Energy Technology Data Exchange (ETDEWEB)
A 2-stage cold (non-tritium) PMR system was tested with the ITER mix in61 days of continuous operation. No decrease in performance was observed over the duration of the test. Decontamination factor (DF) was found to increase with decreasing inlet rate. Decontamination factors in excess of 1.4 {times} 10{sup 5} were obtained, but the exact value of the highest DF could not be determined because of analysis limitations. Results of the 61-day test were used to design a 2-stage PMR system for use in tritium testing. The PMR system was scaled up by a factor of 6 and built into a glovebox in the Tritium Systems Test Assembly (TSTA) of the Los Alamos National Laboratory. This system is approximately 1/5th of the expected full ITER scale. The ITER mix was injected into the PMR system for 31 hours, during which 4.5 g of tritium were processed. The 1st stage had DF = 200 ...
1996-12-31
International Nuclear Information System (INIS)
A 2-stage cold (non-tritium) PMR system was tested with the ITER mix in 61 days of continuous operation. No decrease in performance was observed over the duration of the test. Decontamination factor (DF) was found to increase with decreasing inlet rate. Decontamination factors in excess of 1.4x10"5 were obtained, but the exact value of the highest DF could not be determined because of analysis limitations. Results of the 61-day test were used to design a 2-stage PMR system for use in tritium testing. The PMR system was scaled up by a factor of 6 and built into a glovebox in the Tritium Systems Test Assembly (TSTA) of the Los Alamos National Laboratory. This system is approximately 1/5"t"h of the expected full ITER scale. The ITER mix was injected into the PMR system for 31 hours, during which 4.5 g of tritium were processed. The 1"s"t stage had DF =200 and the ...
1996-06-16
Behavior of tritium in the Purex process
Energy Technology Data Exchange (ETDEWEB)
The tri-n-butyl phosphate(TBP) extraction behavior of tritium was studied to support the evaluation of tritium confinement in the Purex process. The tritium distribution ratio in the system of U - 30% TBP/n-dodecane(nDD) - HNO[sub 3] [minus]H[sub 2]O was measured in batch-wise experiments. The tritium decontamination factor in a tritium scrubbing step was measured in chemical flow sheet experiments using a 6 stage mixer-settler having an internal recycle system of aqueous solution in each stage. Tritium was mainly extracted in the forms of water and nitric acid in the system. Less than 1% of the amount of tritium in the organic phase was fixed in the degradation products of the solvent. A tritium decontamination factor of about 500 in the tritium scrubbing ...
1995-01-01
Tritium contamination and decontamination study on materials for ITER remote handling equipment
Energy Technology Data Exchange (ETDEWEB)
Several materials, lenses, dry bearings and cables were exposed to a tritiated moisture environment to study the behavior of tritium contamination on candidate materials for ITER remote handling equipment. To optimize the tritium removal procedure, decontamination experiments using a gas purge with three different moisture concentrations were also performed. The surface tritium concentrations of CeO{sub 2} containing alkaline barium glass (NB), CeO{sub 2} containing lead glass (LX) and synthetic quartz (Quartz) after the exposure experiments were 7.80, 10.94 and 0.67 Bq/cm{sup 2}, respectively. It was found that the tritium concentration was influenced by the compositions of the materials. The concentrations of tritium on type 831 (solid lubrication material: graphite) and type 237 (solid lubrication material: tungsten disulfate) dry bearings after the exposure ...
2001-09-01
Tritium contamination and decontamination study on materials for ITER remote handling equipment
International Nuclear Information System (INIS)
Several materials, lenses, dry bearings and cables were exposed to a tritiated moisture environment to study the behavior of tritium contamination on candidate materials for ITER remote handling equipment. To optimize the tritium removal procedure, decontamination experiments using a gas purge with three different moisture concentrations were also performed. The surface tritium concentrations of CeO_2 containing alkaline barium glass (NB), CeO_2 containing lead glass (LX) and synthetic quartz (Quartz) after the exposure experiments were 7.80, 10.94 and 0.67 Bq/cm"2, respectively. It was found that the tritium concentration was influenced by the compositions of the materials. The concentrations of tritium on type 831 (solid lubrication material: graphite) and type 237 (solid lubrication material: tungsten disulfate) dry bearings after the exposure experiments ...
2001-09-01
Estimating the tritiated hydrocarbon decontamination factor by heavy methane
International Nuclear Information System (INIS)
As part of the start up of Los Alamos National Laboratory's new tritium-handling facility, the efficiency of a catalytic oxidation tritium decontamination system was investigated using deuterated methane. The tests were performed during the start up of the facility to confirm the operability of the system before introducing tritium and to provide a baseline for comparison. Techniques and instruments normally used for atmospheric tracer experiments using deuterated methane were applied virtually without modification. The sensitivity of this method allowed preliminary checks at the sub-ppm (v/v) level.
Tritium tests with a technical PERMCAT for final clean-up of ITER exhaust gases
Energy Technology Data Exchange (ETDEWEB)
One of the design targets for the ITER Tokamak Exhaust Processing system is not to lose more than 10{sup -5} g h{sup -1} into the Normal Vent Detritiation System of the Tritium Plant. The plasma exhaust gas, therefore, needs to be processed in a way that an overall tritium removal efficiency of about 10{sup 8} is reached. Such a high decontamination factor can only be achieved by multistage processes. The third step of the three step CAPER process developed at the TLK is based on a so-called permeator catalyst (PERMCAT) reactor, a direct combination of a Pd/Ag permeation membrane and a catalyst bed. The PERMCAT principle is based on isotopic swamping in a counter current mode. Previous tritium experiments employing laboratory scale PERMCAT reactors have revealed decontamination factors as high as 10{sup 5} for the third CAPER step. First tritium tests with a ...
2003-09-01
Tritium tests with a technical PERMCAT for final clean-up of ITER exhaust gases
International Nuclear Information System (INIS)
One of the design targets for the ITER Tokamak Exhaust Processing system is not to lose more than 10"-"5 g h"-"1 into the Normal Vent Detritiation System of the Tritium Plant. The plasma exhaust gas, therefore, needs to be processed in a way that an overall tritium removal efficiency of about 10"8 is reached. Such a high decontamination factor can only be achieved by multistage processes. The third step of the three step CAPER process developed at the TLK is based on a so-called permeator catalyst (PERMCAT) reactor, a direct combination of a Pd/Ag permeation membrane and a catalyst bed. The PERMCAT principle is based on isotopic swamping in a counter current mode. Previous tritium experiments employing laboratory scale PERMCAT reactors have revealed decontamination factors as high as 10"5 for the third CAPER step. First tritium tests with a technical scale ...
2003-09-01
Ultra High Strength Beta Titanium Alloy for Fasteners.
... Accession Number : ADD151811. Title : Ultra High Strength Beta Titanium Alloy for Fasteners. Descriptive Note : Journal article,. ...
Development of the ELEX process for tritium separation at reprocessing plants
International Nuclear Information System (INIS)
The ELEX process for isotopic enrichment and separation of tritium from aqueous reprocessing effluents is described. After the development of an appropriate hydrophobic catalyst and the study of the separate constituent steps of the ELEX process, an integrated bench-scale installation with a detritiation capacity of 10 mol water per hour was constructed. It comprises essentially a 1.5 kW electrolyser and two 2 cm diameter by 3 m high exchange columns. In this mini-pilot the ELEX process was successfully demonstrated by detritiating more than 1000 dm"3 water containing up to 100 mCi tritium per dm"3, which is the feed concentration expected for application of the process in a reprocessing plant. The process decontamination factor was always larger than 100 and the overall tritium balance could be kept within the experimental errors of the various measurements. Depending on the duration of the runs, the ...
1985-03-01
Development of ultrafiltration and adsorbents: October 1979-March 1980
Energy Technology Data Exchange (ETDEWEB)
Tests on a sample of trench water from the Maxey Flats burial ground effectively demonstrated the new Reverse Osmosis Pilot Plant. The effluent from the 50% salt-rejection membrane was decontaminated well enough with the exception of tritium to be discharged to the environment. The performance of the 97% salt-rejection membrane was superior to that of the 50% membrane. A breakthrough and capacity experiment was conducted with Durasil 10 on a simulated Three Mile Island solution. The maximum decontamination factor was extrapolated to be 10/sup 6/, which would reduce the cesium level of TMI water to below the discard limit. Capacity (1/DF = 0.5) was reached at 1260 column volumes. Several adsorbents were tested in the engineering columns for decontamination of cesium-bearing solutions. Under the conditions of the experiment, these adsorbents were ineffective in removing cesium from the solution.
1980-07-02
Detritiation of solid waste using superheated steam
International Nuclear Information System (INIS)
Full text: During JET operations, tritium contaminated waste is generated principally but not exclusively from 'intervention' work and from removing or replacing redundant items. It is essential for JET and for any future fusion plant to have available a route for managing each waste stream however large or small, both during operation and decommissioning of the plant. The long term outcome is to have for each tritiated waste stream from JET a route for its management leading to its eventual disposal or recycling (and thus to be available for similar waste streams which will be produced by ITER operations). Since several years SCK#centre dot#CEN has been developing techniques for the treatment of tritiated waste. Amongst them, technologies for water detritiation, for the treatment of tritiated organic liquids and for the decontamination of several types of solid tritiated waste. Our R and D focuses on the development of a system to ...
2005-10-12
Surface Decontamination by Solution
International Science & Technology Center (ISTC)
Development of Technology for Metal Surface Decontamination in Aqueous Solutions
Energy Technology Data Exchange (ETDEWEB)
The ingestion pathway consequences following an accidental tritium release from the Savannah River Site Tritium Facilities are evaluated.
1999-05-18
IAEA RESEARCH CONTRACTS FIRST ANNUAL REPORT. Technical reports Series No. 4
Summaries are included of research contracts which expired prior to Dec. 31, 1960. The contracts were concerned with investigations of: electrophysiological responses of biological systems in nerve cells to irradiation with small doses of ionizing radiations; the mode of the protective action of certain sulfhydryl compounds against radiation effects on the synthesis of deoxyribonucleic acid, using tritium-labeled thymidine; development of a bubble chamber method of monitoring and dosimetry for Low fast neutron fluxes; effects of incorporated radioisotopes on the stability of genetic materials; interrelation of root and leaf absorption of radioisotopes in herbaceous plants; uptake of radioactive wastes by lowland rice from soils contaminated by irrigation water, and decontamination of the rice; and comparison between mutation rates induced by acute and chronic gamma irradiations. (B.O.G.)
1961-01-01
Absorption-Electrochemical Surface Decontamination
International Science & Technology Center (ISTC)
Development of a Comprehensive Decontamination Database and an Absorption-Electrochemical Metal Surface Decontamination Technique Combining Chemical and Electrochemical Process
Core technologies for Tritium removal processes (I).
In case of operating both Wolsung Nuclear Units 1 and 2 without operating tritium removal facilities, it is estimated that tritium in 2013 would be accumulated up to about 30 million Ci that would result in about 2,300 man-rem of tritium exposure to opera...
1992-01-01
Tritium monitor with improved gamma-ray discrimination
Energy Technology Data Exchange (ETDEWEB)
Apparatus and method for selective measurement of tritium oxide in an environment which may include other radioactive components and gamma radiation, the measurement including the selective separation of tritium oxide from a sample gas through a membrane into a counting gas, the generation of electrical pulses individually representative by rise times of tritium oxide and other radioactivity in the counting gas, separation of the pulses by rise times, and counting of those pulses representative of tritium oxide. The invention further includes the separate measurement of any tritium in the sample gas by oxidizing the tritium to tritium oxide and carrying out a second separation and analysis procedure as described above.
1985-01-01
International Science & Technology Center (ISTC)
Development of Method and Technical Project of the Plant for Thermo-Vacuum Desorption of Tritium Oxide (HTO) from the Environmental Samples
Decontamination of nuclear facilities
International Nuclear Information System (INIS)
Thirty-seven papers were presented at this conference in five sessions. Topics covered include regulation, control and consequences of decontamination; decontamination of components and facilities; chemical and non-chemical methods of decontamination; and TMI decontamination experience.
1982-09-19
Ultra high field magnetic resonance imaging
International Nuclear Information System (INIS)
Understanding human brain function, brain development and brain dysfunction is one of the great challenges of the twenty first century. Biomedical imaging has now run up against a number of technical constraints that are exposing limits to its potential. In order to overcome the current limits to high-field magnetic resonance cerebral imaging (MRI) and unleash its fullest potential, the Cea has built NeuroSpin, an ultra-high-field neuroimaging facility at its Saclay centre (in the Essonne). NeuroSpin already boasts three fully operational MRI systems. The first is a 3-tesla high-field system and the second is a very-high-field 7-tesla system, both of which are dedicated to clinical studies and investigations in humans, while the third is an ultra-high-field 17.65-tesla system designed for studies on small animals. In 2011, NeuroSpin will be commissioning an 11.7-tesla ultra-high-field system of unprecedented power that is ...
Optimization of decontamination strategy for CANDU-PHW reactors
International Nuclear Information System (INIS)
Theoretical models of the decontamination process are developed and combined with an existing model of "6"0Co production in CANDU PHW reactors to predict the effects of decontamination on long term "6"0Co build-up in reactor primary heat transport systems. The effects of decontamination interval, decontamination factor, and post-decontamination corrosion release are calculated. An optimum decontamination strategy for a Pickering G.S. type reactor is developed on the basis of a cost-benefit analysis. This study indicates that the optimum decontamination interval is approximately six years. This optimum interval is relatively insensitive to variations in the costs of personnel exposure, the cost of a decontamination, the decontamination factor, and the post-decontamination ...
Development on the technology for tritium removal processes (II).
In order to decrease tritium exposure to workers, the ratio of which is up to 40% of total exposure, tritium removal facility is getting to be one of the considerable parameters in Korea, due to the next CANDUs to be operated at Wolsung NPP. For investiga...
1993-01-01
While tritium exposure to the site-workers in Wolsung NPP is up to about 40% of the total personnel exposure, Ministry of Science and Technology has asked tritium removal facility for requirement of post heavy-water reactor construction. For the purpose o...
1995-01-01
Development on the core technologies for tritium removal processes (I).
At Wolsung NPP, three more CANDU reactors will be operated soon, and the tritium accumulation in the moderator and coolant systems was estimated to be greatly increased. In order to reduce tritium exposure for nuclear safety at Wolsung, a study was carrie...
1993-01-01
BEATRIX-II: In situ tritium test
Energy Technology Data Exchange (ETDEWEB)
The BEATRIX-II irradiation experiment is an in-situ tritium release experiment being carried out in the Fast Flux Test Facility (FFTF) reactor to evaluate the tritium release characteristics of fusion solid breeder materials. A sophisticated tritium gas handling system has been developed to continuously monitor the tritium recovery from the specimens and facilitate tritium removal from the experiment's sweep gas flow stream. The in-situ recovery experiment accommodates two different in-reactor specimen canisters with individual gas streams and temperature monitoring/control. Ionization chambers have been specifically designed to respond to the rapid changes in the tritium release rate at the anticipated tritium concentrations. Two ceramic electrolysis cells have proved effective in reducing the moisture in the gas streams to ...
1990-01-01
Uptake of atmospheric tritium by market foods
Energy Technology Data Exchange (ETDEWEB)
In this paper uptake of tritium by market foods from tritiated water vapor in the air is investigated using cereals and beans purchased in Deep River, Canada. The concentrations of tissue free water tritium (TFWT) and organically bound tritium (OBT) range from 12 to 79% and from 10 to 38% respectively, of that estimated for atmospheric water vapor of the sampling month. The specific activity ratios of OBT to TFWT were constant for cereals, but variable for beans. The elevated OBT was shown to be the result of isotopic exchange of labile hydrogen by the fact that washing the foods with tritium free-water reduced their tritium contents to levels characteristic of their production sites.
1992-03-01
Factoring Potential Accelerator Transmutation of Waste Demonstrations into Accelerator Production of Tritium Design Planning
1998-01-01
International Nuclear Information System (INIS)
During the water detritiation process most of the tritium inventory is transferred from water into the gaseous phase, then it is further enriched and finally extracted and safely stored. The control of tritium inventory is an acute issue from several points of view: - Financially - tritium is an expensive material; - Safeguard - tritium is considered as nuclear material of strategic importance; - Safety - tritium is a radioactive material: requirements for documented safety analysis report (to ensure strict limits on the total tritium allowed) and for evaluation of accident consequences associated with that inventory. Large amounts of tritium can be stored, in a very safely manner, as metal tritides. A bench-scale experiment of a tritium storage bed with integrated system for in-situ tritium ...
2009-10-12
Ultra-high pressure water jet: Baseline report
International Nuclear Information System (INIS)
The ultra-high pressure waterjet technology was being evaluated at Florida International University (FIU) as a baseline technology. In conjunction with FIU's evaluation of efficiency and cost, this report covers the evaluation conducted for safety and health issues. It is a commercially available technology and has been used for various projects at locations throughout the country. The ultra-high pressure waterjet technology acts as a cutting tool for the removal of surface substrates. The Husky trademark pump feeds water to a lance that directs the high pressure water at the surface to be removed. The safety and health evaluation during the testing demonstration focused on two main areas of exposure. These were dust and noise. The dust exposure was found to be minimal, which would be expected due to the wet environment inherent in the technology, but noise exposure was at a significant level. Further testing for noise is recommended because of ...
1997-07-01
Railgun. Challenge to ultra-high speed; Railgun. Chokosoku eno chosen
Energy Technology Data Exchange (ETDEWEB)
A railgun has an armature driven between two rail-like conductors. In other words, it is a linear drive device system that drives airframes by using the Lorentz`s force. The system is expected as a next-generation high-speed transport means, or as a means to create such ultimate fields as ultra-high pressures, ultra-high temperatures, and ultra-ferromagnetic fields. This paper is a report on investigations on the relevant technological trends as surveyed by the investigation committee at the Institute of Electrical Engineers of Japan using research reports published inside and outside the country. The reported themes cover explanations from the construction to the pulse power supply that forms the core of the technology, problems in switching, recent status of research and development, and to application fields. Compatibility in the high-level electrical and mechanical performances demanded in the railgun is not as easy as has been anticipated ...
1995-09-12
Phantom and animal imaging studies using PLS synchrotron X-rays
Ultra-high resolution radiographs can be obtained using synchrotron X-rays. A collaboration team consisting of K-JIST, POSTECH and YUMC has recently commissioned a new beamline (5C1) at Pohang Light Source (PLS) in Korea for medical applications using phase contrast radiology. Relatively simple image acquisition systems were set up on 5C1 beamline, and imaging studies were performed for resolution test patterns, mammographic phantom, and animals. Resolution test patterns and mammographic phantom images showed much better image resolution and quality with the 5C1 imaging system than the mammography system. Both fish and mouse images with 5C1 imaging system also showed much better image resolution with great details of organs and anatomy compared to those obtained with a conventional mammography system. A simple and inexpensive ultra-high resolution imaging system on 5C1 beamline was successfully implemented. The authors were able to acquire ...
2001-01-01
Sorbent materials for fusion reactor tritium processing
Energy Technology Data Exchange (ETDEWEB)
A fusion reactor (such as NET/ITER) which breeds its own tritium fuel requires tritium recovery, purification and separation from the other isotopes. Cyclic adsorption processes are strong candidates for several of the processes involved: amongst other advantages, they promise a low tritium inventory. A good adsorbent for such processes must have high adsorption capacity, high selectivity and very low tritium retention after each cycle. Pure zeolite powder is shown to have an excellent combination of these three properties. However, in practice problems can arise from tritium which is not removed by reactivation. In this paper we show that tritium retention in zeolites can be caused either by water retained in the zeolite structure, which can be removed by ore rigorous activation, or by water tapped on binders in commercial pellets. (orig.).
1995-03-01
British Library Electronic Table of Contents (United Kingdom)
Tailor die quenching in the hot stamping of quenchable steel sheets was developed to produce ultra-high strength steel formed parts having strength distribution. Local portions of the heated sheet were quenched by holding grooved tools at the bottom dead centre during the stamping. Non-contact portions were generated in the sheet by grooving the tools, and thus the strength in the contact portions is high owing to the quenching and that in the non-contact portions is low owing to the lack of the quenching. Hat-shaped products having a tensile strength of approximately 1.5GPa only at four corners were formed.
2010-01-01
Mechanical properties and structure of low-alloy ultra-high strength steels
Energy Technology Data Exchange (ETDEWEB)
Mechanical properties of P-LDHA and V-ROL N steels of the Czech production are compared with other ultra-high strength steels produced in the world. The most important results can be summarized into following points: 1. Optimally heat treated P-LDHA steel exhibits substantially better strength characteristics then the V-ROL N steel. 2. Optimal tempering temperature of the P-LDHA steel is 300 C. 3. Basic mechanical properties of P-LDHA steel belong to the top of the UHS steels ranking and are well comparable with those of American 300 M steel. 4. In the low-cycle fatigue region, the P-LDHA steel exhibits slightly better fatigue resistance then the 300 M steel. On the other hand, the high-cycle fatigue resistance of 300 M steel is slightly better then that of the P-LDHA steel. (orig.)
2000-07-01
Hydrogen transport and embrittlement in 300 M and AerMet100 ultra high strength steels
Energy Technology Data Exchange (ETDEWEB)
This paper describes how hydrogen transport affects the severity of hydrogen embrittlement in 300 M and AerMet100 ultra high strength steels. Slow strain rate tests were carried out on specimens coated with electrodeposited cadmium and aluminium-based SermeTel 1140/962. Hydrogen diffusivities were measured using two-cell permeation and galvanostatic charging methods and values of 8.0 x 10{sup -8} and 1.0 x 10{sup -9} cm{sup 2} s{sup -1} were obtained for 300 M and AerMet100, respectively. A two-dimensional diffusion model was used to predict the hydrogen distributions in the SSR specimens at the time of failure. The superior embrittlement resistance of AerMet100 was attributed to reverted austenite forming around martensite laths during tempering.
2010-05-15
Energy Technology Data Exchange (ETDEWEB)
An experimental verification for long-term performance of a Pd-Ag permeation in ITER tritium fusion cleanup units (FCU) is needed. In addition, information is required on the influence of tritium and {sup 3}He decay on the physical and chemical properties of Pd-Ag alloys (V-1). The results of the investigations of alloys (V-1) (mechanical properties and microstructure) after long-term usage exposition in tritium are given in this report. The experimental conditions (temperature, pressure, clearance, {sup 3}He concentrations) and the previous conclusions on the V-1 alloy performance are presented. (orig.).
1996-10-01
Assessment of tritium in the Savannah River Site environment
Energy Technology Data Exchange (ETDEWEB)
This report is the first revision to a series of reports on radionuclides inn the SRS environment. Tritium was chosen as the first radionuclide in the series because the calculations used to assess the dose to the offsite population from SRS releases indicate that the dose due to tritium, through of small consequence, is one of the most important the radionuclides. This was recognized early in the site operation, and extensive measurements of tritium in the atmosphere, surface water, and ground water exist due to the effort of the Environmental Monitoring Section. In addition, research into the transport and fate of tritium in the environment has been supported at the SRS by both the local Department of Energy (DOE) Office and DOE`s Office of Health and Environmental Research.
1993-10-01
British Library Electronic Table of Contents (United Kingdom)
Dimethyl methylphosphonate (DMMP), a chemical simulant of the nerve gas GB, was decontaminated with a nonthermal atmospheric pressure plasma. The decontamination efficiency was measured qualitatively by means of Fourier transform spectroscopy and quantitatively by means of gas chromatography. With helium gas only, 10g/m2 of DMMP on an aluminum surface was 99.9% decontaminated in 2min, furthermore, with the addition of 5% of oxygen gas, it was 99.99% decontaminated in 10min. Given the low input power (<100W) and temperature (<75degreeC), this plasma is eligible for nondestructive decontamination of almost all material surfaces.
2009-01-01
Decontamination of spent fuel dissolution tank
International Nuclear Information System (INIS)
The decontamination of the dissolution tank from spent fuel reprocessing out-ling device is studied, by using FL-AP decontamination agent. The decontamination factor per step is 2.2, 2.4, respectively for #alpha#, #beta# activities. After dissecting the tank, residual contamination in inner surface of the tank was found to be non-uniform. The exact original contamination value of the tank surface could be approximated by calculating the total amounts of radionuclide distributed on the hanging specimens, the dissecting specimen, and radioactive level in waste decontamination agent. Therefore, it can be concluded that the hanging specimens method is feasible for measuring the decontamination factor of spent fuel dissolution tank. (authors)
2006-01-01
Chemical decontamination methods for coatings
Energy Technology Data Exchange (ETDEWEB)
A review of chemical decontamination methods for coatings indicates the following: the ease of both contamination and decontamination is a function of the radionuclide and the pH of the environment; the coating type is important in determining whether the contamination is loosely adsorbed, complexed, or contained in porous filler material; the condition of the coating is important to the decontamination factor obtained. Thus coatings can be decontaminated provided the solvent is sufficiently acid to solubilize the radionuclide and the complexant strength of the solvent is greater than that of the coating. Difficulties arise if the contamination is associated with fillers. Furthermore, though nothing has been said about temperature, decontamination of metal goes faster and, usually, with better efficiency at high temperatures. 11 references, 3 figures.
1984-05-01
Energy Technology Data Exchange (ETDEWEB)
Promoting the exchange of information related to implementation of the As Low as Reasonably Achievable (ALARA) philosophy is a continuing objective for the Department of Energy (DOE). This report was prepared by the Brookhaven National Laboratory (BNL) ALARA Center for the DOE Office of Health. It contains the fifth in a series of bibliographies on dose reduction at DOE facilities. The BNL ALARA Center was originally established in 1983 under the sponsorship of the Nuclear Regulatory Commission to monitor dose-reduction research and ALARA activities at nuclear power plants. This effort was expanded in 1988 by the DOE`s Office of Environment, Safety and Health, to include DOE nuclear facilities. This bibliography contains abstracts relating to various aspects of ALARA program implementation and dose-reduction activities, with a specific focus on DOE facilities. Abstracts included in this bibliography were selected from proceedings of technical meetings, journals, research reports, ...
1994-01-01
Energy Technology Data Exchange (ETDEWEB)
This bibliography contains abstracts relating to various aspects of ALARA program implementation and dose reduction activities, with a focus on DOE facilities. Abstracts included in this bibliography were selected from proceedings of technical meetings, journals, research reports, searches of the DOE Energy, Science and Technology Database (in general, the citation and abstract information is presented as obtained from this database), and reprints of published articles provided by the authors. Facility types and activities covered in the scope of this report include: radioactive waste, uranium enrichment, fuel fabrication, spent fuel storage and reprocessing, facility decommissioning, hot laboratories, tritium production, research, test and production reactors, weapons fabrication and testing, fusion, uranium and plutonium processing, radiography, and aocelerators. Information on improved shielding design, decontamination, containments, ...
1993-12-01
International Nuclear Information System (INIS)
Various kinds of decontaminations are carried out in atomic power plant. Here current decontamination technologies such as chemical decontamination with chemical solution or blast decontamination have a problem of reduction of secondary radioactive waste generated in the decontamination process. On the other hand, a low pressure arc plasma can remove metal oxide film on the metal substrate without heavy damage on the metal substrate when the object to be treated was set as a cathode. Dry surface decontamination technology with using low-pressure arc plasma can decrease secondary radioactive waste because low-pressure arc plasma does not need any chemical solution. In addition, the time required for treatment can be shorter, so it is possible for the low-pressure arc plasma decontamination technology to interpolate the current ...
2008-12-01
Energy Technology Data Exchange (ETDEWEB)
High and ultra-high strength steels for pipelines are produced by properly handling the steel microstructure. The metallurgical principles involved in the microstructure control are presented, with emphasis on TMCP processing, that comprises conventional controlled rolling followed by accelerated cooling. (author)
2008-05-15
PV Conversion Technologies, Session: OPV, Sensitized, Seed (Presentation)
Energy Technology Data Exchange (ETDEWEB)
The NREL Sensitized Solar Cell (SSC) Core Program supports the Solar America Initiative by: (1) targeting new devices and processes for commercialization by 2015 that are less expensive, more efficient, highly reliable, and environmentally benign; (2) collaborating with DOE OS/BES to conduct basic research targeting breakthroughs in key areas, such as ultra-high efficiency and/or ultra-low cost materials and devices.
2008-04-01
New designs for Ultra High High-Power Single Transverse Mode Cw fibre lasers
International Nuclear Information System (INIS)
Overcoming the limiting constraints of stimulated Raman scattering (SRS) and stimulated Brilluoin scattering (SBS) poses serious fibre design challenges for increasing the output power of optical amplifiers and lasers. New fibre amplifier designs are proposed to break out of these limitations to reach several kWs CW powers. (Author)
2009-04-01
Evaluation of tritium diffusion through the Neutral Beam Injector calorimeter panel
Energy Technology Data Exchange (ETDEWEB)
The Neutral Beam Test Facility (NBTF) to be realized in Padoa will test the Neutral Beam Injection (NBI), one of the Heating and Current Drive Systems foreseen for ITER. The NBI is based on the acceleration of hydrogen or deuterium negative ions up to 1 MeV. This work has been aimed at assessing the tritium release from the NBTF in order to provide data for the safety analysis. In particular, the diffusion of the tritium through the neutral beam target material (the CuCrZr alloy calorimeter panels) has been assessed by using literature data of the diffusion coefficient. The tritium generated inside the calorimeter panels moves into both the vacuum and water side: the tritium diffusion flux has been evaluated during the beam-on (200 deg. C) and the beam-off (20 deg. C) phases of the NBTF experiments consisting of an interim campaign and a final test. The penetration depth of the ...
2009-06-15
Evaluation of tritium diffusion through the Neutral Beam Injector calorimeter panel
International Nuclear Information System (INIS)
The Neutral Beam Test Facility (NBTF) to be realized in Padoa will test the Neutral Beam Injection (NBI), one of the Heating and Current Drive Systems foreseen for ITER. The NBI is based on the acceleration of hydrogen or deuterium negative ions up to 1 MeV. This work has been aimed at assessing the tritium release from the NBTF in order to provide data for the safety analysis. In particular, the diffusion of the tritium through the neutral beam target material (the CuCrZr alloy calorimeter panels) has been assessed by using literature data of the diffusion coefficient. The tritium generated inside the calorimeter panels moves into both the vacuum and water side: the tritium diffusion flux has been evaluated during the beam-on (200 deg. C) and the beam-off (20 deg. C) phases of the NBTF experiments consisting of an interim campaign and a final test. The penetration depth of the ...
2009-06-01
Use of the fast flux test facility for tritium production
Energy Technology Data Exchange (ETDEWEB)
This report provides the results of a JASON review of the technical feasibility of using the Department of Energy`s (DOE`s) Fast Flux Test Facility (FFTF) to generate tritium needed for the enduring United States nuclear weapons stockpile.
1996-10-25
Tritium in surface waters, tap water and in precipitation in Poland during the 1994-1999 period
International Nuclear Information System (INIS)
Concentrations of tritium in environmental waters (precipitation, rivers, lakes, tap water) have been determined using electrolytic enrichment and liquid scintillation counting. In waters of big rivers (the Vistula and the Odra rivers), lakes and tap water the annual average concentrations were similar to each other being from 1.4 to 1.9 Bq x dm"-"3. These concentrations were similar to those in the precipitation in which they ranged from 1.7 to 2.2 Bq x dm"-"3. The lowest tritium concentrations were found in waters of the Seashore Region rivers (average for 1994-1999 was 1.1 Bq x dm"-"3). The tritium concentrations in surface waters and in precipitation are still higher than that of natural level. The data obtained show that tritium concentration in the water of rivers might depend on the size of drainage area. The observed seasonal variations of tritium concentration in the ...
2001-01-01
Environmental levels of tritium, 2
International Nuclear Information System (INIS)
In an attempt to obtain basic data for evaluation of exposure doses in Niigata Prefecture, the concentrations of tritium in atmospheric water, precipitation, river water, and tap water were measured. Samples of atmospheric water, river water, and tap water were collected once for 2 weeks; and precipitation collected for one week was used as sample. The concentration of atmospheric tritium depended on the concentration of tritium in moisture and the content of water in atmosphere. Tritium levels were high in May, November and March, and low in September. Regarding tritium concentrations, there was a good correlation between atmospheric water and precipitation. Tritium concentrations in both of them varied from sample to sample. The concentrations of tritium in river and tap water tended to be high during spring and low during summer and ...
Development of Tritium Removal Technology.
Liquid Phase Catalytic Exchange (LPCE)- Cryogenic Distillation(CD) process was studied which could be available for an optimal tritium removal process of pressurized heavy water reactor system at Wolsung nuclear power plant in the near future. Based upon ...
1986-01-01
Use of evaporation for the treatment of liquids in the nuclear industry
International Nuclear Information System (INIS)
... The results show that a system decontamination factor of 10^ to 10* can be
1994-07-25
Liquid Radioactive Wastes Processing
International Science & Technology Center (ISTC)
Methods of Decontamination, Utilization, and Deactivation of Liquid Radioactive Wastes
Optimum design of the Wolsung tritium removal facility
Energy Technology Data Exchange (ETDEWEB)
Tritium removal from tritiated heavy water in a PHWR is the most effective way in reducing workers` internal dose and radioactivity emissions from Wolsong NPP. The optimum design of the Wolsung TRF(Tritium Removal Facility) was carried out using an approximate short-cut method with an assumption that the TRF, designed to extract 8 MCi per year of elemental tritium from a heavy water feedstream, uses Liquid Phase Catalytic Exchange (LPCE) front-end process and Cryogenic Distillation (CD) process. 19 refs., 6 figs., 2 tabs. (author).
1996-08-01
Optimum design of the Wolsung tritium removal facility
International Nuclear Information System (INIS)
Tritium removal from tritiated heavy water in a PHWR is the most effective way in reducing workers' internal dose and radioactivity emissions from Wolsong NPP. The optimum design of the Wolsung TRF(Tritium Removal Facility) was carried out using an approximate short-cut method with an assumption that the TRF, designed to extract 8 MCi per year of elemental tritium from a heavy water feedstream, uses Liquid Phase Catalytic Exchange (LPCE) front-end process and Cryogenic Distillation (CD) process. 19 refs., 6 figs., 2 tabs. (author).
1996-01-01
Gross decontamination experiment report
International Nuclear Information System (INIS)
A Gross Decontamination Experiment was conducted on various levels and surfaces of the TMI - Unit 2 reactor building in March 1982. The polar crane, D-rings, missile shields, refueling canals, refueling bridges, equipment, and elevations 305' and 347'-6'' were flushed with low pressure water. Additionally, floor surfaces on elevation 305' and floor surfaces and major pieces of equipment on elevation 347'-6'' were sprayed with high pressure water. Selective surfaces were decontaminated with a mechanical scrubber and chemicals. Strippable coating was tested and evaluated on equipment and floor surfaces. The effectiveness, efficiency, and safety of several decontamination techniques were established for the large, complex decontamination effort. Various decontamination equipment was evaluated and its effectiveness was documented. Decontamination training and ...
Energy Technology Data Exchange (ETDEWEB)
It has been reported by the present authors that behavior of tritium release from solid breeder grain is consisted of diffusion in grain, tritium transfer at surface layer and surface reactions on grain surface such as adsorption or isotope exchange reactions. Tritium release curves estimated using the tritium release model gave good agreement with observed tritium release curves from Li{sub 4}SiO{sub 4}, Li{sub 2}ZrO{sub 3} or LiAlO{sub 2}. Tritium release behavior from Li{sub 2}TiO{sub 3} under humid purge gas, dry purge gas and dry purge gas with hydrogen conditions is discussed in this study, tritium release curves using the release model that we proposed previously give a good agreements with experimental tritium release curves. Tritium effective diffusivity in the crystal grain of Li{sub ...
2008-05-15
International Nuclear Information System (INIS)
It has been reported by the present authors that behavior of tritium release from solid breeder grain is consisted of diffusion in grain, tritium transfer at surface layer and surface reactions on grain surface such as adsorption or isotope exchange reactions. Tritium release curves estimated using the tritium release model gave good agreement with observed tritium release curves from Li_4SiO_4, Li_2ZrO_3 or LiAlO_2. Tritium release behavior from Li_2TiO_3 under humid purge gas, dry purge gas and dry purge gas with hydrogen conditions is discussed in this study, tritium release curves using the release model that we proposed previously give a good agreements with experimental tritium release curves. Tritium effective diffusivity in the crystal grain of Li_2TiO_3 is also estimated in this study using ...
2008-05-01
Energy Technology Data Exchange (ETDEWEB)
The present report concerns a research for the tritium and for the carbon 14 in lichens in a spirit of bio-indication: the first results appear in Daillant and al (2004 ) and additional results were presented to the congress B.I.O.M.A.P. in Slovenia, organized collectively by the institute Josef Stefan from Ljubljana and the international atomic energy agency from Vienna (Daillant and al 2003). (N.C.)
2007-07-01
Internal dose from tritium at Wolsung nuclear power plant
International Nuclear Information System (INIS)
Tritium is produced in large quantities at heavy water nuclear power reactors via the neutron activation reaction "2H(n,#gamma#)"3H. At Wolsung nuclear power plant which has a CANDU reactor, the tritium concentrations in coolant and in moderator systems are 1.5 Ci/Kg-D_2O and 35 Ci/kg-D_2O, respectively, after 12 years of operation. The airborne tritium concentration in main access area is normally less than 5 MPCa except short-term peaks. The average tritium concentrations in main access controlled areas are normally less than 100 MPCa. Tritium is mainly present in the air of workplace of CANDU reactors as a tritiated water vapour. Airborne tritiated water vapour enters the workers body via inhalation and absorption through skin and can result in a significant dose. The occupational doses from tritium at Wolsung NPP have been maintained below 1 man-Sv per year ...
1995-02-01
International Nuclear Information System (INIS)
Tritium occurs in nature in trace amounts, but its concentration is changing due to natural and artificial sources. Studies focusing on natural tritium have to take into account the effect of artificial sources. Also, the impact of tritium is an important issue in environmental protection, e.g. in connection with the emissions from nuclear power plants. The present work focuses on the rain washout of tritium emitted from the Paks nuclear power plant in Hungary. Rainwater collectors were placed around the plant and after a period of precipitation, rainwater was collected and analysed for tritium content. Samples were analysed using low-level liquid scintillation counting, with some also subject to the more accurate "3He ingrowth method. The results clearly show the trace of the tritium plume emitted from the plant; however, values are only about one order of ...
2011-01-01
Los Alamos DP West Plutonium Facility decontamination project
Energy Technology Data Exchange (ETDEWEB)
The DP West Plutonium Facility operated by the Los Alamos National Laboratory, Los Alamos, New Mexico, was decontaminated between April 1978 and April 1981. The facility was constructed in 1944 to 1945 to produce plutonium metal and fabricate parts for nuclear weapons. It was continually used as a plutonium processing and research facility until mid-1978. Decontamination operations included dismantling and removing gloveboxes and conveyor tunnels; removing process systems, utilities, and exhaust ducts; and decontaminating all remaining surfaces. This report describes glovebox and conveyor tunnel separations, decontamination techniques, health and safety considerations, waste management procedures, and costs of the operation.
1982-01-01
Decontamination factors and release rates of UO/sub 2/ particles from boiling pools of sodium
Energy Technology Data Exchange (ETDEWEB)
A semi-mechanistic model for calculating solid radionuclide release rates from bubbling pools of sodium was developed. The influence of particle spacial and size distributions on the decontamination of the releases was analysed and found significant. Decontamination factors are shown as a function of pool depth, bubbling characteristics and particle size distribution. The calculation of a decontamination factor for estimating the source term of large scale hypothetical core disruptive accidents is presented. The decontamination factor for a large scale accident was found to be two orders of magnitude greater than results obtained from small scale experiments conducted with uniform particle distributions.
1983-01-01
Decontamination factors and release rates of UO"2 particles from boiling pools of sodium
International Nuclear Information System (INIS)
A semi-mechanistic model for calculating solid radionuclide release rates from bubbling pools of sodium was developed. The influence of particle spacial and size distributions on the decontamination of the releases was analysed and found significant. Decontamination factors are shown as a function of pool depth, bubbling characteristics and particle size distribution. The calculation of a decontamination factor for estimating the source term of large scale hypothetical core disruptive accidents is presented. The decontamination factor for a large scale accident was found to be two orders of magnitude greater than results obtained from small scale experiments conducted with uniform particle distributions. (orig.).
Energy Technology Data Exchange (ETDEWEB)
An estimate of the tritium dose to the public in the vicinity of the heavy water research reactor facility at AECL-Chalk River Laboratories, Ontario, Canada, has largely been accomplished from analyses on regularly-collected samples of air, precipitation, drinking water and foodstuffs (pasture, fruit, vegetables and milk) and environmental dose models. To increase the confidence with which public doses are calculated, tritium doses were estimated directly from the ratio of tritiated species in urine samples from members of the general public. Single cumulative 24 h urine samples from a few adults living in the vicinity of the heavy-water research reactor facility at Chalk River Laboratories, Canada were collected and analysed for tritiated water and organically bound tritium. The participants were from Ottawa (200 km east), Deep River (10 km west) and Chalk River Laboratories. Tritiated water concentrations in urine ranged ...
2001-07-01
Energy Technology Data Exchange (ETDEWEB)
A meeting was held on October 15, 16, 17, 1990 to discuss the state of tritium safety and environmental effects. The meeting was organized with the help of the International Energy Agency planning committee consisting of K. Steinmetz, Y. Seki, G. Nardella, and G. Vivian. Representative of tritium production facilities and heavy water reactor power production were also involved. The meeting was organized to address seven topics in tritium safety that were thought to require further work. The topics were: (1) materials science, (2) environmental models, (3) environmental model validation, (4) tritiated organic compounds, (5) human dosimetry, (6) tritium sampling and measurement, and (7) long-term environmental databases.
1991-04-18
International Nuclear Information System (INIS)
Tarapur Atomic Power Station unit-4 is first 540 MWe pressurized heavy water reactor. Heavy water is used as the coolant and moderator. With reactor operation tritium is formed by absorption of neutron by Deuterium atoms. Experience in the 220 MWe indicates that tritium is main contributor to the internal dose of radiation workers. Study on Tritium build up in Primary Heat Transport (PHT) and Moderator (MOD) system was carried out at the initial stage of the operation of the unit-3 and 4. This paper brings out tritium activity buildup in the PHT and MOD systems and its comparison with 220 MWe reactors. This paper helps in estimation of the internal dose contribution to the radiation workers at TAPS 3 and 4. (author)
2006-11-13
International Nuclear Information System (INIS)
Tarapur Atomic Power Station unit-4 is first 540 MWe pressurized heavy water reactor. Heavy water is used as the coolant and moderator. With reactor operation tritium is formed by absorption of neutron by deuterium atoms. Experience in the 220 MWe indicates that tritium is main contributor to the internal dose of radiation workers. Study on tritium build up in Primary Heat Transport (PHT) and Moderator (MOD) system was carried out at the initial stage of the operation of the unit-4. This paper brings out tritium activity buildup in the PHT and MOD systems and its comparison with 220 MWe reactors. This paper helps in estimation of the internal dose contribution to the radiation workers at TAPS 3 and 4. (author)
2005-11-23
An overview of AECL's participation in the Korean Wolsung Tritium Removal Facility Project (WTRF)
International Nuclear Information System (INIS)
Full text: In heavy-water-moderated power reactors, tritium is primarily produced by neutron capture in deuterium nuclei in the moderator and coolant. For CANDU 6 reactors, the estimated steady-state values are #approx# 3 TBq#centre dot#kg"-"1 D_2O in the moderator and #approx# 74 GBq#centre dot#kg"-"1 D_2O in the coolant. Tritium removal is one option available to reactor operators for use in their heavy water and tritium management strategies. The WTRF is designed to remove tritium from tritiated heavy water in each of the four CANDU units at the Wolsung Site, to immobilize the tritium and to store it on site. The detritiation process is based on three steps: the first one (front-end) involves the transfer of tritium from heavy water to deuterium gas; the second one (enrichment) concentrates the tritium in a cryogenic distillation system ...
2007-11-07
Tritium Release Behavior from Li_4SiO_4
International Nuclear Information System (INIS)
This paper proposes a model to explain tritium release behavior of an irradiated Li_4SiO_4 sample made by Forschungszentrum Karlsruhe. The release curves were obtained in a series of experiments carried out using out-pile temperature programmed desorption techniques in the Kyoto University Reactor (KUR). Tritium release curves obtained for different purge gas compositions (N_2, N_2 + H_2, N_2 + H_2O) were compared for selection of suitable conditions to determine the apparent diffusivity of tritium in a crystal grain of Li_4SiO_4.In the model formation, some mass transfer steps in the bulk of the crystal grain and those on the surface of the grain were taken into account, which were diffusion of tritium in the grain, adsorption and desorption of water on the surface of the grain, two types of isotope exchange reactions, and water formation reaction by the addition of hydrogen to the purge ...
2004-12-01
Energy Technology Data Exchange (ETDEWEB)
For the inventory of water tritium concentration in the Manche department, it is the complementarity that animated the work opened during year 2001. To answer to a commune sensitivity such water quality, particularly drinking water at tap, the A.C.R.O. laboratory brought its know how to make and its technical means in the area of tritium analysis and the general council brought its know how to make and its logistics means in matter of sanitary control. This collaboration has allowed to supply an indication on the tritium content of the distribution waters of thirty of the most important cities of the department. Then, it allowed to inform on the radiological situation (in relation with the tritium presence) of coast waters and principal rivers waters. More than 160 controls have been realised between the months of march 2001 and february 2002. Only the tritium under the shape of ...
2007-07-01
Environmental tritium in the areas adjacent to Wolsong nuclear power plant
International Nuclear Information System (INIS)
The distribution of environmental tritium and the correlation coefficients between tritium concentrations in several environmental samples and the emissions of tritiated water vapor from Wolsong NPP 1 were studied. The annual mean concentrations of atmospheric HTO were in the range 1#centre dot#31-29#centre dot#2 Bq m"-"3 and the long-term atmospheric dilution factors were in the range 10"-"7-10"-"6 s m"-"3. Annual mean concentrations of tritium in ground water were in the range 19#centre dot#2-27#centre dot#9 Bq l"-"1 at N-1 and 64#centre dot#1-189 Bq l"-"1 at S-2, and were generally less than 0#centre dot#2% of MPC_w (222 kBq l"-"1). The concentrations of tritium in precipitation decreased exponentially with distance from Wolsong NPP 1, falling to current global levels at about 25 km off-site. The highest concentration of tritium in soil moisture was observed in May and June, when ...
1998-11-01
Energy Technology Data Exchange (ETDEWEB)
In order to evaluate the effectiveness of some decontamination agents against skin contamination of {sup 60}Co and {sup 137}Cs, the experiments were carried out in this study. In the experiments, pig skin was used instead of human skin, {sup 60}CoCl{sub 2} and {sup 137}CsCl were used the liquid sources of skin contamination. To examine the effectiveness of decontamination agents, skin decontamination was tried using soup, EDTA, DAERICON which was developed for decontamination of radionuclides on the surface of building structure, and new decontamination agents such as IOCON, TRICON, and CHARCON, which were developed in this study. The absorption of radionuclides through the skin was evaluated by the gamma-ray detection on the surface of sample skin after radionuclides were penetrated into the skin during 16 hour soiling time. The results of this absorption experiment indicated that ...
1998-03-01
International Nuclear Information System (INIS)
In order to evaluate the effectiveness of some decontamination agents against skin contamination of "6"0Co and "1"3"7Cs, the experiments were carried out in this study. In the experiments, pig skin was used instead of human skin, "6"0CoCl_2 and "1"3"7CsCl were used the liquid sources of skin contamination. To examine the effectiveness of decontamination agents, skin decontamination was tried using soup, EDTA, DAERICON which was developed for decontamination of radionuclides on the surface of building structure, and new decontamination agents such as IOCON, TRICON, and CHARCON, which were developed in this study. The absorption of radionuclides through the skin was evaluated by the gamma-ray detection on the surface of sample skin after radionuclides were penetrated into the skin during 16 hour soiling time. The results of this absorption experiment indicated that 11.5% and 3.2% of ...
1998-03-01
Oxygen stabilization induced enhancement in superconducting characteristics of high-Tc oxides
International Nuclear Information System (INIS)
In an attempt to enhance the electrical and mechanical properties of the high temperature superconducting oxides, high T(sub c) composites were prepared composed of the 123 compounds and AgO. The presence of extra oxygen due to the decomposition of AgO at high temperature is found to stabilize the superconducting 123 phase. Ag is found to serve as clean flux for grain growth and precipitates as pinning center. Consequently, almost two orders of magnitude enhancement in critical current densities were also observed in these composites. In addition, these composites also show much improvement in workability and shape formation. On the other hand, proper oxygen treatment of Y5Ba6Cu11Oy was found to possibly stabilize superconducting phase with T(sub c) near 250 K. I-V, ac susceptibility, and electrical resistivity measurements indicate the existence of this ultra high T(sub c) phase in this compound. Detailed structure, microstructure, electrical, ...
1991-01-01
Gamma-ray burst (GRB) is one of the candidates of high-energy cosmic-ray acceleration sites. They may be also ultra-high-energy (above 3 EeV) cosmic-ray (UHECR) sources. In this paper, we discuss possibilities and implications of high-energy cosmic-ray acceleration in GRBs. (1) First, we show that not only protons but also heavier nuclei can be accelerated up to ultra-high energies in both usual high-luminosity (HL) and low-luminosity (LL) GRBs by using the Geant4. LL GRBs may also make a significant contribution to the observed UHECR flux if they form a distinct population, and we investigate cosmic-ray acceleration in LL GRBs in detail. (2) Second, we discuss implications of the GRB-UHECR hypothesis (and Hypernova-UHECR hypothesis) to cosmic-ray astronomy. HL GRBs and LL GRBs will lead to different source number densities as UHECR sources, so that the determination of the number density of UHECR sources and strength of the mean extragalactic ...
2008-01-01
Energy Technology Data Exchange (ETDEWEB)
The object of this research is the evaluation of the performance of ultra high speed relays (UHSR's) used for protection of a-c transmission lines. For purposes of this report, these are relays whose response time is less than a quarter of a cycle of the 60 Hz wave (i.e. 4.167 ms.). To identify relaying schemes that may comply with this definition, a literature survey was undertaken. The selected relays were studied in detail and modeled on a digital computer. A theoretical description of these relays is presented. Records of real transient data as well as of simulated data were used as input to the digital models of relays. The real data were recorded by means of monitoring stations connected to the Florida Power and Light Company transmission lines. The simulated data were obtained by modeling the relevant parts of the utility's transmission system using a University of British Columbia simplified version of the well known ...
1984-01-01
Multilayer ultra high gradient insulator technology
Energy Technology Data Exchange (ETDEWEB)
We are investigating a novel insulator concept which involves the use of alternating layers of conductors and insulators with periods less than 1 mm. These structures perform many times better (about 1.5 to 4 times higher breakdown electric field) than conventional insulators in long pulse, short pulse, and alternating polarity applications. We present our ongoing studies investigating the degradation of the breakdown electric field resulting from surface roughness, the effect of gas pressure, and the performance of the insulator structure under bi-polar stress. Further, we present our initial modeling studies.
1998-03-27
Improved formability of ultra high strength steels through local heat treatment
Energy Technology Data Exchange (ETDEWEB)
In this paper it is described how a martensitic steel sheet with tensile strength of 1400 MPa is heat treated locally. The sheet is then formed in the heat treated regions in a way that would be impossible with the untreated material. Mechanical properties and forming limit diagrams of the heat treated material are determined and the forming operations are simulated, which shows that the method can be used by designers. Although the method has been known for decades, it remains to be industrialised and the work presented here is to be seen as a contribution to this development. (orig.)
2005-07-01
Coverage and large scale anisotropies estimation methods for the Pierre Auger Observatory
Energy Technology Data Exchange (ETDEWEB)
When searching for anisotropies in the arrival directions of Ultra High Energy Cosmic Rays, one must estimate the number of events expected in each direction of the sky in the case of a perfect isotropy. We present in this article a new method, developed for the Auger Observatory, based on a smooth estimate of the zenith angle distribution obtained from the data itself (which is essentially unchanged in the case of the presence of a large scale anisotropy pattern). We also study the sensitivity of several methods to detect large-scale anisotropies in the cosmic ray arrival direction distribution : Rayleigh analysis, dipole fitting and angular power spectrum estimation.
2005-07-01
Decontamination for radioactive working dresses using liquid and supercritical carbon dioxide
Energy Technology Data Exchange (ETDEWEB)
A decontamination washer for working dresses using liquid and supercritical carbon dioxide were designed and manufactured. The size of reactor for decontamination and solidification is about 16 liter. The system is a closed one with recycling ability of carbon dioxide. The efficiency of recycling of carbon dioxide and that of separation of solutes in carbon dioxide were checked. They met all the design goals. A remote control system of the carbon dioxide flow was set in a control panel. The manufactured decontamination washer was brought to Wolsung nuclear power plants, and installed to check the efficiency of decontamination and the feasibility of usage in nuclear power plants. The elimination of radioactive oil from the contaminated dresses were very high. However, the decontamination factor was lower than the design goal value. It's due to the low removal rate of ...
2000-05-01
Ultra high vacuum test setup for electron gun
Energy Technology Data Exchange (ETDEWEB)
Ultra High Vacuum (UHV) test setup for electron gun testing has been developed. The development of next generation light sources and accelerators require development of klystron as a radio frequency power source, and in turn electron gun. This UHV electron gun test setup can be used to test the electron guns ranging from high average current, quasi-continuous wave to high peak current, single pulse etc. An electron gun has been designed, fabricated, assembled and tested for insulation up to 80 kV under the programme to develop high power klystron for future accelerators. Further testing includes the electron emission parameters characterization of the cathode, as it determines the development of a reliable and efficient electron gun with high electron emission current and high life time as well. This needs a clean ultra high vacuum to study these parameters particularly at high emission current. The ...
2008-05-01
On-line real-time measurements of decontamination factor for a low-level waste incinerator
Energy Technology Data Exchange (ETDEWEB)
The experiments at the incinerator for low-level wastes processing, (containing transuranium radionuclides) are described. Air decontamination factors and detector readings correction factors for efficiency and absorption are indicated.
1983-01-01
On-line real-time measurements of decontamination factor for a low-level waste incinerator
International Nuclear Information System (INIS)
The experiments at the incinerator for low-level wastes processing, (containing transuranium radionuclides) are described. Air decontamination factors and detector readings correction factors for efficiency and absorption are indicated.
Energy Technology Data Exchange (ETDEWEB)
As evidence of its effectiveness rapidly accumulates, the Lomi process has most recently been used to decontaminate the recirculation loops and the reactor water clean-up unit of a BWR at Monticello in the United States. An average decontamination factor of 23 was achieved in the recirculation loops.
1985-01-01
The pharmacological activity of medical herbs after microbiological decontamination by irradiation
Energy Technology Data Exchange (ETDEWEB)
In the Institute of Nuclear Chemistry and Technology research on microbiological decontamination of medicinal herbs by irradiation has been carried out since 1996. It was shown that using ionizing radiation (a dose of 10 kGy) can obtain satisfactory results of microbiological decontamination of these products. The content of essential biologically active substances such as essential oils, flavonoids, glycosides, anthocyans, antra-compounds, poliphenoloacids, triterpene saponins, oleanosides and plants mucus did not change significantly after irradiation. Pharmacological activity of medicinal herbs has been found satisfactory after microbiological decontamination by irradiation.
2000-03-01
The kinetics of the CAN-DECON process
International Nuclear Information System (INIS)
When decontaminated with continuously replenished CAN-DECON reagent in a once-through system, carbon steel contaminated with "6"0Co during exposure to reducing coolant in stainless steel loops loses up to 90 percent of its radioactivity in the first few minutes. Afterwards, the rate of removal falls to much lower values which persist for many hours to the end of the experiment. The effects of flow rate, temperature and reagent concentration on the initial rates of decontamination indicate that mass transfer in the liquid is an important factor in the decontamination. The decontamination factor is influenced by the initial rate.
1982-09-19
Iodine decontamination factor for liquid radioactive waste volume reduction system
International Nuclear Information System (INIS)
(Jun 1976). United States Tokerud, LD Garcia, R. Aerojet Energy Conversion
1976-06-13
Decontamination of Johnston Island Coral: a preliminary study
International Nuclear Information System (INIS)
A preliminary investigation was completed on the characterization and decontamination of coral samples from Johnston Island. These samples were found to contain individual particles (2 to 0.25 mm) of contaminated coral as well as a piece of contaminated magnetic metal. They ranged in activity from about 70 to 811 nCi Am-241. The decontamination methods investigated were froth flotation, ferrite treatment, attrition scrubbing, ultrasonic treatment and dry sieving. Dry sieving, the more effective technique, separated about 42 wt % of the coral into a decontaminated fraction. This fraction (>4 mm) contained about 0.5% of the total activity. 7 refs., 3 tabs.
Decontamination factor determination for adsorption filters in nuclear power plants
International Nuclear Information System (INIS)
Slovak 1985. p. 110-111. Czechoslovakia Moravek, J. Pietrik, I. Janecka,
1985-08-26
Energy Technology Data Exchange (ETDEWEB)
12 kind of environmental samples such as soil, underground water, seawater, etc. around the Nuclear Power Plants(NPP) and surface seawater around the Korea peninsula were sampled, For the samples of rain, pine-needle, air, seawater, underground water, chinese cabbage, grain of rice and milk sampled around NPP, and surface seawater and rain sampled all around country, tritium concentration was measured, The tritium concentration in the tap water and the gamma activity in the domestic and imported beef that were sampled at ward in the large city in Korea(Seoul, Pusan, Taegu, Taejun, Inchun, Kwangju) were analyzed for the meat and drinking waters. As the results of analyzing, tritium concentration in rain and tap water were very low all around country, but a little higher around the NPP than general surrounding. At the Wolsung NPP, tritium concentration was descend according to distance from the stack. ...
2001-12-15
Dose assessment and behavior of tritium in environmental samples around Wolsong nuclear power plant.
For the estimation of the dispersion trend of tritium discharged from the Wolsung nuclear power plant, the present level of tritium in environmental samples in the vicinity of the Wolsong site has been studied. On the basis of tritium concentrations in environmental samples, the effective dose due to tritium has been estimated for an individual and population within a 16 km radius from the Wolsong site. The annual effective dose of tritium to an inhabitant around the Wolsong site ranged from 0.15 microSv y-1 to 1.3 microSv y-1. The dose level was negligible and much lower than some applicable standards, i.e. the limit on exposure from nuclear fuel cycle to the general public as recommended by ICRP (1 mSv y-1) or US EPA's limit (0.25 mSv y-1). The collective dose to the total population within a 16 km radius from the site, 1.2 x 10(-2) man.Sv y-1 was much lower than 1 man.Sv y-1, an ...
1999-04-01
Tritium bioassay and dosimetry at a CANDU reactors
Energy Technology Data Exchange (ETDEWEB)
Tritium dose management is an important aspect of the radiation protection program at CANDU type reactor sites. This paper describes the bioassay and dosimetry of tritium at CANDU reactor sites, especially for Wolsung Nuclear Power Plant. It presents a compilation of information drawn from published papers, technical reports, international and national guidelines as well as practical experience both in Korean and Canadian CANDU Nuclear Power Plants. The implementation of this program would provide a technical basis for calculations and records should be of acceptable quality and should meet overall radiation protection program objectives.
1996-07-01
Synthesis of high specific activity tritium labelled [2-{sup 3}H]-adenosine-5`-triphosphate
Energy Technology Data Exchange (ETDEWEB)
A procedure for high level tritium labelling at the C2-H position of adenosine 5`-triphosphate ([2-{sup 3}H]-ATP, 1), based on the tritiodehalogenation reaction of 2-bromoadenosine 5`-triphosphate (2) has been elaborated. This precursor was prepared in a six-step synthesis from guanosine. The tritiodehalogenation of (2) for three hours over palladium oxide in phosphate buffer yielded tritium labelled ATP with high specific activity, in good chemical yield. (author).
1996-08-01
Savannah River Technology Center monthly report, January 1994
Energy Technology Data Exchange (ETDEWEB)
This is the monthly progress report for the Savannah River Technology Center, which covers the following areas of interest, Tritium, Separation processes, Environmental Issues, and Waste Management.
1994-01-01
Savannah River Laboratory monthly report, November 1991
Energy Technology Data Exchange (ETDEWEB)
This document details monthly activities at the Savannah River Laboratory. Topics addressed are reactor operation; tritium facilities and production; separation operations; environmental concerns; and waste management. (FI)
1991-01-01
Savannah River Laboratory monthly report, November 1991
Energy Technology Data Exchange (ETDEWEB)
This document details monthly activities at the Savannah River Laboratory. Topics addressed are reactor operation; tritium facilities and production; separation operations; environmental concerns; and waste management. (FI)
1991-12-31
Modelling of tritium behavior in solid breeder blankets of conceptual fusion reactors
International Nuclear Information System (INIS)
1982. p. 1, Paper 11. United States Kessel, CE Jr. Univ. of California,
1982-03-28
Decontamination agent for chemically dissolving radioactive crud and its method
International Nuclear Information System (INIS)
Purpose: To dissolve iron and nickel as well as chromium simultaneously at one step for cruds partially containing chromium, and obtain high decontaminating factor (decontamination factor). Method: Radioactive cruds formed as corrosion products in nuclear reactor primary coolant circuits are subjected to dissolving treatment by using a decontaminating agent composed of cerium sulfate type solution as the dissolving solution. When the treatment is substantially completed, a reducing agent is added to reduce the residual 4-valent cerium into 3-valent cerium. Those having potential lower than the redox potential of cerium are used as the reducing agent so that cerium is not deposited. This can provide high decontaminating factor while preventing the deposition of cerium. (Takahashi, M.).
1986-05-07
The feasibility study of hot cell decontamination by the PFC spray method
International Nuclear Information System (INIS)
The characteristics of per-fluorocarbon compounds (PFC) are colorless, non-toxic, easily vaporized and nonflammable. Also, some of them are liquids of a high density, low surface tension, low latent heat and low specific heat. These particular chemical and physical properties of fluoro-organic compounds permit their use in very different fields such as electronics, medicine, tribology, nuclear and material science. The Sonatol process was developed under a contract with the DOE. The Sonatol process uses an ultrasonic agitation in a PFC solution that contains a fluorinated surfactant to remove radioactive particles from surfaces. Filtering the suspended particles allows the solutions to be reused indefinitely. They applied the Sonatol process to the decontamination of a heterogeneous legacy Pu-238 waste that exhibited an excessive hydrogen gas generation, which prevents a transportation of such a waste to a Waste Isolation Pilot Plant. Korea Atomic Energy Research ...
2008-01-01
International Nuclear Information System (INIS)
The philosophy of containing tritium and activated products very close to the source and of operating by remote techniques is justified by a comparison with other concepts on protection and availability points of view. Several design options are studied according to the optimization protection methodology of ICRP. Provided that an important technological development is accomplished, the utilization of robotics and the limitation of containment volumes should be generalized.
1983-04-26
International Nuclear Information System (INIS)
The tritium in transpired water of plant leaves from four locations within site area (2=0.92) with that of measured values indicating that at Tarapur, the contribution to TFWT of plant is only from air activity and pick up through soil route is negligible during the period of study. (author)
2010-05-13
International Nuclear Information System (INIS)
A Lagrangian atmospheric dispersion model(K-LADM) combining a three dimensional sea-land breeze model has been developed and applied to the estimation of the quaterly and the annual averaged air tritium concentration around Wolsung NPP site. The estimated concentrations were compared with the observed concentration data. The results showed that the present Lagrangian Atmospheric dispersion model(K-LADM) provided very good agreement with the observations.
1998-10-01
International Nuclear Information System (INIS)
Design improvements are being incorporated into the heavy water management systems at Wolsong 2,3 and 4 to reduce the load on the vapour recovery driers and upgraders and the heavy water losses via the stack. There will also be improvements to monitor heavy water and tritium releases. This paper describes the improvements, gives background on heavy water balance mechanism, the historical trends for heavy water recovery/losses and estimated dose to the member of the public critical group resulting from the airborne and waterborne releases. The measured tritium activity levels in the heat transport system (HTS) and moderator system at Wolsong 1 are given. Using these activity levels and heavy water loss data, tritium losses from the dried and ventilated areas are estimated. A qualitative assessment of expected heavy water and tritium releases has been performed for Wolsong 2, 3 and 4. CANDU 6 plants ...
1994-03-01
Isotope exchange reaction between tritiated water and hydrogen on SiC
Energy Technology Data Exchange (ETDEWEB)
SiC has been considered as a primary candidate material for a first wall component in future fusion reactor because it has been claimed that SiC has excellent high-temperature properties, good chemical stability and low activation. However, the behavior of tritium on SiC has not been discussed yet. In this study, tritium trapping capacity on the surface of SiC was experimentally obtained at the temperature range of 25-800 deg. C in consideration of tritium trapping to the experimental system. The capacity, which was independent of the water vapor pressure in the gas phase and the temperature, was determined as about 10{sup 6} Bq/cm{sup 2}. The isotope exchange reaction rate between tritiated water in a gas phase and hydrogen on the surface was quantified at the temperature of 25, 500 and 700 deg. C in consideration of the behavior of tritium trapping at change of experimental condition by the numerical ...
2003-11-15
Isotope exchange reaction between tritiated water and hydrogen on SiC
International Nuclear Information System (INIS)
SiC has been considered as a primary candidate material for a first wall component in future fusion reactor because it has been claimed that SiC has excellent high-temperature properties, good chemical stability and low activation. However, the behavior of tritium on SiC has not been discussed yet. In this study, tritium trapping capacity on the surface of SiC was experimentally obtained at the temperature range of 25-800 deg. C in consideration of tritium trapping to the experimental system. The capacity, which was independent of the water vapor pressure in the gas phase and the temperature, was determined as about 10"6 Bq/cm"2. The isotope exchange reaction rate between tritiated water in a gas phase and hydrogen on the surface was quantified at the temperature of 25, 500 and 700 deg. C in consideration of the behavior of tritium trapping at change of experimental condition by the numerical curve ...
2003-11-15
Development and manufacture of tritium-in-air monitors for Indian PHWRs
International Nuclear Information System (INIS)
Tritium, a beta emitting gas at room temperature causes a biological hazard in the locations where it is present beyond acceptable limits. The hazard can be due to inhalation, and absorption by skin. Hence is the necessity of Tritium monitoring instruments/systems for ensuring safety in the PHWRs and the nuclear research plants and laboratories. It is desirable that the instruments address satisfactorily to certain factors like the following: (i) Wide range of Tritium concentrations - 1 to 104 DAC ( Derived Air Concentration) (ii) On-line monitoring features (iii) Small response time (On-spot instantaneous measurements) (iv) Portability (v) Mitigation of memory effects. This paper presents an overview of the Online Tritium in Air Monitoring Systems manufactured by ECIL for Pressurised Heavy Water Reactors at Tarapur, Kaiga, and Rawatbhata. Significant aspects of design, function, testing, limitations of ...
2009-10-01
Untersuchungen zur Anwendung von UHPFRC-Tubbingen bei der zweischaligen Tunnelbauweise
British Library Electronic Table of Contents (United Kingdom)
Faserbewehrter Beton wird heute zunehmend auch bei Tunnelbauwerken (Tunnelinnenschalen, Tubbinge) eingesetzt. Wesentliche Vorteile sind das hohe Tragvermogen, das daraus entstehende Einsparungspotential an herkommlicher stabformiger Bewehrung (Biegebewehrung, Bugelbewehrung in der Randzone), die Aufnahme von Spaltzugbeanspruchungen durch die Fasern, Rissbreitenbegrenzung, erhohte Dauerhaftigkeit, verbesserter Brandwiderstand (insbesondere bei Verwendung von Kunststofffasern), Optimierung der Arbeitsablaufe etc. Neue Entwicklungen in der Betontechnologie haben in den letzten Jahrzehnten den faserbewehrten ultrahochfesten Beton (engl. UHPFRC - Ultra High Performance Fibre Reinforced Concrete) hervorgebracht. Im Rahmen dieser Arbeit wird der Einsatz des ultrahochfesten, stahlfaserbewehrten Be...
2010-01-01
Ultra high strength beta titanium alloy for fasteners
International Nuclear Information System (INIS)
A new high strength titanium alloy has been developed primarily intended for fastener applications. While Ti-6Al-4V is used extensively as a fastener alloy in the aerospace industry, its shear strength allowable is limited to 655 MPa (95 ksi). For higher shear strength requirements, various steels or nickel-based alloys are used (up to 860 MPa (125 ksi)), but with the attendant density penalty. This new alloy is intended to provide the 860 MPa shear strength at roughly a 40% weight savings. After screening various alloy systems, the optimum chemistry has been selected as follows: Ti-6.0V-6.2Mo-5.7Fe-3Al. In light of its 125 ksi shear strength goal, the alloy has been designated TIMETAL reg-sign 125.
1993-02-21
Separation of rubidium from irradiated aluminum-encapsulated uranium
International Nuclear Information System (INIS)
A procedure was developed for separating rubidium from irradiated aluminum encapsulated uranium. The separations procedure produces a final ultra-high purity RbCl product for subsequent high performance mass spectrometric analysis. The procedure involves first removing most of the macro-components and fission products by strong base anion exchange using, first, concentrated HCl, then oxalic acid media and second, selectively separating rubidium from alkaline-earth ions and other alkali-metal ions, including cesium, using Bio-Rex-40 cation-exchange resin. The resultant RbCl is then put through a final vacuum sublimation step. Ultra-pure reagents and specially clean glassware are used throughout the procedure to minimize contamination by naturally-occurring rubidium.
1993-05-01
Separation of rubidium from irradiated aluminum-encapsulated uranium
Energy Technology Data Exchange (ETDEWEB)
A procedure was developed for separating rubidium from irradiated aluminum encapsulated uranium. The separations procedure produces a final ultra-high purity RbCl product for subsequent high performance mass spectrometric analysis. The procedure involves first removing most of the macro-components and fission products by strong base anion exchange using, first, concentrated HCl, then oxalic acid media and second, selectively separating rubidium from alkaline-earth ions and other alkali-metal ions, including cesium, using Bio-Rex-40 cation-exchange resin. The resultant RbCl is then put through a final vacuum sublimation step. Ultra-pure reagents and specially clean glassware are used throughout the procedure to minimize contamination by naturally-occurring rubidium.
1982-01-01
Pulsed laser deposition of titanium-carbonitride thin films
Energy Technology Data Exchange (ETDEWEB)
The goal of this research program is to determine whether pulsed laser deposition is an effective alternative method for growing TiCN thin films. Pulsed laser deposition (PLD) is chosen because of its well-documented capability for growing uniform, stoichiometric films in ultra-high vacuum or gaseous environments. Processing of thin films by PLD is also achieved at relatively low temperatures compared with CVD processing. Given these attributes, the primary objectives in this article are to determine whether nitrogen may be readily incorporated into films resulting from the laser-ablation of TiC in an N{sub 2} environment, determine what effect nitrogen has on mechanical properties, and determine whether nitrogen incorporation is strongly influenced by processes unrelated to laser deposition (e.g., thermally-activated surface reactions).
1997-05-15
British Library Electronic Table of Contents (United Kingdom)
After irradiation at 254nm of aqueous solutions of the antipsychotic drug flupentixol, the structures of the photodegradation products were determined by ultra high performance liquid-chromatography linked to mass spectrometry. Fragmentation patterns of the parent ions were established on a hybrid linear ion trap-orbitrap mass spectrometer allowing accurate mass measurements of both parent and daughter ions. This allowed to propose plausible structures for the main photolysis products of flupentixol. A total of nine photoproducts were detected after irradiation of the drug. The main photoproduct is generated following the addition of a hydroxyl group on the double bond adjacent to the thioxanthene ring. Secondary photoproducts were also observed.
2010-01-01
Mesodynamics in the SARS nucleocapsid measured by NMR field cycling
Energy Technology Data Exchange (ETDEWEB)
Protein motions on all timescales faster than molecular tumbling are encoded in the spectral density. The dissection of complex protein dynamics is typically performed using relaxation rates determined at high and ultra-high field. Here we expand this range of the spectral density to low fields through field cycling using the nucleocapsid protein of the SARS coronavirus as a model system. The field-cycling approach enables site-specific measurements of R{sub 1} at low fields with the sensitivity and resolution of a high-field magnet. These data, together with high-field relaxation and heteronuclear NOE, provide evidence for correlated rigid-body motions of the entire {beta}-hairpin, and corresponding motions of adjacent loops with a time constant of 0.8 ns (mesodynamics). MD simulations substantiate these findings and provide direct verification of the time scale and collective nature of these motions.
2009-09-15
Hot dip galvanised dual phase steels for automotive applications
Energy Technology Data Exchange (ETDEWEB)
The automotive industry desires to optimize safety and lightweight construction for the production of cars and trucks. The resulting task for steel suppliers is to make steel grades available that can fulfil these requirements. Different projects have shown optimistic outlooks for optimization of safety and reduction of the weight of automobile bodies by using different high strength and ultra high strength steels. In the last group the dual phase steels play the lead. In recent years different steel grades have been developed and optimized for these applications. On one hand developing the mechanical properties as well as joining and forming of dual phase steels is one of the first steps. On the other hand different coated surfaces for various applications of dual phase steels is another step. Starting with characteristic production conditions for cold rolled hot dip galvanised dual phase steels, the mechanical properties for joining and ...
2005-07-01
High-temperature property data: Ferrous alloys
Energy Technology Data Exchange (ETDEWEB)
In this book over 250 alloys are organized by AISI number into 10 major sections: Irons, Carbon Steels, Alloy Steels, Low Alloy Constructional Steels, Ultra High Strength Steels, Tool Steels, Maraging Steels, Wrought Stainless Steels, Heat Resistnat Casting Alloys, and Iron Based Rought Superalloys. Each alloy record lists the designation, specifications, UNS number, composition, product forms and a comment on the high-temperature properties and applications. Referenced data is then given for physical properties such as density, specific heat, thermal conductivity, thermal expansion, electrical conductivity, Poisson's ratio, moduli of elasticity and rigidity, etc. Mechanical properties follow, and include tensile properties, shearing and bearing properties, impact properties, creep, stress rupture and stress relaxation and fatigue properties. The last part of the alloy record gives other effects of temperature, such as hot hardness, ...
1987-01-01
British Library Electronic Table of Contents (United Kingdom)
A qualitative method, involving supported liquid?liquid extraction (SLE) and ultra high pressure liquid chromatography coupled to tandem mass spectrometry (UHPLC-MS?MS), was developed for the rapid tentative identification of various drugs of abuse in urine. In this study, 28 drugs and metabolites were covered by the screening procedure. Before analysis, urine samples were extracted by SLE and good extraction recoveries were obtained for most investigated compounds. The UHPLC strategy was then selected for the rapid separation of amphetamines, cocaine, opiates and related compounds in urine. Using columns packed with sub-2??m particles, analysis time was reduced down to 2?min, while maintaining acceptable performance. Finally, the detection was by tandem MS operating in the single reaction...
2009-01-01
Empirical regularities of order placement in the Chinese stock market
Using ultra-high-frequency data extracted from the order flows of 23 stocks traded on the Shenzhen Stock Exchange, we study the empirical regularities of order placement in the opening call auction, cool period and continuous auction. The distributions of relative logarithmic prices against reference prices in the three time periods are qualitatively the same with quantitative discrepancies. The order placement behavior is asymmetric between buyers and sellers and between the inside-the-book orders and outside-the-book orders. In addition, the conditional distributions of relative prices in the continuous auction are independent of the bid-ask spread and volatility. These findings are crucial to build an empirical behavioral microscopic model based on order flows for Chinese stocks.
2007-01-01
Embedded systems for vacuum control at PEFP
International Nuclear Information System (INIS)
Development of a front end system for a high energy proton accelerator is in progress at Korea Atomic Energy Research Institute (KAERI) for basic science and industrial applications. The proper vacuum components has been installed and operated successfully between ion source and RFQ. The reliable operation of the accelerator has been completed at vacuum system in the high and ultra high vacuum range under operating conditions. Proper control system for the vacuum instruments, based on PC operated by Windows, has been designed and constructed by control group at PAL. As PC operated by windows with inherent instability does not proper, embedded system can be replaced for reliable operation system, such as VME system operated by vxWorks.
2005-05-26
Energy Technology Data Exchange (ETDEWEB)
A thermal-resistant radiation sensing system using optical fiber has been developed. The system is for monitoring progress of chemical decontamination and able to measure the gamma-ray level in a hot solution of decontamination chemicals in situ. Our sensor head makes use of thermal-resistant NaI (T1) and it is connected to an optical fiber bundle. Scintillation photons pass from the NaI (T1) into the end of the bundle. This part of the system can withstand temperatures of over 100degC. At the far end of the optical fiber bundle, the scintillation photons are converted into fluorescent photons using a wavelength-shifting fiber. These photons are transferred to a distant photomultiplier tube through two thin transparent optical fibers. Furthermore, we propose a self-compensation technique for the dependence of scintillator sensitivity on. This compensation method is based on the correlation between temperature, sensitivity, and scintillation ...
1999-07-01
Evaluation of six decontamination processes on actinide and fission product contamination
Energy Technology Data Exchange (ETDEWEB)
In-situ decontamination technologies were evaluated for their ability to: (1) reduce equipment contamination levels to allow either free release of the equipment or land disposal, (2) minimize residues generated by decontamination, and (3) generate residues that are compatible with existing disposal technologies. Six decontamination processes were selected. tested and compared to 4M nitric acid, a traditional decontamination agent: fluoroboric acid (HBF{sub 4}), nitric plus hydrofluoric acid, alkaline persulfate followed by citric acid plus oxalic acid, silver(II) plus sodium persulfate plus nitric acid, oxalic acid plus hydrogen peroxide plus hydrofluoric acid, and electropolishing using nitric acid electrolyte. The effectiveness of these solutions was tested using prepared 304 stainless steel couponds contaminated with uranium, plutonium, americium, or fission products. The ...
1995-12-31
Energy Technology Data Exchange (ETDEWEB)
This study investigates spent fuel cask handling experience at existing nuclear facilities to determine appropriate cask decontamination and maintenance operations at the potential Yucca Mountain repository. These operations are categorized as either routine or nonroutine. Routine cask decontamination and maintenance tasks are performed in the cask preparation area at the repository. Casks are taken offline to a separate cask maintenance area for major nonroutine tasks. The study develops conceptual designs of the cask preparation area and cask maintenance area. The functions, layouts, and major features of these areas are also described.
1992-04-01
Studies on radioactive liquid waste treatment by reverse osmosis
Energy Technology Data Exchange (ETDEWEB)
Reverse osmosis is a simple process and has relatively high decontamination factor compared to other processes used for the treatment of radioactive liquid waste. Furthermore the quantity of secondary waste of this process is small. In this study, test solution containing nine elements such as cesium, strontium, cobalt etc. in chloride forms are treated by reverse osmosis. Permeate rate decreases as the increase of osmotic pressure of feed solution and is expressed by linear equation. Decontamination factor of cations of univalency is more than ten, and about one tenth of that of bivalency. Decontamination factors of all the elements used in this experiment are approximately estimated using the solution-diffusion model.
1982-06-01
Studies on radioactive liquid waste treatment by reverse osmosis
International Nuclear Information System (INIS)
Reverse osmosis is a simple process and has relatively high decontamination factor comparing to other processes used for the treatment of radioactive liquid waste. Furthermore the quantity of secondary waste of this process is small. In this study, test solution containing nine elements such as cesium, strontium, cobalt etc. in chloride forms are treated by reverse osmosis. Permeate rate decreases as the increase of osmotic pressure of feed solution and is expressed by linear equation. Decontamination factor of cations of univalency is more than ten, and about one tenth of that of bivalency. Decontamination factors of all the elements used in this experiment are approximately estimated using the solution-diffusion model. (author).
International Nuclear Information System (INIS)
The document represents a guide for the external decontamination of persons accidentally radio contaminated due to the use, production or transport of radioactive materials. The general conditions, from the medical point of view, to be kept in mind, in the event of accidental overexposures as decontamination treatment and the handling of samples are detailed throughout report. The external contamination without injury in skin or with wound its considered. The distribution of measures and responsibilities for the therapy of the irradiated patients with radioactive materials are enumerated. The preparations of decontaminate solutions are detailed in this work. Moreover, forms for the reception, physical evaluation of the patient and external contamination are presented. (author)
International Nuclear Information System (INIS)
During a high temperature treatment of the radioactive wastes that contain ruthenium, some ruthenium is volatilized and released to the off gas system. The volatilized ruthenium is removed with a scrubber and an adsorber. It was expected that the scrubber was one of the most effective equipments to remove ruthenium and the decontamination factor of the scrubber was studied. The experimental apparatus was simulated as part of an actual perforated plate column scrubber. The non-radioactive ruthenium which simulated the radioactive ruthenium was volatilized and fed into the scrubber. The decontamination factor of the scrubber was determined by the ratio of the ruthenium concentration at the inlet and outlet of the scrubber off gas stream. The results showed that the scrubber removed the volatile ruthenium effectively as expected.
1993-07-01
Energy Technology Data Exchange (ETDEWEB)
In the well-known devices for increasing the decontamination factor in the treatment of radioactive waste water by evaporation, which consist of narrowing devices with evaporator sump and condenser, droplets of liquid and solid particles are carried over from the breeder space, which are radioactive and therefore make the decontamination factor worse. Better results are obtained if one places a fibre bed filter between the evaporator sump and the condenser, preferably in a horizontal connecting pipe between the evaporator sump and the condenser.
1982-06-09
Decontamination of building surface using clay suspension
Energy Technology Data Exchange (ETDEWEB)
The decontamination of the urban building surfaces, based on the covering of clay suspensions, has been studied. Contaminated samples for test purpose were prepared by application of radioactive solution which was extracted from the soil of 2 km zone of the Chernobyl Nuclear Power Plant(ChNPP). The cation converting conditions of clay suspensions were determined by the experiments of swelling and stability of the suspensions. According to the experimental results, the most effective clay suspension was the NH{sub 4}-type which had a 7.1 of decontamination factor(DF) on Cs and 4.5 of DF on total nuclides after 3 times covering on slate.
1994-07-01
A pilot plant demonstration of the vitrification of radioactive solutions using microwave power
Energy Technology Data Exchange (ETDEWEB)
A process has been developed that exploits the characteristics of microwave heating for the vitrification of high-level radioactive liquid waste. This process, microwave vitrification, has been successfully operated at pilot plant scale in an active cell using simulated liquid waste containing several curies of radioactivity. Excellent decontamination factors have been achieved for both volatiles and nonvolatiles with an average ruthenium decontamination factor of 490 and a gross alpha emitter decontamination factor of 100,000. Almost all the radioactivity is incorporated in a glass block.
1986-01-01
A pilot plant demonstration of the vitrification of radioactive solutions using microwave power
International Nuclear Information System (INIS)
A process has been developed that exploits the characteristics of microwave heating for the vitrification of high-level radioactive liquid waste. This process, microwave vitrification, has been successfully operated at pilot plant scale in an active cell using simulated liquid waste containing several curies of radioactivity. Excellent decontamination factors have been achieved for both volatiles and nonvolatiles with an average ruthenium decontamination factor of 490 and a gross alpha emitter decontamination factor of 100,000. Almost all the radioactivity is incorporated in a glass block.
Energy Technology Data Exchange (ETDEWEB)
The small pilot facility of a cyclone type suspension incineration system of radioactive waste was set up in order to evaluate the decontamination efficiency of a high efficiency ceramic filter. The evaluation was made by use of /sup 54/Mn, /sup 59/Fe, /sup 60/Co, /sup 65/Zn and /sup 137/Cs. 1. The decontamination factor by one line of ceramic filter for every species were over 10/sup 5/. 2. The decontamination factor increased by one oder when water vapor exists in off-gas. The same tendency was also observed when iron dioxide existed at the incineration of cation exchange resin.
1987-02-01
International Nuclear Information System (INIS)
The small pilot facility of a cyclone type suspension incineration system of radioactive waste was set up in order to evaluate the decontamination efficiency of a high efficiency ceramic filter. The evaluation was made by use of "5"4Mn, "5"9Fe, "6"0Co, "6"5Zn and "1"3"7Cs. 1. The decontamination factor by one line of ceramic filter for every species were over 10"5. 2. The decontamination factor increased by one oder when water vapor exists in off-gas. The same tendency was also observed when iron dioxide existed at the incineration of cation exchange resin. (author).
Flow rate and decontamination factor of "1"3"7Cs and "1"3"1I through mixed resin bed
International Nuclear Information System (INIS)
(Sep 1971). Japan Yokotsuka, Seiichiro Mitsubishi Chemical Industries, Ltd.,
Decontamination of the reactor coolant pump in Maanshan nuclear power plant
International Nuclear Information System (INIS)
To reduce the radiation dose that accumulated on the reactor coolant pump, decontamination work was carried out at the Maanshan Nuclear Power Plant. A four-step alkaline permanganate (AP)-CanDecon process was applied to remove the activity on the turning vane diffuser and pump impeller. The first step consisted of 8 h of AP treatment and 7 h of decontamination. It was followed by 2.5 h of AP treatment and 5 h of decontamination. An average decontamination factor of 2.9 was obtained. To understand the corrosion of the decontaminating reagents on the materials, coupons were installed in the decontamination tank. These were as-received and sensitized 304SS, alloy 600, casting stainless steel (CF-8), stellite-6, and carbon steels (A508 and A533). The exposure rates (mR h"-"1) of the carbon steels were approximately five times higher in magnitude than those of the ...
Decontamination of a gas-cooler by means of chemical reagent loaded foams
Energy Technology Data Exchange (ETDEWEB)
This paper briefly describes an industrial application of the foam decontamination process applied to large volume components. The process is based on the filling of the component with liquid foam containing suitable chemical reagents, and a circulation loop enables its continuous recycling. The process was successfully validated during the decontamination of a graphite gas-cooler representing a developed area of 1000 m{sup 2}. A decontamination factor up to 190 was obtained leading to a residual activity below 1 Bq/cm{sup 2}. The process only produced 6 m{sup 3} of effluent i.e. about ten times less than for a chemical solution technique. (authors) 2 refs.
1995-12-31
Energy Technology Data Exchange (ETDEWEB)
The development of new steels is always a challenge for the manufacturer of filler metals. In many cases it is obvious that some properties of the base metal cannot be fulfilled with matching filler metals. In some cases, dissimilar filler metals can solve the problem in some cases, there is no chance to meet the requirements of the base metal (for example yield strengths of new ultra high strength steels). This paper deals with different kinds of new steels and the requirements for the weld metal with examples from motor car industry (Mangan Austenite), crane (Ultra high strength steels), earthmoving machinery (Wear-resistant steels) and offshore (Supermartensitic steels). Specific problems will be discussed and best solutions will be highlighted. These examples make clear that the success of new kinds of steels in the market depends on solving the joining problems of these steels. (Abstract Copyright ...
2007-07-15
Ultra-high temperature strength properties on Mod.9Cr-1Mo steel
Energy Technology Data Exchange (ETDEWEB)
A sodium-water reaction drove from the single tube break in steam generator of FBR might overheat labor tubes rapidly under internal pressure loadings. If the temperature of tube wall becomes too high, it has to be evaluated that the stress of tube does not exceed the material strength limit to prevent the propagation of tube rupture. This study clarified the tensile and creep properties of Mod.9Cr-1Mo steel at ultra-high temperature which will be used in evaluation of the tube burst by sodium-water reaction. The strain rates for tensile test are from 10%/min to 10%/sec, and creep-rupture time is maximum 277sec. The range of test temperature is 700degC to 1300degC. The main results obtained were as follows; (1) The evaluation data on the relationship between tensile strength and strain rate and creep-rupture strength in shorter time on Mod.9Cr-1Mo steel were acquired. (2) Short-term mechanical properties of Mod.9Cr-1Mo steel were evaluated based on the results of ...
2000-03-01
Energy Technology Data Exchange (ETDEWEB)
The high-strength and ultra high-strength steels developed and produced by Thyssen Krupp Stahl make a major contribution to automotive lightweighting. Proven and newly-developed coatings are used to meet increasingly important corrosion protection requirements. Design for materials, optimized forming and joining processes and the use of modern simulation techniques help to exploit the potential of the new steels. Future development work will focus on reducing the density of steels without compromising their well-known advantages - in particular their strength. The use of high-strength and ultra high-strength steels in the automotive industry is on the increase. Steel will remain the material of choice for auto manufacture, above all due to its potential for cost-efficient lightweight construction and its full recyclability. (orig.) [German] Einen wesentlichen Beitrag zum Leichtbau im Automobil leisten ...
1999-04-01
The steroidogenic factor 1 (SF-1, also known as NR5A1) is a transcription factor belonging to the nuclear receptor superfamily. Whereas most of the members of this family have been extensively characterized, the therapeutic potential and pharmacology of SF-1 still remains elusive. Described here is the identification and characterization of selective inhibitory chemical probes of SF-1 by a rational ultra-high-throughput screening (uHTS) strategy. A set of 64,908 compounds from the National Institute of Health's Molecular Libraries Small Molecule Repository was screened in a transactivation cell-based assay employing a chimeric SF-1 construct. Two analogous isoquinolinones, ethyl 2-[2-[2-(2,3-dihydro-1,4-benzodioxin-7-ylamino)-2-oxoethyl]-1-oxoisoquinolin-5-yl]oxypropanoate (SID7969543) and ethyl 2-[2-[2-(1,3-benzodioxol-5-ylmethylamino)-2-oxoethyl]-1-oxoisoquinolin-5-yl]oxypropanoate and (SID7970631), were identified as potent submicromolar inhibitors, yielding ...
2008-03-11
Edge biasing in the WEGA stellarator
Energy Technology Data Exchange (ETDEWEB)
The WEGA stellarator is used to confine low temperature, overdense (densities exceeding the cut-off density of the heating wave) plasmas by magnetic fields in the range of B=50-500 mT. Microwave heating systems are used to ignite gas discharges using hydrogen, helium, neon or argon as working gases. The produced plasmas have been analyzed using Langmuir and emissive probes, a single-channel interferometer and ultra-high resolution Doppler spectroscopy. For a typical argon discharge in the low field operation, B=56 mT, the maximum electron density is n{sub e}{proportional_to}10{sup 18} m{sup -3} with temperatures in the range of T=4-12 eV. The plasma parameters are determined by using Langmuir probes and are cross-checked with interferometry. It is demonstrated within this work that the joint use of emissive probes and ultra-high resolution Doppler spectroscopy allows a precise measurement of the radial electric field. The focus of this work is ...
2009-02-27
Energy Technology Data Exchange (ETDEWEB)
The theoretical analysis of a partially-ionized hydrogen gas flow (gas temperatures of approximately 10,000 to 20,000 K) through a particular class of magnetohydrodynamic (MHD) generators and the preliminary design of these MHD generators as open cycle, electric power supplies are performed. Analysis of the gas flow through these ultra-high temperature MHD generators requires a coupled gas dynamics/radiative heat transfer solution. Gas dynamics are modeled by a set of quasi-one-dimensional, nonlinear differential equations which account for friction, convective and radiative heat transfer and the interaction between the ionized gas and applied magnetic field. Radiative heat transfer is modeled using non-gray, absorbing-emitting two- and three-dimensional P-1 approximations which permit an arbitrary variation of the spectral absorption coefficient with frequency. Gas dynamics and radiative heat transfer are coupled through the energy equation, and through the ...
1990-01-01
Savannah River Technology Center monthly report
Energy Technology Data Exchange (ETDEWEB)
This report for the month of June 1995 presents information on the typical topics of tritium processing, environmental studies, waste management issues, and miscellaneous projects. The document consists many small reports by individuals or small groups.
1995-06-01
New intelligent monitor for CANDU type NPP
International Nuclear Information System (INIS)
Nuclear energy provides a third of Europe's electricity with nearly no greenhouse-gas emissions. Sustained efforts are now being conducted to harmonize regulations all over Europe through WENRA and to converge on technical nuclear safety practices within the TSO network ETSON (European Technical Safety Organizations Network). In CANDU type NPP the tritiated water occurs by the neutron bombardment of deuterium. The tritiated water vapors imply health hazard (in the critical organs of the body the water presents a 10 day average biological half-life) and the early detection in nuclear plants of tritium emissions is important because the tritiated water vapors have the same characteristics as of atmospheric water vapors. By detecting tritiated vapors, the monitoring system ensures the following objectives: (a) indicates levels of tritium generally due to heavy water leakage, (b) reduces the possibility of health hazard. In order to attain this ...
2009-10-12
Mixed Waste Management Facility (MWMF) groundwater monitoring report, second quarter 1992
Energy Technology Data Exchange (ETDEWEB)
During second quarter 1992, tritium, trichloroethylene, tetrachloroethylene, chloroethene, antimony, 1,1-dichloroethylene, lead, nonvolatile beta, radium-228, thorium-228, or total alpha-emitting radium (radium-226 and radium-228) exceeded the US Environmental Protection Agency Primary Drinking Water Standards (PDWS) in groundwater samples from monitoring wells at the Mixed Waste Management Facility (MWMF) and adjacent facilities. Tritium and trichloroethylene were the most widespread constituents; 55 (48%) of the 115 monitored wells contained elevated tritium activities, and 23 (20%) wells exhibited elevated trichloroethylene concentrations. Sixty-three downgradient wells screened in Aquifer Zone IIB2 (Water Table), Aquifer Zone IIB[sub 2] (Barnwell/McBean), and Aquifer Unit IIA (Congaree) contained concentrations of tritium, trichloroethylene, tetrachloroethylene, chloroethene, antimony, ...
1992-09-01
Fusion Reactor Radioactive Waste Management.
Quantities and compositions of non-tritium radioactive waste are estimated for some current conceptual fusion reactor designs, and disposal of large amounts of radioactive waste appears necessary. Although the initial radioactivity of fusion reactor and f...
1976-01-01
Energy Technology Data Exchange (ETDEWEB)
It was previously reported that the tritium tracer method is useful for the quantitative consideration of hydrogen behavior in coal during coal liquefaction reaction. Tetralin is excellent hydrogen donating solvent, and is considered as one of the model compounds of coal. In this study, effects of H2S and H2O on the hydrogen exchange reaction between tetralin and gaseous hydrogen labeled by tritium were investigated. It was suggested that the conversion of tetralin and the hydrogen exchange reaction between gaseous hydrogen and tetralin proceed through the radical reaction mechanism with a tetralyl radical as an intermediate product. When H2S existed in this reaction, the hydrogen exchange yield increased drastically without changing the conversion yield. This suggested that the hydrogen exchange reaction proceeds even in the reaction where radical does not give any effect. In the case of H2O addition, the conversion yield and hydrogen exchange ...
1996-10-28
Radioprotective effect of fish products
International Nuclear Information System (INIS)
New fish cans were prepared in the Institute of Fish Industry, Burgas (BG), containing pectin and additives. A biological experimental study was conducted to investigate the decontaminating effect of the new products. The results demonstrated no decontaminating effect in relation to radiocesium and radiostrontium. A pronounced prophylactic effect was observed in case of external irradiation, judged by endogenous spleen colonies. (author).
1993-12-02
International Nuclear Information System (INIS)
Some of the Indian pressurized heavy water reactors (PHWRs) which use Stellite balls in the ball and screw mechanism of the adjustor rod drive mechanism in the moderator circuit have encountered high radiation fields in the moderator system due to "6"0Co. Release of particulate Stellite is responsible for the hotspots in addition to the general uniform contamination of internal surfaces with "6"0Co. Extensive laboratory studies have shown that it is possible to dissolve these Stellite particles by adopting a three-step redox process with permanganic acid as the oxidizing agent. These investigations with inactive Stellite in powder form helped to optimize the process conditions. Permanganic acid was found to have the highest dissolution efficiency as compared to alkaline and nitric acid permanganate. The susceptibility of Stellite to corrode or dissolve was found to depend on the concentration of the permanganate, pH and temperature of the process and microstructure of the Stellite ...
2011-06-01
Dose reduction by chemical decontamination
International Nuclear Information System (INIS)
At the Borssele Nuclear Power Station, which has been in operation since 1973, a comprehensive program of modifications, one of the most extensive of its kind worldwide, was conducted in 1997 within the framework of an integral safety evaluation carried out at ten-year intervals, especially in the nuclear section. The collective dose associated with this activity was greatly reduced by Alara measures, one of which was chemical decontamination of part of the emergency and residual heat removal systems. An average decontamination factor (DF) of 17 was achieved by using the Siemens Cord UV process. Two decontamination cycles were required. The decontamination program took three days to be completed. The planned collective dose was reduced from 1029 mSv (without decontamination) to 335 mSv (on the basis of a DF of 8). Based on the DF of 17 achieved, the planned dose was corrected ...
1998-10-01
Clinoptilolite filter for the removal of tritiated water vapour
International Nuclear Information System (INIS)
The removal of tritiated water vapour was tested by use of a small burning apparatus and a clinoptilolite filter. It was found that decontamination factor of about 10"4 could be obtained by a clinoptilolite filter. The adsorption of HTO in the clinoptilolite is caused by the diffusion, so it is necessary that filtration velocity is maintained below 0.01 m/sec. Decontamination factor was not influence by the moisture content of a clinoptilolite and tritiated water vapour once adsorbed on a filter was hardly removed. (auth.).
Energy Technology Data Exchange (ETDEWEB)
Volume VII of the documentation for the Phase I Data Analysis Task performed in support of the current Regional Flow Model, Transport Model, and Risk Assessment for the Nevada Test Site Underground Test Area Subproject contains the tritium transport model documentation. Because of the size and complexity of the model area, a considerable quantity of data was collected and analyzed in support of the modeling efforts. The data analysis task was consequently broken into eight subtasks, and descriptions of each subtask's activities are contained in one of the eight volumes that comprise the Phase I Data Analysis Documentation.
1996-12-01
Possible influence of vacuum polarization on Q/sub 1//sub //sub s/ in muon catalyzed D-T fusion
Energy Technology Data Exchange (ETDEWEB)
The vacuum polarization splitting of the M-shell states in muonic hydrogen can have a profound influence on the muonit de-excitation cascade in deuterium and tritium targets. The cascade also shows sensitive dependence on the precise rate of transfer processes between certain excited muonic deuterium and tritium atoms. Recent experimental data, where a much greater population of the (d..mu..) qs state (1/sub 1//sub //sub s/) was found than previously predicted, can be explained if the transfer rates from the (d..mu..) M-shell are assumed to be strongly suppressed.
1988-12-27
Analysis of tritium mission FMEF/FAA fuel handling accidents
Energy Technology Data Exchange (ETDEWEB)
The Fuels Material Examination Facility/Fuel Assembly Area is proposed to be used for fabrication of mixed oxide fuel to support the Fast Flux Test Facility (FFTF) tritium/medical isotope mission. The plutonium isotope mix for the new mission is different than that analyzed in the FMEF safety analysis report. A reanalysis was performed of three representative accidents for the revised plutonium mix to determine the impact on the safety analysis. Current versions computer codes and meterology data files were used for the analysis. The revised accidents were a criticality, an explosion in a glovebox, and a tornado. The analysis concluded that risk guidelines were met with the revised plutonium mix.
1997-11-18
Energy Technology Data Exchange (ETDEWEB)
The report addresses the application of reverse osmosis to the treatment of radioactive liquid waste, focusing on the effects of non-radioactive cations and anions, existing in radioactive waste, on the removal of radioactive nuclides. The bivalent cations are generally about ten times as high in decontamination factor as monovalent ones. In the case of anions, the factor of SO{sub 4}{sup 2-} is about ten times that of Cl{sup -} while that of NO{sub 3}{sup -} is somewhat smaller than that of Cl{sup -}. During permeation through membrane, anions tend to accompany cations, and the decontamination factor of accompanying ions is found to increase with that of the paring ions. These results indicate that if one can select components that will remain in the liquid waste, one should consider their effects on the efficiency of its treatment. Furthermore, the interaction between two anions or between two cations can be approximated by a linear equation ...
1991-01-01
International Nuclear Information System (INIS)
A series of tests has been carried out to determine the operating conditions required to remove the corrosion deposit from samples cut from Winfrith Steam Generating Heavy Water Reactor (WSGHWR) primary circuit pipework by submerged water jetting. Two types of samples were used - one set subjected to the normal annual reactor decontamination using TURCO reagents, the other set having been given a LOMI treatment in addition. Tests showed that useful decontamination factors could be achieved on both types of sample, but significantly less severe operating conditions were required to decontaminate the LOMI treated samples. A decontamination factor of 10 was achieved on TURCO treated samples at 360 Bar; only 200 Bar was required to achieve the same decontamination factor on LOMI treated samples. No metal erosion of the stainless steel substrate was found to occur at these pressures. ...
Radiation decontamination of dry food ingredients and processing aids
International Nuclear Information System (INIS)
Radiation decontamination of dry ingredients, herbs and enzyme preparations is a technically feasible, economically viable and safe physical process. The procedure is direct, simple, requires no additives and is highly efficient. Its dose requirement is moderate. Radiation doses of 3-10 kGy (0.3-1 mrad) have proved sufficient to reduce the viable counts to a satisfactory level. Ionising radiations do not cause any significant rise in temperature. The flavour, texture or other important technological or sensory properties of most ingredients are not influenced at radiation doses necessary for satisfactory decontamination, and radiation obviates the chemical residue problem. The microflora surviving radiation decontamination of dry ingredients are more susceptible to subsequent antimicrobial treatments. Recontamination can be prevented as the product can be irradiated in its final packaging. Irradiation could be carried out ...
International Nuclear Information System (INIS)
In nuclear power plant Paks, Hungary, alkaline oxidative (NaOH, KMnO_4, H_2O) and acidic reductive (citric- and oxalic acid, water) liquids are using for the decontamination of primary circuit equipment (main liquid circulating pumps, steam generators, pipelines etc). The above mentioned decontamination liquids are containing "1"1"0"mAg, "9"5Nb, "5"4Mn, "5"8 Co, "6"0Co, "5"1 Cr, "1"2"4 Sb radioisotopes, summarized radioactivity is between 10"3-8x10"4 kBq/dm"3 liquid. The decontamination liquid can be cleaned with reactive adsorption (active carbon) and ion-exchange process at elevated temperature (333-368 K) in multilayered columns. After purification the summarized radioactivity for "5"4Mn, "6"0Co, and "1"1"0"mAg are in the outlet liquid below 1 kBq/dm"3. Decontamination factor DF#approx =#10"3-10"4, volumetric reduction factor VRF#approx =#50-500.
1999-11-04
International Nuclear Information System (INIS)
To raise the efficiency of the redox method and decrease the amount of radioactive wastes, a possibility of improving the decontamination process for NPP heat exchanger tubes made of stainless steel is studied. In the home practice the redox method of equipment decontamination is carried out as a multi-cycle process. In each cycle the surface is treated first with a permanganate alkaline solution ther with an oxalic acid solution, with a condensate washing-at between the treatments. Using samples cut out of the steam generator pipelines of the first and third power units of the Novovoronezh NPP the effect of the oXalic acid concentration, as well as washout time and conditions on the decontamination factor are studied. On the basis of analysis of the obtained data a conclusion is drawn that using oxalic acid of low concentrations and increasing its concentrations from cycle to cycle maximum ...
Decontamination of a gas cooler using foams containing chemical reagents
Energy Technology Data Exchange (ETDEWEB)
This paper deals with an industrial application of the foam decontamination process applied to large volume components. The work presented below was achieved within the context of a CEC contract. The objective of this 4-year programme was to study, develop and demonstrate an effective in-situ decontamination process using foams containing suitable chemical reagents. Laboratory tests were first performed to optimize the chemical formulation of the foams. Pilot tests were then conducted to study the hydrodynamic features of the fluids and to adapt a technique of permanent foam circulation. With these tests completed, it was essential to validate the foam process on an industrial scale and on a representative nuclear component. The objective was successfully achieved. The process was effectively validated during the decontamination of a graphite-gas cooler representing a developed area of 1000 m{sup 2}. Results were quite ...
1994-12-31
Decontamination factor of the commercial detergents for the skin (part 3)
Energy Technology Data Exchange (ETDEWEB)
The commercial detergents, which are cleansing cream, shampoo, neutral detergent, etc., were examined in order to select the body cleaners that are substitutes for the titanium dioxide paste. JNC entrusted Japan Environment Research Corporation Limited with these examinations since 1997. In 1997 and 1998, the commercial detergents were examined for Ce-144, Cs-137 and Ru-106. In 1999, 22 detergents were examined for Co-60 from the result of the past examinations. In this examination, the radioactive solution of Co-60 was dropped on the pig-skin samples. These samples were washed with each detergent after 5 minutes and 40 minutes. The decontamination factors of detergents were estimated by the radioactive ratio of the samples before and after washing. As a result of this examination, the decontamination factors for Co-60 was the same as the decontamination factors for Ce-144 and Cs-137, and 11 detergents were nominated as the ...
2000-08-01
Decontamination factor of the commercial detergents for the skin (part 3)
International Nuclear Information System (INIS)
The commercial detergents, which are cleansing cream, shampoo, neutral detergent, etc., were examined in order to select the body cleaners that are substitutes for the titanium dioxide paste. JNC entrusted Japan Environment Research Corporation Limited with these examinations since 1997. In 1997 and 1998, the commercial detergents were examined for Ce-144, Cs-137 and Ru-106. In 1999, 22 detergents were examined for Co-60 from the result of the past examinations. In this examination, the radioactive solution of Co-60 was dropped on the pig-skin samples. These samples were washed with each detergent after 5 minutes and 40 minutes. The decontamination factors of detergents were estimated by the radioactive ratio of the samples before and after washing. As a result of this examination, the decontamination factors for Co-60 was the same as the decontamination factors for Ce-144 and Cs-137, and 11 detergents were nominated as the ...
Tritium release from lithium orthosilicate pebbles deposited with palladium
International Nuclear Information System (INIS)
Full text of publication follows: Slightly over-stoichiometric lithium orthosilicate pebbles have been selected as one optional breeder material for the European Helium Cooled Pebble Bed (HCPB) blanket. This material has been developed in collaboration of Research Center Karlsruhe and the Schott Glass, Mainz. The lithium orthosilicate pebbles are fabricated from lithium hydroxide and silica by a melting and spraying method in a semi-industrial scale facility. Lithium hydroxide was selected as the precursor since enriched lithium hydroxide is commercially available. The lithium orthosilicate pebbles produced by the process contains oxide phases besides orthosilicate, but it was also found that the oxide phases can be decomposed by annealing at high temperatures. The lithium orthosilicate pebbles produced in this way possesses satisfactory pebble characteristics. Therefore, the authors performed out-of-pile annealing tests using the lithium orthosilicate pebbles irradiated in a research ...
2007-12-10
Incorporation of tritiated stearic acid in polymer
Energy Technology Data Exchange (ETDEWEB)
The chemical fixation of tritium in stearic acid followed by embedding the tritiated stearic acid into an epoxy resin proved to be a good method for permanent waste disposal of tritium gas. Tc-126 and Tc-136 hardener were used for this purpose. The polymerization temperature of the polymer products was found to be highly decreased by adding stearic acid and slightly decreased by adding stearic acid or by raising the temperature of the leachant medium and slightly decreased by irradiation. On the other hand, small improvement in the compressive strength of the polymer products was achieved by adding silica powder. The polymer product showed high flame points above 573 K although it contains stearic acid. DTA and TG analysis indicate that the thermal stability of polymer products containing stearic acid and silica powder is better than samples containing only stearic acid. Stearic acid was found to possess good resistance to irradiation and the ...
1997-10-01
Energy Technology Data Exchange (ETDEWEB)
This study of the hydrogeology of Chicken Creek Canyon wasconducted by the Environmental Restoration Program (ERP) at LawrenceBerkeley National Laboratory (LBNL). This canyon extends downhill fromBuilding 31 at LBNL to Centennial Road below. The leading edge of agroundwater tritium plume at LBNL is located at the top of the canyon.Tritium activities measured in this portion of the plume during thisstudy were approximately 3,000 picocuries/liter (pCi/L), which issignificantly less than the maximum contaminant level (MCL) for drinkingwaterof 20,000 pCi/L established by the Environmental ProtectionAgency.There are three main pathways for tritium migration beyond theLaboratory s boundary: air, surface water and groundwater flow. Thepurpose of this report is to evaluate the groundwater pathway.Hydrogeologic investigation commenced with review of historicalgeotechnical reports including 35 bore logs and 27 test pit/trench logsas ...
2007-10-31
Energy Technology Data Exchange (ETDEWEB)
While tritium exposure to the site-workers in Wolsung NPP is up to about 40% of the total personnel exposure, Ministry of Science and Technology has asked tritium removal facility for requirement of post heavy-water reactor construction. For the purpose of essential removal of tritium from the Wolsung heavy-water reactor system, a preliminary study on the cryogenic Ar-N{sub 2} and H{sub 2}-D{sub 2} distillation process for development of liquid-phase catalytic exchange cryogenic hydrogen distillation process technology. The Ar-N{sub 2} distillation column showed good performance with approximately 97% of final Ar concentration, and a computer simulation code was modified using these data. A simulation code developed for cryogenic hydrogen isotopes (H{sub 2}, HD, D{sub 2}, HT, DT, T{sub 2}) distillation column showed good performance after comparison with the result of a JAERI code, and a H{sub 2}-D{sub 2} distillation ...
1995-12-01
International Nuclear Information System (INIS)
Metal waste generated from domestic nuclear operation for defense and commercial application has led to a growing stockpile of radioactively contaminated scrap metal, much of which is stainless steel. A significant fraction of this material cannot be efficiently surface decontaminated. The burial of this material would be wasteful and expensive, since long term monitoring would be necessary in order to minimize environmental risk. Much of this waste consists of bulky equipment. In many case, this equipment contains valuable material that may be recycled. The piece of equipment considered frequently also has complex geometries, making extremely difficult, time-consuming and expensive to determine the exact location and level of radioactivity on the internal surfaces. After melting, however, the radioactivity may be precisely determined from samples of each ingot. Moreover, an ingot may be released for restricted or unrestricted reuse, or stored for decay to ...
2007-05-10
Use of fuel cells to meet military requirements for mobile power
International Nuclear Information System (INIS)
'Full text:' The use of fuel cell technology in military applications will depend on safe, high energy density systems being developed. An important part of using this technology is also the development of alternative hydrogen producing fuels with high energy densities and are easy to transport. Fuel cells are now a very large R and D effort for several military applications around the world. The major reason is because of the high power demands needed requires electrical energy sources that far exceed the capabilities of batteries currently being fielded for portable applications. Fuel cells are regarded as highly efficient, tactical energy converters that can be adapted for wide range of power requirements. They are potentially the lowest weight power source when coupled with batteries or capacitors to form hybrid systems. Generally electrical power is needed to support a number of applications from ultra-high power for electrical pulses (radios, sensors) to ...
2004-09-25
Ultra high-speed (508 MHz) beam position digital feedback system
Energy Technology Data Exchange (ETDEWEB)
The B-Factory which is constructed by National Laboratory for High Energy Physics is the device for elucidating the breakdown of symmetry of matter and antimatter by studying the behavior of B mesons which are generated in large quantity when the electrons and the positrons which are accelerated to light velocity level are collided. In order to maintain electron beam-positron beam bunch circling the ring at light velocity stably, the instability of the coupled bunch must be overcome. For this purpose, the ultrahigh speed beam position digital feedback control system was developed. This system is composed of the high speed input-output substrate using GaAs LSI, the feedback computation substrate using complementary metal oxide semiconductor and the memory mounted on it, and the real time operation device. The development of both substrates and their functions are explained. The real time data collection and the change of computation parameters for specific bunch in the real time ...
1997-02-01
Energy Technology Data Exchange (ETDEWEB)
This paper describes an investigation of electrodeposited Zn-14% Ni and aluminium-based SermeTel 1140/962 coatings as possible replacements for cadmium. Slow strain rate tests were performed to measure the extent of direct hydrogen embrittlement of a high strength steel substrate as a result of the coating process and of hydrogen re-embrittlement caused by coating corrosion. The level of re-embrittlement was shown to depend on both the electrochemical potential of the coating and its barrier properties. Zn-14% Ni coatings caused the most re-embrittlement as they had the most active potential and contained through-thickness defects which left the steel exposed to hydrogen uptake. The microstructure of the high strength steel was also shown to be an important factor affecting the extent of embrittlement. AerMet 100 steel was more resistant than 300M steel and this was attributed to the presence of reverted austenite surrounding the martensite laths in AerMet 100, which trapped absorbed ...
2008-04-15
The Schenberg spherical antenna: status report
International Nuclear Information System (INIS)
Full text. Here we present a status report of the Schenberg antenna, which started commissioning runs in September 2006 under the full support of FAPESP. In its first commissioning runs we tested three preliminary parametric transducer systems, which did not achieve a high enough performance for placing the antenna sensitivity in the range of the calibrator capacitor. Instead of improving the calibrator, making it capable of introducing a larger input force, we decided to go to a radical upgrading operation: replacing the three transducers for a complete set of six transducers, with better sensitivity and arranged according to the truncated icosahedron configuration, plus two extra ones; starting to install the dilution refrigerator; installing wires, cables, and amplifiers for the complete set of transducer circuits; and a new suspension and vibration isolation system for the cabling and microstrip antennas. We also have been developing a new set of transducers, microwave oscillators, ...
2009-09-14
Energy Technology Data Exchange (ETDEWEB)
Research and development has been performed on photochromic materials expected to be used in ultra-high density recording, high resolution indication and photoswitches. With regard to molecular orientation in the ternary system mixed LB film, the result of structural analysis by XPM spectrum revealed that the acceptor constituent in the LB film is so structured that it is separated and laminated with two other constituents, and that the sensitizer constituent and the donor constituent are not recognized of being separated definitely. Regarding the electron movement reaction in the solid phase system, a photo-current measuring experiment was carried out on the laminated film which is vacuum-deposited with the ternary system comprising of the donor, sensitizer, and acceptor. It was concluded that the observed photo-current reflects the electron movement reaction in the solid phase as it is. For the photo-current in the LB film, increase in the photo-current was ...
1990-03-01
Radiations emitted in the decay of /sup 165/Er: A promising medical radionuclide
The 10.3-h /sup 165/Er, decaying by electron capture to stable /sup 165/Ho, offers an excellent promise for use in diagnostic nuclear medicine, especially in conjuction with multiwire proportional-counter cameras. Using an ultra-high-resolution Si(Li) photon spectrometer, L and K x-ray photon yields in /sup 165/Er decay have been measured. The ratio P/sub L//P/sub K/ of electron-capture probabilities in L and K shells is determined to be 0.196 +- 0.030, in good agreement with theory. Estimates of Auger electron yields and yields of very-low-energy electrons from Coster--Kronig transitions are presented. Levels of /sup 169/Er and /sup 171/Er radioactive impurities in the reactor-produced /sup 165/Er sample are experimentally determined. Whole-body dose estimates for /sup 165/Er are given. These compare favorably with /sup 99/Tc dose.
1977-05-01
Radiations emitted in the decay of "1"6"5Er: A promising medical radionuclide
International Nuclear Information System (INIS)
The 10.3-h "1"6"5Er, decaying by electron capture to stable "1"6"5Ho, offers an excellent promise for use in diagnostic nuclear medicine, especially in conjuction with multiwire proportional-counter cameras. Using an ultra-high-resolution Si(Li) photon spectrometer, L and K x-ray photon yields in "1"6"5Er decay have been measured. The ratio P/sub L//P/sub K/ of electron-capture probabilities in L and K shells is determined to be 0.196 +- 0.030, in good agreement with theory. Estimates of Auger electron yields and yields of very-low-energy electrons from Coster--Kronig transitions are presented. Levels of "1"6"9Er and "1"7"1Er radioactive impurities in the reactor-produced "1"6"5Er sample are experimentally determined. Whole-body dose estimates for "1"6"5Er are given. These compare favorably with "9"9Tc dose.
Energy Technology Data Exchange (ETDEWEB)
A new industrial process allowing to reach very high cooling rates in the cooling section after soaking of a continuous annealing line for steel sheets is presented. This process constitutes the successful conclusion of a long term research programme, jointly carried out at CRM and Arcelor Cockerill-Sambre for three years, including laboratory experiments, pilot scale trials and several industrial campaigns. It is running on from developments performed in the framework of the HOWAQ (Hot Water Quench) process. The process successively combines a moderate cooling step (600 deg C/s for 0.8 mm thick strips), in boiling water, and a faster cooling step (above 700 deg C/s), by impinging turbulent cold water in a box. Its main features are simplicity, resulting from advanced developments, soundness, flexibility and cooling homogeneity. As treated steel products are characterized by improved mechanical properties, outstanding surface quality (corrosion resistance) and exceptional flatness. The ...
2003-08-01
Mechanism of ageing in irradiated polymers
Energy Technology Data Exchange (ETDEWEB)
Samples of ultra-high molecular weight polyethylene (UHMWPE) and nylon 66, of grades suitable for use in medical prostheses, were subjected to irradiation using a /sup 60/Co source. The effects of a 10 Mrad dose on percentage crystallinity, tensile behaviour and dynamic mechanical response were established 3 days after irradiation at intervals over a one year period. Crystallinity in UHMWPE was found to increase progressively during this period with consequent changes in mechanical behaviour. It is proposed that the observed ageing process arises from the breakdown of metastable groups in the polymer, which are formed on irradiation, with consequent release of long inter-lamella tie chains. This removes an inhibition to crystal perfection processes, which can occur at room temperature in polyethylene. Infra-red spectroscopic evidence supports the proposal that the metastable species is peroxy or hydroperoxy and that this decomposes on ageing to a carbonyl group, ...
1988-01-01
Energy Technology Data Exchange (ETDEWEB)
Fe-Ni-Mn martensitic steels are one of the major groups of ultra-high strength steels that have good mechanical properties and ductility in as annealed condition but they suffer from severe inter-granular embitterment after aging. In this paper, the effect of heavy shaped cold rolling and wire drawing on the mechanical properties of Fe-Ni-Mn steel was investigated. This process could provide a large strain deformation in this alloy. The total strain was {epsilon} {approx}7. Aging behavior and tensile properties of Fe-10Ni-7Mn were studied after aging at 753 K. The results showed that the ultimate tensile strength and ductility after cold rolling, wire drawing and aging increased up to 2540 MPa and 7.1 %, respectively, while the conventional steels show a premature fracture stress of 830 MPa with about zero ductility after aging.
2010-07-01
International Nuclear Information System (INIS)
Fe-Ni-Mn martensitic steels are one of the major groups of ultra-high strength steels that have good mechanical properties and ductility in as annealed condition but they suffer from severe inter-granular embitterment after aging. In this paper, the effect of heavy shaped cold rolling and wire drawing on the mechanical properties of Fe-Ni-Mn steel was investigated. This process could provide a large strain deformation in this alloy. The total strain was #epsilon# #approx#7. Aging behavior and tensile properties of Fe-10Ni-7Mn were studied after aging at 753 K. The results showed that the ultimate tensile strength and ductility after cold rolling, wire drawing and aging increased up to 2540 MPa and 7.1 %, respectively, while the conventional steels show a premature fracture stress of 830 MPa with about zero ductility after aging.
2010-07-01
Hybrid electric vehicles and electrochemical storage systems - a technology push-pull couple
Energy Technology Data Exchange (ETDEWEB)
In the advance of fuel cell electric vehicles (EV), hybrid electric vehicles (HEV) can contribute to reduced emissions and energy consumption of personal cars as a short term solution. Trade-offs reveal better emission control for series hybrid vehicles, while parallel hybrid vehicles with different drive trains may significantly reduce fuel consumption as well. At present, costs and marketing considerations favor parallel hybrid vehicles making use of small, high power batteries. With ultra high power density cells in development, exceeding 1 kW/kg, high power batteries can be provided by adapting a technology closely related to consumer cell production. Energy consumption and emissions may benefit from regenerative braking and smoothing of the internal combustion engine (ICE) response as well, with limited additional battery weight. High power supercapacitors may assist the achievement of this goal. Problems to be solved in practice comprise ...
1999-12-01
Hard, infrared black coating with very low outgassing
Energy Technology Data Exchange (ETDEWEB)
Infrared astronomical instruments require absorptive coatings on internal surfaces to trap scattered and stray photons. This is typically accomplished with any one of a number of black paints. Although inexpensive and simple to apply, paint has several disadvantages. Painted surfaces can be fragile, prone to shedding particles, and difficult to clean. Most importantly, the vacuum performance is poor. Recently a plasma enhanced chemical vapor deposition (PECVD) process was developed to apply thick (30 {micro}m) diamond-like carbon (DLC) based protective coatings to the interior of oil pipelines. These DLC coatings show much promise as an infrared black for an ultra high vacuum environment. The coatings are very robust with excellent cryogenic adhesion. Their total infrared reflectivity of < 10% at normal incidence approaches that of black paints. We measured outgas rates of <10{sup -12} Torr liter/sec cm{sup 2}, comparable to bare ...
2008-06-02
Future limits on isotropic Lorentz violation in the photon sector from UHECRs and TeV gamma rays
Present and future ultra-high-energy-cosmic-ray facilities (e.g., the Pierre Auger Observatory with South and North components) and TeV-gamma-ray telescope arrays (e.g., HESS/VERITAS and CTA) have the potential to set stringent indirect bounds on the nine Lorentz-violating parameters of nonbirefringent modified Maxwell theory minimally coupled to standard Dirac theory. Theoretically, the most interesting case is isotropic Lorentz violation, which is described by a single parameter [taken to vanish for the case of the standard Lorentz-invariant theory]. It appears possible to obtain in the future an upper (lower) indirect bound on this single isotropic Lorentz-violating parameter at the +10^{-21} (-10^{-17}) level. Comparison is made with existing and future direct bounds from laboratory experiments. The possible physics implications of upper bounds at the 10^{-21} level are also briefly discussed.
2011-01-01
First plasma experiment on spherical tokamak device UTST
International Nuclear Information System (INIS)
The UTST (University of Tokyo Spherical Tokamak) device was constructed for the purpose of exploring the formation of ultra-high beta ST (Spherical Tokamak) plasma using the double null plasma merging method. When two plasmas merge together to form a single plasma, magnetic field lines reconnect, and the magnetic field energy is converted to the plasma kinetic energy, increasing the plasma beta. The merging start-up has been demonstrated in the TS-3/4, START and MAST devices using coils inside the vacuum vessel and TS-3 plasma obtained 50% beta. In order to demonstrate the start-up in a more reactor relevant situation, UTST has all poloidal field coils outside the vacuum vessel. The first plasma experiment on the UTST was performed from December, 2007. In the result, the plasma obtained 10 kA by using only outer PF coils and single ST was generated at the lower area (z=-0.3 - -1.0[m]) close to a washer gun. This result suggests that another washer gun on the top of ...
2009-04-01
International Nuclear Information System (INIS)
We present an approach for fabrication of intentionally positioned epitaxial InAs QDs in a micron sized light emitting diode. For site-selective growth, a combination of molecular beam epitaxy (MBE) and focused ion beam (FIB) implantation technology in an all-ultra-high-vacuum (UHV) setup has been employed. Single dot occupancy of almost 55 % on FIB patterned nano-depressions was successfully achieved. Thereafter, carrier injection and subsequent radiative recombination from the positioned InAs/GaAs self-assembled QDs was investigated by embedding these QDs in the intrinsic part of a GaAs-based micron sized p-i-n junction device. Few or single dot are expected to be electrically addressed in these devices. We report results from electroluminescence (EL) measurement which proves the single dot characteristics of our device. The EL spectra consist of sharp emission lines and their dependence on injection current shows linear behavior for exciton and quadratic ...
2010-03-21
Energy-filtered electron microscopy for imaging core-shell nanostructures
Energy Technology Data Exchange (ETDEWEB)
CuAg core-shell nanoparticles are synthesized by ultra-high vacuum thermal evaporation. We show on this system how the Energy-Filtered Transmission Electron Microscopy (EFTEM) technique allows one to improve the characterization by precisely pointing out the formation of core-shell arrangements in bimetallic nanoparticle assemblies. A criterion to measure the shell thickness from EFTEM images on unique core-shell nanoparticles is defined, that can be used for core-shell nanoparticles of any sizes, with shell thicknesses over 1 nm. It is based on the intensity variation along a line drawn across a core-shell nanoparticle on a EFTEM image. This criterion has been validated by a close comparison of the shell thickness measurements performed in this work and the ones obtained by acoustic micro-Raman spectroscopy. Using this criterion, we report a strong correlation between the size of the Cu cores and the formation of the core-shell arrangements in the nanoparticle ...
2008-08-15
Energy Technology Data Exchange (ETDEWEB)
Negative ion electrospray ionization (ESI) coupled with high field Fourier transform ion cyclotron resonance mass spectrometry (FT-ICR-MS) allows for the direct detection of acidic NSO compounds in petroleum. The technique requires no chromatographic separation, is able to distinguish 18 different compound classes (e.g., neutral nitrogen, carboxylic acids and oxygenates), and can identify {approx}14,000 distinct masses by ultra-high mass resolution and mass accuracy. We previously studied three crude oils from different geological origins [Organic Geochemistry 33 (2002b) 743-759]. Here, we expand our research by comparing two source-equivalent Smackover oils of different levels of thermal maturity. We observe clear differences in the distribution of NSO compound classes, types (number of rings plus double bonds within a class), and number of alkyl carbons. With increasing thermal stress, the relative amount of sulfur and oxygen containing compounds decreases, ...
2004-07-01
REQUIREMENTS AND GUIDELINES FOR NSLS EXPERIMENTAL BEAM LINE VACUUM SYSTEMS-REVISION B.
Energy Technology Data Exchange (ETDEWEB)
Typical beam lines are comprised of an assembly of vacuum valves and shutters referred to as a ''front end'', optical elements to monochromatize, focus and split the photon beam, and an experimental area where a target sample is placed into the photon beam and data from the interaction is detected and recorded. Windows are used to separate sections of beam lines that are not compatible with storage ring ultra high vacuum. Some experimental beam lines share a common vacuum with storage rings. Sections of beam lines are only allowed to vent up to atmospheric pressure using pure nitrogen gas after a vacuum barrier is established to protect ring vacuum. The front end may only be bled up when there is no current in the machine. This is especially true on the VUV storage ring where for most experiments, windows are not used. For the shorter wavelength, more energetic photons of the x-ray ring, beryllium windows are ...
1999-05-01
Energy Technology Data Exchange (ETDEWEB)
The Air Force`s Armstrong Laboratory at Tyndall Air Force Base, Florida, has supported the research and development of Radio Frequency Soil Decontamination. Radio frequency soil decontamination is essentially a heat-assisted soil vapor extraction process. Site S-1 at Kelly Air Force Base, San Antonio, Texas, was selected for the demonstration of two patented techniques. The site is a former sump that collected spills and surface run-off from a waste petroleum, oils, and lubricants and solvent storage and transfer area. In 1993, a technique developed by the IIT Research Institute using an array of electrodes placed in the soil was demonstrated. In 1994, a technique developed by KAI Technologies, Inc. using a single applicator placed in a vertical borehole was demonstrated. Approximately 120 tons of soil were heated during each demonstration to a temperature of about 150 degrees Celsius.
1995-04-01
Preconcentration and decontamination in radioanalysis
International Nuclear Information System (INIS)
The scope of radioanalysis can be enlarged substantially by preconcentration. The minimal concentration factor required depends on the concentration to be determined, the limit of determination of the analytical technique and the maximal acceptable sample-weight. Simultaneously, the preconcentration step may cause a decontamination. In post-irradiation chemistry this is usually the crucial parameter. The present paper proposes the classification of (pre-) concentration techniques by the relation between the concentration-factor X and the decontamination-factor Y. In addition, three other criteria here are used to judge the applicability in combination with the analytical technique chosen. They stem from the minimal representative and the maximal acceptable sample-weights and the maximal acceptable dose-rate. The features of a particular combination of (pre-) concentration and analytical technique can be visualized in an X-Y graph. (author).
Practical technological benefits of SRE decommissioning
Energy Technology Data Exchange (ETDEWEB)
The decommissioning of the Sodium Reactor Experiment is essentially complete. Contaminated materials, equipment, and soil were removed, decreasing the residual radioactivity to levels acceptable for future unrestricted use of the site. The fuel was removed and declad, tooling and techniques to support the decommissioning were developed, bulk sodium and residual sodium films were removed, coolant systems were dismantled, the reactor vessel was dissected, the interior surfaces of the facilities were decontaminated, and waste materials were packaged and shipped to burial sites. Radiation exposure to workers and the public was within the guidelines and as low as reasonably achievable. In performing the project, new decontamination techniques were tested, decontamination equipment was evaluated, and waste disposal methods were developed.
1982-01-01
Effect of carrier on surface decontamination efficiency
International Nuclear Information System (INIS)
The dependence was determined of the decontamination factor ratio found in the presence of a carrier and in a carrier-free system on carrier concentration at different concentrations of a complexing agent in a solution. Bearing balls were used as contamination materials while a mixture of "1"5"2Eu and "1"5"4Eu isotopes was used as a contaminant, citric acid in a concentration of 5x10"-"3 to 1x10"-"1 mol/dm"3 as a complexing agent, and Eu, lanthanum and aluminium at a concentration range of 1x10"-"5 to 1x10"-"2 mol/dm"3 as carriers. While no increase in the decontamination factor was found for aluminium, a considerable increase was observed in the isotopic and homologic carriers and the concentration dependence of the carrier reached the maximum. An equation was derived explaining the effect by the isotope exchange between the contaminant and the carrier and by the reaction between the carrier and the complexing agent. (J.F.).
Co-product extraction studies on N-reactor PT-57 target materials
International Nuclear Information System (INIS)
Single pellets (of approximately 70 g each) of irradiated lithium aluminate target from N-Reactor test PT-57 were used in a series of experiments to determine the extent to which the product tritium can be recovered by (a) vacuum outgassing of the target (thermal extraction-TX) and (b) in-vacuo chemical dissolution of the target in molten sodium tetraborate (flux extraction-FX). Five TX runs and seven FX runs were made. Thirty-five percent of the tritium was recovered in a form non-condensable at -196"0C. The remainder was recovered in a condensable form (as T_2O, HTO, etc.). Post-extraction analysis of the melt from the seven flux extractions showed that a maximum of 2 percent of the original amount of tritium remained and that target dissolution was essentially complete in 12 hours. Flux extraction of two pellets which had been subjected to thermal extraction showed less than 0.4 percent of the original amount of ...
Analysis of impurities in beryllium, affecting evaluation of the tritium breeding ratio
International Nuclear Information System (INIS)
In most conceptual fusion power reactor designs, it is proposed to use beryllium as a neutron multiplier in the blanket. Detailed chemical composition of beryllium is necessary for evaluation of the tritium breeding ratio, and estimating the activation and transmutation of beryllium in the fusion reactor. In the present report, special attention was paid to a detailed analysis of impurities in beryllium, relevant to the tritium breeding ratio evaluation. Two different methods were used for the study of impurities: an analysis of the local sample by the ICP-MS method, and an integral analysis of the beryllium assembly, using the pulsed neutron method. The latter method was proposed as the most effective way of analyzing the integral effect to impurities in beryllium on production of the tritium on the lithium-6. The evaluation of the integral effect was based on time behaviour observations of the thermal neutron flux, ...
WIS decontamination factor demonstration test with radioactive nuclides
Energy Technology Data Exchange (ETDEWEB)
A radioactive Waste Incineration System (WIS) with suspension combustion is noticed as effective volume reduction technology of low level radiactive wastes that are increasing every year. In order to demonstrate the decontamination efficiency of ceramic filter used on WIS, this test has been carried out with the test facilities as joint research of Central Research Institute of Electric Power Industry (CRIEPI) and Sumitomo Heavy Industries, Ltd. Miscellaneous combustible waste and power resin, to which 5 nuclides (Mn-54, Fe-59, Co-60, Zn-65, Cs-137) were added, were used as samples for incineration. As the result of the test, it was verified that Decontamination Factor (DF) of the single stage ceramic filter was usually kept over 10/sup 5/ for every nuclide, and from the results of above DF, over 10/sup 8/ is expected for real commercial plant as a total system. Therefore, it is realized that the off-gas clean up system of the WIS composed of ...
1987-04-01
WIS decontamination factor demonstration test with radioactive nuclides
International Nuclear Information System (INIS)
A radioactive Waste Incineration System (WIS) with suspension combustion is noticed as effective volume reduction technology of low level radiactive wastes that are increasing every year. In order to demonstrate the decontamination efficiency of ceramic filter used on WIS, this test has been carried out with the test facilities as joint research of Central Research Institute of Electric Power Industry (CRIEPI) and Sumitomo Heavy Industries, Ltd. Miscellaneous combustible waste and power resin, to which 5 nuclides (Mn-54, Fe-59, Co-60, Zn-65, Cs-137) were added, were used as samples for incineration. As the result of the test, it was verified that Decontamination Factor (DF) of the single stage ceramic filter was usually kept over 10"5 for every nuclide, and from the results of above DF, over 10"8 is expected for real commercial plant as a total system. Therefore, it is realized that the off-gas clean up system of the WIS composed of only single ...
Treatment of radioactive liquid waste by reverse osmosis
International Nuclear Information System (INIS)
The report addresses the application of reverse osmosis to the treatment of radioactive liquid waste, focusing on the effects of non-radioactive cations and anions, existing in radioactive waste, on the removal of radioactive nuclides. The bivalent cations are generally about ten times as high in decontamination factor as monovalent ones. In the case of anions, the factor of SO_4"2"- is about ten times that of Cl"- while that of NO_3"- is somewhat smaller than that of Cl"-. During permeation through membrane, anions tend to accompany cations, and the decontamination factor of accompanying ions is found to increase with that of the paring ions. These results indicate that if one can select components that will remain in the liquid waste, one should consider their effects on the efficiency of its treatment. Furthermore, the interaction between two anions or between two cations can be approximated by a linear equation consisting of the logarithm ...
T Plant secondary containment and leak detection upgrades
Energy Technology Data Exchange (ETDEWEB)
The W-259 project will provide upgrades to the 2706-T/TA Facility to comply with Federal and State of Washington environmental regulations for secondary containment and leak detection. The project provides decontamination activities supporting the environmental restoration mission and waste management operations on the Hanford Site.
1995-10-19
Source term attenuation by water in the Mark I boiling water reactor drywell
Energy Technology Data Exchange (ETDEWEB)
Mechanistic models of aerosol decontamination by an overlying water pool during core debris/concrete interactions and spray removal of aerosols from a Mark I drywell atmosphere are developed. Eighteen uncertain features of the pool decontamination model and 19 uncertain features of the model for the rate coefficient of spray removal of aerosols are identified. Ranges for values of parameters that characterize these uncertain features of the models are established. Probability density functions for values within these ranges are assigned according to a set of rules. A Monte Carlo uncertainty analysis of the decontamination factor produced by water pools 30 and 50 cm deep and subcooled 0--70 K is performed. An uncertainty analysis for the rate constant of spray removal of aerosols is done for water fluxes of 0.25, 0.01, and 0.001 cm{sup 3} H{sub 2}O/cm{sup 2}-s and decontamination factors of 1.1, 2, 3.3, ...
1993-09-01
International Nuclear Information System (INIS)
The Gross Decontamination Experiment was conducted on various levels and surfaces of the TMI-2 Reactor Building during February and March 1982 and was designed to investigate the effectiveness of various surface decontamination techniques. The polar crane, D-rings, missile shields, refueling canal, fueling bridge, major equipment, floors and some walls were flushed with low pressure water. Water lances were directed manually and applied water at temperatures between ambient and 60"0C at a flow rate of about 95 liters per minute. In addition, floor surfaces on the 305-ft elevation and floor surfaces and major equipment on the 347-ft elevation were sprayed with high pressure water (floors in the Reactor Building are designated by their elevations above sea level). The water pressure in this case varied between 13.8 and 41.4 mPa and water temperature was at a maximum 60"0C. Certain surfaces were also decontaminated using ...
1984-07-15
Microbial treatment of high explosives
Energy Technology Data Exchange (ETDEWEB)
Both DOE and DOD use water and/or steam in the process of removing high explosives, resulting in large quantities of contaminated water, which is then run through activated carbon, which then has to be decontaminated. Research has been underway to utilize microorganisms to degrade RDX and HMX.
1997-07-01
Lodging - Decommissioning Training Course - Decontamination and...
Hour Fitness Center 24 Hour Market 24 Fitness Center Indoor Heated Pool with Whirlpool Seasonal Outdoor Pool Plaza w/ Outdoor Tiki Bar & Café 1,200 Square Foot Total of...
2011-10-08
Ion exchange at TNX using the SKID unit
Energy Technology Data Exchange (ETDEWEB)
An ion exchange unit has been manufactured for WSRC by British Nuclear Fuels, Ltd. This unit consists of three columns, ancillary valving, pumps, lines, and computer controls. It has been delivered to TNX for use in testing a cesium-specific ion exchange resin, developed at WSRC as a potential second generation process for the decontamination of Defense Waste Processing Facility (DWPF) supernate. This resin also has Department of Energy applications at both Oak Ridge and Hanford. Oak Ridge is interested in decontaminating the Melton Valley storage tank supernate, while Hanford is interested in decontaminating the 101-AW and 101-SY supernate streams. Another potential developmental interest is the Savannah River Site (SRS) DWPF recycle stream. The three primary waste streams of interest are the Oak Ridge, Hanford, and SRS, SWPF supernate streams. For these three waste streams, the cesium decontamination ...
1993-10-21
Energy Technology Data Exchange (ETDEWEB)
A program is currently in progress at Argonne National Laboratory to evaluate and develop evaporator technology for concentrating radioactive waste streams. By concentrating radioactive waste streams, disposal costs can be significantly reduced. To effectively reduce the volume of waste, the evaporator must achieve high decontamination factors so that the distillate is sufficiently free of radioactive material. One technology that shows a great deal of potential for this application is being developed by LICON, Inc. In this program, Argonne plans to apply LICON`s evaporator designs to the processing of radioactive solutions. Concepts that need to be incorporated into the design of the evaporator include, criticality safety, remote operation and maintenance, and materials of construction. To design an effective process for concentrating waste streams, both solubility and vapor-liquid equilibrium data are needed. The key issue, however, is the high ...
1993-10-01
Decontamination factors of ceramic filter in radioactive waste incineration system
International Nuclear Information System (INIS)
A suspension-firing type radioactive waste incineration system is developed and cold demonstration testing of ceramic filters for the system are carried out. The incineration system, which is useful for a wide variety of waste materials, can serve to simplify the facilities and to reduce the costs for waste disposal. The incineration system can be used for drying-processing of concentrated waste liquids and disposal of flame resistant materials including ion exchange resins and rubber, as well as for ordinary combustible solid materials. An on-line backwash system is adopted to allow the ceramic filters to operate stably for a long period of time. For one-step filtering using the ceramic filter, the decontamination factor is greater than 10"5 for the processing of various wastes. In a practical situation, there exist vapor produced by the spray drier and the cladding in used ion exchange resin, which act to increase the decontamination ...
International Nuclear Information System (INIS)
When combining aerosol retention components in the dissolver offgas stream of a reprocessing plant, the behavior both of the individual aerosol filter stages and the overall removal efficiency of all filters connected in series vis-a-vis an aerosol spectrum to be expected must be determined for the benefit of the licensing authority. A fast method of determining removal efficiencies is described, which can also be applied in hot operation. This method was used to demonstrate, with high certainty, decontamination factors of a whole filter train in the range of 10"7.
1983-02-01
Dependence of laser assisted cleaning of clad surfaces on the laser fluence
International Nuclear Information System (INIS)
The decontamination factor is studied as a function of laser fluence for three kinds of clad surfaces viz., plain zircaloy, autoclaved zircaloy and SS with cesium as the test contamination. It has been found that the decontamination factor exhibits a maximal behaviour with the laser fluence and its maximum value occurs at different laser fluences in the three cases. The maximal behaviour is attributed to reduced coupling of energy from the laser beam to the substrate due to the initiation of surface-assisted optical breakdown. The results obtained in the experiment carried out in helium environment qualitatively support this explanation (author)
2005-11-01
The integral experiment on beryllium with D-T neutrons for verification of tritium breeding
Energy Technology Data Exchange (ETDEWEB)
A clean benchmark experiment on beryllium was performed with D-T neutrons at the FNS facility of the Japan Atomic Energy Agency. The main objective was to verify the integral data related to the tritium production on lithium isotopes. Tritium production rates, as well as activation reaction rates were measured inside the beryllium assembly that was shaped as a pseudo-cylindrical slab with an area-equivalent diameter of 628 mm and a thickness of 355 mm. Experimental results were analyzed with a three-dimensional Monte Carlo transport code MCNP-4C and FENDL/MC-2.0, JENDL-3.2/3.3 neutron transport libraries. Evaluation of reaction rates was based on the cross section data taken from the JENDL Dosimetry File and ENDF B-VI data libraries. Analysis shows that all calculation combinations (transport and activation cross section libraries) used for evaluation of reaction rates give data that is agreeable with measured values within 10%.
2007-01-15
Energy Technology Data Exchange (ETDEWEB)
This project was supported through ERDA to demonstrate that the temporal distribution of tritium can be documented by the analysis of bound hydrogen in annual tree-ring samples. The project focuses on two sample locations at the Savannah River Site (SRS), a nuclear material production facility located in Aiken, SC. The SRS provided samples of cross-sections from a single tree that were to be pooled together for analysis. Annual tree-rings were identified in each cross-section sample and separated for the period 1954 to 1993. These annual samples were ground and chemically treated to separate the hollocellulose fraction of the wood, then subsequently combusted and the resulting water counting using low-level liquid scintillation counting equipment. Additionally, the ground annual tree-rings were gamma-counted to determine any temporal variation in radionuclide activity and analyzed with x-ray fluorescence to find any temporal variation in trace-element ...
1995-03-21
A thermochemical hydrogen production system based on a high-temperature fusion reactor blanket
International Nuclear Information System (INIS)
A conceptual fusion synfuel production system has been developed with the unique features of: (1) a fusion blanket producing high-temperature (1250"0C) process heat, and (2) the GA sulfur-iodine thermochemical cycle. The system incorporates a two-zone blanket which achieves a tritium breeding ratio of 1.1 while delivering a high fraction (30%) of the fusion heat at high temperatures (1250"0C). The multiple barriers to tritium permeation in the blanket design permit the hydrogen product to meet 10CFR20 regulatory requirements without stringent requirements on the tritium recovery systems. A ceramic heat exchanger, incorporating SiC tubes and headers to contain the process stream and a cooled, Inconel 718 pressure shell to contain the helium, was designed for transferring the heat from the high-temperature coolant to the process. A good heat-line match of the blanket heatsource temperature distribution to the requirements of ...
1983-04-26
W-12 valve pit decontamination demonstration
Energy Technology Data Exchange (ETDEWEB)
Waste tank W-12 is a tank in the ORNL Low-Level Liquid Waste (LLLW) system that collected waste from Building 3525. Because of a leaking flange in the discharge line from W-12 to the evaporator service tank (W-22) and continual inleakage into the tank from an unknown source, W-12 was removed from service to comply with the Federal Facilities Agreement requirement. The initial response was to decontaminate the valve pit between tank W-12 and the evaporator service tank (W-22) to determine if personnel could enter the pit to attempt repair of the leaking flange. Preventing the spread of radioactive contamination from the pit to the environment and to other waste systems was of concern during the decontamination. The drain in the pit goes to the process waste system; therefore, if high-level liquid waste were generated during decontamination activities, it would have to be removed from the pit by means other than the available ...
1995-12-01
The performance tests used the water scrubber for ruthenium rejection
Energy Technology Data Exchange (ETDEWEB)
LEDF (Large Equipment Dismantling Facility) will be constructed for the purpose of decontaminating the high level {alpha} solid waste generated in oarai engineering center of JNC. And, main processing process of LEDF is incineration and melting system. LEDF will be intended to reduce the secondary waste that occurs along with the operation of the off gas processing equipment of incineration and melting system. It assumed that we are able to eliminate the adsorption tower using silica gel, if the decontamination factor to volatile ruthenium is able to expect in the packed scrubber that is established to remove harmful gas. Thereupon, we carried out this tests that eliminates the adsorption tower and reduces the secondary waste. The decontamination factor (DF) to the volatile ruthenium by the water scrubber is confirmed in the established institution which is in Tokai Works. However, decontamination ...
2002-11-01
The performance tests used the water scrubber for ruthenium rejection
International Nuclear Information System (INIS)
LEDF (Large Equipment Dismantling Facility) will be constructed for the purpose of decontaminating the high level #alpha# solid waste generated in oarai engineering center of JNC. And, main processing process of LEDF is incineration and melting system. LEDF will be intended to reduce the secondary waste that occurs along with the operation of the off gas processing equipment of incineration and melting system. It assumed that we are able to eliminate the adsorption tower using silica gel, if the decontamination factor to volatile ruthenium is able to expect in the packed scrubber that is established to remove harmful gas. Thereupon, we carried out this tests that eliminates the adsorption tower and reduces the secondary waste. The decontamination factor (DF) to the volatile ruthenium by the water scrubber is confirmed in the established institution which is in Tokai Works. However, decontamination ...
Salt decontamination demonstration test results
International Nuclear Information System (INIS)
The Salt Decontamination Demonstration confirmed that the precipitation process could be used for large-scale decontamination of radioactive waste sale solution. Although a number of refinements are necessary to safely process the long-term requirement of 5 million gallons of waste salt solution per year, there were no observations to suggest that any fundamentals of the process require re-evaluation. Major accomplishments were: (1) 518,000 gallons of decontaminated filtrate were produced from 427,000 gallons of waste salt solution from tank 24H. The demonstration goal was to produce a minimum of 200,000 gallons of decontaminated salt solution; (2) cesium activity in the filtrate was reduced by a factor of 43,000 below the cesium activity in the tank 24 solution. This decontamination factor (DF) exceeded the demonstration goal of a DF greater than 10,000; (3) average strontium-90 ...
Summarization of radioactive effluent monitoring in Daya Bay Nuclear Power Station 1994-2002
International Nuclear Information System (INIS)
This paper introduces the radioactive effluent monitoring systems, measurement and quality control methods used in Daya Bay Nuclear Power Station from its commercial operation in 1994. The main work and experiences for the management of effluent release are discussed and analyzed. The radwaste data appear declining trend and are far blow the annual limit approved by the national Environmental Protection Bureau since 1995. The normalized release (unit GBq/GWa) of 9 years is as follows: liquid nuclides (except tritium) 11.1, liquid tritium 1.91 x 10"4, noble gas 2.03 x 10"4, halogen 0.13, aerosol 7.57 x 10"-"3. For "1"1"0"mAg, the average release from 1998 to 2002 has been reduced to 1/7 of the quantity in 1997
2004-05-01
Origin of water salinity in the coastal Sarafand aquifer (South-Lebanon)
International Nuclear Information System (INIS)
Author.The geochemical and isotopic study, based on the analysis of twenty water samples from well in the coastal plain of Sarafand (South-Lebanon), permit to eliminate the hypothesis of marine intrusion in this aquifer. The increase of salinity observed in certain wells is due to the contamination of cretaceous aquifer water by the quaternary formations. The two poles of mixing are respectively characterized: by weak tritium contents (between 2 and 3 UT) and a value of stable isotopes (-5,9<0,18<-5,5) corresponding to the appearance of cretaceous formation area; by the high tritium contents and enrichment relative to heavy isotope in the mineralized water of superficial formations. On the other hand, the isotope contents permit the set a rapid renewal of the cretaceous aquifer water due to quick circulation in the Karstic system
Observation of the microstructural changes in lithium titanate by multi-ion irradiation
Energy Technology Data Exchange (ETDEWEB)
The irradiation behavior of Li{sub 2}TiO{sub 3} under a fusion reactor environment was simulated by simultaneous irradiation of Li{sub 2}TiO{sub 3} by the triple ion beams and the respective single ion beams of O{sup 2+}, He{sup +} and H{sup +}. The microstructural changes in Li{sub 2}TiO{sub 3} caused by the irradiation were measured by Raman spectroscopy and FT-IR photoacoustic spectroscopy. The results suggest that the formation of TiO{sub 2} due to displacements by irradiation occurs, and the irradiation defects generated by irradiation trap hydrogen and increase the amount of hydroxyl near the surface. Such phenomena are believed to significantly affect the chemical form of the released tritium and the tritium inventory in the breeding materials of a fusion reactor.
2004-08-01
Observation of the microstructural changes in lithium titanate by multi-ion irradiation
International Nuclear Information System (INIS)
The irradiation behavior of Li_2TiO_3 under a fusion reactor environment was simulated by simultaneous irradiation of Li_2TiO_3 by the triple ion beams and the respective single ion beams of O"2"+, He"+ and H"+. The microstructural changes in Li_2TiO_3 caused by the irradiation were measured by Raman spectroscopy and FT-IR photoacoustic spectroscopy. The results suggest that the formation of TiO_2 due to displacements by irradiation occurs, and the irradiation defects generated by irradiation trap hydrogen and increase the amount of hydroxyl near the surface. Such phenomena are believed to significantly affect the chemical form of the released tritium and the tritium inventory in the breeding materials of a fusion reactor.
2004-08-01
Lichens as indicators of tritium and radiocarbon contamination
Energy Technology Data Exchange (ETDEWEB)
Lichens were collected in France in the surroundings of a military nuclear facility in Burgundy, near the la Hague reprocessing plant and in an area away from any direct source of contamination. Organically bound tritium (OBT) has been analysed on 18 samples and radiocarbon on 11. It appeared that on the most contaminated spots, the OBT activity in lichens was higher than the background by a factor of 1000 and was still a factor 10-100 at a distance of 20 km from the source. Radiocarbon from la Hague could be traced by lichens. The slow metabolism of lichens makes them suitable for the follow-up of {sup 3}H and {sup 14}C, which have been incorporated by photosynthesis.
2004-05-05
Development of barcode system for internal dose monitoring
International Nuclear Information System (INIS)
In Tarapur Atomic Power Station unit-3 and 4, which is 540 MWe pressurized heavy water reactor, tritium is produced in primary heat transport system and moderator system. Tritium is a major contributor to the internal dose. Internal dose contributes about 30% of the collective dose. Internal dose monitoring and its control are important to control the collective dose. Estimation of internal dose is done by analysis of bioassay samples of radiation workers. In a month, about 7000 bioassay samples are analysed for the internal dose assessment during normal operation, and about 12000 during the biennial shut down of the reactor. To enhance the sample preparation and counting performance, minimize the entry errors and reduce the processing time, barcode based label generation system was developed for the internal dose monitoring. This paper discusses about the use of barcode system in the internal dose monitoring at TAPS 3 and 4. (author)
2008-11-19
Review of tritium metabolism based on urine bioassay results
Energy Technology Data Exchange (ETDEWEB)
The effective half-life based on urine bioassay results of Wolsung NPP's worker was calculated. The effective half-life for tritiated water vapour obtained was 5 {approx} 9 days. In comparison to 10 days reported for ICRP-30, it is lower than the corresponding half-life for Reference Man. Also, the half-life was calculated based on intake amount of daily water. According to this result, the metabolism was reviewed.
2001-05-01
... Targeted fields of research Continuation of ongoing research - Finalising detailed design work on the ITER project; getting JET operational at full power; Improvement of the basic concepts of fusion devices - Fusion plasmas; theoretical studies; technology watch on research into inertial confinement; new experimental concepts and systems; etc.; Long-term technology - Preparations for building a demonstration reactor (development of tritium breeding blankets; prospective ...
Nuclear power plants and the ''dying forests''
International Nuclear Information System (INIS)
Possible causes of forest damage are discussed. Mapping of affected areas by various workers resulted in dissimilar pictures. Release of radioactive rare gases, aerosols, tritium and carbon-14 seems unlikely to have a significant influence on forest damage. Influence of radioactive fallout, ozone formation by high-voltage transmission lines and synergistic effects is also found to be negligible.
1985-01-01
Neutron irradiation effects on plasma facing materials
Energy Technology Data Exchange (ETDEWEB)
This paper reviews the effects of neutron irradiation on thermal and mechanical properties and bulk tritium retention of armour materials (beryllium, tungsten and carbon). For each material, the main properties affected by neutron irradiation are described and the specific tests of neutron irradiated armour materials under thermal shock and disruption conditions are summarized. Based on current knowledge, the expected thermal and structural performance of neutron irradiated armour materials in the ITER plasma facing components are analysed.
2000-12-01
... This is true because a shorter residence time means that ground water moves 'faster.' Thus, contamination will get to the drinking well from the recharge area (point of entry) faster if the ground water is younger. However, it has been difficult to measure the exact age of young ground water. The conventional indicator has been tritium, a radioactive form of hydrogen, but its ...
Lithium question for nuclear fusion
International Nuclear Information System (INIS)
An attempt is made to estimate the lithium reserve (the economically recoverable lithium) for the tritium breeding in D-T fusion reactors and other uses. Similar development patterns for fusion energy and fission energy are assumed to estimate the future lithium requirements. These requirements are grouped into three categories; the commercial uses, the lithium batteries for electric cars, and the fusion reactor uses. 5 refs.
UK PubMed Central (United Kingdom)
The alkylation products formed by in vitro treatment of DNA with tritium-labeled 1,3-bis(2-chloroethyl)-1-nitrosourea (3H-BCNU) were identified and quantified. Twelve adducts were resolved...Full Text Available
2007-01-01
International Nuclear Information System (INIS)
Hydrology and hydrogeochemical are auxiliary techniques to valid conceptual hydrogeology an recharge models. Stable isotopes from water trace sources and path flow and Tritium indicates age. This paper is about the use of D 18, D2H y 3H to study the aquifer system on Bajo Cauca antioqueno.
Energy Technology Data Exchange (ETDEWEB)
It is planned to use the tritium dose model, DCART (Doses from Chronic Atmospheric Releases of Tritium), to reconstruct dose to the hypothetical maximally exposed individual from annual routine releases of tritiated water (HTO) and tritiated hydrogen gas (HT) from all Lawrence Livermore National Laboratory (LLNL) facilities and from the Sandia National (SNL) Laboratory's Tritium Research Laboratory over the last fifty years. DCART has been described in Part 1 of ''Historical Doses From Tritiated Water And Tritiated Hydrogen Gas Released To The Atmosphere from Lawrence Livermore National Laboratory (LLNL)'' (UCRL-TR-205083). This report (Part 2) summarizes information about annual routine releases of tritium from LLNL (and SNL) since 1953. Historical records were used to derive facility-specific annual data (e.g., source terms, dilution factors, ambient air ...
2005-03-07
Development on the technologies for tritium removal processes
Energy Technology Data Exchange (ETDEWEB)
While tritium exposure to the site-workers in Wolsung NPP is upto about 40 % of the total personnel exposure, Korea Institute of Nuclear Safety has asked tritium removal facility, as one of the requirements for post reactor construction, after operation of four CANDU reactors in Wolsung site. For the purpose of essential removal of tritium from the heavy water system of the heavy water reactors, an experiment of Ar-N{sub 2} cryogenic distillation tower was carried out as a preliminary study for development of liquid-phase catalytic exchange - cryogenic hydrogen distillation process. The steady-state reached after 50 minutes under 90 K in the Ar-N{sub 2} distillation column (inner diameter 20 mm, height 500 mm) packed with Dixon ring ({phi} 3 mm x H 3 mm), and the ratios of Ar-concentration at the top and at the bottom measured by gas chromatography within {+-}1 % relative error was approximately 93 : 3. This value was ...
1994-12-01
International Nuclear Information System (INIS)
In a cold fusion method by electrolysis, a hydrogen occluding material mainly comprising vanadium is used as a material for a negative electrode, and lithium isotopes are incorporated in the material by more than 93%. That is, the ratio of lithium 7 ("7Li) isotope is increased to higher than the natural existent ratio, so that tritium ("3H) concentration in the hydrogen occluding material can be increased, to attain energy at high efficiency. (T.M.).
1993-03-02
Accelerator production of tritium pollution prevention design assessment
Energy Technology Data Exchange (ETDEWEB)
This Pollution Prevention Design Assessment (PPDA) provides data for cost-benefit analysis of the potential environmental impact of the APT, is an integral part of pollution prevention/waste minimization, and is required by DOE for any activity generating radioactive, hazardous, and mixed wastes. It will also better position the APT to meet future requirements, since it is anticipated that regulatory and other requirements will continue to become more restrictive and demanding.
1997-09-18
Energy Technology Data Exchange (ETDEWEB)
This paper details the development of a decontamination approach for the West Valley Demonstration Project (WVDP), Decontamination Project Plan (Plan). The WVDP is operated by West Valley Nuclear Services Company (WVNSCO), a subsidiary of Westinghouse Government and Environmental Services, and its parent companies Washington Group International and British Nuclear Fuels Limited (BNFL). The WVDP is a waste management effort being conducted by the United States Department of Energy (DOE) at the site of the only commercial nuclear fuel reprocessing facility to have operated in the United States. This facility is part of the Western New York Nuclear Service Center (WNYNSC), which is owned by the New York State Energy Research and Development Authority (NYSERDA). As authorized by Congress in 1980 through the West Valley Demonstration Project Act (WVDP Act, Public Law 96-368), the DOE's primary mission at the WVDP is to solidify high-level ...
2002-02-25
Removal of iodine species by concentrated nitric acid, (2)
International Nuclear Information System (INIS)
One of the most effective removing processes of iodine species is what is called ''Iodox Process'', which contains oxidation and absorption of iodine species by highly concentrated nitric acid. The result of fundamental test with bubble column in this process had been reported. Present paper describes the fundamental experiment by the use of packed column. This experiment has been carried out to clear the effect of feed gas flow rate, nitric acid flow rate, nitric acid concentration, and methyl iodide concentration on removal efficiency of methyl iodide. The following results were obtained. The decontamination factor of methyl iodide (DF) increases exponentially with nitric acid concentration, which agrees with the result obtained by using the bubble column. The factor is in inverse proportion to feed gas flow rate, and is also almost independent of nitric acid flow rate and methyl iodide concentration. The relation between the decontamination ...
1978-07-01
Process development for remote-handled mixed-waste treatment
Energy Technology Data Exchange (ETDEWEB)
The Oak Ridge National Laboratory (ORNL) is developing a treatment process for remote-handled (RH) liquid transuranic mixed waste governed by the concept of minimizing the volume of waste requiring disposal. This task is to be accomplished by decontaminating the bulk components so the process effluent can be disposed with less risk and expense. Practical processes have been demonstrated on the laboratory scale for removing cesium 137 and strontium 90 isotopes from the waste, generating a concentrated waste volume, and rendering the bulk of the waste nearly radiation free for downstream processing. The process is projected to give decontamination factors of 10{sup 4} for cesium and 10{sup 3} for strontium. Because of the extent of decontamination, downstream processing will be contact handled. The transuranic, radioactive fraction of the mixed waste stream will be solidified using a thin-film evaporator and/or microwave ...
1990-01-01
Pretreatment with U(IV) solution for improving the decontamination of ruthenium
International Nuclear Information System (INIS)
The ruthenium decontamination factor in Purex process falls quickly in successive TBP cycles. So, it is necessary to change the chemical states of RuNO complexes in order to improve DF_R_u in the uranium purification cycle. Hydrazine nitrate is being used to transform RuNO complexes into in-extractable Ru(III)and Ru(IV). However, hydrazine nitrate may be inverted into hydrazoic acid which is dangerous and can bring an unstable factor. Pretreatment using U(IV) solution provides another method to improve the decontamination of ruthenium in Purex process. 0.02 mol/lU(IV) solution can transform RuNO complexes into inextricable species by heating in water bath. The D_R_u can be decreased by a factor of 10-20. U(IV) pretreatment does not bring any harmful chemical in process. The acidity has a very large influence on the effect of pretreatment. The higher the acidity is, the worse the effect will be.
Improving the decontamination of ruthenium with short chain hydroxamic ACTD as complexing agent
International Nuclear Information System (INIS)
The ruthenium decontamination factor in Purex process falls quickly with recycles of TBP. So it is necessary to change the chemical states of RuNO complexes in order to improve DF_R_u in the uranium purification cycle. The retention of RuNO complexes in TBP-kerosenelaurohydroxamic acid is observed to be quite large in our previous work. Therefore, water-soluble short chain hydroxamic acid is used as complexing agent to decrease the distribution coefficient of Ru. Hydroxamic acid can transform RuNO complexes into in-extractable species by TBP-kerosene in certain conditions. The result of cascade experiment indicates that the ruthenium decontamination can be increased by a factor of 40-50. Acidity has more influence on the effect of pretreatment. The higher acidity is, the worse the effect will be. The pretreatment is first carried out in low acidic solution, then extractive acidity is increased. In this way, the distribution of Ru can be ...
International Nuclear Information System (INIS)
Decommissioning of radiological and nuclear installations is for this century the new challenge. One of the performance criteria is the reduction of total quantities of radioactive materials (liquid or solid) arising from dismantling and decontamination of radiological and nuclear installations. In this work we present a new application of the water soluble polymers used as: - flocculation agents in treatment and conditioning process within the management of radioactive liquid materials; - strippable coatings on solid materials based on the water soluble polymers. The parameters of water soluble polymers made in our Institute by radiation processing have been analysed, namely the molecular average weight, composition, and efficiency of utilization of these polymeric materials as well as the content of ash, additives, decontamination factor, consumption per surfaces/liter, corrosion aspects, compatibility with various surfaces (of metal, ...
2003-10-20
Decontamination performance in off-gas cleaning system of radioactive solid waste incineration unit
International Nuclear Information System (INIS)
At the Tokai Research Establishment of Japan Atomic Energy Research Institute, the radioactive solid waste incineration unit with a capacity of 100 kg/h was installed in 1979, since then the unit has been routinly operated. An off-gas cleaning system of the unit consists mainly of a primary and secondary ceramic filters, a heat resistant HEPA filter and a scrubber. A series of hot test was carried out to examine the docontamination performance for radionuclides in the off-gas cleaning system. In the test, simulated wastes contaminated with a known quantity of radionuclides were burned in the unit, and radioactive concentrations in the off-gas were measured. And then, the following data were obtained: a retention factor of radionuclides in a furnace and a decontamination factor for radionuclides in each of off-gas cleaning components. And also overall decontamination factors, defined as the ratio of radioactivities input to the furnace to ...
Basic design of alpha aqueous waste treatment process in NUCEF
Energy Technology Data Exchange (ETDEWEB)
This paper described the basic design of Alpha Aqueous Waste Treatment Process in NUCEF. Since various experiments using the TRU (transuranium) elements are carried out in NUCEF, wastes containing TRU elements arise. The liquid wastes in NUCEF are categorized into three types. Decontamination and volume reduction of the liquid waste mainly of recovery water from acid recovery process which has lowest radioactive concentration is the most important task, because the arising rate of the waste is large. The major function of the Alpha Aqueous Waste Treatment Process is to decontaminate the radioactive concentration below the level which is allowed to discharge into sea. Prior the process design of this facility, the followings are evaluated:property and arising rate of the liquid waste, room space to install and licensing condition. Considering varieties of liquid wastes and their large volume, the very high decontamination ...
1996-11-01
Estimation tests for effecting factor on decontamination property in crystallization process
International Nuclear Information System (INIS)
Crystallization procedure is considered to have adaptability to new reprocessing process based on the PUREX process because it has an advantage in recovering rather pure uranium from contaminated uranium solution without reagent. NEXT (New Extraction System for TRU Recovery) process has been developed by JNC, and applying the crystallization process unit to NEXT process has a capability to contribute to an improvement of economical efficiency and reduction of liquid waste in NEXT process. Thus following studies were carried out. In crystallization process unit, UNH (Uranyl Nitrate Hydrate)-crystals are washed by a nitric acid solution to get high decontamination factor, but the data on UNH-crystals dissolution by washing procedure is insufficient to evaluate the effectiveness of crystallization process unit. So, in this study, the effect of a nitric acid concentration to UNH-crystals dissolution and decontamination factor was tested. As ...
International Nuclear Information System (INIS)
Simple hydroxamic acids are shown to be useful reagents for the separation of Np and Pu from U within simplified, single cycle Purex flowsheets. They are compatible with the use of centrifugal contactors and laboratory scale flowsheet trials with aceto-hydroxamic acid have demonstrated high actinide recoveries and decontamination factors on products for active feeds of up to 40 wt.% Pu. They therefore show many ideal characteristics for Pu and Np recovery within flowsheet options for actinide recovery in advanced fuel cycles. Furthermore, in order to optimise the routing of Np with the Pu product in advanced flowsheets, additional studies of Np extraction in the primary co-decontamination contactor, prior to U/Pu partition, have been undertaken, combining experiment, modelling and flowsheet tests. (author)
2005-10-09
TREATMENT OF RADIOACTIVE EFFLUENTS AT THE MOL LABORATORIES
The cold effluents (sanitary waste and decontaminated radioactive water) are flocculated with sodium phosphate and pumped through a trickling filter. The average decontamination obtained is about 86% for alpha emittera and 76% for beta emitters. The cool effluents (activity < 10/sup -3/ mu c/ml) can be treated by several methods. Provisions have been made for two successive chemical flocculations eventually followed by an adsorptlon. The warm waste treatment (activity between 10/sup -3/ and 1 mu c/ml) is still in the experimental stage. The following methods are used: evaporation for some chemically contaminated wastes, browncoal filtration for reactor effluents, and a combination of chemical treatment and browncoal adsorption in other cases. (auth)
1959-10-31
International Nuclear Information System (INIS)
Studies on the separation of Ag(I) during the recovery of Pu from analytical waste generated during potentiometric determination of Pu using AgO as oxidant, by precipitation of Pu as ammonium plutonium (III) oxalate have shown that most of the Ag(I) is separated during the reduction of Pu to Pu(III) state by ascorbic acid. A decontamination factor of 54 was obtained. Additional a decontamination factor of 5.8 was obtained during the precipitation of Pu as ammonium plutonium (III) oxalate. The Ag content was determined by gamma spectrometry, using "1"1"1Ag as a tracer (T_1_/_2 7.45 d, #gamma# 342.1 keV) and HPGe as detector. The studies indicate that Ag is preferentially separated almost quantitatively during the recovery of plutonium, when acidity adjustment is done with NaOH instead of NH_3. (author)
2007-02-14
Energy Technology Data Exchange (ETDEWEB)
The impacted armor targets used in testing high density armor-piercing ammunition containing depleted uranium (DU) are subject to disposal as low-level radioactive waste. Because of the costs associated with disposal of the entire armor plate and the limited use of secured commercial sites in the future, the U.S. Army is seeking to identify and evaluate new technologies for decontaminating these armor plates. The objectives of this Phase I SBIR program are two-fold, namely: to develop a selective solvent that can decontaminate impacted armor targets containing DU for disposal or recycle, and to identify and characterize technologies that can remove depleted uranium from the solvent for solvent recycle and uranium recovery for easier hazardous-waste disposal.
1987-05-05
Requirement of decontamination factor for near-surface disposal of PEACER wastes
International Nuclear Information System (INIS)
A pyrochemical process has been introduced and utilized so that the transmutation of spent PWR fuel in PEACER can produce mainly low and intermediate level waste for near surface disposal. Major radioactive nuclides from PEACER pyroprocessing are composed of TRU and LLFP. In this study, the requirement for the final waste from PEACER is evaluated based on the methodology for establishment of waste acceptance criteria. Also, sensitivity analysis for several input parameters is conducted in order to determine acceptable decontamination factor (DF) and LLFP removal efficiency and to find out input parameter that extremely have an effect on DF. As a result of the study, TRU DF and LLFP removal efficiency have to be achieved more than 1.0E+04 - 1.0E+05 and 96%, respectively. (author)
2005-10-09
Energy Technology Data Exchange (ETDEWEB)
SZI global distribution due to biogeochemical cycle in environment reservoirs has been studied. It is shown that during the operation of nuclear fuel cycle facilities and at a modern level of the decontamination factor the SZI concentration in some natural media (soil, the Earth biosphere, ocean mixing layer) will increase by 4-5 orders. Recommended gradual increase of the decontamnation factor in time for conserving the SZI concentration level not exceeding one order in comparison with modern one is given. At that to the end of the century the decontamination factor must be of an order of 1 x 10U in the case of SZI intake to the ocean mixing layer and of 1 x 10V in the case of its intake to the atmosphere.
1985-03-01
International Nuclear Information System (INIS)
"1"2"9I global distribution due to biogeochemical cycle in environment reservoirs has been studied. It is shown that during the operation of nuclear fuel cycle facilities and at a modern level of the decontamination factor the "1"2"9I concentration in some natural media (soil, the Earth biosphere, ocean mixing layer) will increase by 4-5 orders. Recommended gradual increase of the decontamnation factor in time for conserving the "1"2"9I concentration level not exceeding one order in comparison with modern one is given. At that to the end fof the centary the decontamination factor must be of an order of 1x10"4 in the case of "1"2"9I intake to the ocean mixing layer and of 1x10"5 in the case of its intake to the atmosphere.
Range of decontamination factor for near-surface disposal of PEACER wastes
Energy Technology Data Exchange (ETDEWEB)
One of the alternative ideas to solve the spent fuel issues, the partitioning and transmutation (P and T) technology has been developed for decades. Moreover, the concept of LILW production from P and T are proposed by Bowman. A PEACER (Proliferationresistant, Environmental-friendly Accident-tolerant, Continuable and Economical Reactor), based on pyrochemical process and Pb-Bi coolant transmutation reactor, has been conceptually designed to be able to convert all PWR spent fuel into low and intermediate level waste for near-surface disposal. In this study, the acceptance criteria for near-surface disposal facility is derived by the methodology for establishment of acceptance criteria. Then acceptable TRU decontamination factor (DF) and LLFP removal efficiency in order to meet acceptance criteria is evaluated.
2005-07-01
Range of decontamination factor for near-surface disposal of PEACER wastes
International Nuclear Information System (INIS)
One of the alternative ideas to solve the spent fuel issues, the partitioning and transmutation (P and T) technology has been developed for decades. Moreover, the concept of LILW production from P and T are proposed by Bowman. A PEACER (Proliferationresistant, Environmental-friendly Accident-tolerant, Continuable and Economical Reactor), based on pyrochemical process and Pb-Bi coolant transmutation reactor, has been conceptually designed to be able to convert all PWR spent fuel into low and intermediate level waste for near-surface disposal. In this study, the acceptance criteria for near-surface disposal facility is derived by the methodology for establishment of acceptance criteria. Then acceptable TRU decontamination factor (DF) and LLFP removal efficiency in order to meet acceptance criteria is evaluated
2005-05-26
British Library Electronic Table of Contents (United Kingdom)
This study was focused on the possibility to inactivate main food pathogens, their spores and biofilms on the surface of packaging material polyolefine by Na-chlorophyllin (Na-Chl)-based photosensitization and to compare efficiency of this treatment with conventional antimicrobials. Data indicate that Bacillus cereus and Listeria monocytogenes were effectively inactivated (7 log) by Na-Chl (7.5x10-7M)-based photosensitization in vitro and on the surface of packaging. Meanwhile to achieve adequate inactivation of thermo-resistant strains, spores or biofilms the higher Na-Chl concentration and longer illumination times had to be used. Comparison of different surface decontamination treatments reveal that photosensitization is much more effective against B. cereus and L. monocytogenes attache...
2011-01-01
Investigation of the removal efficiency of gasborne particles in a scrubber column
Energy Technology Data Exchange (ETDEWEB)
Tests on the scrubbing column have led to the following results: Use of a scrubbing column with Raschig rings is only meaningful for the sedimentation of particles exceeding diameters of 0.5 ..mu..m; drops of diameter size 1.5 ..mu..m are formed in the column; more efficient drop precipitators in the column air flow ease the load on subsequent suspended material filters thereby contributing to a longer life of these filters even at higher sodium ion concentrations in the washing water; with distillate of an 8% rather than 0.8% salt solution a decontamination factor greater than 10 can be calculated since larger particles precipitate more readily. This only applies, however, under the condition that the washing water is renewed regularly, if necessary daily where higher aerosol concentrations are present. If not, the decontamination factor will be reduced through the salt-containing secondary aerosols from the washing water.
1983-01-01
Investigation of the removal efficiency of gasborne particles in a scrubber column
International Nuclear Information System (INIS)
Tests on the scrubbing column have led to the following results: Use of a scrubbing column with Raschig rings is only meaningful for the sedimentation of particles exceeding diameters of 0.5 #mu#m; drops of diameter size 1.5 #mu#m are formed in the column; more efficient drop precipitators in the column air flow ease the load on subsequent suspended material filters thereby contributing to a longer life of these filters even at higher sodium ion concentrations in the washing water; with distillate of an 8% rather than 0.8% salt solution a decontamination factor greater than 10 can be calculated since larger particles precipitate more readily. This only applies, however, under the condition that the washing water is renewed regularly, if necessary daily where higher aerosol concentrations are present. If not, the decontamination factor will be reduced through the salt-containing secondary aerosols from the washing water. (orig.).
Decontamination factor of an incinerator for radioactive solid wastes
International Nuclear Information System (INIS)
An incinerator for the treatment of low-level radioactive solid wastes was installed in Tokai Research Establishment, JAERI, 1966. The incinerator was equipped with a scrubber, cyclone, electrostatic precipitator and HEPA filter. The retention factor (R.F.) of the furnace as well as the decontamination factors (D.F.) of each dust collector were measured using "3"2P as a tracer under various conditions. It was found that the overall D.F. of the incinerator was improved by the increase of the temperature in the furnace, decrease of the off gas flowrate, increase of the charged voltage of the electrostatic precipitator and by the increase of the liquid gas ratio of the scrubber. The overall D.F. of the incinerator (including the R.F. in the furnace) on the standard operating conditions was 9.1x10"6. (auth.).
Cleansing methodology of sites and its applications
International Nuclear Information System (INIS)
The Commissariat a l'Energie Atomique (CEA, French Atomic Energy Commission) has set up over the last 10 years an innovative methodology aiming at characterizing radiological contaminations. The application of the latter relies on various tools such as expertise vehicles with impressive detection performances (VEgAS) and recently developed software platform called Kartotrak. A Geographic Information System tailored to radiological needs constitutes the heart of the platform; it is surrounded by several modules aiming at sampling optimization (Stratege), data analysis and geostatistical modeling (Krigeo), real-time monitoring (Kartotrak- RT) and validation of cleaning efficiency (Pescar). This paper presents the different tools which provide exhaustive instruments for the follow-up of decontamination projects, from doubt removal to the verification of the decontamination process. (authors)
2009-10-12
CTH-process for HLLW treatment. Pt. 1
Energy Technology Data Exchange (ETDEWEB)
A process for separation of actinides and technetium from reprocessing high level liquid waste has been developed, the CTH-process. The main parts are three consecutive solvent extraction cycles followed by an optional step for sorption on inorganic ion exchangers. The first extraction cycle removes and recovers uranium, neptunium, and plutonium by extraction with HDEHP. The second extraction cycle separates technetium and nitric acid from the waste using TBP. In the third extraction cycle Am and Cm are separated from the waste using HDEHP. The actinide free waste is then passed through inorganic ion exchangers to remove most of remaining radionuclides. The process has been tested on an authenic HLLW solution. A decontamination factor > 10/sup 5/ for alpha emitters was measured for the solvent extraction process and the sorption on inorganic ion exchangers gave a decontamination factor > 3x10/sup 4/ for beta emitters.
1984-01-01
Apparatus for measuring the decontamination factor of a multiple filter air-cleaning system
Energy Technology Data Exchange (ETDEWEB)
An apparatus is described for measuring the overall decontamination factor of first and second filters, the first and second filters being located in a plenum having an upstream chamber, an intermediate chamber, and a downstream chamber. The first filter is located between the upstream and intermediate chambers and the second filter is located between the intermediate and downstream chambers. The apparatus comprises a. an aerosol generator for producing a challenge aerosol composed of individual particles, the aerosol generator being in fluid communication with the upstream chamber; b. an upstream collector for collecting the challenge aerosol before the challenge aerosol enters the first filter, the upstream collector being disposed in the upstream chamber; c. an intermediate collector for collecting the challenge aerosol that passes through the first filter, the intermediate collector being disposed in the intermediate chamber; and d. a downstream collector for ...
1986-10-28
Apparatus for measuring the decontamination factor of a multiple filter air-cleaning system
Energy Technology Data Exchange (ETDEWEB)
An apparatus for measuring the overall decontamination factors of first and second filters located in a plenum. The first filter separates the plenum's upstream and intermediate chambers. The second filter separates the plenum's intermediate and downstream chambers. The apparatus comprises an aerosol generator that generates a challenge aerosol. An upstream collector collects unfiltered aerosol which is piped to first and second dilution stages and then to a laser aerosol spectrometer. An intermediate collector collects challenge aerosol that penetrates the first filter. The filtered aerosol is piped to the first dilution stage, diluted, and then piped to the laser aerosol spectrometer which detects single particles. A downstream collector collects challenge aerosol that penetrates both filters. The twice-filtered aerosol is piped to the aerosol spectrometer. A pump and several valves control the movement of aerosol within the apparatus.
1985-07-03
International Nuclear Information System (INIS)
Two inactive tracer techniques for determination of the decontamination factor (DF) of evaporation plants for radioactive waste water are described. One method was used for determination of the DF of an one stage pilot plant. The elements Mg, Cd and Co were employed as tracers. The analyses were performed by atomic absorption spectroscopy. The measurements being fast and simple are especially advantageous with test series in pilot plants. In the second method activation analysis was used for measurement of the tracer to determine the DF of a two stage evaporation plant. Europium is added to the stock solution in a concentration of 70 ppm only. With this method a DF of up to 3 . 10"8 can still be determined. (Auth.).
Energy Technology Data Exchange (ETDEWEB)
An approach to the ductile fracture of ultra high strength steels has been evaluated. According to this approach the critical crack tip opening, delta/sub IC/, will scale with X/sub 0/(R/sub V//R/sub I/vertical bar/sub R//sub 0/. X/sub 0/ is an average inclusion spacing and (R/sub V/R/sub I/)vertical bar/sub R//sub 0/ is the void radius divided by the radius of the inclusion nucleating the void evaluated at the average inclusion size. AF1410 was selected to test this approach because it has exceptionally high fracture toughness on aging at 510/sup 0/C and because its toughness varies markedly with aging temperature. The results from this and earlier work showed a linear relationship exists between delta/sub IC/ and X/sub 0/(R/sub V//R/sub I/)vertical bar /sub R//sub 0/ for values of delta/sub IC/ ranging from about 8 ..mu..m to 60 ..mu..m. The values of (R/sub V//R/sub I/)vertical bar /sub R//sub 0/ for AF1410 aged at 425/sup 0/C and 510/sup ...
1987-07-01
Surface Roughness of Stainless Steel Bender Mirrors for FocusingSoft X-rays
Energy Technology Data Exchange (ETDEWEB)
We have used polished stainless steel as a mirror substrate to provide focusing of soft x-rays in grazing incidence reflection. The substrate is bent to an elliptical shape with large curvature and high stresses in the substrate require a strong elastic material. Conventional material choices of silicon or of glass will not withstand the stress required. The use of steel allows the substrates to be polished and installed flat, using screws in tapped holes. The ultra-high-vacuum bender mechanism is motorized and computer controlled. These mirrors are used to deliver focused beams of soft x-rays onto the surface of a sample for experiments at the Advanced Light Source (ALS). They provide an illumination field that can be as small as the mirror demagnification allows, for localized study, and can be enlarged, under computer control,for survey measurements over areas of the surface up to several millimeters. The critical issue of the quality of the steel surface, ...
2005-10-11
Spin-resolved magnetic studies of focused ion beam etched nano-sized magnetic structures
International Nuclear Information System (INIS)
Scanning ion microscopy with polarization analysis (SIMPA) is used to study the spin-resolved surface magnetic structure of nano-sized magnetic systems. SIMPA is utilized for in situ topographic and spin-resolved magnetic domain imaging as well as for focused ion beam (FIB) etching of desired structures in magnetic or non-magnetic systems. Ultra-thin Co films are deposited on surfaces of Si(1 0 0) substrates, and ultra-thin, tri-layered, bct Fe(1 0 0)/Mn/bct Fe(1 0 0) wedged magnetic structures are deposited on fcc Pd(1 0 0) substrates. SIMPA experiments clearly show that ion-induced electrons emitted from magnetic surfaces exhibit non-zero electron spin polarization (ESP), whereas electrons emitted from non-magnetic surfaces such as Si and Pd exhibit zero ESP, which can be used to calibrate sputtering rates in situ. We report on new, spin-resolved magnetic microstructures, such as magnetic 'C' states and magnetic vortices, found at surfaces of FIB patterned magnetic elements. It is ...
2005-04-01
SERAPHIM: A propulsion technology for fast trains
Energy Technology Data Exchange (ETDEWEB)
The Segmented Rail Phased Induction Motor (SERAPHIM) is a compact, pulsed linear induction motor (LIM) offering a unique capability for very high speed train propulsion. It uses technology developed for the Sandia coilgun, an electromagnetic launcher designed to accelerate projectiles to several kilometers per second. Both aluminum cylinders and plates were accelerated to a kilometer per second (Mach 3) by passing through a sequence of coils which were energized at the appropriate time. Although this technology was developed for ultra-high velocity, it can be readily adapted to train propulsion for which, at sea level, the power required to overcome air resistance limits the operational speed to a more modest 300 mph. Here, the geometry is reversed. The coils are on the vehicle and the ``projectiles`` are fixed along the roadbed. SERAPHIM operates not by embedding flux in a conductor, but by excluding it. In this propulsion scheme, pairs of closely spaced coils on ...
1995-06-01
Materials research and beam line operation utilizing NSLS. Progress report
Energy Technology Data Exchange (ETDEWEB)
MATRIX, a participating research team of Midwest x-ray scattering specialists, continues to operate beam line X-18A at NSLS. Operations of this line now provides state-of-the-art capabilities to a wide range of people in the Materials Science and Engineering research community. Improvements of the beam line continue to be a focus of MATRIX. Throughout this past year the emphasis has been shifting towards improvement in ``user friendly`` aspects. Simplified control operations and a shift to single-user personal computer has been a major part of the effort. Over the past year the full 242 operational days were utilized. Beam line test and evaluation consumed 21 days with eight MATRIX groups combining to use 170 days. General user demand for use of the beam line continues to be strong and three groups were provided 51 operating days. Research production has been growing as NSLS and the beam line become a more stable type of operation. For 1990 the MATRIX group published nine articles. To ...
1991-10-01
Energy efficient soil disinfestation by microwaves
Energy Technology Data Exchange (ETDEWEB)
A major obstacle prohibiting the use of microwaves for soil disinfection and disinfestation is the large amount of energy required to obtain sufficient results. The present work presents an experimental study of the effect of initial soil temperature and soil moisture on energy consumption by application of microwaves for soil disinfection. All experiments were carried out by using a microwave generator of a nominal power output of 900 W. The ultra-high-frequency field (2450{+-}2 MHZ) was produced by a magnetron tube and channelled through a metal waveguide. The output opening of the waveguide was placed directly on the soil surface. It was found that a soil with 15% moisture content (w.b.) and an initial temperature of 20degC requires energy to be heated at a depth of 10 cm up to 61degC which is 3.2 times more than the energy required to heat the soil up to 5 cm depth at the same initial temperature. In general, the conversion of electric energy to useful ...
2000-02-01
Low temperature irradiations in FFTF [Fast Flux Test Facility
International Nuclear Information System (INIS)
The fusion materials program has little irradiation effects data at temperatures from 100 to 350 degree C. Near-term machines such as the International Thermonuclear Engineering Reactor (ITER) will expose materials to neutron doses of 38 to 50 dpa at 150 degree C or less. The data base for structural materials must be extended into this range. Also, lower temperatures are needed to investigate the lower bound for tritium release from solid breeder materials. A low temperature test vehicle is proposed for the Fast Flux Test Facility (FFTF), which will provide test temperatures of 100 to 350 degree C. An 8.5-cm dia. by 100-cm test volume will be instrumented to collect temperature data and provide feedback for control. The spectrum and flux will provide accelerated damage accumulation for structural materials testing and the best available approximation of fusion reactor conditions for solid breeder materials testing. Breeder samples can be equipped with sweep gas ...
1988-10-09
Identification of recharge sources and dating of groundwater using isotope and CFC techniques
International Nuclear Information System (INIS)
Due to severe drought conditions in Pakistan over the past several years, most of the areas are facing extinction of its potable water reserves and inadequate replenishment of groundwater aquifers. Due to over exploitation, the groundwater flow dynamics is changing and water quality is degrading due to induced infiltration from polluted surface sources. Isotope hydrology is relatively a new discipline having great potential for studying various water-related problems. RIAD, PINSTECH has established analytical facilities for commonly used environmental isotopes and applied to investigate various hydrological problems. This paper briefly describes practical examples on recharge mechanism and dating of groundwater in Lahore and Ziarat areas using isotopes like deuterium (/sup 2/H), Oxygen-18 (/sup 18/O), Tritium (/sup 3/H) and CFCs in water. In Lahore, the areas having different contribution of the river Ravi in groundwater recharge have been marked and on the basis ...
2004-06-07
Fast Flux Test Facility (FFTF) standby plan
Energy Technology Data Exchange (ETDEWEB)
The FFTF Standby Plan, Revision 0, provides changes to the major elements and project baselines to maintain the FFTF plant in a standby condition and to continue washing sodium from irradiated reactor fuel. The Plan is consistent with the Memorandum of Decision approved by the Secretary of Energy on January 17, 1997, which directed that FFTF be maintained in a standby condition to permit the Department to make a decision on whether the facility should play a future role in the Department of Energy`s dual track tritium production strategy. This decision would be made in parallel with the intended December 1998 decision on the selection of the primary, long- term source of tritium. This also allows the Department to review the economic and technical feasibility of using the FFTF to produce isotopes for the medical community. Formal direction has been received from DOE-RL and Fluor 2020 Daniel Hanford to implement the FFTF standby decision. The ...
1997-03-06
Environmental distribution and behavior of 3H and 14C around Wolsong Nuclear Power Plants.
To estimate of the dispersion trend of 3H and 14C discharged from the Wolsung Nuclear Power Plants, the present level of 3H and 14C in environmental samples in the vicinity of the Wolsong site was studied. Tree-ring cellulose analyses were carried out for retrospective evaluation of 3H and 14C in the environment around the Wolsong Nuclear Power Plants. 3H released from the Wolsong Nuclear Power Plants has affected an area up to a 25-km radius from the site, while almost all 14C was deposited within a 2-km radius, reaching to a natural level over 2 km. Organically bound tritium concentrations in tree rings were strongly correlated with the gaseous tritium discharge rate, while delta14C (excess) in tree rings ranged from 204 per thousand to 460 per thousand, which did not significantly vary with year. PMID:10832930
2000-06-01
Current status and future plan of JMTR Hot Laboratory
Energy Technology Data Exchange (ETDEWEB)
The newly developed techniques by the Hot Laboratory (JMTR HL) have provided for us the key information on behavior of specimens due to mechanical / physical / chemical / synergistic effects of radiation, stress and water for fission and fusion reactor environment. These techniques are focused on several topics as follows; (1) miniaturized specimen test for the development of fusion reactor materials, (2) slow strain rate tensile testing (SSRT) and crack propagation measuring tests for the study of Irradiation Assisted Stress Corrosion Cracking (IASCC) of core internals of LWR, (3) handling technique on specimens including tritium for the research and development of tritium breeders and neutron multiplier as fusion blanket materials, (4) joining method using the Tungsten Inert Gas (TIG) welding technique for re-assembling of capsule and re-fabrication of specimen and (5) nondestructive evaluation using ultrasonic wave and infrared thermography ...
1999-08-01
Energy Technology Data Exchange (ETDEWEB)
ESH-19 personnel collected soil and single-stage water samples around the perimeter of Area G at Los Alamos National Laboratory (LANL) during FY 95 to characterize possible radionuclide movement out of Area G through surface water and entrained sediment runoff. Soil samples were analyzed for tritium, total uranium, isotopic plutonium, americium-241, and cesium-137. The single-stage water samples were analyzed for tritium and plutonium isotopes. All radiochemical data was compared with analogous samples collected during FY 93 and 94 and reported in LA-12986 and LA-13165-PR. Six surface soils were also submitted for metal analyses. These data were included with similar data generated for soil samples collected during FY 94 and compared with metals in background samples collected at the Area G expansion area.
1997-09-01
International Nuclear Information System (INIS)
Lithium carbonate pellets are frequently used for estimation of tritium production rate in irradiated samples in fusion blanket neutronics experiment and the activity is measured by liquid scintillation counting technique. In this measurement, it is essential to solve the lithium carbonate pellet as much as possible and to mix the pellet solution into scintillation cocktail homogeneously at stable condition. For this purpose, a novel binary-acid method has been developed to solve lithium carbonate and to mix the pellet solution into scintillation cocktail. High solubility is attained by adopting two acids, HNO_3 and CH_3COOH, and a good compatibility of the pellet solution with scintillator is obtained by emulsion cocktail resulting in high counting efficiency. Defining a product of dissolved mass and counting efficiency as a Figure of Merit (FOM), the present method has higher FOM value than the conventional method and is extremely simple in a sample preparation ...
Energy Technology Data Exchange (ETDEWEB)
Argonne National Laboratory (ANL) is implementing waste minimization and pollution prevention activities into its conduct of decontamination and decommissioning (D&D) projects. Many of these activities are rather straight forward and simple approaches, yet they are often overlooked and not implemented as often as they should or could be. Specific activities involving recycling and reuse of materials and structures, which have proven useful in lowering decommissioning and disposal costs on D&D projects at ANL are presented.
1996-07-01
Treatment of radioactive metallic waste by the electro-slag melting method
Energy Technology Data Exchange (ETDEWEB)
The applicability of the electro-slag melting method for treating plutonium contaminated metallic waste was studied. A 100kg test furnace was built and simulated metallic waste was melted and solidified in this furnace. Waste volume was reduced to 1/25 with a decontamination factor of 25 and the slag and the copper mold are repeatedly usable. The process is expected to be employed in the project of PWTF (Plutonium contaminated Waste Treatment Facilities).
1983-01-01
International Nuclear Information System (INIS)
Most of the low-level liquid radioactive wastes generated from PWR plants are classified into high or low total suspended solid(HTDS or LTDS), and into radiochemical and radioactive laundry waste. Although the evaporation process has a high decontamination ability, it has several problems such as corrosion, foam, and congestion. A new liquid waste disposal process using the ion-exchange demineralizer(IED), instead of the current evaporation process, has been introduced into the Yonggwang NPP No 5 and 6. These two methods have been compared to understand the differences in this study. Aspects compared here were the released radioactivity amount of the liquid radioactive wastes, the dose of off-site residents, the decontamination factor, and the amount of the solid radioactive wastes. The IED system is designed to discharge higher radioactivity about 20% than the evaporating system, and the actual radioactivity released from the evaporating and ...
2004-09-01
Teleobservation in hostile environment
International Nuclear Information System (INIS)
In order to meet the needs of remote servicing performed in nuclear power plants, in fuel reprocessing plants and in atomic research centers three companies: - STMI, subsidiary of CEA, EDF and SGN, specialized in decontamination and dismantling, - La Calhene, subsidiary of CEA and SGN, specialized in robotics, - Inspectronic, manufacturer of closed circuit television cameras, have combined to create the Visionic Society, the main objectives of which are observation by television and inspections in radioactive environment.
Sweden employs a multi venturi scrubber for containment venting
Energy Technology Data Exchange (ETDEWEB)
The Filtra-MVSS for filtered venting of containment overpressure is a flexible system capable of covering a wide range of hypothetical design basis events for BWRs and PWRs. The system encompasses a number of special features, can be optimized for a specified decontamination factor, and can accommodate a wide range of off-gas flow rates.
1988-03-01
Strontium removal from caustic carbonate waste solutions using carrier coprecipitation
Energy Technology Data Exchange (ETDEWEB)
A carrier coprecipitation procedures has been developed for the removal of radioactive strontium from caustic liquid low-level waste (LLLW) generated at Oak Ridge National Laboratory. The two-step treatment process involves the addition of normal Sr (as SrCl{sub 2}) to the waste matrix, which is composed primarily of 0.3 M NaOH and 0.6 M Na{sub 2}CO{sub 3}. The active Sr equilibrates with the normal Sr carrier and coprecipitates as SrCO{sub 3} at pH 13. A liquid/solid separation is made before the pH of the supernate is reduced to pH 8 with sulfuric acid. During the neutralization step, the aluminum is the waste precipitates as Al(OH){sub 3}. Further Sr decontamination is achieved as traces of active Sr sorb to the Al(OH){sub 3} that precipitates during the neutralization step. A final liquid/solid separation is made at pH 8 to remove the sorbed active Sr. Maximum Sr decontamination of the LLLW is obtained when at least 50 ppm normal Sr is ...
1994-12-31
SOLVENT EXTRACTION OF CESIUM BY DIPICRYLAMINE. III. SEMIWORKS DEMONSTRATION
The extraction and recovery of cesium from simulated Purex waste solutions was successfully demonstrated in the pilot plant pulse column. Stable volumetric capacities as high as 670 gph/ft/sup 2/ (sum of both phases) were obtained for alkaline supernate-type waste; however, for efficient operation (transfer unit height - HTU -of two feet or less), the maximum throughput rate was limited to about 500 gph/ft/sup 2/. This rate could be achieved with feeds diluted to densities within 0.08 g/cc of the solvent density. Stable feed was prepared from simulated current, denitrated waste by addition of citric acid to complex the iron before neutralization to the desired operating pH of 7 to 8. Capacities of 500 gph/ft/sup 2/ were readily achieved with this feed, together with HTU's of 1.0 to 1.3 feet. Sodium extracted with the cesium was satisfactorily scrubbed from the solvent with a dilute citric acid solution. Scrub section sodium ...
1963-03-15
Energy Technology Data Exchange (ETDEWEB)
A borohydride, for instance sodium borohydride, is added to the radioactive effluent, with eventually a carrier such as Cu{sup +}, to give a precipitate containing ruthenium. The processing can be combined to Sr and Cs precipitation be know processes giving barium sulfate and nickel ferrocyamide precipitates. Influence of borohydride concentration on decontamination factor is given.
1989-08-25
Radiation treatment of some poultry products
International Nuclear Information System (INIS)
Practical procedures were developed for large-scale microbial decontamination of dry egg powder and gelatine with gamma radiation ("6"0Co). The formation and lifes of free organic radicals in these materials were examined by ESR measurements of powder samples. The concentration of these radicals was studied in dependence on the time of storage. Secondary oxidation of egg fats by air oxygen was investigated. Sensoric tests of irradiated gelatine, both in powder and hydrogel form, were performed. (author). 4 figs., 2 tabs., 2 refs.
1988-09-26
Energy Technology Data Exchange (ETDEWEB)
This Test Plan outlines the testing to be done on the Special Protective Coating (SPC) Polyurea which includes: Tank Waste Compatibility, Decontamination Factor Testing, and Adhesion Strength Testing after a sample has been exposed to Radiation.
2001-01-15
International Nuclear Information System (INIS)
This book contains the proceedings of the International Topical Meeting on Remote Systems and Robotics in Hostile Environments. It is organized under the following sessions: Worldwide Applications Overview; Operating Mobile Systems; Sensors and Control Systems; Space Applications; Reactor Operations and Surveillance; Remote Equipment for Hazardous Operations; Future Mobile System; Mining and Construction Operations; Special Applications; Hot Cell Applications; Processing; Reactor Operations and Maintenance; Decontamination and Waste Handling; Remote Handling Development and Demonstration.
Energy Technology Data Exchange (ETDEWEB)
A krypton recovery pilot plant has been completed for the Power Reactor and Nuclear Fuel Development Corporation. This is the first industrial facility in the world to make practical use of development results for offgas treatment and storage from nuclear facilities. The cryogenic distillation process was adopted as a proven and reliable method to separate krypton and xenon, and to reduce gas effuents to a level so low that the decontamination factor amounts to more than 1000.
1983-01-01
Experimental verification of caustic-side solvent extraction for removal of cesium from tank waste.
Energy Technology Data Exchange (ETDEWEB)
The objectives of this report are: to demonstrate complete CSSX process flowsheet (proof of concept)--decontamination factor {ge} 40,000, and concentration factor {approx}15; Scientific and technical issues evaluated--stage efficiency, temperature control, hydraulic performance, long time (multi-day) operation, short-term shutdown, effect of solids, and recovery from Cs moving through strip section.
2001-09-21
Energy Technology Data Exchange (ETDEWEB)
This document provides data on aerosol concentrations in tank headspaces, total mass of aerosols in the tank headspace, and mass of aerosols sent to the exhauster during rotary mode core sampling from November 1994 through June 1999. A decontamination factor for the RMCS exhauster filter housing is calculated based upon operational data and non-destructive assay.
2001-03-23
Energy Technology Data Exchange (ETDEWEB)
This document provides data on aerosol concentrations in tank head spaces, total mass of aerosols in the tank head space and mass of aerosols sent to the exhauster during Rotary Mode Core Sampling from November 1994 through June 1999. A decontamination factor for the RMCS exhauster filter housing is calculated based on operation data.
2000-01-24
Estimating demolition cost of plutonium buildings for dummies
Energy Technology Data Exchange (ETDEWEB)
The primary purpose of the Rocky Flats Field Office of the US Department of Energy is to decommission the entire plant. In an effort to improve the basis and the accuracy of the future decommissioning cost, Rocky Flats has developed a powerful but easy-to-use tool to determine budget cost estimates to characterize, decontaminate, and demolish all its buildings. The parametric cost-estimating tool is called the Facilities Disposition Cost Model (FDCM).
2000-07-01
Development of an incinerator using ceramic filters for low level radioactive solid waste treatment
International Nuclear Information System (INIS)
This facility has treatment capacity of 12 kg/hr, and is equipped with a furnace, two ceramic filter chambers, each of which hangs inside the 36 ceramic filter elements having mean pore size of 44 #mu#m. Three series of experiments were performed during a period from October 1972 to August 1973. The first was measurement of the change of pressure drop of the primary and the secondary filters after an operation of 52 days (352 hours). The pressure drop of the primary filter did not change during the operation, but the secondary brought a fairly large increment, from 79 to 140 mmAq. The second was measurement of the after-burning effect of the primary filter for the soot and tar in the off-gas. Through the after-burning most of the soot was removed from the off-gas, though the tar was not perfectly taken off. At the secondary filter, some of the tar was burnt, but most of it was caught by the filter as aerosol. The third was measurement of decontamination factors of ...
Determination of [sup 99]Tc in sea water at ultra low levels
Energy Technology Data Exchange (ETDEWEB)
A method based on the collection of [sup 99]Tc from 500 l sea water samples by anion exchange and further extraction of TcO[sub 4][sup -] into 5% triisooctylamine-xylene has been improved to include a decontamination factor 6.5x10[sup 5] for uranium. The detection limit for [sup 99]Tc is thereby reduced to 3 mBq/m[sup 3].
1994-01-20
Decontamination of LRW of low and intermediate level of activity with a new bio-sorbent mycoton
International Nuclear Information System (INIS)
An absorption method of elimination of liquid radioactive wastes (LRW) of low and intermediate activity level by decreasing their contamination up to the level permitting their discharge into the environment is proposed in the paper. The LRW decontamination is accompanied with efficient compacting the resulting secondary solid wastes. The method is based on the use of a new very efficient, chitin containing natural fiber bio-sorbent, Mycoton, which is manufactured commercially in Ukraine. The chemical composition of the sorbent and its highly developed surface provide practically unrestricted opportunities for producing its modifications having any necessary absorption and operational characteristics. The effects of pH, the presence of various salts and complexing agents, as well as of some other factors to the distribution coefficients of the most important radionuclides have been carefully studied in experiments with Mycoton and its modifications. It appeared, ...
2005-10-09
De-entrainment of boron by evaporation
Energy Technology Data Exchange (ETDEWEB)
The purpose of this research was to investigate the de-entrainment of boron for evaporators used in nuclear power plants. The forced circulation and semi-continuous type evaporator was used in the experiment. Cyclone and glass-wool packed column which is supposed to provide good decontamination factor as well as easy maintenance, were selected as de-entrainment device to be used in the evaporation of radioactive liquid wastes. The de-entrainment device combined with cyclone and glass-wool column has shown overall DF more than 1000 for boron.
1986-12-01
Contamination preventive method and decontaminating method for equipment
Energy Technology Data Exchange (ETDEWEB)
The method of the present invention comprises a step of previously coating a positive type resist on the surface of equipment, a step of solidifying the coated positive type resist and a step of bringing the coated equipment to circumstances for use and cleaning the positive type resist. With such procedures, the amount of radioactive materials deposited on the equipment can be reduced, and redeposition of nuclides on the surface to be cleaned can be prevented. (T.M.)
1998-12-04
Cation exchange separation of trace amounts of {sup 203}Hg and {sup 181}Hf
Energy Technology Data Exchange (ETDEWEB)
A radiochemical method of separation of {sup 203}Hg from {sup 181}Hf is described. The method involves separation by Dowex 50W- X 8, 100-200 mesh, cation exchange resin using 1 M hydrochloric acid as the eluant. The chemical yield for the separation of mercury is > 85% and the decontamination factor is >10{sup 4}. The {sup 181}Hf can be eluted from the column by 4 M HCl.
2000-02-01
International Nuclear Information System (INIS)
Most of the low-level liquid radioactive wastes generated from PWR plants are classified into high or low total suspended solid(HTDS or LTDS), radio-chemical waste and radioactive laundry waste. Although the evaporation process has a high decontamination ability, it has several problems such as corrosion, foaming, and congestion. A new liquid waste disposal process using the ion-exchange demineralizer(IED) has been introduced into the Yonggwang NPP 5 and 6 to complement the current evaporation process. To determine the differences, these two methods have been compared in this study. Those aspects compared here were the released radioactivity volume of the liquid radioactive wastes, The dose of off-site residents, the decontamination factor, and the amount of the solid radioactive wastes. While it was expected that the liquid radioactive waste volume in the evaporating system would be 20 percent higher than in the IED, the actual volume of the ...
2003-11-05
Thermonuclear reactivity of D-T fusion plasma with spin-polarized fuel
Energy Technology Data Exchange (ETDEWEB)
The thermonuclear reactivity of deuterium(D) - tritium(T) fusion plasma with spin-polarized fuel has been studied. Two mechanisms of depolarization, collisions and waves, in the high temperature fusion plasma have been considered. The binary collisions have been found not to change the nuclear spin states. The waves with a frequency of a few GHz, however, changes the spin states appreciably, when {delta}B/B{sub 0} (the ratio of the amplitude of the fluctuating magnetic field to the external field) becomes larger than 10{sup -5}. (author)
1999-04-01
Stress analysis of hydride bed vessels used for tritium storage
Energy Technology Data Exchange (ETDEWEB)
A prototype hydride storage bed, using LaNi{sub 4.25}Al{sub 0.75} as the storage material, was fitted with strain gages to measure strains occurring in the stainless steel bed vessel caused by expansion of the storage powder upon uptake of hydrogen. The strain remained low in the bed as hydrogen was added, up to a bed loading of about 0.5 hydrogen to metal atom ratio (H/M). The strain then increased with increasing hydrogen loading ({approximately} 0.8 H/M). Different locations exhibited greatly different levels of maximum strain. In no case was the design stress of the vessel exceeded.
1991-01-01
Loss of flow accident analysis of a water-cooled fusion reactor
International Nuclear Information System (INIS)
Within the APROS simulation environment we have built a thermo-hydraulic model of a conceptual fusion power plant which is water cooled and uses lithium-lead for tritium breeding. For the safety assessment of this design we have studied an accident sequence which starts from a loss or coolant flow then leads to first wall breach and pressurisation of the vacuum vessel. Simulations have revealed strong pressure transients which can be alleviated by design changes. One goal is to verify the adequacy of the containment design: it remains intact at least 14 h without any mitigating efforts. Estimates for radioactive releases are obtained. (author)
2003-08-25
JET contribution to ITER fuel cycle issues
Energy Technology Data Exchange (ETDEWEB)
The Joint European Torus (JET) fusion machine is the only device capable of operation with tritium (as fuel) and Be (as plasma facing component), what makes it best suited to study ITER relevant issues. A large variety of activities are performed within the JET Fusion Technology Task Force. In this paper, some topics such as erosion/deposition and material transport, flakes characterization and detritiation techniques are highlighted. Recent results obtained using a pumping cryo-panel and on plasma facing component characterisation are given. Finally, issues that will be addressed in the forthcoming JET work-programme are presented, such as a beryllium main wall for JET and in-situ laser detritiation. (authors)
2005-07-01
Evaluation of tritiated water retention capacity of fusion reactor concrete building
Energy Technology Data Exchange (ETDEWEB)
In this paper the diffusion of tritiated water vapor into concrete walls is studied to evaluate tritiated water retention capacity of a fusion reactor concrete building. Using a model of the tritiated water diffusion determined form experimental results, depth profiles of tritiated water in concrete are calculated in the case of being exposed to air containing tritiated water vapor during the normal operational condition of a fusion reactor. A 0.5-m-thick concrete is sufficient for reactor hall walls from a viewpoint of the tritium containment.
1992-03-01
Evaluation of tritiated water retention capacity of fusion reactor concrete building
International Nuclear Information System (INIS)
In this paper the diffusion of tritiated water vapor into concrete walls is studied to evaluate tritiated water retention capacity of a fusion reactor concrete building. Using a model of the tritiated water diffusion determined form experimental results, depth profiles of tritiated water in concrete are calculated in the case of being exposed to air containing tritiated water vapor during the normal operational condition of a fusion reactor. A 0.5-m-thick concrete is sufficient for reactor hall walls from a viewpoint of the tritium containment.
An Evaluation of Dual-Media Contaminant Transport for SRS Environmental Applications
The dual-media approach to contaminant transport modeling has emerged over the years as a clear improvement over the conventional Fickian advection-dispersion, or single-medium model, in an increasing number of settings. Recent application to the MADE-2 tracer test at Columbus Air Force Base has extended interest to field-scale plume migration in unconsolidated sediments. Subsequent application to tritium migration from the SRS F- and H-area seepage basins within this study also demonstrated improved transport predictions.
2002-12-19
Energy Technology Data Exchange (ETDEWEB)
This paper describes the results of a model intercomparision exercise for predicting tritium transport through foodchains. Modellers were asked to assume that farmland was exposed for one hour to an average concentration in air of 10{sup 4} MBq tritium m{sup -3}. They were given the initial soil moisture content and 30 days of hourly averaged historical weather and asked to predict HTO and OBT concentrations in foods at selected times up to 30 days later when crops were assumed to be harvested. Two fumigations were postulated, one at 10.00 h (i.e., in day-light), and the other at 24.00 h (i.e., in darkness).Predicted environmental media concentrations after the daytime exposure agreed within an order of magnitude in most cases. Important sources of differences were variations in choices of numerical values for transport parameters. The different depths of soil layers used in the models appeared to make important contributions to differences in ...
1998-01-01
Energy Technology Data Exchange (ETDEWEB)
This report describes experimental results for the selective removal of strontium and cesium from simulated waste solutions using monosodium titanate (MST) and crystalline silicotitanate (CST)-laden filter cartridges. Four types of ion exchange cartridge media (CST and MST designed by both 3M and POROX{reg_sign}) were evaluated. In these proof-of-principle tests effective uptake of both Sr-85 and Cs-137 was observed. However, the experiments were not performed long enough to determine the saturation levels or breakthrough curve for each filter cartridge. POREX{reg_sign} MST cartridges, which by design were based on co-sintering of the active titanates with polyethylene particles, seem to perform as well as the 3M-designed MST cartridges (impregnated filter membrane design) in the uptake of strontium. At low salt simulant conditions (0.29 M Na{sup +}), the instantaneous decontamination factor (D{sub F}) for Sr-85 with the 3M-design MST cartridge measured 26, ...
2011-05-26
International Nuclear Information System (INIS)
Interest to thin film of metals' silicides first of all is conditioned intrinsic al them unique physical properties. On their basis of it is possible to produce extremely sophisticated devices of solid-state electronics, production which needs the controlled change of physics, chemical and electrical properties with high-level of accuracy. On the present time most are in detail investigated composition, structure and properties of three-dimensional samples of metals' silicides. In the last years the intensive are led to researches in the direction of creation and study of physical-chemical properties thin (500-1000 Angstroms) and ultrafine (100-120 Angstroms) films silicides. It has information about composition, morphology of surface and emission of properties of thin film of silicides of barium, of cobalt and of palladium, was obtained in conditions of ultra-high vacuum. Low energy ion implantation and further annealing on composition, electronic and crystalline ...
Direct Comparison of the X-Ray Emission and Absorption of Cerium Oxide
Energy Technology Data Exchange (ETDEWEB)
Bremstrahlung Isochromat Spectroscopy (BIS). The XES spectra were collected using a Specs electron gun for the excitation and the XES 350 grating monochromator and channel plate system from Scienta as the photon detection. Spectra were collected in 'normal mode,' where the electron gun kinetic energy (KE) and the energy position of the center of the channel plate were both fixed and the energy distribution in the photon (hv) spectrum was derived from the intensities distributed across the channel plate detector in the energy dispersal direction. The polycrystalline Ce sample was oxidized by exposure to air at ambient pressures. After introduction to the ultra-high vacuum system, the oxidized sample was bombarded with Ar, to clean the topmost surface region and stabilize the surface and near surface regions. Although CeO{sub 2} would be the thermodynamically preferred composition in an oxygen rich environment, the combination of a vacuum ...
2010-11-24
Energy Technology Data Exchange (ETDEWEB)
Some hypo-stoichiometric Zr-based Laves phase alloys were prepared and studied from a viewpoint of discharge capacity for electrochemical application. After careful alloy design of ZrMn{sub 2}-based hydrogen storage alloys through changing their stoichiometry while substituting or adding some alloying elements, the Zr(Mn{sub 0.2}V{sub 0.2}Ni{sub 0.6}){sub 1.8} alloy reveals relatively good properties with regard to hydrogen storage capacity, hydrogen equilibrium pressure and electrochemical discharge capacity. In order to improve the discharge capacity and rate-capability, Zr is partially replaced by Ti. The discharge capacity of Zr{sub 1-x}Ti{sub x}(Mn{sub 0.2}V{sub 0.2}Ni{sub 0.6}){sub 1.8} (x=0.0, 0.2, 0.3, 0.4, 0.6) alloy electrodes at 30 C reaches a maximum value and decreases as the Ti fraction increases. In view of electrochemical and thermodynamic characteristics, the occurrence of a maximal phenomenon of the electrochemical discharge capacity of the alloy is attributed to a ...
2000-08-10
Volume reduction of reactor wastes by spray drying
International Nuclear Information System (INIS)
Three simulated low-level reactor wastes were dried using a spray dryer-baghouse system. The three aqueous feedstocks were sodium sulfate waste characteristic of a BWR, boric acid waste characteristic of a PWR, and a waste mixture of ion exchange resins and filter aid. These slurries were spiked with nonradioactive iron, cobalt, and manganese (representing corrosion products) and nonradioactive cesium and iodine (representing fission products). The throughput for the 2.1-m-diameter spray dryer and baghouse system was 160-180 kg/h, which is comparable to the requirements for a full-scale commercial installation. A free-flowing, dry product was produced in all of the tests. The volume reduction factor ranged from 2.5 to 5.8; the baghouse decontamination factor was typically in the range of 10"3 to 10"4. Using an overall system decontamination factor of 10"6, the activity of the off-gas was calculated to be one to two orders of magnitude less than ...
Toxicity of radioactive wastes generated from PEACER spent fuel
Energy Technology Data Exchange (ETDEWEB)
Assessment on the back end fuel cycle, in PEACER (Proliferation-resistant Environmental-friendly Accident-tolerant Continuable and Economical Reactor) that was designated as a new transmutation concept, was performed. Recovery system of uranium and TRU for PEACER is based on pyroprocessing. In the assessment of Long-Lived Fission Products (LLFP) wastes, initially {sup 90}Sr and {sup 137}Cs are dominant contributor nuclides until 30 years and especially {sup 90}Sr and {sup 137}Cs have the highest activity and decay heat than other LLFP. In this study, recovery of {sup 90}Sr and {sup 137}Cs is recommended for reducing of wastes loading. The acceptable decontamination factor is investigated by the toxicity of PEACER spent fuel. The acceptable decontamination factor is about 1.02E+05 for the actinides from PEACER spent fuel after 10 years cooling, 4.26E+05 after 100 years cooling, 1.97E+04 after 300 years cooling, 9.52E+03 after 1000 years cooling.
2003-10-01
Toxicity of radioactive wastes generated from PEACER spent fuel
International Nuclear Information System (INIS)
Assessment on the back end fuel cycle, in PEACER (Proliferation-resistant Environmental-friendly Accident-tolerant Continuable and Economical Reactor) that was designated as a new transmutation concept, was performed. Recovery system of uranium and TRU for PEACER is based on pyroprocessing. In the assessment of Long-Lived Fission Products (LLFP) wastes, initially "9"0Sr and "1"3"7Cs are dominant contributor nuclides until 30 years and especially "9"0Sr and "1"3"7Cs have the highest activity and decay heat than other LLFP. In this study, recovery of "9"0Sr and "1"3"7Cs is recommended for reducing of wastes loading. The acceptable decontamination factor is investigated by the toxicity of PEACER spent fuel. The acceptable decontamination factor is about 1.02E+05 for the actinides from PEACER spent fuel after 10 years cooling, 4.26E+05 after 100 years cooling, 1.97E+04 after 300 years cooling, 9.52E+03 after 1000 years cooling.
2003-10-01
Toxicity of Radioactive Wastes Generated from PEACER in Korea
International Nuclear Information System (INIS)
Assessment on the back end fuel cycle, in PEACER (Proliferation-resistant Environmental-friendly Accident-tolerant Continuable and Economical Reactor) that was designated as a new transmutation concept, was performed. Recovery system of uranium and TRU for PEACER is based on pyro-processing. In the assessment of long-lived fission products (LLFP) wastes, initially "9"0Sr and "1"3"7Cs are dominant contributor nuclides until 30 years and especially "9"0Sr and "1"3"7Cs have the highest activity and decay heat than other LLFP. In this study, recovery of "9"0Sr and "1"3"7Cs is recommended for reducing of wastes loading. The acceptable decontamination factor is investigated by the toxicity of PEACER spent fuel. The acceptable decontamination factor is about 1.02 E+05 for the actinides from PEACER spent fuel after 10 years cooling, 4.26 E+05 after 100 years cooling, 1.97 E+04 after 300 years cooling, 9.52 E+03 after 1000 years cooling. (authors)
2006-06-04
The RADionuclide transport, removal, and dose (RADTRAD) code
International Nuclear Information System (INIS)
The RADionuclide Transport, Removal, And Dose (RAD-TRAD) code is designed for U.S. Nuclear Regulatory Commission (USNRC) use to calculate the radiological consequences to the off-site population and to control room operators following a design-basis accident at light water reactor (LWR) power plants. This code utilizes updated reactor accident source terms published in draft NUREG-1465. The code will track the transport of radionuclides as they are released from the reactor pressure vessel, travel through the primary containment and other buildings, and are released to the environment. As the radioactive material is transported through the primary containment and other buildings, credit for several removal mechanisms may be taken, including sprays, suppression pools, overlying pools, filters, and natural deposition. Simple models are available for these different removal mechanisms that use, as input, information about the conditions in the plant and predict either a removal ...
1993-11-14
The RADionuclide Transport, Removal, and Dose (RADTRAD) code
Energy Technology Data Exchange (ETDEWEB)
The RADionuclide Transport, Removal, And Dose (RADTRAD) code is designed for US Nuclear Regulatory Commission (USNRC) use to calculate the radiological consequences to the offsite population and to control room operators following a design-basis accident at Light Water Reactor (LWR) power plants. This code utilizes updated reactor accident source terms published in draft NUREG-1465, ``Accident Source Terms for Light-Water Nuclear Power Plants.`` The code will track the transport of radionuclides as they are released from the reactor pressure vessel, travel through the primary containment and other buildings, and are released to the environment. As the radioactive material is transported through the primary containment and other buildings, credit for several removal mechanisms may be taken including sprays, suppression pools, overlying pools, filters, and natural deposition. Simple models are available for these different removal mechanisms that use, as input, information about the ...
1993-07-01
Testing of the SpinTek Rotary Microfilter Using Actual Waste
Energy Technology Data Exchange (ETDEWEB)
The Department of Energy selected caustic-side solvent extraction (CSSX) as the preferred cesium-removal technology for SRS high-level waste. In the pretreatment step of the CSSX flowsheet, the incoming salt solution, which contains entrained sludge, is contacted with MST to adsorb strontium and selected actinides. An alternative approach replaces MST with the addition of sodium permanganate, strontium nitrate, and hydrogen peroxide. The pretreatment operation then filters the resulting slurry to remove the sludge and MST or manganese oxide and strontium carbonate solids. The filtrate receives further treatment in the solvent extraction system. SRTC personnel coordinated tests using a SpinTek rotary microfilter at the vendor location in FY01. These tests demonstrated a significant improvement - 2.5 to 6 times increase - in performance relative to the conventional cross-flow filter units. Rotary microfilter testing used a filter disk with nominal pore size of either 0.1-micron or 0. ...
2004-02-13
Separation of trace radionuclides by ion exchange in the presence of competing ions
International Nuclear Information System (INIS)
The performance of larger than bench scale ion exchange systems is evaluated by using solutions containing trace amounts of "1"3"7Cs, "8"5Kr, and "1"3"1I, and large amounts of either NaCl or Na_2HPO_4, H_3BO_3, and LiOH. The significant finding in this study is that the empirical rules of ionic selectivity of strong acid cation and strong base anion resins were followed by all ionic species, even though concentrations of some macrocomponents were nearly 10"6 times those of trace components. Other results of possible importance are the correlation between the instantaneous decontamination factor (DF) and the efficiency of column exchange capacity utilization, and the concept of time average decontamination factor (anti DF). The plot of anti DF vs. feed throughput will serve as a guide in determining when the feed should be discontinued in order to achieve a desired anti DF. Both of these correlations are derived from the breakthrough curves.
Safety assessment for clearance of radioactive metal wastes from nuclear facility
Energy Technology Data Exchange (ETDEWEB)
Safety assessments for clearance of H-beam and valves, main radioactive metal wastes in Kori nuclear power plants, were carried out to derivate a decontamination factor for satisfying the dose limits of clearance level (Maximum individual dose: 10 {mu}Sv/y, collective dose: 1 man{center_dot}Sv/y) in Korea. Maximum individual dose and collective dose were evaluated by internal dose conversion factor which based on the concept of effective dose in ICRP publication 60. The results of maximum individual dose and collective dose is 139 {mu}Sv per year and 0.166 man{center_dot}Sv per year about H-beam, and 158 {mu}Sv per year and 0.468 man{center_dot}Sv per year about valves respectively. Demand decontamination factor satisfied with, which is respectively more than 13.9 and 15.8 for satisfying clearance level.
2003-10-01
Safety assessment for clearance of radioactive metal wastes from nuclear facility
International Nuclear Information System (INIS)
Safety assessments for clearance of H-beam and valves, main radioactive metal wastes in Kori nuclear power plants, were carried out to derivate a decontamination factor for satisfying the dose limits of clearance level (Maximum individual dose: 10 #mu#Sv/y, collective dose: 1 man#centre dot#Sv/y) in Korea. Maximum individual dose and collective dose were evaluated by internal dose conversion factor which based on the concept of effective dose in ICRP publication 60. The results of maximum individual dose and collective dose is 139 #mu#Sv per year and 0.166 man#centre dot#Sv per year about H-beam, and 158 #mu#Sv per year and 0.468 man#centre dot#Sv per year about valves respectively. Demand decontamination factor satisfied with, which is respectively more than 13.9 and 15.8 for satisfying clearance level.
2003-10-01
Energy Technology Data Exchange (ETDEWEB)
The {sup 176}Ybn,{gamma}{sup 177}Yb-{beta}{sup -}{yields}{sup 177}Lu process was investigated to provide no-carrier-added (nca) {sup 177}Lu. The radiochemical separation of the {sup 177}Lu from the macro-amounts of the ytterbium target based on the cementation process, i.e. the selective extraction of Yb by Na(Hg) amalgam from Cl{sup -}/CH{sub 3}COO{sup -} electrolytes, followed by a final cation exchange purification. The cementation separation process provides a decontamination factor of Yb(III) of 10{sup 4}, the cation exchange purification adding a decontamination factor of >10{sup 2}. The nca {sup 177}Lu is available in radiochemically pure form despite the chemical similarity of the lanthanides with 75{+-}5% overall separation yield within 4-5 h. It can be used to synthesise nca {sup 177}Lu labelled radiotherapeuticals.
2000-09-15
Pyrochemical Processing for Low-Level Waste Production in PEACER
A pyrochemical partitioning process has been conceptually designed so that the transmutation of spent LWR fuels in PEACER can produce mainly low-level waste (Class C waste) for near-surface burial. Chloride salt technology developed for IFR has been employed as the baseline. Electrorefining, reductive extraction and salt recycling steps are used to construct overall flowsheet in order to support PEACER operation. The decontamination factor for transuranic elements was estimated based on both thermodynamic models and reported experimental data. It is expected that overall decontamination factor can be as high as 10{sup 5} for transuranic elements. Final wastes from pyrochemical processing for PEACER are noble metals, alkaline earth metal, and lanthanides. The final wastes are stabilized by mixing with zeolite and glass-frits such that concentration limit for class C waste can be met. The volume of Class C waste is estimated to be small enough to ...
2002-07-01
Pyrochemical Processing for Low-Level Waste Production in PEACER
International Nuclear Information System (INIS)
A pyrochemical partitioning process has been conceptually designed so that the transmutation of spent LWR fuels in PEACER can produce mainly low-level waste (Class C waste) for near-surface burial. Chloride salt technology developed for IFR has been employed as the baseline. Electrorefining, reductive extraction and salt recycling steps are used to construct overall flowsheet in order to support PEACER operation. The decontamination factor for transuranic elements was estimated based on both thermodynamic models and reported experimental data. It is expected that overall decontamination factor can be as high as 10"5 for transuranic elements. Final wastes from pyrochemical processing for PEACER are noble metals, alkaline earth metal, and lanthanides. The final wastes are stabilized by mixing with zeolite and glass-frits such that concentration limit for class C waste can be met. The volume of Class C waste is estimated to be small enough to make ...
2002-06-09
Production of "8"3Rb and development of a generator for the separation of sup(83m)Kr from "8"3Rb
International Nuclear Information System (INIS)
"8"3Rb was produced from rubidium by a (#gamma#,2n)-reaction. The specific activity in the irradiated samples of RbCl was 0.2 to 0.3mCi"8"3Rb/gRb. For the separation of the sup(83m)Kr in the liquid phase the cation exchanger Dowex-50WX12 proved to be a suitable carrier. sup(83m)Kr was eluted by bidistilled water. The yield ranged from 85-95%, at an elution time of 3 minutes. The decontamination factor was > 10"6. The separation of sup(83m)Kr in the gaseous phase was effected by floating a "8"3Rb loaded column with an elution gas. The best results were obtained with a generator containing aluminium oxide as carrier for "8"3Rb. The yield of sup(83m)Kr was 90-100%, the decontamination factor > 10"4, the time needed for the separation 20-60 seconds. All generators proved to be very safe even after long time of use. (orig.).
Pilot-scale testing of pyrolysis for the volume reduction of organic waste
Energy Technology Data Exchange (ETDEWEB)
Pilot-scale pyrolysis units have been in operation since 1980 to test the efficiency of thermal treatment of transuranic (TRU) solid waste to retrieve the TRUs and to reduce the volume of wastes such as spent solvent, spent resin, and others. These wastes are generated by reprocessing, fuel production, and utilities. NUKEM has developed a criticality-safe, ring-slab reactor to decompose solid TRU waste. The plant processes 25 kg/h with a polyvinyl chloride content up to 70%. The overall throughput (inactive) up to the spring of 1982 was 2000 kg. The decontamination factor for the reactor itself is 1000. The liquid wastes, mainly spent solvent, are cracked under nitrogen at 400 to 700/sup 0/C in a reactor that is filled by a packed bed kept in motion by a specially designed agitator. This unit was built for 15 kg/h water equivalent evaporation. Up to 1982 the unit processed 2000 kg of spent solvent (simulated) overall. The decontamination factor ...
1982-11-01
Pilot-scale testing of pyrolysis for the volume reduction of organic waste
International Nuclear Information System (INIS)
Pilot-scale pyrolysis units have been in operation since 1980 to test the efficiency of thermal treatment of transuranic (TRU) solid waste to retrieve the TRUs and to reduce the volume of wastes such as spent solvent, spent resin, and others. These wastes are generated by reprocessing, fuel production, and utilities. NUKEM has developed a criticality-safe, ring-slab reactor to decompose solid TRU waste. The plant processes 25 kg/h with a polyvinyl chloride content up to 70%. The overall throughput (inactive) up to the spring of 1982 was 2000 kg. The decontamination factor for the reactor itself is 1000. The liquid wastes, mainly spent solvent, are cracked under nitrogen at 400 to 700"0C in a reactor that is filled by a packed bed kept in motion by a specially designed agitator. This unit was built for 15 kg/h water equivalent evaporation. Up to 1982 the unit processed 2000 kg of spent solvent (simulated) overall. The decontamination factor is ...
Multiple Ion Exchange Column Tests for Technetium Removal from Hanford Tank Waste Supernate
Five cycles of loading, elution, and regeneration were performed to remove technetium from a Hanford waste sample retrieved from Tank 241-AW-101 using SuperLig 639 resin. The waste sample was diluted to 4.95 M Na plus and then was processed to remove 137Cs through dual ion exchange columns each containing 15 mL of SuperLig 644. To remove 99Tc, the cesium decontaminated solution was processed downwards through two ion exchange columns, each containing 12 mL of SuperLig 639 resin. The columns, designated as lead and lag, each had an inside diameter of 1.45 cm and a height of 30 cm. The columns were loaded in series, but were eluted and then regenerated separately. The average technetium loading for the cycles was 250 BV at 10 percent breakthrough. There was no significant difference in the loading performances among the five cycles. The percent removal of 99Tc was greater than 99.94 percent and the average decontamination factor (DF) was ...
2004-02-27
Energy Technology Data Exchange (ETDEWEB)
Gallium is present in surplus weapons-grade plutonium (WG-Pu) at a concentration of approximately 1 wt %. Plans are to dispose of surplus WG-Pu by converting it to UO{sub 2}-PuO{sub 2} mixed oxide (MOX) fuel and irradiating it in commercial power reactors. However, the presence of high concentrations of gallium in plutonium poses a potential corrosion problem during the process of MOX fuel irradiation. The batch experiments performed in this study were designed to measure the capability of the PUREX solvent extraction process to separate gallium from plutonium under idealized conditions. Radioactive tracing of the gallium with {sup 72}Ga enabled the accurate measurement of low concentrations of extractable gallium. The experiments approximated the proposed flowsheet for WG-Pu purification, except that only one stage was used for each process: extraction, scrubbing, and stripping. The gallium decontamination factor (DF) obtained after one extraction stage was about ...
2000-07-01
Kinetic aspects of the photolysis of in-station airborne methyl iodide
International Nuclear Information System (INIS)
A method for converting organic iodides to elemental iodine would be advantageous in improving the performance of charcoal filters for the removal of radio iodines from reactor off gases. A photochemical method has been developed. The HAVCHM code was used to establish the relevant process time scales on a complete set of rate equations describing the primary and secondary reactions occurring in a plug-flow reactor containing low levels of elemental iodine and methyl iodide in air, which is irradiated by intense u.v. light. These simulations were used to justify the contraction of the complete set of reactions to the most significant elementary processes. The contracted set of rate equations are then solved analytically to render the concentration-time profiles of methyl iodide, total inorganic iodine and total oxidized organics, consistent with the achievement of a desirable radioiodine decontamination factor. For the short contact times available, the flux of ...
International Nuclear Information System (INIS)
The Swedish State Power Board has together with Nukem, Hanau, West-Germany carried out pyrolysis o powder resins in a pilot plant with a capacity of about 30 kg/hr. The pyrolysis reactor with its afterburner and offgas scrubber system has been operated under steady state condition. About 2200 kg resins have been pyrolysed under November-December 1983 and the decontamination factor for Cs has been measured. Solidification of the residues from the pyrolysis reactor and scrubber water solutions has been carried out and various recipes with cement have been tested. The pyrolysis process has high decontamination factors and no offgas problems as the operating temperature of the reactor is Low. The residues from the reactor are chemically dead and can not cause swelling problems. Compared with a normal cementation process the final waste volume will be reduced with a factor of 4 if also the scrubber water after neutralization is solidified. The ...
International Nuclear Information System (INIS)
To reduce the volume of radioactive wastes after evaporation, activity carriers can be separated from the inactive salt load. Boric acid separation from PWR concentrates was considered a preliminary stage for nuclide precipitation. In connection with the precipitation process, the reaction conditions for boric acid separation were determined by bench-scale experiments. After evaluating the known purification processes, crystallization was suggested as a practicable method. After inactive bench-scale experiments, mixed crystal formation with iron hexacyanoferrate for Cs removal was chosen. The disturbing effect of the complexing agents was neutralized by a pre-dose of iron-III-salts. By specifying the precipitation conditions, for Cs-134 an activity separation from 3,0 E + 06 Bg/l to 1,9 E + 02 Bg/l, and for Cs-137 from 5,9 E + 06 Bg/l to 1,2 E + 02 Bg/l was achieved. Accordingly, the decontamination factor for Cs-134 was 16000, and for Cs-137 48000. For the ...
Decontamination factor of air filter against /sup 198/Au aerosol particles
Energy Technology Data Exchange (ETDEWEB)
DF (decontamination factor) of two types of air filter was investigated against /sup 198/Au aerosol particles with AMAD (activity median aerodynamic diameter) = 1.2 ..mu..m and sigmag (geometric standard deviation) = 2.0. One of the filters, SO filter, is HEPA (high efficiency particulate air) filter media with 46 mmphi, and the other is HE-40T (cellulose-glass fiber filter for dust sampling) filter media with 40 mmphi. DF of the SO filter was found to be over 5 x 10/sup 4/ at air flow rate of 1 lmin. And DF of HE-40 T filter was determined to be 94+-4 at the same airflow rate. In the multistage HE-40 T filter system, DF decreased at each succeeding stage. It was confirmed by numerical simulation that the decrease of DF was not inconsistent with the decrease of collection performance in each successive filter. It was also confirmed that DF could be predicted by the numerical simulaiton, if particle penetration function of filter and size distribution function of ...
1987-12-01
Decontamination factor of air filter against "1"9"8Au aerosol particles
International Nuclear Information System (INIS)
DF (decontamination factor) of two types of air filter was investigated against "1"9"8Au aerosol particles with AMAD (activity median aerodynamic diameter) = 1.2 #mu#m and #sigma#g (geometric standard deviation) = 2.0. One of the filters, SO filter, is HEPA (high efficiency particulate air) filter media with 46 mm#phi#, and the other is HE-40T (cellulose-glass fiber filter for dust sampling) filter media with 40 mm#phi#. DF of the SO filter was found to be over 5 x 10"4 at air flow rate of 1 l/min. And DF of HE-40 T filter was determined to be 94#+-#4 at the same airflow rate. In the multistage HE-40 T filter system, DF decreased at each succeeding stage. It was confirmed by numerical simulation that the decrease of DF was not inconsistent with the decrease of collection performance in each successive filter. It was also confirmed that DF could be predicted by the numerical simulaiton, if particle penetration function of filter and size distribution function of ...
Collection efficiency and decontamination factor of HEPA filter
International Nuclear Information System (INIS)
It is very important in a nuclear air cleaning system that HEPA (High Efficiency Particulate Air) filter is for reduction of releasing amounts of airborne radioactive particles. HEPA filter, by definition, has a minimum collection efficiency of 99.97 % for 0.3 #mu#m particles. However, DF (Decontamination Factor), which is necessary for safety management, can not be directly derived from the efficiency. And the current standard defined for 0.3 #mu#m particles has no scientific justification, because it has been found that the most penetrating particle size through HEPA filter is not always 0.3 #mu#m. In the present paper, a numerical experiment was made in order to estimate a relationship between DF and the efficiency. And new standard, in which the minimum DF is able to be easily obtained, was proposed. In the multistage filtration system, it was found that lower values of DF was possible to be experimentally indicated in the second and the third stages, even if ...
CTH-process for HLLW treatment. Pt. 2
Energy Technology Data Exchange (ETDEWEB)
The results from a hot test, using authentic HLLW solution, of the CTH actinide separation process are reported. The process consists of three solvent extraction cycles for separation of actinides and technetium from reprocessing high level liquid waste, utilizing HDEHP, TBP, and HDEHP in sequence, and an optional step for sorption on inorganic ion exchangers of the fission product content in the process raffinate. In general the process worked according to predictions but a malfunctioning feed pump gave a 10% loss of Pu to one stream. The hot test indicating that U and Pu can be recovered with losses below 0.1% and Am, Cm with a loss below 0.2%. Np and Tc were difficult to follow because of the low activity of /sup 237/Np and because /sup 99/Tc is a pure beta emitter, but the results indicate that also these elements behaved according to predictions, i.e., that recoveries >= 99.8% for Np and >= 97% for Tc can be achieved. For the HLLW stream the solvent extraction process gave a ...
1984-01-01
Acceptable requirement of decontamination factor for LLW disposal of PEACER pyro-processing wastes
International Nuclear Information System (INIS)
A pyrochemical process has been introduced and utilized so that the transmutation of spent PWR fuel in PEACER can produce mainly low and intermediate level waste for near surface disposal. Major radioactive nuclides from PEACER pyro-processing are composed of TRU and LLFP. In this study, the requirement for the final waste from PEACER is evaluated based on the methodology for establishment of waste acceptance criteria. Also, sensitivity analysis for several input parameters is conducted in order to determine acceptable decontamination factor (DF) and LLFP removal efficiency and to find out input parameter that extremely have an effect on DF. As a result of the study, LLFP removal efficiency, especially Sr-90 and Tc-99, is proved to be a major nuclide which contributes to annual dose by human intrusion scenario rather than TRU DF. More than 98.5% of LLFP have to be removed to meet below dose constraint within the DF more than 5.0E+03. Besides, because of the ...
2007-09-09
Acceptable decontamination factor for near-surface disposal of PEACER wastes
Energy Technology Data Exchange (ETDEWEB)
A pyrochemical process has been introduced and utilized so that the transmutation of spent PWR fuel in PEACER can produce mainly low and intermediate level waste for near surface disposal. Major radioactive nuclides from PEACER pyroprocessing are composed of TRU and LLFP. In this study, the requirement for the final waste from PEACER is evaluated based on the methodology for establishment of waste acceptance criteria. Also, sensitivity analysis for several input parameters is conducted in order to determine acceptable decontamination factor (DF) and LLFP removal efficiency and to find out input parameter that extremely have an effect on DF. As a result of the study, LLFP removal efficiency, especially Sr-90 and Tc-99, is proved to be a major nuclide which contributes to annual dose by human intrusion scenario rather than TRU DF. More than 98.5% of LLFP have to be removed to meet below dose constraint within the DF more than 5.0E + 03. Besides, because of the ...
2005-11-15
Acceptable decontamination factor for near-surface disposal of PEACER wastes
International Nuclear Information System (INIS)
A pyrochemical process has been introduced and utilized so that the transmutation of spent PWR fuel in PEACER can produce mainly low and intermediate level waste for near surface disposal. Major radioactive nuclides from PEACER pyroprocessing are composed of TRU and LLFP. In this study, the requirement for the final waste from PEACER is evaluated based on the methodology for establishment of waste acceptance criteria. Also, sensitivity analysis for several input parameters is conducted in order to determine acceptable decontamination factor (DF) and LLFP removal efficiency and to find out input parameter that extremely have an effect on DF. As a result of the study, LLFP removal efficiency, especially Sr-90 and Tc-99, is proved to be a major nuclide which contributes to annual dose by human intrusion scenario rather than TRU DF. More than 98.5% of LLFP have to be removed to meet below dose constraint within the DF more than 5.0E + 03. Besides, because of the ...
2005-11-01
ALARA{trademark} 1146 strippable coating
Energy Technology Data Exchange (ETDEWEB)
Strippable or temporary coatings are innovative technologies for decontamination that effectively reduce loose contamination at low cost. These coatings have become a viable option during the deactivation and decommissioning of both US Department of Energy (DOE) and commercial nuclear facilities to remove or fix loose contamination on both vertical and horizontal surfaces. The ALARA{trademark} 1146 strippable coating was demonstrated as part of the Savannah River Site LSDDP and successfully removed transferable (surface) contamination from multiple surfaces (metal and concrete) with an average decontamination factor for alpha contamination of 6.68 and an average percentage of alpha contamination removed of 85.0%. Beta contamination removed was an average DF of 5.55 and an average percentage removed of 82.0%. This paper is an Innovative Technology Summary Report designed to provide potential users with the information they need to quickly ...
1999-12-17
A study on the treatment of radioactive liquid wastes using synthetic by air intake system
International Nuclear Information System (INIS)
In this study based on the mass transfer theory, experiments for the evaporation rates depending on various conditions were carried out through the operation of the existing Natural Evaporation Facility in KAERI. Evaporation media were made of the cotton and polyester. Air circulation in the facility was forced by exhausting fans. The evaporation rate and the decontamination factor were calculated by the result of experiment. The evaporation rate increased as the flow rate of air supply, the feed rate of liquid waste, and the temperature of supplied air increased. As for the humility of supplied air, the evaporation rate was getting higher as the humidity was getting lower. As the result of this study, operation conditions of the Natural Evaporation Facility are optimized as follows; The air temperature above 8C .deg., the air humidity below 70%, the air flow rate 1.14-1.47 m/sec, and the liquid waste feed rate 4.6l/hr.m"2. The decontamination ...
2003-11-27
Thermal treatment of dusts from non ferrous metallurgical industries
Energy Technology Data Exchange (ETDEWEB)
Three samples of dusts generated by the non ferrous metallurgical industries are treated between 200 and 800 degree centigree in controlled oxidizing and reducing atmospheres. The objective of this study is to recover the valuable metals from these wastes. The treatments of these solids under oxidizing conditions at 700 degree centigree are well adapted for two samples. The totality of valuable elements are concentrated in the treatments residues. The use of hydrogen at 600 degree centigree, permits the removal of up to 100 % of valuable metals contained in the treated industrial wastes. The recovery rate of valuable metals (Pb, Zn, Cu) as well as the Global Decontamination Factor are reported. (Author) 9 refs.
2000-07-01
Technical area status report for chemical/physical treatment. Volume 2, Appendices
Energy Technology Data Exchange (ETDEWEB)
These Appendices describe various technologies that may be applicable to the Mixed Waste Treatment Plant (MWTP) Chemical/Physical Treatment System (CPTS). These technologies were identified by the CPTS Technical Support Group (TSG) as potentially applicable to a variety of separation, volume reduction, and decontamination requirements. The purpose was to identify all available and developing technologies, and their characteristics, for subsequent evaluation for specific requirements identified for the CPTS. However, the technologies described herein are not necessarily all inclusive, nor are they necessarily all applicable.
1993-08-01
Quality engineering and control. Semiannual progress report, May-October 1979
International Nuclear Information System (INIS)
The following are reported: colorimetric determination of Ti in Cr, decontamination of metals by anodic dissolution, computer code for x-ray peak identification, gel-permeation chromatography of CoRezyn 1664 polyester resin, infrared monitoring of gases and vapors, particle size analysis of dusts, nondestructive analysis of Oralloy for removable alpha contamination, dissolution (digestion) of high-fired oxides, assay of U in a Pu-U alloy, measurement of oxide thickness on Pu metal by x-ray diffraction, analysis of precipitated Pu peroxide, differentiation of Dowex SBR and 11 resins, and determination of Pu solubility in simulated lung fluid.
Production of the radioisotope "8"8Y
International Nuclear Information System (INIS)
Carrier-free "8"8Y radioisotope, which has the longest half life (T=106.6 d) of yttrium radioisotopes and is a #gamma#-ray emitter, was obtained by proton irradiation of strontium, followed by cooling for one month. Then, "8"8Y was purified by precipitating strontium as strontium nitrate and extracting yttrium with tri-n-butyl phosphate (TBP). The decontamination factor of strontium to yttrium was more than 4x10"3 and chemically pure yttrium radioisotope was obtained. (author) 6 refs.
International Nuclear Information System (INIS)
The use of finely powdered ion exchange resins improve loading of specific ion exchange materials with better performance but as such these materials are not suitable for column operation. However, by proper selection of ion exchange support medium, it is possible to get better product. The radioactive solution can be treated by suspending this material, stirring and allowing to settle. The present method gives DF in the range of 70 - 80 even after repeated use as compared to DF in the range of 5 to 10 by single conventional chemical treatment process. (author)
2001-02-07
In-place testing of HEPA filter systems by the single-particle, particle-size spectrometer method
Energy Technology Data Exchange (ETDEWEB)
This standard describes the procedure and equipment for in-place testing of HEPA filter systems by the single-particle, particle-size (SPPS) spectrometer method. This method provides the capability for evaluating the effectiveness (i.e., decontamination factor or DF) of systems consisting of one or more stages of HEPA filters against submicrometer aerosols in discrete particle-size ranges. It is particularly useful for testing of multi-stage HEPA filter installations and for testing of very large (50,000 cfm installed capacity) single-stage systems where it is desired to minimize the quantity of challenge aerosol required.
1981-12-01
Entrained Solids, Strontium-Transuranic Precipitation, and Crossflow Filtration of AN102 Small C
Energy Technology Data Exchange (ETDEWEB)
This work is the first active crossflow filter testing of the new strontium-permanganate process for Envelope C at the Savannah River Technology Center. Extreme filtration difficulties with the ferric hydroxide precipitation led to investigations of other chemistries with simulants. The current process includes the isotopic dilution by precipitation from inactive strontium nitrate addition. A permanganate strike to replace ferric reagents was found to provide practical filterability and good lanthanide or transuranic decontamination. That work had been supported with simulant and active beaker testing.
2000-09-27
Demonstration experiment on improved radwaste evaporator
Energy Technology Data Exchange (ETDEWEB)
High conductivity liquid waste, which is produced in nuclear power plants, is now processed with radwaste evaporator. The concentrated liquid waste in the evaporator is so highly radioactive and corrosive that the improvement on maintenability and reduction of exposure dose rate are desirable as well as high decontamination factor (DF). Fuji Electric constructed the improved experimental facility of evaporator and carried out an experiment to demonstrate DF, maintenability and controllability of system. As the results, DF, maintenability and controllability were proved to be excellent and its applicability to nuclear power plant was well established.
1988-07-01
Aqueous radioactive waste bituminization
International Nuclear Information System (INIS)
The bituminzation of decontamination and ion exchange resin stripping wastes with four grades of asphalt was investigated to determine the effects of asphalt type on the properties of the final products. All waste forms deformed readily under light loads indicating they would flow if not restrained. It was observed in all cases that product leaching rates increased as the hardness of the asphalt used to treat the waste increased. If bituminization is adopted for any Ontario Hydro aqueous radioactive wastes they should be treated with soft asphalt to obtain optimum leaching resistance and mechanical stability during interim storage should be provided by a corrosion resistant container.
5049-01-01
Energy Technology Data Exchange (ETDEWEB)
The UFIP (French Petroleum Industry Association) studies concerning polluted sites and soils and their rehabilitation are presented: characterization of the admissible maximum fuel or gas oil content in the ground, the issue of time effects, and the risks it may induce for public health; study on the various pollutant impacts on the environment (underground waters, biotope...); approach to the development of a dynamical model describing these phenomena and their influence on man, in order to derive consistent and reasonable decontamination objectives
1996-12-31
A two-cycle process for enhanced actinide separation from radioactive liquid wastes
Energy Technology Data Exchange (ETDEWEB)
A two-cycle process using O{Phi}CMPO and HDEHP as extractants to achieve an alpha decontamination factor of HLLW greater than 10{sup 3} together with a reduction of the lanthanides/americium weight ratio by a factor of about 200 is considered. Experimentally measured distribution ratios have been employed as input data of a suitable computer code to define operating conditions and M/S stage numbers of a process flow-sheet able to meet the above-mentioned objectives.
1996-09-01
Energy Technology Data Exchange (ETDEWEB)
Corrective Action Unit (CAU) No. 92, the Area 6 Decontamination Pond Facility (DPF), is an historic disposal unit located at the Nevada Test Site (NTS) in Nye County, Nevada (Figures 1 - 1, 1-2, and 1-3). The NTS is operated by the U.S. Department of Energy, Nevada Operations Office (DOE/NV), which has been required by the Nevada Division of Environmental Protection (NDEP) to characterize the DPF under the requirements of the Resource Conservation and Recovery Act (RCRA) Part A Permit (NDEP, 1995) for the NTS and Title 40 Code of Federal Regulations (CFR) Part 265 (1996c). The DPF is prioritized in the Federal Facility Agreement and Consent Order (FFACO, 1996) but is governed by the permit. The DPF was characterized through sampling events in 1994, 1996, and 1997. The results of these sampling events are contained in the Final Resource Conservation and Recovery Act Industrial Site Environmental Restoration Site Characterization Report, Area 6 ...
1997-10-01
Removal of radioactive ions from nuclear waste solutions by electrodialysis
International Nuclear Information System (INIS)
Removal of radioactive ions was studied from low and medium level radioactive waste solutions by electrodialysis using ion exchange membranes. The test solutions contained "1"3"7Cs"+, "1"0"6Ru"3"+ or fission products (F.P.) as active ions and NaCl, Na_2SO_4 or Ca(NO_3)_2 as inactive coexisting salts. The decontamination factor of the active ions was in the order: "1"3"7Cs"+ (greater than 99%) > "9"0Sr"2"+ > F.P. > "1"0"6Ru"3"+. The dialysis time required to attain the saturation was the shortest for monovalent cations K"+, Cs"+ and Na"+, intermediate for divalent cation Sr"2"+, and the longest for trivalent cation Ru"3"+. The ratio of the decontamination factor of an active ion eta sub( a) to the desalination factor of an inactive ion eta sub( b) was nearly equal to unity for "2"4Na, "4"2K, "1"3"7Cs and "9"0Sr. On the other hand, the apparent selective permeability of an active ion (A"+) against Na"+ ion, T sub(Na"+) sup( a) was higher ...
Energy Technology Data Exchange (ETDEWEB)
Potential maximum radiation dose rates over a 1,000-year time horizon were calculated for exposure to the decontaminated concrete removed from the 183-H Solar Evaporation Basins at the Hanford Site, Richland, Washington. The RESRAD computer code, Version 5.62, which implements the methodology described in the US Department of Energy`s manual for developing residual radioactive material guidelines, was used in this evaluation. Currently, the concrete is not being used. Four potential exposure scenarios were developed for the land area where the decontaminated concrete will be stored. In Scenario A industrial use of the land is assumed; in Scenario B recreational use of the land is assumed; in Scenario C residential use of the land is assumed; and in Scenario D (a plausible but unlikely land-use scenario), the presence of a subsistence farmer in the immediate vicinity of the land is assumed. For Scenarios A and B, water used for drinking is ...
1997-01-01
Present status of study on reduced-moderation water reactors
Energy Technology Data Exchange (ETDEWEB)
The Reduced-Moderation Water Reactor (RMWR) is a next generation water-cooled reactor, based on the experienced light water reactor (LWR) technology, aiming at effective utilization of uranium resources, high burn-up and long operation cycle and plutonium multiple recycling. These characteristics can be achieved by the high conversion ratio from {sup 238}U to {sup 239}Pu resulted from the higher neutron energy spectrum in comparison to conventional LWRs. Considering the extension of LWR utilization, Japan Atomic Energy Research Institute (JAERI) started the research on it in 1997 and then started a collaboration in the conceptual design study with the Japan Atomic Power Company (JAPC) in 1998, under technical cooperation with three Japanese reactor vendors. In the core design study of the RMWR, several basic core designs with the high conversion ratio more than 1 and the negative void reactivity coefficient have been proposed, and then, subsequent investigation on the effects of ...
2001-09-01
International Nuclear Information System (INIS)
To demonstrate that the caustic-side solvent extraction (CSSX) process could remove cesium from Savannah River Site (SRS) high-level waste over long periods of time, an improved minicontactor (2-cm centrifugal contactor) was needed that could be operated for several days. In particular, the contractor temperature had to be controlled and contactor hydraulic performance needed to be improved. Because the process was to be continuous, provisions were made for a three-shift operation. With the improvements made and the operators trained, the CSSX process was run in a 33-stage minicontactor over a period of three days to remove cesium from an average SRS siumulant for the waste feed. The two key process goals were achieved: (1) the cesium was removed from the waste with decontamination factors greater than 40,000 and (2) the recovered cesium was concentrated by a factor of 15 in dilute nitric acid. These goals were maintained for 71 h as 1.4 L of solvent was recycled ...
Experiences in radioactive gaseous effluent management in JAERI
International Nuclear Information System (INIS)
In the Japan Research Reactor-II (JRR-2), the main source of _4_1Ar generation is the exhaust air from the horizontal experimental holes and the pneumatic tubes. For the horizontal experimental holes, the flow of exhaust air through the holes was decreased by improving the airtightness, and a decay duct of capacity 2.4 m_3 was installed in the middle of the exhaust line. In consequence, the release rate of _4_1Ar was reduced by 6-8%. For the pneumatic tubes, a mechanical shutter was installed in the tube. The shutter stops the exhaust air flow, except when the pneumatic tube is used. Prior to the use, the activated air in the tube is led to a decay tank. As a result, the _4_1Ar release rate was reduced by 10-20%. By the above means, the yearly exposure at the site boundary was reduced to 0.36 mR from 2.6 mR. In Hot Laboratory for metallurgical examination of spent fuel, the exhaust filtration system consists of filters in the cave, i.e. frame trap, prefilter, HEPA filter, and the main ...
1983-05-01
Thermal conductivity of sintered lithium orthosilicate compacts
British Library Electronic Table of Contents (United Kingdom)
The design of solid breeder blankets is strongly affected by the low values of thermal conductivity and density of ceramic breeder pebble beds. A significant rise of both quantities would enhance the thermal performance and lead to an increased tritium breeding ratio. In order to improve these quantities pretreated lithium orthosilicate pebble material was dry pressed and subsequently sintered. The thermal conductivity of cylindrical pellets was determined by the heat pulse method using a laser flash device. A pebble bed characteristic sample was also investigated in order to check the measurement accuracy in comparison with previous results. Furthermore, two samples of low density cellular ceramics were also prepared by infiltration of polymer foams with a ceramic slurry. The thermal cond...
2009-01-01
TIG of Reduced Activation Ferrite/Martensitic Steel for the Korean ITER-TBM
International Nuclear Information System (INIS)
Test Blanket Modules (TBM) will be tested in ITER to verify the capability of tritium breeding and recovery and the extraction of thermal energy suitable for the production of electricity. A Helium Cooled Solid Breeder (HCSB) TBM has been developed in Korea to accomplish these goals. Reduced Activation Ferritic/Martensitic (RAFM) steel has been chosen as the primary candidate structural material for Korean TBM. Due to the complexity of the First wall (FW) and Side wall (SW), it is necessary to develop various joining technologies, such as Hot Isostatic Pressing (HIP), Electron Beam Welding (EBW) and Tungsten Inert Gas (TIG) welding, for the successful fabrication of TBM. In this study, the mechanical properties of TIG welded RAFM steel were investigated. Various mechanical tests of TIG-welded RAFM steel were performed to obtain the optimized TIG welding process for RAFM steel
2010-10-01
Energy Technology Data Exchange (ETDEWEB)
We find dosage of gamma emitters radionuclides of samples collected in the environment of the Chinon nuclear power plant for 2002 and 2003, these results are presented in two tables: concentrations in gamma emitter radionuclides of samples collected in the terrestrial environment (soils) and aquatic environment (sediments) of the site of Chinon in june 2002 in the frame of the annual surveillance, the second table concerns the concentrations in gamma emitter radionuclides of samples collected in the terrestrial environment (soils and lichens) of the site of Chinon in may 2003 in the frame of the annual surveillance. We find also the dosage of free tritium in the water of the Loire river for 2002 and 2003, upstream and downstream to the power plant of Chinon. (N.C.)
2003-07-01
Parameter study of the LIFE engine nuclear design
British Library Electronic Table of Contents (United Kingdom)
LLNL is developing the nuclear fusion based Laser Inertial Fusion Energy (LIFE) power plant concept. The baseline design uses a depleted uranium (DU) fission fuel blanket with a flowing molten salt coolant (flibe) that also breeds the tritium needed to sustain the fusion energy source. Indirect drive targets, similar to those that will be demonstrated on the National Ignition Facility (NIF), are ignited at 13Hz providing a 500MW fusion source. The DU is in the form of a uranium oxycarbide kernel in modified TRISO-like fuel particles distributed in a carbon matrix forming 2-cm-diameter pebbles. The thermal power is held at 2000MW by continuously varying the 6Li enrichment in the coolants. There are many options to be considered in the engine design including target yield, U-to-C ratio in th...
2010-01-01
PROSPECTS AND STATUS OF LOW-ASPECT-RATIO TOKAMAKS
Energy Technology Data Exchange (ETDEWEB)
The prospects for the low-aspect-ratio (A) tokamak to fulfill the requirements of viable fusion power plants are considered relative to the present status in data and modeling. Desirable physics and design features for an attractive Blanket Test Facility and power reactors are estimated for low-A tokamaks based on calculations improved with the latest data from small pioneering experiments. While these experiments have confirmed some of the recent predictions for low-A, they also identify the remaining issues that require verification before reliable projections can be made for these deuterium-tritium applications. The results show that the low-A regime of small size, modest field, and high current offers a path complementary to the standard and high A tokamaks in developing the full potential of fusion power.
1995-01-01
Mechanical design of a PERMCAT reactor module
International Nuclear Information System (INIS)
The PERMCAT is a membrane reactor proposed for processing fusion reactor plasma exhaust gas: tritium removal is obtained by isotopic swamping operating in counter-current mode. In this work, a membrane reactor using a permeator tube of length about 500 mm produced via diffusion welding of Pd-Ag thin foils is described. An appropriate mechanical design of the membrane module has been developed in order to avoid any significant compressive and bending stresses on the very long and thin wall permeator tube: two expanded bellows have been applied to the Pd-Ag tube, so that it has been pre-tensioned before operating. The elongation of the metal permeator under hydrogenation has been theoretically estimated and experimentally verified for properly designing the membrane reactor.
2007-02-01
Measurement of induced radioactivity in materials found around a neutron generator
The induced radioactivity in the construction materials of a Cockcroft-- Walton type neutron generator was measured. Major activation products (/sup 24/ Na, /sup 28/Al, /sup 56/Mn, /sup 64/Cu, /sup 65/Ni, /sup 69m/Zn, /sup 88/Rb /sup 91/Sr /sup 101/Mo, /sup 187/W/ and resulting doses are tabulated. Results show that the highest gamma activities would be observed in the fluorescent bulbs, copper pipe, aluminum lattice rod, and the aluminum pipe clamp. Thermoluminescent dosimeter readings yield the highest doses for the copper pipe tee, copper pipe, and aluminum lattice rod. Results of measuremerts of the neutron and gamma dose profiles of the facility are shown. However the indication is clearly that the tritium target, compared to other components, is the major source of radiation both during and after shutdown. (UK)
1974-01-01
Learning and case-based reasoning for faults diagnosis-aiding in nuclear power plants
International Nuclear Information System (INIS)
The aim of this thesis is the design of a faults diagnosis-aiding system in a nuclear facility of the Cea. Actually the existing system allows the optimization of the production processes in regular operating conditions. Meanwhile during accidental events, the alarms, managed by threshold, are bringing no relevant information. To increase the reliability and the safety, the human operator needs a faults diagnosis-aiding system. The developed system, SECAPI, combines problem solving techniques and automatic learning techniques, that allow the diagnosis and the the simulation of various faults happening on nuclear facilities. Its reasoning principle uses case-based and rules-based techniques. SECAPI owns a learning module which reads out knowledge connected with faults. It can then simulate various faults, using the inductive logical computing. SECAPI has been applied on a radioactive tritium treatment operating channel, at the Cea with good results. (A.L.B.)
1998-01-01
HYFIRE: a tokamak- high-temperature electrolysis system
Energy Technology Data Exchange (ETDEWEB)
Brookhaven National Laboratory is involved in a conceptual design study of a commercial nuclear power system which utilizes high-temperature electrolysis to produce synthetic fuels. The system is called HYFIRE. It includes a tokamak fusion power reactor supplying electrical and thermal energy to an array of electrolytes. The electrolytes produce hydrogen which can be used either directly as a fuel or in the production of hydrocarbons. The purpose of the study is to provide a mechanism for DOE to further assess the commercial potential of fusion using a tokamak reactor to produce synthetic fuel. The HYFIRE design is based on the tokamak commercial power reactor, STARFIRE. STARFIRE uses the deuterium/tritium/lithium fuel cycle. The HYFIRE study assumes the plasma shape and characteristics of STARFIRE study but uses a different blanket design. This study is particularly interested in the possibility of using the STARFIRE tokamak in the production of synthetic fuels.
1980-01-01
International Nuclear Information System (INIS)
The nuclear complex in Tarapur, Maharashtra is a multi facility nuclear site comprising of power reactors and research facilities. Each facility has independent liquid effluent discharge line to Arabian Sea. Experimental studies were conducted to evaluate dilution factors in the aquatic environment using liquid effluent releases as tracer from one of the facilities. 3H and 137Cs radioisotopes present in the routine releases were used as simulated tracer nuclides. The dilution factors(D.F) observed for tritium were in the range of 20-20000 in a distance range of 10 m to 1500 m respectively and for 137Cs the D.F. were in the range of 50 to 900 over a distance range of 10-200 m. The paper describes the analytical methodology and sampling scenarios and the results of dilution factors obtained for Tarapur aquatic environment. (author)
2007-06-05
Calorimetric sensors for energy deposition measurements
Energy Technology Data Exchange (ETDEWEB)
A calorimetric sensor with several novel design features has been developed. These sensors will provide an accurate sampling of thermal power density and energy deposition from proton beams incident on target components of accelerator-based systems, such as the Accelerator Production of Tritium Project (APT) and the Spallation Neutron Source (SNS). A small, solid slug (volume = 0.347 cc) of target material is suspended by kevlar fibers and surrounded by an adiabatic enclosure in an insulating vacuum canister of stainless steel construction. The slug is in thermal contact with a low-mass, calibrated, 100-k{Omega} thermistor. Power deposition caused by the passage of radiation through the slug is calculated from the rate of temperature rise of the slug. The authors have chosen slugs composed of Pb, Al, and LiAl.
1998-12-31
Energy Technology Data Exchange (ETDEWEB)
It is planned to bulk-heat a unit cell of a fusion reactor solid-breeder blanket in a fission reactor to study thermo-mechanical and thermal-hydraulic properties of fusion blankets. This study investigates the neutronic feasibility of using the Power Burst Facility (PBF) for this purpose. Heating rates were calculated for a Li/sub 2/O experiment placed in the PBF test space. The ANISN code and a 56-group coupled neutron-gamma library based on FLUNG and VITAMIN C were used to compute the heating rates. The results show that an average heating rate level of 1-3 W/cc can be produced in PBF with a local power profile that should be typical of a fusion blanket unit cell.
1982-11-01
ARIES-AT safety design and analysis
British Library Electronic Table of Contents (United Kingdom)
ARIES-AT is a 1000MWe conceptual fusion power plant design with a very low projected cost of electricity. The design contains many innovative features to improve both the physics and engineering performance of the system. From the safety and environmental perspective, there is greater depth to the overall analysis than in past ARIES studies. For ARIES-AT, the overall spectrum of off-normal events to be examined has been broadened. They include conventional loss of coolant and loss of flow events, an ex-vessel loss of coolant, and in-vessel off-normal events that mobilize in-vessel inventories (e.g., tritium and tokamak dust) and bypass primary confinement such as a loss of vacuum and an in-vessel loss of coolant with bypass. This broader examination of accidents improves the robustness of ...
2006-01-01
Thermal release of volatile fission products from irradiated nuclear fuel
International Nuclear Information System (INIS)
An effective procedure for removing _3H, Xe and Kr from irradiated fuels was demonstrated using Shippingport UO"2 fuel. The release characteristics of _3H, Kr, Xe, and I from irradiated nuclear fuel have been determined as a function of temperature and gaseous environment. Vacuum outgassing and a flowing gas stream have been used to vary the gaseous environment. Vacuum outgassing released about 99% of the _3H and 20% of both Kr and Xe within a 3 h at 1500_0C. Similar results were obtained using a carrier gas of He containing 6% H"2. However, a carrier gas containing only He resulted in the release of approximately 80% of the _3H and 99% of both Kr and Xe. These results indicate that the release of these volatile fission products from irradiated nuclear fuel is a function of the chemical composition of the gaseous environment. The rate of tritium release increased with increasing temperature (1100 to 1500_0C) and with the addition of hydrogen to the gas stream. ...
Incorporation of tritium into body constituent molecules
International Nuclear Information System (INIS)
Incorporation of tritium into body constituent molecules from tritiated water and its in vivo behaviors were studies using rats. In single administration of HTO, "3H behaviors were studied in lipids that are rich in hydrogen. Incorporation of "3H into the lipid fraction from HTO and its release differed by each organ and by the type of lipid components. Of routes of administration, the oral and parenteral routes showed same results, and no prominent difference was noted by inhalation. By consecutive administration, the urine "3H concentration showed no difference according to the route, but increased as the concentration of administered HTO increased. When administration was discontinued after the urine "3H concentration reached a plateau, the biological half-life was about 4.5 days, almost in agreement with the value by single administration. In relation to water intake, increase in the urine volume and accompanying promotion of urine "3H excretion in approximate ...
1981-12-03
ITER Core Imaging X-Ray Spectrometer Conceptual Design and Performance Assessment - Phase 2
International Nuclear Information System (INIS)
During Phase 2 of our study of the CIXS conceptual design we have tackled additional important issues that are unique to the ITER environment. These include the thermal control of the crystal and detector enclosures located in an environment with a 100-250 C ambient temperature, tritium containment, and the range of crystal and detector movement based on the need for spectral adjustments and the desire to make measurements of colder plasmas. In addressing these issues we have selected a ''Dewar''-type enclosure for the crystals and detectors. Applying realistic view factors for radiant heat and making allowance for conduction we have made engineering studies of this enclosure and showed that the cooling requirements can be solved and the temperature can be kept sufficiently constant without compromising the specification parameters of the CIXS. We have chosen a minimum 3 mm combined thickness of the six beryllium windows needed in a Dewar-type enclosure and showed ...
Energy Technology Data Exchange (ETDEWEB)
Copper coatings deposited on Al-6061 substrates by radio frequency magnetron sputtering, to prevent the retention and permeation of energetically implanted tritium in Al-6061, were evaluated by a variety of characterization techniques. The coatings, weighing in the 0.03 to 0.088 kg/m{sup 2} range, were smooth and had a fine grain structure. They contained the intermetallic phases Cu{sub 9}Al{sub 4} and CuAl{sub 2} as well as copper. The fractions of Al and Cu in any coating increased and decreased, respectively, with increasing depth below the surface. Furthermore, the fractions of Al and Cu on the coating surface decreased and increased, respectively, with increasing coating weight. There was no texture or preferred orientation in the Cu phase of the coatings. A significant amount of oxygen was also detected at the original substrate surface. Residual stress measurements revealed that, in both Cu and CuAl{sub 2}, the stresses in the coating plane were compressive, ...
1999-08-01
Uptake of cesium and strontium by crystalline silicotitanates from radioactive wastes
British Library Electronic Table of Contents (United Kingdom)
Crystalline silicotitanate inorganic ion exchanger, with a sitinakite structure is candidate material for remediation of aqueous nuclear waste streams. The syntheses of crystalline silicotitanate (CST) and Nb-substituted crystalline silcotitanate (Nb-CST) were carried out under hydrothermal conditions and the products were characterized using techniques viz., XRD, SEM/EDS, DTA/TGA, surface area respectively. Batch experiments were carried out to study the kinetics of uptake of 137Cs and 90Sr, to estimate the decontamination factor (DF) values and distribution coefficients (K d) for the above synthesized CST and Nb-CST samples from actual radioactive waste solutions. The DF values for uptake of Cs and Sr by Nb-CST after 24?h of equilibration was 355 and 136 whereas for CST it was found to b...
2011-01-01
Transuranic separation using organophophorus extractants adsorbed onto superparamagnetic carriers.
Energy Technology Data Exchange (ETDEWEB)
Polymeric coated ferromagnetic carriers with an absorbed layer of octyl(phenyl)-N,N-diisobutylcarbamoylmethylphosphine oxide (CMPO) diluted by tributyl phosphate (TBP) are being evaluated for application in the separation and the recovery of low concentrations of americium, plutonium, and uranium from nuclear waste solutions. Due to their chemical nature, these extractants selectively complex americium and plutonium contaminants onto the particles and the complexed particles can be recovered from the solution using a magnet. Physical and chemical characterization of the extractant-absorbed particles were performed by gamma and liquid scintillation counting, scanning electron microscopic (SEM) micrograph, and other physical measurements. Plutonium, americium, and uranium separations have been performed at various HNO{sub 3} and HCl concentrations. Parameters were studied to determine the limitations and capacity of the process. The status of the chemistry and application of the process ...
1998-10-07
Thermoactivation of viruses by microwaves
Energy Technology Data Exchange (ETDEWEB)
Eight different viruses, suspended in drinking water, were examined for their ability to be inactivated by microwaves from a microwave oven. Up to a virus content of 10/sup 5/ TCID/sub 50//ml inactivation was successful within a few minutes of microwave treatment and occurred in parallel to the heat stability of the viruses. Evidence for direct effects of microwaves on viruses could not be detected. 7 of the viruses studied were inactivated rapidly when temperatures of 50 to 65/sup 0/C under microwave treatment were reached in the flowing water, while a bovine parvovirus was only inactivated by temperatures above 90/sup 0/C. The advantages of a thermal virus-decontamination of fluids and material by microwaves are discussed.
1981-01-01
Scientific report 1997; Rapport scientifique 1997
Energy Technology Data Exchange (ETDEWEB)
In this book are found technical and scientific papers on the main works of the Direction of the Fuel Cycle (DCC) in France. The study fields are: the up-side of the nuclear fuel cycle with theoretical studies (plasma simulation) and technological developments and instrumentation (lasers diodes, carbides plasma projection, carbon 13 enrichment); the down-side nuclear fuel cycle with theoretical studies (ion Eu{sup 3+} complexation simulation, decay simulation, uranium and plutonium diffusion study, electrolyser operating simulation), scenario studies ( recycling, wastes management), experimental studies; dismantling and cleaning (soils cleaning, surface-active agent for decontamination, fault tree analysis); analysis with expert systems and mass spectrometry. (A.L.B.)
1998-07-01
Natural radioactive materials in oil and gas industry
International Nuclear Information System (INIS)
Oil and gas production and processing operations sometimes cause naturally occurring radioactive materials (NORM) to accumulate at elevated concentrations in by-product waste streams. The sources of most of the radioactivity are isotopes of "2"3"8U and "2"3"2Th series, which are naturally present in the subsurface formations from which oil and gas are produced. NORM waste may cause problems in the operations of installations by plugging perforations, clogging tubular and valves then restricting flow. Therefore, plants or equipment have to be refurbished and decontaminated before reuse to avoid radioactive waste or surface contaminated object. There are two options for safe disposal of scale and sludge produced from NORM Descaling Facility : 1- Injection into an abandoned production well. 2- The construction of a near surface depository. These options are assumed to be environmental friendly disposal options. (author)
2010-03-01
MODELING AN ION EXCHANGE PROCESS FOR CESIUM REMOVAL FROM ALKALINE RADIOACTIVE WASTE SOLUTIONS
Energy Technology Data Exchange (ETDEWEB)
The performance of spherical Resorcinol-Formaldehyde ion-exchange resin for the removal of cesium from alkaline radioactive waste solutions has been investigated through computer modeling. Cesium adsorption isotherms were obtained by fitting experimental data using a thermodynamic framework. Results show that ion-exchange is an efficient method for cesium removal from highly alkaline radioactive waste solutions. On average, two 1300 liter columns operating in series are able to treat 690,000 liters of waste with an initial cesium concentration of 0.09 mM in 11 days achieving a decontamination factor of over 50,000. The study also tested the sensitivity of ion-exchange column performance to variations in flow rate, temperature and column dimensions. Modeling results can be used to optimize design of the ion exchange system.
2008-08-26
Selenium 79 is a beta emitter produced from (235)U fission and is one of the long half-life radionuclides of interest in nuclear waste disposal problematic because of its potential migration capacity to the surface environment. Measurement of (79)Se is particularly difficult due to its low activity in waste matrices (about 10(-3)Bqg(-1)). A radiochemical procedure based on ion exchange separations was already described in a previous paper. This work presents different applications of the radiochemical separation to waste samples and an improvement of this procedure, including a selective extraction of selenium as diethylselenium in an organic solvent followed by a re-extraction in aqueous medium. This additional step allows the decontamination factor to be increased with the aim of counting (79)Se by liquid scintillation counting. PMID:19071740
2007-01-14
Evaporation behavior of water and concentration of technetium and rhenium using thin film evaporator
International Nuclear Information System (INIS)
The nuclear energy cycle requires the recycling of nuclear fuel, water, chemical reagents, and the volume reduction of radioactive liquid wastes. A fundamental technique for continuous recovery of water using a thin-film evaporator was examined. Appropriate recovery measurements were: an evaporator heat temperature of 323 K, a feed rate of 0.23 cm"3 x s"-"1, a vacuum pressure of 15 mmHg (2 kPa), and impeller rotational speeds of 500#approx#600 rpm (min"-"1). The concentration of trace technetium and rhenium in aqueous solutions was also studied. A decontamination factor of 10"5 for rhenium was obtained. (author)
1999-06-01
Energy Technology Data Exchange (ETDEWEB)
With the issuance of the Decommissioning Rule (July 27, 1988), nuclear power plant licensees are required to submit to the US Regulatory Commission (NRC) for review, decommissioning plans and cost estimates. This user`s manual and the accompanying Cost Estimating Computer Program (CECP) software provide a cost-calculating methodology to the NRC staff that will assist them in assessing the adequacy of the licensee submittals. The CECP, designed to be used on a personnel computer, provides estimates for the cost of decommissioning PWR plant stations to the point of license termination. Such cost estimates include component, piping, and equipment removal costs; packaging costs; decontamination costs; transportation costs; burial costs; and manpower costs. In addition to costs, the CECP also calculates burial volumes, person-hours, crew-hours, and exposure person-hours associated with decommissioning.
1993-10-01
Energy Technology Data Exchange (ETDEWEB)
Normal butylamine compounds are studied as salt-free wash reagents for degraded solvent used in PUREX process in spent fuel reprocessing. The solvent wash tests were carried out with two types of butylamine compounds, n-butylamine oxalate and n-butylamine bicarbonate, by counter-current mode using a small size mixer-settler composed of two 4-stage wash steps. Di-n-butyl phosphoric acid (HDBP), the main degradation product from TBP, was removed from real degraded solvent with decontamination factor of 2.5 {approx} 7.9. The study on electrolytic decomposition of butylamine compounds was also conducted for waste treatment.
2003-02-27
Concentration of Melton Valley Storage Tank surrogates with a wiped film evaporator
Energy Technology Data Exchange (ETDEWEB)
This report describes experiments to determine whether a wiped film evaporator (WFE) might be used to concentrate low-level liquid radioactive waste (LLLW). Solutions used in these studies were surrogates that contain no radionuclides. The compositions of the surrogates were based on one of Oak Ridge National Laboratory`s (ORNL`s) Melton Valley Storage Tanks (MVSTs). It was found that a WFE could be used to concentrate LLLW to varying degrees by manipulating various parameters. The parameters studied were rotor speed, process fluid feed temperature and feed rate, and evaporator temperature. Product consistency varied from an unsaturated liquid to a dry powder. Volume reductions up to 68% were achieved. System decontamination factors were consistently in the range of 10{sup 4}.
1994-08-01
Energy Technology Data Exchange (ETDEWEB)
Decontamination and decommission activities related to the Molten Salt Reactor Experiment (MSRE) involve the trapping and recovery of radiolitically generated uranium hexafluoride and fluorine. Although fission product radiolysis was known to generate F{sub 2}, the formation of UF{sub 6} and its transport from the fuel salt was unexpected. Some of these gaseous radiolysis products have been moving through the gas piping to a charcoal bed since the reactor was shut down in 1969. Current and planned remediation and clean-up activities involve the trapping of the gaseous products, deactivation and treatment of the activated charcoal bed, stabilization and reconditioning of the fuel salt, and recovery of the uranium. The chemical aspects of these processes, including radiolytic generation mechanisms, reactions between uranium hexafluoride and fluorine and trapping materials such as activated charcoal, activated alumina, and sodium fluoride, along with the analytical ...
1996-10-01
Energy Technology Data Exchange (ETDEWEB)
The ventilation requirements for decontamination are normally determined with a static calculation method. In some cases, the pollutant emission is intermittent, for example in the car park of an office building, where all the cars enter and leave the place nearly at the same time. Generally, in such a case, the volume of the garage is large, consequently the time constant of the system has a high value. So a static approach would no longer stay accurate and a dynamic evaluation is needed. With the help of some assumptions, calculations remain rather simple and results can be plotted on nomographs or computed on a programmable handheld calculator. The amount of energy saved may appear very large in some cases. A sizing optimization will be required but also remains easy to compute. The paper presents the method of calculation for a single ventilation level and the optimization of a two-level ventilation.
1982-01-01
CLOSURE OF THE FAST FLUX TEST FACILITY (FFTF) HISTORY & STATUS & FUTURE PLANS
Energy Technology Data Exchange (ETDEWEB)
In 1993, the US Department of Energy (DOE) decided to shut down the Fast Flux Test Facility (FFTF) due to lack of national missions that justified the annual operating budget of approximately $88M/year. The initial vision was to ''deactive'' the facility to an industrially and radiologically safe condition to allow long-term, minimal surveillance storage until approximately 2045. This approach would minimize near term cash flow and allow the radioactive decay of activated components. The final decontamination and decommissioning (D and D) would then be performed using then-current methodology in a safe and efficient manner. the philosophy has now changed to close coupling the initial deactivation with final D and D. This paper presents the status of the facility and focuses on the future challenge of sodium removal.
2006-02-24
Britain's dirty deeds at Maralinga
Energy Technology Data Exchange (ETDEWEB)
Following the United Kingdom's nuclear tests at Maralinga in Australia in the 1960's, the Australian government signed away its rights to claim compensation for decontamination costs in a 1968 agreement. Controversy now rages as the Australian government is claiming pound33 million for this purpose from the United Kingdom to compensate the Maralinga Tjarutja for the loss of access to their traditional lands. They claim that the UK clean-up operation was inadequate and that much plutonium was spread over the land, rather than contained in pits. Measurements of contamination at the site were wrong by a factor of ten according to a 1984 visit when Australian scientists were horrified to realize that an Aboriginal child living near Taranaki could inhale more than 460 millisieverts a year. As ministers from both countries meet in June 1993 the debate is likely to be heated and hotly defended. (UK).
1993-06-12
Energy Technology Data Exchange (ETDEWEB)
The T Plant facilities in the 200-West Area of the Hanford site were constructed in the early 1940s to produce nuclear materials in support of national defense activities. T Plant includes the 271-T facility, the 221-T facility, and several support facilities (eg, 2706-T), utilities, and tanks/piping systems. T Plant has been recommended as the primary interim decontamination facility for the Hanford site. Project W-259 will provide capital upgrades to the T Plant facilities to comply with Federal and State of Washington environmental regulations for secondary containment and leak detection. This document provides an advanced conceptual design concept that complies with functional requirements for the T Plant Secondary Containment and Leak Detection upgrades.
1995-05-12
A brief history of the PUREX and UO{sub 3} facilities
Energy Technology Data Exchange (ETDEWEB)
The Plutonium-Uranium Extraction (PUREX) Plant, conceived during the early Cold War years, was a vehicle to increase significantly US nuclear weapons production capacity. The original PUREX Plant was a concrete rectangle 1,005 feet long and 61.5 feet wide. The shielding capacity of the concrete was designed so that personnel in non-regulated service areas would not receive radiation in excess of 0.1 millirem per hour. This report discusses the design of the PUREX Plant, the production chronology, projects and equipment changes, equipment decontamination and reuse, waste management, and contamination events that have occurred during the operation of the plant. Additionally, the development and history of the Uranium Trioxide Plant are also covered.
1993-11-01
Energy Technology Data Exchange (ETDEWEB)
The transport and partitioning of {sup 129}I has been examined for a shallow groundwater flow system at Sturgeon Falls in northeastern Ontario. Recharge into a sandy surficial postglacial deltaic aquifer occurs in the vicinity of a seasonally-wet boreal forest. Concentrations of stable iodine, {sup 129}I, tritium, radiocarbon, stable isotopes and major ions were measured on samples of groundwater and precipitation. The present-day tritium profile delineates the position of the early 1960's above-ground nuclear weapons pulse at a depth of approximately 12 m. The concentrations of stable iodine for groundwaters above, near and below the above-ground nuclear weapons pulse range from 0.07 to 1.7 ppb. Over that same interval {sup 129}I concentrations decreased from 1.9 x 10{sup 6} atoms/L at 9 m, to approximately 1.9 x 10{sup 5} atoms/L in tritium-depleted waters at 35 m, below the present-day depth of the recharging ...
2005-07-01
Energy Technology Data Exchange (ETDEWEB)
Neutron and gamma ray energy spectra were measured using an NE-213 scintillator at depths of 7.2, 15.2, and 22.2 cm in a tissue-equivalent phantom which was uniformly irradiated on one face by deuterium--tritium (DT) neutrons. Coupled neutron--gamma ray multigroup discrete-ordinates calculations were performed using semi-infinite slab geometry. These calculations were used to supplement the measured spectra below 1 MeV. Similar calculations were performed to study the perturbation in the phantom due to the detector. The measured and calculated spectra were used to determine the kerma distributions for neutrons and gamma rays at each location. The gamma radiation was determined to contribute more than 10% of the total dose at each depth. The calculated kerma also reveals that a knowledge of the gamma ray spectra below 1 MeV is desirable. Key words: neutron--gamma spectra, spectrometry, kerma distributions, coupled multigroup calculations
1983-01-01
International Nuclear Information System (INIS)
Neutron and gamma ray energy spectra were measured using an NE-213 scintillator at depths of 7.2, 15.2, and 22.2 cm in a tissue-equivalent phantom which was uniformly irradiated on one face by deuterium--tritium (DT) neutrons. Coupled neutron--gamma ray multigroup discrete-ordinates calculations were performed using semi-infinite slab geometry. These calculations were used to supplement the measured spectra below 1 MeV. Similar calculations were performed to study the perturbation in the phantom due to the detector. The measured and calculated spectra were used to determine the kerma distributions for neutrons and gamma rays at each location. The gamma radiation was determined to contribute more than 10% of the total dose at each depth. The calculated kerma also reveals that a knowledge of the gamma ray spectra below 1 MeV is desirable. Key words: neutron--gamma spectra, spectrometry, kerma distributions, coupled multigroup calculations.
7871-01-01
Tritium and "1"4C in the environment around Wolsong nuclear power plant
International Nuclear Information System (INIS)
To understand the environmental dispersion trend of "3H and "1"4C discharged from the Wolsung nuclear power plant, the present levels of "3H and "1"4C in environmental samples in the vicinity of the Wolsong site were studied. During 1992 through 2002, the annual means of HTO and "1"4C concentrations in air collected at three sampling stations around Wolsong nuclear power plant were in the range of 1.13 #approx# 29.2 Bq m"-"3 and 0.33 #approx# 0.40 Bq g-C"-"1 respectively, decreasing with distance from the site. The annual mean of TFWT concentrations in pine needle was in the range of 104 #approx# 790 Bq L"-"1 at N-1 and 62.8 #approx# 298 Bq L"-"1 at S"-"2, while the annual mean of "1"4C concentration was in the range of 0.335 #approx# 0.897 g-C"-"1 at N-1 and 0.254 #approx# 0.332 Bq g-C"-"1 #approx# at S"-"2, showing elevated value than a 0.25 Bq g-C"-"1 of background level. (author)
2003-09-01
Thermal conductivity of sintered lithium orthosilicate compacts
International Nuclear Information System (INIS)
The design of solid breeder blankets is strongly affected by the low values of thermal conductivity and density of ceramic breeder pebble beds. A significant rise of both quantities would enhance the thermal performance and lead to an increased tritium breeding ratio. In order to improve these quantities pretreated lithium orthosilicate pebble material was dry pressed and subsequently sintered. The thermal conductivity of cylindrical pellets was determined by the heat pulse method using a laser flash device. A pebble bed characteristic sample was also investigated in order to check the measurement accuracy in comparison with previous results. Furthermore, two samples of low density cellular ceramics were also prepared by infiltration of polymer foams with a ceramic slurry. The thermal conductivity results show that the values are affected both by the particle size and the sample density. Thermal conductivity values of higher than 2 W/m K were obtained using large ...
2009-04-30
T-2 mycotoxin inhibits mitochondrial protein synthesis
Energy Technology Data Exchange (ETDEWEB)
The authors investigated the effect of T-2 toxin on rat liver mitochondrial protein synthesis. Isolated rat liver mitochondria were supplemented with an S-100 supernatant from rat liver and an external ATP-generating system. An in-vitro assay employing cycloheximide, and inhibitor of cytoplasmic protein synthesis, and chloramphenicol, and inhibitor of mitochondrial protein synthesis, to distinguish mitochondrial protein synthesis from the cytoplasmic process. Amino acid incorporation into mitochondria was dependent on the concentration of mitochondria and was inhibited by chloramphenicol. The rate of uptake of tritium leucine into mitochondrial protein was unaffected by the addition of T-2 toxin and was not a rate-limiting step in incorporation. However, 0.02 micrograms/ml of T-2 toxin decreased the rate of protein synthesis inhibition correlated with the amount of T-2 toxin taken up by the mitochondria. While T-2 toxin is known to inhibit eukaryotic protein ...
1988-01-01
We study the sensitivity to neutrino masses of a Galactic supernova neutrino signal as could be measured with the detectors presently in operation and with future large volume water \\v{C}erencov and scintillator detectors. The analysis uses the full statistics of neutrino events. The method proposed uses the principles of Bayesian inference reasoning and has shown a remarkably independence of astrophysical assumptions. We show that, after accounting for the uncertainties in the detailed astrophysical description of the neutrino signal and taking into account the effects of neutrino oscillations in the supernova mantle, detectors presently in operation can have enough sensitivity to reveal a neutrino mass (or to set upper limits) at the level of 1 eV. This is sensibly better than present results from tritium $\\beta$-decay experiments, competitive with the most conservative limits from neutrinoless double $\\beta$-decay and less precise but remarkably less ...
2005-01-01
Research on development of adsorbent for separating and collecting light element isotopes
International Nuclear Information System (INIS)
Lithium isotopes are used as the raw material of tritium which is the fuel for fusion power generation and the material for fusion reactors, accordingly those are indispensable for future nuclear fusion power generation. As for boron isotopes, the neutron absorption corss section is very large, therefore, they are used for shielding neutrons and controlling fast neutron reactors. In order to further develop the utilization of nuclear power, it is important to develop the technology for separating and refining light element isotopes in large amount. In fiscal year 1995, the relation of the ion sieve characteristics of inorganic ion exchanger and the behavior of lithium isotope separation was examined. The behavior of forming boron complex of polyol amine was examined by B-11 NMR. These experiments and the results are reported. It was shown to be feasible that lithium is adsorbed from seawater, and isotopes are concentrated. Titanium phosphate and its heat treated ...
Energy Technology Data Exchange (ETDEWEB)
The use of deuterium-tritium fuel in the Compact Ignition Tokamak will require applying remote handling technology for ex-vessel maintenance and replacement of machine components. Highly activated and contaminated components of the fusion devices auxiliary systems, such as diagnostics and RF heating, must be replaced using remotely operated maintenance equipment in the test cell. In-vessel remote maintenance included replacement of divertor and first wall hardware, faraday shields, and for an in-vessel inspection system. Provision for remote replacement of a vacuum vessel sector, toroidal field coil or poloidal field ring coil was not included in the project baseline. As a result of recent coil failures experienced at a number of facilities, the CIT project decided to reconsider the question of remote recovery from a coil failure and, in January of 1990, initiated a coil replacement study. This study focused on the technical requirements and impact on fusion ...
1990-01-01
International Nuclear Information System (INIS)
A critical issues study of a symmetric illumination, direct drive laser fusion reactor called SIRIUS has been conducted. In particular, the uniformity requirements for direct drive targets have been assessed and it is shown that respectable gains (more than 60) could be obtained at modest (2MJ) KrF laser energies. Previous ICF cavity designs have been examined for use in a symmetric illumination geometry and features from several designs have been combined into a dry wall cavity design with a radius of 8 meters. Neutronic and photonic analysis shows that the present SIRIUS cavity design can breed sufficient tritium (breeding ratio = 1.17) even with 32 laser ports penetrating the cavity. However, it was found that there are a few critical issues that remain to be solved before a self-consistent reactor design could be initiated. Radiation damage to final optics, thermal performance of SiC tiles on the SIRIUS cavity wall, and performance of direct drive targets to ...
1984-01-01
Parameter study of the LIFE engine nuclear design
International Nuclear Information System (INIS)
LLNL is developing the nuclear fusion based Laser Inertial Fusion Energy (LIFE) power plant concept. The baseline design uses a depleted uranium (DU) fission fuel blanket with a flowing molten salt coolant (flibe) that also breeds the tritium needed to sustain the fusion energy source. Indirect drive targets, similar to those that will be demonstrated on the National Ignition Facility (NIF), are ignited at #approx#13 Hz providing a 500 MW fusion source. The DU is in the form of a uranium oxycarbide kernel in modified TRISO-like fuel particles distributed in a carbon matrix forming 2-cm-diameter pebbles. The thermal power is held at 2000 MW by continuously varying the "6Li enrichment in the coolants. There are many options to be considered in the engine design including target yield, U-to-C ratio in the fuel, fission blanket thickness, etc. Here we report results of design variations and compare them in terms of various figures of merit such as time to reach a ...
2010-09-01
Energy Technology Data Exchange (ETDEWEB)
Examination of a chloroform extract of Dracaena loureiri Gagnep (Agavaceae), a Thia medicinal plant possessing antibacterial activity, has led to the isolation of fifteen flavenoids. The biogenic relationships among these flavenoids isolated were briefly discussed. Definition of the skeleton and the unambiguous assignment of all of the protons of the isolates was achieved through extensive 2D-homonuclear chemical shift correlation, nuclear Overhauser effect (NOE) difference spectroscopy and 2D-NOE experiments. The {sup 1}H and {sup 13}C NMR spectra of staurosporine, a potent biologically active agent from Streptomyces staurosporeus, were unambiguously assigned by using 2D homonuclear chemical shift correlation, NOE, {sup 1}H-detected heteronuclear multiple-quantum coherence via direct coupling and via multiple-bond coupling for resonance assignments of protonated and nonprotonated carbons, respectively. S. Staurosporeus was found to utilize endogenous and exogenous D- and L-isomers of ...
1988-01-01
High resolution alpha-particle spectroscopy using CR-39 plastic track detector
Energy Technology Data Exchange (ETDEWEB)
A technique has been developed for high resolution alpha particle spectroscopy from track length determination in CR-39 plastic. On individual tracks an energy resolution deltaE close to the range straggling limit is obtainable. For 6 MeV alpha-particle deltaE is proportional 35 keV on individual particles and for groups of particles deltaE proportional 20 keV can be achieved using certain data selection criteria. At 100 keV on individual particles deltaE is proportional 20 keV. The analysis requires 1) a knowledge of the track-etch rate (Vsub(T))-range relationship and 2) a theoretical understanding of alpha-particle track structure in CR-39 as a function of particle energy, dip angle and degree of etching. The structure of alpha-particle etched tracks in CR-39 is described and two methods of analysis discussed. Examples are given of the resolution attainable on tracks of alpha-particles as natural decay energy and from alpha-particles generated in laser driven deuterium and ...
1984-06-15
Fusion power and the environment
Environmental characteristics of conceptual fusion-reactor systems based on magnetic confinement are examined quantitatively, and some comparisons with fission systems are made. Fusion, like all other energy sources, will not be completely free of environmental liabilities, but the most obvious of these-- tritium leakage and activation of structural materials by neutron bombardment-- are susceptible to significant reduction by ingenuity in choice of materials and design. Large fusion reactors can probably be designed so that worst-case releases of radioactivity owing to accident or sabotage would produce no prompt fatalities in the public. A world energy economy relying heavily on fusion could make heavy demands on scarce nonfuel materials, a topic deserving further attention. Fusion's potential environmental advantages are not entirely ''automatic'', converting them into practical reality will ...
1975-06-01
Energy Technology Data Exchange (ETDEWEB)
The PERMCAT process chosen for the final clean-up stage of the Tokamak Exhaust Processing system of the ITER tritium plant combines in a single component a catalytic reactor and a permeator using Pd/Ag membranes. This study covers the mechanical behaviour of a Pd/Ag membrane under different operating conditions. The consequences of hydrogen uptake by the membrane during nominal operation but also during off-normal events are presented. Depending on the operating conditions, expansions around 2% and significant deformations are observed. Different mechanical designs of PERMCAT reactors are then discussed. The first generation comprises finger-type membranes and two new mechanical designs use either additional edge welded bellows or a special corrugated Pd/Ag membrane. These upgraded designs improve the robustness and simplify the geometry of the component. The experimental validation of these new units has been carried out based on the measurements of the processing ...
2007-10-15
International Nuclear Information System (INIS)
The PERMCAT process chosen for the final clean-up stage of the Tokamak Exhaust Processing system of the ITER tritium plant combines in a single component a catalytic reactor and a permeator using Pd/Ag membranes. This study covers the mechanical behaviour of a Pd/Ag membrane under different operating conditions. The consequences of hydrogen uptake by the membrane during nominal operation but also during off-normal events are presented. Depending on the operating conditions, expansions around 2% and significant deformations are observed. Different mechanical designs of PERMCAT reactors are then discussed. The first generation comprises finger-type membranes and two new mechanical designs use either additional edge welded bellows or a special corrugated Pd/Ag membrane. These upgraded designs improve the robustness and simplify the geometry of the component. The experimental validation of these new units has been carried out based on the measurements of the processing ...
2007-10-01
Energy Technology Data Exchange (ETDEWEB)
ACRO, a NGO equipped with a laboratory to measure radioactivity, runs the Citizen Watchdog of Radioactivity in the Environment. Involving many volunteers, it monitors regularly the French coast of the Channel and many rivers of the North half of France. It also makes investigations in other places. Such an action is aimed to supplement the official monitoring, not to replace it, in order to answer to the worries of the population. This monitoring shows that some radioelements, such as iodine 129, cobalt 60, tritium, etc. released in the environment by nuclear facilities can be detected on very large areas. Carbon 14 was detected up to almost 4 times the background in vegetables around the reprocessing plant of La Hague. ACRO also sits in many official committees to transmit the point of view of the populations exposed to the radioactive pollution. It is lobbying for a decrease of the release authorization, especially for the elements that are discharged in large ...
2010-06-15
Effects of multi-ion irradiation on microstructural changes in lithium titanate
Energy Technology Data Exchange (ETDEWEB)
The irradiation behavior of Li{sub 2}TiO{sub 3} under a fusion reactor environment was simulated by simultaneous irradiation of Li{sub 2}TiO{sub 3} by the triple ion beams and the respective single ion beams of O{sup 2+}, He{sup +} and H{sup +}. The microstructural changes in Li{sub 2}TiO{sub 3} caused by the irradiation were measured by FT-IR photoacoustic spectroscopy. The results suggest that the amount of TiO{sub 2} formed is proportional to the dpa and that the method of irradiation does not affect the dependence of formation of TiO{sub 2}. On the other hand, the amount of defects and/or radiolytic products generated by irradiation, which is considered to trap hydrogen near the surface, is found to be affected by the method of irradiation. Such phenomena are believed to affect the tritium release behavior from Li{sub 2}TiO{sub 3}, and durability of Li{sub 2}TiO{sub 3} and compatibility of Li{sub 2}TiO{sub 3} with other components of the breeder blanket such as ...
2009-04-30
Effects of multi-ion irradiation on microstructural changes in lithium titanate
International Nuclear Information System (INIS)
The irradiation behavior of Li_2TiO_3 under a fusion reactor environment was simulated by simultaneous irradiation of Li_2TiO_3 by the triple ion beams and the respective single ion beams of O"2"+, He"+ and H"+. The microstructural changes in Li_2TiO_3 caused by the irradiation were measured by FT-IR photoacoustic spectroscopy. The results suggest that the amount of TiO_2 formed is proportional to the dpa and that the method of irradiation does not affect the dependence of formation of TiO_2. On the other hand, the amount of defects and/or radiolytic products generated by irradiation, which is considered to trap hydrogen near the surface, is found to be affected by the method of irradiation. Such phenomena are believed to affect the tritium release behavior from Li_2TiO_3, and durability of Li_2TiO_3 and compatibility of Li_2TiO_3 with other components of the breeder blanket such as structural materials in the fusion reactor system under operation.
2009-04-30
Development of the Regulation Concept for a Fusion Reactor
International Nuclear Information System (INIS)
Fusion energy has been studied in many countries such as U.S., France, Japan, Korea etc. Because it would provide much more energy for a given weight of fuel than any technology currently in use, and the fuel itself (primarily deuterium) exists abundantly in the Earth's ocean. Nuclear fusion reactor uses tritium and deuterium as fuel while nuclear fission reactor uses uranium and plutonium as fuel. Besides, inherent design characteristics and driving condition of nuclear fusion reactor is different from those of nuclear fission reactor. Therefore, we cannot apply the regulation rules of nuclear fission reactor to nuclear fusion reactor without change and thus it is needed to development of the safety regulation concept which reflects the characteristics of nuclear fusion reactor. Safety regulation of nuclear fusion reactor employs deterministic approach until sufficient data are secured. However, regulation methodology of nuclear fusion reactor should be based on ...
2010-10-01
International Nuclear Information System (INIS)
Changes in contents of the two kinds of neuropeptides have been measured in the brains of postnatal G57BL/6J strain mice that received accumulative doses of 0, 0.05, 0.10 or 0.30 Gy respectively in utero from tritium #beta#-irradiation during the mother mice's pregnancy from the 12.5th day of gestation to the day of delivery. Dose response relationship for alteration in somatostatin content due to exposure to 0.10 Gy or above was observed, and it was also noted that 0.30 Gy could cause decrease in arginine vasopressin in hypothalamus. These results were consistent with findings in research on brain development and reflex behavior in the literature. 0.10 Gy exposure may represent a threshold for exposure to tritiated water within the range from day 12.5 of gestation to the day of delivery using change in content of somatostatin in hypophysis as a parameter.
Energy Technology Data Exchange (ETDEWEB)
ESH-19 personnel collected soil and single-stage water samples around the perimeter of Area G at Los Alamos National Laboratory during FY94 to characterize possible contaminant movement out of Area G through surface-water and sediment runoff. These samples were analyzed for tritium, total uranium, isotopic plutonium, americium-241, and cesium-137. Ten metals were also analyzed on selected soils using analytical laboratory techniques. All radiochemical data are compared with analogous samples collected during FY 93 and reported in LA-12986. Baseline concentrations for future disposal operations were established for metals and radionuclides by a sampling program in the proposed Area G Expansion Area. Considering the amount of radioactive waste that has been disposed at Area G, there is evidence of only low concentrations of radionuclides on perimeter surface soils. Consequently, little radioactivity is leaving the confines of Area G via the surface water runoff ...
1996-08-01
Application of variational methods to fusion reactor blanket studies
International Nuclear Information System (INIS)
The general development of variational methods for fusion reactor blanket studies is given. Important quantities such as tritium breeding ratio and total nuclear heating are linear functionals of the solutions to the Boltzmann transport equation. To estimate a neutronic quantity by variational methods is, in general, to carry out the scalar product formulation of the Roussopoulos variational principle, or the Schwinger variational principle, with the help of the associated adjoint transport equation where the appropriate response function for the estimate is taken as the source. A multipoint interpolation method based on the above variational principles has been developed and compared to other variational approaches. The method of variational interpolation removes the need to compute both forward and adjoint solutions while the error has the characteristic of cancellation of errors between interpolation reference points. Finally, the practical computational ...
Analysis of the requirements for economic magnetic fusion
Energy Technology Data Exchange (ETDEWEB)
A generic reactor model is used to examine the economic viability of electricity generation by magnetic fusion. The simple model uses components which are representative of those used in previous reactor studies of deuterium-tritium burning tokamaks, stellarators, bumpy tori, reverse field pinches and tandem mirrors. Conservative costing assumptions are made. The generic reactor is not a tokamak but rather it is intended to emphasize what is common to all magnetic fusion reactors. The reactor uses a superconducting toroidal coil set to produce the dominant magnetic field. To this extent it is a less good approximation to systems, such as the reversed field pinch in which the main field is produced by a plasma current. The main output of the study is the cost of electricity as a function of the weight and size of the fusion core - blanket, shield, structure and coils. The model shows that a 1200 MW/sub e/ power plant with a fusion core weight of about 10,000 tonnes ...
1986-01-01
ARIES-AT safety design and analysis
Energy Technology Data Exchange (ETDEWEB)
ARIES-AT is a 1000 MWe conceptual fusion power plant design with a very low projected cost of electricity. The design contains many innovative features to improve both the physics and engineering performance of the system. From the safety and environmental perspective, there is greater depth to the overall analysis than in past ARIES studies. For ARIES-AT, the overall spectrum of off-normal events to be examined has been broadened. They include conventional loss of coolant and loss of flow events, an ex-vessel loss of coolant, and in-vessel off-normal events that mobilize in-vessel inventories (e.g., tritium and tokamak dust) and bypass primary confinement such as a loss of vacuum and an in-vessel loss of coolant with bypass. This broader examination of accidents improves the robustness of the design from the safety perspective and gives additional confidence that the facility can meet the no-evacuation requirement under average weather conditions. We also provide ...
2006-01-15
ARIES-AT safety design and analysis
International Nuclear Information System (INIS)
ARIES-AT is a 1000 MWe conceptual fusion power plant design with a very low projected cost of electricity. The design contains many innovative features to improve both the physics and engineering performance of the system. From the safety and environmental perspective, there is greater depth to the overall analysis than in past ARIES studies. For ARIES-AT, the overall spectrum of off-normal events to be examined has been broadened. They include conventional loss of coolant and loss of flow events, an ex-vessel loss of coolant, and in-vessel off-normal events that mobilize in-vessel inventories (e.g., tritium and tokamak dust) and bypass primary confinement such as a loss of vacuum and an in-vessel loss of coolant with bypass. This broader examination of accidents improves the robustness of the design from the safety perspective and gives additional confidence that the facility can meet the no-evacuation requirement under average weather conditions. We also provide ...
2006-01-01
2008 Data Report: Groundwater Monitoring Program Area 5 Radioactive Waste Management Site
This report is a compilation of the groundwater sampling results from the Area 5 Radioactive Waste Management Site (RWMS) including calendar year 2008 results. Each of the three Pilot Wells was sampled on March 11, 2008, and September 10, 2008. These wells were sampled for the following indicators of contamination: pH, specific conductance, total organic carbon, total organic halides, and tritium. Indicators of general water chemistry (cations and anions) were also monitored. Results from all samples collected in 2008 were within the limits established by agreement with the Nevada Division of Environmental Protection for each analyte. These data indicate that there has been no measurable impact to the uppermost aquifer from the Area 5 RWMS. There were no significant changes in measured groundwater parameters compared to previous years. Other information in the report includes an updated Cumulative Chronology for the Area 5 RWMS Groundwater Monitoring Program and ...
2009-01-13
2006 Data Report: Groundwater Monitoring Program Area 5 Radioactive Waste Management Site
This report is a compilation of the groundwater sampling results from the Area 5 Radioactive Waste Management Site (RWMS) for calendar year 2006. Pilot wells UE5PW-1, UE5PW-2, and UE5PW-3 were sampled in April and October 2006 for the following indicators of contamination: pH, specific conductance, total organic carbon, total organic halides, and tritium. Indicators of general water chemistry (cations and anions) were also monitored. Results from all samples collected in 2006 were within the limits established by agreement with the Nevada Division of Environmental Protection for each analyte. These data indicate that there has been no measurable impact to the uppermost aquifer from the Area 5 RWMS. There were no significant changes in measured groundwater parameters compared to previous years. Other information in the report includes an updated Cumulative Chronology for the Area 5 RWMS Groundwater Monitoring Program and a brief description of the site hydrogeology.
2007-02-01
International Nuclear Information System (INIS)
A multielement apparatus for the removal of aerosols formed in the vitrification of simulated high-activity accident wastes from the decommissioned nuclear power plant A-1 has been designed, manufactured and tested. The apparatus consists of two cooling and condensing steps connected in series, and of five filtration steps also connected in series. The five filtration steps allowed to achieve a decontamination factor of 1x10"5 in the case of removal of a NaCl("2"4Na) testing model aerosol. The decontamination factor for removal of the cesium aerosol by the whole apparatus was 3.3x10"6. In the first filtration step the aerosols are removed by the cartridge with a filtration fabric made of polyethylene fibers, in the second step by the cartridge with a granulated natural material, in the third step by the cartridge with glass-fiber filtration paper, in the fourth and fifth steps by the cartridge with high-efficiency filtration paper made of glass ...
The interaction of Np(V), Pu(VI) and Tc(VII) with metal in alkaline solutions
International Nuclear Information System (INIS)
The interaction of Np(V), Pu(VI) and Tc(VII) with metal reductants Zn, Cr, Sn and their alloys was investigated in 0.5-4 mol l"-"1 NaOH solutions in static and dynamic conditions (by filtration of solutions through the column filled with grains of metal). In this paper, it was found that the reduction and succeeding precipitation hydroxides of these elements, on the surface of metal grains from 0.5 to 4 mol l"-"1 NaOH solutions, gives a decontamination factor (DF) from 1.1 to 67. The best result was achieved for Pu (DF=67) on Cr grains after 2.5 h contact at 60 C with 0.5 mol l"-"1 NaOH solution containing Pu(VI). Increasing the NaOH concentration, and the addition of chromate ions and complex-forming agents to alkaline solution results in a decrease of the decontamination factor (DF). A better result for Np sorption from 1 mol l"-"1 NaOH solutions was achieved after longer contact, than for Pu, with Cr and Zn grains. The maximum DF=8.9 was ...
1998-06-12
Stationary low power reactor No. 1 (SL-1) accident site decontamination & dismantlement project
The Army Reactor Area (ARA) II was constructed in the late 1950s as a test site for the Stationary Low Power Reactor No. 1 (SL-1). The SL-1 was a prototype power and heat source developed for use at remote military bases using a direct cycle, boiling water, natural circulation reactor designed to operate at a thermal power of 3,000 kW. The ARA II compound encompassed 3 acres and was comprised of (a) the SL-1 Reactor Building, (b) eight support facilities, (c) 50,000-gallon raw water storage tank, (d) electrical substation, (e) aboveground 1,400-gallon heating oil tank, (f) underground 1,000-gallon hazardous waste storage tank, and (g) belowground power, sewer, and water systems. The reactor building was a cylindrical, aboveground facility, 39 ft in diameter and 48 ft high. The lower portion of the building contained the reactor pressure vessel surrounded by gravel shielding. Above the pressure vessel, in the center portion of the building, was a turbine generator and plant support ...
1995-11-01
International Nuclear Information System (INIS)
With the aim of preparing carrier-free "2"8Mg and "4"7Ca simultaneously, Ti, V and Fe targets were examined by irradiating with high-energy ions of "1"2C, "1"4N and "1"6O accelerated by the RIKEN ring cyclotron. Among the targets, V gave the highest cross section for the formation of both "2"8Mg and "4"7Ca irrespective of the kind of beams. The cross section for the formation of "2"8Mg by the reactions of Ti, V and Fe targets with ion beams increased in the order of "1"2C<"1"6O<"1"4N. On the other hand, the three beams exhibited almost the same cross sections for the formation of "4"7Ca by the reaction of a given target. Titanium and V were selected as prospective targets and "1"4N as a suitable beam for the production of "2"8Mg and "4"7Ca. Chemical separation procedures of the radiotracers in carrier- and salt-free states have been established by using cation exchange resins. The recovery yields of "2"8Mg and "4"7Ca from Ti target were 70 and 90%, respectively, and the ...
Reprocessed uranium fuel fabrication in Japan
International Nuclear Information System (INIS)
Nuclear fuel vendors in Japan are now studying reprocessed uranium (RepU) fuel in order to prepare for full scale utilization in the future. Separate studies are made for PWR and BWR fuel. The study consists of 2 phrases. The purposes of phase-1 are to understand various RepU characteristics in the fuel fabrication process, to analyze the core characteristics by loading RepU assemblies, to solve the problems clarified in the study, and to collect basic data for licensing. In phase-2, the effects of impurities on the fabrication process will be evaluated, and the safety of RepU fuel manufacturing will be confirmed with a RepU fuel fabrication campaign in 1990. The neutronic data will be collected after insertion into power reactors, and the data will be used to verify plant safety for full utilization of RepU in the future. This paper summarizes the phase-1 study results. 1. RepU Characteristics. The internal and external radiation exposures due to nuclide impurities in RepU, were ...
1990-12-01
Recovery and mutual separation of noble metals from the simulated insoluble residue of spent fuel
International Nuclear Information System (INIS)
The recovery of noble metals from the quaternary Mo-Ru-Rh-Pd alloy in the simulated insoluble residue was studied by means of Pb extraction and the recovery yield was found to be more than 90% for Ru, Rh and Pd. The recovery yield of Mo was very small due to the oxidative vaporization in air. The decontamination factor for Ce as a stand-in of Pu was determined to be around 200 for one stage. These results on the recovery yields of noble metals from the quaternary alloy and the decontamination factor for Ce are in good agreement with those for the ternary Mo-Ru-Pd alloy previously reported by the present authors. The mutual separation of noble metal elements recovered in Pb button was examined by means of re-extraction with molten Zn and the dissolution in boiling 3M or 6M nitric acid solution. The dissolution fractions of Pd and Rh recovered in the Pb button in boiling 3M and 6M nitric acid solution for 12 h were about 90 and 30%, respectively, ...
International Nuclear Information System (INIS)
A new method that allows rapid preconcentration and separation of plutonium and neptunium in water samples was developed for the measurement of "2"3"7Np and Pu isotopes by inductively-coupled plasma mass spectrometry (ICP-MS) and alpha spectrometry. "2"3"8U can interfere with "2"3"9Pu measurement by ICP-MS as "2"3"8UH"+ mass overlap and "2"3"7Np via peak tailing. The method provide enhanced removal of uranium by separating Pu and Np initially on TEVA Resin, then moving Pu to DGA resin for additional removal of uranium. The decontamination factor for uranium from Pu is almost 100,000 and the decontamination factor for U from Np is greater than 10,000. This method uses stacked extraction chromatography cartridges and vacuum box technology to facilitate rapid separations. Preconcentration is performed using a streamlined calcium phosphate precipitation method. Purified solutions are split between ICP-MS and alpha spectrometry so that long and ...
2011-01-01
Energy Technology Data Exchange (ETDEWEB)
A new method that allows rapid preconcentration and separation of plutonium and neptunium in water samples was developed for the measurement of {sup 237}Np and Pu isotopes by inductively-coupled plasma mass spectrometry (ICP-MS) and alpha spectrometry; a hybrid approach. {sup 238}U can interfere with {sup 239}Pu measurement by ICP-MS as {sup 238}UH{sup +} mass overlap and {sup 237}Np via peak tailing. The method provide enhanced removal of uranium by separating Pu and Np initially on TEVA Resin, then moving Pu to DGA resin for additional removal of uranium. The decontamination factor for uranium from Pu is almost 100,000 and the decontamination factor for U from Np is greater than 10,000. This method uses stacked extraction chromatography cartridges and vacuum box technology to facilitate rapid separations. Preconcentration is performed using a streamlined calcium phosphate precipitation method. Purified solutions are split between ICP-MS and ...
2010-06-23
Energy Technology Data Exchange (ETDEWEB)
The performance of PAN-based composite absorbers was evaluated in dynamic experiments at flow rates ranging from 25--100 bed volumes (BV) per hour. Composite absorbers with active components of ammonium molybdophosphate (AMP) PAN and K-Co ferrocyanide (KCoFC) PAN were used for separating Cs from a 1 M HNO{sub 3} + 1 M NaNO{sub 3} + 2 {times} 10{sup {minus}5} M CsCl acidic simulant solution. KCoFC-PAN and two other FC-based composite absorbers were tested for separating Cs from alkaline simulant solutions containing 0.01 M to 1 M NaOH and 1 M NaNO{sub 3} + x {times} 10{sup {minus}4} M CsCl. The efficiency of the Cs sorption on the AMP-PAN absorber from acidic simulant solutions was negatively influenced by the dissolution of the AMP active component. At flow rates of 50 BV/hr, the decontamination factor of about 10{sup 3} could be maintained for treatment of 380 BV of the feed. With the KCoFC-PAN absorber, the decontamination factor of about ...
1996-05-01
International Nuclear Information System (INIS)
In the case where uranium recovered by an advanced aqueous reprocessing is utilized in light water reactors (LWRs) with the thermal neutron spectrum, the effects of the decontamination factor (DF) of the reprocessing on core neutronic characteristics were examined. The amounts of transuranium (TRU) elements and fission products (FPs) contained in the recovered uranium depend on the DF of reprocessing, and also "2"3"6U is generated by neutron capture of "2"3"5U during a reactor operation. These all act as poisons in the fuel. Therefore, in this paper, the additional "2"3"5U enrichment necessary to compensate for the produced TRU elements, FPs, and "2"3"6U was evaluated for three representative DF values: 10"2, 10"3, and infinity. The low value of 10"2 corresponds to the advanced aqueous reprocessing investigated here. An APWR core with a discharge burnup of 49 GWd/t when the initial "2"3"5U enrichment is 4.6% was considered as the reference core. Uranium of the ...
2009-05-01
Development of low-level liquid-waste treatment systems: April-September 1982
Energy Technology Data Exchange (ETDEWEB)
A preliminary investigation was conducted on ion specific membranes. This investigation concentrated on testing candidate organic compounds for transporting cesium ions through a membrane composed of the organic compound supported on a substrate. Solid PVC membranes were initially tried, but were found to be too slow. Thereafter, only liquid membranes were tested. These were faster and cesium concentration factors up to 2.96 were achieved in a single membrane cell. A cell with two membranes achieved a cesium concentration factor of 4.19. Cesium precipitation with sodium tetraphenyl borate in high sodium concentrations was explored. No interference from sodium was found until the sodium nitrite concentration reached 4.5 moles. Concurrently, cesium concentrations as high as 5.4 g/L were precipitated. Potassium tetraphenyl borate is being investigated for use in exchange columns for the removal of cesium from solutions. Initial investigations show that cesium removal is affected by (K/sup ...
1982-12-22
Development of low-level liquid-waste treatment systems: April-September 1982
International Nuclear Information System (INIS)
A preliminary investigation was conducted on ion specific membranes. This investigation concentrated on testing candidate organic compounds for transporting cesium ions through a membrane composed of the organic compound supported on a substrate. Solid PVC membranes were initially tried, but were found to be too slow. Thereafter, only liquid membranes were tested. These were faster and cesium concentration factors up to 2.96 were achieved in a single membrane cell. A cell with two membranes achieved a cesium concentration factor of 4.19. Cesium precipitation with sodium tetraphenyl borate in high sodium concentrations was explored. No interference from sodium was found until the sodium nitrite concentration reached 4.5 moles. Concurrently, cesium concentrations as high as 5.4 g/L were precipitated. Potassium tetraphenyl borate is being investigated for use in exchange columns for the removal of cesium from solutions. Initial investigations show that cesium removal is affected by [K"+] ...
International Nuclear Information System (INIS)
A series of separation experiment was performed in order to study a multi-functional spent fuel reprocessing process based on ion-exchange technique. The tertiary pyridine-type anion-exchange resin was used in this experiment and the mixed oxide fuel highly irradiated in the experimental fast reactor ''JOYO'' was used as a reference spent fuel. As the result, "1"0"6Ru + "1"2"5Sb, "1"3"7Cs + "1"5"5Eu + "1"4"4Ce, plutonium, americium and curium could be separated from the irradiated fuel by only three steps of ion-exchange. The decontamination factor of "1"3"7Cs and trivalent lanthanides ("1"5"5Eu, "1"4"4Ce) in the final americium product exceeded 3.9 x 10"4 and 1.0 x 10"5, respectively. The decontamination factor for the mutual separation of "2"4"3Cm and "2"4"1Am was larger than 2.2 x 10"3 for the americium product and, moreover, the content of "1"3"7Cs, trivalent lanthanides and "2"4"3Cm included in "2"4"1Am product did not exceed 2 ppm. These ...
2006-06-01
Decontamination of cesium, strontium, and cobalt from aqueous solutions by bentonite
Energy Technology Data Exchange (ETDEWEB)
Sorption studies of cesium, strontium, and cobalt (Cs, Sr, and Co) on bentonite under various experimental conditions, such as contact time, pH, sorbent and sorbate concentration, and temperature, have been performed. The sorption data for all these metals have been interpreted in terms of Freundlich, Langmuir, and Dubinin-Radushkevich equations. Thermodynamics parameters, such as heat of sorption {Delta}H{degrees}, free energy change {Delta}G{degrees}, and entropy change {Delta}S{degrees}, for the sorption of these metals on bentonite have been calculated. The value of {Delta}H{degrees} shows that the sorption of Cs was exothermic, while the sorption of Sr and Co on bentonite were endothermic in nature. The value of {Delta}G{degrees} for their sorption was negative, showing the spontaneity of the process. The maximum loading capacity of Cs, Sr, and Co were 75.5, 22, and 27.5 meq, respectively, for 100 g of bentonite. The mean free energy E of Cs, Sr, and Co sorption on bentonite was ...
1996-12-31
Chemical, sensory and microbiological changes of gamma irradiated coconut cream powder
Energy Technology Data Exchange (ETDEWEB)
A study was carried out to determine optimum decontamination dose for a locally manufactured coconut cream powder. Samples were gamma irradiated (0-15 kGy) and ageing process was achieved using GEER oven at 60 deg. C for 7 days, which is equivalent to one-year storage at room temperature. Iodine value (IV), ranging from 4.8 to 6.4, was not affected by radiation doses and storage, however peroxide value and thiobarbituric acid (TBA) generally increased with radiation doses. In most samples, peroxide value (meq/kg) reduced after storage, whilst the TBA (mg malonaldehyde/kg), indicator for product quality, slightly increased. The sensory evaluation conducted using 25 taste panellists indicated that scores on odour, creamy taste and overall acceptance for all irradiated samples at more than 5 kGy were significantly lower (P<0.05) than the control. However, the panellists could not detect any significant differences among the irradiation doses (P>0.05). ...
2007-11-15
A study on the treatment of radioactive liquid wastes using synthetic by air intake system
Energy Technology Data Exchange (ETDEWEB)
In this study based on the mass transfer theory, experiments for the evaporation rates depending on various conditions were carried out through the operation of the existing Natural Evaporation Facility in KAERI. Evaporation media were made of the cotton and polyester. Air circulation in the facility was forced by exhausting fans. The evaporation rate and the decontamination factor were calculated by the result of experiment. The evaporation rate increased as the flow rate of air supply, the feed rate of liquid waste, and the temperature of supplied air increased. As for the humility of supplied air, the evaporation rate was getting higher as the humidity was getting lower. As the result of this study, operation conditions of the Natural Evaporation Facility are optimized as follows; The air temperature above 8C .deg., the air humidity below 70%, the air flow rate 1.14-1.47 m/sec, and the liquid waste feed rate 4.6l/hr.m{sup 2}. The ...
2003-07-01
Environmental monitoring data were collected at and around the Area 3 and Area 5 Radioactive Waste Management Sites (RWMSs) at the Nevada Test Site. These data are associated with radiation exposure, air, groundwater, meteorology, vadose zone, subsidence, and biota. This report summarizes the 2006 environmental data to provide an overall evaluation of RWMS performance and to support environmental compliance and performance assessment (PA) activities. Some of these data (e.g., radiation exposure, air, and groundwater) are presented in other reports (U.S. Department of Energy, 2006; Warren and Grossman, 2007; National Security Technologies, LLC, 2007). Direct radiation monitoring data indicate that exposure levels around the RWMSs are at or below background levels. Air monitoring data at the Area 3 and Area 5 RWMSs indicate that tritium concentrations are slightly above background levels. There is no detectable man-made radioactivity by gamma spectroscopy, and ...
2007-06-30
Effects of Multi-ion Irradiation on Microstructural Changes in Lithium Titanate
Energy Technology Data Exchange (ETDEWEB)
Full text of publication follows: Li{sub 2}TiO{sub 3} is regarded as one of the most suitable candidates for the solid tritium breeder material of D-T fusion reactors. It is known that, in an operating fusion reactor, the radiation damage in Li{sub 2}TiO{sub 3} will be caused by fast neutrons, energetic tritons and helium ions generated in {sup 6}Li(n,{alpha}){sup 3}H reaction. The irradiation damage caused by such radiation may result in the microstructural changes, and the changes may affect the characteristics of Li{sub 2}TiO{sub 3} such as tritium release behavior. Thus the study of irradiation defects and microstructural changes caused by irradiation in Li{sub 2}TiO{sub 3} is essential to evaluate its irradiation performance. Simulation of the fusion reactor environment and hence the study of a synergistic effect of atomic displacement damage in Li{sub 2}TiO{sub 3} are approached by a simultaneous irradiation with ...
2007-07-01
ETE-EVAL: a methodology for D and D cost estimation
International Nuclear Information System (INIS)
In compliance with Article 20 of the sustainable radioactive materials and waste management act dated 28 June 2006, the CEA and AREVA are required every three years to revise the cost of decommissioning their facilities and to provide the necessary assets by constituting a dedicated fund. For the 2007 revision the CEA used ETE-EVAL V5. Similarly, AREVA reevaluated the cost of decontaminating and dismantling its facilities at La Hague, as the previous estimate in 2004 did not take into account the complete cleanup of all the structural work. ETE-EVAL V5 is a computer application designed to estimate the cost of decontamination and dismantling of basic nuclear installations (INB). It has been qualified by Bureau Veritas and audited. ETE-EVAL V5 has become the official software for cost assessment of CEA civilian and AREVA decommissioning projects. It has been used by the DPAD (Decontamination and Dismantling Projects ...
Energy Technology Data Exchange (ETDEWEB)
The project involved several studies of vesicles and micelles and their constituent surfactants. The primary objective of the project was an elucidation of factors involved in the stabilization and destabilization of vesicles and micelles. Work was performed on seven individual studies. Several different types of novel cleavable surfactants were synthesized, including systems with two chains and two head groups, and their aqueous micelles and vesicles were characterized by methods including dynamic laser light scattering (to give aggregate sizes) and differential scanning calorimetry (to give vesicle bilayer phase transition temperatures). A cleavable surfactant is stable under certain conditions but liable under other conditions with respect to cleavage to give nonsurfactant products and/or other surfactants with different properties. The destruction of several cleavable surfactant-derived aggregates was demonstrated, indicating that they have potential as entrapment and release ...
1996-03-19
Trapping technology for gaseous fission products from voloxidation process
Energy Technology Data Exchange (ETDEWEB)
The objective of this report is to review the different technologies for trapping the gaseous wastes containing Cs, Ru, Tc, {sup 14}C, Kr, Xe, I and {sup 3}H from a voloxidation process. Based on literature reviews and KAERI's experimental results on the gaseous fission products trapping, appropriate trapping method for each fission product has been selected considering process reliability, simplicity, decontamination factor, availability, and disposal. Specifically, the most promising trapping method for each fission product has been proposed for the development of the INL off-gas trapping system. A fly ash filter is proposed as a trapping media for a cesium trapping unit. In addition, a calcium filter is proposed as a trapping media for ruthenium, technetium, and {sup 14}C trapping unit. In case of I trapping unit, AgX is proposed. For Kr and Xe, adsorption on solid is proposed. SDBC (Styrene Divinyl Benzene Copolymer) is also proposed as a conversion ...
2005-05-15
The application of irradiation techniques for food preservation and processing improvement
Energy Technology Data Exchange (ETDEWEB)
This project has intended to develop alternative techniques to be used in food industry for food processing and utilization by safe irradiation methods. For improvement of rheology and processing in corn starch by irradiation, the production of modified starch with low viscosity as well as with excellent viscosity stability became feasible by the control of gamma irradiation dose levels and the amount of added inorganic peroxides to starch. Also, this project was developed the improvement methods of hygienic quality and long-term storage of dried red pepper by gamma irradiation. And, in Korean medicinal plants, 10 kGy gamma irradiation was effective for improving sanitary quality and increasing extraction yield of major components. For the sanitization of health and convenience foods, gamma irradiation was more effective than ozone treatment in decontamination of microorganisms, with minimal effect on the physicochemical properties analysed. In evaluation of ...
1997-09-01
International Nuclear Information System (INIS)
The interest for medicinal plants has raised again in the last decades, after overcoming a declination period caused by the advances in the researches and development of the synthetic drugs industries. This growing interest has been stimulated mainly by searching cheap and accessible alternative therapies. However, in order to have natural products based treatment in an efficient and safety way, it is necessary to guarantee the plant authenticity, finding adulterations and to assure a low level of microbiological contaminations to avoid damages to consumer's health. The decontamination method should be chosen for eliminating or reduce the microorganisms level without loss of the plant active constituents that would destroy its therapeutic action. At the present work, the possibility of using #gamma# and X electromagnetic radiations to sterilize a Brazilian medicinal plant (Maytenus aquifolium Martius, Celastraceae), which shows anti-ulcer activity, was studied by ...
Energy Technology Data Exchange (ETDEWEB)
Food irradiation is the processing of food products by ionizing radiation in order, among other things, to control food borne pathogens, reduce microbial load and insect infestation, inhibit the germination of root crops, and extend the durable life of perishable products. Irradiation of dried food ingredients, particularly herbs and spices, has a great application potential, and has already been implemented in many countries. Spice irradiation is performed to increase the hygienic quality and used as decontamination processes instead of fumigation methods. European Community approves irradiation processing as an effective residue-free alternative. The present paper evaluates the effect of ionizing radiation on sensorial properties of cinnamon (Laurus cinnamomum) and nut meg (Myristica fragans). The samples have been irradiated in multipurpose irradiator of {sup 60}Co in the doses: 0, 5, 10, 15, 20 e 25 kGy. (author)
2007-07-01
Salmonella radicidation of poultry carcasses
International Nuclear Information System (INIS)
This thesis reports investigations using gamma-radiation to decontaminate poultry carcasses. The application to foods of doses of ionizing radiation sufficient to reduce the number of viable specific non-sporeforming pathogenic microorganisms so that none is detectable in the treated food by any standard method is termed radicidation. The doses used in this study were at such a level that no undesirable or unfavourable side-effects occurred. The effects of these doses were studied on salmonellae and other microorganisms present in, or associated with poultry carcasses and in liquid and on solid culture media as well. Decimal reduction (D_1_0) values were estimated. These represent the dose (kGy) required to achieve a reduction in initial colony count from N_0 to 0.1 N_0. Together with the estimation of the numbers of Salmonella present per carcass the data were used to predict the effect of an ionizing radiation treatment of poultry. Data on the effect of ionizing ...
2005-09-22
Removal of iodine from nuclear fuel reprocessing plant off-gases by Corona discharge
International Nuclear Information System (INIS)
Corona discharge has been investigated for the treatment of off-gases arising from nuclear fuel reprocessing operations, in particular Dissolver off-Gases (DOG). Results are presented of studies carried out on single tube, wire-in-tube experimental rigs to examine the behaviour of molecular iodine, organic iodine and oxides of nitrogen (NOx). The effect of corona current, gas residence time, electrode configuration, oxygen concentration and moisture content are discussed. Decontamination Factors (DF's) of greater than 104 (> 99.99% removal) have been achieved for both molecular and organic iodine. Efficient NOx removal has also been demonstrated. Moisture and NOx both interfere with iodine removal above certain concentrations. To overcome this a two stage corona system has been developed consisting of a primary continuously irrigated corona unit followed by a dehumidifier prior to a secondary dry corona unit.
1991-10-21
Energy Technology Data Exchange (ETDEWEB)
The ROTAMIX process for the treatment of contaminated soils, developed by GSI Environment of Sherbrooke, Quebec, is described. The technology combines the use of a self-propelled rotary turner with bioactivating nutrients and structuring agents. Results of various trials using this process showed that soils contaminated with pentachlorophenol and heavy petroleum hydrocarbons, substances that do not easily break down, were decontaminated to a level that corresponds to the C criterion of the Quebec Ministry of the Environment. The ROTAMIX process was found to improve solid/liquid/gas exchanges, and increased water retention capacity of the treated soil. The technology is not constrained by the fine particle concentration that may result from the addition of structuring agents. It produces no leachate water or gaseous emissions. It broadens the range of contaminants that can be treated, including contaminants that resist biodegradation. The process is relatively cheap ...
1999-02-01
Proposed fuel cycle for the Integral Fast Reactor
Energy Technology Data Exchange (ETDEWEB)
One of the key features of ANL's Integral Fast Reactor (IFR) concept is a close-coupled fuel cycle. The proposed fuel cycle is similar to that demonstrated over the first five to six years of operation of EBR-II, when a fuel cycle facility adjacent to EBR-II was operated to reprocess and refabricate rapidly fuel discharged from the EBR-II. Locating the IFR and its fuel cycle facility on the same site makes the IFR a self-contained system. Because the reactor fuel and the uranium blanket are metals, pyrometallurgical processes (shortned to ''pyroprocesses'') have been chosen. The objectives of the IFR processes for the reactor fuel and blanket materials are to (1) recover fissionable materials in high yield; (2) remove fission products adequately from the reactor fuel, e.g., a decontamination factor of 10 to 100; and (3) upgrade the concentration of plutonium in uranium sufficiently to replenish the fissile-material ...
1985-01-01
Low-Level waste phase 1 melter testing off gas and mass balance evaluation
Energy Technology Data Exchange (ETDEWEB)
Commercially available melter technologies were tested during 1994-95 as part of a multiphase program to test candidate technologies for vitrification of the low-level waste (LLW) stream to be derived from retrieval and pretreatment of Hanford Site tank wastes. Seven vendors were selected for Phase 1 testing to demonstrate vitrification of a high sodium content liquid LLW simulant. The tested melter technologies included four Joule-heated melters, a carbon electrode melter, a combustion melter, and a plasma melter. Various dry and slurry melter feed preparation processes were also tested. Various feed material samples, product glass samples, and process offgas streams were characterized to provide data for evaluation of process decontamination factors and material mass balances for each vitrification technology. This report describes the melter mass balance evaluations and results for six of the Phase 1 LLW melter vendor demonstration tests.
1996-06-28
Energy Technology Data Exchange (ETDEWEB)
The first equipment installed at KfK-HDB was a system with a thin-film evaporator. This was later replaced by two vapor compression evaporating units with forced circulation, for evaporation of liquid LAW, and a steam-heated natural circulation evaporator, for evaporation of liquid MAW. Nuclear activities of the Karlsruhe Nuclear Research Center phasing out, the liquid radwaste quantities to be treated have been shrinking accordingly, so that the current system is planned to be replaced by a smaller system with a thin-film evaporator. (orig./HP) [Deutsch] Im Laufe der Jahre wurde die Anlage mit Duennschichtverdampfer durch zwei Bruedenkompressionsverdampfer mit Zwangsumwaelzung fuer die Eindampfung leicht aktiver waessriger Abfaelle und einem dampfbeheizten Naturumlaufverdampfer fuer die Eindampfung mittelaktiver waessriger Abfaelle ersetzt. Mittlerweile sinkt der Abwasseranfall seit Jahren stetig aufgrund der sinkenden Aktivitaeten des Zentrums auf dem Gebiet der Kerntechnik. Die ...
1994-05-01
International Nuclear Information System (INIS)
Processing of food with ionizing radiation is a method suitable to enhance shelf-life and hygienic quality. Up to a dose of 10 kGy the method is considered wholesome. In many countries the practical use of food irradiation is increasing, however, in the Federal Republic of Germany the process is strictly forbidden. Applications and methods for radiation processing of food are compiled, limits and prospects are explained, and advantages and disadvantages are compared with traditional methods. Identification of irradiated foods and dosimetry and process control for radiation processing of food are areas where further research is needed. Continuous processing of particulate foods in bulk is an application where electron accelerators might be profitable. Beam parameters and velocity distribution of food particles in the treatment area can be matched for an effective result. Thus, dose distribution can be adjusted for homogeneous treatment and at the same time radiation energy is absorbed ...
Intervention for recovery after accidents
International Nuclear Information System (INIS)
The purpose of this document is to provide a framework for developing protective strategies in the longer term following an accidental release of radionuclides to the offsite environment. This advice covers all forms and scales of accidental release, including releases from nuclear sites and reactors, weapons accidents, and damaged industrial or medical sealed sources. The countermeasures considered are those intended to protect the public from external irradiation from radionuclides deposited in the environment, from the inhalation of resuspended radionuclides, and from inadvertent ingestion of radionuclides resulting from contact with contaminated surfaces. The Board terms these recovery countermeasures. They can be broadly grouped as either decontamination measures (ie measures that deal directly with the radionuclides, whether by removing them, shielding them or physically or chemically bonding them) or as restricted access measures (ie measures that reduce ...
Evaluation of actinide biosorption by microorganisms
Energy Technology Data Exchange (ETDEWEB)
Conventional methods for removing metals from aqueous solutions include chemical precipitation, chemical oxidation or reduction, ion exchange, reverse osmosis, electrochemical treatment and evaporation. The removal of radionuclides from aqueous waste streams has largely relied on ion exchange methods which can be prohibitively costly given increasingly stringent regulatory effluent limits. The use of microbial cells as biosorbants for heavy metals offers a potential alternative to existing methods for decontamination or recovery of heavy metals from a variety of industrial waste streams and contaminated ground waters. The toxicity and the extreme and variable conditions present in many radionuclide containing waste streams may preclude the use of living microorganisms and favor the use of non-living biomass for the removal of actinides from these waste streams. In the work presented here, we have examined the biosorption of uranium by non-living, non-metabolizing ...
1996-06-01
International Nuclear Information System (INIS)
The efficacy of gamma irradiation as a method of decontamination for food and herbal materials is well established. In the present study, Glycyrrhiza glabra roots were irradiated at doses 5, 10, 15, 20 and 25 kGy in a cobalt-60 irradiator. The irradiated and un-irradiated control samples were evaluated for phenolic contents, antimicrobial activities and DPPH scavenging properties. The result of the present study showed that radiation treatment up to 20 kGy does not affect the antifungal and antibacterial activity of the plant. While sample irradiated at 25 kGy does showed changes in the antibacterial activity against some selected pathogens. No significant differences in the phenolic contents were observed for control and samples irradiated at 5, 10 and 15 kGy radiation doses. However, phenolic contents increased in samples treated with 20 and 25 kGy doses. The DPPH scavenging activity significantly (p<0.05) increased in all irradiated samples of the plant.
2010-04-01
Development of fission Mo-99 production technology
Energy Technology Data Exchange (ETDEWEB)
This R and D project is planed to supply domestic demands of Mo-99 through fission route, and consequently this project will be expected to rise up utilization of HANARO and KAERI's capability for marketing extension into domestic and oversea radiopharmaceutical market. HEU and LEU target types are decided and designed for fission Mo-99 production in domestic. Experimental study of target fabrication technology was performed and developed processing equipments. And conceptual design of target loading/unloading in/from HANARO device are performed. Tracer test of Mo-99 separation and purification process was performed, test results reach to Mo-99 recovery yield above 80% and decontamination factor above 1600. Combined Mo-99 separation and purification process was decided for hot test scheduled from next year, and performance test was performed. Conceptual design for modification of existing hot cell for fission Mo-99 production facility was performed and ...
2001-05-01
Development of a new evaporator using hydrophobic membrane for radioactive liquid waste
Energy Technology Data Exchange (ETDEWEB)
An evaporator using a hydrophobic membrane made from a polytetrafluoroethylene (PTFE) was developed to improve DF (Decontamination Factor) and to reduce evaporator size. The membrane distillation, provided by the evaporator, is a new technique for liquid purification. Fundamental experiments were carried out to develop the membrane filter (tube type, outer diameter, 8 mm; membrane thickness, 500 {mu}m) for radioactive liquid treatment. The continuous operation test using actual liquid waste was also made during about 3,000 h. (This is almost equal to the operation time of an actual evaporator per year.) The evaporation rate decreased with increase an operation time due to contamination of waste impurity. But the rate was recovered by washing the membrane with hot water and then drying it. DF was over 10{sup 4} which is ten times larger than that for a conventional system. A pilot plant (capacity, 200 kg-liquid waste/h) was constructed and its performance test was ...
1996-10-01
Detection of concealed mercury with thermal neutrons
Energy Technology Data Exchange (ETDEWEB)
In the United States today, governments at all levels and the citizenry are paying increasing attention to the effects, both real and hypothetical, of industrial activity on the environment. Responsible modem industries, reflecting this heightened public and regulatory awareness, are either substituting benign materials for hazardous ones, or using hazardous materials only under carefully controlled conditions. In addition, present-day environmental consciousness dictates that we deal responsibly with legacy wastes. The decontamination and decommissioning (D&D) of facilities at which mercury was used or processed presents a variety of challenges. Elemental mercury is a liquid at room temperature and readily evaporates in air. In large mercury-laden buildings, droplets may evaporate from one area only to recondense in other cooler areas. The rate of evaporation is a function of humidity and temperature; consequently, different parts of a building may be sources ...
1994-08-18
Design and safety evaluation of radioactive gas handling and storage in the FFTF
International Nuclear Information System (INIS)
During the operation of the Fast Flux Test Facility (FFTF), radioactive gases, primarily xenon and krypton, will be produced which will require processing and storing. Two systems have been installed in the FFTF for handling these gases: (1) one to handle, primarily, the reactor cover gas system, and (2) a second to handle the cells and cover gas systems, other than the reactor, whose atmosphere may become contaminated. The system that processes the reactor cover gas, which is argon, is called the Radioactive Argon Processing System (RAPS). The effluent argon from RAPS will normally be sufficiently decontaminated to allow its reuse as the reactor cover gas. If the radioactive level in the RAPS becomes too high, the exhaust stream will be diverted to the Cell Atmosphere Processing System (CAPS), a system which can function as a backup to RAPS. The design and operation of the RAPS and CAPS systems are described and certain safety aspects of the systems are discussed. ...
1976-06-13
Energy Technology Data Exchange (ETDEWEB)
Users of pesticides may have waste or surplus quantities or spills for disposal. One alternative is to deactivate the pesticide at the handling site by using a straightforward chemical reaction. This option can be practical for those who use relatively small quantities of a large variety of pesticides, for example, greenhouse workers, small farmers, and agricultural researchers. This paper describes practical on-site methods for the disposal of spills or small waste quantities of five commonly used pesticides, Diazinon, Chlorpyrifos, Iprodione, 2,4-D, and Captan. These have been tested in the laboratory for the rate of disappearance of the pesticide, the degree of conversion to nontoxic products, the nature and identity of the products, the practicality of the method, and the ease of reproducibility. Methods selected were shown to be safe for the operator, reliable, and reproducible. Greater than 99% of the starting material had to be reacted under reasonable conditions and length of ...
1996-12-31
Energy Technology Data Exchange (ETDEWEB)
A new method for the determination of {sup 237}Np and Pu isotopes in large soil samples has been developed that provides enhanced uranium removal to facilitate assay by inductively coupled plasma mass spectrometry (ICP-MS). This method allows rapid preconcentration and separation of plutonium and neptunium in large soil samples for the measurement of {sup 237}Np and Pu isotopes by ICP-MS. {sup 238}U can interfere with {sup 239}Pu measurement by ICP-MS as {sup 238}UH{sup +} mass overlap and {sup 237}Np via {sup 238}U peak tailing. The method provides enhanced removal of uranium by separating Pu and Np initially on TEVA Resin, then transferring Pu to DGA resin for additional purification. The decontamination factor for removal of uranium from plutonium for this method is greater than 1 x 10{sup 6}. Alpha spectrometry can also be applied so that the shorter-lived {sup 238}Pu isotope can be measured successfully. {sup 239}Pu, {sup 242}Pu and {sup 237}Np were measured ...
2010-07-26
Coir pith of the green coconut in the decontamination of radioactive aqueous effluent
International Nuclear Information System (INIS)
Industrial segments as plant of mining, hospitals and university generate considerable volumes of radioactive wastewater containing uranium. The increasing development of the use of the nuclear energy to lead away to an expansion of the sectors of the nuclear fuel cycle, but it leads to security problems and it appears the necessity of control of the removing of uranium and radioactive effluent treatments. Researches evaluate if the technique of the biosorption would promote an alternative process with attractive characteristics of cost-benefit. The residual biomass from agricultural activities has been studied and used as adsorbent of metals and organic composts by low cost, abundance and for being biodegradable. In this work, it is presented the efficiency of the coir pith for the adsorption of ions UO_2"2"+. The coir pith is a by-product of the harvest of the coconut, a renewable natural source. The study was accomplished using the batch techniques. The influence from pH 2 to 5, the ...
Energy Technology Data Exchange (ETDEWEB)
An economic analysis of the potential advantages of alternatives for recycling and reusing equipment now stored in Building 865 at the Rocky Flats Plant (RFP) in Colorado has been conducted. The inventory considered in this analysis consists primarily of metallurgical and process equipment used before January 1992, during development and production of nuclear weapons components at the site. The economic analysis consists of a thorough building inventory and cost comparisons for four equipment dispositions alternatives. The first is a baseline option of disposal at a Low Level Waste (LLW) landfill. The three alternatives investigated are metal recycling, reuse with the government sector, and release for unrestricted use. This report provides item-by-item estimates of value, disposal cost, and decontamination cost. The economic evaluation methods documented here, the simple cost comparisons presented, and the data provided as a supplement, should provide a foundation ...
1993-08-01
Advanced evaporator technology progress report FY 1992
Energy Technology Data Exchange (ETDEWEB)
This report summarizes the work that was completed in FY 1992 on the program {open_quotes}Technology Development for Concentrating Process Streams.{close_quotes} The purpose of this program is to evaluate and develop evaporator technology for concentrating radioactive waste and product streams such as those generated by the TRUEX process. Concentrating these streams and minimizing the volume of waste generated can significantly reduce disposal costs; however, equipment to concentrate the streams and recycle the decontaminated condensates must be installed. LICON, Inc., is developing an evaporator that shows a great deal of potential for this application. In this report, concepts that need to be incorporated into the design of an evaporator operated in a radioactive environment are discussed. These concepts include criticality safety, remote operation and maintenance, and materials of construction. Both solubility and vapor-liquid equilibrium data are needed to ...
1995-01-01
A simple model for strontium breakthrough on zeolite columns
The Process Waste Treatment Plant (PWTP) at the Oak Ridge National Laboratory is designed to remove radioactive contaminants, principally {sup 90}Sr, from process wastewater. Planned upgrades to the PWTP will use chabazite zeolite columns. Pilot-scale studies have shown that mass transfer zone lengths increase from 10 to about 30 cm as the superficial velocity increases from 5.5 to 22 cm/min. Calculations with a multicomponent equilibrium model showed that the distribution coefficient for strontium remains essentially constant over the process conditions, suggesting that a simple kinetic model (the Rosen long-bed solution) should adequately represent breakthrough behavior. Using a distribution coefficient of 4.87 L/g predicted by the equilibrium model, good agreement was found between experimental breakthrough curves and those calculated with the Rosen solution. This model allows prediction of bed depths and cycle times necessary to achieve the required ...
1995-04-01
Energy Technology Data Exchange (ETDEWEB)
LEDF(Large Equipment Dismantling Facility) is the solid waste processing technology development facility that carries out high-volume reduction and low dosage processing. The high-volume reduction processing of the high dose {alpha}-waste configured with combustible waste, pvc and rubber, spent ion exchange resin, and noncombustible waste have been planned the incinerating and melting facility using the in-can type high frequency induction heating in LEDF. This test is intended to clarify the design data. It was confirmed that the incinerating and melting performance, molten solid properties and exhaust gas processing performance with pilot testing equipment and bench scale equipment. The result of this test are as follows. 1. Processing speed is 6.7 kg/h for the combustible waste, 13.0 kg/h for the ion exchange resin, and 30.0 kg/h for the noncombustible waste. For above optimum processing conditions are as follows. Operating temperature is 1000degC for the combustible waste, 1300degC ...
1999-12-01
All the Spent Nuclear Wastes to Low and Intermediate Level Wastes: PyroGreen
International Nuclear Information System (INIS)
Spent nuclear wastes are inevitable issues to use nuclear power as a sustainable energy. Therefore, every country has their fuel cycles which are best for their environmental and/or political circumstances for the use of nuclear energy. These days agreements are made that spent nuclear fuels should be recycled to minimize waste volume and its toxicity all around the world. Republic of Korea also has a plan to recycle the spent nuclear fuels by using Gen-IV concept burner reactors and pyro-process plants. Not many options of national nuclear strategies are exist because Korea has too many people for its limited land space. KAERI already has been proposing a national fuel cycle concept called 'KIEP-21' that encompasses all the requirements of the advanced nuclear fuel cycle such as reduction of volume, toxicity, HLW heat load and so on. Authors suggest non-national fuel cycle concept called 'PyroGreen' for the sustainable nuclear energy system. PyroGreen is also comprised of ...
2009-06-01
TRITEX. A ferritic steel loop with Pb-15.8Li. Facility and operation
Energy Technology Data Exchange (ETDEWEB)
TRITEX was a pumped loop with Pb-15.8Li, fabricated from steel 1.4922. In contact with the molten eutectic were also molybdenum, vanadium and armco-iron. The loop was originally designed to investigate tritium extraction using solid getter metals. Over the years the goal changed to the study of metals, corrosion products and purification of the eutectic mixture. Therefore many modifications were done. The first part of this report describes TRITEX. All parts were enclosed in thermoboxes for a homogeneous temperature. One test section was in an argon glove box and could be opened during operation. Other special equipment`s were: permeation membranes and liquid-metal-covergas-interfaces to study the transport of H{sub 2}, D{sub 2} and {sup 3}H, different purification devices, a quartz observation window to see the liquid metal surface, 4 different kinds of flow measurements, level indicators, freeze valves. The second part describes loop operation. Between 1989 and ...
1999-05-01
Performance Assessment Monitoring Plan for the Hanford Site Low-Level Burial Grounds
Energy Technology Data Exchange (ETDEWEB)
The U.S. Department of Energy Order 435.1, Radioactive Waste Management, requires a disposal authorization statement authorizing operation (or continued operation) for low-level waste disposal facilities. In fulfillment of these requirements, a disposal authorization statement was issued on October 25, 1999, authorizing the Hanford Site to transfer, receive, possess, and dispose of low-level radioactive waste at the 200 East Area burial grounds and the 200 West Area burial grounds. One of the conditions is that monitoring plans for the 200 East Area and 200 West Area low-level burial grounds be written and approved by the Richland Operations Office. As a result of a record of decision for the Hanford Site Solid Waste Program and acceptance of the Hanford Site Solid Waste Environmental Impact Statement, the use of the low-level burial ground (LLBG) as a disposal facility for low-level and mixed low-level wastes has been restricted to lined trenches and the Navy reactor-compartment ...
2006-03-30
Energy Technology Data Exchange (ETDEWEB)
(methine-{sup 3}H)1,1-Di-(4-chlorophenyl)-2,2,2-trichloroethane ((methine-{sup 3}H)DDT) and its di-(4-nitrophenyl) analog, both of high purity with a moderately high specific activity were prepared. Chloro-benzene was condensed with (1-{sup 3}H)1-(4-chlorophenyl)-2,2,2-trichloro-ethanol, which has been synthesized by sodium boro({sup 3}H)hydride reduction of 4-chlorophenyl trichloromethyl ketone. The purified ({sup 3}H)DDT had a specific activity of 0.77 Ci/mmol (28.49 GBq/mmol). (methine-{sup 3}H)1,1-Diphenyl-2,2,2-trichloroethane was similarly synthesized and was nitrated to give (methine-{sup 3}H)1,1-di-(4-nitrophenyl)-2,2,2-trichloro-ethane of 1.63 Ci/mmol (60.31 GBq/mmol). Dehydrochlorination with housefly enzyme (glutathione-dependent DDT dehydrochlorinase) showed a remarkable isotope effect. For DDT, the observed tritium isotope effect on V{sub max}/K{sub m} was 11.51{plus minus}0.52. For the nitro-analog, the value was 11.3{plus minus}1.2. We measured ...
1989-08-01
Simplified fusion power plant costing. A general prognosis and call for `new think`
Energy Technology Data Exchange (ETDEWEB)
A top-level costing model is developed and used to project the cost of electricity (COE) (in mills per kilo watt-hour) expected from conceptual fusion power plants. Application is restricted to magnetic fusion energy (MFE) concepts. These costs are estimated parametrically in terms of the mass of the fusion-power-core (FPC) heater, the power required to sustain a reacting deuterium-tritium plasma, the heat transport/transfer system that delivers the fusion power to the balance of plant (BOP), and the BOP needed to convert the fusion heat to electrical power. Although the highly integrated (simplified) cost-estimating relationships (CERs) used to express COE in terms of FPC mass power density (MPD) [in kilowatt(electric) per tonne] and the engineering gain Q{sub E} (inverse of fraction of gross electric power recirculated to the fusion power plant) apply primarily to MFE approaches to fusion power, the costing gauge thus results is generally independent of ...
1995-03-01
Shell Temperatures for a Single-Heater Diffuser
Energy Technology Data Exchange (ETDEWEB)
A new diffuser/permeator design has been proposed for a new Savannah River Site tritium project. The use of a single heater well in the center of the shell had raised concerns that the Pd/Ag coils may be shielding radiative heat transfer to the walls thus reducing Pd/Ag tube temperatures near the shell below the recommended minimum operating temperature. The diffuser was fitted with thermocouples to measure shell temperatures during testing. Tests were run with the shell evacuated, helium feed flows of 0, 1000, and 2000 sccm; bleed pressures ranging from 0 to 203 kPa, and heater temperatures of 650, 675, and 700 degrees C. Hydrogen permeation tests were run with two hydrogen/helium mixtures and feed rates to simulate 1st and 2nd stage diffuser operations. Approximately 20 hours were required to bring the diffuser from ambient temperature to steady-state conditions. For tests with a heater temperature of 675 degrees C and no hydrogen flow, helium flow rate and ...
2004-11-01
Role of Fusion Energy in a Sustainable Global Energy Strategy
Energy Technology Data Exchange (ETDEWEB)
Fusion energy is one of only a few truly long-term energy options. Since its inception in the 1950s, the vision of the fusion energy research program has been to develop a viable means of harnessing the virtually unlimited energy stored in the nuclei of light atoms--the primary fuel deuterium is present as one part in 6,500 of all hydrogen. This vision grew out of the recognition that the immense power radiated by the sun is fueled by nuclear fusion in its hot core. Such high temperatures are a prerequisite for driving significant fusion reactions. The fascinating fourth state of matter at high temperatures is known as plasma. It is only in this fourth state of matter that the nuclei of two light atoms can fuse, releasing the excess energy that was needed to separately bind each of the original two nuclei. Because the nuclei of atoms carry a net positive electric charge, they repel each other. Hydrogenic nuclei, such as deuterium and tritium, must be heated to ...
2001-03-07
Energy Technology Data Exchange (ETDEWEB)
Set up in 2004 by the A.C.R.O. the citizens network of radioecological surveillance, information and evaluation (R.I.V.I.E.R.E.) aims at making a follow-up of the radioactive contamination of the aquatic ecosystems on the scale of the Seine-Normandy pond: from Nogent-on-Seine to La Hague and from the Mont-Saint-Michel to the Treport. The peculiarity of this network, which also makes its strength is to associate strictly all those who wish to appropriate the knowledge of the radioactivity levels around to them. With R.I.V.I.E.R.E., the citizen is at the same moment an author and an actor of the surveillance of his environment as his information. An approach defended by the A.C.R.O. since about 20 years and which has no equivalent anywhere else. This project has four main objectives: to know the levels and the tendencies of the present radioactivity in the main aquatic ecosystems of the Seine-Normandy widened pond, and so feed a data base including more than 3000 analysis (limited to the ...
2005-07-01
Research and development on plasma facing components for fusion reactors in JAEA
International Nuclear Information System (INIS)
This paper presents the present status of R and D activities on plasma facing components for fusion reactors, such as International Thermonuclear Experimental Reactor (ITER) and fusion demonstration reactor (DEMO). The plasma facing components (PFCs) as typified by divertor and first wall components are subjected to high heat flux and particle flux from fusion plasma. It is essential for these components to have sufficient heat removal capability and robust structure against those loadings. JAEA has been carried out to develop the ITER-PFCs which consist of copper alloys and armor materials with high thermal conductivity, such as carbon fiber composites, tungsten and beryllium. The demonstration of the thermomechanical performance of the ITER-PFCs by using mock-ups has successfully been made under close mutual cooperation between the participant countries of ITER. Currently, the activity on the development of the ITER-PFCs is in a qualification phase prior to the bulk production for ...
2008-10-13
Modelling of multifrequency IRMPD for laser isotope separation
International Nuclear Information System (INIS)
The process of infrared multiple photon dissociation (IRMPD) of molecules is of great fundamental importance and has practical significance, such as isotope separation etc. Unfortunately, a clear insight into the process has been hindered by the bewildering array of important variables affecting MPD. The dissociation probability #gamma#(#phi#) i.e. the yield has been found to be a sensitive function of laser fluence #phi# along with numerous other parameters like laser frequency, gas pressure etc. We have shown that in single frequency IRMPD an accurate quantitative characterization of the dissociation probability can be adequately expressed by a 'power law' model with two fitting parameters namely critical fluence, #phi#c and multi photon order, m. This model was exploited in analysing our MPD results on various systems. However, the small isotope shift encountered in heavy elements and the sticking phenomenon observed in small light molecules restrict respectively the separation ...
2002-12-01
F-Area Seepage Basins groundwater monitoring report -- third and fourth quarters 1993. Volume 1
Energy Technology Data Exchange (ETDEWEB)
During the second half of 1993, the groundwater at the F-Area Seepage Basins (FASB) was monitored in compliance with Module 3, Section C, of South Carolina Hazardous Waste Permit SC1-890-008-989, effective November 2, 1992. The monitoring well network is composed of 87 FSB wells screened in the three hydrostratigraphic units that make up the uppermost aquifer beneath the FASB. A detailed description of the uppermost aquifer is included in the Resource Conservation and Recovery Act Part B post-closure care permit application for the F-Area Hazardous Waste Management Facility submitted to the South Carolina Department of Health and Environmental Control (SCDHEC) in December 1990. Beginning in the first quarter of 1993, the standard for comparison became the SCDHEC Groundwater Protection Standard (GWPS) specified in the approved F-Area Seepage Basins Part B permit. Currently and historically, gross alpha, nitrate, nonvolatile beta, and tritium are among the primary ...
1994-03-01
Excitation function of "5"9 Co (n, 2n) "5"8 Co process in the energy range 13.9-14.7 MeV
International Nuclear Information System (INIS)
The objective of the study is to measure the neutron cross sections for the "5"9 Co (n, 2n) "5"8 Co reaction around the 14 MeV energy region. Neutron activation cross section for almost all the nuclei, mostly in the medium energy region e.g., 7 to 20 MeV are reported in literature. Neutron cross section data around 14 MeV is of immense importance for the design of D + T fusion reactors. The accuracy of the cross section data at this energy region is a requirement for correct prediction of reactor parameters e.g., tritium breeding, nuclear heating, induced activity, etc. In order to perform the experiment, the Co-sample sandwiched in Ni foils was irradiated employing the J-25 Neutron Generator at the AERE, Savar, Dhaka. After irradiation, the counting was done by the activation technique using a high resolution Hp Ge gamma ray spectrometer. The gamma ray spectra was analyzed in a Canberra series-40 Multi-channel Analyzer. Calculations for cross sections were done at ...
Electrodeless, multi-megawatt reactor for room-temperature, lithium-6/deuterium nuclear reactions
International Nuclear Information System (INIS)
This paper describes a reactor design to facilitate a room-temperature nuclear fusion/fission reaction to generate heat without generating unwanted neutrons, gamma rays, tritium, or other radioactive products. The room-temperature fusion/fission reaction involves the sequential triggering of billions of single-molecule, "6LiD 'fusion energy pellets' distributed in lattices of a palladium ion accumulator that also acts as a catalyst to produce the molecules of "6LiD from a solution comprising D_2O, "6LiOD with D_2 gas bubbling through it. The D_2 gas is the source of the negative deuterium ions in the "6LiD molecules. The next step is to trigger a first nuclear fusion/fission reaction of some of the "6LiD molecules, according to the well-known nuclear reaction: "6Li + D #-># 2"4He + 22.4 MeV. The highly energetic alpha particles ("4He nuclei) generated by this nuclear reaction within the palladium will cause shock and vibrations in the palladium lattices, leading ...
Diffusion of lithium-6 isotopes in lithium aluminate ceramics using neutron depth profiling
International Nuclear Information System (INIS)
Lithium Ceramics offer tremendous potential as a source for the production of tritium ("3H) for fusion power reactors. Their successful application will depend to a great extent upon the diffusion properties of the "6Li within the matrix. Consequently knowledge of "6Li concentration gradients in the ceramic matrices is an important requirement in the continued development of the technology. In this investigation, the neutron depth profile (NDP) technique has been applied to the study of concentration profiles of "6Li in lithium aluminate ceramics, doped with 1.8%, 50% and 95% "6Li isotopic concentrations. Specimen for analysis were prepared at Battelle (PNL) as pellet discs. Samples for diffusion studies were arranged as diffusion couples in the following manner: 1.8% "6Li discs/85% "6Li powder. Experiments were performed at the Texas A and M Nuclear Science Center Reactor Building, utilizing 1 MW equivalent thermal neutron fluxes 3x10"1"1 n/m"2 s. The depth probed ...
APSTNG: Neutron interrogation for detection of nuclear and CW weapons, explosives, and drugs
Energy Technology Data Exchange (ETDEWEB)
A recently developed neutron diagnostic probe system has the potential to satisfy a significant number of van-mobile and fixed- portal requirements for nondestructive verification of sealed munitions and detection of contraband explosives and drugs. The probe is based on a unique associated-particle sealed-tube neutron generator (APSTNG) that interrogates the object of interest with a low-intensity beam of 14-MeV neutrons generated from the deuterium-tritium reaction and that detects the alpha-particle associated with each neutron. Gamma-ray spectra of resulting neutron inelastic scattering and fission reactions identify nuclides associated with all major chemicals in chemical warfare agents, explosives, and drugs, as well as many pollutants and fissile and fertile special nuclear material. Flight times determined from determined from detection times of the gamma-rays and alpha-particles yield a separate tomographic image of each identified nuclide. The APSTNG also ...
1992-07-01
A.C.R.O. activity report 1999; A.C.R.O. rapport d'activite scientifique 1999
Energy Technology Data Exchange (ETDEWEB)
The work of this association is cut according to 6 axes. Three publications: radiological quality of marine and continental waters of the Normandy coast (synthesis 1997 and 1998); preliminary study of the iodine 129 distribution in the environment of the reprocessing plant of La Hague with terrestrial moss (Homalotecium sericeum); radiological surveillance of the aquatic environment of the nuclear facilities on the area of La Hague (1997 and 1998). The second axis concerns the radiation protection with a campaign of radon measures in a school of the Vire rural district (june 1999). The third part is devoted to the radioecology with the surveillance of radioactivity in the aquatic continental environment of nuclear facilities and the radioecological surveillance (1999) of the building site of Cogema la Hague in the area of tidal range of the Moulinets cove. The fourth part concerns the radioactive waste and environment, with the study of the distribution of the artificial gamma emitters ...
1999-07-01
Energy Technology Data Exchange (ETDEWEB)
This report is a compilation of the calendar year 2003 groundwater sampling results from the Area 5 Radioactive Waste Management Site, Nevada Test Site. Wells Ue5PW-1, Ue5PW-2, and Ue5PW-3 were sampled semi-annually for the required analytes: pH, specific conductance, total organic carbon (TOC), total organic halides (TOX), tritium, and major cations/anions. Results from all samples collected in 2003 were within established criteria. These data indicate that there has been no measurable impact to the uppermost aquifer from the Resource Conservation and Recovery Act (RCRA) regulated unit within the Area 5 Radioactive Waste Management Site and confirm that any previous detections of TOC and TOX were false positives. Contamination indicator data are presented in control chart and tabular form with investigation levels indicated. Gross water chemistry data are presented in graphical and tabular form. There were no major changes noted in the monitored groundwater ...
2004-02-01
International Nuclear Information System (INIS)
An efficient adsorption process is developed for the decontamination of trivalent chromium from tannery effluents. A low cost activated carbon (ATFAC) was prepared from coconut shell fibers (an agricultural waste), characterized and utilized for Cr(III) removal from water/wastewater. A commercially available activated carbon fabric cloth (ACF) was also studied for comparative evaluation. All the equilibrium and kinetic studies were conducted at different temperatures, particle size, pHs, and adsorbent doses in batch mode. The Langmuir and Freundlich isotherm models were applied. The Langmuir model best fit the equilibrium isotherm data. The maximum adsorption capacities of ATFAC and ACF at 25 deg. C are 12.2 and 39.56 mg/g, respectively. Cr(III) adsorption increased with an increase in temperature (10 deg. C: ATFAC-10.97 mg/g, ACF-36.05 mg/g; 40 deg. C: ATFAC-16.10 mg/g, ACF-40.29 mg/g). The kinetic studies were conducted to delineate the effect of temperature, ...
2006-07-31
Energy Technology Data Exchange (ETDEWEB)
Since the 1970 innovations have allowed both active and passive neutron techniques to address various safeguards and waste measurement needs in the DOE complex. Much research was focused on satisfjring the 100-nCi/g detection limit for TRU waste in 208-liter drums. The emphasis on measuring drum-sized containers for disposal at WIPP has resulted in improved waste assay capability that now needs to be extended to larger containers. The desire to expedite the decontamination and decommissioning of certtain DOE facilities, and the large waste encountered in that process, has prompted the need for increasingly large disposal containers. Instruments have recently been built to accommodate crates that are nearly 100 cubic feet in volume, such as a B-25 box or Standard Waste 13ox. The density of hydrogen inside a waste container profoundly affects the accuracy of neutron measurements, and the metal content greatly affects sensitivity. Depending on the matrix, and ...
2001-01-01
D & D screening risk evaluation guidance
Energy Technology Data Exchange (ETDEWEB)
The Screening Risk Evaluation (SRE) guidance document is a set of guidelines provided for the uniform implementation of SREs performed on decontamination and decommissioning (D&D) facilities. Although this method has been developed for D&D facilities, it can be used for transition (EM-60) facilities as well. The SRE guidance produces screening risk scores reflecting levels of risk through the use of risk ranking indices. Five types of possible risk are calculated from the SRE: current releases, worker exposures, future releases, physical hazards, and criticality. The Current Release Index (CRI) calculates the current risk to human health and the environment, exterior to the building, from ongoing or probable releases within a one-year time period. The Worker Exposure Index (WEI) calculates the current risk to workers, occupants and visitors inside contaminated D&D facilities due to contaminant exposure. The Future Release Index (FRI) calculates the ...
1995-09-01
Closure Report for Corrective Action Unit 543: Liquid Disposal Units, Nevada Test Site, Nevada
Energy Technology Data Exchange (ETDEWEB)
This Closure Report (CR) documents closure activities for Corrective Action Unit (CAU) 543, Liquid Disposal Units, according to the Federal Facility Agreement and Consent Order (FFACO, 1996) and the Corrective Action Plan (CAP) for CAU 543 (U.S. Department of Energy, National Nuclear Security Administration Nevada Site Office [NNSA/NSO], 2007). CAU 543 is located at the Nevada Test Site (NTS), Nevada (Figure 1), and consists of the following seven Corrective Action Sites (CASs): CAS 06-07-01, Decon Pad; CAS 15-01-03, Aboveground Storage Tank; CAS 15-04-01, Septic Tank; CAS 15-05-01, Leachfield; CAS 15-08-01, Liquid Manure Tank; CAS 15-23-01, Underground Radioactive Material Area; CAS 15-23-03, Contaminated Sump, Piping; and CAS 06-07-01 is located at the Decontamination Facility in Area 6, adjacent to Yucca Lake. The remaining CASs are located at the former U.S. Environmental Protection Agency (EPA) Farm in Area 15. The purpose of this CR is to provide a summary of ...
2008-01-01
Energy Technology Data Exchange (ETDEWEB)
The precipitation of heavy metals as hydroxides is the standard technique for the decontamination of waste water streams polluted by these elements. On the other side, progress in research has been made concerning the biosorption onto dead biomass and bioprecipitation supported by physiologically active bacteria. As the aim of this study, a flexible strategy has been envisaged cleaning a waste water with definite heavy metal load underlying the process mentioned above. Suitable bacteria were enriched and the process was tested in a technical plant. As result, a very high efficiency of heavy metal elimination has been found. The field of application covered by the acquired process is identical with the whole range of the waste water streams polluted by heavy metals. In addition, a second stage may be necessary if there are any further contaminants to be removed. (orig.) [Deutsch] Bei der Reinigung von schwermetallhaltigen Abwaessern ist der derzeitige Stand der ...
1996-12-31
Biological and Chemical Security
The LLNL Chemical & Biological National Security Program (CBNP) provides science, technology and integrated systems for chemical and biological security. Our approach is to develop and field advanced strategies that dramatically improve the nation's capabilities to prevent, prepare for, detect, and respond to terrorist use of chemical or biological weapons. Recent events show the importance of civilian defense against terrorism. The 1995 nerve gas attack in Tokyo's subway served to catalyze and focus the early LLNL program on civilian counter terrorism. In the same year, LLNL began CBNP using Laboratory-Directed R&D investments and a focus on biodetection. The Nunn-Lugar-Domenici Defense Against Weapons of Mass Destruction Act, passed in 1996, initiated a number of U.S. nonproliferation and counter-terrorism programs including the DOE (now NNSA) Chemical and Biological Nonproliferation Program (also known as CBNP). In 2002, the Department of Homeland Security ...
2002-12-19
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