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Sample records for 46ti 64zn 114sn

  1. Evaluation of Excitation Function for 64Zn

    Institute of Scientific and Technical Information of China (English)

    2008-01-01

    <正>Present work concerns the evaluated neutron induced excitation function data for 64Zn, and mainly on (n, γ) reaction channel. The related experimental data were collected, analyzed and corrected for 64Zn

  2. Comparison between the exact and the thermal description of the pairing interaction in 114Sn

    International Nuclear Information System (INIS)

    The pairing interaction is solved exactly in the 114Sn nucleus using a realistic strength parameter as well as standard energy levels for the shell seniority zero states. The same single-particle and two-body Hamiltonian is treated with finite-temperature BCS and the thermal random-phase approximation. The results obtained through these calculations are compared to obtain insight about the suitability of the thermal approach to the description of nuclear phenomena

  3. Thermal quantities of 46Ti

    Science.gov (United States)

    Rahmatinejad, A.; Razavi, R.; Kakavand, T.

    2015-07-01

    Thermodynamic quantities of 46Ti have been calculated in the framework of the BCS model with inclusion of modified nuclear pairing gap (MPBCS) that was proposed in our previous publication. Using modified paring gap results in an S-shaped heat capacity curve at critical temperature with a smooth behavior instead of singular behavior of the same curve in the BCS calculations. In addition the thermal quantities have been extracted within the framework of a canonical ensemble according to the new experimental data on nuclear level densities measured by the Oslo group. Comparison shows a good agreement between our calculations in MPBCS and the extracted quantities in the canonical ensemble framework.

  4. Enhanced $0_{g.s.}^+ \\to 2_1^+$ E2 Transition Strength in $^{112,114}$Sn

    CERN Document Server

    Kumar, R; Jhingan, A; Muralithar, S; Mukherjee, S; Reiter, P; Gorska, M; Bhowmik, R K; Cederkall, J; Siwal, D; Doornenbal, P; Garg, R; Appannababu, S; Kojouharov, I; Grawe, H; Singh, P P; Mandal, S; Sharma, A; Schaffner, H; Ekstrom, A; Caceres, L; Prokopowicz, W; Kaur, J; Gerl, J; Singh, R P; Bednarczyk, P

    2011-01-01

    The poorly known B(E2; 0(+) -> 2(+)) values of (112)Sn and (114)Sn have been measured to high precision. Two Coulomb excitation experiments were performed to determine the reduced transition probabilities relative to (116)Sn in order to minimize the systematic errors. The obtained B(E2 up arrow) values of 0.242(8) e(2)b(2) for (112)Sn and 0.232(8) e(2)b(2) for (114)Sn confirm the tendency of large B(E2 up arrow) values for the lighter tin isotopes below the midshell (116)Sn that has been observed recently in various radioactive ion beam experiments.

  5. Effects of nuclear breakup channel on fusion of 6Li+64Zn system around barrier energies

    International Nuclear Information System (INIS)

    We have studied the effects of breakup, occurring due to the nuclear interaction between weakly bound 6Li and tightly bound 64Zn isotopes, on the fusion reaction at near barrier energies within the framework of dynamic polarization potential (DPP) approach. When the nuclear induced dynamic polarization potential is taken into account sub barrier enhancement and above barrier suppression have been found which improves the matching between the fusion excitation function data and predictions for 6Li+64Zn system significantly. (author)

  6. Thermal quantities of {sup 46}Ti

    Energy Technology Data Exchange (ETDEWEB)

    Rahmatinejad, A. [Department of Physics, Faculty of Science, University of Zanjan, Zanjan (Iran, Islamic Republic of); Razavi, R., E-mail: rrazavin@ihu.ac.ir [Physics Department, Faculty of Science, Imam Hossein Comprehensive University, Tehran (Iran, Islamic Republic of); Kakavand, T. [Department of Physics, Faculty of Science, Imam Khomeini International University, Qazvin (Iran, Islamic Republic of)

    2015-07-15

    Thermodynamic quantities of {sup 46}Ti have been calculated in the framework of the BCS model with inclusion of modified nuclear pairing gap (MPBCS) that was proposed in our previous publication. Using modified paring gap results in an S-shaped heat capacity curve at critical temperature with a smooth behavior instead of singular behavior of the same curve in the BCS calculations. In addition the thermal quantities have been extracted within the framework of a canonical ensemble according to the new experimental data on nuclear level densities measured by the Oslo group. Comparison shows a good agreement between our calculations in MPBCS and the extracted quantities in the canonical ensemble framework.

  7. Deformed shell model studies of spectroscopic properties of 64Zn and 64Ni and the positron double beta decay of 64Zn

    Indian Academy of Sciences (India)

    R Sahu; V K B Kota

    2014-04-01

    The spectroscopic properties of 64Zn and 64Ni are calculated within the framework of the deformed shell model (DSM) based on Hartree–Fock states. GXPF1A interaction in 1 $f_{7/2}$, 2$p_{3/2}$, 1$f_{5/2}$ and 2$p_{1/2}$ space with 40Ca as the core is employed. After ensuring that DSM gives good description of the spectroscopic properties of low-lying levels in these two nuclei considered, nuclear transition matrix elements (NTME) for the neutrinoless positron double beta decay (0 + and 0 +EC) of 64Zn are calculated. The two-neutrino positron double beta decay halflife is also calculated for this nucleus.

  8. Double folding model analysis of elastic scattering of halo nucleus 11Be from 64Zn

    Indian Academy of Sciences (India)

    M Hemalatha

    2014-05-01

    Calculations of elastic scattering cross-sections for 9,10,11Be+64Zn at near-Coulomb barrier energy have been performed using a potential obtained from the double folding model and are compared with the experiment. In the framework of the double folding model, the nuclear matter densities of 9,10,11Be projectiles and a 64Zn target are folded with the complex energydependent effective M3Y interaction. The angular distributions of the differential cross-section for 9,10Be scattering from 64Zn at $E_{c.m.} ≈$24.5 MeV agree remarkably well with the data, while in case of 11Be, calculations show a Coulomb–nuclear interference peak which is not observed in the data.

  9. Elastic scattering and fusion studies in the reactions $^{10,11}$Be + $^{64}$Zn

    CERN Multimedia

    2002-01-01

    We propose to measure elastic scattering and fusion excitation functions for the reactions $^{10,11}$Be + $^{64}$Zn at 3.1 MeV/u . The aim of the experiment is to investigate possible effects of the halo structure of the $^{11}$Be nucleus on the reaction mechanisms at energy around the Coulomb barrier. For this purpose a comparison with the reaction induced by the $^{10}$Be nucleus is required.

  10. Gamma-ray spectroscopy for investigation of the co-existence of deformed and spherical states in the magic nucleus of 114Sn

    International Nuclear Information System (INIS)

    The term diagram of the 50114Sn64 magic nucleus could be enlarged by 77 newly identified gamma transitions and 47 novel energy levels identified by way of a gamma-gamma coincidence measurement using the OSIRIS hexahedral spectrometer and by means of the high-spin reaction of 100Mo(18O,4n)114Sn at an injection energy of E(18O) = 70 MeV. Spins up to an excitation energy of ∝ 11.2 MeV and up to a maximum spin of 23 h have been occupied. For identification of the multipolarities of low-intensity γ-transitions which deplete the high-spin states, γγ-angular correlations have been evaluated, and 26 energy levels could be clearly assigned for the first time to measured spin values. For an interpretation of further nuclear structural states of 114Sn theoretical calculation have been made based on the shell model of nucleus. (orig./DG)

  11. Elastic scattering of the halo nucleus 11Be on 64Zn

    International Nuclear Information System (INIS)

    The elastic scattering cross-sections for the halo nucleus 11Be incident on 64Zn in the vicinity of Coulomb barrier are calculated using the microscopic double folding model. The parametrized densities taking into account for the halo part are folded with the effective nucleon-nucleon interaction (M3Y) to yield the microscopic double folded potential. The dynamic polarization potential (DPP) has been computed using the dipole strength distribution from the cluster model and from experiments. The calculated differential cross-section with the inclusion of the imaginary part of the dynamic polarization potential to the double folded potential shows a significant suppression of the differential cross-section in the Coulomb-nuclear interference region. This indicates that DPP effects due to B(E1) distribution are crucial in explaining the elastic scattering cross section of halo nuclei at incident energies in the vicinity of Coulomb barrier

  12. High spin levels in 62Zn, 64Zn, 66Zn, and 68Zn

    International Nuclear Information System (INIS)

    Investigation by in-beam gamma spectroscopy of high-spin states in the even zinc isotopes has been made using the Ni(α,2nγ)Zn reactions at Esub(α) approximately equal to 30MeV for 62Zn, 64Zn and 66Zn, and the 65Cu(α,pγ) reaction at Esub(α) approximately equal to 18MeV for 68Zn. The high-spin states feeding by varying the incident particles: p,3He,α,12C is discussed. It is pointed out that the gsub(9/2) orbital plays an important role in the structure of the high-spin states. The variation of the inertia momentum throughout the yrast line shows a backbending behavior and a shape transition associated to the occurence, for J>6, of rotational states is speculated

  13. Evidence for the Jacobi shape transition in hot 46Ti

    CERN Document Server

    Maj, A; Bracco, A; Camera, F; Bednarczyk, P; Herskind, B; Brambilla, S; Benzoni, G; Brekiesz, M; Curien, D; De Angelis, G F; Farnea, E; Grebosz, J; Kicinska-Habior, M; Leoni, S; Meczynski, W; Million, B; Napoli, D R; Nyberg, J; Petrache, C M; Styczen, J; Wieland, O; Zieblinski, M; Zuber, K; Dubray, N; Dudek, J; Pomorski, K

    2004-01-01

    The gamma-rays from the decay of the GDR in 46Ti compound nucleus formed in the 18O+28Si reaction at bombarding energy 105 MeV have been measured in an experiment using a setup consisting of the combined EUROBALL IV, HECTOR and EUCLIDES arrays. A comparison of the extracted GDR lineshape data with the predictions of the thermal shape fluctuation model shows evidence for the Jacobi shape transition in hot 46Ti. In addition to the previously found broad structure in the GDR lineshape region at 18-27 MeV caused by large deformations, the presence of a low energy component (around 10 MeV), due to the Coriolis splitting in prolate well deformed shape, has been identified for the first time.

  14. Cyclotron production of {sup 64}Cu by deuteron irradiation of {sup 64}Zn

    Energy Technology Data Exchange (ETDEWEB)

    Abbas, K. [Institute for Health and Consumer Protection, Joint Research Centre, European Commission, TP 500, I-21020 Ispra (Vatican City State, Holy See,) (Italy)]. E-mail: kamel.abbas@jrc.it; Kozempel, J. [Institute for Health and Consumer Protection, Joint Research Centre, European Commission, TP 500, I-21020 Ispra (VA) (Italy); Charles University Prague, Faculty of Science, Department of Organic and Nuclear Chemistry, 128 43 Prague (Czech Republic); Bonardi, M. [LASA, Radiochemistry Laboratory, University and INFN, via F.lli Cervi 201, I-20090 Segrate (MI) (Italy); Groppi, F. [LASA, Radiochemistry Laboratory, University and INFN, via F.lli Cervi 201, I-20090 Segrate (MI) (Italy); Alfarano, A. [Institute for Health and Consumer Protection, Joint Research Centre, European Commission, TP 500, I-21020 Ispra (VA) (Italy); Holzwarth, U. [Institute for Health and Consumer Protection, Joint Research Centre, European Commission, TP 500, I-21020 Ispra (VA) (Italy); Simonelli, F. [Institute for Health and Consumer Protection, Joint Research Centre, European Commission, TP 500, I-21020 Ispra (VA) (Italy); Hofman, H. [Institute for Health and Consumer Protection, Joint Research Centre, European Commission, TP 500, I-21020 Ispra (VA) (Italy); Horstmann, W. [Institute for Health and Consumer Protection, Joint Research Centre, European Commission, TP 500, I-21020 Ispra (VA) (Italy); Menapace, E. [ENEA, Applied Physics Division, Bologna (Italy); Leseticky, L. [Charles University Prague, Faculty of Science, Department of Organic and Nuclear Chemistry, 128 43 Prague (Czech Republic); Gibson, N. [Institute for Health and Consumer Protection, Joint Research Centre, European Commission, TP 500, I-21020 Ispra (VA) (Italy)

    2006-09-15

    The short-lived (12.7 h half-life) {sup 64}Cu radioisotope is both a {beta} {sup +} and a {beta} {sup -} emitter. This property makes {sup 64}Cu a promising candidate for novel medical applications, since it can be used simultaneously for therapeutic application of radiolabelled biomolecules and for diagnosis with PET. Following previous work on {sup 64}Cu production by deuteron irradiation of natural zinc, we report here the production of this radioisotope by deuteron irradiation of enriched {sup 64}Zn. In addition, yields of other radioisotopes such as {sup 61}Cu, {sup 67}Cu, {sup 65}Zn, {sup 69m}Zn, {sup 66}Ga and {sup 67}Ga, which were co-produced in this process, were also measured. The evaporation code ALICE-91 and the transport code SRIM 2003 were used to determine the excitation functions and the stopping power, respectively. All the nuclear reactions yielding the above-mentioned radioisotopes were taken into account in the calculations both for the natural and enriched Zn targets. The experimental and calculated yields were shown to be in reasonable agreement. The work was carried out at the Scanditronix MC-40 Cyclotron of the Institute for Health and Consumer Protection of the Joint Research Centre of the European Commission (Ispra site, Italy). The irradiations were carried out with 19.5 MeV deuterons, the maximum deuteron energy obtainable with the MC-40 cyclotron.

  15. Strong Deformation Effects in Hot Rotating 46Ti

    CERN Document Server

    Kmiecik, M; Brekiesz, M; Mazurek, K; Bednarczyk, P; Grebosz, J; Meczynski, W; Styczen, J; Zieblinski, M; Zuber, K; Papka, P; Beck, C; Curien, D; Haas, F; Rauch, V; Rousseau, M; Dudek, J; Schunck, N; Bracco, A; Camera, F; Benzoni, G; Wieland, O; Herskind, B; Farnea, E; De Angelis, G

    2007-01-01

    Exotic-deformation effects in 46Ti nucleus were investigated by analysing the high-energy gamma-ray and the alpha-particle energy spectra. One of the experiments was performed using the charged-particle multi-detector array ICARE together with a large volume (4"x4") BGO detector. The study focused on simultaneous measurement of light charged particles and gamma-rays in coincidence with the evaporation residues. The experimental data show a signature of very large deformations of the compound nucleus in the Jacobi transition region at the highest spins. These results are compared to data from previous experiments performed with the HECTOR array coupled to the EUROBALL array, where it was found that the GDR strength function is highly fragmented, strongly indicating a presence of nuclei with very large deformation.

  16. Coupled-channel analysis for 20.4 MeV energy of p-^{64}Zn inelastic scattering

    Indian Academy of Sciences (India)

    Harun Yücel; Müşfik Taşan

    2012-02-01

    In this study, a coupled-channel (CC) analysis of the elastic and the inelastic scattering of 20.4 MeV polarized protons from a 64Zn target leading to the deformed 2+, $3^−$, $2^+_2$ states was performed. The CC potential parameters and the deformation parameters of the excited states corresponding to the best fit to the experimental differential cross-sections and the analysing powers data were determined. For $2^+_2$ excited state, a mixed type was used and a good fit to the data was provided. The CC calculation results were compared to the pure distorted wave Born approximation (DWBA) calculation results which were calculated using the new parameters. All calculations were conducted using the computer code ECIS06.

  17. Comparison of the effects of couplings to breakup channels in reactions induced by {sup 6}Li and {sup 6}He on the same {sup 64}Zn target

    Energy Technology Data Exchange (ETDEWEB)

    Fernández-García, J. P., E-mail: fernandez@lns.infn.it; Di Pietro, A.; Figuera, P.; Fisichella, M. [INFN, Laboratori Nazionali del Sud, via S. Sofia 62, 1-95123 Catania (Italy); Lattuada, M.; Musumarra, A.; Pellegriti, M. G.; Scuderi, V.; Torresi, D. [INFN, Laboratori Nazionali del Sud, via S. Sofia 62, 1-95123 Catania (Italy); Dipartamento di Fisica e Astronomia, via S. Sofia 64, I-95123 Catania (Italy); Moro, A. M. [Departamento de FAMN, Universidad de Sevilla, Apartado 1065, E-41080 Seville (Spain); Zadro, M. [Ruder Bošković Institute, Bijenička cesta 54, HR-10000 Zagreb (Croatia)

    2015-10-15

    The experimental elastic scattering angular distributions for the weakly bound nuclei {sup 6,7}Li and for the halo nucleus {sup 6}He on the same {sup 64}Zn target at several energies around the Coulomb barrier were measured at the Laboratori Nazionali del Sud (LNS, Italy) and at the Cyclotron Research Center, Louvain La Neuve (Belgium), respectively. The measured elastic scattering angular distributions of these three systems at the same center of mass energy have been compared. The experimental data of the {sup 6,7}Li+ {sup 64}Zn systems have been analyzed within the CDCC method, while the {sup 6}He+{sup 64}Zn data have been compared with both both CDCC and CRC calculations.

  18. MICROSTRUCTURE OF Mg-6.4Zn-1.1Y ALLOY FABRICATED BY RAPID SOLIDIFICATION AND RECIPROCATING EXTRUSION

    Institute of Scientific and Technical Information of China (English)

    Z.M. Zhang; C.J. Xu; X.F. Guo

    2008-01-01

    In order to explore the methods to prepare high-strength quasicrystal-reinforced magnesium alloys, the flakes of rapidly solidified Mg-6.4Zn-1.1 Y magnesium alloy with a thickness of 50-60 um were obtained by a melt spinning single-roller device, and the flakes were then processed into rods by reciprocating extrusion and direct extrusion. The microstructure of the alloy was analyzed by optical microscope and SEM, and the constituent phases were identified by XRD. Phase transformation and its onset temperature were determined by differential thermal analyzer (DTA). The analysis result shows that rapid solidification for Mg-6.4Zn-1.1Y alloy can inhibit the eutectic reactions, broaden the solid solubility of Zn in a-Mg solute solution, and impede the formation of Mg3 Y2 Zn3 and MgZn2 compounds, and thus help the icosahedral Mg3 YZn6 quasicrystal formed directly from the melt. The mierostrueture of the flakes consists of the a-Mg solid solution and icosahedral Mg3 YZn6 quasierystal. Dense rods can be made from the flakes by two-pass reciprocating extrusion and direct extrusion. The interfaces between flakes in the rods can be welded and jointed perfectly. During the reciprocating extrusion and direct extrusion process, more Mg3 YZn6 compounds are precipitated and distributed uniformly, whereas the rods possess fine microstructures inherited from rapidly solidified flakes. The rods contain only two phases: amagnesium solid solution as matrix and fine icosahedral Mg3 YZn6 quasicrystal which disperses uniformly in the matrix.

  19. Search for 2{beta} processes in {sup 64}Zn with the help of ZnWO{sub 4} crystal scintillator

    Energy Technology Data Exchange (ETDEWEB)

    Belli, P. [Dipartimento di Fisica, Universita di Roma ' Tor Vergata' and INFN, Sezione di Roma Tor Vergata, I-00133 Rome (Italy); Bernabei, R. [Dipartimento di Fisica, Universita di Roma ' Tor Vergata' and INFN, Sezione di Roma Tor Vergata, I-00133 Rome (Italy)], E-mail: rita.bernabei@roma2.infn.it; Cappella, F. [Dipartimento di Fisica, Universita di Roma ' La Sapienza' and INFN, Sezione di Roma, I-00185 Rome (Italy); Cerulli, R. [INFN, Laboratori Nazionali del Gran Sasso, 67010 Assergi (AQ) (Italy); Dai, C.J. [IHEP, Chinese Academy, P.O. Box 918/3, Beijing 100039 (China); Danevich, F.A. [Institute for Nuclear Research, MSP 03680 Kyiv (Ukraine); Grinyov, B.V. [Institute for Scintillation Materials, 61001 Kharkiv (Ukraine); Incicchitti, A. [Dipartimento di Fisica, Universita di Roma ' La Sapienza' and INFN, Sezione di Roma, I-00185 Rome (Italy); Kobychev, V.V. [Institute for Nuclear Research, MSP 03680 Kyiv (Ukraine); Nagornaya, L.L. [Institute for Scintillation Materials, 61001 Kharkiv (Ukraine); Nagorny, S.S. [Institute for Nuclear Research, MSP 03680 Kyiv (Ukraine); Nozzoli, F. [Dipartimento di Fisica, Universita di Roma ' Tor Vergata' and INFN, Sezione di Roma Tor Vergata, I-00133 Rome (Italy); Poda, D.V. [Institute for Nuclear Research, MSP 03680 Kyiv (Ukraine); Prosperi, D. [Dipartimento di Fisica, Universita di Roma ' La Sapienza' and INFN, Sezione di Roma, I-00185 Rome (Italy); Tretyak, V.I.; Yurchenko, S.S. [Institute for Nuclear Research, MSP 03680 Kyiv (Ukraine)

    2008-01-10

    Double beta processes in {sup 64}Zn were searched for with the help of a low background ZnWO{sub 4} crystal scintillator (mass of 117 g) at the Gran Sasso National Laboratories of the INFN. Total time of measurements was 1902 h. New improved half-life limits on different modes of double electron capture and electron capture with positron emission were established as: T{sub 1/2}{sup 2{nu}}{sup 2K}{>=}6.2x10{sup 18} yr, T{sub 1/2}{sup 0{nu}}{sup 2K}{>=}4.0x10{sup 18} yr, T{sub 1/2}{sup 0{nu}}{sup 2{epsilon}}{>=}3.4x10{sup 18} yr, T{sub 1/2}{sup 2{nu}}{sup {epsilon}}{sup {beta}{sup +}}{>=}2.1x10{sup 20} yr, and T{sub 1/2}{sup 0{nu}}{sup {epsilon}}{sup {beta}{sup +}}{>=}2.2x10{sup 20} yr, all at 90% C.L.

  20. SIMS depth profiling of rubber-tyre cord bonding layers prepared using 64Zn depleted ZnO

    International Nuclear Information System (INIS)

    Zinc oxide and copper/zinc sulphide layers are formed during vulcanisation and moulding of rubber to brass-coated steel tyre reinforcing cords. Previous studies have described how zinc diffuses through the rubber-brass interface to form zinc sulphide, and combines with oxygen to create zinc oxide during dezincification. The zinc is usually assumed to originate in the brass of the tyre cord, however, zinc oxide is also present in the rubber formulation. We reveal how zinc from these sources is distributed within the interfacial bonding layers, before and after heat and humidity ageing. Zinc oxide produced using 64Zn-isotope depleted zinc was mixed in the rubber formulation in place of the natural ZnO and the zinc isotope ratios within the interfacial layers were followed by secondary ion mass spectroscopy (SIMS) depth profiling. Variations in the relative ratios of the zinc isotopes during depth profiling were measured for unaged, heat-aged and humidity-aged wire samples and in each case a relatively large proportion of the zinc incorporated into the interfacial layer as zinc sulphide was shown to have originated from ZnO in the rubber compound

  1. Search for the Jacobi Instability in Rapidly Rotating 46Ti* Nuclei

    CERN Document Server

    Maj, A; Krolas, W; Styczen, J; Bracco, A; Camera, F; Million, B; Gaardhøje, J J; Herskind, B; Kicinska-Habior, M; Kownacki, J P; Ormand, W E

    2001-01-01

    The possible existence of Jacobi shape transition in hot 46Ti at high angular momenta was investigated with the Giant Dipole Resonance exclusive experiments. The GDR spectra and the angular distributions are consistent with predictions of the thermal shape fluctuation model indicating elongated nuclear shapes.

  2. Disappearance of flow and the in-medium nucleon-nucleon cross section for {sup 64}Zn+{sup 27}Al collisions at intermediate energies

    Energy Technology Data Exchange (ETDEWEB)

    Zhi-Yong He [Caen Univ., 14 (France). Lab. de Physique Corpusculaire]|[Academia Sinica, Lanzhou, GS (China). Inst. of Modern Physics; Peter, J.; Angelique, J.C.; Bizard, G.; Brou, R.; Cussol, D. [Caen Univ., 14 (France). Lab. de Physique Corpusculaire; Auger, A.; Cabot, C.; Crema, E. [Grand Accelerateur National d`Ions Lourds (GANIL), 14 - Caen (France); Buta, A. [Caen Univ., 14 (France). Lab. de Physique Corpusculaire]|[Institute of Atomic Physics, Bucharest (Romania)] [and others

    1996-09-01

    Experimental measurement and theoretical comparison of collective flow can give important information about the nuclear equation of state (EOS) and the in-medium nucleon-nucleon cross section. Experimental measurements of {sup 64}Zn+{sup 27}Al collision from 35 to 79 MeV/u with the 4{pi} array MUR=TONNEAU are presented. The results are compared to BUU calculations. (K.A.).

  3. Measurement of the thermal cross section of the reaction 64Zn(n,γ)65Zn in a mixed neutron flux

    International Nuclear Information System (INIS)

    Zinc is an element that is present in a great variety of biological and geological samples.For its determination by Instrumental Neutron Activation Analysis, the reaction 64Zn(n,γ)65Zn is used, due to the long half life of the reaction product, the target's bigger isotopic abundance, and an easily measurable 1115 keV main gamma line.In a recent evaluation of thermal cross sections and resonance integrals, a thermal cross section value that is 44.7% bigger than the previous evaluation has been published by the same reference.This difference is not within reported uncertainties.Besides, the relative uncertainty of the new evaluation is much bigger than the one corresponding to the previous evaluation.The adoption of the thermal cross section corresponding to different evaluations may imply, in the case of an irradiation in the peripheral I 6 position at the R A-6 reactor, discrepancies of about 43% in the calculated concentrations.These inconsistencies were evident during the irradiation of certified standard materials.This motivated the measurement of the thermal cross section for the reaction 64Zn(n,γ)65Zn in the I 6 position at the R A-6 reactor.For the analysis of results, a code was written in order to calculate correction factors from an accurate characterization of the neutron spectrum.The thermal cross section value of the reaction 64Zn(n,γ)65Zn measured is (0.76± 0.03) b

  4. Measurements of the 64Zn(n,a)61Ni cross section at En=5.0-6.75 MeV

    OpenAIRE

    Gledenov, Yu. M.; Sedysheva, M. V.; Sedyshev, P. V.; Oprea, A.; Chen, Z.; Chen, Y; Yuan, J.; Zhang, G.; Tang, G.; Khuukhenkhuu, G.; Szalanski, P.

    2002-01-01

    The experiment of determination of the 64Zn(n,a)61Ni reaction cross section in the 5.0-6.75 MeV neutron energy range was performed at the 4.5 MV Van de Graaf accelerator at the Institute of Heavy Ion Physics, Peking University, Beijing. Double section ionization chamber with grid was used for direct registration of the reaction products. The cross sections and angular distributions were extracted from the experimental data. The obtained values were compared with the results of other authors a...

  5. Study of Deformation Effects in the Charged Particle Emission from 46Ti*

    Science.gov (United States)

    Brekiesz, M.; Papka, P.; Maj, A.; Kmiecik, M.; Beck, C.; Bednarczyk, P.; Grebosz, J.; Haas, F.; Meczynski, W.; Rauch, V.; Rousseau, M.; Zafra, A. Sanchez I.; Styczen, J.; Thummerer, S.; Zieblinski, M.; Zuber, K.

    2005-04-01

    The 46Ti* compound nucleus, as populated by the fusion--evaporation reaction 27Al + 19F at the bombarding energy of 144MeV, has been investigated by charged particle spectroscopy using the multidetector array ICARE at the VIVITRON tandem facility of the IReS (Strasbourg). The light charged particles have been measured in coincidence with evaporation residues. The CACARIZO} code, a Monte Carlo implementation of the statistical model code CASCADE, has been used to calculate the spectral shapes of evaporated α -particles which are compared with the experimental spectra. This comparison indicates the possible signature of large deformations of the compound nucleus.

  6. Study of Deformation Effects in the Charged Particle Emission from 46Ti

    CERN Document Server

    Brekiesz, M; Maj, A; Kmiecik, M; Beck, C; Bednarczyk, P; Grebosz, J; Haas, F; Meczynski, W; Rauch, V; Rousseau, M; Zafra, A S; Styczen, J; Thummerer, S; Zieblinski, M; Zuber, K

    2004-01-01

    The 46Ti compound nucleus, as populated by the fusion-evaporation reaction 27Al + 19F at the bombarding energy of 144 MeV, has been investigated by charged particle spectroscopy using the multidetector array ICARE at the VIVITRON tandem facility of the IReS (Strasbourg). The light charged particles have been measured in coincidence with evaporation residues. The CACARIZO code, a Monte Carlo implementation of the statistical-model code CASCADE, has been used to calculate the spectral shapes of evaporated alpha-particles which are compared with the experimental spectra. This comparison indicates the possible signature of large deformations of the compound nucleus.

  7. A Comprehensive Theoretical Analysis of 6,7Li + 64Zn Elastic Scattering in a Wide Angular Range Around the Coulomb Barrier

    Science.gov (United States)

    Ibraheem, Awad A.; Aygun, M.

    2016-08-01

    In this paper, the elastic scattering angular distributions of 6,7Li on 64Zn have been investigated by using various nuclear potentials. For this, we use the phenomenological Woods-Saxon potential, the real double folding potential with the density-independent M3Y effective interaction supplemented with an imaginary part in Woods-Saxon form and the double folding potentials multiplied with a normalization factor of the real and imaginary parts via the density-independent and CDM3Y6 density-dependent versions of the M3Y effective interaction have been used. The results have been compared with each other as well as with the experimental data. It has been observed that the agreement between the theoretical results and earlier reported data is perfect. Finally, the change of the total reaction cross sections with energy has been investigated.

  8. Reconstructed primary fragments and symmetry energy, temperature and density of the fragmenting source in $^{64}$Zn + $^{112}$Sn at 40 MeV/nucleon

    CERN Document Server

    Liu, X; Wada, R; Huang, M; Zhang, S; Ren, P; Chen, Z; Wang, J; Xiao, G Q; Han, R; Liu, J; Shi, F; Rodrigues, M R D; Kowalski, S; Keutgen, T; Hagel, K; Barbui, M; Zheng, H; Bonasera, A; Natowitz, J B

    2014-01-01

    Symmetry energy, temperature and density at the time of the intermediate mass fragment formation are determined in a self-consistent manner, using the experimentally reconstructed primary hot isotope yields and anti-symmetrized molecular dynamics (AMD) simulations. The yields of primary hot fragments are experimentally reconstructed for multifragmentation events in the reaction system $^{64}$Zn + $^{112}$Sn at 40 MeV/nucleon. Using the reconstructed hot isotope yields and an improved method, based on the modified Fisher model, symmetry energy values relative to the apparent temperature, $a_{sym}/T$, are extracted. The extracted values are compared with those of the AMD simulations, extracted in the same way as that for the experiment, with the Gogny interaction with three different density-dependent symmetry energy terms. $a_{sym}/T$ values change according to the density-dependent symmetry energy terms used. Using this relation, the density of the fragmenting system is extracted first. Then symmetry energy a...

  9. A Comprehensive Theoretical Analysis of 6,7Li + 64Zn Elastic Scattering in a Wide Angular Range Around the Coulomb Barrier

    Science.gov (United States)

    Ibraheem, Awad A.; Aygun, M.

    2016-06-01

    In this paper, the elastic scattering angular distributions of 6,7Li on 64Zn have been investigated by using various nuclear potentials. For this, we use the phenomenological Woods-Saxon potential, the real double folding potential with the density-independent M3Y effective interaction supplemented with an imaginary part in Woods-Saxon form and the double folding potentials multiplied with a normalization factor of the real and imaginary parts via the density-independent and CDM3Y6 density-dependent versions of the M3Y effective interaction have been used. The results have been compared with each other as well as with the experimental data. It has been observed that the agreement between the theoretical results and earlier reported data is perfect. Finally, the change of the total reaction cross sections with energy has been investigated.

  10. Direct study of the alpha-nucleus optical potential at astrophysical energies using the 64Zn(p,alpha)61Cu reaction

    CERN Document Server

    Gyürky, Gy; Halász, Z; Kiss, G G; Szücs, T

    2014-01-01

    In the model calculations of heavy element nucleosynthesis processes the nuclear reaction rates are taken from statistical model calculations which utilize various nuclear input parameters. It is found that in the case of reactions involving alpha particles the calculations bear a high uncertainty owing to the largely unknown low energy alpha-nucleus optical potential. Experiments are typically restricted to higher energies and therefore no direct astrophysical consequences can be drawn. In the present work a (p,alpha) reaction is used for the first time to study the alpha-nucleus optical potential. The measured 64Zn(p,alpha)61Cu cross section is uniquely sensitive to the alpha-nucleus potential and the measurement covers the whole astrophysically relevant energy range. By the comparison to model calculations, direct evidence is provided for the incorrectness of global optical potentials used in astrophysical models.

  11. Evidence for the Jacobi shape transition in hot {sup 46}Ti

    Energy Technology Data Exchange (ETDEWEB)

    Maj, A.; Kmiecik, M.; Bracco, A.; Camera, F.; Bednarczyk, P.; Herskind, B.; Brambilla, S.; Benzoni, G.; Brekiesz, M.; Curien, D.; De Angelis, G.; Farnea, E.; Grebosz, J.; Kicinska-Habior, M.; Leoni, S.; Meczynski, W.; Million, B.; Napoli, D.R.; Nyberg, J.; Petrache, C.M.; Styczen, J.; Wieland, O.; Zieblinski, M.; Zuber, K.; Dubray, N.; Dudek, J.; Pomorski, K

    2004-02-09

    The {gamma}-ras from the decay of the GDR in the compound nucleus reaction {sup 18}O+{sup 28}Si at bombarding energy of 105 MeV have been measured in an experiment using a setup consisting of the combined EUROBALL IV, HECTOR and EUCLIDES arrays. The shape of the rotating compound nucleus, {sup 46}Ti, is expected to undergo the Jacobi transition around spin 28 {Dirac_h}. A comparison of the GDR lineshape data with the predictions of the thermal shape fluctuation model, based on the most recent rotating liquid drop LSD calculations, shows evidence for such Jacobi shape transition. In addition to the previously found broad structure in the GDR lineshape region at 18-25 MeV caused by large deformations, the presence of a low energy component (around 10 MeV), due to the Coriolis splitting in prolate, well deformed shape has been identified for the first time.

  12. Deformation Effects in Hot Rotating 46Ti Probed by the Charged Particle Emission and GDR γ-Decay

    Science.gov (United States)

    Brekiesz, M.; Maj, A.; Kmiecik, M.; Mazurek, K.; Mȩczyński, W.; Styczeń, J.; Zuber, K.; Papka, P.; Beck, C.; Haas, F.; Rauch, V.; Rousseau, M.; Sànchez i Zafra, A.; Dudek, J.; Schunck, N.

    2007-05-01

    The 46Ti * compound nucleus, as populated by the fusion-evaporation reaction 27Al + 19F at the bombarding energy of Elab = 144 MeV, has been investigated by charged particle spectroscopy using the multidetector array ICARE at the VIVITRON tandem facility of the IReS (Strasbourg). The light charged particles and high-energy γ-rays from the GDR decay have been measured in coincidence with selected evaporation residues. The CACARIZO code, a Monte Carlo implementation of the statistical-model code CASCADE, has been used to calculate the spectral shapes of evaporated α-particles which are compared with the experimental coincident spectra. This comparison indicates the signature of large deformations (possibly superdeformed and hyperdeformed shapes) present in the compound nucleus decay. The occurrence of the Jacobi shape transition is also discussed in the framework of a newly developed rotating liquid drop model.

  13. Deformation Effects in Hot Rotating $^{46}Ti$ Probed by the Charged Particle Emission and GDR $\\gamma-Decay$

    CERN Document Server

    Brekiesz, M; Kmiecik, M; Mazurek, K; Meczynski, W; Styczen, J; Zuber, K; Papka, P; Beck, C; Haas, F; Rauch, V; Rousseau, M; Zafra, A S; Dudek, J; Schunck, N

    2007-01-01

    The 46Ti* compound nucleus, as populated by the fusion-evaporation reaction 27Al+19F at the bombarding energy of E_lab=144 MeV, has been investigated by charged particle spectroscopy using the multidetector array ICARE at the VIVITRON tandem facility of the IReS (Strasbourg). The light charged particles and high-energy gamma-rays from the GDR decay have been measured in coincidence with selected evaporation residues. The CACARIZO code, a Monte Carlo implementation of the statistical-model code CASCADE, has been used to calculate the spectral shapes of evaporated alpha-particles which are compared with the experimental coincident spectra. This comparison indicates the signature of large deformations (possibly superdeformed and hyperdeformed shapes) present in the compound nucleus decay. The occurrence of the Jacobi shape transition is also discussed in the framework of a newly developed rotating liquid drop model.

  14. Deformation Effects in Hot Rotating {sup 46}Ti Probed by the Charged Particle Emission and GDR {gamma}-Decay

    Energy Technology Data Exchange (ETDEWEB)

    Brekiesz, M. [H. Niewodniczanski Institute of Nuclear Physics, PAN, 31-342 Cracow (Poland); Maj, A. [H. Niewodniczanski Institute of Nuclear Physics, PAN, 31-342 Cracow (Poland); Kmiecik, M. [H. Niewodniczanski Institute of Nuclear Physics, PAN, 31-342 Cracow (Poland); Mazurek, K. [H. Niewodniczanski Institute of Nuclear Physics, PAN, 31-342 Cracow (Poland); Meczynski, W. [H. Niewodniczanski Institute of Nuclear Physics, PAN, 31-342 Cracow (Poland); Styczen, J. [H. Niewodniczanski Institute of Nuclear Physics, PAN, 31-342 Cracow (Poland); Zuber, K. [H. Niewodniczanski Institute of Nuclear Physics, PAN, 31-342 Cracow (Poland); Papka, P. [IPHC and ULP (Strasbourg I), B.P. 28 F-67037 Strasbourg Cedex 2 (France); iThemba LABS, 7129 Somerset West (South Africa); Beck, C. [IPHC and ULP (Strasbourg I), B.P. 28 F-67037 Strasbourg Cedex 2 (France); Haas, F. [IPHC and ULP (Strasbourg I), B.P. 28 F-67037 Strasbourg Cedex 2 (France); Rauch, V. [IPHC and ULP (Strasbourg I), B.P. 28 F-67037 Strasbourg Cedex 2 (France); Rousseau, M. [IPHC and ULP (Strasbourg I), B.P. 28 F-67037 Strasbourg Cedex 2 (France); Sanchez i Zafra, A. [IPHC and ULP (Strasbourg I), B.P. 28 F-67037 Strasbourg Cedex 2 (France); Dudek, J. [IPHC and ULP (Strasbourg I), B.P. 28 F-67037 Strasbourg Cedex 2 (France); Schunck, N. [H. Niewodniczanski Institute of Nuclear Physics, PAN, 31-342 Cracow (Poland); Departamento de Fisica Teorica, Universidad Autonoma de Madrid (Spain)

    2007-05-15

    The {sup 46}Ti * compound nucleus, as populated by the fusion-evaporation reaction {sup 27}Al + {sup 19}F at the bombarding energy of E {sub lab} = 144 MeV, has been investigated by charged particle spectroscopy using the multidetector array ICARE at the VIVITRON tandem facility of the IReS (Strasbourg). The light charged particles and high-energy {gamma}-rays from the GDR decay have been measured in coincidence with selected evaporation residues. The CACARIZO code, a Monte Carlo implementation of the statistical-model code CASCADE, has been used to calculate the spectral shapes of evaporated {alpha}-particles which are compared with the experimental coincident spectra. This comparison indicates the signature of large deformations (possibly superdeformed and hyperdeformed shapes) present in the compound nucleus decay. The occurrence of the Jacobi shape transition is also discussed in the framework of a newly developed rotating liquid drop model.

  15. Re-evaluation of microscopic and integral cross-section data for important dosimetry reactions. Re-evaluation of the excitation functions for the 24Mg(n,p)24Na, 32S(n,p)32P, 60Ni(n,p)60m+gCo, 63Cu(n,2n)62Cu, 65Cu(n,2n)64Cu, 64Zn(n,p)64Cu, 115In(n,2n)114mIn, 127I(n,2n)126I, 197Au(n,2n)196Au and 199Hg(n,n')199mHg reactions

    International Nuclear Information System (INIS)

    Re-evaluations of cross sections and their associated covariance matrices have been carried out for ten dosimetry reactions: - excitation functions for the 63Cu(n,2n)62Cu, 65Cu(n,2n)64Cu, 64Zn(n,p)64Cu, 115In(n,2n)114mIn and 199Hg(n,n')199mHg reactions were re-evaluated over the neutron energy range from threshold to 20 MeV; - excitation functions for the 24Mg(n,p)24Na, 32S(n,p)32P and 60Ni(n,p)60m+gCo were reevaluated in the energy range from threshold to 21 MeV; - excitation functions for the 127I(n,2n)126I and 197Au(n,2n)196Au reactions were reevaluated in the energy range from threshold to 32 and 40 MeV, respectively. Benchmark calculations performed for 235U thermal fission and 252Cf spontaneous fission neutron spectra show that the integral cross sections derived from the newly evaluated excitation functions exhibit improved agreement with related experimental data when compared with the equivalent data from the IRDF-2002 library. (author)

  16. On the Contribution of Gamma Ray Bursts to the Galactic Inventory of Some Intermediate Mass Nuclei

    Energy Technology Data Exchange (ETDEWEB)

    Pruet, J; Surman, R; McLaughlin, G C

    2004-01-23

    Light curves from a growing number of Gamma Ray Bursts (GRBs) indicate that GRBs copiously produce radioactive Ni moving outward at fractions of the speed of light. We calculate nuclear abundances of elements accompanying the outflowing Ni under the assumption that this Ni originates from a wind blown off of a viscous accretion disk. We also show that GRB's likely contribute appreciably to the galactic inventory of {sup 42}Ca, {sup 45}Sc, {sup 46}Ti, {sup 49}Ti, {sup 63}Cu, and may be an important site for the production of {sup 64}Zn.

  17. On the Contribution of Gamma Ray Bursts to the Galactic Inventory of Some Intermediate Mass Nuclei

    CERN Document Server

    Pruet, J; McLaughlin, G C; Pruet, Jason; Surman, Rebecca; Laughlin, Gail C. Mc

    2004-01-01

    Light curves from a growing number of Gamma Ray Bursts (GRBs) indicate that GRBs copiously produce radioactive Ni moving outward at fractions of the speed of light. We calculate nuclear abundances of elements accompanying the outflowing Ni under the assumption that this Ni originates from a wind blown off of a viscous accretion disk. We also show that GRB's likely contribute appreciably to the galactic inventory of 42Ca, 45Sc, 46Ti, 49Ti, 63Cu, and may be a principal site for the production of 64Zn.

  18. Integral cross section measurements of a few threshold reactions induced by Am/Be neutrons

    Energy Technology Data Exchange (ETDEWEB)

    Uddin, Md. Shuza; Hossain, Syed Mohammad; Rumman-Uz-Zaman, Md. [Atomic Energy Research Establishment, Dhaka (Bangladesh). Institute of Nuclear Science and Technology (INST); Spahn, Ingo; Qaim, Syed M. [Forschungszentrum Juelich GmbH (Germany). Inst. fuer Neurowissenschaften und Medizin (INM), Nuklearchemie (INM-5); Rakib-Uz-Zaman, Md. [Rajshahi Univ. (Bangladesh). Dept. of Applied Chemistry and Chemical Engineering

    2015-07-01

    Integral cross sections of the reactions {sup 46}Ti(n,p){sup 46}Sc, {sup 47}Ti(n,p){sup 47}Sc, {sup 48}Ti(n,p){sup 48}Sc, {sup 60}Ni(n,p){sup 60}Co and {sup 64}Zn(n,p){sup 64}Cu were measured with fast neutrons (E{sub n} > 1.5 MeV) from an Am/Be source. The results were compared with data calculated using the neutron spectral distribution and the excitation function of each reaction given in the data libraries ENDF/B-VII.0, IRDF-2002, JEFF-3.2 and JENDL-4.0. In general, the integral measurement and the integrated value agreed within ±4%, except for the {sup 46}Ti(n,p){sup 46}Sc reaction where JEFF-3.2 shows a deviation of 7% and the {sup 60}Ni(n,p){sup 60}Co reaction where ENDF/B-VII.0 and IRDF-2002 exhibit deviations upto 8%.

  19. Ferroelectromagnetic solid solutions on the base piezoelectric ceramic materials for components of micromechatronics

    Science.gov (United States)

    Bochenek, Dariusz; Zachariasz, Radosław; Niemiec, Przemysław; Ilczuk, Jan; Bartkowska, Joanna; Brzezińska, Dagmara

    2016-10-01

    In the presented work, a ferroelectromagnetic solid solutions based on PZT and ferrite powders have been obtained. The main aim of combination of ferroelectric and magnetic powders was to obtain material showing both electric and magnetic properties. Ferroelectric ceramic powder (in amount of 90%) was based on the doped PZT type solid solution while magnetic component was nickel-zinc ferrite Ni1-xZnxFe2O4 (in amount of 10%). The synthesis of components of ferroelectromagnetic solid solutions was performed using the solid phase sintering. Final densification of synthesized powder has been done using free sintering. The aim of the work was to obtain and examine in the first multicomponent PZT type ceramics admixed with chromium with the following chemical composition Pb0.94Sr0.06(Zr0.46Ti0.54)O3+0.25 at% Cr2O3 and next ferroelectromagnetic solid solution based on a PZT type ferroelectric powder (Pb0.94Sr0.06(Zr0.46Ti0.54)O3+0.25 at% Cr2O3) and nickel-zinc ferrite (Ni0.64Zn0.36Fe2O4), from the point of view of their mechanical and electric properties, such as: electric permittivity, ε; dielectric loss, tanδ; mechanical losses, Q-1; and Young modulus, E.

  20. The PSIMECX medium-energy neutron activation cross-section library. Part 1: Description and procedures for use

    Energy Technology Data Exchange (ETDEWEB)

    Atchison, F.

    1998-09-01

    The PSIMECX library contains calculated nuclide production cross-sections from neutron-induced reactions in the energy range about 2 to 800 MeV in the following 72 stable isotopes of 24 elements: {sup 12}C, {sup 13}C, {sup 16}O, {sup 17}O, {sup 18}O, {sup 23}Na, {sup 24}Mg, {sup 25}Mg, {sup 26}Mg, {sup 27}Al, {sup 28}Si, {sup 29}Si, {sup 30}Si, {sup 31}P, {sup 32}S, {sup 33}S, {sup 34}S, {sup 36}S, {sup 35}Cl, {sup 37}Cl, {sup 39}K, {sup 40}K, {sup 41}K, {sup 40}Ca, {sup 42}Ca, {sup 43}Ca, {sup 44}Ca, {sup 46}Ca, {sup 48}Ca, {sup 46}Ti, {sup 47}Ti, {sup 48}Ti, {sup 49}Ti, {sup 50}Ti, {sup 50}V, {sup 51}V, {sup 50}Cr, {sup 52}Cr, {sup 53}Cr, {sup 54}Cr, {sup 55}Mn, {sup 54}Fe, {sup 56}Fe, {sup 57}Fe, {sup 58}Fe, {sup 58}Ni, {sup 60}Ni, {sup 61}Ni, {sup 62}Ni, {sup 64}Ni, {sup 63}Cu, {sup 65}Cu, {sup 64}Zn, {sup 66}Zn, {sup 67}Zn, {sup 68}Zn, {sup 70}Zn, {sup 92}Mo, {sup 94}Mo, {sup 95}Mo, {sup 96}Mo, {sup 97}Mo, {sup 98}Mo, {sup 100}Mo, {sup 121}Sb, {sup 123}Sb, {sup 204}Pb, {sup 206}Pb, {sup 207}Pb, {sup 208}Pb, {sup 232}Th and {sup 238}U. The energy range covers essentially all transmutation channels other than capture. The majority of the selected elements are principal constituents of normal materials of construction used in and around accelerator facilities and the library is, first and foremost, designed to be a tool for the estimation of their activation in wide-band neutron fields. This first report, from a set of three, describes the form and usage of the library; the other two reports document the calculational methods. The present organisation of the library is the author's first idea and adequate for the intended use (activation calculations); being machine readable, translation of the library into other formats is straightforward. (author)

  1. The PSIMECX medium-energy neutron activation cross-section library. Part II: Calculational methods for light to medium mass nuclei

    Energy Technology Data Exchange (ETDEWEB)

    Atchison, F.

    1998-09-01

    The PSIMECX library contains calculated nuclide production cross-sections from neutron-induced reactions in the energy range about 2 to 800 MeV in the following 72 stable isotopes of 24 elements: {sup 12}C, {sup 13}C, {sup 16}O, {sup 17}O, {sup 18}O, {sup 23}Na, {sup 24}Mg, {sup 25}Mg, {sup 26}Mg, {sup 27}Al, {sup 28}Si, {sup 29}Si, {sup 30}Si, {sup 31}P, {sup 32}S, {sup 33}S, {sup 34}S, {sup 36}S, {sup 35}Cl, {sup 37}Cl, {sup 39}K, {sup 40}K, {sup 41}K, {sup 40}Ca, {sup 42}Ca, {sup 43}Ca, {sup 44}Ca, {sup 46}Ca, {sup 48}Ca, {sup 46}Ti, {sup 47}Ti, {sup 48}Ti, {sup 49}Ti, {sup 50}Ti, {sup 50}V, {sup 51}V, {sup 50}Cr, {sup 52}Cr, {sup 53}Cr, {sup 54}Cr, {sup 55}Mn, {sup 54}Fe, {sup 56}Fe, {sup 57}Fe, {sup 58}Fe, {sup 58}Ni, {sup 60}Ni, {sup 61}Ni, {sup 62}Ni, {sup 64}Ni, {sup 63}Cu, {sup 65}Cu, {sup 64}Zn, {sup 66}Zn, {sup 67}Zn, {sup 68}Zn, {sup 70}Zn, {sup 92}Mo, {sup 94}Mo, {sup 95}Mo, {sup 96}Mo, {sup 97}Mo, {sup 98}Mo, {sup 100}Mo, {sup 121}Sb, {sup 123}Sb, {sup 204}Pb, {sup 206}Pb, {sup 207}Pb, {sup 208}Pb, {sup 232}Th and {sup 238}U. The energy range covers essentially all transmutation channels other than capture. The majority of the selected elements are principal constituents of normal materials of construction used in and around accelerator facilities and the library is, first and foremost, designed to be a tool for the estimation of their activation in wide-band neutron fields. This second report, of a series of three, describes and discusses the calculational methods used for the stable isotopes up to and including {sup 123}Sb. The library itself has been described in the first report of the series and the treatment for the heavy nuclei is given in the third. (author)

  2. ZZ KAFAX-F31, 150 and 12 Groups Cross Section Library in MATXS Format based on JEFF-3.1 for Fast Reactors

    International Nuclear Information System (INIS)

    1 - Description: Format: MATXS, 142 nuclides processed with NJOY99.245. Number of groups: 150 neutron-, 12 photon-groups. 142 nuclides: H-1, H-2, He-3, He-4, Li-6, Li-7, Be-9, B-10, B-11, C-nat, N-14, N-15, O-16, F-19, Na-23, Mg-24, Mg-25, Mg-26, Al-27, Si-28, Si-29, Si-30, P-31, Cl-35, Cl-37, Ar-40, K-39, K-40, K-41, Ca-40, Ca-42, Ca-43, Ca-44, Ca-46, Ca-48, Ti-46, Ti-47, Ti-48, Ti-49, Ti-50, V-nat, Cr-50, Cr-52, Cr-53, Cr-54, Mn-55, Fe-54, Fe-56, Fe-57, Fe-58, Co-59, Ni-58, Ni-60, Ni-61, Ni-62, Ni-64, Cu-63, Cu-65, Ga-nat, Y-89, Zr-90, Zr-91, Zr-92, Zr-93, Zr-94, Zr-95, Zr-96, Nb-93, Mo-92, Mo-94, Mo-95, Mo-96, Mo-97, Mo-98, Mo-99, Mo-100, Ag-107, Ag-109, Cd-106, Cd-108, Cd-110, Cd-111, Cd-112, Cd-113, Cd-114, Cd-115m, Cd-116, Sn-112, Sn-114, Sn-115, Sn-116, Sn-117, Sn-118, Sn-119, Sn-120, Sn-122, Sn-123, Sn-124, Sn-125, Sn-126, Eu-151, Eu-153, Gd-152, Gd-154, Gd-155, Gd-156, Gd-157, Gd-158, Gd-160, W-182, W-183, W-184, W-186, Re-185, Re-187, Au-197, Pb-206, Pb-207, Pb-208, Bi-209, Th-232, Pa-233, U-233, U-234, U-235, U-236, U-238, Np-237, Pu-238, Pu-239, Pu-240, Pu-241, Pu-242, Am-241, Am-242, Am-242m, Am-243, Cm-242, Cm-243, Cm-244, Cm-245, Cm-246. Origin: JEFF-3.1. Weighting spectrum: 300, 600, 900, 1200 K. The KAFAX-F31 is a MATXS-format, 150-group neutron and 12-group photon cross section library for fast reactors based on JEFF-3.1. This library was originally generated for the KALIMER (Korea Advanced LIquid Metal Reactor) core analyses. It includes 142 nuclide data (Table 1) processed by the NJOY99.245 code patched with NEA020. The library can be utilized to generate the problem-dependent group constants for neutron and/or photon transport calculations through the DANTSYS, DOORS, or PARTISN code systems. 2 - Methods: The KAFAX-F31 was generated at 300, 600, 900, and 1200 K. It contains the self-shielded cross sections for 5 to 10 background cross sections depending on the nuclides. The neutron group structure consists of one-eighth lethargy widths in almost

  3. ZZ KAFAX-E70, 150 and 12 Groups Cross Section Library in MATXS Format based on ENDF/B-VII.0 for Fast Reactors

    International Nuclear Information System (INIS)

    1 - Description: Format: MATXS, 144 nuclides processed with NJOY99.245. Number of groups: 150 neutron-, 12 photon-groups. 144 nuclides: H-1, H-2, He-3, He-4, Li-6, Li-7, Be-9, B-10, B-11, C-nat, N-14, N-15, O-16, F-19, Na-23, Mg-24, Mg-25, Mg-26, Al-27, Si-28, Si-29, Si-30, P-31, Cl-35, Cl-37, Ar-40, K-39, K-40, K-41, Ca-40, Ca-42, Ca-43, Ca-44, Ca-46, Ca-48, Ti-46, Ti-47, Ti-48, Ti-49, Ti-50, V-nat, Cr-50, Cr-52, Cr-53, Cr-54, Mn-55, Fe-54, Fe-56, Fe-57, Fe-58, Co-59, Ni-58, Ni-60, Ni-61, Ni-62, Ni-64, Cu-63, Cu-65, Ga-69, Ga-71, Y-89, Zr-90, Zr-91, Zr-92, Zr-93, Zr-94, Zr-95, Zr-96, Nb-93, Mo-92, Mo-94, Mo-95, Mo-96, Mo-97, Mo-98, Mo-99, Mo-100, Ag-107, Ag-109, Cd-106, Cd-108, Cd-110, Cd-111, Cd-112, Cd-113, Cd-114, Cd-115m, Cd-116, Sn-112, Sn-113, Sn-114, Sn-115, Sn-116, Sn-117, Sn-118, Sn-119, Sn-120, Sn-122, Sn-123, Sn-124, Sn-125, Sn-126, Eu-151, Eu-153, Gd-152, Gd-154, Gd-155, Gd-156, Gd-157, Gd-158, Gd-160, W-182, W-183, W-184, W-186, Re-185, Re-187, Au-197, Pb-206, Pb-207, Pb-208, Bi-209, Th-232, Pa-233, U-233, U-234, U-235, U-236, U-238, Np-237, Pu-238, Pu-239, Pu-240, Pu-241, Pu-242, Am-241, Am-242, Am-242m, Am-243, Cm-242, Cm-243, Cm-244, Cm-245, Cm-246. Origin: ENDF/B-VII.0. Weighting spectrum: 300, 600, 900, 1200 k. The ZZ-KAFAX-E70 is a MATXS-format, 150-group neutron and 12-group photon cross section library for fast reactors based on ENDF/B-VII.0. This library was originally generated for the KALIMER (Korea Advanced Liquid Metal Reactor) core analyses. It includes 144 nuclide data processed with the NJOY99.245 code patched with NEA020. The library can be used to generate the problem-dependent group constants for neutron and/or photon transport calculations through the DANTSYS, DOORS, or PARTISN code systems. 2 - Methods: The KAFAX-E70 was generated at 300, 600, 900, and 1200 K. It contains the self-shielded cross sections for 5 to 10 background cross sections depending on the nuclides. The neutron group structure consists of one-eighth lethargy

  4. ZZ KAFAX-J33, 150 and 12 Groups Cross Section Library in MATXS Format based on JENDL-3.3 for Fast Reactors

    International Nuclear Information System (INIS)

    1 - Description: Format: MATXS, 136 nuclides processed with NJOY99.245. Number of groups: 150 neutron-, 12 photon-groups. 136 Nuclides: H-1, H-2, He-3, He-4, Li-6, Li-7, Be-9, B-10, B-11, C-nat, N-14, N-15, O-16, F-19, Na-23, Mg-24, Mg-25, Mg-26, Al-27, Si-28, Si-29, Si-30, P-31, Cl-35, Cl-37, Ar-40, K-39, K-40, K-41, Ca-40, Ca-42, Ca-43, Ca-44, Ca-46, Ca-48, Ti-46, Ti-47, Ti-48, Ti-49, Ti-50, V-nat, Cr-50, Cr-52, Cr-53, Cr-54, Mn-55, Fe-54, Fe-56, Fe-57, Fe-58, Co-59, Ni-58, Ni-60, Ni-61, Ni-62, Ni-64, Cu-63, Cu-65, Ga-69, Ga-71, Y-89, Zr-90, Zr-91, Zr-92, Zr-93, Zr-94, Zr-95, Zr-96, Mo-92, Mo-94, Mo-95, Mo-96, Mo-97, Mo-98, Mo-99, Mo-100, Ag-107, Ag-109, Cd-106, Cd-108, Cd-110, Cd-111, Cd-112, Cd-113, Cd-114, Cd-116, Sn-112, Sn-114, Sn-115, Sn-116, Sn-117, Sn-118, Sn-119, Sn-120, Sn-122, Sn-123, Sn-124, Sn-126, Eu-151, Eu-153, Gd-152, Gd-154, Gd-155, Gd-156, Gd-157, Gd-158, Gd-160, W-182, W-183, W-184, W-186, Pb-206, Pb-208, Bi-209, Th-232, Pa-233, U-233, U-234, U-235, U-236, U-238, Np-237, Pu-238, Pu-239, Pu-240, Pu-241, Pu-242, Am-241, Am-242, Am-242m, Am-243, Cm-242, Cm-243, Cm-244, Cm-245, Cm-246. Origin: JENDL-3.3. Weighting spectrum: 300, 600, 900, 1200 K. The KAFAX-J33 is a MATXS-format, 150-group neutron and 12-group photon cross section library for fast reactors based on JENDL-3.3. This library was originally generated for the KALIMER (Korea Advanced LIquid Metal Reactor) core analyses. It includes 136 nuclide data processed by the NJOY99.245 code patched with NEA020. The library can be utilized to generate the problem-dependent group constants for neutron and/or photon transport calculations through the DANTSYS, DOORS, or PARTISN code systems. 2 - Methods: The KAFAX-J33 was generated at 300, 600, 900, and 1200 K. It contains the self-shielded cross sections for 5 to 10 background cross sections depending on the nuclides. The neutron group structure consists of one-eighth lethargy widths in almost all the energy ranges, except between 1 and 10 keV in

  5. Zinc separation by using a liquid membrane

    International Nuclear Information System (INIS)

    We have performed the isotopic separation of 64Zn and 66Zn by using a liquid membrane with chloroform diluent and dicyclohexano - 18 - crown - 6 as carrier. The isotopic separation factor was the same as for liquid-liquid extraction

  6. Zinc isotope separation in acetone by displacement chromatography using benzo-15-crown-5 resin

    International Nuclear Information System (INIS)

    Zinc isotope separation was studied by column chromatographies using resorcinol-formaldehyde-resin grafted with benzo-15-crown-5 in the porous silica beads. Chromatography was performed in a break-through manner by feeding the acetone solution of zinc chloride into the columns. Zinc isotopic abundance ratios of 66Zn/64Zn and 68Zn/64Zn were measured by ICP-MS. It has been found that the heavier isotopes are preferentially enriched at the front boundary region. This result proves 64Zn depleted zinc can be obtained by collecting the effluents of front boundary region. The separation coefficient (ε) observed by five meters migration treatment is 0.81 x 10-3 for the isotopic pair of 68Zn/64Zn at 25 deg C and higher separation coefficient was obtained from more concentrated zinc chloride solution. (author)

  7. Role of projectile breakup in {sup 6}He and {sup 6}Li induced fusion reactions around barrier energies

    Energy Technology Data Exchange (ETDEWEB)

    Kumari, Anju; Kharab, Rajesh, E-mail: kharabrajesh@rediffmail.com

    2015-09-15

    The influence of projectile breakup on fusion cross section for {sup 6}He + {sup 209}Bi, {sup 6}He + {sup 64}Zn, {sup 6}Li + {sup 209}Bi and {sup 6}Li + {sup 64}Zn reactions at near barrier energies is studied within the framework of quantum diffusion approach. The breakup does not affect the fusion induced by {sup 6}He, whereas a significant suppression for {sup 6}Li induced reaction is observed in below barrier energy region.

  8. Overview

    International Nuclear Information System (INIS)

    The year 2003 can be called a real breakthrough for our Institute. We managed to have our Institute transferred to the Polish Academy of Sciences. Furthermore, we succeeded in joining several programmes of the EU. These programmes are usually oriented towards improving the quality of life and applied research. Our scientific activities throughout 2003 led to 325 publications. In addition, we published 210 conference reports and scientific articles. In the field of particle physics the outstanding result was precise determination of the φ1 angle of the unitarity triangle, sin2φ1 0.733±0.057, in the CP violation studies based on B-mesons decays. This result was the outcome of the Belle collaboration. Here, our contribution was the Si Vertex Detector. An interesting result was obtained in the studies of the B0→φK0s decay driven by the b→sss transition. The time-dependent CP asymmetry in this channel measured with high statistics hinted at the CP asymmetry being inconsistent with the Standard Model (SM) prediction. This may be a sign of new physics. In central Au + Au collisions at 200 GeV/nucleon pair, the Phobos group discovered creation of a new type of highly excited hadronic matter which strongly absorbs the jets. This result indicates that a sort of critical state for dense excited hadronic matter has been reached. The Coriolis splitting of the GDR components in 46Ti was observed, and a link to the low excited states of 42Co established. This may point to a kind of memory in the compound nucleus. The spectra of pions from hadronic reaction were calculated using unintegrated parton distributions known from lepton inelastic scattering experiments. It was shown that the spectra cannot be explained by the gluonic mechanism only. Complete Two-Loop Bosonic contributions to the Muon Lifetime in the Standard Model were calculated. These results will serve as a test of the SM in future e+e- colliders. Within the Na49 collaboration the existence of the S=-2, Q =-2

  9. ZZ MATXSLIBJ33, JENDL-3.3 based, 175 N-42 photon groups (VITAMIN-J) MATXS library for discrete ordinates multi-group

    International Nuclear Information System (INIS)

    1 - Description of program or function: JENDL-3.3 based, 175 neutron-42 photon groups (VITAMIN-J) MATXS library for discrete ordinates multi-group transport codes. Format: MATXS. Number of groups: 175 neutron, 42 gamma-ray. Nuclides: 337 nuclides contained in JENDL-3.3: H-1, H-2, He-3, He-4, Li-6, Li-7, Be-9, B-10, B-11, C-Nat, N-14, N-15, O-16, F-19, Na-23, Mg-24, Mg-25, Mg-26, Al-27, Si-28, Si-29, Si-30, P-31, S-32, S-33, S-34, S-36, Cl-35, Cl-37, Ar-40, K-39, K-40, K-41, Ca-40, Ca-42, Ca-43, Ca-44, Ca-46, Ca-48, Sc-45, Ti-46, Ti-47, Ti-48, Ti-49, Ti-50, V-Nat, Cr-50, Cr-52, Cr-53, Cr-54, Mn-55, Fe-54, Fe-56, Fe-57, Fe-58, Co-59, Ni-58, Ni-60, Ni-61, Ni-62, Ni-64, Cu-63, Cu-65, Ga-69, Ga-71, Ge-70, Ge-72, Ge-73, Ge-74, Ge-76, As-75, Se-74, Se-76, Se-77, Se-78, Se-79, Se-80, Se-82, Br-79, Br-81, Kr-78, Kr-80, Kr-82, Kr-83, Kr-84, Kr-85, Kr-86, Rb-85, Rb-87, Sr-86, Sr-87, Sr-88, Sr-89, Sr-90, Y-89, Y-91, Zr-90, Zr-91, Zr-92, Zr-93, Zr-94, Zr-95, Zr-96, Nb-93, Nb-94, Nb-95, Mo-92, Mo-94, Mo-95, Mo-96, Mo-97, Mo-98, Mo-99, Mo-100, Tc-99, Ru-96, Ru-98, Ru-99, Ru-100, Ru-101, Ru-102, Ru-103, Ru-104, Ru-106, Rh-103, Rh-105, Pd-102, Pd-104, Pd-105, Pd-106, Pd-107, Pd-108, Pd-110, Ag-107, Ag-109, Ag-110m, Cd-106, Cd-108, Cd-110, Cd-111, Cd-112, Cd-113, Cd-114, Cd-116, In-113, In-115, Sn-112, Sn-114, Sn-115, Sn-116, Sn-117, Sn-118, Sn-119, Sn-120, Sn-122, Sn-123, Sn-124, Sn-126, Sb-121, Sb-123, Sb-124, Sb-125, Te-120, Te-122, Te-123, Te-124, Te-125, Te-126, Te-127m, Te-128, Te-129m, Te-130, I-127, I-129, I-131, Xe-124, Xe-126, Xe-128, Xe-129, Xe-130, Xe-131, Xe-132, Xe-133, Xe-134, Xe-135, Xe-136, Cs-133, Cs-134, Cs-135, Cs-136, Cs-137, Ba-130, Ba-132, Ba-134, Ba-135, Ba-136, Ba-137, Ba-138, Ba-140, La-138, La-139, Ce-140, Ce-141, Ce-142, Ce-144, Pr-141, Pr-143, Nd-142, Nd-143, Nd-144, Nd-145, Nd-146, Nd-147, Nd-148, Nd-150, Pm-147, Pm-148, Pm-148m, Pm-149, Sm-144, Sm-147, Sm-148, Sm-149, Sm-150, Sm-151, Sm-152, Sm-153, Sm-154, Eu-151, Eu-152, Eu-153, Eu-154, Eu-155, Eu

  10. Zinc isotope separation in acetone by displacement chromatography using benzo-15-crown-5 resin

    International Nuclear Information System (INIS)

    Zinc is considered as a useful material for cooling water treatment in light water plants. Injection of 64Zn depleted Zinc is expected to further reduce the radiation in the reactor water system. For such a purpose of Zinc isotope separation, chemical exchange method has been studied. Breakthrough methods of chromatography experiments were performed. 0.5 mol/dm3 ZnCl2 dissolved in acetone solution was fed to glass columns packed with benzo-15-crown-5 resin at 35 degree C. The effluent was collected in fractions of which zinc concentration was determined by atomic adsorption spectrometer and isotope ratio was measured by ICP-MS. Observed enrichment ratios defined as, (iZn/64Zn)sample/ (iZn/64Zn)original, where i=66,68, are plotted in Figure. From the results of experiment, it was confirmed that heavier zinc is preferentially enriched in the eluted samples of front band regions. The separation coefficient (ε) for 66Zn/64Zn and 68Zn/64Zn of five meters migration was obtained as 5.2 x 10-4 and 8.1 x 10-4, respectively. The error is estimated to be 20% of the values.

  11. Zinc isotope separation with crown ether by column chromatography

    International Nuclear Information System (INIS)

    Depleted 64Zn is a new useful material and can be widely used in the cooling water treatment in light water nuclear power plants. In the present work, column chromatographic zinc isotope separation was performed by crown ether resin which was synthesized by ourselfs, the experimental results shown that benzo-15-crown-5 resin could effectively separate the zinc isotopes. High temperature could improve the separation coefficient, while the migration distance has no effect on separation coefficient. The height equivalent to a theoretical plate increase with the increasing of the migration distance. The separation coefficients (68Zn/64Zn=6.03 x 10-4, 66Zn/64Zn=3.52 x 10-4, respectively) and the height equivalent to a theoretical plate (0.204 cm) were obtained by 20 meters chromatographic operation with the temperature of 328 K. (authors)

  12. Spin distribution as a probe to investigate the dynamical effects in fusion reactions

    Directory of Open Access Journals (Sweden)

    Kaur Maninder

    2015-01-01

    Full Text Available The spin distributions are measured for the compound nucleus 80Sr populated in the reactions 16O+64Zn and 32S+48Ti. The comparison of the experimental results for both the systems shows that the mean γ-ray multiplicity values for the system 32S+48Ti are lower than those for 16O+64Zn. The spin distribution of the compound nucleus populated through the symmetric channel is also found to be lower than the asymmetric channel. Present investigation directly shows the effect of entrance channel mass asymmetry on the reaction dynamics.

  13. Search for double beta decay of zinc and tungsten with low background ZnWO{sub 4} crystal scintillators

    Energy Technology Data Exchange (ETDEWEB)

    Bernabei, R; Nozzoli, F [Dip. di Fisica, Universita di Roma ' Tor Vergata' , I-00133 Rome (Italy); Belli, P [INFN, sez. Roma ' Tor Vergata' , I-00133 Rome (Italy); Cappella, F; Prosperi, D [Dip. di Fisica, Universita di Roma ' La Sapienza' , I-00185 Rome (Italy); Cerulli, R; Nisi, S [INFN, Laboratori Nazionali del Gran Sasso, 67010 Assergi (Italy); Danevich, F A; Kobychev, V V; Mokina, V M; Nagorny, S S; Poda, D V; Tretyak, V I; Yurchenko, S S [Institute for Nuclear Research, MSP 03680 Kyiv (Ukraine); Grinyov, B V; Nagornaya, L L [Institute for Scintillation Materials, 61001 Kharkiv (Ukraine); Incicchitti, A [INFN, sez. Roma, I-00185 Rome (Italy)

    2010-01-01

    Double beta processes in {sup 64}Zn, {sup 70}Zn, {sup 180}W, and {sup 186}W have been searched for with the help of low background ZnWO4 crystal scintillators at the Gran Sasso National Laboratories of the INFN (Italy). The total measurement time exceeds ten thousand hours. New improved half-life (T{sub 1/2}) limits on double electron capture and electron capture with positron emission in {sup 64}Zn have been set. New T{sub 1/2} bounds were also set on different modes of 2{beta} processes in {sup 70}Zn, {sup 180}W, and {sup 186}W. Future perspectives are considered.

  14. New lifetime measurements in the stable semimagic Sn isotopes using the Doppler-shift attenuation technique

    Science.gov (United States)

    Jungclaus, A.; Walker, J.; Leske, J.; Speidel, K.-H.; Stuchbery, A. E.; East, M.; Boutachkov, P.; Cederkäll, J.; Doornenbal, P.; Egido, J. L.; Ekström, A.; Gerl, J.; Gernhäuser, R.; Goel, N.; Górska, M.; Kojouharov, I.; Maier-Komor, P.; Modamio, V.; Naqvi, F.; Pietralla, N.; Pietri, S.; Prokopowicz, W.; Schaffner, H.; Schwengner, R.; Wollersheim, H.-J.

    2011-09-01

    Precise measurements of lifetimes in the picosecond range of excited states in the stable even-A Sn isotopes 112,114,116,122Sn have been performed using the Doppler shift attenuation technique. For the first excited 2+ states in 112Sn, 114Sn and 116Sn the E2 transition strengths deduced from the measured lifetimes are in disagreement with the previously adopted values. They indicate a shallow minimum at N = 66 in contrast to the maximum at mid-shell predicted by modern shell model calculations.

  15. Resonant Continuum in the Relativistic Mean-Field Theory

    Institute of Scientific and Technical Information of China (English)

    CAOLi-Gang; MAZhong-Yu

    2002-01-01

    Energies,widths and wave functions of the single-particle resonant continuum are determined by solving scattering states of the Dirac equation with proper asymptotic conditions for the continuous spectrum in the relativistic mean-field theory.The relativistic regular and irregular Coulomb wave functions are calculated numerically.The resonance states in the continum for some closed-or sub-closed-shell nucleus in Sn-isotopes,such as 114Sn,116Sn,118Sn,and 120Sn are calculated.Results show that the S-matrix method is a reliable and straightforward way in determining energies and widths of resonant states.

  16. New lifetime measurements in the stable semimagic Sn isotopes using the Doppler-shift attenuation technique

    International Nuclear Information System (INIS)

    Precise measurements of lifetimes in the picosecond range of excited states in the stable even-A Sn isotopes 112,114,116,122Sn have been performed using the Doppler shift attenuation technique. For the first excited 2+ states in 112Sn, 114Sn and 116Sn the E2 transition strengths deduced from the measured lifetimes are in disagreement with the previously adopted values. They indicate a shallow minimum at N = 66 in contrast to the maximum at mid-shell predicted by modern shell model calculations.

  17. Combinatorial Level Densities from a Microscopic Relativistic Structure Model

    OpenAIRE

    Pezer, R.; Ventura, A.; Vretenar, D.

    2002-01-01

    A new model for calculating nuclear level densities is investigated. The single-nucleon spectra are calculated in a relativistic mean-field model with energy-dependent effective mass, which yields a realistic density of single-particle states at the Fermi energy. These microscopic single-nucleon states are used in a fast combinatorial algorithm for calculating the non-collective excitations of nuclei. The method, when applied to magic and semi-magic nuclei, such as $^{60}$Ni, $^{114}$Sn and $...

  18. ZZ FSXJ32, MCNP nuclear data library based on JENDL-3.2. ZZ FSXLIBJ33, MCNP nuclear data library based on JENDL-3.3

    International Nuclear Information System (INIS)

    1 - Description of program or function: - NEA-1424/03: JENDL-3.2 based MCNP library. Format: MCNP. Number of groups: Continuous energy cross section library. Nuclides: H, He, Li, Be, B, C, N, O, F, Na, Mg, Al, Si, P, S, Cl, Ar, K, Ca, Sc, Ti, V, Cr, Mn, Fe, Co, Ni, Cu, Ga, Ge, As, Se, Br, Kr, Rb, Sr, Y, Zr, Nb, Mo, Tc, Ru, Rh, Pd, Ag, Cd, In, Sn, Sb, Te, I, Xe, Cs, Ba, La, Ce, Pr, Nd, Pm, Sm, Eu, Gd, Hf, Ta, W, Pb, Bi, Ra, Ac, Th, Pa, U, Np, Pu, Am, Cm, Bk, Cf, Es, Fm. Temperatures: 293 K, 600 K, 900 K, 1200 K, 1500 K, 2000 K. Origin: JENDL-3.2. The temperature-dependent continuous energy cross section library for MCNP, FSXJ32, was prepared from JENDL-3.2 for a variety of applications in the field of atomic energy. - NEA-1424/06: April 2005: This is the DVD version of ZZ-FSXJ32 NEA-1424/03. - NEA-1424/07: This version differs from version NEA-1424/05 in the following: Index files xsdir.fsxlb331 and xsdir.fsxlb332 have been updated, since atomic weights were missing for 23 nuclides. JENDL-3.3 based MCNP library. Format: MCNP. Number of groups: Continuous energy cross section library. Nuclides: 337 nuclides contained in JENDL-3.3. H-1, H-2, He-3, He-4, Li-6, Li-7, Be-9, B-10, B-11, C-Nat, N-14, N-15, O-16, F-19, Na-23, Mg-24, Mg-25, Mg-26, Al-27, Si-28, Si-29, Si-30, P-31, S-32, S-33, S-34, S-36, Cl-35, Cl-37, Ar-40, K-39, K-40, K-41, Ca-40, Ca-42, Ca-43, Ca-44, Ca-46, Ca-48, Sc-45, Ti-46, Ti-47, Ti-48, Ti-49, Ti-50, V-Nat, Cr-50, Cr-52, Cr-53, Cr-54, Mn-55, Fe-54, Fe-56, Fe-57, Fe-58, Co-59, Ni-58, Ni-60, Ni-61, Ni-62, Ni-64, Cu-63, Cu-65, Ga-69, Ga-71, Ge-70, Ge-72, Ge-73, Ge-74, Ge-76, As-75, Se-74, Se-76, Se-77, Se-78, Se-79, Se-80, Se-82, Br-79, Br-81, Kr-78, Kr-80, Kr-82, Kr-83, Kr-84, Kr-85, Kr-86, Rb-85, Rb-87, Sr-86, Sr-87, Sr-88, Sr-89, Sr-90, Y-89, Y-91, Zr-90, Zr-91, Zr-92, Zr-93, Zr-94, Zr-95, Zr-96, Nb-93, Nb-94, Nb-95, Mo-92, Mo-94, Mo-95, Mo-96, Mo-97, Mo-98, Mo-99, Mo-100, Tc-99, Ru-96, Ru-98, Ru-99, Ru-100, Ru-101, Ru-102, Ru-103, Ru-104, Ru-106, Rh

  19. Isotopic fractionation of zinc in tektites

    Science.gov (United States)

    Moynier, Frederic; Beck, Pierre; Jourdan, Fred; Yin, Qing-Zhu; Reimold, Uwe; Koeberl, Christian

    2009-01-01

    Tektites are terrestrial natural glasses produced during a hypervelocity impact of an extraterrestrial projectile onto the Earth's surface. The similarity between the chemical and isotopic compositions of tektites and terrestrial upper continental crust implies that the tektites formed by fusion of such target rock. Tektites are among the driest rocks on Earth. Although volatilization at high temperature may have caused this extreme dryness, the exact mechanism of the water loss and the behavior of other volatile species during tektite formation are still debated. Volatilization can fractionate isotopes, therefore, comparing the isotope composition of volatile elements in tektites with that of their source rocks may help to understand the physical conditions during tektite formation. For this study, we have measured the Zn isotopic composition of 20 tektites from four different strewn fields. Almost all samples are enriched in heavy isotopes of Zn compared to the upper continental crust. On average, the different groups of tektites are isotopically distinct (listed from the isotopically lightest to the heaviest): Muong-Nong type indochinites ( δ66/64Zn = 0.61 ± 0.30‰); North American bediasites ( δ66/64Zn = 1.61 ± 0.49‰); Ivory Coast tektites ( δ66/64Zn = 1.66 ± 0.18‰); the Australasian tektites (others than the Muong Nong-type indochinites) ( δ66/64Zn = 1.84 ± 0.42‰); and Central European moldavites ( δ66/64Zn = 2.04 ± 0.19‰). These results are contrasted with a narrow range of δ66/64Zn = 0-0.7‰ for a diverse spectrum of upper continental crust materials. The elemental abundance of Zn is negatively correlated with δ66/64Zn, which may reflect that isotopic fractionation occurred by evaporation during the heating event upon tektite formation. Simple Rayleigh distillation predicts isotopic fractionations much larger than what is actually observed, therefore, such a model cannot account for the observed Zn isotope fractionation in tektites. We

  20. Shell Model Analysis of the ^45V(p,γ) thermonuclear reaction rate relevant to ^44Ti production in core-collapse supernovae

    Science.gov (United States)

    Horoi, M.; Jora, R.; Zelevinsky, V.; Murphy, A. St. J.; Boyd, R. N.

    2001-10-01

    A reliable estimate of the ^45V(p,γ) reaction rate is necessary in order to reduce a large uncertainty in the production of ^44Ti in core collapse supernovae. We performed a theoretical analysis of the astrophysical factors and reaction rates including resonances in ^46Cr associated with the analog states in ^46Ti. Full fp shell model calculations are performed to predict positive parity states in ^46Ti situated in the Gamow window, which have a significant proton spectroscopic factor. The uncertainty of the reaction rate associated with electric dipole gamma decays to the negative parity low-lying states is also discussed.

  1. Asymptotic and near-target direct breakup of 6Li and 7Li

    Science.gov (United States)

    Kalkal, Sunil; Simpson, E. C.; Luong, D. H.; Cook, K. J.; Dasgupta, M.; Hinde, D. J.; Carter, I. P.; Jeung, D. Y.; Mohanto, G.; Palshetkar, C. S.; Prasad, E.; Rafferty, D. C.; Simenel, C.; Vo-Phuoc, K.; Williams, E.; Gasques, L. R.; Gomes, P. R. S.; Linares, R.

    2016-04-01

    Background: Li,76 and 9Be are weakly bound against breakup into their cluster constituents. Breakup location is important for determining the role of breakup in above-barrier complete fusion suppression. Recent works have pointed out that experimental observables can be used to separate near-target and asymptotic breakup. Purpose: Our purpose is to distinguish near-target and asymptotic direct breakup of Li,76 in reactions with nuclei in different mass regions. Method: Charged particle coincidence measurements are carried out with pulsed Li,76 beams on 58Ni and 64Zn targets at sub-barrier energies and compared with previous measurements using 208Pb and 209Bi targets. A detector array providing a large angular coverage is used, along with time-of-flight information to give definitive particle identification of the direct breakup fragments. Results: In interactions of 6Li with 58Ni and 64Zn, direct breakup occurs only asymptotically far away from the target. However, in interactions with 208Pb and 209Bi, near-target breakup occurs in addition to asymptotic breakup. Direct breakup of 7Li into α -t is not observed in interactions with 58Ni and 64Zn. However, near-target dominated direct breakup was observed in measurements with 208Pb and 209Bi. A modified version of the Monte Carlo classical trajectory model code platypus, which explicitly takes into account lifetimes associated with unbound states, is used to simulate sub-barrier breakup reactions. Conclusions: Near-target breakup in interactions with Li,76 is an important mechanism only for the heavy targets 208Pb and 209Bi. There is insignificant near-target direct breakup of 6Li and no direct breakup of 7Li in reactions with 58Ni and 64Zn. Therefore, direct breakup is unlikely to suppress the above-barrier fusion cross section in reactions of Li,76 with 58Ni and 64Zn nuclei.

  2. Risk of overestimation of urinary cadmium concentrations: interference from molybdenum

    Directory of Open Access Journals (Sweden)

    Cañas A.I.

    2013-04-01

    Full Text Available We show here that the selection of analytical method is critical when measuring low levels of cadmium in human urine. Cadmium is today usually analyzed by Inductively Coupled Plasma Mass Spectrometry (ICP-MS, which has a higher sensitivity than Atomic Absorption Spectroscopy (AAS. ICP-MS cadmium measurements show interference from tin (114Sn and molybdenum oxides, which can result in an overestimation of cadmium levels. The 114Sn interference is stable and can be mathematically corrected. Molybdenum concentrations in urine are variable and different from individual to individual. We have estimated the degree of error which molybdenum interference introduces in the measurement of cadmium in urine by conventional ICP-MS. 268 urine samples from mothers and their children were measured. Removal of the molybdenum oxide interference (DRC-ICP-MS method reduced urinary cadmium concentrations significantly (47.8%. The urinary molybdenum concentration in children was higher than in their mothers, resulting in greater overestimation. Our results clearly show that the DRC method is essential for reliable measurements of urinary cadmium concentrations, particularly in children. Furthermore, care should be taken when comparing Human Biomonitoring data for cadmium in urine and attention should be paid to which analytical method has been used (e.g. AAS and ICP-Ms, and especially if the measurements have been corrected for molybdenum interference.

  3. Origins of dipole resonance strength fragmentation in calcium and titanium isotopes

    Directory of Open Access Journals (Sweden)

    Skorodumina Iu. A.

    2012-12-01

    Full Text Available Theoretical description of dipole resonances in 46Ti, 48Ti, 50Ti, 48Ca, 40Ca was performed. The distribution of the “hole” among the states of final nuclei was taken into account using information on pick-up reactions. The obtained results are in reasonable agreement with experimental data.

  4. Evaluation of zinc, cadmium and lead isotope fractionation during smelting and refining

    International Nuclear Information System (INIS)

    To evaluate metallurgical processing as a source of Zn and Cd isotopic fractionation and to potentially trace their distribution in the environment, high-precision MC-ICP-MS Zn, Cd and Pb isotope ratio measurements were made for samples from the integrated Zn-Pb smelting and refining complex in Trail, B.C., Canada. Significant fractionation of Zn and Cd isotopes during processing of ZnS and PbS ore concentrates is demonstrated by the total variation in δ66/64Zn and δ114/110Cd values of 0.42 per mille and 1.04 per mille , respectively, among all smelter samples. No significant difference is observed between the isotopic compositions of the Zn ore concentrates (δ66/64Zn = 0.09 to 0.17 per mille ; δ114/110Cd = - 0.13 to 0.18 per mille ) and the roasting product, calcine (δ66/64Zn = 0.17 per mille ; δ114/110Cd = 0.05 per mille ), due to ∼ 100% recovery from roasting. The overall Zn recovery from metallurgical processing is ∼ 98%, thus the refined Zn metal (δ66/64Zn = 0.22 per mille ) is not significantly fractionated relative to the starting materials despite significantly fractionated fume (δ66/64Zn = 0.43 per mille ) and effluent (δ66/64Zn = 0.41 to 0.51 per mille ). Calculated Cd recovery from metallurgical processing is 72-92%, with the majority of the unrecovered Cd lost during Pb operations (δ114/110Cd = - 0.38 per mille ). The refined Cd metal is heavy (δ114/110Cd = 0.39 to 0.52 per mille ) relative to the starting materials. In addition, significant fractionation of Cd isotopes is evidenced by the relatively light and heavy isotopic compositions of the fume (δ114/110Cd = - 0.52 per mille ) and effluent (δ114/110Cd = 0.31 to 0.46 per mille ). In contrast to Zn and Cd, Pb isotopes are homogenized by mixing during processing. The total variation observed in the Pb isotopic compositions of smelter samples is attributed to mixing of ore sources with different radiogenic signatures.

  5. Study on bioavailability of zinc for children's diet by using activable isotopic tracer 70Zn and neutron activation analysis techniques

    International Nuclear Information System (INIS)

    Bioavailability of zinc for three groups (low amount of diet zinc, balance amount of diet zinc and high amount of diet zinc) of children's diet is studied by using activable isotopic tracer 70Zn and neutron activation analysis techniques. The results indicate that the fractional absorption of zinc from balance diet zinc group is the highest, up to 33.9%. A procedure of pre-irradiation concentration zinc for fecal samples using anion exchanger is developed, and the enriched 70Zn with isotopic abundance of 18.3% is used for tracer. The mass ratios between 70Zn and 68Zn or 64Zn and their contents between natural zinc and enriched zinc are used to calculate the bioavailability of zinc. Instrumental neutron activation analysis of 64Zn of each original fecal samples and pre-irradiation concentrated zinc samples are used to normalize the chemical yield in order to reduce the uncertainty during the chemical separation procedure

  6. Production and separation of 64Cu and 67Cu using 14 MeV neutrons

    International Nuclear Information System (INIS)

    64Cu and 67Cu were produced from 14 MeV neutron irradiated natural ZnO and enriched 64ZnO targets via 64Zn(n,p)64Cu and 67Zn(n,p)67Cu reactions. The ZnO disc targets were irradiated for 6 hours by 14 MeV neutrons, which are generated by bombarding a tritiated titanium target with deuteron beam at the Fusion Neutronics Source (FNS) at Japan Atomic Energy Agency (JAEA). After irradiation, ion chromatographic separations were carried out to obtain purified no-carrier-added Cu radionuclides. Elution pattern clearly showed separation of 64Cu and 67Cu giving a yield of > 90%, and a very low radionuclide impurity ratio of 65Zn within the purified 64Cu. (author)

  7. Zinc isotope fractionation on benzo-15-crown-5 resin by liquid chromatography

    International Nuclear Information System (INIS)

    Chromatographic fractionation of zinc isotopes was performed on the synthesized benzo-15-crown-5 resin as a column packing material at 323 K in the breakthrough manner for both a frontal and a rear bands. Zinc adsorption capacity was affected by anion chloride concentration and solvent dielectric constant. The heavier zinc isotopes were found enriched to the solution phase and the lighter zinc isotope was concentrated on the resin phase. The frontal maximum enrichment ratio for isotopic pair of 68Zn/64Zn was 1.0081. The isotope separation coefficients for isotopic pair of 68Zn/64Zn for frontal and rear band, were 5.3x10-4, 4.5x10-4, respectively. (author)

  8. Search for double beta decay of Zinc and Tungsten with the help of low-background ZnWO4 crystal scintillators

    CERN Document Server

    Belli, P; Cappella, F; Cerulli, R; Danevich, F A; Grinyov, B V; Incicchitti, A; Kobychev, V V; Mokina, V M; Nagorny, S S; Nagornaya, L L; Nisi, S; Nozzoli, F; Poda, D V; Prosperi, D; Tretyak, V I; Yurchenko, S S

    2008-01-01

    Double beta processes in 64-Zn, 70-Zn, 180-W, and 186-W have been searched for with the help of large volume (0.1-0.7 kg) low background ZnWO4 crystal scintillators at the Gran Sasso National Laboratories of the INFN. Total time of measurements exceeds 10 thousands hours. New improved half-life limits on double electron capture and electron capture with positron emission in 64-Zn have been set, in particular (all the limits are at 90% C.L.): T1/2(0nu2EC)> 1.1e20 yr, T1/2(2nuECbeta+)>7.0e20 yr, and T1/2(0nuECbeta+)>4.3e20 yr. The different modes of double beta processes in 70-Zn, 180-W, and 186-W have been restricted at the level of 1e17-1e20 yr.

  9. Final results of an experiment to search for 2beta processes in zinc and tungsten with the help of radiopure ZnWO4 crystal scintillators

    CERN Document Server

    Belli, P; Cappella, F; Cerulli, R; Danevich, F A; d'Angelo, S; Incicchitti, A; Kobychev, V V; Poda, D V; Tretyak, V I

    2011-01-01

    A search for the double beta decay of zinc and tungsten isotopes has been performed with the help of radiopure ZnWO4 crystal scintillators (0.1-0.7 kg) at the Gran Sasso National Laboratories of the INFN. The total exposure of the low background measurements is 0.529 kg yr. New improved half-life limits on the double beta decay modes of 64Zn, 70Zn, 180W, and 186W have been established at the level of 10^{18}-10^{21} yr. In particular, limits on double electron capture and electron capture with positron emission in 64Zn have been set: T_{1/2}(2\

  10. Continuum effects in the scattering of exotic nuclei

    Energy Technology Data Exchange (ETDEWEB)

    Druet, T. [Universite Libre de Bruxelles (ULB), Physique Quantique, C.P. 165/82, Brussels (Belgium); Universite Libre de Bruxelles (ULB), Physique Nucleaire Theorique et Physique Mathematique, Brussels (Belgium); Descouvemont, P. [Universite Libre de Bruxelles (ULB), Physique Nucleaire Theorique et Physique Mathematique, Brussels (Belgium)

    2012-10-15

    We discuss continuum effects in the scattering of exotic nuclei, and more specifically on the {sup 11}Be + {sup 64}Zn scattering. {sup 11}Be is a typical example of an exotic nucleus, with a low binding energy. Elastic, inelastic and breakup cross-sections of the {sup 11}Be + {sup 64}Zn system are computed in the Continuum Discretized Coupled Channel formalism, at energies near the Coulomb barrier. We show that converged cross-sections need high angular momenta as well as as large excitation energies in the wave functions of the projectile. Extensions to other systems are simulated by different collision energies, and by varying the binding energy of {sup 11}Be. (orig.)

  11. Determination of activable isotopic tracers of zinc by neutron activation analysis for study of bioavailability of zinc

    International Nuclear Information System (INIS)

    A procedure of pre-irradiation concentration of zinc in fecal samples using anion exchanger was developed for the study of the bioavailability of zinc by neutron activation analysis. The mass ratios between 70Zn and 68Zn, or 64Zn and their contents between natural zinc and enriched zinc are used to calculate the bioavailability of zinc when the abundance of the isotope 70Zn is not high enough. (author) 9 refs.; 1 fig.; 2 tabs

  12. Thermal properties of a rotating nucleus in a fluctuating mean field approach

    OpenAIRE

    B K Agrawal; Ansari, A

    1993-01-01

    The static path approximation to the path integral representation of partition function provides a natural microscopic basis to deal with thermal fluctuations around mean field configurations. Using this approach for one-dimensional cranking Hamiltonian with quadrupole- quadrupole interaction term we have studied a few properties like energy, level density, level density parameter($a$) and moment of inertia as a function of temperature and spin for $^{64}Zn$ taking it as an illustrative examp...

  13. Properties of rotational bands at the spin limit in A {approximately} 50, A {approximately} 65 and A {approximately} 110 nuclei

    Energy Technology Data Exchange (ETDEWEB)

    Janzen, V.P.; Andrews, H.R.; Ball, G.C. [Chalk River Labs., Ontario (Canada)] [and others

    1996-12-31

    There is now widespread evidence for the smooth termination of rotational bands in A {approx_equal} 110 nuclei at spins of 40-to-50{Dirac_h}s. The characteristics of these bands are compared to those of bands recently observed to high spin in {sup 64}Zn and {sup 48}Cr, studied with the 8{pi} {gamma}-ray spectrometer coupled to the Chalk River miniball charged-particle-detector array.

  14. Mediating conducting polymer growth within hydrogels by controlling nucleation

    OpenAIRE

    A. J. Patton; Green, R A; L. A. Poole-Warren

    2015-01-01

    This study examines the efficacy of primary and secondary nucleation for electrochemical polymerisation of conductive polymers within poly(vinyl alcohol) methacrylate hydrogels. The two methods of nucleation investigated were a primary heterogeneous mechanism via introduction of conductive bulk metallic glass (Mg64Zn30Ca5Na1) particles and a secondary mechanism via introduction of “pre-polymerised” conducting polymer within the hydrogel (PEDOT:PSS). Evidence of nucleation was not seen in the ...

  15. Enrichment of zinc isotopes by a liquid membrane system using a crown ether

    International Nuclear Information System (INIS)

    A liquid membrane system to enrich zinc isotope was investigated. The liquid membrane was composed of a solution of dicyclohexano-18-crown-6 in chloroform. Zinc chloride dissolved in diluted hydrochloric acid was used as a feed phase. A receiving phase was made of a 0.001 M HCl solution. The zinc isotopes were enriched (1) at the interface of the liquid-membrane/feed-phase and (2) at that of the liquid-membrane/receiving-phase. The separation factor attained in the system was α = 1.049 for the separation of 64Zn and 66Zn. The enrichment factor of 66Zn relative to 67Zn was ε = -0.053, which is in the inverse direction of enrichment by a liquid-liquid extraction. The enrichment factor of 64Zn to 66Zn showed a different value from that of 66Zn to 68Zn, regardless of their similar mass difference. The isotope effects in the Zn-crown complex were dominated by the field shift of electronic energy in the isotope atom. This is in contrast to the Bigeleisen-Mayer approximation for a chemical exchange reaction. Trace amounts of zinc are injected into the primary coolant of boiling water reactors in order to suppress 60Co build-up. The use of 64Zn-depleted zinc suppresses the production of 65Zn within the reactor. Zinc isotopes are also useful precursors of radiopharmaceuticals

  16. Isotope separation of zinc by ion cyclotron resonance

    International Nuclear Information System (INIS)

    The separation of zinc isotopes has been performed in CEA Saclay by ion cyclotron resonance (ICR). Zinc, enriched in the isotope 68 is needed for medical applications and zinc, depleted in the isotope 64, in nuclear water reactors. A high density (up to 8 x 1011 cm-3), low electronic temperature (1-3 eV) plasma has been obtained, using Joule heating combined with electron cyclotron resonance heating. The density and electronic radial profiles have been measured as well as the multicharged ions, which have been found negligible. The selective resonant heating of 68 Zn, measured with an electrostatic analyser, has reached 180 eV, while the ionic energy of non resonant isotopes remains around 3 eV. In the so-called depletion experiments, we choose to have 64 Zn resonant; in this case, the 64 Zn ion energy was increased up to 150 eV. The conditions for depleting the initial natural zinc in 64 Zn have been optimised: i.e. the rich collector bias and the spacing of the blades of the 'rich'collector. It has been easy to get a depletion factor of 0.26 with a high flow rate. As a conclusion, operating conditions that make the ICR process attractive in the depletion mode have been derived. (author)

  17. Zinc isotope effects observed by liquid chromatography with benzo-15-crown-5 resin

    International Nuclear Information System (INIS)

    The chromatographic fractionation in Zn isotopes was performed on the synthesized benzo-15-crown-5 resin at 313 and 343 K. The lighter isotopes were found enriched in the resin phase. The isotope fractionation coefficients (ε) were 3.4 and 2.9x10-4, 4.7 and 4.7x10-4, and 6.7 and 5.7x10-4 for the 66Zn/64Zn, 67Zn/64Zn and 68Zn/64Zn isotopic pairs at 313 and 343 K, respectively. They reflected mass-dependence among the Zn isotopes at each operated temperature but did not show 1/T2-temperature proportionality. The temperature effects of the composition of Zn species both in the solution phase and in the resin phase may account in part for the latter observation. The magnitudes of ε's in this study were comparable to the ones obtained by ion exchange chromatography, but much smaller than those observed in the solvent extraction systems with a crown ether in the organic phase. (author)

  18. Study of the giant dipole resonance built on highly excited states in Sn and Dy nuclei

    International Nuclear Information System (INIS)

    A study is presented of the giant dipole resonance built on highly excited states. The aim is to get more detailed information on the properties of the GDR and to use it as a tool for the investigation of nuclear structure at high excitation energy. The high energy γ-rays seen from the decay of excited state GDRs in heavy ion fusion reactions reflect the average properties of the states populated by the γ-emission. The measurements at different initial excitation energies of 114Sn provide information on the nuclear level density near the particle separation energy at an average angular momentum of 10ℎ. The study of shape changes at very high spin in 152-156Dy nuclei is presented. A theoretical model developed to describe fusion-evaporation reactions is presented. 149 refs.; 63 figs.; 13 tabs

  19. Search for the Jacobi shape transition in light nuclei

    CERN Document Server

    Maj, A; Brekiesz, M; Grebosz, J; Meczynski, W; Styczen, J; Zieblinski, M; Zuber, K; Bracco, A; Camera, F; Benzoni, G; Million, B; Blasi, N; Brambilla, S; Leoni, S; Pignanelli, M; Wieland, O; Nyberg, J; Kicinska-Habior, M; Petrache, C M; Dudek, J; Pomorski, K

    2003-01-01

    The gamma-rays following the reaction 105 MeV 18O + 28Si have been measured using the EUROBALL IV, HECTOR and EUCLIDES arrays in order to investigate the predicted Jacobi shape transition. The high-energy gamma-ray spectrum from the GDR decay indicates a presence of large deformations in hot 46Ti nucleus, in agreement with new theoretical calculations based on the Rotating Liquid Drop model.

  20. Search for the Jacobi shape transition in light nuclei

    Energy Technology Data Exchange (ETDEWEB)

    Maj, A.; Kmiecik, M.; Brekiesz, M.; Grebosz, J.; Meczynski, W.; Styczen, J.; Zieblinski, M.; Zuber, K. [The Niewodniczanski Institute of Nuclear Physics, Polish Academy of Sciences, ul. Radzikowskiego 152, PL-31342, Krakow (Poland); Bracco, A.; Camera, F.; Benzoni, G.; Million, B.; Blasi, N.; Brambilla, S.; Leoni, S.; Pignanelli, M.; Wieland, O. [Dipartimento di Fisica and INFN sez. Milano, I-20133, Milano (Italy); Herskind, B. [The Niels Bohr Insitute, Blegdamsvej 17, DK-2100, Copenhagen (Denmark); Bednarczyk, P. [The Niewodniczanski Institute of Nuclear Physics, Polish Academy of Sciences, ul. Radzikowskiego 152, PL-31342, Krakow (Poland); Institut de Recherches Subatomiques, 23 rue du Loess, BP28, F-67037, Strasbourg (France); Curien, D. [Institut de Recherches Subatomiques, 23 rue du Loess, BP28, F-67037, Strasbourg (France); Vivien, J.P.; Farnea, E.; De Angelis, G.; Napoli, D.R.; Nyberg, J.; Kicinska-Habior, M.; Petrache, C.M.; Dudek, J.; Pomorski, K.

    2004-04-01

    The {gamma}-rays following the reaction 105 MeV {sup 18}O+{sup 28}Si have been measured using the EUROBALL IV, HECTOR and EUCLIDES arrays in order to investigate the predicted Jacobi shape transition. The high-energy {gamma}-ray spectrum from the GDR decay indicates the presence of large deformations in the hot {sup 46}Ti nucleus, in agreement with new theoretical calculations based on the rotating liquid-drop model. (orig.)

  1. High-Spin States in Odd-Odd N=Z {sup 46}V

    Energy Technology Data Exchange (ETDEWEB)

    O' Leary, C.D.; Bentley, M.A.; Appelbe, D.E.; Bark, R.A.; Cullen, D.M.; Erturk, S.; Maj. A.; Sheikh, J.A.; Warner, D.D.

    1999-12-31

    High-spin states up to the F{sub 7/2}-shell band termination at J{pi}=15+ have been observed for the first time in the odd-odd N=Z=23 nucleous {sup 46}V. The new level scheme has two separate structures corresponding to spherical and prolate shapes. A rotational band has very similar energies to the yrast sequence in {sup 46}Ti and is therefore assumed to be a T=1 configuration.

  2. INFLUENCE OF AGEING ON THE INTERNAL FRICTION OF Nb-Ti-N ALLOYS

    OpenAIRE

    Heulin, B.; Clauss, A.

    1981-01-01

    We have studied the influence of ageing on the internal friction of various Nb-4.6Ti-N alloys at 1Hz, annealed for 24 hours at 400, 600, and 800°C. This study shows the influence of temperature, beginning at 400°C, on the measurements of internal friction and allows a more complete description of the structure and behaviour of Nb-Ti-N alloys.

  3. Do light nuclei display a universal γ-ray strength function?

    Directory of Open Access Journals (Sweden)

    Voinov A.

    2012-02-01

    Full Text Available In this work we focus on properties in the quasi-continuum of light nuclei. Generally, both level density and γ-ray strength function (γ-SF differ from nucleus to nucleus. In order to investigate this closer, we have performed particle-γ coincidences using the reactions (p, p', (p, d and (p, t on a 46Ti target. In particular, the very rich data set of the 46Ti(p, p'46Ti inelastic scattering reaction allows analysis of the coincidence data for many independent data sets. Using the Oslo method, we find one common level density for all data sets. If transitions to well-separated low-energy levels are included, the deduced γ-SF may change by a factor of 2 – 3, due strong to Porter-Thomas fluctuations. However, a universal γ-SF with small fluctuations is found provided that only excitation energies above 3 MeV are taken into account. The nuclear structure of the titaniums is discussed within a combinatorial quasi-particle model, showing that only few Nilsson orbitals participate in building up the level density for these light nuclei.

  4. Theoretical and experimental cross sections for neutron reactions on 64Zinc

    International Nuclear Information System (INIS)

    Accurate measurements of the 64Zn (n,2n) 64Cu and 64Zn (n,p) 63Zn cross sections at 14.8 MeV have been made using a Texas Nuclear Neutron Generator and the activation technique. A NaI(T1) spectrometer (using two 6'' x 6'' NaI detectors/crystals) was used to measure the gamma radiation emitted in coincidence from the positron-emitting decay products. The measurements were made relative to 65Cu (n,2n) /64/Cu and 63Cu (n,2n) 62Cu cross sections, which have similar half-lives, radiation emission, and were previously measured to high accuracy (2 percent). The value obtained for the (n,2n) measurement was 199 /+-/ 6 millibarns, and a value of 176 /+-/ 4.5 millibarns was obtained for the (n,p) measurement. In concert, a theoretical analysis of neutron induced reactions on /64/Zn was performed at Los Alamos National Laboratory using the Hauser-Feshbach statistical theory in the GNASH code over an energy range of 100 keV to 20 MeV. Calculations included width fluctuation corrections, direct reaction contributions, and preequilibrium corrections above 6 MeV. Neutron optical model potentials were determined for zinc. The theoretical values agree with the new 14.8 MeV measurements approximately within experimental error, with calculations of 201 millibarns for the (n,2n) cross section and 170 millibarns for the (n,p) cross section. Results from the analysis will be made available in National Evaluated Nuclear Data Format (ENDF/B) for fusion energy applications. 50 refs., 34 figs., 10 tabs

  5. Zn isotopic fractionation caused by sorption on goethite and 2-Lines ferrihydrite

    Science.gov (United States)

    Juillot, F.; Maréchal, C.; Ponthieu, M.; Cacaly, S.; Morin, G.; Benedetti, M.; Hazemann, J. L.; Proux, O.; Guyot, F.

    2008-10-01

    Zn isotopic fractionation caused by sorption on 2-Lines ferrihydrite (Fh2L) and goethite was investigated to assess the role of reactions at the Fe-oxyhydroxide/water interface in changes of the isotopic distribution of Zn. Since sorption reactions are ubiquitous in Earth's surface environments, it is important to evaluate their influence on the isotopic distribution of Zn before it can be used to track and quantify contributions of various sources and/or biogeochemical processes involving this element. Our results show that Zn isotopes are fractionated upon sorption on Fe-oxyhydroxides with an enrichment of the heavy isotopes present on the solid's surface. This fractionation appears to proceed through an equilibrium mechanism and yields different (Δ 66/64Zn) sorbed-aqueous values for Zn sorption on goethite [(Δ 66/64Zn) sorbed-aqueous around +0.29‰] and Fh2L [(Δ 66/64Zn) sorbed-aqueous around +0.53‰]. These different magnitudes of Zn fractionation are related to structural differences between Zn complexes existing on the surface of goethite (octahedrally coordinated Zn by oxygen atoms) and Fh2L (tetrahedrally coordinated Zn by oxygen atoms), as evidenced by Extended X-ray Absorption Fine Structure (EXAFS) spectroscopy and CD-MUSIC modeling. These results show the importance of accounting for reactions at the Fe-oxyhydroxide/water interface when dealing with the isotopic distribution of Zn at the Earth's surface. Considering the large range of other possible sorbents (Mn or Al oxides, phyllosilicates, carbonates, biologic surfaces, etc.) and the importance of reactions at sorbent/water interfaces for other non-traditional stable isotopes (i.e. Cr, Fe, Ni and Cu) that are increasingly used in environmental studies, these results emphasize the need for further experimental studies that are needed to quantify the isotopic fractionation of these elements possibly accompanying their sorption.

  6. Theoretical and experimental cross sections for neutron reactions on /sup 64/Zinc

    Energy Technology Data Exchange (ETDEWEB)

    Rutherford, D.A.

    1988-03-01

    Accurate measurements of the /sup 64/Zn (n,2n)/sup 63/Zn and /sup 64/Zn (n,p)/sup 64/Cu cross sections at 14.8 MeV have been made using a Texas Nuclear Neutron Generator and the activation technique. A NaI(Tl) spectrometer (using two 6'' x 6'' NaI detectors/crystals) was ued to measure the gamma radiation emitted in coincidence from the positron-emitting decay products. The measurements were made relative to /sup 65/Cu (n,2n)/sup 64/Cu and /sup 63/Cu (n,2n)/sup 62/Cu cross sections, which have similar half-lives, radiation emission, and were previously measured to high accuracy (2%). The value obtained for the (n,2n) measurement was 199 +- 6 millibarns, and a value of 176 +- 4.5 millibarns was obtained for the (n,p) measurement. In concert, a theoretical analysis of neutron induced reactions on /sup 64/Zn was performed at Los Alamos National Laboratory using the Hauser-Feshbach statistical theory in the GNASH code over an energy range of 100 keV to 20 MeV. Calculations included width fluctuation corrections, direct reaction contributions, and preequilibrium corrections above 6 MeV. Neutron optical model potentials were determined for zinc. The theoretical values agree with the new 14.8 MeV measurements approximately within experimental error, with calculations of 201 millibarns for the (n,2n) cross section and 170 millibarns for the (n,p) cross section. Results from the analysis will be made available in National Evaluated Nuclear Data Format (ENDF/B) for fusion energy applications. 50 refs., 34 figs., 10 tabs.

  7. Structure of high-spin states in A {approx} 60 region

    Energy Technology Data Exchange (ETDEWEB)

    Nakada, Hitoshi [Chiba Univ. (Japan); Furutaka, K.; Hatsukawa, Y. [and others

    1998-03-01

    High-spin states in the proton-rich Cu-Zn nuclei are investigated by the experiments at JAERI. New levels and {gamma}-rays are identified by the particle-{gamma}-{gamma} coincidence, and J{sup P} assignments are made via the DCO ratio analysis. Yrast sequences are observed up to J {approx} 18 for {sup 62}Zn, and {sup 64}Zn, J {approx} 27/2 for {sup 61}Cu and J {approx} 23/2 for {sup 63}Cu. Though we cannot settle new J{sup P} values for {sup 61,63}Zn, their yrast sequence is also extended. In {sup 64}Zn, a doublet of {gamma}-rays is discovered at 1315 keV, clarifying the similarity in the level scheme between {sup 62}Zn and {sup 64}Zn. We reproduce the yrast levels by a shell-model calculation, by which structure of the high-spin states is further studied. A parity change in the yrast sequence is established, in which the unique-parity orbit 0g{sub 9/2} plays an essential role; one nucleon excitation to g{sub 9/2} gains high angular momentum with low seniority, at the cost of the single-parity energy. Second parity-change is also suggested by the calculation. Such parity change seems characteristic to spherical or nearly spherical nuclei. In {sup 61}Cu, concentration of the {gamma}-ray intensity is observed. This happens because a stretched 3-quasiparticle configuration including 0g{sub 9/2} is relatively stable, similarly to some isomers. Thus, by studying the structure of the high-spin states of the A {approx} 60 nuclei, we have clarified the role of unique-parity orbit in high-spin states, which may be generic to spherical and nearly spherical nuclei. (J.P.N.)

  8. Isotope effects of zinc in crown ether chromatography

    International Nuclear Information System (INIS)

    Isotope separation of zinc has been studied with a polymer-supported crown ether resin packed in glass columns. Chromatography was performed in a break-through manner by feeding a zinc chloride solution into the columns. The mass analysis revealed that the heavier isotope was enriched at the front part of the zinc adsorption band. This result means that the heavier isotopes are preferentially fractionated into the solution phase. The largest single-stage separation coefficient (ε) in the present work is 1.0 x 10-3 for the isotopic pair of 64Zn and 66Zn at 35degC. (author)

  9. Isotope enrichment of metal in the process of zone melting

    International Nuclear Information System (INIS)

    The possibility of using the zone melting technique with the purpose of isotope enrichment of metal has been checked. The experiments have been carried out with zinc and cadmium wires. After the experiment the long wire has been sectioned by 15 mm and in such a state has been subjected to mass spectrometric and neutron activation analysis. The dependence of isotope enrichment with zone passage is shown. The light isotopes 64Zn in zinc and 106Cd and 108Cd in cadmium move following the zone enriching at the wire end

  10. Centrifugal enrichment of zinc isotopes, their application in medicine and in increasing radiation safety in nuclear power plants

    International Nuclear Information System (INIS)

    This paper contains the results of our research on the complete cycle of centrifuge enrichment of all zinc isotopes. The centrifuge cascade that was used to obtain the world's first zinc isotope, 7Zn, with an enrichment of more than 99.3% in gram quantities, is described. As a result of this work, gram quantities of all highly enriched zinc isotopes and hundreds of grams of depleted zinc (in the form of ZnO) with concentrations of less than 0.5% 64Zn were obtained

  11. Dominance of binary dissipative reactions in nearly symmetric nucleus-nucleus collisions above 35 MeV/U

    International Nuclear Information System (INIS)

    Incomplete fusion or massive transfer mechanisms were invoked to explain the observed distributions of products, especially for heavy residues, for the nearly symmetric systems, 36Ar on 27Al from 55 to 95 MeV/u, and 64Zn on natTi, from 35 to 79 MeV/u. Charged products were detected in a nearly 4π geometry using two complementary multidetector systems. Lorentz invariant cross section maps plotted for different products show three sources for Z=1 and 2 particles: quasi-projectile, quasi-target and a third source, located at mid-rapidity. For heavier fragments, the mid-rapidity contribution vanishes. (K.A.)

  12. Improvements on the present theoretical understanding of octupole correlations

    International Nuclear Information System (INIS)

    Some intriguing results, obtained in a recent survey of octupole properties for all even-even nuclei, are reanalyzed in order to understand the origin of the strong disagreement with experimental data and/or the strange behaviours observed. The limitations of the rotational formula to describe E1 and E3 transition strengths are discussed as well as the role played by octupole-quadrupole coupling in some specific nuclei such as 20Ne, 64Zn, 158Gd, 208Pb and 224Ra

  13. Elastic and break-up of the 1n-halo 11Be nucleus

    Science.gov (United States)

    Di Pietro, A.; Moro, A. M.; Acosta, L.; Amorini, F.; Borge, M. J. G.; Figuera, P.; Fisichella, M.; Fraile, L. M.; Gomez-Camacho, J.; Jeppesen, H.; Lattuada, M.; Martel, I.; Milin, M.; Musumarra, A.; Papa, M.; Pellegriti, M. G.; Perez-Bernal, F.; Raabe, R.; Randisi, G.; Rizzo, F.; Scuderi, V.; Tengblad, O.; Torresi, D.; Vidal, A. Maira; Voulot, D.; Wenander, F.; Zadro, M.

    2014-03-01

    The elastic and break-up angular distributions of the 10,11Be+64Zn reactions measured at Ec.m.≈1.4 VC have been analysed within the CCDC and O.M. frameworks. The suppression of the Coulomb-nuclear interference, observed in the 11Be scattering case with respect to the 10Be, has been interpreted as due to a long range absorption owing to the coupling with the break-up (Coulomb and nuclear) channels. The presence of 10Be events on the 11Be experiment data have been explained as due mainly to break-up processes.

  14. Elastic and break-up of the 1n-halo 11Be nucleus

    Directory of Open Access Journals (Sweden)

    Di Pietro A.

    2014-03-01

    Full Text Available The elastic and break-up angular distributions of the 10,11Be+64Zn reactions measured at Ec.m.≈1.4 VC have been analysed within the CCDC and O.M. frameworks. The suppression of the Coulomb-nuclear interference, observed in the 11Be scattering case with respect to the 10Be, has been interpreted as due to a long range absorption owing to the coupling with the break-up (Coulomb and nuclear channels. The presence of 10Be events on the 11Be experiment data have been explained as due mainly to break-up processes.

  15. Double beta decay of ^{64,70}Zn and ^{180,186}W isotopes

    CERN Document Server

    Poda, D V

    2011-01-01

    The results of the experimental investigations of double beta processes in Zinc and Tungsten isotopes with the help of middle volume (117 g, 168 g and 699 g) low-background ZnWO_4 crystal scintillators are presented. The experiment was carried out in the low-background "DAMA/R&D" set-up at the Gran Sasso National Laboratories of the INFN (Italy) at a depth of \\approx3600 m w.e. The total measurement time exceeds ten thousand hours. New improved half-life limits on double electron capture and electron capture with positron emission in ^{64}Zn have been set: T^{2\

  16. Giant Dipole Resonance in the Hot and Thermalized Ce132 Nucleus: Damping of Collective Modes at Finite Temperature

    Science.gov (United States)

    Wieland, O.; Bracco, A.; Camera, F.; Benzoni, G.; Blasi, N.; Brambilla, S.; Crespi, F.; Giussani, A.; Leoni, S.; Mason, P.; Million, B.; Moroni, A.; Barlini, S.; Kravchuk, V. L.; Gramegna, F.; Lanchais, A.; Mastinu, P.; Maj, A.; Brekiesz, M.; Kmiecik, M.; Bruno, M.; Geraci, E.; Vannini, G.; Casini, G.; Chiari, M.; Nannini, A.; Ordine, A.; Ormand, E.

    2006-07-01

    The γ decay of the giant dipole resonance (GDR) in the Ce132 compound nucleus with temperature up to ≈4MeV has been measured, using the reaction Ni64+Zn68 at Ebeam=300, 400, and 500 MeV. The γ and charged particles measured in coincidence with recoils are consistent with a fully equilibrated compound nucleus emission. The GDR width, obtained with the statistical model analysis, is found to increase almost linearly with temperature. This increase is rather well reproduced within a model including thermal shape fluctuations and the lifetime of the compound nucleus.

  17. Enhanced production possibility of the therapeutic radionuclides 64Cu, 67Cu and 89Sr via (n,p) reactions induced by fast spectral neutrons

    OpenAIRE

    Spahn, I.; Coenen, H. H.; Qaim, S. M.

    2004-01-01

    Spectrum averaged cross sections for the Zn-64(n, p)Cu-64, Zn-67(n, p)Cu-67 and Y-89(n, p)Sr-89 reactions were measured using a 14 MeV d(Be) neutron source. In each case a clean radiochemical separation was performed and the radioactivity of the product was determined via high-resolution gamma-ray spectrometry or anticoincidence beta(-) counting. The cross sections are three to five times higher than with a fission neutron spectrum. It is postulated that at an intense fast spectral neutron so...

  18. Diffraction structures in high-energy electron–nucleus bremsstrahlung

    Energy Technology Data Exchange (ETDEWEB)

    Jakubassa-Amundsen, D.H.

    2013-10-30

    The emission of hard bremsstrahlung during the collision of relativistic spin-polarized electrons with inert spin 0 and spin 1/2 nuclei is calculated within the weak-potential approximation. Diffraction structures in the polarization correlations between the beam electron and the emitted photon are predicted for collision energies in the region 50–120 MeV if the photon is emitted at backward angles. The dynamical recoil plays a dominant role concerning the location and the shape of the structures. The target nuclei {sup 19}F, {sup 64}Zn and {sup 89}Y are investigated.

  19. Fusion and neutron transfer reactions with weakly bound nuclei within time-dependent and coupled channel approaches

    Science.gov (United States)

    Samarin, V. V.

    2016-05-01

    The time-dependent Schrödinger equation and the coupled channel approach based on the method of perturbed stationary two-center states are used to describe nucleon transfers and fusion in low-energy nuclear reactions. Results of the cross sections calculation for the formation of the 198Au and fusion in the 6He+197Au reaction and for the formation of the 65Zn in 6He+64Zn reaction agree satisfactorily with the experimental data near the barrier. The Feynman's continual integrals calculations for a few-body systems were used for the proposal of the new form of the shell model mean field for helium isotopes.

  20. Chromatographic zinc isotope separation by phenol formaldehyde benzo crown resin.

    Science.gov (United States)

    Ding, Xingcheng; Nomura, Masao; Suzuki, Tatsuya; Sugiyama, Yuichi; Kaneshiki, Toshitaka; Fujii, Yasuhiko

    2006-04-28

    New types of phenol formaldehyde resin having benzo crown as a functional group were synthesized and applied to zinc isotope chromatographic operation. Zinc adsorption and isotope separation capacities were dramatically improved by using phenol formaldehyde benzo-15-crown-5 resin. Zinc batch adsorption tests were performed by various dehydrated organic solvents. Separation coefficient, epsilon 8.1 x 10(-4) and height equivalent to a theoretical plate (HETP) 0.105 cm for the isotopic pair of 68Zn/64Zn in phenol formaldehyde benzo-15-crown-5 resin were obtained in the case of acetone as the solvent at 298+/-1K.

  1. Correlations between the fragmentation modes and light charged particles emission in heavy ion collisions

    CERN Document Server

    Zhang, Yingxun; Chen, Jixian; Wang, Ning; Zhao, Kai; Li, Zhuxia

    2015-01-01

    The correlations between the shape of rapidity distribution of the yield of light charged particles and the fragmentation modes in semi-peripheral collisions for $^{70}$Zn+$^{70}$Zn, $^{64}$Zn+$^{64}$Zn and $^{64}$Ni+$^{64}$Ni at the beam energy of 35MeV/nucleon are investigated based on ImQMD05 code. Our studies show there is an interplay between the binary, ternary and multi-fragmentation break-up modes. The binary and ternary break-up modes more prefer to emit light charged particles at middle rapidity and give larger values of $R_{yield}^{mid}$ compared with the multi-fragmentation break-up mode does. The reduced rapidity distribution for the normalized yields of p, d, t, $^3$He, $^4$He and $^6$He and the corresponding values of $R_{yield}^{mid}$ can be used to estimate the probability of multi-fragmentation break-up modes. By comparing to experimental data, our results illustrate that $\\ge$40\\% of the collisions events belong to the multi-fragmentation break-up mode for the reactions we studied.

  2. Search for double beta decay of zinc and tungsten with low background ZnWO{sub 4} crystal scintillators

    Energy Technology Data Exchange (ETDEWEB)

    Belli, P. [Dipartimento di Fisica, Universita di Roma ' Tor Vergata' and INFN, Sezione di Roma Tor Vergata, I-00133 Rome (Italy); Bernabei, R. [Dipartimento di Fisica, Universita di Roma ' Tor Vergata' and INFN, Sezione di Roma Tor Vergata, I-00133 Rome (Italy)], E-mail: rita.bernabei@roma2.infn.it; Cappella, F. [Dipartimento di Fisica, Universita di Roma ' La Sapienza' and INFN, Sezione di Roma, I-00185 Rome (Italy); Cerulli, R. [INFN, Laboratori Nazionali del Gran Sasso, 67010 Assergi (AQ) (Italy); Danevich, F.A. [Institute for Nuclear Research, MSP 03680 Kyiv (Ukraine); Grinyov, B.V. [Institute for Scintillation Materials, 61001 Kharkiv (Ukraine); Incicchitti, A. [Dipartimento di Fisica, Universita di Roma ' La Sapienza' and INFN, Sezione di Roma, I-00185 Rome (Italy); Kobychev, V.V.; Mokina, V.M.; Nagorny, S.S. [Institute for Nuclear Research, MSP 03680 Kyiv (Ukraine); Nagornaya, L.L. [Institute for Scintillation Materials, 61001 Kharkiv (Ukraine); Nisi, S. [INFN, Laboratori Nazionali del Gran Sasso, 67010 Assergi (AQ) (Italy); Nozzoli, F. [Dipartimento di Fisica, Universita di Roma ' Tor Vergata' and INFN, Sezione di Roma Tor Vergata, I-00133 Rome (Italy); Poda, D.V. [Institute for Nuclear Research, MSP 03680 Kyiv (Ukraine); Prosperi, D. [Dipartimento di Fisica, Universita di Roma ' La Sapienza' and INFN, Sezione di Roma, I-00185 Rome (Italy); Tretyak, V.I.; Yurchenko, S.S. [Institute for Nuclear Research, MSP 03680 Kyiv (Ukraine)

    2009-08-01

    Double beta processes in {sup 64}Zn, {sup 70}Zn, {sup 180}W, and {sup 186}W have been searched for with the help of large volume (0.1-0.7 kg) low background ZnWO{sub 4} crystal scintillators at the Gran Sasso National Laboratories of the INFN (Italy). The total measurement time exceeds ten thousand hours. New improved half-life limits on double electron capture and electron capture with positron emission in {sup 64}Zn have been set, in particular (all the limits are at 90% C.L.): T{sub 1/2}{sup 0{nu}}{sup 2{epsilon}}{>=}1.1x10{sup 20} yr, T{sub 1/2}{sup 2{nu}}{sup {epsilon}}{sup {beta}{sup +}}{>=}7.0x10{sup 20} yr, and T{sub 1/2}{sup 0{nu}}{sup {epsilon}}{sup {beta}{sup +}}{>=}4.3x10{sup 20} yr. In addition, new T{sub 1/2} bounds were set for different modes of 2{beta} processes in {sup 70}Zn, {sup 180}W, and {sup 186}W at the level of 10{sup 17}-10{sup 20} yr.

  3. Neutron activation of natural zinc samples at kT = 25 keV

    CERN Document Server

    Reifarth, R; Heil, M; Käppeler, F; Plag, R; Sonnabend, K; Uberseder, E

    2013-01-01

    The neutron-capture cross sections of 64Zn, 68Zn, and 70Zn have been measured with the activation technique in a quasistellar neutron spectrum corresponding to a thermal energy of kT = 25 keV. By a series of repeated irradiations with different experimental conditions, an uncertainty of 3% could be achieved for the 64Zn(n,g)65Zn cross section and for the partial cross section 68Zn(n,g)69Zn-m feeding the isomeric state in 69Zn. For the partial cross sections 70Zn(n,g)71Zn-m and 70Zn(n,g)71Zn-g, which had not been measured so far, uncertainties of only 16% and 6% could be reached because of limited counting statistics and decay intensities. Compared to previous measurements on 64,68Zn, the uncertainties could be significantly improved, while the 70Zn cross section was found to be two times smaller than existing model calculations. From these results Maxwellian average cross sections were determined between 5 and 100 keV. Additionally, the beta-decay half-life of 71Zn-m could be determined with significantly imp...

  4. Correlations with projectile-like fragments and emission order of light charged particles

    Science.gov (United States)

    Kohley, Z.; Bonasera, A.; Galanopoulos, S.; Hagel, K.; May, L. W.; McIntosh, A. B.; Stein, B. C.; Souliotis, G. A.; Tripathi, R.; Wuenschel, S.; Yennello, S. J.

    2012-10-01

    Correlations of midrapidity light charged particles (LCPs) and intermediate mass fragments (IMFs) with projectile-like fragments (PLFs) have been examined from the 35 MeV/u 70Zn+70Zn, 64Zn+64Zn, and 64Ni+64Ni reaction systems. A new method was developed to examine the flow of the particles with respect to the PLF. The invariant PLF-scaled flow allowed for the dynamics of the midrapidity Z=1-4 particles to be studied. Strong differences in the PLF-scaled flow were observed between the different isotopes. In particular, the most n-rich LCPs exhibited a negative PLF-scaled flow in comparison to the other LCPs. A classical molecular dynamics model and a three-body Coulomb trajectory simulation were both used to show that the PLF-scaled flow observable could be connected to the average order of emission of the LCPs. The experimental results suggest that the midrapidity region is preferentially populated with neutron-rich LCPs and Z=3-4 IMFs at a relatively early stage in the collision. The deuteron and 3He particles are emitted later followed, lastly, by protons and alphas. The average order of emission of the midrapidity LCPs was extracted from the constrained molecular dynamics simulations and showed good agreement with the emission order suggested by the experimental PLF-scaled flow results.

  5. Studying dispersions of ferroelectric nanopowders in dioctyl phthalate as dielectric media for capacitive electronic components

    Science.gov (United States)

    Gorokhovskii, A. V.; Gorshkov, N. V.; Burmistrov, I. N.; Goffman, V. G.; Tret'yachenko, E. V.; Sevryugin, A. V.; Fedorov, F. S.; Kovyneva, N. N.

    2016-06-01

    The electrical properties of dispersions of a powdered ferroelectric nanocomposite based on ilmenite (FeTiO3) and hollandite (K1.46Ti7.2Fe0.8O16) in dioctyl phthalate have been studied by impedance spectroscopy techniques in a frequency range of 10-1-106 Hz. The influence of stabilizing additives of cationic and anionic surfactants and iron acetylacetonate on the permittivity, conductivity, and dielectric losses was determined for dispersions containing 40 mass % of the solid composite. The influence of composition on the mechanisms of relaxation processes in the system is discussed.

  6. Spin and temperature dependence of nuclear deformation using alpha-gamma angular correlations

    International Nuclear Information System (INIS)

    Alpha-particle angular distributions with respect to the spin direction of residual nuclei have been measured in heavy-ion fusion reactions. The spin direction was determined by measuring the γ-ray angular distributions, for each event, using the spin spectrometer. α-particle anisotropies have been extracted for the compound nuclear systems: 110Sn*(94 MeV), 114Sn*(80 MeV), 138Nd*(82 MeV), 164Yb*(67 MeV) and 170Yb*(135 MeV) as a function of the α-particle energy and γ-ray multiplicity. The results are compared with statistical model calculations using transmission coefficients from a spherically symmetric optical model potential. The trend of the anisotropy coefficients below the evaporation Coulomb barrier is consistent with spherical emitting shapes in the case of the Sn* isotopes. Small deformation effects are suggested by the 138Nd* and 164Yb* data. The 170Yb* data indicate a large deformation which increases considerably with increasing spin. These results are in agreement with findings for similar systems in which the decay of the giant resonances built on excited states have been studied. 16 refs., 5 figs

  7. Collective and non-collective structures in nuclei of mass region A ≈ 125

    International Nuclear Information System (INIS)

    Generation of angular momentum in nuclei is a key question in nuclear structure studies. In single particle model, it is due to alignment of spin of individual nucleon available in the valence space, whereas coherent motion of nucleons are assumed in the collective model. The nuclei near the closed shell at Z = 50 with mass number A ≈ 120-125 represent ideal cases to explore the interplay between these competing mechanisms and the transition from non-collective to collective behavior or vice versa. Recent spectroscopic studies of nuclei in this region reveal several non-collective maximally aligned states representing the first kind of excitation mechanism, where 8-12 particles above the 114Sn align their spins to generate these states. Deformed rotational bands feeding the non-collective states in the spin range I=20-25 and excitation energies around 10 MeV have also been observed. Structure of the collective and non-collective states are discussed in the framework of Cranked-Nilsson-Strutinsky model

  8. Reactor production of 64Cu and 67Cu using enriched zinc target material

    International Nuclear Information System (INIS)

    Initial development work and trial irradiations were conducted to produce the in-demand medical isotopes 64Cu and 67Cu via the reactor-based fast neutron 64Zn(n,p)64Cu and 67Zn(n,p)67Cu reactions using enriched zinc targets. Boron-nitride shielded sample holders were used to reduce the thermal neutron flux to the zinc targets and diminish the production of undesired 65Zn. Irradiated oxide targets were dissolved and preliminary separations achieved copper yields of ∼95 % and zinc separations factors greater than 103 after one ion exchange pass. Further development would allow the production of mCi levels of 64Cu and 67Cu per irradiation, providing sufficient activity for small mammal research studies. (author)

  9. Diffusion studies in ZnTe for an active role of vacancies

    International Nuclear Information System (INIS)

    Investigations on the jump frequencies for various isotopes of cations and anions in ZnTe for an active role of vacancies are reported. Lattice dynamical calculations of diffusion are carried out using the scattering matrix formalism and reaction co-ordinates. The jump frequency and isotope effect for 126Te, 128Te, 64Zn, 66Zn, 68Zn are estimated for temperatures 1000, 1200, and 1500 K. The isotope effect in the case of Te diffusion is of the order of 50%. The diffusion of Zn in ZnTe can be explained lattice dynamically only by considering the contributions from various defects (single vacancies, Frenkel defect pairs). It can be concluded that Zn diffusion in ZnTe is different from Te diffusion in ZnTe

  10. A study on zinc isotope fractionation in a benzo crown resin/acetone system

    International Nuclear Information System (INIS)

    Zinc isotope fractionation has been studied in different cavities of crown ether resins that were synthesized in porous silica beads. Displacement chromatography was performed, as a breakthrough manner, in glass columns by feeding in a zinc chloride solution. From the mass analysis of effluents, the heavier isotopes of zinc were enriched at the beginning of the zinc adsorption band. The front maximum enrichment (1.0168), separation coefficient (8.1 x 10-4), and smaller HETP (0.205 cm) for the isotopic pair 68Zn/64Zn were obtained with the use of the benzo-15-crown-5 resin. Zinc isotope fractionation was obviously affected by the cavity size of the crown ethers. (author)

  11. Zinc isotope separation by phenol formaldehyde type 15-crown-5 resin in organic solvents

    International Nuclear Information System (INIS)

    Zinc adsorption and isotope separation by newly synthesized benzo-15-crown-5 resin was evaluated using various solvents. This resin was synthesized in the pores of silica beads for chromatography use. Larger adsorption of zinc was obtained in the case of acetic acid derivatives than in protic solvent such as water and alcohol by the batch treatment. The displacement chromatography was conducted to study zinc isotope separation. The isotope separation coefficient ε=0.32x10-3, 0.69x10-3 and HETP=0.2268, 0.3968 cm were determined for isotopic pair of 68Zn/64Zn at 25degC by five meters migration experiment using methyl isobutyl ketone and acetic acid, respectively. The improvement of enrichment ratio is very small between 1 and 5 m migration. Hydrogen chloride and/or water obviously reduce zinc adsorption to this resin. (author)

  12. The $^{63}$Ni(n,$\\gamma$) cross section measured with DANCE

    CERN Document Server

    Weigand, M; Couture, A; Göbel, K; Heftrich, T; Jandel, M; Käppeler, F; Lederer, C; Kivel, N; Korschinek, G; Krticka, M; O'Donnell, J M; Ostermöller, J; Plag, R; Reifarth, R; Schumann, D; Ullmann, J L; Wallner, A

    2015-01-01

    The neutron capture cross section of the s-process branch nucleus $^{63}$Ni affects the abundances of other nuclei in its region, especially $^{63}$Cu and $^{64}$Zn. In order to determine the energy dependent neutron capture cross section in the astrophysical energy region, an experiment at the Los Alamos National Laboratory has been performed using the calorimetric 4$\\pi$ BaF$_2$ array DANCE. The (n,$\\gamma$) cross section of $^{63}$Ni has been determined relative to the well known $^{197}$Au standard with uncertainties below 15%. Various $^{63}$Ni resonances have been identified based on the Q-value. Furthermore, the s-process sensitivity of the new values was analyzed with the new network calculation tool NETZ.

  13. 63Ni (n ,γ ) cross sections measured with DANCE

    Science.gov (United States)

    Weigand, M.; Bredeweg, T. A.; Couture, A.; Göbel, K.; Heftrich, T.; Jandel, M.; Käppeler, F.; Lederer, C.; Kivel, N.; Korschinek, G.; Krtička, M.; O'Donnell, J. M.; Ostermöller, J.; Plag, R.; Reifarth, R.; Schumann, D.; Ullmann, J. L.; Wallner, A.

    2015-10-01

    The neutron capture cross section of the s -process branch nucleus 63Ni affects the abundances of other nuclei in its region, especially 63Cu and 64Zn. In order to determine the energy-dependent neutron capture cross section in the astrophysical energy region, an experiment at the Los Alamos National Laboratory has been performed using the calorimetric 4 π BaF2 array DANCE. The (n ,γ ) cross section of 63Ni has been determined relative to the well-known 197Au standard with uncertainties below 15%. Various 63Ni resonances have been identified based on the Q value. Furthermore, the s -process sensitivity of the new values was analyzed with the new network calculation tool NETZ.

  14. Thermal properties of zinc isotopes in the static path approximation

    International Nuclear Information System (INIS)

    Employing a quadrupole-quadrupole interaction Hamiltonian in the so-called static path approximation, which is based on path integration in the space of single-particle potential fields, we have calculated the excitation energy, level density, and level density parameter of some of the zinc isotopes with neutron numbers, N=34, 40, 44, and 46 at finite temperatures, T≤2.0 MeV. Using a cranking Hamiltonian (with rotation about the X axis) in the same approach we have also studied the behavior of the moment of inertia as a function of rotational frequency (ω) and temperature for 64Zn, taking it as an illustrative example. At low temperature (T∼0.5 MeV) the effect of rotation alignment is seen at ω∼1.0 MeV whereas at T∼2.0 MeV the moment of inertia becomes almost independent of ω, indicative of a rigid body behavior

  15. Application of Zn + p reactions for production of copper radioisotopes for medical studies

    Energy Technology Data Exchange (ETDEWEB)

    Szelecsenyi, F.; Kovacs, Z. [Institute of Nuclear Research of the Hungarian Academy of Sciences (ATOMKI), Debrecen (Hungary); Steyn, G.F.; Van der Walt, T.N.; Vermeulen, C.; Van der Meulen, N.P.; Dolley, S.G. [iThemba Laboratory for Accelerator Based Sciences (South Africa); Suzuki, K.; Mukai, K. [National Institute of Radiological Sciences, Chiba (Japan)

    2008-07-01

    The production possibility of four medically important copper radioisotopes via Zn + p reactions was studied up to 80 MeV. Based on experimentally evaluated excitation function curves of the {sup 64}Zn(p,x){sup 61}Cu, {sup nat}Zn(p,x){sup 62}Zn {yields} {sup 62}Cu; {sup 66}Zn(p,2pn){sup 64}Cu, {sup 68}Zn(p,x){sup 64}Cu and {sup 68}Zn(p,2p){sup 67}Cu reactions, production energy windows are recommended for the {sup 61}Cu, {sup 62}Cu, {sup 64}Cu and {sup 67}Cu isotopes. The available yields for these radioisotopes as well as the predicted yields of the major contaminants are also presented, it is concluded that the Zn + p route can produce sufficient activity of {sup 61,62,64,67}Cu (with low contamination level) to be considered for practical purposes.

  16. ZnWO_4 crystals as detectors for double beta decay and dark matter experiments

    CERN Document Server

    Danevich, F A; Nagorny, S S; Poda, D V; Tretyak, V I; Yurchenko, S S; Zdesenko, Y G; Zdesenko, Yu.G.

    2004-01-01

    Energy resolution, alpha/beta ratio, and the pulse shape discrimination ability of the ZnWO_4 crystal scintillators were studied. The radioactive contamination of a ZnWO_4 crystal was investigated in the Solotvina Underground Laboratory. Possibilities to apply ZnWO_4 crystals for the dark matter and double beta decay searches are discussed. New improved half-life limits on double beta decay in zinc isotopes were established, in particular, for EC\\beta^+ decay of 64-Zn as: T_1/2^2nu > 8.9 10^18 yr and T_1/2^0nu > 3.6 10^18 yr, both at 68% CL.

  17. ZnWO{sub 4} crystals as detectors for 2{beta} decay and dark matter experiments

    Energy Technology Data Exchange (ETDEWEB)

    Danevich, F.A. [Institute for Nuclear Research, Prospekt Nauki 47, MSP 03680 Kiev (Ukraine)]. E-mail: danevich@kinr.kiev.ua; Kobychev, V.V. [Institute for Nuclear Research, Prospekt Nauki 47, MSP 03680 Kiev (Ukraine); Nagorny, S.S. [Institute for Nuclear Research, Prospekt Nauki 47, MSP 03680 Kiev (Ukraine); Poda, D.V. [Institute for Nuclear Research, Prospekt Nauki 47, MSP 03680 Kiev (Ukraine); Tretyak, V.I. [Institute for Nuclear Research, Prospekt Nauki 47, MSP 03680 Kiev (Ukraine); Yurchenko, S.S. [Institute for Nuclear Research, Prospekt Nauki 47, MSP 03680 Kiev (Ukraine); Zdesenko, Yu.G. [Institute for Nuclear Research, Prospekt Nauki 47, MSP 03680 Kiev (Ukraine)

    2005-06-01

    Energy resolution, {alpha}/{beta} ratio, and the pulse shape discrimination ability of the ZnWO{sub 4} crystal scintillators were studied. The radioactive contamination of a ZnWO{sub 4} crystal was investigated in the Solotvina Underground Laboratory. Possibilities to apply ZnWO{sub 4} crystals for the dark matter and double beta decay searches are discussed. New improved half-life limits on double beta decay in zinc isotopes were established, in particular, for -bar {beta}{sup +} decay of {sup 64}Zn as: T{sub 1/2}{sup 2{nu}}>=8.9x10{sup 18} years and T{sub 1/2}{sup 0{nu}}>=3.6x10{sup 18} years, both at 68% CL.

  18. Zinc isotope ratios of bones and teeth as new dietary indicators: results from a modern food web (Koobi Fora, Kenya)

    Science.gov (United States)

    Jaouen, Klervia; Beasley, Melanie; Schoeninger, Margaret; Hublin, Jean-Jacques; Richards, Michael P.

    2016-05-01

    In order to explore the possibilities of using zinc (Zn) stable isotope ratios as dietary indicators, we report here on the measurements of the ratio of stable isotopes of zinc (66Zn/64Zn, expressed here as δ66Zn) in bioapatite (bone and dental enamel) of animals from a modern food web in the Koobi Fora region of the Turkana Basin in Kenya. We demonstrate that δ66Zn values in both bone and enamel allow a clear distinction between carnivores and herbivores from this food web. Differences were also observed between browsers and grazers as well as between carnivores that consumed bone (i.e. hyenas) compared to those that largely consume flesh (i.e. lions). We conclude that Zn isotope ratio measurements of bone and teeth are a new and promising dietary indicator.

  19. Market of stable isotopes produced by gas centrifuges: status and prospects

    International Nuclear Information System (INIS)

    The major consumers on the market of enriched stable isotopes traditionally include nuclear industry, medicine and life sciences, and new technical and scientific applications. The beginning of new millennium has brought the wide application of enriched stable isotopes in fundamental physics experiments that needed tens and hundreds kilograms of various stable isotopes of middle and heavy masses. In addition, the needs of nuclear power industry to develop materials to be used in nuclear power plants capable to reduce formation of radioactive by-products and to prevent cracking in certain metallic components led to production of big amounts of different compounds of zinc depleted with the 64Zn isotope. All these problems have been solved successfully by means of the gas centrifuge technology applied for separation of isotopes other than uranium. As a result the market of enriched/depleted stable isotopes has changed radically in recent years. (authors)

  20. Nuclear level densities of 64,66Zn from neutron evaporation

    Science.gov (United States)

    Ramirez, A. P. D.; Voinov, A. V.; Grimes, S. M.; Schiller, A.; Brune, C. R.; Massey, T. N.; Salas-Bacci, A.

    2013-12-01

    Double differential cross sections of neutrons from d+63,65Cu reactions have been measured at deuteron energies of 6 and 7.5 MeV. The cross sections measured at backward angles have been compared to theoretical calculations in the framework of the statistical Hauser-Feshbach model. Three different level density models were tested: the Fermi-gas model, the Gilbert-Cameron model, and the microscopic approach through the Hartree-Fock-Bogoliubov method (HFBM). The calculations using the Gilbert-Cameron model are in best agreement with our experimental data. Level densities of the residual nuclei 64Zn and 66Zn have been obtained from statistical neutron evaporation spectra. The angle-integrated cross sections have been analyzed with the exciton model of nuclear reaction.

  1. Zinc isotope ratios of bones and teeth as new dietary indicators: results from a modern food web (Koobi Fora, Kenya)

    Science.gov (United States)

    Jaouen, Klervia; Beasley, Melanie; Schoeninger, Margaret; Hublin, Jean-Jacques; Richards, Michael P.

    2016-01-01

    In order to explore the possibilities of using zinc (Zn) stable isotope ratios as dietary indicators, we report here on the measurements of the ratio of stable isotopes of zinc (66Zn/64Zn, expressed here as δ66Zn) in bioapatite (bone and dental enamel) of animals from a modern food web in the Koobi Fora region of the Turkana Basin in Kenya. We demonstrate that δ66Zn values in both bone and enamel allow a clear distinction between carnivores and herbivores from this food web. Differences were also observed between browsers and grazers as well as between carnivores that consumed bone (i.e. hyenas) compared to those that largely consume flesh (i.e. lions). We conclude that Zn isotope ratio measurements of bone and teeth are a new and promising dietary indicator. PMID:27189145

  2. Mediating conducting polymer growth within hydrogels by controlling nucleation

    Directory of Open Access Journals (Sweden)

    A. J. Patton

    2015-01-01

    Full Text Available This study examines the efficacy of primary and secondary nucleation for electrochemical polymerisation of conductive polymers within poly(vinyl alcohol methacrylate hydrogels. The two methods of nucleation investigated were a primary heterogeneous mechanism via introduction of conductive bulk metallic glass (Mg64Zn30Ca5Na1 particles and a secondary mechanism via introduction of “pre-polymerised” conducting polymer within the hydrogel (PEDOT:PSS. Evidence of nucleation was not seen in the bulk metallic glass loaded gels, however, the PEDOT:PSS loaded gels produced charge storage capacities over 15 mC/cm2 when sufficient polymer was loaded. These studies support the hypothesis that secondary nucleation is an efficient approach to producing stand-alone conducting hydrogels.

  3. Reaction mechanisms in collisions induced by 8B beam close to the barrier

    CERN Multimedia

    The aim of the proposed experiment is to investigate on the reaction dynamics of proton-halo induced collisions at energies around the Coulomb barrier where coupling to continuum effects are expected to be important. We propose to measure $^{8}$B+$^{64}$Zn elastic scattering angular distribution together with the measurement, for the first time, of p-$^{7}$Be coincidences coming from transfer and/or break-up of $^{8}$B. The latter will allow a better understanding of the relative contribution of elastic $\\textit{vs}$ non-elastic break-up in reactions induced by extremely weakly-bound nuclei. We believe that with the availability of the post accelerated $^{8}$B beam at REX-ISOLDE we will be able to collect for the first time high quality data for the study of such an important topic.

  4. Neutrinoless double positron decay and positron emitting electron capture in the interacting boson model

    CERN Document Server

    Barea, J; Iachello, F

    2015-01-01

    Neutrinoless double-$\\beta$ decay is of fundamental importance for determining the neutrino mass. Although double electron ($\\beta^-\\beta^-$) decay is the most promising mode, in very recent years interest in double positron ($\\beta^+\\beta^+$) decay, positron emitting electron capture ($EC\\beta^+$), and double electron capture ($ECEC$) has been renewed. We present here results of a calculation of nuclear matrix elements for neutrinoless double-$\\beta^+$ decay and positron emitting electron capture within the framework of the microscopic interacting boson model (IBM-2) for $^{58}$Ni, $^{64}$Zn, $^{78}$Kr, $^{96}$Ru, $^{106}$Cd, $^{124}$Xe, $^{130}$Ba, and $^{136}$Ce decay. By combining these with a calculation of phase space factors we calculate expected half-lives.

  5. Experimental reconstruction of primary fragments with kinematical focusing method

    International Nuclear Information System (INIS)

    An experimental method was used to evaluate the primary isotope yields of semi-central collisions in the reaction system 64Zn+112Sn at 40A MeV, The characteristic nature of the hot nuclear matter at the time of the isotope formation was studied. The multiplicities of light particles (LPs) associated with intermediate mass fragments (IMFs) were determined experimentally by using a kinematical focusing technique. The primary isotope distributions, reconstructed by a Monte Carlo method, were compared with those of the AMD-Gemini simulations. ac/T=0.11 and asym/T=3.34 were extracted from the reconstructed primary fragments yield. These are consistent with those of the primary fragments of the AMD simulation. (authors)

  6. Anomalous behaviour of transition probabilities in 75Kr

    International Nuclear Information System (INIS)

    The two collective bands of 75Kr have been extended up to spin 21/2 using the compound reactions 64Zn(14N, p2n)75Kr and 50Cr(28Si, 2pn)75Kr. Spins and parities were assigned from neutron-gated γ angular-distributions and excitation functions using the OSIRIS Anti Compton Spectrometer. The bands are interpreted to be built on well-deformed Nilsson states: [442]5/2 and [301]3/2. Energies and mixing ratios for both bands can be reproduced within the 'single particle and rotor' model, while the experimental Q0(I->I-1)/Q0(I->I-2) ratios exhibit large deviations by a factor 4 to 6 from theoretical values. (orig.)

  7. Nuclear structure effects in high-energy bremsstrahlung from spin-0 and spin-1/2 nuclei

    Energy Technology Data Exchange (ETDEWEB)

    Jakubassa-Amundsen, Doris [University of Munich (Germany)

    2014-07-01

    Bremsstrahlung from relativistic spin-polarized electrons colliding with inert nuclei is calculated by taking into account the nuclear form factors and the kinematical recoil. For the spin-1/2 nuclei additional contributions from the anomalous magnetic moment and the dynamical recoil are considered. Electron bremsstrahlung is described with the help of semirelativistic wavefunctions while nuclear bremsstrahlung, when present, is treated within the Born approximation. The triply differential bremsstrahlung cross section is integrated over the electron scattering angle to study the polarization correlations between the beam electron and the emitted photon. Results are shown for 20-120 MeV electrons colliding with protons, 19F, 64Zn and 89Y. It is also attempted to explain the background in electron spectra from nuclear excitation in terms of bremsstrahlung. As an example the 180 degree spectrum from exciting the giant M2 resonance in 90Zr by 42.7 MeV electrons is analyzed.

  8. Neutron capture cross section of unstable 63Ni implications for stellar nucleosynthesis

    CERN Document Server

    Lederer, C; Altstadt, S; Andrzejewski, J; Audouin, L; Barbagallo, M; Becares, V; Becvar, F; Belloni, F; Berthoumieux, E; Billowes, J; Boccone, V; Bosnar, D; Brugger, M; Calviani, M; Calvino, F; Cano-Ott, D; Carrapico, C; Cerutti, F; Chiaveri, E; Chin, M; Colonna, N; Cortes, G; Cortes-Giraldo, M.A; Diakaki, M; Domingo-Pardo, C; Duran, I; Dressler, R; Dzysiuk, N; Eleftheriadis, C; Ferrari, A; Fraval, K; Ganesan, S; Garcia, A R; Giubrone, G; Gomez-Hornillos, M B; Goncalves, I F; Gonzalez-Romero, E; Griesmayer, E; Guerrero, C; Gunsing, F; Gurusamy, P; Jenkins, D G; Jericha, E; Kadi, Y; Kappeler, F; Karadimos, D; Kivel, N; Koehler, P; Kokkoris, M; Korschinek, G; Krticka, M; Kroll, J; Langer, C; Leeb, H; Leong, L S; Losito, R; Manousos, A; Marganiec, J; Martinez, T; Mastinu, P F; Mastromarco, M; Meaze, M; Mendoza, E; Mengoni, A; Milazzo, P M; Mingrone, F; Mirea, M; Mondelaers, W; Paradela, C; Pavlik, A; Perkowski, J; Pignatari, M; Plompen, A; Praena, J; Quesada, J M; Rauscher, T; Reifarth, R; Riego, A; Roman, F; Rubbia, C; Sarmento, R; Schillebeeckx, P; Schmidt, S; Schumann, D; Tagliente, G; Tain, J L; Tarrio, D; Tassan-Got, L; Tsinganis, A; Valenta, S; Vannini, G; Variale, V; Vaz, P; Ventura, A; Versaci, R; Vermeulen, M J; Vlachoudis, V; Vlastou, R; Wallner, A; Ware, T; Weigand, M; Weiss, C; Wright, T J; Zugec, P

    2013-01-01

    The $^{63}$Ni($n, \\gamma$) cross section has been measured for the first time at the neutron time-of-flight facility n\\_TOF at CERN from thermal neutron energies up to 200 keV. In total, capture kernels of 12 (new) resonances were determined. Maxwellian Averaged Cross Sections were calculated for thermal energies from kT = 5 keV to 100 keV with uncertainties around 20%. Stellar model calculations for a 25 M$_\\odot$ star show that the new data have a significant effect on the $s$-process production of $^{63}$Cu, $^{64}$Ni, and $^{64}$Zn in massive stars, allowing stronger constraints on the Cu yields from explosive nucleosynthesis in the subsequent supernova.

  9. Realization of a gamma multiplicity filter and gamma multiplicity measurements

    International Nuclear Information System (INIS)

    A gamma multiplicity filter for the study of reaction mechanism has been realised. It's composed of six NaI(Tl) counters. The flexibility of the geometry allows many configurations. This set up has been tested with gamma radioactive sources and with the 252Cf source to resolve problems of gamma-efficiency of the NaI(Tl) counters and the contamination of neutrons in these detectors. A logical electronic unit (Encodeur) has been constructed and the around electronic has been developped. This gamma multiplicity filter has been coupled with a detector of high resolution Ge(Li), and used in two reactions: 12C + 55Mn at E(12C) = 54 MeV; α + 63Cu at E(α) = 52 MeV. The dominant process is the fusion-evaporation. The compound nucleus 67Ga, is formed at the same excitation energy. The values of multiplicities Msub(γ) have been extracted using a program based on the formalism of W.J. Ockels. The fractionalization of the angular momentum is well observed for some residual nuclei (63Zn, 64Zn, 65Zn), and for each residual nucleus, the average gamma multiplicity is lower with projectile α than that with projectile 12C. For the most strongly output channel p2n, an entry point for the 64Zn has been determined in the reactions. All these observations are in good agreement with those published, in the same region (f-p shell) of nuclei. This set up can be coupled with different central detector as, ''X'', neutrons charged particles detectors, and will be used with the new machine SARA to make a systematic study of transfer of angular momentum to the fragments at 30 MeV/A

  10. Dependence of strength og polycrystalline ferroelectric TsTS-22 on loading velocity

    International Nuclear Information System (INIS)

    The strength of polycrystalline ferroelectric Pb0.95Sr0,05(Zr0,46Ti0.54)O3 + 0.78 wt. % Cr2O3 (TsTS-22) by bending is measured within the range of loading velocities of 5 x 10-2 MPa/s and temperatures of 293-873 K (including Curie temperature Tc = 593 K). The interpretation of results is presented within the frames of the relaxation model of the friable destruction. The effective activation volume of destruction process is determined with application of the strength dependence on the sample loading velocity under various temperatures. Changes in the activation features in the phase transition area are discussed

  11. Onset of collectivity in the ground-state band of 50Cr

    International Nuclear Information System (INIS)

    Transient field precessions of the first excited states in 50Cr have been measured. The states were excited by the inverse 12C(40Ca, 2p)50Cr reaction and the recoil nuclei traversed a thick gadolinium foil, where they experienced the rotation. The observed precessions, for the 2+,4+,6+,8+ states of the ground-state band, were equal within experimental error indicating these states have g factors similar to that of the 2+ state value of 0.55±0.10 measured previously. This feature is contrary to the predictions of the shell model and suggests a higher collectivity for the ground-state band. Limited results were also obtained for the cross conjugate nucleus 46Ti supporting this conclusion

  12. Nuclear structure theory in spin- and number-conserving quasiparticle configuration spaces: First applications

    Energy Technology Data Exchange (ETDEWEB)

    Schmid, K.W.; Gruemmer, F.; Faessler, A.

    1984-01-01

    In the first part of the present series of two papers we discussed several nuclear structure models all working in configuration spaces consisting of spin- and number-projected quasiparticle determinants. In the present paper a particular version of the numerically simplest of these models is presented. This model approximates the nuclear wave functions by linear combinations of the angular momentum- and particle number-projected Hartree-Fock-Bogoliubov vacuum and the equally spin- and number-projected two quasiparticle excitations with respect to it. The model allows the use of realistic two body interactions and rather large model spaces. It can hence be applied to a large number of nuclear structure problems in various mass regions. First applications have been performed for the nuclei /sup 20/Ne, /sup 22/Ne, /sup 46/Ti, and /sup 164/Er. In all these cases the results are very encouraging.

  13. Isospin aspects in nuclear reactions involving Ca beams at 25 MeV/nucleon

    Energy Technology Data Exchange (ETDEWEB)

    Lombardo, I., E-mail: ilombardo@lns.infn.it; Agodi, C.; Alba, R.; Amorini, F.; Anzalone, A. [INFN Laboratori Nazionali del Sud (Italy); Auditore, L. [Universita di Messina, and INFN-Gr. Coll. Messina, Dipartimento di Fisica (Italy); Berceanu, I. [Institute for Physics and Nuclear Engineering (Romania); Cardella, G. [INFN, Sezione di Catania (Italy); Cavallaro, S. [INFN Laboratori Nazionali del Sud (Italy); Chatterjee, M. B. [Saha Institute of Nuclear Physics (India); Filippo, E. De [INFN, Sezione di Catania (Italy); Di Pietro, A.; Figuera, P. [INFN Laboratori Nazionali del Sud (Italy); Giuliani, G.; Geraci, E.; Grassi, L. [Dipartimento di Fisica e Astronomia Universita di Catania (Italy); Grzeszczuk, A. [University of Silesia, Institute of Physics (Poland); Han, J. [INFN Laboratori Nazionali del Sud (Italy); La Guidara, E. [INFN, Sezione di Catania (Italy); Lanzalone, G. [INFN Laboratori Nazionali del Sud (Italy); and others

    2011-11-15

    Isospin dependence of dynamical and thermodynamical properties observed in reactions {sup 40}Ca+ {sup 40,48}Ca and {sup 40}Ca + {sup 46}Ti at 25 MeV/nucleon has been studied. We used the CHIMERA multi-detector array. Strong isospin effects are seen in the isotopic distributions of light nuclei and in the competition between different reaction mechanisms in semi-central collisions. We will show also preliminary results obtained in nuclear collision {sup 48}Ca + {sup 48}Ca at 25MeV/nucleon, having very high N/Z value in the entrance channel (N/Z = 1.4). The enhancement of evaporation residue production confirms the strong role played by the N/Z degree of freedom in nuclear dynamics.

  14. Isospin Dependence of Incomplete Fusion Reactions at 25 Mev/a

    CERN Document Server

    Amorini, F; Giuliani, G; Papa, M; Agodi, C; Alba, R; Anzalone, A; Berceanu, I; Cavallaro, S; Chatterjee, M B; Coniglione, R; De Filippo, E; Di Pietro, A; Geraci, E; Grassi, L; Grzeszczuk, A; Figuera, P; La Guidara, E; Lanzalone, G; Neindre, N Le; Lombardo, I; Maiolino, C; Pagano, A; Pirrone, S; Politi, G; Pop, A; Porto, F; Rizzo, F; Russotto, P; Santonocito, D; Sapienza, P; Verde, G

    2008-01-01

    40Ca+40,48Ca,46Ti reactions at 25 MeV/A have been studied using the 4p CHIMERA detector. An isospin effect on the competition between incomplete fusion and dissipative binary reaction mechanisms has been observed. The probability of producing a compound system is observed to be lower in the case of N=Z colliding systems as compared to the case of reactions induced on the more neutron rich 48Ca target. Predictions based on CoMD-II calculations show that the competition between fusion-like and dissipative reactions, for the selected centrality, can strongly constraint the parameterization of symmetry energy and its density dependence in the nuclear equation of state.

  15. Synthesis of amorphous Ti-Al alloys by mechanical alloying of elemental powders

    Institute of Scientific and Technical Information of China (English)

    张俊红; 黄伯云; 贺跃辉; 周科朝; 刘咏

    2002-01-01

    Blended elemental powders with the nominal compositions (mole fraction, %) of Ti54Al46, Ti52Al48 and Ti50Al50 were mechanically alloyed in a planetary ball milling system for up to 100h.The structure evolution in these powders was characterized by scanning electron microscope, X-ray diffraction and differential thermal a nalysis techniques. It was found that elemental powders were progressively trans formed into nanocrystalline Ti(Al) supersaturated solid solution, then into amor phous phase. With increasing Al content, the formation of a fully Ti(Al) supersa turated solid solution and amorphous phase were accelerated, which are attributed to the fine grain size. And the grain size condition for formation of amorpho us phase in this system is ≤16 nm.

  16. Evaluation of the (n,p) cross sections of natural Ti and its isotopes from thresholds to 20 MeV

    International Nuclear Information System (INIS)

    The titanium isotopes (n,p) cross sections are based upon renormalized experimental data or deduced from statistical model calculations where measurements were not available. Some of these cross sections, notably the 46Ti (n,p), 47Ti (n,p) and 48Ti (n,p), which find wide use as dosimetry indicators, are compared here with the corresponding ENDF/BIV dosimetry file data. The (n,p) elemental cross section is constructed from the weighted isotopic components. Our evaluation and the corresponding ENDF/BIV data are compared showing the great difference between both results, especially below 10 MeV. Moreover the new data exhibit some structure characteristics of the 47Ti (n,p) cross section. The present Ti (n,p) data are intended to be included in the ENDF/BV evaluation

  17. Angular momentum projection of cranked Hartree-Fock states: Application to terminating bands in A∼44 nuclei

    International Nuclear Information System (INIS)

    We present the first systematic calculations based on the angular momentum projection of cranked Slater determinants. We propose the Iy→I scheme, by which one projects the angular momentum I from the one-dimensional cranked state constrained to the average spin projection of y>=I. Calculations performed for the rotational band in 46Ti show that the AMP Iy→I scheme offers a natural mechanism for correcting the cranking moment of inertia at low spins and shifting the terminating state up by ∼2 MeV, in accordance with data. We also apply this scheme to high-spin states near the band termination in A∼44 nuclei and compare results thereof with experimental data, shell-model calculations, and results of the approximate analytical symmetry-restoration method proposed previously

  18. Zinc isotope fractionation during adsorption on calcite

    Science.gov (United States)

    Dong, S.; Wasylenki, L. E.

    2013-12-01

    Zinc is an important element as a nutrient in the marine biosphere. However, our understanding of its biogeochemical cycling in the oceans is relatively limited. The Zn stable isotope system holds the promise of providing novel insights, since published Zn isotopic values for various natural samples reveal significant fractionations in the marine environment. Surface seawater, basalts, shales, deep-sea clay sediments, sediment trap material, bulk plankton and zooplankton samples, and eolian dust fall within a tight range (δ66/64Zn from -0.1 to 0.5‰), but modern ferromanganese crusts (δ66/64Zn from 0.5 to 1.2‰), as well as carbonates (δ66/64Zn from 0.3 to 1.4‰), are notably enriched in heavy Zn isotopes [1-4]. In this study we seek to constrain the mechanism by which carbonates are enriched in heavier isotopes. In particular, we have conducted experiments to quantify isotope fractionation during adsorption of Zn onto the surfaces of calcite crystals that are in equilibrium with solution. The adsorption experiments were carried out in a series of small-volume batch reactions in a clean laboratory environment, using high-purity reagents and calcite seed crystals. The calcite was equilibrated with the solution prior to addition of Zn at atmospheric CO2 pressure (i.e., in air) for 5 days until a stable pH of 8.3 was reached. Later, a small aliquot of dissolved ZnCl2 was added such that the solution remained undersaturated with respect to hydrozincite. Experimental duration varied among the replicates from 6 to 144 hours, and then all solids and solutions were separated by filtration, purified by ion exchange chromatography, and analyzed by MC-ICP-MS. Zn adsorbed on calcite is isotopically heavier than in the co-existing solutions, with Δ68/66Zncalcite-solution of approximately 0.3‰. The variation of Δ68/66Zncalcite-solution beyond 24 hours is insignificant, so we infer that isotopic equilibrium is reached by this time. Previous work strongly suggests that a

  19. Calculation and measurement of helium generation and solid transmutations in Cu-Zn-Ni alloys

    Energy Technology Data Exchange (ETDEWEB)

    Greenwood, L.R.; Oliver, B.M.; Garner, F.A. [Pacific Northwest National Lab., Richland, WA (United States); Muroga, T. [National Inst. of Fusion Science, Nagoya (Japan)

    1998-03-01

    A method was recently proposed by Garner and Greenwood that would allow the separation of the effects of solid and gaseous transmutation for Cu-Zn-Ni alloys. Pure copper produces zinc and nickel during neutron irradiation. {sup 63}Cu transmutes to {sup 64}Ni and {sup 64}Zn, in about a 2-to-1 ratio, and {sup 65}Cu transmutes to {sup 66}Zn. The {sup 64}Zn further transmutes to {sup 65}Zn which has been shown to have a high thermal neutron (n,{alpha}) cross-section. Since a three-step reaction sequence is required for natural copper, the amount of helium produced is much smaller than would be produced for the two-step, well-known {sup 58}Ni (n,{gamma}) {sup 59}Ni (n,{alpha}) reaction sequence. The addition of natural Zn and Ni to copper leads to greatly increased helium production in neutron spectra with a significant thermal component. Using a suitable Cu-Zn-Ni alloy matrix and comparative irradiation of thermal neutron-shielded and unshielded specimens, it should be possible to distinguish the separate influences of the solid and gaseous transmutants. Whereas helium generation rates have been previously measured for natural nickel and copper, they have not been measured for natural Zn or Cu-Ni-Zn alloys. The (N,{alpha}) cross section for {sup 65}Zn was inferred from helium measurements made with natural copper. By comparing helium production in Cu and Cu-Zn alloys, this cross section can be determined more accurately. In the current study, both the solid and helium transmutants were measured for Cu, Cu-5Ni, Cu-3.5Zn and Cu-5Ni-2Zn, irradiated in each of two positions in the HFIR JP-23 test. Highly accurate helium measurements were performed on these materials by isotope dilution mass spectrometry using a facility that was recently moved from Rockwell International to PNNL. It is shown that both the helium and solid transmutants for Cu-zn-Ni alloys can be calculated with reasonable certainty, allowing the development of a transmutation experiment as proposed by

  20. Study of angular momentum variation due to entrance channel effect in heavy ion fusion reactions

    Science.gov (United States)

    Kumar, Ajay

    2014-05-01

    A systematic investigation of the properties of hot nuclei may be studied by detecting the evaporated particles. These emissions reflect the behavior of the nucleus at various stages of the deexcitation cascade. When the nucleus is formed by the collision of a heavy nucleus with a light particle, the statistical model has done a good job of predicting the distribution of evaporated particles when reasonable choices were made for the level densities and yrast lines. Comparison to more specific measurements could, of course, provide a more severe test of the model and enable one to identify the deviations from the statistical model as the signature of other effects not included in the model. Some papers have claimed that experimental evaporation spectra from heavy-ion fusion reactions at higher excitation energies and angular momenta are no longer consistent with the predictions of the standard statistical model. In order to confirm this prediction we have employed two systems, a mass-symmetric (31P+45Sc) and a mass-asymmetric channel (12C+64Zn), leading to the same compound nucleus 76Kr* at the excitation energy of 75 MeV. Neutron energy spectra of the asymmetric system (12C+64Zn) at different angles are well described by the statistical model predictions using the normal value of the level density parameter a = A/8 MeV-1. However, in the case of the symmetric system (31P+45Sc), the statistical model interpretation of the data requires the change in the value of a = A/10 MeV-1. The delayed evolution of the compound system in case of the symmetric 31P+45Sc system may lead to the formation of a temperature equilibrated dinuclear complex, which may be responsible for the neutron emission at higher temperature, while the protons and alpha particles are evaporated after neutron emission when the system is sufficiently cooled down and the higher g-values do not contribute in the formation of the compound nucleus for the symmetric entrance channel in case of charged

  1. Effects of thermal treatment and depth profiling analysis of solution processed bulk-heterojunction organic photovoltaic cells.

    Science.gov (United States)

    Mbule, Pontsho S; Swart, Hendrik C; Ntwaeaborwa, Odireleng M

    2014-12-15

    We report the use of solution processed zinc oxide (ZnO) nanoparticles as a buffer layer inserted between the top metal electrode and the photo-active layer in bulk-heterojunction (BHJ) organic solar cell (OSC) devices. The photovoltaic properties were compared for devices annealed before (Device A) or after (Device B) the deposition of the Al top electrode. The post-annealing treatment was shown to improve the power conversion efficiency up to 2.93% and the fill factor (FF) up to 63% under AM1.5 (100mW/cm(2)) illumination. We performed the depth profile/interface analysis and elemental mapping using the time-of-flight secondary ion mass spectrometry (TOF-SIMS). Signals arising from (27)Al, (16)O, (12)C, (32)S, (64)Zn, (28)Si, (120)Sn and (115)In give an indication of successive deposition of Al, ZnO, P3HT:PCBM and PEDOT:PSS layers on ITO coated glass substrates. Furthermore, we discuss the surface imaging and visualize the chemical information on the surface of the devices.

  2. The measurement of the isotope ratios and concentrations of zinc by thermal ionization mass spectrometry using double isotope dilution

    International Nuclear Information System (INIS)

    The isotope ratios and concentrations of zinc are measured by silicagel-thermal ionization mass spectrometry using the double isotope spikers. The double isotope spikers (70Zn and 67Zn-enriched isotopes) are used to correct the isotope mass fractionation for the zinc isotope ratios, and to certify the zinc concentrations in the unknown samples. The zinc concentrations of these double isotope spikers are surveyed by a spiker made of pure (99.99%) natural zinc metal powder. The correcting factors (fa, ft and fn) of the zinc isotope ratios in the spiked mixture, spike and unspiked samples for the isotope mass fractionation, and the spike-to-unspiked ratios (Xr) of the zinc isotope r in the spiked mixture samples can be obtained to solve the matrix equations by numerical approximation. The natural zinc isotope ratios are: 64Zn/67Zn = 11.8498, 66Zn/67Zn = 6.7977, 68Zn/67Zn = 4.5730 and 70Zn/67Zn = 0.1520. The uncertainties determined of the isotope ratios and concentrations of zinc are +- 0.16% and +-0.31%, respectively

  3. Discussion on the Key Factors of Abundance Ratios About Zn Isotope Measurement

    International Nuclear Information System (INIS)

    The application of Zn isotope analysis is well known in geochemistry and diet study. An inter-lab comparison of five samples with isotopic ratio covering from 0.02 to 15.00 was organized in order to develop measurement ability and keep consistency of the results of isotopic ratios measurement among the participants. Multi-collector inductively coupled plasma mass spectrometry (MC-ICP-MS) and multi-collector thermal ionization mass spectrometry (MC-TIMS) were used. For MC-ICP-MS, blank-corrected and blank-no corrected results were submitted. For MC-TIMS, total evaporation method (TE) was applied to the samples while a certified reference material IRMM3702 was analyzed together. All the results showed that the uncertainties were 1.29%-0.03% for 64Zn/66Zn, and the uncertainty was obviously relative to isotopic abundances. The blank-corrected and blank-no corrected and the influence of blank and non-linear of K factor of mass discrimination for MC-ICP-MS were convinced of contributing to the unsatisfied uncertainties. (authors)

  4. Competition between collective and single particle excitations in nuclear structure description

    International Nuclear Information System (INIS)

    The microscopic description of the quadrupole collective dynamics in even krypton isotopes is presented. A microscopic calculation of Bohr's collective Hamiltonian is used to describe the collective motion in 76Kr. A single-particle basis calculated in a deformed Woods-Saxon potential leads to the potential energy surface obtained by the Strutinsky renormalization procedure, and to the inertial functions determined in the cranking model approximation. The collective Schroedinger equation is solved numerically to analyse the low-energy, even parity states in 76Kr. A good agreement between experiment and theory is obtained without specifically adjusting any parameter in the model for this nucleus. Some results regarding statical and dynamical characteristics of sup(74,78,80)Kr isotopes are also presented. The asymmetric rotor model with admixture of two quasiparticles is used to describe the sup(66,68,70)Ge and the sup(64,66)Zn isotopes. The interplay of collective and single particle motions is further investigated by magnetic moment measurements using the method of integral angular correlations perturbed by recoil into gas. The results involve g-factor measurements for 166Ho, 68Ge, 64Zn, 66Zn and 68Ga nuclei. Finally, a discussion of further possible improvements and more general developments of the problems under investigation is given. (author)

  5. Sensitivity of N/Z ratio in projectile break-up of isobaric systems

    Directory of Open Access Journals (Sweden)

    De Filippo E.

    2016-01-01

    Full Text Available The binary break-up of projectile-like fragments in non central heavy-ion collisions follows different decay patterns, from equilibrated emission towards dynamical (prompt fission. Recently, comparing two systems with different N/Z in the entrance channel, it has been shown that the dynamical emission cross-section is enhanced for the most neutron rich system while the statistical emission cross-section is independent from the isotopic composition. In order to understand this dependence and disentangle it from the initial size of the nuclei, we have studied the two isobaric systems 124Xe+64 Zn and 124Xe+64 Ni at 35 A MeV (InKiIsSy experiment, in comparison with the previous studied reactions (124Sn +64 Ni and 112Sn +58 Ni at the same bombarding energy. We present the first results evidencing a striking similar effect in the dynamical decay as a function of the N/Z of the target for equal size systems.

  6. Preparation of [61Cu]-2-acetylpyridine thiosemicarbazone complex as a possible PET tracer for malignancies

    International Nuclear Information System (INIS)

    Due to the interesting anti-proliferative properties of copper-thiosemicarbazone complexes, the production of a 61Cu-labeled thiosemicarbazone, i.e. 2-acetylpyridine thiosemicarbazone (APTS) was investigated. Copper-61 (T1/2=3.33h) was produced via the 64Zn(p,α)61Cu nuclear reaction using a natural zinc target irradiated with 22MeV protons for 500μAh. The 61Cu was separated from the irradiated target material by a two-step method and converted to acetate; this yielded a final activity of 222GBq (6.0Ci), with a radiochemical yield of >95%. The 61Cu-acetate was mixed with 2-acetylpyridine thiosemicarbazone for 30min at room temperature to yield [61Cu]APTS with a radiochemical yield of more than 80%. Colorimetric methods showed that residual chemical impurities in the product were below the accepted limits. Radio thin layer chromatography (RTLC) showed a radiochemical purity of more than 99% after C18 column chromatography. A specific activity of about 370-740MBq/mmol (10-20Ci/mmol) was obtained. The stability of the final product was checked in the absence and presence of human serum at 37oC for up to 3h. The partition coefficient of the final complex was also determined

  7. Preparation of [{sup 61}Cu]-2-acetylpyridine thiosemicarbazone complex as a possible PET tracer for malignancies

    Energy Technology Data Exchange (ETDEWEB)

    Jalilian, A.R. [Cyclotron and Nuclear Medicine Department, Nuclear Research Center for Agriculture and Medicine (NRCAM), Atomic Energy Organization of Iran, Moazzen Boulevard, Rajaeeshahr, P.O. Box 31485-498 Karaj (Iran, Islamic Republic of)]. E-mail: ajalilian@nrcam.org; Rowshanfarzad, P. [Cyclotron and Nuclear Medicine Department, Nuclear Research Center for Agriculture and Medicine (NRCAM), Atomic Energy Organization of Iran, Moazzen Boulevard, Rajaeeshahr, P.O. Box 31485-498 Karaj (Iran, Islamic Republic of); Sabet, M. [SSDL and Health Physics Department, Nuclear Research Center for Agriculture and Medicine (NRCAM), Atomic Energy Organization of Iran, Moazzen Boulevard, Rajaeeshahr, P.O. Box 31485-498 Karaj, Iran. (Iran); Shafiee, A. [Faculty of Pharmacy and Pharmaceutical Sciences Research center, Tehran University of Medical Sciences, P.O. Box 14155-6451 Tehran (Iran, Islamic Republic of)

    2006-03-15

    Due to the interesting anti-proliferative properties of copper-thiosemicarbazone complexes, the production of a {sup 61}Cu-labeled thiosemicarbazone, i.e. 2-acetylpyridine thiosemicarbazone (APTS) was investigated. Copper-61 (T{sub 1/2}=3.33h) was produced via the {sup 64}Zn(p,{alpha}){sup 61}Cu nuclear reaction using a natural zinc target irradiated with 22MeV protons for 500{mu}Ah. The {sup 61}Cu was separated from the irradiated target material by a two-step method and converted to acetate; this yielded a final activity of 222GBq (6.0Ci), with a radiochemical yield of >95%. The {sup 61}Cu-acetate was mixed with 2-acetylpyridine thiosemicarbazone for 30min at room temperature to yield [{sup 61}Cu]APTS with a radiochemical yield of more than 80%. Colorimetric methods showed that residual chemical impurities in the product were below the accepted limits. Radio thin layer chromatography (RTLC) showed a radiochemical purity of more than 99% after C{sub 18} column chromatography. A specific activity of about 370-740MBq/mmol (10-20Ci/mmol) was obtained. The stability of the final product was checked in the absence and presence of human serum at 37{sup o}C for up to 3h. The partition coefficient of the final complex was also determined.

  8. Correlation between the fragmentation modes and light charged particles emission in heavy ion collisions

    Institute of Scientific and Technical Information of China (English)

    ZHANG YingXun[1; ZHOU ChengShuang[1,2; CHEN JiXian[1,2; WANG Ning[2; ZHAO Kai[1; LI ZhuXia[1

    2015-01-01

    The correlation between the shape of rapidity distribution of the yield of light charged particles and the fragmentation modes in semi-peripheral collisions for 70Zn+70Zn, 64Zn+64Zn and 64Ni+64Ni at the beam energy of 35 MeV/nucleon is investigated based on ImQMD05 code. Our studies show there is an interplay between the binary, ternary and multi-fragmentation break-up modes. The binary and ternary break-up modes more prefer to emit light charged particles at middle rapidity and give larger values of Rmid compared with the multi-fragmentation break-up mode does. The reduced rapidity distribution for the normalized yields of yield p, d, t, 3He, 4He and 6He and the corresponding values ~ Rmid oI yield can be used to estimate the probability of multi-fragmentation break-up modes. By comparing to experimental data, our results illustrate that ~40% of the collisions events belong to the multi- fragmentation break-up mode for the reactions we studied.

  9. Heterogeneous distribution of Zn stable isotopes in mice and applications to medical sciences

    Science.gov (United States)

    Moynier, F.; Fujii, T.; Shaw, A.; Le Borgne, M.

    2013-12-01

    Zinc is required for the function of more than 300 enzymes involved in many metabolic pathways, and is a vital micronutrient for living organisms. To investigate if Zn isotopes could be used to better understand metal homeostasis, as well as a biomarker for diseases, we assessed the distribution of natural Zn isotopes in various mouse tissues. We found that, with respect to Zn isotopes, most mouse organs are isotopically distinct and that the total range of variation within one mouse encompasses the variations observed in the Earth's crust. Therefore, biological activity must have a major impact on the distribution of Zn isotopes in inorganic materials. The most striking aspect of the data is that red blood cells and bones are enriched by ~0.5 per mil in 66Zn relative to 64Zn when compared to serum, and up to ~1 per mil when compared to the brain and liver. This fractionation is well explained by the equilibrium distribution of isotopes between different bonding environments of Zn in different organs. Differences in gender and genetic background did not appear to affect the isotopic distribution of Zn. Together, these results suggest that potential use of Zn isotopes as a tracer for dietary Zn, and for detecting disturbances in Zn metabolism due to pathological conditions.

  10. Thermal properties of a rotating nucleus in a fluctuating mean-field approach

    International Nuclear Information System (INIS)

    The static-path approximation to the path integral representation of partition function provides a natural microscopic basis to deal with thermal fluctuations around mean-field configurations. Using this approach for a one-dimensional cranking hamiltonian with quadrupole-quadrupole interaction term we have studied a few properties like energy, level-density, level-density parameter (a) and moment of inertia as a function of temperature and spin for 64Zn taking it as an illustrative example. We have also investigated the effects of variation in interaction strength on the level density and the parameter a as a function of temperature. The moment of inertia, I, versus rotational frequency, ω, plot shows a sudden rise in the value of I due to the rotation alignment of Og9/2 orbitals at ω ∼ 1.0 MeV for a small temperature T ∼ 0.5 MeV. At high T ∼ 2.0 MeV about 40-45% of each angular momentum is generated by the alignment of Og9/2 orbitals with an interesting result that at ω ∼ 1.0 MeV and spin J ∼ 16 the moment of inertia has almost a constant, temperature-independent value. (orig.)

  11. Interaction of an aluminum atom with a closed subshell metal atom: Spectroscopic analysis of AlZn

    Science.gov (United States)

    Behm, Jane M.; Blume, Thorsten; Morse, Michael D.

    1994-10-01

    Resonant two-photon ionization spectroscopy has been employed to investigate diatomic AlZn produced by laser vaporization of a 1:2 Al:Zn alloy target disk in a supersonic expansion of helium. Several discrete transitions are reported in the energy range from 18 400 to 19 100 cm-1. Most of these are assigned as members of the B 2Π←X 2Π system, although an isolated band has been observed and assigned as the 2-0 band of the A Ω'=0.5←X 2Π1/2 system. A pair of strongly mixed levels are identified as resulting from a homogeneous spin-orbit perturbation between the A Ω=0.5, v'=3 and the B 2Π1/2, v'=1 levels, and the perturbation matrix element has been deduced to be 8.11 cm-1 for 27Al64Zn, 8.23 cm-1 for 27Al66Zn. The ground state has been unambiguously identified as a 2Πr state with a bond length of 2.6957±0.0004 Å. Comparisons to the results of the preceding article on the spectroscopy of AlCa are also provided, along with a discussion of the chemical bonding in AlZn in relation to AlCa, AlAr, and AlKr.

  12. Radiochemical measurement of neutron-spectrum averaged cross sections for the formation of {sup 64}Cu and {sup 67}Cu via the (n,p) reaction at a TRIGA Mark-II reactor. Feasibility of simultaneous production of the theragnostic pair {sup 64}Cu/{sup 67}Cu

    Energy Technology Data Exchange (ETDEWEB)

    Uddin, M. Shuza; Hossain, Syed Mohammod [Atomic Energy Research Establishment, Dhaka (Bangladesh). Inst. of Nuclear Science and Technology; Rumman-uz-Zaman, M. [Atomic Energy Research Establishment, Dhaka (Bangladesh). Inst. of Nuclear Science and Technology; Dhaka Univ. (Bangladesh). Dept. of Applied Chemistry and Chemical Engineering; Qaim, Syed M. [Forschungszentrum Juelich GmbH (Germany). Inst. fuer Neurowissenschaften und Medizin (INM-5) - Nuklearchemie

    2014-09-01

    Integral cross sections of the {sup 64}Zn(n,p){sup 64}Cu and {sup 67}Zn(n,p){sup 67}Cu reactions were measured for the fast neutron spectrum of TRIGA Mark-II reactor at Savar, Dhaka, Bangladesh. A clean radiochemical separation was performed to isolate the copper radionuclides from the target element zinc. The radioactivities produced in the irradiation were measured by HPGe γ-ray spectroscopy. The neutron flux over the energy range 0.5-20 MeV was determined using the {sup 58}Ni(n,p){sup 58}Co monitor reaction. The measured results amount to 28.9 ± 2.0 mb and 0.84 ± 0.07 mb for the formation of {sup 64}Cu and {sup 67}Cu, respectively. These values are slightly lower than the respective values for a pure fission spectrum. The present results were compared with data calculated using the neutron spectral distribution and the recently critically analysed excitation function of each reaction given in the literature. The good agreement validates the reliability of those excitation functions. The feasibility of simultaneous production of {sup 64}Cu and {sup 67}Cu with fast neutrons is discussed. (orig.)

  13. Hypernova Nucleosynthesis and Galactic Chemical Evolution

    CERN Document Server

    Nomoto, K; Umeda, H; Nakamura, T

    2001-01-01

    We study nucleosynthesis in 'hypernovae', i.e., supernovae with very large explosion energies ($ \\gsim 10^{52} $ ergs) for both spherical and aspherical explosions. The hypernova yields compared to those of ordinary core-collapse supernovae show the following characteristics: 1) Complete Si-burning takes place in more extended region, so that the mass ratio between the complete and incomplete Si burning regions is generally larger in hypernovae than normal supernovae. As a result, higher energy explosions tend to produce larger [(Zn, Co)/Fe], small [(Mn, Cr)/Fe], and larger [Fe/O], which could explain the trend observed in very metal-poor stars. 2) Si-burning takes place in lower density regions, so that the effects of $\\alpha$-rich freezeout is enhanced. Thus $^{44}$Ca, $^{48}$Ti, and $^{64}$Zn are produced more abundantly than in normal supernovae. The large [(Ti, Zn)/Fe] ratios observed in very metal poor stars strongly suggest a significant contribution of hypernovae. 3) Oxygen burning also takes place in...

  14. Hypernovae and their Nucleosynthesis

    CERN Document Server

    Nomoto, K; Umeda, H; Ohkubo, T; Deng, J; Mazzali, P A; Nomoto, Ken'ichi; Maeda, Keiichi; Umeda, Hideyuki; Ohkubo, Takuya; Deng, Jingsong; Mazzali, Paolo

    2002-01-01

    We review the characteristics of nucleosynthesis in 'Hypernovae', i.e., core-collapse supernovae with very large explosion energies ($ \\gsim 10^{52} $ ergs). The hypernova yields show the following characteristics: 1) The mass ratio between the complete and incomplete Si burning regions is larger in hypernovae than normal supernovae. As a result, higher energy explosions tend to produce larger [(Zn, Co, V)/Fe] and smaller [(Mn, Cr)/Fe], which could explain the trend observed in very metal-poor stars. 2) Because of enhanced $\\alpha$-rich freezeout, $^{44}$Ca, $^{48}$Ti, and $^{64}$Zn are produced more abundantly than in normal supernovae. The large [(Ti, Zn)/Fe] ratios observed in very metal poor stars strongly suggest a significant contribution of hypernovae. 3) Oxygen burning takes place in more extended regions in hypernovae to synthesize a larger amount of Si, S, Ar, and Ca ("Si"), which makes the "Si"/O ratio larger. The abundance pattern of the starburst galaxy M82 may be attributed to hypernova explosio...

  15. Hypernova Nucleosynthesis and Early Chemical Evolution

    CERN Document Server

    Nomoto, K; Umeda, H; Nomoto, Ken'ichi; Maeda, Keiichi; Umeda, Hideyuki

    2001-01-01

    We review the characteristics of nucleosynthesis in 'Hypernovae', i.e., supernovae with very large explosion energies ($ \\gsim 10^{52} $ ergs). The hypernova yields compared to those of ordinary core-collapse supernovae show the following characteristics: 1) Complete Si-burning takes place in more extended region, so that the mass ratio between the complete and incomplete Si burning regions is generally larger in hypernovae than normal supernovae. As a result, higher energy explosions tend to produce larger [(Zn, Co)/Fe], smaller [(Mn, Cr)/Fe], and larger [Fe/O], which could explain the trend observed in very metal-poor stars. 2) Si-burning takes place in lower density regions, so that the effects of $\\alpha$-rich freezeout is enhanced. Thus $^{44}$Ca, $^{48}$Ti, and $^{64}$Zn are produced more abundantly than in normal supernovae. The large [(Ti, Zn)/Fe] ratios observed in very metal-poor stars strongly suggest a significant contribution of hypernovae. 3) Oxygen burning also takes place in more extended regi...

  16. Probing the nuclear multipole response with intermediate energy heavy ions

    International Nuclear Information System (INIS)

    Intermediate energy (∼100 MeV/nucleon) heavy ion inelastic scattering excites low multipolarity giant resonances (GR) with very large cross sections (∼barns/sr for states which exhaust a large fraction of the relevant energy-weighted sum rule), and excites the continuum underlying the GR very weakly compared to light hadronic probes. These two features, combined with the fact that high resolution magnetic spectrometers are available at intermediate-energy heavy ion facilities, mean that heavy ion scattering has enormous promise for use in DR decay studies, and for isolating and studying weak states lying above the GDR. The author illustrates some of this promise with the results of experiments employing inelastic scattering of 17O, 36Ar, 86Kr, and 64Zn at energies ranging from 60 to 95 MeV/nucleon. These experiments were carried out at GANIL, and employed a high resolution magnetic spectrograph to detect the inelastically scattered particle, a large array of BaF2 detectors and a plastic open-quotes forward wallclose quotes hodoscope to study decay products. Results of studies of the decay of the GDR and the investigation of exotic strength above the GDR, including the identification and study of two-phonon strength, are discussed. The work involves scientists from ORNL, MSU, GANIL, KVI, GSI, Giessen, and Valencia

  17. Application of elemental bioimaging using laser ablation ICP-MS in forest pathology: distribution of elements in the bark of Picea sitchensis following wounding

    Energy Technology Data Exchange (ETDEWEB)

    Siebold, Magdalena [University of Aberdeen, Department of Plant and Soil Science, Institute of Biological and Environmental Sciences, Aberdeen (United Kingdom); University of Natural Resources and Applied Life Sciences Vienna, Department of Forest and Soil Sciences, Institute of Forest Entomology, Forest Pathology and Forest Protection, Vienna (Austria); Georg-August University Goettingen, Division of Plant Pathology and Crop Protection, Department of Crop Sciences, Goettingen (Germany); Leidich, Patrick; Bertini, Martina; Feldmann, Joerg [University of Aberdeen, TESLA, Trace Element Speciation Laboratory, Department of Chemistry, Aberdeen (United Kingdom); Deflorio, Giuliana; Woodward, Steve [University of Aberdeen, Department of Plant and Soil Science, Institute of Biological and Environmental Sciences, Aberdeen (United Kingdom); Krupp, Eva M. [University of Aberdeen, TESLA, Trace Element Speciation Laboratory, Department of Chemistry, Aberdeen (United Kingdom); University of Aberdeen, ACES, Aberdeen Centre of Environmental Sustainability, Aberdeen (United Kingdom); Halmschlager, Erhard [University of Natural Resources and Applied Life Sciences Vienna, Department of Forest and Soil Sciences, Institute of Forest Entomology, Forest Pathology and Forest Protection, Vienna (Austria)

    2012-04-15

    Element distribution in the bark of two 20-year-old clones of Picea sitchensis following wounding was studied using laser ablation inductively coupled plasma mass spectrometry (LA-ICP-MS). Bark was sampled at 0, 3, and 43 days after wounding and analysed using a focused Nd:YAG laser (266 nm). Intensities of {sup 13} C, {sup 25}Mg, {sup 27}Al, {sup 31}P, {sup 32}S, {sup 39}K, {sup 48}Ca, {sup 55}Mn, {sup 57}Fe, {sup 63}Cu and {sup 64}Zn were measured by ICP-MS to study elemental distribution across the bark samples during the wound repair process. A clear accumulation of Mg, P and K at the boundary zone between the lesion and healthy tissue was detected in the wounded samples and was more distinctive at 43 than at 3 days after treatment. This zone of accumulation mapped onto the position of formation of the ligno-suberised boundary zone and differentiation of the wound periderm. These accumulations suggest major roles for Mg, P and K in the non-specific response of Sitka spruce both to wounding, possibly as co-factors to enzymes and energy utilisation. The LA-ICP-MS method developed in this work proved useful to study spatial element distribution across bark samples and has great potential for applications in other areas of plant pathology research. (orig.)

  18. Evidence for a large radius of the 11Be projectile

    Science.gov (United States)

    So, W. Y.; Choi, K. S.; Cheoun, Myung-Ki; Kim, K. S.

    2016-05-01

    We investigate ratios of the elastic scattering cross section to Rutherford cross section, PE, and angular distributions of breakup cross section by using an optical model which exploits various long-range dynamic polarization potentials as well as short-range nuclear bare potentials for the 11Be projectile. From these simultaneous analyses, we extract a large radius of a halo projectile from the experimental data for PE and the angular distribution of the breakup cross section of the 11Be + 64Zn and 11 + 120Sn systems. It results from the fact that a large radius for the long-range nuclear potential is more reasonable for properly explaining these data simultaneously. The extracted reduced interaction radius turns out to be r0=3.18 ˜3.61 fm for 11Be nucleus, which is larger than the conventional value of r0=1.1 ˜1.5 fm used in the standard radius form R =r0A1 /3 . Furthermore, the larger radius as well as the normalization constant N is shown to be important for understanding Coulomb dipole strength distribution.

  19. Communication of nuclear data progress No.25 (2001. 6)

    International Nuclear Information System (INIS)

    This is the 25th issue of Communication of Nuclear Data Progress (CNDP), in which the achievements in nuclear data field for the last year in China are carried. It includes the measurements of 10B(n, γ)7Li and 64Zn(n,α) 61Ni angular distributions and cross sections, 75As(n,γ) 76As cross section and fission product yields of n + 235,238U; theoretical calculations of n + 23Na, 93,95Nb, 99Tc, 99-105Ru, 132,134-138Ba, 133-135,137Cs, 136,138,140,142NatCe, 142-148,150Nd, 175,176NatLu, 174,176-180NatHf; evaluations of reference fission yield data and n + 93,95Nb, 99,100Ru, 121,123Sb, 127,135I and 241,242Pu complete data; method to set up file 6 in neutron data library of light nuclei, Kerma factor calculation, a code for automatically searching optimal optical potential parameters below 300 MeV, internal conversion electrons data calculation, a code for composition of a nuclear data file of natural element from its isotope files; and the developments of CWIMS code and its 69-group library. Also the activities and cooperation on nuclear data in China are summarized

  20. Abundance and Impact of Doubly Charged Polyatomic Argon Interferences in ICPMS Spectra.

    Science.gov (United States)

    Hattendorf, Bodo; Gusmini, Bianca; Dorta, Ladina; Houk, Robert S; Günther, Detlef

    2016-07-19

    Doubly charged molecular ions of alkaline earth metals and argon could be identified as spectral interferences in an inductively coupled plasma mass spectrometer. These molecular ions were found to occur at abundances reaching about 10(-4) relative to the alkaline earth atomic ion abundances. They can thus substantially affect ultratrace analyses and, when present at similar concentration as the analyte elements, also isotope ratio measurements. For the case of Cu and Zn isotope ratio analyses, the same mass concentration of Sr was found to alter the measured (63)Cu/(65)Cu and (64)Zn/(66)Zn isotope ratios by -0.036‰ to -0.95‰ due to SrAr(2+), appearing at m/Q 63 and 64. BaAr(2+) can affect Sr isotope analyses, MgAr(2+) may impair S isotope ratio measurements, while CaAr(2+) may cause interference to Ca(+) isotopes. The abundances of the doubly charged molecular ions were higher than those of the corresponding singly charged species, which is in accordance with their generally higher bond dissociation energies. The relative abundances were found to depend significantly on the inductively coupled plasma (ICP) operating conditions and generally increase with increasing carrier gas flow rates or lower gas temperature of the ICP. They also increase by about an order of magnitude when a desolvated aerosol is introduced to the ICP. PMID:27306032

  1. Zinc isotope fractionation during magmatic differentiation and the isotopic composition of the bulk Earth

    Science.gov (United States)

    Chen, Heng; Savage, Paul S.; Teng, Fang-Zehn; Helz, Rosalind T.; Moynier, Frédéric

    2013-01-01

    he zinc stable isotope system has been successfully applied to many and varied fields in geochemistry, but to date it is still not completely clear how this isotope system is affected by igneous processes. In order to evaluate the potential application of Zn isotopes as a proxy for planetary differentiation and volatile history, it is important to constrain the magnitude of Zn isotopic fractionation induced by magmatic differentiation. In this study we present high-precision Zn isotope analyses of two sets of chemically diverse, cogenetic samples from Kilauea Iki lava lake, Hawaii, and Hekla volcano, Iceland, which both show clear evidence of having undergone variable and significant degrees of magmatic differentiation. The Kilauea Iki samples display small but resolvable variations in Zn isotope composition (0.26‰66Zn66Zn defined as the per mille deviation of a sample's 66Zn/64Zn compositional ratio from the JMC-Lyon standard), with the most differentiated lithologies exhibiting more positive δ66Zn values. This fractionation is likely a result of the crystallization of olivine and/or Fe–Ti oxides, which can both host Zn in their crystal structures. Samples from Hekla have a similar range of isotopic variation (0.22‰66Zn66Zn=0.28±0.05‰ (2s.d.).

  2. Utilization and operating experience of the 250 kw TRIGA Mark II research reactor in Ljubljana

    International Nuclear Information System (INIS)

    In its 35th year, the TRIGA Mark II 250 kW pulsing research reactor in Ljubljana is continuing its busy operation. With the maximum neutron flux in the central thimble of 10 13 n/cm 2 sec and many sample radiation positions the reactor has been used to perform many experiments in the following fields: solid state physics (elastic and inelastic neutron scattering), neutron dosimetry, neutron radiography, reactor physics including burn up measurements and calculations, boron neutron capture therapy and neutron activation analysis which represents one of the major usage of our reactor. Besides these, applied research around the reactor has been conducted, such as doping of silicon monocrystals, a routine production of various radioactive isotopes for industry ( 60Co, 64Zn, 24Na, 82Br) and medical use ( 18F, 99m Tc, etc.) and other activities. During the past decade the reactor was almost completely reconstructed (new grid plates, the control mechanisms and the control unit, modification of the spent fuel storage pool, etc). The main novelty in the reactor physics and operation features of the reactor was the installation of a pulse rod, therefore the reactor can be operated in a pulse mode. After reconstruction, the core was loaded with fresh 20% enriched fuel elements. In 1999 all spent fuel elements were shipped to the USA. (author)

  3. Investigation of dynamics of fusion reactions through cross-section and spin distribution measurements

    International Nuclear Information System (INIS)

    The CN populated at high excitation energy and angular momentum in fusion reactions can undergo decay through fission or emission of different light particles (α-particles, neutrons and protons). The statistical model has been extensively used to explain the evaporation spectra of these light particles and to extract important information about the properties of the CN. However, many of the evaporation studies show anomalous results from the statistical model predictions, for the mass symmetric systems. With this motivation we have performed the ER-gated spin distribution and the cross-section measurements for two systems 16O + 64Zn (mass asymmetric) and 32S + 48Ti (mass symmetric) populating the same CN (80Sr) for which the evaporation spectra studies have reported the existence of deviations for the symmetric system. Present measurements have been performed using 15 UD Pelletron accelerator and Heavy Ion Reaction Analyzer (HIRA) facility at Inter University Accelerator Centre (IUAC), New Delhi. The details of these measurements and analysis procedure have been described elsewhere

  4. Response of unirradiated and neutron-irradiated vanadium alloys to Charpy-impact loading

    International Nuclear Information System (INIS)

    The ductile-brittle transition temperature (DBTT) was determined by Charpy-impact impact tests for dehydrogenated (<30 appm H) and hydrogenated (400--1200 appm H) V-7.2Cr-14.5Ti, V-9.9Cr-9.2Ti, V-13.5Cr-5.2Ti, V-17.7Ti, V-9.2Cr-4.9Ti, V-9.0Cr-3.2Fe-1.2Zr, V-3.1Ti-0.5Si, V-4.1Cr-4.3Ti, V-4.6Ti, and V-2.5Ti-1.0Si alloys. The DBTT was also determined for the V-13.5Cr-5.2Ti, V-9.2Cr-4.9Ti, V-7.2Cr-14.5Ti, and V-17.7Ti alloys after neutron irradiation at 420 and 600 degrees C to 41--44 atom displacements per atom. The DBTTs determined for these vanadium alloys show that a vanadium alloy containing Cr and/or Ti and Si alloying additions to be used as a structural material in a fusion reactor should contain 3--11 wt % total alloying addition for maximum resistance to hydrogen- and/or irradiation-induced embrittlement. 4 refs., 3 figs., 2 tabs

  5. Synthesis and structural and thermodynamical characterization of hollandite type material intended for the specific containment of cesium; Synthese et caracterisation de ceramiques de type hollandite destinees au conditionnement specifique du cecium

    Energy Technology Data Exchange (ETDEWEB)

    Leinekugel-Le-Cocq-Errien, A.Y

    2005-09-15

    This thesis deals with the characterization of the Ba{sub 1}Cs{sub 0.28}Fe{sub 0.82}Al{sub 1.46}Ti{sub 5.72}O{sub 16} hollandite envisaged for Cs containment. Techniques used are essentially classical powder XRD or synchrotron radiation at the absorption threshold of Ba and Cs, TEM and high-temperature calorimetry. Two syntheses have been studied: an alcoxide route and a dry route. After sintering, both routes lead to an incommensurate modulated tetragonal hollandite structure (space group: I4/m(00{gamma})00) with a modulation vector distribution. Before sintering, the material obtained by the alcoxide route is composed of three phases: a tetragonal hollandite like above, a monoclinic Ba-free hollandite and a weak-coherence-length phase containing only Ba. On contrary, the dry route already leads to the tetragonal hollandite at this step of the synthesis. High temperature oxide melt solution calorimetry was used to derive standard enthalpy of formation of hollandite to deduce its free enthalpy of formation. (author)

  6. Probing the systematics for low energy incomplete fusion with universal fusion function model

    International Nuclear Information System (INIS)

    In the recent years, a renewed interest has emerged, in the study of heavy ion (HI) reactions to investigate the effects of breakup and fusion processes at energies around the Coulomb barrier. In HI reactions the complete fusion (CF) takes place when all the nucleons of the projectile and target nuclei lose their identity to form a single complex system followed by equilibration of the compound system. On the other hand, incomplete fusion (ICF) occurs, when only a part of projectile fuses with the target nucleus and remaining part escapes with nearly incident beam velocity. In order to explore the dynamics of HI reactions, a number of studies has been done within the framework of entrance channel parameters with weakly as well as strongly bound projectiles. In the present work, an attempt has been made to study the target dependence on experimentally modified fusion function as suggested by Canto et al.. The experimental data from the experiment performed at IUAC, New Delhi for the 12C projectile on 159Tb target along with 12C+46Ti, 12C+48Ti, 12C+50Ti from the available literature has been renormalized within the framework of recently proposed Universal Fusion Function (UFF) approach

  7. Study of dynamics and ground state structure of low and medium mass double hypernuclei

    Indian Academy of Sciences (India)

    M D Abdul Khan; Tapan Kumar Das

    2001-01-01

    We critically review the dynamics by examining - and -nucleon phenomenological potentials in the study of the bound state properties of double- hypernuclei $^{6}_{}$He, $^{10}_{}$Be, $^{14}_{}$C, $^{18}_{}$O, $^{22}_{}$Ne, $^{26}_{}$Mg, $^{30}_{}$Si, $^{34}_{}$S, $^{38}_{}$Ar, $^{42}_{}$Ca, $^{46}_{}$Ti, $^{50}_{}$Cr, $^{54}_{}$Fe, $^{58}_{}$Ni, $^{62}_{}$Zn, $^{66}_{}$Ge, $^{70}_{}$Se, $^{74}_{}$Kr, $^{78}_{}$Sr, $^{82}_{}$Zr, $^{86}_{}$Mo, $^{90}_{}$Ru, $^{94}_{}$Pd, $^{98}_{}$Cd, $^{102}_{}$Sn in the frame work of (core ++) three body model. An effective potential is obtained by folding the phenomenological potential into the density distribution of the core nuclei. The former two cases (i.e. $^{6}_{}$He and $^{10}_{}$Be) are revisited to justify the correctness of the present potential model. Assuming the same potential model we predicted some of the structural properties of heavier doubly -hypernuclei. The hyperspherical harmonics expansion method, which is an essentially exact method has been employed for the three body system. A convergence in binding energy up to 0.15% for max = 20 has been achieved. In our calculation we have made no approximation in restricting the allowed -values of the interacting pairs.

  8. Mass measurements and superallowed beta decay

    CERN Document Server

    Hardy, J C; Towner, I S

    2005-01-01

    A recent Penning-trap measurement of the masses of 46V and 46Ti leads to a Qec value that disagrees significantly with the previously accepted value, and destroys overall consistency among the nine most precisely characterized T=1 superallowed beta emitters. This raises the possibility of a systematic discrepancy between Penning-trap measurements and the reaction-based measurements upon which the Qec values depended in the past. We carefully re-analyze (n,gamma) and (p,gamma) reaction measurements in the 24 \\leq A \\leq 28 mass region, and compare the results to very precise Penning-trap measurements of the stable nuclei 24Mg, 26Mg and 28Si. We thus determine upper limits to possible systematic effects in the reaction results, and go on to establish limits for the mass of radioactive 26Al, to which future on-line Penning-trap measurements can be compared. We stress the urgency of identifying or ruling-out possible systematic effects.

  9. Comparison of the charge distributions of the titanium isotopes

    International Nuclear Information System (INIS)

    Measurements have been made of the elastic electron scattering from the three even isotopes of titanium, Ti46, Ti48, and Ti50, with the objective of determining the differences in their ground state charge distributions. The experiment measures the ratios of the elastic cross sections of the three isotopes, thereby eliminating many of the uncertainties peculiar to an absolute cross section measurement. The experiment was done at the NBS Linac in Gaithersburg, Maryland. Theoretical calculations using a partial wave elastic scattering program, showed that the ratios of cross sections arising from scattering from two slightly different Fermi type 2 parameter charge distributions, depended strongly on the differences in the parameter describing the charge distribution, but only weakly on the actual values of these parameters. These ratio curves, considered as a function of momentum transfer, achieved their extreme values at momenta transfer near 1.0 F-1, which is near the point where the Born approximation form factor goes to zero. Therefore, ratios of cross sections were measured at momenta transfer ranging from .55 to 1.1 F-1; by holding the scattering angle fixed at 127.50 and varying the incident beam energy from 60 to 123 MeV. 43 refs., 45 figs., 9 tabs

  10. Design status of KOBRA for rare isotope production and direct measurements of radiative capture cross sections

    Science.gov (United States)

    Tshoo, K.; Chae, H.; Park, J.; Moon, J. Y.; Kwon, Y. K.; Souliotis, G. A.; Hashimoto, T.; Akers, C.; Berg, G. P. A.; Choi, S.; Jeong, S. C.; Kato, S.; Kim, Y. K.; Kubono, S.; Lee, K. B.; Moon, C.-B.

    2016-06-01

    KOBRA (KOrea Broad acceptance Recoil spectrometer and Apparatus) facility being designed at Rare Isotope Science Project in Korea will be utilized to produce rare isotope beams by employing multi-nucleon transfer reactions at about 20 MeV/nucleon for studies of nuclear structure. KOBRA will also provide high suppression of beam induced background for direct measurements of radiative-capture cross sections in the astrophysical energy range. The present design status of the KOBRA facility is reported along with a brief introduction to the facility. We have studied the feasibility of production of 44Ti based on the present design of KOBRA as an example, and calculated the intensity of 44Ti secondary beam, to be about 105 particles per second, for 1 pnA 46Ti primary beam with a carbon target for a beam energy of 25 MeV/nucleon. A Monte Carlo simulation with a ray-tracing code has been performed to show that recoil products 66Se are well separated from a 65As beam by KOBRA for the 65As (p, γ)66Se reaction at a beam energy of 1 MeV/nucleon.

  11. The ground state infrared spectra of several isotopic forms of the CdH and ZnH radicals

    International Nuclear Information System (INIS)

    The infrared spectra of six isotopic forms of cadmium monohydride, [116CdH (7.6%), 114CdH (28.9%), 113CdH (12.3%), 112CdH (24.1%), 111CdH (12.7%), and 110CdH (12.4%)] and four isotopic forms of zinc hydride [68ZnH (18.6%), 67ZnH (4.1%), 66ZnH (27.8%), and 64ZnH (48.9%)] have been observed in natural abundance in their ground electronic state (2Σ+) in the gas phase using a diode laser spectrometer. A number of transitions of 108CdH (0.9%) and 106CdH (1.2%) and 70ZnH (0.6%) were also observed, but too little data was accumulated to allow a good analysis. The hydrides were produced by reaction of hydrogen with metal vapor at elevated temperature in an electric discharge. The analysis of the experimental data was carried out in two ways. (a) A complete set of Dunham parameters and spin--rotation parameters (γ parameters) was determined for each isotopic species of the two radicals and (b) a set of mass-independent parameters were calculated for both ZnH and CdH. Since only information over the isotopic species of the heavy atom was produced in each case, effects arising from a breakdown of the Born--Oppenheimer approximation were negligible. The effects of the strong anharmonicity present in these two molecules on the values of the parameters are discussed

  12. Systematics of gamma decay through low-lying vibrational levels of even--even nuclei excited by (p,p') and (n,n') reactions

    Energy Technology Data Exchange (ETDEWEB)

    Koopman, R.P.

    1977-06-30

    A series of experiments was performed in which gamma-ray spectra were measured, using a Ge(Li) detector, for incident 7 to 26-MeV protons on the even-even vibrational nuclei /sup 56/Fe, /sup 62/Ni, /sup 64/Zn, /sup 108/Pd, /sup 110/Cd, /sup 114/Cd, /sup 116/Cd, /sup 116/Sn, /sup 120/Sn, and /sup 206/Pb, and for incident 14-MeV neutrons on natural Fe, Ni, Zn, Cd, Sn, and Pb. These measurements yielded gamma-ray cross sections from which it was inferred that almost all of the gamma cascades from (p,p') and (n,n') reactions passed down through the first 2/sup +/ levels. Consequently, the strength of the 2/sup +/ ..-->.. 0/sup +/ gamma transitions were found to be an indirect measure of the (p,p') or (n,n') cross sections. Several types of nuclear model calculations were performed and compared with experimental results. These calculations included coupled-channel calculations to reproduce the direct, collective excitation of the low-lying levels, and statistical plus pre-equilibrium model calculations to reproduce the (p,p') and the (n,n') cross sections for comparison with the 2/sup +/ ..-->.. 0/sup +/ gamma measurements. The agreement between calculation and experiment was generally good except at high energies, where pre-equilibrium processes dominate (i.e. around 26-MeV). Here discrepancies between calculations from the two different pre-equilibrium models and between the data and the calculations were found. Significant isospin mixing of T/sub greater than/ into T/sub less than/ states was necessary in order to have the calculations match the data for the (p,p') reactions, up to about 18-MeV.

  13. Validation of minor actinides fission neutron cross-sections

    Directory of Open Access Journals (Sweden)

    Pešić Milan P.

    2015-01-01

    Full Text Available Verification of neutron fission cross-sections of minor actinides from some recently available evaluated nuclear data libraries was carried out by comparison of the reaction rates calculated by the MCNP6.1 computer code to the experimental values. The experimental samples, containing thin layers of 235U, 237Np, 238,239,240,241Pu, 242mAm, 243Cm, 245Cm, and 247Cm, deposited on metal support and foils of 235U (pseudo-alloy 27Al + 235U, 238U, natIn, 64Zn, 27Al, and multi-component sample alloy 27Al + 55Mn + natCu + natLu + 197Au, were irradiated in the channels of the tank containing fluorine salts 0.52NaF + 0.48ZrF4, labelled as the Micromodel Salt Blanket, inserted in the lattice centre of the MAKET heavy water critical assembly at the Institute for Theoretical and Experimental Physics, Moscow. This paper is a continuation of earlier initiated scientific-research activities carried out for validation of the evaluated fission cross-sections of actinides that were supposed to be used for the quality examination of the fuel design of the accelerator driven systems or fast reactors, and consequently, determination of transmutation rates of actinides, and therefore, determination of operation parameters of these reactor facilities. These scientific-research activities were carried out within a frame of scientific projects supported by the International Science and Technology Center and the International Atomic Energy Agency co-ordinated research activities, from 1999 to 2010. Obtained results confirm that further research is needed in evaluations in order to establish better neutron cross-section data for the minor actinides and selected nuclides which could be used in the accelerator driven systems or fast reactors.

  14. Mass and beta decay of the N = Z isotope {sup 68}Se

    Energy Technology Data Exchange (ETDEWEB)

    Blumenthal, D.J.; Davids, C.N.; Lister, C.J. [and others

    1995-08-01

    An experiment to measure the mass and beta decay of the N = Z nuclide {sup 68}Se was performed. The properties of {sup 68}Se are important for determining the abundance of proton-rich nuclei such as {sup 60}Ni and {sup 64}Zn, which are thought to be formed in the alpha-rich freezeout stage of a giant star. The abundances of the even-even N = Z nuclei such as {sup 60}Zn, {sup 64}Ge, and {sup 68}Se depend on the competition between ({alpha},{gamma}) and ({gamma},{alpha}) reactions, whose rates depend sensitively on the reaction Q-values. In addition, the half-life of {sup 68}Se is important in determining the path of the explosive rp-process, since reactions such as (p,{gamma}) must compete with beta decay in order to push the rp path to heavier nuclei. Using the moving tape collector system and the {sup 12}C({sup 58}Ni,2n){sup 68}Se reaction at 200 MeV, recoils were mass-selected by a slit at the FMA focal plane and implanted into the tape. After a 50-second collection period, the accumulated activity was moved to the counting position between two Ge gamma-ray detectors or a plastic scintillator beta detector and a Ge detector. The half-life of {sup 68}Se was determined to be 37 {plus_minus} 5 s, in agreement with other measurements. Gamma-gamma and beta-gamma coincidence data are under analysis, to produce the decay scheme and the electron capture decay energy.

  15. Zinc isotope and transition-element dynamics accompanying hydrozincite biomineralization in the Rio Naracauli, Sardinia, Italy

    Science.gov (United States)

    Wanty, Richard B.; Podda, F.; De Giudici, Giovanni; Cidu, R.; Lattanzi, Pierfranco

    2013-01-01

    The Rio Naracauli in SW Sardinia drains part of the Ingurtosu Zn–Pb mining district, and contains extreme concentrations of dissolved Zn at near-neutral pH. In the upper reaches of the stream, pH, alkalinity and Zn concentrations are such that hydrozincite [Zn5(CO3)2(OH)6] precipitates in a biologically mediated process facilitated by a microalga (Chlorella sp.) and a cyanobacterium (Scytonema sp.). Values of δ66Zn in water and solid samples ranged from − 0.35‰ to + 0.5‰ relative to the JMC 3-0749-Lyon standard, and closely follow a mass-dependent fractionation line. Two composite samples of sphalerite, the primary ore mineral in the Ingurtosu deposits, had an average δ66Zn of + 0.15‰, similar to sphalerite measured elsewhere in hydrothermal mineral deposits. Zinc isotope measurements of the stream water and the hydrozincite forming in the stream show a consistent preference for the heavy isotope, 66Zn, in the hydrozincite relative to 64Zn. Synthetic hydrozincites produced without added bacteria have δ66Zn identical to the dissolved Zn, thus suggesting a biologically mediated mineralization process in Rio Naracauli. The average fractionation, Δhdz-water, is 0.35‰, the magnitude of which is consistent with other studies, and suggests an extracellular mechanism of the biomineralization process. Zinc concentration and dissolved δ66Zn steadily decrease in the reach of the stream where the biomineralization occurs. The biomineralization process also leads to the sequestration of Pb, Cu and Ni in the hydrozincite lattice, and the coeval precipitation of an amorphous CdCO3 solid, prompting the suggestion that if optimized, the biomineralization process might represent a feasible passive remediation strategy for streams with high Zn and other metals, and with near-neutral pH.

  16. Exploiting dynamic reaction cell inductively coupled plasma mass spectrometry (DRC-ICP-MS) for sequential determination of trace elements in blood using a dilute-and-shoot procedure.

    Science.gov (United States)

    Batista, Bruno Lemos; Rodrigues, Jairo Lisboa; Nunes, Juliana Andrade; Souza, Vanessa Cristina de Oliveira; Barbosa, Fernando

    2009-04-20

    Inductively coupled plasma mass spectrometry with quadrupole (q-ICP-MS) and dynamic reaction cell (DRC-ICP-MS) were evaluated for sequential determination of As, Cd, Co, Cr, Cu, Mn, Pb, Se, Tl, V and Zn in blood. The method requires as little as 100 microL of blood. Prior to analysis, samples (100 microL) were diluted 1:50 in a solution containing 0.01% (v/v) Triton X-100 and 0.5% (v/v) nitric acid. The use of the DRC was only mandatory for Cr, Cu, V and Zn. For the other elements the equipment may be operated in a standard mode (q-ICP-MS). Ammonia was used as reaction gas. Selection of best flow rate of ammonium gas and optimization of the quadrupole dynamic band-pass tuning parameter (RPq) were carried out, using a ovine base blood for Cr and V and a synthetic matrix solution (SMS) for Zn and Cu diluted 1:50 and spiked to contain 1 microg L(-1) of each element. Method detection limits (3 s) for (75)As, (114)Cd, (59)Co, (51)Cr, (63)Cu (55)Mn, (208)Pb, (82)Se, (205)Tl, (51)V, and (64)Zn were 14.0, 3.0, 11.0, 7.0, 280, 9.0, 3.0, 264, 0.7, 6.0 and 800 ng L(-1), respectively. Method validation was accomplished by the analysis of blood Reference Materials produced by the L'Institut National de Santé Publique du Quebec (Canada).

  17. Fractionation of Cu and Zn isotopes during adsorption onto amorphous Fe(III) oxyhydroxide: Experimental mixing of acid rock drainage and ambient river water

    Science.gov (United States)

    Balistrieri, L.S.; Borrok, D.M.; Wanty, R.B.; Ridley, W.I.

    2008-01-01

    Fractionation of Cu and Zn isotopes during adsorption onto amorphous ferric oxyhydroxide is examined in experimental mixtures of metal-rich acid rock drainage and relatively pure river water and during batch adsorption experiments using synthetic ferrihydrite. A diverse set of Cu- and Zn-bearing solutions was examined, including natural waters, complex synthetic acid rock drainage, and simple NaNO3 electrolyte. Metal adsorption data are combined with isotopic measurements of dissolved Cu (65Cu/63Cu) and Zn (66Zn/64Zn) in each of the experiments. Fractionation of Cu and Zn isotopes occurs during adsorption of the metal onto amorphous ferric oxyhydroxide. The adsorption data are modeled successfully using the diffuse double layer model in PHREEQC. The isotopic data are best described by a closed system, equilibrium exchange model. The fractionation factors (??soln-solid) are 0.99927 ?? 0.00008 for Cu and 0.99948 ?? 0.00004 for Zn or, alternately, the separation factors (??soln-solid) are -0.73 ?? 0.08??? for Cu and -0.52 ?? 0.04??? for Zn. These factors indicate that the heavier isotope preferentially adsorbs onto the oxyhydroxide surface, which is consistent with shorter metal-oxygen bonds and lower coordination number for the metal at the surface relative to the aqueous ion. Fractionation of Cu isotopes also is greater than that for Zn isotopes. Limited isotopic data for adsorption of Cu, Fe(II), and Zn onto amorphous ferric oxyhydroxide suggest that isotopic fractionation is related to the intrinsic equilibrium constants that define aqueous metal interactions with oxyhydroxide surface sites. Greater isotopic fractionation occurs with stronger metal binding by the oxyhydroxide with Cu > Zn > Fe(II).

  18. Imaging of copper, zinc, and other elements in thin section of human brain samples (hippocampus) by laser ablation inductively coupled plasma mass spectrometry.

    Science.gov (United States)

    Becker, J S; Zoriy, M V; Pickhardt, C; Palomero-Gallagher, N; Zilles, K

    2005-05-15

    Laser ablation inductively coupled plasma mass spectrometry (LA-ICPMS) was used to produce images of element distribution in 20-microm thin sections of human brain tissue. The sample surface was scanned (raster area approximately 80 mm(2)) with a focused laser beam (wavelength 213 nm, diameter of laser crater 50 microm, and laser power density 3 x 10(9) W cm(-2)) in a cooled laser ablation chamber developed for these measurements. The laser ablation system was coupled to a double-focusing sector field ICPMS. Ion intensities of 31P+, 32S+, 56Fe+, 63Cu+, 64Zn+, 232Th+, and 238U+ were measured within the area of interest of the human brain tissue (hippocampus) by LA-ICPMS. The quantitative determination of copper, zinc, uranium, and thorium distribution in thin slices of the human hippocampus was performed using matrix-matched laboratory standards. In addition, a new arrangement in solution-based calibration using a micronebulizer, which was inserted directly into the laser ablation chamber, was applied for validation of synthetic laboratory standard. The mass spectrometric analysis yielded an inhomogeneous distribution (layered structure) for P, S, Cu, and Zn in thin brain sections of the hippocampus. In contrast, Th and U are more homogeneously distributed at a low-concentration level with detection limits in the low-nanogram per gram range. The unique analytical capability and the limits of LA-ICPMS will be demonstrated for the imaging of element distribution in thin cross sections of brain tissue from the hippocampus. LA-ICPMS provides new information on the spatial element distribution of the layered structure in thin sections of brain tissues from the hippocampus. PMID:15889910

  19. Synthesis, characterization and thermochemistry of Cs-, Rb- and Sr-substituted barium aluminium titanate hollandites

    International Nuclear Information System (INIS)

    Highlights: • Cs-, Rb- and Sr-substituted barium titanate hollandites were synthesized using sol–gel methods. • Chemical compositions were determined by electron microprobe analyses. • Crystal structures were analyzed using powder synchrotron X-ray diffraction coupled with Rietveld refinements. • Enthalpies of formation were measured using high temperature oxide melt solution calorimetry. • Stability relations with respect to BaTiO3 and SrTiO3 perovskites and other oxides were determined. - Abstract: Titanate hollandites are of considerable interest for immobilization of radioactive Cs, its daughter product Ba and related radionuclides Rb and Sr. In this study, we synthesized three hollandites, Ba1.18Cs0.21Al2.44Ti5.53O16, Ba1.17Rb0.19Al2.46Ti5.53O16 and Ba1.14Sr0.10Al2.38Ti5.59O16, using sol–gel methods. Rietveld analysis of synchrotron XRD data shows that they adopt the tetragonal structure (space group I4/m), and their cell parameters increase with increasing cation size (Sr2+ → Rb+ → Cs+). Standard enthalpies of formation of these hollandites were determined from drop solution calorimetric measurements with lead borate as the solvent at 973 K. Their formation enthalpies are similar, consistent with the occurrence of extensive cation substitutions in hollandites. Further energetic analysis with respect to BaTiO3 and SrTiO3 perovskites and other oxides reveals decreased thermodynamic stability from Cs- to Rb- to Sr-hollandite. This trend is consistent with the phase assemblage observed in Synroc, where Cs+, Rb+ and Ba2+ enter into hollandite, whereas Sr2+ occurs in perovskite

  20. RoSiB - a 4π silicon ball for charged-particle detection in EUROBALL

    Science.gov (United States)

    Pausch, G.; Prade, H.; Sobiella, M.; Schnare, H.; Schwengner, R.; Käubler, L.; Borcan, C.; Ortlepp, H.-G.; Oehmichen, U.; Grawe, H.; Schubart, R.; Gerl, J.; Cederkäll, J.; Johnson, A.; Kerek, A.; Klamra, W.; Moszyński, M.; Wolski, D.; Kapusta, M.; Axelsson, A.; Weiszflog, M.; Härtlein, T.; Pansegrau, D.; de Angelis, G.; Ashrafi, S.; Likar, A.; Lipoglavšek, M.

    2000-04-01

    A 4π silicon ball for detection and identification of light charged particles in large multidetector γ-arrays as EUROBALL is presented. The design is based on a N=42 ball with 12 pentagons and 30 hexagons as used in the GASP array. The absorptive material for γ-rays is minimized to the detector thickness of 300 or 500 μm and a 0.63 mm ceramic backing. The geometrical coverage is designed for about 90% of 4π. A pulse shape discrimination method with totally depleted detectors working in the reverse mount allows identifying protons and α-particles above an energy threshold of about 2 MeV. The performances of the ball were tested at the tandem - booster accelerator combination of the MPI Heidelberg in two experiments using the high-recoil reaction of 228 MeV 58Ni+ 46Ti and the low-recoil reaction of 95 MeV 16O+ 58Ni . The two-dimensional spectra of zero-crossing (ZC) versus energy confirmed an excellent discrimination of protons and α-particles in all the detectors at different angles. The energy spectra of protons and α-particles measured in the experiments are presented, too. The γ-spectra measured in coincidence with various combinations of emitted particles showed a high selectivity of the ball. The reduced total efficiency for protons of 59% and 55% and α-particles of 44% and 32% measured in a nuclear spectroscopy application is analyzed in a Monte-Carlo simulation (GEANT). It is due to a combined influence of a thick target needed to stop the recoiling residual nuclei and thick absorbers needed to protect the Si-detectors from scattered beam. The results along with the GEANT extrapolation to optimum experimental conditions confirm that RoSiB is a highly efficient and selective device for identification of rare reaction channels with heavy ions.

  1. Temperature-dependent wear mechanisms for magnetron-sputtered AlTiTaN hard coatings.

    Science.gov (United States)

    Khetan, Vishal; Valle, Nathalie; Duday, David; Michotte, Claude; Mitterer, Christian; Delplancke-Ogletree, Marie-Paule; Choquet, Patrick

    2014-09-10

    AlTiTaN coatings have been demonstrated to have high thermal stability at temperatures up to 900 °C. It has been speculated that the high oxidation resistance promotes an improved wear resistance, specifically for dry machining applications. This work reports on the influence of temperature up to 900 °C on the wear mechanisms of AlTiTaN hard coatings. DC magnetron-sputtered coatings were obtained from an Al(46)Ti(42)Ta(12) target, keeping the substrate bias at -100 V and the substrate temperature at 265 °C. The coatings exhibited a single-phase face-centered cubic AlTiTaN structure. The dry sliding tests revealed predominant abrasion and tribo-oxidation as wear mechanisms, depending on the wear debris formed. At room temperature, abrasion leading to surface polishing was observed. At 700 and 800 °C, slow tribo-oxidation and an amorphous oxide formed reduced the wear rate of the coating compared to room temperature. Further, an increase in temperature to 900 °C increased the wear rate significantly due to fast tribo-oxidation accompanied by grooving. The friction coefficient was found to decrease with temperature increasing from 700 to 900 °C due to the formation of oxide scales, which reduce adhesion of asperity contacts. A relationship between the oxidation and wear mechanisms was established using X-ray diffraction, Raman spectroscopy, scanning electron microscopy, surface profilometry, confocal microscopy, and dynamic secondary ion mass spectrometry.

  2. Thermochemical investigations of zirconolite, pyrochlore and brannerite: Three materials relevant to issues of plutonium immobilization

    Science.gov (United States)

    Helean, Katheryn Bridget

    For the purpose of immobilizing plutonium, a crystalline ceramic waste form is being developed that can be described as a pseudo-quaternary system consisting of CaHfTi2O7- CaPuTi2O7- CaUTi2O7- GdTi2O7. High-temperature oxide melt solution calorimetry offers an effective methodology for the determination of enthalpies of formation of rare earth-bearing and other refractory oxides relevant to the proposed waste form. Calorimetric investigations of the waste form end-member phases (using Ce as a Pu analogue) plus brannerite, the major waste form impurity, were conducted using 3Na2O•4MoO3 solvent at 975 K. Standard enthalpies of formation, DeltaH°f (kJ/mol), were derived for three pyrochlore phases: Ca0.93Ce1.00Ti 2.035O7.00 (-3656.0 +/- 5.6), Ca1.46U 4+0.23U6+0.46Ti1.85O 7.00 (-3610.6 +/- 4.1) and Gd2Ti2O 7 (-3822.5 +/- 4.9). Enthalpies of formation with respect to an oxide phase assemblage, DeltaH°f-ox: CaO+MO2+2TiO2=CaMTi2O7 or Gd 2O3+2TiO2=Gd2Ti2O7 , and an oxide/perovskite phase assemblage, DeltaH° f-pv+ox: CaTiO3+MO2+TiO2=CaMTi 2O7, M = Ce, U were also calculated. DeltaH° f-ox (kJ/mol): Gd2Ti2O7 (-113.4 +/- 2.8); Ca1.46U4+0.23U 6+0.46Ti1.85O7.00 (-123.1 +/- 3.4); Ca0.93Ce1.00Ti2.035O7.00 (-54.1 +/- 5.2). DeltaH°f-pv+ox (kJ/mol): Ca1.46U4+0.23U6+ 0.46Ti1.85O7.00 (-5.1 +/- 4.0); Ca 0.93Ce1.00Ti2.035O7.00 (+21.0 +/- 5.5). A significant metastability field was defined with respect to an oxide/perovskite phase assemblage. DeltaH°f (kJ/mol) were derived for two zirconolite phases: CaZr1.03Ti1.97O7 (-3719.4 +/- 3.9) and CaHf1.02Ti1.98O 7 (-3720.5 +/- 3.9). DeltaH° f-ox (kJ/mol): CaZr1.03Ti1.97O7 (-89.6 +/- 2.8); CaHf1.02Ti1.98O7 (-74.8 +/- 3.1). CaZr1.03Ti1.97O7 was stable with respect to a perovskite plus oxides assemblage (DeltaH° f-pv+ox = -8.8 +/- 3.3 kJ/mol). CaHf1.02Ti 1.98O7 was marginally metastable in enthalpy (Delta H°f-pv+ox = +6.0 +/- 3.5 kJ/mol). DeltaH°f (kJ/mol) were derived for three brannerites: CeTi2O6 (-2948.8 +/- 4.3); U0.97Ti2.03O6

  3. Separation of Radiocopper 64/67Cu from the Matrix of Neutron-Irradiated Natural Zinc Applicable for 64Cu Production

    International Nuclear Information System (INIS)

    Radioisotope 64Cu is a promising radiometallic-isotope for molecular-targeted-radiopharmaceuticals. Having a half-life of 12.70 hours and emitting β+-radiation (Eβ+ = 0.6531 MeV) as well as β-ray (Eβ- = 0.5787 MeV), it is widely used in the form of biomedical-substrate-radiopharmaceutical for positron emission tomography (PET) diagnosis and simultaneously for targeted radiotherapy of cancer. The potential needs on the availability of 64Cu-labeled pharmaceuticals for domestic nuclear medicine hospitals lead to a necessity for the local production of carrier-free 64Cu using BATAN's G.A. Siwabessy reactor because of the technical and economical constraints in the production using BATAN's cyclotron. The presented work is accordingly to study whether the radioisotope 64Cu can be produced and separated from the matrix of post-neutron-irradiated-natural zinc. This study is expected can be further improved and implemented in production technology of carrier-free 64Cu based on 64Zn (n,p) 64Cu nuclear reaction exploiting the fast neutron fraction among the major thermal fraction due to unavailability of fast-neutron-irradiation facility in the BATAN's G.A. Siwabessy reactor. The solution of post-neutron-irradiated-natural zinc in 1M acetic acid was loaded into Chelex-100 cation exchanger resin column to pass out the Zn/Zn* fraction whereas the Cu* fraction which remained in the column was then eluted out from the column by using 1.5 M HCl and loaded into the second column containing Dowex-1X8 anion exchanger resin. The second column was then eluted with 0.5 M HCl. The collected eluate was expected to be zinc-free Cu* fraction. It was observed from the half-life and the γ-spectrometric analysis that radioactive copper-64Cu containing 67Cu was produced by neutron activation on the natural Zn-foil target and can be separated from the target matrix by the presented two-steps-column-chromatographic separation technique. The radioactivity measurement showed that wrapping the

  4. Nano confinement induced isotope separation of zinc: density functional theoretical modelling

    International Nuclear Information System (INIS)

    Crown ether has shown potential for isotope separation. Zinc has five stable isotopes of masses 64, 66, 67, 68 and 70 with natural abundances 48.63, 27.90, 4.10, 18.75 and 0.62%, respectively. 64Zn-depleted zinc is used in the primary coolant of nuclear power plant to reduce the formation of radioactive cobalt isotope, 60Co, presence of which leads to radiation threat to the working personal. It will be worthwhile to investigate whether crown ether can also be used for isotope separation of Zinc. DFT based electronic structure calculation using Turbomole package was performed to evaluate the isotope separation factor of Zn with crown ether of different nano confinement. In order to compute the isotope separation factor for any biphasic system we need to know the value of reduced partition function ratio (RPFR) for a pair of isotope in the feed solvent phase and the product complex phase. Hence, first the RPFR of hydrated Zn2+-(H2O)n (n=1-6) cluster system was calculated for different pair of Zn isotope. The computed value of RPFR was found to be increased from n=1 then shows maximum at n=4 and then further reduced. The working value of RPFR at n=4 were taken as 1.0098 for Zn (68/64); 1.005 for Zn (66/64) and 1.0047 for Zn (68/66). The highest separation factor is limited by the value of RPFR in water system. Next, the values of RPFR of complexes of Zn2+ ion with different crown ethers were computed. It is interesting to mention that the RPFR was found to be decreased from B12C4 to DB18C6 for all the pair of Zn isotopes studied here. The RPFR was found to be highest with B12C4 and lowest with DB18C6 leading to lowest separation factor in B12C4 and highest separation factor in DB18C6. Further, the separation factor was found to be highest for Zn (68/64) pair and lowest for Zn (68/66) pair as expected because in the former pair the mass difference is highest. It is worth noting that the RPFR can be correlated with the binding energy and free energy of complexation

  5. Zinc and volatile element loss during planetary magma ocean phases

    Science.gov (United States)

    Dhaliwal, Jasmeet K.; Day, James M. D.; Moynier, Frédéric

    2016-10-01

    Zinc is a moderately volatile element and a key tracer of volatile depletion on planetary bodies due to lack of significant isotopic fractionation under high-temperature processes. Terrestrial basalts have δ66Zn values similar to some chondrites (+ 0.15 to 0.3‰ where [{66Zn/64Znsample/66Zn/64ZnJMC-Lyon-1} × 1000]) and elevated Zn concentrations (100 ppm). Lunar mare basalts yield a mean δ66Zn value of +1.4 ± 0.5‰ and have low Zn concentrations (~2 ppm). Late-stage lunar magmatic products, such as ferroan anorthosite, Mg-suite and Alkali suite rocks exhibit heavier δ66Zn values (+3 to +6‰). The heavy δ66Zn lunar signature is thought to reflect evaporative loss and fractionation of zinc, either during a giant impact or in a magma ocean phase.We explore conditions of volatile element loss within a lunar magma ocean (LMO) using models of Zn isotopic fractionation that are widely applicable to planetary magma oceans. For the Moon, our objective was to identify conditions that would yield a δ66Zn signature of ~ +1.4‰ within the mantle, assuming a terrestrial mantle zinc starting composition.We examine two cases of zinc evaporative fractionation: (1) lunar surface zinc fractionation that was completed prior to LMO crystallization and (2) lunar surface zinc fractionation that was concurrent with LMO crystallization. The first case resulted in a homogeneous lunar mantle and the second case yielded a stratified lunar mantle, with the greatest zinc isotopic enrichment in late-stage crystallization products. This latter case reproduces the distribution of zinc isotope compositions in lunar materials quite well.We find that hydrodynamic escape was not a dominant process in losing Zn, but that erosion of a nascent lunar atmosphere, or separation of condensates into a proto-lunar crust are possible. While lunar volatile depletion is still possible as a consequence of the giant impact, this process cannot reproduce the variable δ66Zn found in the Moon. Outgassing

  6. Separation of Radiocopper 64/67Cu from the Matrix of Neutron-Irradiated Natural Zinc Applicable for 64Cu Production

    Directory of Open Access Journals (Sweden)

    S. Soenarjo

    2012-04-01

    Full Text Available Radioisotope 64Cu is a promising radiometallic-isotope for molecular-targeted-radiopharmaceuticals. Having a half-life of 12.70 hours and emitting β+-radiation (E+ = 0.6531 MeV as well as β—ray (E = 0.5787 MeV, it is widely used in the form of biomedical-substrate-radiopharmaceutical for positron emission tomography (PET diagnosis and simultaneously for targeted radiotherapy of cancer. The potential needs on the availability of 64Cu-labeled pharmaceuticals for domestic nuclear medicine hospitals lead to a necessity for the local production of carrier-free 64Cu using BATAN’s G.A. Siwabessy reactor because of the technical and economical constraints in the production using BATAN’s cyclotron. The presented work is accordingly to study whether the radioisotope 64Cu can be produced and separated from the matrix of post-neutron-irradiated-natural zinc. This study is expected can be further improved and implemented in production technology of carrier-free 64Cu based on 64Zn (n,p 64Cu nuclear reaction exploiting the fast neutron fraction among the major thermal fraction due to unavailability of fast-neutron-irradiation facility in the BATAN’s G.A. Siwabessy reactor. The solution of post-neutron-irradiated-natural zinc in 1M acetic acid was loaded into Chelex-100 cation exchanger resin column to pass out the Zn/Zn* fraction whereas the Cu* fraction which remained in the column was then eluted out from the column by using 1.5 M HCl and loaded into the second column containing Dowex-1X8 anion exchanger resin. The second column was then eluted with 0.5 M HCl. The collected eluate was expected to be zinc-free Cu* fraction. It was observed from the half-life and the -spectrometric analysis that radioactive copper-64Cu containing 67Cu was produced by neutron activation on the natural Zn-foil target and can be separated from the target matrix by the presented two-steps-column-chromatographic separation technique. The radioactivity

  7. Fast neutron radiography using photoluminescent imaging plates

    International Nuclear Information System (INIS)

    Fast neutron radiography (FNR) and resonance neutron radiography (RNR) are complementary to the conventional radiography with high energy gamma-rays or brems-strahlung radiation used for the inspection of thick metal objects. In both non-destructive methods, the contrast sensitivity and the penetration power can be improved by using higher energy neutrons. At present direct techniques based either n Solid State Nuclear Track detectors (SSNTDs) or scintillating screens and transfer techniques using activation threshold detectors and radiographic films are applied for the detection of fast neutron images. Rather low detection sensitivity of film and SSNTD based fast neutron imaging methods and also rather poor inherent image contrast of SSNTD pose a problem for FNR in the fast neutron energy region 1-15 MeV interesting for NDT. For more efficient detection of fast neutron images the use of novel highly sensitive photoluminescent imaging plates (IP) in combination with threshold at the KFKI research reactor. The conventional IP produced by FUJI Photo Film Co. for the detection of beta and X-ray radiation were used. The threshold activation detectors were the reactions 115In(n, n') 115mIn, 64Zn(n,p) 64Cu, 56Fe(n, p)56Mn, 24Mg(n, p)24Na and 27Al(n, α)24Na. These threshold reactions cover the fast neutron energy region between 0,7 MeV and 12 MeV. Pure, commercially available metals 0,1 mm to 0,25 mm thick made of In, Zn, Fe, Mg and Al were used as converter screens. The very high sensitivity of IP, the linearity of their response over 5 decades of exposure dose and the high dynamic digitalisation latitude enabled fast neutron radiography of image quality comparable to the quality of thermal NR. In our experimental conditions (φn∼ 108 n/cm2s, RCd ∼ 2) the neutron exposure and IP exposure periods were still practical and comparable to the half life of the corresponding reaction products (half an hour to several hours). Even with the 27Al(n.α)24Na reaction having a

  8. Lithium-bearing fluor-arfvedsonite from Hurricane Mountain, New Hampshire: A crystal-chemical study

    Science.gov (United States)

    Hawthorne, F.C.; Oberti, R.; Ottolini, L.; Foord, E.E.

    1996-01-01

    The structures of two crystals of Li-bearing fluor-arfvedsonite (1) (K0.32Na0.68)Na2(Li0.48Fe 2+2.83Mn2+0.10Zn 0.06Fe3+1.46Ti0.07) (Si7.88Al0.12)O22[Fu1.15(OH) 0.85] and (2) (K0.25Na0.75)Na2(Li0.48Fe 2+2.84Mn2+0.11Zn 0.05Fe3+1.45Ti0.07)(Si 7.89Al0.11)O22[F1.35(OH) 0.65] from a granitic pegmatite, Hurricane Mountain, New Hampshire, have been refined to R indices of 1.5(1.6)% based on 1380(1387) reflections measured with MoK?? X-radiation. The unit cell parameters are (1) a 9.838(4), b 17.991(6), c 5.315(2) A??, 103.78(3)??, V 913.7 A??3 and (2) a 9.832(3), b 17.990(7), c 5.316(3) A??, ?? 103.79(3)??, V 913.2 A??3. Site-scattering refinement shows Li to be completely ordered at the M(3) site in these crystals. The amphibole composition is intermediate between fluor-arfvedsonite and fluor-ferro-leakeite with a small component (???10%) of fluor-ferro-ferri-nybo??ite. These amphibole crystals project into miarolitic cavities in a pegmatitic phase of a riebeckite granite. The early-crystallizing amphibole is close to fluor-ferro-leakeite in composition, but becomes progressively depleted in Li and F as crystals project out into miarolitic cavities; the final amphibole to crystallize is a fibrous Li-poor riebeckite. Li plays a significant role in late-stage fractionation involving the crystallization of alkali amphibole in peralkaline granitic environments.

  9. Synthesis, characterization and thermochemistry of Cs-, Rb- and Sr-substituted barium aluminium titanate hollandites

    Energy Technology Data Exchange (ETDEWEB)

    Xu, H., E-mail: hxu@lanl.gov [Earth and Environmental Sciences Division, Los Alamos National Laboratory, Los Alamos, NM 87545 (United States); Wu, L. [Peter A. Rock Thermochemistry Laboratory and NEAT ORU, University of California at Davis, Davis, CA 95616 (United States); Zhu, J. [Los Alamos Neutron Science Center, Los Alamos National Laboratory, Los Alamos, NM 87545 (United States); Navrotsky, A. [Peter A. Rock Thermochemistry Laboratory and NEAT ORU, University of California at Davis, Davis, CA 95616 (United States)

    2015-04-15

    Highlights: • Cs-, Rb- and Sr-substituted barium titanate hollandites were synthesized using sol–gel methods. • Chemical compositions were determined by electron microprobe analyses. • Crystal structures were analyzed using powder synchrotron X-ray diffraction coupled with Rietveld refinements. • Enthalpies of formation were measured using high temperature oxide melt solution calorimetry. • Stability relations with respect to BaTiO{sub 3} and SrTiO{sub 3} perovskites and other oxides were determined. - Abstract: Titanate hollandites are of considerable interest for immobilization of radioactive Cs, its daughter product Ba and related radionuclides Rb and Sr. In this study, we synthesized three hollandites, Ba{sub 1.18}Cs{sub 0.21}Al{sub 2.44}Ti{sub 5.53}O{sub 16}, Ba{sub 1.17}Rb{sub 0.19}Al{sub 2.46}Ti{sub 5.53}O{sub 16} and Ba{sub 1.14}Sr{sub 0.10}Al{sub 2.38}Ti{sub 5.59}O{sub 16}, using sol–gel methods. Rietveld analysis of synchrotron XRD data shows that they adopt the tetragonal structure (space group I4/m), and their cell parameters increase with increasing cation size (Sr{sup 2+} → Rb{sup +} → Cs{sup +}). Standard enthalpies of formation of these hollandites were determined from drop solution calorimetric measurements with lead borate as the solvent at 973 K. Their formation enthalpies are similar, consistent with the occurrence of extensive cation substitutions in hollandites. Further energetic analysis with respect to BaTiO{sub 3} and SrTiO{sub 3} perovskites and other oxides reveals decreased thermodynamic stability from Cs- to Rb- to Sr-hollandite. This trend is consistent with the phase assemblage observed in Synroc, where Cs{sup +}, Rb{sup +} and Ba{sup 2+} enter into hollandite, whereas Sr{sup 2+} occurs in perovskite.

  10. Determination of copper isotope ratios by LA-MC-ICP-MS

    International Nuclear Information System (INIS)

    Full text: The stable isotope ratios of metals commonly found in sulphide ore deposits (e.g., Cu, Zn. Fe, Sb, Ag) may be fractionated significantly during ore-forming processes (redox reactions, etc.) and thus provide important information on the source, transport and depositional mechanisms of these metals. However, little work has been done on these isotopic systems because of past analytical difficulties in making precise measurements. Recently developed laser ablation (LA)-multi-collector (MC)-ICP-MS technology now allows routine rapid, in situ determination of the isotope ratios of these metals. This study reports on: (a) the development of an analytical protocol for the measurement of the 65Cu/63Cu ratio of chalcopyrite, (b) preliminary data for samples from a wide range of copper-bearing mineral deposits, and (c) a preliminary study of the spatial distribution of Cu isotope ratios within the Cadia Hill porphyry Cu-Au deposit. The instrumentation used in this study was a Merchantek LUV266 laser sampler operated with either Ar or He as the sample carrier gas. The ablated material was transported into a Plasma MC-ICP-MS for isotopic determination. Instrumental mass bias was corrected using the measured 66Zn/64Zn ratio of a Zn-bearing aerosol added continuously to the ablated sample carrier gas flow via a T-junction. The isotopes of copper (and other metals) are fractionated significantly by volatilisation and condensation processes operative during the laser sampling/transport processes, both of which favour depletion of 65Cu relative to 63Cu in the transported material. This fractionation may be reduced by using high laser pulse energies, low repetition rates and, most significantly, by ablation in He, which reduces dramatically the condensation blanket of sulphidic material around the ablation site. Using these conditions, relatively stable Cu isotope ratios may be maintained over a long ablation period (up to 4 minutes). However, absolute ratios are still

  11. Twenty years of operation of Ljubljana's TRIGA Mark II reactor

    International Nuclear Information System (INIS)

    Twenty years have now passed since the start of the TRIGA Mark II reactor in Ljubljana. The reactor was critical on May 31, 1966. The total energy produced until the end of May 1986 was 14.048 MWh or 585 MWd. For the first 14 years (until 1981) the yearly energy produced was about 600 MWh, since 1981 the yearly energy produced was 1000 MWh when a routine radioactive isotopes production started for medical use as well as other industrial applications, such as doping and irradiation with fast neutrons of silicon monocrystals, production of level indicators (irradiated cobalt wire), production of radioactive iridium for gamma-radiography, leak detection in pipes by sodium, etc. Besides these, applied research around the reactor is being conducted in the following main fields, where- many unique methods have been developed or have found their way into the local industry or hospitals: neutron radiography, neutron induced auto-radiography using solid state nuclear track detectors, nondestructive methods for assessment of nuclear burn-up, neutron dosimetry, calculation of core burn-up for the optimal in-core fuel management strategy. The solvent extraction method was developed for the everyday production of 99mTc, which is the most widely used radionuclide in diagnostic nuclear medicine. The methods were developed for the production of the following isotopes: 18F, 85mKr, 24Na, 82Br, 64Zn, 125I. Neutron activation analysis represents one of the major usages for the TRIGA reactor. Basic research is being conducted in the following main fields: solid state physics (elastic and inelastic scattering of the neutrons), neutron dosimetry, neutron radiography, reactor physics and neutron activation analysis. The reactor is used very extensively as a main instrument in the Reactor Training Centre in Ljubljana where manpower training for our nuclear power plant and other organisations has been performed. Although the reactor was designed very carefully in order to be used for

  12. Biogeochemical Processes Related to Metal Removal and Toxicity Reduction in the H-02 Constructed Wetland, Savannah River Site

    Science.gov (United States)

    Burgess, E. A.; Mills, G. L.; Harmon, M.; Samarkin, V.

    2011-12-01

    The H-02 wetland system was designed to treat building process water and storm water runoff from multiple sources associated with the Tritium Facility at the DOE-Savannah River Site, Aiken, SC. The wetland construction included the addition of gypsum (calcium sulfate) to foster a sulfate-reducing bacterial population. Conceptually, the wetland functions as follows: ? Cu and Zn initially bind to both dissolved and particulate organic detritus within the wetland. ? A portion of this organic matter is subsequently deposited into the surface sediments within the wetland. ? The fraction of Cu and Zn that is discharged in the wetland effluent is organically complexed, less bioavailable, and consequently, less toxic. ? The Cu and Zn deposited in the surface sediments are eventually sequestered into insoluble sulfide minerals in the wetland. Development of the H-02 system has been closely monitored; sampling began in August 2007, shortly after its construction. This monitoring has included the measurement of water quality parameters, Cu and Zn concentrations in surface water and sediments, as well as, characterization of the prokaryotic (e.g., bacterial) component of wetland biogeochemical processes. Since the beginning of the study, the mean influent Cu concentration was 31.5±12.1 ppb and the mean effluent concentration was 11.9±7.3 ppb, corresponding to an average Cu removal of 64%. Zn concentrations were more variable, averaging 39.2±13.8 ppb in the influent and 25.7±21.3 ppb in the effluent. Average Zn removal was 52%. The wetland also ameliorated high pH values associated with influent water to values similar to those measured at reference sites. Seasonal variations in DOC concentration corresponded to seasonal variations in Cu and Zn removal efficiency. The concentration of Cu and Zn in the surface layer of the sediments has increased over the lifetime of the wetland and, like removal efficiency, demonstrated seasonal variation. Within its first year, the H-02

  13. Experimental Research on Magnetic Separation of Ilmenite Placer of Yun Nan%云南钛铁矿砂矿磁选试验研究

    Institute of Scientific and Technical Information of China (English)

    徐明; 张渊; 傅文章; 洪秉信

    2011-01-01

    The main useful components of ilmenite placers of Yun Nan are ilmenite and titanium magnetite and the ores are extremely sliming. Experimental research on magnetic separation for this ore was adopted. When the technology of selective scrubbing dissociation was carried on, +0.030mm products of 35. 31%TiO2 with the yield of 78.25% and -0.030mm products of 8.46% TiO2 with the yield of 21.75% were obtained respectively. Directed at + 0.030mm products,low -intensity magnetic separation was adopted to remove iron,the tailings of which was carried on titanium beneficiation by adopting the technology of grading-high - intensity magnetic separation and the concentrate was carried on separating iron and titanium by using low - intensity magnetic separation-high - intensity magnetic separation. Directed at the -0.030mm products,fine particle titanium separation was carried on by using the technology of desliming-magnetic separation. Finally, titanium concentrate of 48. 83%TiO2 with recovery of 85.51% and iron concentrate of 56.62% Tfe with recovery of 25.17% were obtained. This technology is rational and feasible and the separation index is satisfactory.%云南钛铁矿石中主要有用矿物为钛铁矿、钛磁铁矿,矿石泥化较严重,针对该矿石进行了磁选试验研究.对原矿采用选择性擦洗解离,可以得到TiO2品位35.31%,产率78.25%的+0.030mm产品及TiO2品位8.46%,产率21.75%的-0.030mm产品.+0.030mm粒级采用弱磁除铁,弱磁尾矿采用分级-强磁选工艺进行选钛试验,对弱磁精矿再磨后采用弱磁-强磁工艺进行钛、铁分离;-0.030mm粒级采用脱泥-磁选工艺进行细粒选钛试验.最终可得到TiO2品位48.83%的钛精矿,回收率85.51%,TFe晶位56.62%的铁精矿,回收率25.17%.该工艺合理可行,选矿指标较为理想.

  14. ZZ IRDF-2002, 640-Group Cross-Section Library and Spectra for Dosimetry Calculation in ENDF-6 Format. ZZ IRDF-2002-ACE, Cross-Section Library and Spectra for Dosimetry Calculation in ACE Format for Monte Carlo methods. ZZ IRDF-90, 640-Group Cross-Section Library and Spectra for Dosimetry Calculation in ENDF-6 Format. ZZ IRDF-82, 620-Group Cross-Section Library and Spectra for Dosimetry Calculation in ENDF-5 Format

    International Nuclear Information System (INIS)

    sections, using the SAND-II group structure. (2) The reactions 19F(n,2n), 24Mg(n,p), 31P(n,p), 29Cu(n,2n), 64Zn(n,p), 90Zr(n,2n), 93Nb(n,n') and 103(Rh(n,n'), supplied by Vonach. This data was converted to the ENDF/B-V Format, which in turn was converted to 620 group form. (3) The reaction 23Na(n,2n) provided by Marcinkowski. This data was converted to the ENDF/B-V Format (5) and then converted to 620 group Format. (4) The reaction 241Am(n,f) as supplied by Patrick. This data was converted to the ENDF/B-V Format at Stuttgart and then converted to 620 group form. (5) ASTM and EUR standards damage Cross sections for iron as provided by Zijp (10) in the form of 620 group Cross sections. This data was converted to the ENDF/B-V Format. II) The Benchmark Spectra library contains ten benchmark spectra, including: (1) The NBS 252Cf spontaneous fission; the NBS 235U and ENDF/B-V 235U thermal fission, the Intermediate-Energy Standard Neutron Field (ISNF), the Coupled Fast Reactivity Measurement Facility (CFRMF), the 10 % Enriched Uranium Cylindrical Critical Assembly (BIG-TEN) and the Coupled Thermal/Fast Uranium and Boron Carbide Spherical Assembly (SIGMA-SIGMA) spectra, all of which were provided by Eisenhauer in 620 group form. (2) The ORR and YAYOI Spectra, which were provided by Greenwood in 100 group form. (3) The Central Zone Flux of the NEACRP Benchmark Spectra provided by Goel in 208 group form. - (B) ZZ-IRDF-90: The following changes compared to the 1982 version should be noted: - IRDF-90 is mainly based on the ENDF/B-IV data and its present version contains cross section values for 51 different dosimetry reactions. Damage Cross sections are given for three different materials: Fe, Cr, Ni. - The library is written in the ENDF-6 Format. - Gas production reactions are completely missing from IRDF-90.V.1 and other important dosimetry reactions are also not yet present. At the same time, double cross section information is given for the following reactions Ni582, Cu632 and Fe

  15. Overview

    International Nuclear Information System (INIS)

    of the baryonic chemical potential consistently decreases down to the value of μB = 29 MeV at the collision energy √sNN = 200 GeV for the Au + Au system. The time scale of the thermal multifragmentation of 197Au nuclei induced by a fast proton of the energy of 8.1 GeV was established. It was proved that it is a fast process, with characteristic decay time τ of the order of 10-22 s. The first observation of the Jacobi shape transition accompanying the fast rotation of the 46Ti nucleus was made. For the first time, non-hem iron was found in the low - spin state of Fe2+ which indicates that NHFe initiates the cyclic transport of electrons in photosystem II. The result was published in Applied Organometallic Chemistry. The medium T-matrix theory was developed for superfluid nuclear matter. This new theoretical achievement was published in Phys. Rev. C. Using the ''ab initio'' method for structure calculation of the FeBO3 compound, a special phase transition with spatial group symmetry unchanged, was found for the metal - isolator and magnetic - nonmagnetic cases. The advantage of the ''ab initio'' method is that the phase transition can be studied in the region of pressure values often difficult to access experimentally. A high level of the concentration of Pu and Am was found in sculls of prehistoric fossil animals. Legal accreditation for measuring individual radiation doses was granted to our second laboratory. Together with the laboratory for scaling and legalizing portable dosimeters, it should resume public services in 2003, hopefully providing some additional income for the Institute. Two doctors obtained their habilitation degrees, and three Associate Professors became full Professors. A group of laboratories from different departments formed a Centre of Excellence in the field of the Quality of Life, which was approved by the European Union. This may help us to obtain additional money for research as well. The Henryk Niewodniczanski prize was given to Dr

  16. 41Ca in Circumstellar Graphite from Supernovae

    Science.gov (United States)

    Amari, S.; Zinner, E.; Lewis, R. S.

    1995-09-01

    We have measured isotopic ratios of C, N, O, Si, K, Ca, and Ti in 13 carbon grains from the low density graphite fraction KE3 (1.65-1.72g/cm3). These grains show the same isotopic signatures as KE3 grains previously measured [1]. Many of them have isotopically heavy C (up to x13 solar) and heavy N (up to x9.7 solar); nine have ^18O excesses (up to x183 solar); 26Al/27Al ratios range up to 0.07. Type II supernovae have previously been proposed as stellar sources of low density graphite grains [1,2,3]. Grain KE3c-551 (14 micrometers in size) has the most extreme C-, N-, and O-isotopic ratios ever measured in a graphite grain (^12C/^13C=7223+/-111, 14N/15N=28+/-2, 16O/18O=2.72+/-0.08). Interestingly, the isotopic ratios of these elements changed during analysis, becoming more anomalous with time. This suggests that isotopically "normal" components had been absorbed onto the grain surface or that partial exchange of the indigenous component had occurred. The above ratios are therefore lower (for C) and upper (for N and O) limits. High ^12C/^13C and ^16O/^17O (4595+/-858) and low ^16O/^18O ratios as well as the Ti isotopic ratios of the grain (delta 46Ti/48Ti=12+/-10 permil, delta ^47Ti/^48Ti=-62+/-9 permil, delta ^49Ti/^48Ti=901+/-16 permil, delta ^50Ti/^48Ti=200+/-12 permil) show the signature of the He/C zone in presupernova stars [4]. Eleven grains were measured for their K, Ca, and Ti isotopic ratios. Four of them, including KE3c-551, have ^41K excesses (218+/-50 permil to 10610+/-326 permil), apparently due to the decay of ^41Ca (T(sub)1/2=1.03 x 10^5a). Inferred ^41Ca/^40Ca ratios range from (1.94+/-0.43) x 10^-3 to (1.65+/-0.38) x 10^-2. In supernovae, ^41Ca is produced by neutron capture in the He/C, the O/C, and the O/Ne zones, as well as by explosive nucleosynthesis in the Si/S zone [4,5]. The expected ^41Ca/^40Ca ratios in the neutron capture zones are 1.6-1.8 x 10^-2 and in the Si/S zone 8 x 10^-4. Two of the 4 grains with ^41K excesses have Ca isotopic

  17. ZZ KASHIL-E70, 199 N, 42 Photon Groups Cross Sections in MATXS Format Based on ENDF/B-VII.0 for Shielding Applications

    International Nuclear Information System (INIS)

    1 - Description: Format: MATXS, 204 nuclides processed with NJOY99.245. Number of groups: 199 neutron-, 42 photon-groups. 204 Nuclides including 8 thermal scattering law data: H-1, H-2, H-3, He-3, He-4, Li-6, Li-7, Be-9, Be-9, Be-9, B-10, B-11, C-nat, C-nat, N-14, N-15, O-16, O-17, F-19, Na-23, Mg-24, Mg-25, Mg-26, Al-27, Si-28, Si-29, Si-30, P-31, S-32, S-33, S-34, S-36, Cl-35, Cl-37, K-39, K-40, K-41, Ca-40, Ca-42, Ca-43, Ca-44, Ca-46, Ca-48, Sc-45, Ti-46, Ti-47, Ti-48, Ti-49, Ti-50, V-nat, Cr-50, Cr-52, Cr-53, Cr-54, Mn-55, Fe-54, Fe-56, Fe-57, Fe-58, Co-59, Ni-58, Ni-60, Ni-61, Ni-62, Ni-64, Cu-63, Cu-65, Ga-69, Ga-71, Y-89, Zr-90, Zr-91, Zr-92, Zr-94, Zr-96, Nb-93, Mo-92, Mo-94, Mo-95, Mo-96, Mo-97, Mo-98, Mo-100, Pd-102, Pd-104, Pd-105, Pd-106, Pd-108, Pd-110, Ag-107, Ag-109, Cd-106, Cd-108, Cd-110, Cd-112, Cd-113, Cd-114, Cd-116, In-113, In-115, I-127, Xe-124, Xe-126, Xe-128, Xe-129, Xe-130, Xe-131, Xe-132, Xe-134, Xe-136, Cs-133, Ba-138, Pr-141, Nd-143, Nd-145, Nd-146, Nd-148, Nd-150, Pm-147, Sm-147, Sm-151, Sm-152, Eu-151, Eu-152, Eu-153, Eu-154, Eu-155, Gd-152, Gd-154, Gd-155, Gd-156, Gd-157, Gd-158, Gd-160, Dy-164, Ho-165, Lu-175, Lu-176, Hf-174, Hf-176, Hf-177, Hf-178, Hf-179, Hf-180, Ta-181, Ta-182, W-182, W-183, W-184, W-186, Re-185, Re-187, Ir-191, Ir-193, Au-197, Pb-206, Pb-207, Pb-208, Bi-209, Th-230, Th-232, Pa-231, Pa-233, U-232, U-233, U-234, U-235, U-236, U-237, U-238, Np-237, Np-238, Np-239, Pu-236, Pu-237, Pu-238, Pu-239, Pu-240, Pu-241, Pu-242, Pu-243, Pu-244, Am-241, Am-242, Am-242m, Am-243, Cm-241, Cm-242, Cm-243, Cm-244, Cm-245, Cm-246, Cm-247, Cm-248, Bk-249, Cf-249, Cf-250, Cf-251, Cf-252, Cf-253, Es-253. Origin: ENDF/B-VII.0. Weighting spectrum: 300, 600, 1000, 2100 K. The KASHIL-E70 is a MATXS-format, 199-group neutron and 42-group photon cross section library for shielding applications based on ENDF/B-VII.0. The library contains 204 nuclide data including 8 thermal scattering law data processed by the NJOY99.259 code patched with NEA

  18. Overview

    International Nuclear Information System (INIS)

    the first time. Many topics were covered, like: physics of the W bosons and four-fermion processes at LEP2/TESLA energies, as well as two-fermion production processes at both present and future colliders. A detailed analysis of the response of detectors like ATLAS to the supersymmetric particles possibly created in p-p collisions at LHC energies was performed. Several experiments at the HERA collider at DESY based on the model calculations by our theorists were performed. The nuclear structure studies were conducted mainly with the use of multidetector arrays (GASP, GAMASPHERE, HECTOR and EUROBALL). The experimental data from GDR on highly excited 46Ti nuclei and their comparison with model predictions involving thermal shape fluctuations seem to indicate a Jacobi transition at high angular momenta to very elongated prolate shape. Among the achievements in the physics of condensed matter, a new evidence of a low-energy excitation, the so-called boson peak, was found by neutron scattering in glass-forming organic materials like cyclohexanol, glycerol, neohexanol, and in some mezogenic compounds. Perturbed angular correlation measurements of the Fe3Sn compounds revealed a unique quadrupole interaction above the Curie point and a combined interaction with the magnetic field of 435 kG below this point. The first-principle calculations of structure and dynamics of crystals were continued. Within this approach it has been shown that the perovskite structure of MgSiO3 remains stable to the highest pressure of 150 GPa present in the Earth, where MgSiO3 makes up 64% of the volume. Intermediate phase under pressure was formed between NaCl- and CsCl-type phase transitions of AgBr crystal. For the first time the phonon dispersion curves were calculated for ZnSnP2 and Mg2Si04 crystals. We joined two new international collaborations i.e. project AUGER (search for the highest-energy particles in the Universe) and project ICARUS (search for high-energy-accelerator neutrino