Electron Interference in Molecular Circular Polarization Attosecond XUV Photoionization

Directory of Open Access Journals (Sweden)

Kai-Jun Yuan

2015-01-01

Full Text Available Two-center electron interference in molecular attosecond photoionization processes is investigated from numerical solutions of time-dependent Schrödinger equations. Both symmetric H\\(_2^+\\ and nonsymmetric HHe\\(^{2+}\\ one electron diatomic systems are ionized by intense attosecond circularly polarized XUV laser pulses. Photoionization of these molecular ions shows signature of interference with double peaks (minima in molecular attosecond photoelectron energy spectra (MAPES at critical angles \\(\\vartheta_c\\ between the molecular \\(\\textbf{R}\\ axis and the photoelectron momentum \\(\\textbf{p}\\. The interferences are shown to be a function of the symmetry of electronic states and the interference patterns are sensitive to the molecular orientation and pulse polarization. Such sensitivity offers possibility for imaging of molecular structure and orbitals.

Secondary-electron cascade in attosecond photoelectron spectroscopy from metals

DEFF Research Database (Denmark)

Baggesen, Jan Conrad; Madsen, Lars Bojer

2009-01-01

an analytical model based on an approximate solution to Boltzmann's transport equation to account for the amount and energy distribution of these secondary electrons. Our theory is in good agreement with the electron spectrum found in a recent attosecond streaking experiment. To suppress the background and gain......Attosecond spectroscopy is currently restricted to photon energies around 100 eV. We show that under these conditions, electron-electron scatterings, as the photoelectrons leave the metal, give rise to a tail of secondary electrons with lower energies and hence a significant background. We develop...

Connecting Lab-Based Attosecond Science with FEL research

CERN Multimedia

CERN. Geneva

2011-01-01

In the last few years laboratory-scale femtosecond laser-based research using XUV light has developed dramatically following the successful development of attosecond laser pulses by means of high-harmonic generation. Using attosecond laser pulses, studies of electron dynamics on the natural timescale that electronic processes occur in atoms, molecules and solids can be contemplated, providing unprecedented insight into the fundamental role that electrons play in photo-induced processes. In my talk I will briefly review the present status of the attosecond science research field in terms of present and foreseen capabilities, and discuss a few recent applications, including a first example of the use of attosecond laser pulses in molecular science. In addition, I will discuss very recent results of experiments where photoionization of dynamically aligned molecules is investigated using a high-harmonics XUV source. Photoionization of aligned molecules becomes all the more interesting if the experiment is perfo...

The dynamics of electron and ion holes in a collisionless plasma

Directory of Open Access Journals (Sweden)

B. Eliasson

2005-01-01

Full Text Available We present a review of recent analytical and numerical studies of the dynamics of electron and ion holes in a collisionless plasma. The new results are based on the class of analytic solutions which were found by Schamel more than three decades ago, and which here work as initial conditions to numerical simulations of the dynamics of ion and electron holes and their interaction with radiation and the background plasma. Our analytic and numerical studies reveal that ion holes in an electron-ion plasma can trap Langmuir waves, due the local electron density depletion associated with the negative ion hole potential. Since the scale-length of the ion holes are on a relatively small Debye scale, the trapped Langmuir waves are Landau damped. We also find that colliding ion holes accelerate electron streams by the negative ion hole potentials, and that these streams of electrons excite Langmuir waves due to a streaming instability. In our Vlasov simulation of two colliding ion holes, the holes survive the collision and after the collision, the electron distribution becomes flat-topped between the two ion holes due to the ion hole potentials which work as potential barriers for low-energy electrons. Our study of the dynamics between electron holes and the ion background reveals that standing electron holes can be accelerated by the self-created ion cavity owing to the positive electron hole potential. Vlasov simulations show that electron holes are repelled by ion density minima and attracted by ion density maxima. We also present an extension of Schamel's theory to relativistically hot plasmas, where the relativistic mass increase of the accelerated electrons have a dramatic effect on the electron hole, with an increase in the electron hole potential and in the width of the electron hole. A study of the interaction between electromagnetic waves with relativistic electron holes shows that electromagnetic waves can be both linearly and nonlinearly

Attosecond Electron Wave Packet Dynamics in Strong Laser Fields

International Nuclear Information System (INIS)

Johnsson, P.; Remetter, T.; Varju, K.; L'Huillier, A.; Lopez-Martens, R.; Valentin, C.; Balcou, Ph.; Kazamias, S.; Mauritsson, J.; Gaarde, M. B.; Schafer, K. J.; Mairesse, Y.; Wabnitz, H.; Salieres, P.

2005-01-01

We use a train of sub-200 attosecond extreme ultraviolet (XUV) pulses with energies just above the ionization threshold in argon to create a train of temporally localized electron wave packets. We study the energy transfer from a strong infrared (IR) laser field to the ionized electrons as a function of the delay between the XUV and IR fields. When the wave packets are born at the zero crossings of the IR field, a significant amount of energy (∼20 eV) is transferred from the field to the electrons. This results in dramatically enhanced above-threshold ionization in conditions where the IR field alone does not induce any significant ionization. Because both the energy and duration of the wave packets can be varied independently of the IR laser, they are valuable tools for studying and controlling strong-field processes

Correlated nuclear and electronic dynamics in photoionized systems studied by quantum and mixed quantum-classical approaches

International Nuclear Information System (INIS)

Li, Zheng

2014-09-01

The advent of free electron lasers and high harmonic sources enables the investigation of electronic and nuclear dynamics of molecules and solids with atomic spatial resolution and femtosecond/attosecond time resolution, using bright and ultrashort laser pulses of frequency from terahertz to hard x-ray range. With the help of ultrashort laser pulses, the nuclear and electronic dynamics can be initiated, monitored and actively controlled at the typical time scale in the femtosecond to attosecond realm. Meanwhile, theoretical tools are required to describe the underlying mechanism. This doctoral thesis focuses on the development of theoretical tools based on full quantum mechanical multiconfiguration time-dependent Hartree (MCTDH) and mixed quantum classical approaches, which can be applied to describe the dynamical behavior of gas phase molecules and strongly correlated solids in the presence of ultrashort laser pulses. In the first part of this thesis, the focus is on the motion of electron holes in gas phase molecular ions created by extreme ultraviolet (XUV) photoionization and watched by spectroscopic approaches. The XUV photons create electron-hole in the valence orbitals of molecules by photoionization, the electron hole, as a positively charged quasi-particle, can then interact with the nuclei and the rest of electrons, leading to coupled non-Born-Oppenheimer dynamics. I present our study on electron-hole relaxation dynamics in valence ionized molecular ions of moderate size, using quantum wave packet and mixed quantum-classical approaches, using photoionized [H + (H 2 O) n ] + molecular ion as example. We have shown that the coupled motion of the electron-hole and the nuclei can be mapped out with femtosecond resolution by core-level x-ray transient absorption spectroscopy. Furthermore, in specific cases, the XUV photon can create a coherent electron hole, that can maintain its coherence to time scales of ∝ 1 picosecond. Employing XUV pump - IR probe

Attosecond time-energy structure of X-ray free-electron laser pulses

Science.gov (United States)

Hartmann, N.; Hartmann, G.; Heider, R.; Wagner, M. S.; Ilchen, M.; Buck, J.; Lindahl, A. O.; Benko, C.; Grünert, J.; Krzywinski, J.; Liu, J.; Lutman, A. A.; Marinelli, A.; Maxwell, T.; Miahnahri, A. A.; Moeller, S. P.; Planas, M.; Robinson, J.; Kazansky, A. K.; Kabachnik, N. M.; Viefhaus, J.; Feurer, T.; Kienberger, R.; Coffee, R. N.; Helml, W.

2018-04-01

The time-energy information of ultrashort X-ray free-electron laser pulses generated by the Linac Coherent Light Source is measured with attosecond resolution via angular streaking of neon 1s photoelectrons. The X-ray pulses promote electrons from the neon core level into an ionization continuum, where they are dressed with the electric field of a circularly polarized infrared laser. This induces characteristic modulations of the resulting photoelectron energy and angular distribution. From these modulations we recover the single-shot attosecond intensity structure and chirp of arbitrary X-ray pulses based on self-amplified spontaneous emission, which have eluded direct measurement so far. We characterize individual attosecond pulses, including their instantaneous frequency, and identify double pulses with well-defined delays and spectral properties, thus paving the way for X-ray pump/X-ray probe attosecond free-electron laser science.

Investigation of attosecond ionization dynamics in gases and solids with intense few-cycle laser pulses

International Nuclear Information System (INIS)

Mitrofanov, A. V.

2011-01-01

Interaction of intense light fields with dielectric materials has fascinated scientists since the invention of pulsed lasers in the early sixties. Despite the many decades of research, the interest in the field keeps growing because of the potential technological applications of optical (meta-) materials and the prospects of light-controlled peta-Hertz electronics as well as the improving understanding of the fundamental processes behind light-matter interactions. The progress in the short-pulse laser technology that delivered ever-shorter light pulses was echoed by the discoveries of different progressively shorter time scales in the cycle of excitation and energy/charge relaxation in transparent solids, many parts of which are now well understood. The ultimate challenge lies in recovering the earliest stages of the dynamics which are linked to optical-field-ionization that proceeds within a fraction of an optical cycle. One of the complications of advancing the attosecond science to the bulk media is the problem of inducing and detecting a synchronized attosecond response. The charged particles spectroscopy, well developed in gaseous media during last decade and capable of reaching an attosecond temporal resolution cannot be used as an experimental tool for investigation since direct detection of charged particles is impossible in the volume of a solid material. However, solids are the natural place where electronic processes on the sub-femtosecond or attosecond time scale are expected. Very recently several methods for measuring attosecond dynamics in condensed media have been proposed utilizing optical fields in the transparency range of the material. In this thesis a method, suggested in our scientific group is presented. It is an all-optical method based on the detection of optical harmonics originating from ultrafast modulation of a free electron current due to ionization in the field of intense few-cycle laser pulses. This technique will allow retrieving

Coherent control of atto-second emission from aligned molecules

Energy Technology Data Exchange (ETDEWEB)

Boutu, W; Haessler, S; Merdji, H; Breger, P; Monchicourt, P; Carre, B; Salieres, P [CEA Saclay, DSM, Serv Photons Atomes Mol, F-91191 Gif Sur Yvette, (France); Waters, G [Univ Reading, JJ Thomson Phys Lab, Reading RG6 6AF, Berks, (United Kingdom); Stankiewicz, M [Jagiellonian Univ, Inst Phys, PL-30059 Krakow, (Poland); Frasinski, L J [Univ London Imperial Coll Sci Technol and Med, Blackett Lab, London SW7 2BW, (United Kingdom); Taieb, R; Caillat, J; Maquet, A [Univ Paris 06, UMR 7614, Lab Chim Phys Matiere Rayonnement, F-75231 Paris 05, (France); Taieb, R; Caillat, J; Maquet, A [LCPMR, UMR 7614, CNRS, F-75005 Paris, (France)

2008-07-01

Controlling atto-second electron wave packets and soft X-ray pulses represents a formidable challenge of general implication to many areas of science. A strong laser field interacting with atoms or molecules drives ultrafast intra-atomic/molecular electron wave packets on a sub femtosecond timescale, resulting in the emission of atto-second bursts of extreme-ultraviolet light. Controlling the intra-atomic/molecular electron dynamics enables steering of the atto-second emission. Here, we carry out a coherent control in linear molecules, where the interaction of the laser-driven electron wave packet with the core leads to quantum interferences. We demonstrate that these interferences can be finely controlled by turning the molecular axis relative to the laser polarization, that is, changing the electron re-collision angle. The wave-packet coulombic distortion modifies the spectral phase jump measured in the extreme-ultraviolet emission. Our atto-second control of the interference results in atto-second pulse shaping, useful for future applications in ultrafast coherent control of atomic and molecular processes. (authors)

Velocity map imaging of attosecond and femtosecond dynamics in atoms and small molecules in strong laser fields

International Nuclear Information System (INIS)

Kling, M.F.; Ni, Yongfeng; Lepine, F.; Khan, J.I.; Vrakking, M.J.J.; Johnsson, P.; Remetter, T.; Varju, K.; Gustafsson, E.; L'Huillier, A.; Lopez-Martens, R.; Boutu, W.

2005-01-01

Full text: In the past decade, the dynamics of atomic and small molecular systems in strong laser fields has received enormous attention, but was mainly studied with femtosecond laser fields. We report on first applications of attosecond extreme ultraviolet (XUV) pulse trains (APTs) from high-order harmonic generation (HHG) for the study of atomic and molecular electron and ion dynamics in strong laser fields utilizing the Velocity Map Imaging Technique. The APTs were generated in argon from harmonics 13 to 35 of a 35 fs Ti:sapphire laser, and spatially and temporally overlapped with an intense IR laser field (up to 5x10 13 W/cm 2 ) in the interaction region of a Velocity Map Imaging (VMI) machine. In the VMI setup, electrons and ions that were created at the crossing point of the laser fields and an atomic or molecular beam were accelerated in a dc-electric field towards a two-dimensional position-sensitive detector, allowing to reconstruct the full initial three-dimensional velocity distribution. The poster will focus on results that were obtained for argon atoms. We recorded the velocity distribution of electron wave packets that were strongly driven in the IR laser field after their generation in Ar via single-photon ionization by attosecond XUV pulses. The 3D evolution of the electron wave packets was observed on an attosecond timescale. In addition to earlier experiments with APTs using a magnetic bottle electron time-of-flight spectrometers and with single attosecond pulses, the angular dependence of the electrons kinetic energies can give further insight into the details of the dynamics. Initial results that were obtained for molecular systems like H 2 , D 2 , N 2 , and CO 2 using the same powerful approach will be highlighted as well. We will show, that detailed insight into the dynamics of these systems in strong laser fields can be obtained (e.g. on the alignment, above-threshold ionization, direct vs. sequential two-photon ionization, dissociation, and

Theory of attosecond delays in molecular photoionization.

Science.gov (United States)

Baykusheva, Denitsa; Wörner, Hans Jakob

2017-03-28

We present a theoretical formalism for the calculation of attosecond delays in molecular photoionization. It is shown how delays relevant to one-photon-ionization, also known as Eisenbud-Wigner-Smith delays, can be obtained from the complex dipole matrix elements provided by molecular quantum scattering theory. These results are used to derive formulae for the delays measured by two-photon attosecond interferometry based on an attosecond pulse train and a dressing femtosecond infrared pulse. These effective delays are first expressed in the molecular frame where maximal information about the molecular photoionization dynamics is available. The effects of averaging over the emission direction of the electron and the molecular orientation are introduced analytically. We illustrate this general formalism for the case of two polyatomic molecules. N 2 O serves as an example of a polar linear molecule characterized by complex photoionization dynamics resulting from the presence of molecular shape resonances. H 2 O illustrates the case of a non-linear molecule with comparably simple photoionization dynamics resulting from a flat continuum. Our theory establishes the foundation for interpreting measurements of the photoionization dynamics of all molecules by attosecond metrology.

Attosecond control of electron beams at dielectric and absorbing membranes

Science.gov (United States)

Morimoto, Yuya; Baum, Peter

2018-03-01

Ultrashort electron pulses are crucial for time-resolved electron diffraction and microscopy of the fundamental light-matter interaction. In this work, we study experimentally and theoretically the generation and characterization of attosecond electron pulses by optical-field-driven compression and streaking at dielectric or absorbing interaction elements. The achievable acceleration and deflection gradient depends on the laser-electron angle, the laser's electric and magnetic field directions, and the foil orientation. Electric and magnetic fields have similar contributions to the final effect and both need to be considered. Experiments and theory agree well and reveal the optimum conditions for highly efficient, velocity-matched electron-field interactions in the longitudinal or transverse direction. We find that metallic membranes are optimum for light-electron control at mid-infrared or terahertz wavelengths, but dielectric membranes are excellent in the visible and near-infrared regimes and are therefore ideal for the formation of attosecond electron pulses.

Attosecond experiments on plasmonic nanostructures principles and experiments

CERN Document Server

Schötz, Johannes

2016-01-01

Johannes Schötz presents the first measurements of optical electro-magnetic near-fields around nanostructures with subcycle-resolution. The ability to measure and understand light-matter interactions on the nanoscale is an important component for the development of light-wave-electronics, the control and steering of electron dynamics with the frequency of light, which promises a speed-up by several orders of magnitude compared to conventional electronics. The experiments presented here on metallic nanotips, widely used in experiments and applications, do not only demonstrate the feasibility of attosecond streaking as a unique tool for fundamental studies of ultrafast nanophotonics but also represent a first important step towards this goal. Contents Electron Scattering in Solids Attosecond Streaking from Metal Nanotips Target Groups Lecturers and students of physics, especially in the area of nanophotonics and attosecond physics About the Author Johannes Schötz received his Master's degree in physics and cu...

Generation of attosecond electron packets via conical surface plasmon electron acceleration

Science.gov (United States)

Greig, S. R.; Elezzabi, A. Y.

2016-01-01

We present a method for the generation of high kinetic energy attosecond electron packets via magnetostatic and aperture filtering of conical surface plasmon (SP) accelerated electrons. The conical SP waves are excited by coupling an ultrafast radially polarized laser beam to a conical silica lens coated with an Ag film. Electromagnetic and particle tracking models are employed to characterize the ultrafast electron packets. PMID:26764129

Génération d'impulsions attosecondes sur miroir plasma à très haute cadence

OpenAIRE

Borot , Antonin

2012-01-01

Focusing an intense laser pulse onto a solid surface leads to the almost complete ionisation of matter and the creation of a plasma of near-solid electronic density. Collective charge dynamic of the plasma electrons is then driven by the laser field and can give birth to a train of XUV attosecond pulses. This work aims at demonstrating that plasma dynamics can be driven with attosecond precison by the laser field in order to generate reproducible attosecond XUV pulses. Therfore we built up th...

Molecular electron recollision dynamics in intense circularly polarized laser pulses

Science.gov (United States)

Bandrauk, André D.; Yuan, Kai-Jun

2018-04-01

Extreme UV and x-ray table top light sources based on high-order harmonic generation (HHG) are focused now on circular polarization for the generation of circularly polarized attosecond pulses as new tools for controlling electron dynamics, such as charge transfer and migration and the generation of attosecond quantum electron currents for ultrafast magneto-optics. A fundamental electron dynamical process in HHG is laser induced electron recollision with the parent ion, well established theoretically and experimentally for linear polarization. We discuss molecular electron recollision dynamics in circular polarization by theoretical analysis and numerical simulation. The control of the polarization of HHG with circularly polarized ionizing pulses is examined and it is shown that bichromatic circularly polarized pulses enhance recollision dynamics, rendering HHG more efficient, especially in molecules because of their nonspherical symmetry. The polarization of the harmonics is found to be dependent on the compatibility of the rotational symmetry of the net electric field created by combinations of bichromatic circularly polarized pulses with the dynamical symmetry of molecules. We show how the field and molecule symmetry influences the electron recollision trajectories by a time-frequency analysis of harmonics. The results, in principle, offer new unique controllable tools in the study of attosecond molecular electron dynamics.

Attosecond transient absorption spectroscopy of molecular hydrogen

International Nuclear Information System (INIS)

Martín, Fernando; González-Castrillo, Alberto; Palacios, Alicia; Argenti, Luca; Cheng, Yan; Chini, Michael; Wang, Xiaowei; Chang, Zenghu

2015-01-01

We extend attosecond transient absorption spectroscopy (ATAS) to the study of hydrogen molecules, demonstrating the potential of the technique to resolve – simultaneously and with state resolution – both the electronic and nuclear dynamics. (paper)

Laser-plasma accelerator-based single-cycle attosecond undulator source

Science.gov (United States)

Tibai, Z.; Tóth, Gy.; Nagyváradi, A.; Sharma, A.; Mechler, M. I.; Fülöp, J. A.; Almási, G.; Hebling, J.

2018-06-01

Laser-plasma accelerators (LPAs), producing high-quality electron beams, provide an opportunity to reduce the size of free-electron lasers (FELs) to only a few meters. A complete system is proposed here, which is based on FEL technology and consists of an LPA, two undulators, and other magnetic devices. The system is capable to generate carrier-envelope phase stable attosecond pulses with engineered waveform. Pulses with up to 60 nJ energy and 90-400 attosecond duration in the 30-120 nm wavelength range are predicted by numerical simulation. These pulses can be used to investigate ultrafast field-driven electron dynamics in matter.

Attosecond-resolved photoionization of chiral molecules.

Science.gov (United States)

Beaulieu, S; Comby, A; Clergerie, A; Caillat, J; Descamps, D; Dudovich, N; Fabre, B; Géneaux, R; Légaré, F; Petit, S; Pons, B; Porat, G; Ruchon, T; Taïeb, R; Blanchet, V; Mairesse, Y

2017-12-08

Chiral light-matter interactions have been investigated for two centuries, leading to the discovery of many chiroptical processes used for discrimination of enantiomers. Whereas most chiroptical effects result from a response of bound electrons, photoionization can produce much stronger chiral signals that manifest as asymmetries in the angular distribution of the photoelectrons along the light-propagation axis. We implemented self-referenced attosecond photoelectron interferometry to measure the temporal profile of the forward and backward electron wave packets emitted upon photoionization of camphor by circularly polarized laser pulses. We measured a delay between electrons ejected forward and backward, which depends on the ejection angle and reaches 24 attoseconds. The asymmetric temporal shape of electron wave packets emitted through an autoionizing state further reveals the chiral character of strongly correlated electronic dynamics. Copyright © 2017 The Authors, some rights reserved; exclusive licensee American Association for the Advancement of Science. No claim to original U.S. Government Works.

Feasibility analysis for attosecond X-ray pulses at FERMI@ELETTRA free electron laser

Energy Technology Data Exchange (ETDEWEB)

Zholents, Alexander

2004-09-01

We present preliminary analysis for the feasibility of the attosecond x-ray pulses at a proposed FERMI@ELETTRA free electron laser (FEL) [1]. In part 1 we restrict ourselves to minimal modifications to the proposed FEL and consider a scheme for attosecond x-ray production which can be qualified as a small add-on to a primary facility. We demonstrate that at 5-nm wavelength our scheme is capable for production of pulses with an approximate duration of 100 attoseconds at approximately 2 MW peak power and with an absolute temporal synchronization to a pump laser pulse. In part 2 we propose to use an FEL amplifier seeded by a VUV signal and to follow it by the scheme for attosecond x-ray production described in part 1.

Next Generation Driver for Attosecond and Laser-plasma Physics.

Science.gov (United States)

Rivas, D E; Borot, A; Cardenas, D E; Marcus, G; Gu, X; Herrmann, D; Xu, J; Tan, J; Kormin, D; Ma, G; Dallari, W; Tsakiris, G D; Földes, I B; Chou, S-W; Weidman, M; Bergues, B; Wittmann, T; Schröder, H; Tzallas, P; Charalambidis, D; Razskazovskaya, O; Pervak, V; Krausz, F; Veisz, L

2017-07-12

The observation and manipulation of electron dynamics in matter call for attosecond light pulses, routinely available from high-order harmonic generation driven by few-femtosecond lasers. However, the energy limitation of these lasers supports only weak sources and correspondingly linear attosecond studies. Here we report on an optical parametric synthesizer designed for nonlinear attosecond optics and relativistic laser-plasma physics. This synthesizer uniquely combines ultra-relativistic focused intensities of about 10 20  W/cm 2 with a pulse duration of sub-two carrier-wave cycles. The coherent combination of two sequentially amplified and complementary spectral ranges yields sub-5-fs pulses with multi-TW peak power. The application of this source allows the generation of a broad spectral continuum at 100-eV photon energy in gases as well as high-order harmonics in relativistic plasmas. Unprecedented spatio-temporal confinement of light now permits the investigation of electric-field-driven electron phenomena in the relativistic regime and ultimately the rise of next-generation intense isolated attosecond sources.

Decoherence in attosecond photoionization.

Science.gov (United States)

Pabst, Stefan; Greenman, Loren; Ho, Phay J; Mazziotti, David A; Santra, Robin

2011-02-04

The creation of superpositions of hole states via single-photon ionization using attosecond extreme-ultraviolet pulses is studied with the time-dependent configuration-interaction singles (TDCIS) method. Specifically, the degree of coherence between hole states in atomic xenon is investigated. We find that interchannel coupling not only affects the hole populations, but it also enhances the entanglement between the photoelectron and the remaining ion, thereby reducing the coherence within the ion. As a consequence, even if the spectral bandwidth of the ionizing pulse exceeds the energy splittings among the hole states involved, perfectly coherent hole wave packets cannot be formed. For sufficiently large spectral bandwidth, the coherence can only be increased by increasing the mean photon energy.

Generation of attosecond electron beams in relativistic ionization by short laser pulses

Science.gov (United States)

Cajiao Vélez, F.; Kamiński, J. Z.; Krajewska, K.

2018-03-01

Ionization by relativistically intense short laser pulses is studied in the framework of strong-field quantum electrodynamics. Distinctive patterns are found in the energy probability distributions of photoelectrons, which are sensitive to the properties of a driving laser field. It is demonstrated that these electrons are generated in the form of solitary attosecond wave packets. This is particularly important in light of various applications of attosecond electron beams such as in ultrafast electron diffraction and crystallography, or in time-resolved electron microscopy of physical, chemical, and biological processes. We also show that, for intense laser pulses, high-energy ionization takes place in narrow regions surrounding the momentum spiral, the exact form of which is determined by the shape of a driving pulse. The self-intersections of the spiral define the momenta for which the interference patterns in the energy distributions of photoelectrons are observed. Furthermore, these interference regions lead to the synthesis of single-electron wave packets characterized by coherent double-hump structures.

Monitoring conical intersections in the ring opening of furan by attosecond stimulated X-ray Raman spectroscopy

Directory of Open Access Journals (Sweden)

Weijie Hua

2016-03-01

Full Text Available Attosecond X-ray pulses are short enough to capture snapshots of molecules undergoing nonadiabatic electron and nuclear dynamics at conical intersections (CoIns. We show that a stimulated Raman probe induced by a combination of an attosecond and a femtosecond pulse has a unique temporal and spectral resolution for probing the nonadiabatic dynamics and detecting the ultrafast (∼4.5 fs passage through a CoIn. This is demonstrated by a multiconfigurational self-consistent-field study of the dynamics and spectroscopy of the furan ring-opening reaction. Trajectories generated by surface hopping simulations were used to predict Attosecond Stimulated X-ray Raman Spectroscopy signals at reactant and product structures as well as representative snapshots along the conical intersection seam. The signals are highly sensitive to the changes in nonadiabatically coupled electronic structure and geometry.

Obtaining attosecond x-ray pulses using a self-amplified spontaneous emission free electron laser

Directory of Open Access Journals (Sweden)

A. A. Zholents

2005-05-01

Full Text Available We describe a technique for the generation of a solitary attosecond x-ray pulse in a free-electron laser (FEL, via a process of self-amplified spontaneous emission. In this method, electrons experience an energy modulation upon interacting with laser pulses having a duration of a few cycles within single-period wiggler magnets. Two consecutive modulation sections, followed by compression in a dispersive section, are used to obtain a single, subfemtosecond spike in the electron peak current. This region of the electron beam experiences an enhanced growth rate for FEL amplification. After propagation through a long undulator, this current spike emits a ∼250   attosecond x-ray pulse whose intensity dominates the x-ray emission from the rest of the electron bunch.

Attosecond pulse trains generated using two color laser fields

International Nuclear Information System (INIS)

Mauritsson, J.; Louisiana State University, Baton Rouge, LA; Johnsson, P.; Gustafsson, E.; L'Hullier, A.; Schafer, K.J.; Gaarde, M.B.

2006-01-01

parameters trains of attosecond pulses with only one pulse per IR cycle are generated. The presence of one attosecond pulse per IR cycle may furthermore be taken as evidence that consecutive pulses in the train have the same carrier envelope phase. When the attosecond pulses interact with a gas of atoms, electron wave packets are created if the photon energy exceeds the ionization potential. The wave packets are temporally localized with properties that are directly inherited from the attosecond pulses. If the ionization takes place in the presence of a strong IR field an energy exchange between the electrons and the field occurs. The amount of energy exchanged depends on the timing with respect to the phase of the IR field when the electrons are injected into the the continuum. Using trains with only one pulse per IR cycle, all the wave packets are injected with the same timing with respect to the IR field, thus enabling us to measure their dynamics in the dressed continuum. Using a velocity map imaging spectrometer we can measure a projection of the three dimensional electron distributions.

Ultrafast carrier dynamics in tetrahedral amorphous carbon: carrier trapping versus electron-hole recombination

International Nuclear Information System (INIS)

Carpene, E; Mancini, E; Dallera, C; Schwen, D; Ronning, C; Silvestri, S De

2007-01-01

We report the investigation of the ultrafast carrier dynamics in thin tetrahedral amorphous carbon films by means of femtosecond time-resolved reflectivity. We estimated the electron-phonon relaxation time of a few hundred femtoseconds and we observed that under low optical excitation photo-generated carriers decay according to two distinct mechanisms attributed to trapping by defect states and direct electron-hole recombination. With high excitation, when photo-carrier and trap densities are comparable, a unique temporal evolution develops, as the time dependence of the trapping process becomes degenerate with the electron-hole recombination. This experimental evidence highlights the role of defects in the ultrafast electronic dynamics and is not specific to this particular form of carbon, but has general validity for amorphous and disordered semiconductors

Generation of atto-second pulses in atoms and molecules

International Nuclear Information System (INIS)

Haessler, St.

2009-12-01

When a low-frequency laser pulse is focused to a high intensity into a gas, the electric field of the laser light may become of comparable strength to that felt by the electrons bound in an atom or molecule. A valence electron can then be 'freed' by tunnel ionization, accelerated by the strong oscillating laser field and can eventually re-collide and recombine with the ion. The gained kinetic energy is then released as a burst of coherent X-UV light and the macroscopic gas medium then becomes a source of X-UV light pulses of atto-second (1 as equals 10 -18 s) duration. This is the natural time-scale of electron dynamics in atoms and molecules. The largest part of this thesis deals with experiments where molecules are the harmonic generation medium and the re-colliding electron wave packet acts as a 'self-probe'. In several experiments, we demonstrate the potential of this scheme to observe or image ultra-fast intra-molecular electronic and nuclear dynamics. In particular, we have performed the first phase measurements of the high harmonic emission from aligned molecules and we have extracted the recombination dipole matrix element. This observable contains signatures of quantum interference between the continuum and bound parts of the total electronic wavefunction. It is shown how this quantum interference can be utilized to shape the atto-second light emission from the molecules. In a second part of this thesis, we use the well characterized coherent X-UV light emitted by rare gas atoms to photo-ionize molecules. Measuring the ejected photoelectron wave packet then allows to extract information on the photoionization process itself, and possibly about the initial bound and final continuum states of the electron. The last chapter of this manuscript describes studies of high harmonic and atto-second light pulse generation in a different medium: ablation plasmas. (author)

Nano-electron beam induced current and hole charge dynamics through uncapped Ge nanocrystals

Energy Technology Data Exchange (ETDEWEB)

Marchand, A.; El Hdiy, A.; Troyon, M. [Laboratoire de Recherche en Nanosciences, Bat. 6, case no 15, UFR Sciences, Universite de Reims Champagne Ardenne, 51687 Reims Cedex 2 (France); Amiard, G.; Ronda, A.; Berbezier, I. [IM2NP, Faculte des Sciences et Techniques, Campus de Saint Jerome - Case 142, Avenue Escadrille Normandie Niemen, 13397 Marseille Cedex 20 (France)

2012-04-16

Dynamics of hole storage in spherical Ge nanocrystals (NCs) formed by a two step dewetting/nucleation process on an oxide layer grown on an n-doped <001> silicon substrate is studied using a nano-electron beam induced current technique. Carrier generation is produced by an electron beam irradiation. The generated current is collected by an atomic force microscope--tip in contact mode at a fixed position away from the beam spot of about 0.5 {mu}m. This distance represents the effective diffusion length of holes. The time constants of holes charging are determined and the effect of the NC size is underlined.

Molecular alignment dependent electron interference in attosecond ultraviolet photoionization

Directory of Open Access Journals (Sweden)

Kai-Jun Yuan

2015-01-01

Full Text Available We present molecular photoionization processes by intense attosecond ultraviolet laser pulses from numerical solutions of time-dependent Schrödinger equations. Simulations preformed on a single electron diatomic H2+ show minima in molecular photoelectron energy spectra resulting from two center interference effects which depend strongly on molecular alignment. We attribute such sensitivity to the spatial orientation asymmetry of the photoionization process from the two nuclei. A similar influence on photoelectron kinetic energies is also presented.

Molecular alignment dependent electron interference in attosecond ultraviolet photoionization

Science.gov (United States)

Yuan, Kai-Jun; Bandrauk, André D.

2015-01-01

We present molecular photoionization processes by intense attosecond ultraviolet laser pulses from numerical solutions of time-dependent Schrödinger equations. Simulations preformed on a single electron diatomic H2+ show minima in molecular photoelectron energy spectra resulting from two center interference effects which depend strongly on molecular alignment. We attribute such sensitivity to the spatial orientation asymmetry of the photoionization process from the two nuclei. A similar influence on photoelectron kinetic energies is also presented. PMID:26798785

Charge migration induced by attosecond pulses in bio-relevant molecules

International Nuclear Information System (INIS)

Calegari, Francesca; Castrovilli, Mattea C; Nisoli, Mauro; Trabattoni, Andrea; Palacios, Alicia; Ayuso, David; Martín, Fernando; Greenwood, Jason B; Decleva, Piero

2016-01-01

After sudden ionization of a large molecule, the positive charge can migrate throughout the system on a sub-femtosecond time scale, purely guided by electronic coherences. The possibility to actively explore the role of the electron dynamics in the photo-chemistry of bio-relevant molecules is of fundamental interest for understanding, and perhaps ultimately controlling, the processes leading to damage, mutation and, more generally, to the alteration of the biological functions of the macromolecule. Attosecond laser sources can provide the extreme time resolution required to follow this ultrafast charge flow. In this review we will present recent advances in attosecond molecular science: after a brief description of the results obtained for small molecules, recent experimental and theoretical findings on charge migration in bio-relevant molecules will be discussed. (topical review)

Practical issues of retrieving isolated attosecond pulses

International Nuclear Information System (INIS)

Wang He; Chini, Michael; Khan, Sabih D; Chen, Shouyuan; Gilbertson, Steve; Feng Ximao; Mashiko, Hiroki; Chang Zenghu

2009-01-01

The attosecond streaking technique is used for the characterization of isolated extreme ultraviolet (XUV) attosecond pulses. This type of measurement suffers from low photoelectron counts in the streaked spectrogram, and is thus susceptible to shot noise. For the retrieval of few- or mono-cycle attosecond pulses, high-intensity streaking laser fields are required, which cause the energy spectrum of above-threshold ionized (ATI) electrons to overlap with that of the streaked photoelectrons. It is found by using the principal component generalized projections algorithm that the XUV attosecond pulse can accurately be retrieved for simulated and experimental spectrograms with a peak value of 50 or more photoelectron counts. Also, the minimum streaking intensity is found to be more than 50 times smaller than that required by the classical streaking camera for retrieval of pulses with a spectral bandwidth supporting 90 as transform-limited pulse durations. Furthermore, spatial variation of the streaking laser intensity, collection angle of streaked electrons and time delay jitter between the XUV pulse and streaking field can degrade the quality of the streaked spectrogram. We find that even when the XUV and streaking laser focal spots are comparable in size, the streaking electrons are collected from a 4π solid angle, or the delay fluctuates by more than the attosecond pulse duration, the attosecond pulses can still be accurately retrieved. In order to explain the insusceptibility of the streaked spectrogram to these factors, the linearity of the streaked spectrogram with respect to the streaking field is derived under the saddle point approximation.

Extracting attosecond delays from spectrally overlapping interferograms

Science.gov (United States)

Jordan, Inga; Wörner, Hans Jakob

2018-02-01

Attosecond interferometry is becoming an increasingly popular technique for measuring the dynamics of photoionization in real time. Whereas early measurements focused on atomic systems with very simple photoelectron spectra, the technique is now being applied to more complex systems including isolated molecules and solids. The increase in complexity translates into an augmented spectral congestion, unavoidably resulting in spectral overlap in attosecond interferograms. Here, we discuss currently used methods for phase retrieval and introduce two new approaches for determining attosecond photoemission delays from spectrally overlapping photoelectron spectra. We show that the previously used technique, consisting in the spectral integration of the areas of interest, does in general not provide reliable results. Our methods resolve this problem, thereby opening the technique of attosecond interferometry to complex systems and fully exploiting its specific advantages in terms of spectral resolution compared to attosecond streaking.

On the fly quantum dynamics of electronic and nuclear wave packets

Science.gov (United States)

Komarova, Ksenia G.; Remacle, F.; Levine, R. D.

2018-05-01

Multielectronic states quantum dynamics on a grid is described in a manner motivated by on the fly classical trajectory computations. Non stationary electronic states are prepared by a few cycle laser pulse. The nuclei respond and begin moving. We solve the time dependent Schrödinger equation for the electronic and nuclear dynamics for excitation from the ground electronic state. A satisfactory accuracy is possible using a localized description on a discrete grid. This enables computing on the fly for both the nuclear and electronic dynamics including non-adiabatic couplings. Attosecond dynamics in LiH is used as an example.

Electron Dynamics in a Subproton-Gyroscale Magnetic Hole

Science.gov (United States)

Gershman, Daniel J.; Dorelli, John C.; Vinas, Adolfo F.; Avanov, Levon A.; Gliese, Ulrik B.; Barrie, Alexander C.; Coffey, Victoria; Chandler, Michael; Dickson, Charles; MacDonald, Elizabeth A.;

Optical circular deflector with attosecond resolution for ultrashort electron beam

Directory of Open Access Journals (Sweden)

Zhen Zhang

2017-05-01

Full Text Available A novel method using high-power laser as a circular deflector is proposed for the measurement of femtosecond (fs and sub-fs electron beam. In the scheme, the electron beam interacts with a laser pulse operating in a radially polarized doughnut mode (TEM_{01^{*}} in a helical undulator, generating angular kicks along the beam in two directions at the same time. The phase difference between the two angular kicks makes the beam form a ring after a propagation section with appropriate phase advance, which can reveal the current profile of the electron beam. Detailed theoretical analysis of the method and numerical results with reasonable parameters are both presented. It is shown that the temporal resolution can reach up to ∼100 attosecond, which is a significant improvement for the diagnostics of ultrashort electron beam.

Generation and Characterization of Attosecond Pulses

Energy Technology Data Exchange (ETDEWEB)

Ian A. Walmsley; Robert W. Boyd

2006-04-24

The research undertaken in this project has been directed toward the area of attoscience, in particular the problem of attosecond metrology. That is, the accurate determination of the electric field of attosecond XUV radiation. This outstanding problem has been identified as a critical technology for further development of the field, and our research adds to the area by providing the first method for characterization using the harmonic radiation itself as a tool. The technical effectiveness of this approach is very high, since it is vastly easier to detect XUV radiation directly than via the spectrum of photoelectrons liberated from atoms by it. This means that the experimental data rate can be much higher in principle using all-optical detection that electron detection, which will greatly aid the utility of harmonic XUV sources in attoscience applications. There are as yet no direct public benefits from this area of scientific research, though access to material structural dynamics on unprecedented brief timescales are expected to yield significant benefits for the future.

Dynamical effects of electron-hole correlation and giant quantum attenuation of ultrasound in semimetals

International Nuclear Information System (INIS)

Kuramoto, Y.

1982-01-01

The giant quantum attenuation of ultrasound in bismuth and other semimetals is noticeably enhanced when certain pair of Landau subbands of electrons and holes participate simultaneously in an attenuation peak. A theoretical analysis is presented which emphasizes importance of dynamical effects of the electron-hole correlation. In the temperature range between 1K and 4K covered by most experiments, the correlation effect is found to be weak on the real part of the relevant response function which gives change in sound velocity. This implies that equilibrium properties of the system are not much influenced by the correlation effect. Nonetheless, the electron-hole correlation is shown to have a drastic consequence on the imaginary part of the response function probed by the ultrasonic attenuation. Proposal for experiment is advanced to discriminate relative importance of this exciton-like correlation from that of repulsive correlation between carriers with the same charge. (orig.)

Attosecond Coherent Control of the Photo-Dissociation of Oxygen Molecules

Science.gov (United States)

Sturm, Felix; Ray, Dipanwita; Wright, Travis; Shivaram, Niranjan; Bocharova, Irina; Slaughter, Daniel; Ranitovic, Predrag; Belkacem, Ali; Weber, Thorsten

2016-05-01

Attosecond Coherent Control has emerged in recent years as a technique to manipulate the absorption and ionization in atoms as well as the dissociation of molecules on an attosecond time scale. Single attosecond pulses and attosecond pulse trains (APTs) can coherently excite multiple electronic states. The electronic and nuclear wave packets can then be coupled with a second pulse forming multiple interfering quantum pathways. We have built a high flux extreme ultraviolet (XUV) light source delivering APTs based on HHG that allows to selectively excite neutral and ion states in molecules. Our beamline provides spectral selectivity and attosecond interferometric control of the pulses. In the study presented here, we use APTs, generated by High Harmonic Generation in a high flux extreme ultraviolet light source, to ionize highly excited states of oxygen molecules. We identify the ionization/dissociation pathways revealing vibrational structure with ultra-high resolution ion 3D-momentum imaging spectroscopy. Furthermore, we introduce a delay between IR pulses and XUV/IR pulses to constructively or destructively interfere the ionization and dissociation pathways, thus, enabling the manipulation of both the O2+and the O+ ion yields with attosecond precision. Supported by DOE under Contract No. DE-AC02-05CH11231.

Theory of strong-field attosecond transient absorption

International Nuclear Information System (INIS)

Wu, Mengxi; Chen, Shaohao; Camp, Seth; Schafer, Kenneth J; Gaarde, Mette B

2016-01-01

Attosecond transient absorption is one of the promising new techniques being developed to exploit the availability of sub-femtosecond extreme ultraviolet (XUV) pulses to study the dynamics of the electron on its natural time scale. The temporal resolution in a transient absorption setup comes from the control of the relative delay and coherence between pump and probe pulses, while the spectral resolution comes from the characteristic width of the features that are being probed. In this review we focus on transient absorption scenarios where an attosecond pulse of XUV radiation creates a broadband excitation that is subsequently probed by a few cycle infrared (IR) laser. Because the attosecond XUV pulses are locked to the IR field cycle, the exchange of energy in the laser–matter interaction can be studied with unprecedented precision. We focus on the transient absorption by helium atoms of XUV radiation around the first ionization threshold, where we can simultaneoulsy solve the time-dependent Schrödinger equation for the single atom response and the Maxwell wave equation for the collective response of the nonlinear medium. We use a time-domain method that allows us to treat on an equal footing all the different linear and nonlinear processes by which the medium can exchange energy with the fields. We present several simple models, based on a few-level system interacting with a strong IR field, to explain many of the novel features found in attosecond transient absorption spectrograms. These include the presence of light-induced states, which demonstrate the ability to probe the dressed states of the atom. We also present a time-domain interpretation of the resonant pulse propagation features that appear in absorption spectra in dense, macroscopic media. We close by reviewing several recent experimental results that can be explained in terms of the models we discuss. Our aim is to present a road map for understanding future attosecond transient absorption

Electron-phonon thermalization in a scalable method for real-time quantum dynamics

Science.gov (United States)

Rizzi, Valerio; Todorov, Tchavdar N.; Kohanoff, Jorge J.; Correa, Alfredo A.

2016-01-01

We present a quantum simulation method that follows the dynamics of out-of-equilibrium many-body systems of electrons and oscillators in real time. Its cost is linear in the number of oscillators and it can probe time scales from attoseconds to hundreds of picoseconds. Contrary to Ehrenfest dynamics, it can thermalize starting from a variety of initial conditions, including electronic population inversion. While an electronic temperature can be defined in terms of a nonequilibrium entropy, a Fermi-Dirac distribution in general emerges only after thermalization. These results can be used to construct a kinetic model of electron-phonon equilibration based on the explicit quantum dynamics.

Dynamics of valence-shell electrons and nuclei probed by strong-field holography and rescattering

Science.gov (United States)

Walt, Samuel G.; Bhargava Ram, Niraghatam; Atala, Marcos; Shvetsov-Shilovski, Nikolay I; von Conta, Aaron; Baykusheva, Denitsa; Lein, Manfred; Wörner, Hans Jakob

2017-01-01

Strong-field photoelectron holography and laser-induced electron diffraction (LIED) are two powerful emerging methods for probing the ultrafast dynamics of molecules. However, both of them have remained restricted to static systems and to nuclear dynamics induced by strong-field ionization. Here we extend these promising methods to image purely electronic valence-shell dynamics in molecules using photoelectron holography. In the same experiment, we use LIED and photoelectron holography simultaneously, to observe coupled electronic-rotational dynamics taking place on similar timescales. These results offer perspectives for imaging ultrafast dynamics of molecules on femtosecond to attosecond timescales. PMID:28643771

Few-cycle isolated attosecond pulses

International Nuclear Information System (INIS)

Sansone, G.; Benedetti, E.; Calegari, F.; Stagira, S.; Vozzi, C.; Silvestri De, S.; Nisoli, M.

2006-01-01

Complete test of publication follows. In the last few years the field of attosecond science has shown impressive and rapid progress, mainly due to the introduction of novel experimental methods for the characterization of extreme ultraviolet (XUV) pulses and attosecond electron wave packets. This development has been also triggered by significant improvements in the control of the electric field of the driving infrared pulses. Particularly interesting for the applications is the generation of isolated attosecond XUV pulses using few-cycle driving pulses. In this case significant progresses have been achieved thanks to the stabilization of the carrier-envelope phase (CEP) of amplified light pulses. In this work we demonstrate that the polarization gating (PG) method with few-cycle phase-stabilized driving pulses allows one to generate few-cycle isolated attosecond pulses tunable on a very broad spectral region. The PG method is based on temporal modulation of the ellipticity of a light pulse, which confines the XUV emission in the temporal gate where the polarization is close to linear. The time-dependent polarization of phase-stabilized sub-6-fs pulses, generated by the hollow fiber technique, has been obtained using two birefringent plates. It is possible to create a linear polarization gate, whose position is imposed by the intensity profile of the pulse whilst the emission time is linked to the CEP of the electric field. The pulses have been analyzed by using a flat-field spectrometer. Continuous XUV spectra, corresponding to the production of isolated attosecond pulses, have been generated for particular CEP values. Upon changing the rotation of the first plate it was possible to tune the XUV emission in a broad spectra range. We have then achieved a complete temporal characterization of the generated isolated attosecond pulses using frequency-resolved optical gating for complete reconstruction of attosecond bursts (FROG CRAB). The measured parabolic phase

Dynamical spin susceptibility of electron-doped high-Tc cuprates. Comparison with hole-doped systems

International Nuclear Information System (INIS)

Suzuki, Atsuo; Mutou, Tetsuya; Tanaka, Syunsuke; Hirashima, Dai S.

2010-01-01

The magnetic excitation spectrum of electron-doped copper oxide superconductors is studied by calculating the dynamical spin susceptibility of the two-dimensional Hubbard model in which a d x2-y2 -wave superconducting order parameter is assumed. The spectrum of electron-doped systems is compared with that of hole-doped systems, and the relationship between the frequency at which a peak grows in the spectrum and the superconducting energy gap at a hot spot is investigated. A peak may be observed even when the magnetic resonance condition is not exactly satisfied. We find that, in the electron-doped systems, the resonance condition is less likely to be satisfied than in the hole-doped systems because of the small density of states around the hot spots, and the peak frequency is close to twice the gap magnitude at the hot spots. (author)

Time-resolved imaging of purely valence-electron dynamics during a chemical reaction

DEFF Research Database (Denmark)

Hockett, Paul; Bisgaard, Christer Z.; Clarkin, Owen J.

2011-01-01

Chemical reactions are manifestations of the dynamics of molecular valence electrons and their couplings to atomic motions. Emerging methods in attosecond science can probe purely electronic dynamics in atomic and molecular systems(1-6). By contrast, time-resolved structural-dynamics methods...... such as electron(7-10) or X-ray diffraction(11) and X-ray absorption(12) yield complementary information about the atomic motions. Time-resolved methods that are directly sensitive to both valence-electron dynamics and atomic motions include photoelectron spectroscopy(13-15) and high-harmonic generation(16......,17): in both cases, this sensitivity derives from the ionization-matrix element(18,19). Here we demonstrate a time-resolved molecular-frame photoelectron-angular-distribution (TRMFPAD) method for imaging the purely valence-electron dynamics during a chemical reaction. Specifically, the TRMFPADs measured during...

Generation of Attosecond Light Pulses from Gas and Solid State Media

Directory of Open Access Journals (Sweden)

Stefanos Chatziathanasiou

2017-03-01

Full Text Available Real-time observation of ultrafast dynamics in the microcosm is a fundamental approach for understanding the internal evolution of physical, chemical and biological systems. Tools for tracing such dynamics are flashes of light with duration comparable to or shorter than the characteristic evolution times of the system under investigation. While femtosecond (fs pulses are successfully used to investigate vibrational dynamics in molecular systems, real time observation of electron motion in all states of matter requires temporal resolution in the attosecond (1 attosecond (asec = 10−18 s time scale. During the last decades, continuous efforts in ultra-short pulse engineering led to the development of table-top sources which can produce asec pulses. These pulses have been synthesized by using broadband coherent radiation in the extreme ultraviolet (XUV spectral region generated by the interaction of matter with intense fs pulses. Here, we will review asec pulses generated by the interaction of gas phase media and solid surfaces with intense fs IR laser fields. After a brief overview of the fundamental process underlying the XUV emission form these media, we will review the current technology, specifications and the ongoing developments of such asec sources.

Generation and Characterization of Attosecond Pulses. Final report

International Nuclear Information System (INIS)

Ian A. Walmsley; Robert W. Boyd

2006-01-01

The research undertaken in this project has been directed toward the area of attoscience, in particular the problem of attosecond metrology. That is, the accurate determination of the electric field of attosecond XUV radiation. This outstanding problem has been identified as a critical technology for further development of the field, and our research adds to the area by providing the first method for characterization using the harmonic radiation itself as a tool. The technical effectiveness of this approach is very high, since it is vastly easier to detect XUV radiation directly than via the spectrum of photoelectrons liberated from atoms by it. This means that the experimental data rate can be much higher in principle using all-optical detection that electron detection, which will greatly aid the utility of harmonic XUV sources in attoscience applications. There are as yet no direct public benefits from this area of scientific research, though access to material structural dynamics on unprecedented brief timescales are expected to yield significant benefits for the future

Correlated proton-electron hole dynamics in protonated water clusters upon extreme ultraviolet photoionization

Directory of Open Access Journals (Sweden)

Zheng Li

2016-07-01

Full Text Available The ultrafast nuclear and electronic dynamics of protonated water clusters H+(H2On after extreme ultraviolet photoionization is investigated. In particular, we focus on cluster cations with n = 3, 6, and 21. Upon ionization, two positive charges are present in the cluster related to the excess proton and the missing electron, respectively. A correlation is found between the cluster's geometrical conformation and initial electronic energy with the size of the final fragments produced. For situations in which the electron hole and proton are initially spatially close, the two entities become correlated and separate in a time-scale of 20 to 40 fs driven by strong non-adiabatic effects.

Correlated proton-electron hole dynamics in protonated water clusters upon extreme ultraviolet photoionization

Science.gov (United States)

Li, Zheng; Vendrell, Oriol

2016-01-01

The ultrafast nuclear and electronic dynamics of protonated water clusters H+(H2O)n after extreme ultraviolet photoionization is investigated. In particular, we focus on cluster cations with n = 3, 6, and 21. Upon ionization, two positive charges are present in the cluster related to the excess proton and the missing electron, respectively. A correlation is found between the cluster's geometrical conformation and initial electronic energy with the size of the final fragments produced. For situations in which the electron hole and proton are initially spatially close, the two entities become correlated and separate in a time-scale of 20 to 40 fs driven by strong non-adiabatic effects. PMID:26798842

Dynamics of electrons and holes at surfaces

International Nuclear Information System (INIS)

Chulkov, E.V.; Leonardo, A.; Sklyadneva, I.Yu.; Silkin, V.M.

2007-01-01

We present ab initio calculation results for electron-phonon (e-ph) contribution to hole lifetime broadening of the X-bar surface state on Al(0 0 1). We show that e-ph coupling in this state is significantly stronger than in bulk Al at the Fermi level. It makes the e-ph decay channel very important in the formation of the hole decay in the surface state at X-bar. We also present the results for e-e lifetime broadening in a quantum-well state in 1 ML K/Cu(1 1 1). We show that this contribution is not negligible and is much larger than that in a surface state on Ag(1 1 1)

A novel optical tool for controlling and probing ultrafast surface dynamics

International Nuclear Information System (INIS)

Yang, Yudong

2017-12-01

Ultrashort pulse laser sources have been greatly developed over the past few decades. The available pulse duration has been reduced to the single-cycle pulse regime. The discovery of high harmonic generation has freed us from the limitation of the laser wavelength. Moreover, the demonstration of isolated attosecond pulse generation has indicated the advent of the attosecond science era. Attosecond pulses undoubtedly allow one to study ultrafast dynamics with unprecedented time resolution. However, physical systems with genuine attosecond time scale dynamics are rather challenging to find. Ultrafast surface charge transfer, which is an important process in photochemistry and electrochemistry, is a good candidate experimental system exhibiting attosecond electronic dynamics. Specifically, the ultrafast surface charge transfer on the c(4 x 2)S/Ru(0001) surface was previously studied and the charge transfer time inferred to be 320 as using core-hole clock spectroscopy at a synchrotron facility. In order to measure this benchmark attosecond electronic dynamics with real time-resolving methods, pump pulses centered at 160 eV and probe pulses centered at 40 eV are required. To this end, a dedicated attosecond experimental beamline including an ultrashort laser pulse source and an attosecond pulse generation and characterization setup has been designed and is being developed. The author of this thesis was responsible for the construction of the attosecond experimental beamline which will be used ultrafast surface charge transfer studies. In this thesis, a completely functional attosecond extreme ultraviolet (XUV) beamline, which includes a few-cycle laser pulse source, an attosecond pulse generation and characterization setup, is described. A commercial Ti:sapphire-based chirped-pulse amplification (CPA) laser system is the overall source of the beamline. The laser system is actively carrier-envelope phase (CEP) stabilized and the output pulse duration is ∝35 fs. The

A novel optical tool for controlling and probing ultrafast surface dynamics

Energy Technology Data Exchange (ETDEWEB)

Yang, Yudong

2017-12-15

Ultrashort pulse laser sources have been greatly developed over the past few decades. The available pulse duration has been reduced to the single-cycle pulse regime. The discovery of high harmonic generation has freed us from the limitation of the laser wavelength. Moreover, the demonstration of isolated attosecond pulse generation has indicated the advent of the attosecond science era. Attosecond pulses undoubtedly allow one to study ultrafast dynamics with unprecedented time resolution. However, physical systems with genuine attosecond time scale dynamics are rather challenging to find. Ultrafast surface charge transfer, which is an important process in photochemistry and electrochemistry, is a good candidate experimental system exhibiting attosecond electronic dynamics. Specifically, the ultrafast surface charge transfer on the c(4 x 2)S/Ru(0001) surface was previously studied and the charge transfer time inferred to be 320 as using core-hole clock spectroscopy at a synchrotron facility. In order to measure this benchmark attosecond electronic dynamics with real time-resolving methods, pump pulses centered at 160 eV and probe pulses centered at 40 eV are required. To this end, a dedicated attosecond experimental beamline including an ultrashort laser pulse source and an attosecond pulse generation and characterization setup has been designed and is being developed. The author of this thesis was responsible for the construction of the attosecond experimental beamline which will be used ultrafast surface charge transfer studies. In this thesis, a completely functional attosecond extreme ultraviolet (XUV) beamline, which includes a few-cycle laser pulse source, an attosecond pulse generation and characterization setup, is described. A commercial Ti:sapphire-based chirped-pulse amplification (CPA) laser system is the overall source of the beamline. The laser system is actively carrier-envelope phase (CEP) stabilized and the output pulse duration is ∝35 fs. The

Isolated sub-100-as pulse generation via controlling electron dynamics

International Nuclear Information System (INIS)

Lan Pengfei; Lu Peixiang; Cao Wei; Li Yuhua; Wang Xinlin

2007-01-01

A method to coherently control electron dynamics is proposed using a few-cycle laser pulse in combination with a controlling field. It is shown that this method not only broadens the attosecond pulse bandwidth, but also reduces the chirp; thus an isolated 80-as pulse is straightforwardly obtained, and even shorter pulses are achievable by increasing the intensity of the controlling field. Such ultrashort pulses allow one to investigate ultrafast electronic processes. In addition, the few-cycle synthesized pulse is expected to be useful for manipulating a wide range of laser-atom interactions

Attosecond control of orbital parity mix interferences and the relative phase of even and odd harmonics in an attosecond pulse train.

Science.gov (United States)

Laurent, G; Cao, W; Li, H; Wang, Z; Ben-Itzhak, I; Cocke, C L

2012-08-24

We experimentally demonstrate that atomic orbital parity mix interferences can be temporally controlled on an attosecond time scale. Electron wave packets are formed by ionizing argon gas with a comb of odd and even high-order harmonics, in the presence of a weak infrared field. Consequently, a mix of energy-degenerate even and odd parity states is fed in the continuum by one- and two-photon transitions. These interfere, leading to an asymmetric electron emission along the polarization vector. The direction of the emission can be controlled by varying the time delay between the comb and infrared field pulses. We show that such asymmetric emission provides information on the relative phase of consecutive odd and even order harmonics in the attosecond pulse train.

Assembly and application of an instrument for attosecond-time-resolved ionization chronoscopy

International Nuclear Information System (INIS)

Uphues, T.

2006-11-01

In the framework of this thesis a new setup for attosecond time-resolved measurements has been built and observations of ionization dynamics in rare gas atoms have been made. This new technique is entitled Ionization Chronoscopy and gives further evidence that time-resolved experiments in the attosecond regime will become a powerful tool for investigations in atomic physics. (orig.)

Measurement and Control of Attosecond Pulses

Science.gov (United States)

2016-04-25

highest power or the shortest duration attosecond pulses. Results: We have adapted the attosecond lighthouse to gases and confirmed isolated...simplifying attosecond metrology so it becomes more widely accessible. Result: This goal was completely accomplished. Aim 2: To exploit few- cycle ...μm driver. Aim 3: To compare attosecond gating methods, selecting the most efficient way to produce the highest power or the shortest duration

Attosecond interference control of XUV photoionization

Energy Technology Data Exchange (ETDEWEB)

Cao Wei; Lu Peixiang; Lan Pengfei; Li Yuhua; Wang Xinlin [Wuhan National Laboratory for Optoelectronics and School of Optoelectronics Science and Engineering, Huazhong University of Science and Technology, Wuhan 430074 (China)], E-mail: lupeixiang@mail.hust.edu.cn

2008-04-28

The characterizing of attosecond pulses has great importance for the investigation of ultrafast phenomena. Here, we proposed a novel and efficient scheme for measuring attosecond XUV pulses, which is based on laser-dressed XUV photoionization. The ultrashort attosecond gating of photoionization leads to an interference structure in the photoelectron spectrum. Then the duration of the attosecond XUV pulse can be retrieved directly from the photoelectron spectrum with a rather high resolution.

Attosecond interference control of XUV photoionization

International Nuclear Information System (INIS)

Cao Wei; Lu Peixiang; Lan Pengfei; Li Yuhua; Wang Xinlin

2008-01-01

The characterizing of attosecond pulses has great importance for the investigation of ultrafast phenomena. Here, we proposed a novel and efficient scheme for measuring attosecond XUV pulses, which is based on laser-dressed XUV photoionization. The ultrashort attosecond gating of photoionization leads to an interference structure in the photoelectron spectrum. Then the duration of the attosecond XUV pulse can be retrieved directly from the photoelectron spectrum with a rather high resolution

AXSIS: Exploring the frontiers in attosecond X-ray science, imaging and spectroscopy

Energy Technology Data Exchange (ETDEWEB)

Kärtner, F.X., E-mail: franz.kaertner@cfel.de [Center for Free-Electron Laser Science, Hamburg (Germany); Institute for Experimental Physics, University of Hamburg, Hamburg (Germany); The Hamburg Center for Ultrafast Imaging, Hamburg (Germany); DESY, Hamburg (Germany); Research Laboratory of Electronics, Massachusetts Institute of Technology, Cambridge, MA (United States); Ahr, F. [Center for Free-Electron Laser Science, Hamburg (Germany); Institute for Experimental Physics, University of Hamburg, Hamburg (Germany); DESY, Hamburg (Germany); Max Planck Institute for the Structure and Dynamics of Matter, Hamburg (Germany); Calendron, A.-L. [Center for Free-Electron Laser Science, Hamburg (Germany); Institute for Experimental Physics, University of Hamburg, Hamburg (Germany); The Hamburg Center for Ultrafast Imaging, Hamburg (Germany); DESY, Hamburg (Germany); Çankaya, H. [Center for Free-Electron Laser Science, Hamburg (Germany); The Hamburg Center for Ultrafast Imaging, Hamburg (Germany); DESY, Hamburg (Germany); Carbajo, S. [Center for Free-Electron Laser Science, Hamburg (Germany); Institute for Experimental Physics, University of Hamburg, Hamburg (Germany); DESY, Hamburg (Germany); Chang, G.; Cirmi, G. [Center for Free-Electron Laser Science, Hamburg (Germany); The Hamburg Center for Ultrafast Imaging, Hamburg (Germany); DESY, Hamburg (Germany); Dörner, K. [Center for Free-Electron Laser Science, Hamburg (Germany); DESY, Hamburg (Germany); Dorda, U. [DESY, Hamburg (Germany); Fallahi, A. [Center for Free-Electron Laser Science, Hamburg (Germany); DESY, Hamburg (Germany); Hartin, A. [Center for Free-Electron Laser Science, Hamburg (Germany); Institute for Experimental Physics, University of Hamburg, Hamburg (Germany); DESY, Hamburg (Germany); Hemmer, M. [Center for Free-Electron Laser Science, Hamburg (Germany); DESY, Hamburg (Germany); and others

2016-09-01

X-ray crystallography is one of the main methods to determine atomic-resolution 3D images of the whole spectrum of molecules ranging from small inorganic clusters to large protein complexes consisting of hundred-thousands of atoms that constitute the macromolecular machinery of life. Life is not static, and unravelling the structure and dynamics of the most important reactions in chemistry and biology is essential to uncover their mechanism. Many of these reactions, including photosynthesis which drives our biosphere, are light induced and occur on ultrafast timescales. These have been studied with high time resolution primarily by optical spectroscopy, enabled by ultrafast laser technology, but they reduce the vast complexity of the process to a few reaction coordinates. In the AXSIS project at CFEL in Hamburg, funded by the European Research Council, we develop the new method of attosecond serial X-ray crystallography and spectroscopy, to give a full description of ultrafast processes atomically resolved in real space and on the electronic energy landscape, from co-measurement of X-ray and optical spectra, and X-ray diffraction. This technique will revolutionize our understanding of structure and function at the atomic and molecular level and thereby unravel fundamental processes in chemistry and biology like energy conversion processes. For that purpose, we develop a compact, fully coherent, THz-driven attosecond X-ray source based on coherent inverse Compton scattering off a free-electron crystal, to outrun radiation damage effects due to the necessary high X-ray irradiance required to acquire diffraction signals. This highly synergistic project starts from a completely clean slate rather than conforming to the specifications of a large free-electron laser (FEL) user facility, to optimize the entire instrumentation towards fundamental measurements of the mechanism of light absorption and excitation energy transfer. A multidisciplinary team formed by laser

Fundamentals of attosecond optics

CERN Document Server

Chang, Zenghu

2011-01-01

Attosecond optical pulse generation, along with the related process of high-order harmonic generation, is redefining ultrafast physics and chemistry. A practical understanding of attosecond optics requires significant background information and foundational theory to make full use of these cutting-edge lasers and advance the technology toward the next generation of ultrafast lasers. Fundamentals of Attosecond Optics provides the first focused introduction to the field. The author presents the underlying concepts and techniques required to enter the field, as well as recent research advances th

Separation of electron and hole dynamics in the semimetal LaSb

Energy Technology Data Exchange (ETDEWEB)

Han, F.; Xu, J.; Botana, A. S.; Xiao, Z. L.; Wang, Y. L.; Yang, W. G.; Chung, D. Y.; Kanatzidis, M. G.; Norman, M. R.; Crabtree, G. W.; Kwok, W. K.

2017-09-01

We report investigations on the magnetotransport in LaSb, which exhibits extremely large magnetoresistance (XMR). Foremost, we demonstrate that the resistivity plateau can be explained without invoking topological protection. We then determine the Fermi surface from Shubnikov–de Haas (SdH) quantum oscillation measurements and find good agreement with the bulk Fermi pockets derived from first-principles calculations. Using a semiclassical theory and the experimentally determined Fermi pocket anisotropies, we quantitatively describe the orbital magnetoresistance, including its angle dependence.We show that the origin of XMR in LaSb lies in its high mobility with diminishing Hall effect, where the high mobility leads to a strong magnetic-field dependence of the longitudinal magnetoconductance. Unlike a one-band material, when a system has two or more bands (Fermi pockets) with electron and hole carriers, the added conductance arising from the Hall effect is reduced, hence revealing the latent XMR enabled by the longitudinal magnetoconductance. With diminishing Hall effect, the magnetoresistivity is simply the inverse of the longitudinal magnetoconductivity, enabling the differentiation of the electron and hole contributions to the XMR, which varies with the strength and orientation of the magnetic field. This work demonstrates a convenient way to separate the dynamics of the charge carriers and to uncover the origin of XMR in multiband materials with anisotropic Fermi surfaces. Our approach can be readily applied to other XMR materials.

Ultrafast quantum control of ionization dynamics in krypton.

Science.gov (United States)

Hütten, Konrad; Mittermair, Michael; Stock, Sebastian O; Beerwerth, Randolf; Shirvanyan, Vahe; Riemensberger, Johann; Duensing, Andreas; Heider, Rupert; Wagner, Martin S; Guggenmos, Alexander; Fritzsche, Stephan; Kabachnik, Nikolay M; Kienberger, Reinhard; Bernhardt, Birgitta

2018-02-19

Ultrafast spectroscopy with attosecond resolution has enabled the real time observation of ultrafast electron dynamics in atoms, molecules and solids. These experiments employ attosecond pulses or pulse trains and explore dynamical processes in a pump-probe scheme that is selectively sensitive to electronic state of matter via photoelectron or XUV absorption spectroscopy or that includes changes of the ionic state detected via photo-ion mass spectrometry. Here, we demonstrate how the implementation of combined photo-ion and absorption spectroscopy with attosecond resolution enables tracking the complex multidimensional excitation and decay cascade of an Auger auto-ionization process of a few femtoseconds in highly excited krypton. In tandem with theory, our study reveals the role of intermediate electronic states in the formation of multiply charged ions. Amplitude tuning of a dressing laser field addresses different groups of decay channels and allows exerting temporal and quantitative control over the ionization dynamics in rare gas atoms.

Attosecond physics attosecond measurements and control of physical systems

CERN Document Server

Torres, Ricardo; Zaïr, Amelle

2013-01-01

Attophysics is an emerging field in physics devoted to the study and characterization of matter dynamics in the sub-femtosecond time scale. This book gives coverage of a broad set of selected topics in this field, exciting by their novelty and their potential impact. The book is written review-like. It also includes fundamental chapters as introduction to the field for non-specialist physicists. The book is structured in four sections: basics, attosecond pulse technology, applications to measurements and control of physical processes and future perspectives. It is a valuable reference tool for researchers in the field as well as a concise introduction to non-specialist readers.

Attosecond Delays in Molecular Photoionization.

Science.gov (United States)

Huppert, Martin; Jordan, Inga; Baykusheva, Denitsa; von Conta, Aaron; Wörner, Hans Jakob

2016-08-26

We report measurements of energy-dependent photoionization delays between the two outermost valence shells of N_{2}O and H_{2}O. The combination of single-shot signal referencing with the use of different metal foils to filter the attosecond pulse train enables us to extract delays from congested spectra. Remarkably large delays up to 160 as are observed in N_{2}O, whereas the delays in H_{2}O are all smaller than 50 as in the photon-energy range of 20-40 eV. These results are interpreted by developing a theory of molecular photoionization delays. The long delays measured in N_{2}O are shown to reflect the population of molecular shape resonances that trap the photoelectron for a duration of up to ∼110 as. The unstructured continua of H_{2}O result in much smaller delays at the same photon energies. Our experimental and theoretical methods make the study of molecular attosecond photoionization dynamics accessible.

Attosecond delays in photoionization: time and quantum mechanics

International Nuclear Information System (INIS)

Maquet, Alfred; Caillat, Jérémie; Taïeb, Richard

2014-01-01

This article addresses topics regarding time measurements performed on quantum systems. The motivation is linked to the advent of ‘attophysics’ which makes feasible to follow the motion of electrons in atoms and molecules, with time resolution at the attosecond (1 as = 10 −18 s) level, i.e. at the natural scale for electronic processes in these systems. In this context, attosecond ‘time-delays’ have been recently measured in experiments on photoionization and the question arises if such advances could cast a new light on the still active discussion on the status of the time variable in quantum mechanics. One issue still debatable is how to decide whether one can define a quantum time operator with eigenvalues associated to measurable ‘time-delays’, or time is a parameter, as it is implicit in the Newtonian classical mechanics. One objective of this paper is to investigate if the recent attophysics-based measurements could shed light on this parameter–operator conundrum. To this end, we present here the main features of the theory background, followed by an analysis of the experimental schemes that have been used to evidence attosecond ‘time-delays’ in photoionization. Our conclusion is that these results reinforce the view that time is a parameter which cannot be defined without reference to classical mechanics. (tutorial)

Correlation effects on spin-polarized electron-hole quantum bilayer

Energy Technology Data Exchange (ETDEWEB)

Saini, L. K., E-mail: drlalitsaini75@gmail.com; Sharma, R. O., E-mail: sharmarajesh0387@gmail.com [Department of Applied Physics, S. V. National Institute of Technology, Surat – 395 007 (India); Nayak, Mukesh G. [Department of Physics, Silvassa College (Silvassa Institute of Higher Learning), Silvassa 396 230 (India)

2016-05-06

We present a numerical calculation for the intra- and interlayer pair-correlation functions, g{sub ll’}(r), of spin-polarized electron-hole quantum bilayers at zero temperature. The calculations of g{sub ll’}(r) are performed by including electron correlations within the dynamical version of the self-consistent mean-field approximation of Singwi, Tosi, Land and Sjölander (qSTLS). Our study reveals that the critical layer density decreases (increases) due to the inclusion of finite width (mass-asymmetry) effect during the phase-transition from charge-density wave to Wigner crystal ground-state by yielding the pronounced oscillatory behavior ing{sub ll}(r). The results are compared with recent findings of spin-polarized electron-hole quantum bilayers with mass-symmetry and zero width effects. To highlight the importance of dynamical character of correlations, we have also compared our results with the STLS results.

Observing electron motion in molecules

International Nuclear Information System (INIS)

Chelkowski, S; Yudin, G L; Bandrauk, A D

2006-01-01

We study analytically the possibility for monitoring electron motion in a molecule using two ultrashort laser pulses. The first prepares a coherent superposition of two electronic molecular states whereas the second (attosecond pulse) photoionizes the molecule. We show that interesting information about electron dynamics can be obtained from measurement of the photoelectron spectra as a function of the time delay between two pulses. In particular, asymmetries in photoelectron angular distribution provide a simple signature of the electron motion within the initial time-dependent coherently coupled two molecular states. Both asymmetries and electron spectra show very strong two-centre interference patterns. We illustrate these effects using as an example a dissociating hydrogen molecular ion probed by the attosecond pulses

Generation of atto-second pulses on relativistic mirror plasma

International Nuclear Information System (INIS)

Vincenti, H.

2012-12-01

When an ultra intense femtosecond laser (I > 10 16 W.cm -2 ) with high contrast is focused on a solid target, the laser field at focus is high enough to completely ionize the target surface during the rising edge of the laser pulse and form a plasma. This plasma is so dense (the electron density is of the order of hundred times the critical density) that it completely reflects the incident laser beam in the specular direction: this is the so-called 'plasma mirror'. When laser intensity becomes very high, the non-linear response of the plasma mirror to the laser field periodically deforms the incident electric field leading to high harmonic generation in the reflected beam. In the temporal domain this harmonic spectrum is associated to a train of atto-second pulses. The goals of my work were to get a better comprehension of the properties of harmonic beams produced on plasma mirrors and design new methods to control theses properties, notably in order to produce isolated atto-second pulses instead of trains. Initially, we imagined and modeled the first realistic technique to generate isolated atto-second on plasma mirrors. This brand new approach is based on a totally new physical effect: 'the atto-second lighthouse effect'. Its principle consists in sending the atto-second pulses of the train in different directions and selects one of these pulses by putting a slit in the far field. Despite its simplicity, this technique is very general and applies to any high harmonic generation mechanism. Moreover, the atto-second lighthouse effect has many other applications (e.g in metrology). In particular, it paves the way to atto-second pump-probe experiments. Then, we studied the spatial properties of these harmonics, whose control and characterization are crucial if one wants to use this source in future application experiments. For instance, we need to control very precisely the harmonic beam divergence in order to achieve the atto-second lighthouse effect and get

Reflection of attosecond x-ray free electron laser pulses

International Nuclear Information System (INIS)

Hau-Riege, Stefan P.; Chapman, Henry N.

2007-01-01

In order to utilize hard x-ray free electron lasers (XFEL's) when they are extended to attosecond pulse lengths, it is necessary to choose optical elements with minimal response time. Specular grazing-incidence optics made of low-Z materials are popular candidates for reflectors since they are likely to withstand x-ray damage and provide sufficiently large reflectivities. Using linear-optics reflection theory, we calculated the transient reflectivity of a delta-function electric pulse from a homogenous semi-infinite medium as a function of angle of incidence for s- and p-polarized light. We specifically considered the pulse response of beryllium, diamond, silicon carbide, and silicon, all of which are of relevance to the XFEL's that are currently being built. We found that the media emit energy in a damped oscillatory way, and that the impulse-response times are shorter than 0.3 fs for normal incidence. For grazing incidence, the impulse-response time is substantially shorter, making grazing-incidence mirrors a good choice for deep subfemtosecond reflective optics

High Harmonic Radiation Generation and Attosecond pulse generation from Intense Laser-Solid Interactions

Energy Technology Data Exchange (ETDEWEB)

Thomas, Alexander Roy [Univ. of Michigan, Ann Arbor, MI (United States); Krushelnick, Karl [Univ. of Michigan, Ann Arbor, MI (United States)

2016-09-08

We have studied ion motion effects in high harmonic generation, including shifts to the harmonics which result in degradation of the attosecond pulse train, and how to mitigate them. We have examined the scaling with intensity of harmonic emission. We have also switched the geometry of the interaction to measure, for the first time, harmonics from a normal incidence interaction. This was performed by using a special parabolic reflector with an on axis hole and is to allow measurements of the attosecond pulses using standard techniques. Here is a summary of the findings: First high harmonic generation in laser-solid interactions at 10²¹ Wcm^-2, demonstration of harmonic focusing, study of ion motion effects in high harmonic generation in laser-solid interactions, and demonstration of harmonic amplification.

Attosecond-controlled photoemission from metal nanowire tips in the few-electron regime

KAUST Repository

Ahn, B.

2017-02-07

Metal nanotip photoemitters have proven to be versatile in fundamental nanoplasmonics research and applications, including, e.g., the generation of ultrafast electron pulses, the adiabatic focusing of plasmons, and as light-triggered electron sources for microscopy. Here, we report the generation of high energy photoelectrons (up to 160 eV) in photoemission from single-crystalline nanowire tips in few-cycle, 750-nm laser fields at peak intensities of (2-7.3) × 1012 W/cm2. Recording the carrier-envelope phase (CEP)-dependent photoemission from the nanowire tips allows us to identify rescattering contributions and also permits us to determine the high-energy cutoff of the electron spectra as a function of laser intensity. So far these types of experiments from metal nanotips have been limited to an emission regime with less than one electron per pulse. We detect up to 13 e/shot and given the limited detection efficiency, we expect up to a few ten times more electrons being emitted from the nanowire. Within the investigated intensity range, we find linear scaling of cutoff energies. The nonlinear scaling of electron count rates is consistent with tunneling photoemission occurring in the absence of significant charge interaction. The high electron energy gain is attributed to field-induced rescattering in the enhanced nanolocalized fields at the wires apex, where a strong CEP-modulation is indicative of the attosecond control of photoemission.

Electron-hole liquid in semiconductors and low-dimensional structures

Science.gov (United States)

Sibeldin, N. N.

2017-11-01

The condensation of excitons into an electron-hole liquid (EHL) and the main EHL properties in bulk semiconductors and low-dimensional structures are considered. The EHL properties in bulk materials are discussed primarily in qualitative terms based on the experimental results obtained for germanium and silicon. Some of the experiments in which the main EHL thermodynamic parameters (density and binding energy) have been obtained are described and the basic factors that determine these parameters are considered. Topics covered include the effect of external perturbations (uniaxial strain and magnetic field) on EHL stability; phase diagrams for a nonequilibrium exciton-gas-EHL system; information on the size and concentration of electron-hole drops (EHDs) under various experimental conditions; the kinetics of exciton condensation and of recombination in the exciton-gas-EHD system; dynamic EHD properties and the motion of EHDs under the action of external forces; the properties of giant EHDs that form in potential wells produced by applying an inhomogeneous strain to the crystal; and effects associated with the drag of EHDs by nonequilibrium phonons (phonon wind), including the dynamics and formation of an anisotropic spatial structure of the EHD cloud. In discussing EHLs in low-dimensional structures, a number of studies are reviewed on the observation and experimental investigation of phenomena such as spatially indirect (dipolar) electron-hole and exciton (dielectric) liquids in GaAs/AlGaAs structures with double quantum wells (QWs), EHDs containing only a few electron-hole pairs (dropletons), EHLs in type-I silicon QWs, and spatially direct and dipolar EHLs in type-II silicon-germanium heterostructures.

Atomic and molecular dynamics triggered by ultrashort light pulses on the atto- to picosecond time scale

Science.gov (United States)

Pabst, Stefan

2013-04-01

Time-resolved investigations of ultrafast electronic and molecular dynamics were not possible until recently. The typical time scale of these processes is in the picosecond to attosecond realm. The tremendous technological progress in recent years made it possible to generate ultrashort pulses, which can be used to trigger, to watch, and to control atomic and molecular motion. This tutorial focuses on experimental and theoretical advances which are used to study the dynamics of electrons and molecules in the presence of ultrashort pulses. In the first part, the rotational dynamics of molecules, which happens on picosecond and femtosecond time scales, is reviewed. Well-aligned molecules are particularly suitable for angle-dependent investigations like x-ray diffraction or strong-field ionization experiments. In the second part, the ionization dynamics of atoms is studied. The characteristic time scale lies, here, in the attosecond to few-femtosecond regime. Although a one-particle picture has been successfully applied to many processes, many-body effects do constantly occur. After a broad overview of the main mechanisms and the most common tools in attosecond physics, examples of many-body dynamics in the attosecond world (e.g., in high-harmonic generation and attosecond transient absorption spectroscopy) are discussed.

Formation and Coalescence of Electron Solitary Holes

DEFF Research Database (Denmark)

Saeki, K.; Michelsen, Poul; Pécseli, H. L.

1979-01-01

Electron solitary holes were observed in a magnetized collisionless plasma. These holes were identified as Bernstein-Green-Kruskal equilibria, thus being purely kinetic phenomena. The electron hole does not damp even though its velocity is close to the electron thermal velocity. Two holes attract...

Attosecond time delay in the valence photoionization of C240 versus C60

International Nuclear Information System (INIS)

Shi, Kele; Magrakvelidze, Maia; Anstine, Dylan; Chakraborty, Himadri; Madjet, Mohamed

2015-01-01

We investigate effects of electron correlations on the attosecond time delay of the photoionization from HOMO and HOMO-1 electrons in C 240 . A comparison with earlier C 60 results assesses the molecular size effect. (paper)

Generation of Attosecond X-Ray Pulse through Coherent Relativistic Nonlinear Thomson Scattering

CERN Document Server

Lee, K; Jeong, Y U; Lee, B C; Park, S H

2005-01-01

In contrast to some recent experimental results, which state that the Nonlinear Thomson Scattered (NTS) radiation is incoherent, a coherent condition under which the scattered radiation of an incident laser pulse by a bunch of electrons can be coherently superposed has been investigated. The Coherent Relativistic Nonlinear Thomson Scattered (C-RNTS) radiation makes it possible utilizing the ultra-short pulse nature of NTS radiation with a bunch of electrons, such as plasma or electron beams. A numerical simulation shows that a 25 attosecond X-ray pulse can be generated by irradiating an ultra-intense laser pulse of 4x10(19) W/cm2 on an ultra-thin solid target of 50 nm thickness, which is commercially available. The coherent condition can be easily extended to an electron beam from accelerators. Different from the solid target, much narrower electron beam is required for the generation of an attosecond pulse. Instead, this condition could be applied for the generation of intense Compton scattered X-rays with a...

Relativistic attosecond electron bunch emission from few-cycle laser irradiated nanoscale droplets

Directory of Open Access Journals (Sweden)

Laura Di Lucchio

2015-02-01

Full Text Available Attosecond electron bunches produced at the surface of nanometer-scale droplets illuminated by a two-cycle laser pulse are investigated for the purpose of determining their optimal emission characteristics. Significant departures from Mie theory are found for electron bunch emission from droplets whose radii satisfy the condition δ_{r}

Attosecond delay in the molecular photoionization of asymmetric molecules.

Science.gov (United States)

Chacón, Alexis; Ruiz, Camilo

2018-02-19

We report theoretical calculations of the delay in photoemission from CO with particular emphasis on the role of the ultrafast electronic bound dynamics. We study the delays in photoionization in the HOMO and HOMO-1 orbitals of the CO molecule by looking into the stereo Wigner time delay technique. That compares the delay in photoemission from electrons emitted to the left and right to extract structural and dynamical information of the ionization process. For this we apply two techniques: The attosecond streak camera and the time of flight technique. Although they should provide the same results we have found large discrepancies of up to 36 in the case of HOMO, while for the HOMO-1 we obtain the same results with the two techniques. We have found that the large time delays observed in the HOMO orbital with the streaking technique are a consequence of the resonant transition triggered by the streaking field. This resonant transition produces a bound electron wavepacket that modifies the measurements of delay in photoionization. As a result of this observation, our technique allows us to reconstruct the bound wavepacket dynamics induced by the streaking field. By measuring the expected value of the electron momentum along the polarization direction after the streaking field has finished, we can recover the relative phase between the complex amplitudes of the HOMO and LUMO orbitals. These theoretical calculations pave the way for the measurement of ultrafast bound-bound electron transitionsand its crucial role for the delay in photoemission observation.

Vlasov simulations of electron hole dynamics in inhomogeneous magnetic field

Science.gov (United States)

Kuzichev, Ilya; Vasko, Ivan; Agapitov, Oleksiy; Mozer, Forrest; Artemyev, Anton

2017-04-01

Electron holes (EHs) or phase space vortices are solitary electrostatic waves existing due to electrons trapped within EH electrostatic potential. Since the first direct observation [1], EHs have been widely observed in the Earth's magnetosphere: in reconnecting current sheets [2], injection fronts [3], auroral region [4], and many other space plasma systems. EHs have typical spatial scales up to tens of Debye lengths, electric field amplitudes up to hundreds of mV/m and propagate along magnetic field lines with velocities of about electron thermal velocity [5]. The role of EHs in energy dissipation and supporting of large-scale potential drops is under active investigation. The accurate interpretation of spacecraft observations requires understanding of EH evolution in inhomogeneous plasma. The critical role of plasma density gradients in EH evolution was demonstrated in [6] using PIC simulations. Interestingly, up to date no studies have addressed a role of magnetic field gradients in EH evolution. In this report, we use 1.5D gyrokinetic Vlasov code to demonstrate the critical role of magnetic field gradients in EH dynamics. We show that EHs propagating into stronger (weaker) magnetic field are decelerated (accelerated) with deceleration (acceleration) rate dependent on the magnetic field gradient. Remarkably, the reflection points of decelerating EHs are independent of the average magnetic field gradient in the system and depend only on the EH parameters. EHs are decelerated (accelerated) faster than would follow from the "quasi-particle" concept assuming that EH is decelerated (accelerated) entirely due to the mirror force acting on electrons trapped within EH. We demonstrate that EH propagation in inhomogeneous magnetic fields results in development of a net potential drop along an EH, which depends on the magnetic field gradient. The revealed features will be helpful for interpreting spacecraft observations and results of advanced particle simulations. In

Plasma electron hole kinematics. I. Momentum conservation

Energy Technology Data Exchange (ETDEWEB)

Hutchinson, I. H.; Zhou, C. [Plasma Science and Fusion Center, Massachusetts Institute of Technology, Cambridge, Massachusetts 02139 (United States)

2016-08-15

We analyse the kinematic properties of a plasma electron hole: a non-linear self-sustained localized positive electric potential perturbation, trapping electrons, which behaves as a coherent entity. When a hole accelerates or grows in depth, ion and electron plasma momentum is changed both within the hole and outside, by an energization process we call jetting. We present a comprehensive analytic calculation of the momentum changes of an isolated general one-dimensional hole. The conservation of the total momentum gives the hole's kinematics, determining its velocity evolution. Our results explain many features of the behavior of hole speed observed in numerical simulations, including self-acceleration at formation, and hole pushing and trapping by ion streams.

Nondipole effects in attosecond photoelectron streaking

DEFF Research Database (Denmark)

Spiewanowski, Maciek; Madsen, Lars Bojer

2012-01-01

The influence of nondipole terms on the time delay in photoionization by an extreme-ultraviolet attosecond pulse in the presence of a near-infrared femtosecond laser pulse from 1s, 2s, and 2p states in hydrogen is investigated. In this attosecond photoelectron streaking process, the relative...

Breaking the Attosecond, Angstrom and TV/m Field Barriers with Ultrafast Electron Beams

International Nuclear Information System (INIS)

Rosenzweig, J. B.; Andonian, G.; Fukasawa, A.; Hemsing, E.; Marcus, G.; Marinelli, A.; Musumeci, P.; O'Shea, B.; O'Shea, F.; Pellegrini, C.; Schiller, D.; Travish, G.; Bucksbaum, P.; Hogan, M.; Krejcik, Patrick; Ferrario, M.; Muggli, Patric

2010-01-01

Recent initiatives at UCLA concerning ultra-short, GeV electron beam generation have been aimed at achieving sub-fs pulses capable of driving X-ray free-electron lasers (FELs) in single-spike mode. This scheme uses very low charge beams, which may allow existing FEL injectors to produce few-100 attosecond pulses, with very high brightness. Towards this end, recent experiments at the Stanford X-ray FEL (LCLS, first of its kind, built with essential UCLA leadership) have produced ∼2 fs, 20 pC electron pulses. We discuss here extensions of this work, in which we seek to exploit the beam brightness in FELs, in tandem with new developments at UCLA in cryogenic undulator technology, to create compact accelerator/undulator systems that can lase below 0.15 Angst , or be used to permit 1.5 Angst operation at 4.5 GeV. In addition, we are now developing experiments which use the present LCLS fs pulses to excite plasma wakefields exceeding 1 TV/m, permitting a table-top TeV accelerator for frontier high energy physics applications. We discuss the experimental issues associated with this initiative.

Hole dynamics and spin currents after ionization in strong circularly polarized laser fields

International Nuclear Information System (INIS)

Barth, Ingo; Smirnova, Olga

2014-01-01

We apply the time-dependent analytical R-matrix theory to develop a movie of hole motion in a Kr atom upon ionization by strong circularly polarized field. We find rich hole dynamics, ranging from rotation to swinging motion. The motion of the hole depends on the final energy and the spin of the photoelectron and can be controlled by the laser frequency and intensity. Crucially, hole rotation is a purely non-adiabatic effect, completely missing in the framework of quasistatic (adiabatic) tunneling theories. We explore the possibility to use hole rotation as a clock for measuring ionization time. Analyzing the relationship between the relative phases in different ionization channels we show that in the case of short-range electron-core interaction the hole is always initially aligned along the instantaneous direction of the laser field, signifying zero delays in ionization. Finally, we show that strong-field ionization in circular fields creates spin currents (i.e. different flow of spin-up and spin-down density in space) in the ions. This phenomenon is intimately related to the production of spin-polarized electrons in strong laser fields Barth and Smirnova (2013 Phys. Rev. A 88 013401). We demonstrate that rich spin dynamics of electrons and holes produced during strong field ionization can occur in typical experimental conditions and does not require relativistic intensities or strong magnetic fields. (paper)

Isolated elliptically polarized attosecond soft X-ray with high-brilliance using polarization gating of harmonics from relativistic plasmas at oblique incidence.

Science.gov (United States)

Chen, Zi-Yu; Li, Xiao-Ya; Li, Bo-Yuan; Chen, Min; Liu, Feng

2018-02-19

The production of intense isolated attosecond pulse is a major goal in ultrafast research. Recent advances in high harmonic generation from relativistic plasma mirrors under oblique incidence interactions gave rise to photon-rich attosecond pulses with circular or elliptical polarization. However, to achieve an isolated elliptical attosecond pulse via polarization gating using currently available long driving pulses remains a challenge, because polarization gating of high harmonics from relativistic plasmas is assumed only possible at normal or near-normal incidence. Here we numerically demonstrate a scheme around this problem. We show that via control of plasma dynamics by managing laser polarization, it is possible to gate an intense single attosecond pulse with high ellipticity extending to the soft X-ray regime at oblique incidence. This approach thus paves the way towards a powerful tool enabling high-time-resolution probe of dynamics of chiral systems and magnetic materials with current laser technology.

Multiphoton Processes and Attosecond Physics

CERN Document Server

Midorikawa, Katsumi; 12th International Conference on Multiphoton Processes; 3rd International Conference on Attosecond Physics

2012-01-01

Recent advances in ultrashort pulsed laser technology have opened new frontiers in atomic, molecular and optical sciences. The 12th International Conference on Multiphoton Processes (ICOMP12) and the 3rd International Conference on Attosecond Physics (ATTO3), held jointly in Sapporo, Japan, during July 3-8, showcased studies at the forefront of research on multiphoton processes and attosecond physics. This book summarizes presentations and discussions from these two conferences.

Reconstruction of Attosecond Pulse Trains

Science.gov (United States)

Mairesse, Y.; Agostini, P.; Breger, P.; Carre, B.; Merdji, A.; Monchicourt, P.; Salieres, P.; Varju, K.; Gustafsson, E.; Johnsson, P.; Mauritsson, J.; Remetter, T.; L'Huillier, A.; Frasinski, L. J.

2006-11-01

We show that it is possible to completely reconstruct the intensity profile of the attosecond bursts emitted as a superposition of high harmonics from a series of RABBIT measurements carried out at different infrared intensities. The electric field can be recovered from a measurement of the central harmonic chirp. Timing, chirp and variations of the carrier-to-envelope phase of the attosecond bursts are accessible to the proposed method.

Time-resolved photoelectron spectroscopy of IR-driven electron dynamics in a charge transfer model system.

Science.gov (United States)

Falge, Mirjam; Fröbel, Friedrich Georg; Engel, Volker; Gräfe, Stefanie

2017-08-02

If the adiabatic approximation is valid, electrons smoothly adapt to molecular geometry changes. In contrast, as a characteristic of diabatic dynamics, the electron density does not follow the nuclear motion. Recently, we have shown that the asymmetry in time-resolved photoelectron spectra serves as a tool to distinguish between these dynamics [Falge et al., J. Phys. Chem. Lett., 2012, 3, 2617]. Here, we investigate the influence of an additional, moderately intense infrared (IR) laser field, as often applied in attosecond time-resolved experiments, on such asymmetries. This is done using a simple model for coupled electronic-nuclear motion. We calculate time-resolved photoelectron spectra and their asymmetries and demonstrate that the spectra directly map the bound electron-nuclear dynamics. From the asymmetries, we can trace the IR field-induced population transfer and both the field-driven and intrinsic (non-)adiabatic dynamics. This holds true when considering superposition states accompanied by electronic coherences. The latter are observable in the asymmetries for sufficiently short XUV pulses to coherently probe the coupled states. It is thus documented that the asymmetry is a measure for phases in bound electron wave packets and non-adiabatic dynamics.

Dynamical thermalization in isolated quantum dots and black holes

Science.gov (United States)

Kolovsky, Andrey R.; Shepelyansky, Dima L.

2017-01-01

We study numerically a model of quantum dot with interacting fermions. At strong interactions with small conductance the model is reduced to the Sachdev-Ye-Kitaev black-hole model while at weak interactions and large conductance it describes a Landau-Fermi liquid in a regime of quantum chaos. We show that above the Åberg threshold for interactions there is an onset of dynamical themalization with the Fermi-Dirac distribution describing the eigenstates of an isolated dot. At strong interactions in the isolated black-hole regime there is also the onset of dynamical thermalization with the entropy described by the quantum Gibbs distribution. This dynamical thermalization takes place in an isolated system without any contact with a thermostat. We discuss the possible realization of these regimes with quantum dots of 2D electrons and cold ions in optical lattices.

Theory of laser-assisted autoionization by attosecond light pulses

International Nuclear Information System (INIS)

Zhao, Z.X.; Lin, C.D.

2005-01-01

We present a quantum theory of the decay of an autoionizing state created in the attosecond xuv (extreme ultraviolet) pump and laser probe measurements within the strong field approximation employing resonance parameters from Fano's theory. From the electron spectra versus the pump-probe time delay, we show how the lifetimes of the resonances can be extracted directly from the time domain measurements

Attosecond-correlated dynamics of two electrons in argon

Indian Academy of Sciences (India)

2014-01-11

Jan 11, 2014 ... 2Max-Planck-Institut für Kernphysik, 69117 Heidelberg, Germany ... involving a highly correlated electronic transition state. ... laser is low, the recolliding electron can have a maximum energy of about 15 eV which.

Electron Hole Plasma in Solids Induced by Ultrashort XUV Laser Pulses

International Nuclear Information System (INIS)

Rethfeld, B.; Medvedev, N.

2013-01-01

Irradiation of solids with ultrashort XUV laser pulses leads to an excitation of electrons from the valence band and deeper shells to the conduction band leading to a nonequilibrium highly energetic electron hole plasma. We investigate the transient electron dynamics in a solid semiconductor and metal (silicon and aluminum, respectively) under irradiation with a femtosecond VUV to XUV laser pulse as used in experiments with the Free Electron Laser FLASH at DESY in Hamburg, Germany. Applying the Asymptotical Trajectory Monte-Carlo technique, we obtain the transient energy distribution of the excited and ionized electrons within the solid. Photon absorption by electrons in different bands and secondary excitation and ionization processes are simulated event by event. The method was extended in order to take into account the electronic band structure and Pauli's principle for electrons in the conduction band. In this talk we review our results on the dynamics of the transient electron-hole plasma, in particular its transient density and energy distribution in dependence on laser and material parameters. For semiconductors we introduce the concept of an ''effective energy gap'' for collective electronic excitation, which can be applied to estimate the free electron density after high-intensity ultrashort XUV laser pulse irradiation. For aluminum we demonstrate that the electronic spectra depend on the relaxation kinetics of the excited electronic subsystem. Experimentally observed spectra of emitted photons from irradiated aluminum can be explained well with our results. (author)

Cascading electron and hole transfer dynamics in a CdS/CdTe core-shell sensitized with bromo-pyrogallol red (Br-PGR): slow charge recombination in type II regime.

Science.gov (United States)

Maity, Partha; Debnath, Tushar; Chopra, Uday; Ghosh, Hirendra Nath

2015-02-14

Ultrafast cascading hole and electron transfer dynamics have been demonstrated in a CdS/CdTe type II core-shell sensitized with Br-PGR using transient absorption spectroscopy and the charge recombination dynamics have been compared with those of CdS/Br-PGR composite materials. Steady state optical absorption studies suggest that Br-PGR forms strong charge transfer (CT) complexes with both the CdS QD and CdS/CdTe core-shell. Hole transfer from the photo-excited QD and QD core-shell to Br-PGR was confirmed by both steady state and time-resolved emission spectroscopy. Charge separation was also confirmed by detecting electrons in the conduction band of the QD and the cation radical of Br-PGR as measured from femtosecond transient absorption spectroscopy. Charge separation in the CdS/Br-PGR composite materials was found to take place in three different pathways, by transferring the photo-excited hole of CdS to Br-PGR, electron injection from the photo-excited Br-PGR to the CdS QD, and direct electron transfer from the HOMO of Br-PGR to the conduction band of the CdS QD. However, in the CdS/CdTe/Br-PGR system hole transfer from the photo-excited CdS to Br-PGR and electron injection from the photo-excited Br-PGR to CdS take place after cascading through the CdTe shell QD. Charge separation also takes place via direct electron transfer from the Br-PGR HOMO to the conduction band of CdS/CdTe. Charge recombination (CR) dynamics between the electron in the conduction band of the CdS QD and the Br-PGR cation radical were determined by monitoring the bleach recovery kinetics. The CR dynamics were found to be much slower in the CdS/CdTe/Br-PGR system than in the CdS/Br-PGR system. The formation of the strong CT complex and the separation of charges cascading through the CdTe shell help to slow down charge recombination in the type II regime.

Dynamic study of a compressed electron layer during the hole-boring stage in a sharp-front laser interaction region

Directory of Open Access Journals (Sweden)

W. P. Wang

2012-08-01

Full Text Available This study investigates the dynamics of a compressed electron layer (CEL when a circularly polarized laser pulse with a sharp front irradiates a high-density foil. A time-dependent model for CEL motion during the hole-boring stage is proposed to describe details of the interaction for any shape of laser pulse. The opacity case, where the laser pulse is totally reflected, is investigated using this model. The results obtained are consistent with the results from particle-in-cell (PIC simulations. A relaxation distance determined by the laser-front steepness is necessary to build a stable CEL state before ions rejoin into the CEL. For the transparent case, the laser-front steepness is important for the formation of the stable CEL state at the back surface of the target. Considering the motion of ions, both the CEL and ion dynamics are important to rebalance the laser pressure and electrostatic charge-separation force as the hole-boring stage changes to the light-sail stage.

Particle creation rate for dynamical black holes

Energy Technology Data Exchange (ETDEWEB)

Firouzjaee, Javad T. [School of Astronomy, Institute for Research in Fundamental Sciences (IPM), Tehran (Iran, Islamic Republic of); University of Oxford, Department of Physics (Astrophysics), Oxford (United Kingdom); Ellis, George F.R. [University of Cape Town, Mathematics and Applied Mathematics Department, Rondebosch (South Africa)

2016-11-15

We present the particle creation probability rate around a general black hole as an outcome of quantum fluctuations. Using the uncertainty principle for these fluctuation, we derive a new ultraviolet frequency cutoff for the radiation spectrum of a dynamical black hole. Using this frequency cutoff, we define the probability creation rate function for such black holes. We consider a dynamical Vaidya model and calculate the probability creation rate for this case when its horizon is in a slowly evolving phase. Our results show that one can expect the usual Hawking radiation emission process in the case of a dynamical black hole when it has a slowly evolving horizon. Moreover, calculating the probability rate for a dynamical black hole gives a measure of when Hawking radiation can be killed off by an incoming flux of matter or radiation. Our result strictly suggests that we have to revise the Hawking radiation expectation for primordial black holes that have grown substantially since they were created in the early universe. We also infer that this frequency cut off can be a parameter that shows the primordial black hole growth at the emission moment. (orig.)

Single attosecond pulse from terahertz-assisted high-order harmonic generation

Science.gov (United States)

Balogh, Emeric; Kovacs, Katalin; Dombi, Peter; Fulop, Jozsef A.; Farkas, Gyozo; Hebling, Janos; Tosa, Valer; Varju, Katalin

2011-08-01

High-order harmonic generation by few-cycle 800 nm laser pulses in neon gas in the presence of a strong terahertz (THz) field is investigated numerically with propagation effects taken into account. Our calculations show that the combination of THz fields with up to 12 fs laser pulses can be an effective gating technique to generate single attosecond pulses. We show that in the presence of the strong THz field only a single attosecond burst can be phase matched, whereas radiation emitted during other half cycles disappears during propagation. The cutoff is extended and a wide supercontinuum appears in the near-field spectra, extending the available spectral width for isolated attosecond pulse generation from 23 to 93 eV. We demonstrate that phase-matching effects are responsible for the generation of isolated attosecond pulses, even in conditions when single-atom response yields an attosecond pulse train.

Single attosecond pulse from terahertz-assisted high-order harmonic generation

International Nuclear Information System (INIS)

Balogh, Emeric; Kovacs, Katalin; Dombi, Peter; Farkas, Gyozo; Fulop, Jozsef A.; Hebling, Janos; Tosa, Valer; Varju, Katalin

2011-01-01

High-order harmonic generation by few-cycle 800 nm laser pulses in neon gas in the presence of a strong terahertz (THz) field is investigated numerically with propagation effects taken into account. Our calculations show that the combination of THz fields with up to 12 fs laser pulses can be an effective gating technique to generate single attosecond pulses. We show that in the presence of the strong THz field only a single attosecond burst can be phase matched, whereas radiation emitted during other half cycles disappears during propagation. The cutoff is extended and a wide supercontinuum appears in the near-field spectra, extending the available spectral width for isolated attosecond pulse generation from 23 to 93 eV. We demonstrate that phase-matching effects are responsible for the generation of isolated attosecond pulses, even in conditions when single-atom response yields an attosecond pulse train.

Single attosecond pulse from terahertz-assisted high-order harmonic generation

Energy Technology Data Exchange (ETDEWEB)

Balogh, Emeric [Department of Optics and Quantum Electronics, University of Szeged, H-6701 Szeged (Hungary); Kovacs, Katalin [Department of Optics and Quantum Electronics, University of Szeged, H-6701 Szeged (Hungary); National Institute for R and D of Isotopic and Molecular Technologies, RO-400293 Cluj-Napoca (Romania); Dombi, Peter; Farkas, Gyozo [Research Institute for Solid State Physics and Optics, H-1525 Budapest (Hungary); Fulop, Jozsef A.; Hebling, Janos [Department of Experimental Physics, University of Pecs, H-7624 Pecs (Hungary); Tosa, Valer [National Institute for R and D of Isotopic and Molecular Technologies, RO-400293 Cluj-Napoca (Romania); Varju, Katalin [HAS Research Group on Laser Physics, University of Szeged, H-6701 Szeged (Hungary)

2011-08-15

High-order harmonic generation by few-cycle 800 nm laser pulses in neon gas in the presence of a strong terahertz (THz) field is investigated numerically with propagation effects taken into account. Our calculations show that the combination of THz fields with up to 12 fs laser pulses can be an effective gating technique to generate single attosecond pulses. We show that in the presence of the strong THz field only a single attosecond burst can be phase matched, whereas radiation emitted during other half cycles disappears during propagation. The cutoff is extended and a wide supercontinuum appears in the near-field spectra, extending the available spectral width for isolated attosecond pulse generation from 23 to 93 eV. We demonstrate that phase-matching effects are responsible for the generation of isolated attosecond pulses, even in conditions when single-atom response yields an attosecond pulse train.

Spectral Caustics in Attosecond Science

Directory of Open Access Journals (Sweden)

Dudovich N.

2013-03-01

Full Text Available A unique type of singularity common in wave phenomena, known as caustics, links processes observed in many different branches of physics [1]. We investigate the role of caustics in attosecond science and in particular the physical process behind high harmonic generation. By exploiting singularities of the three-step model that describes HHG, we can manipulate and enhance specific features in the emitted harmonic spectrum. This new level of control holds promises in both scientific and technological aspects of attosecond science, and provides a deeper insight into the basic mechanism underlying the high harmonic generation process.

Generation of attosecond soft X-ray pulses in a longitudinal space charge amplifier

Energy Technology Data Exchange (ETDEWEB)

Dohlus, M.; Schneidmiller, E.A.; Yurkov, M.V. [Deutsches Elektronen-Synchrotron (DESY), Hamburg (Germany)

2011-03-15

A longitudinal space charge amplifier (LSCA), operating in soft X-ray regime, was recently proposed. Such an amplifier consists of a few amplification cascades (focusing channel and chicane) and a short radiator undulator in the end. Broadband nature of LSCA supports generation of few-cycle pulses as well as wavelength compression. In this paper we consider an application of these properties of LSCA for generation of attosecond X-ray pulses. It is shown that a compact and cheap addition to the soft X-ray free electron laser facility FLASH would allow to generate 60 attosecond (FWHM) long X-ray pulses with the peak power at 100 MW level and a contrast above 98%. (orig.)

Generation of attosecond soft X-ray pulses in a longitudinal space charge amplifier

International Nuclear Information System (INIS)

Dohlus, M.; Schneidmiller, E.A.; Yurkov, M.V.

2011-03-01

A longitudinal space charge amplifier (LSCA), operating in soft X-ray regime, was recently proposed. Such an amplifier consists of a few amplification cascades (focusing channel and chicane) and a short radiator undulator in the end. Broadband nature of LSCA supports generation of few-cycle pulses as well as wavelength compression. In this paper we consider an application of these properties of LSCA for generation of attosecond X-ray pulses. It is shown that a compact and cheap addition to the soft X-ray free electron laser facility FLASH would allow to generate 60 attosecond (FWHM) long X-ray pulses with the peak power at 100 MW level and a contrast above 98%. (orig.)

Towards attosecond X-ray pulses from the FEL

International Nuclear Information System (INIS)

Zholents, Alexander A.; Fawley, William M.

2004-01-01

The ability to study ultrafast phenomena has been recently advanced by the demonstrated production and measurement of a single, 650-attosecond (10 18 sec), VUV x-ray pulse[1] and, latter, a 250-attosecond pulse[2]. The next frontier is a production of the x-ray pulses with shorter wavelengths and in a broader spectral range. Several techniques for a generation of an isolated, attosecond duration, short-wavelength x-ray pulse based upon the ponderomotive laser acceleration [3], SASE and harmonic cascade FELs ([4] - [6]) had been already proposed. In this paper we briefly review a technique proposed in [5] and present some new results

Control of the launch of attosecond pulses

International Nuclear Information System (INIS)

Cao Wei; Lu Peixiang; Lan Pengfei; Wang Xinlin; Li Yuhua

2007-01-01

We propose an approach to steer the launch of attosecond (as) pulses with a high precision. We numerically demonstrate that by adding a weak second-harmonic (SH) field to the fundamental beam the ionization and recollision process of the electron will be perturbed, which can induce a variation of the emission time of high harmonics. Through modifying the relative intensity of the SH and fundamental fields, the launch of as pulses can be manipulated with a resolution less than 40 as. This will show significant potential for ultrafast optics

Coherent dynamics of plasma mirrors

Energy Technology Data Exchange (ETDEWEB)

Thaury, C; George, H; Quere, F; Monot, P; Martin, Ph [CEA, DSM, IRAMIS, Serv Photons Atomes and Mol, F-91191 Gif Sur Yvette, (France); Loch, R [Univ Twente, Laser Phys and Nonlinear Opt Grp, Fac Sci and Technol, MESA Inst Nanotechnol, NL-7500 AE Enschede, (Netherlands); Geindre, J P [Ecole Polytech, Lab Pour Utilisat Lasers Intenses, CNRS, F-91128 Palaiseau, (France)

2008-07-01

Coherent ultrashort X-ray pulses provide new ways to probe matter and its ultrafast dynamics. One of the promising paths to generate these pulses consists of using a nonlinear interaction with a system to strongly and periodically distort the waveform of intense laser fields, and thus produce high-order harmonics. Such distortions have so far been induced by using the nonlinear polarizability of atoms, leading to the production of atto-second light bursts, short enough to study the dynamics of electrons in matter. Shorter and more intense atto-second pulses, together with higher harmonic orders, are expected by reflecting ultra intense laser pulses on a plasma mirror - a dense (approximate to 10{sup 23} electrons cm{sup -3}) plasma with a steep interface. However, short-wavelength-light sources produced by such plasmas are known to generally be incoherent. In contrast, we demonstrate that like in usual low-intensity reflection, the coherence of the light wave is preserved during harmonic generation on plasma mirrors. We then exploit this coherence for interferometric measurements and thus carry out a first study of the laser-driven coherent dynamics of the plasma electrons. (authors)

Photoelectron spectrometer for attosecond spectroscopy of liquids and gases

Energy Technology Data Exchange (ETDEWEB)

Jordan, I.; Huppert, M.; Wörner, H. J., E-mail: hwoerner@ethz.ch [Laboratory of Physical Chemistry, ETH Zurich, Vladimir-Prelog-Weg 2, 8093 Zurich (Switzerland); Brown, M. A. [Laboratory for Surface Science and Technology, Department of Materials, ETH Zurich, Vladimir-Prelog-Weg 5, 8093 Zurich (Switzerland); Bokhoven, J. A. van [Institute for Chemical and Bioengineering, ETH Zurich, Vladimir-Prelog-Weg 1, 8093 Zurich (Switzerland); Laboratory for Catalysis and Sustainable Chemistry, Paul Scherrer Institute, 5232 Villigen (Switzerland)

2015-12-15

A new apparatus for attosecond time-resolved photoelectron spectroscopy of liquids and gases is described. It combines a liquid microjet source with a magnetic-bottle photoelectron spectrometer and an actively stabilized attosecond beamline. The photoelectron spectrometer permits venting and pumping of the interaction chamber without affecting the low pressure in the flight tube. This pressure separation has been realized through a sliding skimmer plate, which effectively seals the flight tube in its closed position and functions as a differential pumping stage in its open position. A high-harmonic photon spectrometer, attached to the photoelectron spectrometer, exit port is used to acquire photon spectra for calibration purposes. Attosecond pulse trains have been used to record photoelectron spectra of noble gases, water in the gas and liquid states as well as solvated species. RABBIT scans demonstrate the attosecond resolution of this setup.

Photoelectron spectrometer for attosecond spectroscopy of liquids and gases

International Nuclear Information System (INIS)

Jordan, I.; Huppert, M.; Wörner, H. J.; Brown, M. A.; Bokhoven, J. A. van

2015-01-01

A new apparatus for attosecond time-resolved photoelectron spectroscopy of liquids and gases is described. It combines a liquid microjet source with a magnetic-bottle photoelectron spectrometer and an actively stabilized attosecond beamline. The photoelectron spectrometer permits venting and pumping of the interaction chamber without affecting the low pressure in the flight tube. This pressure separation has been realized through a sliding skimmer plate, which effectively seals the flight tube in its closed position and functions as a differential pumping stage in its open position. A high-harmonic photon spectrometer, attached to the photoelectron spectrometer, exit port is used to acquire photon spectra for calibration purposes. Attosecond pulse trains have been used to record photoelectron spectra of noble gases, water in the gas and liquid states as well as solvated species. RABBIT scans demonstrate the attosecond resolution of this setup

Photoelectron spectrometer for attosecond spectroscopy of liquids and gases

Science.gov (United States)

Jordan, I.; Huppert, M.; Brown, M. A.; van Bokhoven, J. A.; Wörner, H. J.

2015-12-01

A new apparatus for attosecond time-resolved photoelectron spectroscopy of liquids and gases is described. It combines a liquid microjet source with a magnetic-bottle photoelectron spectrometer and an actively stabilized attosecond beamline. The photoelectron spectrometer permits venting and pumping of the interaction chamber without affecting the low pressure in the flight tube. This pressure separation has been realized through a sliding skimmer plate, which effectively seals the flight tube in its closed position and functions as a differential pumping stage in its open position. A high-harmonic photon spectrometer, attached to the photoelectron spectrometer, exit port is used to acquire photon spectra for calibration purposes. Attosecond pulse trains have been used to record photoelectron spectra of noble gases, water in the gas and liquid states as well as solvated species. RABBIT scans demonstrate the attosecond resolution of this setup.

Dynamics of an excess hole in the 1-methyl-1-butyl-pyrrolidinium dicyanamide ionic-liquid

Science.gov (United States)

Wu, Fei; Xu, Changhui; Margulis, Claudio J.

2018-05-01

In a set of recent publications [C. J. Margulis et al., J. Am. Chem. Soc. 133, 20186 (2011); C. H. Xu et al., J. Am. Chem. Soc. 135, 17528 (2013); C. H. Xu and C. J. Margulis, J. Phys. Chem. B 119, 532 (2015); and K. B. Dhungana et al., J. Phys. Chem. B 121, 8809 (2017)], we explored for selected ionic liquids the early stages of excess charge localization and reactivity relevant both to electrochemical and radiation chemistry processes. In particular, Xu and Margulis [J. Phys. Chem. B 119, 532 (2015)] explored the dynamics of an excess electron in 1-methyl-1-butyl-pyrrolidinium dicyanamide. When electrons are produced from an ionic liquid, the more elusive hole species are also generated. Depending on the nature of cations and anions and the relative alignment of their electronic states in the condensed phase, the very early hole species can nominally be neutral radicals—if the electron is generated from anions—or doubly charged radical cations if their origin is from cations. However, in reality early excess charge localization is more complex and often involves more than one ion. The dynamics and the transient spectroscopy of the hole are the main objects of this study. We find that in the case of 1-methyl-1-butyl-pyrrolidinium dicyanamide, it is the anions that can most easily lose an electron becoming radical species, and that hole localization is mostly on anionic nitrogen. We also find that the driving force for localization of an excess hole appears to be smaller than that for an excess electron in 1-methyl-1-butyl-pyrrolidinium dicyanamide. The early transient hole species can absorb light in the visible, ultraviolet, and near infrared regions, and we are able to identify the type of states being connected by these transitions.

Black hole dynamics at large D

CERN Multimedia

CERN. Geneva

2016-01-01

We demonstrate that the classical dynamics of black holes can be reformulated as a dynamical problem of a codimension one membrane moving in flat space. This membrane - roughly the black hole event horizon - carries a conserved charge current and stress tensor which source radiation. This `membrane paradigm' may be viewed as a simplification of the equations of general relativity at large D, and suggests the possibility of using 1/D as a useful expansion parameter in the analysis of complicated four dimensional solutions of general relativity, for instance the collision between two black holes.

High-throughput beamline for attosecond pulses based on toroidal mirrors with microfocusing capabilities

International Nuclear Information System (INIS)

Frassetto, F.; Poletto, L.; Trabattoni, A.; Anumula, S.; Sansone, G.; Calegari, F.; Nisoli, M.

2014-01-01

We have developed a novel attosecond beamline designed for attosecond-pump/attosecond probe experiments. Microfocusing of the Extreme-ultraviolet (XUV) radiation is obtained by using a coma-compensated optical configuration based on the use of three toroidal mirrors controlled by a genetic algorithm. Trains of attosecond pulses are generated with a measured peak intensity of about 3 × 10 11 W/cm 2

High-throughput beamline for attosecond pulses based on toroidal mirrors with microfocusing capabilities

Energy Technology Data Exchange (ETDEWEB)

Frassetto, F.; Poletto, L., E-mail: poletto@dei.unipd.it [National Research Council, Institute of Photonics and Nanotechnologies, via Trasea 7, 35131 Padova (Italy); Trabattoni, A.; Anumula, S.; Sansone, G. [Department of Physics, Politecnico di Milano, Piazza L. Da Vinci 32, 20133 Milano (Italy); Calegari, F. [National Research Council, Institute of Photonics and Nanotechnologies, Piazza L. da Vinci 32, 20133 Milano (Italy); Nisoli, M. [Department of Physics, Politecnico di Milano, Piazza L. Da Vinci 32, 20133 Milano (Italy); National Research Council, Institute of Photonics and Nanotechnologies, Piazza L. da Vinci 32, 20133 Milano (Italy)

2014-10-15

We have developed a novel attosecond beamline designed for attosecond-pump/attosecond probe experiments. Microfocusing of the Extreme-ultraviolet (XUV) radiation is obtained by using a coma-compensated optical configuration based on the use of three toroidal mirrors controlled by a genetic algorithm. Trains of attosecond pulses are generated with a measured peak intensity of about 3 × 10{sup 11} W/cm{sup 2}.

Self-probing spectroscopy of XUV photo-ionization dynamics in atoms subjected to a strong-field environment.

Science.gov (United States)

Azoury, Doron; Krüger, Michael; Orenstein, Gal; Larsson, Henrik R; Bauch, Sebastian; Bruner, Barry D; Dudovich, Nirit

2017-11-13

Single-photon ionization is one of the most fundamental light matter interactions in nature, serving as a universal probe of the quantum state of matter. By probing the emitted electron, one can decode the full dynamics of the interaction. When photo-ionization is evolving in the presence of a strong laser field, the fundamental properties of the mechanism can be signicantly altered. Here we demonstrate how the liberated electron can perform a self-probing measurement of such interaction with attosecond precision. Extreme ultraviolet attosecond pulses initiate an electron wavepacket by photo-ionization, a strong infrared field controls its motion, and finally electron-ion collision maps it into re-emission of attosecond radiation bursts. Our measurements resolve the internal clock provided by the self-probing mechanism, obtaining a direct insight into the build-up of photo-ionization in the presence of the strong laser field.

Large-scale laser-microwave synchronization for attosecond photon science facilities

Energy Technology Data Exchange (ETDEWEB)

Shafak, Kemal

2017-04-15

Low-noise transfer of time and frequency standards over large distances provides high temporal resolution for ambitious scientific explorations such as sensitive imaging of astronomical objects using multi-telescope arrays, comparison of distant optical clocks or gravitational-wave detection using large laser interferometers. In particular, rapidly expanding photon science facilities such as X-ray free-electron lasers (FELs) and attoscience centers have the most challenging synchronization requirements of sub-fs timing precision to generate ultrashort X-ray pulses for the benefit of creating super-microscopes with sub-atomic spatiotemporal resolution. The critical task in these facilities is to synchronize various pulsed lasers and microwave sources across multi-kilometer distances as required for seeded FELs and attosecond pump-probe experiments. So far, there has been no timing distribution system meeting this strict requirement. Therefore, insufficient temporal precision provided by the current synchronization systems hinders the development of attosecond hard X-ray photon science facilities. The aim of this thesis is to devise a timing distribution system satisfying the most challenging synchronization requirements in science mandated by the next-generation photon science facilities. Using the pulsed-optical timing distribution approach, attosecond timing precision is realized by thoroughly investigating and eliminating the remaining noise sources in the synchronization system. First, optical and microwave timing detection schemes are further developed to support long-term stable, attosecond-precision measurements. Second, the feasibility of the master laser to support a kilometer-scale timing network with attosecond precision is examined by experimentally characterizing its free-running timing jitter and improving its long-term frequency stability with a sophisticated environmental insulation. Third, nonlinear pulse propagation inside optical fibers is studied

Large-scale laser-microwave synchronization for attosecond photon science facilities

International Nuclear Information System (INIS)

Shafak, Kemal

2017-04-01

Low-noise transfer of time and frequency standards over large distances provides high temporal resolution for ambitious scientific explorations such as sensitive imaging of astronomical objects using multi-telescope arrays, comparison of distant optical clocks or gravitational-wave detection using large laser interferometers. In particular, rapidly expanding photon science facilities such as X-ray free-electron lasers (FELs) and attoscience centers have the most challenging synchronization requirements of sub-fs timing precision to generate ultrashort X-ray pulses for the benefit of creating super-microscopes with sub-atomic spatiotemporal resolution. The critical task in these facilities is to synchronize various pulsed lasers and microwave sources across multi-kilometer distances as required for seeded FELs and attosecond pump-probe experiments. So far, there has been no timing distribution system meeting this strict requirement. Therefore, insufficient temporal precision provided by the current synchronization systems hinders the development of attosecond hard X-ray photon science facilities. The aim of this thesis is to devise a timing distribution system satisfying the most challenging synchronization requirements in science mandated by the next-generation photon science facilities. Using the pulsed-optical timing distribution approach, attosecond timing precision is realized by thoroughly investigating and eliminating the remaining noise sources in the synchronization system. First, optical and microwave timing detection schemes are further developed to support long-term stable, attosecond-precision measurements. Second, the feasibility of the master laser to support a kilometer-scale timing network with attosecond precision is examined by experimentally characterizing its free-running timing jitter and improving its long-term frequency stability with a sophisticated environmental insulation. Third, nonlinear pulse propagation inside optical fibers is studied

Attosecond control of dissociative ionization of O{sub 2} molecules

Energy Technology Data Exchange (ETDEWEB)

Siu, W.; Kelkensberg, F.; Gademann, G. [FOM Institute AMOLF, Science Park 104, NL-1098 XG Amsterdam (Netherlands); Rouzee, A.; Vrakking, M. J. J. [FOM Institute AMOLF, Science Park 104, NL-1098 XG Amsterdam (Netherlands); Max-Born-Institut, Max-Born Strasse 2A, D-12489 Berlin (Germany); Johnsson, P. [FOM Institute AMOLF, Science Park 104, NL-1098 XG Amsterdam (Netherlands); Department of Physics, Lund University, Post Office Box 118, SE-221 00 Lund (Sweden); Dowek, D. [Laboratoire des Collisions Atomiques et Moleculaires (UMR Universite Paris-Sud et CNRS, 8625), Batiment 351, Universite Paris-Sud, F-91405 Orsay Cedex (France); Lucchini, M.; Calegari, F. [Department of Physics, Politecnico di Milano, Istituto di Fotonica e Nanotecnologie CNR-IFN, Piazza Leonardo da Vinci 32, 20133 Milano (Italy); De Giovannini, U.; Rubio, A. [Nano-bio Spectroscopy Group, ETSF Scientific Development Centre, Universidad del Pais Vasco, Avenida Tolosa 72, E-20018 San Sebastian (Spain); Lucchese, R. R. [Department of Chemistry, Texas A and M University, Post Office Box 30012, College Station, Texas 77842-3012 (United States); Kono, H. [Department of Chemistry, Graduate School of Science, Tohoku University, Sendai 980-8578 (Japan); Lepine, F. [Universite Lyon 1/CNRS/LASIM, UMR 5579, 43 Boulevard Du 11 Novembre 1918, F-69622 Villeurbane (France)

2011-12-15

We demonstrate that dissociative ionization of O{sub 2} can be controlled by the relative delay between an attosecond pulse train (APT) and a copropagating infrared (IR) field. Our experiments reveal a dependence of both the branching ratios between a range of electronic states and the fragment angular distributions on the extreme ultraviolet (XUV) to IR time delay. The observations go beyond adiabatic propagation of dissociative wave packets on IR-induced quasistatic potential energy curves and are understood in terms of an IR-induced coupling between electronic states in the molecular ion.

Density matrix-based time-dependent configuration interaction approach to ultrafast spin-flip dynamics

Science.gov (United States)

Wang, Huihui; Bokarev, Sergey I.; Aziz, Saadullah G.; Kühn, Oliver

2017-08-01

Recent developments in attosecond spectroscopy yield access to the correlated motion of electrons on their intrinsic timescales. Spin-flip dynamics is usually considered in the context of valence electronic states, where spin-orbit coupling is weak and processes related to the electron spin are usually driven by nuclear motion. However, for core-excited states, where the core-hole has a nonzero angular momentum, spin-orbit coupling is strong enough to drive spin-flips on a much shorter timescale. Using density matrix-based time-dependent restricted active space configuration interaction including spin-orbit coupling, we address an unprecedentedly short spin-crossover for the example of L-edge (2p→3d) excited states of a prototypical Fe(II) complex. This process occurs on a timescale, which is faster than that of Auger decay (∼4 fs) treated here explicitly. Modest variations of carrier frequency and pulse duration can lead to substantial changes in the spin-state yield, suggesting its control by soft X-ray light.

Generation of attosecond soft x-ray pulses in a longitudinal space charge amplifier

Directory of Open Access Journals (Sweden)

M. Dohlus

2011-09-01

Full Text Available A longitudinal space charge amplifier (LSCA, operating in soft x-ray regime, was recently proposed. Such an amplifier consists of a few amplification cascades (focusing channel and chicane and a short radiator undulator in the end. The broadband nature of LSCA supports generation of few-cycle pulses as well as wavelength compression. In this paper we consider an application of these properties of LSCA for generation of attosecond x-ray pulses. It is shown that a compact and cheap addition to the soft x-ray free-electron laser facility FLASH would allow one to generate 60 attosecond (FWHM long x-ray pulses with the peak power at the 100 MW level and a contrast above 98%.

Black hole dynamics in Einstein-Maxwell-dilaton theory

Science.gov (United States)

Hirschmann, Eric W.; Lehner, Luis; Liebling, Steven L.; Palenzuela, Carlos

2018-03-01

We consider the properties and dynamics of black holes within a family of alternative theories of gravity, namely Einstein-Maxwell-dilaton theory. We analyze the dynamical evolution of individual black holes as well as the merger of binary black hole systems. We do this for a wide range of parameter values for the family of Einstein-Maxwell-dilaton theories, investigating, in the process, the stability of these black holes. We examine radiative degrees of freedom, explore the impact of the scalar field on the dynamics of merger, and compare with other scalar-tensor theories. We argue that the dilaton can largely be discounted in understanding merging binary systems and that the end states essentially interpolate between charged and uncharged, rotating black holes. For the relatively small charge values considered here, we conclude that these black hole systems will be difficult to distinguish from their analogs within General Relativity.

Carrier-envelope phase-stabilized attosecond pulses from asymmetric molecules

International Nuclear Information System (INIS)

Lan Pengfei; Lu Peixiang; Cao Wei; Li Yuhua; Wang Xinlin

2007-01-01

High-order harmonic generation from asymmetric molecules is investigated, and the concept of phase-stabilized infrared ultrashort laser pulses is extended to the extreme ultraviolet regime. It is shown that the ionization symmetry in consecutive half optical cycles is broken for asymmetric molecules, and both even and odd harmonics with comparable intensity are produced. In the time domain, only one attosecond pulse is generated in each cycle of the driving field, and the carrier-envelope phases of the attosecond pulses are equal. Consequently, a clean attosecond pulse train with the same carrier-envelope phase from pulse to pulse is obtained in the extreme ultraviolet regime

Subfemtosecond electron dynamics of H{sub 2} in strong fields or the quest for the molecular clock

Energy Technology Data Exchange (ETDEWEB)

Staudte, A.

2005-07-01

In this work we have studied experimentally and theoretically hydrogen and deuterium molecules in strong laser fields. We wanted to demonstrate that control of dynamical processes on the time scale below a single laser cycle (2.7 fs) can be achieved even without using attosecond pulses just by employing the advanced experimental technique COLTRIMS. In order to do this, we have pursued two goals: 1. To examine, whether laser steered electron wavepackets can be used for laser induced electron diffraction (LIED) on molecules. 2. To demonstrate, that the double ionization of H{sub 2} can be followed with sub laser cycle temporal resolution (the molecular clock). Laser induced electron diffraction needs linearly polarized light since its mechanism relies on rescattering of the ionized electron in the molecular potential. With rescattering occurring within a few hundred attoseconds, LIED is really a process of attosecond physics. In principle, two extreme scattering geometries are possible for a homonuclear diatomic molecule like H{sub 2}: the perpendicular geometry, which corresponds to the classical double slit experiment where the electron microbunch is steered transversely to the molecular axis, and the tangential geometry with the electron moving parallel to the molecular axis. Experimental restrictions prevented us to investigate the perpendicular geometry. The molecular clock, on the other hand, employs circularly polarized light to map the absolute phase of the laser electric field onto the spatial direction of the electron momentum. Thereby, a full laser cycle is mapped onto 360 in momentum space. Thus, different electron ejection angles in the laboratory frame correspond to different ejection times. Together with the correlated kinetic energy release of the Coulomb exploding molecules an unambiguous clock running from 0-8 fs with a few 100 as resolution can be envisioned. In direct relation to this experiment, we studied the influence of the long range

Macroscopic effects in attosecond pulse generation

International Nuclear Information System (INIS)

Ruchon, T; Varju, K; Mansten, E; Swoboda, M; L'Huillier, A; Hauri, C P; Lopez-Martens, R

2008-01-01

We examine how the generation and propagation of high-order harmonics in a partly ionized gas medium affect their strength and synchronization. The temporal properties of the resulting attosecond pulses generated in long gas targets can be significantly influenced by macroscopic effects, in particular by the intensity in the medium and the degree of ionization which control the dispersion. Under some conditions, the use of gas targets longer than the absorption length can lead to the generation of compressed attosecond pulses. We show these macroscopic effects experimentally, using a 6 mm-long argon-filled gas cell as the generating medium

Macroscopic effects in attosecond pulse generation

Energy Technology Data Exchange (ETDEWEB)

Ruchon, T; Varju, K; Mansten, E; Swoboda, M; L' Huillier, A [Department of Physics, Lund University, PO Box 118, SE-221 00 Lund (Sweden); Hauri, C P; Lopez-Martens, R [Laboratoire d' Optique Appliquee, Ecole Nationale Superieure des Techniques Avancees (ENSTA)-Ecole Polytechnique CNRS UMR 7639, 91761 Palaiseau (France)], E-mail: anne.lhuillier@fysik.lth.se

2008-02-15

We examine how the generation and propagation of high-order harmonics in a partly ionized gas medium affect their strength and synchronization. The temporal properties of the resulting attosecond pulses generated in long gas targets can be significantly influenced by macroscopic effects, in particular by the intensity in the medium and the degree of ionization which control the dispersion. Under some conditions, the use of gas targets longer than the absorption length can lead to the generation of compressed attosecond pulses. We show these macroscopic effects experimentally, using a 6 mm-long argon-filled gas cell as the generating medium.

Black Hole Dynamic Potentials Koustubh Ajit Kabe

Indian Academy of Sciences (India)

Abstract. In the following paper, certain black hole dynamic potentials have been developed definitively on the lines of classical thermodynam- ics. These potentials have been refined in view of the small differences in the equations of the laws of black hole dynamics as given by Bekenstein and those of thermodynamics.

Reconstruction of Attosecond Pulse Trains Using an Adiabatic Phase Expansion

International Nuclear Information System (INIS)

Varju, K.; Gustafsson, E.; Johnsson, P.; Mauritsson, J.; L'Huillier, A.; Mairesse, Y.; Agostini, P.; Breger, P.; Carre, B.; Merdji, H.; Monchicourt, P.; Salieres, P.; Frasinski, L.J.

2005-01-01

We propose a new method to reconstruct the electric field of attosecond pulse trains. The phase of the high-order harmonic emission electric field is Taylor expanded around the maximum of the laser pulse envelope in the time domain and around the central harmonic in the frequency domain. Experimental measurements allow us to determine the coefficients of this expansion and to characterize the radiation with attosecond accuracy over a femtosecond time scale. The method gives access to pulse-to-pulse variations along the train, including the timing, the chirp, and the attosecond carrier envelope phase

Influence of heat treatment on hole transfer dynamics in core-shell quantum dot/organic hole conductor hybrid films

Science.gov (United States)

Sun, Mingye; Zheng, Youjin; Zhang, Lei; Zhao, Liping; Zhang, Bing

2017-08-01

The influence of heat treatment on hole transfer (HT) processes from the CdSe/ZnS and CdSe/CdS/ZnS quantum dots (QDs) to 4,4‧,4″-Tris(carbazol-9-yl)-triphenylamine (TCTA) in QD/TCTA hybrid films has been researched with time-resolved photoluminescence (PL) spectroscopy. The PL dynamic results demonstrated a heat-treatment-temperature-dependent HT process from the core-shell CdSe QDs to TCTA. The HT rates and efficiencies can be effectively increased due to reduced distance between core-shell CdSe QDs and TCTA after heat treatment. The CdS shell exhibited a more obvious effect on HT from the core-shell CdSe QDs to TCTA than on electron transfer to TiO2, due to higher barrier for holes to tunnel through CdS shell and larger effective mass of holes in CdS than electrons. These results indicate that heat treatment would be an effective means to further optimize solid-state QD sensitized solar cells and rational design of CdS shell is significant.

Soft hair of dynamical black hole and Hawking radiation

Science.gov (United States)

Chu, Chong-Sun; Koyama, Yoji

2018-04-01

Soft hair of black hole has been proposed recently to play an important role in the resolution of the black hole information paradox. Recent work has emphasized that the soft modes cannot affect the black hole S-matrix due to Weinberg soft theorems. However as soft hair is generated by supertranslation of geometry which involves an angular dependent shift of time, it must have non-trivial quantum effects. We consider supertranslation of the Vaidya black hole and construct a non-spherical symmetric dynamical spacetime with soft hair. We show that this spacetime admits a trapping horizon and is a dynamical black hole. We find that Hawking radiation is emitted from the trapping horizon of the dynamical black hole. The Hawking radiation has a spectrum which depends on the soft hair of the black hole and this is consistent with the factorization property of the black hole S-matrix.

Energy of ground state of laminar electron-hole liquid

International Nuclear Information System (INIS)

Andryushin, E.A.

1976-01-01

The problem of a possible existence of metal electron-hole liquid in semiconductors is considered. The calculation has been carried out for the following model: two parallel planes are separated with the distance on one of the planes electrons moving, on the other holes doing. Transitions between the planes are forbidden. The density of particles for both planes is the same. The energy of the ground state and correlation functions for such electron-and hole system are calculated. It is shown that the state of a metal liquid is more advantageous against the exciton gas. For the mass ratio of electrons and holes, msub(e)/msub(h) → 0 a smooth rearrangement of the system into a state with ordered heavy particles is observed

Dynamics of test black holes

International Nuclear Information System (INIS)

Epikhin, E.N.

1981-01-01

A concept of a test object is introduced. This definition includes also small black holes. Reduced approximation of testing permits to unambiguously introduce a concept of background space-time. Dynamic values for test objects are introduced by means of the Noether theorem which gave the possibility to covariantly generalize pseudotensor of the Papapetru energy-momentum for the case of curved background space-time. Additional use of radiation approximation and the accountancy of the zero and first momenta of dynamic values lead to the conclusion that motion of the test object (including small black holes) is subordinated to the Matthiessen-Papapetru equations. The above results are testified to the accountancy of a proper gravitational field of the test object in integrated dynamic values [ru

Dynamical 3-Space: Black Holes in an Expanding Universe

Directory of Open Access Journals (Sweden)

Rothall D. P.

2013-10-01

Full Text Available Black holes are usually studied without including effects of the expanding universe. However in some recent studies black holes have been embedded in an expanding universe, in order to determine the interplay, if any, of these two dynamical processes. Dynamical 3-space theory contains time independent solutions for black holes, which are spatial in-flows, and separately the time dependent Hubble expansion. This theory has explained numerous puzzles in observational astrophysics and contains 3 constants; G, - which from experimental data turns out to be the fine structure constant, and - which is a small but nonzero distance, possibly a Planck-type length. The Hubble expansion in the dynamical 3-space theory cannot be “switched o”, forcing the study, first, of isolated black holes coexisting with the expanding universe. It is shown that a time dependent black hole and expanding universe solution exists. The nature and implications of these solutions are discussed as they evolve over time. A dynamical network of black holes and induced linking cosmic filaments forming bubble structures is discussed, as a consequence of dynamical 3-space undergoing a dynamical breakdown of homogeneity and isotropy, even in the absence of baryonic matter.

Broadband Cooling Spectra of Hot Electrons and Holes in PbSe Quantum Dots

NARCIS (Netherlands)

Spoor, F.C.M.; Tomić, Stanko; Houtepen, A.J.; Siebbeles, L.D.A.

2017-01-01

Understanding cooling of hot charge carriers in semiconductor quantum dots (QDs) is of fundamental interest and useful to enhance the performance of QDs in photovoltaics. We study electron and hole cooling dynamics in PbSe QDs up to high energies where carrier multiplication occurs. We

Thermoelectric performance of electron and hole doped PtSb2

KAUST Repository

Saeed, Yasir; Singh, Nirpendra; Parker, D.; Schwingenschlö gl, Udo

2013-01-01

We investigate the thermoelectric properties of electron and hole doped PtSb2. Our results show that for doping of 0.04 holes per unit cell ( 1.5×1020 cm−3 ) PtSb2 shows a high Seebeck coefficient at room temperature, which can also be achieved at other temperatures by controlling the carrier concentration (both electron and hole). The electrical conductivity becomes temperature independent when the doping exceeds some 0.2 electrons/holes per unit cell. The figure of merit at 800 K in electron and hole doped PtSb2 is comparatively low at 0.13 and 0.21, respectively, but may increase significantly with As alloying due to the likely opening of a band gap and reduction of the lattice thermal conductivity.

Thermoelectric performance of electron and hole doped PtSb2

KAUST Repository

Saeed, Yasir

2013-04-30

We investigate the thermoelectric properties of electron and hole doped PtSb2. Our results show that for doping of 0.04 holes per unit cell ( 1.5×1020 cm−3 ) PtSb2 shows a high Seebeck coefficient at room temperature, which can also be achieved at other temperatures by controlling the carrier concentration (both electron and hole). The electrical conductivity becomes temperature independent when the doping exceeds some 0.2 electrons/holes per unit cell. The figure of merit at 800 K in electron and hole doped PtSb2 is comparatively low at 0.13 and 0.21, respectively, but may increase significantly with As alloying due to the likely opening of a band gap and reduction of the lattice thermal conductivity.

Analysis and simulation of BGK electron holes

Directory of Open Access Journals (Sweden)

L. Muschietti

1999-01-01

Full Text Available Recent observations from satellites crossing regions of magnetic-field-aligned electron streams reveal solitary potential structures that move at speeds much greater than the ion acoustic/thermal velocity. The structures appear as positive potential pulses rapidly drifting along the magnetic field, and are electrostatic in their rest frame. We interpret them as BGK electron holes supported by a drifting population of trapped electrons. Using Laplace transforms, we analyse the behavior of one phase-space electron hole. The resulting potential shapes and electron distribution functions are self-consistent and compatible with the field and particle data associated with the observed pulses. In particular, the spatial width increases with increasing amplitude. The stability of the analytic solution is tested by means of a two-dimensional particle-in-cell simulation code with open boundaries. We consider a strongly magnetized parameter regime in which the bounce frequency of the trapped electrons is much less than their gyrofrequency. Our investigation includes the influence of the ions, which in the frame of the hole appear as an incident beam, and impinge on the BGK potential with considerable energy. The nonlinear structure is remarkably resilient

Electron and hole transport in ambipolar, thin film pentacene transistors

International Nuclear Information System (INIS)

Saudari, Sangameshwar R.; Kagan, Cherie R.

2015-01-01

Solution-processed, ambipolar, thin-film pentacene field-effect transistors were employed to study both electron and hole transport simultaneously in a single, organic solid-state device. Electron and hole mobilities were extracted from the respective unipolar saturation regimes and show thermally activated behavior and gate voltage dependence. We fit the gate voltage dependent saturation mobility to a power law to extract the characteristic Meyer-Neldel (MN) energy, a measure of the width of the exponential distribution of localized states extending into the energy gap of the organic semiconductor. The MN energy is ∼78 and ∼28 meV for electrons and holes, respectively, which reflects a greater density of localized tail states for electrons than holes. This is consistent with the lower measured electron than hole mobility. For holes, the well-behaved linear regime allows for four-point probe measurement of the contact resistance independent mobility and separate characterization of the width of the localized density of states, yielding a consistent MN energy of 28 meV

Electron and hole transport in ambipolar, thin film pentacene transistors

Energy Technology Data Exchange (ETDEWEB)

Saudari, Sangameshwar R. [Department of Materials Science and Engineering, University of Pennsylvania, Philadelphia, Pennsylvania 19104 (United States); Kagan, Cherie R. [Department of Materials Science and Engineering, University of Pennsylvania, Philadelphia, Pennsylvania 19104 (United States); Department of Electrical and Systems Engineering, University of Pennsylvania, Philadelphia, Pennsylvania 19104 (United States); Department of Chemistry, University of Pennsylvania, Philadelphia, Pennsylvania 19104 (United States)

2015-01-21

Solution-processed, ambipolar, thin-film pentacene field-effect transistors were employed to study both electron and hole transport simultaneously in a single, organic solid-state device. Electron and hole mobilities were extracted from the respective unipolar saturation regimes and show thermally activated behavior and gate voltage dependence. We fit the gate voltage dependent saturation mobility to a power law to extract the characteristic Meyer-Neldel (MN) energy, a measure of the width of the exponential distribution of localized states extending into the energy gap of the organic semiconductor. The MN energy is ∼78 and ∼28 meV for electrons and holes, respectively, which reflects a greater density of localized tail states for electrons than holes. This is consistent with the lower measured electron than hole mobility. For holes, the well-behaved linear regime allows for four-point probe measurement of the contact resistance independent mobility and separate characterization of the width of the localized density of states, yielding a consistent MN energy of 28 meV.

Magnetic holes in the dipolarized magnetotail: ion and electron anisotropies

Science.gov (United States)

Shustov, P.; Artemyev, A.; Zhang, X. J.; Yushkov, E.; Petrukovich, A. A.

2017-12-01

We conduct statistics on magnetic holes observed by THEMIS spacecraft in the near-Earth magnetotail. Groups of holes are detected after dipolarizations in the quiet, equatorial plasma sheet. Magnetic holes are characterized by significant magnetic field depressions (up to 50%) and strong electron currents ( 10-50 nA/m2), with spatial scales much smaller than the ion gyroradius. These magnetic holes are populated by hot (>10 keV), transversely anisotropic electrons supporting the pressure balance. We present statistical properties of these sub-ion scale magnetic holes and discuss possible mechanisms on the hole formation.

Dynamics of Coronal Hole Boundaries

Energy Technology Data Exchange (ETDEWEB)

Higginson, A. K.; Zurbuchen, T. H. [Department of Climate and Space Sciences and Engineering, University of Michigan, Ann Arbor, MI 48109 (United States); Antiochos, S. K.; DeVore, C. R. [Heliophysics Science Division, NASA Goddard Space Flight Center, Greenbelt, MD 20771 (United States); Wyper, P. F. [Universities Space Research Association, NASA Goddard Space Flight Center, 8800 Greenbelt Road, Greenbelt, MD 20771 (United States)

2017-03-10

Remote and in situ observations strongly imply that the slow solar wind consists of plasma from the hot, closed-field corona that is released onto open magnetic field lines. The Separatrix Web theory for the slow wind proposes that photospheric motions at the scale of supergranules are responsible for generating dynamics at coronal-hole boundaries, which result in the closed plasma release. We use three-dimensional magnetohydrodynamic simulations to determine the effect of photospheric flows on the open and closed magnetic flux of a model corona with a dipole magnetic field and an isothermal solar wind. A rotational surface motion is used to approximate photospheric supergranular driving and is applied at the boundary between the coronal hole and helmet streamer. The resulting dynamics consist primarily of prolific and efficient interchange reconnection between open and closed flux. The magnetic flux near the coronal-hole boundary experiences multiple interchange events, with some flux interchanging over 50 times in one day. Additionally, we find that the interchange reconnection occurs all along the coronal-hole boundary and even produces a lasting change in magnetic-field connectivity in regions that were not driven by the applied motions. Our results show that these dynamics should be ubiquitous in the Sun and heliosphere. We discuss the implications of our simulations for understanding the observed properties of the slow solar wind, with particular focus on the global-scale consequences of interchange reconnection.

Plasma effects in attosecond pulse generation from ultra-relativistic laser-plasma interactions

International Nuclear Information System (INIS)

Boyd, T.J.M.

2010-01-01

Complete text of publication follows. Particle-in-cell simulations were performed to examine the influence of plasma effects on high harmonic spectra from the interaction of ultra-intense p-polarized laser pulses with overdense plasma targets. Furthermore, a theoretical model is proposed to explain the radiation mechanism that leads to attosecond pulse generation in the reflected field. It is shown that plasma harmonic emission affects the spectral characteristics, causing deviations in the harmonic power decay as compared with the so-called universal 8/3-decay. These deviations may occur, in a varying degree, as a consequence of the extent to which the plasma line and its harmonics affect the emission. It is also found a strong correlation of the emitted attosecond pulses with electron density structures within the plasma, responsible to generate intense localised electrostatic fields. A theoretical model based on the excitation of Langmuir waves by the re-entrant Brunel electron beams in the plasma and their electromagnetic interaction with the laser field is proposed to explain the flatter power spectral emission - described by a weaker 5/3 index and observed in numerical simulations - than that of the universal decay.

Generation of Attosecond x-ray pulse using Coherent Relativistic Nonlinear Thomson Scattering

Energy Technology Data Exchange (ETDEWEB)

Lee, Ki Tae; Park, Seong Hee; Cha, Yong Ho; Jeong, Young Uk; Lee, Byung Cheol [Korea Atomic Energy Research Institute, Daejeon (Korea, Republic of)

2005-07-01

Relativistic plasma, a new regime in physics, has been opened due to the development in ultra-intense laser technology during the past decade. Not only the fundamental aspect of relativistic plasma are attractive but also its potential application seems to be significant especially in the area of the generation of high energy particles such as electrons, ions, positrons, and {gamma}-rays. The generation of x-ray radiation with a pulse width of sub-femtoseconds presently draws much attention because such a radiation allows one to explore ultra-fast dynamics of electrons and nucleons. Several schemes have been proposed and/or demonstrated to generate an ultra-short x-ray pulse: the relativistic Doppler shift of a backscattered laser pulse by a relativistic electron beam, the harmonic frequency upshift of a laser pulse by relativistic nonlinear motion of electrons, high order harmonic generation in the interaction of intense laser pulse with noble gases and solids The train of a few 100 attosecond pulses has been observed in the case of laser-noble gas interaction. When a low-intensity laser pulse is irradiated on an electron, the electron undergoes a harmonic oscillatory motion and generates a dipole radiation with the same frequency as the incident laser pulse, which is called Thomson scattering. As the laser intensity increases, the oscillatory motion of the electron becomes relativistically nonlinear, which leads to the generation of harmonic radiations, referred to as Relativistic Nonlinear Thomson Scattered (RNTS) radiation. The motion of the electron begins to be relativistic as the following normalized vector potential approaches to unity: a{sub 0}=8.5 x 10{sup -10} {lambda}{iota}{sup 1/2} , (1) where {lambda} is the laser wavelength in {mu}m and I the laser intensity in W/cm{sup 2} The RNTS radiation has been investigated in analytical ways. Recently, indebted to the development of the ultra-intense laser pulse, experiments on RNTS radiation have been carried

Volkov transform generalized projection algorithm for attosecond pulse characterization

International Nuclear Information System (INIS)

Keathley, P D; Bhardwaj, S; Moses, J; Laurent, G; Kärtner, F X

2016-01-01

An algorithm for characterizing attosecond extreme ultraviolet pulses that is not bandwidth-limited, requires no interpolation of the experimental data, and makes no approximations beyond the strong-field approximation is introduced. This approach fully incorporates the dipole transition matrix element into the retrieval process. Unlike attosecond retrieval methods such as phase retrieval by omega oscillation filtering (PROOF), or improved PROOF, it simultaneously retrieves both the attosecond and infrared (IR) pulses, without placing fundamental restrictions on the IR pulse duration, intensity or bandwidth. The new algorithm is validated both numerically and experimentally, and is also found to have practical advantages. These include an increased robustness to noise, and relaxed requirements for the size of the experimental dataset and the intensity of the streaking pulse. (paper)

On Electron Hole Evolution in Inhomogeneous Plasmas

Science.gov (United States)

Kuzichev, I.; Vasko, I.; Agapitov, O. V.; Mozer, F.; Artemyev, A.

2017-12-01

Electron holes (EHs) are the stationary localized non-linear structures in phase space existing due to an electron population trapped within EH electrostatic potential. EHs were found to be a common phenomenon in the Earth's magnetosphere. Such structures were observed in reconnecting current sheets, injection fronts in the outer radiation belt, and in many other situations. EHs usually propagate along magnetic field lines with velocities about electron thermal velocity, are localized on the scale of about 4-10 Debye lengths, and have the field amplitude up to hundreds of mV/m. Generation of these structures, evolution, and their role in relaxation of instabilities and energy dissipation, particle energization, supporting large-scale potential drops is under active investigation. In this report, we present the results of 1.5D gyrokinetic Vlasov-Maxwell simulations of the EH evolution in plasmas with inhomogeneous magnetic field and inhomogeneous density. Our calculations show that the inhomogeneity has a critical effect on the EH dynamics. EHs propagating into stronger (weaker) magnetic field are decelerated (accelerated) with deceleration (acceleration) rate dependent on the magnetic field gradient. During the deceleration of EH, the potential drop (weak double layer) along EH is generated. Such a potential drop might be experimentally observable even for single EH in the reconnecting current sheets. The same holds for the propagation in the plasma with inhomogeneous density. For some parameters of the system, the deceleration results in the turning of the hole. The interesting feature of this process is that the turning point depends only on the EH parameters, being independent of the average inhomogeneity scale. Our calculations also demonstrate the significant difference between "quasi-particle" concept and real evolution of the hole. Indeed, the EH is accelerated (decelerated) faster than it follows from a quasi-particle energy conservation law. It indicates

Electron holes observed in the Moon Plasma Wake

Science.gov (United States)

Hutchinson, I. H.; Malaspina, D.; Zhou, C.

2017-10-01

Electrostatic instabilities are predicted in the magnetized wake of plasma flowing past a non-magnetic absorbing object such as a probe or the moon. Analysis of the data from the Artemis satellites, now orbiting the moon at distances ten moon radii and less, shows very clear evidence of fast-moving isolated solitary potential structures causing bipolar electric field excursions as they pass the satellite's probes. These structures have all the hallmarks of electron holes: BGK solitons typically a few Debye-lengths in size, self-sustaining by a deficit of phase-space density on trapped orbits. Electron holes are now observed to be widespread in space plasmas. They have been observed in PIC simulations of the moon wake to be the non-linear consequence of the predicted electron instabilities. Simulations document hole prevalence, speed, length, and depth; and theory can explain many of these features from kinetic analysis. The solar wind wake is certainly the cause of the overwhelming majority of the holes observed by Artemis, because we observe almost all holes to be in or very near to the wake. We compare theory and simulation of the hole generation, lifetime, and transport mechanisms with observations. Work partially supported by NASA Grant NNX16AG82G.

Two types of fundamental luminescence of ionization-passive electrons and holes in optical dielectrics—Intraband-electron and interband-hole luminescence (theoretical calculation and comparison with experiment)

Science.gov (United States)

Vaisburd, D. I.; Kharitonova, S. V.

1997-11-01

A short high-power pulse of ionizing radiation creates a high concentration of nonequilibrium electrons and holes in a dielectric. They quickly lose their energy, generating a multiplicity of secondary quasiparticles: electron—hole pairs, excitons, plasmons, phonons of all types, and others. When the kinetic energy of an electron becomes less that some value EΔ≈(1.3-2)Eg it loses the ability to perform collisional ionization and electron excitations of the dielectric medium. Such an electron is said to be ionization-passive. It relaxes to the bottom of the lower conduction band by emitting phonons. Similarly a hole becomes ionization-passive when it “floats up” above some level EH and loses the ability for Auger ionization of the dielectric medium. It continues to float upward to the ceiling of the upper valance band only by emitting phonons. The concentrations of ionization-passive electrons and holes are larger by several orders of magnitude than those of the active electrons and holes and consequently make of a far larger contribution to many kinetic processes such as luminescence. Intraband and interband quantum transitions make the greatest contribution to the fundamental (independent of impurities and intrinsic defects) electromagnetic radiation of ionization-passive electrons and holes. Consequently the brightest types of purely fundamental luminescence of strongly nonequilibrium electrons and holes are intraband and interband luminescence. These forms of luminescence, discovered relatively recently, carry valuable information on the high-energy states of the electrons in the conduction band and of the holes in the valence band of a dielectric. Experimental investigations of these types of luminescence were made, mainly on alkali halide crystals which were excited by nanoseconal pulses of high-current-density electrons and by two-photon absorption of the ultraviolet harmonics of pulsed laser radiation beams of nanosecond and picosecond duration. The

Laboratory Observation of Electron Phase-Space Holes during Magnetic Reconnection

International Nuclear Information System (INIS)

Fox, W.; Porkolab, M.; Egedal, J.; Katz, N.; Le, A.

2008-01-01

We report the observation of large-amplitude, nonlinear electrostatic structures, identified as electron phase-space holes, during magnetic reconnection experiments on the Versatile Toroidal Facility at MIT. The holes are positive electric potential spikes, observed on high-bandwidth (∼2 GHz) Langmuir probes. Investigations with multiple probes establish that the holes travel at or above the electron thermal speed and have a three-dimensional, approximately spherical shape, with a scale size ∼2 mm. This corresponds to a few electron gyroradii, or many tens of Debye lengths, which is large compared to holes considered in simulations and observed by satellites, whose length scale is typically only a few Debye lengths. Finally, a statistical study over many discharges confirms that the holes appear in conjunction with the large inductive electric fields and the creation of energetic electrons associated with the magnetic energy release

Coherent electron - hole state and femtosecond cooperative emission in bulk GaAs

International Nuclear Information System (INIS)

Vasil'ev, Petr P; Kan, H; Ohta, H; Hiruma, T

2002-01-01

The conditions for obtaining a collective coherent electron - hole state in semiconductors are discussed. The results of the experimental study of the regime of cooperative recombination of high-density electrons and holes (more than 3 x 10 18 cm -3 ) in bulk GaAs at room temperature are presented. It is shown that the collective pairing of electrons and holes and their condensation cause the formation of a short-living coherent electron - hole BCS-like state, which exhibits radiative recombination in the form of high-power femtosecond optical pulses. It is experimentally demonstrated that almost all of the electrons and holes available are condensed at the very bottoms of the bands and are at the cooperative state. The average lifetime of this state is measured to be of about 300 fs. The dependences of the order parameter (the energy gap of the spectrum of electrons and holes) and the Fermi energy of the coherent BCS state on the electron - hole concentration are obtained. (special issue devoted to the 80th anniversary of academician n g basov's birth)

Correlation induced electron-hole asymmetry in quasi- two-dimensional iridates.

Science.gov (United States)

Pärschke, Ekaterina M; Wohlfeld, Krzysztof; Foyevtsova, Kateryna; van den Brink, Jeroen

2017-09-25

The resemblance of crystallographic and magnetic structures of the quasi-two-dimensional iridates Ba 2 IrO 4 and Sr 2 IrO 4 to La 2 CuO 4 points at an analogy to cuprate high-Tc superconductors, even if spin-orbit coupling is very strong in iridates. Here we examine this analogy for the motion of a charge (hole or electron) added to the antiferromagnetic ground state. We show that correlation effects render the hole and electron case in iridates very different. An added electron forms a spin polaron, similar to the cuprates, but the situation of a removed electron is far more complex. Many-body 5d 4 configurations form which can be singlet and triplet states of total angular momentum that strongly affect the hole motion. This not only has ramifications for the interpretation of (inverse-)photoemission experiments but also demonstrates that correlation physics renders electron- and hole-doped iridates fundamentally different.Some iridate compounds such as Sr 2 IrO 4 have electronic and atomic structures similar to quasi-2D copper oxides, raising the prospect of high temperature superconductivity. Here, the authors show that there is significant electron-hole asymmetry in iridates, contrary to expectations from the cuprates.

Nonadiabatic electron wavepacket dynamics behind molecular autoionization

Science.gov (United States)

Matsuoka, Takahide; Takatsuka, Kazuo

2018-01-01

A theoretical method for real-time dynamics of nonadiabatic reorganization of electronic configurations in molecules is developed, with dual aim that the intramolecular electron dynamics can be probed by means of direct and/or indirect photoionizations and that the physical origins behind photoionization signals attained in the time domain can be identified in terms of the language of time-dependent quantum chemistry. In doing so, we first formulate and implement a new computational scheme for nonadiabatic electron dynamics associated with molecular ionization, which well fits in the general theory of nonadiabatic electron dynamics. In this method, the total nonadiabatic electron wavepackets are propagated in time directly with complex natural orbitals without referring to Hartree-Fock molecular orbitals, and the amount of electron flux from a molecular region leading to ionization is evaluated in terms of the relevant complex natural orbitals. In the second half of this paper, we apply the method to electron dynamics in the elementary processes consisting of the Auger decay to demonstrate the methodological significance. An illustrative example is taken from an Auger decay starting from the 2a1 orbital hole-state of H2O+. The roles of nuclear momentum (kinetic) couplings in electronic-state mixing during the decay process are analyzed in terms of complex natural orbitals, which are schematically represented in the conventional language of molecular symmetry of the Hartree-Fock orbitals.

Interaction between Electron Holes in a Strongly Magnetized Plasma

DEFF Research Database (Denmark)

Lynov, Jens-Peter; Michelsen, Poul; Pécseli, Hans

1980-01-01

The interaction between electron holes in a strongly magnetized, plasma-filled waveguide is investigated by means of computer simulation. Two holes may or may not coalesce, depending on their amplitudes and velocities. The interaction between holes and Trivelpiece-Gould solitons is demonstrated...

Femtosecond few- to single-electron point-projection microscopy for nanoscale dynamic imaging

Directory of Open Access Journals (Sweden)

A. R. Bainbridge

2016-03-01

Full Text Available Femtosecond electron microscopy produces real-space images of matter in a series of ultrafast snapshots. Pulses of electrons self-disperse under space-charge broadening, so without compression, the ideal operation mode is a single electron per pulse. Here, we demonstrate femtosecond single-electron point projection microscopy (fs-ePPM in a laser-pump fs-e-probe configuration. The electrons have an energy of only 150 eV and take tens of picoseconds to propagate to the object under study. Nonetheless, we achieve a temporal resolution with a standard deviation of 114 fs (equivalent to a full-width at half-maximum of 269 ± 40 fs combined with a spatial resolution of 100 nm, applied to a localized region of charge at the apex of a nanoscale metal tip induced by 30 fs 800 nm laser pulses at 50 kHz. These observations demonstrate real-space imaging of reversible processes, such as tracking charge distributions, is feasible whilst maintaining femtosecond resolution. Our findings could find application as a characterization method, which, depending on geometry, could resolve tens of femtoseconds and tens of nanometres. Dynamically imaging electric and magnetic fields and charge distributions on sub-micron length scales opens new avenues of ultrafast dynamics. Furthermore, through the use of active compression, such pulses are an ideal seed for few-femtosecond to attosecond imaging applications which will access sub-optical cycle processes in nanoplasmonics.

Electronic structure and electron dynamics at Si(100)

Energy Technology Data Exchange (ETDEWEB)

Weinelt, M. [Universitaet Erlangen-Nuernberg, Lehrstuhl fuer Festkoerperphysik, Erlangen (Germany); Max-Born-Institut, Berlin (Germany); Kutschera, M.; Schmidt, R.; Orth, C.; Fauster, T. [Universitaet Erlangen-Nuernberg, Lehrstuhl fuer Festkoerperphysik, Erlangen (Germany); Rohlfing, M. [International University Bremen, School of Engineering and Science, P.O. Box 750 561, Bremen (Germany)

2005-02-01

The electronic structure and electron dynamics at a Si(100) surface is studied by two-photon photoemission (2PPE). At 90 K the occupied D{sub up} dangling-bond state is located 150{+-}50 meV below the valence-band maximum (VBM) at the center of the surface Brillouin zone anti {gamma} and exhibits an effective hole mass of (0.5{+-}0.15)m{sub e}. The unoccupied D{sub down} band has a local minimum at anti {gamma} at 650{+-}50 meV above the VBM and shows strong dispersion along the dimer rows of the c(4 x 2) reconstructed surface. At 300 K the D{sub down} position shifts comparable to the Si conduction-band minimum by 40 meV to lower energies but the dispersion of the dangling-bond states is independent of temperature. The surface band bending for p-doped silicon is less than 30 meV, while acceptor-type defects cause significant and preparation-dependent band bending on n-doped samples. 2PPE spectra of Si(100) are dominated by interband transitions between the occupied and unoccupied surface states and emission out of transiently and permanently charged surface defects. Including electron-hole interaction in many-body calculations of the quasi-particle band structure leads us to assign a dangling-bond split-off state to a quasi-one-dimensional surface exciton with a binding energy of 130 meV. Electrons resonantly excited to the unoccupied D{sub down} dangling-bond band with an excess energy of about 350 meV need 1.5{+-}0.2 ps to scatter via phonon emission to the band bottom at anti {gamma} and relax within 5 ps with an excited hole in the occupied surface band to form an exciton living for nanoseconds. (orig.)

Observation of Internal Photoinduced Electron and Hole Separation in Hybrid Two-Dimentional Perovskite Films.

Science.gov (United States)

Liu, Junxue; Leng, Jing; Wu, Kaifeng; Zhang, Jun; Jin, Shengye

2017-02-01

Two-dimensional (2D) organolead halide perovskites are promising for various optoelectronic applications. Here we report a unique spontaneous charge (electron/hole) separation property in multilayered (BA) 2 (MA) n-1 Pb n I 3n+1 (BA = CH 3 (CH 2 ) 3 NH 3 + , MA = CH 3 NH 3 + ) 2D perovskite films by studying the charge carrier dynamics using ultrafast transient absorption and photoluminescence spectroscopy. Surprisingly, the 2D perovskite films, although nominally prepared as "n = 4", are found to be mixture of multiple perovskite phases, with n = 2, 3, 4 and ≈ ∞, that naturally align in the order of n along the direction perpendicular to the substrate. Driven by the band alignment between 2D perovskites phases, we observe consecutive photoinduced electron transfer from small-n to large-n phases and hole transfer in the opposite direction on hundreds of picoseconds inside the 2D film of ∼358 nm thickness. This internal charge transfer efficiently separates electrons and holes to the upper and bottom surfaces of the films, which is a unique property beneficial for applications in photovoltaics and other optoelectronics devices.

Thermodynamical and dynamical properties of charged BTZ black holes

Energy Technology Data Exchange (ETDEWEB)

Tang, Zi-Yu; Wang, Bin [Shanghai Jiao Tong University, Department of Physics and Astronomy, Center for Astronomy and Astrophysics, Shanghai (China); Zhang, Cheng-Yong [Peking University, Center for High-Energy Physics, Beijing (China); Kord Zangeneh, Mahdi [Shanghai Jiao Tong University, Department of Physics and Astronomy, Center for Astronomy and Astrophysics, Shanghai (China); Shahid Chamran University of Ahvaz, Physics Department, Faculty of Science, Ahvaz (Iran, Islamic Republic of); Research Institute for Astronomy and Astrophysics of Maragha (RIAAM)-Maragha, P. O. Box: 55134-441, Maragha (Iran, Islamic Republic of); Shiraz University, Physics Department and Biruni Observatory, College of Sciences, Shiraz (Iran, Islamic Republic of); Saavedra, Joel [Pontificia Universidad Catolica de Valparaiso, Instituto de Fisica, Valparaiso (Chile)

2017-06-15

We investigate the spacetime properties of BTZ black holes in the presence of the Maxwell field and Born-Infeld field and find rich properties in the spacetime structures when the model parameters are varied. Employing Landau-Lifshitz theory, we examine the thermodynamical phase transition in the charged BTZ black holes. We further study the dynamical perturbation in the background of the charged BTZ black holes and find different properties in the dynamics when the thermodynamical phase transition occurs. (orig.)

Mapping the spectral phase of isolated attosecond pulses by extreme-ultraviolet emission spectrum.

Science.gov (United States)

Liu, Candong; Zeng, Zhinan; Li, Ruxin; Xu, Zhizhan; Nisoli, Mauro

2015-04-20

An all-optical method is proposed for the measurement of the spectral phase of isolated attosecond pulses. The technique is based on the generation of extreme-ultraviolet (XUV) radiation in a gas by the combination of an attosecond pulse and a strong infrared (IR) pulse with controlled electric field. By using a full quantum simulation, we demonstrate that, for particular temporal delays between the two pulses, the IR field can drive back to the parent ions the photoelectrons generated by the attosecond pulse, thus leading to the generation of XUV photons. It is found that the generated XUV spectrum is notably sensitive to the chirp of the attosecond pulse, which can then be reliably retrieved. A classical quantum-path analysis is further used to quantitatively explain the main features exhibited in the XUV emission.

Direct Visualization of Valence Electron Motion Using Strong-Field Photoelectron Holography

Science.gov (United States)

He, Mingrui; Li, Yang; Zhou, Yueming; Li, Min; Cao, Wei; Lu, Peixiang

2018-03-01

Watching the valence electron move in molecules on its intrinsic timescale has been one of the central goals of attosecond science and it requires measurements with subatomic spatial and attosecond temporal resolutions. The time-resolved photoelectron holography in strong-field tunneling ionization holds the promise to access this realm. However, it remains to be a challenging task hitherto. Here we reveal how the information of valence electron motion is encoded in the hologram of the photoelectron momentum distribution (PEMD) and develop a novel approach of retrieval. As a demonstration, applying it to the PEMDs obtained by solving the time-dependent Schrödinger equation for the prototypical molecule H2+ , the attosecond charge migration is directly visualized with picometer spatial and attosecond temporal resolutions. Our method represents a general approach for monitoring attosecond charge migration in more complex polyatomic and biological molecules, which is one of the central tasks in the newly emerging attosecond chemistry.

Observations of electron vortex magnetic holes and related wave-particle interactions in the turbulent magnetosheath

Science.gov (United States)

Huang, S.; Sahraoui, F.; Yuan, Z.; He, J.; Zhao, J.; Du, J.; Le Contel, O.; Wang, X.; Deng, X.; Fu, H.; Zhou, M.; Shi, Q.; Breuillard, H.; Pang, Y.; Yu, X.; Wang, D.

2017-12-01

Magnetic hole is characterized by a magnetic depression, a density peak, a total electron temperature increase (with a parallel temperature decrease but a perpendicular temperature increase), and strong currents carried by the electrons. The current has a dip in the core region of the magnetic hole and a peak in the outer region of the magnetic hole. There is an enhancement in the perpendicular electron fluxes at 90° pitch angles inside the magnetic hole, implying that the electrons are trapped within it. The variations of the electron velocity components Vem and Ven suggest that an electron vortex is formed by trapping electrons inside the magnetic hole in the circular cross-section. These observations demonstrate the existence of a new type of coherent structures behaving as an electron vortex magnetic hole in turbulent space plasmas as predicted by recent kinetic simulations. We perform a statistically study using high time solution data from the MMS mission. The magnetic holes with short duration (i.e., < 0.5 s) have their cross section smaller than the ion gyro-radius. Superposed epoch analysis of all events reveals that an increase in the electron density and total temperature, significantly increase (resp. decrease) the electron perpendicular (resp. parallel) temperature, and an electron vortex inside the holes. Electron fluxes at 90° pitch angles with selective energies increase in the KSMHs, are trapped inside KSMHs and form the electron vortex due to their collective motion. All these features are consistent with the electron vortex magnetic holes obtained in 2D and 3D particle-in-cell simulations, indicating that the observed the magnetic holes seem to be best explained as electron vortex magnetic holes. It is furthermore shown that the magnetic holes are likely to heat and accelerate the electrons. We also investigate the coupling between whistler waves and electron vortex magnetic holes. These whistler waves can be locally generated inside electron

Transverse Space-Charge Field-Induced Plasma Dynamics for Ultraintense Electron-Beam Characterization

Directory of Open Access Journals (Sweden)

R. Tarkeshian

2018-05-01

Full Text Available Similarly to laser or x-ray beams, the interaction of sufficiently intense particle beams with neutral gases will result in the creation of plasma. In contrast to photon-based ionization, the strong unipolar field of a particle beam can generate a plasma where the electron population receives a large initial momentum kick and escapes, leaving behind unshielded ions. Measuring the properties of the ensuing Coulomb exploding ions—such as their kinetic energy distribution, yield, and spatial distribution—can provide information about the peak electric fields that are achieved in the electron beams. Particle-in-cell simulations and analytical models are presented for high-brightness electron beams of a few femtoseconds or even hundreds of attoseconds, and transverse beam sizes on the micron scale, as generated by today’s free electron lasers. Different density regimes for the utilization as a potential diagnostics are explored, and the fundamental differences in plasma dynamical behavior for e-beam or photon-based ionization are highlighted. By measuring the dynamics of field-induced ions for different gas and beam densities, a lower bound on the beam charge density can be obtained in a single shot and in a noninvasive way. The exponential dependency of the ionization yield on the beam properties can provide unprecedented spatial and temporal resolution, at the submicrometer and subfemtosecond scales, respectively, offering a practical and powerful approach to characterizing beams from accelerators at the frontiers of performance.

Dynamical evolution of quasicircular binary black hole data

International Nuclear Information System (INIS)

Alcubierre, Miguel; Bruegmann, Bernd; Diener, Peter; Guzman, F. Siddhartha; Hawke, Ian; Hawley, Scott; Herrmann, Frank; Pollney, Denis; Thornburg, Jonathan; Koppitz, Michael; Seidel, Edward

2005-01-01

We study the fully nonlinear dynamical evolution of binary black hole data, whose orbital parameters are specified via the effective potential method for determining quasicircular orbits. The cases studied range from the Cook-Baumgarte innermost stable circular orbit (ISCO) to significantly beyond that separation. In all cases we find the black holes to coalesce (as determined by the appearance of a common apparent horizon) in less than half an orbital period. The results of the numerical simulations indicate that the initial holes are not actually in quasicircular orbits, but that they are in fact nearly plunging together. The dynamics of the final horizon are studied to determine physical parameters of the final black hole, such as its spin, mass, and oscillation frequency, revealing information about the inspiral process. We show that considerable resolution is required to extract accurate physical information from the final black hole formed in the merger process, and that the quasinormal modes of the final hole are strongly excited in the merger process. For the ISCO case, by comparing physical measurements of the final black hole formed to the initial data, we estimate that less than 3% of the total energy is radiated in the merger process

Electron holes in phase space: What they are and why they matter

Science.gov (United States)

Hutchinson, I. H.

2017-05-01

This is a tutorial and selective review explaining the fundamental concepts and some currently open questions concerning the plasma phenomenon of the electron hole. The widespread occurrence of electron holes in numerical simulations, space-craft observations, and laboratory experiments is illustrated. The elementary underlying theory is developed of a one-dimensional electron hole as a localized potential maximum, self-consistently sustained by a deficit of trapped electron phase-space density. The spatial extent of a hole is typically a few Debye lengths; what determines the minimum and maximum possible lengths is explained, addressing the key aspects of the as yet unsettled dispute between the integral and differential approaches to hole structure. In multiple dimensions, holes tend to form less readily; they generally require a magnetic field and distribution-function anisotropy. The mechanisms by which they break up are explained, noting that this transverse instability is not fully understood. Examples are given of plasma circumstances where holes play an important role, and of recent progress on understanding their holistic kinematics and self-acceleration.

Luminescence of high density electron-hole plasma in CdS and CdSe in a wide temperature range

International Nuclear Information System (INIS)

Yoshida, H.; Shionoya, S.

1983-01-01

Time-resolved spectra of the spontaneous luminescence of the high density electron-hole plasma (EHP) in CdS and CdSe are observed in a wide range of temperature which is surely higher than the calculated critical temperature for electron-hole liquid formation, in order to carry forward discussion on dynamic nature of the EHP previously observed in 4.2 K experiments. Spectra in the late stage are analyzed, and obtained values of the reduced bandgap energy and chemical potential are compared with those theoretically calculated for higher temperatures. The aspects of the change of the spectral shape in the late stage are hard to understand. Unfortunately no clear conclusion is drawn on the nature of the EHP produced at 4.2 K. The only thing one can say is that the condensed electron-hole liquid state, which is in equilibrium with the exciton state, is not realized. (author)

Magnetospheric Multiscale Observations of Electron Vortex Magnetic Hole in the Turbulent Magnetosheath Plasma

Energy Technology Data Exchange (ETDEWEB)

Huang, S. Y.; Yuan, Z. G.; Wang, D. D.; Yu, X. D. [School of Electronic Information, Wuhan University, Wuhan (China); Sahraoui, F.; Contel, O. Le [Laboratoire de Physique des Plasmas, CNRS-Ecole Polytechnique-UPMC, Palaiseau (France); He, J. S. [School of Earth and Space Sciences, Peking University, Beijing (China); Zhao, J. S. [Key Laboratory of Planetary Sciences, Purple Mountain Observatory, Chinese Academy of Sciences, Nanjing (China); Deng, X. H.; Pang, Y.; Li, H. M. [Institute of Space Science and Technology, Nanchang University, Nanchang (China); Zhou, M. [Department of Physics and Astronomy, University of California, Los Angeles, CA (United States); Fu, H. S.; Yang, J. [School of Space and Environment, Beihang University, Beijing (China); Shi, Q. Q. [Shandong Provincial Key Laboratory of Optical Astronomy and Solar-Terrestrial Environment, Institute of Space Sciences, Shandong University, Weihai (China); Lavraud, B. [Institut de Recherche and Astrophysique et Planétologie, Université de Toulouse (UPS), Toulouse (France); Pollock, C. J.; Giles, B. L. [NASA, Goddard Space Flight Center, Greenbelt, MD (United States); Torbert, R. B. [University of New Hampshire, Durham, NH (United States); Russell, C. T., E-mail: shiyonghuang@whu.edu.cn [Department of Earth, Planetary and Space Sciences, University of California, Los Angeles, CA (United States); and others

2017-02-20

We report on the observations of an electron vortex magnetic hole corresponding to a new type of coherent structure in the turbulent magnetosheath plasma using the Magnetospheric Multiscale mission data. The magnetic hole is characterized by a magnetic depression, a density peak, a total electron temperature increase (with a parallel temperature decrease but a perpendicular temperature increase), and strong currents carried by the electrons. The current has a dip in the core region and a peak in the outer region of the magnetic hole. The estimated size of the magnetic hole is about 0.23 ρ {sub i} (∼30 ρ {sub e}) in the quasi-circular cross-section perpendicular to its axis, where ρ {sub i} and ρ {sub e} are respectively the proton and electron gyroradius. There are no clear enhancements seen in high-energy electron fluxes. However, there is an enhancement in the perpendicular electron fluxes at 90° pitch angle inside the magnetic hole, implying that the electrons are trapped within it. The variations of the electron velocity components V {sub em} and V {sub en} suggest that an electron vortex is formed by trapping electrons inside the magnetic hole in the cross-section in the M – N plane. These observations demonstrate the existence of a new type of coherent structures behaving as an electron vortex magnetic hole in turbulent space plasmas as predicted by recent kinetic simulations.

Binary black holes: Spin dynamics and gravitational recoil

International Nuclear Information System (INIS)

Herrmann, Frank; Hinder, Ian; Shoemaker, Deirdre M.; Laguna, Pablo; Matzner, Richard A.

2007-01-01

We present a study of spinning black hole binaries focusing on the spin dynamics of the individual black holes as well as on the gravitational recoil acquired by the black hole produced by the merger. We consider two series of initial spin orientations away from the binary orbital plane. In one of the series, the spins are antialigned; for the second series, one of the spins points away from the binary along the line separating the black holes. We find a remarkable agreement between the spin dynamics predicted at 2nd post-Newtonian order and those from numerical relativity. For each configuration, we compute the kick of the final black hole. We use the kick estimates from the series with antialigned spins to fit the parameters in the Kidder kick formula, and verify that the recoil in the direction of the orbital angular momentum is ∝sinθ and on the orbital plane ∝cosθ, with θ the angle between the spin directions and the orbital angular momentum. We also find that the black hole spins can be well estimated by evaluating the isolated horizon spin on spheres of constant coordinate radius

Amplitude and phase control of attosecond light pulses

International Nuclear Information System (INIS)

Lopez-Martens, Rodrigo; Varju, Katalin; Johnsson, Per; Mauritsson, Johan; Persson, Anders; Svanberg, Sune; Wahlstroem, Claes-Goeran; L'Huillier, Anne; Mairesse, Yann; Salieres, Pascal; Gaarde, Mette B.; Schafer, Kenneth J.

2005-01-01

We report the generation, compression, and delivery on target of ultrashort extreme-ultraviolet light pulses using external amplitude and phase control. Broadband harmonic radiation is first generated by focusing an infrared laser with a carefully chosen intensity into a gas cell containing argon atoms. The emitted light then goes through a hard aperture and a thin aluminum filter that selects a 30-eV bandwidth around a 30-eV photon energy and synchronizes all of the components, thereby enabling the formation of a train of almost Fourier-transform-limited single-cycle 170 attosecond pulses. Our experiment demonstrates a practical method for synthesizing and controlling attosecond waveforms

Phase-resolved attosecond near-threshold photoionization of molecular nitrogen

International Nuclear Information System (INIS)

Haessler, S.; Ruchon, T.; Breger, P.; Carre, B.; Salieres, P.; Fabre, B.; Higuet, J.; Constant, E.; Mevel, E.; Mairesse, Y.; Caillat, J.; Maquet, A.; Taieeb, R.

2009-01-01

We photoionize nitrogen molecules with a train of extreme ultraviolet attosecond pulses together with a weak infrared field. We measure the phase of the two-color two-photon ionization transition (molecular phase) for different states of the ion. We observe a 0.9π shift for the electrons produced in the ionization channels leading to the X 2 Σ g + , v ' =1, and v ' =2 states. We relate this phase shift to the presence of a complex resonance in the continuum. By providing both a high spectral and temporal resolution, this general approach gives access to the evolution of extremely short-lived states, which is often not accessible otherwise.

Producing High Intense Attosecond Pulse Train by Interaction of Three-Color Pulse and Overdense Plasma

Science.gov (United States)

Salehi, M.; Mirzanejad, S.

2017-05-01

Amplifying the attosecond pulse by the chirp pulse amplification method is impossible. Furthermore, the intensity of attosecond pulse is low in the interaction of laser pulse and underdense plasma. This motivates us to propose using a multi-color pulse to produce the high intense attosecond pulse. In the present study, the relativistic interaction of a three-color linearly-polarized laser-pulse with highly overdense plasma is studied. We show that the combination of {{ω }}1, {{ω }}2 and {{ω }}3 frequencies decreases the instance full width at half maximum reflected attosecond pulse train from the overdense plasma surface. Moreover, we show that the three-color pulse increases the intensity of generated harmonics, which is explained by the relativistic oscillating mirror model. The obtained results demonstrate that if the three-color laser pulse interacts with overdense plasma, it will enhance two orders of magnitude of intensity of ultra short attosecond pulses in comparison with monochromatic pulse.

Interlayer electron-hole pair multiplication by hot carriers in atomic layer semiconductor heterostructures

Science.gov (United States)

Barati, Fatemeh; Grossnickle, Max; Su, Shanshan; Lake, Roger; Aji, Vivek; Gabor, Nathaniel

Two-dimensional heterostructures composed of atomically thin transition metal dichalcogenides provide the opportunity to design novel devices for the study of electron-hole pair multiplication. We report on highly efficient multiplication of interlayer electron-hole pairs at the interface of a tungsten diselenide / molybdenum diselenide heterostructure. Electronic transport measurements of the interlayer current-voltage characteristics indicate that layer-indirect electron-hole pairs are generated by hot electron impact excitation. Our findings, which demonstrate an efficient energy relaxation pathway that competes with electron thermalization losses, make 2D semiconductor heterostructures viable for a new class of hot-carrier energy harvesting devices that exploit layer-indirect electron-hole excitations. SHINES, an Energy Frontier Research Center funded by the U.S. Department of Energy, Air Force Office of Scientific Research.

Global structure of exact scalar hairy dynamical black holes

Energy Technology Data Exchange (ETDEWEB)

Fan, Zhong-Ying [Center for High Energy Physics, Peking University,No. 5 Yiheyuan Rd, Beijing, 100871 P.R. (China); Chen, Bin [Center for High Energy Physics, Peking University,No. 5 Yiheyuan Rd, Beijing, 100871 P.R. (China); Department of Physics and State Key Laboratory of Nuclear Physics and Technology,Peking University, No. 5 Yiheyuan Rd, Beijing, 100871 P.R. (China); Collaborative Innovation Center of Quantum Matter,No. 5 Yiheyuan Rd, Beijing, 100871 P.R. (China); Lü, H. [Center for Advanced Quantum Studies, Department of Physics, Beijing Normal University,Beijing, 100875 P.R. (China)

2016-05-30

We study the global structure of some exact scalar hairy dynamical black holes which were constructed in Einstein gravity either minimally or non-minimally coupled to a scalar field. We find that both the apparent horizon and the local event horizon (measured in luminosity coordinate) monotonically increase with the advanced time as well as the Vaidya mass. At late advanced times, the apparent horizon approaches the event horizon and gradually becomes future outer. Correspondingly, the space-time arrives at stationary black hole states with the relaxation time inversely proportional to the 1/(n−1) power of the final black hole mass, where n is the space-time dimension. These results strongly support the solutions describing the formation of black holes with scalar hair. We also obtain new charged dynamical solutions in the non-minimal theory by introducing an Maxwell field which is non-minimally coupled to the scalar. The presence of the electric charge strongly modifies the dynamical evolution of the space-time.

Effects of density imbalance on the BCS-BEC crossover in semiconductor electron-hole bilayers

International Nuclear Information System (INIS)

Pieri, P.; Strinati, G. C.; Neilson, D.

2007-01-01

We study the occurrence of excitonic superfluidity in electron-hole bilayers at zero temperature. We not only identify the crossover in the phase diagram from the BCS limit of overlapping pairs to the BEC limit of nonoverlapping tightly bound pairs but also, by varying the electron and hole densities independently, we can analyze a number of phases that occur mainly in the crossover region. With different electron and hole effective masses, the phase diagram is asymmetric with respect to excess electron or hole densities. We propose, as the criterion for the onset of superfluidity, the jump of the electron and hole chemical potentials when their densities cross

Quantum dynamic imaging theoretical and numerical methods

CERN Document Server

Ivanov, Misha

2011-01-01

Studying and using light or "photons" to image and then to control and transmit molecular information is among the most challenging and significant research fields to emerge in recent years. One of the fastest growing areas involves research in the temporal imaging of quantum phenomena, ranging from molecular dynamics in the femto (10-15s) time regime for atomic motion to the atto (10-18s) time scale of electron motion. In fact, the attosecond "revolution" is now recognized as one of the most important recent breakthroughs and innovations in the science of the 21st century. A major participant in the development of ultrafast femto and attosecond temporal imaging of molecular quantum phenomena has been theory and numerical simulation of the nonlinear, non-perturbative response of atoms and molecules to ultrashort laser pulses. Therefore, imaging quantum dynamics is a new frontier of science requiring advanced mathematical approaches for analyzing and solving spatial and temporal multidimensional partial differ...

Attosecond pulse trains from long laser-gas interaction targets

International Nuclear Information System (INIS)

Hauri, C.P.; Lopez-Martens, R.; Varju, K.; Ruchon, T.; Gustafsson, E.; L'Huillier, A.

2006-01-01

Complete test of publication follows. Many experiments in attosecond physics require high XUV photon flux as well as a clean attosecond pulse train (APT) temporal structure. Temporal characterization of high-order harmonic generation (HHG) in long interaction targets is thus of high interest. HHG being a very inefficient process, a large effort has been made to increase the amount of XUV photons emitted per infrared laser pulse. Besides quasi phase-matching in a modulated capillary, loose driving laser focusing conditions and subsequent self-channeling have shown to significantly increase the conversion efficiency. We characterized the temporal structure of APTs generated during the self-channeling of an intense IR driving laser pulse. Our first results indicate, however, that the temporal structure of the APT generated during the HHG process might be affected by quantum path interference and spectral phase distortion due to the self-channeling process itself. In particular, our measurements show that the relative spectral phase between consecutive harmonics can strongly vary depending on the target length and the position of the laser focus with respect to the target. In general for short gas targets, no clean APT structure can be expected since the individual attosecond pulses carry significant chirp. For longer targets, however, we observe a flattening of the harmonic spectral phase, resulting in near-transform-limited attosecond pulse trains. A complete analysis of the process is complex and involves detailed knowledge of the spatial and temporal evolution of the self-channeling driver laser pulse throughout the gas target.

Breakdown of the one-electron picture in XPS, XES and AES spectra involving 4s and 4p holes in Pd to Xe

International Nuclear Information System (INIS)

Ohno, M.; Wendin, G.

1981-01-01

Certain XES spectra of Pd to Xe have been calculated using diagrammatic many-body theory within the framework of a free atom calculation. Both XPS an XES spectra demonstrate breakdown of the one-electron picture of a 4p hole due to strong dynamical grant-Coster Kronig (gCK) fluctuation and decay processes. For a 4s hole, there is a large energy shift due to gCK fluctuation, but an effective one-electron model of the 4s hole is valid. For elements Cd to Te, gCK fluctuation and decay lead to broad continuance spectrum and breakdown of the 4p model. Breakdown of the one-electron, or even quasi-particle, model must occur when 4s and 4p holes are part of multiple vacancies

Black hole dynamics in general relativity

Indian Academy of Sciences (India)

Abstract. Basic features of dynamical black holes in full, non-linear general relativity are summarized in a pedagogical fashion. Qualitative properties of the evolution of various horizons follow directly from the celebrated Raychaudhuri equation.

Intense isolated attosecond pulse generation from relativistic laser plasmas using few-cycle laser pulses

International Nuclear Information System (INIS)

Ma, Guangjin; Dallari, William; Borot, Antonin; Tsakiris, George D.; Veisz, Laszlo; Krausz, Ferenc; Yu, Wei

2015-01-01

We have performed a systematic study through particle-in-cell simulations to investigate the generation of attosecond pulse from relativistic laser plasmas when laser pulse duration approaches the few-cycle regime. A significant enhancement of attosecond pulse energy has been found to depend on laser pulse duration, carrier envelope phase, and plasma scale length. Based on the results obtained in this work, the potential of attaining isolated attosecond pulses with ∼100 μJ energy for photons >16 eV using state-of-the-art laser technology appears to be within reach

High level harmonic radiation: atto-second impulse generation, application to coherent radiation

International Nuclear Information System (INIS)

Kovacev, Milutin

2003-01-01

The work presented in this thesis is dedicated to the characterization and optimization of the unique properties of high order harmonic generation in a rare gas: high brilliance, short pulse duration (femtosecond to atto-second, 1 as = 10"-"1"8 s and good mutual coherence. In the first part of this work, we concentrate on the exploitation of a scaling law using a high-energy laser loosely focused inside an extended gaseous medium. For the first time, the generated harmonic energy exceeds the 1 μJ level per laser pulse using the fifteenth harmonic order at a wavelength of 53 nm. The conversion efficiency reaches 4.10"-"5, which results from the combination of a strong dipolar response and a good phase matching within a generating volume that is extended by self guiding of the generating laser pulse. In the second part, our interest is devoted to the temporal profile of the harmonic emission and its atto-second structure. We first demonstrate the feasibility of a spatial/spectral selection of the contributions associated to the two main electronic trajectories, allowing thereby the generation of regular atto-second pulse trains. We then characterize such a pulse train by the measurement of the relative phases of consecutive harmonics. Finally, we describe an original technique for the temporal confinement of the harmonic emission by manipulating the ellipticity of the generating laser beam. In the third part, our interest is dedicated to the mutual coherence properties of the harmonic emission. We first demonstrate the precise control of the relative phase of the harmonic pulses by multiple beam interference in the XUV. This frequency-domain interferometry using four phase-locked temporally separated pulses shows an extreme sensitivity to the relative phase of the pulses on an atto-second time scale. We then measure the first order autocorrelation trace of the harmonic beam thanks to the generation of two harmonic sources mutually coherent and spatially separated

Negligible Electronic Interaction between Photoexcited Electron-Hole Pairs and Free Electrons in Phosphorus-Boron Co-Doped Silicon Nanocrystals

Energy Technology Data Exchange (ETDEWEB)

Limpens, Rens [National Renewable Energy Laboratory (NREL), Golden, CO (United States); Neale, Nathan R [National Renewable Energy Laboratory (NREL), Golden, CO (United States); Fujii, Minoru [Kobe University; Gregorkiewicz, Tom [University of Amsterdam

2018-03-05

Phosphorus (P) and boron (B) co-doped Si nanocrystals (NCs) have raised interest in the optoelectronic industry due to their electronic tunability, optimal carrier multiplication properties, and straightforward dispersibility in polar solvents. Yet a basic understanding of the interaction of photoexcited electron-hole (e-h) pairs with new physical features that are introduced by the co-doping process (free carriers, defect states, and surface chemistry) is missing. Here, we present the first study of the ultrafast carrier dynamics in SiO2-embedded P-B co-doped Si NC ensembles using induced absorption spectroscopy through a two-step approach. First, the induced absorption data show that the large fraction of the dopants residing on the NC surface slows down carrier relaxation dynamics within the first 20 ps relative to intrinsic (undoped) Si NCs, which we interpret as enhanced surface passivation. On longer time-scales (picosecond to nanosecond regime), we observe a speeding up of the carrier relaxation dynamics and ascribe it to doping-induced trap states. This argument is deduced from the second part of the study, where we investigate multiexciton interactions. From a stochastic modeling approach we show that localized carriers, which are introduced by the P or B dopants, have minor electronic interactions with the photoexcited e-h pairs. This is understood in light of the strong localization of the introduced carriers on their original P- or B-dopant atoms, due to the strong quantum confinement regime in these relatively small NCs (<6 nm).

Spin relaxation dynamics of holes in intrinsic GaAs quantum wells studied by transient circular dichromatic absorption spectroscopy at room temperature.

Science.gov (United States)

Fang, Shaoyin; Zhu, Ruidan; Lai, Tianshu

2017-03-21

Spin relaxation dynamics of holes in intrinsic GaAs quantum wells is studied using time-resolved circular dichromatic absorption spectroscopy at room temperature. It is found that ultrafast dynamics is dominated by the cooperative contributions of band filling and many-body effects. The relative contribution of the two effects is opposite in strength for electrons and holes. As a result, transient circular dichromatic differential transmission (TCD-DT) with co- and cross-circularly polarized pump and probe presents different strength at several picosecond delay time. Ultrafast spin relaxation dynamics of excited holes is sensitively reflected in TCD-DT with cross-circularly polarized pump and probe. A model, including coherent artifact, thermalization of nonthermal carriers and the cooperative contribution of band filling and many-body effects, is developed, and used to fit TCD-DT with cross-circularly polarized pump and probe. Spin relaxation time of holes is achieved as a function of excited hole density for the first time at room temperature, and increases with hole density, which disagrees with a theoretical prediction based on EY spin relaxation mechanism, implying that EY mechanism may be not dominant hole spin relaxation mechanism at room temperature, but DP mechanism is dominant possibly.

Value and Anisotropy of the Electron and Hole Mass in Pure Wurtzite InP Nanowires.

Science.gov (United States)

Tedeschi, D; De Luca, M; Granados Del Águila, A; Gao, Q; Ambrosio, G; Capizzi, M; Tan, H H; Christianen, P C M; Jagadish, C; Polimeni, A

2016-10-12

The effective mass of electrons and holes in semiconductors is pivotal in determining the dynamics of carriers and their confinement energy in nanostructured materials. Surprisingly, this quantity is still unknown in wurtzite (WZ) nanowires (NWs) made of III-V compounds (e.g., GaAs, InAs, GaP, InP), where the WZ phase has no bulk counterpart. Here, we investigate the magneto-optical properties of InP WZ NWs grown by selective-area epitaxy that provides perfectly ordered NWs featuring high-crystalline quality. The combined analysis of the energy of free exciton states and impurity levels under magnetic field (B up to 29 T) allows us to disentangle the dynamics of oppositely charged carriers from the Coulomb interaction and thus to determine the values of the electron and hole effective mass. By application of B⃗ along different crystallographic directions, we also assess the dependence of the transport properties with respect to the NW growth axis (namely, the WZ ĉ axis). The effective mass of electrons along ĉ is m e ∥ = (0.078 ± 0.002) m 0 (m 0 is the electron mass in vacuum) and perpendicular to ĉ is m e ⊥ = (0.093 ± 0.001) m 0 , resulting in a 20% mass anisotropy. Holes exhibit a much larger (∼320%) and opposite mass anisotropy with their effective mass along and perpendicular to ĉ equal to m h ∥ = (0.81 ± 0.18) m 0 and m h ⊥ = (0.250 ± 0.016) m 0 , respectively. While no full consensus is found with current theoretical results on WZ InP, our findings show trends remarkably similar to the experimental data available in WZ bulk materials, such as InN, GaN, and ZnO.

Classical black holes: the nonlinear dynamics of curved spacetime.

Science.gov (United States)

Thorne, Kip S

2012-08-03

Numerical simulations have revealed two types of physical structures, made from curved spacetime, that are attached to black holes: tendexes, which stretch or squeeze anything they encounter, and vortexes, which twist adjacent inertial frames relative to each other. When black holes collide, their tendexes and vortexes interact and oscillate (a form of nonlinear dynamics of curved spacetime). These oscillations generate gravitational waves, which can give kicks up to 4000 kilometers per second to the merged black hole. The gravitational waves encode details of the spacetime dynamics and will soon be observed and studied by the Laser Interferometer Gravitational Wave Observatory and its international partners.

Linked-cluster formulation of electron-hole interaction kernel in real-space representation without using unoccupied states.

Science.gov (United States)

Bayne, Michael G; Scher, Jeremy A; Ellis, Benjamin H; Chakraborty, Arindam

2018-05-21

Electron-hole or quasiparticle representation plays a central role in describing electronic excitations in many-electron systems. For charge-neutral excitation, the electron-hole interaction kernel is the quantity of interest for calculating important excitation properties such as optical gap, optical spectra, electron-hole recombination and electron-hole binding energies. The electron-hole interaction kernel can be formally derived from the density-density correlation function using both Green's function and TDDFT formalism. The accurate determination of the electron-hole interaction kernel remains a significant challenge for precise calculations of optical properties in the GW+BSE formalism. From the TDDFT perspective, the electron-hole interaction kernel has been viewed as a path to systematic development of frequency-dependent exchange-correlation functionals. Traditional approaches, such as MBPT formalism, use unoccupied states (which are defined with respect to Fermi vacuum) to construct the electron-hole interaction kernel. However, the inclusion of unoccupied states has long been recognized as the leading computational bottleneck that limits the application of this approach for larger finite systems. In this work, an alternative derivation that avoids using unoccupied states to construct the electron-hole interaction kernel is presented. The central idea of this approach is to use explicitly correlated geminal functions for treating electron-electron correlation for both ground and excited state wave functions. Using this ansatz, it is derived using both diagrammatic and algebraic techniques that the electron-hole interaction kernel can be expressed only in terms of linked closed-loop diagrams. It is proved that the cancellation of unlinked diagrams is a consequence of linked-cluster theorem in real-space representation. The electron-hole interaction kernel derived in this work was used to calculate excitation energies in many-electron systems and results

Local and dynamic properties of light interacting with subwavelength holes

NARCIS (Netherlands)

Prangsma, Jord

2009-01-01

The discovery of the extraordinary transmission phenomena has initiated an intense study of the interaction of light with subwavelength holes. In this thesis the dynamic and local properties of light interacting with subwavelength holes are investigated. First of all the role of hole shape on the

Hole-spin dynamics in p-doped GaAs/AlGaAs heterostructures; Lochspindynamik in p-dotierten GaAs/AlGaAs-Heterostrukturen

Energy Technology Data Exchange (ETDEWEB)

Kugler, Michael

2012-11-15

This work investigates the spin dynamics of holes in p-doped GaAs/AlGaAs quantum wells (QW) at low temperatures. To examine the energetic structure of the used samples, PL and PLE-spectroscopy were employed. Time resolved Kerr and Faraday-Rotation (TRKR/FR) and 'Resonant Spin Amplification' (RSA) were used to analyse the spin dynamics. First, the signal formation in TRKR/FR and RSA experiments is discussed taking into account the interconnected charge carrier dynamics and spin dynamics of electrons and holes. An excitation energy dependent sign change of the Kerr signal amplitude could be observed, whose energetic position corresponds to an absorption maximum in PLE experiments. This behavior could be explained by an energy dependent splitting of the spin niveaus, which leads to an energy dependence of the Faraday and Kerr signal. Furthermore, two initialization processes were investigated, which could be used to transfer optically generated spin information into the resident hole spin system. This could be achieved by either applying a magnetic field, or by rapid dephasing of hole spins immediately after excitation. Changes in excitation energy, excitation density or temperature could be used to influence the fast dephasing processes and therefore the initial ratio of hole to electron spins. The complex, interconnected charge carrier and spin dynamics of electrons and holes could be accurately reproduced using a rate equation model. This allowed for the extraction of physically relevant parameters like spin lifetimes and g-factors from RSA and TRKR/FR data. An analytical model that was developed at the Wroclaw University of Technology delivered matching results. In the second part of the experimental work, the dependence of the hole spin lifetime and the hole g-factor on various parameters was analysed. Here, the RSA method could for the first time be applied to two-dimensional hole systems, allowing for new insights into the regime of long lived hole

Electron vortex magnetic holes: A nonlinear coherent plasma structure

Energy Technology Data Exchange (ETDEWEB)

Haynes, Christopher T., E-mail: c.t.haynes@qmul.ac.uk; Burgess, David; Sundberg, Torbjorn [School of Physics and Astronomy, Queen Mary University of London, Mile End Road, London E1 4NS (United Kingdom); Camporeale, Enrico [Multiscale Dynamics, Centrum Wiskunde and Informatica (CWI), Amsterdam (Netherlands)

2015-01-15

We report the properties of a novel type of sub-proton scale magnetic hole found in two dimensional particle-in-cell simulations of decaying turbulence with a guide field. The simulations were performed with a realistic value for ion to electron mass ratio. These structures, electron vortex magnetic holes (EVMHs), have circular cross-section. The magnetic field depression is associated with a diamagnetic azimuthal current provided by a population of trapped electrons in petal-like orbits. The trapped electron population provides a mean azimuthal velocity and since trapping preferentially selects high pitch angles, a perpendicular temperature anisotropy. The structures arise out of initial perturbations in the course of the turbulent evolution of the plasma, and are stable over at least 100 electron gyroperiods. We have verified the model for the EVMH by carrying out test particle and PIC simulations of isolated structures in a uniform plasma. It is found that (quasi-)stable structures can be formed provided that there is some initial perpendicular temperature anisotropy at the structure location. The properties of these structures (scale size, trapped population, etc.) are able to explain the observed properties of magnetic holes in the terrestrial plasma sheet. EVMHs may also contribute to turbulence properties, such as intermittency, at short scale lengths in other astrophysical plasmas.

Generation of isolated attosecond pulses using a plasmonic funnel-waveguide

International Nuclear Information System (INIS)

Choi, Joonhee; Kim, Seungchul; Park, In-Yong; Lee, Dong-Hyub; Han, Seunghwoi; Kim, Seung-Woo

2012-01-01

We theoretically investigated the possibility of generating attosecond pulses by means of plasmonic field enhancement induced in a nano-structured metallic funnel-waveguide. This study was motivated by our recent experimental demonstration of ultrashort extreme-ultraviolet (EUV) pulses using the same type of three-dimensional waveguides. Here, with emphasis on generation of isolated attosecond pulses, the finite-domain time-difference method was used to analyze the funnel-waveguide with respect to the geometry-dependent plasmonic features such as the field enhancement factor, enhanced plasmonic field profile and hot-spot location. Then an extended semi-classical model of high-order harmonic generation was adopted to predict the EUV spectra generated from the funnel-waveguide in consideration of the spatial inhomogeneity of the plasmonic field within the hot-spot volume. Our simulation finally proved that isolated attosecond pulses can be produced at fast repetition rates directly from a few-cycle femtosecond laser or by synthesizing a two-color laser consisting of two multi-cycle pulses of cross-polarized configuration. (paper)

Black Hole Universe Model for Explaining GRBs, X-Ray Flares, and Quasars as Emissions of Dynamic Star-like, Massive, and Supermassive Black Holes

Science.gov (United States)

Zhang, Tianxi

2014-01-01

Slightly modifying the standard big bang theory, the author has recently developed a new cosmological model called black hole universe, which is consistent with Mach’s principle, governed by Einstein’s general theory of relativity, and able to explain all observations of the universe. Previous studies accounted for the origin, structure, evolution, expansion, cosmic microwave background radiation, and acceleration of the black hole universe, which grew from a star-like black hole with several solar masses through a supermassive black hole with billions of solar masses to the present state with hundred billion-trillions of solar masses by accreting ambient matter and merging with other black holes. This study investigates the emissions of dynamic black holes according to the black hole universe model and provides a self-consistent explanation for the observations of gamma ray bursts (GRBs), X-ray flares, and quasars as emissions of dynamic star-like, massive, and supermassive black holes. It is shown that a black hole, when it accretes its ambient matter or merges with other black holes, becomes dynamic. Since the event horizon of a dynamic black hole is broken, the inside hot (or high-frequency) blackbody radiation leaks out. The leakage of the inside hot blackbody radiation leads to a GRB if it is a star-like black hole, an X-ray flare if it is a massive black hole like the one at the center of the Milky Way, or a quasar if it is a supermassive black hole like an active galactic nucleus (AGN). The energy spectra and amount of emissions produced by the dynamic star-like, massive, and supermassive black holes can be consistent with the measurements of GRBs, X-ray flares, and quasars.

Generation of Electron Whistler Waves at the Mirror Mode Magnetic Holes: MMS Observations and PIC Simulation

Science.gov (United States)

Ahmadi, N.; Wilder, F. D.; Usanova, M.; Ergun, R.; Argall, M. R.; Goodrich, K.; Eriksson, S.; Germaschewski, K.; Torbert, R. B.; Lindqvist, P. A.; Le Contel, O.; Khotyaintsev, Y. V.; Strangeway, R. J.; Schwartz, S. J.; Giles, B. L.; Burch, J.

2017-12-01

The Magnetospheric Multiscale (MMS) mission observed electron whistler waves at the center and at the gradients of magnetic holes on the dayside magnetosheath. The magnetic holes are nonlinear mirror structures which are anti-correlated with particle density. We used expanding box Particle-in-cell simulations and produced the mirror instability magnetic holes. We show that the electron whistler waves can be generated at the gradients and the center of magnetic holes in our simulations which is in agreement with MMS observations. At the nonlinear regime of mirror instability, the proton and electron temperature anisotropy are anti-correlated with the magnetic hole. The plasma is unstable to electron whistler waves at the minimum of the magnetic field structures. In the saturation regime of mirror instability, when magnetic holes are dominant, electron temperature anisotropy develops at the edges of the magnetic holes and electrons become isotropic at the magnetic field minimum. We investigate the possible mechanism for enhancing the electron temperature anisotropy and analyze the electron pitch angle distributions and electron distribution functions in our simulations and compare it with MMS observations.

Observation of preformed electron-hole Cooper pairs in highly excited ZnO

NARCIS (Netherlands)

Versteegh, M.A.M.; van Lange, A.J.; Stoof, H.T.C.; Dijkhuis, J.I.

2012-01-01

Electrons and holes in a semiconductor form hydrogen-atom-like bound states, called excitons. At high electron-hole densities the attractive Coulomb force becomes screened and excitons can no longer exist. Bardeen-Cooper-Schrieffer theory predicts that at such high densities co-operative many-body

Solution-processable ambipolar diketopyrrolopyrrole-selenophene polymer with unprecedentedly high hole and electron mobilities.

Science.gov (United States)

Lee, Junghoon; Han, A-Reum; Kim, Jonggi; Kim, Yiho; Oh, Joon Hak; Yang, Changduk

2012-12-26

There is a fast-growing demand for polymer-based ambipolar thin-film transistors (TFTs), in which both n-type and p-type transistor operations are realized in a single layer, while maintaining simplicity in processing. Research progress toward this end is essentially fueled by molecular engineering of the conjugated backbones of the polymers and the development of process architectures for device fabrication, which has recently led to hole and electron mobilities of more than 1.0 cm(2) V(-1) s(-1). However, ambipolar polymers with even higher performance are still required. By taking into account both the conjugated backbone and side chains of the polymer component, we have developed a dithienyl-diketopyrrolopyrrole (TDPP) and selenophene containing polymer with hybrid siloxane-solubilizing groups (PTDPPSe-Si). A synergistic combination of rational polymer backbone design, side-chain dynamics, and solution processing affords an enormous boost in ambipolar TFT performance, resulting in unprecedentedly high hole and electron mobilities of 3.97 and 2.20 cm(2) V(-1) s(-1), respectively.

Many-particle correlations in quasi-two-dimensional electron-hole systems

International Nuclear Information System (INIS)

Nikolaev, Valentin

2002-01-01

This thesis reports a theoretical investigation of many-particle correlation effects in semiconductor heterostructures containing quantum wells. Particular attention is paid towards quasi-particle pair correlations. Using the Green's function technique and the ladder approximation as a basis, the generalized mass action law, which describes the redistribution of particles between correlated and uncorrelated states in quasi-two-dimensional systems for different temperatures and total densities, is derived. The expression is valid beyond the low-density limit, which allows us to investigate the transition of the system from a dilute exciton gas to a dense electron-hole plasma. A generalized Levinson theorem, which takes k-space filling into account, is formulated. Screening in quasi-two-dimensional systems is analyzed rigorously. Firstly, the qualitatively new mechanism of static local screening by indirect excitons is studied using the simple Thomas-Fermi approximation. Then, a detailed many-body description suitable for a proper account of dynamic screening by a quasi-2D electron-hole plasma, and consistent with the previously derived mass action law, is provided. The generalized Lindhard approximation and excitonic plasmon-pole approximations are also derived. The theory is applied to single and double quantum wells. A self-consistent procedure is developed for numerical investigation of the ionization degree of an electron-hole plasma at different values of temperature/exciton Rydberg ratios. This procedure accounts for screening, k-space filling (exciton bleaching), and the formation of excitons. An abrupt jump in the value of the ionization degree that happens with an increase of the carrier density or temperature (Mott transition) is found in a certain density-temperature region. It has been found that the critical density of the Mott transition for indirect excitons may be much smaller than that for direct excitons. A suggestion has been made that some of the

Relaxation processes in aqueous solutions upon X-ray exposure. Entanglement of electronic and nuclear dynamics

Energy Technology Data Exchange (ETDEWEB)

Unger, Isaak

2017-07-01

About a decade ago new types of electronic non-radiative relaxation processes, involving the environment of an electronically excited or ionized monomer, have been predicted for van der Waals clusters and these were also the first systems where such processes have been detected experimentally. These new autoionization channels encompass the recombination of an electron and a hole, and the energy transfer to a neighboring atom or molecule. Two processes can be distinguished here. In the intermolecular Coulombic decay (ICD) the hole created upon ionization of a monomer is filled by a valence electron of the same species, and the energy released in this electron-hole recombination is used to ionize a neighboring species. In the electron transfer mediated decay (ETMD) the initial hole is filled by an electron from a neighboring species, and the energy released by this recombination is either used to ionize the same neighbor species, or to ionize a third monomer. In more recent experiments on liquid water it has been discovered that these non- local autoionization processes are strongly coupled with ultrafast nuclear dynamics. The core ionization initiates proton motion along a hydrogen donor-bond of the electronically excited water cation. This nuclear dynamics leads to the formation of transient cationic species where a proton is shared by two neighboring water molecules. Subsequent autoionization, either via Auger decay, ICD or ETMD, then occurs from any of such structure transients. This relaxation process is termed proton transfer mediated charge separation, PTM-CS. It has been found in a number of experiments that the probability of PTM-CS to occur depends on the hydrogen-bond strength between the core-ionized molecule and solvent molecules.

Electron-hole pair effects in methane dissociative chemisorption on Ni(111)

Energy Technology Data Exchange (ETDEWEB)

Luo, Xuan; Jiang, Bin, E-mail: bjiangch@ustc.edu.cn [Department of Chemical Physics, University of Science and Technology of China, Hefei, Anhui 230026 (China); Juaristi, J. Iñaki [Centro de Física de Materiales CFM/MPC(CSIC-UPV/EHU), P. Manuel de Lardizabal 5, 20018 San Sebastián (Spain); Donostia International Physics Center DIPC, P. Manuel de Lardizabal 4, 20018 San Sebastián (Spain); Departamento de Física de Materiales, Facultad de Químicas, Universidad del País Vasco (UPV/EHU), Apartado 1072, 20080 San Sebastián (Spain); Alducin, Maite [Centro de Física de Materiales CFM/MPC(CSIC-UPV/EHU), P. Manuel de Lardizabal 5, 20018 San Sebastián (Spain); Donostia International Physics Center DIPC, P. Manuel de Lardizabal 4, 20018 San Sebastián (Spain); Guo, Hua [Department of Chemistry and Chemical Biology, University of New Mexico, Albuquerque, New Mexico 87131 (United States)

2016-07-28

The dissociative chemisorption of methane on metal surfaces has attracted much attention in recent years as a prototype of gas-surface reactions in understanding the mode specific and bond selective chemistry. In this work, we systematically investigate the influence of electron-hole pair excitations on the dissociative chemisorption of CH{sub 4}/CH{sub 3}D/CHD{sub 3} on Ni(111). The energy dissipation induced by surface electron-hole pair excitations is modeled as a friction force introduced in the generalized Langevin equation, in which the independent atomic friction coefficients are determined within the local-density friction approximation. Quasi-classical trajectory calculations for CH{sub 4}/CH{sub 3}D/CHD{sub 3} have been carried out on a recently developed twelve-dimensional potential energy surface. Comparing the dissociation probabilities obtained with and without friction, our results clearly indicate that the electron-hole pair effects are generally small, both on absolute reactivity of each vibrational state and on the mode specificity and bond selectivity. Given similar observations in both water and methane dissociation processes, we conclude that electron-hole pair excitations would not play an important role as long as the reaction is direct and the interaction time between the molecule and metal electrons is relatively short.

Observations of electron phase-space holes driven during magnetic reconnection in a laboratory plasma

Science.gov (United States)

Fox, W.; Porkolab, M.; Egedal, J.; Katz, N.; Le, A.

2012-03-01

This work presents detailed experimental observations of electron phase-space holes driven during magnetic reconnection events on the Versatile Toroidal Facility. The holes are observed to travel on the order of or faster than the electron thermal speed, and are of large size scale, with diameter of order 60 Debye lengths. In addition, they have 3D spheroidal structure with approximately unity aspect ratio. We estimate the direct anomalous resistivity due to ion interaction with the holes and find it to be too small to affect the reconnection rate; however, the holes may play a role in reining in a tail of accelerated electrons and they indicate the presence of other processes in the reconnection layer, such as electron energization and electron beam formation.

Electron-hole collision limited transport in charge-neutral bilayer graphene

Science.gov (United States)

Nam, Youngwoo; Ki, Dong-Keun; Soler-Delgado, David; Morpurgo, Alberto F.

2017-12-01

Ballistic transport occurs whenever electrons propagate without collisions deflecting their trajectory. It is normally observed in conductors with a negligible concentration of impurities, at low temperature, to avoid electron-phonon scattering. Here, we use suspended bilayer graphene devices to reveal a new regime, in which ballistic transport is not limited by scattering with phonons or impurities, but by electron-hole collisions. The phenomenon manifests itself in a negative four-terminal resistance that becomes visible when the density of holes (electrons) is suppressed by gate-shifting the Fermi level in the conduction (valence) band, above the thermal energy. For smaller densities, transport is diffusive, and the measured conductivity is reproduced quantitatively, with no fitting parameters, by including electron-hole scattering as the only process causing velocity relaxation. Experiments on a trilayer device show that the phenomenon is robust and that transport at charge neutrality is governed by the same physics. Our results provide a textbook illustration of a transport regime that had not been observed previously and clarify the nature of conduction through charge-neutral graphene under conditions in which carrier density inhomogeneity is immaterial. They also demonstrate that transport can be limited by a fully electronic mechanism, originating from the same microscopic processes that govern the physics of Dirac-like plasmas.

Photoinduced electron transfer and persistent spectral hole-burning in natural emerald.

Science.gov (United States)

Riesen, Hans

2011-06-02

Wavelength-selective excited-state lifetime measurements and absorption, luminescence, and hole-burning spectra of a natural African emerald crystal are reported. The (2)E excited-state lifetime displays an extreme wavelength dependence, varying from 190 to 37 μs within 1.8 nm of the R(1)-line. Overall, the excited state is strongly quenched, in comparison to laboratory-created emerald (τ=1.3 ms), with an average quenching rate of ∼6 × 10(3) s(-1) at 2.5 K. This quenching is attributed to photoinduced electron transfer caused by a relatively high concentration of Fe(2+) ions. The forward electron-transfer rate, k(f), from the nearest possible Fe(2+) sites at around 5 Å is estimated to be ∼20 × 10(3) s(-1) at 2.5 K. The photoreductive quenching of the excited Cr(3+) ions by Fe(2+) is followed by rapid electron back-transfer in the ground state upon deactivation. The exchange interaction based quenching can be modeled by assuming a random quencher distribution within the possible Fe(2+) sites with the forward electron-transfer rate, k(f), given as a function of acceptor-donor separation R by exp[(R(f)-R)/a(f)]; R(f) and a(f) values of 13.5 and 2.7 Å are obtained at 2.5 K. The electron transfer/back-transfer reorganizes the local crystal lattice, occasionally leading to a minor variation of the short-range structure around the Cr(3+) ions. This provides a mechanism for spectral hole-burning for which a moderately high quantum efficiency of about ∼0.005% is observed. Spectral holes are subject to spontaneous hole-filling and spectral diffusion, and both effects can be quantified within the standard two-level systems for non-photochemical hole-burning. Importantly, the absorbance increases on both sides of broad spectral holes, and isosbestic points are observed, in accord with the expected distribution of the "photoproduct" in a non-photochemical hole-burning process. © 2011 American Chemical Society

Deriving the coronal hole electron temperature: electron density dependent ionization / recombination considerations

International Nuclear Information System (INIS)

Doyle, John Gerard; Perez-Suarez, David; Singh, Avninda; Chapman, Steven; Bryans, Paul; Summers, Hugh; Savin, Daniel Wolf

2010-01-01

Comparison of appropriate theoretically derived line ratios with observational data can yield estimates of a plasma's physical parameters, such as electron density or temperature. The usual practice in the calculation of the line ratio is the assumption of excitation by electrons/protons followed by radiative decay. Furthermore, it is normal to use the so-called coronal approximation, i.e. one only considers ionization and recombination to and from the ground-state. A more accurate treatment is to include ionization/recombination to and from metastable levels. Here, we apply this to two lines from adjacent ionization stages, Mg IX 368 A and Mg X 625 A, which has been shown to be a very useful temperature diagnostic. At densities typical of coronal hole conditions, the difference between the electron temperature derived assuming the zero density limit compared with the electron density dependent ionization/recombination is small. This, however, is not the case for flares where the electron density is orders of magnitude larger. The derived temperature for the coronal hole at solar maximum is around 1.04 MK compared to just below 0.82 MK at solar minimum.

Giant electron-hole transport asymmetry in ultra-short quantum transistors

Science.gov (United States)

McRae, A. C.; Tayari, V.; Porter, J. M.; Champagne, A. R.

2017-01-01

Making use of bipolar transport in single-wall carbon nanotube quantum transistors would permit a single device to operate as both a quantum dot and a ballistic conductor or as two quantum dots with different charging energies. Here we report ultra-clean 10 to 100 nm scale suspended nanotube transistors with a large electron-hole transport asymmetry. The devices consist of naked nanotube channels contacted with sections of tube under annealed gold. The annealed gold acts as an n-doping top gate, allowing coherent quantum transport, and can create nanometre-sharp barriers. These tunnel barriers define a single quantum dot whose charging energies to add an electron or a hole are vastly different (e−h charging energy asymmetry). We parameterize the e−h transport asymmetry by the ratio of the hole and electron charging energies ηe−h. This asymmetry is maximized for short channels and small band gap tubes. In a small band gap device, we demonstrate the fabrication of a dual functionality quantum device acting as a quantum dot for holes and a much longer quantum bus for electrons. In a 14 nm-long channel, ηe−h reaches up to 2.6 for a device with a band gap of 270 meV. The charging energies in this device exceed 100 meV. PMID:28561024

Electronic properties of electron and hole in type-II semiconductor nano-heterostructures

Science.gov (United States)

Rahul, K. Suseel; Souparnika, C.; Salini, K.; Mathew, Vincent

2016-05-01

In this project, we record the orbitals of electron and hole in type-II (CdTe/CdSe/CdTe/CdSe) semiconductor nanocrystal using effective mass approximation. In type-II the band edges of both valance and conduction band are higher than that of shell. So the electron and hole get confined in different layers of the hetero-structure. The energy eigen values and eigen functions are calculated by solving Schrodinger equation using finite difference matrix method. Based on this we investigate the effect of shell thickness and well width on energy and probability distribution of ground state (1s) and few excited states (1p,1d,etc). Our results predict that, type-II quantum dots have significant importance in photovoltaic applications.

Electronic properties of electron and hole in type-II semiconductor nano-heterostructures

Energy Technology Data Exchange (ETDEWEB)

Rahul, K. Suseel [Department of Physics, Central University of Kerala, Riverside Transit Campus, Kasaragod, Kerala. India (India); Department of Physics, Sri Vyasa NSS College, Wadakkancheri, Thrissur, Kerala, PIN:680623. India (India); Souparnika, C. [Department of Physics, Sri Vyasa NSS College, Wadakkancheri, Thrissur, Kerala, PIN:680623. India (India); Salini, K.; Mathew, Vincent, E-mail: vincent@cukerala.ac.in [Department of Physics, Central University of Kerala, Riverside Transit Campus, Kasaragod, Kerala. India (India)

2016-05-06

In this project, we record the orbitals of electron and hole in type-II (CdTe/CdSe/CdTe/CdSe) semiconductor nanocrystal using effective mass approximation. In type-II the band edges of both valance and conduction band are higher than that of shell. So the electron and hole get confined in different layers of the hetero-structure. The energy eigen values and eigen functions are calculated by solving Schrodinger equation using finite difference matrix method. Based on this we investigate the effect of shell thickness and well width on energy and probability distribution of ground state (1s) and few excited states (1p,1d,etc). Our results predict that, type-II quantum dots have significant importance in photovoltaic applications.

Laser plasma as a source of intense attosecond pulses via high-order harmonic generation

International Nuclear Information System (INIS)

Ozaki, T.

2013-01-01

The incredible progress in ultrafast laser technology and Ti:sapphire lasers have lead to many important applications, one of them being high-order harmonic generation (HHG). HHG is a source of coherent extreme ultraviolet (XUV) radiation, which has opened new frontiers in science by extending nonlinear optics and time-resolved spectroscopy to the XUV region, and pushing ultrafast science to the attosecond domain. Progress in attosecond science has revealed many new phenomena that have not been seen with femtosecond pulses. Clearly, the next frontier is to study nonlinear effects at the attosecond timescale and in the XUV. However, a problem with present-day attosecond pulses is that they are just too weak to induce measurable nonlinearities, which severely limits the application of this source. While HHG from solid targets has shown promise for higher conversion efficiency, there is no experiment so far that demonstrates isolated attosecond pulse generation. The generation of isolated, several 100-as pulses with few-µJ energy will enable us to enter a completely new phase in attoscience. In past works, we have demonstrated that high-order harmonics from lowly ionized plasma is a highly efficient method to generate coherent XUV pulses. For example, indium plasma has been shown to generate intense 13th harmonic of the Ti:sapphire laser, with conversion efficiency of 10-4. However, the quasi-monochromatic nature of indium harmonics would make it difficult to generate attosecond pulses. We have also demonstrated that one could increase the harmonic yield by using nanoparticle targets. Specifically, we showed that by using indium oxide nanoparticles or C60 film, we could obtain intense harmonics between wavelengths of 50 to 90 nm. The energy in each of these harmonic orders was measured to be a few µJ, which is sufficient for many applications. However, the problem of using nanoparticle or film targets is the rapid decrease in the harmonic intensity, due to the rapid

Late-time dynamics of rapidly rotating black holes

International Nuclear Information System (INIS)

Glampedakis, K.; Andersson, N.

2001-01-01

We study the late-time behaviour of a dynamically perturbed rapidly rotating black hole. Considering an extreme Kerr black hole, we show that the large number of virtually undamped quasinormal modes (that exist for nonzero values of the azimuthal eigenvalue m) combine in such a way that the field (as observed at infinity) oscillates with an amplitude that decays as 1/t at late times. For a near extreme black hole, these modes, collectively, give rise to an exponentially decaying field which, however, is considerably 'long-lived'. Our analytic results are verified using numerical time-evolutions of the Teukolsky equation. Moreover, we argue that the physical mechanism behind the observed behaviour is the presence of a 'superradiance resonance cavity' immediately outside the black hole. We present this new feature in detail, and discuss whether it may be relevant for astrophysical black holes. (author)

Attosecond relative delay among xenon 5p, 5s, and 4d photoionization

Science.gov (United States)

Magrakvelidze, Maia; Madjet, Mohamed; Chakraborty, Himadri

2017-04-01

Attosecond Wigner-Smith (WS) time delays of the photoemissions of Xe valence 5p, 5s, and core 4d electrons are investigated in details using the time-dependent local density approximation (TDLDA). Electron correlations determine the energy-dependent structures in ionization phases of the dipole channels and in the resulting WS delays at various shape resonances, induced by the collective motion of 4d electrons, and at various Cooper minima. We find that our calculation closely agrees with the streaking measurement for the delay of 4d relative to 5s, and predicts accelerated emission of 5p with respect to 4d as was experimentally observed at similar photon energies for Xe atoms adsorbed on the tungsten surface. This work was supported by the U.S. National Science Foundation.

Nonadiabatic Response Model of Laser-Induced Ultrafast π-Electron Rotations in Chiral Aromatic Molecules

International Nuclear Information System (INIS)

Kanno, Manabu; Kono, Hirohiko; Fujimura, Yuichi; Lin, Sheng H.

2010-01-01

We theoretically investigated the nonadiabatic couplings between optically induced π-electron rotations and molecular vibrations in a chiral aromatic molecule irradiated by a nonhelical, linearly polarized laser pulse. The results of wave packet dynamics simulation show that the vibrational amplitudes strongly depend on the initial rotation direction, clockwise or counterclockwise, which is controlled by the polarization direction of the incident pulse. This suggests that attosecond π-electron rotations can be observed by spectroscopic detection of femtosecond molecular vibrations.

Electron-phonon contribution to the phonon and excited electron (hole) linewidths in bulk Pd

International Nuclear Information System (INIS)

Sklyadneva, I Yu; Leonardo, A; Echenique, P M; Eremeev, S V; Chulkov, E V

2006-01-01

We present an ab initio study of the electron-phonon (e-ph) coupling and its contribution to the phonon linewidths and to the lifetime broadening of excited electron and hole states in bulk Pd. The calculations, based on density-functional theory, were carried out using a linear-response approach in the plane-wave pseudopotential representation. The obtained results for the Eliashberg spectral function α 2 F(ω), e-ph coupling constant λ, and the contribution to the lifetime broadening, Γ e-ph , show strong dependence on both the energy and momentum of an electron (hole) state. The calculation of phonon linewidths gives, in agreement with experimental observations, an anomalously large broadening for the transverse phonon mode T 1 in the Σ direction. In addition, this mode is found to contribute most strongly to the electron-phonon scattering processes on the Fermi surface

Double optical gating

Science.gov (United States)

Gilbertson, Steve

The observation and control of dynamics in atomic and molecular targets requires the use of laser pulses with duration less than the characteristic timescale of the process which is to be manipulated. For electron dynamics, this time scale is on the order of attoseconds where 1 attosecond = 10 -18 seconds. In order to generate pulses on this time scale, different gating methods have been proposed. The idea is to extract or "gate" a single pulse from an attosecond pulse train and switch off all the other pulses. While previous methods have had some success, they are very difficult to implement and so far very few labs have access to these unique light sources. The purpose of this work is to introduce a new method, called double optical gating (DOG), and to demonstrate its effectiveness at generating high contrast single isolated attosecond pulses from multi-cycle lasers. First, the method is described in detail and is investigated in the spectral domain. The resulting attosecond pulses produced are then temporally characterized through attosecond streaking. A second method of gating, called generalized double optical gating (GDOG), is also introduced. This method allows attosecond pulse generation directly from a carrier-envelope phase un-stabilized laser system for the first time. Next the methods of DOG and GDOG are implemented in attosecond applications like high flux pulses and extreme broadband spectrum generation. Finally, the attosecond pulses themselves are used in experiments. First, an attosecond/femtosecond cross correlation is used for characterization of spatial and temporal properties of femtosecond pulses. Then, an attosecond pump, femtosecond probe experiment is conducted to observe and control electron dynamics in helium for the first time.

Attosecond Electron Processes in Materials: Excitons, Plasmons, and Charge Dynamics

Science.gov (United States)

2015-05-19

focused using a f=1.5 m lens into a 250 micron hollow core fiber (HCF) filled with neon gas at atmospheric pressure to stretch the pulse spectrum from... insulator to metal transition. Introduction: The goal of this work was to understand the generation, transport, and manipulation of electronic charge...chemically sensitive probe pulse utilizing specific core level transitions in atoms that are part of a material under study. The measurements follow

Direct Observation of Electron-to-Hole Energy Transfer in CdSe Quantum Dots

NARCIS (Netherlands)

Hendry, E.; Koeberg, M.; Wang, F.; Zhang, H.; de Mello Donega, C.; Vanmaekelbergh, D.; Bonn, M.

2006-01-01

We independently determine the subpicosecond cooling rates for holes and electrons in CdSe quantum dots. Time-resolved luminescence and terahertz spectroscopy reveal that the rate of hole cooling, following photoexcitation of the quantum dots, depends critically on the electron excess energy. This

Thermal radiation and nonthermal radiation of the slowly changing dynamic Kerr–Newman black hole

International Nuclear Information System (INIS)

Meng Qingmiao; Wang Shuai; Jiang Jijian; Deng Deli

2008-01-01

Using the related formula of dynamic black hole, we have calculated the instantaneous radiation energy density of the slowly changing dynamic Kerr–Newman black hole. It is found that the instantaneous radiation energy density of a black hole is always proportional to the quartic of the temperature of the event horizon in the same direction. By using the Hamilton–Jacobin equation of scalar particles in the curved spacetime, the spontaneous radiation of the slowly changing dynamic Kerr–Newman black hole is studied. The energy condition for the occurrence of the spontaneous radiation is obtained. (general)

Balancing Hole and Electron Conduction in Ambipolar Split-Gate Thin-Film Transistors.

Science.gov (United States)

Yoo, Hocheon; Ghittorelli, Matteo; Lee, Dong-Kyu; Smits, Edsger C P; Gelinck, Gerwin H; Ahn, Hyungju; Lee, Han-Koo; Torricelli, Fabrizio; Kim, Jae-Joon

2017-07-10

Complementary organic electronics is a key enabling technology for the development of new applications including smart ubiquitous sensors, wearable electronics, and healthcare devices. High-performance, high-functionality and reliable complementary circuits require n- and p-type thin-film transistors with balanced characteristics. Recent advancements in ambipolar organic transistors in terms of semiconductor and device engineering demonstrate the great potential of this route but, unfortunately, the actual development of ambipolar organic complementary electronics is currently hampered by the uneven electron (n-type) and hole (p-type) conduction in ambipolar organic transistors. Here we show ambipolar organic thin-film transistors with balanced n-type and p-type operation. By manipulating air exposure and vacuum annealing conditions, we show that well-balanced electron and hole transport properties can be easily obtained. The method is used to control hole and electron conductions in split-gate transistors based on a solution-processed donor-acceptor semiconducting polymer. Complementary logic inverters with balanced charging and discharging characteristics are demonstrated. These findings may open up new opportunities for the rational design of complementary electronics based on ambipolar organic transistors.

Massive Black Hole Binaries: Dynamical Evolution and Observational Signatures

Directory of Open Access Journals (Sweden)

M. Dotti

2012-01-01

Full Text Available The study of the dynamical evolution of massive black hole pairs in mergers is crucial in the context of a hierarchical galaxy formation scenario. The timescales for the formation and the coalescence of black hole binaries are still poorly constrained, resulting in large uncertainties in the expected rate of massive black hole binaries detectable in the electromagnetic and gravitational wave spectra. Here, we review the current theoretical understanding of the black hole pairing in galaxy mergers, with a particular attention to recent developments and open issues. We conclude with a review of the expected observational signatures of massive binaries and of the candidates discussed in literature to date.

Plasma phase transition in dense hydrogen and electron-hole plasmas

CERN Document Server

Filinov, V S; Levashov, P R; Fortov, V E; Ebeling, W; Schlanges, M; Koch, S W

2003-01-01

Plasma phase transitions in dense hydrogen and electron-hole plasmas are investigated by direct path integral Monte Carlo methods. The phase boundary of the electron-hole liquid in germanium is calculated and is found to agree reasonably well with the known experimental results. Analogous behaviour is found for high-density hydrogen. For a temperature of T = 10 000 K it is shown that the internal energy is lowered due to droplet formation for densities between 10 sup 2 sup 3 cm sup - sup 3 and 10 sup 2 sup 4 cm sup - sup 3.

Dynamics at Solid State Surfaces and Interfaces, Volume 1 Current Developments

CERN Document Server

Bovensiepen, Uwe; Wolf, Martin

2010-01-01

This two-volume work covers ultrafast structural and electronic dynamics of elementary processes at solid surfaces and interfaces, presenting the current status of photoinduced processes. Providing valuable introductory information for newcomers to this booming field of research, it investigates concepts and experiments, femtosecond and attosecond time-resolved methods, as well as frequency domain techniques. The whole is rounded off by a look at future developments.

Quantum simulations of small electron-hole complexes

International Nuclear Information System (INIS)

Lee, M.A.; Kalia, R.K.; Vashishta, P.D.

1984-09-01

The Green's Function Monte Carlo method is applied to the calculation of the binding energies of electron-hole complexes in semiconductors. The quantum simulation method allows the unambiguous determination of the ground state energy and the effects of band anisotropy on the binding energy. 22 refs., 1 fig

Computational Benchmarking for Ultrafast Electron Dynamics: Wave Function Methods vs Density Functional Theory.

Science.gov (United States)

Oliveira, Micael J T; Mignolet, Benoit; Kus, Tomasz; Papadopoulos, Theodoros A; Remacle, F; Verstraete, Matthieu J

2015-05-12

Attosecond electron dynamics in small- and medium-sized molecules, induced by an ultrashort strong optical pulse, is studied computationally for a frozen nuclear geometry. The importance of exchange and correlation effects on the nonequilibrium electron dynamics induced by the interaction of the molecule with the strong optical pulse is analyzed by comparing the solution of the time-dependent Schrödinger equation based on the correlated field-free stationary electronic states computed with the equationof-motion coupled cluster singles and doubles and the complete active space multi-configurational self-consistent field methodologies on one hand, and various functionals in real-time time-dependent density functional theory (TDDFT) on the other. We aim to evaluate the performance of the latter approach, which is very widely used for nonlinear absorption processes and whose computational cost has a more favorable scaling with the system size. We focus on LiH as a toy model for a nontrivial molecule and show that our conclusions carry over to larger molecules, exemplified by ABCU (C10H19N). The molecules are probed with IR and UV pulses whose intensities are not strong enough to significantly ionize the system. By comparing the evolution of the time-dependent field-free electronic dipole moment, as well as its Fourier power spectrum, we show that TD-DFT performs qualitatively well in most cases. Contrary to previous studies, we find almost no changes in the TD-DFT excitation energies when excited states are populated. Transitions between states of different symmetries are induced using pulses polarized in different directions. We observe that the performance of TD-DFT does not depend on the symmetry of the states involved in the transition.

Fermi-edge superfluorescence from a quantum-degenerate electron-hole gas

Science.gov (United States)

Kim, Ji-Hee; , G. Timothy Noe, II; McGill, Stephen A.; Wang, Yongrui; Wójcik, Aleksander K.; Belyanin, Alexey A.; Kono, Junichiro

2013-11-01

Nonequilibrium can be a source of order. This rather counterintuitive statement has been proven to be true through a variety of fluctuation-driven, self-organization behaviors exhibited by out-of-equilibrium, many-body systems in nature (physical, chemical, and biological), resulting in the spontaneous appearance of macroscopic coherence. Here, we report on the observation of spontaneous bursts of coherent radiation from a quantum-degenerate gas of nonequilibrium electron-hole pairs in semiconductor quantum wells. Unlike typical spontaneous emission from semiconductors, which occurs at the band edge, the observed emission occurs at the quasi-Fermi edge of the carrier distribution. As the carriers are consumed by recombination, the quasi-Fermi energy goes down toward the band edge, and we observe a continuously red-shifting streak. We interpret this emission as cooperative spontaneous recombination of electron-hole pairs, or superfluorescence (SF), which is enhanced by Coulomb interactions near the Fermi edge. This novel many-body enhancement allows the magnitude of the spontaneously developed macroscopic polarization to exceed the maximum value for ordinary SF, making electron-hole SF even more ``super'' than atomic SF.

Interacting Electrons and Holes in Quasi-2D Quantum Dots in Strong Magnetic Fields

Science.gov (United States)

Hawrylak, P.; Sheng, W.; Cheng, S.-J.

2004-09-01

Theory of optical properties of interacting electrons and holes in quasi-2D quantum dots in strong magnetic fields is discussed. In two dimensions and the lowest Landau level, hidden symmetries control the interaction of the interacting system with light. By confining electrons and holes into quantum dots hidden symmetries can be removed and the excitation spectrum of electrons and excitons can be observed. We discuss a theory electronic and of excitonic quantum Hall droplets at a filling factorν=2. For an excitonic quantum Hall droplet the characteristic emission spectra are predicted to be related to the total spin of electron and hole configurations. For the electronic droplet the excitation spectrum of the droplet can be mapped out by measuring the emission for increasing number of electrons.

Interacting electrons and holes in quasi-2D quantum dots in strong magnetic fields

International Nuclear Information System (INIS)

Hawrylak, P.; Sheng, W.; Cheng, S.-J.

2004-01-01

Theory of optical properties of interacting electrons and holes in quasi-2D quantum dots in strong magnetic fields is discussed. In two dimensions and the lowest Landau level, hidden symmetries control the interaction of the interacting system with light. By confining electrons and holes into quantum dots hidden symmetries can be removed and the excitation spectrum of electrons and excitons can be observed. We discuss a theory electronic and excitonic quantum Hall droplets at a filling factor υ = 2. For an excitonic quantum Hall droplet the characteristic emission spectra are predicted to be related to the total spin of electron and hole configurations. For the electronic droplet the excitation spectrum of the droplet can be mapped out by measuring the emission for increasing number of electrons. (author)

Attosecond physics at the nanoscale

Czech Academy of Sciences Publication Activity Database

Ciappina, Marcelo F.; Perez-Hernandez, J.A.; Landsman, A.S.; Okell, W.A.; Zherebtsov, S.; Foerg, B.; Schoetz, J.; Seiffert, L.; Fennel, T.; Shaaran, T.; Zimmermann, T.; Chacon, A.; Guichard, R.; Zair, A.; Tisch, J.W.G.; Marangos, J.P.; Witting, T.; Braun, A.; Maier, S. A.; Roso, L.; Krueger, M.; Hommelhoff, P.; Kling, M.F.; Krausz, F.; Lewenstein, M.

2017-01-01

Roč. 80, č. 5 (2017), 1-50, č. článku 054401. ISSN 0034-4885 R&D Projects: GA MŠk EF15_008/0000162; GA MŠk LQ1606 Grant - others:ELI Beamlines(XE) CZ.02.1.01/0.0/0.0/15_008/0000162 Institutional support: RVO:68378271 Keywords : attosecond physics * plasmonic fields * strong field physics Subject RIV: BH - Optics, Masers, Laser s OBOR OECD: Optics (including laser optics and quantum optics) Impact factor: 14.311, year: 2016

Mesoscopic chaos mediated by Drude electron-hole plasma in silicon optomechanical oscillators

Science.gov (United States)

Wu, Jiagui; Huang, Shu-Wei; Huang, Yongjun; Zhou, Hao; Yang, Jinghui; Liu, Jia-Ming; Yu, Mingbin; Lo, Guoqiang; Kwong, Dim-Lee; Duan, Shukai; Wei Wong, Chee

2017-01-01

Chaos has revolutionized the field of nonlinear science and stimulated foundational studies from neural networks, extreme event statistics, to physics of electron transport. Recent studies in cavity optomechanics provide a new platform to uncover quintessential architectures of chaos generation and the underlying physics. Here, we report the generation of dynamical chaos in silicon-based monolithic optomechanical oscillators, enabled by the strong and coupled nonlinearities of two-photon absorption induced Drude electron–hole plasma. Deterministic chaotic oscillation is achieved, and statistical and entropic characterization quantifies the chaos complexity at 60 fJ intracavity energies. The correlation dimension D2 is determined at 1.67 for the chaotic attractor, along with a maximal Lyapunov exponent rate of about 2.94 times the fundamental optomechanical oscillation for fast adjacent trajectory divergence. Nonlinear dynamical maps demonstrate the subharmonics, bifurcations and stable regimes, along with distinct transitional routes into chaos. This provides a CMOS-compatible and scalable architecture for understanding complex dynamics on the mesoscopic scale. PMID:28598426

Electron-electron correlation in two-photon double ionization of He-like ions

Science.gov (United States)

Hu, S. X.

2018-01-01

Electron correlation plays a crucial role in quantum many-body physics ranging from molecular bonding and strong-field-induced multielectron ionization, to superconducting in materials. Understanding the dynamic electron correlation in the photoionization of relatively simple quantum three-body systems, such as He and He-like ions, is an important step toward manipulating complex systems through photoinduced processes. Here we have performed ab initio investigations of two-photon double ionization (TPDI) of He and He-like ions (L i+,B e2 + , and C4 +) exposed to intense attosecond x-ray pulses. Results from such fully correlated quantum calculations show weaker and weaker electron correlation effects in TPDI spectra as the ionic charge increases, which is opposite to the intuition that the absolute increase of correlation in the ground state should lead to more equal energy sharing in photoionization. These findings indicate that the final-state electron-electron correlation ultimately determines the energy sharing of the two ionized electrons in TPDI.

Atomic and molecular phases through attosecond streaking

DEFF Research Database (Denmark)

Baggesen, Jan Conrad; Madsen, Lars Bojer

2011-01-01

phase of the atomic or molecular ionization matrix elements from the two states through the interference from the two channels. The interference may change the phase of the photoelectron streaking signal within the envelope of the infrared field, an effect to be accounted for when reconstructing short...... pulses from the photoelectron signal and in attosecond time-resolved measurements....

Kinematical vortices in double photoionization of helium by attosecond pulses

Science.gov (United States)

Djiokap, J. M. Ngoko; Meremianin, A. V.; Manakov, N. L.; Hu, S. X.; Madsen, L. B.; Starace, Anthony F.

2017-07-01

Two-armed helical vortex structures are predicted in the two-electron momentum distributions produced in double photoionization (DPI) of the He atom by a pair of time-delayed elliptically polarized attosecond pulses with opposite helicities. These predictions are based upon both a first-order perturbation theory analysis and numerical solutions of the two-electron, time-dependent Schrödinger equation in six spatial dimensions. The helical vortex structures originate from Ramsey interference of a pair of ionized two-electron wave packets, each having a total angular momentum of unity, and appear in the sixfold differential DPI probability distribution for any energy partitioning between the two electrons. The vortex structures are exquisitely sensitive to the time delay between the two pulses, their relative phase, their ellipticity, and their handedness; moreover, they occur in a variety of electron detection geometries. However, the vortex structures only occur when the angular separation β =cos-1(p̂1.p̂2) between the electron momenta p1 and p2 is held fixed. The vortex structures can also be observed in the fourfold differential DPI probability distribution obtained by averaging the sixfold differential probability over the emission angles of one electron. Such kinematical vortices are a general phenomenon that may occur in any ionization process, initiated by two time-delayed short pulses with opposite ellipticities, for particular detection geometries.

Doping Phosphorene with Holes and Electrons through Molecular Charge Transfer.

Science.gov (United States)

Vishnoi, Pratap; Rajesh, S; Manjunatha, S; Bandyopadhyay, Arkamita; Barua, Manaswee; Pati, Swapan K; Rao, C N R

2017-11-03

An important aspect of phosphorene, the novel two-dimensional semiconductor, is whether holes and electrons can both be doped in this material. Some reports found that only electrons can be preferentially doped into phosphorene. There are some theoretical calculations showing charge-transfer interaction with both tetrathiafulvalene (TTF) and tetracyanoethylene (TCNE). We have carried out an investigation of chemical doping of phosphorene by a variety of electron donor and acceptor molecules, employing both experiment and theory, Raman scattering being a crucial aspect of the study. We find that both electron acceptors and donors interact with phosphorene by charge-transfer, with the acceptors having more marked effects. All the three Raman bands of phosphorene soften and exhibit band broadening on interaction with both donor and acceptor molecules. First-principles calculations establish the occurrence of charge-transfer between phosphorene with donors as well as acceptors. The absence of electron-hole asymmetry is noteworthy. © 2017 Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim.

Energy-resolved attosecond interferometric photoemission from Ag(111) and Au(111) surfaces

Science.gov (United States)

Ambrosio, M. J.; Thumm, U.

2018-04-01

Photoelectron emission from solid surfaces induced by attosecond pulse trains into the electric field of delayed phase-coherent infrared (IR) pulses allows the surface-specific observation of energy-resolved electronic phase accumulations and photoemission delays. We quantum-mechanically modeled interferometric photoemission spectra from the (111) surfaces of Au and Ag, including background contributions from secondary electrons and direct emission by the IR pulse, and adjusted parameters of our model to energy-resolved photoelectron spectra recently measured at a synchrotron light source by Roth et al. [J. Electron Spectrosc. 224, 84 (2018), 10.1016/j.elspec.2017.05.008]. Our calculated spectra and photoelectron phase shifts are in fair agreement with the experimental data of Locher et al. [Optica 2, 405 (2015), 10.1364/OPTICA.2.000405]. Our model's not reproducing the measured energy-dependent oscillations of the Ag(111) photoemission phases may be interpreted as evidence for subtle band-structure effects on the final-state photoelectron-surface interaction not accounted for in our simulation.

Dynamically important magnetic fields near accreting supermassive black holes.

Science.gov (United States)

Zamaninasab, M; Clausen-Brown, E; Savolainen, T; Tchekhovskoy, A

2014-06-05

Accreting supermassive black holes at the centres of active galaxies often produce 'jets'--collimated bipolar outflows of relativistic particles. Magnetic fields probably play a critical role in jet formation and in accretion disk physics. A dynamically important magnetic field was recently found near the Galactic Centre black hole. If this is common and if the field continues to near the black hole event horizon, disk structures will be affected, invalidating assumptions made in standard models. Here we report that jet magnetic field and accretion disk luminosity are tightly correlated over seven orders of magnitude for a sample of 76 radio-loud active galaxies. We conclude that the jet-launching regions of these radio-loud galaxies are threaded by dynamically important fields, which will affect the disk properties. These fields obstruct gas infall, compress the accretion disk vertically, slow down the disk rotation by carrying away its angular momentum in an outflow and determine the directionality of jets.

Emulating Molecular Orbitals and Electronic Dynamics with Ultracold Atoms

Directory of Open Access Journals (Sweden)

Dirk-Sören Lühmann

2015-08-01

Full Text Available In recent years, ultracold atoms in optical lattices have proven their great value as quantum simulators for studying strongly correlated phases and complex phenomena in solid-state systems. Here, we reveal their potential as quantum simulators for molecular physics and propose a technique to image the three-dimensional molecular orbitals with high resolution. The outstanding tunability of ultracold atoms in terms of potential and interaction offer fully adjustable model systems for gaining deep insight into the electronic structure of molecules. We study the orbitals of an artificial benzene molecule and discuss the effect of tunable interactions in its conjugated π electron system with special regard to localization and spin order. The dynamical time scales of ultracold atom simulators are on the order of milliseconds, which allows for the time-resolved monitoring of a broad range of dynamical processes. As an example, we compute the hole dynamics in the conjugated π system of the artificial benzene molecule.

Exchange electron-hole interaction of two-dimensional magnetoexcitons under the influence of the Rashba spin-orbit coupling

International Nuclear Information System (INIS)

Moskalenko, S.A.; Podlesny, I.V.; Lelyakov, I.A.; Novikov, B.V.; Kiselyova, E.S.; Gherciu, L.

2011-01-01

The Rashba spin-orbit coupling (RSOC) in the case of two-dimensional (2D) electrons and holes in a strong perpendicular magnetic field was studied. The spinor-type wave functions are characterized by different numbers of Landau levels in different spin projections. For electrons they differ by 1 as was established earlier by Rashba, whereas for holes they differ by 3. Two lowest electron states and four lowest hole states of Landau quantization give rise to eight 2D magnetoexciton states. The exchange electron-hole interaction in the frame of these states is investigated.

Black Holes Versus Firewalls and Thermo-Field Dynamics

Science.gov (United States)

Chowdhury, Borun D.

2013-09-01

In this paper, we examine the implications of the ongoing black holes versus firewalls debate for the thermo-field dynamics of black holes by analyzing a conformal field theory (CFT) in a thermal state in the context of anti-de Sitter/CFT. We argue that the thermo-field doubled copy of the thermal CFT should be thought of not as a fictitious system, but as the image of the CFT in the heat bath. In case of strong coupling between the CFT and the heat bath, this image allows for free infall through the horizon and the system is described by a black hole. Conversely, firewalls are the appropriate dual description in case of weak interaction of the CFT with its heat bath.

Coulomb drag in electron-hole bilayer: Mass-asymmetry and exchange correlation effects

Science.gov (United States)

Arora, Priya; Singh, Gurvinder; Moudgil, R. K.

2018-04-01

Motivated by a recent experiment by Zheng et al. [App. Phys. Lett. 108, 062102 (2016)] on coulomb drag in electron-hole and hole-hole bilayers based on GaAs/AlGaAs semiconductor heterostructure, we investigate theoretically the influence of mass-asymmetry and temperature-dependence of correlations on the drag rate. The correlation effects are dealt with using the Vignale-Singwi effective inter-layer interaction model which includes correlations through local-field corrections to the bare coulomb interactions. However, in this work, we have incorporated only the intra-layer correlations using the temperature-dependent Hubbard approximation. Our results display a reasonably good agreement with the experimental data. However, it is crucial to include both the electron-hole mass-asymmetry and temperature-dependence of correlations. Mass-asymmetry and correlations are found to result in a substantial enhancement of drag resistivity.

High-speed nanoscale characterization of dewetting via dynamic transmission electron microscopy

International Nuclear Information System (INIS)

Hihath, Sahar; Santala, Melissa K.; Campbell, Geoffrey; Benthem, Klaus van

2016-01-01

The dewetting of thin films can occur in either the solid or the liquid state for which different mass transport mechanisms are expected to control morphological changes. Traditionally, dewetting dynamics have been examined on time scales between several seconds to hours, and length scales ranging between nanometers and millimeters. The determination of mass transport mechanisms on the nanoscale, however, requires nanoscale spatial resolution and much shorter time scales. This study reports the high-speed observation of dewetting phenomena for kinetically constrained Ni thin films on crystalline SrTiO_3 substrates. Movie-mode Dynamic Transmission Electron Microscopy (DTEM) was used for high-speed image acquisition during thin film dewetting at different temperatures. DTEM imaging confirmed that the initial stages of film agglomeration include edge retraction, hole formation, and growth. Finite element modeling was used to simulate temperature distributions within the DTEM samples after laser irradiation with different energies. For pulsed laser irradiation at 18 μJ, experimentally observed hole growth suggests that Marangoni flow dominates hole formation in the liquid nickel film. After irradiation with 13.8 μJ, however, the observations suggest that dewetting was initiated by nucleation of voids followed by hole growth through solid-state surface diffusion.

High-speed nanoscale characterization of dewetting via dynamic transmission electron microscopy

Energy Technology Data Exchange (ETDEWEB)

Hihath, Sahar [Department of Materials Science and Engineering, University of California, Davis, 1 Shields Ave., Davis, California 95616 (United States); Department of Physics, University of California, Davis, 1 Shields Ave., Davis, California 95616 (United States); Santala, Melissa K.; Campbell, Geoffrey [Materials Science Division, Lawrence Livermore National Laboratory, 7000 East Ave., Livermore, California 94550 (United States); Benthem, Klaus van, E-mail: benthem@ucdavis.edu [Department of Materials Science and Engineering, University of California, Davis, 1 Shields Ave., Davis, California 95616 (United States)

2016-08-28

The dewetting of thin films can occur in either the solid or the liquid state for which different mass transport mechanisms are expected to control morphological changes. Traditionally, dewetting dynamics have been examined on time scales between several seconds to hours, and length scales ranging between nanometers and millimeters. The determination of mass transport mechanisms on the nanoscale, however, requires nanoscale spatial resolution and much shorter time scales. This study reports the high-speed observation of dewetting phenomena for kinetically constrained Ni thin films on crystalline SrTiO{sub 3} substrates. Movie-mode Dynamic Transmission Electron Microscopy (DTEM) was used for high-speed image acquisition during thin film dewetting at different temperatures. DTEM imaging confirmed that the initial stages of film agglomeration include edge retraction, hole formation, and growth. Finite element modeling was used to simulate temperature distributions within the DTEM samples after laser irradiation with different energies. For pulsed laser irradiation at 18 μJ, experimentally observed hole growth suggests that Marangoni flow dominates hole formation in the liquid nickel film. After irradiation with 13.8 μJ, however, the observations suggest that dewetting was initiated by nucleation of voids followed by hole growth through solid-state surface diffusion.

Timing analysis of two-electron photoemission

International Nuclear Information System (INIS)

Kheifets, A S; Ivanov, I A; Bray, Igor

2011-01-01

We predict a significant delay of two-electron photoemission from the helium atom after absorption of an attosecond XUV pulse. We establish this delay by solving the time-dependent Schroedinger equation and by subsequently tracing the field-free evolution of the two-electron wave packet. This delay can also be related to the energy derivative of the phase of the complex double-photoionization (DPI) amplitude which we evaluate by using the convergent close-coupling method. Our observations indicate that future attosecond time delay measurements on DPI of He can provide information on the absolute quantum phase and elucidate various mechanisms of this strongly correlated ionization process. (fast track communication)

The Dynamical Evolution of Stellar-Mass Black Holes in Dense Star Clusters

Science.gov (United States)

Morscher, Maggie

Globular clusters are gravitationally bound systems containing up to millions of stars, and are found ubiquitously in massive galaxies, including the Milky Way. With densities as high as a million stars per cubic parsec, they are one of the few places in the Universe where stars interact with one another. They therefore provide us with a unique laboratory for studying how gravitational interactions can facilitate the formation of exotic systems, such as X-ray binaries containing black holes, and merging double black hole binaries, which are produced much less efficiently in isolation. While telescopes can provide us with a snapshot of what these dense clusters look like at present, we must rely on detailed numerical simulations to learn about their evolution. These simulations are quite challenging, however, since dense star clusters are described by a complicated set of physical processes occurring on many different length and time scales, including stellar and binary evolution, weak gravitational scattering encounters, strong resonant binary interactions, and tidal stripping by the host galaxy. Until very recently, it was not possible to model the evolution of systems with millions of stars, the actual number contained in the largest clusters, including all the relevant physics required describe these systems accurately. The Northwestern Group's Henon Monte Carlo code, CMC, which has been in development for over a decade, is a powerful tool that can be used to construct detailed evolutionary models of large star clusters. With its recent parallelization, CMC is now capable of addressing a particularly interesting unsolved problem in astrophysics: the dynamical evolution of stellar black holes in dense star clusters. Our current understanding of the stellar initial mass function and massive star evolution suggests that young globular clusters may have formed hundreds to thousands of stellar-mass black holes, the remnants of stars with initial masses from 20 - 100

Excitons formed from spatially separated electrons and holes in Ge/Si geterostructures with Ge quantum dots

International Nuclear Information System (INIS)

Pokutnyj, S.I.

2016-01-01

The effect of a significant increase in the exciton binding energy of space-separated electrons and holes (hole moves in the volume of the quantum dot, and the electron is localized on a spherical surface section quantum dot-matrix) in nanosystems containing germanium quantum dots grown in a matrix of silicon by compared with the binding energy of an exciton in a silicon single crystal. It was found that in such nanosystems in the conduction band silicon matrix is first a zone of states of electron-hole pairs, which with increasing radius of the quantum dot becomes a zone of exciton states, located in the band gap of silicon matrix. It is shown that the mechanism of light absorption in nanosystems due to transitions between quantum-electron levels of the electron-hole pairs, as well as the electron transitions between quantum-exciton levels.

Observation of hole accumulation in Ge/Si core/shell nanowires using off-axis electron holography.

Science.gov (United States)

Li, Luying; Smith, David J; Dailey, Eric; Madras, Prashanth; Drucker, Jeff; McCartney, Martha R

2011-02-09

Hole accumulation in Ge/Si core/shell nanowires (NWs) has been observed and quantified using off-axis electron holography and other electron microscopy techniques. The epitaxial [110]-oriented Ge/Si core/shell NWs were grown on Si (111) substrates by chemical vapor deposition through the vapor-liquid-solid growth mechanism. High-angle annular-dark-field scanning transmission electron microscopy images and off-axis electron holograms were obtained from specific NWs. The excess phase shifts measured by electron holography across the NWs indicated the presence of holes inside the Ge cores. Calculations based on a simplified coaxial cylindrical model gave hole densities of (0.4 ± 0.2) /nm(3) in the core regions.

Electron-Hole Asymmetry of Spin Injection and Transport in Single-Layer Graphene

OpenAIRE

Han, Wei; Wang, W. H.; Pi, K.; McCreary, K. M.; Bao, W.; Li, Yan; Miao, F.; Lau, C. N.; Kawakami, R. K.

2009-01-01

Spin-dependent properties of single-layer graphene (SLG) have been studied by non-local spin valve measurements at room temperature. Gate voltage dependence shows that the non-local magnetoresistance (MR) is proportional to the conductivity of the SLG, which is the predicted behavior for transparent ferromagnetic/nonmagnetic contacts. While the electron and hole bands in SLG are symmetric, gate voltage and bias dependence of the non-local MR reveal an electron-hole asymmetry in which the non-...

Investigation of novel shape-controlled linearly and circularly polarized attosecond pulse sources

International Nuclear Information System (INIS)

Tóth, György; Tibai, Zoltán; Nagy-Csiha, Zsuzsanna; Márton, Zsuzsanna; Almási, Gábor; Hebling, János

2016-01-01

In this article, we investigate the temporal shape of one- or few-cycle, 20–180 nm central wavelength attosecond pulses that are produced in a scheme based on coherent undulator radiation. It is demonstrated, that the carrier–envelope phase (CEP) of the radiated electric field can be chosen arbitrarily by shaping the magnetic field of the radiator undulator appropriately. It is shown that the temporal shape and the spectrum of the generated electric field are influenced by the spatial shape and amplitude of the magnetic field of the radiator undulator for different central wavelength pulses, while both are practically independent of the energy of the initial electron bunch. Shape distortions at high K undulator parameters are also discussed.

Investigation of novel shape-controlled linearly and circularly polarized attosecond pulse sources

Energy Technology Data Exchange (ETDEWEB)

Tóth, György [MTA-PTE High-Field Terahertz Research Group, 7624 Pécs (Hungary); Tibai, Zoltán; Nagy-Csiha, Zsuzsanna [Institute of Physics, University of Pécs, 7624 Pécs (Hungary); Márton, Zsuzsanna [MTA-PTE High-Field Terahertz Research Group, 7624 Pécs (Hungary); Institute of Physics, University of Pécs, 7624 Pécs (Hungary); Almási, Gábor; Hebling, János [MTA-PTE High-Field Terahertz Research Group, 7624 Pécs (Hungary); Institute of Physics, University of Pécs, 7624 Pécs (Hungary); Szentágothai Research Centre, 7624 Pécs (Hungary)

2016-02-15

In this article, we investigate the temporal shape of one- or few-cycle, 20–180 nm central wavelength attosecond pulses that are produced in a scheme based on coherent undulator radiation. It is demonstrated, that the carrier–envelope phase (CEP) of the radiated electric field can be chosen arbitrarily by shaping the magnetic field of the radiator undulator appropriately. It is shown that the temporal shape and the spectrum of the generated electric field are influenced by the spatial shape and amplitude of the magnetic field of the radiator undulator for different central wavelength pulses, while both are practically independent of the energy of the initial electron bunch. Shape distortions at high K undulator parameters are also discussed.

Lewis Base Passivation of Hybrid Halide Perovskites Slows Electron-Hole Recombination: Time-Domain Ab Initio Analysis.

Science.gov (United States)

Liu, Lihong; Fang, Wei-Hai; Long, Run; Prezhdo, Oleg V

2018-03-01

Nonradiative electron-hole recombination plays a key role in determining photon conversion efficiencies in solar cells. Experiments demonstrate significant reduction in the recombination rate upon passivation of methylammonium lead iodide perovskite with Lewis base molecules. Using nonadiabatic molecular dynamics combined with time-domain density functional theory, we find that the nonradiative charge recombination is decelerated by an order of magnitude upon adsorption of the molecules. Thiophene acts by the traditional passivation mechanism, forcing electron density away from the surface. In contrast, pyridine localizes the electron at the surface while leaving it energetically near the conduction band edge. This is because pyridine creates a stronger coordinative bond with a lead atom of the perovskite and has a lower energy unoccupied orbital compared with thiophene due to the more electronegative nitrogen atom relative to thiophene's sulfur. Both molecules reduce two-fold the nonadiabatic coupling and electronic coherence time. A broad range of vibrational modes couple to the electronic subsystem, arising from inorganic and organic components. The simulations reveal the atomistic mechanisms underlying the enhancement of the excited-state lifetime achieved by the perovskite passivation, rationalize the experimental results, and advance our understanding of charge-phonon dynamics in perovskite solar cells.

Electrostatics of electron-hole interactions in van der Waals heterostructures

Science.gov (United States)

Cavalcante, L. S. R.; Chaves, A.; Van Duppen, B.; Peeters, F. M.; Reichman, D. R.

2018-03-01

The role of dielectric screening of electron-hole interaction in van der Waals heterostructures is theoretically investigated. A comparison between models available in the literature for describing these interactions is made and the limitations of these approaches are discussed. A simple numerical solution of Poisson's equation for a stack of dielectric slabs based on a transfer matrix method is developed, enabling the calculation of the electron-hole interaction potential at very low computational cost and with reasonable accuracy. Using different potential models, direct and indirect exciton binding energies in these systems are calculated within Wannier-Mott theory, and a comparison of theoretical results with recent experiments on excitons in two-dimensional materials is discussed.

Generation of an isolated sub-30 attosecond pulse in a two-color laser field and a static electric field

International Nuclear Information System (INIS)

Zhang Gang-Tai; Zhang Mei-Guang; Bai Ting-Ting

2012-01-01

We theoretically investigate high-order harmonic generation (HHG) from a helium ion model in a two-color laser field, which is synthesized by a fundamental pulse and its second harmonic pulse. It is shown that a supercontinuum spectrum can be generated in the two-color field. However, the spectral intensity is very low, limiting the application of the generated attosecond (as) pulse. By adding a static electric field to the synthesized two-color field, not only is the ionization yield of electrons contributing to the harmonic emission remarkably increased, but also the quantum paths of the HHG can be significantly modulated. As a result, the extension and enhancement of the supercontinuum spectrum are achieved, producing an intense isolated 26-as pulse with a bandwidth of about 170.5 eV. In particular, we also analyse the influence of the laser parameters on the ultrabroad supercontinuum spectrum and isolated sub-30-as pulse generation. (electromagnetism, optics, acoustics, heat transfer, classical mechanics, and fluid dynamics)

Laser control of electron matter waves

NARCIS (Netherlands)

Jones, E.; Becker, M.; Luiten, O.J.; Batelaan, H.

2016-01-01

In recent years laser light has been used to control the motion of electron waves. Electrons can now be diffracted by standing waves of light. Laser light in the vicinity of nanostructures is used to affect free electrons, for example, femto-second and atto-second laser-induced electrons are emitted

Ultrafast Electron Dynamics in Solar Energy Conversion.

Science.gov (United States)

Ponseca, Carlito S; Chábera, Pavel; Uhlig, Jens; Persson, Petter; Sundström, Villy

2017-08-23

Electrons are the workhorses of solar energy conversion. Conversion of the energy of light to electricity in photovoltaics, or to energy-rich molecules (solar fuel) through photocatalytic processes, invariably starts with photoinduced generation of energy-rich electrons. The harvesting of these electrons in practical devices rests on a series of electron transfer processes whose dynamics and efficiencies determine the function of materials and devices. To capture the energy of a photogenerated electron-hole pair in a solar cell material, charges of opposite sign have to be separated against electrostatic attractions, prevented from recombining and being transported through the active material to electrodes where they can be extracted. In photocatalytic solar fuel production, these electron processes are coupled to chemical reactions leading to storage of the energy of light in chemical bonds. With the focus on the ultrafast time scale, we here discuss the light-induced electron processes underlying the function of several molecular and hybrid materials currently under development for solar energy applications in dye or quantum dot-sensitized solar cells, polymer-fullerene polymer solar cells, organometal halide perovskite solar cells, and finally some photocatalytic systems.

Harvesting multiple electron-hole pairs generated through plasmonic excitation of Au nanoparticles.

Science.gov (United States)

Kim, Youngsoo; Smith, Jeremy G; Jain, Prashant K

2018-05-07

Multi-electron redox reactions, although central to artificial photosynthesis, are kinetically sluggish. Amidst the search for synthetic catalysts for such processes, plasmonic nanoparticles have been found to catalyse multi-electron reduction of CO 2 under visible light. This example motivates the need for a general, insight-driven framework for plasmonic catalysis of such multi-electron chemistry. Here, we elucidate the principles underlying the extraction of multiple redox equivalents from a plasmonic photocatalyst. We measure the kinetics of electron harvesting from a gold nanoparticle photocatalyst as a function of photon flux. Our measurements, supported by theoretical modelling, reveal a regime where two-electron transfer from the excited gold nanoparticle becomes prevalent. Multiple electron harvesting becomes possible under continuous-wave, visible-light excitation of moderate intensity due to strong interband transitions in gold and electron-hole separation accomplished using a hole scavenger. These insights will help expand the utility of plasmonic photocatalysis beyond CO 2 reduction to other challenging multi-electron, multi-proton transformations such as N 2 fixation.

Delayed electron emission in strong-field driven tunnelling from a metallic nanotip in the multi-electron regime

Science.gov (United States)

Yanagisawa, Hirofumi; Schnepp, Sascha; Hafner, Christian; Hengsberger, Matthias; Kim, Dong Eon; Kling, Matthias F.; Landsman, Alexandra; Gallmann, Lukas; Osterwalder, Jürg

2016-01-01

Illuminating a nano-sized metallic tip with ultrashort laser pulses leads to the emission of electrons due to multiphoton excitations. As optical fields become stronger, tunnelling emission directly from the Fermi level becomes prevalent. This can generate coherent electron waves in vacuum leading to a variety of attosecond phenomena. Working at high emission currents where multi-electron effects are significant, we were able to characterize the transition from one regime to the other. Specifically, we found that the onset of laser-driven tunnelling emission is heralded by the appearance of a peculiar delayed emission channel. In this channel, the electrons emitted via laser-driven tunnelling emission are driven back into the metal, and some of the electrons reappear in the vacuum with some delay time after undergoing inelastic scattering and cascading processes inside the metal. Our understanding of these processes gives insights on attosecond tunnelling emission from solids and should prove useful in designing new types of pulsed electron sources. PMID:27786287

ACCRETION DISKS AROUND KICKED BLACK HOLES: POST-KICK DYNAMICS

International Nuclear Information System (INIS)

Ponce, Marcelo; Faber, Joshua A.; Lombardi, James C.

2012-01-01

Numerical calculations of merging black hole binaries indicate that asymmetric emission of gravitational radiation can kick the merged black hole at up to thousands of km s –1 , and a number of systems have been observed recently whose properties are consistent with an active galactic nucleus containing a supermassive black hole moving with substantial velocity with respect to its broader accretion disk. We study here the effect of an impulsive kick delivered to a black hole on the dynamical evolution of its accretion disk using a smoothed particle hydrodynamics code, focusing attention on the role played by the kick angle with respect to the orbital angular momentum vector of the pre-kicked disk. We find that for more vertical kicks, for which the angle between the kick and the normal vector to the disk θ ∼ 45°, matter rapidly accretes toward the black hole. There is a systematic trend for higher potential luminosities for more oblique kick angles for a given black hole mass, disk mass, and kick velocity, and we find large amplitude oscillations in time in the case of a kick oriented 60° from the vertical.

Electrogenerated chemiluminescence induced by sequential hot electron and hole injection into aqueous electrolyte solution

Energy Technology Data Exchange (ETDEWEB)

Salminen, Kalle; Kuosmanen, Päivi; Pusa, Matti [Aalto University, Department of Chemistry, Laboratory of Analytical Chemistry, P.O. Box 16100, FI-00076 Aalto (Finland); Kulmala, Oskari [University of Helsinki, Department of Physics, P.O. Box 64, FI-00014 (Finland); Håkansson, Markus [Aalto University, Department of Chemistry, Laboratory of Analytical Chemistry, P.O. Box 16100, FI-00076 Aalto (Finland); Kulmala, Sakari, E-mail: sakari.kulmala@aalto.fi [Aalto University, Department of Chemistry, Laboratory of Analytical Chemistry, P.O. Box 16100, FI-00076 Aalto (Finland)

2016-03-17

Hole injection into aqueous electrolyte solution is proposed to occur when oxide-coated aluminum electrode is anodically pulse-polarized by a voltage pulse train containing sufficiently high-voltage anodic pulses. The effects of anodic pulses are studied by using an aromatic Tb(III) chelate as a probe known to produce intensive hot electron-induced electrochemiluminescence (HECL) with plain cathodic pulses and preoxidized electrodes. The presently studied system allows injection of hot electrons and holes successively into aqueous electrolyte solutions and can be utilized in detecting electrochemiluminescent labels in fully aqueous solutions, and actually, the system is suggested to be quite close to a pulse radiolysis system providing hydrated electrons and hydroxyl radicals as the primary radicals in aqueous solution without the problems and hazards of ionizing radiation. The analytical power of the present excitation waveforms are that they allow detection of electrochemiluminescent labels at very low detection limits in bioaffinity assays such as in immunoassays or DNA probe assays. The two important properties of the present waveforms are: (i) they provide in situ oxidation of the electrode surface resulting in the desired oxide film thickness and (ii) they can provide one-electron oxidants for the system by hole injection either via F- and F{sup +}-center band of the oxide or by direct hole injection to valence band of water at highly anodic pulse amplitudes. - Highlights: • Hot electrons injected into aqueous electrolyte solution. • Generation of hydrated electrons. • Hole injection into aqueous electrolyte solution. • Generation of hydroxyl radicals.

Reemission spectra and inelastic processes at interaction of attosecond and shorter duration electromagnetic pulses with atoms

International Nuclear Information System (INIS)

Makarov, D.N.; Matveev, V.I.

2017-01-01

Inelastic processes and the reemission of attosecond and shorter electromagnetic pulses by atoms have been considered within the analytical solution of the Schrödinger equation in the sudden perturbation approximation. A method of calculations with the exact inclusion of spatial inhomogeneity of the field of an ultrashort pulse and the momenta of photons in the reemission processes has been developed. The probabilities of inelastic processes and spectra of reemission of ultrashort electromagnetic pulses by one- and many-electron atoms have been calculated. The results have been presented in the form of analytical formulas.

Auger electron emission initiated by the creation of valence-band holes in graphene by positron annihilation.

Science.gov (United States)

Chirayath, V A; Callewaert, V; Fairchild, A J; Chrysler, M D; Gladen, R W; Mcdonald, A D; Imam, S K; Shastry, K; Koymen, A R; Saniz, R; Barbiellini, B; Rajeshwar, K; Partoens, B; Weiss, A H

2017-07-13

Auger processes involving the filling of holes in the valence band are thought to make important contributions to the low-energy photoelectron and secondary electron spectrum from many solids. However, measurements of the energy spectrum and the efficiency with which electrons are emitted in this process remain elusive due to a large unrelated background resulting from primary beam-induced secondary electrons. Here, we report the direct measurement of the energy spectra of electrons emitted from single layer graphene as a result of the decay of deep holes in the valence band. These measurements were made possible by eliminating competing backgrounds by employing low-energy positrons (holes by annihilation. Our experimental results, supported by theoretical calculations, indicate that between 80 and 100% of the deep valence-band holes in graphene are filled via an Auger transition.

Desorption by Femtosecond Laser Pulses : An Electron-Hole Effect?

OpenAIRE

D. M., NEWNS; T. F., HEINZ; J. A., MISEWICH; IBM Research Division, T. J. Watson Research Center; IBM Research Division, T. J. Watson Research Center; IBM Research Division, T. J. Watson Research Center

1992-01-01

Desorption of molecules from metal surfaces induced by femtosecond visible laser pulses has been reported. Since the lattice temperature rise is insufficient to explain desorption, an electronic mechanism is clearly responsible. It is shown that a theory based on direct coupling between the center-of-mass degree of freedom of the adsorbate and the electron-hole excitations of the substrate provides a satisfactory explanation of the various experimental findings.

The causal structure of dynamical charged black holes

International Nuclear Information System (INIS)

Hong, Sungwook E; Hwang, Dong-il; Stewart, Ewan D; Yeom, Dong-han

2010-01-01

We study the causal structure of dynamical charged black holes, with a sufficient number of massless fields, using numerical simulations. Neglecting Hawking radiation, the inner horizon is a null Cauchy horizon and a curvature singularity due to mass inflation. When we include Hawking radiation, the inner horizon becomes space-like and is separated from the Cauchy horizon, which is parallel to the out-going null direction. Since a charged black hole must eventually transit to a neutral black hole, we studied the neutralization of the black hole and observed that the inner horizon evolves into a space-like singularity, generating a Cauchy horizon which is parallel to the in-going null direction. Since the mass function is finite around the inner horizon, the inner horizon is regular and penetrable in a general relativistic sense. However, since the curvature functions become trans-Planckian, we cannot say more about the region beyond the inner horizon, and it is natural to say that there is a 'physical' space-like singularity. However, if we assume an exponentially large number of massless scalar fields, our results can be extended beyond the inner horizon. In this case, strong cosmic censorship and black hole complementarity can be violated.

The causal structure of dynamical charged black holes

Energy Technology Data Exchange (ETDEWEB)

Hong, Sungwook E; Hwang, Dong-il; Stewart, Ewan D; Yeom, Dong-han, E-mail: eostm@muon.kaist.ac.k, E-mail: enotsae@gmail.co, E-mail: innocent@muon.kaist.ac.k [Department of Physics, KAIST, Daejeon 305-701 (Korea, Republic of)

2010-02-21

We study the causal structure of dynamical charged black holes, with a sufficient number of massless fields, using numerical simulations. Neglecting Hawking radiation, the inner horizon is a null Cauchy horizon and a curvature singularity due to mass inflation. When we include Hawking radiation, the inner horizon becomes space-like and is separated from the Cauchy horizon, which is parallel to the out-going null direction. Since a charged black hole must eventually transit to a neutral black hole, we studied the neutralization of the black hole and observed that the inner horizon evolves into a space-like singularity, generating a Cauchy horizon which is parallel to the in-going null direction. Since the mass function is finite around the inner horizon, the inner horizon is regular and penetrable in a general relativistic sense. However, since the curvature functions become trans-Planckian, we cannot say more about the region beyond the inner horizon, and it is natural to say that there is a 'physical' space-like singularity. However, if we assume an exponentially large number of massless scalar fields, our results can be extended beyond the inner horizon. In this case, strong cosmic censorship and black hole complementarity can be violated.

Diffusive scattering of electrons by electron holes around injection fronts

Science.gov (United States)

Vasko, I. Y.; Agapitov, O. V.; Mozer, F. S.; Artemyev, A. V.; Krasnoselskikh, V. V.; Bonnell, J. W.

2017-03-01

Van Allen Probes have detected nonlinear electrostatic spikes around injection fronts in the outer radiation belt. These spikes include electron holes (EH), double layers, and more complicated solitary waves. We show that EHs can efficiently scatter electrons due to their substantial transverse electric fields. Although the electron scattering driven by EHs is diffusive, it cannot be evaluated via the standard quasi-linear theory. We derive analytical formulas describing local electron scattering by a single EH and verify them via test particle simulations. We show that the most efficiently scattered are gyroresonant electrons (crossing EH on a time scale comparable to the local electron gyroperiod). We compute bounce-averaged diffusion coefficients and demonstrate their dependence on the EH spatial distribution (latitudinal extent and spatial filling factor) and individual EH parameters (amplitude of electrostatic potential, velocity, and spatial scales). We show that EHs can drive pitch angle scattering of ≲5 keV electrons at rates 10-2-10-4 s-1 and, hence, can contribute to electron losses and conjugated diffuse aurora brightenings. The momentum and pitch angle scattering rates can be comparable, so that EHs can also provide efficient electron heating. The scattering rates driven by EHs at L shells L ˜ 5-8 are comparable to those due to chorus waves and may exceed those due to electron cyclotron harmonics.

Stability of Sarma phases in density imbalanced electron-hole bilayer systems

International Nuclear Information System (INIS)

Subasi, A. L.; Tanatar, B.; Pieri, P.; Senatore, G.

2010-01-01

We study excitonic condensation in an electron-hole bilayer system with unequal layer densities at zero temperature. Using mean-field theory we solve the Bardeen-Cooper-Schrieffer (BCS) gap equations numerically and investigate the effects of intralayer interactions. The electron-hole system evolves from BCS in the weak coupling limit to Bose-Einstein condensation (BEC) in the strong coupling limit. We analyze the stability of the Sarma phase with k,-k pairing by calculating the superfluid mass density and also by checking the compressibility matrix. We find that with bare Coulomb interactions the superfluid density is always positive in the Sarma phase, due to a peculiar momentum structure of the gap function originating from the singular behavior of the Coulomb potential at zero momentum and the presence of a sharp Fermi surface. Introducing a simple model for screening, we find that the superfluid density becomes negative in some regions of the phase diagram, corresponding to an instability toward a Fulde-Ferrel-Larkin-Ovchinnikov-type superfluid phase. Thus, intralayer interaction and screening together can lead to a rich phase diagram in the BCS-BEC crossover regime in electron-hole bilayer systems.

Attosecond Time Delay in Photoionization of Noble-Gas and Halogen Atoms

Directory of Open Access Journals (Sweden)

Liang-Wen Pi

2018-02-01

Full Text Available Ultrafast processes are now accessible on the attosecond time scale due to the availability of ultrashort XUV laser pulses. Noble-gas and halogen atoms remain important targets due to their giant dipole resonance and Cooper minimum. Here, we calculate photoionization cross section, asymmetry parameter and Wigner time delay using the time-dependent local-density approximation (TDLDA, which includes the electron correlation effects. Our results are consistent with experimental data and other theoretical calculations. The asymmetry parameter provides an extra layer of access to the phase information of the photoionization processes. We find that halogen atoms bear a strong resemblance on cross section, asymmetry parameter and time delay to their noble-gas neighbors. Our predicted time delay should provide a guidance for future experiments on those atoms and related molecules.

First Principles Modeling and Interpretation of Ionization-Triggered Charge Migration in Molecules

Science.gov (United States)

Bruner, Adam; Hernandez, Sam; Mauger, Francois; Abanador, Paul; Gaarde, Mette; Schafer, Ken; Lopata, Ken

Modeling attosecond coherent charge migration in molecules is important for understanding initial steps of photochemistry and light harvesting processes. Ionization triggered hole migration can be difficult to characterize and interpret as the dynamics can be convoluted with excited states. Here, we introduce a real-time time-dependent density functional theory (RT-TDDFT) approach for modeling such dynamics from first principles. To isolate the specific hole dynamics from excited states, Fourier transform analysis and orbital occupations are used to provide a spatial hole representation in the frequency domain. These techniques are applied to hole transfer across a thiophene dimer as well as core-hole triggered valence motion in nitrosobenzene. This work was supported by U.S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Award No. DE-SC0012462.

Propagation of an attosecond pulse in a dense two-level medium

International Nuclear Information System (INIS)

Song Xiaohong; Gong Shangqing; Yang Weifeng; Xu Zhizhan

2004-01-01

We investigate the propagation of attosecond pulse in a dense two-level medium by using an iterative predictor-corrector finite-difference time-domain method. We find when attosecond pulse is considered, that the standard area theorem will break down even for small area pulses: ideal self-induced transparency cannot occur even for a 2π pulse, while the pulses whose areas are not integer multiples of 2π, such as 1.8π and 2.2π pulses, cannot evolve to 2π pulses as predicted by the standard area theorem. Significantly higher spectra components can occur on all these small area propagating pulses due to strong carrier reshaping. Furthermore, these higher spectral components dependent sensitively on the pulse area: the larger the pulse area is, the more evident are these higher spectral components

How electronic dynamics with Pauli exclusion produces Fermi-Dirac statistics.

Science.gov (United States)

Nguyen, Triet S; Nanguneri, Ravindra; Parkhill, John

2015-04-07

It is important that any dynamics method approaches the correct population distribution at long times. In this paper, we derive a one-body reduced density matrix dynamics for electrons in energetic contact with a bath. We obtain a remarkable equation of motion which shows that in order to reach equilibrium properly, rates of electron transitions depend on the density matrix. Even though the bath drives the electrons towards a Boltzmann distribution, hole blocking factors in our equation of motion cause the electronic populations to relax to a Fermi-Dirac distribution. These factors are an old concept, but we show how they can be derived with a combination of time-dependent perturbation theory and the extended normal ordering of Mukherjee and Kutzelnigg for a general electronic state. The resulting non-equilibrium kinetic equations generalize the usual Redfield theory to many-electron systems, while ensuring that the orbital occupations remain between zero and one. In numerical applications of our equations, we show that relaxation rates of molecules are not constant because of the blocking effect. Other applications to model atomic chains are also presented which highlight the importance of treating both dephasing and relaxation. Finally, we show how the bath localizes the electron density matrix.

How electronic dynamics with Pauli exclusion produces Fermi-Dirac statistics

International Nuclear Information System (INIS)

Nguyen, Triet S.; Nanguneri, Ravindra; Parkhill, John

2015-01-01

It is important that any dynamics method approaches the correct population distribution at long times. In this paper, we derive a one-body reduced density matrix dynamics for electrons in energetic contact with a bath. We obtain a remarkable equation of motion which shows that in order to reach equilibrium properly, rates of electron transitions depend on the density matrix. Even though the bath drives the electrons towards a Boltzmann distribution, hole blocking factors in our equation of motion cause the electronic populations to relax to a Fermi-Dirac distribution. These factors are an old concept, but we show how they can be derived with a combination of time-dependent perturbation theory and the extended normal ordering of Mukherjee and Kutzelnigg for a general electronic state. The resulting non-equilibrium kinetic equations generalize the usual Redfield theory to many-electron systems, while ensuring that the orbital occupations remain between zero and one. In numerical applications of our equations, we show that relaxation rates of molecules are not constant because of the blocking effect. Other applications to model atomic chains are also presented which highlight the importance of treating both dephasing and relaxation. Finally, we show how the bath localizes the electron density matrix

Probing charge transfer dynamics in self-assembled monolayers by core hole clock approach

International Nuclear Information System (INIS)

Zharnikov, Michael

2015-01-01

This article reviews recent progress in the application of core hole clock approach in the framework of resonant Auger electron spectroscopy to the monomolecular assembles of alkyl, oligophenyl, and oligo(phenylene–ethynylene) based molecules on Au(1 1 1) substrates, referring mostly to the work by the author et al. The major goal was to study electron transfer (ET) dynamics in these systems serving as prototypes of molecular electronics (ME) devices. The ET pathway to the conductive substrate was unambiguously defined by resonant excitation of the nitrile tailgroup attached to the molecular backbone. Characteristic ET times within the femtosecond domain were determined, along with the attenuation factors for the ET dynamics, analogous to the case of the static transport. The above parameters were found to exhibit strong dependence on the character of the molecular orbital which mediates the ET process. In addition, certain spectral features, which can be associated with an inverse ET from the molecular backbone to the excitation site, were observed upon exchange of the nitrile group by strongly electronegative nitro moiety. The reported results represent a valuable input for theory and a certain potential for applications such as ME devices where optimization of ET can have significant technological impact.

Dynamical Formation and Merger of Binary Black Holes

Science.gov (United States)

Stone, Nicholas

2017-01-01

The advent of gravitational wave (GW) astronomy began with Advanced LIGO's 2015 discovery of GWs from coalescing black hole (BH) binaries. GW astronomy holds great promise for testing general relativity, but also for investigating open astrophysical questions not amenable to traditional electromagnetic observations. One such question concerns the origin of stellar mass BH binaries in the universe: do these form primarily from evolution of isolated binaries of massive stars, or do they form through more exotic dynamical channels? The best studied dynamical formation channel involves multibody interactions of BHs and stars in dense globular cluster environments, but many other dynamical scenarios have recently been proposed, ranging from the Kozai effect in hierarchical triple systems to BH binary formation in the outskirts of Toomre-unstable accretion disks surrounding supermassive black holes. The BH binaries formed through these processes will have different distributions of observable parameters (e.g. mass ratios, spins) than BH binaries formed through the evolution of isolated binary stars. In my talk I will overview these and other dynamical formation scenarios, and summarize the key observational tests that will enable Advanced LIGO or other future detectors to determine what formation pathway creates the majority of binary BHs in the universe. NCS thanks NASA, which has funded his work through Einstein postdoctoral grant PF5-160145.

Quantum coherent optical phase modulation in an ultrafast transmission electron microscope.

Science.gov (United States)

Feist, Armin; Echternkamp, Katharina E; Schauss, Jakob; Yalunin, Sergey V; Schäfer, Sascha; Ropers, Claus

2015-05-14

Coherent manipulation of quantum systems with light is expected to be a cornerstone of future information and communication technology, including quantum computation and cryptography. The transfer of an optical phase onto a quantum wavefunction is a defining aspect of coherent interactions and forms the basis of quantum state preparation, synchronization and metrology. Light-phase-modulated electron states near atoms and molecules are essential for the techniques of attosecond science, including the generation of extreme-ultraviolet pulses and orbital tomography. In contrast, the quantum-coherent phase-modulation of energetic free-electron beams has not been demonstrated, although it promises direct access to ultrafast imaging and spectroscopy with tailored electron pulses on the attosecond scale. Here we demonstrate the coherent quantum state manipulation of free-electron populations in an electron microscope beam. We employ the interaction of ultrashort electron pulses with optical near-fields to induce Rabi oscillations in the populations of electron momentum states, observed as a function of the optical driving field. Excellent agreement with the scaling of an equal-Rabi multilevel quantum ladder is obtained, representing the observation of a light-driven 'quantum walk' coherently reshaping electron density in momentum space. We note that, after the interaction, the optically generated superposition of momentum states evolves into a train of attosecond electron pulses. Our results reveal the potential of quantum control for the precision structuring of electron densities, with possible applications ranging from ultrafast electron spectroscopy and microscopy to accelerator science and free-electron lasers.

Exciton and Hole-Transfer Dynamics in Polymer: Fullerene Blends

Directory of Open Access Journals (Sweden)

van Loosdrecht P. H. M.

2013-03-01

Full Text Available Ultrafast hole transfer dynamics from fullerene derivative to polymer in bulk heterojunction blends are studied with visible-pump - IR-probe spectroscopy. The hole transfer process is found to occur in 50/300 fs next to the interface, while a longer 15-ps time is attributed to exciton diffusion towards interface in PC71BM domains. High polaron generation efficiency in P3HT blends indicates excellent intercalation between the polymer and the fullerene even at highest PC71BM concentration thereby yielding a valuable information on the blend morphology.

Plasma dynamics near critical density inferred from direct measurements of laser hole boring

Science.gov (United States)

Gong, Chao; Tochitsky, Sergei Ya.; Fiuza, Frederico; Pigeon, Jeremy J.; Joshi, Chan

2016-06-01

We have used multiframe picosecond optical interferometry to make direct measurements of the hole boring velocity, vHB, of the density cavity pushed forward by a train of C O2 laser pulses in a near critical density helium plasma. As the pulse train intensity rises, the increasing radiation pressure of each pulse pushes the density cavity forward and the plasma electrons are strongly heated. After the peak laser intensity, the plasma pressure exerted by the heated electrons strongly impedes the hole boring process and the vHB falls rapidly as the laser pulse intensity falls at the back of the laser pulse train. A heuristic theory is presented that allows the estimation of the plasma electron temperature from the measurements of the hole boring velocity. The measured values of vHB, and the estimated values of the heated electron temperature as a function of laser intensity are in reasonable agreement with those obtained from two-dimensional numerical simulations.

Direct longitudinal laser acceleration of electrons in free space

Directory of Open Access Journals (Sweden)

Sergio Carbajo

2016-02-01

Full Text Available Compact laser-driven accelerators are pursued heavily worldwide because they make novel methods and tools invented at national laboratories widely accessible in science, health, security, and technology [V. Malka et al., Principles and applications of compact laser-plasma accelerators, Nat. Phys. 4, 447 (2008]. Current leading laser-based accelerator technologies [S. P. D. Mangles et al., Monoenergetic beams of relativistic electrons from intense laser-plasma interactions, Nature (London 431, 535 (2004; T. Toncian et al., Ultrafast laser-driven microlens to focus and energy-select mega-electron volt protons, Science 312, 410 (2006; S. Tokita et al. Single-shot ultrafast electron diffraction with a laser-accelerated sub-MeV electron pulse, Appl. Phys. Lett. 95, 111911 (2009] rely on a medium to assist the light to particle energy transfer. The medium imposes material limitations or may introduce inhomogeneous fields [J. R. Dwyer et al., Femtosecond electron diffraction: “Making the molecular movie,”, Phil. Trans. R. Soc. A 364, 741 (2006]. The advent of few cycle ultraintense radially polarized lasers [S. Carbajo et al., Efficient generation of ultraintense few-cycle radially polarized laser pulses, Opt. Lett. 39, 2487 (2014] has ushered in a novel accelerator concept [L. J. Wong and F. X. Kärtner, Direct acceleration of an electron in infinite vacuum by a pulsed radially polarized laser beam, Opt. Express 18, 25035 (2010; F. Pierre-Louis et al. Direct-field electron acceleration with ultrafast radially polarized laser beams: Scaling laws and optimization, J. Phys. B 43, 025401 (2010; Y. I. Salamin, Electron acceleration from rest in vacuum by an axicon Gaussian laser beam, Phys. Rev. A 73, 043402 (2006; C. Varin and M. Piché, Relativistic attosecond electron pulses from a free-space laser-acceleration scheme, Phys. Rev. E 74, 045602 (2006; A. Sell and F. X. Kärtner, Attosecond electron bunches accelerated and

Helical edge states and fractional quantum Hall effect in a graphene electron-hole bilayer.

Science.gov (United States)

Sanchez-Yamagishi, Javier D; Luo, Jason Y; Young, Andrea F; Hunt, Benjamin M; Watanabe, Kenji; Taniguchi, Takashi; Ashoori, Raymond C; Jarillo-Herrero, Pablo

2017-02-01

Helical 1D electronic systems are a promising route towards realizing circuits of topological quantum states that exhibit non-Abelian statistics. Here, we demonstrate a versatile platform to realize 1D systems made by combining quantum Hall (QH) edge states of opposite chiralities in a graphene electron-hole bilayer at moderate magnetic fields. Using this approach, we engineer helical 1D edge conductors where the counterpropagating modes are localized in separate electron and hole layers by a tunable electric field. These helical conductors exhibit strong non-local transport signals and suppressed backscattering due to the opposite spin polarizations of the counterpropagating modes. Unlike other approaches used for realizing helical states, the graphene electron-hole bilayer can be used to build new 1D systems incorporating fractional edge states. Indeed, we are able to tune the bilayer devices into a regime hosting fractional and integer edge states of opposite chiralities, paving the way towards 1D helical conductors with fractional quantum statistics.

Identification of electron and hole traps in KH2PO4 crystals

International Nuclear Information System (INIS)

Garces, N. Y.; Stevens, K. T.; Halliburton, L. E.; Demos, S. G.; Radousky, H. B.; Zaitseva, N. P.

2001-01-01

Electron paramagnetic resonance (EPR) has been used to characterize a hole trap and several electron traps in single crystals of potassium dihydrogen phosphate (KH 2 PO 4 or KDP). The paramagnetic charge states of these centers are produced by ionizing radiation (e.g., x rays or a 266 nm beam from a pulsed Nd:YAG laser) and are stable for days and even weeks at room temperature. One center consists of a hole trapped on an oxygen ion adjacent to a silicon impurity located on a phosphorus site. This defect has a small, but easily observed, hyperfine interaction with the adjacent substitutional proton. The other centers are formed when an electron is trapped at an oxygen vacancy. These latter defects are best described as (PO 3 ) 2- molecular ions, where the primary phosphorus nucleus is responsible for a large hyperfine splitting (500--800 G in magnitude). Five EPR spectra representing variations of these oxygen vacancy centers are observed, with the differences being attributed to the relative position of a nearby cation vacancy, either a missing proton or potassium. An angular study of the EPR spectra, conducted at room temperature, provided principal values and principal directions for the g matrices and hyperfine matrices for the hole center and two of the electron centers

Many-body correlation effects in the spatially separated electron and hole layers in the coupled quantum wells

Energy Technology Data Exchange (ETDEWEB)

Babichenko, V.S. [RRC Kurchatov Institute, Kurchatov Sq., 1, 123182 Moscow (Russian Federation); Polishchuk, I.Ya., E-mail: iyppolishchuk@gmail.com [RRC Kurchatov Institute, Kurchatov Sq., 1, 123182 Moscow (Russian Federation); Moscow Institute of Physics and Technology, 141700, 9, Institutskii per., Dolgoprudny, Moscow Region (Russian Federation)

2014-11-15

The many-body correlation effects in the spatially separated electron and hole layers in the coupled quantum wells are investigated. A special case of the many-component electron–hole system is considered. It is shown that if the hole mass is much greater than the electron mass, the negative correlation energy is mainly determined by the holes. The ground state of the system is found to be the 2D electron–hole liquid with the energy smaller than the exciton phase. It is shown that the system decays into the spatially separated neutral electron–hole drops if the initially created charge density in the layers is smaller than the certain critical value n{sub eq}.

The effects of electron-hole separation on the photoconductivity of individual metal oxide nanowires

International Nuclear Information System (INIS)

Prades, J D; Hernandez-Ramirez, F; Jimenez-Diaz, R; Manzanares, M; Andreu, T; Cirera, A; Romano-Rodriguez, A; Morante, J R

2008-01-01

The responses of individual ZnO nanowires to UV light demonstrate that the persistent photoconductivity (PPC) state is directly related to the electron-hole separation near the surface. Our results demonstrate that the electrical transport in these nanomaterials is influenced by the surface in two different ways. On the one hand, the effective mobility and the density of free carriers are determined by recombination mechanisms assisted by the oxidizing molecules in air. This phenomenon can also be blocked by surface passivation. On the other hand, the surface built-in potential separates the photogenerated electron-hole pairs and accumulates holes at the surface. After illumination, the charge separation makes the electron-hole recombination difficult and originates PPC. This effect is quickly reverted after increasing either the probing current (self-heating by Joule dissipation) or the oxygen content in air (favouring the surface recombination mechanisms). The model for PPC in individual nanowires presented here illustrates the intrinsic potential of metal oxide nanowires to develop optoelectronic devices or optochemical sensors with better and new performances.

Interaction of non-equilibrium phonons with electron-hole plasmas in germanium

International Nuclear Information System (INIS)

Kirch, S.J.

1985-01-01

This thesis presents results of experiments on the interaction of phonons and photo-excited electron-hole plasmas in Ge at low temperature. The first two studies involved the low-temperature fluid phase known as the electron-hole liquid (EHL). The third study involved a wider range of temperatures and includes the higher temperature electron-hole plasma (EHP). In the first experiment, superconducting tunnel junctions are used to produce quasi-monochromatic phonons, which propagate through the EHL. The magnitude of the absorption of these non-equilibrium phonons gives a direct measure of the coupling constant, the deformation potential. In the second experiment, the nonequilibrium phonons are generated by laser excitation of a metal film. An unusual sample geometry allows examination of the EHL-phonon interaction near the EHL excitation surface. This coupling is examined for both cw and pulsed EHL excitation. In the third experiment, the phonons are byproducts of the photo-excited carrier thermalization. The spatial, spectral and temporal dependence of the recombination luminescence is examined. A phonon wind force is observed to dominate the transport properties of the EHL and the EHP. These carriers are never observed to move faster than the phonon velocity even during the laser pulse

Ultrafast dynamics of correlated electrons

International Nuclear Information System (INIS)

Rettig, Laurenz

2012-01-01

This work investigates the ultrafast electron dynamics in correlated, low-dimensional model systems using femtosecond time- and angle-resolved photoemission spectroscopy (trARPES) directly in the time domain. In such materials, the strong electron-electron (e-e) correlations or coupling to other degrees of freedom such as phonons within the complex many-body quantum system lead to new, emergent properties that are characterized by phase transitions into broken-symmetry ground states such as magnetic, superconducting or charge density wave (CDW) phases. The dynamical processes related to order like transient phase changes, collective excitations or the energy relaxation within the system allow deeper insight into the complex physics governing the emergence of the broken-symmetry state. In this work, several model systems for broken-symmetry ground states and for the dynamical charge balance at interfaces have been studied. In the quantum well state (QWS) model system Pb/Si(111), the charge transfer across the Pb/Si interface leads to an ultrafast energetic stabilization of occupied QWSs, which is the result of an increase of the electronic confinement to the metal film. In addition, a coherently excited surface phonon mode is observed. In antiferromagnetic (AFM) Fe pnictide compounds, a strong momentum-dependent asymmetry of electron and hole relaxation rates allows to separate the recovery dynamics of the AFM phase from electron-phonon (e-ph) relaxation. The strong modulation of the chemical potential by coherent phonon modes demonstrates the importance of e-ph coupling in these materials. However, the average e-ph coupling constant is found to be small. The investigation of the excited quasiparticle (QP) relaxation dynamics in the high-T c 4 superconductor Bi 2 Sr 2 CaCu 2 O 8+δ reveals a striking momentum and fluence independence of the QP life times. In combination with the momentum-dependent density of excited QPs, this demonstrates the suppression of momentum

Semiconducting Polymer Photodetectors with Electron and Hole Blocking Layers: High Detectivity in the Near-Infrared

Directory of Open Access Journals (Sweden)

Xiong Gong

2010-07-01

Full Text Available Sensing from the ultraviolet-visible to the infrared is critical for a variety of industrial and scientific applications. Photodetectors with broad spectral response, from 300 nm to 1,100 nm, were fabricated using a narrow-band gap semiconducting polymer blended with a fullerene derivative. By using both an electron-blocking layer and a hole-blocking layer, the polymer photodetectors, operating at room temperature, exhibited calculated detectivities greater than 1013 cm Hz1/2/W over entire spectral range with linear dynamic range approximately 130 dB. The performance is comparable to or even better than Si photodetectors.

Individual identification of free hole and electron dynamics in CuIn{sub 1−x}Ga{sub x}Se{sub 2} thin films by simultaneous monitoring of two optical transitions

Energy Technology Data Exchange (ETDEWEB)

Okano, Makoto [Institute for Chemical Research, Kyoto University, Uji, Kyoto 611-0011 (Japan); Hagiya, Hideki; Sakurai, Takeaki; Akimoto, Katsuhiro [Institute of Applied Physics, University of Tsukuba, Tsukuba, Ibaraki 305-8573 (Japan); Shibata, Hajime; Niki, Shigeru [National Institute of Advanced Industrial Science and Technology (AIST), Tsukuba, Ibaraki 305-8568 (Japan); Kanemitsu, Yoshihiko, E-mail: kanemitu@scl.kyoto-u.ac.jp [Institute for Chemical Research, Kyoto University, Uji, Kyoto 611-0011 (Japan); Japan Science and Technology Agency, CREST, Kyoto University, Uji, Kyoto 611-0011 (Japan)

2015-05-04

The photocarrier dynamics of CuIn{sub 1−x}Ga{sub x}Se{sub 2} (CIGS) thin films were studied using white-light transient absorption (TA) measurements, as an understanding of this behavior is essential for improving the performance of solar cells composed of CIGS thin films. A characteristic double-peak structure due to the splitting of the valence bands in the CIGS was observed in the TA spectra under near-band-gap resonant excitation. From a comparison of the TA decay dynamics monitored at these two peaks, it was found that the slow-decay components of the electron and hole relaxation are on the nanosecond timescale. This finding is clear evidence of the long lifetimes of free photocarriers in polycrystalline CIGS thin films.

σ-holes and π-holes: Similarities and differences.

Science.gov (United States)

Politzer, Peter; Murray, Jane S

2018-04-05

σ-Holes and π-holes are regions of molecules with electronic densities lower than their surroundings. There are often positive electrostatic potentials associated with them. Through these potentials, the molecule can interact attractively with negative sites, such as lone pairs, π electrons, and anions. Such noncovalent interactions, "σ-hole bonding" and "π-hole bonding," are increasingly recognized as being important in a number of different areas. In this article, we discuss and compare the natures and characteristics of σ-holes and π-holes, and factors that influence the strengths and locations of the resulting electrostatic potentials. © 2017 Wiley Periodicals, Inc. © 2017 Wiley Periodicals, Inc.

Ultrafast Interfacial Electron and Hole Transfer from CsPbBr3 Perovskite Quantum Dots.

Science.gov (United States)

Wu, Kaifeng; Liang, Guijie; Shang, Qiongyi; Ren, Yueping; Kong, Degui; Lian, Tianquan

2015-10-14

Recently reported colloidal lead halide perovskite quantum dots (QDs) with tunable photoluminescence (PL) wavelengths covering the whole visible spectrum and exceptionally high PL quantum yields (QYs, 50-90%) constitute a new family of functional materials with potential applications in light-harvesting and -emitting devices. By transient absorption spectroscopy, we show that the high PL QYs (∼79%) can be attributed to negligible electron or hole trapping pathways in CsPbBr3 QDs: ∼94% of lowest excitonic states decayed with a single-exponential time constant of 4.5 ± 0.2 ns. Furthermore, excitons in CsPbBr3 QDs can be efficiently dissociated in the presence of electron or hole acceptors. The half-lives of electron transfer (ET) to benzoquinone and subsequent charge recombination are 65 ± 5 ps and 2.6 ± 0.4 ns, respectively. The half-lives for hole transfer (HT) to phenothiazine and the subsequent charge recombination are 49 ± 6 ps and 1.0 ± 0.2 ns, respectively. The lack of electron and hole traps and fast interfacial ET and HT rates are key properties that may enable the development of efficient lead halide perovskite QDs-based light-harvesting and -emitting devices.

Local Hawking temperature for dynamical black holes

International Nuclear Information System (INIS)

Hayward, S A; Criscienzo, R Di; Nadalini, M; Vanzo, L; Zerbini, S

2009-01-01

A local Hawking temperature is derived for any future outer trapping horizon in spherical symmetry, using a Hamilton-Jacobi variant of the Parikh-Wilczek tunneling method. It is given by a dynamical surface gravity as defined geometrically. The operational meaning of the temperature is that Kodama observers just outside the horizon measure an invariantly redshifted temperature, diverging at the horizon itself. In static, asymptotically flat cases, the Hawking temperature as usually defined by the Killing vector agrees in standard cases, but generally differs by a relative redshift factor between the horizon and infinity, this being the temperature measured by static observers at infinity. Likewise, the geometrical surface gravity reduces to the Newtonian surface gravity in the Newtonian limit, while the Killing definition instead reflects measurements at infinity. This may resolve a long-standing puzzle concerning the Hawking temperature for the extremal limit of the charged stringy black hole, namely that it is the local temperature which vanishes. In general, this confirms the quasi-stationary picture of black-hole evaporation in early stages. However, the geometrical surface gravity is generally not the surface gravity of a static black hole with the same parameters. (fast track communication)

Dynamic hole closure behind a deep ocean sediment penetrator

International Nuclear Information System (INIS)

Dzwilewski, P.T.; Karnes, C.H.

1982-01-01

A freefall or boosted penetrator is one concept being considered to dispose of nuclear waste in the deep ocean seabed. For this technique to be acceptable, the sediment must be an effective barrier to the migration of radioactive nuclides, which means that the hole behind the advancing penetrator must close. One mechanism which can cause the hole to close immediately behind the penetrator is the reduction in water pressure in the wake as water tries to follow the penetrator into the sediment. An approximate solution to this complex problem is presented which analyzes the deformation of the sediment with a nonlinear, large displacement and strain, Lagrangian finite-difference computer code (STEALTH). The water was treated by Bernoulli's Principle for flow in a pipe resulting in a pressure boundary condition applied to the sediment surface along the path after passage of the penetrator. Two one-dimensional and eight two-dimensional calculations were performed with various penetrator velocities (15, 30, and 60 m/s) and sediment shear strengths. In two of the calculations, the dynamic pressure reduction was neglected to see if geostatic stresses alone would close the hole. The results of this study showed that geostatic stresses alone would not close the hole but the dynamic pressure reduction would. The largest uncertainty in the analysis was the pressure conditions in the water behind the penetrator in which frictionless, steady-state flow, in a uniform diameter pipe was assumed. A more sophisticated and realistic pressure condition has been formulated and will be implemented in the computer code in the near future

Could the dynamics of the Universe be influenced by what is going on inside black holes?

Energy Technology Data Exchange (ETDEWEB)

Avelino, P.P., E-mail: pedro.avelino@astro.up.pt [Instituto de Astrofísica e Ciências do Espaço, Universidade do Porto, CAUP, Rua das Estrelas, PT4150-762 Porto (Portugal)

2015-04-01

We investigate the potential impact of mass inflation inside black holes on the dynamics of the Universe, considering a recent reformulation of general relativity, proposed in [1], which prevents the vacuum energy from acting as a gravitational source. The interior dynamics of accreting black holes is studied, at the classical level, using the homogeneous approximation and taking charge as a surrogate for angular momentum. We show that, depending on the accreting fluid properties, mass inflation inside black holes could influence the value of the cosmological constant and thus the dynamics of the Universe. A full assessment of the cosmological role played by black holes will require a deeper understanding of the extremely energetic regimes expected inside real astrophysical black holes, including their relation with the physics of the very early Universe, and may eventually lead to an entirely new paradigm for the origin and evolution of the Universe.

Phase-space holes due to electron and ion beams accelerated by a current-driven potential ramp

Directory of Open Access Journals (Sweden)

M. V. Goldman

2003-01-01

Full Text Available One-dimensional open-boundary simulations have been carried out in a current-carrying plasma seeded with a neutral density depression and with no initial electric field. These simulations show the development of a variety of nonlinear localized electric field structures: double layers (unipolar localized fields, fast electron phase-space holes (bipolar fields moving in the direction of electrons accelerated by the double layer and trains of slow alternating electron and ion phase-space holes (wave-like fields moving in the direction of ions accelerated by the double layer. The principal new result in this paper is to show by means of a linear stability analysis that the slow-moving trains of electron and ion holes are likely to be the result of saturation via trapping of a kinetic-Buneman instability driven by the interaction of accelerated ions with unaccelerated electrons.

Hole growth dynamics in a two dimensional Leidenfrost droplet

Science.gov (United States)

Raufaste, Christophe; Celestini, Franck; Barzyk, Alexandre; Frisch, Thomas

2015-03-01

We studied the behaviors of Leidenfrost droplets confined in a Hele-Shaw cell. These droplets are unstable above a critical size and a hole grows at their center. We experimentally investigate two different systems for which the hole growth dynamics exhibits peculiar features that are driven by capillarity and inertia. We report a first regime characterized by the liquid reorganization from a liquid sheet to a liquid torus with similarities to the burst of micron-thick soap films. In the second regime, the liquid torus expands and thins before fragmentation. Finally, we propose models to account for the experimental results.

Relation between bulk compressibility and surface energy of electron-hole liquids

International Nuclear Information System (INIS)

Singwi, K.S.; Tosi, M.P.

1979-08-01

Attention is drawn to the existence of an empirical relation chiσ/asup(*)sub(B) approximately 1 between the compressibility, the surface energy and the excitonic radius in electron-hole liquids. (author)

Impact ionization coefficients for electrons and holes in In0.14Ga0.86As

International Nuclear Information System (INIS)

Pearsall, T.P.; Nahory, R.E.; Pollack, M.A.

1975-01-01

We report the measurement of impact ionization rates for electrons and holes in the direct band-gap semiconductor alloy In 0 . 14 Ga 0 . 86 As. Our results show clearly that the ionization rate for holes is greater than that for electrons. The measurments were made for electric fields between 2.6times10 5 and 3.4times10 5 V cm -1 . In this range, the ionization coefficients can be expressed as α=α/sub infinity/ exp(-A/E) for electrons and β=β/sub infinity/ exp(-B/E) for holes with α/sub infinity/=1.0times10 9 cm -1 , A=3.6times10 6 V cm -1 , and β/sub infinity/=1.3times10 8 cm -1 , B=2.7times10 6 V cm -1

On the existence and dynamics of braneworld black holes

International Nuclear Information System (INIS)

Fitzpatrick, Andrew Liam; Randall, Lisa; Wiseman, Toby

2006-01-01

Based on holographic arguments Tanaka and Emparan et al have claimed that large localized static black holes do not exist in the one-brane Randall-Sundrum model. If such black holes are time-dependent as they propose, there are potentially significant phenomenological and theoretical consequences. We revisit the issue, arguing that their reasoning does not take into account the strongly coupled nature of the holographic theory. We claim that static black holes with smooth metrics should indeed exist in these theories, and give a simple example. However, although the existence of such solutions is relevant to exact and numerical solution searches, such static solutions might be dynamically unstable, again leading to time dependence with phenomenological consequences. We explore a plausible instability, suggested by Tanaka, analogous to that of Gregory and Laflamme, but argue that there is no reliable reason at this point to assume it must exist

Time-dependence hole and electron trapping effects in SIMOX buried oxides

International Nuclear Information System (INIS)

Boesch, H.E. Jr.; Taylor, T.L.; Hite, L.R.; Bailey, W.E.

1990-01-01

Back-channel threshold shift associated with the buried oxide layers of separation by implanted oxygen (SIMOX) and zone-melted recrystallization (ZMR) field-effect transistors (FETs) was measured following pulsed irradiation as a function of temperature and back-gate bias using a fast time-resolved I-V measurement technique. The SIMOX FETs showed large initial negative voltage shifts at 0.2 ms after irradiation followed by temperature- and bias-dependent additional negative shifts to 800s. Analysis and modeling of the results indicate efficient deep trapping of radiation-generated holes in the bulk of the oxide, substantial initial trapping of radiation-generated electrons in the oxide, and rapid removal of the trapped electrons by a thermal detrapping process. The ZMR FETs showed evidence of substantial trapping of holes alone in the oxide bulk

Cluster dynamics transcending chemical dynamics toward nuclear fusion.

Science.gov (United States)

Heidenreich, Andreas; Jortner, Joshua; Last, Isidore

2006-07-11

Ultrafast cluster dynamics encompasses femtosecond nuclear dynamics, attosecond electron dynamics, and electron-nuclear dynamics in ultraintense laser fields (peak intensities 10(15)-10(20) W.cm(-2)). Extreme cluster multielectron ionization produces highly charged cluster ions, e.g., (C(4+)(D(+))(4))(n) and (D(+)I(22+))(n) at I(M) = 10(18) W.cm(-2), that undergo Coulomb explosion (CE) with the production of high-energy (5 keV to 1 MeV) ions, which can trigger nuclear reactions in an assembly of exploding clusters. The laser intensity and the cluster size dependence of the dynamics and energetics of CE of (D(2))(n), (HT)(n), (CD(4))(n), (DI)(n), (CD(3)I)(n), and (CH(3)I)(n) clusters were explored by electrostatic models and molecular dynamics simulations, quantifying energetic driving effects, and kinematic run-over effects. The optimization of table-top dd nuclear fusion driven by CE of deuterium containing heteroclusters is realized for light-heavy heteroclusters of the largest size, which allows for the prevalence of cluster vertical ionization at the highest intensity of the laser field. We demonstrate a 7-orders-of-magnitude enhancement of the yield of dd nuclear fusion driven by CE of light-heavy heteroclusters as compared with (D(2))(n) clusters of the same size. Prospective applications for the attainment of table-top nucleosynthesis reactions, e.g., (12)C(P,gamma)(13)N driven by CE of (CH(3)I)(n) clusters, were explored.

Effect of hole size on fluid dynamics of a posterior-chamber phakic intraocular lens with a central perforation by using computational fluid dynamics.

Science.gov (United States)

Kawamorita, Takushi; Shimizu, Kimiya; Shoji, Nobuyuki

2016-04-01

A modified implantable collamer lens (ICL) with a central hole with a diameter of 0.36 mm, referred to as a hole-ICL, was created to improve aqueous humour circulation. The aim of this study is to investigate the ideal hole size in a hole-ICL from the standpoint of the fluid dynamic characteristics of the aqueous humour using computational fluid dynamics. Fluid dynamics simulation using an ICL was performed with thermal-hydraulic analysis software FloEFD V 12.2 (Mentor Graphics Corp.). In the simulation, three-dimensional eye models based on a modified Liou-Brennan model eye with a conventional ICL (Model ICM, Staar Surgical) and a hole-ICL were used. The hole-ICL was -9.0 dioptres (D) and 12.0 mm in length, with an optic zone of 5.5 mm. The vaulting was 0.50 mm. The quantity of aqueous humour produced by the ciliary body was set at 2.80 μL/min. Flow distribution between the anterior surface of the crystalline lens and the posterior surface of the ICL was calculated, and trajectory analysis was performed. With an increase in the central hole size, the velocity of the aqueous humour increased, with the peak velocity occurring at a diameter of approximately 0.4 mm. Once the diameter had increased above 0.4 mm, the velocity then decreased. The velocity difference between the cases of a central hole size of 0.1 mm and 0.2 mm was significant. The desirable central hole size was 0.2 mm or larger in terms of flow dynamics. The current model, based on a central hole size of 0.36 mm, was close to ideal. The optimisation of the hole size should be performed based on results from a long-term clinical study so as to analyse the incidence rate of secondary cataract and optical performance.

Ultrafast dynamics of correlated electrons

Energy Technology Data Exchange (ETDEWEB)

Rettig, Laurenz

2012-07-09

This work investigates the ultrafast electron dynamics in correlated, low-dimensional model systems using femtosecond time- and angle-resolved photoemission spectroscopy (trARPES) directly in the time domain. In such materials, the strong electron-electron (e-e) correlations or coupling to other degrees of freedom such as phonons within the complex many-body quantum system lead to new, emergent properties that are characterized by phase transitions into broken-symmetry ground states such as magnetic, superconducting or charge density wave (CDW) phases. The dynamical processes related to order like transient phase changes, collective excitations or the energy relaxation within the system allow deeper insight into the complex physics governing the emergence of the broken-symmetry state. In this work, several model systems for broken-symmetry ground states and for the dynamical charge balance at interfaces have been studied. In the quantum well state (QWS) model system Pb/Si(111), the charge transfer across the Pb/Si interface leads to an ultrafast energetic stabilization of occupied QWSs, which is the result of an increase of the electronic confinement to the metal film. In addition, a coherently excited surface phonon mode is observed. In antiferromagnetic (AFM) Fe pnictide compounds, a strong momentum-dependent asymmetry of electron and hole relaxation rates allows to separate the recovery dynamics of the AFM phase from electron-phonon (e-ph) relaxation. The strong modulation of the chemical potential by coherent phonon modes demonstrates the importance of e-ph coupling in these materials. However, the average e-ph coupling constant is found to be small. The investigation of the excited quasiparticle (QP) relaxation dynamics in the high-T{sub c}4 superconductor Bi{sub 2}Sr{sub 2}CaCu{sub 2}O{sub 8+δ} reveals a striking momentum and fluence independence of the QP life times. In combination with the momentum-dependent density of excited QPs, this demonstrates the

Electron-hole pairing and anomalous properties of layered high-Tc compounds

International Nuclear Information System (INIS)

Efetov, K.B.

1991-01-01

Band-structure pictures for layered high-T c materials available in the literature show that, besides the dispersive broad band responsible for metallic properties, there are at least two additional bands having minima and maxima near the Fermi surface. These additional bands belong to different planes (for example, CuO planes and BiO planes in Bi 2 Sr 2 CaCu 2 O 8 ) or to planes and chains (in YBa 2 Cu 3 O 7 ). Provided the Coulomb repulsion is not very weak, pairing of electrons and holes belonging to these additional bands in different planes or planes and chains is possible. It is shown that, if this possibility is realized, a transition in the additional bands into a state of an excitonic dielectric occurs. The spin of an electron-hole pair can be both 0 and 1. Due to the fact that the electron and the hole of the pair belong to different planes, there are no charge- or spin-density waves. This excitonic insulator can serve as a polarizing substance and give a strong attraction between electrons of the metallic band even if the bare interaction is repulsive. It is also shown that some interesting gapless excitations exist. Provided there are impurities in the system that scatter from plane to plane, these excitations are coupled to the electrons of the metallic band. This effective interaction can be described in terms of an effective mode P(ω) with ImP(ω)∼-sgnω. As a result, one can obtain such properties of the normal state as a linear dependence of the resistivity on temperature, linear dependence of the density of states on energy, constant background in the Raman-scattering intensity, large nuclear relaxation rate, etc., which are very well known from experiments

Potential beneficial effects of electron-hole plasmas created in silicon sensors by XFEL-like high intensity pulses for detector development

Energy Technology Data Exchange (ETDEWEB)

Weiss, Joel T.; Becker, Julian; Shanks, Katherine S.; Philipp, Hugh T.; Tate, Mark W. [Laboratory of Atomic and Solid State Physics, Cornell University, Ithaca, NY 14853 (United States); Gruner, Sol M., E-mail: smg26@cornell.edu [Laboratory of Atomic and Solid State Physics, Cornell University, Ithaca, NY 14853 (United States); Cornell High Energy Synchrotron Source (CHESS), Cornell University, Ithaca, NY 14853 (United States)

2016-07-27

There is a compelling need for a high frame rate imaging detector with a wide dynamic range, from single x-rays/pixel/pulse to >10{sup 6} x-rays/pixel/pulse, that is capable of operating at both x-ray free electron laser (XFEL) and 3rd generation sources with sustained fluxes of > 10{sup 11} x-rays/pixel/s [1, 2, 3]. We propose to meet these requirements with the High Dynamic Range Pixel Array Detector (HDR-PAD) by (a) increasing the speed of charge removal strategies [4], (b) increasing integrator range by implementing adaptive gain [5], and (c) exploiting the extended charge collection times of electron-hole pair plasma clouds that form when a sufficiently large number of x-rays are absorbed in a detector sensor in a short period of time [6]. We have developed a measurement platform similar to the one used in [6] to study the effects of high electron-hole densities in silicon sensors using optical lasers to emulate the conditions found at XFELs. Characterizations of the employed tunable wavelength laser with picosecond pulse duration have shown Gaussian focal spots sizes of 6 ± 1 µm rms over the relevant spectrum and 2 to 3 orders of magnitude increase in available intensity compared to previous measurements presented in [6]. Results from measurements on a typical pixelated silicon diode intended for use with the HDR-PAD (150 µm pixel size, 500 µm thick sensor) are presented.

Dynamics of toroidal spiral strings around five-dimensional black holes

International Nuclear Information System (INIS)

Igata, Takahisa; Ishihara, Hideki

2010-01-01

We examine the separability of the Nambu-Goto equation for test strings in a shape of toroidal spiral in a five-dimensional Kerr-AdS black hole. In particular, for a 'Hopf loop' string which is a special class of the toroidal spiral strings, we show the complete separation of variables occurs in two cases, Kerr background and Kerr-AdS background with equal angular momenta. We also obtain the dynamical solution for the Hopf loop around a black hole and for the general toroidal spiral in Minkowski background.

Monte Carlo studies of thermalization of electron-hole pairs in spin-polarized degenerate electron gas in monolayer graphene

Science.gov (United States)

Borowik, Piotr; Thobel, Jean-Luc; Adamowicz, Leszek

2018-02-01

Monte Carlo method is applied to the study of relaxation of excited electron-hole (e-h) pairs in graphene. The presence of background of spin-polarized electrons, with high density imposing degeneracy conditions, is assumed. To such system, a number of e-h pairs with spin polarization parallel or antiparallel to the background is injected. Two stages of relaxation: thermalization and cooling are clearly distinguished when average particles energy and its standard deviation σ _E are examined. At the very beginning of thermalization phase, holes loose energy to electrons, and after this process is substantially completed, particle distributions reorganize to take a Fermi-Dirac shape. To describe the evolution of and σ _E during thermalization, we define characteristic times τ _ {th} and values at the end of thermalization E_ {th} and σ _ {th}. The dependence of these parameters on various conditions, such as temperature and background density, is presented. It is shown that among the considered parameters, only the standard deviation of electrons energy allows to distinguish between different cases of relative spin polarizations of background and excited electrons.

Optical and magneto-optical properties of the electron-doped and hole-doped C{sub 82} crystal

Energy Technology Data Exchange (ETDEWEB)

Rostampour, E., E-mail: el_rostampour@yahoo.com [Plasma Physics Research Center, Science and Research Branch, Islamic Azad University, Tehran (Iran, Islamic Republic of); Koohi, A. [Plasma Physics and Nuclear Fusion Research School, Nuclear Science and Technology Research Institute, AEOI, Tehran (Iran, Islamic Republic of)

2015-01-15

The optical and magnetic properties of the doped C{sub 82} crystal have been investigated by Su–Schrieffer–Heeger (SSH) model, which is based on the Ewald method. When the C{sub 82} molecule is doped with one electron (or hole), a single electron is remained in the energy level that affects the optical and magnetic properties of the C{sub 82} crystal. The lattice and electronic structures of C{sub 82} changed with doping electron (or hole) in the molecule of C{sub 82}. Therefore, polarons are predicted in doped fullerenes. The obtained results showed that the dielectric tensor of the C{sub 82} crystal increased with doping electron (or hole) in the molecule of C{sub 82}. The spectral shapes of the dielectric tensor, circular dichroism and birefringence coefficient of the C{sub 82} crystal turn out to be determined mainly by the geometrical distributions of the pentagons in the fullerene structures.

Recent advances in imaging of properties and growth of low dimensional structures for photonics and electronics by XPEEM

International Nuclear Information System (INIS)

Zakharov, A.A.; Mikkelsen, A.; Andersen, J.N.

2012-01-01

Highlights: ► 3d electronic band mapping is made using XPEEM. ► Free-standing graphene on SiC can be made by atomic intercalation. ► XPEEM gives a deeper insight into growth of self-seeded III–V nanowires. ► Presents controlled self-propelled droplet dynamics on GaP surface. ► Presents punp-probe experiments in the attosecond time range. -- Abstract: Spectroscopic Photoemission and Low Energy Electron Microscopy (SPELEEM) is a very powerful and diverse microscopy technique for the investigation of surfaces, interfaces, buried layers and nanoscale objects like nanoparticles and nanowires. The many significant results from photoemission Electron microscopy (PEEM) in recent years are linked with the exploitation of advanced light sources such as synchrotrons and new advanced laser systems. Combined also with low energy electron microscopy (LEEM) it allows a complementary chemical and structural analysis making LEEM/PEEM a versatile multitechnique instrument. To illustrate the extreme diversity, we give a summary of the recent studies with the SPELEEM installed at the soft X-ray beamline I311 at the MAXII synchrotron storage ring and a portable electrostatic PEEM used with ultra-fast XUV laser technology. The examples cover topics such as full-cone 3D band mapping by using the photoelectron diffraction mode of the microscope, growth mechanism and detailed doping profile of III–V nanowires, growth and intercalation of graphene on SiC substrates, droplet dynamics on GaP(1 1 1) surface, surface chemistry and control of nanostructure fabrication. Moreover, the first results of PEEM experiments using extreme ultraviolet attosecond pulse trains are discussed.

Lightwave-driven quasiparticle collisions on a subcycle timescale.

Science.gov (United States)

Langer, F; Hohenleutner, M; Schmid, C P; Poellmann, C; Nagler, P; Korn, T; Schüller, C; Sherwin, M S; Huttner, U; Steiner, J T; Koch, S W; Kira, M; Huber, R

2016-05-12

Ever since Ernest Rutherford scattered α-particles from gold foils, collision experiments have revealed insights into atoms, nuclei and elementary particles. In solids, many-body correlations lead to characteristic resonances--called quasiparticles--such as excitons, dropletons, polarons and Cooper pairs. The structure and dynamics of quasiparticles are important because they define macroscopic phenomena such as Mott insulating states, spontaneous spin- and charge-order, and high-temperature superconductivity. However, the extremely short lifetimes of these entities make practical implementations of a suitable collider challenging. Here we exploit lightwave-driven charge transport, the foundation of attosecond science, to explore ultrafast quasiparticle collisions directly in the time domain: a femtosecond optical pulse creates excitonic electron-hole pairs in the layered dichalcogenide tungsten diselenide while a strong terahertz field accelerates and collides the electrons with the holes. The underlying dynamics of the wave packets, including collision, pair annihilation, quantum interference and dephasing, are detected as light emission in high-order spectral sidebands of the optical excitation. A full quantum theory explains our observations microscopically. This approach enables collision experiments with various complex quasiparticles and suggests a promising new way of generating sub-femtosecond pulses.

Electron-hole drop (EHD) stability in deformation potential well

International Nuclear Information System (INIS)

Makarov, A.G.; Tikhodeev, S.G.

1984-01-01

In heterogeneously-deformed Ge the stability of electron-hole droplets (EHD) being in a potential well is considered. It is shown that the potential well effect is equivalent to the decrease of effective density of phonon EHD charge. It is pointed out that heating EHD (for example, by IR radiation), can increase the phonon droplet charge and affect its stability

Interference Processes During Reradiation of Attosecond Pulses of Electromagnetic Field by Graphene

Science.gov (United States)

Makarov, D. N.; Matveev, V. I.; Makarova, K. A.

2018-05-01

Interference spectra during reradiation of attosecond pulses of electromagnetic field by graphene sheets are considered. Analytical expressions for calculations of spectral distributions are derived. As an example, the interference spectra of a graphene sheet and a flat rectangular lattice are compared.

Activity coefficients of electrons and holes in semiconductors

International Nuclear Information System (INIS)

Orazem, M.E.; Newman, J.

1984-01-01

Dilute-solution transport equations with constant activity coefficients are commonly used to model semiconductors. These equations are consistent with a Boltzmann distribution and are invalid in regions where the species concentration is close to the respective site concentration. A more rigorous treatment of transport in a semiconductor requires activity coefficients which are functions of concentration. Expressions are presented for activity coefficients of electrons and holes in semiconductors for which conduction- and valence-band energy levels are given by the respective bandedge energy levels. These activity coefficients are functions of concentration and are thermodynamically consistent. The use of activity coefficients in macroscopic transport relationships allows a description of electron transport in a manner consistent with the Fermi-Dirac distribution

On the theory of hole propagation in an antiferromagnetic background

International Nuclear Information System (INIS)

Kuzemsky, A.L.

1994-10-01

The spectrum of hole quasiparticles and the role of magnetic correlations has been considered in the self-consistent Irreducible Green Functions formalism, motivated from Strongly Correlated Electron systems for correlated electron models of high-Tc superconductivity. The hole quasiparticle dynamics has been discussed for t-J model and compared with that of the spin-fermion model. For this Kondo-Heisenberg-type model it was clearly pointed out on the self-energy level, beyond Hartree-Fock approximation, how the one-and two magnon processes define the true nature of carriers in HTSC. (author). 57 refs

Tailoring of polarization in electron blocking layer for electron confinement and hole injection in ultraviolet light-emitting diodes

International Nuclear Information System (INIS)

Lu, Yu-Hsuan; Pilkuhn, Manfred H.; Fu, Yi-Keng; Chu, Mu-Tao; Huang, Shyh-Jer; Su, Yan-Kuin; Wang, Kang L.

2014-01-01

The influence of the AlGaN electron blocking layer (EBL) with graded aluminum composition on electron confinement and hole injection in AlGaN-based ultraviolet light-emitting diodes (LEDs) are investigated. The light output power of LED with graded AlGaN EBL was markedly improved, comparing to LED with conventional EBL. In experimental results, a high increment of 86.7% can be obtained in light output power. Simulation analysis shows that via proper modification of the barrier profile from the last barrier of the active region to EBL, not only the elimination of electron overflow to p-type layer can be achieved but also the hole injection into the active region can be enhanced, compared to a conventional LED structure. The dominant factor to the performance improvement is shown to be the modulation of polarization field by the graded Al composition in EBL

Tailoring of polarization in electron blocking layer for electron confinement and hole injection in ultraviolet light-emitting diodes

Energy Technology Data Exchange (ETDEWEB)

Lu, Yu-Hsuan; Pilkuhn, Manfred H. [Department of Electrical Engineering, Institute of Microelectronics and Advanced Optoelectronic Technology Center, National Cheng Kung University, Tainan 70101, Taiwan (China); Fu, Yi-Keng; Chu, Mu-Tao [Electronics and Optoelectronics Research Laboratories, Industrial Technology Research Institute, Hsinchu 31040, Taiwan (China); Huang, Shyh-Jer, E-mail: yksu@mail.ncku.edu.tw, E-mail: totaljer48@gmail.com [Department of Electrical Engineering, Institute of Microelectronics and Advanced Optoelectronic Technology Center, National Cheng Kung University, Tainan 70101, Taiwan (China); Department of Electrical Engineering, University of California at Los Angeles, Los Angeles, California 90095 (United States); Su, Yan-Kuin, E-mail: yksu@mail.ncku.edu.tw, E-mail: totaljer48@gmail.com [Department of Electrical Engineering, Institute of Microelectronics and Advanced Optoelectronic Technology Center, National Cheng Kung University, Tainan 70101, Taiwan (China); Department of Electronic Engineering, Kun-Shan University, Tainan 71003, Taiwan (China); Wang, Kang L. [Department of Electrical Engineering, University of California at Los Angeles, Los Angeles, California 90095 (United States)

2014-03-21

The influence of the AlGaN electron blocking layer (EBL) with graded aluminum composition on electron confinement and hole injection in AlGaN-based ultraviolet light-emitting diodes (LEDs) are investigated. The light output power of LED with graded AlGaN EBL was markedly improved, comparing to LED with conventional EBL. In experimental results, a high increment of 86.7% can be obtained in light output power. Simulation analysis shows that via proper modification of the barrier profile from the last barrier of the active region to EBL, not only the elimination of electron overflow to p-type layer can be achieved but also the hole injection into the active region can be enhanced, compared to a conventional LED structure. The dominant factor to the performance improvement is shown to be the modulation of polarization field by the graded Al composition in EBL.

INTERCHANGE RECONNECTION AND CORONAL HOLE DYNAMICS

International Nuclear Information System (INIS)

Edmondson, J. K.; Antiochos, S. K.; DeVore, C. R.; Lynch, B. J.; Zurbuchen, T. H.

2010-01-01

We investigate the effect of magnetic reconnection between open and closed fields, often referred to as 'interchange' reconnection, on the dynamics and topology of coronal hole boundaries. The most important and most prevalent three-dimensional topology of the interchange process is that of a small-scale bipolar magnetic field interacting with a large-scale background field. We determine the evolution of such a magnetic topology by numerical solution of the fully three-dimensional MHD equations in spherical coordinates. First, we calculate the evolution of a small-scale bipole that initially is completely inside an open field region and then is driven across a coronal hole boundary by photospheric motions. Next the reverse situation is calculated in which the bipole is initially inside the closed region and driven toward the coronal hole boundary. In both cases, we find that the stress imparted by the photospheric motions results in deformation of the separatrix surface between the closed field of the bipole and the background field, leading to rapid current sheet formation and to efficient reconnection. When the bipole is inside the open field region, the reconnection is of the interchange type in that it exchanges open and closed fields. We examine, in detail, the topology of the field as the bipole moves across the coronal hole boundary and find that the field remains well connected throughout this process. Our results, therefore, provide essential support for the quasi-steady models of the open field, because in these models the open and closed flux are assumed to remain topologically distinct as the photosphere evolves. Our results also support the uniqueness hypothesis for open field regions as postulated by Antiochos et al. On the other hand, the results argue against models in which open flux is assumed to diffusively penetrate deeply inside the closed field region under a helmet streamer. We discuss the implications of this work for coronal observations.

The effect of particle-hole interaction on the XPS core-hole spectrum

International Nuclear Information System (INIS)

Ohno, Masahide; Sjoegren, Lennart

2004-01-01

How the effective particle-hole interaction energy, U, or the polarization effect on a secondary electron in a final two-hole one-particle (2h1p) state created by the Coster-Kronig (CK) transition can solely affect the density of the CK particle states and consequently the core-hole spectral function, is discussed. The X-ray photoelectron spectroscopy (XPS) core-hole spectrum is predominantly governed by the unperturbed initial core-hole energy relative to the zero-point energy. At the latter energy, the real part of the initial core-hole self-energy becomes zero (no relaxation energy shift) and the imaginary part (the lifetime broadening) approximately maximizes. The zero-point energy relative to the double-ionization threshold energy is governed by the ratio of U relative to the bandwidth of the CK continuum. As an example, we study the 5p XPS spectra of atomic Ra (Z=88), Th (Z=90) and U (Z=92). The spectra are interpreted in terms of the change in the unperturbed initial core-hole energy relative to the zero-point energy. We explain why in general an ab initio atomic many-body calculation can provide an overall good description of solid-state spectra predominantly governed by the atomic-like localized core-hole dynamics. We explain this in terms of the change from free atom to metal in both U and the zero-point energy (self-energy)

Theory of the electronic structure and carrier dynamics of strain-induced (Ga, In)As quantum dots

International Nuclear Information System (INIS)

Boxberg, Fredrik; Tulkki, Jukka

2007-01-01

Strain-induced quantum dots (SIQD) confine electrons and holes to a lateral potential minimum within a near-surface quantum well (QW). The potential minimum is located in the QW below a nanometre-sized stressor crystal grown on top of the QW. SIQD exhibit well-resolved and prominently atomic-like optical spectra, making them ideal for experimental and theoretical studies of mesoscopic phenomena in semiconductor nanocrystals. In this report we review the theory of strain-induced confinement, electronic structure, photonics and carrier relaxation dynamics in SIQD. The theoretical results are compared with available experimental data. Electronic structure calculations are mainly performed using the multiband envelope function approach. Many-body effects are discussed using a direct diagonalization method, albeit, for the sake of computational feasibility, within a two-band model. The QD carrier dynamics are discussed in terms of a master equation model, which accounts for the details of the electronic structure as well as the leading photon, phonon and Coulomb interaction processes. We also discuss the quantum confined Stark effect, the Zeeman splitting and the formation of Landau levels in external fields. Finally, we review a recent theory of the cooling of radiative QD excitons by THz radiation. In particular we discuss the resonance charge transfer of holes between piezoelectric trap states and the deformation potential minima. The agreement between the theory and experiment is fair throughout, but calls for further investigations

Investigation of dynamic characteristics of shells with holes and added mass

Directory of Open Access Journals (Sweden)

Seregin Sergey Valer’evich

2014-04-01

Full Text Available Thin cylindrical shells are widely used in construction, engineering and other industries. In case of designing a reservoir for the isothermal storage of liquefied gases such cases are inevitable, when housing requires various technical holes. A point wise added mass can appear into practice in the form of suspended spotlights, radar, architectural inclusions in buildings and structures of various purposes. It is known, that the dynamic asymmetry as an initial irregular geometric shape, including holes, and the added mass leads to specific effects in shells. In the paper the impact of a cut on the frequency and form of its own vibrations of thin circular cylindrical shells is theoretically examined with the help of the equations of linear shallow shell theory. For modal equations with Nav’e boundary conditions, we used the Bubnov - Galerkin method. The authors have expressed a formula for finding the lowest of the split-frequency vibrations of a shell with a cutout. It is stated, that in case of an appropriate choice of added mass value the lower frequencies are comparable with the case of vibrations of a shell with a hole. By numerical and experimental modeling and finite element method in the environment of MSC "Nastran" oscillation frequencies a shell supporting a concentrated mass and a shell with a cutout were compared. It is shown, that the results of the dynamic analysis of shells with holes with a suitable choice of the attached mass values are comparable with the results of the analysis of shells carrying a point mass. It was concluded that the edges in the holes, significantly affect the reduction in the lowest frequency, and need to be strengthened.

Particle Dynamics around Weakly Magnetized Reissner-Nordström Black Hole

International Nuclear Information System (INIS)

Jamil, Mubasher; Majeed, Bushra; Hussain, Saqib

2015-01-01

Considering the geometry of Reissner-Nordström (RN) black hole immersed in magnetic field, we have studied the dynamics of neutral and charged particles. A collision of particles in the inner stable circular orbit is considered and the conditions for the escape of colliding particles from the vicinity of black hole are given. The trajectories of the escaping particle are discussed. Also, the velocity required for this escape is calculated. It is observed that there is more than one stable region if magnetic field is present in the accretion disk of black hole, so the stability of ISCO increases in the presence of magnetic field. Effect of magnetic field on the angular motion of neutral and charged particles is observed graphically.

Electronic correlations in hole- and electron-doped Fe-based superconductors

Science.gov (United States)

Hardy, Frederic; Boehmer, Anna; Schweiss, Peter; Wolf, Thomas; Heid, Rolf; Eder, Robert; Fisher, Robert A.; Meingast, Christoph

2015-03-01

High-temperature superconductivity in the cuprates occurs at the crossover from a highly-correlated Mott insulating state to a weaker correlated Fermi liquid as a function of hole doping. The iron pnictides were initially thought to be fairly weakly correlated. However, we have recently shown using transport and thermodynamic measurements that KFe2As2 is strongly correlated. Both the Sommerfeld coefficient and the Pauli susceptibility are strongly enhanced with respect to their bare DFT values. These correlations are even further enhanced in RbFe2As2andCsFe2As2. The temperature dependence of both the susceptibility and the thermal expansion provides strong experimental evidence for the existence of a coherence-incoherence crossover; similar to what is found in heavy-fermion compounds. Whereas the correlations in the cuprates result from a large value of the Hubbard U, recent works have stressed the particular relevance of Hund's coupling in the pnictides. Our data may be interpreted in terms of a close proximity of KFe2As2 to an orbital-selective Mott transition. We now have good thermodynamic data covering both the hole and electron sides of the BaFe2As2 system and we will discuss how these correlations are modified by doping.

Molecular origin of differences in hole and electron mobility in amorphous Alq3--a multiscale simulation study.

Science.gov (United States)

Fuchs, Andreas; Steinbrecher, Thomas; Mommer, Mario S; Nagata, Yuki; Elstner, Marcus; Lennartz, Christian

2012-03-28

In order to determine the molecular origin of the difference in electron and hole mobilities of amorphous thin films of Alq(3) (meridional Alq(3) (tris(8-hydroxyquinoline) aluminium)) we performed multiscale simulations covering quantum mechanics, molecular mechanics and lattice models. The study includes realistic disordered morphologies, polarized site energies to describe diagonal disorder, quantum chemically calculated transfer integrals for the off-diagonal disorder, inner sphere reorganization energies and an approximative scheme for outer sphere reorganization energies. Intermolecular transfer rates were calculated via Marcus-theory and mobilities were simulated via kinetic Monte Carlo simulations and by a Master Equation approach. The difference in electron and hole mobility originates from the different localization of charge density in the radical anion (more delocalized) compared to the radical cation (more confined). This results in higher diagonal disorder for holes and less favourable overlap properties for the hole transfer integrals leading to an overall higher electron mobility.

Observing the dynamics of supermassive black hole binaries with pulsar timing arrays.

Science.gov (United States)

Mingarelli, C M F; Grover, K; Sidery, T; Smith, R J E; Vecchio, A

2012-08-24

Pulsar timing arrays are a prime tool to study unexplored astrophysical regimes with gravitational waves. Here, we show that the detection of gravitational radiation from individually resolvable supermassive black hole binary systems can yield direct information about the masses and spins of the black holes, provided that the gravitational-wave-induced timing fluctuations both at the pulsar and at Earth are detected. This in turn provides a map of the nonlinear dynamics of the gravitational field and a new avenue to tackle open problems in astrophysics connected to the formation and evolution of supermassive black holes. We discuss the potential, the challenges, and the limitations of these observations.

Direct probing of electron and hole trapping into nano-floating-gate in organic field-effect transistor nonvolatile memories

Energy Technology Data Exchange (ETDEWEB)

Cui, Ze-Qun; Wang, Shun; Chen, Jian-Mei; Gao, Xu; Dong, Bin, E-mail: wangsd@suda.edu.cn, E-mail: chilf@suda.edu.cn, E-mail: bdong@suda.edu.cn; Chi, Li-Feng, E-mail: wangsd@suda.edu.cn, E-mail: chilf@suda.edu.cn, E-mail: bdong@suda.edu.cn; Wang, Sui-Dong, E-mail: wangsd@suda.edu.cn, E-mail: chilf@suda.edu.cn, E-mail: bdong@suda.edu.cn [Jiangsu Key Laboratory for Carbon-Based Functional Materials and Devices, Institute of Functional Nano and Soft Materials (FUNSOM), Soochow University, Suzhou, Jiangsu 215123 (China)

2015-03-23

Electron and hole trapping into the nano-floating-gate of a pentacene-based organic field-effect transistor nonvolatile memory is directly probed by Kelvin probe force microscopy. The probing is straightforward and non-destructive. The measured surface potential change can quantitatively profile the charge trapping, and the surface characterization results are in good accord with the corresponding device behavior. Both electrons and holes can be trapped into the nano-floating-gate, with a preference of electron trapping than hole trapping. The trapped charge quantity has an approximately linear relation with the programming/erasing gate bias, indicating that the charge trapping in the device is a field-controlled process.

Direct probing of electron and hole trapping into nano-floating-gate in organic field-effect transistor nonvolatile memories

International Nuclear Information System (INIS)

Cui, Ze-Qun; Wang, Shun; Chen, Jian-Mei; Gao, Xu; Dong, Bin; Chi, Li-Feng; Wang, Sui-Dong

2015-01-01

Electron and hole trapping into the nano-floating-gate of a pentacene-based organic field-effect transistor nonvolatile memory is directly probed by Kelvin probe force microscopy. The probing is straightforward and non-destructive. The measured surface potential change can quantitatively profile the charge trapping, and the surface characterization results are in good accord with the corresponding device behavior. Both electrons and holes can be trapped into the nano-floating-gate, with a preference of electron trapping than hole trapping. The trapped charge quantity has an approximately linear relation with the programming/erasing gate bias, indicating that the charge trapping in the device is a field-controlled process

Enhancement of tunnel conductivity by Cooper pair fluctuations in electron-hole bilayer

International Nuclear Information System (INIS)

Efimkin, D K; Lozovik, Yu E

2012-01-01

Influence of Cooper pair fluctuations that are precursor of pairing of electrons and holes located on opposite surfaces of topological insulator film on tunnel conductivity between the surfaces is investigated. Due to restrictions caused by momentum and energy conservation dependence of tunnel conductivity on external bias voltage has peak that becomes more prominent with decreasing of disorder and temperature. We have shown that Cooper pair fluctuations considerably enhance tunneling and height of the peak diverges in vicinity of critical temperature with critical index ν = 2. Width of the peak tends to zero in proximity of critical temperature. Pairing of electrons and holes can be suppressed by disorder and in vicinity of quantum critical point height of the peak also diverges as function of Cooper pair damping with critical index μ = 2.

Electron and hole drift mobility measurements on methylammonium lead iodide perovskite solar cells

Energy Technology Data Exchange (ETDEWEB)

Maynard, Brian; Long, Qi; Schiff, Eric A. [Department of Physics, Syracuse University, Syracuse, New York 13244 (United States); Yang, Mengjin; Zhu, Kai [National Renewable Energy Laboratory, Golden, Colorado 80401 (United States); Kottokkaran, Ranjith; Abbas, Hisham; Dalal, Vikram L. [Iowa State University, Ames, Iowa 50011 (United States)

2016-04-25

We report nanosecond domain time-of-flight measurements of electron and hole photocarriers in methylammonium lead iodide perovskite solar cells. The mobilities ranged from 0.06 to 1.4 cm{sup 2}/Vs at room temperature, but there is little systematic difference between the two carriers. We also find that the drift mobilities are dispersive (time-dependent). The dispersion parameters are in the range of 0.4–0.7, and they imply that terahertz domain mobilities will be much larger than nanosecond domain mobilities. The temperature-dependences of the dispersion parameters are consistent with confinement of electron and hole transport to fractal-like spatial networks within nanoseconds of their photogeneration.

High-temperature electron-hole superfluidity with strong anisotropic gaps in double phosphorene monolayers

Science.gov (United States)

Saberi-Pouya, S.; Zarenia, M.; Perali, A.; Vazifehshenas, T.; Peeters, F. M.

2018-05-01

Excitonic superfluidity in double phosphorene monolayers is investigated using the BCS mean-field equations. Highly anisotropic superfluidity is predicted where we found that the maximum superfluid gap is in the Bose-Einstein condensate (BEC) regime along the armchair direction and in the BCS-BEC crossover regime along the zigzag direction. We estimate the highest Kosterlitz-Thouless transition temperature with maximum value up to ˜90 K with onset carrier densities as high as 4 ×1012cm-2 . This transition temperature is significantly larger than what is found in double electron-hole few-layers graphene. Our results can guide experimental research toward the realization of anisotropic condensate states in electron-hole phosphorene monolayers.

Ballistic hole magnetic microscopy

NARCIS (Netherlands)

Haq, E.; Banerjee, T.; Siekman, M.H.; Lodder, J.C.; Jansen, R.

2005-01-01

A technique to study nanoscale spin transport of holes is presented: ballistic hole magnetic microscopy. The tip of a scanning tunneling microscope is used to inject hot electrons into a ferromagnetic heterostructure, where inelastic decay creates a distribution of electron-hole pairs.

Transport Properties of an Electron-Hole Bilayer in Contact with a Superconductor Hybrid Junction

Science.gov (United States)

Bercioux, D.; Klapwijk, T. M.; Bergeret, F. S.

2017-08-01

We investigate the transport properties of a junction consisting of an electron-hole bilayer in contact with normal and superconducting leads. The electron-hole bilayer is considered as a semimetal with two electronic bands. We assume that in the region between the contacts the system hosts an exciton condensate described by a BCS-like model with a gap Γ in the quasiparticle density of states. We first discuss how the subgap electronic transport through the junction is mainly governed by the interplay between two kinds of reflection processes at the interfaces: the standard Andreev reflection at the interface between the superconductor and the exciton condensate, and a coherent crossed reflection at the semimetal-exciton-condensate interface that converts electrons from one layer into the other. We show that the differential conductance of the junction shows a minimum at voltages of the order of Γ /e . Such a minimum can be seen as a direct hallmark of the existence of the gapped excitonic state.

Emission of ultrashort electromagnetic pulses from electron bunches formed and accelerated by laser beams with tilted amplitude fronts

International Nuclear Information System (INIS)

Galkin, A.L.; Korobkin, V.V.; Romanovsky, M.Yu.; Shiryaev, O.B.; Trofimov, V.A.

2013-01-01

The dynamics of an electron in a standing wave generated by a pair of counterpropagating linearly polarized relativistically intense laser pulses and the emission of electromagnetic radiation by the electron are analyzed. The pulses are assumed to have tilted amplitude fronts and asymmetric focal spots. The analysis of the dynamics is performed by solving numerically the Newton equation with the corresponding Lorentz force, and the emission of radiation is simulated based on the Lienard-Wiechert potentials. The electrons are accelerated by the direct action of the standing wave field and are shown to form a small short bunch. For relativistic intensities, the energies gained by the electrons reach several GeV. It is demonstrated that the radiation emitted by the electrons in the bunch is a single electromagnetic pulse confined to a narrow solid angle and having an attosecond duration. (copyright 2013 WILEY-VCH Verlag GmbH and Co. KGaA, Weinheim) (orig.)

Generation of a strong attosecond pulse train with an orthogonally polarized two-color laser field

International Nuclear Information System (INIS)

Kim, Chul Min; Kim, I Jong; Nam, Chang Hee

2005-01-01

We theoretically investigate the high-order harmonic generation from a neon atom irradiated by an intense two-color femtosecond laser pulse, in which the fundamental field and its second harmonic are linearly polarized and orthogonal to each other. In contrast to usual high-harmonic generation with linearly polarized fundamental field alone, a very strong and clean high-harmonic spectrum, consisting of both odd and even orders of harmonics, can be generated in the orthogonally polarized two-color laser field with proper selection of the relative phase between the fundamental and second-harmonic fields. In time domain, this results in a strong and regular attosecond pulse train. The origin of these behaviors is elucidated by analyzing semiclassical electron paths and by simulating high-harmonic generation quantum mechanically

Spectral Interferometry with Electron Microscopes

Science.gov (United States)

Talebi, Nahid

2016-01-01

Interference patterns are not only a defining characteristic of waves, but also have several applications; characterization of coherent processes and holography. Spatial holography with electron waves, has paved the way towards space-resolved characterization of magnetic domains and electrostatic potentials with angstrom spatial resolution. Another impetus in electron microscopy has been introduced by ultrafast electron microscopy which uses pulses of sub-picosecond durations for probing a laser induced excitation of the sample. However, attosecond temporal resolution has not yet been reported, merely due to the statistical distribution of arrival times of electrons at the sample, with respect to the laser time reference. This is however, the very time resolution which will be needed for performing time-frequency analysis. These difficulties are addressed here by proposing a new methodology to improve the synchronization between electron and optical excitations through introducing an efficient electron-driven photon source. We use focused transition radiation of the electron as a pump for the sample. Due to the nature of transition radiation, the process is coherent. This technique allows us to perform spectral interferometry with electron microscopes, with applications in retrieving the phase of electron-induced polarizations and reconstructing dynamics of the induced vector potential. PMID:27649932

Numerical simulation of evolution of electron-hole avalanches and streamers in silicon in a uniform electric field

International Nuclear Information System (INIS)

Kyuregyan, A. S.

2010-01-01

Numerical simulation of origination and evolution of streamers in Si is performed for the first time. It is assumed that an external electric field E 0 is constant and uniform, the avalanche and streamer are axially symmetric, and background electrons and holes are absent. The calculations have been performed in the context of the diffusion-drift approximation with impact and tunneling ionization, Auger recombination, and electron-hole scattering taken into account. The most realistic values of the ionization and recombination rates, diffusion coefficients, and drift mobilities of electrons and holes have been used. It is shown that the features of evolution of avalanches and streamers are generally consistent with the result obtained previously for a hypothetic semiconductor with equal kinetic coefficients for electrons and holes. Asymmetry of these coefficients (mostly, the impact-ionization coefficients) manifests itself only at the initial stage of evolution. However, with time, two exponentially self-similar streamers are formed, differing only in the sign of charge of fronts and directions of their propagation. Empirical dependences of the main parameters of streamers on E 0 in the range of 0.34-0.75 MV/cm have been derived for this most important stage of evolution.

Dynamics of particles around a pseudo-Newtonian Kerr black hole with halos

International Nuclear Information System (INIS)

Wang Ying; Wu Xin

2012-01-01

The regular and chaotic dynamics of test particles in a superposed field between a pseudo-Newtonian Kerr black hole and quadrupolar halos is detailed. In particular, the dependence of dynamics on the quadrupolar parameter of the halos and the spin angular momentum of the rotating black hole is studied. It is found that the small quadrupolar moment, in contrast with the spin angular momentum, does not have a great effect on the stability and radii of the innermost stable circular orbits of these test particles. In addition, chaos mainly occurs for small absolute values of the rotating parameters, and does not exist for the maximum counter-rotating case under some certain initial conditions and parameters. This means that the rotating parameters of the black hole weaken the chaotic properties. It is also found that the counter-rotating system is more unstable than the co-rotating one. Furthermore, chaos is absent for small absolute values of the quadrupoles, and the onset of chaos is easier for the prolate halos than for the oblate ones. (general)

Theory of magnetostriction of electron-hole drops in Ge

International Nuclear Information System (INIS)

Markiewicz, R.S.

1978-01-01

A large mass of electron-hole liquid (γ drop) formed in a strain-induced potential well in Ge is known to distort its shape significantly in a magnetic field B > or approx. = 1 kG. It is shown in this paper that the shape change can be understood in detail as due to a ''recombination current'' of electron-hole pairs needed to replace those pairs which recombine in the drop volume. The Lorentz force deflects this current and produces a macroscopic dipole current loop inside the drop. The drop then changes shape to minimize its total energy, including magnetic, strain, and surface energies. While the drop usually flattens along the field direction, both para- and diamagnetic effects (elongated drops) are found to be possible, depending on excitation conditions, in accord with experiment. Similar effects are predicted to occur in small drops in unstrained Ge. This paper presents a magnetohydrodynamic theory of the magnetostriction which takes into account density variations which occur in the strain well and in high magnetic fields. A simpler theory is given for the special case in which the drop may be considered incompressible (small drops and moderate fields). Effects of carrier mass anisotropy and fluid viscosity are taken into consideration

Interaction of attosecond electromagnetic pulses with atoms: The exactly solvable model

International Nuclear Information System (INIS)

Popov, Yu. V.; Kouzakov, K. A.; Vinitsky, S. I.; Gusev, A. A.

2007-01-01

We consider the exactly solvable model of interaction of zero-duration electromagnetic pulses with an atom. The model has a number of peculiar properties which are outlined in the cases of a single pulse and two opposite pulses. In perspective, it can be useful in different fields of physics involving interaction of attosecond laser pulses with quantum systems

Crossover between the dense electron-hole phase and the BCS excitonic phase in quantum dots

International Nuclear Information System (INIS)

Rodriguez, B.A.; Gonzalez, A.; Quiroga, L.; Capote, R.; Rodriguez, F.J.

1999-09-01

Second order perturbation theory and a Lipkin-Nogami scheme combined with an exact Monte Carlo projection after variation are applied to compute the ground-state energy of 6 ≤ N ≤ 210 electron-hole pairs confined in a parabolic two-dimensional quantum dot. The energy shows nice scaling properties as N or the confinement strength is varied. A crossover from the high-density electron-hole phase to the BCS excitonic phase is found at a density which is roughly four times the close-packing density of excitons. (author)

Electron, hole and exciton self-trapping in germanium doped silica glass from DFT calculations with self-interaction correction

International Nuclear Information System (INIS)

Du Jincheng; Rene Corrales, L.; Tsemekhman, Kiril; Bylaska, Eric J.

2007-01-01

Density functional theory (DFT) calculations were employed to understand the refractive index change in germanium doped silica glasses for the trapped states of electronic excitations induced by UV irradiation. Local structure relaxation and excess electron density distribution were calculated upon self-trapping of an excess electron, hole, and exciton in germanium doped silica glass. The results show that both the trapped exciton and excess electron are highly localized on germanium ion and, to some extent, on its oxygen neighbors. Exciton self-trapping is found to lead to the formation of a Ge E' center and a non-bridging hole center. Electron trapping changes the GeO 4 tetrahedron structure into trigonal bi-pyramid with the majority of the excess electron density located along the equatorial line. The self-trapped hole is localized on bridging oxygen ions that are not coordinated to germanium atoms that lead to elongation of the Si-O bonds and change of the Si-O-Si bond angles. We carried out a comparative study of standard DFT versus DFT with a hybrid PBE0 exchange and correlation functional. The results show that the two methods give qualitatively similar relaxed structure and charge distribution for electron and exciton trapping in germanium doped silica glass; however, only the PBE0 functional produces the self-trapped hole

Electron-positron pairs in physics and astrophysics: From heavy nuclei to black holes

Science.gov (United States)

Ruffini, Remo; Vereshchagin, Gregory; Xue, She-Sheng

2010-02-01

scales. What has become clear in the last ten years is that all the three above mentioned processes, duly extended in the general relativistic framework, are necessary for the understanding of the physics of the gravitational collapse to a black hole. Vice versa, the natural arena where these processes can be observed in mutual interaction and on an unprecedented scale, is indeed the realm of relativistic astrophysics. We systematically analyze the conceptual developments which have followed the basic work of Dirac and Breit-Wheeler. We also recall how the seminal work of Born and Infeld inspired the work by Sauter, Heisenberg and Euler on effective Lagrangian leading to the estimate of the rate for the process of electron-positron production in a constant electric field. In addition to reviewing the intuitive semi-classical treatment of quantum mechanical tunneling for describing the process of electron-positron production, we recall the calculations in Quantum Electro-Dynamics of the Schwinger rate and effective Lagrangian for constant electromagnetic fields. We also review the electron-positron production in both time-alternating electromagnetic fields, studied by Brezin, Itzykson, Popov, Nikishov and Narozhny, and the corresponding processes relevant for pair production at the focus of coherent laser beams as well as electron-beam-laser collision. We finally report some current developments based on the general JWKB approach which allows us to compute the Schwinger rate in spatially varying and time varying electromagnetic fields. We also recall the pioneering work of Landau and Lifshitz, and Racah on the collision of charged particles as well as the experimental success of AdA and ADONE in the production of electron-positron pairs. We then turn to the possible experimental verification of these phenomena. We review: (A) the experimental verification of the e+e-→2γ process studied by Dirac. We also briefly recall the very successful experiments of e

Dynamical manifestations of quantum chaos: correlation hole and bulge

Science.gov (United States)

Torres-Herrera, E. J.; Santos, Lea F.

2017-10-01

A main feature of a chaotic quantum system is a rigid spectrum where the levels do not cross. We discuss how the presence of level repulsion in lattice many-body quantum systems can be detected from the analysis of their time evolution instead of their energy spectra. This approach is advantageous to experiments that deal with dynamics, but have limited or no direct access to spectroscopy. Dynamical manifestations of avoided crossings occur at long times. They correspond to a drop, referred to as correlation hole, below the asymptotic value of the survival probability and to a bulge above the saturation point of the von Neumann entanglement entropy and the Shannon information entropy. By contrast, the evolution of these quantities at shorter times reflects the level of delocalization of the initial state, but not necessarily a rigid spectrum. The correlation hole is a general indicator of the integrable-chaos transition in disordered and clean models and as such can be used to detect the transition to the many-body localized phase in disordered interacting systems. This article is part of the themed issue 'Breakdown of ergodicity in quantum systems: from solids to synthetic matter'.

On the physics of electron ejection from laser-irradiated overdense plasmas

Energy Technology Data Exchange (ETDEWEB)

Thévenet, M.; Vincenti, H.; Faure, J. [Laboratoire d' Optique Appliquée, ENSTA ParisTech, CNRS, Ecole Polytechnique, Université Paris-Saclay, 828 bd des Maréchaux, 91762 Palaiseau Cedex (France)

2016-06-15

Using 1D and 2D PIC simulations, we describe and model the backward ejection of electron bunches when a laser pulse reflects off an overdense plasma with a short density gradient on its front side. The dependence on the laser intensity and gradient scale length is studied. It is found that during each laser period, the incident laser pulse generates a large charge-separation field, or plasma capacitor, which accelerates an attosecond bunch of electrons toward vacuum. This process is maximized for short gradient scale lengths and collapses when the gradient scale length is comparable to the laser wavelength. We develop a model that reproduces the electron dynamics and the dependence on laser intensity and gradient scale length. This process is shown to be strongly linked with high harmonic generation via the Relativistic Oscillating Mirror mechanism.

Femtosecond-laser induced dynamics of CO on Ru(0001): Deep insights from a hot-electron friction model including surface motion

Science.gov (United States)

Scholz, Robert; Floß, Gereon; Saalfrank, Peter; Füchsel, Gernot; Lončarić, Ivor; Juaristi, J. I.

2016-10-01

A Langevin model accounting for all six molecular degrees of freedom is applied to femtosecond-laser induced, hot-electron driven dynamics of Ru(0001)(2 ×2 ):CO. In our molecular dynamics with electronic friction approach, a recently developed potential energy surface based on gradient-corrected density functional theory accounting for van der Waals interactions is adopted. Electronic friction due to the coupling of molecular degrees of freedom to electron-hole pairs in the metal are included via a local density friction approximation, and surface phonons by a generalized Langevin oscillator model. The action of ultrashort laser pulses enters through a substrate-mediated, hot-electron mechanism via a time-dependent electronic temperature (derived from a two-temperature model), causing random forces acting on the molecule. The model is applied to laser induced lateral diffusion of CO on the surface, "hot adsorbate" formation, and laser induced desorption. Reaction probabilities are strongly enhanced compared to purely thermal processes, both for diffusion and desorption. Reaction yields depend in a characteristic (nonlinear) fashion on the applied laser fluence, as well as branching ratios for various reaction channels. Computed two-pulse correlation traces for desorption and other indicators suggest that aside from electron-hole pairs, phonons play a non-negligible role for laser induced dynamics in this system, acting on a surprisingly short time scale. Our simulations on precomputed potentials allow for good statistics and the treatment of long-time dynamics (300 ps), giving insight into this system which hitherto has not been reached. We find generally good agreement with experimental data where available and make predictions in addition. A recently proposed laser induced population of physisorbed precursor states could not be observed with the present low-coverage model.

Electron-hole pairs generated in ZrO2 nanoparticle resist upon exposure to extreme ultraviolet radiation

Science.gov (United States)

Kozawa, Takahiro; Santillan, Julius Joseph; Itani, Toshiro

2018-02-01

Metal oxide nanoparticle resists have attracted much attention as the next-generation resist used for the high-volume production of semiconductor devices. However, the sensitization mechanism of the metal oxide nanoparticle resists is unknown. Understanding the sensitization mechanism is important for the efficient development of resist materials. In this study, the energy deposition in a zirconium oxide (ZrO2) nanoparticle resist was investigated. The numbers of electron-hole pairs generated in a ZrO2 core and an methacrylic acid (MAA) ligand shell upon exposure to 1 mJ cm-2 (exposure dose) extreme ultraviolet (EUV) radiations were theoretically estimated to be 0.16 at most and 0.04-0.17 cm2 mJ-1, respectively. By comparing the calculated distribution of electron-hole pairs with the line-and-space patterns of the ZrO2 nanoparticle resist fabricated by an EUV exposure tool, the number of electron-hole pairs required for the solubility change of the resist films was estimated to be 1.3-2.2 per NP. NP denotes a nanoparticle consisting of a metal oxide core with a ligand shell. In the material design of metal oxide nanoparticle resists, it is important to efficiently use the electron-hole pairs generated in the metal oxide core for the chemical change of ligand molecules.

A theory of electron baths: One-electron system dynamics

International Nuclear Information System (INIS)

McDowell, H.K.

1992-01-01

The second-quantized, many-electron, atomic, and molecular Hamiltonian is partitioned both by the identity or labeling of the spin orbitals and by the dynamics of the spin orbitals into a system coupled to a bath. The electron bath is treated by a molecular time scale generalized Langevin equation approach designed to include one-electron dynamics in the system dynamics. The bath is formulated as an equivalent chain of spin orbitals through the introduction of equivalent-chain annihilation and creation operators. Both the dynamics and the quantum grand canonical statistical properties of the electron bath are examined. Two versions for the statistical properties of the bath are pursued. Using a weak bath assumption, a bath statistical average is defined which allows one to achieve a reduced dynamics description of the electron system which is coupled to the electron bath. In a strong bath assumption effective Hamiltonians are obtained which reproduce the dynamics of the bath and which lead to the same results as found in the weak bath assumption. The effective (but exact) Hamiltonian is found to be a one-electron Hamiltonian. A reduced dynamics equation of motion for the system population matrix is derived and found to agree with a previous version. This equation of motion is useful for studying electron transfer in the system when coupled to an electron bath

Membrane viewpoint on black holes: Dynamical electromagnetic fields near the horizon

International Nuclear Information System (INIS)

Macdonald, D.A.; Suen, W.

1985-01-01

This paper is part of a series of papers with the aim of developing a complete self-consistent formalism for the treatment of electromagnetic and gravitational fields in the neighborhood of a black-hole horizon. In this membrane formalism, the horizon is treated as a closed two-dimensional membrane lying in a curved three-dimensional space, and endowed with familiar physical properties such as entropy and temperature, surface pressure and viscosity, and electrical conductivity, charge, and current. This paper develops the concept of the ''stretched horizon,'' which will be vital for both the electromagnetic and gravitational aspects of the formalism, and it presents several model problems illustrating the interaction of dynamical electromagnetic fields with stationary black-hole horizons: The field of a test charge in various states of motion outside the Schwarzschild horizon is analyzed in the near-horizon limit, where the spatial curvature may be ignored and the metric may be approximated by that of Rindler. This analysis elucidates the influence of the horizon on the shapes and motions of electric and magnetic field lines when external agents move the field lines in arbitrary manners. It also illustrates how the field lines interact with the horizon's charge and current to produce an exchange of energy and momentum between the external agent and the horizon. A numerical calculation of the dynamical relaxation of a magnetic field threading a Schwarzschild black hole is also presented, illustrating the ''cleaning'' of a complicated field structure by a black-hole horizon, and elucidating the constraints on the location of the stretched horizon

Frequency chirp of harmonic and attosecond pulses

International Nuclear Information System (INIS)

Varju, K.; Johansson, P; L'Huillier, A.L.; Mairesse, Y.; Salieres, P.

2005-01-01

Full text: We have explored in detail the first- and second-order variations of the atomic phase as a function of the laser intensity and harmonic order. This unravels the similitudes and differences existing between the chirp of individual harmonic pulses and the chirp of the attosecond pulses. We show that the two techniques XFROG and RABITT used to characterize the two chirps (respectively) converge to give the same information, namely the values of the mixed partial derivatives of the atomic phase. This underlines the common physical origin of all these phenomena and provides a unified frame for their description and understanding. Ref. 1 (author)

Spectral hole-burning and carrier-heating dynamics in InGaAs quantum-dot amplifiers

DEFF Research Database (Denmark)

Borri, Paola; Langbein, Wolfgang Werner; Hvam, Jørn Märcher

2000-01-01

recovery of the spectral hole within ~100 fs is measured, comparable to bulk and quantum-well amplifiers, which is contradicting a carrier relaxation bottleneck in electrically pumped QD devices. The CH dynamics in the QD is quantitatively compared with results on an InGaAsP bulk amplifier. Reduced CH......The ultrafast gain and index dynamics in a set of InAs-InGaAs-GaAs quantum-dot (QD) amplifiers are measured at room temperature with femtosecond resolution. The role of spectral hole-burning (SHB) and carrier heating (CH) in the recovery of gain compression is investigated in detail. An ultrafast...

Landau damping effects on collision-induced quantum interference in electron-hole plasmas

International Nuclear Information System (INIS)

Hwa-Min, Kim; Young-Dae, Jung

2007-01-01

The Landau damping effects on the quantum interference in electron collisions are investigated in a quantum plasma composed of electrons and holes. The Born method and the total spin states are considered to obtain the scattering cross-section by using the effective screened potential model. It is found that the Landau damping effects enhance the scattering cross-section, especially, near the scattering angle θ L = π/4. (authors)

Landau damping effects on collision-induced quantum interference in electron-hole plasmas

Energy Technology Data Exchange (ETDEWEB)

Hwa-Min, Kim [Daegu Univ. Catholic, Dept. of Electronics Engineering (Korea, Republic of); Young-Dae, Jung [Hanyang Univ., Dept. of Applied Physics, Seoul (Korea, Republic of)

2007-07-15

The Landau damping effects on the quantum interference in electron collisions are investigated in a quantum plasma composed of electrons and holes. The Born method and the total spin states are considered to obtain the scattering cross-section by using the effective screened potential model. It is found that the Landau damping effects enhance the scattering cross-section, especially, near the scattering angle {theta}{sub L} = {pi}/4. (authors)

Assessment of pseudo-bilayer structures in the heterogate germanium electron-hole bilayer tunnel field-effect transistor

International Nuclear Information System (INIS)

Padilla, J. L.; Alper, C.; Ionescu, A. M.; Medina-Bailón, C.; Gámiz, F.

2015-01-01

We investigate the effect of pseudo-bilayer configurations at low operating voltages (≤0.5 V) in the heterogate germanium electron-hole bilayer tunnel field-effect transistor (HG-EHBTFET) compared to the traditional bilayer structures of EHBTFETs arising from semiclassical simulations where the inversion layers for electrons and holes featured very symmetric profiles with similar concentration levels at the ON-state. Pseudo-bilayer layouts are attained by inducing a certain asymmetry between the top and the bottom gates so that even though the hole inversion layer is formed at the bottom of the channel, the top gate voltage remains below the required value to trigger the formation of the inversion layer for electrons. Resulting benefits from this setup are improved electrostatic control on the channel, enhanced gate-to-gate efficiency, and higher I ON levels. Furthermore, pseudo-bilayer configurations alleviate the difficulties derived from confining very high opposite carrier concentrations in very thin structures

Assessment of pseudo-bilayer structures in the heterogate germanium electron-hole bilayer tunnel field-effect transistor

Energy Technology Data Exchange (ETDEWEB)

Padilla, J. L., E-mail: jose.padilladelatorre@epfl.ch; Alper, C.; Ionescu, A. M. [Nanoelectronic Devices Laboratory, École Polytechnique Fédérale de Lausanne, Lausanne CH-1015 (Switzerland); Medina-Bailón, C.; Gámiz, F. [Departamento de Electrónica y Tecnología de los Computadores, Universidad de Granada, Avda. Fuentenueva s/n, 18071 Granada (Spain)

2015-06-29

We investigate the effect of pseudo-bilayer configurations at low operating voltages (≤0.5 V) in the heterogate germanium electron-hole bilayer tunnel field-effect transistor (HG-EHBTFET) compared to the traditional bilayer structures of EHBTFETs arising from semiclassical simulations where the inversion layers for electrons and holes featured very symmetric profiles with similar concentration levels at the ON-state. Pseudo-bilayer layouts are attained by inducing a certain asymmetry between the top and the bottom gates so that even though the hole inversion layer is formed at the bottom of the channel, the top gate voltage remains below the required value to trigger the formation of the inversion layer for electrons. Resulting benefits from this setup are improved electrostatic control on the channel, enhanced gate-to-gate efficiency, and higher I{sub ON} levels. Furthermore, pseudo-bilayer configurations alleviate the difficulties derived from confining very high opposite carrier concentrations in very thin structures.

Interaction of relativistic electrons with an intense laser pulse: High-order harmonic generation based on Thomson scattering

International Nuclear Information System (INIS)

Hack, Szabolcs; Varró, Sándor; Czirják, Attila

2016-01-01

We investigate nonlinear Thomson scattering as a source of high-order harmonic radiation with the potential to enable attosecond light pulse generation. We present a new analytic solution of the electron’s relativistic equations of motion in the case of a short laser pulse with a sine-squared envelope. Based on the single electron emission, we compute and analyze the radiated amplitude and phase spectrum for a realistic electron bunch, with special attention to the correct initial values. These results show that the radiation spectrum of an electron bunch in head-on collision with a sufficiently strong laser pulse of sine-squared envelope has a smooth frequency dependence to allow for the synthesis of attosecond light pulses.

Interaction of relativistic electrons with an intense laser pulse: High-order harmonic generation based on Thomson scattering

Energy Technology Data Exchange (ETDEWEB)

Hack, Szabolcs [ELI-ALPS, ELI-HU Non-Profit Ltd., Dugonics tér 13, H-6720 Szeged (Hungary); Department of Theoretical Physics, University of Szeged, Tisza L. krt. 84-86, H-6720 Szeged (Hungary); Varró, Sándor [ELI-ALPS, ELI-HU Non-Profit Ltd., Dugonics tér 13, H-6720 Szeged (Hungary); Wigner Research Center for Physics, SZFI, PO Box 49, H-1525 Budapest (Hungary); Czirják, Attila [ELI-ALPS, ELI-HU Non-Profit Ltd., Dugonics tér 13, H-6720 Szeged (Hungary); Department of Theoretical Physics, University of Szeged, Tisza L. krt. 84-86, H-6720 Szeged (Hungary)

2016-02-15

We investigate nonlinear Thomson scattering as a source of high-order harmonic radiation with the potential to enable attosecond light pulse generation. We present a new analytic solution of the electron’s relativistic equations of motion in the case of a short laser pulse with a sine-squared envelope. Based on the single electron emission, we compute and analyze the radiated amplitude and phase spectrum for a realistic electron bunch, with special attention to the correct initial values. These results show that the radiation spectrum of an electron bunch in head-on collision with a sufficiently strong laser pulse of sine-squared envelope has a smooth frequency dependence to allow for the synthesis of attosecond light pulses.

Is there a hole in the topside, equatorial ionosphere?

Directory of Open Access Journals (Sweden)

D. Gallagher

Full Text Available A paper in 2000 (Huba, 2000 found a depression in electron density in the topside ionosphere near the magnetic equator, based on the SAMI-2 physical ionospheric model. The model showed, for the first time, the formation of a hole in electron density in the altitude range 1500–2500 km at geomagnetic equatorial latitudes. The model produced the hole because of transhemispheric O+ flows that collisionally couple to H+, transporting it to lower altitudes, and thereby reducing the electron density at high altitudes. At that time and until now, no published observations have been reported to confirm or refute this numerical result. Recent, new analysis of Dynamics Explorer 1 Retarding Ion Mass Spectrometer measurements provides the first tentative experimental support for this model result. Keywords: Ionosphere, Topside, Magnetic equator, Plasmasphere

Control of electron localization to isolate and enhance molecular harmonic plateau in asymmetric HeH2+ system

International Nuclear Information System (INIS)

Lu, Ruifeng; Yu, Chao; Wang, Yunhui; Shi, Qi; Zhang, Yadong

2014-01-01

High-order harmonic generation from the asymmetric molecular ion HeH 2+ exposed to intense laser fields was investigated by quantum wave packet calculations in which the initial wave packet of HeH 2+ was prepared in the first excited 2pσ state. The calculated molecular harmonic plateau at low frequencies was effectively isolated and enhanced by adjusting the carrier-envelope phase (CEP) of the laser field. Furthermore, double-well model, time-dependent electronic density, electronic state population, and time-frequency analyses were presented to explain the underlying mechanism of the efficient isolated molecular plateau. By taking advantage of the CEP effect to control the electronic dynamics, this isolated molecular plateau can be used to generate high-intensity single attosecond pulses.

New theoretical approaches to atomic and molecular dynamics triggered by ultrashort light pulses on the atto- to picosecond time scale

International Nuclear Information System (INIS)

Pabst, Stefan Ulf

2013-04-01

The concept of atoms as the building blocks of matter has existed for over 3000 years. A revolution in the understanding and the description of atoms and molecules has occurred in the last century with the birth of quantum mechanics. After the electronic structure was understood, interest in studying the dynamics of electrons, atoms, and molecules increased. However, time-resolved investigations of these ultrafast processes were not possible until recently. The typical time scale of atomic and molecular processes is in the picosecond to attosecond realm. Tremendous technological progress in recent years makes it possible to generate light pulses on these time scales. With such ultrashort pulses, atomic and molecular dynamics can be triggered, watched, and controlled. Simultaneously, the need rises for theoretical models describing the underlying mechanisms. This doctoral thesis focuses on the development of theoretical models which can be used to study the dynamical behavior of electrons, atoms, and molecules in the presence of ultrashort light pulses. Several examples are discussed illustrating how light pulses can trigger and control electronic, atomic, and molecular motions. In the first part of this work, I focus on the rotational motion of asymmetric molecules, which happens on picosecond and femtosecond time scales. Here, the aim is to align all three axes of the molecule as well as possible. To investigate theoretically alignment dynamics, I developed a program that can describe alignment motion ranging from the impulsive to the adiabatic regime. The asymmetric molecule SO 2 is taken as an example to discuss strategies of optimizing 3D alignment without the presence of an external field (i.e., field-free alignment). Field-free alignment is particularly advantageous because subsequent experiments on the aligned molecule are not perturbed by the aligning light pulse. Wellaligned molecules in the gas phase are suitable for diffraction experiments. From the

New theoretical approaches to atomic and molecular dynamics triggered by ultrashort light pulses on the atto- to picosecond time scale

Energy Technology Data Exchange (ETDEWEB)

Pabst, Stefan Ulf

2013-04-15

The concept of atoms as the building blocks of matter has existed for over 3000 years. A revolution in the understanding and the description of atoms and molecules has occurred in the last century with the birth of quantum mechanics. After the electronic structure was understood, interest in studying the dynamics of electrons, atoms, and molecules increased. However, time-resolved investigations of these ultrafast processes were not possible until recently. The typical time scale of atomic and molecular processes is in the picosecond to attosecond realm. Tremendous technological progress in recent years makes it possible to generate light pulses on these time scales. With such ultrashort pulses, atomic and molecular dynamics can be triggered, watched, and controlled. Simultaneously, the need rises for theoretical models describing the underlying mechanisms. This doctoral thesis focuses on the development of theoretical models which can be used to study the dynamical behavior of electrons, atoms, and molecules in the presence of ultrashort light pulses. Several examples are discussed illustrating how light pulses can trigger and control electronic, atomic, and molecular motions. In the first part of this work, I focus on the rotational motion of asymmetric molecules, which happens on picosecond and femtosecond time scales. Here, the aim is to align all three axes of the molecule as well as possible. To investigate theoretically alignment dynamics, I developed a program that can describe alignment motion ranging from the impulsive to the adiabatic regime. The asymmetric molecule SO{sub 2} is taken as an example to discuss strategies of optimizing 3D alignment without the presence of an external field (i.e., field-free alignment). Field-free alignment is particularly advantageous because subsequent experiments on the aligned molecule are not perturbed by the aligning light pulse. Wellaligned molecules in the gas phase are suitable for diffraction experiments. From the

Peripheral Hole Acceptor Moieties on an Organic Dye Improve Dye‐Sensitized Solar Cell Performance

Science.gov (United States)

Hao, Yan; Gabrielsson, Erik; Lohse, Peter William; Yang, Wenxing; Johansson, Erik M. J.; Hagfeldt, Anders

2015-01-01

Investigation of charge transfer dynamics in dye‐sensitized solar cells is of fundamental interest and the control of these dynamics is a key factor for developing more efficient solar cell devices. One possibility for attenuating losses through recombination between injected electrons and oxidized dye molecules is to move the positive charge further away from the metal oxide surface. For this purpose, a metal‐free dye named E6 is developed, in which the chromophore core is tethered to two external triphenylamine (TPA) units. After photoinduced electron injection into TiO2, the remaining hole is rapidly transferred to a peripheral TPA unit. Electron–hole recombination is slowed down by 30% compared to a reference dye without peripheral TPA units. Furthermore, it is found that the added TPA moieties improve the electron blocking effect of the dye, retarding recombination of electrons from TiO2 to the cobalt‐based electrolyte. PMID:27722076

Vibrational lifetimes of hydrogen on lead films: An ab initio molecular dynamics with electronic friction (AIMDEF) study

Energy Technology Data Exchange (ETDEWEB)

Saalfrank, Peter [Institut für Chemie, Universität Potsdam, Karl-Liebknecht-Strasse 24-25, D-14476 Potsdam (Germany); Donostia International Physics Center (DIPC), Paseo Manuel de Lardizabal 4, 20018 Donostia-San Sebastián (Spain); Juaristi, J. I. [Donostia International Physics Center (DIPC), Paseo Manuel de Lardizabal 4, 20018 Donostia-San Sebastián (Spain); Centro de Física de Materiales CFM/MPC (CSIC-UPV/EHU), Paseo Manuel de Lardizabal 5, 20018 Donostia-San Sebastián (Spain); Departamento de Física de Materiales, Facultad de Químicas UPV/EHU, Apartado 1072, 20018 Donostia-San Sebastián (Spain); Alducin, M.; Muiño, R. Díez [Donostia International Physics Center (DIPC), Paseo Manuel de Lardizabal 4, 20018 Donostia-San Sebastián (Spain); Centro de Física de Materiales CFM/MPC (CSIC-UPV/EHU), Paseo Manuel de Lardizabal 5, 20018 Donostia-San Sebastián (Spain); Blanco-Rey, M. [Donostia International Physics Center (DIPC), Paseo Manuel de Lardizabal 4, 20018 Donostia-San Sebastián (Spain); Departamento de Física de Materiales, Facultad de Químicas UPV/EHU, Apartado 1072, 20018 Donostia-San Sebastián (Spain)

2014-12-21

Using density functional theory and Ab Initio Molecular Dynamics with Electronic Friction (AIMDEF), we study the adsorption and dissipative vibrational dynamics of hydrogen atoms chemisorbed on free-standing lead films of increasing thickness. Lead films are known for their oscillatory behaviour of certain properties with increasing thickness, e.g., energy and electron spillout change in discontinuous manner, due to quantum size effects [G. Materzanini, P. Saalfrank, and P. J. D. Lindan, Phys. Rev. B 63, 235405 (2001)]. Here, we demonstrate that oscillatory features arise also for hydrogen when chemisorbed on lead films. Besides stationary properties of the adsorbate, we concentrate on finite vibrational lifetimes of H-surface vibrations. As shown by AIMDEF, the damping via vibration-electron hole pair coupling dominates clearly over the vibration-phonon channel, in particular for high-frequency modes. Vibrational relaxation times are a characteristic function of layer thickness due to the oscillating behaviour of the embedding surface electronic density. Implications derived from AIMDEF for frictional many-atom dynamics, and physisorbed species will also be given.

Angular dependence of the attosecond time delay in the H 2 + ion

Science.gov (United States)

Kheifets, Anatoli; Serov, Vladislav

2016-05-01

Angular dependence of attosecond time delay relative to polarization of light can now be measured using combination of RABBITT and COLTRIMS techniques. This dependence brings particularly useful information in molecules where it is sensitive to the orientation of the molecular axis. Here we extend the theoretical studies of and consider a molecular ion H2+in combination of an attosecond pulse train and a dressing IR field which is a characteristic set up of a RABBIT measurement. We solve the time-dependent Schrödinger equation using a fast spherical Bessel transformation (SBT) for the radial variable, a discrete variable representation for the angular variables and a split-step technique for the time evolution. The use of SBT ensures correct phase of the wave function for a long time evolution which is especially important in time delay calculations. To speed up computations, we implement an expanding coordinate (EC) system which allows us to reach space sizes and time periods unavailable by other techniques. Australian Research Council DP120101805.

Geometry and dynamics of a tidally deformed black hole

International Nuclear Information System (INIS)

Poisson, Eric; Vlasov, Igor

2010-01-01

The metric of a nonrotating black hole deformed by a tidal interaction is calculated and expressed as an expansion in the strength of the tidal coupling. The expansion parameter is the inverse length scale R -1 , where R is the radius of curvature of the external spacetime in which the black hole moves. The expansion begins at order R -2 , and it is carried out through order R -4 . The metric is parametrized by a number of tidal multipole moments, which specify the black hole's tidal environment. The tidal moments are freely-specifiable functions of time that are related to the Weyl tensor of the external spacetime. At order R -2 the metric involves the tidal quadrupole moments E ab and B ab . At order R -3 it involves the time derivative of the quadrupole moments and the tidal octupole moments E abc and B abc . At order R -4 the metric involves the second time derivative of the quadrupole moments, the first time derivative of the octupole moments, the tidal hexadecapole moments E abcd and B abcd , and bilinear combinations of the quadrupole moments. The metric is presented in a light-cone coordinate system that possesses a clear geometrical meaning: The advanced-time coordinate v is constant on past light cones that converge toward the black hole; the angles θ and φ are constant on the null generators of each light cone; and the radial coordinate r is an affine parameter on each generator, which decreases as the light cones converge toward the black hole. The coordinates are well-behaved on the black-hole horizon, and they are adjusted so that the coordinate description of the horizon is the same as in the Schwarzschild geometry: r=2M+O(R -5 ). At the order of accuracy maintained in this work, the horizon is a stationary null hypersurface foliated by apparent horizons; it is an isolated horizon in the sense of Ashtekar and Krishnan. As an application of our results we examine the induced geometry and dynamics of the horizon, and calculate the rate at which the

Different regimes of electronic coupling and their influence on exciton recombination in vertically stacked InAs/InP quantum wires

International Nuclear Information System (INIS)

Fuster, David; Martinez-Pastor, Juan; Gonzalez, Luisa; Gonzalez, Yolanda

2006-01-01

In the present work we study the influence of stacking self-assembled InAs quantum wires (QWRs) on the emission wavelength and the excitonic recombination dynamics. The reduction in the InP spacer layer thickness, d(InP), produces both a size filtering effect towards large wire ensembles and an increase in the vertical coupling for electrons and holes along the stack direction. The different vertical coupling for electrons and holes induces a different behaviour in the exciton recombination dynamics, depending on the InP spacer layer thickness: weak electron coupling and negligible hole coupling for d(InP) > 10 nm, intermediate electron coupling and weak hole coupling for 5 nm ≤ d(InP) ≤ 10 nm and strong electron coupling and moderate hole coupling for d(InP) < 5 nm. Such exciton dynamics have been established by comparing the experimental time decay results with a multi-quantum well model accounting for the vertical carrier coupling

Hole and electron extraction layers based on graphene oxide derivatives for high-performance bulk heterojunction solar cells.

Science.gov (United States)

Liu, Jun; Xue, Yuhua; Gao, Yunxiang; Yu, Dingshan; Durstock, Michael; Dai, Liming

2012-05-02

By charge neutralization of carboxylic acid groups in graphene oxide (GO) with Cs(2)CO(3) to afford Cesium-neutralized GO (GO-Cs), GO derivatives with appropriate modification are used as both hole- and electron-extraction layers for bulk heterojunction (BHJ) solar cells. The normal and inverted devices based on GO hole- and GO-Cs electron-extraction layers both outperform the corresponding standard BHJ solar cells. Copyright © 2012 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

Magnetometry of low-dimensional electron and hole systems

Energy Technology Data Exchange (ETDEWEB)

Usher, A [School of Physics, University of Exeter, Stocker Road, Exeter EX4 4QL (United Kingdom); Elliott, M [School of Physics and Astronomy, Cardiff University, Queens Buildings, Cardiff CF24 3AA (United Kingdom)], E-mail: a.usher@exeter.ac.uk, E-mail: elliottm@cf.ac.uk

2009-03-11

The high-magnetic-field, low-temperature magnetic properties of low-dimensional electron and hole systems reveal a wealth of fundamental information. Quantum oscillations of the thermodynamic equilibrium magnetization yield the total density of states, a central quantity in understanding the quantum Hall effect in 2D systems. The magnetization arising from non-equilibrium circulating currents reveals details, not accessible with traditional measurements, of the vanishingly small longitudinal resistance in the quantum Hall regime. We review how the technique of magnetometry has been applied to these systems, the most important discoveries that have been made, and their theoretical significance. (topical review)

K-shell-hole production, multiple-hole production, charge transfer, and antisymmetry

International Nuclear Information System (INIS)

Reading, J.F.; Ford, A.L.

1980-01-01

In calculating K-shell-hole production when an ion collides with an atom, account must be taken of the fact that processes involving electrons other than the K-shell electron can occur. For example, after making a K-shell hole an L-shell electron may be knocked into it, or an L-shell vacancy may be produced and the K-shell electron promoted to that vacancy in the ''Fermi sea'' of the target-atom orbitals. In 1973 a theorem was proved by one of the present authors demonstrating that all these multielectron processes cancel in an independent-particle model for the target atom. In this paper it is shown that the same thing occurs for hole production by charge transfer to the ion. The authors demonstrate that multihole production does not obey this simple rule and that the probability for multihole production is not the product of independent single-electron probabilities. The correct expressions that should be used for these processes are given, together with new results for charge-transfer processes accompanied by hole production

Resonant third-harmonic generation of a short-pulse laser from electron-hole plasmas

Energy Technology Data Exchange (ETDEWEB)

Kant, Niti [Department of Physics, Lovely Professional University, Phagwara, Punjab 144 402 (India); Nandan Gupta, Devki [Department of Physics and Astrophysics, University of Delhi, Delhi 110 007 (India); Suk, Hyyong [Advanced Photonics Research Institute (APRI) and Graduate Program of Photonics and Applied Physics, Gwangju Institute of Science and Technology, Gwangju 500 712 (Korea, Republic of)

2012-01-15

In semiconductors, free carriers are created in pairs in inter-band transitions and consist of an electron and its corresponding hole. At very high carrier densities, carrier-carrier collisions dominate over carrier-lattice collisions and carriers begin to behave collectively to form plasma. Here, we apply a short-pulse laser to generate third-harmonic radiation from a semiconductor plasma (electron-hole plasma) in the presence of a transverse wiggler magnetic-field. The process of third-harmonic generation of an intense short-pulse laser is resonantly enhanced by the magnetic wiggler, i.e., wiggler magnetic field provides the necessary momentum to third-harmonic photons. In addition, a high-power laser radiation, propagating through a semiconductor imparts an oscillatory velocity to the electrons and exerts a ponderomotive force on electrons at the third-harmonic frequency of the laser. This oscillatory velocity produces a third-harmonic longitudinal current. And due to the beating of the longitudinal electron velocity and the wiggler magnetic field, a transverse third-harmonic current is produced that drives third-harmonic electromagnetic radiation. It is finally observed that for a specific wiggler wave number value, the phase-matching conditions for the process are satisfied, leading to resonant enhancement in the energy conversion efficiency.

Resonant third-harmonic generation of a short-pulse laser from electron-hole plasmas

International Nuclear Information System (INIS)

Kant, Niti; Nandan Gupta, Devki; Suk, Hyyong

2012-01-01

In semiconductors, free carriers are created in pairs in inter-band transitions and consist of an electron and its corresponding hole. At very high carrier densities, carrier-carrier collisions dominate over carrier-lattice collisions and carriers begin to behave collectively to form plasma. Here, we apply a short-pulse laser to generate third-harmonic radiation from a semiconductor plasma (electron-hole plasma) in the presence of a transverse wiggler magnetic-field. The process of third-harmonic generation of an intense short-pulse laser is resonantly enhanced by the magnetic wiggler, i.e., wiggler magnetic field provides the necessary momentum to third-harmonic photons. In addition, a high-power laser radiation, propagating through a semiconductor imparts an oscillatory velocity to the electrons and exerts a ponderomotive force on electrons at the third-harmonic frequency of the laser. This oscillatory velocity produces a third-harmonic longitudinal current. And due to the beating of the longitudinal electron velocity and the wiggler magnetic field, a transverse third-harmonic current is produced that drives third-harmonic electromagnetic radiation. It is finally observed that for a specific wiggler wave number value, the phase-matching conditions for the process are satisfied, leading to resonant enhancement in the energy conversion efficiency.

Observation of topological surface states and strong electron/hole imbalance in extreme magnetoresistance compound LaBi

Science.gov (United States)

Jiang, J.; Schröter, N. B. M.; Wu, S.-C.; Kumar, N.; Shekhar, C.; Peng, H.; Xu, X.; Chen, C.; Yang, H. F.; Hwang, C.-C.; Mo, S.-K.; Felser, C.; Yan, B. H.; Liu, Z. K.; Yang, L. X.; Chen, Y. L.

2018-02-01

The recent discovery of the extreme magnetoresistance (XMR) in the nonmagnetic rare-earth monopnictides La X (X = P, As, Sb, Bi,), a recently proposed new topological semimetal family, has inspired intensive research effort in the exploration of the correlation between the XMR and their electronic structures. In this work, using angle-resolved photoemission spectroscopy to investigate the three-dimensional band structure of LaBi, we unraveled its topologically nontrivial nature with the observation of multiple topological surface Dirac fermions, as supported by our ab initio calculations. Furthermore, we observed substantial imbalance between the volume of electron and hole pockets, which rules out the electron-hole compensation as the primary cause of the XMR in LaBi.

Hole and electron extraction layers based on graphene oxide derivatives for high-performance bulk heterojunction solar cells

Energy Technology Data Exchange (ETDEWEB)

Liu, Jun; Gao, Yunxiang; Yu, Dingshan; Dai, Liming [Center of Advanced Science and Engineering for Carbon, Department of Macromolecular, Science and Engineering, Case School of Engineering, Case Western Reserve University, Cleveland, Ohio (United States); Xue, Yuhua [Center of Advanced Science and Engineering for Carbon, Department of Macromolecular, Science and Engineering, Case School of Engineering, Case Western Reserve University, Cleveland, Ohio (United States); Institute of Advanced Materials for Nano-Bio Applications, School of Ophthalmology and Optometry, Wenzhou Medical College, Zhejiang 325027 (China); Durstock, Michael [Materials and Manufacturing Directorate, Air Force Research Laboratory, RXBP, Wright-Patterson Air Force Base, Ohio 45433 (United States)

2012-05-02

By charge neutralization of carboxylic acid groups in graphene oxide (GO) with Cs{sub 2}CO{sub 3} to afford Cesium-neutralized GO (GO-Cs), GO derivatives with appropriate modification are used as both hole- and electron-extraction layers for bulk heterojunction (BHJ) solar cells. The normal and inverted devices based on GO hole- and GO-Cs electron-extraction layers both outperform the corresponding standard BHJ solar cells. (Copyright copyright 2012 WILEY-VCH Verlag GmbH and Co. KGaA, Weinheim)

Electron dynamics in the core-excited CS2 molecule revealed through resonant inelastic x-ray scattering spectroscopy

International Nuclear Information System (INIS)

Marchenko, T; Carniato, S; Journel, L; Guillemin, R; Kawerk, E; Simon, M; Žitnik, M; Kavčič, M; Bučar, K; Bohinc, R; Petric, M; Da Cruz, V Vaz; Gel'mukhanov, F

2015-01-01

We present an experimental and theoretical study of resonant inelastic x-ray scattering (RIXS) in the CS 2 molecule near the S 1s edge. We show that localization of the S 1s core-hole occurs in CS 2 during the RIXS process due to the orientational dephasing of interference between the waves scattering on the two sulfur atoms. Strong evolution of the RIXS profile with the excitation energy far below the first absorption resonance reflects the onset of electron dynamics triggered by a coherent excitation of multiple electronic states. (paper)

Electronic hole localization in rutile and anatase TiO2 - Self-interaction correction in Delta-SCF DFT

DEFF Research Database (Denmark)

Zawadzki, Pawel; Jacobsen, Karsten Wedel; Rossmeisl, Jan

2011-01-01

We study electronic hole localization in rutile and anatase titanium dioxide by means of Δ-Self-Consistent Field Density Functional Theory. In order to compare stabilities of the localized and the delocalized hole states we introduce a simple correction to the wrong description of the localizatio...

The effects of electron and hole transport layer with the electrode work function on perovskite solar cells

Science.gov (United States)

Deng, Quanrong; Li, Yiqi; Chen, Lian; Wang, Shenggao; Wang, Geming; Sheng, Yonglong; Shao, Guosheng

2016-09-01

The effects of electron and hole transport layer with the electrode work function on perovskite solar cells with the interface defects were simulated by using analysis of microelectronic and photonic structures-one-dimensional (AMPS-1D) software. The simulation results suggest that TiO2 electron transport layer provides best device performance with conversion efficiency of 25.9% compared with ZnO and CdS. The threshold value of back electrode work function for Spiro-OMeTAD, NiO, CuI and Cu2O hole transport layer are calculated to be 4.9, 4.8, 4.7 and 4.9 eV, respectively, to reach the highest conversion efficiency. The mechanisms of device physics with various electron and hole transport materials are discussed in details. The device performance deteriorates gradually as the increased density of interface defects located at ETM/absorber or absorber/HTM. This research results can provide helpful guidance for materials and metal electrode choice for perovskite solar cells.

Coupled quantum-classical method for long range charge transfer: relevance of the nuclear motion to the quantum electron dynamics

International Nuclear Information System (INIS)

Da Silva, Robson; Hoff, Diego A; Rego, Luis G C

2015-01-01

Charge and excitonic-energy transfer phenomena are fundamental for energy conversion in solar cells as well as artificial photosynthesis. Currently, much interest is being paid to light-harvesting and energy transduction processes in supramolecular structures, where nuclear dynamics has a major influence on electronic quantum dynamics. For this reason, the simulation of long range electron transfer in supramolecular structures, under environmental conditions described within an atomistic framework, has been a difficult problem to study. This work describes a coupled quantum mechanics/molecular mechanics method that aims at describing long range charge transfer processes in supramolecular systems, taking into account the atomistic details of large molecular structures, the underlying nuclear motion, and environmental effects. The method is applied to investigate the relevance of electron–nuclei interaction on the mechanisms for photo-induced electron–hole pair separation in dye-sensitized interfaces as well as electronic dynamics in molecular structures. (paper)

Black holes in binary stars

NARCIS (Netherlands)

Wijers, R.A.M.J.

1996-01-01

Introduction Distinguishing neutron stars and black holes Optical companions and dynamical masses X-ray signatures of the nature of a compact object Structure and evolution of black-hole binaries High-mass black-hole binaries Low-mass black-hole binaries Low-mass black holes Formation of black holes

Electron Cyclotron Resonances in Electron Cloud Dynamics

International Nuclear Information System (INIS)

Celata, Christine; Celata, C.M.; Furman, Miguel A.; Vay, J.-L.; Yu, Jennifer W.

2008-01-01

We report a previously unknown resonance for electron cloud dynamics. The 2D simulation code 'POSINST' was used to study the electron cloud buildup at different z positions in the International Linear Collider positron damping ring wiggler. An electron equilibrium density enhancement of up to a factor of 3 was found at magnetic field values for which the bunch frequency is an integral multiple of the electron cyclotron frequency. At low magnetic fields the effects of the resonance are prominent, but when B exceeds ∼(2 pi mec/(elb)), with lb = bunch length, effects of the resonance disappear. Thus short bunches and low B fields are required for observing the effect. The reason for the B field dependence, an explanation of the dynamics, and the results of the 2D simulations and of a single-particle tracking code used to elucidate details of the dynamics are discussed

Chemical dynamics of the first proton-coupled electron transfer of water oxidation on TiO2 anatase.

Science.gov (United States)

Chen, Jia; Li, Ye-Fei; Sit, Patrick; Selloni, Annabella

2013-12-18

Titanium dioxide (TiO2) is a prototype, water-splitting (photo)catalyst, but its performance is limited by the large overpotential for the oxygen evolution reaction (OER). We report here a first-principles density functional theory study of the chemical dynamics of the first proton-coupled electron transfer (PCET), which is considered responsible for the large OER overpotential on TiO2. We use a periodic model of the TiO2/water interface that includes a slab of anatase TiO2 and explicit water molecules, sample the solvent configurations by first principles molecular dynamics, and determine the energy profiles of the two electronic states involved in the electron transfer (ET) by hybrid functional calculations. Our results suggest that the first PCET is sequential, with the ET following the proton transfer. The ET occurs via an inner sphere process, which is facilitated by a state in which one electronic hole is shared by the two oxygen ions involved in the transfer.

Uncorrelated electron-hole transition energy in GaN|InGaN|GaN spherical QDQW nanoparticles

International Nuclear Information System (INIS)

Haddou El Ghazi; Anouar Jorio and Izeddine Zorkani

2013-01-01

The electron (hole) energy and uncorrelated 1S e - 1S h electron-hole transition in Core(GaN)|well(In x Ga 1-x N)|shell(GaN) spherical QDQW nanoparticles is investigated as a function of the inner and the outer radii. The calculations are performed within the framework of the effective-mass approximation and the finite parabolic potential confinement barrier in which two confined parameters are taking account. The Indium composition effect is also investigated. A critical value of the outer and the inner ratio is obtained which constitutes the turning point of two indium composition behaviors. (author)

Dynamics of Dwarf Galaxies Disfavor Stellar-Mass Black Holes as Dark Matter.

Science.gov (United States)

Koushiappas, Savvas M; Loeb, Abraham

2017-07-28

We study the effects of black hole dark matter on the dynamical evolution of stars in dwarf galaxies. We find that mass segregation leads to a depletion of stars in the center of dwarf galaxies and the appearance of a ring in the projected stellar surface density profile. Using Segue 1 as an example we show that current observations of the projected surface stellar density rule out at the 99.9% confidence level the possibility that more than 6% of the dark matter is composed of black holes with a mass of few tens of solar masses.

Formation of electrostatic double-layers and electron-holes in a low pressure mercury plasma column

International Nuclear Information System (INIS)

Petraconi, G; Maciel, Homero S

2003-01-01

Experimental studies of the formation of electrostatic double layers (DLs) and electron-holes (e-holes) are reported. The measurements were performed in the positive column of a mercury arc discharge operating in the low-pressure range of (2.0-14.0) x 10 -2 Pa with current density in the range of (3.0-8.0) x 10 3 A m -2 . Stable and unstable modes of the discharge were identified as the current was gradually increased, keeping constant the vapour pressure. The discharge remains stable until a critical current from which a slight increase of the current leads to an unstable regime characterized by high discharge impedance and strong oscillations. This mode ceased after a DL was formed in the plasma column. To induce the DL formation and to transport it smoothly along the discharge column, a low intensity B-field (7-10) x 10 -3 T produced by a movable single coil was used. The B-field locally increases the electron current density and makes the DL form at the centre of the magnetic constriction where it remained at rest. Electrostatic potential structures compatible with ordinary DLs and multiple-layers could be formed in the plasma column by dealing with the combined effects of the operational parameters of the discharge. It is noticeable that a pure e-hole, which is a symmetric triple-layer having a bell shape potential profile, could easily be formed by means of this experimental technique. A partial kinetic description, based on the space charge structure derived from an experimental e-hole, is presented in order to infer the charged particle populations that could contribute to the space charge of the e-hole. Evidence is shown that strong e-hole formation might be driven by an ion beam, therefore it could not be formed in isolation since its formation requires a nearby ion accelerating potential structure. Probe measurements of the plasma properties, at various radial positions of the stable positive column, are also presented. In the stable mode, prior to

Photoconversion and dynamic hole recycling process in anion vacancies in neutron-irradiated MgO crystals

International Nuclear Information System (INIS)

Monge, M.A.; Gonzalez, R.; Munoz Santiuste, J.E.; Pareja, R.; Chen, Y.; Kotomin, E.A.; Popov, A.I.

1999-01-01

Optical spectroscopy and theory demonstrate that photon excitation of the positively charged anion vacancies (F + centers) at 5.0 eV in neutron-irradiated MgO crystals releases holes that are subsequently trapped at V-type centers, which are cation vacancies charge compensated by impurities, such as Al 3+ , F - , and OH - ions. The concentration of trapped-hole centers was found to exceed that of available anion vacancies. The disproportionately large amount of holes produced is attributed to a dynamic recycling process, by which the F + center serves to release a hole to the V-type centers and subsequently trap a hole from an Fe 3+ ion. The net effect was the increase of V-type centers mostly at the expense of Fe 3+ ions. It was also shown that concurrently there was a component which distributed holes directly from Fe 3+ to the V-type centers. copyright 1999 The American Physical Society

Effects of Collisionality on the Nonlinear Characteristics of Boundary Turbulence and Blob/hole Transport in Tokamak Plasmas

Energy Technology Data Exchange (ETDEWEB)

Li, J.; Yasuaki, K., E-mail: lijq@energy.kyoto-u.ac.jp [Kyoto University, Kyoto (Japan); Cheng, J.; Longwen, Y.; Jiaqi, D. [Southwestern Institute of Physics, Chengdu (China)

2012-09-15

Full text: Blob/hole dynamics near tokamak separatrix is of striking importance in determining the boundary transport. Based on simulations using an extended 2-region (edge/SOL) fluid model, we found that blob/hole dynamics are sensitively influenced by the plasma collisionality, i.e., ion-electron and ion-neutral collisions. Namely, the holes are enhanced in highly collisional edge whereas the blobs are weakened at the SOL, causing larger particle convection. These blob/hole dynamics are closely correlated with potential dipoles. The trends are experimentally evidenced on the HL-2A tokamak. Moreover, as the neutral-ion collision increases, the blobs at the SOL tend to develop into streamers propagating outwards with reduced amplitude while the holes inwards are suppressed, showing a key role in nonlinear structure regulation and resultant transport suppression. Results suggest that adjusting the plasma collisionality by fueling, e.g., gas puffing, could serve as a method to nonlinearly select turbulent structures, i.e., blobs, holes or streamers, to access the control of boundary transport. (author)

Enhanced asymmetry in few-cycle attosecond pulse ionization of He in the vicinity of autoionizing resonances

International Nuclear Information System (INIS)

Djiokap, J M Ngoko; Starace, Anthony F; Hu, S X; Jiang Weichao; Peng Liangyou

2012-01-01

By solving the two-active-electron, time-dependent Schrödinger equation in its full dimensionality, we investigate the carrier-envelope phase (CEP) dependence of single ionization of He to the He + (1s) state triggered by an intense few-cycle attosecond pulse with carrier frequency ω corresponding to the energy ℏω = 36 eV. Effects of electron correlations are probed by comparing projections of the final state of the two-electron wave packet onto field-free highly correlated Jacobi matrix wave functions with projections onto uncorrelated Coulomb wave functions. Significant differences are found in the vicinity of autoionizing resonances. Owing to the broad bandwidths of our 115 and 230 as pulses and their high intensities (1–2 PW cm −2 ), asymmetries are found in the differential probability for ionization of electrons parallel and antiparallel to the linear polarization axis of the laser pulse. These asymmetries stem from interference of the one- and two-photon ionization amplitudes for producing electrons with the same momentum along the linear polarization axis. Whereas these asymmetries generally decrease with increasing ionized electron kinetic energy, we find a large enhancement of the asymmetry in the vicinity of two-electron doubly excited (autoionizing) states on an energy scale comparable to the widths of the autoionizing states. The CEP dependence of the energy-integrated asymmetry agrees very well with the predictions of time-dependent perturbation theory (Pronin et al 2009 Phys. Rev. A 80 063403). (paper)

Real-Space Imaging of Carrier Dynamics of Materials Surfaces by Second-Generation Four-Dimensional Scanning Ultrafast Electron Microscopy

KAUST Repository

Sun, Jingya

2015-09-14

In the fields of photocatalysis and photovoltaics, ultrafast dynamical processes, including carrier trapping and recombination on material surfaces, are among the key factors that determine the overall energy conversion efficiency. A precise knowledge of these dynamical events on the nanometer (nm) and femtosecond (fs) scales was not accessible until recently. The only way to access such fundamental processes fully is to map the surface dynamics selectively in real space and time. In this study, we establish a second generation of four-dimensional scanning ultrafast electron microscopy (4D S-UEM) and demonstrate the ability to record time-resolved images (snapshots) of material surfaces with 650 fs and ∼5 nm temporal and spatial resolutions, respectively. In this method, the surface of a specimen is excited by a clocking optical pulse and imaged using a pulsed primary electron beam as a probe pulse, generating secondary electrons (SEs), which are emitted from the surface of the specimen in a manner that is sensitive to the local electron/hole density. This method provides direct and controllable information regarding surface dynamics. We clearly demonstrate how the surface morphology, grains, defects, and nanostructured features can significantly impact the overall dynamical processes on the surface of photoactive-materials. In addition, the ability to access two regimes of dynamical probing in a single experiment and the energy loss of SEs in semiconductor-nanoscale materials will also be discussed.

Linking high harmonics from gases and solids.

Science.gov (United States)

Vampa, G; Hammond, T J; Thiré, N; Schmidt, B E; Légaré, F; McDonald, C R; Brabec, T; Corkum, P B

2015-06-25

When intense light interacts with an atomic gas, recollision between an ionizing electron and its parent ion creates high-order harmonics of the fundamental laser frequency. This sub-cycle effect generates coherent soft X-rays and attosecond pulses, and provides a means to image molecular orbitals. Recently, high harmonics have been generated from bulk crystals, but what mechanism dominates the emission remains uncertain. To resolve this issue, we adapt measurement methods from gas-phase research to solid zinc oxide driven by mid-infrared laser fields of 0.25 volts per ångström. We find that when we alter the generation process with a second-harmonic beam, the modified harmonic spectrum bears the signature of a generalized recollision between an electron and its associated hole. In addition, we find that solid-state high harmonics are perturbed by fields so weak that they are present in conventional electronic circuits, thus opening a route to integrate electronics with attosecond and high-harmonic technology. Future experiments will permit the band structure of a solid to be tomographically reconstructed.

The 2002 Antarctic Ozone Hole

Science.gov (United States)

Newman, P. A.; Nash, E. R.; Douglass, A. R.; Kawa, S. R.

2003-01-01

Since 1979, the ozone hole has grown from near zero size to over 24 Million km2. This area is most strongly controlled by levels of inorganic chlorine and bromine oncentrations. In addition, dynamical variations modulate the size of the ozone hole by either cooling or warming the polar vortex collar region. We will review the size observations, the size trends, and the interannual variability of the size. Using a simple trajectory model, we will demonstrate the sensitivity of the ozone hole to dynamical forcing, and we will use these observations to discuss the size of the ozone hole during the 2002 Austral spring. We will further show how the Cly decreases in the stratosphere will cause the ozone hole to decrease by 1-1.5% per year. We will also show results from a 3-D chemical transport model (CTM) that has been continuously run since 1999. These CTM results directly show how strong dynamics acts to reduce the size of the ozone hole.

Skyrmion dynamics in single-hole Neel ordered doped two-dimensional antiferromagnets with arbitrary spin

International Nuclear Information System (INIS)

Moura, A.R.; Pereira, A.R.; Moura-Melo, W.A.; Pires, A.S.T.

2008-01-01

We develop an effective theory to study the skyrmion dynamics in the presence of a hole (removed spins from the lattice) in Neel ordered two-dimensional antiferromagnets with arbitrary spin value S. The general equation of motion for the 'mass center' of this structure is obtained. The frequency of small amplitude oscillations of pinned skyrmions around the defect center is calculated. It is proportional to the hole size and inversely proportional to the square of the skyrmion size

One-Shot Decoupling and Page Curves from a Dynamical Model for Black Hole Evaporation.

Science.gov (United States)

Brádler, Kamil; Adami, Christoph

2016-03-11

One-shot decoupling is a powerful primitive in quantum information theory and was hypothesized to play a role in the black hole information paradox. We study black hole dynamics modeled by a trilinear Hamiltonian whose semiclassical limit gives rise to Hawking radiation. An explicit numerical calculation of the discretized path integral of the S matrix shows that decoupling is exact in the continuous limit, implying that quantum information is perfectly transferred from the black hole to radiation. A striking consequence of decoupling is the emergence of an output radiation entropy profile that follows Page's prediction. We argue that information transfer and the emergence of Page curves is a robust feature of any multilinear interaction Hamiltonian with a bounded spectrum.

Rate constant of free electrons and holes recombination in thin films CdSe

International Nuclear Information System (INIS)

Radychev, N.A.; Novikov, G.F.

2006-01-01

Destruction kinetics of electrons generated in thin films CdSe by laser impulse (wave length is 337 nm, period of impulse - 8 nc) is studied by the method of microwave photoconductivity (36 GHz) at 295 K. Model of the process was suggested using the analysis of kinetics of photo-responses decay, and it allowed determination of rate constant of recombination of free electrons and holes in cadmium selenide - (4-6)x10 -11 cm 3 s -1 [ru

ULTRAMASSIVE BLACK HOLE COALESCENCE

International Nuclear Information System (INIS)

Khan, Fazeel Mahmood; Holley-Bockelmann, Kelly; Berczik, Peter

2015-01-01

Although supermassive black holes (SMBHs) correlate well with their host galaxies, there is an emerging view that outliers exist. Henize 2-10, NGC 4889, and NGC 1277 are examples of SMBHs at least an order of magnitude more massive than their host galaxy suggests. The dynamical effects of such ultramassive central black holes is unclear. Here, we perform direct N-body simulations of mergers of galactic nuclei where one black hole is ultramassive to study the evolution of the remnant and the black hole dynamics in this extreme regime. We find that the merger remnant is axisymmetric near the center, while near the large SMBH influence radius, the galaxy is triaxial. The SMBH separation shrinks rapidly due to dynamical friction, and quickly forms a binary black hole; if we scale our model to the most massive estimate for the NGC 1277 black hole, for example, the timescale for the SMBH separation to shrink from nearly a kiloparsec to less than a parsec is roughly 10 Myr. By the time the SMBHs form a hard binary, gravitational wave emission dominates, and the black holes coalesce in a mere few Myr. Curiously, these extremely massive binaries appear to nearly bypass the three-body scattering evolutionary phase. Our study suggests that in this extreme case, SMBH coalescence is governed by dynamical friction followed nearly directly by gravitational wave emission, resulting in a rapid and efficient SMBH coalescence timescale. We discuss the implications for gravitational wave event rates and hypervelocity star production

Gravitational waves from quasicircular black-hole binaries in dynamical Chern-Simons gravity.

Science.gov (United States)

Yagi, Kent; Yunes, Nicolás; Tanaka, Takahiro

2012-12-21

Dynamical Chern-Simons gravity cannot be strongly constrained with current experiments because it reduces to general relativity in the weak-field limit. This theory, however, introduces modifications in the nonlinear, dynamical regime, and thus it could be greatly constrained with gravitational waves from the late inspiral of black-hole binaries. We complete the first self-consistent calculation of such gravitational waves in this theory. For favorable spin orientations, advanced ground-based detectors may improve existing solar system constraints by 6 orders of magnitude.

Electron and hole spectrum in InAs quantum dot renormalized by InAs/GaAs heterostructure deformation

International Nuclear Information System (INIS)

Dan'kiv, O.O.; Peleshchak, R.M.

2005-01-01

Analytical expressions describing the energy spectrum of electrons and holes are obtained for a quantum dot occurring in a self-consistent strain field created by an array of coherently stressed quantum dots. A method of taking into account the lattice mismatch at the quantum dot-matrix interface is proposed that allows for the dependence of the mismatch parameter on the quantum dot size and the matrix layer thickness. It is shown that the internal elastic strain arising at the quantum dot-matrix interface influences the energy spectrum of electrons more significantly than the spectrum of holes [ru

The inversion layer of electric fields and electron phase-space-hole structure during two-dimensional collisionless magnetic reconnection

International Nuclear Information System (INIS)

Chen Lijen; Lefebvre, Bertrand; Torbert, Roy B.; Daughton, William S.

2011-01-01

Based on two-dimensional fully kinetic simulations that resolve the electron diffusion layer in undriven collisionless magnetic reconnection with zero guide field, this paper reports the existence and evolution of an inversion layer of bipolar electric fields, its corresponding phase-space structure (an electron-hole layer), and the implication to collisionless dissipation. The inversion electric field layer is embedded in the layer of bipolar Hall electric field and extends throughout the entire length of the electron diffusion layer. The electron phase-space hole structure spontaneously arises during the explosive growth phase when there exist significant inflows into the reconnection layer, and electrons perform meandering orbits across the layer while being cyclotron-turned toward the outflow directions. The cyclotron turning of meandering electrons by the magnetic field normal to the reconnection layer is shown to be a primary factor limiting the current density in the region where the reconnection electric field is balanced by the gradient (along the current sheet normal) of the off-diagonal electron pressure-tensor.

Electron and hole photoemission detection for band offset determination of tunnel field-effect transistor heterojunctions

International Nuclear Information System (INIS)

Li, Wei; Zhang, Qin; Kirillov, Oleg A.; Levin, Igor; Richter, Curt A.; Gundlach, David J.; Nguyen, N. V.; Bijesh, R.; Datta, S.; Liang, Yiran; Peng, Lian-Mao; Liang, Xuelei

2014-01-01

We report experimental methods to ascertain a complete energy band alignment of a broken-gap tunnel field-effect transistor based on an InAs/GaSb hetero-junction. By using graphene as an optically transparent electrode, both the electron and hole barrier heights at the InAs/GaSb interface can be quantified. For a Al 2 O 3 /InAs/GaSb layer structure, the barrier height from the top of the InAs and GaSb valence bands to the bottom of the Al 2 O 3 conduction band is inferred from electron emission whereas hole emissions reveal the barrier height from the top of the Al 2 O 3 valence band to the bottom of the InAs and GaSb conduction bands. Subsequently, the offset parameter at the broken gap InAs/GaSb interface is extracted and thus can be used to facilitate the development of predicted models of electron quantum tunneling efficiency and transistor performance

Theory of Weak Bipolar Fields and Electron Holes with Applications to Space Plasmas

International Nuclear Information System (INIS)

Goldman, Martin V.; Newman, David L.; Mangeney, Andre

2007-01-01

A theoretical model of weak electron phase-space holes is used to interpret bipolar field structures observed in space. In the limit eφ max /T e max sech 4 (x/α), where φ max depends on the derivative of the trapped distribution at the separatrix, while α depends only on a screening integral over the untrapped distribution. Idealized trapped and passing electron distributions are inferred from the speed, amplitude, and shape of satellite waveform measurements of weak bipolar field structures

Electron and hole doping effects in Sr{sub 2}FeMoO{sub 6} double perovskites

Energy Technology Data Exchange (ETDEWEB)

Sanchez, D. E-mail: diana.sanchez@icmm.csic.es; Alonso, J.A.; Garcia-Hernandez, M.; Martinez-Lope, M.J.; Casais, M.T.; Martinez, J.L.; Fernandez-Diaz, M.T

2004-05-01

Electron and hole doping effects in the ferromagnetic and structural properties of the double perovskite Sr{sub 2}FeMoO{sub 6} are studied along the series Sr{sub 2-x}La{sub x}FeMoO{sub 6} (0{<=}x{<=}1) and Sr{sub 2-x}FeMoO{sub 6} (0{<=}x{<=}0.4) from neutron powder diffraction and magnetization data. Sr-deficient samples (hole doped) show moderate changes in the structure and both T{sub c} and M{sub s} rapidly decrease with x. On the contrary, a change from tetragonal to monoclinic symmetry and a non monotonic behaviour in T{sub c} is found in the La-substituted series (electron doped)

Dynamic screening and electron dynamics in low-dimensional metal systems

International Nuclear Information System (INIS)

Silkin, V.M.; Quijada, M.; Vergniory, M.G.; Alducin, M.; Borisov, A.G.; Diez Muino, R.; Juaristi, J.I.; Sanchez-Portal, D.; Chulkov, E.V.; Echenique, P.M.

2007-01-01

Recent advances in the theoretical description of dynamic screening and electron dynamics in metallic media are reviewed. The time-dependent building-up of screening in different situations is addressed. Perturbative and non-perturbative theories are used to study electron dynamics in low-dimensional systems, such as metal clusters, image states, surface states and quantum wells. Modification of the electronic lifetimes due to confinement effects is analyzed as well

Effects of irradiation and isochronal anneal temperature on hole and electron trapping in MOS devices

International Nuclear Information System (INIS)

Fleetwood, D.M.; Winokur, P.S.; Shaneyfelt, M.R.; Riewe, L.C.; Flament, O.; Paillet, P.; Leray, J.L.

1998-02-01

Capacitance-voltage and thermally-stimulated-current techniques are used to estimate trapped hole and electron densities in MOS oxides as functions of irradiation and isochronal anneal temperature. Trapped-charge annealing and compensation effects are discussed

Fractional high-harmonic combs by attosecond-precision split-spectrum pulse control

Directory of Open Access Journals (Sweden)

Laux Martin

2013-03-01

Full Text Available Few-cycle laser fields enable pulse-shaping control of high-order harmonic generation by time delaying variable broadband spectral sections. We report the experimental generation of fractional (noninteger high-harmonic combs by the controlled interference of two attosecond pulse trains. Additionally the energy of the high harmonics is strongly tuned with the relative time delay. We quantify the tuning to directly result from the controlled variation of the instantaneous laser frequency at the shaped driver pulse intensity maximum.

Design and Analysis of CMOS-Compatible III-V Compound Electron-Hole Bilayer Tunneling Field-Effect Transistor for Ultra-Low-Power Applications.

Science.gov (United States)

Kim, Sung Yoon; Seo, Jae Hwa; Yoon, Young Jun; Lee, Ho-Young; Lee, Seong Min; Cho, Seongjae; Kang, In Man

2015-10-01

In this work, we design and analyze complementary metal-oxide-semiconductor (CMOS)-compatible III-V compound electron-hole bilayer (EHB) tunneling field-effect transistors (TFETs) by using two-dimensional (2D) technology computer-aided design (TCAD) simulations. A recently proposed EHB TFET exploits a bias-induced band-to-band tunneling (BTBT) across the electron-hole bilayer by an electric field from the top and bottom gates. This is in contrast to conventional planar p(+)-p(-)-n TFETs, which utilize BTBT across the source-to-channel junction. We applied III-V compound semiconductor materials to the EHB TFETs in order to enhance the current drivability and switching performance. Devices based on various compound semiconductor materials have been designed and analyzed in terms of their primary DC characteristics. In addition, the operational principles were validated by close examination of the electron concentrations and energy-band diagrams under various operation conditions. The simulation results of the optimally designed In0.533Ga0.47As EHB TFET show outstanding performance, with an on-state current (Ion) of 249.5 μA/μm, subthreshold swing (S) of 11.4 mV/dec, and threshold voltage (Vth) of 50 mV at VDS = 0.5 V. Based on the DC-optimized InGaAs EHB TFET, the CMOS inverter circuit was simulated in views of static and dynamic behaviors of the p-channel device with exchanges between top and bottom gates or between source and drain electrodes maintaining the device structure.

Generation and characterization of atto second pulses

International Nuclear Information System (INIS)

Mairesse, Y.

2005-07-01

Atto-second pulse trains in the extreme ultraviolet range can be produced by high-order harmonic generation, by focusing an intense femtosecond pulse in a rare gas jet. In this thesis, we present a temporal characterization of this radiation on the femtosecond and atto-second timescales. By transposing a spectral interferometry technique commonly used in the infrared range (SPIDER), we make a complete single-shot characterization of the temporal profile of individual harmonics, on the femtosecond timescale. In a second part, we study experimentally the atto-second structure of the harmonic radiation, and demonstrate a temporal drift in the emission: the lowest harmonics are emitted before the highest ones. This chirp, which is directly related to the electron dynamics in the generation process, imposes a lower limit to the duration that can be achieved by increasing the spectral range. We show how generating conditions can be optimized in order to enhance the synchronization in the emission, and how atto-second pulses can be re-compressed. Last, we propose a new technique for the complete characterization of arbitrary atto-second pulses: FROGCRAB. This method would allow simultaneous measurements of the femtosecond and atto-second structures of the radiation, and thus a complete knowledge of the atto-second light source in the perspective of applications. (author)

Charge transport in organic molecular semiconductors from first principles: The bandlike hole mobility in a naphthalene crystal

Science.gov (United States)

Lee, Nien-En; Zhou, Jin-Jian; Agapito, Luis A.; Bernardi, Marco

2018-03-01

Predicting charge transport in organic molecular crystals is notoriously challenging. Carrier mobility calculations in organic semiconductors are dominated by quantum chemistry methods based on charge hopping, which are laborious and only moderately accurate. We compute from first principles the electron-phonon scattering and the phonon-limited hole mobility of naphthalene crystal in the framework of ab initio band theory. Our calculations combine GW electronic bandstructures, ab initio electron-phonon scattering, and the Boltzmann transport equation. The calculated hole mobility is in very good agreement with experiment between 100 -300 K , and we can predict its temperature dependence with high accuracy. We show that scattering between intermolecular phonons and holes regulates the mobility, though intramolecular phonons possess the strongest coupling with holes. We revisit the common belief that only rigid molecular motions affect carrier dynamics in organic molecular crystals. Our paper provides a quantitative and rigorous framework to compute charge transport in organic crystals and is a first step toward reconciling band theory and carrier hopping computational methods.

In situ measurement of plasma and shock wave properties inside laser-drilled metal holes

Science.gov (United States)

Brajdic, Mihael; Hermans, Martin; Horn, Alexander; Kelbassa, Ingomar

2008-10-01

High-speed imaging of shock wave and plasma dynamics is a commonly used diagnostic method for monitoring processes during laser material treatment. It is used for processes such as laser ablation, cutting, keyhole welding and drilling. Diagnosis of laser drilling is typically adopted above the material surface because lateral process monitoring with optical diagnostic methods inside the laser-drilled hole is not possible due to the hole walls. A novel method is presented to investigate plasma and shock wave properties during the laser drilling inside a confined environment such as a laser-drilled hole. With a novel sample preparation and the use of high-speed imaging combined with spectroscopy, a time and spatial resolved monitoring of plasma and shock wave dynamics is realized. Optical emission of plasma and shock waves during drilling of stainless steel with ns-pulsed laser radiation is monitored and analysed. Spatial distributions and velocities of shock waves and of plasma are determined inside the holes. Spectroscopy is accomplished during the expansion of the plasma inside the drilled hole allowing for the determination of electron densities.

Optical conductivity calculation of a k.p model semiconductor GaAs incorporating first-order electron-hole vertex correction

Science.gov (United States)

Nurhuda, Maryam; Aziz Majidi, Muhammad

2018-04-01

The role of excitons in semiconducting materials carries potential applications. Experimental results show that excitonic signals also appear in optical absorption spectra of semiconductor system with narrow gap, such as Gallium Arsenide (GaAs). While on the theoretical side, calculation of optical spectra based purely on Density Functional Theory (DFT) without taking electron-hole (e-h) interactions into account does not lead to the appearance of any excitonic signal. Meanwhile, existing DFT-based algorithms that include a full vertex correction through Bethe-Salpeter equation may reveal an excitonic signal, but the algorithm has not provided a way to analyze the excitonic signal further. Motivated to provide a way to isolate the excitonic effect in the optical response theoretically, we develop a method of calculation for the optical conductivity of a narrow band-gap semiconductor GaAs within the 8-band k.p model that includes electron-hole interactions through first-order electron-hole vertex correction. Our calculation confirms that the first-order e-h vertex correction reveals excitonic signal around 1.5 eV (the band gap edge), consistent with the experimental data.

Atomistic Tight-Binding Theory of Electron-Hole Exchange Interaction in Morphological Evolution of CdSe/ZnS Core/Shell Nanodisk to CdSe/ZnS Core/Shell Nanorod

Directory of Open Access Journals (Sweden)

Worasak Sukkabot

2016-01-01

Full Text Available Based on the atomistic tight-binding theory (TB and a configuration interaction (CI description, the electron-hole exchange interaction in the morphological transformation of CdSe/ZnS core/shell nanodisk to CdSe/ZnS core/shell nanorod is described with the aim of understanding the impact of the structural shapes on the change of the electron-hole exchange interaction. Normally, the ground hole states confined in typical CdSe/ZnS core/shell nanocrystals are of heavy hole-like character. However, the atomistic tight-binding theory shows that a transition of the ground hole states from heavy hole-like to light hole-like contribution with the increasing aspect ratios of the CdSe/ZnS core/shell nanostructures is recognized. According to the change in the ground-state hole characters, the electron-hole exchange interaction is also significantly altered. To do so, optical band gaps, ground-state electron character, ground-state hole character, oscillation strengths, ground-state coulomb energies, ground-state exchange energies, and dark-bright (DB excitonic splitting (stoke shift are numerically demonstrated. These atomistic computations obviously show the sensitivity with the aspect ratios. Finally, the alteration in the hole character has a prominent effect on dark-bright (DB excitonic splitting.

High-order harmonic generation spectra and isolated attosecond pulse generation with a two-color time delayed pulse

International Nuclear Information System (INIS)

Feng Liqiang; Chu Tianshu

2012-01-01

Highlights: ► Investigation of HHG spectra and single isolated attosecond pulse generation. ► Irradiation from a model Ne atom by two-color time delayed pulse. ► Observation of time delay effect and relative phase effect. ► Revelation of the optimal condition for generating isolated attosecond pulse. ► Generation of a single isolated attosecond pulse of 45as. - Abstract: In this paper, we theoretically investigate the delay time effect on the high-order harmonic generation (HHG) when a model Ne atom is exposed to a two-color time delayed pulse, consisting of a 5fs/800 nm fundamental field and a 20fs/2000 nm controlling field. It shows that the HHG spectra are strongly sensitive to the delay time between the two laser fields, in particular, for the zero carrier-envelope phase (CEP) φ case (corresponding to the 800 nm fundamental field), the maximum cutoff energy has been achieved at zero delay time. However, with the introduction of the CEP (φ = 180°), the delay effect on HHG is changed, exhibiting a ‘U’ structure harmonic emission from −1 T to 1 T. In addition, the combinations of different controlling pulse frequencies and pulse intensities have also been considered, showing the similar results as the original controlling field case, but with some characteristics. Finally, by properly superposing the optimal harmonic spectrum, an isolated 45as pulse is generated without phase compensation.

Impact of Relativistic Electron Beam on Hole Acoustic Instability in Quantum Semiconductor Plasmas

Science.gov (United States)

Siddique, M.; Jamil, M.; Rasheed, A.; Areeb, F.; Javed, Asif; Sumera, P.

2018-01-01

We studied the influence of the classical relativistic beam of electrons on the hole acoustic wave (HAW) instability exciting in the semiconductor quantum plasmas. We conducted this study by using the quantum-hydrodynamic model of dense plasmas, incorporating the quantum effects of semiconductor plasma species which include degeneracy pressure, exchange-correlation potential and Bohm potential. Analysis of the quantum characteristics of semiconductor plasma species along with relativistic effect of beam electrons on the dispersion relation of the HAW is given in detail qualitatively and quantitatively by plotting them numerically. It is worth mentioning that the relativistic electron beam (REB) stabilises the HAWs exciting in semiconductor (GaAs) degenerate plasma.

On the ultrafast charge migration and subsequent charge directed reactivity in Cl⋯N halogen-bonded clusters following vertical ionization

International Nuclear Information System (INIS)

Chandra, Sankhabrata; Bhattacharya, Atanu; Periyasamy, Ganga

2015-01-01

In this article, we have presented ultrafast charge transfer dynamics through halogen bonds following vertical ionization of representative halogen bonded clusters. Subsequent hole directed reactivity of the radical cations of halogen bonded clusters is also discussed. Furthermore, we have examined effect of the halogen bond strength on the electron-electron correlation- and relaxation-driven charge migration in halogen bonded complexes. For this study, we have selected A-Cl (A represents F, OH, CN, NH 2 , CF 3 , and COOH substituents) molecules paired with NH 3 (referred as ACl:NH 3 complex): these complexes exhibit halogen bonds. To the best of our knowledge, this is the first report on purely electron correlation- and relaxation-driven ultrafast (attosecond) charge migration dynamics through halogen bonds. Both density functional theory and complete active space self-consistent field theory with 6-31 + G(d, p) basis set are employed for this work. Upon vertical ionization of NCCl⋯NH 3 complex, the hole is predicted to migrate from the NH 3 -end to the ClCN-end of the NCCl⋯NH 3 complex in approximately 0.5 fs on the D 0 cationic surface. This hole migration leads to structural rearrangement of the halogen bonded complex, yielding hydrogen bonding interaction stronger than the halogen bonding interaction on the same cationic surface. Other halogen bonded complexes, such as H 2 NCl:NH 3 , F 3 CCl:NH 3 , and HOOCCl:NH 3 , exhibit similar charge migration following vertical ionization. On the contrary, FCl:NH 3 and HOCl:NH 3 complexes do not exhibit any charge migration following vertical ionization to the D 0 cation state, pointing to interesting halogen bond strength-dependent charge migration

Isolating strong-field dynamics in molecular systems

Science.gov (United States)

Orenstein, Gal; Pedatzur, Oren; Uzan, Ayelet J.; Bruner, Barry D.; Mairesse, Yann; Dudovich, Nirit

2017-05-01

Strong-field ionization followed by recollision provides a unique pump-probe measurement which reveals a range of electronic processes, combining sub-Angstrom spatial and attosecond temporal resolution. A major limitation of this approach is imposed by the coupling between the spatial and temporal degrees of freedom. In this paper we focus on the study of high harmonic generation and demonstrate the ability to isolate the internal dynamics—decoupling the temporal information from the spatial one. By applying an in situ approach we reveal the universality of the intrinsic pump-probe measurement and establish its validity in molecular systems. When several orbitals are involved we identify the fingerprint of the transition from the single-channel case into the multiple-channel dynamics, where complex multielectron phenomena are expected to be observed.

Gamma ray bursts of black hole universe

Science.gov (United States)

Zhang, T. X.

2015-07-01

Slightly modifying the standard big bang theory, Zhang recently developed a new cosmological model called black hole universe, which has only a single postulate but is consistent with Mach's principle, governed by Einstein's general theory of relativity, and able to explain existing observations of the universe. In the previous studies, we have explained the origin, structure, evolution, expansion, cosmic microwave background radiation, quasar, and acceleration of black hole universe, which grew from a star-like black hole with several solar masses through a supermassive black hole with billions of solar masses to the present state with hundred billion-trillions of solar masses by accreting ambient matter and merging with other black holes. This study investigates gamma ray bursts of black hole universe and provides an alternative explanation for the energy and spectrum measurements of gamma ray bursts according to the black hole universe model. The results indicate that gamma ray bursts can be understood as emissions of dynamic star-like black holes. A black hole, when it accretes its star or merges with another black hole, becomes dynamic. A dynamic black hole has a broken event horizon and thus cannot hold the inside hot (or high-frequency) blackbody radiation, which flows or leaks out and produces a GRB. A star when it collapses into its core black hole produces a long GRB and releases the gravitational potential energy of the star as gamma rays. A black hole that merges with another black hole produces a short GRB and releases a part of their blackbody radiation as gamma rays. The amount of energy obtained from the emissions of dynamic star-like black holes are consistent with the measurements of energy from GRBs. The GRB energy spectra derived from this new emission mechanism are also consistent with the measurements.

Communication: The electronic structure of matter probed with a single femtosecond hard x-ray pulse

Directory of Open Access Journals (Sweden)

J. Szlachetko

2014-03-01

Full Text Available Physical, biological, and chemical transformations are initiated by changes in the electronic configuration of the species involved. These electronic changes occur on the timescales of attoseconds (10−18 s to femtoseconds (10−15 s and drive all subsequent electronic reorganization as the system moves to a new equilibrium or quasi-equilibrium state. The ability to detect the dynamics of these electronic changes is crucial for understanding the potential energy surfaces upon which chemical and biological reactions take place. Here, we report on the determination of the electronic structure of matter using a single self-seeded femtosecond x-ray pulse from the Linac Coherent Light Source hard x-ray free electron laser. By measuring the high energy resolution off-resonant spectrum (HEROS, we were able to obtain information about the electronic density of states with a single femtosecond x-ray pulse. We show that the unoccupied electronic states of the scattering atom may be determined on a shot-to-shot basis and that the measured spectral shape is independent of the large intensity fluctuations of the incoming x-ray beam. Moreover, we demonstrate the chemical sensitivity and single-shot capability and limitations of HEROS, which enables the technique to track the electronic structural dynamics in matter on femtosecond time scales, making it an ideal probe technique for time-resolved X-ray experiments.

Post-Newtonian Dynamics in Dense Star Clusters: Highly Eccentric, Highly Spinning, and Repeated Binary Black Hole Mergers.

Science.gov (United States)

Rodriguez, Carl L; Amaro-Seoane, Pau; Chatterjee, Sourav; Rasio, Frederic A

2018-04-13

We present models of realistic globular clusters with post-Newtonian dynamics for black holes. By modeling the relativistic accelerations and gravitational-wave emission in isolated binaries and during three- and four-body encounters, we find that nearly half of all binary black hole mergers occur inside the cluster, with about 10% of those mergers entering the LIGO/Virgo band with eccentricities greater than 0.1. In-cluster mergers lead to the birth of a second generation of black holes with larger masses and high spins, which, depending on the black hole natal spins, can sometimes be retained in the cluster and merge again. As a result, globular clusters can produce merging binaries with detectable spins regardless of the birth spins of black holes formed from massive stars. These second-generation black holes would also populate any upper mass gap created by pair-instability supernovae.

Post-Newtonian Dynamics in Dense Star Clusters: Highly Eccentric, Highly Spinning, and Repeated Binary Black Hole Mergers

Science.gov (United States)

Rodriguez, Carl L.; Amaro-Seoane, Pau; Chatterjee, Sourav; Rasio, Frederic A.

2018-04-01

We present models of realistic globular clusters with post-Newtonian dynamics for black holes. By modeling the relativistic accelerations and gravitational-wave emission in isolated binaries and during three- and four-body encounters, we find that nearly half of all binary black hole mergers occur inside the cluster, with about 10% of those mergers entering the LIGO/Virgo band with eccentricities greater than 0.1. In-cluster mergers lead to the birth of a second generation of black holes with larger masses and high spins, which, depending on the black hole natal spins, can sometimes be retained in the cluster and merge again. As a result, globular clusters can produce merging binaries with detectable spins regardless of the birth spins of black holes formed from massive stars. These second-generation black holes would also populate any upper mass gap created by pair-instability supernovae.

Static and dynamic behaviours of railway prestressed concrete sleepers with longitudinal through hole