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1

[sup 3]He([ital n],[gamma])[sup 4]He cross section and the photodisintegration of [sup 4]He  

Energy Technology Data Exchange (ETDEWEB)

The absolute cross section of the [sup 3]He([ital n],[gamma])[sup 4]He reaction was measured at five energies between [ital E][sub [ital n

1993-11-01

2

Geometrical aspects of reaction cross sections for {sup 3}He, {sup 4}He and {sup 12}C projectiles  

Energy Technology Data Exchange (ETDEWEB)

A black-disc model combined with accurate matter densities has been used for an investigation of reaction cross sections for {sup 3}He, {sup 4}He and {sup 12}C projectiles. A simple relation is derived between the energy dependence of the reaction cross sections and the strength of the nucleon-nucleon interaction. A comparison is also made of the reaction cross sections for {sup 3}He and {sup 4}He for six different nuclei {sup 12}C, {sup 16}O, {sup 40}Ca, {sup 58,60}Ni and {sup 208}Pb.

2003-04-01

3

Traditional Fusion reaction: D + T n (14.07 MeV) + 4He (3.52 MeV ...  

Science.gov (United States)

as for direct energy conversion in specialized direct electrical energy conversion plants. Figure 1. An energetic (~163KeV) proton and a 11boron nucleus fuse ...

4

Superfluid 4He interferometer operating near 2 K  

International Nuclear Information System (INIS)

We report the observation of quantum interference in superfluid 4He. The interferometer, an analog of a dc-superconducting quantum interference device (SQUID), employs a recently reported phenomenon wherein superfluid 4He exhibits Josephson frequency oscillations in an array of submicron apertures. An interference pattern is generated by reorienting the loop of the superfluid 'SQUID' with respect to the Earth's rotation vector, thereby varying the rotation flux in the loop. The experiment is performed at 2 K, a temperature 2000 times higher than previously achieved with superfluid 3He. We find that the interference exists not only when the aperture array current-phase relation is a sinusoidal function characteristic of the Josephson effect, but also at lower temperatures where it is linear and oscillations occur by phase slips. The modest requirements for the interferometer (2 K cryogenics and ...

2006-09-01

5

Pion-induced fission  

Energy Technology Data Exchange (ETDEWEB)

The A(..pi../sup +/,/sup 3/He)B reaction near threshold is studied in a model where the pion is absorbed by an /sup 4/He constituent of the target nucleus. The predictions of this model using harmonic oscillator cluster wave functions agree semi-quantitatively with the experimental data on the inverse reaction.

1982-03-10

6

Heat capacity measurements of atoms and molecules adsorbed on evaporated metal films  

Energy Technology Data Exchange (ETDEWEB)

Investigations of the properties of absorbed monolayers have received great experimental and theoretical attention recently, both because of the importance of surface processes in practical applications such as catalysis, and the importance of such systems to the understanding of the fundamentals of thermodynamics in two dimensions. We have adapted the composite bolometer technology to the construction of microcalorimeters. For these calorimeters, the adsorption substrate is an evaporated film deposited on one surface of an optically polished sapphire wafer. This approach has allowed us to make the first measurements of the heat capacity of submonolayer films of /sup 4/He adsorbed on metallic films. In contrast to measurements of /sup 4/He adsorbed on all other insulating substrates, we have shown that /sup 4/He on silver films occupies a two-dimensional gas ...

1989-05-01

7

Big bang nucleosynthesis  

Energy Technology Data Exchange (ETDEWEB)

The concordance of standard big bang nucleosynthesis theory and the related observations of the light element isotopes (including some new higher {sup 4}He abundances) will be reviewed. Implications of BBN on chemical evolution, dark matter and constraints on particle properties will be discussed.

1999-01-01

8

Annealing behavior of radiation damages in metal-silicides  

International Nuclear Information System (INIS)

The annealing behavior of the radiation damage in epitaxial Pd_2Si and NiSi_2 films on Si, due to the implantation of 100 keV Ar ions, is investigated by using the channeling technique with "4He ions. (U.K.).

9

Effects of the variation of fundamental constants on Pop III stellar evolution  

International Nuclear Information System (INIS)

The effect of variations of the fundamental constants on the thermonuclear rate of the triple alpha reaction, "4He(#alpha##alpha#, #gamma#)"1"2C, that bridges the gap between "4He and "1"2C is investigated. We have followed the evolution of 15 and 60 M#centre dot# zero metallicity stellar models, up to the end of core helium burning. They are assumed to be representative of the first (Population III) stars. The calculated oxygen carbon abundances resulting from helium burning can then be used to constrain the variation of the fundamental constants.

2010-08-12

10

Neutron magnetic form factor G{sub M}{sup n}(Q{sup 2}) from quasielastic inclusive scattering data on D and {sup 4}He  

Science.gov (United States)

We analyze cross sections for quasielastic inclusive scattering of electrons on nuclei and show that the observed isolated peaks for relatively low Q{sup 2} are unique for the lightest targets. Focusing, in particular, on D and {sup 4}He, we investigate in two ways to what measure the above peaks can be allocated to nucleon-elastic processes. We first compute approximate upper limits for the nucleon-inelastic background in the quasielastic region due to inclusive {delta} excitation, and find those to be small. Far more precise is a semiphenomenological approach, where the dominance of nucleon-elastic processes is translated into a set of stringent requirements. We show that those are very well fulfilled for recent D data, and to a somewhat lesser extent for older D and {sup 4}He data. With knowledge of G{sub E,M}{sup p} and information on G{sub E}{sup n}, we then extract G{sub M}{sup n} and find ...

2004-07-01

11

Neutron magnetic form factor G_M"n(Q"2) from quasielastic inclusive scattering data on D and "4He  

International Nuclear Information System (INIS)

We analyze cross sections for quasielastic inclusive scattering of electrons on nuclei and show that the observed isolated peaks for relatively low Q"2 are unique for the lightest targets. Focusing, in particular, on D and "4He, we investigate in two ways to what measure the above peaks can be allocated to nucleon-elastic processes. We first compute approximate upper limits for the nucleon-inelastic background in the quasielastic region due to inclusive #DELTA# excitation, and find those to be small. Far more precise is a semiphenomenological approach, where the dominance of nucleon-elastic processes is translated into a set of stringent requirements. We show that those are very well fulfilled for recent D data, and to a somewhat lesser extent for older D and "4He data. With knowledge of G_E_,_M"p and information on G_E"n, we then extract G_M"n and find agreement with values obtained by alternative ...

2004-07-01

12

Energy spectra and electromagnetic properties in lithium isotopes  

International Nuclear Information System (INIS)

Li shell-model calculation has been made in the isospin formalism in the complete (0 + n)#Planck constant##omega# model space with the assumption of a closed core "4He. The calculation could probably be improved by use of a better effective interaction and increasing shell model space. With the use of faster computer with large memories, the authors are in hope of calculation in spsd shell-model space

13

Tensor polarization of the residual nucleus in the "6Li (#alpha#, #alpha#') "6Li (2.18 MeV, 3"+) reaction at E_#alpha# = 27.2 MeV  

International Nuclear Information System (INIS)

The experiment on the determination of the tensor polarization of the residual nucleus is described for the reaction "6Li (#alpha#, #alpha#') "6Li. It is based on the unique connection of polarization tensors t_l_m of the residual nucleus for the reaction (#alpha#, #alpha#') and the angular correlation function W (#omega#_1, #omega#_2) for #alpha#'-particle and decay product of this nucleus, where #omega#_1, #omega#_2 are motion directions of #alpha#'-particle and decay product. The angular correlations of #alpha#'-particle and deuteron are measured for the "6Li (#alpha#, #alpha#', d)"4He reaction on the 27.2 MeV #alpha#-particle beam. The recording system consists of six silicon detectors and provides the energy resolution about 0.8 MeV and the angular resolution #+-# 3 deg. The polarization tensors of the residual nucleus "6Li (2.185 MeV, 3"+) are determined as the result of measuring the angular correlations of products of the "6Li (#alpha#, ...

1999-01-01

14

Multi-nucleon transfer reactions and the formation of light charged particles in the system sup(nat)Ag + /sup 40/Ar(285MeV)  

Energy Technology Data Exchange (ETDEWEB)

In the reaction sup(nat)Ag + /sup 40/Ar (285 MeV) there have been measured the energy spectra of the isotopes of elements from H to Cl at an emission angle of 40/sup 0/, the energy spectra and angular distributions of /sup 1/H, /sup 2/H, /sup 3/H, and /sup 4/He, and the angular distributions of Li, Be, B, and C. The contribution from multinucleon transfer reactions to the formation of light charged particles is discussed.

1981-11-01

15

Distribution of 6 q functions in nuclei and quark enhancement of hard processes with deuteron emission  

International Nuclear Information System (INIS)

"2H, "4He, "1"6O, "4"0Ca, "8"0Zr, "1"4"0Yb, "2"2"4112, "3"3"6168 nuclei are invesigated in terms of flucton model. Effective numbers of nuclear fluctons and deuterons are calculated. Values of complete effective numbers of low-radius deuterons and fluctons with S=1 spin and T=0 isospin are presented. Investigation results of inclusive reactions of quasi-elastic knock-out of deuterons by fast protons are discussed. 9 refs.; 1 fig.; 1 tab.

1988-06-14

16

Light charged particles and intermediate mass fragments from the reactions 486, 550, 640, and 730 MeV [sup 86]Kr + [sup 63]Cu  

Energy Technology Data Exchange (ETDEWEB)

A study has been made of the reaction [sup 86]Kr + [sup 63]Cu at incident energies of 486, 550, 640, and 730 MeV. Measurements include cross sections, angular distributions, and energy spectra for light charged particles ([sup 1,2,3]H and [sup 4]He), intermediate mass fragments (IMF) (4 [le] Z [le] 17), and heavy fragments (Z [ge] 18). Coincidences between light charged particles and between particles and fragments have been measured to obtain cross sections, energy spectra, and angular distributions. Statistical model analysis of the energy spectra for [sup 1]H and [sup 4]He detected in coincidence with the fragments has allowed estimation of [sup 1]H and [sup 4]He multiplicities associated with the evaporation residues, fragments, and composite nuclei prior to scission. A comparison of cross sections, energy spectra, angular distributions, and particle ...

1992-01-01

17

Total nuclear photoabsorption cross section in the range 0.2-1.0 GeV for nuclei throughout the periodic table  

International Nuclear Information System (INIS)

An analysis of the total photoabsorption cross section for nuclei ranging from "4He up to "2"3"8U has been performed in the energy range 0.2-1.0 GeV. Mean total photoabsorption cross sections have been obtained by summing up the contributions from partial photoreactions, and found to follow an A"1-dependence in the 0.2-1.0 GeV range. A review of the available total photoabsorption cross section data is also presented. Comparisons have been made with cross section values calculated by considering both the quasi-deuteron and #pi#-meson photoproduction mechanism of primary nuclear photointeraction. (orig.).

18

Radiochemical investigations of nuclear properties. Progress report, October 1, 1976--September 30, 1977  

International Nuclear Information System (INIS)

Progress in experimental investigations of high spin excitations in spherical and transitional nuclei in the A = 180 to 204 mass range is described. Most of the experiments were performed by in-beam #gamma#-ray spectroscopy using beams of "3He, "4He, and "1"2C ions from the Michigan State University cyclotron. The main results of studies of the nuclei "1"9"5 "1"9"7 "1"9"9 "2"0"1 "2"0"2 "2"0"3Pb, "1"9"6 "1"9"7 "1"9"9 "2"0"0Hg and "1"8"6 "1"8"7 "1"8"8 "1"8"9Pt are summarized.

19

Neutrino cross sections with the MINER?A Experiment  

British Library Electronic Table of Contents (United Kingdom)

MINER?A is a high resolution, fully active detector designed to study neutrino interactions on nuclei in the NuMI beam at Fermi National Accelerator Laboratory. The active volume of the detector consists of 3 tons of plastic scintillator and includes embedded targets of 4He, C, H2O, Fe and Pb. The MINER?A collaboration expects to perform precision, A-dependent neutrino cross section measurements in the 1?10 GeV region, measure the axial form factor, and study nuclear shadowing of F2, quark-hadron duality and coherent pion production, among other topics. MINER?A began data taking in the fall of 2009. This paper describes the MINER?A experiment and provides an overview of the physics objectives along with estimated uncertainties of the measurements and the tentative projected schedule of dat...

2011-01-01

20

Near-threshold {eta}-meson production in the dd{yields}He{eta} reaction  

Energy Technology Data Exchange (ETDEWEB)

The dd{yields}{sup 4}He{eta} reaction has been investigated near threshold using the ANKE facility at COSY-Juelich. Both total and differential cross-sections have been measured at two excess energies, Q=2.6 MeV and 7.7 MeV, with a subthreshold measurement being undertaken at Q=-2.6 MeV to study the physical background. While consistent with isotropy at the lower energy, the angular distribution reveals a pronounced anisotropy at the higher one, indicating the presence of higher partial waves. Options for the decomposition into partial amplitudes and their consequences for the determination of the s-wave {eta}{alpha} scattering length are discussed. (orig.)

2005-12-01

 
 
 
 
21

Momentum transfer in 30-200 MeV/sup 4/He induced reaction with /sup 59/Co  

Energy Technology Data Exchange (ETDEWEB)

Thick-target recoil ranges of radioactive nuclei produced in 30-200 MeV alpha-particle bombardment of /sup 59/Co have been used to deduce the longitudinal momentum transfer per projectile nucleon (psub(parallel)/A) as a function of residue mass and bombarding energy. The average value of psub(parallel)/A increases monotonically with bombarding energy and reaches a maximum value of proportional160 MeV/c at proportional23 MeV/u, and decreases thereafter. The maximum value of psub(parallel)/A is equal to the incident momentum up to proportional23 MeV/u and saturates at a value of proportional220 MeV/c beyond this energy.

1984-03-01

22

Measurements and calculations of M-shell X-ray production in Er, Yb and Lu by 0.75-6 MeV He ions  

Energy Technology Data Exchange (ETDEWEB)

M-shell X-ray production cross sections for the light rare-earth elements of {sup 68}Er, {sup 7}Yb and {sup 71}Lu have been measured for incident {sup 4}He{sup +} ions in the energy range from 0.75 to 6 MeV. The measured X-ray production cross sections are compared to the predictions of the First Born approximation, the ECPSSR theory and the ECUSAR theory. A comparison of the ytterbium M-shell X-ray production cross sections with these theories is made for two different sets of fluorescence yields and Coster-Kronig factors that are further modified for multiple ionization.

2005-12-15

23

Ion-induced phase formation in metal-silicon systems. [Xenon ion implantation effects  

Energy Technology Data Exchange (ETDEWEB)

By using megaelectronvolt /sup 4/He ion backscattering techniques and transmission electron microscopy, the authors have investigated the interactions of ion beams with thin film structures in a number of silicide-forming systems. The mixed layer was found to be an equilibrium compound for near-noble metals and an amorphous phase for refractory metals. Differences in behavior have also been observed in near-noble metal systems. For palladium, the Pd/sub 2/Si phase grew with ion dose and remained crystalline up to high dose. For nickel, the compound Ni/sub 2/Si was formed initially and became amorphous on prolonged irradiation. All the results indicate the significance of atomic mobility at target temperatures in determining the phase formation and in explaining the sensitivity of the silicides to ion bombardment.

1985-01-11

24

Ion-induced phase formation in metal-silicon systems  

International Nuclear Information System (INIS)

By using megaelectronvolt "4He ion backscattering techniques and transmission electron microscopy, the authors have investigated the interactions of ion beams with thin film structures in a number of silicide-forming systems. The mixed layer was found to be an equilibrium compound for near-noble metals and an amorphous phase for refractory metals. Differences in behavior have also been observed in near-noble metal systems. For palladium, the Pd_2Si phase grew with ion dose and remained crystalline up to high dose. For nickel, the compound Ni_2Si was formed initially and became amorphous on prolonged irradiation. All the results indicate the significance of atomic mobility at target temperatures in determining the phase formation and in explaining the sensitivity of the silicides to ion bombardment. (Auth.).

25

Investigation of nuclear fusion in reaction of "4","6He and "7Li on "2"0"8Pb and "2"0"9Bi nuclei  

International Nuclear Information System (INIS)

One measured fission and fusion cross sections of "4","6He+"2"0"9Bi and "7Li+"2"0"8Pb reactions within the range from the Coulomb barrier up to 200 MeV. The measured functions of fission and fusion for the mentioned reactions are shown to have close values within the excitation energy wide range. One analyzed the excitation functions of fusion and fission for "4He+"2"0"9Bi, "6He+"2"0"9Bi and "7Li+"2"0"8Pb reactions resulting in formation of "2"1"3","2"1"5At compound systems

2006-11-01

26

Determination of the helium thermal diffusion coefficient in britholite using a NRA method: new results  

International Nuclear Information System (INIS)

Dimensioning of actinides waste packages for long duration storage has to take into account helium production from natural decay and release rates from the material. For the latter, we propose here an improved method for the determination of the helium diffusion coefficient in britholite, to be used for minor actinides storage. This work is based on results we previously published using the classical three steps method: "3He implantation on a Van de Graaff facility, "3He profile determination analysing the protons resulting from the "3He(d,p)"4He reaction in a nuclear microprobe, evolution of the helium profile during annealings. Taking explicitly into account the incident deuterons energy stragglings allows us to show that the implanted helium profiles are bimodal, each component leading to a different helium diffusion coefficient.

2005-02-01

27

Cyclotron produced lead-203  

International Nuclear Information System (INIS)

The radioactive isotopes of lead are reviewed with respect to their choice for in vitro tracer studies. The #gamma#-photon energy and absence of particle emission in the decay of "2"0"3Pb makes it particularly suitable for these applications. Reaction yields of "2"0"3Pb using "2"0"3Tl targets and proton, deuteron, "3He and "4He beams are listed. Using the preferred reaction "2"0"3Tl (d, 2n)"2"0"3Pb with a 15 MeV deuteron beam, yields of about 75 #mu#Ci #mu#Ahr"-"1, after chemical separation, are reported. Details of target design and chemical separation are given. (U.K.).

28

Studies of weak hcp "3He-"4He solution decomposition and magnetic properties of decomposed samples  

International Nuclear Information System (INIS)

The information is reported on the kinetics of decomposition of weak hcp "3He-"4He solutions with the starting "3He concentration 0.5#+-#0.1% and 1.20#+-#0.2% under the sample pressure 3.5 to 3.8 MPa before the decomposition. The NMR technique of the prompt control of the phase separation process is developed. To accelerate the metastable phase decomposition, the samples were thermally cycled at temperatures below 100 mK. Using the pulse NMR method, the magnetic susceptibility of "3He nuclei and the spin-lattice T_1 and spin-spin T_2 relaxation times were measured on three samples of the decomposed solid solutions with the starting "3He concentration 0.5% at the pressures 3.53, 3.71 and 3.78 MPa. Above 10 mK the Curie-Weiss constant was two to three times higher than the values typical of bulk bcc "3He of the corresponding density. Below 10 mK the magnetic susceptibility was observed to deviate from the Curie-Weiss law. One of the samples ...

29

Electrodeless, multi-megawatt reactor for room-temperature, lithium-6/deuterium nuclear reactions  

International Nuclear Information System (INIS)

This paper describes a reactor design to facilitate a room-temperature nuclear fusion/fission reaction to generate heat without generating unwanted neutrons, gamma rays, tritium, or other radioactive products. The room-temperature fusion/fission reaction involves the sequential triggering of billions of single-molecule, "6LiD 'fusion energy pellets' distributed in lattices of a palladium ion accumulator that also acts as a catalyst to produce the molecules of "6LiD from a solution comprising D_2O, "6LiOD with D_2 gas bubbling through it. The D_2 gas is the source of the negative deuterium ions in the "6LiD molecules. The next step is to trigger a first nuclear fusion/fission reaction of some of the "6LiD molecules, according to the well-known nuclear reaction: "6Li + D #-># 2"4He + 22.4 MeV. The highly energetic alpha particles ("4He nuclei) generated by this nuclear reaction within the palladium ...

30

High spin states of some nuclei around the N=Z=28 double closed shell  

Energy Technology Data Exchange (ETDEWEB)

A spectroscopic study is performed for high spin states of {sup 55}Fe, {sup 55}Co and {sup 57}Ni. To populate the investigated residues with a relevant cross section, the fusion evaporation reactions of {sup 30}Si({sup 28}Si, 2pn){sup 55}Fe, {sup 30}Si({sup 28}Si, 2pn){sup 55}Co and {sup 4}He({sup 54}Fe, n){sup 57}Ni were chosen. To identify the new {gamma} transitions and to build the energy level schemes, {gamma}-{gamma} coincidence techniques together with excitation functions were employed. Angular distributions and {gamma}-{gamma} angular correlations allowed us to assign the spin values of the nuclear states. The previous level scheme of {sup 55}Fe is extended into the region between 6.5-11 MeV of excitation energy, up to spin 27/2, while the yrast decay pathos of {sup 57}Ni and {sup 55}Co are reported here for the first time. Experimental data are fairly well reproduced by Glaudemans' shell model calculations. (orig.).

1989-12-01

31

High spin states of some nuclei around the N=Z=28 double closed shell  

International Nuclear Information System (INIS)

A spectroscopic study is performed for high spin states of "5"5Fe, "5"5Co and "5"7Ni. To populate the investigated residues with a relevant cross section, the fusion evaporation reactions of "3"0Si("2"8Si, 2pn)"5"5Fe, "3"0Si("2"8Si, 2pn)"5"5Co and "4He("5"4Fe, n)"5"7Ni were chosen. To identify the new #gamma# transitions and to build the energy level schemes, #gamma#-#gamma# coincidence techniques together with excitation functions were employed. Angular distributions and #gamma#-#gamma# angular correlations allowed us to assign the spin values of the nuclear states. The previous level scheme of "5"5Fe is extended into the region between 6.5-11 MeV of excitation energy, up to spin 27/2, while the yrast decay pathos of "5"7Ni and "5"5Co are reported here for the first time. Experimental data are fairly well reproduced by Glaudemans' shell model calculations. (orig.).

1989-01-01

32

Effect of chemical composition of SiOx films on rapid formation of Si nanocrystals induced by thermal plasma jet irradiation  

British Library Electronic Table of Contents (United Kingdom)

Si nanocrystal floating gate MOS capacitors were formed on p-Si (100) wafers by thermal plasma jet (TPJ) annealing of SiO2/SiOx /SiO2/Si(100) stacked structure. The chemical composition of SiOx layer was controlled by changing the SiH4, He, and O2 gas flow ratio during plasma enhanced chemical vapour deposition. The MOS capacitors showed clear hysteresis in capacitance-voltage (CV) characteristics after TPJ annealing. The hysteresis width shows maximum value when initial composition x =1.7, which shows the maximum photoluminescence (PL) intensity. The maximum hysteresis width of 6.8 V was observed with gate voltage swept between 20 and -20 V in x = 1.7 sample. The result means 7.4 x 1012 cm-2 carriers are injected to or emitted from Si nanocrystals. The duration of 1 V shift in flatband vo...

2010-01-01

33

PRELIMINARY CROSS SECTION AND NU-BAR COVARIANCES FOR WPEC SUBGROUP 26  

Energy Technology Data Exchange (ETDEWEB)

We report preliminary cross section covariances developed for the WPEC Subgroup 26 for 45 out of 52 requested materials. The covariances were produced in 15- and 187-group representations as follows: (1) 36 isotopes ({sup 16}O, {sup 19}F, {sup 23}Na, {sup 27}Al, {sup 28}Si, {sup 52}Cr, {sup 56,56}Fe, {sup 58}Ni, {sup 90,91,92,94}Zr, {sup 166,167,168,170}Er, {sup 206,207,208}Pb, {sup 209}Bi, {sup 233,234,236}U, {sup 237}Np, {sup 238,240,241,242}Pu, {sup 241,242m,243}Am, {sup 242,243,244,245}Cm) were evaluated using the BNL-LANL methodology. For the thermal region and the resolved and unresolved resonance regions, the methodology has been based on the Atlas-Kalman approach, in the fast neutron region the Empire-Kalman method has been used; (2) 6 isotopes ({sup 155,156,157,158,160}Gd and {sup 232}Th) were taken from ENDF/B-VII.0; and (3) 3 isotopes ({sup 1}H, {sup 238}U and {sup 239}Pu) were taken from JENDL-3.3. For 6 light nuclei ({sup 4}He, ...

2007-01-31

34

Ion backscattering, channeling and nuclear reaction analysis study of passive films formed on FeCrNi and FeCrNiMo (100) single crystals  

Energy Technology Data Exchange (ETDEWEB)

The compositions of passive films formed on Fe-17Fr-13Ni (at. %) and Fe-18.5Cr-14Ni-1.5Mo (100) single crystals have been determined and the structure of the alloy under the film has been investigated. The alloys were passivated in 0.05M H{sub 2}SO{sub 4} at 250 mV/SHE for 30 min. The oxygen content was measured by nuclear microanalysis using the {sup 16}O(d,p) {sup 17}O* reaction. The oxygen content in the passive film is similar for the two alloys and equal to (12{plus minus}2) 10{sup 15} O/cm{sup 2}. The cationic compositions of the passive films have been determined by {sup 4}He channeling at two incident beam energies: 0.8 and 2.0 MeV. For the two alloys studied, a total cation content of (5{plus minus}2)10{sup 15} at/cm{sup 2} is found in the passive films. The corresponding thickness is about 12 A. There is an excess of oxygen, which can be attributed to the presence of hydroxyls and sulfate. A strong chromium enrichment is found in the ...

1990-01-01

35

Ion backscattering, channeling and nuclear reaction analysis study of passive films formed on FeCrNi and FeCrNiMo (100) single crystals  

International Nuclear Information System (INIS)

The compositions of passive films formed on Fe-17Fr-13Ni (at. %) and Fe-18.5Cr-14Ni-1.5Mo (100) single crystals have been determined and the structure of the alloy under the film has been investigated. The alloys were passivated in 0.05M H_2SO_4 at 250 mV/SHE for 30 min. The oxygen content was measured by nuclear microanalysis using the "1"6O(d,p) "1"7O* reaction. The oxygen content in the passive film is similar for the two alloys and equal to (12#+-#2) 10"1"5 O/cm"2. The cationic compositions of the passive films have been determined by "4He channeling at two incident beam energies: 0.8 and 2.0 MeV. For the two alloys studied, a total cation content of (5#+-#2)10"1"5 at/cm"2 is found in the passive films. The corresponding thickness is about 12 A. There is an excess of oxygen, which can be attributed to the presence of hydroxyls and sulfate. A strong chromium enrichment is found in the passive film formed on both alloys: chromium represents ...

1989-09-24

36

High-precision Penning-Trap measurements of light-ion masses  

International Nuclear Information System (INIS)

The UW-Penning Trap Mass Spectrometer (PTMs) is ideally suited for high precision measurements of atomic masses throughout the periodic table upon using highly-stripped ions. However, at the present time, this device has been applied extensively to the light elements ("1H, "2H, "3H, "3He, "4He, "1"2C, "1"3C, "1"4N, "1"6O) due to their fundamental importance. Atomic masses follow immediately from a comparison with some multiply-charged carbon ion, after correcting for the lost electrons and their corresponding binding energies. For instance, the most recent C"5"+/C"6"+ comparison yielded a discrepancy of -0.30(33) ppb, limited only by the magnetic field instability for a 40-h run. The initial emphasis on hydrogen has now produced a 1-ppb value for the proton's atomic mass and similar work with deuterium has yielded a 2.5-ppb value for the neutron's atomic mass. However, the most significant result is the "3H-"3He mass difference = 18,590.1(17) ...

1993-04-12

37

Effect of chemical composition of SiO{sub x} films on rapid formation of Si nanocrystals induced by thermal plasma jet irradiation  

Energy Technology Data Exchange (ETDEWEB)

Si nanocrystal floating gate MOS capacitors were formed on p-Si (100) wafers by thermal plasma jet (TPJ) annealing of SiO{sub 2}/SiO{sub x} /SiO{sub 2}/Si(100) stacked structure. The chemical composition of SiO{sub x} layer was controlled by changing the SiH{sub 4}, He, and O{sub 2} gas flow ratio during plasma enhanced chemical vapour deposition. The MOS capacitors showed clear hysteresis in capacitance-voltage (CV) characteristics after TPJ annealing. The hysteresis width shows maximum value when initial composition x =1.7, which shows the maximum photoluminescence (PL) intensity. The maximum hysteresis width of 6.8 V was observed with gate voltage swept between 20 and -20 V in x = 1.7 sample. The result means 7.4 x 10{sup 12} cm{sup -2} carriers are injected to or emitted from Si nanocrystals. The duration of 1 V shift in flatband voltage was {proportional_to}0.1 ms with 20 V pulse, and charged carriers were stably maintained for ...

2010-04-15

38

Determination of the helium diffusion coefficient in nuclear waste storage ceramics by a nuclear reaction analysis method  

International Nuclear Information System (INIS)

Host matrices for actinide immobilisation will undergo the formation of large helium quantities due to alpha decay. Helium diffusion rate has to be known in order to predict the long-term behaviour of the material, and particularly, the influence of helium accumulation on mechanical properties. A nuclear reaction analysis method, namely the "3He(d, p)"4He reaction, has been used to analyse the evolution of "3He profiles after ion implantations at 1 and 3 MeV in two materials, monoclinic ZrO_2 (as a test material) and Ca_9Nd(PO_4)_5(SiO_4)F_1_._5(OH)_0_._5 britholite (envisaged for Am and Pu long-term storage). Two data processing methods are used: the classical excitation curve (proton yields versus deuteron energy) and second, the proton energy spectrum for a given deuteron energy. The characteristics of the "3He profiles (depth, width) obtained by both methods are compared to SRIM estimations. Their evolution during subsequent annealings ...

2002-06-01