn, T.; Klimentov, A.; Kossakowski, R.; Kounine, A.; Koutsenko, V.; Kraeber, M.; Laborie, G.; Laitinen, T.; Lamanna, G.; Laurenti, G.; Lebedev, A.; Lechanoine-Leluc, C.; Lee, M. W.; Lee, S. C.; Levi, G.; Lin, C. H.; Liu, H. T.; Lu, G.; Lu, Y. S.; Lübelsmeyer, K.; Luckey, D.; Lustermann, W.; Maña, C.; Margotti, A.; Mayet, F.; McNeil, R. R.; Menichelli, M.; Mihul, A.; Mujunen, A.; Natale, S.; Oliva, A.; Palmonari, F.; Paniccia, M.; Park, H. B.; Park, W. H.; Pauluzzi, M.; Pauss, F.; Pereira, R.; Perrin, E.; Pevsner, A.; Pilo, F.; Pimenta, M.; Plyaskin, V.; Pojidaev, V.; Pohl, M.; Produit, N.; Quadrani, L.; Rancoita, P. G.; Rapin, D.; Ren, D.; Ren, Z.; Ribordy, M.; Riihonen, E.; Ritakari, J.; Ro, S.; Roeser, U.; Sagdeev, R.; Santos, D.; Sartorelli, G.; Saouter, P.; Sbarra, C.; Schael, S.; Schultz von Dratzig, A.; Schwering, G.; Seo, E. S.; Shin, J. W.; Shoumilov, E.; Shoutko, V.; Siedenburg, T.; Siedling, R.; Son, D.; Song, T.; Spada, F. R.; Spinella, F.; Steuer, M.; Sun, G. S.; Suter, H.; Tang, X. W.; Ting, Samuel C. C.; Ting, S. M.; Tomassetti, N.; Tornikoski, M.; Torsti, J.; Trümper, J.; Ulbricht, J.; Urpo, S.; Valtonen, E.; Vandenhirtz, J.; Velikhov, E.; Verlaat, B.; Vetlitsky, I.; Vezzu, F.; Vialle, J. P.; Viertel, G.; Vité, D.; Von Gunten, H.; Waldmeier Wicki, S.; Wallraff, W.; Wang, J. Z.; Wiik, K.; Williams, C.; Wu, S. X.; Xia, P. C.; Xu, S.; Xu, Z. Z.; Yan, J. L.; Yan, L. G.; Yang, C. G.; Yang, J.; Yang, M.; Ye, S. W.; Zhang, H. Y.; Zhang, Z. P.; Zhao, D. X.; Zhou, F.; Zhou, Y.; Zhu, G. Y.; Zhu, W. Z.; Zhuang, H. L.; Zichichi, A.; Zimmermann, B.; Zuccon, P.

    2011-08-01

    The variety of isotopes in cosmic rays allows us to study different aspects of the processes that cosmic rays undergo between the time they are produced and the time of their arrival in the heliosphere. In this paper, we present measurements of the isotopic ratios 2H/4He, 3He/4He, 6Li/7Li, 7Be/(9Be+10Be), and 10B/11B in the range 0.2-1.4 GeV of kinetic energy per nucleon. The measurements are based on the data collected by the Alpha Magnetic Spectrometer, AMS-01, during the STS-91 flight in 1998 June.

  6. Isotopic Composition of Light Nuclei in Cosmic Rays: Results from AMS-01

    CERN Document Server

    Aguilar, M; Wiik, K; Grimm, O; Sartorelli, G; Zhou, Y; Pauss, F; Alpat, B; Capell, M; Djambazov, L; Yang, M; Yang, J; Extermann, P; Arefiev, A; Zhuang, H L; Hermel, V; Mihul, A; Galaktionov, Y; Park, H B; Von Gunten, H; Vetlitsky, I; Zhou, F; Vandenhirtz, J; Ambrosi, G; Suter, H; Becker, U; Zhang, H Y; Alcaraz, J; Casaus, J; Ren, Z; Fiandrini, E; Hungerford, W; Ren, D; Wicki, S W; Eppling, F J; Flugge, G; Karlamaa, K; Boella, G; Levi, G; Choi, Y Y; Laborie, G; Lubelsmeyer, K; Gervasi, M; Kirn, T; Azzarello, P; Kounine, A; Barreira, G; Yan, L G; Burger, W J; Koutsenko, V; Grandi, D; Ribordy, M; Gu, W Q; Bindi, V; Favier, J; Haino, S; Shin, J W; Mana, C; Seo, E S; Plyaskin, V; Shoumilov, E; Cannarsa, P; Xia, P C; Ionica, M; Jongmanns, M; Shoutko, V; Wallraff, W; Margotti, A; Lee, S C; Giovacchini, F; Schael, S; Bourquin, M; Roeser, U; Lu, Y S; Torsti, J; Kossakowski, R; Chang, Y H; Menichelli, M; Verlaat, B; Paniccia, M; Steuer, M; Fouque, N; Boschini, M; Zimmermann, B; Song, T; Zuccon, P; Contin, A; Produit, N; Laitinen, T; Kim, K S; Viertel, G; Lin, C H; Lechanoine-Leluc, C; Delgado, C; Lu, G; Pohl, M; Yang, C G; Tornikoski, M; Duranti, M; Cindolo, F; Xu, S; Lebedev, A; Xu, Z Z; Crespo, D; Cristinziani, M; Tomassetti, N; Kim, D H; Biland, A; Bertucci, B; Trumper, J; Buenerd, M; Hangarter, K; Kenney, G; Quadrani, L; Hofer, H; Berdugo, J; Siedenburg, T; Chen, Z G; Ting, S M; Vezzu, F; Cortina-Gil, E; Dai, T S; Barao, F; Commichau, V; Zhang, Z P; Sun, G S; Zhu, W Z; Laurenti, G; Chen, H S; Kim, G N; Sagdeev, R; Wu, S X; Urpo, S; Lee, M W; Rapin, D; Kraeber, M; Chen, H F; Engelberg, J; Ritakari, J; Di Falco, S; Zhu, G Y; Vite, D; Ulbricht, J; Bruni, G; Bellagamba, L; Williams, C; Fisher, P H; D'Antone, I; Pevsner, A; Castellini, G; Chernoplekov, N A; Ao, L; Giusti, P; McNeil, R R; Allaby, J; Yan, J L; Son, D; Santos, D; Cai, X D; Rancoita, P G; Becker, R; Wang, J Z; Oliva, A; Karpinski, W; Cernuda, I; Saouter, P; Ro, S; Anderhub, H; Dela Guia, C; Schwering, G; Ting, S C C; Lamanna, G; Pauluzzi, M; Berges, P; Riihonen, E; Pojidaev, V; Chiueh, T H; Valtonen, E; Pereira, R; Spinella, F; Perrin, E; Park, W H; Dong, Z R; Zichichi, A; Battiston, R; von Dratzig, A S; Vialle, J P; Klimentov, A; Liu, H T; Bartoloni, A; Arruda, L; Tang, X W; Mujunen, A; Pimenta, M; Casadei, D; Spada, F R; Eronen, T; Mayet, F; Palmonari, F; Lustermann, W; Velikhov, E; Pilo, F; Zhao, D X; Luckey, D; Basile, M; Sbarra, C; Natale, S; Siedling, R; Ye, S W; Burger, J D

    2011-01-01

    The variety of isotopes in cosmic rays allows us to study different aspects of the processes that cosmic rays undergo between the time they are produced and the time of their arrival in the heliosphere. In this paper, we present measurements of the isotopic ratios (2)H/(4)He, (3)He/(4)He, (6)Li/(7)Li, (7)Be/((9)Be+(10)Be), and (10)B/(11)B in the range 0.2-1.4 GeV of kinetic energy per nucleon. The measurements are based on the data collected by the Alpha Magnetic Spectrometer, AMS-01, during the STS-91 flight in 1998 June.

  7. A test of the cosmogenic 10Be(meteoric)/9Be proxy for simultaneously determining basin-wide erosion rates, denudation rates, and the degree of weathering in the Amazon basin

    Science.gov (United States)

    Wittmann, H.; Blanckenburg, F.; Dannhaus, N.; Bouchez, J.; Gaillardet, J.; Guyot, J. L.; Maurice, L.; Roig, H.; Filizola, N.; Christl, M.

    2015-12-01

    We present an extensive investigation of a new erosion and weathering proxy derived from the 10Be(meteoric)/9Be(stable) ratio in the Amazon River basin. This new proxy combines a radioactive atmospheric flux tracer, meteoric cosmogenic 10Be, with 9Be, a trace metal released by weathering. Results show that meteoric 10Be concentrations ([10Be]) and 10Be/9Be ratios increase by >30% from the Andes to the lowlands. We can calculate floodplain transfer times of 2-30 kyr from this increase. Intriguingly however, the riverine exported flux of meteoric 10Be shows a deficit with respect to the atmospheric depositional 10Be flux. Most likely, the actual area from which the 10Be flux is being delivered into the mainstream is smaller than the basin-wide one. Despite this imbalance, denudation rates calculated from 10Be/9Be ratios from bed load, suspended sediment, and water samples from Amazon Rivers agree within a factor of 2 with published in situ 10Be denudation rates. Erosion rates calculated from meteoric [10Be], measured from depth-integrated suspended sediment samples, agree with denudation rates, suggesting that grain size-induced variations in [10Be] are minimized when using such sampling material instead of bed load. In addition, the agreement between erosion and denudation rates implies minor chemical weathering intensity in most Amazon tributaries. Indeed, the Be-specific weathering intensity, calculated from mobilized 9Be comprising reactive and dissolved fractions that are released during weathering, is constant at approximately 40% of the total denudation from the Andes across the lowlands to the Amazon mouth. Therefore, weathering in the Amazon floodplain is not detected.

  8. Li2ZrO3-coated 0.4Li2MnO3·0.6LiNi1/3Co1/3Mn1/3O2 for high performance cathode material in lithium-ion battery

    Science.gov (United States)

    Miao, Xiaowei; Ni, Huan; Zhang, Han; Wang, Chunguang; Fang, Jianhui; Yang, Gang

    2014-10-01

    To improve the high-rate capacity and cycle ability, minor Li2ZrO3 successfully coat the nanoparticles of 0.4Li2MnO3·0.6LiNi1/3Co1/3Mn1/3O2 (LMO) via sol-gel method. The crystal structure and electrochemical properties of the bare and coated material are studied by X-ray diffractometry (XRD), transmission electron microscopy (TEM), cyclic voltammetry (CV), galvanostatic intermittent titration technique (GITT), and charge-discharge tests. The lithium diffusion coefficient of LMO increases one to two orders of magnitude after Li2ZrO3 coating. Li2ZrO3 coating improves the rate capability and cycling stability of LMO. Within the cut-off voltage of 2.5-4.8 V, the initial discharge capacity of Li2ZrO3-coated 0.4Li2MnO3·0.6LiNi1/3Co1/3Mn1/3O2 (LZO-LMO) reaches to 264 mAh g-1 at 0.1 C rate, and the capacity remains 235 mAh g-1 after 100 cycles. At the current rates of 1, 2, 5 and 10 C, the maximum discharge capacities of LZO-LMO are 205.6, 161, 153.8 and 106 mAh g-1, respectively. Minor Li2ZrO3 modification plays an important role to enhance the high-rate capability and cycle ability of LMO.

  9. Study of elastic pion scattering from /sup 9/Be, /sup 28/Si, /sup 58/Ni, and /sup 208/Pb at 162 MeV. [Total and differential cross sections, scattering yields, scattering amplitudes

    Energy Technology Data Exchange (ETDEWEB)

    Devereux, M.J.

    1979-05-01

    Elastic pion scattering from /sup 9/Be, /sup 28/Si, /sup 58/Ni, and /sup 208/Pb at 162 MeV is analyzed and compared with an optical model theory which incorporates a pion--nucleon range. Excellent fits to the data are obtained in all but one case. The fitted values of the pion--nucleon range, as well as other fitted values are listed. 108 references.

  10. Heavy-ion fusion cross sections of weakly bound {sup 9}Be on {sup 27}Al, {sup 64}Zn and tightly bound {sup 16}O on {sup 64}Zn target using Coulomb and proximity potential

    Energy Technology Data Exchange (ETDEWEB)

    Santhosh, K.P., E-mail: drkpsanthosh@gmail.com; Bobby Jose, V.

    2014-02-15

    The total fusion cross sections for the fusion of weakly bound {sup 9}Be on {sup 27}Al and {sup 64}Zn targets at near and above the barrier have been calculated using one dimensional barrier penetration model, taking scattering potential as the sum of Coulomb and proximity potential and the calculated values are compared with experimental data. For the purpose of comparison of the fusion of weakly bound projectiles and strongly bound projectiles, the total fusion cross sections for the reaction of tightly bound nucleus {sup 16}O on {sup 64}Zn have also been computed using a similar procedure. The calculated values of total fusion cross sections in all cases are compared with coupled channel calculations using the code CCFULL. The computed cross sections using Coulomb and proximity potential explain the fusion reactions well in both cases of weakly bound and strongly bound projectiles. Reduced reaction cross sections for the systems {sup 9}Be+{sup 27}Al, {sup 9}Be+{sup 64}Zn and {sup 16}O+{sup 64}Zn have also been described.

  11. Heavy-ion fusion cross sections of weakly bound $^{9}$Be on $^{27}$Al, $^{64}$Zn and tightly bound $^{16}$O on $^{64}$Zn target using Coulomb and proximity potential

    CERN Document Server

    Santhosh, K P

    2013-01-01

    The total fusion cross sections for the fusion of weakly bound $^{9}$Be on $^{27}$Al and $^{64}$Zn targets at near and above the barrier have been calculated using one dimensional barrier penetration model, taking scattering potential as the sum of Coulomb and proximity potential and the calculated values are compared with experimental data. For the purpose of comparison of the fusion of weakly bound projectiles and strongly bound projectiles, the total fusion cross sections for the reaction of tightly bound nucleus $^{16}$O on $^{64}$Zn have also been computed using a similar procedure. The calculated values of total fusion cross sections in all cases are compared with coupled channel calculations using the code CCFULL. The computed cross sections using Coulomb and proximity potential explain the fusion reactions well in both cases of weakly bound and strongly bound projectiles. Reduced reaction cross sections for the systems $^{9}$Be + $^{27}$Al, $^{9}$Be+ $^{64}$Zn and $^{16}$O + $^{64}$Zn have also been d...

  12. Nature of mixed symmetry 2{sup +} states in {sup 94}Mo from high resolution electron and proton scattering and line shape of the first excited 1/2{sup +} state in {sup 9}Be

    Energy Technology Data Exchange (ETDEWEB)

    Burda, Oleksiy

    2007-07-15

    The present work contains two parts. The first one is devoted to the investigation of mixed-symmetry structure in {sup 94}Mo and the second one to the astrophysical relevant line shape of the first excited 1/2{sup +} state in {sup 9}Be. In the first part of the thesis the nature of one- and two-phonon symmetric and mixed-symmetric 2{sup +} states in {sup 94}Mo is investigated with high-resolution inelastic electron and proton scattering experiments in a combined analysis. The (e,e') experiments were carried out at the 169 magnetic spectrometer at the S-DALINAC. Data were taken at a beam energy E e=70 MeV and scattering angles {theta}{sub e}=93 -165 . In dispersion-matching mode an energy resolution {delta}{sub E}=30-45 keV (full width at half maximum) was achieved. The (p,p') measurements were performed at iThemba LABS, South Africa, using a K600 magnetic spectrometer at a proton energy E p=200 MeV and scattering angles {theta}{sub p}=4.5 -26 . Typical energy resolutions were {delta}{sub E}{approx_equal}35 keV. The combined analysis reveals a dominant one-phonon structure of the transitions to the first and third 2{sup +} states, as well as an isovector character of the transition to the one-phonon mixed-symmetric state within the valence shell. Quantitatively consistent estimates of the one-phonon admixtures are obtained from both experimental probes when two-step contributions to the proton scattering cross sections are taken into account. In the second part of the thesis the line shape of the first excited 1/2{sup +} state in {sup 9}Be is studied. Spectra of the {sup 9}Be(e,e') reaction were measured at the S-DALINAC at an electron energy E e=73 MeV and scattering angles of 93 and 141 with high energy resolution up to excitation energies E{sub x}=8 MeV. The form factor of the first excited state has been extracted from the data. The astrophysical relevant {sup 9}Be({gamma},n) cross sections have been extracted from the (e,e') data. The

  13. Table of charged particle energies versus magnetic field strength x orbit radius (B{rho}) for A = 1 to 7 (100< (B{rho}) < 1200 kG.cm); Table des energies des particules chargees en fonction de la rigidite magnetique (B{rho}) pour A = 1 a 7 (100< (B{rho}) < 1200 kG.cm)

    Energy Technology Data Exchange (ETDEWEB)

    Bianchi, L. [Commissariat a l' Energie Atomique, Saclay (France). Centre d' Etudes Nucleaires

    1969-07-01

    A table of charged particle energies versus magnetic field strength x orbit radius (B{sub {rho}}) is presented. Particles p, d, t, {sup 3}He{sup ++}, {sup 4}He{sup +}, {sup 4}He{sup ++}, {sup 6}Li{sup +}, {sup 6}Li{sup ++}, {sup 6}Li{sup +++}, {sup 7}Li{sup +}, {sup 7}Li{sup ++}, {sup 7}Li{sup +++}. Values of B{sub {rho}}: 100 to 1200 kG.cm by steps of 0.5 kG.cm. Values of energies are given in keV. (author) [French] Nous presentons une table des energies de protons, deutons, tritons, {sup 3}He{sup ++}, {sup 4}He{sup +}, {sup 4}He{sup ++}, {sup 6}Li{sup +}, {sup 6}Li{sup ++}, {sup 6}Li{sup +++}, {sup 7}Li{sup +}, {sup 7}Li{sup ++}, {sup 7}Li{sup +++} en fonction de leur rigidite magnetique (B{sub {rho}}). Les valeurs de B{sub {rho}} sont comprises entre 100 et 1200 kG.cm par pas de 0.5 kG.cm. Les valeurs des energies sont donnees en keV. (auteur)

  14. Crystal structure of a new variety of lead dodecaborate Pb{sub 6}(Li{sub 0.65}Na{sub 0.19})[B{sub 12}O{sub 24}]I{sub 0.84} {center_dot} 0.168H{sub 2}O and its comparison with beryl and cordierite

    Energy Technology Data Exchange (ETDEWEB)

    Belokoneva, E. L., E-mail: elbel@geol.msu.ru; Derkach, I. K.; Dimitrova, O. V. [Moscow State University, Faculty of Geology (Russian Federation)

    2013-05-15

    Crystals of a new representative of ring-radical dodecaborates Pb{sub 6}(Li{sub 0.65}Na{sub 0.19})[B{sub 12}O{sub 24}]I{sub 0.84} {center_dot} 0.168H{sub 2}O, space group R3bar m , are obtained under hydrothermal conditions. The structure is determined with-out preliminary knowledge of the chemical formula. It is close to that of the Pb{sub 6}[B{sub 12}O{sub 24}] {center_dot} H{sub 2}O dodecaborate studied earlier, but unlike the latter structure it contains admixtures of iodide anion, lithium cation, and water molecule, which incompletely populate positions in channels. The formation of the second variety, which brings to light ion-exchange properties of the crystals, is due to mineralizing ions available in the concen-trated solution in the course of crystallization. The new compound is compared with beryl and cordierite, which have close structures with channels capable of capturing various groups. Structures of synthetic Na and Ag dodecaborates with analogous but distorted ring dodecaborate radicals are discussed.

  15. Computational assessment of deep-seated tumor treatment capability of the 9Be(d,n)10B reaction for accelerator-based boron neutron capture therapy (AB-BNCT).

    Science.gov (United States)

    Capoulat, M E; Minsky, D M; Kreiner, A J

    2014-03-01

    The 9Be(d,n)10B reaction was studied as an epithermal neutron source for brain tumor treatment through Boron Neutron Capture Therapy (BNCT). In BNCT, neutrons are classified according to their energies as thermal (epithermal (from 0.5 eV to 10 keV) or fast (>10 keV). For deep-seated tumors epithermal neutrons are needed. Since a fraction of the neutrons produced by this reaction are quite fast (up to 5-6 MeV, even for low-bombarding energies), an efficient beam shaping design is required. This task was carried out (1) by selecting the combinations of bombarding energy and target thickness that minimize the highest-energy neutron production; and (2) by the appropriate choice of the Beam Shaping Assembly (BSA) geometry, for each of the combinations found in (1). The BSA geometry was determined as the configuration that maximized the dose deliverable to the tumor in a 1 h treatment, within the constraints imposed by the healthy tissue dose adopted tolerance. Doses were calculated through the MCNP code. The highest dose deliverable to the tumor was found for an 8 μm target and a deuteron beam of 1.45 MeV. Tumor weighted doses ≥40 Gy can be delivered up to about 5 cm in depth, with a maximum value of 51 Gy at a depth of about 2 cm. This dose performance can be improved by relaxing the treatment time constraint and splitting the treatment into two 1-h sessions. These good treatment capabilities strengthen the prospects for a potential use of this reaction in BNCT.

  16. Light elements depletion in stellar environments.

    Science.gov (United States)

    Pizzone, R. G.; Lamia, L.; Romano, S.; Spitaleri, C.; Szanto de Toledo, A.; Blagus, S.; Bogovac, M.; Carlin, N.; Cherubini, S.; Crucillá, V.; Milin, M.; De Moura, M. M.; Gameiro Munhoz, M.; Gimenez del Santo, M.; Gulino, M.; La Cognata, M.; Liguori Neto, R.; Miljanić, D.; Puglia, S. M. R.; Rapisarda, G. G.; Sergi, M. L.; Soić, N.; Souza, F. A.; Suaide, A. A. P.; Szanto, E.; Tudisco, S.; Tumino, A.; Typel, S.

    Big efforts have been devoted in the last years to the study of light elements abundances. Definitively their importance is strongly related to cosmology as well as to stellar structure and evolution. In fact hints on the primordial nucleosynthesis can be achieved from Li, Be and B primordial abundances. Moreover these studies can be a precious tool for testing and understanding the inner stellar structure, especially for what regards the mixing processes in stellar envelopes \\citep{boesgard04}. In this framework the different nuclear processes which produce or destroy Li, Be and B must be studied in details and an accurate knowledge of the involved nuclear cross sections is necessary. In particular we will focus our attention on one of the main destruction channels for these elements in stellar environments, the (p,alpha ) reactions. In particular this work will review the last results achieved by the Trojan Horse Method (THM) for the 6Li(p,alpha )3He, 6Li(d,alpha )4He, 7Li(p,alpha )4He, 10B(p,alpha )7Be, 9Be(p,alpha )6Li and 11B(p,alpha )8Be.

  17. New lithium copper borates with BO3 triangles: Li6CuB4O10, Li3CuB3O7, Li8Cu7B14O32, and Li2Cu9B12O28.

    Science.gov (United States)

    Kuratieva, N V; Bànki, M; Tsirlin, A A; Eckert, J; Ehrenberg, H; Mikhailova, D

    2013-12-16

    Crystal structures of three new lithium copper borates, Li3CuB3O7, Li8Cu7B14O32, and Li2Cu9B12O28, and a new Li6CuB4O10 polymorph were solved by single-crystal X-ray diffraction. In all of the structures, the boron cations form BO3 triangles, which are connected with each other and with copper polyhedra only via corners in Li6CuB4O10 and Li3CuB3O7 and via both corners and edges in Li8Cu7B14O32 and Li2Cu9B12O28. The Li3CuB3O7 and Li8Cu7B14O32 compounds were synthesized as pure samples with only trace amounts of impurities; hence, their magnetic properties could be investigated and analyzed in terms of underlying magnetic couplings. Other compositions always represented multiphase mixtures. Li3CuB3O7 features infinite Cu,O chains formed by Cu2O6 units consisting of edge-shared CuO4 squares. Together with two apical oxygen atoms with long interatomic Cu-O distances of 2.7-2.8 Å, the Cu2O6 units form chains extended along the a axis. These pseudochains are responsible for strong anisotropic thermal expansion behavior. The temperature dependence of the magnetization between 4 and 380 K for Li3CuB3O7 could be fit well by a spin-dimer model. The magnetic susceptibility of Li8Cu7B14O32 showed a more complex temperature dependence, with two different Curie-Weiss regimes in the temperature range of 2-380 K.

  18. Study of the (p,d/sup 3/He) reaction as a quasi-free reaction process

    Energy Technology Data Exchange (ETDEWEB)

    Cowley, A. A.; Roos, P. G.; Chant, N. S.; Woody, R. III; Holmgren, H. D.; Goldberg, D. A.

    1976-11-01

    The (p,d/sup 3/He) reaction on /sup 6/Li, /sup 7/Li, /sup 9/Be, and /sup 12/C has been investigated in conjunction with studies of the (p,p..cap alpha..) reaction on the same targets. Coincident data for all four targets were obtained at a bombarding energy of 100 MeV for numerous angle pairs in order to test the reaction mechanism. Comparisons of the (p,d/sup 3/He) data to both (p,p..cap alpha..) data and distorted wave impulse approximation calculations (DWIA) indicate a dominance of the direct quasi-free reaction process (p + alpha yields d + /sup 3/He). The absolute alpha-particle spectroscopic factors extracted using DWIA analysis are in agreement with the values obtained in the (p,p..cap alpha..) reaction.

  19. Neutrino-Nucleus Reaction Cross Sections for Light Element Synthesis in Supernova Explosions

    CERN Document Server

    Yoshida, T; Chiba, S; Kajino, T; Yokomakura, H; Kimura, K; Takamura, A; Hartmann, D H

    2008-01-01

    The neutrino-nucleus reaction cross sections of 4He and 12C are evaluated using new shell model Hamiltonians. Branching ratios of various decay channels are calculated to evaluate the yields of Li, Be, and B produced through the nu-process in supernova explosions. The new cross sections enhance the yields of 7Li and 11B produced during the supernova explosion of a 16.2 M_odot star model compared to the case using the conventional cross sections by about 10%. On the other hand, the yield of 10B decreases by a factor of two. The yields of 6Li, 9Be, and the radioactive nucleus 10Be are found at a level of 10^{-11} M_odot. The temperature of nu_{mu,tau}- and bar{nu}_{mu,tau}-neutrinos inferred from the supernova contribution of 11B in Galactic chemical evolution models is constrained to the 4.3 MeV to 6.5 MeV range. The increase in the 7Li and 11B yields due to neutrino oscillations is demonstrated with the new cross sections.

  20. Primordial Nucleosynthesis

    CERN Document Server

    Coc, Alain

    2012-01-01

    Primordial nucleosynthesis, or Big-Bang Nucleosynthesis (BBN), is one of the three evidences for the Big-Bang model, together with the expansion of the Universe and the Cosmic Microwave Background. There is a good global agreement over a range of nine orders of magnitude between abundances of 4He, D, 3He and 7Li deduced from observations, and calculated in primordial nucleosynthesis. This comparison was used to determine the baryonic density of the Universe. For this purpose, it is now superseded by the analysis of the Cosmic Microwave Background (CMB) radiation anisotropies. However, there remain, a yet unexplained, discrepancy of a factor 3-5, between the calculated and observed lithium primordial abundances, that has not been reduced, neither by recent nuclear physics experiments, nor by new observations. We review here the nuclear physics aspects of BBN for the production of 4He, D, 3He and 7Li, but also 6Li, 9Be, 11B and up to CNO isotopes. These are, for instance, important for the initial composition o...

  1. Determination of the {sup 9}Be({sup 3}He,p{sub i}){sup 11}B (i = 0,1,2,3) cross section at 135° in the energy range 1–2.5 MeV

    Energy Technology Data Exchange (ETDEWEB)

    Barradas, N.P., E-mail: nunoni@ctn.ist.utl.pt [Centro de Ciências e Tecnologias Nucleares, Instituto Superior Técnico, Universidade de Lisboa, E.N. 10 ao km 139,7, 2695-066 Bobadela LRS (Portugal); Catarino, N.; Mateus, R. [Instituto de Plasmas e Fusão Nuclear, Instituto Superior Técnico, Universidade de Lisboa, E.N. 10 ao km 139,7, 2695-066 Bobadela LRS (Portugal); Magalhães, S. [Centro de Ciências e Tecnologias Nucleares, Instituto Superior Técnico, Universidade de Lisboa, E.N. 10 ao km 139,7, 2695-066 Bobadela LRS (Portugal); Alves, E. [Instituto de Plasmas e Fusão Nuclear, Instituto Superior Técnico, Universidade de Lisboa, E.N. 10 ao km 139,7, 2695-066 Bobadela LRS (Portugal); Siketić, Z.; Radović, I. Bogdanović [Ruđer Bošković Institute, P.O. Box 180, 10002 Zagreb (Croatia)

    2015-03-01

    The {sup 9}Be({sup 3}He,p{sub i}){sup 11}B cross sections for i = 0,1,2,3 at an angle of 135° in the energy range 1–2.5 MeV have been measured using two thin films with different Be thickness at selected energies. The new data extend previous results, that only existed at 90°, 120° and 150° angles, and down to 1.8 MeV, which prevented use of this reaction for samples containing Be at larger depths.

  2. Study of the primordial lithium abundance

    Institute of Scientific and Technical Information of China (English)

    2011-01-01

    Lithium isotopes have attracted an intense interest because the abundance of both 6Li and 6Li from big bang nucleosynthesis (BBN) is one of the puzzles in nuclear astrophysics. Many investigations of both astrophysical observation and nucleosynthesis calculation have been carried out to solve the puzzle, but it is not solved yet. Several nuclear reactions involving lithium have been indirectly measured at China Institute of Atomic Energy, Beijing. The Standard BBN (SBBN) network calculations are then performed to investigate the primordial Lithium abundance. The result shows that these nuclear reactions have minimal effect on the SBBN abundances of 6Li and 7Li.

  3. Atomic lithium vapor laser isotope separation

    CERN Document Server

    Olivares, I E

    2002-01-01

    An atomic vapor laser isotope separation in lithium was performed using tunable diode lasers. The method permits also the separation of the isotopes between the sup 6 LiD sub 2 and the sup 7 LiD sub 1 lines using a self-made mass separator which includes a magnetic sector and an ion beam designed for lithium. (Author)

  4. Diode laser absorption spectroscopy of lithium isotopes

    Science.gov (United States)

    Olivares, Ignacio E.; González, Iván A.

    2016-10-01

    We study Doppler-limited laser intensity absorption, in a thermal lithium vapor containing 7Li and 6Li atoms in a 9 to 1 ratio, using a narrow-linewidth single-longitudinal-mode tunable external cavity diode laser at the wavelength of 670.8 nm. The lithium vapor was embedded in helium or argon buffer gas. The spectral lineshapes were rigorously predicted for D_1 and D_2 for the lithium 6 and 7 isotope lines using reduced optical Bloch equations, specifically derived, from a density matrix analysis. Here, a detailed comparison is provided of the predicted lineshapes with the measured 7Li-D_2, 7Li-D_1, 6Li-D_2 and 6Li-D_1 lines, in the case of high vapor density and with intensity above the saturation intensity. To our knowledge, this is the first time that such detailed comparison is reported in the open literature. The calculations were also extended to saturated absorption spectra and compared to measured Doppler-free 7Li-D_2 and 6Li-D_2 hyperfine lines.

  5. Sol-gel chemistry synthesis and DTA-TGA, XRPD, SIC and {sup 7}Li, {sup 31}P, {sup 29}Si MAS-NMR studies on the Li-NASICON Li{sub 3}Zr{sub 2-y}Si{sub 2-4y}P{sub 1+4y}O{sub 12} (0 Less-Than-Or-Slanted-Equal-To y Less-Than-Or-Slanted-Equal-To 0.5) system

    Energy Technology Data Exchange (ETDEWEB)

    Belam, W., E-mail: WahidBelam@yahoo.fr [Chemistry Department, Bizerta Science Faculty, 7021 Jarzouna, Bizerta (Tunisia)

    2013-02-25

    Highlights: Black-Right-Pointing-Pointer The samples of Li-NASICON were elaborated by sol-gel chemistry. Black-Right-Pointing-Pointer The calcined temperatures of the studied samples were deduced from their thermograms. Black-Right-Pointing-Pointer The recorded X-ray powder diffractograms were indexed in the rhombohedral system. Black-Right-Pointing-Pointer The synthesized Li-NASICON materials are excellent lithium fast cation conductors. - Abstract: Five selected compounds of Li-NASICON, Li{sub 3}Zr{sub 2-y}Si{sub 2-4y}P{sub 1+4y}O{sub 12} (0 Less-Than-Or-Slanted-Equal-To y Less-Than-Or-Slanted-Equal-To 0.5), were synthesized by sol-gel chemistry in order to obtain pure polycrystalline powder and then analyzed by different physicochemical characterizations such as coupled DTA (differential thermal analysis)-TGA (thermogravimetric analysis), XRPD (X-ray powder diffraction), CIS (complex impedance spectroscopy) and MAS (magic angle spinning)-NMR (nuclear magnetic resonance). So the calcined temperature of each sample has been deduced from its corresponding DTA-TGA thermogram. However, the recorded X-ray powder diffractograms were indexed in the rhombohedral system with R3{sup Macron }c space group which corresponds to the ideal structure of NASICON. Whereas, the complex impedance spectroscopy study showed that these Li-NASICON materials are excellent lithium fast cation conductors with total electric conductivity maximal value 1.97 Multiplication-Sign 10{sup -3} S cm{sup -1} at 293 K in the case of Li{sub 3}Zr{sub 1.5}P{sub 3}O{sub 12}. Furthermore, {sup 7}Li, {sup 31}P and {sup 29}Si MAS-NMR spectroscopy study and DFT/B3LYP theoretical calculations of chemical shifts were performed to discuss the ambiguousness that exists between the resonance peak number in the experimental spectrum and the crystallographic site number relative to Li{sub 3}Zr{sub 2}Si{sub 2}PO{sub 12}.

  6. Lithium isotopic abundances in metal-poor halo stars

    CERN Document Server

    Asplund, M; Nissen, P E; Primas, F; Smith, V V; Asplund, Martin; Lambert, David L.; Nissen, Poul Erik; Primas, Francesca; Smith, Verne V.

    2005-01-01

    Very high-quality spectra of 24 metal-poor halo dwarfs and subgiants have been acquired with ESO's VLT/UVES for the purpose of determining Li isotopic abundances. The derived 1D, non-LTE 7Li abundances from the LiI 670.8nm line reveal a pronounced dependence on metallicity but with negligible scatter around this trend. Very good agreement is found between the abundances from the LiI 670.8nm line and the LiI 610.4nm line. The estimated primordial 7Li abundance is $7Li/H = 1.1-1.5 x 10^-10, which is a factor of three to four lower than predicted from standard Big Bang nucleosynthesis with the baryon density inferred from the cosmic microwave background. Interestingly, 6Li is detected in nine of our 24 stars at the >2sigma significance level. Our observations suggest the existence of a 6Li plateau at the level of log 6Li = 0.8; however, taking into account predictions for 6Li destruction during the pre-main sequence evolution tilts the plateau such that the 6Li abundances apparently increase with metallicity. Ou...

  7. Nucleon polarization in three-body models of polarized \\bbox{^6}Li

    CERN Document Server

    Schellingerhout, N W; Coon, S A; Adam, R M

    1993-01-01

    Just as $^3\\roarrow{\\rm He}$ can be approximately characterized as a polarized neutron target, polarized \\Li6D has been advocated as a good {\\em isoscalar} nuclear target for the extraction of the polarized gluon content of the nucleon. The original argument rests upon a presumed ``alpha + deuteron'' picture of \\Li6, with the polarization of the nucleus carried by the polarization of the deuteron. We have calculated the polarization of the constituents of \\Li6 as a three-body bound state of $\\alpha + n + p$ interacting with local potentials fitted to the scattering data. It is necessary to include partial waves up to $j=17/2$ (75 channels, or, when including the $T=1$ state, 150 channels) in the Faddeev equations before the energy eigenvalue converges. The longitudinal formfactors are then described well by the wave function. Various combinations of $\\alpha$N and NN strong and Coulomb potentials yield a straight line in the charge radius {\\em vs.} energy plane which, unlike those of previous calculations, pas...

  8. Geometric Scaling of Efimov States in a 6Li - 133Cs Mixture

    Science.gov (United States)

    Tung, Shih-Kuang; Jiménez-García, Karina; Johansen, Jacob; Parker, Colin V.; Chin, Cheng

    2014-12-01

    In few-body physics, Efimov states are an infinite series of three-body bound states that obey universal discrete scaling symmetry when pairwise interactions are resonantly enhanced. Despite abundant reports of Efimov states in recent cold atom experiments, direct observation of the discrete scaling symmetry remains an elusive goal. Here we report the observation of three consecutive Efimov resonances in a heteronuclear Li-Cs mixture near a broad interspecies Feshbach resonance. The positions of the resonances closely follow a geometric series 1, λ , λ2. The observed scaling constant λexp=4.9 (4 ) is in good agreement with the predicted value of 4.88.

  9. Determination of $^{6}Li - ^{4}He$ interaction from multi-energy scattering data

    CERN Document Server

    MacIntosh, R S; Kukulin, V I

    1999-01-01

    We present the first successful potential model description of Li-6 -- He-4 scattering. The differential cross-sections for three energies and the vector analyzing powers for two energies were fitted by a single potential with energy dependent imaginary components. An essential ingredient is a set of Majorana terms in each component. The potential was determined using a recently developed direct data-to-potential inversion method which is a generalisation of the IP S-matrix-to-potential inversion algorithm. We discuss the problems related to this phenomenological approach, and discuss the relationship of our results to existing and future theories.

  10. Development and Characterization of 6Li-doped Liquid Scintillator Detectors for PROSPECT

    Science.gov (United States)

    Gaison, Jeremy; Prospect Collaboration

    2016-09-01

    PROSPECT, the Precision Reactor Oscillation and Spectrum experiment, is a phased reactor antineutrino experiment designed to search for eV-scale sterile neutrinos via short-baseline neutrino oscillations and to make a precision measurement of the 235U reactor antineutrino spectrum. A multi-ton, optically segmented detector will be deployed at Oak Ridge National Laboratory's (ORNL) High Flux Isotope Reactor (HFIR) to measure the reactor spectrum at baselines ranging from 7-12m. A two-segment detector prototype with 50 liters of active liquid scintillator target has been built to verify the detector design and to benchmark its performance. In this presentation, we will summarize the performance of this detector prototype and describe the optical and energy calibration of the segmented PROSPECT detectors.

  11. A Solution to Lithium Problem by Long-Lived Stau

    CERN Document Server

    Sato, Joe; Yamanaka, Masato

    2016-01-01

    We review a non-standard Big-Bang nucleosynthesis (BBN) scenario within the minimal supersymmetric standard model, and propose an idea to solve both ${}^{7}$Li and ${}^{6}$Li problems. Each problem is a discrepancy between the predicted abundance in the standard BBN and observed one. We focus on the stau, a supersymmetric partner of tau lepton, which is a long-lived charged particle when it is the next lightest supersymmetric particle and is degenerate in mass with the lightest supersymmetric particle. The long-lived stau forms a bound state with a nucleus, and provide non-standard nuclear reactions. One of those, the internal conversion process, accelerates the destruction of ${}^{7}$Be and ${}^{7}$Li, and leads to a solution to the ${}^{7}$Li problem. On the other hand, the bound state of the stau and ${}^{4}$He enhances productions of n, d, t, and ${}^{6}$Li. The over-production of ${}^{6}$Li could solve the ${}^{6}$Li problem. While, the over-productions of d and t could conflict with observations, and th...

  12. Investigation of DNA Damage Induced by 7Li and 12C Ions

    Institute of Scientific and Technical Information of China (English)

    SUILi; ZHAOKui; NIMei-nan; GUOJi-yu; LUOHong-bing; MEIJun-ping; KONGFu-quan; LUXiu-qin; ZHOUPing

    2003-01-01

    Deoxyribonucleic acid(DNA) is an important biomacromolecule. It is a carrier of genetic information and a critical target for radiobiological effects. Numerous lesions have been identified in irradiated DNA.DNA double strand breaks (DSBs) are considered as the most important initial damage of all biological effects induced by ionizing radiation. The goal of this experiment is to investigate DNA DSBs induced by heavy ions with atomic force microscopy (AFM).

  13. Study of the Pion Production Mechanisms in Nucleus-Nucleus Collisions at the CERN SC using the Omicron Spectrometer

    CERN Multimedia

    2002-01-01

    The aim of this experiment is to study the pion production mechanism in nucleus-nucleus collisions with the |3He and |1|2C beams of the CERN SC using the Omicron Spectrometer. The high intensity ion beams delivered now by the SC combined with the favourable characteristics of the Omicron Spectrometer offer a unique possibility of measuring very low cross-sections (typically in the order of 1 pb/(sr~MeV/c). In a first stage we will measure with an energy resolution of about 3~MeV the spectra of @p@+ emitted at 0|0 in two-body reactions induced by |3He ions of 910~MeV on targets of |6Li, |7Li, |9Be and |1|2C. The aim is to understand the reaction mechanisms and the nuclear wave functions most appropriate to describe the formation of nuclear bound states at momentum transfers of about 1.6@/1.7~GeV/c. The apparatus is shown in the figure. The same instrument will allow the measurement of the @p@+ inclusive spectra emitted at 0|0 after the interaction of the |1|2C|4|+ beam at 1032 MeV with the same targets. At 86 ...

  14. Production of secondary particles and nuclei in cosmic rays collisions with the interstellar gas using the FLUKA code

    CERN Document Server

    Mazziotta, M N; Ferrari, A; Gaggero, D; Loparco, F; Sala, P R

    2016-01-01

    The measured fluxes of secondary particles produced by the interactions of Cosmic Rays (CRs) with the astronomical environment play a crucial role in understanding the physics of CR transport. In this work we present a comprehensive calculation of the secondary hadron, lepton, gamma-ray and neutrino yields produced by the inelastic interactions between several species of stable or long-lived cosmic rays projectiles (p, D, T, 3He, 4He, 6Li, 7Li, 9Be, 10Be, 10B, 11B, 12C, 13C, 14C, 14N, 15N, 16O, 17O, 18O, 20Ne, 24Mg and 28Si) and different target gas nuclei (p, 4He, 12C, 14N, 16O, 20Ne, 24Mg, 28Si and 40Ar). The yields are calculated using FLUKA, a simulation package designed to compute the energy distributions of secondary products with large accuracy in a wide energy range. The present results provide, for the first time, a complete and self-consistent set of all the relevant inclusive cross sections regarding the whole spectrum of secondary products in nuclear collisions. We cover, for the projectiles, a ki...

  15. Two-dimensional cross-section sensitivity and uncertainty analysis of the LBM (Lithium Blanket Module) experiments at LOTUS

    Energy Technology Data Exchange (ETDEWEB)

    Davidson, J.W.; Dudziak, D.J.; Pelloni, S.; Stepanek, J.

    1988-01-01

    In a recent common Los Alamos/PSI effort, a sensitivity and nuclear data uncertainty path for the modular code system AARE (Advanced Analysis for Reactor Engineering) was developed. This path includes the cross-section code TRAMIX, the one-dimensional finite difference S/sub N/-transport code ONEDANT, the two-dimensional finite element S/sub N/-transport code TRISM, and the one- and two-dimensional sensitivity and nuclear data uncertainty code SENSIBL. Within the framework of the present work a complete set of forward and adjoint two-dimensional TRISM calculations were performed both for the bare, as well as for the Pb- and Be-preceeded, LBM using MATXS8 libraries. Then a two-dimensional sensitivity and uncertainty analysis for all cases was performed. The goal of this analysis was the determination of the uncertainties of a calculated tritium production per source neutron from lithium along the central Li/sub 2/O rod in the LBM. Considered were the contributions from /sup 1/H, /sup 6/Li, /sup 7/Li, /sup 9/Be, /sup nat/C, /sup 14/N, /sup 16/O, /sup 23/Na, /sup 27/Al, /sup nat/Si, /sup nat/Cr, /sup nat/Fe, /sup nat/Ni, and /sup nat/Pb. 22 refs., 1 fig., 3 tabs.

  16. Influence of projectile breakup on complete fusion

    Indian Academy of Sciences (India)

    A Mukherjee; M K Pradhan

    2010-07-01

    Complete fusion excitation functions for 11,10B+159Tb and 6,7Li+159Tb have been reported at energies around the respective Coulomb barriers. The measurements show significant suppression of complete fusion cross-sections at energies above the barrier for 10B+159Tb and 6,7Li+159Tb reactions, when compared to those for 11B+159Tb. The comparison shows that the extent of suppression of complete fusion cross-sections is correlated with the -separation energies of the projectiles. Also, the measured incomplete fusion cross-sections show that the -particle emanating channel is the favoured incomplete fusion process. Inclusive measurement of the -particles produced in 6Li+159Tb reaction has been carried out. Preliminary CDCC calculations carried out to estimate the - yield following 6Li breaking up into + fail to explain the measured -yield. Transfer processes seem to be important contributors.

  17. Identification of a $9/2^-$[505] isomer in the neutron-rich $^{193}$Os nucleus

    OpenAIRE

    Gao, B. S.; Zhou, X. H.; Fang, Y. D.; Zhang, Y.H.; Liu, M.L.; Wang, S C; Wang, J.G.; F. Ma; Guo, Y. X.; Wu, X. G.; He, C.Y.(China Institute of Atomic Energy, Beijing, 102413, China); Zheng, Y.; Wang, Z. M.; Yan, X. L.; Wang, Z.G.

    2013-01-01

    The neutron rich nucleus $^{193}$Os was produced in the $^{192}$Os($^{7}$Li,$^{6}$Li)$^{193}$Os reaction. An isomeric state based on the $9/2^-$[505] nilsson orbital was identified in the present work. Half-life of the isomeric state was extracted and discussed in terms of the $K$ quantum number. Level scheme built on the isomeric state was proposed based on the experimental data.

  18. Radiation-Induced Color Centers in LiF for Dosimetry at High Absorbed Dose Rates

    DEFF Research Database (Denmark)

    McLaughlin, W. L.; Miller, Arne; Ellis, S. C.

    1980-01-01

    Color centers formed by irradiation of optically clear crystals of pure LiF may be analyzed spectrophotometrically for dosimetry in the absorbed dose range from 102 to 107 Gy. Routine monitoring of intense electron beams is an important application. Both 6LiF and 7LiF forms are commercially avail...... available, and when used with filters as albedo dosimeters in pairs, they provide discrimination of neutron and gamma-ray doses....

  19. α and 3He production in the 7Be+28Si reaction at near-barrier energies: Direct versus compound-nucleus mechanisms

    Science.gov (United States)

    Sgouros, O.; Pakou, A.; Pierroutsakou, D.; Mazzocco, M.; Acosta, L.; Aslanoglou, X.; Betsou, Ch.; Boiano, A.; Boiano, C.; Carbone, D.; Cavallaro, M.; Grebosz, J.; Keeley, N.; La Commara, M.; Manea, C.; Marquinez-Duran, G.; Martel, I.; Nicolis, N. G.; Parascandolo, C.; Rusek, K.; Sánchez-Benítez, A. M.; Signorini, C.; Soramel, F.; Soukeras, V.; Stefanini, C.; Stiliaris, E.; Strano, E.; Strojek, I.; Torresi, D.

    2016-10-01

    The production of α and 3He particles, the cluster constituents of 7Be, in the 7Be+28Si reaction was studied at three near-barrier energies, namely 13, 20, and 22 MeV. Angular distribution measurements were performed at each energy, and the data were analyzed in both statistical model and Distorted-Wave Born Approximation (DWBA) frameworks in order to disentangle the degree of competition between direct and compound channels. The energy evolution of the ratio of direct to total reaction cross section was mapped in comparison with similar data for 6Li and 7Li projectiles on a 28Si target. The results indicate larger transfer contributions for collisions involving the mirror nuclei 7Be and 7Li than in the 6Li case. Fusion cross sections were deduced, taking into account the α -particle cross sections due to compound-nucleus formation and particle multiplicities deduced from our statistical model framework. It was found that fusion is compatible with systematics and single-barrier penetration cross sections to within an uncertainty band of 10% to 20%. Indications of fusion hindrance for 7Li and 7Be compared to 6Li, starting from the barrier and below it, are given. This hindrance is attributed to the existence of large transfer channels. Furthermore, the experimental results, analyzed in the DWBA framework, suggest 3He and 4He transfer as the dominant direct reaction mechanism.

  20. SoLid: Search for Oscillation with a 6Li Detector at the BR2 research reactor

    CERN Document Server

    Michiels, Ianthe

    2016-01-01

    In the past decades, various nuclear reactor neutrino experiments have measured a deficit in the flux of antineutrinos coming from the reactor at short reactor-detector distances, when compared to theoretical calculations. One of the experiments designed to investigate this reactor antineutrino anomaly is the SoLid experiment. It uses the compact BR2 research reactor from the SCK-CEN in Mol, Belgium, to perform reactor antineutrino flux measurements at very short baseline. These proceedings discuss the general detection concepts of the SoLid experiment and its novel detector technology. The performance of the SoLid design is demonstrated with some results of the analysis of the data gathered with the experiment's first large scale test module, SM1.

  1. All-optical production and transport of a large $^6$Li quantum gas in a crossed optical dipole trap

    CERN Document Server

    Gross, Ch; Dieckmann, K

    2016-01-01

    We report on an efficient production scheme for a large quantum degenerate sample of fermionic lithium. The approach is based on our previous work on narrow-line $ 2S_{1/2}\\rightarrow 3P_{3/2} $ laser cooling resulting in a high phase-space density of up to $3\\times10^{-4}$. This allows utilizing a large volume crossed optical dipole trap with a total power of $45\\,\\textrm{W}$, leading to high loading efficiency and $8\\times10^6$ trapped atoms. The same optical trapping configuration is used for rapid adiabatic transport over a distance of $25\\,\\textrm{cm}$ in $0.9\\,\\textrm{s}$, and subsequent evaporative cooling. With optimized evaporation we achieve a degenerate Fermi gas with $1.7\\times 10^{6}$ atoms at a temperature of $60 \\, \\textrm{nK}$, corresponding to $T/T_{\\text{F}}=0.16\\left(2 \\right)$. Furthermore, the performance is demonstrated by evaporation near a broad Feshbach resonance creating a molecular Bose-Einstein condensate of $3\\times10^5$ lithium dimers.

  2. Immunofluorescence Detection of γ-H2AX Foci Induced by ~7Li Ions and γ-rays Radiation

    Institute of Scientific and Technical Information of China (English)

    2011-01-01

    DNA double strand breaks (DSBs) are considered as the most critical type of lesions. Correct and complete repair of DSBs guarantees cellular survival, while incorrect repair and residual DNA damage may lead to cell killing, mutation or transformation. Following induction of DNA double strand breaks,

  3. Optical absorption of isotopically enriched Li{sub 2}B{sub 4}O{sub 7} single crystals irradiated by thermal neutrons

    Energy Technology Data Exchange (ETDEWEB)

    Burak, Ya.V. E-mail: burak@ifo.lviv.ua; Adamiv, V.T.; Teslyuk, I.M.; Shevel, V.M

    2004-12-01

    Induced absorption spectra in the range 200-900 nm at 77 and 290 K for Li{sub 2}B{sub 4}O{sub 7} single crystals, isotopically Li and B enriched are presented after irradiation of these crystals by thermal neutrons with fluence 1.8x10{sup 16} cm{sup -2}. The dependence of induced absorption spectra on the isotope composition was revealed: for {sup 6}Li{sub 2}{sup 10}B{sub 4}O{sub 7} and {sup 7}Li{sub 2}{sup 10}B{sub 4}O{sub 7} crystals intensive band in the region of 280-294 nm was observed. Under substitution of {sup 7}Li isotope by {sup 6}Li in the lithium tetraborate lattice no changes in the absorption spectra were observed. The nuclear reaction {sup 10}B(n,{alpha}){sup 7}Li is proposed to be the main mechanism of formation of the radiation defects.

  4. 2p1v states populated in 135Te from 9Be induced reactions with a 132Sn beam

    Energy Technology Data Exchange (ETDEWEB)

    Allmond, James M [ORNL; Stuchbery, Andrew E [ORNL; Brown, Alex [National Superconducting Cyclotron Laboratory (NSCL), Michigan State University; Beene, James R [ORNL; Galindo-Uribarri, Alfredo {nmn} [ORNL; Gross, Carl J [ORNL; Liang, J Felix [ORNL; Padilla-Rodal, Elizabeth [Universidad Nacional Autonoma de Mexico (UNAM); Radford, David C [ORNL; Varner Jr, Robert L [ORNL; Ayres, A. [University of Tennessee, Knoxville (UTK); Batchelder, J. C. [Oak Ridge Associated Universities (ORAU); Bey, A. [University of Tennessee, Knoxville (UTK); Bingham, C. R. [University of Tennessee, Knoxville (UTK); Howard, Meredith E [ORNL; Jones, K. L. [University of Tennessee, Knoxville (UTK); Manning, Brett M [ORNL; Mueller, Paul Edward [ORNL; Nesaraja, Caroline D [ORNL; Pain, Steven D [ORNL; Peters, William A [ORNL; Ratkiewicz, Andrew J [ORNL; Schmitt, Kyle [University of Tennessee, Knoxville (UTK); Shapira, Dan [ORNL; Smith, Michael Scott [ORNL; Stone, N. J. [University of Tennessee, Knoxville (UTK); Stracener, Daniel W [ORNL; Yu, Chang-Hong [ORNL

    2014-01-01

    Gamma-ray transitions in $^{134}$\\textrm{Te}, $^{135}$\\textrm{Te}, and $^{136}$\\textrm{Te} were measured from $^{9}$\\textrm{Be} induced reactions with a radioactive $^{132}$\\textrm{Sn} beam at a sub-Coulomb barrier energy of $3$~MeV per nucleon using particle-$\\gamma$ coincidence spectroscopy. The transitions were selected by gating on alpha-like particles in a \\textrm{CsI} detector following a combination of ($^{9}$\\textrm{Be},$\\alpha 1n$), ($^{9}$\\textrm{Be},$\\alpha 2n$), and ($^{9}$\\textrm{Be},$\\alpha 3n$) reactions. Distorted wave Born approximation calculations suggest little to no contribution from the ($^{9}$\\textrm{Be},$^{7}$\\textrm{He}), ($^{9}$\\textrm{Be},$^{6}$\\textrm{He}), and ($^{9}$\\textrm{Be},$^{5}$\\textrm{He}) direct reactions. Gamma-ray transitions from previously known $2^+\\otimes \

  5. Thermoluminescence measurements of neutron streaming through JET Torus Hall ducts

    Energy Technology Data Exchange (ETDEWEB)

    Obryk, Barbara, E-mail: barbara.obryk@ifj.edu.pl [Institute of Nuclear Physics Polish Academy of Sciences, Radzikowskiego 152, 31-342 Kraków (Poland); Batistoni, Paola [Associazione EURATOM-ENEA sulla Fusione, Via Enrico Fermi 45, 00044 Frascati, Rome (Italy); EURATOM–CCFE Fusion Association, Culham Science Centre, Abingdon OX14 3DB (United Kingdom); Conroy, Sean [EURATOM-VR Association, Department of Physics and Astronomy, Uppsala University, Box 516, 75120 Uppsala (Sweden); EURATOM–CCFE Fusion Association, Culham Science Centre, Abingdon OX14 3DB (United Kingdom); Syme, Brian D.; Popovichev, Sergey [EURATOM–CCFE Fusion Association, Culham Science Centre, Abingdon OX14 3DB (United Kingdom); Stamatelatos, Ion E.; Vasilopoulou, Theodora [Institute of Nuclear and Radiological Sciences, Energy, Technology and Safety, NCSR “Demokritos”, Athens (Greece); Bilski, Paweł [Institute of Nuclear Physics Polish Academy of Sciences, Radzikowskiego 152, 31-342 Kraków (Poland)

    2014-10-15

    Highlights: •Thermoluminescence detectors (TLDs) were used for dose measurements at JET. •Pairs of {sup 6}LiF/{sup 7}LiF TLDs allow to measure thermal neutron component of a radiation field. •For detection of neutrons of higher energy, polyethylene (PE-300) moderators were used. •TLDs were installed at eleven positions in the JET hall and the hall labyrinth. •The experimental results are compared with calculations using the MCNP code. -- Abstract: Thermoluminescence detectors (TLD) were used for dose measurements at JET. Several hundreds of LiF detectors of various types, standard LiF:Mg,Ti and highly sensitive LiF:Mg,Cu,P were produced. LiF detectors consisting of natural lithium are sensitive to slow neutrons, their response to neutrons being enhanced by {sup 6}Li-enriched lithium or suppressed by using lithium consisting entirely of {sup 7}Li. Pairs of {sup 6}LiF/{sup 7}LiF detectors allow distinguishing between neutron/non-neutron components of a radiation field. For detection of neutrons of higher energy, polyethylene (PE-300) moderators were used. TLDs, located in the centre of cylindrical moderators, were installed at eleven positions in the JET hall and the hall labyrinth in July 2012, and exposure took place during the last two weeks of the experimental campaign. Measurements of the gamma dose were obtained for all positions over a range of about five orders of magnitude variation. As the TLDs were also calibrated in a thermal neutron field, the neutron fluence at the experimental position could be derived. The experimental results are compared with calculations using the MCNP code. The results confirm that the TLD technology can be usefully applied to measurements of neutron streaming through JET Torus Hall ducts.

  6. Laserspectroscopic investigations of the lithium- D-lines in magnetic fields

    Science.gov (United States)

    Windholz, L.; Jäger, H.; Musso, M.; Zerza, G.

    1990-03-01

    Laser-atomic-beam investigations of the lithium D 1- and D 2-line in magnetic fields were performed using cw-laser excitation and fluorescence detection. For both isotopes6Li and7Li, the hyperfine splittings of the ground level 22 S 1/2 and the upper level of the D 1-line, 22 P 1/2, as well as the isotopic shifts of the D 1- and the D 2-line were determined from the registrations without field. In magnetic fields, Zeeman- and Paschen-Back-effects of the lines were studied. Using the Zeeman pattern of the D 1-line for a calibration of the field strength, values for the hyperfine constants A and B of the 22 P 3/2-level of7Li could be derived from the Zeeman pattern of the D 2-line.

  7. Bethe logarithm and QED shift for lithium.

    Science.gov (United States)

    Yan, Zong-Chao; Drake, G W F

    2003-09-12

    A novel finite basis set method is used to calculate the Bethe logarithm for the ground 2 (2)S(1/2) and excited 3 (2)S(1/2) states of lithium. The basis sets are constructed to span a huge range of distance scales within a single calculation, leading to well-converged values for the Bethe logarithm. The results are used to calculate an accurate value for the complete quantum electrodynamic energy shift up to order alpha(3) Ry. The calculated 3 (2)S(1/2)-2 (2)S(1/2) transition frequency for 7Li is 27 206.092 6(9) cm(-1), and the ionization potential for the 2 (2)S(1/2) state is 43 487.158 3(6) cm(-1). The 7Li-6Li isotope shift is also considered, and all the results compared with experiment.

  8. Target structure independent $^7\\vec{Li}$ elastic scattering at low momentum transfers

    CERN Document Server

    Momotyuk, O A; Crisp, A M; Keeley, N; Kemper, K W; Liendo, J; Maréchal, F; Mezhevych, S Y; Roeder, B T; Rusek, K; Schmidt, B G; Wiedeking, M

    2006-01-01

    Analyzing powers and cross sections for the elastic scattering of polarized 7Li by targets of 6Li, 7Li and 12C are shown to depend only on the properties of the projectile for momentum transfers of less than 1.0 fm-1. The result of a detailed analysis of the experimental data within the framework of the coupled channels model with ground state reorientation and transitions to the excited states of the projectile and targets included in the coupling schemes are presented. This work suggests that nuclear properties of weakly-bound nuclei can be tested by elastic scattering experiments, independent of the target used, if data are acquired for momentum transfers less than ~1.0 fm-1.

  9. Quantum Defect Theory description of weakly bound levels and Feshbach resonances in LiRb

    CERN Document Server

    Pérez-Ríos, Jesús; Chen, Yong P; Greene, Chris H

    2014-01-01

    The multichannel quantum defect theory (MQDT) in combination with the frame transformation (FT) approach is applied to model the Fano-Feshbach resonances measured for $^{7}$Li$^{87}$Rb and $^{6}$Li$^{87}$Rb [Marzok {\\it et al.} Phys. Rev. A {\\bf 79} 012717 (2009)]. The MQDT results show a level of accuracy comparable to that of previous models based on direct, fully numerical solutions of the the coupled channel Schr\\"odinger equations (CC). Here, energy levels deduced from 2-photon photoassociation spectra for $^{7}$Li$^{85}$Rb are assigned by applying the MQDT approach, obtaining the bound state energies for the coupled channel problem. Our results confirm that MQDT yields a compact description of photoassociation observables as well as the Fano-Feshbach resonance positions and widths.

  10. Coupled-channels effects in elastic scattering and near-barrier fusion induced by weakly bound nuclei and exotic halo nuclei

    Energy Technology Data Exchange (ETDEWEB)

    Beck, C. [Institut Pluridisciplinaire Hubert Curien, UMR 7178, IN2P3-CNRS et Universite Louis Pasteur (Strasbourg I), 23 rue du Loess - BP28, F-67037 Strasbourg Cedex 2 (France); Keeley, N. [DSM/DAPNIA/SPhN CEA Saclay, Orme des Merisiers, F-91191 Gif-sur-Yvette Cedex (France); Diaz-Torres, A. [Department of Nuclear Physics, Research School of Physical Sciences and Engineering, The Australian National University, Canberra ACT 0200 (Australia)

    2007-03-15

    The influence on fusion of coupling to the breakup process is investigated for reactions where at least one of the colliding nuclei has a sufficiently low binding energy for breakup to become an important process. Elastic scattering, excitation functions for sub-and near-barrier fusion cross sections, and breakup yields are analyzed for {sup 6,7}Li+{sup 59}Co. Continuum-Discretized Coupled-Channels (CDCC) calculations describe well the data at and above the barrier. Elastic scattering with {sup 6}Li (as compared to {sup 7}Li) indicates the significant role of breakup for weakly bound projectiles. A study of {sup 4,6}He induced fusion reactions with a three-body CDCC method for the {sup 6}He halo nucleus is presented. The relative importance of breakup and bound-state structure effects on total fusion is discussed. (authors)

  11. Coincidence in the two-photon spectra of Li and Li2 at 735 nm

    Science.gov (United States)

    DeGraffenreid, W.; Sansonetti, Craig J.

    2005-02-01

    A coincidence between the 22S1/2-32S1/2 two-photon transition in the atomic spectrum of 6Li and the X 1Σ+g→ E 1Σ+g two-photon ro-vibrational series of 7Li2 was observed near 735 nm in a heat pipe oven using a tunable laser and thermionic diode detection scheme. The molecular transition obscures one component of the 6Li atomic transition. Selective detection of the atomic transition was obtained by adding an intensity-modulated laser that drives atoms from the 3S to 16P state. The coincident molecular transition and four nearby molecular lines were identified using previously determined Dunham coefficients.

  12. Coincidence in the two-photon spectra of Li and Li{sub 2} at 735 nm

    Energy Technology Data Exchange (ETDEWEB)

    DeGraffenreid, W [Department of Physics and Astronomy, California State University, Sacramento, Sacramento, CA 95819-6041 (United States); Sansonetti, Craig J [National Institute of Standards and Technology, Gaithersburg, MD 20899-8422 (United States)

    2005-02-28

    A coincidence between the 2{sup 2}S{sub 1/2}-3{sup 2}S{sub 1/2} two-photon transition in the atomic spectrum of {sup 6}Li and the X {sup 1}{sigma}{sup +}{sub g}{yields} E {sup 1}{sigma}{sup +}{sub g} two-photon ro-vibrational series of {sup 7}Li{sub 2} was observed near 735 nm in a heat pipe oven using a tunable laser and thermionic diode detection scheme. The molecular transition obscures one component of the {sup 6}Li atomic transition. Selective detection of the atomic transition was obtained by adding an intensity-modulated laser that drives atoms from the 3S to 16P state. The coincident molecular transition and four nearby molecular lines were identified using previously determined Dunham coefficients.

  13. Infrared length scale and extrapolations for the no-core shell model

    CERN Document Server

    Wendt, K A; Papenbrock, T; Sääf, D

    2015-01-01

    We precisely determine the infrared (IR) length scale of the no-core shell model (NCSM). In the NCSM, the $A$-body Hilbert space is truncated by the total energy, and the IR length can be determined by equating the intrinsic kinetic energy of $A$ nucleons in the NCSM space to that of $A$ nucleons in a $3(A-1)$-dimensional hyper-radial well with a Dirichlet boundary condition for the hyper radius. We demonstrate that this procedure indeed yields a very precise IR length by performing large-scale NCSM calculations for $^{6}$Li. We apply our result and perform accurate IR extrapolations for bound states of $^{4}$He, $^{6}$He, $^{6}$Li, $^{7}$Li. We also attempt to extrapolate NCSM results for $^{10}$B and $^{16}$O with bare interactions from chiral effective field theory over tens of MeV.

  14. Dissociation Energies of Diatomic Molecules

    Institute of Scientific and Technical Information of China (English)

    FAN Qun-Chao; SUN Wei-Guo

    2008-01-01

    Molecular dissociation energies of 10 electronic states of alkali molecules of KH, 7LID, 7LiH, 6LiH, NaK, NaLi and NaRb are studied using the highest three accurate vibrational energies of each electronic state, and an improved parameter-free analytical formula which is obtained starting from the LeRoy-Bernstein vibrational energy expression near the dissociation limit. The results show that as long as the highest three vibrational energies are accurate, the current analytical formula will give accurate theoretical dissociation energies Detheory, which are in excellent agreement with the experimental dissociation energies Dexpte.

  15. 吉林陨石锂同位素相对丰度的初步探讨

    Institute of Scientific and Technical Information of China (English)

    李肇辉

    1977-01-01

    Relative abundances of lithium isotopes are determined for Kirin chcndric meteorite and Hainan tektite with ion microprobe mass spectrometer. The appareut results of 7Li/6Li are 17.03±7 and 12.18±1.67 for Kirin ehondric meteorite and Hainan tektite respectively. If this result can be taken as a reflection of the real case, an anomalous distribution with respect, to lithium isotopes in micro-area scale is thus evidenced in Kirin meteorites. Possible reasons are suggested for this anomaly,

  16. Several Light Nulcie Evaluations Testing With LLNL Pulsed Sphere Benchmarks

    Institute of Scientific and Technical Information of China (English)

    ZHANG; Huan-yu

    2012-01-01

    <正>In this work, Lawrence Livermore pulsed sphere experiments were modeled using Monte Carlo N-particle code (MCNP) for the purpose of benchmarking the new release of nuclear data librarys (CENDL-3[1], ENDF/B-Ⅶ.1[2], JENDL-4.0[3]). This program consisted of 12 different spheres, including 6 Li, 7Li, Be, C, N, O, LiD, Air, H2O, D2O, polythene and teflon. The calculated results were compared to experimental results[4-5].

  17. Spectroscopic Factors for Low-lying 16N Levels and Astrophysical 15N(n, γ)16N Reaction Rate

    Institute of Scientific and Technical Information of China (English)

    WU; Zhi-dan; GUO; Bing; LI; Zhi-hong; LI; Yun-ju; SU; Jun; PAN; Dan-yang; YAN; Sheng-quan; LI; Er-tao; BAI; Xi-xiang; DU; Xian-chao; FAN; Qi-wen; GAN; Lin; HE; Jian-jun; JIN; Sun-jun; JING; Long; LI; Long; LI; Zhi-chang; LIAN; Gang; LIU; Jian-cheng; SHEN; Yang-ping; WANG; You-bao; YU; Xiang-qing; ZENG; Sheng; ZHANG; Li-yong; ZHANG; Wei-jie; LIU; Wei-ping

    2013-01-01

    Fluorine is a key element for nucleosynthetic studies since it is extremely sensitive to the physical conditions within stars.The astrophysical site to produce fluorine is suggested to be asymptotic giant branch stars.In these stars the 15N(n,γ)16N reaction could affect the abundance of fluorine by competing with 15N(α,γ)19F.In the present work,the angular distribution of the 15N(7Li,6Li)16N reaction populating

  18. Formates and dithionates: sensitive EPR-dosimeter materials for radiation therapy

    Energy Technology Data Exchange (ETDEWEB)

    Lund, E. [Department of Medicine and Care, Radiation Physics, Faculty of Health Sciences, University of Linkoeping, S-581 85 Linkoeping (Sweden)]. E-mail: eva.lund@imv.liu.se; Gustafsson, H. [Department of Medicine and Care, Radiation Physics, Faculty of Health Sciences, University of Linkoeping, S-581 85 Linkoeping (Sweden); Danilczuk, M. [Chemical Physics Laboratory, IFM, University of Linkoeping, S-581 83 Linkoeping (Sweden); Sastry, M.D. [Chemical Physics Laboratory, IFM, University of Linkoeping, S-581 83 Linkoeping (Sweden); Lund, A. [Chemical Physics Laboratory, IFM, University of Linkoeping, S-581 83 Linkoeping (Sweden); Vestad, T.A. [Department of Physics, University of Oslo, P.O. Box 1048 Blindern, N-0316 Oslo (Norway); Malinen, E. [Department of Physics, University of Oslo, P.O. Box 1048 Blindern, N-0316 Oslo (Norway); Hole, E.O. [Department of Physics, University of Oslo, P.O. Box 1048 Blindern, N-0316 Oslo (Norway); Sagstuen, E. [Department of Physics, University of Oslo, P.O. Box 1048 Blindern, N-0316 Oslo (Norway)

    2005-02-01

    Polycrystalline formates and dithionates are promising materials for EPR dosimetry, as large yields of radiation induced stable radicals are formed with a linear dose response. Rapid spin relaxation rates were detected in many of the substances, indicating that a high microwave power can be applied during EPR acquisition in order to improve sensitivity. Different techniques used to further improve the sensitivity, such as the replacement of {sup 7}Li with {sup 6}Li or exchange of protons with deuterons in the corresponding crystalline matrices and metal ion doping are discussed. It is concluded that formates and dithionates may be up to 10 times as sensitive as L-{alpha}-alanine.

  19. Production of {sup 48}V in a nuclear reactor via secondary tritons

    Energy Technology Data Exchange (ETDEWEB)

    Siri, S. [Comision Nacional de Energia Atomica, Centro Atomico Ezeiza, Gerencia de Capacitacion, Quimica Nuclear y Ciencias de la Salud, Ezeiza, Buenos Aires (Argentina); Cohen, I.M. [Univ. Tecnologica Nacional, Dept. de Ingenieria Quimica, Buenos Aires (Argentina)

    2009-07-01

    The production of {sup 48}V in a nuclear reactor, induced on titanium by tritons generated from the {sup 6}Li(n, t){sup 4} He reaction, and eventually {sup 7}Li(n, n't){sup 4}He, is described. Samples of lithium titanate were irradiated for an irradiation cycle (120 h) in the RA-3 reactor, belonging to Ezeiza Atomic Centre. After a radiochemical separation, the characteristic radiations from {sup 48}V were identified in the gamma ray spectra of the vanadium fractions. (orig.)

  20. Investigating sorption on iron-oxyhydroxide soil minerals by solid-state NMR spectroscopy: a 6Li MAS NMR study of adsorption and absorption on goethite

    DEFF Research Database (Denmark)

    Nielsen, Ulla Gro; Paik, Younkee; Julmis, Keinia;

    2005-01-01

    High-resolution 2H MAS NMR spectra can be obtained for nanocrystalline particles of goethite (alpha-FeOOH, particle size approximately 4-10 nm) at room temperature, facilitating NMR studies of sorption under environmentally relevant conditions. Li sorption was investigated as a function of pH, th...

  1. Production of antimatter $^{5,6}$Li nuclei in central Au+Au collisions at $\\sqrt{s_{NN}} = 200$ GeV

    CERN Document Server

    Sun, Kai-Jia

    2015-01-01

    Combining the covariant coalescence model and a blast-wave-like analytical parametrization for (anti-)nucleon phase-space freezeout configuration, we explore light (anti-)nucleus production in central Au+Au collisions at $\\sqrt{s_{NN}} = 200$ GeV. Using the nucleon freezeout configuration (denoted by FO1) determined from the measured spectra of protons (p), deutrons (d) and $^{3}$He, we find the predicted yield of $^{4}$He is significantly smaller than the experimental data. We show this disagreement can be removed by using a nucleon freezeout configuration (denoted by FO2) in which the nucleons are assumed to freeze out earlier than those in FO1 to effectively consider the effect of large binding energy value of $^{4}$He. Assuming the binding energy effect also exists for the production of $^5\\text{Li}$, $^5\\overline{\\text{Li}}$, $^6\\text{Li}$ and $^6\\overline{\\text{Li}}$ due to their similar binding energy values as $^{4}$He, we find the yields of these heavier (anti-)nuclei can be enhanced by a factor of a...

  2. Study of the $\\bm{p+^6}$Li$\\bm{\\to\\eta+^7}$Be reaction 11.3 MeV above threshold

    CERN Document Server

    Budzanowski, A; Hawranek, P; Jahn, R; Jha, V; Kilian, K; Kliczewski, S; Kirillov, Da; Kirillov, Di; Kolev, D; Kravcikova, M; Lesiak, M; Lieb, J; Machner, H; Magiera, A; Maier, R; Martinska, G; Piskunov, N; Protić, D; Ritman, J; von Rossen, P; Roy, B J; Sitnik, I; Siudak, R; Tsenov, R; Urban, J; Vankova, G

    2010-01-01

    The cross section for the reaction $p+^6\\text{Li}\\to\\eta+^7\\text{Be}$ was measured at an excess energy of 11.28 MeV above threshold by detecting the recoiling $^7$Be nuclei. A dedicated set of focal plane detectors was built for the magnetic spectrograph Big Karl and was used for identification and four momentum measurement of the $^7$Be. A differential cross section of $\\frac{d\\sigma}{d\\Omega}=(0.69\\pm{0.20}\\text{(stat.)}\\pm 0.20\\text{(syst.)})\\text{nb/sr}$ for the ground state plus the 1/2$^-$ was measured. The result is compared to model calculations.

  3. A universal, post Big-Bang Nucleo-synthesis, pre-Galactic, origin of the Lithium (Spite) Plateau

    CERN Document Server

    Ouyed, Rachid

    2012-01-01

    (Abridged abstract) We investigate the lithium plateau in the context of primordial dual-shock quark novae (dsQNe; i.e. a QN occurring a few days to a few weeks following the preceding SN explosion) going off in the wake of Pop. III stars. The neutron-rich relativistic QN ejecta leads to spallation of 56Ni processed in the ejecta of the preceding SN ejecta and thus to "iron impoverishment" of the primordial gas swept by dsQNe. We show that the generation of stars formed from fragmentation of pristine clouds swept-up by dsQNe acquire a metallicity with -7.5 2 (and up to [C/Fe] ~ 5) can be accounted for in our model for dsQNe with t_delay 10-11 days (i.e. [Fe/H] > -3). For shorter delays the temperature of the SN shell is too hot (> 2.5x10^6 K) for the spallated 7Li to survive. We find a corresponding 6Li plateau with 6Li/7Li < 0.3.

  4. Isotope shifts and transition frequencies for the S and P states of lithium: Bethe logarithms and second-order relativistic recoil

    Science.gov (United States)

    Wang, L. M.; Li, Chun; Yan, Z.-C.; Drake, G. W. F.

    2017-03-01

    Isotope shifts and total transition frequencies are calculated for the 2 2S-3 2S transition of the lithium isotopes 6Li, 7Li, 8Li, 9Li, and the halo nucleus 11Li. The accuracy is improved for previously calculated relativistic and quantum electrodynamic corrections, and in particular a disagreement for the Bethe logarithm is resolved for the ground 2S state. Our previous result is confirmed for the 2 2P state. We use the pseudostate expansion method to perform the sum over virtual intermediate states. Results for the second-order relativistic recoil term of order α2(μ/M ) 2 Ry are shown to make a significant contribution relative to the theoretical uncertainty, but because of accidental cancellations the final result for the isotope shift is nearly unchanged. However, the spin-orbit term makes an unexpectedly large contribution to the splitting isotope shift (SIS) for the 2 1/2 2P -2 3/2 2P fine structure, increasing the theoretical value for the 6Li-7Li isotopes to 0.556 31 (7 )±0.001 MHz. A comparison is made with high-precision measurements and other calculations for the SIS and for the total 2 2S-3 2S transition frequency.

  5. Mixtures of ultracold gases: Fermi sea and Bose-Einstein condensate of lithium isotopes

    Science.gov (United States)

    Schreck, F.

    2003-03-01

    This thesis presents studies of quantum degenerate atomic gases of fermionic ^6Li and bosonic ^7Li. Degeneracy is reached by evaporative cooling of ^7Li in a strongly confining magnetic trap. Since at low temperatures direct evaporative cooling is not possible for a polarized fermionic gas, ^6Li is sympathetically cooled by thermal contact with ^7Li. In a first series of experiments both isotopes are trapped in their low-field seeking higher hyperfine states. A Fermi degeneracy of T/T_F=0.25(5) is achieved for 10^5 fermions. For more than 300 atoms, the ^7Li condensate collapses, due to the attractive interatomic interaction in this state. This limits the degeneracy reached for both species. To overcome this limit, in a second series of experiments ^7Li and ^6Li atoms are transferred to their low field seeking lower hyperfine states, where the boson-boson interaction is repulsive but weak. The inter-isotope collisions are used to thermalize the mixture. A ^7Li Bose-Einstein condensate (BEC) of 10^4 atoms immersed in a Fermi sea is produced. The BEC is quasi-one-dimensional and the thermal fraction can be negligible. The measured degeneracies are T/T_C=T/T_F=0.2(1). The temperature is measured using the bosonic thermal fraction, which vanishes at the lowest temperatures, limiting our measurement sensitivity. In a third series of experiments, the bosons are transferred into an optical trap and their internal state is changed to |F=1,m_F=1rangle, the lowest energy state. A Feshbach resonance is detected and used to produce a BEC with tunable atomic interactions. When the effective interaction between atoms is tuned to be small and attractive, we observe the formation of a matter-wave bright soliton. Propagation of the soliton without spreading over a macroscopic distance of 1.1 mm is observed. Mélanges de gaz ultrafroids: mer de Fermi et condensat de Bose-Einstein des isotopes du lithium Cette thèse décrit l'étude des gaz de fermions ^6Li et de bosons ^7Li dans le

  6. Investigation of neutron converters for production of optically stimulated luminescence (OSL) neutron dosimeters using Al{sub 2}O{sub 3}:C

    Energy Technology Data Exchange (ETDEWEB)

    Mittani, J.C.R. [Department of Physics, Oklahoma State University, Stillwater, OK 74078-3072 (United States); Silva, A.A.R. da [Department of Physics, Oklahoma State University, Stillwater, OK 74078-3072 (United States); Vanhavere, F. [SCK.CEN, Belgian Nuclear Research Centre, Boeretang 200, 2400 Mol (Belgium); Akselrod, M.S. [Landauer, Inc., Stillwater Crystal Growth Division, 723 1/2 Eastgate Rd., Stillwater, OK 74074 (United States); Yukihara, E.G. [Department of Physics, Oklahoma State University, Stillwater, OK 74078-3072 (United States)]. E-mail: eduardo.yukihara@okstate.edu

    2007-07-15

    This paper presents the optically stimulated luminescence (OSL) properties of neutron dosimeters in powder and in the form of pellets prepared with a mixture of Al{sub 2}O{sub 3}:C and neutron converters. The neutron converters investigated were high density polyethylene (HDPE), lithium fluoride (LiF), lithium fluoride 95% enriched with {sup 6}Li ({sup 6}LiF), lithium carbonate 95% enriched with {sup 6}Li ({sup 6}Li{sub 2}CO{sub 3}), boric acid enriched with 99% of {sup 10}B (H{sub 3}{sup 10}BO{sub 3}) and gadolinium oxide (Gd{sub 2}O{sub 3}). The proportion of Al{sub 2}O{sub 3}:C and neutron converter in the mixture was varied to optimize the total OSL signal and neutron sensitivity. The neutron sensitivity and dose-response were determined for the OSL dosimeters using a bare {sup 252}Cf source and compared to the response of Harshaw TLD-600 and TLD-700 dosimeters ({sup 6}LiF:Mg,Ti and {sup 7}LiF:Mg,Ti). The results demonstrate the possibility of developing an OSL dosimeter made of Al{sub 2}O{sub 3}:C powder and neutron converter with a neutron sensitivity (defined as the ratio between the {sup 60}Co equivalent gamma dose and the reference neutron absorbed dose) and neutron-gamma discrimination comparable to the TLD-600/TLD-700 combination. It was shown that the shape of the OSL decay curves varied with the type of the neutron converter, demonstrating the influence of the energy deposition mechanism and ionization density on the OSL process in Al{sub 2}O{sub 3}:C.

  7. Synthesis of 8-(dimethylamino)-1-naphthyllithium etherate. Its structure in the solid (X-ray) and in Solution (7Li and 1H NMR)

    NARCIS (Netherlands)

    Koten, G. van; Jastrzebski, J.T.B.H.; Goubitz, K.; Arlen, C.; Pfeffer, M.

    1983-01-01

    The reaction of Bu{4}Li{4} with 4 molar equivalents of 1-(dimethylamino)naphthalene in diethyl ether affords novel 8-(dimethylamino)-1-naphthyllithium. Its molecular structure (X-ray) consists of two 8-(dimethylamino)-1-naphthyl groups each 3 center-2 electron bonded via C(1) to two lithium atoms an

  8. Long-term corrosion behavior of ODS-Eurofer in flowing Pb-15.7Li at 550°C

    Directory of Open Access Journals (Sweden)

    W. Krauss

    2016-12-01

    In this paper results from long-term corrosion testing of ODS-Eurofer will be reported for exposure times up to 1.5 years at a flow velocity of 0.1m/s. The evaluated data for ODS-Eurofer corrosion will be compared with values of ‘single’ phase ’classical‘ Eurofer. The observed corrosion attack and mechanisms will be discussed in detail considering the testing conditions and the microstructure of the RAFM-steels.

  9. Verification test for three WindCube WLS7 LiDARs at the Høvsøre test site

    DEFF Research Database (Denmark)

    Gottschall, Julia; Courtney, Michael

    The report describes the procedure of testing ground-based WindCube lidars (manufactured by the French company Leosphere) at the Høvsøre test site in comparison to reference sensors mounted at a meteorological mast. Results are presented for three tested units – in detail for unit WLS7...

  10. Evaluation of target photon dose mixed in mono-energetic neutron fields using {sup 7}Li(p,n){sup 7}Be reaction

    Energy Technology Data Exchange (ETDEWEB)

    Tanimura, Y., E-mail: tanimura.yoshihiko@jaea.go.j [Department of Radiation Protection, Nuclear Science and Research Institute, Japan Atomic Energy Agency, 2-4 Shirakata-Shirane, Tokai-mura, Ibaraki 319-1195 (Japan); Tsutsumi, M.; Saegusa, J.; Shikaze, Y.; Yoshizawa, M. [Department of Radiation Protection, Nuclear Science and Research Institute, Japan Atomic Energy Agency, 2-4 Shirakata-Shirane, Tokai-mura, Ibaraki 319-1195 (Japan)

    2010-12-15

    Target photons mixed in the 144, 250 and 565 keV mono-energetic neutron calibration fields were measured using a cylindrical NaI(Tl) detector with 7.62 cm both in diameter and in length. The ambient dose equivalent H*(10) of the photons was evaluated by applying the 'G(E) function' to the measured pulse height spectrum. Neutrons induce photons by nuclear reactions in the NaI(Tl) detector and affect the pulse height spectrum. In order to eliminate the influence of these neutron events, the time-of-flight technique was applied with operating the accelerator in the pulse mode. The ratios by the ambient dose equivalent H*(10) of the photons to the 144, 250 and 565 keV neutrons were evaluated to be 3.3%, 4.7% and 0.9%, respectively. Although high energy photons ranging from 6 to 7 MeV are emitted by the {sup 19}F(p,{alpha}{gamma}){sup 16}O reactions, the dose of the target photons is low enough to calibrate neutron dosemeters except for ones with high sensitivity to the photons.

  11. Complete determination of neutron yield from 62 MeV protons on 9Be for the design of a low - power ADS

    Science.gov (United States)

    Schillaci, Maria; Osipenko, Mikhail; Ripani, Marco; Alba, Rosa; Ricco, Giovanni; Barbagallo, Massimo; Celentano, Andrea; Boccaccio, Pasquale; Cosentino, Luigi; Del Zoppo, Antonio; Di Pietro, Alessia; Esposito, Juan; Finocchiaro, Paolo; Kostyukov, Alexander; Maiolino, Concettina; Santonocito, Domenico; Viberti, Carlo Maria

    2014-03-01

    Within the European Partitioning & Transmutation research programs, infrastructures specifically dedicated to the study of fundamental reactor physics of future fast neutron-based reactors are very important. In this respect, an Accelerator Driven System low-power prototype, based on a 70 MeV proton beam impinging on a thick Beryllium converter, was recently proposed and designed within the INFN-E project. The world data on neutron yield from Be target are scarce in this proton energy range. This lack of data calls for a dedicated measurement which was performed at INFN Laboratori Nazionali del Sud, covering a wide angular range, from 0 to 150 degrees, and an almost complete neutron energy interval, from thermal up to the beam energy. In this contribution the results are discussed together with the description of the proposed ADS facility.

  12. Complete determination of neutron yield from 62 MeV protons on 9Be for the design of a low – power ADS

    Directory of Open Access Journals (Sweden)

    Schillaci Maria

    2014-03-01

    Full Text Available Within the European Partitioning & Transmutation research programs, infrastructures specifically dedicated to the study of fundamental reactor physics of future fast neutron-based reactors are very important. In this respect, an Accelerator Driven System low-power prototype, based on a 70 MeV proton beam impinging on a thick Beryllium converter, was recently proposed and designed within the INFN-E project. The world data on neutron yield from Be target are scarce in this proton energy range. This lack of data calls for a dedicated measurement which was performed at INFN Laboratori Nazionali del Sud, covering a wide angular range, from 0 to 150 degrees, and an almost complete neutron energy interval, from thermal up to the beam energy. In this contribution the results are discussed together with the description of the proposed ADS facility.

  13. Production of secondary particles and nuclei in cosmic rays collisions with the interstellar gas using the FLUKA code

    Science.gov (United States)

    Mazziotta, M. N.; Cerutti, F.; Ferrari, A.; Gaggero, D.; Loparco, F.; Sala, P. R.

    2016-08-01

    The measured fluxes of secondary particles produced by the interactions of Cosmic Rays (CRs) with the astronomical environment play a crucial role in understanding the physics of CR transport. In this work we present a comprehensive calculation of the secondary hadron, lepton, gamma-ray and neutrino yields produced by the inelastic interactions between several species of stable or long-lived cosmic rays projectiles (p, D, T, 3He, 4He, 6Li, 7Li, 9Be, 10Be, 10B, 11B, 12C, 13C, 14C, 14N, 15N, 16O, 17O, 18O, 20Ne, 24Mg and 28Si) and different target gas nuclei (p, 4He, 12C, 14N, 16O, 20Ne, 24Mg, 28Si and 40Ar). The yields are calculated using FLUKA, a simulation package designed to compute the energy distributions of secondary products with large accuracy in a wide energy range. The present results provide, for the first time, a complete and self-consistent set of all the relevant inclusive cross sections regarding the whole spectrum of secondary products in nuclear collisions. We cover, for the projectiles, a kinetic energy range extending from 0.1 GeV/n up to 100 TeV/n in the lab frame. In order to show the importance of our results for multi-messenger studies about the physics of CR propagation, we evaluate the propagated spectra of Galactic secondary nuclei, leptons, and gamma rays produced by the interactions of CRs with the interstellar gas, exploiting the numerical codes DRAGON and GammaSky. We show that, adopting our cross section database, we are able to provide a good fit of a complete sample of CR observables, including: leptonic and hadronic spectra measured at Earth, the local interstellar spectra measured by Voyager, and the gamma-ray emissivities from Fermi-LAT collaboration. We also show a set of gamma-ray and neutrino full-sky maps and spectra.

  14. Tritium breeding mock-up experiments containing lithium titanate ceramic pebbles and lead irradiated with DT neutrons

    Energy Technology Data Exchange (ETDEWEB)

    Jakhar, Shrichand; Abhangi, M.; Tiwari, S. [Institute for Plasma Research, Bhat, Gandhinagar 382 428 (India); Makwana, R. [Department of Physics, MS University, Vadodara (India); Chaudhari, V.; Swami, H.L.; Danani, C.; Rao, C.V.S.; Basu, T.K. [Institute for Plasma Research, Bhat, Gandhinagar 382 428 (India); Mandal, D.; Bhade, Sonali; Kolekar, R.V.; Reddy, P.J. [Bhabha Atomic Research Center, Trombay, Mumbai 400 085 (India); Bhattacharyay, R.; Chaudhuri, P. [Institute for Plasma Research, Bhat, Gandhinagar 382 428 (India)

    2015-06-15

    Highlights: • Breeding benchmark experiment on LLCB TBM in ITER was performed. • Nuclear responses measured are TPR and reaction rate of {sup 115}In(n, n′){sup 115m}In reaction. • Measured responses are compared with calculations by MCNP and FENDL 2.1 library. • TPR measurements agree with calculations in the estimated error bar. • Measured {sup 115}In(n, n′){sup 115m}In reaction rates are underestimated by the calculations. - Abstract: Experiments were conducted with breeding blanket mock-up consisting of two layers of breeder material lithium titanate pebbles and three layers of pure lead as neutron multiplier. The radial dimensions of breeder, neutron multiplier and structural material layers are similar to the current design of the Indian Lead–Lithium cooled Ceramic Breeder (LLCB) blanket. The mock-up assembly was irradiated with 14 MeV neutrons from DT neutron generator. The local tritium production rates (TPR) from {sup 6}Li and {sup 7}Li in breeder layers were measured with the help of two different compositions of Li isotopes (60.69% {sup 6}Li and 7.54% {sup 6}Li) in Li{sub 2}CO{sub 3}. Tritium production in the multiplication layers were also measured with above mentioned two types of pellets to compare the experimental tritium production with calculations. TPR from {sup 6}Li at one location in the breeder layer was also measured by direct online measurement of tritons from {sup 6}Li(n, t){sup 4}He reaction using silicon surface barrier detector and {sup 6}Li to triton converter. Additional verification of neutron spectra (E{sub n} > 0.35 MeV) in the mock-up zones were obtained by measuring {sup 115}In(n, n′){sup 115m}In reaction rate and comparing it with calculated values in all five layers of mock-up. All the measured nuclear responses were compared with transport calculations using code MCNP with FENDL2.1 and FENDL3.0 cross-section libraries. The average C/E ratio for tritium production in enriched Li{sub 2}CO{sub 3} pellets was 1

  15. Coulomb explosion of nanodroplets drives the conversion of laser energy to nuclear energy

    Institute of Scientific and Technical Information of China (English)

    Isidore; Last; Shlomo; Ron; Andreas; Heidenreich; Joshua; Jortner

    2013-01-01

    Theoretical–computational studies of table-top laser-driven nuclear fusion of high-energy(up to 15 MeV)deuterons with7Li,6Li,and D nuclei demonstrate the attainment of high fusion yields within a source–target reaction design.This constitutes a source of Coulomb-exploding deuterium nanodroplets driven by an ultraintense femtosecond near-infrared laser and a solid hollow cylindrical target containing the second element.The source–target reaction design attains the highest table-top fusion efficiencies(up to 4×109J 1per laser pulse)obtained to date.The highest conversion efficiency of laser energy to nuclear energy(10 2–10 3)for table-top DD fusion attained in the source–target design is comparable to that for DT fusion currently accomplished for‘big science’inertial fusion setups.

  16. Ionic Debye Screening in Dense Liquid Plasmas Observed for Li+p,d Reactions with Liquid Li Target

    Institute of Scientific and Technical Information of China (English)

    J.Kasagi; H.Yonemura; Y.Toriyabe; A.Nakagawa; T.Sugawara; WANG Tie-shan

    2009-01-01

    Thick target yields of a particles emitted in the ~6Li(d,a)~4 He and ~7Li(p,a)~4 He reactions were measured for Li target in the solid and liquid phase.Observed reaction rates for the liquid Li are always larger than those for the solid.This suggests that the stopping power of hydrogen ion in the liquid Li metal might be smaller than in the solid.Using the empirically obtained stopping power for the liquid Li,we have deduced the screening potentials of the Li+p and Li+d reactions in both phases.The deduced screening potential for the liquid Li is about 500 eV larger than for the solid.This difference is attributed to the effect of liquefied Li~+ ions.It is concluded that the ionic screening is much stronger than the electronic screening in a low-temperature dense plasmas.

  17. On the 14C(alpha,gamma) reaction rate

    CERN Document Server

    Johnson, E D; Mitchell, J; Miller, L; Kemper, K W

    2009-01-01

    The 14C(alpha,gamma) reaction rate at temperatures below 0.3 GK depends on the properties of two near threshold resonances in 18O, the 1- at 6.198 MeV and the 3- at 6.404 MeV. The alpha+14C Asymptotic Normalization Coefficients (ANCs) for these resonances were determined using the alpha-transfer reactions 14C(7Li,t) and 14C(6Li,d) at sub-Coulomb energies. The 14C(alpha,gamma) reaction rate at low temperatures has been evaluated. Implications of the new reaction rate on the evolution of accreting helium white dwarfs and on the nucleosynthesis of low mass stars during the asymptotic giant branch (AGB) phase are discussed.

  18. Multiheteromacrocycles that Complex Metal Ions. Sixth Progress Report, 1 May 1979-30 April 1980

    Science.gov (United States)

    Cram, D. J.

    1980-01-15

    Objective is to design synthesize, and evaluate cyclic and polycyclic host organic compounds for their abilities to complex and lipophilize guest metal ions, their complexes, and their clusters. Host organic compounds consist of strategically placed solvating, coordinating, and ion-pairing sites tied together by covalent bonds through hydrocarbon units around cavities shaped to be occupied by guest metal ions or by metal ions plus their ligands. Specificity in complexation is sought by matching the following properties of host and guest: cavity and metal ion sizes; geometric arrangements of binding sites; number of binding sites; character of binding sites; and valences. During this period, hemispherands based on an aryloxy or cyclic urea unit, spherands based on aryloxyl units only, and their complexes with alkali metals and alkaline earths were investigated. An attempt to separate {sup 6}Li and {sup 7}Li by gel permeation chromatography of lithiospherium chloride failed. (DLC)

  19. Connecting Few-Body Inelastic Decay to Quantum Correlations in a Many-Body System: A Weakly Coupled Impurity in a Resonant Fermi Gas.

    Science.gov (United States)

    Laurent, Sébastien; Pierce, Matthieu; Delehaye, Marion; Yefsah, Tarik; Chevy, Frédéric; Salomon, Christophe

    2017-03-10

    We study three-body recombination in an ultracold Bose-Fermi mixture. We first show theoretically that, for weak interspecies coupling, the loss rate is proportional to Tan's contact. Second, using a ^{7}Li/^{6}Li mixture we probe the recombination rate in both the thermal and dual superfluid regimes. We find excellent agreement with our model in the BEC-BCS crossover. At unitarity where the fermion-fermion scattering length diverges, we show that the loss rate is proportional to n_{f}^{4/3}, where n_{f} is the fermionic density. This unusual exponent signals nontrivial two-body correlations in the system. Our results demonstrate that few-body losses can be used as a quantitative probe of quantum correlations in many-body ensembles.

  20. Experimental differential cross sections, level densities, and spin cutoffs as a testing ground for nuclear reaction codes

    Science.gov (United States)

    Voinov, A. V.; Grimes, S. M.; Brune, C. R.; Bürger, A.; Görgen, A.; Guttormsen, M.; Larsen, A. C.; Massey, T. N.; Siem, S.

    2013-11-01

    Proton double-differential cross sections from 59Co(α,p)62Ni, 57Fe(α,p)60Co, 56Fe(7Li,p)62Ni, and 55Mn(6Li,p)60Co reactions have been measured with 21-MeV α and 15-MeV lithium beams. Cross sections have been compared against calculations with the empire reaction code. Different input level density models have been tested. It was found that the Gilbert and Cameron [A. Gilbert and A. G. W. Cameron, Can. J. Phys.0008-420410.1139/p65-139 43, 1446 (1965)] level density model is best to reproduce experimental data. Level densities and spin cutoff parameters for 62Ni and 60Co above the excitation energy range of discrete levels (in continuum) have been obtained with a Monte Carlo technique. Excitation energy dependencies were found to be inconsistent with the Fermi-gas model.

  1. Development of Tritium Permeation Analysis Code and Tritium Transport in a High Temperature Gas-Cooled Reactor Coupled with Hydrogen Production System

    Energy Technology Data Exchange (ETDEWEB)

    Chang H. Oh; Eung S. Kim; Mike Patterson

    2010-06-01

    Abstract – A tritium permeation analyses code (TPAC) was developed by Idaho National Laboratory for the purpose of analyzing tritium distributions in very high temperature reactor (VHTR) systems, including integrated hydrogen production systems. A MATLAB SIMULINK software package was used in developing the code. The TPAC is based on the mass balance equations of tritium-containing species and various forms of hydrogen coupled with a variety of tritium sources, sinks, and permeation models. In the TPAC, ternary fission and neutron reactions with 6Li, 7Li 10B, and 3He were taken into considerations as tritium sources. Purification and leakage models were implemented as main tritium sinks. Permeation of tritium and H2 through pipes, vessels, and heat exchangers were considered as main tritium transport paths. In addition, electroyzer and isotope exchange models were developed for analyzing hydrogen production systems, including high temperature electrolysis and sulfur-iodine processes.

  2. In-situ Isotopic Analysis at Nanoscale using Parallel Ion Electron Spectrometry: A Powerful New Paradigm for Correlative Microscopy

    Science.gov (United States)

    Yedra, Lluís; Eswara, Santhana; Dowsett, David; Wirtz, Tom

    2016-01-01

    Isotopic analysis is of paramount importance across the entire gamut of scientific research. To advance the frontiers of knowledge, a technique for nanoscale isotopic analysis is indispensable. Secondary Ion Mass Spectrometry (SIMS) is a well-established technique for analyzing isotopes, but its spatial-resolution is fundamentally limited. Transmission Electron Microscopy (TEM) is a well-known method for high-resolution imaging down to the atomic scale. However, isotopic analysis in TEM is not possible. Here, we introduce a powerful new paradigm for in-situ correlative microscopy called the Parallel Ion Electron Spectrometry by synergizing SIMS with TEM. We demonstrate this technique by distinguishing lithium carbonate nanoparticles according to the isotopic label of lithium, viz. 6Li and 7Li and imaging them at high-resolution by TEM, adding a new dimension to correlative microscopy. PMID:27350565

  3. Summary documentation of LASL nuclear data evaluations for ENDF/B-V

    Energy Technology Data Exchange (ETDEWEB)

    Young, P.G. (comp.)

    1979-01-01

    Summaries are presented of nuclear data evaluations performed at Los Alamos Scientific Laboratory (LASL) that will comprise part of Version V of the Evaluated Nuclear Data File, ENDF/B. A total of 18 general purpose evaluations of neutron-induced data are summarized, together with 6 summaries directed specifically at covariance data evaluations. The general purpose evaluation summaries cover the following isotopes: /sup 1 -3/H, /sup 3/ /sup 4/He, /sup 6/ /sup 7/Li, /sup 10/B, /sup 14/ /sup 15/N, /sup 16/O, /sup 27/Al, /sup 182/ /sup 183/ /sup 184/ /sup 186/W, /sup 233/U, and /sup 242/Pu. The covariance data summaries are given for /sup 1/H, /sup 6/Li, /sup 10/B, /sup 14/N, /sup 16/O, and /sup 27/Al. 28 figures.

  4. Parameters of Fermi-motion from Quasielastic Backward Pion-Proton Scattering on Nuclei

    CERN Document Server

    Abramov, B M; Dukhovskoy, I A; Khanov, A I; Krestnikov, Yu S; Krutenkova, A P; Kulikov, V V; Matsuk, M A; Radkevich, I A; Turdakina, E N

    1999-01-01

    In experiment on the study of the quasielastic pion-proton scattering at large momentum transfer on nuclei the proton Fermi-momentum distributions have been analysed in plane-wave approximation for light nuclei $^6$Li, $^7$Li and $^{12}$C. It was found that, contrary to (e,e') experiments, that the oscillator model gives slightly better description of our data than the Fermi - gas model. But the values of parameters of the distributions obtained in our analysis are considerably smaller, than in (e,e') experiments. It gives evidence that the plane-wave approximation is not sufficient and more complicated theoretical models which take into account the effects of distortion of pion-nucleon amplitude in a nuclear medium are necessary for analysis of our data.

  5. Neutrino-Induced Nucleosynthesis in Helium Shells of Early Core-Collapse Supernovae

    Directory of Open Access Journals (Sweden)

    Banerjee Projjwal

    2016-01-01

    Full Text Available We summarize our studies on neutrino-driven nucleosynthesis in He shells of early core-collapse supernovae with metallicities of Z ≲ 10−3 Z⊙. We find that for progenitors of ∼ 11–15 M⊙, the neutrons released by 4He(ν¯ee, e+n3H in He shells can be captured to produce nuclei with mass numbers up to A ∼ 200. This mechanism is sensitive to neutrino emission spectra and flavor oscillations. In addition, we find two new primary mechanisms for neutrino-induced production of 9Be in He shells. The first mechanism produces 9Be via 7Li(n,γ8Li(n,γ9Li(e− ν¯ee9Be and relies on a low explosion energy for its survival. The second mechanism operates in progenitors of ∼ 8 M⊙, where 9Be can be produced directly via 7Li(3H, n09Be during the rapid expansion of the shocked Heshell material. The light nuclei 7Li and 3H involved in these mechanisms are produced by neutrino interactions with 4He. We discuss the implications of neutrino-induced nucleosynthesis in He shells for interpreting the elemental abundances in metal-poor stars.

  6. Investigation of the lithium 670.7 nm wavelength range in the solar spectrum

    Science.gov (United States)

    Caffau, Elisabetta; Mott, Alessandro; Harutyunyan, Gohar; Malherbe, Jean-Marie; Steffen, Matthias

    2016-07-01

    Lithium is a key chemical element, with a chemical evolution that is different from that of most other elements. It is also very fragile, as it is destroyed by nuclear reactions with protons at temperatures higher than about 2.5 million K. According to standard Big Bang nucleosynthesis, only the isotope 7Li is produced in significant amounts, while the primordial abundance of the lighter isotope 6Li is negligible. Lithium is not produced by nucleosynthesis in normal stars, except in peculiar phases of stellar evolution (e.g. in AGB stars and Novae). Lithium may also be formed as a result of flares in the atmospheres of young, active stars. To investigate the history of Li production and depletion in the Galaxy, it is necessary to analyse stars of all ages, including those at solar metallicity. In this case, the spectroscopic determination of the Li abundance is complicated by the presence of other spectral lines overlapping with the Li doublet at 670.7 nm. The correct identification and knowledge of the atomic parameters of these blend lines is critical, especially if the 6LI/7Li isotopic ratio is to be derived. In this investigation, we consider several line lists of the blending components available in the literature and use them to compute synthetic spectra, performing the line formation computations both for the classical 1D Holweger-Mueller model and a CO5BOLD 3D hydrodynamical simulation of the solar atmosphere. The synthetic spectra are then compared to the solar spectrum observed at different limb angles. This allows us to check the quality of existing line lists, to find potentially misidentified blend lines, and to construct an optimized line list for solar-type stars.

  7. Differences in TLD 600 and TLD 700 glow curves derived from distict mixed gamma/neutron field irradiations

    Energy Technology Data Exchange (ETDEWEB)

    Cavalieri, Tassio A.; Castro, Vinicius A.; Siqueira, Paulo T.D., E-mail: tassio.cavalieri@usp.br [Instituto de Pesquisas Energeticas e Nucleares (IPEN/CNEN-SP), Sao Paulo, SP (Brazil). Centro de Engenharia Nuclear

    2013-07-01

    In Neutron Capture Therapy, a thermal neutron beam shall impinge on a specific nuclide, such as {sup 10}B, to promote a nuclear reaction which releases the useful therapeutic energy. A nuclear reactor is usually used as the neutron source, and therefore field contaminants such as gamma and high energy neutrons are also present in the field. However, mixed field dosimetry still stands as a challenge in some cases, due to the difficulty to experimentally discriminate the dose from each field component. For the mixed field dosimetry, the International Commission on Radiation end Units (ICRU) recommends the use of detector pairs with different responses for each beam component. The TLD 600/700 pair meets this need, because these LiF detectors have different Li isotopes concentration, with distinct thermal neutron responses because {sup 6}Li presents a much higher neutron capture cross section than does {sup 7}Li for low energy neutrons. TLD 600 is {sup 6}Li enriched while TLD 700 is {sup 7}Li enriched. However, depending on the neutron spectrum presented in the mixed field, TLD 700 response to thermal neutrons cannot be disregarded. This work aims to study the difference in TLD 600 and TLD 700 glow curves when these TLDs are submitted to mixed fields of different energy spectra and components balance. The TLDs were irradiated in a pure gamma source, and in mixed fields from an AmBe sealed source and from the IPEN/MB-01 reactor. These TLDs were read and had their two main dosimetric regions analyzed to observe the differences in the glow curves of these TLDs in each irradiation. Field components discrimination was achieved through Monte Carlo simulations run with MCNP radiation transport code. (author)

  8. Interplay of projectile breakup and target excitation in reactions induced by weakly bound nuclei

    Science.gov (United States)

    Gómez-Ramos, M.; Moro, A. M.

    2017-03-01

    Background: Reactions involving weakly bound nuclei require formalisms able to deal with continuum states. The majority of these formalisms struggle to treat collective excitations of the systems involved. For continuum-discretized coupled channels (CDCC), extensions to include target excitation have been developed but have only been applied to a small number of cases. Purpose: In this work, we reexamine the extension of the CDCC formalism to include target excitation and apply it to a variety of reactions to study the effect of breakup on inelastic cross sections. Methods: We use a transformed oscillator basis to discretize the continuum of the projectiles in the different reactions and use the extended CDCC method developed in this work to solve the resulting coupled differential equations. A new code has been developed to perform the calculations. Results: Reactions 58Ni(d ,d )*58Ni , 24Mg(d ,d )*24Mg , 144Sm(6Li,6Li)*144Sm , and 9Be(6Li,6Li)*9Be are studied. Satisfactory agreement is found between experimental data and extended CDCC calculations. Conclusions: The studied CDCC method has proven to be an accurate tool to describe target excitation in reactions with weakly bound nuclei. Moderate effects of breakup on inelastic observables are found for the reactions studied. Cross-section magnitudes are not modified much, but angular distributions present smoothing when opposed to calculations without breakup.

  9. Interplay of projectile breakup and target excitation in reactions induced by weakly-bound nuclei

    CERN Document Server

    Gomez-Ramos, M

    2016-01-01

    In this work, we reexamine the extension of the CDCC formalism to include target excitation and apply it to a variety of reactions to study the effect of breakup on inelastic cross sections. We use a transformed oscillator basis to discretize the continuum of the projectiles in the different reactions and use the extended CDCC method developed in this work to solve the resulting coupled differential equations. A new code has been developed to perform the calculations. Reactions 58Ni(d, d) 58Ni*, 24Mg(d, d) 24Mg* , 144Sm( 6Li, 6Li) 144Sm* and 9Be( 6Li, 6Li) 9Be* are studied. Satisfactory agreement is found between experimental data and extended CDCC calculations. The studied CDCC method is proved to be an accurate tool to describe target excitation in reactions with weakly-bound nuclei. Moderate effects of breakup on inelastic observables are found for the reactions studied. Cross section magnitudes are not modified much, but angular distributions present smoothing when opposed to calculations without breakup.

  10. Isotope and ion selectivity in reverse osmosis desalination: geochemical tracers for man-made freshwater.

    Science.gov (United States)

    Kloppmann, Wolfram; Vengosh, Avner; Guerrot, Catherine; Millot, Romain; Pankratov, Irena

    2008-07-01

    A systematic measurement of ions and 2H/1H, 7Li/6Li, 11B/10B, 18O/ 16O, and 87Sr/86Sr isotopes in feed-waters, permeates, and brines from commercial reverse osmosis (RO) desalination plants in Israel (Ashkelon, Eilat, and Nitzana) and Cyprus (Larnaca) reveals distinctive geochemical and isotopic fingerprints of fresh water generated from desalination of seawater (SWRO) and brackish water (BWRO). The degree of isotope fractionation during the passage of water and solutes through the RO membranes depends on the medium (solvent-water vs. solutes), chemical speciation of the solutes, their charge, and their mass difference. O, H, and Sr isotopes are not fractionated during the RO process. 7Li is preferentially rejected in low pH RO, and B isotope fractionation depends on the pH conditions. Under low pH conditions, B isotopes are not significantly fractionated, whereas at high pH, RO permeates are enriched by 20 per thousand in 11B due to selective rejection of borate ion and preferential permeation of 11B-enriched boric acid through the membrane. The specific geochemical and isotopic fingerprints of SWRO provide a unique tool for tracing "man-made" fresh water as an emerging recharge component of natural water resources.

  11. Study of structure of nuclei with neutrons and nuclear data measurements for MFE. Progress report, September 1, 1979-August 31, 1980

    Energy Technology Data Exchange (ETDEWEB)

    Lane, R. O.

    1980-01-01

    Measurements of neutron differential elastic and inelastic scattering cross sections have been made for /sup 6/Li, /sup 7/Li, /sup 11/B and /sup 13/C. For /sup 7/Li + n, a multichannel R-matrix analysis has been completed, providing much new structure information for the compound /sup 8/Li system. These results are in very good agreement with recent theoretical model calculations, so that together the two provide considerable advancement in the state of our knowledge of /sup 8/Li. R-matrix analyses of /sup 11/B + n and /sup 13/C + n elastic scattering data have also been completed. For /sup 13/C + n theoretical model calculations have also been carried out and comparisons of these theoretical results with the R-matrix analysis are made. The triplet quadrupole spectrometer (TQS) is now fully operational. Development of new detectors, techniques, data analysis codes and theoretical model codes for use with the TQS system is complete. Measurements of (n,z) cross sections for fusion reactor structural materials e.g. /sup 58/Ni are currently underway. Construction of the long-flight-path tunnel for the swinger magnet facility has begun and development for this facility will continue in the coming year.

  12. Analytic potentials and vibrational energies for Li$_{2}$ states dissociating to $\\mbox{Li}\\left(2S\\right)+\\mbox{Li}\\left(3P\\right)$. Part 1: The $^{2S+1}\\Pi_{u/g}$ states

    CERN Document Server

    Dattani, Nikesh S

    2015-01-01

    Analytic potentials are built for all four $^{2S+1}\\Pi_{u/g}$ states of Li$_{2}$ dissociating to Li$(2S)$ + Li$(3P)$: $3b(3^{3}\\Pi_{u})$, $3B(3^{1}\\Pi_{u})$, $3C(3^{1}\\Pi_{g}),$ and $3d(3^{3}\\Pi_{g})$. These potentials include the effect of spin-orbit coupling for large internuclear distances, and include state of the art long-range constants. This is the first successful demonstration of fully analytic diatomic potentials that capture features that are usually considered too difficult to capture without a point-wise potential, such as multiple minima, and shelves. Vibrational energies for each potential are presented for the isotopologues $^{6,6}$Li$_{2}$, $^{6,7}$Li$_{2}$, $^{7,7}$Li$_{2}$, and the elusive `halo nucleonic molecule' $^{11,11}$Li$_{2}$. These energies are claimed to be accurate enough for new high-precision experimental setups such as the one presented in {[}Sebastian \\emph{et al.} Phys. Rev. A, \\textbf{90}, 033417 (2014){]} to measure and assign energy levels of these electronic states, all ...

  13. The Production of Negative Lithium Beams by Charge Exchange in Cesium Vapours

    CERN Document Server

    Re, Maurizio; Chines, Francesco; Cuttone, Giacomo; Menna, Mariano; Messina, Esteban; Stracener, Dan

    2005-01-01

    These measurements were carried out at the Holifield Radioactive Ion Beam Facility of the Oak Ridge National Laboratory (ORNL-HRIBF) by researchers from the Istituto Nazionale di Fisica Nucleare - Laboratori Nazionali del Sud (INFN-LNS), Catania, Italy and local staff. The Charge Exchange Cell (CEC) consisted of a vacuum chamber containing cesium vapours at a variable temperature, T, in which positive ions accelerated from an ion source were transformed into negative ones by collisions with the Cs atoms. The main goal of this test was to measure the production efficiency for 7Li- ions at different operating conditions, such as 7Li+ beam energy (5 to 55 keV) and Cs temperature (190 to 300 °C). Moreover, the efficiency measurements performed with a 6Li+ projectile beam gave clear indications about the isotopic shift effect. These results are useful to estimate the charge exchange efficiency for 8, 9Li, which will be the first radioactive beams to be produced at the EXCYT facility (EXotics with CYclotro...

  14. B and Li isotopes as intrinsic tracers for injection tests in aquifer storage and recovery systems

    Energy Technology Data Exchange (ETDEWEB)

    Kloppmann, Wolfram, E-mail: w.kloppmann@brgm.fr [BRGM, French Geological Survey, 3 Av. Claude Guillemin B.P. 6009, F-45000 Orleans (France); Chikurel, Haim [Mekorot National Water Company, Tel Aviv (Israel); Picot, Geraldine [BRGM, French Geological Survey, 3 Av. Claude Guillemin B.P. 6009, F-45000 Orleans (France); Guttman, Joseph [Mekorot National Water Company, Tel Aviv (Israel); Pettenati, Marie [BRGM, French Geological Survey, 3 Av. Claude Guillemin B.P. 6009, F-45000 Orleans (France); Aharoni, Avi [Mekorot National Water Company, Tel Aviv (Israel); Guerrot, Catherine; Millot, Romain; Gaus, Irina [BRGM, French Geological Survey, 3 Av. Claude Guillemin B.P. 6009, F-45000 Orleans (France); Wintgens, Thomas [Rheinisch Westfaelische Technische Hochschule, RWTH, Aachen (Germany)

    2009-07-15

    Boron and Li isotopes have been tested as environmental tracers of treated sewage injected into a sandy aquifer (Shafdan reclamation project, Israel). During a 38 days injection test in a newly dug injection well, a conservative artificial tracer (Br{sup -}) was monitored together with {delta}{sup 11}B and {delta}{sup 7}Li in the injectate, in the unsaturated soil zone (porous cup) and an observation well in the aquifer. In spite of B and Li concentrations in the injectate close to background values, significant shifts of the isotope signatures could be observed over the duration of the injection test. Boron isotope ratios show a breakthrough curve delayed with respect to Br{sup -} breakthrough due to some reversible sorption on the aquifer material. No isotope fractionation was observed in the unsaturated or the saturated zone so that B isotopes can be considered as conservative in the investigated part of the aquifer system. Lithium isotopes are strongly fractionated, probably due to sorption processes. Lithium concentrations point to a Li sink in the system, {delta}{sup 7}Li values vary strongly with a tendency of {sup 7}Li depletion in the liquid phase over the duration of the experiment. This is opposite to the expected preferential sorption of {sup 6}Li onto clay minerals. Boron isotopes reveals a valuable tracer of artificial recharge of freshwaters derived from treated sewage, both for short term tracer tests and for long-term monitoring of artificial recharge, even if in aquifers with higher clay contents, sorption-linked isotope fractionation cannot be excluded. More data are needed on Li isotope fractionation in natural groundwater systems to assess the potential of this tracer as monitoring tool.

  15. A super lithium-rich red-clump star in the open cluster Trumpler 5

    CERN Document Server

    Monaco, L; Bonifacio, P; Villanova, S; Carraro, G; Caffau, E; Steffen, M; Ahumada, J A; Beletsky, Y; Beccari, G

    2014-01-01

    Context. The existence of lithium-rich low-mass red giant stars still represents a challenge for stellar evolution models. Stellar clusters are privileged environments for this kind of investigation. Aims. To investigate the chemical abundance pattern of the old open cluster Trumpler\\,5, we observed a sample of four red-clump stars with high-resolution optical spectrographs. One of them (#3416) reveals extremely strong lithium lines in its spectrum. Methods. One-dimensional, local thermodynamic equilibrium analysis was performed on the spectra of the observed stars. A 3D-NLTE analysis was performed to derive the lithium abundance of star #3416. Results. Star #3416 is super Li-rich with A(Li)=3.75\\,dex. The lack of $^6$Li enrichment ($^6$Li/$^7$Li$<$2%), the low carbon isotopic ratio ($^{12}$C/$^{13}$C=14$\\pm$3), and the lack of evidence for radial velocity variation or enhanced rotational velocity ($v\\sin i = 2.8\\,$\\kms) all suggest that lithium production has occurred in this star through the Cameron &...

  16. The lithium isotopic ratio in very metal-poor stars

    CERN Document Server

    Lind, Karin; Asplund, Martin; Collet, Remo; Magic, Zazralt

    2013-01-01

    Un-evolved, very metal-poor stars are the most important tracers of the cosmic abundance of lithium in the early universe. Combining the standard Big Bang nucleosynthesis model with Galactic production through cosmic ray spallation, these stars at [Fe/H]<-2 are expected to show an undetectably small 6Li/7Li isotopic signature. Evidence to the contrary may necessitate an additional pre-galactic production source or a revision of the standard model of Big Bang nucleosynthesis. We revisit the isotopic analysis of four halo stars, two with claimed 6Li-detections in the literature, to investigate the influence of improved model atmospheres and line formation treatment. For the first time, a combined 3D, NLTE (non-local thermodynamic equilibrium) modelling technique for Li, Na, and Ca lines is utilised to constrain the intrinsic line-broadening and to determine the Li isotopic ratio. We discuss the influence of 3D NLTE effects on line profile shapes and assess the realism of our modelling using the Ca excitation...

  17. A super lithium-rich red-clump star in the open cluster Trumpler 5

    Science.gov (United States)

    Monaco, L.; Boffin, H. M. J.; Bonifacio, P.; Villanova, S.; Carraro, G.; Caffau, E.; Steffen, M.; Ahumada, J. A.; Beletsky, Y.; Beccari, G.

    2014-04-01

    Context. The existence of lithium-rich low-mass red giant stars still represents a challenge for stellar evolution models. Stellar clusters are privileged environments for this kind of investigation. Aims: To investigate the chemical abundance pattern of the old open cluster Trumpler 5, we observed a sample of four red-clump stars with high-resolution optical spectrographs. One of them (#3416) reveals extremely strong lithium lines in its spectrum. Methods: One-dimensional, local thermodynamic equilibrium analysis was performed on the spectra of the observed stars. A 3D-NLTE analysis was performed to derive the lithium abundance of star #3416. Results: Star #3416 is super Li-rich with A(Li) = 3.75 dex. The lack of 6Li enrichment (6Li/7Li Cameron & Fowler mechanism. Conclusions: We identified a super Li-rich core helium-burning, red-clump star in an open cluster. Internal production is the most likely cause of the observed enrichment. Given the expected short duration of a star's Li-rich phase, enrichment is likely to have occurred at the red clump or in the immediately preceding phases, namely during the He-flash at the tip of the red giant branch (RGB) or while ascending the brightest portion of the RGB. Based on observations made with ESO Telescopes at the La Silla Paranal Observatory under program ID 088.D-0045(A).Appendix A is available in electronic form at http://www.aanda.org

  18. The CLYC-6 and CLYC-7 response to γ-rays, fast and thermal neutrons

    Science.gov (United States)

    Giaz, A.; Pellegri, L.; Camera, F.; Blasi, N.; Brambilla, S.; Ceruti, S.; Million, B.; Riboldi, S.; Cazzaniga, C.; Gorini, G.; Nocente, M.; Pietropaolo, A.; Pillon, M.; Rebai, M.; Tardocchi, M.

    2016-02-01

    The crystal Cs2LiYCl6:Ce (CLYC) is a very interesting scintillator material because of its good energy resolution and its capability to identify γ-rays and fast/thermal neutrons. The crystal Cs2LiYCl6:Ce contains 6Li and 35Cl isotopes, therefore, it is possible to detect thermal neutrons through the reaction 6Li(n, α)t while 35Cl ions allow to measure fast neutrons through the reactions 35Cl(n, p)35S and 35Cl(n, α)32P. In this work two CLYC 1″×1″ crystals were used: the first crystal, enriched with 6Li at 95% (CLYC-6) is ideal for thermal neutron measurements while the second one, enriched with 7Li at >99% (CLYC-7) is suitable for fast neutron measurements. The response of CLYC scintillators was measured with different PMT models: timing or spectroscopic, with borosilicate glass or quartz window. The energy resolution, the neutron-γ discrimination and the internal activity are discussed. The capability of CLYC scintillators to discriminate γ rays from neutrons was tested with both thermal and fast neutrons. The thermal neutrons were measured with both detectors, using an AmBe source. The measurements of fast neutrons were performed at the Frascati Neutron Generator facility (Italy) where a deuterium beam was accelerated on a deuterium or on a tritium target, providing neutrons of 2.5 MeV or 14.1 MeV, respectively. The different sensitivity to thermal and fast neutrons of a CLYC-6 and of a CLYC-7 was additionally studied.

  19. The CLYC-6 and CLYC-7 response to γ-rays, fast and thermal neutrons

    Energy Technology Data Exchange (ETDEWEB)

    Giaz, A.; Pellegri, L. [INFN Milano, Via Celoria 16, 20133 Milano (Italy); Camera, F., E-mail: franco.camera@mi.infn.it [INFN Milano, Via Celoria 16, 20133 Milano (Italy); Università degli Studi di Milano, Physics Department, Via Celoria 16, 20133 Milano (Italy); Blasi, N.; Brambilla, S. [INFN Milano, Via Celoria 16, 20133 Milano (Italy); Ceruti, S. [INFN Milano, Via Celoria 16, 20133 Milano (Italy); Università degli Studi di Milano, Physics Department, Via Celoria 16, 20133 Milano (Italy); Million, B. [INFN Milano, Via Celoria 16, 20133 Milano (Italy); Riboldi, S. [INFN Milano, Via Celoria 16, 20133 Milano (Italy); Università degli Studi di Milano, Physics Department, Via Celoria 16, 20133 Milano (Italy); Cazzaniga, C.; Gorini, G.; Nocente, M. [University of Milano Bicocca, Physics Department, Piazza della Scienza 3, 20126 Milano (Italy); Istituto di Fisica del Plasma, Associazione EURATOM-ENEA-CNR, via Roberto Cozzi 53, 20125 Milano (Italy); Pietropaolo, A.; Pillon, M. [Associazione EURATOM-ENEA sulla Fusione ENEA C.R. Frascati, Via E. Fermi 45, 00044 Frascati, Roma (Italy); Rebai, M. [University of Milano Bicocca, Physics Department, Piazza della Scienza 3, 20126 Milano (Italy); Tardocchi, M. [Istituto di Fisica del Plasma, Associazione EURATOM-ENEA-CNR, via Roberto Cozzi 53, 20125 Milano (Italy)

    2016-02-21

    The crystal Cs{sub 2}LiYCl{sub 6}:Ce (CLYC) is a very interesting scintillator material because of its good energy resolution and its capability to identify γ-rays and fast/thermal neutrons. The crystal Cs{sub 2}LiYCl{sub 6}:Ce contains {sup 6}Li and {sup 35}Cl isotopes, therefore, it is possible to detect thermal neutrons through the reaction {sup 6}Li(n, α)t while {sup 35}Cl ions allow to measure fast neutrons through the reactions {sup 35}Cl(n, p){sup 35}S and {sup 35}Cl(n, α){sup 32}P. In this work two CLYC 1″×1″ crystals were used: the first crystal, enriched with {sup 6}Li at 95% (CLYC-6) is ideal for thermal neutron measurements while the second one, enriched with {sup 7}Li at >99% (CLYC-7) is suitable for fast neutron measurements. The response of CLYC scintillators was measured with different PMT models: timing or spectroscopic, with borosilicate glass or quartz window. The energy resolution, the neutron-γ discrimination and the internal activity are discussed. The capability of CLYC scintillators to discriminate γ rays from neutrons was tested with both thermal and fast neutrons. The thermal neutrons were measured with both detectors, using an AmBe source. The measurements of fast neutrons were performed at the Frascati Neutron Generator facility (Italy) where a deuterium beam was accelerated on a deuterium or on a tritium target, providing neutrons of 2.5 MeV or 14.1 MeV, respectively. The different sensitivity to thermal and fast neutrons of a CLYC-6 and of a CLYC-7 was additionally studied.

  20. Neutron dosimetric measurements in shuttle and MIR.

    Science.gov (United States)

    Reitz, G

    2001-06-01

    Detector packages consisting of thermoluminescence detectors (TLD), nuclear emulsions and plastic track detectors were exposed at identical positions inside MIR space station and on shuttle flights inside Spacelab and Spacehab during different phases of the solar cycle. The objectives of the investigations are to provide data on charge and energy spectra of heavy ions, and the contribution of events with low-energy deposit (protons, electrons, gamma, etc.) to the dose, as well as the contribution of secondaries, such as nuclear disintegration stars and neutrons. For neutron dosimetry 6LiF (TLD600) and 7LiF (TLD700) chips were used both of which have almost the same response to gamma rays but different response to neutrons. Neutrons in space are produced mainly in evaporation and knock-on processes with energies mainly of 1-10 MeV and up to several 100 MeV, respectively. The energy spectrum undergoes continuous changes toward greater depth in the attenuating material until an equilibrium is reached. In equilibrium, the spectrum is a wide continuum extending down to thermal energies to which the 6LiF is sensitive. Based on the difference of absorbed doses in the 6LiF and 7LiF chips, thermal neutron fluxes from 1 to 2.3 cm-2 s-1 are calculated using the assumption that the maximum induced dose in TLD600 for 1 neutron cm-2 is 1.6 x 10(-10) Gy (Horowitz and Freeman, Nucl. Instr. and Meth. 157 (1978) 393). It is assumed that the flux of high-energy neutrons is at least of that quantity. Tissue doses were calculated taking as a mean ambient absorbed dose per neutron 6 x10(-12) Gy cm2 (for a10 MeV neutron). The neutron equivalent doses for the above-mentioned fluxes are 52 micro Gy d-1 and 120 micro Gy d-1. In recent experiments, a personal neutron dosimeter was integrated into the dosimeter packages. First results of this dosimeter which is based on nuclear track detectors with converter foils are reported. For future measurements, a scintillator counter with

  1. Study of the poly-aniline complexed with Li Cl O{sub 4} by Lithium-7 NMR; Estudo da polianilina complexada com Li Cl O{sub 4} por RMN do {sup 7} Li

    Energy Technology Data Exchange (ETDEWEB)

    Giotto, M.V.; Bonagamba, T.J.; Panepucci, H. [Sao Paulo Univ., Sao Carlos, SP (Brazil). Inst. de Fisica e Quimica; Mattoso, L.H.C.; Valenciano, G.R. [EMBRAPA, Sao Carlos, SP (Brazil). CNPDIA

    1997-12-31

    This work presents the chemical structure study of poly-aniline. The chemical preparation of the samples is presented. Also studied are the electric conductivity of the complexes of poly-aniline with Lithium. The samples were analysed by NMR. The spectra are presented 3 refs., 11 figs., 3 tabs.

  2. Magnetic structure of low-dimensional LiCu{sub 2}O{sub 2} multiferroic according to {sup 63,65}Cu and {sup 7}Li NMR studies

    Energy Technology Data Exchange (ETDEWEB)

    Sadykov, A. F., E-mail: sadykov@imp.uran.ru; Gerashchenko, A. P.; Piskunov, Yu. V.; Ogloblichev, V. V.; Smol' nikov, A. G.; Verkhovskii, S. V. [Russian Academy of Sciences, Institute of Metal Physics, Ural Division (Russian Federation); Yakubovskii, A. Yu. [National Research Centre Kurchatov Institute (Russian Federation); Tishchenko, E. A. [Russian Academy of Sciences, Kapitza Institute for Physical Problems (Russian Federation); Bush, A. A. [Moscow State Technical University of Radio Engineering, Electronics, and Automation (Russian Federation)

    2012-10-15

    The complex NMR study of the magnetic structure of LiCu{sub 2}O{sub 2} multiferroic has been performed. It has been shown that the spin spirals in LiCu{sub 2}O{sub 2} are beyond the ab, bc, and ac crystallographic planes. The external magnetic field applied along the c axis of the crystal does not change the spatial orientation of spirals in Cu{sup 2+} chains. A magnetic field of H{sub 0} = 94 kOe applied along the a and b axes rotates the planes of spin spirals in chains, tending to orient the normal n of spirals along the external magnetic field. The rotation angle of the planes of the magnetic moments are maximal at H{sub 0} Double-Vertical-Line b.

  3. A twin ionization chamber setup as detector for light charged particles with energies around 1 MeV applied to the sup 1 sup 0 B(n, alpha) sup 7 Li reaction

    CERN Document Server

    Göpfert, A; Bax, H

    2000-01-01

    The setup and operating conditions of a gridded twin ionization chamber with sample change facility to study light charged particle properties in the 1 MeV region is described. Detailed studies of different grid geometries in connection with the choice of an eligible counting gas mixture and the applied high voltage have been performed. Due to the high overall amplification of the small electrical chamber signals obtained from such low-energy particles, special filters have been developed in order to increase the signal-to-noise ratio. Timing properties of the chamber signals are discussed in detail. Information available from chamber signals and encoding methods are elucidated by spectra of alpha particles created by sup 2 sup 3 sup 4 sup , sup 2 sup 3 sup 5 U spontaneous alpha decay. The detector permits the independent and simultaneous measurement of energy and angular distribution of particles in both sides of the chamber. Finally, preliminary results and related analysis methods will be presented for the...

  4. L-Phenylalanine preloading reduces the (10)B(n, α)(7)Li dose to the normal brain by inhibiting the uptake of boronophenylalanine in boron neutron capture therapy for brain tumours.

    Science.gov (United States)

    Watanabe, Tsubasa; Tanaka, Hiroki; Fukutani, Satoshi; Suzuki, Minoru; Hiraoka, Masahiro; Ono, Koji

    2016-01-01

    Boron neutron capture therapy (BNCT) is a cellular-level particle radiation therapy that combines the selective delivery of boron compounds to tumour tissue with neutron irradiation. Previously, high doses of one of the boron compounds used for BNCT, L-BPA, were found to reduce the boron-derived irradiation dose to the central nervous system. However, injection with a high dose of L-BPA is not feasible in clinical settings. We aimed to find an alternative method to improve the therapeutic efficacy of this therapy. We examined the effects of oral preloading with various analogues of L-BPA in a xenograft tumour model and found that high-dose L-phenylalanine reduced the accumulation of L-BPA in the normal brain relative to tumour tissue. As a result, the maximum irradiation dose in the normal brain was 19.2% lower in the L-phenylalanine group relative to the control group. This study provides a simple strategy to improve the therapeutic efficacy of conventional boron compounds for BNCT for brain tumours and the possibility to widen the indication of BNCT to various kinds of other tumours.

  5. Measurement of Total Cross Sections of Nuclei Produced by 20 Ne Bombing at 9 Be Target%80MeV/u 20 Ne轰击9Be碎裂产物反应总截面的测量

    Institute of Scientific and Technical Information of China (English)

    李加兴; 郭忠言; 肖国青; 詹文龙; 孙志宇; 王建松; 田文栋; 王猛; 陈志强; 王武生; 宁振江; 王建峰; 毛瑞士

    2002-01-01

    介绍了用透射法测量中能区20Ne打9Be靶碎裂产生的次级束与Si靶作用的核反应总截面的方法,以及实验的探测器布局、实验过程和实验结果. 并对理论上预言有奇异结构的核12N,17Ne和17F的实验结果与其相邻核进行了比较.

  6. Experimental study to explore the $\\rm ^8Be$ induced nuclear reaction via the Trojan Horse Method

    CERN Document Server

    Qun-Gang, Wen; Shu-Hua, Zhou; Irgaziev, Bakhadir; Yuan-Yong, Fu; Spitaleri, Claudio; La Cognata, Marco; Jing, Zhou; Qiu-Ying, Meng; Lamia, Livio; Lattuada, Marcello

    2014-01-01

    To explore a possible indirect method for $\\rm ^8Be$ induced astrophysical reactions, the $\\rm ^9Be=({}^8Be+\\it n)$ cluster structure was studied via the Trojan Horse Method. It is the first time to study a super short life nucleus $\\rm ^8Be$ via the Trojan Horse Method, and it is the first time to make a valid test for $l=1$ Trojan-horse nucleus. The $\\rm ^9Be$ nucleus is assumed to have a ($\\rm {}^8Be+\\it n$) cluster structure and used as the Trojan-horse nucleus. The $\\rm ^8Be$ nucleus acts as a participant, while the neutron is a spectator to the virtual $\\rm ^8Be +{\\it d}\\rightarrow \\alpha + {}^6Li$ reaction via a suitable 3-body reaction $\\rm ^9Be +{\\it d}\\rightarrow \\alpha + {}^6Li +\\it n$. The experimental neutron momentum distribution inside $\\rm ^9Be$ was reconstructed. The agreement between experimental and theoretical momentum distribution indicates that there should be a ($\\rm {}^8Be+\\it n$) cluster structure inside $\\rm ^9Be$. Therefor the experimental study of $\\rm ^8Be$ induced reactions, for ...

  7. 离子液体/苯并15-冠-5浸渍XAD-7树脂萃取分离锂同位素%Extraction Separation of Lithium Isotopes by Using XAD-7 Resins Impregnated With Ionic Liquid and Benzo-15-Crown-5

    Institute of Scientific and Technical Information of China (English)

    顾玲; 孙晓利; 任冬红; 邱丹; 顾志国; 李在均

    2015-01-01

    Imidazolium-type ionic liquid ([C8 mim][BF4 ],[C8 mim][PF6 ]and [C8 mim] [(SO2 CF3 )2 N])and benzo-15-crown-5 were immobilized on XAD-7 resin to obtain the im-pregnated resin for lithium isotopes separation.IR and SEM characterizations of the impreg-nated resins indicate that ionic liquids and benzo-15-crown-5 are immobilized in the resins successfully and the thermal analysis indicates that the materials are thermally stable.The optimum E was obtained in the initial solution at pH=5.55.The larger extraction percenta-ges and separation factors values were obtained from LiSCN solution and CF3 COOLi solu-tion,respectively.The maximum single-stage isotopes separation factor of 6 Li/7 Li is up to 1.045±0.002.The equilibrium time of extraction is attained in 2.5-3 h.The thermodynamic parameters of the system were presented and revealed that the extraction reaction was a spontaneous process and the temperature had slight influence on the extraction separation of lithium isotopes.The mechanism of extraction system show that 6 Li enriches in the solid phase and 7 Li concentrates in the aqueous phase.The impregnated resins can be regenerated and reused for lithium isotopes separation.%以 XAD-7树脂为支撑担体制备了含有三种不同咪唑型离子液体([C8 mim][BF4]、[C8 mim][PF6]、[C8 mim][(SO2 CF3)2 N])和萃取剂(苯并15-冠-5)的浸渍树脂,并用于锂同位素的萃取分离。浸渍树脂的红外和扫描电镜表征表明,离子液体成功负载到了树脂上;热重分析表明,该浸渍树脂具有良好的热稳定性。在水相初始 pH=5.55时,浸渍树脂具有最佳萃取率。浸渍树脂在 LiSCN 溶液中具有较高的萃取率,而在CF3 COOLi 溶液中呈现较大的单级分离因子,最大单级分离因子达到1.045±0.002。浸渍树脂的萃取平衡时间为2.5~3 h。萃取热力学研究表明,该反应为自发过程,温度对体系的影响较小。6 Li 富集于固相,7 Li 富集在水相。该系列浸渍树脂易于再生,可循环使用。

  8. Study of the response to neutrons of a personal dosemeter in mixed fields (n, {gamma}) in function of Hp(10); Estudio de la respuesta a neutrones de un dosimetro personal en campos mixtos (n, {gamma}) en funcion de Hp(10)

    Energy Technology Data Exchange (ETDEWEB)

    Cruzate, J.; Gregori, B.; Carelli, J.; Aguerre, L.; Discacciatti, A. [Autoridad REgulatoria Nuclear, Av. del Libertador 8250 (1429), Buenos Aires (Argentina)]. e-mail: cruzate@cae.arn.gov.ar

    2006-07-01

    In this work it is presented the theoretical study and their experimental validation of the answer of the personal dosimetro in terms of the component of neutrons of the personal equivalent dose Hpn(10) in function of the energy, in presence of fields of neutrons and range. The personal dosimetro, based on detecting termoluminiscentes (TLD), it consists of two detectors 7LiF and two 6LiF, located low filters of plastic and cadmium starting from whose information is evaluated the component range and of neutrons of the dose. Additionally it consists of a detecting CaF2, used basically to discriminate against the energy of the component range and to make the corresponding corrections on the evaluation of the dose range obtained with the 7LiF. The answer to neutrons in function of the energy, defined as the quotient among the one I number of reactions 6Li(n, a)4He taken place in each TLD and the Hpn(10), it was calculated using the code MCNPX and the library ENDF/B-VI. You model the dosimetro under the irradiation conditions proposed by the ISO8529-3. Faces monoenergeticos were simulated in the range of energy understood between 70 keV and 5 MeV. The dispersion in each one of the results of the simulation is smaller than 3%. You I study the existent relationship among the answer te6rica, reactions (n,a)/Hpn(10) and the experimental one, nC/Hpn(10), for a given thermal treatment. The factor of resulting conversion is constant in the energy and similar to 1,71 104 reacciones(n, a)/nC, with a smaller standard deviation to 10%. The experimental answer was obtained starting from the irradiations carried out in the mark of the International Intercomparacion of Dosimetria in Mixed Campos (n,) 2004 organized by the OIEA next to the PTB (Germany) and the IRSN (France). The extension of these calculations to other spectra of neutrons of fields real they will allow to obtain group of factors of application conversion in routine and accidental situations. (Author)

  9. Experimental study to explore the 8Be-induced nuclear reaction via the Trojan horse method

    Science.gov (United States)

    Wen, Qun-Gang; Li, Cheng-Bo; Zhou, Shu-Hua; Irgaziev, Bakhadir; Fu, Yuan-Yong; Spitaleri, Claudio; La Cognata, Marco; Zhou, Jing; Meng, Qiu-Ying; Lamia, Livio; Lattuada, Marcello

    2016-03-01

    To explore a possible indirect method for 8Be induced astrophysical reactions, the 8Be=(8Be+n ) cluster structure has been studied via the Trojan horse method. For the first time a 8Be nucleus having an ultrashort lifetime is studied by the Trojan horse method and a 9Be nucleus in the ground state is used for this purpose. The 9Be nucleus is assumed to have a (8Be+n ) cluster structure and used as a Trojan horse nucleus. The 8Be nucleus acts as a participant, while the neutron is a spectator to the virtual 8Be+d →α +6Li reaction via the 3-body reaction 8Be+d →α +6Li+n . The experimental neutron momentum distribution inside 9Be has been reconstructed. The agreement between the experimental momentum distribution and the theoretical one indicates that a (8Be+n ) cluster structure inside 9Be is very likely. Therefore, the experimental study of 8Be induced reactions, for example, the measurement of the 8Be+α →12C reaction proceeding through the Hoyle state, is possible.

  10. Accelerator-based epithermal neutron beam design for neutron capture therapy.

    Science.gov (United States)

    Yanch, J C; Zhou, X L; Shefer, R E; Klinkowstein, R E

    1992-01-01

    Recent interest in the production of epithermal neutrons for use in boron neutron capture therapy (BNCT) has promoted an investigation into the feasibility of generating such neutrons with a high current proton accelerator. Energetic protons (2.5 MeV) on a 7Li target produce a spectrum of neutrons with maximum energy of roughly 800 keV. A number of combinations of D2O moderator, lead reflector, 6Li thermal neutron filtration, and D2O/6Li shielding will result in a useful epithermal flux of 1.6 x 10(8) n/s at the patient position. The neutron beam is capable of delivering 3000 RBE-cGy to a tumor at a depth of 7.5 cm in a total treatment time of 60-93 min (depending on RBE values used and based on a 24-cm diameter x 19-cm length D2O moderator). Treatment of deeper tumors with therapeutic advantage would also be possible. Maximum advantage depths (RBE weighted) of 8.2-9.2 (again depending on RBE values and precise moderator configuration) are obtained in a right-circular cylindrical phantom composed of brain-equivalent material with an advantage ratio of 4.7-6.3. A tandem cascade accelerator (TCA), designed and constructed at Science Research Laboratory (SRL) in Somerville MA, can provide the required proton beam parameters for BNCT of deep-seated tumors. An optimized configuration of materials required to shift the accelerator neutron spectrum down to therapeutically useful energies has been designed using Monte Carlo simulation in the Whitaker College Biomedical Imaging and Computation Laboratory at MIT. Actual construction of the moderator/reflector assembly is currently underway.

  11. New insights into the structural and dynamical features of lithium hexaoxometalates Li7MO6 (M = Nb, Ta, Sb, Bi).

    Science.gov (United States)

    Mühle, Claus; Dinnebier, Robert E; van Wüllen, Leo; Schwering, Georg; Jansen, Martin

    2004-02-09

    We present a (re)investigation of the hexaoxometalates Li(8)MO(6) (M = Sn, Pb, Zr, Hf) and Li(7)MO(6) (M = Nb, Ta, Sb, Bi). Lithium motion and ionic conductivity in the hexaoxometalates were studied using impedance spectroscopy (for Li(7)MO(6), M = Sb, Bi, Ta) and (6)Li and (7)Li solid-state nuclear magnetic resonance (for Li(7)TaO(6)). The NMR data indicate a considerable exchange of Li among the tetrahedral and octahedral voids even at ambient temperature. In an investigation of the crystal structures using laboratory and synchrotron X-ray powder diffraction techniques, the structures of Li(7)TaO(6), Li(7)NbO(6), and Li(7)SbO(6) could be solved and refined. All three reveal a triclinic metric (Li(7)SbO(6), triclinic, P1, a = 5.38503(6) A, b = 5.89164(7) A, c = 5.43074(6) A, alpha = 117.2210(6) degrees, beta = 119.6311(6) degrees, gamma = 63.2520(7) degrees, V = 127.454(3) A(3), Z = 1; Li(7)NbO(6), triclinic, P1, a = 5.37932(9) A, b = 5.91942(11) A, c = 5.37922(9) A, alpha = 117.0033(9) degrees, beta = 119.6023(7) degrees, gamma = 63.2570(9) degrees, V = 126.938(4) A(3), Z = 1; Li(7)TaO(6), triclinic, P1, a = 5.38486(2) A, b = 5.92014(3) A, c = 5.38551(2) A, alpha = 117.0108(2) degrees, beta = 119.6132(2) degrees, gamma = 63.2492(2) degrees, V = 127.208(1) A(3), Z = 1.

  12. MC-ICP-MS高精度测定Li同位素分析方法%High-precision measurement of lithium isotopes using MC-ICP-MS.

    Institute of Scientific and Technical Information of China (English)

    苏嫒娜; 杨竹森; 田世洪; 李真真; 侯增谦; 侯可军; 胡文洁; 高延光; 杨丹; 李延河

    2011-01-01

    A high-yield lithium separation technique for rock samples has been established together with precise Li isotope analysis by MC-ICP-MS. The solutions with different concentration of lithiumelement standard reference materials and single element standard samples of potassium, calcium, sodium, magnesium and iron were used to evaluate the analytical methods applied. Three separate stages of ion-exchange chromatography were carried out using organic cation exchange resin (AG 50W-XS,200-400 mesh). Lithium was enriched in different eluants for the different stages. 2. 8 mol/L HCI, 0. 15 mol/L HCI and 0. 5 rnol/L HCI in 30% ethanol were used for the different three stages. Two kinds of columns which are made of polypropylene for the first and second stages and quartz for the third stage were used, which is different from those used abroad.Total reagent volume for the entire chemical process was reduced to 38 mL for the rock samples and the recovery is more than 97. 6%. The precision of this technique is conservatively estimated to be ±0. 60%0-0. 94%(2σ population), which is similar to the precision of other methods used abroad. The δ7Li value (7Li/6Li relative to the IRMM-016 standard) determined for AGV-2 is 5. 13%. The δ7Li values determined for BHVO-2 (7Li/6Li relative to the IRMM-016 standard) and IRMM-016 (7Li/6Li relative to the L-SVEC standard) are 4.08%0 and 0. 038%0, respectively. In addition, the results for the same kinds of samples analyzed by my lab are the same as those by isotope lab of Maryland University. All the analytical results are consistent with those reported by others. Moreover, the δ7I.i value (7Li/61.i relative to the IRMM-016 standard) determined for substandard NKT-1 nephelinite obtained from the United States Geological Survey (USGS) is 8. 71%0 and its precision is ±0. 46%0. According to the experiments, it is concluded that this proposed procedure is a suitable method for determining the lithium isotopic composition of

  13. Investigation of a measure of robustness in inductively coupled plasma mass spectrometry

    Science.gov (United States)

    Makonnen, Yoseif; Beauchemin, Diane

    2015-01-01

    In industrial/commercial settings where operators often have minimal expertise in inductively coupled plasma (ICP) mass spectrometry (MS), there is a prevalent need for a response factor indicating robust plasma conditions, which is analogous to the Mg II/Mg I ratio in ICP optical emission spectrometry (OES), whereby a Mg II/Mg I ratio of 10 constitutes robust conditions. While minimizing the oxide ratio usually corresponds to robust conditions, there is no specific target value that is widely accepted as indicating robust conditions. Furthermore, tuning for low oxide ratios does not necessarily guarantee minimal matrix effects, as they really address polyatomic interferences. From experiments, conducted in parallel for both MS and OES, there were some element pairs of similar mass and very different ionization potential that were exploited for such a purpose, the rationale being that, if these elements were ionized to the same extent, then that could be indicative of a robust plasma. The Be II/Li I intensity ratio was directly related to the Mg II/Mg I ratio in OES. Moreover, the 9Be+/7Li+ ratio was inversely related to the CeO+/Ce+ and LaO+/La+ oxide ratios in MS. The effects of different matrices (i.e. 0.01-0.1 M Na) were also investigated and compared to a conventional argon plasma optimized for maximum sensitivity. The suppression effect of these matrices was significantly reduced, if not eliminated in the case of 0.01 M Na, when the 9Be+/7Li+ ratio was around 0.30 on the Varian 820 MS instrument. Moreover, a very similar ratio (0.28) increased robustness to the same extent on a completely different ICP-MS instrument (PerkinElmer NEXION). Much greater robustness was achieved using a mixed-gas plasma with nitrogen in the outer gas and either nitrogen or hydrogen as a sheathing gas, as the 9Be+/7Li+ ratio was then around 1.70. To the best of our knowledge, this is the first report on using a simple analyte intensity ratio, 9Be+/7Li+, to gauge plasma robustness.

  14. Experimental Evidence for Fast Lithium Diffusion and Isotope Fractionation in Water-bearing Rhyolitic Melts at Magmatic Conditions

    Science.gov (United States)

    Cichy, S. B.; Till, C. B.; Roggensack, K.; Hervig, R. L.; Clarke, A. B.

    2015-12-01

    The aim of this work is to extend the existing database of experimentally-determined lithium diffusion coefficients to more natural cases of water-bearing melts at the pressure-temperature range of the upper crust. In particular, we are investigating Li intra-melt and melt-vapor diffusion and Li isotope fractionation, which have the potential to record short-lived magmatic processes (seconds to hours) in the shallow crust, especially during decompression-induced magma degassing. Hydrated intra-melt Li diffusion-couple experiments on Los Posos rhyolite glass [1] were performed in a piston cylinder at 300 MPa and 1050 °C. The polished interfaces between the diffusion couples were marked by addition of Pt powder for post-run detection. Secondary ion mass spectrometry analyses indicate that lithium diffuses extremely fast in the presence of water. Re-equilibration of a hydrated ~2.5 mm long diffusion-couple experiment was observed during the heating period from room temperature to the final temperature of 1050 °C at a rate of ~32 °C/min. Fractionation of ~40‰ δ7Li was also detected in this zero-time experiment. The 0.5h and 3h runs show progressively higher degrees of re-equilibration, while the isotope fractionation becomes imperceptible. Li contamination was observed in some experiments when flakes filed off Pt tubing were used to mark the diffusion couple boundary, while the use of high purity Pt powder produced better results and allowed easier detection of the diffusion-couple boundary. The preliminary lithium isotope fractionation results (δ7Li vs. distance) support findings from [2] that 6Li diffuses substantially faster than 7Li. Further experimental sets are in progress, including lower run temperatures (e.g. 900 °C), faster heating procedure (~100 °C/min), shorter run durations and the extension to mafic systems. [1] Stanton (1990) Ph.D. thesis, Arizona State Univ., [2] Richter et al. (2003) GCA 67, 3905-3923.

  15. Study the effect of beryllium reflector poisoning on the Syrian MNSR.

    Science.gov (United States)

    Omar, H; Ghazi, N; Haddad, Kh; Ezzuddin, H

    2012-06-01

    Neutron interactions with beryllium lead to formation of (3)H and strong neutron absorbers (3)He and (6)Li in the reflector (so called beryllium poisoning). After the reactor shutdown, the concentration of (3)He increases in time due to tritium decay. This paper illustrates the impact of poisoning accumulation in the beryllium reflectors on reactivity for the Syrian MNSR research reactor. The prediction of (6)Li and (3)He poison concentrations, initiated by the 9Be(n,α) reaction, in the beryllium reflectors of the MNSR was also presented. The results were based on MCNP Monte Carlo calculations and solutions to the differential equations which describe the time dependent poison concentrations as a function of reactor operation time and shutdown periods. The whole reactor history was taken into account to predict reliable values of parasitic isotope concentrations. It was found that the (3)He and (6)Li accumulations in the beryllium reflectors during the actual working history decreased the excess reactivity by about 28%. While, the effect became more significant at the reactor life's end and the reactor became subcritical after 25,000 h operation. The results contained in this paper could be used in assess the safety analysis of the MNSR reactor.

  16. Ultracold lithium-6 atoms in the BEC-BCS crossover: experiments and the construction of a new apparatus; Atomes de lithium-6 ultra froids dans la transition BEC-BCS: experiences et construction d'un montage experimental

    Energy Technology Data Exchange (ETDEWEB)

    Teichmann, M

    2007-09-15

    We use a fermionic gas of Lithium-6 as a model system to study superfluidity. The limiting cases of superfluidity are Bose-Einstein condensation (BEC) and superconductivity, described by the theory by Bardeen, Cooper and Schrieffer (BCS). In Lithium-6 gases, we can explore the whole range between the two cases, known as the BEC-BCS crossover, using a Feshbach resonance. We study the change of the momentum distribution of the gas in this cross-over and compare to theoretical models. We also investigate the hydrodynamic expansion, characteristic for a superfluid gas. We observe a sudden change of the ellipticity of the gas close to the transition to the superfluid phase. Moreover, we localized heteronuclear Feshbach resonances between {sup 6}Li and {sup 7}Li. We are currently constructing a second generation of the experimental setup. An new laser system, based on high power laser diodes, was developed. Changes in the vacuum chamber, including a complete reconstruction of the Zeeman slower, have increased the atomic flux, allowing us to increase the repetition rate of our experiment. Modifications of the geometry of the magnetic traps lead to a higher number of trapped atoms. (author)

  17. Big bang nucleosynthesis: Present status

    Science.gov (United States)

    Cyburt, Richard H.; Fields, Brian D.; Olive, Keith A.; Yeh, Tsung-Han

    2016-01-01

    Big bang nucleosynthesis (BBN) describes the production of the lightest nuclides via a dynamic interplay among the four fundamental forces during the first seconds of cosmic time. A brief overview of the essentials of this physics is given, and new calculations presented of light-element abundances through 6Li and 7Li, with updated nuclear reactions and uncertainties including those in the neutron lifetime. Fits are provided for these results as a function of baryon density and of the number of neutrino flavors Nν. Recent developments are reviewed in BBN, particularly new, precision Planck cosmic microwave background (CMB) measurements that now probe the baryon density, helium content, and the effective number of degrees of freedom Neff. These measurements allow for a tight test of BBN and cosmology using CMB data alone. Our likelihood analysis convolves the 2015 Planck data chains with our BBN output and observational data. Adding astronomical measurements of light elements strengthens the power of BBN. A new determination of the primordial helium abundance is included in our likelihood analysis. New D/H observations are now more precise than the corresponding theoretical predictions and are consistent with the standard model and the Planck baryon density. Moreover, D/H now provides a tight measurement of Nν when combined with the CMB baryon density and provides a 2 σ upper limit Nνpointing to new physics. This paper concludes with a look at future directions including key nuclear reactions, astronomical observations, and theoretical issues.

  18. Desorption of alkali atoms from 4He nanodroplets.

    Science.gov (United States)

    Hernando, Alberto; Barranco, Manuel; Pi, Martí; Loginov, Evgeniy; Langlet, Marina; Drabbels, Marcel

    2012-03-21

    The dynamics following the photoexcitation of Na and Li atoms located on the surface of helium nanodroplets has been investigated in a joint experimental and theoretical study. Photoelectron spectroscopy has revealed that excitation of the alkali atoms via the (n + 1)s ←ns transition leads to the desorption of these atoms. The mean kinetic energy of the desorbed atoms, as determined by ion imaging, shows a linear dependence on excitation frequency. These experimental findings are analyzed within a three-dimensional, time-dependent density functional approach for the helium droplet combined with a Bohmian dynamics description of the desorbing atom. This hybrid method reproduces well the key experimental observables. The dependence of the observables on the impurity mass is discussed by comparing the results obtained for the (6)Li and (7)Li isotopes. The calculations show that the desorption of the excited alkali atom is accompanied by the creation of highly non-linear density waves in the helium droplet that propagate at supersonic velocities.

  19. Thermal neutron capture cross sections resonance integrals and g-factors

    CERN Document Server

    Mughabghab, S F

    2003-01-01

    The thermal radiative capture cross sections and resonance integrals of elements and isotopes with atomic numbers from 1 to 83 (as well as sup 2 sup 3 sup 2 Th and sup 2 sup 3 sup 8 U) have been re-evaluated by taking into consideration all known pertinent data published since 1979. This work has been undertaken as part of an IAEA co-ordinated research project on 'Prompt capture gamma-ray activation analysis'. Westcott g-factors for radiative capture cross sections at a temperature of 300K were computed by utilizing the INTER code and ENDF-B/VI (Release 8) library files. The temperature dependence of the Westcott g-factor is illustrated for sup 1 sup 1 sup 3 Cd, sup 1 sup 2 sup 4 Xe and sup 1 sup 5 sup 7 Gd at temperatures of 150, 294 and 400K. Comparisons have also been made of the newly evaluated capture cross sections of sup 6 Li, sup 7 Li, sup 1 sup 2 C and sup 2 sup 0 sup 7 Pb with those determined by the k sub 0 method.

  20. Development of detector for neutron monitor of wide energy range. Joint research

    CERN Document Server

    Kim, E; Nakamura, T; Rasolonjatovo, D R D; Shiomi, T; Tanaka, S; Yamaguchi, Y; Yoshizawa, M

    2002-01-01

    Radiation monitoring of neutrons in high-power proton accelerator facilities is very important for radiation safety management for workers and members of the public. In the present study, a neutron detector that can evaluate dose of neutrons in the energy range from thermal energy to 100MeV was developed using an organic liquid scintillator, a boron-loaded scintillator and a sup 6 Li glass scintillator. First, a method was developed to evaluate neutron doses above several MeV by a spectrum weight function (G-function) which is applied to the organic liquid scintillator, and the validity of the methods was confirmed by dose evaluation in some neutron fields. Second, the G-function was applied to the boron-loaded scintillator which detects thermal neutrons by sup 1 sup 0 B(n, alpha) sup 7 Li reaction, in order to expand the covering neutron energy range. The response function and the G-function of the scintillator were evaluated by experiment and calculation, and the characteristics of dose measurement were ana...

  1. ANSL-V: ENDF/B-V based multigroup cross-section libraries for Advanced Neutron Source (ANS) reactor studies. Supplement 1

    Energy Technology Data Exchange (ETDEWEB)

    Wright, R.Q.; Renier, J.P.; Bucholz, J.A.

    1995-08-01

    The original ANSL-V cross-section libraries (ORNL-6618) were developed over a period of several years for the physics analysis of the ANS reactor, with little thought toward including the materials commonly needed for shielding applications. Materials commonly used for shielding applications include calcium barium, sulfur, phosphorous, and bismuth. These materials, as well as {sup 6}Li, {sup 7}Li, and the naturally occurring isotopes of hafnium, have been added to the ANSL-V libraries. The gamma-ray production and gamma-ray interaction cross sections were completely regenerated for the ANSL-V 99n/44g library which did not exist previously. The MALOCS module was used to collapse the 99n/44g coupled library to the 39n/44g broad- group library. COMET was used to renormalize the two-dimensional (2- D) neutron matrix sums to agree with the one-dimensional (1-D) averaged values. The FRESH module was used to adjust the thermal scattering matrices on the 99n/44g and 39n/44g ANSL-V libraries. PERFUME was used to correct the original XLACS Legendre polynomial fits to produce acceptable distributions. The final ANSL-V 99n/44g and 39n/44g cross-section libraries were both checked by running RADE. The AIM module was used to convert the master cross-section libraries from binary coded decimal to binary format (or vice versa).

  2. Microanalysis system of ppm-order 10B concentrations in tissue for neutron capture therapy by prompt gamma-ray spectrometry

    Science.gov (United States)

    Kobayashi, Tooru; Kanda, Keiji

    1983-01-01

    For neutron capture therapy, a new technique for measuring 10B concentrations of ppm order in tissue has been developed by using 10B(n, α) 7Li ∗ prompt gamma-ray spectrometry. The measuring system consists of a Ge(Li) detector and a 6LiF tile neutron shield attached to the neutron guide tube of the Kyoto University Reactor (KUR) with very low background gamma-rays. The 10B concentrations of unknown samples were determined in comparison with gamma-ray data obtained from known samples. The detection limit of the system is 0.1-0.5 ppm 10B concentration. In the practical use of the system for neutron capture therapy, 10B concentrations of 10 ppm, which is ordinarily pre-injected into the tumor, can be measured in less than 30 s with 10% accuracy by using 1 g samples. Moreover, the system has the advantage that pre-treatment of the sample is not required. As a neutron monitor in a homogeneous sample, gamma-rays emitted from H(n, γ)D reactions are used. Therefore, neutron irradiation conditions of this system, i.e. fluence rate, energy spectrum, and distribution in the sample do not affect the analyzing results, and the quantity and dimensions of the sample are also not restricted.

  3. Local field in LiD polarized target material

    CERN Document Server

    Kisselev, Yu V; Baum, G; Berglund, P; Doshita, N; Gautheron, F; Görtz, S; Horikawa, N; Koivuniemi, J H; Kondo, K; Magnon, A; Meyer, Werner T; Reicherz, G

    2004-01-01

    We have experimentally studied the first and the second moments of D, **6Li and **7Li (I greater than 1/2) NMR lines in a granulated LiD- target material as a function of nuclear polarizations and the data has been compared with a theory elaborated by Abragam, Roinel and Bouffard for monocrystalline samples. The experiments were carried out in the large COMPASS twin-target at CERN. The static local magnetic field of the polarized nuclei was measured by frequency shift between the NMR-signals in the two oppositely polarized cells and lead to the first moment, whereas the investigation of the second moment was done through Gaussian approximation. The average field magnitude in granulated material was estimated 20% larger than the value given by the calculations for monocrystalline samples of cylindrical shape. The second moment shows a qualitative agreement with the theory but it is slightly larger at the negative than at the positive polarization. In a polarized mode, the moments depend on the saturated microw...

  4. Scoping Analyses on Tritium Permeation to VHTR Integarted Industrial Application Systems

    Energy Technology Data Exchange (ETDEWEB)

    Chang H. Oh; Eung S. Kim

    2011-03-01

    Tritium permeation is a very important current issue in the very high temperature reactor (VHTR) because tritium is easily permeated through high temperature metallic surfaces. Tritium permeations in the VHTR-integrated systems were investigated in this study using the tritium permeation analysis code (TPAC) that was developed by Idaho National Laboratory (INL). The INL TPAC is a numerical tool that is based on the mass balance equations of tritium containing species and hydrogen (i.e. HT, H2, HTO, HTSO4, TI) coupled with a variety of tritium sources, sink, and permeation models. In the TPAC, ternary fission and thermal neutron caption reactions with 6Li, 7Li 10B, 3He were taken into considerations as tritium sources. Purification and leakage models were implemented as main tritium sinks. Permeation of tritium and H2 through pipes, vessels, and heat exchangers were considered as main tritium transport paths. In addition, electroyzer and isotope exchange models were developed for analyzing hydrogen production systems including high temperature electrolysis (HTSE) and sulfur-iodine processes.

  5. Magic wavelengths for optical cooling and trapping of lithium

    CERN Document Server

    Safronova, M S; Clark, Charles W

    2012-01-01

    Using first-principles calculations, we identify magic wavelengths for the 2s-2p and 2s-3p transitions in lithium. The ns and np atomic levels have the same ac Stark shifts at the corresponding magic wavelength, which facilitates state-insensitive optical cooling and trapping. Tune-out wavelengths for which the ground-state frequency-dependent polarizability vanishes are also calculated. Differences of these wavelengths between 6Li and 7Li are reported. Our approach uses high-precision, relativistic all-order methods in which all single, double, and partial triple excitations of the Dirac-Fock wave functions are included to all orders of perturbation theory. Recommended values are provided for a large number of Li electric-dipole matrix elements. Static polarizabilities for the 2s, 2p, 3s, 3p, and 3d levels are compared with other theory and experiment where available. Uncertainties of all recommended values are estimated. The magic wavelengths for the uv 2s-3p transition are of particular interest for the pr...

  6. Neutron spectral measurements in an intense photon field associated with a high-energy x-ray radiotherapy machine.

    Science.gov (United States)

    Holeman, G R; Price, K W; Friedman, L F; Nath, R

    1977-01-01

    High-energy x-ray radiotherapy machines in the supermegavoltage region generate complex neutron energy spectra which make an exact evaluation of neutron shielding difficult. Fast neutrons resulting from photonuclear reactions in the x-ray target and collimators undergo successive collisions in the surrounding materials and are moderated by varying amounts. In order to examine the neutron radiation exposures quantitatively, the neutron energy spectra have been measured inside and outside the treatment room of a Sagittaire medical linear accelerator (25-MV x rays) located at Yale-New Haven Hospital. The measurements were made using a Bonner spectrometer consisting of 2-, 3-, 5-, 8-, 10- and 12-in.-diameter polyethylene spheres with 6Li and 7Li thermoluminescent dosimeter (TLD) chips at the centers, in addition to bare and cadmium-covered chips. The individual TLD chips were calibrated for neutron and photon response. The spectrometer was calibrated using a known PuBe spectrum Spectrometer measurements were made at Yale Electron Accelerator Laboratory and results compared with a neutron time-of-flight spectrometer and an activation technique. The agreement between the results from these independent methods is found to be good, except for the measurements in the direct photon beam. Quality factors have been inferred for the neutron fields inside and outside the treatment room. Values of the inferred quality factors fall primarily between 4 and 8, depending on location.

  7. Relative Composition and Energy Spectra of Light Nuclei in Cosmic Rays: Results from AMS-01

    Science.gov (United States)

    Aguilar, M.; Alcaraz, J.; Allaby, J.; Alpat, B.; Ambrosi, G.; Anderhub, H.; Ao, L.; Arefiev, A.; Arruda, L.; Azzarello, P.; Basile, M.; Barao, F.; Barreira, G.; Bartoloni, A.; Battiston, R.; Becker, R.; Becker, U.; Bellagamba, L.; Béné, P.; Berdugo, J.; Berges, P.; Bertucci, B.; Biland, A.; Bindi, V.; Boella, G.; Boschini, M.; Bourquin, M.; Bruni, G.; Buénerd, M.; Burger, J. D.; Burger, W. J.; Cai, X. D.; Cannarsa, P.; Capell, M.; Casadei, D.; Casaus, J.; Castellini, G.; Cernuda, I.; Chang, Y. H.; Chen, H. F.; Chen, H. S.; Chen, Z. G.; Chernoplekov, N. A.; Chiueh, T. H.; Choi, Y. Y.; Cindolo, F.; Commichau, V.; Contin, A.; Cortina-Gil, E.; Crespo, D.; Cristinziani, M.; Dai, T. S.; dela Guia, C.; Delgado, C.; Di Falco, S.; Djambazov, L.; D'Antone, I.; Dong, Z. R.; Duranti, M.; Engelberg, J.; Eppling, F. J.; Eronen, T.; Extermann, P.; Favier, J.; Fiandrini, E.; Fisher, P. H.; Flügge, G.; Fouque, N.; Galaktionov, Y.; Gervasi, M.; Giovacchini, F.; Giusti, P.; Grandi, D.; Grimm, O.; Gu, W. Q.; Haino, S.; Hangarter, K.; Hasan, A.; Hermel, V.; Hofer, H.; Hungerford, W.; Ionica, M.; Jongmanns, M.; Karlamaa, K.; Karpinski, W.; Kenney, G.; Kim, D. H.; Kim, G. N.; Kim, K. S.; Kirn, T.; Klimentov, A.; Kossakowski, R.; Kounine, A.; Koutsenko, V.; Kraeber, M.; Laborie, G.; Laitinen, T.; Lamanna, G.; Laurenti, G.; Lebedev, A.; Lechanoine-Leluc, C.; Lee, M. W.; Lee, S. C.; Levi, G.; Lin, C. H.; Liu, H. T.; Lu, G.; Lu, Y. S.; Lübelsmeyer, K.; Luckey, D.; Lustermann, W.; Maña, C.; Margotti, A.; Mayet, F.; McNeil, R. R.; Menichelli, M.; Mihul, A.; Mujunen, A.; Oliva, A.; Palmonari, F.; Park, H. B.; Park, W. H.; Pauluzzi, M.; Pauss, F.; Pereira, R.; Perrin, E.; Pevsner, A.; Pilo, F.; Pimenta, M.; Plyaskin, V.; Pojidaev, V.; Pohl, M.; Produit, N.; Quadrani, L.; Rancoita, P. G.; Rapin, D.; Ren, D.; Ren, Z.; Ribordy, M.; Richeux, J. P.; Riihonen, E.; Ritakari, J.; Ro, S.; Roeser, U.; Sagdeev, R.; Santos, D.; Sartorelli, G.; Sbarra, C.; Schael, S.; Schultz von Dratzig, A.; Schwering, G.; Seo, E. S.; Shin, J. W.; Shoumilov, E.; Shoutko, V.; Siedenburg, T.; Siedling, R.; Son, D.; Song, T.; Spada, F. R.; Spinella, F.; Steuer, M.; Sun, G. S.; Suter, H.; Tang, X. W.; Ting, Samuel C. C.; Ting, S. M.; Tomassetti, N.; Tornikoski, M.; Torsti, J.; Trümper, J.; Ulbricht, J.; Urpo, S.; Valtonen, E.; Vandenhirtz, J.; Velikhov, E.; Verlaat, B.; Vetlitsky, I.; Vezzu, F.; Vialle, J. P.; Viertel, G.; Vité, D.; Von Gunten, H.; Waldmeier Wicki, S.; Wallraff, W.; Wang, J. Z.; Wiik, K.; Williams, C.; Wu, S. X.; Xia, P. C.; Xu, S.; Xu, Z. Z.; Yan, J. L.; Yan, L. G.; Yang, C. G.; Yang, J.; Yang, M.; Ye, S. W.; Zhang, H. Y.; Zhang, Z. P.; Zhao, D. X.; Zhou, F.; Zhou, Y.; Zhu, G. Y.; Zhu, W. Z.; Zhuang, H. L.; Zichichi, A.; Zimmermann, B.; Zuccon, P.

    2010-11-01

    Measurement of the chemical and isotopic composition of cosmic rays is essential for the precise understanding of their propagation in the galaxy. While the model parameters are mainly determined using the B/C ratio, the study of extended sets of ratios can provide stronger constraints on the propagation models. In this paper, the relative abundances of light-nuclei lithium, beryllium, boron, and carbon are presented. The secondary-to-primary ratios Li/C, Be/C, and B/C have been measured in the kinetic energy range 0.35-45 GeV nucleon-1. The isotopic ratio 7Li/6Li is also determined in the magnetic rigidity interval 2.5-6.3 GV. The secondary-to-secondary ratios Li/Be, Li/B, and Be/B are also reported. These measurements are based on the data collected by the Alpha Magnetic Spectrometer AMS-01 during the STS-91 space shuttle flight in 1998 June. Our experimental results are in substantial agreement with other measurements, where they exist. We describe our light-nuclei data with a diffusive-reacceleration model. A 10%-15% overproduction of Be is found in the model predictions and can be attributed to uncertainties in the production cross-section data.

  8. Relative Composition and Energy Spectra of Light Nuclei in Cosmic Rays. Results from AMS-01

    CERN Document Server

    Aguilar, M; Allaby, J; Alpat, B; Ambrosi, G; Anderhub, H; Ao, L; Arefiev, A; Arruda, L; Azzarello, P; Basile, M; Barao, F; Barreira, G; Vartoloni, A; Battiston, R; Becker, R; Becker, U; Bellagamba, L; Bene, P; Berdugo, J; Berges, P; Bertucci, B; Biland, A; Bindi, V; Boella, G; Boschini, M; Bourquin, M; Bruni, G; Buenerd, M; Burger, J D; Burger, W J; Cai, X D; Cannarsa, P; Capell, M; Casadei, D; Casaus, J; Castellini, G; Cernuda, I; Chang, Y H; Chen, H F; Chen, H S; Chen, Z G; Chernoplekov, N A; Chiueh, T H; Choi, Y Y; Cindolo, F; Commichau, V; Contin, A; Cortina-Gil, E; Crespo, D; Cristinziani, M; Dai, T S; Dela Guia, C; Delgado, C; Di Falco, S; Djambazov, L; D'Antoine, I; Dong, Z R; Duranti, M; Engelberg, J; Eppling, F J; Eronen, T; Extermann, P; Favier, J; Fiandrini, E; Fisher, P H; Flugge, G; Fouque, N; Galaktionov, Y; Gervasi, M; Giovacchini, F; Giusti, P; Grandi, D; Grimm, O; Gu, W Q; Haino, S; Hangarter, K; Hasan, A; Hermel, V; Hofer, H; Hungerford, W; Ionica, M; Jongmanns, M; Karlamaa, K; Karpinski, W; Kenney, G; Kim, D H; Kim, G N; Kim, K S; Kirn, T; Klimentov, A; Kossakowski, R; Kounine, A; Koutsenko, V; Kraeber, M; Laborie, G; Laitinen, T; Lamanna, G; Laurenti, G; Lebedev, A; Lechanoine-Leluc, C; Lee, M W; Lee, S C; Levi, G; Lin, C H; Liu, H T; Lu, G; Lubelsmeyer, K; Luckey, D; Lustermann, W; Mana, C; Margotti, A; Mayet, F; McNeil, R R; Menichelli, M; Mihul, A; Mujunen, A; Oliva, A; Palmonari, F; Park, H B; Park, W H; Pauluzzi, M; Pauss, F; Pereira, R; Perrin, E; Pevsner, A; Pilo, F; Pimenta, M; Plyaskin, V; Pojidaev, V; Pohl, M; Produit, N; Quadrani, L; Rancoita, P G; Rapin, D; Ren, D; Ren, Z; Ribordy, M; Richeux, J P; Riihonen, E; Ritakari, J; Ro, S; Roeser, U; Sagdeev, R; Santos, D; Sartorelli, G; Sbarra, C; Schael, S; Schultz von Dratzig, A; Schwering, G; Seo, E S; Shin, J W; Shoumilov, E; Shoutko, V; Siedenburg, T; Siedling, R; Son, D; Song, T; Spada, F R; Spinella, F; Steuer, M; Sun, G S; Suter, H; Tang, X W; Ting, Samuel C C; Ting, S M; Tomassetti, N; Tornikoski, M; Torsti, J; Trumper, J; Ulbricht, J; Urpo, S; Valtonen, E; Vandenhirtz, J; Velikhov, E; Verlaat, B; Vetlitsky, I; Vezzu, F; Vialle, J P; Viertel, G; Vite, D; Von Gunten, H; Waldmeier Wicki, S; Wallraff, W; Wang, J Z; Wiik, K; Williams, C; Wu, S X; Xia, P C; Xu, S; Xu, Z Z; Yan, J L; Yan, L G; Yang, C G; Yang, J; Yang, M; Ye, S W; Zhang, H Y; Zhang, Z P; Zhao, D X; Zhou, F; Zhou, Y; Zhu, G Y; Zhu, W Z; Zhuang, H L; Zichichi, A; Zimmermann, B; Zuccon, P

    2010-01-01

    Measurement of the chemical and isotopic composition of cosmic rays is essential for the precise understanding of their propagation in the galaxy. While the model parameters are mainly determined using the B/C ratio, the study of extended sets of ratios can provide stronger constraints on the propagation models. In this paper the relative abundances of the light nuclei lithium, beryllium, boron and carbon are presented. The secondary to primary ratios Li/C, Be/C and B/C have been measured in the kinetic energy range 0.35-45 GeV/nucleon. The isotopic ratio 7Li/6Li is also determined in the magnetic rigidity interval 2.5-6.3 GV. The secondary to secondary ratios Li/Be, Li/B and Be/B are also reported. These measurements are based on the data collected by the Alpha Magnetic Spectrometer AMS-01 during the STS-91 space shuttle flight in 1998 June. Our experimental results are in substantial agreement with other measurements, where they exist. We describe our light-nuclei data with a diffusive-reacceleration model....

  9. High accuracy measurement of the $^{235}$U(n,f) reaction cross-section in the 10-30 keV neutron energy range

    CERN Multimedia

    The analysis of the neutron flux of n_TOF (in EAR1) revealed an anomaly in the 10-30 keV neutron energy range. While the flux extracted on the basis of the $^{6}$Li(n,t)$^{4}$He and $^{10}$B(n,$\\alpha$)$^{7}$Li reactions mostly agreed with each other and with the results of FLUKA simulations of the neutron beam, the one based on the $^{235}$U(n,f) reaction was found to be systematically lower, independently of the detection system used. A possible explanation is that the $^{235}$U(n,f) crosssection in that energy region, where in principle should be known with an uncertainty of 1%, may be systematically overestimated. Such a finding, which has a negligible influence on thermal reactors, would be important for future fast critical or subcritical reactors. Furthermore, its interest is more general, since the $^{235}$U(n,f) reaction is often used at that energy to determine the neutron flux, or as reference in measurements of fission cross section of other actinides. We propose to perform a high-accuracy, high-r...

  10. Integrating techniques for neutron dosimetry in Linac 18 MV; Integrando tecnicas para dosimetria de neutrones en un Linac de 18 MV

    Energy Technology Data Exchange (ETDEWEB)

    Ceron R, P. V.; Diaz G, J. A. I.; Rivera M, T. [IPN, Centro de Investigacion en Ciencia Aplicada y Tecnologia Avanzada, Av. Legaria 694, 11500 Mexico D. F. (Mexico); Paredes G, L. C. [ININ, Carretera Mexico-Toluca s/n, 52750 Ocoyoacac, Estado de Mexico (Mexico); Vega C, H. R. [Universidad Autonoma de Zacatecas, Unidad Academica de Estudios Nucleares, Cipres No. 10, Fracc. La Penuela, 98068 Zacatecas, Zac. (Mexico)

    2015-10-15

    In this paper thermoluminescent dosimetry, analytical techniques and Monte Carlo calculations were used to estimate the neutron dose equivalent in a radiotherapy room with a linear electron accelerator of 18 MV. The equivalent dose was measured at isocenter to 1.42 m of target and at the entrance of the labyrinth of the room of a Novalis Tx. The neutron detectors were constructed with pairs of thermoluminescent dosimeters TLD 600 ({sup 6}LiF: Mg, Ti) and TLD 700 ({sup 7}LiF: Mg, Ti) which are placed inside a paraffin sphere of 20 cm in diameter. These measurements enabled the calculation of equivalent dose in the gate and the source term, using the relationships contained in the NCRP-151. Through the models carried out with the code MCNPX the absorbed dose distribution with regard to depth in a paraffin phantom are included and the neutron spectrum produced by the head, taking into account the geometry and component materials. The results are in the order of neutron milli sievert by gray of X-rays (mSv/Gy x) which are in the same order as those found in other reports for different accelerators. (Author)

  11. Compression and phase diagram of lithium hydrides at elevated pressures and temperatures by first-principles calculations

    CERN Document Server

    Chen, Yang M; Wu, Qiang; Geng, Hua Y; Yan, Xiao Z; Wang, Yi X; Wang, Zi W

    2016-01-01

    High pressure and high temperature properties of AB (A = $^6$Li, $^7$Li; B = H, D, T) are investigated with first-principles method comprehensively. It is found that the H$^{-}$ sublattice features in the low-pressure electronic structure near the Fermi level of LiH are shifted to that dominated by the Li$^{+}$ sublattice in compression. The lattice dynamics is studied in quasi-harmonic approximation, from which the phonon contribution to the free energy and the isotopic effects are accurately modelled with the aid of a parameterized double-Debye model. The obtained equation of state (EOS) matches perfectly with available static experimental data. The calculated principal Hugoniot is also in accordance with that derived from shock wave experiments. Using the calculated principal Hugoniot and the previous theoretical melting curve, we predict a shock melting point at 56 GPa and 1923 K. In order to establish the phase diagram for LiH, the phase boundaries between the B1 and B2 solid phases are explored. The B1-...

  12. Structural characterisation of amorphous materials by solid state NMR

    CERN Document Server

    Mollison, N B

    2002-01-01

    Solid state nuclear magnetic resonance (NMR) is a structural elucidation technique that is ideal as a probe in the investigation of atomic structure of highly complex amorphous materials. In this study, NMR is employed in the structural characterisation of a series of sodium-lithium disilicate glasses. These so-called 'mixed-alkali' glasses are of great scientific interest, since they exhibit non-linear ionic transport related properties; the theory of which is not understood, but is thought to be related to the cation distribution in the disilicate network. This project attempts to utilise solid state NMR to its fullest potential, by combining several techniques, including the novel MQMAS experiment and a series of double resonance measurements. The double resonance techniques TRAPDOR and SEDOR have been attempted to measure sup 2 sup 9 Si-left brace sup 2 sup 3 Na right brace and sup 6 sup , sup 7 Li-left brace sup 7 sup , sup 6 Li right brace interactions respectively. Since these experiments rely on the d...

  13. Neutron-photon mixed field dosimetry by TLD-700 glow curve analysis and its implementation in dose monitoring for Boron Neutron Capture Therapy (BNCT) treatments

    Energy Technology Data Exchange (ETDEWEB)

    Boggio, E. F.; Longhino, J. M. [Centro Atomico Bariloche, Departamento de Fisica de Reactores y Radiaciones / CNEA, Av. E. Bustillo Km 9.5, R8402AGP San Carlos de Bariloche (Argentina); Andres, P. A., E-mail: efboggio@cab.cnea.gov.ar [Centro Atomico Bariloche, Division Proteccion Radiologica / CNEA, Av. E. Bustillo Km 9.5, R8402AGP San Carlos de Bariloche (Argentina)

    2015-10-15

    BNCT is a cancerous cells selective, non-conventional radiotherapy modality to treat malignant tumors such as glioblastoma, melanoma and recurrent head and neck cancer. It consists of a two-step procedure: first, the patient is injected with a tumor localizing drug containing a non-radioactive isotope (Boron-10) with high slow neutron capture cross-section. In a second step, the patient is irradiated with neutrons, which are absorbed by the Boron-10 agent with the subsequently nuclear reaction B- 10(n,a)Li-7, thereby resulting in dose at cellular level due to the high-Let particles. The neutron fields suitable for BNCT are characterized by high neutron fluxes and low gamma dose. Determination of each component is not an easy task, especially when the volume of measurement is quite small or inaccessible for a miniature ionization chamber, for example. A method of measuring the photon and slow neutron dose(mainly by N-14 and B-10) from the glow curve (GC) analysis of a single {sup 7}LiF thermoluminescence detector is evaluated. This method was suggested by the group headed by Dr. Grazia Gambarini. The dosemeters used were TLD-600 ({sup 6}LiF:Mg,Ti with 95.6% {sup 6}Li) and TLD-700 ({sup 7}LiF:Mg,Ti with 99.9% {sup 7}LiF) from Harshaw. Photon dose measurement using the GC analysis method with TLD-700 in mixed fields requires the relation of the two main peaks of a TLD-600 GC shape obtained from an exposition to the same neutron field, and a photon calibrated GC with TLD-700. The requirements for slow neutron dose measurements are similar. In order to properly apply the GC analysis method at the Ra-6 Research Reactor BNCT facility, measurements were carried out in a standard water phantom, fully characterized on the BNCT beam by conventional techniques (activation detectors and paired ionization chambers technique). Next, the method was implemented in whole body dose monitoring of a patient undergoing a BNCT treatment, using a Bo MAb (Bottle Manikin Absorption) phantom

  14. Search for the existence of the tetra-neutron through the He{sup 8}(d,Li{sup 6})4n nuclear reaction; Recherche de l'existence eventuelle du tetraneutron via la reaction de transfert {sup 8}He(d, {sup 6}Li)4n

    Energy Technology Data Exchange (ETDEWEB)

    Rich, E

    2005-10-15

    The He{sup 8}(d,Li{sup 6})4n reaction is studied through reverse kinematics: a radioactive beam of He{sup 8} nuclei impinges on a CD{sub 2} target. The measurement of the energy spectrum and emission angle distribution of Li{sup 6} has allowed us to determine by applying kinematics laws the excitation energy spectrum of the 4 neutrons system released in the reaction. The first chapter recalls the main features of the nucleon-nucleon interaction and reviews recent experiments on multi-neutrons. The second chapter presents the experimental setting from the production of the He{sup 8} beam at GANIL to the detection system of the reaction products via the data acquisition system. The method of the missing mass gives the mass of the 4 neutron system. The third and fourth chapters deal with the calibration of the detection system, the missing mass method is applied to the following reactions: C{sup 12}(d,Li{sup 6})Be{sup 8}, C{sup 12}(d,t)C{sup 11} and C{sup 12}(d,He{sup 3})B{sup 11}. The last chapter presents the experimental results. The analysis of the excitation energy spectrum of the 4 neutron systems shows no evidence for the existence of a bound state. We get a maximal limit of 60 {mu}b for the production cross section of a bound state. Complementary results concerning the excitation energy spectra of the di-neutron and tri-neutron released in the reactions: He{sup 8}(d,Li{sup 8})2n and He{sup 8}(d,Li{sup 7})3n are also presented. (A.C.)

  15. Cs7Sm11[TeO3]12Cl16 and Rb7Nd11[TeO3]12Br16, the new tellurite halides of the tetragonal Rb6LiNd11[SeO3]12Cl16 structure type

    OpenAIRE

    Dmitri O. Charkin; Black, Cameron; Downie, Lewis James; Sklovsky, Dmitry E.; Peter S. Berdonosov; Olenev, Andrei V.; Zhou, Wuzong; Lightfoot, Philip; Dolgikh, Valery A.

    2015-01-01

    The authors thank the Russian Foundation for Basic Researches for the support of this work under Grants No. 14-03-00604_a and 12-03-92604-KO_a. The X-ray study of compound II was made possible due to M.V. Lomonosov Moscow State University Programm of Development. PL thanks the University of St Andrews and EPSRC for DTA Studentships to CB and LJD. Two new rare-earth – alkali – tellurium oxide halides were synthesized by a salt flux technique and characterized by single-crystal X-ray diffrac...

  16. Calorimetria nucleare in collisioni tra ioni pesanti ad energie intermedie

    Science.gov (United States)

    Spezzi, L.

    2002-07-01

    Nel presente lavoro di tesi ci si e' occupati di uno studio sistematico di misure di temperatura ed energia di eccitazione in sistemi nucleari formati in reazioni tra ioni pesanti ad energie intermedie. La temperatura a stata misurata tramite due diversi metodi: rapporto tra le rese di isotopi che differiscono di uno stesso numero di nucleoni ( d/t-3He/4He , 3He/4He -6Li/7Li) - temperatura isotopica -, e rapporto tra le popolazioni degli stati eccitati in frammenti instabili (5Li e 6Li) che decadono in particelle leggere in coincidenza - temperatura di emissione. Le misure in esame sono state effettuate presso i Laboratori Nazionali del Sud per i sistemi 93Nb+93Nb, 93Nb+116,124Sn, 116,120Sn+116,124Sn e 116Sn+93Nb ad energie comprese tra 17 e 40 A MeV. L'apparato di rivelazione era costituito da un odoscopio ad alta granularite (96 telescopi Si (50micron)-Si(300micron)-CsI(Tl) ) e basse soglie di rivelazione, utilizzato sia per identificare risonanze in frammenti eccitati che per misure di rese di isotopi di frammenti con 2<=Z<=6, e dal multirivelatore FIASCO che, grazie alla misura contemporanea di posizione e tempo di volo dei frammenti provenienti dal proiettile (PLF - Projectile Like Fragments) e dal bersaglio (TLF - Target Like Fragment), e' stato utilizzato per misurare direttamente l'energia di eccitazione del sistema in studio. Analisi precedenti, condotte nell'ambito di varie collaborazioni, hanno messo in evidenza la possible esistenza di una transizione di fase liquido-gas del primo ordine nella materia nucleare. In tale contesto, ci siamo occupati di una verifica della curva calorica nucleare, ovvero della correlazione esistente fra temperatura ed energia di eccitazione del sistema, indagando, nel contempo, sulla sua dipendenza dalla massa del sistema che si frammenta. Si e' effettuato, inoltre, un confronto fra i due diversi metodi di misura della temperatura (temperatura isotopica e di emissione): l'andamento plateau-like della curva calorica e' stato

  17. HELIX: The High Energy Light Isotope Experiment

    Science.gov (United States)

    Wakely, Scott

    stage, which is the subject of this proposal, will focus on the design and construction of the main HELIX instrument, and the measurement of key light isotope ratios from ~200 MeV/n to ~3GeV/n. A future stage 2 will build on this work, incorporating evolutionary enhancements to the instrumentation to extend the energy reach into the challenging ~10 GeV/n range. The stage 1 instrument achieves a maximum detectable rigidity of ~800GV and charge range from Z=1 to Z=10. The high field of the HEAT magnet will make it possible to reach the required mass resolution dm/m = 2.5% over the energy range of concern with very small systematic limitations due to multiple Coulomb scattering in the thin tracker. This is a decisive advantage over the current AMS-02 instrument which employs a permanent magnet with an average field ~7 times smaller than that of HELIX. The primary scientific goals of the full HELIX program are: - a high-statistics measurement of the 10Be/9Be 'clock ratio' to ~10 GeV/nuc - a high-statistics measurement of the 3He/4He ratio to ~12GeV/nuc - the first measurements of 22Ne/20Ne above 1 GeV/nuc - the first measurements of 7Li/6Li, and 10B/11B above 1 GeV//nuc A number of secondary goals will also be pursued including the measurement of several other isotopic and elemental abundance ratios and fluxes, as well as the primary Helium flux to ~125 GeV/nuc, where there is currently disagreement between AMS-02 and PAMELA on the shape of the energy spectrum. The proposed work will be conducted by a team of US scientists and engineers with extensive experience in cosmic-ray observations on balloons or in space, and, specifically in magnet spectroscopy, with the SMILI, P-BAR, and HEAT programs. Significant participation from a crew of more than 10 graduate and undergraduate students forms an important educational element of the program.

  18. Using R-matrix Theory to Analyze Resonant Reactions

    Energy Technology Data Exchange (ETDEWEB)

    Hale, G.M. [Theoretical Division Los Alamos National Laboratory (United States)

    2006-07-01

    Full text of publication follows: We begin with a summary of R-matrix theory, formulated in terms of Green's functions that include the Bloch operator to apply the boundary conditions. This is a general approach, not restricted to any particular reaction mechanism, that nevertheless is particularly well-suited to describing resonant reactions. We then give a brief description of the capabilities of the general Los Alamos R-matrix code, EDA. This code can fit the data for any type of measurement for a reaction involving any types of two-body channels (including charged particles and photons), using an automated chi-square minimization algorithm that has quadratic convergence and yields the covariance matrix of the fitting parameters at a local chi-square minimum. This allows covariance information to be produced for the calculated (cross-section) data. As time allows, several examples will be given for light systems, including reactions initiated by n+p ({sup 2}H), n+{sup 6}Li ({sup 7}Li), n+{sup 10}B ({sup 11}B), and n+{sup 16}O ({sup 17}O). These systems have varying numbers of visible resonances, ranging from none in the {sup 2}H system up to many in the {sup 17}O system. However, the same R-matrix approach gives a good description of the data in all cases, several of which were used in the recent IAEA standards evaluation, and in Endf/B7 general-purpose files. Some aspects of the output covariances that result from such R-matrix analyses will be discussed. (authors)

  19. SU-E-T-594: Out-Of-Field Neutron and Gamma Dose Estimated Using TLD-600/700 Pairs in the Wobbling Proton Therapy System

    Energy Technology Data Exchange (ETDEWEB)

    Chen, Y [College of Medicine, Chang Gung University, Linkou, Taoyuan, Taiwan (China); Lin, Y [College of Medicine, Chang Gung University, Linkou, Taoyuan, Taiwan (China); Medical Physics Research Center, Institute for Radiological Research, Chang Gung University / Chang Gung Memorial Hospital, Linkou, Taoyuan, Taiwan (China); Chen, H [College of Medicine, Chang Gung University, Linkou, Taoyuan, Taiwan (China); Chang Gung Memorial Hospital, Linkou, Taoyuan, Taiwan (China); Tsai, H [College of Medicine, Chang Gung University, Linkou, Taoyuan, Taiwan (China); Medical Physics Research Center, Institute for Radiological Research, Chang Gung University / Chang Gung Memorial Hospital, Linkou, Taoyuan, Taiwan (China); Healthy Aging Research Center, Chang Gung University, Linkou, Taoyuan, Taiwan (China)

    2015-06-15

    Purpose: Secondary fast neutrons and gamma rays are mainly produced due to the interaction of the primary proton beam with the beam delivery nozzle. These secondary radiation dose to patients and radiation workers are unwanted. The purpose of this study is to estimate the neutron and gamma dose equivalent out of the treatment volume during the wobbling proton therapy system. Methods: Two types of thermoluminescent (TL) dosimeters, TLD-600 ({sup 6}LiF: Mg, Ti) and TLD-700 ({sup 7}LiF: Mg, Ti) were used in this study. They were calibrated in the standard neutron and gamma sources at National Standards Laboratory. Annealing procedure is 400°C for 1 hour, 100°C for 2 hours and spontaneously cooling down to the room temperature in a programmable oven. Two-peak method (a kind of glow curve analysis technique) was used to evaluate the TL response corresponding to the neutron and gamma dose. The TLD pairs were placed outside the treatment field at the neutron-gamma mixed field with 190-MeV proton beam produced by the wobbling system through the polyethylene plate phantom. The results of TLD measurement were compared to the Monte Carlo simulation. Results: The initial experiment results of calculated dose equivalents are 0.63, 0.38, 0.21 and 0.13 mSv per Gy outside the field at the distance of 50, 100, 150 and 200 cm. Conclusion: The TLD-600 and TLD-700 pairs are convenient to estimate neutron and gamma dosimetry during proton therapy. However, an accurate and suitable glow curve analysis technique is necessary. During the wobbling system proton therapy, our results showed that the neutron and gamma doses outside the treatment field are noticeable. This study was supported by the grants from the Chang Gung Memorial Hospital (CMRPD1C0682)

  20. SRAG Measurements Performed During the Orion EFT-1 Mission

    Science.gov (United States)

    Gaza, Ramona

    2015-01-01

    The Exploration Flight Test 1 (EFT-1) was the first flight of the Orion Multi-Purpose Crew Vehicle (MPCV). The flight was launched on December 5, 2014, by a Delta IV Heavy rocket and lasted 4.5 hours. The EFT-1 trajectory involved one low altitude orbit and one high altitude orbit with an apogee of almost 6000 km. As a result of this particular flight profile, the Orion MPCV passed through intense regions of trapped protons and electron belts. In support of the radiation measurements aboard the EFT-1, the Space Radiation Analysis Group (SRAG) provided a Battery-operated Independent Radiation Detector (BIRD) based on Timepix radiation monitoring technology similar to that employed by the ISS Radiation Environmental Monitors (REM). In addition, SRAG provided a suite of optically and thermally stimulated luminescence detectors, with 2 Radiation Area Monitor (RAM) units collocated with the BIRD instrument for comparison purposes, and 6 RAM units distributed at different shielding configurations within the Orion MPCV. A summary of the EFT-1 Radiation Area Monitors (RAM) mission dose results obtained from measurements performed in the Space Radiation Dosimetry Laboratory at the NASA Johnson Space Center will be presented. Each RAM included LiF:Mg,Ti (TLD-100), (6)LiF:Mg,Ti (TLD-600), (7)LiF:Mg,Ti (TLD-700), Al2O3:C (Luxel trademark), and CaF2:Tm (TLD-300). The RAM mission dose values will be compared with the BIRD instrument total mission dose. In addition, a similar comparison will be shown for the ISS environment by comparing the ISS RAM data with data from the six Timepix-based REM units deployed on ISS as part of the NASA REM Technology Demonstration.

  1. Properties of A = 7-9 Drip-Line Nuclei in RMF Theory

    Institute of Scientific and Technical Information of China (English)

    WANG Cheng-Bin; DONG Tie-Kuang; REN Zhong-Zhou; ZHU Zhi-Yuan

    2009-01-01

    The relativistic mean-field (RMF) theory is used to calculate the properties of A = 7-9 drip-line nuclei 7Li, 7;9Be, 8;9B, and 9C. Systematic deviations between experimental and theoretical binding energies are found. Possible reasons of these systematic deviations are discussed in terms of pairing energy. The root-mean-square (rms) radii of matter distributions for these nuclei agree with the experimental data quite well. The one-proton halo structure in 8B is reproduced well, and the two-proton halo in 9C is predicted. The calculations show that the RMF theory is valid in studying the properties of light drip-line nuclei.

  2. Light elements burning reaction rates at stellar temperatures as deduced by the Trojan Horse measurements

    Energy Technology Data Exchange (ETDEWEB)

    Lamia, L. [Dipartimento di Fisica e Astronomia, Università degli Studi di Catania, Catania (Italy); Spitaleri, C. [Dipartimento di Fisica e Astronomia, Università degli Studi di Catania, Catania, Italy and INFN-Laboratori Nazionali del Sud, Catania (Italy); La Cognata, M.; Palmerini, S.; Sergi, M. L. [INFN-Laboratori Nazionali del Sud, Catania (Italy); Puglia, S. M. R. [INFN-Laboratori Nazionali del Sud, Catania, Italy and Dipartimento di Fisica e Astronomia, Università degli Studi di Catania, Catania (Italy)

    2015-02-24

    Experimental nuclear astrophysics aims at determining the reaction rates for astrophysically relevant reactions at their Gamow energies. For charged-particle induced reactions, the access to these energies is usually hindered, in direct measurements, by the presence of the Coulomb barrier between the interacting particles or by electron screening effects, which make hard the determination of the bare-nucleus S(E)-factor of interest for astrophysical codes. The use of the Trojan Horse Method (THM) appears as one of the most suitable tools for investigating nuclear processes of interest for astrophysics. Here, in view of the recent TH measurements, the main destruction channels for deuterium ({sup 2}H), for the two lithium {sup 6,7}Li isotopes, for the {sup 9}Be and the one for the two boron {sup 10,11}B isotopes will be discussed.

  3. The behaviour of Li and Mg isotopes during primary phase dissolution and secondary mineral formation in basalt

    Science.gov (United States)

    Wimpenny, Josh; Gíslason, Sigurður R.; James, Rachael H.; Gannoun, Abdelmouhcine; Pogge Von Strandmann, Philip A. E.; Burton, Kevin W.

    2010-09-01

    fluid become increasingly heavy with time, consistent with previous experimental work and natural data indicating that 6Li is preferentially incorporated into secondary minerals, leaving the solution enriched in 7Li. The behaviour of Mg isotopes is different from that anticipated or observed in natural systems. Similar to the far from equilibrium experiments initially light Mg is lost during olivine dissolution, but with time the δ 26Mg value of the solution becomes increasingly heavy. This suggests either preferential loss of light, and then heavy Mg from olivine, or that the secondary phase preferentially incorporates light Mg from solution. Assuming that the secondary phase is chrysotile, a Mg-silicate, the sense of Mg fractionation is opposite to that previously associated with silicate soils and implies that the fractionation of Mg isotopes during silicate precipitation may be mineral specific. If secondary silicates do preferentially remove light Mg from solution then this could be a possible mechanism for the relatively heavy δ 26Mg value of seawater. This study highlights the utility of experimental studies to quantify the effects of natural weathering reactions on the Li and Mg geochemical cycles.

  4. Development and Verification of Tritium Analyses Code for a Very High Temperature Reactor

    Energy Technology Data Exchange (ETDEWEB)

    Chang H. Oh; Eung S. Kim

    2009-09-01

    A tritium permeation analyses code (TPAC) has been developed by Idaho National Laboratory for the purpose of analyzing tritium distributions in the VHTR systems including integrated hydrogen production systems. A MATLAB SIMULINK software package was used for development of the code. The TPAC is based on the mass balance equations of tritium-containing species and a various form of hydrogen (i.e., HT, H2, HTO, HTSO4, and TI) coupled with a variety of tritium source, sink, and permeation models. In the TPAC, ternary fission and neutron reactions with 6Li, 7Li 10B, 3He were taken into considerations as tritium sources. Purification and leakage models were implemented as main tritium sinks. Permeation of HT and H2 through pipes, vessels, and heat exchangers were importantly considered as main tritium transport paths. In addition, electroyzer and isotope exchange models were developed for analyzing hydrogen production systems including both high-temperature electrolysis and sulfur-iodine process. The TPAC has unlimited flexibility for the system configurations, and provides easy drag-and-drops for making models by adopting a graphical user interface. Verification of the code has been performed by comparisons with the analytical solutions and the experimental data based on the Peach Bottom reactor design. The preliminary results calculated with a former tritium analyses code, THYTAN which was developed in Japan and adopted by Japan Atomic Energy Agency were also compared with the TPAC solutions. This report contains descriptions of the basic tritium pathways, theory, simple user guide, verifications, sensitivity studies, sample cases, and code tutorials. Tritium behaviors in a very high temperature reactor/high temperature steam electrolysis system have been analyzed by the TPAC based on the reference indirect parallel configuration proposed by Oh et al. (2007). This analysis showed that only 0.4% of tritium released from the core is transferred to the product hydrogen

  5. Kinetic Isotopic Fractionation During Diffusion of Ionic Speciesin Water

    Energy Technology Data Exchange (ETDEWEB)

    Richter, Frank M.; Mendybaev, Ruslan A.; Christensen, John; Hutcheon, Ian D.; Williams, Ross W.; Sturchio, Neil C.; Beloso Jr.,Abelardo D.

    2005-06-09

    Experiments specifically designed to measure the ratio of the diffusivities of ions dissolved in water were used to determine D{sub Li}/D{sub K}, D{sub 7{sub Li}}/D{sub 6{sub Li}}, D{sub 25{sub Mg}}/D{sub 24{sub Mg}}, D{sub 26{sub Mg}}/D{sub 25{sub Mg}}, and D{sub 37{sub Cl}}/D{sub 35{sub Cl}}. The measured ratio of the diffusion coefficients for Li and K in water (D{sub Li}/D{sub K} = 0.6) is in good agreement with published data, providing evidence that the experimental design being used resolves the relative mobility of ions with adequate precision to also be used for determining the fractionation of isotopes by diffusion in water. In the case of Li we found measurable isotopic fractionation associated with the diffusion of dissolved LiCl (D{sub 7{sub Li}}/D{sub 6{sub Li}} = 0.99772 {+-} 0.00026). This difference in the diffusion coefficient of {sup 7}Li compared to {sup 6}Li is significantly less than reported in an earlier study, a difference we attribute to the fact that in the earlier study Li diffused through a membrane separating the water reservoirs. Our experiments involving Mg diffusing in water found no measurable isotopic fractionation (D{sub 25{sub Mg}}/D{sub 24{sub Mg}} = 1.00003 {+-} 0.00006). Cl isotopes were fractionated during diffusion in water (D{sub 37{sub Cl}}/D{sub 35{sub Cl}} = 0.99857 {+-} 0.00080) whether or not the co-diffuser (Li or Mg) was isotopically fractionated. The isotopic fractionation associated with the diffusion of ions in water is much smaller than values we found previously for the isotopic fractionation of Li and Ca isotopes by diffusion in molten silicate liquids. A major distinction between water and silicate liquids is that water, being a polar liquid, surrounds dissolved ions with hydration shells, which very likely play an important but still poorly understood role in reducing isotopic fractionation associated with diffusion.

  6. CO2 capture properties of lithium silicates with different ratios of Li2O/SiO2: an ab initio thermodynamic and experimental approach.

    Science.gov (United States)

    Duan, Yuhua; Pfeiffer, Heriberto; Li, Bingyun; Romero-Ibarra, Issis C; Sorescu, Dan C; Luebke, David R; Halley, J Woods

    2013-08-28

    The lithium silicates have attracted scientific interest due to their potential use as high-temperature sorbents for CO2 capture. The electronic properties and thermodynamic stabilities of lithium silicates with different Li2O/SiO2 ratios (Li2O, Li8SiO6, Li4SiO4, Li6Si2O7, Li2SiO3, Li2Si2O5, Li2Si3O7, and α-SiO2) have been investigated by combining first-principles density functional theory with lattice phonon dynamics. All these lithium silicates examined are insulators with band-gaps larger than 4.5 eV. By decreasing the Li2O/SiO2 ratio, the first valence bandwidth of the corresponding lithium silicate increases. Additionally, by decreasing the Li2O/SiO2 ratio, the vibrational frequencies of the corresponding lithium silicates shift to higher frequencies. Based on the calculated energetic information, their CO2 absorption capabilities were extensively analyzed through thermodynamic investigations on these absorption reactions. We found that by increasing the Li2O/SiO2 ratio when going from Li2Si3O7 to Li8SiO6, the corresponding lithium silicates have higher CO2 capture capacity, higher turnover temperatures and heats of reaction, and require higher energy inputs for regeneration. Based on our experimentally measured isotherms of the CO2 chemisorption by lithium silicates, we found that the CO2 capture reactions are two-stage processes: (1) a superficial reaction to form the external shell composed of Li2CO3 and a metal oxide or lithium silicate secondary phase and (2) lithium diffusion from bulk to the surface with a simultaneous diffusion of CO2 into the shell to continue the CO2 chemisorption process. The second stage is the rate determining step for the capture process. By changing the mixing ratio of Li2O and SiO2, we can obtain different lithium silicate solids which exhibit different thermodynamic behaviors. Based on our results, three mixing scenarios are discussed to provide general guidelines for designing new CO2 sorbents to fit practical needs.

  7. Space radiation absorbed dose distribution in a human phantom

    Science.gov (United States)

    Badhwar, G. D.; Atwell, W.; Badavi, F. F.; Yang, T. C.; Cleghorn, T. F.

    2002-01-01

    -rate predictions are 20% lower than the observations. Assuming that the trapped-belt models lead to a correct orbit-averaged energy spectrum, the measurements of dose rates inside the phantom cannot be fully understood. Passive measurements using 6Li- and 7Li-based detectors on the astronauts and inside the brain and thyroid of the phantom show the presence of a significant contribution due to thermal neutrons, an area requiring additional study.

  8. Experimental investigations of the neutron contamination in high-energy photon fields at medical linear accelerators

    Energy Technology Data Exchange (ETDEWEB)

    Brunckhorst, Elin

    2009-02-26

    The scope of this thesis was to develop a device for the detection of the photoneutron dose inside the high-energy photon field. The photoneutron contamination of a Siemens PRIMUS linear accelerator was investigated in detail in its 15 MV photon mode. The experimental examinations were performed with three ionisation chambers (a tissue equivalent chamber, a magnesium chamber and a {sup 10}B-coated magnesium chamber) and two types of thermoluminescence detectors (enriched with {sup 6}Li and {sup 7}Li, respectively). The detectors have different sensitivities to photons and neutrons and their combination allows the dose separation in a mixed neutron/photon field. The application of the ionisation chamber system, as well as the present TLD system for photoneutron detection in high-energy photon beams is a new approach. The TLD neutron sensitivity was found to be too low for a measurement inside the open photon field and the further investigation focused on the ionisation chambers. The three ionisation chambers were calibrated at different photon and neutron sources and a the borated magnesium chamber showed a very high response to thermal neutrons. For a cross check of the calibration, the three chambers were also used for dose separation of a boron neutron capture therapy beam where the exact determination of the thermal neutron dose is essential. Very accurate results were achieved for the thermal neutron dose component. At the linear accelerator the chamber system was reduced to a paired chamber system utilising the two magnesium chambers, since the fast neutron component was to small to be separated. The neutron calibration of the three chambers could not be applied, instead a conversion of measured thermal neutron signal by the borated chamber to Monte Carlo simulated total neutron dose was performed. Measurements for open fields in solid water and liquid water were performed with the paired chamber system. In larger depths the neutron dose could be determined

  9. Rb-Sr isotopic composition of granites in the Western Krušné hory/Erzgebirge pluton, Central Europe: record of variations in source lithologies, mafic magma input and postmagmatic hydrothermal events

    Science.gov (United States)

    Dolejš, David; Bendl, Jiří; Štemprok, Miroslav

    2016-10-01

    The late Variscan (327-318 Ma) Western Krušné hory/Erzgebirge pluton (Czech Republic and Germany) represents a multiply emplaced intrusive sequence ranging from low-F biotite monzogranites (with rare minor bodies of gabbrodiorites and granodiorites) to high-F topaz-zinnwaldite alkali-feldspar granites. This granite suite is characterized by progressively increasing concentrations of incompatible elements (Li, Rb, F), monotonous decrease in mafic components and compatible elements (FeOtot, MgO, TiO2, CaO, Sr) with increasing silica. Consequently, this leads to extreme variations in the Rb/Sr ratios (0.52 to 59), which impose highly variable 87Rb/86Sr and 87Sr/86Sr signatures. The low-F biotite monzogranites represent isotopically heterogeneous mixture with (87Sr/86Sr)323 = 0.707-0.709 between partial melts from the Saxothuringian metasediments and mantle-derived mafic precursors. The medium-F two-mica microgranites show variable (87Sr/86Sr)323 = 0.708-0.714, indicating involvement of multiple precursors and more mature crustal protoliths. The evolved high-F topaz-zinnwaldite alkali-feldspar granites were derived from a precursor with (87Sr/86Sr)320 = 0.707-0.708 at 324-317 Ma by differentiation, which produced the extreme Rb/Sr enrichment and variations. The Li/Rb ratios remain nearly constant (~0.5), thus insensitive to the degree of geochemical differentiation. In comparison to terrestrial variations, the high Li/Rb values indicate derivation of granitic magmas from predominantly sedimentary precursors, in accord with 7Li-6Li and 143Nd-144Nd isotope composition reported previously. The Rb-Sr element variations in each granite unit are sligthly different and indicate ascent and emplacement of separate magma batches, which do not form a single liquid line of descent. We consider the enrichment of granites in incompatible elements (Li, Rb, F) and compatible depletion of ferromagnesian components, CaO and Sr as a combined effect of multiple precursors, changes in

  10. Lifetime of the metastable 2/sup 3/S/sub 1/ state in stored Li/sup +/ ions

    Energy Technology Data Exchange (ETDEWEB)

    Knight, R.D.

    1979-04-01

    A laser-induced fluorescence technique combined with the observation of spontaneous magnetic dipole photons from the highly metastable 2/sup 3/S/sub 1/ state of Li/sup +/ was used to measure the radiative lifetime of this state. The ions are created by electron impact on a lithium atomic beam and are subsequently stored for periods of many seconds in an RF-quadrupole ion trap. A tunable dye laser excites the 2/sup 3/S--2/sup 3/P, transition at 5485A, and the intercombination electric dipole transition 2/sup 3/P/sub 1/--1 /sup 1/S/sub 0/ at 202A is observed. This process depletes the metastable population in a time tau/sub d/ < 1 sec < < tau/sub /sup 3/S/sub 1// and provides a measure of the total number of metastables. Comparison with the rate of 210A spontaneously emitted photons yields a measured value for the 2/sup 3/S/sub 1/ radiative lifetime of tau/sub rad/ = 58.6 +- 12.9 sec, where the quoted error represents 95% confidence levels. The theoretical lifetime is tau/sub theory/ = 49.0 sec. The measured value includes data taken with both /sup 6/Li/sup +/ and /sup 7/Li/sup +/ isotopes and was corrected for the slightly different detector efficiencies at 202A and 210A. A careful study of nonradiative quenching of the metastable state was necessary to understand observed differences between tau/sub rad/ and tau/sub /sup 3/S/sub 1//, the total metastable lifetime. Spatial density profiles of the ions within the trap, useful for determining the ion temperature, were obtained by scanning the laser beam horizontally across the ion trap while storing 2/sup 3/P/sub 1/--/sup 1/S/sub 0/ photon counts as a function of the laser beam's position. Agreement with a simple equilibrium model, including space charge effects, is satisfactory. A study of the optical pumping process is necessary to understand the laser-ion interaction, and observational and theoretical data are presented. 47 references.

  11. Unstable nuclei in dissociation of light stable and radioactive nuclei in nuclear track emulsion

    CERN Document Server

    Artemenkov, D A; Zarubin, P I

    2016-01-01

    A role of the unstable nuclei ${}^{6}$Be, ${}^{8}$Be and ${}^{9}$B in the dissociation of relativistic nuclei ${}^{7,9}$Be, ${}^{10}$B and ${}^{10,11}$C is under study on the basis of nuclear track emulsion exposed to secondary beams of the JINR Nuclotron. Contribution of the configuration ${}^{6}$Be + $\\mit{n}$ to the ${}^{7}$Be nucleus structure is 8 $\\pm$ 1% which is near the value for the configuration ${}^{6}$Li + $\\mit{p}$. Distributions over the opening angle of $\\alpha$-particle pairs indicate to a simultaneous presence of virtual ${}^{8}$Be$_{g.s.}$ and ${}^{8}$Be$_{2^+}$ states in the ground states of the ${}^{9}$Be and ${}^{10}$C nuclei. The core ${}^{9}$B is manifested in the {${}^{10}$C} nucleus with a probability of 30 $\\pm$ 4%. Selection of the ${}^{10}$C "white" stars accompanied by ${}^{8}$Be$_{g.s.}$ (${}^{9}$B) leads to appearance in the excitation energy distribution of 2$\\alpha$2$\\mit{p}$ "quartets" of the distinct peak with a maximum at 4.1 $\\pm$ 0.3 MeV. ${}^{8}$Be$_{g.s.}$ decays are p...

  12. Development and construction of a neutron beam line for accelerator-based boron neutron capture synovectomy.

    Science.gov (United States)

    Gierga, D P; Yanch, J C; Shefer, R E

    2000-01-01

    A potential application of the 10B(n, alpha)7Li nuclear reaction for the treatment of rheumatoid arthritis, termed Boron Neutron Capture Synovectomy (BNCS), is under investigation. In an arthritic joint, the synovial lining becomes inflamed and is a source of great pain and discomfort for the afflicted patient. The goal of BNCS is to ablate the synovium, thereby eliminating the symptoms of the arthritis. A BNCS treatment would consist of an intra-articular injection of boron followed by neutron irradiation of the joint. Monte Carlo radiation transport calculations have been used to develop an accelerator-based epithermal neutron beam line for BNCS treatments. The model includes a moderator/reflector assembly, neutron producing target, target cooling system, and arthritic joint phantom. Single and parallel opposed beam irradiations have been modeled for the human knee, human finger, and rabbit knee joints. Additional reflectors, placed to the side and back of the joint, have been added to the model and have been shown to improve treatment times and skin doses by about a factor of 2. Several neutron-producing charged particle reactions have been examined for BNCS, including the 9Be(p,n) reaction at proton energies of 4 and 3.7 MeV, the 9Be(d,n) reaction at deuteron energies of 1.5 and 2.6 MeV, and the 7Li(p,n) reaction at a proton energy of 2.5 MeV. For an accelerator beam current of 1 mA and synovial boron uptake of 1000 ppm, the time to deliver a therapy dose of 10,000 RBEcGy ranges from 3 to 48 min, depending on the treated joint and the neutron producing charged particle reaction. The whole-body effective dose that a human would incur during a knee treatment has been estimated to be 3.6 rem or 0.75 rem, for 1000 ppm or 19,000 ppm synovial boron uptake, respectively, although the shielding configuration has not yet been optimized. The Monte Carlo design process culminated in the construction, installation, and testing of a dedicated BNCS beam line on the high

  13. Absolute level-resolved reactive and inelastic rate constants in Li+Li2*

    Science.gov (United States)

    Coppage, Steven; Matei, Paula; Stewart, Brian

    2008-06-01

    We have used nuclear parity-changing collisions to obtain absolute level-to-level rate constants for reactive scattering in a triatomic system with identical nuclei. We have determined rate constants for the system 7Li2*(A 1Σu+)(vi=2,ji=19)+7Li-->7Li+7Li2*(A 1Σu+)(vf,jf), from laser-induced fluorescence spectra of lithium vapor in a heat pipe oven. Parity-preserving collisions yielded measurements of absolute rotationally and vibrationally inelastic rate constants as well. We compare the reactive rate constants with statistical prior distributions and the inelastic results with previously measured results on the Ne+7Li2* system.

  14. A new capability for ANTARES: {sup 7}Be by AMS for ice samples

    Energy Technology Data Exchange (ETDEWEB)

    Smith, A.M., E-mail: ams@ansto.gov.au [Australian Nuclear Science and Technology Organisation (ANSTO), Locked Bag 2001, Kirrawee, NSW 2232 (Australia); Mokhber-Shahin, L.; Simon, K.J. [Australian Nuclear Science and Technology Organisation (ANSTO), Locked Bag 2001, Kirrawee, NSW 2232 (Australia)

    2013-01-15

    ANSTO, in collaboration with Australian Antarctic Division (AAD) and the Antarctic Climate and Ecosystems Cooperative Research Centre (ACE CRC), has an on-going program of {sup 10}Be (t{sub Vulgar-Fraction-One-Half} = 1.39 Multiplication-Sign 10{sup 6} a) concentration measurement in firn and ice at Law Dome, Antarctica. In recent years snow pit samples have also been measured for {sup 7}Be (t{sub Vulgar-Fraction-One-Half} = 53.28 d) concentration as this isotope has the potential to give further insight into the transport and deposition of cosmogenic beryllium to Law Dome and so improve the use of {sup 10}Be as a proxy for solar activity. Early {sup 7}Be measurements were made by gamma-ray spectrometry (GRS) with typical counting times of 3 days. In 2010, we developed the capability for {sup 7}Be/{sup 9}Be measurement on the 10 MV ANTARES (Australian National Tandem Accelerator for Applied Research) accelerator using carbon foil post-stripping of {sup 7}Be{sup 3+} to {sup 7}Be{sup 4+} to eliminate the {sup 7}Li isobar. We describe the method and explain the advantages of using accelerator mass spectrometry (AMS) over GRS for {sup 7}Be analysis.

  15. Search for a bound K− pp system

    Directory of Open Access Journals (Sweden)

    Camerini P.

    2010-04-01

    Full Text Available Data from the K− absorption reaction on 6,7Li, 9Be, 13C and 16O have recently been collected by FINUDA at the DAΦNE φ-factory (Laboratori Nazionali di Frascati-INFN, following an earlier lower statitics run on 12C and some other targets. FINUDA is a high acceptance magnetic spectrometer which performed a wide range of studies by detecting the charged particles and neutrons exiting the targets after the absorption event. In this paper it is discussed about the study of the A(K− , Λp reaction in the context of the search for deeply bound $ar{K}$ - nuclear states. The observation of a bump in the Λp invariant mass distribution is discussed in terms of a possible signature of a deeply bound K− pp kaonic cluster as well as of more conventional physics. An overview of the experimental situation in this field will be given.

  16. A new capability for ANTARES: 7Be by AMS for ice samples

    Science.gov (United States)

    Smith, A. M.; Mokhber-Shahin, L.; Simon, K. J.

    2013-01-01

    ANSTO, in collaboration with the Australian Antarctic Division (AAD) and the Antarctic Climate and Ecosystems Cooperative Research Centre (ACE CRC), has an on-going program of 10Be (t½ = 1.39 × 106 a) concentration measurement in firn and ice at Law Dome, Antarctica. In recent years snow pit samples have also been measured for 7Be (t½ = 53.28 d) concentration as this isotope has the potential to give further insight into the transport and deposition of cosmogenic beryllium to Law Dome and so improve the use of 10Be as a proxy for solar activity. Early 7Be measurements were made by gamma-ray spectrometry (GRS) with typical counting times of 3 days. In 2010, we developed the capability for 7Be/9Be measurement on the 10 MV ANTARES (Australian National Tandem Accelerator for Applied Research) accelerator using carbon foil post-stripping of 7Be3+ to 7Be4+ to eliminate the 7Li isobar. We describe the method and explain the advantages of using accelerator mass spectrometry (AMS) over GRS for 7Be analysis.

  17. Study of neutron-induced background and its impact on the search of 0$\

    CERN Document Server

    Dokania, N; Mathimalar, S; Ghosh, C; Nanal, V; Pillay, R G; Pal, S; Bhushan, K G; Shrivastava, A

    2014-01-01

    Neutron-induced background has been studied in various components of the TIN.TIN detector, which is under development for the search of Neutrinoless Double Beta Decay in $\\rm^{124}Sn$. Fast neutron flux $\\sim10^{6}~n~cm^{-2}s^{-1}$ covering a broad energy range ($ \\sim0.1$ to $ \\sim18$~MeV) was generated using $^{9}Be(p,n)^{9}B$ reaction. In addition, reactions with quasi-monoenergetic neutrons were also studied using $^{7}Li(p,n)^{7}Be$ reaction. Among the different cryogenic support structures studied, Teflon is found to be preferable compared to Torlon as there is no high energy gamma background ($E_\\gamma >$ 1 MeV). Contribution of neutron-induced reactions in $\\rm ^{nat, 124} $Sn from other Sn isotopes (A = 112 -- 122) in the energy region of interest, namely, around the $Q_{\\beta\\beta}$ of $\\rm^{124}Sn$ ($E \\sim$ 2.293 MeV), is also investigated.

  18. Decay analysis of compound nuclei with mass A$\\sim 30-200$ formed in the reactions involving loosely bound projectiles

    CERN Document Server

    Kaur, Mandeep; Sharma, Manoj K; Gupta, Raj K

    2015-01-01

    The dynamics of the reactions forming compound nuclei using loosely bound projectiles is analysed within the framework of dynamical cluster decay model (DCM) of Gupta and Collaborators. We have analysed different reactions with $^{7}Li$, $^{9}Be$ and $^{7}Be$ as neutron rich and neutron deficient projectiles, respectively, on different targets at the three $E_{lab}$ values, forming compound nuclei within the mass region A$\\sim 30-200$. The contributions of light particles LPs ($A\\le4$) cross sections $\\sigma_{LP}$, energetically favoured intermediate mass fragments IMFs ($5 \\le A_2 \\le 20$) cross sections $\\sigma_{IMF}$ as well as fusion-fission $\\it{ff}$ cross sections $\\sigma_{ff}$ constitute the $\\sigma_{fus}$ (=$\\sigma_{LP}$+$\\sigma_{IMF}$+$\\sigma_{ff}$) for these reactions. The contribution of the emitted LPs, IMFs and ff fragments is added for all the angular momentum upto the $\\ell_{max}$ value, for the resepctive reactions. Interestingly, we find that the $\\Delta R^{emp}$, the only parameter of model ...

  19. Annual report of the Tandem Accelerator Center, University of Tsukuba. April 1, 1997 - March 31, 1998

    Energy Technology Data Exchange (ETDEWEB)

    NONE

    1998-06-01

    This report briefly described the investigations performed during the period from April 1997 to March 1998 in Tandem Accelerator Center. The 12 UD Pelletron tandem accelerator was reconstructed and the first beam test was carried out in Nov. 1997. In nuclear physics, the measurement of total reaction cross sections, the non-resonant breakup of {sup 7}Li and {sup 9}Be, the investigation of hole states via (p,d) reaction, nuclear structure physics by means of in-beam {gamma} ray spectroscopy and the study of the three dimensional cranking model have been performed. In interdisciplinary fields, the development of AMS system has been continued. The trace element analysis of mineral samples has been carried out by means of PIXE with the proton beam which was focused on the sample as narrow as 50 {mu}m{sup 2}. The hydrogen analysis using H({sup 19}F,{alpha}{gamma}) reaction has been started aiming at the extension of the measurement of depth profile down to a few tens of {mu}m deep region. (M.N.)

  20. Review of Big Bang Nucleosynthesis and Primordial Abundances

    Science.gov (United States)

    Tytler, David; O'Meara, John M.; Suzuki, Nao; Lubin, Dan

    2001-03-01

    the light nuclei, but unfortunately in most cases we are not yet seeing much improvement in the accuracy of the primordial abundances. Since we are now interested in the highest accuracy and reliability for all nuclei, the few objects with the most extensive observations give by far the most convincing results. Earlier measurements of 4He may have obtained too low a value because the He emission line strengths were reduced by undetected stellar absorption lines. The systematic errors associated with the 4He abundance have frequently been underestimated in the past, and this problem persists. When two groups use the same data and different ways to estimate the electron density and 4He abundance, the results differ by more than the quoted systematic errors. While the methods used by Izotov and Thuan [1] seem to be an advance on those used before, the other method is reasonable, and hence the systematic error should encompass the range in results. The abundance of 7Li is measured to high accuracy, but we do not know how much was produced prior to the formation of the stars, and how much was destroyed (depleted) in the stars. 6Li helps limit the amount of depletion of 7Li, but by an uncertain amount since it too has been depleted. BBN is successful because it uses known physics and measured cross-sections for the nuclear reactions. It gives accurate predictions for the abundances of five light nuclei as a function of the one free parameter η. The other initial conditions seem natural: the universe began homogeneous and hotter than T > 1011 K (30 Mev). The predicted abundances agree with most observations, and the required η is consistent with other, less accurate, measurements of the baryon density. Abundance measurements of the baryon density, from the CMB, clusters of galaxies and the Lyα forest, will give η. Although the accuracy might not exceed that obtained from D/H, this is an important advance because BBN then gives abundance predictions with no adjustable

  1. Transparent lithiated polymer films for thermal neutron detection

    Science.gov (United States)

    Mabe, Andrew N.; Auxier, John D.; Urffer, Matthew J.; Penumadu, Dayakar; Schweitzer, George K.; Miller, Laurence F.

    2013-09-01

    Novel water-soluble 6Li loaded copolymer scintillation films have been designed and fabricated to detect thermal neutrons. Styrene and maleic anhydride were copolymerized to form an alternating copolymer, then the anhydride functionality was hydrolyzed using 6Li hydroxide. The resulting poly(styrene-co-lithium maleate) was mixed with salicylic acid as a fluor and cast as a thin film from water. The maximum 6Li loading obtained that resulted in a transparent film was 4.36% by mass (6Li to polymer). The optimum fluorescence output was obtained for 11.7% salicylic acid by mass, presumably in the form of lithium salicylate, resulting in an optimum film containing 3.85% by mass of 6Li. A facile and robust synthesis method, film fabrication protocol, photoluminescence results, and scintillation responses are reported herein.

  2. {sup 8}Li + p reaction and the primordial nucleosynthesis

    Energy Technology Data Exchange (ETDEWEB)

    Mendes Junior, D.R.; Lepine-Szily, A.; Lichtenthaeler, Rubens; Guimaraes, Valdir; Faria, P.N. de; Barioni, Adriana; Camargo Junior, Orli; Pires, K.C.C.; Morcelle, Viviane; Morais, Maria Carmen; Candori, R. Pampa; Scarduelli, Valdir; Leistenschneider, Erick [Universidade de Sao Paulo (IF/USP), SP (Brazil). Inst. de Fisica. Dept. de Fisica Nuclear; Assuncao, Marlete [Universidade Federal de Sao Paulo (UNIFESP), SP (Brazil); Descouvemont, P. [Universite Libre de Bruxelles, Brussels (Belgium). Physique Theorique et Mathematique

    2011-07-01

    Full text: We present a direct measurement of the {sup 8}Li(p,{alpha}){sup 5}He cross section, using a radioactive {sup 8}Li beam impinging on target of CH{sub 2}. This target has a thickness of 6.8 mg/cm{sup 2}, that is thick enough to stop the {sup 8}Li beam in it. The {sup 8}Li beam was produced at the primary target by the reaction {sup 9}Be({sup 7}Li,{sup 8}Li){sup 8}Be and was focalized by the first superconductor solenoid of RIBRAS on a secondary CH{sub 2} target. The reaction products were measured with four silicon barrier detectors, mounted as {Delta}E-E telescopes, where the {Delta}E detectors were 20{mu}m thick and the E detectors were 1000 {mu}m thick. The measurements were performed between Ecm=0.2 and 2.5 MeV at several laboratory angles. They show a broad peak around 1.7 MeV where the cross-section is almost isotropic. At low energies the data show a clear evidence for an increase of the S-factor. This suggests the importance of subthreshold states in {sup 9}Be. An R-matrix analysis of the experimental data has been performed in order to derive spectroscopic information (such as energies, neutron and alpha widths) of some resonances and to extrapolate the data down to zero energy. This R-matrix fit is then used to determine the {sup 8}Li(p,{alpha}){sup 5}He reaction rate, which is compared to the {sup 8}Li({alpha},n){sup 11}B reaction rate. (author)

  3. Lithium isotope behaviour during weathering in the Ganges Alluvial Plain

    Science.gov (United States)

    Pogge von Strandmann, Philip A. E.; Frings, Patrick J.; Murphy, Melissa J.

    2017-02-01

    The Ganges river system is responsible for the transportation of a large flux of dissolved materials derived from Himalayan weathering to the oceans. Silicate weathering-driven cooling resulting from uplift of the Himalayas has been proposed to be a key player in Cenozoic climate variation. This study has analysed Li isotope (δ7Li) ratios from over 50 Ganges river waters and sediments, in order to trace silicate weathering processes. Sediments have δ7Li of ∼0‰, identical to bulk continental crust, however suspended sediment depth profiles do not display variations associated with grain size that have been observed in other large river systems. Dissolved δ7Li are low (∼11‰) in the Ganges headwaters, but reach a constant value of 21 ± 1.6‰ within a relatively short distance downstream, which is then maintained for almost 2000 km to the Ganges mouth. Given that Li isotopes are controlled by the ratio of primary mineral dissolution to secondary mineral formation, this suggests that the Ganges floodplain is at steady-state in terms of these processes for most of its length. Low δ7Li in the mountainous regions suggest silicate weathering is therefore at its most congruent where uplift and fresh silicate exposure rates are high. However, there is no correlation between δ7Li and the silicate weathering rate in these rivers, suggesting that Li isotopes cannot be used as a weathering-rate tracer, although they do inform on weathering congruency and intensity. The close-to-constant δ7Li values for the final 2000 km of Ganges flow also suggest that once the size of the alluvial plain reached more than ∼500 km (the flow distance after which riverine δ7Li stops varying), the Ganges exerted little influence on the changing Cenozoic seawater δ7Li, because riverine δ7Li attained a near steady-state composition.

  4. Reaction cross sections and elastic scattering energy dependence around the Coulomb barrier for the {sup 7}Be+{sup 27}Al system

    Energy Technology Data Exchange (ETDEWEB)

    Morcelle, Viviane; Gomes, P.R.S.; Lubian, J.; Mendes Junior, D.R. [Universidade Federal Fluminense (UFF), Niteroi, RJ (Brazil); Lichtenthaeler, R.; Guimaraes, V.; Lepine-Szily, A.; Camargo, O.; Faria, P.N. de; Gasquez, L.; Morais, M.C.; Condori, R.P.; Pires, K.C.C.; Scarduelli, V. [Universidade de Sao Paulo (USP), SP (Brazil); Barioni, A. [Universidade Federal da Bahia (UFBA), Salvador, BA (Brazil); Shorto, J.M.B. [Instituto de Pesquisas Energeticas e Nucleares (IPEN/CNEN-SP), Sao Paulo, SP (Brazil); Zamora, J.C. [Technische Universitaet Darmstadt (Germany); Aguilera, E.; Martinez-Quiroz, E. [Instituto Nacional de Investigaciones Nucleares (Mexico); Kolata, J.; Jiang, H. [University of Notre Dame, IN (United States); Bechetti, F.D.; Lamm, L.O. [Michigan University, MI (United States); Lizcano, D. [Universidad Autonoma del Estado de Mexico (Mexico)

    2012-07-01

    Full text: Elastic scattering measurements were performed at energies around the Coulomb barrier at the Tandem Accelerators of the Sao Paulo (USP - Brazil ) and Notre Dame (UND - USA) Universities. The {sup 7}Be is a radioactive nucleus and has been produced by the reaction {sup 6}He({sup 6}Li,{sup 9}Be) and impinged on {sup 27}Al and {sup 197}Au secondary targets using a double superconducting systems RIBRAS ( USP ) and Twinsol (UND). The elastic scattering angular distributions were analyzed through the optical model calculations, using the Woods- Saxon form factors [1] and the Sao Paulo potential [2] to fit the experimental data. The total reaction cross sections were also derived and compared with others presented at the literature for other systems. In addition, a study of the nuclear potential energy dependence has been carried out in this work in the dispersion relation context. Due to the fact that {sup 7}Be has a small breakup threshold energy, the results can provide significant information of the influence of the breakup channel on the reactions involving this projectile. For this purpose, {chi}{sup 2}- data analysis with different kind of potentials were performed to identify the energy dependence of the real (V) and imaginary (W) parts of the potential. [1] L.C. Chamon et al., Phys. Rev. C 66, (2002) 014610. [2] R.D. Wood e D.S. Saxon, Phys. Rev. 95 ( 1954) 577. (author)

  5. Disentangling the transfer and breakup contributions from the inclusive ^{8}Li+ ^{208}Pb reaction

    CERN Document Server

    Moro, A M; García-Martínez, H; Aguilera, E F; Martínez-Quiroz, E; Gómez-Camacho, J

    2003-01-01

    An analysis of the elastic and one-neutron removal channel for the reaction (^{8})Li+(^{208})Pb reaction at energies around the Coulomb barrier is presented. For the elastic scattering, an optical model analysis of the experimental data is performed. The observed (^{7})Li is interpreted as the superposition of the one-neutron transfer reaction, (^{208})Pb((^{8})Li,(^{7} )Li)(^{209})Pb, and the breakup reaction. The separate contribution of each one of these processes has been calculated within the DWBA formalism. The sum of both contributions explains adequately the experimental angular distribution of (^{7})Li.

  6. Natural ageing responses of duplex structured Mg-Li based alloys

    Science.gov (United States)

    Li, C. Q.; Xu, D. K.; Wang, B. J.; Sheng, L. Y.; Qiao, Y. X.; Han, E. H.

    2017-01-01

    Natural ageing responses of duplex structured Mg-6%Li and Mg-6%Li-6%Zn-1.2%Y alloys have been investigated. Microstructural analyses revealed that the precipitation and coarsening process of α-Mg particles could occur in β-Li phases of both two alloys during ageing process. Since a certain amount of Mg atoms in β-Li phases were consumed for the precipitation of abundant tiny MgLiZn particles, the size of α-Mg precipitates in Mg-6%Li-6%Zn-1.2%Y alloy was relatively smaller than that in Mg-6%Li alloy. Micro hardness measurements demonstrated that with the ageing time increasing, the α-Mg phases in Mg-6%Li alloy could have a constant hardness value of 41 HV, but the contained β-Li phases exhibited a slight age-softening response. Compared with the Mg-6%Li alloy, the age-softening response of β-Li phases in Mg-6%Li-6%Zn-1.2%Y alloy was much more profound. Meanwhile, a normal age-hardening response of α-Mg phases was maintained. Tensile results indicated that obvious ageing-softening phenomenon in terms of macro tensile strength occurred in both two alloys. Failure analysis demonstrated that for the Mg-6%Li alloy, cracks were preferentially initiated at α-Mg/β-Li interfaces. For the Mg-6%Li-6%Zn-1.2%Y alloy, cracks occurred at both α-Mg/β-Li interfaces and slip bands in α-Mg and β-Li phases.

  7. Getting the Most Neutrinos out of IsoDAR

    CERN Document Server

    Ciuffoli, Emilio; Mohammed, Hosam; Zhao, Fengyi; Deliyergiyev, Maksym

    2016-01-01

    Several experimental collaborations worldwide intend to test sterile neutrino models by measuring the disappearance of antineutrinos produced via isotope decay at rest (IsoDAR). The most advanced of these proposals have very similar setups, in which a proton beam strikes a target yielding neutrons which are absorbed by a high isotopic purity 7Li converter, yielding 8Li whose resulting decay yields the antineutrinos. In this note, we use FLUKA and GEANT4 simulations to investigate three proposed modifications of this standard proposal. In the first, the 7Li is replaced with 7Li compounds including a deuterium moderator. In the second, a gap is placed between the target and the converter to reduce the neutron bounce-back. Finally, we consider cooling the converter with liquid nitrogen. We find that these modifications can increase the antineutrino yield by as much as 50 percent. The first also substantially reduces the quantity of high purity 7Li which is needed.

  8. Sympathetic cooling in an optically trapped mixture of alkali and spin-singlet atoms.

    Science.gov (United States)

    Ivanov, Vladyslav V; Khramov, Alexander; Hansen, Anders H; Dowd, William H; Münchow, Frank; Jamison, Alan O; Gupta, Subhadeep

    2011-04-15

    We report on the realization of a stable mixture of ultracold lithium and ytterbium atoms confined in a far-off-resonance optical dipole trap. We observe sympathetic cooling of 6Li by 174Yb and extract the s-wave scattering length magnitude |a(6Li-174Yb)|=(13±3)a0 from the rate of interspecies thermalization. Using forced evaporative cooling of 174Yb, we achieve reduction of the 6Li temperature to below the Fermi temperature, purely through interspecies sympathetic cooling.

  9. Using Inertial Fusion Implosions to Measure the T+^{3}He Fusion Cross Section at Nucleosynthesis-Relevant Energies.

    Science.gov (United States)

    Zylstra, A B; Herrmann, H W; Johnson, M Gatu; Kim, Y H; Frenje, J A; Hale, G; Li, C K; Rubery, M; Paris, M; Bacher, A; Brune, C R; Forrest, C; Glebov, V Yu; Janezic, R; McNabb, D; Nikroo, A; Pino, J; Sangster, T C; Séguin, F H; Seka, W; Sio, H; Stoeckl, C; Petrasso, R D

    2016-07-15

    Light nuclei were created during big-bang nucleosynthesis (BBN). Standard BBN theory, using rates inferred from accelerator-beam data, cannot explain high levels of ^{6}Li in low-metallicity stars. Using high-energy-density plasmas we measure the T(^{3}He,γ)^{6}Li reaction rate, a candidate for anomalously high ^{6}Li production; we find that the rate is too low to explain the observations, and different than values used in common BBN models. This is the first data directly relevant to BBN, and also the first use of laboratory plasmas, at comparable conditions to astrophysical systems, to address a problem in nuclear astrophysics.

  10. Using Inertial Fusion Implosions to Measure the T + 3He Fusion Cross Section at Nucleosynthesis-Relevant Energies

    Science.gov (United States)

    Zylstra, A. B.; Herrmann, H. W.; Johnson, M. Gatu; Kim, Y. H.; Frenje, J. A.; Hale, G.; Li, C. K.; Rubery, M.; Paris, M.; Bacher, A.; Brune, C. R.; Forrest, C.; Glebov, V. Yu.; Janezic, R.; McNabb, D.; Nikroo, A.; Pino, J.; Sangster, T. C.; Séguin, F. H.; Seka, W.; Sio, H.; Stoeckl, C.; Petrasso, R. D.

    2016-07-01

    Light nuclei were created during big-bang nucleosynthesis (BBN). Standard BBN theory, using rates inferred from accelerator-beam data, cannot explain high levels of 6Li in in low-metallicity stars. Using high-energy-density plasmas we measure the T (3He, ,γ )6Li reaction rate, a candidate for anomalously high 6Li production; we find that the rate is too low to explain the observations, and different than values used in common BBN models. This is the first data directly relevant to BBN, and also the first use of laboratory plasmas, at comparable conditions to astrophysical systems, to address a problem in nuclear astrophysics.

  11. The observation of charge exchange of pions captured in several nuclei

    Science.gov (United States)

    Bassalleck, B.; Corriveau, F.; Hasinoff, M. D.; Marks, T.; Measday, D. F.; Poutissou, J.-M.; Salomon, M.

    1981-06-01

    We have measured for the first time the branching ratios of the charge exchange of stopped negative pions in targets of 6Li, Al, Ti, Cu, Nb and Pb. These branching ratios are of the order of 10 -6, about an order of magnitude smaller than the upper limit previously established. Using the branching ratio for radiative pion capture in 6Li to the ground state of 6He we obtain the Panofsky ratio in 6Li, P6 = (8.7 ± 2.3) × 10 -4.

  12. Implanted $^{7}$Be targets for the study of neutron interactions with $^{7}$Be

    CERN Multimedia

    The disagreement of the predicted abundance of primordial $^{7}$Li with the observed abundance is a longstanding problem in Big Bang Nucleosynthesis (BBN) theory (“Primordial $^{7}$Li problem”). While BBN theory correctly predicts the relative abundances of $^{2}$H/$^{1}$H, $^{3}$He/$^{1}$H and $^{4}$He/$^{1}$H (that vary over four orders of magnitudes), but it over-predicts the relative abundance of primordial $^{7}$Li/$^{1}$H by a factor of approximately 3-4 larger than observed (approximately 4-5$\\sigma$ discrepancy). Primordial $^{7}$Li is destroyed during the first 15 minutes primarily via the $^{7}$Li(p,$\\alpha$) reaction. Hence most of the primordial $^7$Li is predicted as the result of the (later when atoms are formed) electron capture $\\beta$-decay of the primordial $^{7}$Be that is produced primarily in the $^{3}$He($\\alpha$,$\\gamma$) )$^{7}$Be reaction. We propose to investigate the direct destruction of $^{7}$Be during (the first 15 minutes of) BBN via the $^{7}$Be(n,$\\alpha$) reaction to ch...

  13. Abnormal lithium isotope composition from the ancient lithospheric mantle beneath the North China Craton.

    Science.gov (United States)

    Tang, Yan-Jie; Zhang, Hong-Fu; Deloule, Etienne; Su, Ben-Xun; Ying, Ji-Feng; Santosh, M; Xiao, Yan

    2014-03-04

    Lithium elemental and isotopic compositions of olivines in peridotite xenoliths from Hebi in the North China Craton provide direct evidence for the highly variable δ(7)Li in Archean lithospheric mantle. The δ(7)Li in the cores of olivines from the Hebi high-Mg# peridotites (Fo > 91) show extreme variation from -27 to +21, in marked deviation from the δ(7)Li range of fresh MORB (+1.6 to +5.6) although the Li abundances of the olivines are within the range of normal mantle (1-2 ppm). The Li abundances and δ(7)Li characteristics of the Hebi olivines could not have been produced by recent diffusive-driven isotopic fractionation of Li and therefore the δ(7)Li in the cores of these olivines record the isotopic signature of the subcontinental lithospheric mantle. Our data demonstrate that abnormal δ(7)Li may be preserved in the ancient lithospheric mantle as observed in our study from the central North China Craton, which suggest that the subcontinental lithospheric mantle has experienced modification of fluid/melt derived from recycled oceanic crust.

  14. Benchmarking ENDF/B-VII.0

    Science.gov (United States)

    van der Marck, Steven C.

    2006-12-01

    The new major release VII.0 of the ENDF/B nuclear data library has been tested extensively using benchmark calculations. These were based upon MCNP-4C3 continuous-energy Monte Carlo neutronics simulations, together with nuclear data processed using the code NJOY. Three types of benchmarks were used, viz., criticality safety benchmarks, (fusion) shielding benchmarks, and reference systems for which the effective delayed neutron fraction is reported. For criticality safety, more than 700 benchmarks from the International Handbook of Criticality Safety Benchmark Experiments were used. Benchmarks from all categories were used, ranging from low-enriched uranium, compound fuel, thermal spectrum ones (LEU-COMP-THERM), to mixed uranium-plutonium, metallic fuel, fast spectrum ones (MIX-MET-FAST). For fusion shielding many benchmarks were based on IAEA specifications for the Oktavian experiments (for Al, Co, Cr, Cu, LiF, Mn, Mo, Si, Ti, W, Zr), Fusion Neutronics Source in Japan (for Be, C, N, O, Fe, Pb), and Pulsed Sphere experiments at Lawrence Livermore National Laboratory (for 6Li, 7Li, Be, C, N, O, Mg, Al, Ti, Fe, Pb, D 2O, H 2O, concrete, polyethylene and teflon). For testing delayed neutron data more than thirty measurements in widely varying systems were used. Among these were measurements in the Tank Critical Assembly (TCA in Japan) and IPEN/MB-01 (Brazil), both with a thermal spectrum, and two cores in Masurca (France) and three cores in the Fast Critical Assembly (FCA, Japan), all with fast spectra. In criticality safety, many benchmarks were chosen from the category with a thermal spectrum, low-enriched uranium, compound fuel (LEU-COMP-THERM), because this is typical of most current-day reactors, and because these benchmarks were previously underpredicted by as much as 0.5% by most nuclear data libraries (such as ENDF/B-VI.8, JEFF-3.0). The calculated results presented here show that this underprediction is no longer there for ENDF/B-VII.0. The average over 257

  15. A Record of Oceanic Lithium Isotope Composition for the Last 7Ma

    Science.gov (United States)

    Marriott, C. S.; Henderson, G. M.

    2003-12-01

    Continental weathering plays an important role in global climate change but has proved difficult to reconstruct for the past. New geological tools with which to assess the past rate and style of weathering are therefore urgently required. One such tool is Li isotope fractionation. Recent studies [1,2] have shown preferential release of 7Li into the aqueous phase and retention/adsorption of 6Li during weathering processes such as partial dissolution and secondary mineral formation. Lithium behaves conservatively in the oceans, with a residence time of ˜1Ma, so that a history of ocean Li isotope composition provides information about the average rate and style of global continental weathering on long timescales. The incorporation of lithium as a trace element in marine carbonates enables the construction of a record of oceanic Li-isotopic variation and is the focus of this work. Carbonate Li-isotope compositions are lighter than seawater by ˜8 per mil, but this fractionation is not temperature dependent. This has been demonstrated by measurement of Li isotopes in inorganically precipitated calcites (5-30° C) [3], in coralline aragonite (25-30° C) [3] and in benthic foraminifera Uvigerina (7-23° C). This lack of T-dependent fractionation suggests that the variation in the isotope composition of planktonic foraminifera will solely reflect changes in oceanic Li isotope composition, which in turn is strongly influence by changes in continental weathering. ODP site 758, located on the Ninetyeast Ridge in the Indian Ocean (5° N, 90° E; 2925m), was sampled at 2m intervals, over a depth corresponding to the last 7Ma, to produce 55 samples with a temporal resolution of approximately 130Ka. Site 758 is previously well studied with an existing chronology and high resolution Sr, O and Nd isotope data. Individual foram species in the core top were first investigated to assess inter-species fractionation effects. Down core lithium isotope variation was examined by

  16. Detnex Project: Dispersion, Structure and Tracking of Exotic Nuclei

    Science.gov (United States)

    Alvarez, M. A. G.; Gómez-Camacho, J.; Espino, J. M.; Mukha, I.; Martel, I.

    2007-05-01

    Since 1970's when double-folding model, based on M3Y interaction, had to be renormalized to fit the elastic scattering of weakly bound 6,7Li and 9Be nuclei, we learned that preconceptions based on the highly successful experience of the optical model on stable nuclei could not be simply extrapolated to the scattering of exotic nuclei. Recently, we have shown some evidences of long range mechanisms in 6He induced reactions that lead to the loss of flux in the elastic channel at kinematic conditions that suggest the nuclei are well beyond the strong absorption radius [O. R. Kakuee, M. A. G. Alvarez, M. V. Andrés, S. Cherubini, T. Davinson, A. Di Pietro, W. Galster, J. Gómez-Camacho, A. M. Laird, M. Lamehi-Rachti, I. Martel, A. M. Moro, J. Rahighi, A. M. Sánchez-Benitez, A. C. Shotter, W. B. Smith, J. Vervier, P. J. Woods. Nucl. Phys. A 765, (2006) 294]. Even so, the use of nuclear reactions as an spectroscopic tool to investigate the nuclear structure of weakly bound nuclei requires a deep understanding of the reactions induced by these nuclei. Therefore, precise experimental measurements of the elastic scattering of exotic nuclei on a variety of targets, as well as the measurements of the main reaction channels are required in order to converge experimentally and theoretically to this understanding. With this aim a campaign of experiments involving different institutions and collaborations is being carefully established and going ahead at several radioactive ion beam (RIB) facilities: ISOLDE (CERN), CRC (Be), GSI (Ge) and TRIUMPH (Ca). The main idea is to measure the scattering of He, Li, and Be isotopes, and perform an intensive theoretical treatment, besides promoting some necessary instrumental development. In particular we participate in the low energy branch of the FAIR project where we take part in the tracking studies and developments.

  17. Detnex Project: Dispersion, Structure and Tracking of Exotic Nuclei

    Energy Technology Data Exchange (ETDEWEB)

    Alvarez, M.A.G. [Universidad de Sevilla, P.O. Box 1065, E-41080, Seville (Spain); Gomez-Camacho, J. [Universidad de Sevilla, P.O. Box 1065, E-41080, Seville (Spain); Espino, J.M. [Universidad de Sevilla, P.O. Box 1065, E-41080, Seville (Spain); Mukha, I. [Universidad de Sevilla, P.O. Box 1065, E-41080, Seville (Spain); Martel, I. [Universidad de Huelva, Departamento de Fisica Aplicada, E-21819 Huelva (Spain)

    2007-05-01

    Since 1970's when double-folding model, based on M3Y interaction, had to be renormalized to fit the elastic scattering of weakly bound {sup 6,7}Li and {sup 9}Be nuclei, we learned that preconceptions based on the highly successful experience of the optical model on stable nuclei could not be simply extrapolated to the scattering of exotic nuclei. Recently, we have shown some evidences of long range mechanisms in {sup 6}He induced reactions that lead to the loss of flux in the elastic channel at kinematic conditions that suggest the nuclei are well beyond the strong absorption radius [O. R. Kakuee, M. A. G. Alvarez, M. V. Andres, S. Cherubini, T. Davinson, A. Di Pietro, W. Galster, J. Gomez-Camacho, A. M. Laird, M. Lamehi-Rachti, I. Martel, A. M. Moro, J. Rahighi, A. M. Sanchez-Benitez, A. C. Shotter, W. B. Smith, J. Vervier, P. J. Woods. Nucl. Phys. A 765 (2006) 294]. Even so, the use of nuclear reactions as an spectroscopic tool to investigate the nuclear structure of weakly bound nuclei requires a deep understanding of the reactions induced by these nuclei. Therefore, precise experimental measurements of the elastic scattering of exotic nuclei on a variety of targets, as well as the measurements of the main reaction channels are required in order to converge experimentally and theoretically to this understanding. With this aim a campaign of experiments involving different institutions and collaborations is being carefully established and going ahead at several radioactive ion beam (RIB) facilities: ISOLDE (CERN), CRC (Be), GSI (Ge) and TRIUMPH (Ca). The main idea is to measure the scattering of He, Li, and Be isotopes, and perform an intensive theoretical treatment, besides promoting some necessary instrumental development. In particular we participate in the low energy branch of the FAIR project where we take part in the tracking studies and developments.

  18. Coulomb excitation of {sup 8}Li

    Energy Technology Data Exchange (ETDEWEB)

    Assuncao, Marlete; Britos, Tatiane Nassar [Universidade Federal de Sao Paulo (UNIFESP), SP (Brazil). Dept. de Ciencias Exatas e da Terra; Descouvemont, Pierre [Universite Libre de Bruxelles (ULB), Brussels (Belgium). Physique Nucleaire Theorique et Physique Mathematique; Lepine-Szily, Alinka; Lichtenthaler Filho, Rubens; Barioni, Adriana; Silva, Diego Medeiros da; Pereira, Dirceu; Mendes Junior, Djalma Rosa; Pires, Kelly Cristina Cezaretto; Gasques, Leandro Romero; Morais, Maria Carmen; Added, Nemitala; Neto Faria, Pedro; Rec, Rafael [Universidade de Sao Paulo (IF/USP), SP (Brazil). Inst. de Fisica. Dept. de Fisica Nuclear

    2012-07-01

    Full text: This work shows the Coulomb Excitation of {sup 8}Li on targets that have effectively behavior of Rutherford in angles and energies of interest for determining the value of the B(E2) electromagnetic transition. Theoretical aspects involved in this type of measure, known as COULEX [1], and some results in the literature [2-3] will be presented. Some problems with the targets and measurement system while performing an experiment on Coulomb Excitation of {sup 8}Li will be discussed: the energy resolution, background, possible contributions of the primary beam and also the excited states of the target near the region of elastic and inelastic peaks. They will be illustrated by measurements of the Coulomb Excitation of {sup 8}Li on targets of {sup 197}Au and {sup 208}Pb using the system RIBRAS(Brazilian Radioactive Ion Beam). In this case, the {sup 8}Li beam(T{sub 1/2} = 838 ms)is produced by {sup 9}Be({sup 7}Li;{sup 8} Li){sup 8}Be reaction from RIBRAS system which is installed at Instituto de Fisica of the Universidade de Sao Paulo. The primary {sup 7L}i beam is provided by Pelletron Accelerator. [1] K. Alder and A. Winther, Electromagnetic Excitation, North-Holland, New York, 1975; [2] P. Descouvemont and D. Baye, Phys. Letts. B 292, 235-238, 1992; [3] J. A. Brown, F. D. Becchetti, J. W. Jaenecke, K, Ashktorab, and D. A. Roberts, J. J. Kolata, R. J. Smith, and K. Lamkin, R. E. Warner, Phys. Rev. Letts., 66, 19, 1991; [4] R. J. Smith, J. J Kolata, K. Lamkin and A. Morsard, F. D. Becchetti, J. A. Brown, W. Z. Liu, J. W. Jaenecke, and D. A. Roberts, R. E. Warner, Phys. Rev. C, 43, 5, 1991. (author)

  19. PRELIMINARY CROSS SECTION AND NU-BAR COVARIANCES FOR WPEC SUBGROUP 26

    Energy Technology Data Exchange (ETDEWEB)

    ROCHMAN,D.

    2007-01-31

    We report preliminary cross section covariances developed for the WPEC Subgroup 26 for 45 out of 52 requested materials. The covariances were produced in 15- and 187-group representations as follows: (1) 36 isotopes ({sup 16}O, {sup 19}F, {sup 23}Na, {sup 27}Al, {sup 28}Si, {sup 52}Cr, {sup 56,56}Fe, {sup 58}Ni, {sup 90,91,92,94}Zr, {sup 166,167,168,170}Er, {sup 206,207,208}Pb, {sup 209}Bi, {sup 233,234,236}U, {sup 237}Np, {sup 238,240,241,242}Pu, {sup 241,242m,243}Am, {sup 242,243,244,245}Cm) were evaluated using the BNL-LANL methodology. For the thermal region and the resolved and unresolved resonance regions, the methodology has been based on the Atlas-Kalman approach, in the fast neutron region the Empire-Kalman method has been used; (2) 6 isotopes ({sup 155,156,157,158,160}Gd and {sup 232}Th) were taken from ENDF/B-VII.0; and (3) 3 isotopes ({sup 1}H, {sup 238}U and {sup 239}Pu) were taken from JENDL-3.3. For 6 light nuclei ({sup 4}He, {sup 6,7}Li, {sup 9}Be, {sup 10}B, {sup 12}C), only partial cross section covariance results were obtained, additional work is needed and they do not report the results here. Likewise, the cross section covariances for {sup 235}U, which they recommend to take from JENDL-3.3, will be included once the multigroup processing is successfully completed. Covariances for the average number of neutrons per fission, total {nu}-bar, are provided for 10 actinides identified as priority by SG26. Further work is needed to resolve some of the issues and to produce covariances for the full set of 52 materials.

  20. Precise atomic radiative lifetime via photoassociative spectroscopy of ultracold lithium

    NARCIS (Netherlands)

    McAlexander, W.I.; Abraham, E.R.I.; Ritchie, N.W.M.; Williams, C.J.; Stoof, H.T.C.; Hulet, R.G.

    1995-01-01

    We have obtained spectra of the high-lying vibrational levels of the 13Σg+ state of 6Li2 via photoassociation of ultracold 6Li atoms confined in a magneto-optical trap. The 13Σg+ state of the diatomic molecule correlates to a 2S1/2 state atom plus a 2P1/2 state atom. The long-range part of the molec

  1. Lithium isotope separation by laser

    Energy Technology Data Exchange (ETDEWEB)

    Arisawa, T.; Maruyama, Y.; Suzuki, Y.; Shiba, K.

    1982-01-01

    A lithium isotope separation was performed using a laser isotope separation method. It was found that the lithium atoms with a natural isotopic abundance enhanced its /sup 6/Li concentration up to over 90% by tuning the laser wavelength to the /sup 2/Psub(1/2) of /sup 6/Li. Too high power, however, leads to a loss of enrichment due to the power broadening effect which was analysed by the equation of motion of density matrices.

  2. GAMBE: multipurpose sandwich detector for neutrons and photons

    Science.gov (United States)

    Ahmed, A.; Burdin, S.; Casse, G.; van Zalinge, H.; Powel, S.; Rees, J.; Smith, A.; Tsurin, I.

    2016-10-01

    Detectors made with semiconductors such as silicon can be efficiently used for detecting and imaging neutrons when coated with suitable materials. They detect the charged reaction products resulting from the interaction of thermal neutrons with materials with high capture cross section like 10B, 6Li, and 6LiF. This work describes the performance of a thermal neutron detector system, GAMBE, which is based on silicon sensors and a layer of neutron-sensitive material, such as a lithium fluoride film or a lithium-6 foil, in a sandwich configuration. This arrangement has a total detection efficiency of 4 +/- 2 %, 7 +/- 1 %, and12 +/- 1 % for 7 μm 6LiF film, 40 μm and 70 μm 6Li foil respectively. Also, it enhances the rejection of fake hits using a simple coincidence method. The coincidence that defines a true neutron hit is the simultaneous signal recorded by the two sensors facing the conversion layer (or foil). These coincidences provide a very good method for rejecting the spurious hits coming from gamma-rays, which are usually present in the neutron field under measurement. The GAMBE system yields a rejection factor at the level of 108 allowing very pure neutron detection in high gamma background conditions. However, the price to pay is a reduction of the detection efficiency of 1 +/- 1 % or 0:9 +/- 0:3 % for 7 μm 6LiF film and 40 μm 6Li foil respectively.

  3. Transparent lithiated polymer films for thermal neutron detection

    Energy Technology Data Exchange (ETDEWEB)

    Mabe, Andrew N., E-mail: andrew.n.mabe@gmail.com [Department of Chemistry, University of Tennessee, Knoxville, TN 37996 (United States); Auxier, John D. [Department of Chemistry, University of Tennessee, Knoxville, TN 37996 (United States); Urffer, Matthew J. [Department of Nuclear Engineering, University of Tennessee, Knoxville, TN 37996 (United States); Penumadu, Dayakar [Department of Civil and Environmental Engineering, University of Tennessee, Knoxville, TN 37996 (United States); Schweitzer, George K. [Department of Chemistry, University of Tennessee, Knoxville, TN 37996 (United States); Miller, Laurence F. [Department of Nuclear Engineering, University of Tennessee, Knoxville, TN 37996 (United States)

    2013-09-11

    Novel water-soluble {sup 6}Li loaded copolymer scintillation films have been designed and fabricated to detect thermal neutrons. Styrene and maleic anhydride were copolymerized to form an alternating copolymer, then the anhydride functionality was hydrolyzed using {sup 6}Li hydroxide. The resulting poly(styrene-co-lithium maleate) was mixed with salicylic acid as a fluor and cast as a thin film from water. The maximum {sup 6}Li loading obtained that resulted in a transparent film was 4.36% by mass ({sup 6}Li to polymer). The optimum fluorescence output was obtained for 11.7% salicylic acid by mass, presumably in the form of lithium salicylate, resulting in an optimum film containing 3.85% by mass of {sup 6}Li. A facile and robust synthesis method, film fabrication protocol, photoluminescence results, and scintillation responses are reported herein. -- Highlights: • A transparent polymer scintillator containing 3.85 wt% {sup 6}Li has been synthesized. • This class of polymeric thermal neutron scintillation detector is water-soluble. • Salicylic acid, presumably in the form of lithium salicylate, is used as a fluor. • The material emits 373 photons/α ({sup 241}Am) and an average of 139 photons/β ({sup 36}Cl). • The material emits 360 photons per thermal neutron capture event.

  4. Sustainability of thorium-uranium in pebble-bed fluoride salt-cooled high temperature reactor

    Directory of Open Access Journals (Sweden)

    Zhu Guifeng

    2016-01-01

    Full Text Available Sustainability of thorium fuel in a Pebble-Bed Fluoride salt-cooled High temperature Reactor (PB-FHR is investigated to find the feasible region of high discharge burnup and negative Flibe (2LiF-BeF2 salt Temperature Reactivity Coefficient (TRC. Dispersion fuel or pellet fuel with SiC cladding and SiC matrix is used to replace the tristructural-isotropic (TRISO coated particle system for increasing fuel loading and decreasing excessive moderation. To analyze the neutronic characteristics, an equilibrium calculation method of thorium fuel self-sustainability is developed. We have compared two refueling schemes (mixing flow pattern and directional flow pattern and two kinds of reflector materials (SiC and graphite. This method found that the feasible region of breeding and negative Flibe TRC is between 20 vol% and 62 vol% fuel loading in the fuel. A discharge burnup could be achieved up to about 200 MWd/kgHM. The case with directional flow pattern and SiC reflector showed superior burnup characteristics but the worst radial power peak factor, while the case with mixing flow pattern and SiC reflector, which was the best tradeoff between discharge burnup and radial power peak factor, could provide burnup of 140 MWd/kgHM and about 1.4 radial power peak factor with 50 vol% dispersion fuel. In addition, Flibe salt displays good neutron properties as a coolant of quasi-fast reactors due to the strong 9Be(n,2n reaction and low neutron absorption of 6Li (even at 1000 ppm in fast spectrum. Preliminary thermal hydraulic calculation shows good safety margin. The greatest challenge of this reactor may be the decades irradiation time of the pebble fuel.

  5. Standard model contribution to the electric dipole moment of the deuteron, 3H, and 3He nuclei

    Science.gov (United States)

    Yamanaka, Nodoka; Hiyama, Emiko

    2016-02-01

    We calculate for the first time the electric dipole moment (EDM) of the deuteron, 3H, and 3He nuclei generated by the one-meson exchange CP-odd nuclear force in the standard model. The effective |Δ S| = 1 four-quark operators are matched to the |Δ S| = 1 standard model processes involving the CP phase of the Cabibbo-Kobayashi-Maskawa matrix at the electroweak scale and run down to the hadronic scale μ = 1 GeV according to the renormalization group evolution in the next-to-leading logarithmic order. At the hadronic scale, the hadron matrix elements are modeled in the factorization approach. We then obtain the one-meson (pion, eta meson, and kaon) exchange CP-odd nuclear force, which is the combination of the |Δ S| = 1 meson-baryon vertices which issue from the penguin operator and the hyperon-nucleon transition. From this CP-odd nuclear force, the nuclear EDM is calculated with the realistic Argonne v18 interaction and the CP-odd nuclear force using the Gaussian expansion method. It is found that the EDMs of light nuclear systems are of order O (10-31) e cm. We also estimate the standard model contribution to other hadronic CP violating observables such as the EDMs of 6Li, 9Be nuclei, and the atomic EDMs of 129Xe, 199Hg, 211Rn, and 225Ra generated through the nuclear Schiff moment. We then analyze the source of theoretical uncertainties and show some possible ways to overcome them.

  6. Effect of exotic long-lived sub-strongly interacting massive particles in big bang nucleosynthesis and a new solution to the Li problem

    Directory of Open Access Journals (Sweden)

    Kawasaki Masahiro

    2012-02-01

    Full Text Available The plateau of 7Li abundance as a function of the iron abundance by spectroscopic observations of metal-poor halo stars (MPHSs indicates its primordial origin. The observed abundance levels are about a factor of three smaller than the primordial 7Li abundance predicted in the standard Big Bang Nucleosynthesis (BBN model. This discrepancy might originate from exotic particle and nuclear processes operating in BBN epoch. Some particle models include heavy (m >> 1 GeV long-lived colored particles which would be confined inside exotic heavy hadrons, i.e., strongly interacting massive particles (SIMPs. We have found reactions which destroy 7Be and 7Li during BBN in the scenario of BBN catalyzed by a long-lived sub-strongly interacting massive particle (sub-SIMP, X. The reactions are non radiative X captures of 7 Be and 7Li which can be operative if the X particle interacts with nuclei strongly enough to drive 7 Be destruction but not strongly enough to form a bound state with 4 He of relative angular momentum L = 1. We suggest that 7Li problem can be solved as a result of a new process beyond the standard model through which the observable signature was left on the primordial Li abundance.

  7. Isotope compositions of dissolved lithium in the rivers Jinshajiang, Lancangjiang, and Nujiang: Implications for weathering in Qinghai-Tibet Plateau

    Energy Technology Data Exchange (ETDEWEB)

    Liu Congqiang, E-mail: liucongqiang@vip.skleg.cn [State Key Laboratory of Environmental Geochemistry, Institute of Geochemistry, Chinese Academy of Sciences, No. 46, Guanshui Rd., Guiyang 550002 (China); Zhao Zhiqi; Wang Qilian; Gao Bo [State Key Laboratory of Environmental Geochemistry, Institute of Geochemistry, Chinese Academy of Sciences, No. 46, Guanshui Rd., Guiyang 550002 (China)

    2011-06-15

    The Li isotope geochemistry of the Jinshajiang (upper reach of the Changjiang), Lancangjiang (Meckong) and the Nujiang (Salween) rivers have been studied to better understanding the weathering of continental crust. The three rivers show different water geochemistry, the Jinshajiang followed by the Lancangjiang contains much solute from dissolution of evaporites; the Jinshajiang has the highest average Li content and {delta}{sup 7}Li values. The relatively low {delta}{sup 7}Li values (+4.74{approx}+12.9 per mille) of the river waters, compared to those of large rivers in the world, probably reflect less weathering intensity in this arid and cold region. The Jinshajiang water has relatively high and constant {delta}{sup 7}Li values, and is considered to be affected by evaporite dissolution and the high {delta}{sup 7}Li values indicating that precipitation of salt minerals might have resulted in enrichment of {sup 7}Li in the remaining water. It is thought that H{sub 2}SO{sub 4} has been involved in crustal weathering in the region, especially in the Nujiang basin.

  8. Supernova Neutrino Nucleosynthesis of Light Elements with Neutrino Oscillations

    CERN Document Server

    Yoshida, T; Yokomakura, H; Kimura, K; Takamura, A; Hartmann, D H

    2006-01-01

    Light element synthesis in supernovae through neutrino-nucleus interactions, i.e., the nu-process, is affected by neutrino oscillations in the supernova environment. There is a resonance of 13-mixing in the O/C layer, which increases the rates of charged-current nu-process reactions in the outer He-rich layer. The yields of 7Li and 11B increase by about a factor of 1.9 and 1.3, respectively, for a normal mass hierarchy and an adiabatic 13-mixing resonance, compared to those without neutrino oscillations. In the case of an inverted mass hierarchy and a non-adiabatic 13-mixing resonance, the increase in the 7Li and 11B yields is much smaller. Observations of the 7Li/11B ratio in stars showing signs of supernova enrichment could thus provide a unique test of neutrino oscillations and constrain their parameters and the mass hierarchy.

  9. Photoassociation of ultracold LiRb* molecules: observation of high efficiency and unitarity-limited rate saturation

    CERN Document Server

    Dutta, Sourav; Altaf, Adeel; Elliott, D S; Chen, Yong P

    2013-01-01

    We report the production of ultracold heteronuclear 7Li85Rb molecules in excited electronic states by photoassociation (PA) of ultracold 7Li and 85Rb atoms. PA is performed in a dual-species 7Li-85Rb magneto-optical trap (MOT) and the PA resonances are detected using trap loss spectroscopy. We identify several strong PA resonances below the Li (2s 2S1/2) + Rb (5p 2P3/2) asymptote and experimentally determine the long range C6 dispersion coefficients. We find a molecule formation rate (P_LiRb) of 3.5x10^7 s^-1 and a PA rate coefficient (K_PA) of 1.3x10^-10 cm^3/s, the highest among heteronuclear bi-alkali molecules. At large PA laser intensity, we observe the saturation of the PA rate coefficient (K_PA) close to the theoretical value at the unitarity limit.

  10. Near threshold ⁷Li(p,n) ⁷Be reaction as neutron source for BNCT.

    Science.gov (United States)

    Minsky, D M; Kreiner, A J

    2015-12-01

    (7)Li(p,n)(7)Be is an endothermic reaction and working near its threshold (1.88 MeV) has the advantage of neutron spectra with maximum energies of about 100 keV, considerably lower than at higher beam energies, or than using other neutron-producing reactions or as for the uranium fission spectrum, relevant for BNCT based on nuclear reactors. With this primary energy it is much easier to obtain the energies needed for treating deep seated tumors by BNCT (about 10 keV). This work studies bombarding energies up to 2.05 MeV, different beam incidence angles and the effect of the undesirable gamma production via the (7)Li(p,γp') (7)Li reaction.

  11. Response of TL dosemeters to cosmic radiation on board passenger aircraft

    CERN Document Server

    Bilski, P; Marczewska, B; Olko, P

    2002-01-01

    Measurements were performed with various LiF based TLDs on board seven Polish aircraft, flying long-distance or middle-distance routes. All of the /sup 7/LiF detectors used (various types of /sup 7 /LiF:Mg, Ti and /sup 7/LiF:Mg, Cu, P detectors), which measure the non-neutron component of the radiation field, produced consistent results. It was found that the characteristics of the TLD response (ratio of different detector responses, glow curve shapes) after doses of radiation at flying altitudes differ from those obtained after exposure at the CERN facility (CERF), suggesting a lower contribution of densely ionising radiation. The neutron induced TL signal was also more affected by the thickness of the holder, suggesting the presence of a softer neutron energy spectrum at flight altitudes. Further in-flight and CERF exposures of detectors are planned to resolve these issues. (5 refs).

  12. Evolution of fusion hindrance for asymmetric systems at deep sub-barrier energies

    Science.gov (United States)

    Shrivastava, A.; Mahata, K.; Pandit, S. K.; Nanal, V.; Ichikawa, T.; Hagino, K.; Navin, A.; Palshetkar, C. S.; Parkar, V. V.; Ramachandran, K.; Rout, P. C.; Kumar, Abhinav; Chatterjee, A.; Kailas, S.

    2016-04-01

    Measurements of fusion cross-sections of 7Li and 12C with 198Pt at deep sub-barrier energies are reported to unravel the role of the entrance channel in the occurrence of fusion hindrance. The onset of fusion hindrance has been clearly observed in 12C +198Pt system but not in 7Li +198Pt system, within the measured energy range. Emergence of the hindrance, moving from lighter (6,7Li) to heavier (12C, 16O) projectiles is explained employing a model that considers a gradual transition from a sudden to adiabatic regime at low energies. The model calculation reveals a weak effect of the damping of coupling to collective motion for the present systems as compared to that obtained for systems with heavier projectiles.

  13. Evolution of fusion hindrance for asymmetric systems at deep sub barrier energies

    CERN Document Server

    Shrivastavaa, A; Pandit, S K; Nanal, V; Ichikawa, T; Hagino, K; Navin, A; Palshetkar, C S; Parkar, V V; Ramachandran, K; Rout, P C; Kumar, Abhinav; Chatterjee, A; Kailas, S

    2016-01-01

    Measurements of fusion cross-sections of 7Li and 12C with 198Pt at deep sub-barrier energies are reported to unravel the role of the entrance channel in the occurrence of fusion hindrance. The onset of fusion hindrance has been clearly observed in 12C + 198Pt system but not in 7Li + 198Pt system, within the measured energy range. Emergence of the hindrance, moving from lighter (6,7Li) to heavier (12C,16O) projectiles is explained employing a model that considers a gradual transition from a sudden to adiabatic regime at low energies. The model calculation reveals a weak effect of the damping of coupling to collective motion for the present systems as compared to that obtained for systems with heavier projectiles.

  14. Supernova neutrino nucleosynthesis of light elements with neutrino oscillations.

    Science.gov (United States)

    Yoshida, Takashi; Kajino, Toshitaka; Yokomakura, Hidekazu; Kimura, Keiichi; Takamura, Akira; Hartmann, Dieter H

    2006-03-10

    Light element synthesis in supernovae through neutrino-nucleus interactions, i.e., the v process, is affected by neutrino oscillations in the supernova environment. There is a resonance of 13-mixing in the O/C layer, which increases the rates of charged-current -process reactions in the outer He-rich layer. The yields of 7Li and 11B increase by about a factor of 1.9 and 1.3, respectively, for a normal mass hierarchy and an adiabatic 13-mixing resonance, compared to those without neutrino oscillations. In the case of an inverted mass hierarchy and a nonadiabatic 13-mixing resonance, the increase in the 7Li and 11B yields is much smaller. Observations of the 7Li/11B ratio in stars showing signs of supernova enrichment could thus provide a unique test of neutrino oscillations and constrain their parameters and the mass hierarchy.

  15. Transparent plastic scintillators for neutron detection based on lithium salicylate

    Energy Technology Data Exchange (ETDEWEB)

    Mabe, Andrew N., E-mail: mabe2@llnl.gov; Glenn, Andrew M.; Carman, M. Leslie; Zaitseva, Natalia P.; Payne, Stephen A.

    2016-01-11

    Transparent plastic scintillators with pulse shape discrimination containing {sup 6}Li salicylate have been synthesized by bulk polymerization with a maximum {sup 6}Li loading of 0.40 wt%. Photoluminescence and scintillation responses to gamma-rays and neutrons are reported herein. Plastics containing {sup 6}Li salicylate exhibit higher light yields and permit a higher loading of {sup 6}Li as compared to previously reported plastics based on lithium 3-phenylsalicylate. However, pulse shape discrimination performance is reduced in lithium salicylate plastics due to the requirement of adding more nonaromatic monomers to the polymer matrix as compared to those based on lithium 3-phenylsalicylate. Reduction in light yield and pulse shape discrimination performance in lithium-loaded plastics as compared to pulse shape discrimination plastics without lithium is interpreted in terms of energy transfer interference by the aromatic lithium salts. - Highlights: • Plastic scintillator with 0.4% {sup 6}Li loading is reported using lithium salicylate. • Influence of lithium salts on the scintillation mechanism is explored. • New lithium-loaded scintillator provides improved light yield and reduced cost.

  16. Light element evolution resulting from WMAP data

    CERN Document Server

    Romano, D; Matteucci, F; Chiappini, C; Romano, Donatella; Tosi, Monica; Matteucci, Francesca; Chiappini, Cristina

    2003-01-01

    The recent determination of the baryon-to-photon ratio from WMAP data by Spergel et al. (2003) allows one to fix with unprecedented precision the primordial abundances of the light elements D, 3He, 4He and 7Li in the framework of the standard model of big bang nucleosynthesis. We adopt these primordial abundances and discuss the implications for Galactic chemical evolution, stellar evolution and nucleosynthesis of the light elements. The model predictions on D, 3He and 4He are in excellent agreement with the available data, while a significant depletion of 7Li in low-metallicity stars is required to reproduce the Spite plateau.

  17. Gamma-decay study of sup 2 sup 1 Na and sup 2 sup 1 Ne, octupole bands in sup 2 sup 1 Ne

    CERN Document Server

    Thummerer, S; Kokalova, T; Bohlen, H G; Gebauer, B; Tumino, A; Massey, T N; Angelis, G D; Axiotis, M; Gadea, A; Kröll, T; Marginean, N; Napoli, D R; Poli, M; Ur, C; Bazzacco, D; Lenzi, S M; Alvarez, C R; Lunardi, S; Menegazzo, R; Bizzeti, P G; Bizzeti-Sona, A M

    2003-01-01

    The reactions sup 1 sup 6 O( sup 7 Li, 2n) and sup 1 sup 6 O( sup 7 Li, np) populating sup 2 sup 1 Na and sup 2 sup 1 Ne have been studied at E sub L = 27 MeV using the GASP gamma-detector array. The level scheme for sup 2 sup 1 Na and sup 2 sup 1 Ne has been extended to higher excitation energy. Spins and parities of the observed levels are assigned tentatively supporting the identification of opposite parity structures connected by strong dipole transitions. The structure of these bands is interpreted as based on a reflection asymmetric cluster structure.

  18. Experimental Study of High-spin States in ~(127)I~1

    Institute of Scientific and Technical Information of China (English)

    2001-01-01

    Study of in-bearn γ-ray spectroscopy o~(127)I has been carried out by using~(124)Sn(~7Li,4n)~(127)I reaction.The ~7Li beam was delivered by the Tandem Accelerator in the University of Tsukuba,Japan.The target was an enriched self-supporting~(124)Sn metallic foil of 4 mg/cm~2 thickness.A γ-ray detector array composed of one planar detector and 9 BGO-Compton-suppressed Ge detectors was used.Five Ge detectors were positioned at

  19. Radioactive proton capture on {sup 6}He

    Energy Technology Data Exchange (ETDEWEB)

    Sauvan, E.; Marques, F.M. [Caen Univ., 14 (France). Lab. de Physique Corpusculaire; Wilschut, H.W. [Kernfysich Versneller Instituut, Groningen (Netherlands)

    2001-03-01

    Radiative capture of protons is investigated as a probe of clustering in nuclei far from stability. The first such measurement on a halo nucleus is reported here for the reaction {sup 6}He(p,{gamma}) at 40 MeV. Capture into {sup 7}Li is observed as the strongest channel. In addition, events have been recorded that may be described by quasi-free capture on halo neutron, the {alpha} core and {sup 5}He. The possibility of describing such events by capture into the continuum of {sup 7}Li is also discussed. (authors)

  20. Pulse-shape analysis for gamma background rejection in thermal neutron radiation using CVD diamond detectors

    Energy Technology Data Exchange (ETDEWEB)

    Kavrigin, P., E-mail: pavel.kavrigin@cividec.at [Vienna University of Technology (Austria); Finocchiaro, P., E-mail: finocchiaro@lns.infn.it [INFN Laboratori Nazionali del Sud, via S.Sofia 62, 95123 Catania (Italy); Griesmayer, E., E-mail: erich.griesmayer@cividec.at [Vienna University of Technology (Austria); Jericha, E., E-mail: jericha@ati.ac.at [Vienna University of Technology (Austria); Pappalardo, A., E-mail: apappalardo@lns.infn.it [INFN Laboratori Nazionali del Sud, via S.Sofia 62, 95123 Catania (Italy); Weiss, C., E-mail: Christina.Weiss@cern.ch [Vienna University of Technology (Austria); European Organisation for Nuclear Research (CERN), Geneva (Switzerland)

    2015-09-21

    A novel technique for the rejection of gamma background from charged-particle spectra was demonstrated using a CVD diamond detector with a {sup 6}Li neutron converter installed at a thermal neutron beamline of the TRIGA research reactor at the Atominstitut (Vienna University of Technology). Spectra of the alpha particles and tritons of {sup 6}Li(n,T){sup 4}He thermal neutron capture reaction were separated from the gamma background by a new algorithm based on pulse-shape analysis. The thermal neutron capture in {sup 6}Li is already used for neutron flux monitoring, but the ability to remove gamma background allows using a CVD diamond detector for thermal neutron counting. The pulse-shape analysis can equally be applied to all cases where the charged products of an interaction are absorbed in the diamond and to other background particles that fully traverse the detector.