Positron Annihilation Induced Auger and Gamma Spectroscopy of Catalytically Important Surfaces

Science.gov (United States)

Weiss, A. H.; Nadesalingam, M. P.; Sundaramoorthy, R.; Mukherjee, S.; Fazleev, N. G.

2006-10-01

The annihilation of positrons with core electrons results in unique signatures in the spectra of Auger-electron and annihilation-gamma rays that can be used to make clear chemical identification of atoms at the surface. Because positrons implanted at low energies are trapped with high efficiency in the image-correlation well where they are localized just outside the surface it is possible to use annihilation induced Auger and Gamma signals to probe the surfaces of solids with single atomic layer depth resolution. In this talk we will report recent applications of Positron Annihilation Induced Auger Electron Spectroscopy (PAES) and Auger-Gamma Coincidence Spectroscopy (AGCS) to the study of surface structure and surface chemistry. Our research has demonstrated that PAES spectra can provide new information regarding the composition of the top-most atomic layer. Applications of PAES to the study of catalytically important surfaces of oxides and wide band-gap semiconductors including TiO2, SiO2,Cu2O, and SiC will be presented. We conclude with a discussion of the use of Auger-Gamma and Gamma-Gamma coincidence spectroscopy for the study of surfaces at pressures closer to those found in practical chemical reactors. Research supported by the Welch Foundation Grant Number Y-1100.

High resolution gamma spectroscopy well logging system

International Nuclear Information System (INIS)

Giles, J.R.; Dooley, K.J.

1997-01-01

A Gamma Spectroscopy Logging System (GSLS) has been developed to study sub-surface radionuclide contamination. The absolute counting efficiencies of the GSLS detectors were determined using cylindrical reference sources. More complex borehole geometries were modeled using commercially available shielding software and correction factors were developed based on relative gamma-ray fluence rates. Examination of varying porosity and moisture content showed that as porosity increases, and as the formation saturation ratio decreases, relative gamma-ray fluence rates increase linearly for all energies. Correction factors for iron and water cylindrical shields were found to agree well with correction factors determined during previous studies allowing for the development of correction factors for type-304 stainless steel and low-carbon steel casings. Regression analyses of correction factor data produced equations for determining correction factors applicable to spectral gamma-ray well logs acquired under non-standard borehole conditions

Nuclear Forensics using Gamma-ray Spectroscopy

Directory of Open Access Journals (Sweden)

Norman E. B.

2016-01-01

Full Text Available Much of George Dracoulis’s research career was devoted to utilising gamma-ray spectroscopy in fundamental studies in nuclear physics. This same technology is useful in a wide range of applications in the area of nuclear forensics. Over the last several years, our research group has made use of both high- and low-resolution gamma-ray spectrometers to: identify the first sample of plutonium large enough to be weighed; determine the yield of the Trinity nuclear explosion; measure fission fragment yields as a function of target nucleus and neutron energy; and observe fallout in the U. S. from the Fukushima nuclear reactor accident.

Gamma and Xray spectroscopy at high performance

International Nuclear Information System (INIS)

Borchert, G.L.

1984-01-01

The author determines that for many interesting problems in gamma and Xray spectroscopy it is necessary to use crystal diffractometers. The basic features of such instruments are discussed and the special performance of crystal spectrometers is demonstrated by means of typical examples of various applications

Gamma-ray spectroscopy with relativistic exotic heavy-ions

Indian Academy of Sciences (India)

Abstract. Feasibility of gamma-ray spectroscopy at relativistic energies with exotic heavy-ions and new generation of germanium detectors (segmented Clover) is discussed. An experiment with such detector array and radioactive is discussed.

Experimental approaches for the development of gamma spectroscopy well logging system

Energy Technology Data Exchange (ETDEWEB)

Shin, Jehyun; Hwang, Seho; Kim, Jongman [Korea Institute of Geoscience and Mineral Resources (124 Gwahang-no, Yuseong-gu, Daejeon, Korea) (Korea, Republic of); Won, Byeongho [Heesong Geotek Co., Ltd (146-8 Sangdaewon-dong, Jungwon-gu, Seongnam-si, Gyeonggi-do, Korea) (Korea, Republic of)

2015-03-10

This article discusses experimental approaches for the development of gamma spectroscopy well logging system. Considering the size of borehole sonde, we customize 2 x 2 inches inorganic scintillators and the system including high voltage, preamplifier, amplifier and multichannel analyzer (MCA). The calibration chart is made by test using standard radioactive sources so that the measured count rates are expressed by energy spectrum. Optimum high-voltage supplies and the measurement parameters of each detector are set up by experimental investigation. Also, the responses of scintillation detectors have been examined by analysis according to the distance between source and detector. Because gamma spectroscopy well logging needs broad spectrum, high sensitivity and resolution, the energy resolution and sensitivity as a function of gamma ray energy are investigated by analyzing the gamma ray activities of the radioactive sources.

Gamma ray spectroscopy monitoring method and apparatus

Science.gov (United States)

Stagg, William R; Policke, Timothy A

2017-05-16

The present invention relates generally to the field of gamma ray spectroscopy monitoring and a system for accomplishing same to monitor one or more aspects of various isotope production processes. In one embodiment, the present invention relates to a monitoring system, and method of utilizing same, for monitoring one or more aspects of an isotope production process where the monitoring system comprises: (A) at least one sample cell; (B) at least one measuring port; (C) at least one adjustable collimator device; (D) at least one shutter; and (E) at least one high resolution gamma ray spectrometer.

Fast amplification system for gamma spectroscopy

International Nuclear Information System (INIS)

Jesus, E.F.O.; Lopes, R.T.

1992-01-01

An amplification system for gamma spectroscopy with high counting rates was developed. The system was constructed with operational amplifiers, and tested and compared with ORTEC conventional system, using Iridium-192 as source of 9,25 x 10 1 0 Bq of activity and NaI (Tl) detector. The constructed system showed a better performance in relation to efficiency and resolution parameters, tested before. (C.G.C.)

Gamma-ray spectrometry applied to down-hole logging

International Nuclear Information System (INIS)

Dumesnil, P.; Umiastowsky, K.

1983-11-01

Gamma-ray spectrometry permits to improve the accuracy of natural gamma, gamma-gamma and neutron-gamma geophysical measurements. The probe developed at Centre d'Etudes Nucleaires de Saclay allows down-hole gamma-ray spectrometry. Among others, this probe can be applied to the uranium content determination by selective natural gamma method, down-hole determination of the ash content in the coal by gamma-gamma selective method and elemental analysis by neutron-gamma method. For the calibration and an exact interpretation of the measurements it is important to know the gamma-ray and neutron characteristics of the different kinds of rocks considered as probabilistic variables

Multielement CdZnTe detectors for high-efficiency, ambient-temperature gamma-ray spectroscopy

International Nuclear Information System (INIS)

Prettyman, T.H.; Moss, C.E.; Sweet, M.R.; Ianakiev, K.; Reedy, R.C.; Li, J.; Valentine, J.D.

1998-01-01

CdZnTe is an attractive alternative to scintillator-based technology for ambient-temperature, gamma-ray spectroscopy. Large, single-element devices up to 3500 mm 3 have been developed for gamma-ray spectroscopy and are now available commercially. Because CdZnTe is a wide band-gap semiconductor, it can operate over a wide range of ambient temperatures with minimal power consumption. Over this range, CdZnTe detectors routinely yield better overall performance for gamma-ray spectroscopy than scintillator detectors. Manufacturing issues and material electronic properties limit the maximum size of single-element CdZnTe detectors. The authors are investigating methods to combine CdZnTe detectors together to improve detection efficiency and overall performance of gamma-ray spectroscopy. The applications include the assay and identification of radioisotopes for nuclear material safeguards and nonproliferation (over the energy range 50 keV to 1 MeV), and the analysis of elemental composition for planetary science (over the energy range 1 MeV to 10 MeV). Design issues for the two energy ranges are summarized

Quantitative portable gamma-spectroscopy sample analysis for non-standard sample geometries

International Nuclear Information System (INIS)

Ebara, S.B.

1998-01-01

Utilizing a portable spectroscopy system, a quantitative method for analysis of samples containing a mixture of fission and activation products in nonstandard geometries was developed. This method was not developed to replace other methods such as Monte Carlo or Discrete Ordinates but rather to offer an alternative rapid solution. The method can be used with various sample and shielding configurations where analysis on a laboratory based gamma-spectroscopy system is impractical. The portable gamma-spectroscopy method involves calibration of the detector and modeling of the sample and shielding to identify and quantify the radionuclides present in the sample. The method utilizes the intrinsic efficiency of the detector and the unattenuated gamma fluence rate at the detector surface per unit activity from the sample to calculate the nuclide activity and Minimum Detectable Activity (MDA). For a complex geometry, a computer code written for shielding applications (MICROSHIELD) is utilized to determine the unattenuated gamma fluence rate per unit activity at the detector surface. Lastly, the method is only applicable to nuclides which emit gamma-rays and cannot be used for pure beta or alpha emitters. In addition, if sample self absorption and shielding is significant, the attenuation will result in high MDA's for nuclides which solely emit low energy gamma-rays. The following presents the analysis technique and presents verification results using actual experimental data, rather than comparisons to other approximations such as Monte Carlo techniques, to demonstrate the accuracy of the method given a known geometry and source term. (author)

CsI(Tl)-photodiode detectors for gamma-ray spectroscopy

CERN Document Server

Fioretto, E; Viesti, G; Cinausero, M; Zuin, L; Fabris, D; Lunardon, M; Nebbia, G; Prete, G

2000-01-01

We report on the performances of CsI(Tl)-photodiode detectors for gamma-ray spectroscopy applications. Light output yield and energy resolution have been measured for different crystals and read-out configurations.

Gamma spectroscopy: from steady beams to radioactive beams

International Nuclear Information System (INIS)

Stezowski, O.

2008-06-01

The author gives an overview of his research works in the field of gamma spectroscopy. First, he recalls some results of experiments performed for the study of peculiar structures associated with different modes of nucleus rotation, and notably in the case of collective rotation of deformed and even super-deformed nuclei. Then, he details tools and methods used to experimentally determine the level scheme. The main characteristics of steady and radioactive beams are briefly presented, and their complementarities and differences are highlighted. Specific spectrometers and sensors are described. In a last chapter, the author discusses several research projects he is involved in, and more particularly the 'gamma tracking' which is the fundamental principle for gamma multi-sensors of the next generations

A phoswich detector for simultaneous alpha–gamma spectroscopy

Energy Technology Data Exchange (ETDEWEB)

Moghadam, S. Rajabi [Department of Radiation Application, Shahid Beheshti University G.C., Tehran (Iran, Islamic Republic of); Feghhi, S.A.H., E-mail: A_feghhi@sbu.ac.ir [Department of Radiation Application, Shahid Beheshti University G.C., Tehran (Iran, Islamic Republic of); Safari, M.J. [Amirkabir University of Technology, Department of Energy Engineering and Physics, Tehran (Iran, Islamic Republic of)

2015-11-01

Phoswich detectors are of value for radiation spectroscopy, especially in cases where a low-cost solution for a mixed radiation field is desired. Meanwhile, simultaneous spectroscopy of alpha particles and gamma-rays has many applications in quantification and distinguishing the alpha-emitting radionuclides which usually occur in the analysis of environmental solid samples. Here, we have developed a system for detection of radioactive actinides (e.g., {sup 241}Am) based on the alpha–gamma coincidence technique. The underlying concept, is to assemble two appropriately selected scintillators (i.e., a fast and a slow one) together with a discriminating unit for analysis of their data. Detailed Monte Carlo simulation procedure has been developed using the GEANT4 toolkit to design and find enough knowledge about the response of the system in the studied radiation field. Various comparisons were made between experimental and simulation data which showed appropriate agreement between them. The calibration was performed and the MDA was estimated as 60 mBq for the phoswich system.

A phoswich detector for simultaneous alpha–gamma spectroscopy

International Nuclear Information System (INIS)

Moghadam, S. Rajabi; Feghhi, S.A.H.; Safari, M.J.

2015-01-01

Phoswich detectors are of value for radiation spectroscopy, especially in cases where a low-cost solution for a mixed radiation field is desired. Meanwhile, simultaneous spectroscopy of alpha particles and gamma-rays has many applications in quantification and distinguishing the alpha-emitting radionuclides which usually occur in the analysis of environmental solid samples. Here, we have developed a system for detection of radioactive actinides (e.g., 241 Am) based on the alpha–gamma coincidence technique. The underlying concept, is to assemble two appropriately selected scintillators (i.e., a fast and a slow one) together with a discriminating unit for analysis of their data. Detailed Monte Carlo simulation procedure has been developed using the GEANT4 toolkit to design and find enough knowledge about the response of the system in the studied radiation field. Various comparisons were made between experimental and simulation data which showed appropriate agreement between them. The calibration was performed and the MDA was estimated as 60 mBq for the phoswich system

Nuclear Gamma-Ray Spectroscopy at the Limit of Particle Stability

International Nuclear Information System (INIS)

Dr. Norbert Pietralla

2006-01-01

The research project ''Nuclear Gamma-Ray Spectroscopy at the Limit of Particle Stability'' with sponsor ID ''DE-FG02-04ER41334'' started late-summer 2004 and aims at the investigation of highly excited low-spin states of selected key-nuclei in the vicinity of the particle separation threshold by means of high-resolution gamma-ray spectroscopy in electromagnetic excitation reactions. This work addresses nuclear structures with excitation energies close to the binding energy or highly excited off-yrast states in accordance with the NSAC milestones. In 2005 the program was extended towards additional use of virtual photons and theoretical description of the low-lying collective excitations in the well deformed nuclei

The Northern Marshall Islands radiological survey: A quality control program for radiochemical and gamma spectroscopy analysis

International Nuclear Information System (INIS)

Kehl, S.R.; Mount, M.E.; Robison, W.L.

1995-09-01

From 1979 to 1989, approximately 25,000 Post Northern Marshall Islands Radiological Survey (PNMIRS) samples were collected, and over 71,400 radiochemical and gamma spectroscopy analyses were performed to establish the concentration of 90 Sr, 137 Cs, 241 Am, and plutonium isotopes in soil, vegetation, fish, and animals in the Northern Marshall Islands. While the Low Level Gamma Counting Facility (B379) in the Health and Ecological Assessment (HEA) division accounted for over 80% of all gamma spectroscopy analyses, approximately 4889 radiochemical and 5437 gamma spectroscopy analyses were performed on 4784 samples of soil, vegetation, terrestrial animal, and marine organisms by outside laboratories. Four laboratories were used by Lawrence Livermore National Laboratory (LLNL) to perform the radiochemical analyses: Thermo Analytical Norcal, Richmond, California (TMA); Nuclear Energy Services, North Carolina State University (NCSU); Laboratory of Radiation Ecology, University of Washington (LRE); and Health and Ecological Assessment (HEA) division, LLNL, Livermore, California. Additionally, LRE and NCSU were used to perform gamma spectroscopy analyses. The analytical precision and accuracy were monitored by including blind duplicates and natural matrix standards in each group of samples analyzed. On the basis of reported analytical values for duplicates and standards, 88% of the gamma and 87% of the radiochemical analyses in this survey were accepted. By laboratory, 93% of the radiochemical analyses by TMA; 88% of the gamma-ray spectrometry and 100% of the radiochemistry analyses by NCSU; 89% of the gamma spectroscopy and 87% of the radiochemistry analyses by LRE; and 90% of the radiochemistry analyses performed by HEA's radiochemistry department were accepted

Use of gamma spectroscopy in activation analysis; Utilisation de la spectrographie gamma dans l'analyse par activation

Energy Technology Data Exchange (ETDEWEB)

Leveque, [Commissariat a l' Energie Atomique, Saclay (France).Centre d' Etudes Nucleaires

1959-07-01

Brief review of the principles of activation analysis: calculation of activities, decay curves, {beta} absorption curves, examples of application. - Principle and description of the {gamma} spectrograph. - Practical utilisation of the {gamma} spectrograph: analysis by activation, analysis by {beta} - x fluorescence. - Sensitivity limit of the method and precision of the measurements. - Possible improvements to the method: {gamma} spectroscopy with elimination of the Compton effect. (author) [French] Bref rappel des principes de l'analyse par activation: calcul des activites, courbes de decroissance, courbes d'absorption {beta}, exemples d'utilisation. - Principe et description du spectrographe {gamma}. - Utilisation pratique de la spectrographie {gamma}: analyse par activation, analyse par fluorescence {beta} - x. - Limite de sensibilite de la methode et precision des mesures. - Ameliorations possibles de la methode: spectrographe {gamma} avec elimination de l'effet Compton. (auteur)

Delayed Gamma-Ray Spectroscopy for Non-Destructive Assay of Nuclear Materials

International Nuclear Information System (INIS)

Ludewigt, Bernhard; Mozin, Vladimir; Campbell, Luke; Favalli, Andrea; Hunt, Alan W.; Reedy, Edward T.E.; Seipel, Heather

2015-01-01

High-energy, beta-delayed gamma-ray spectroscopy is a potential, non-destructive assay techniques for the independent verification of declared quantities of special nuclear materials at key stages of the fuel cycle and for directly assaying nuclear material inventories for spent fuel handling, interim storage, reprocessing facilities, repository sites, and final disposal. Other potential applications include determination of MOX fuel composition, characterization of nuclear waste packages, and challenges in homeland security and arms control verification. Experimental measurements were performed to evaluate fission fragment yields, to test methods for determining isotopic fractions, and to benchmark the modeling code package. Experimental measurement campaigns were carried out at the IAC using a photo-neutron source and at OSU using a thermal neutron beam from the TRIGA reactor to characterize the emission of high-energy delayed gamma rays from 235 U, 239 Pu, and 241 Pu targets following neutron induced fission. Data were collected for pure and combined targets for several irradiation/spectroscopy cycle times ranging from 10/10 seconds to 15/30 minutes.The delayed gamma-ray signature of 241 Pu, a significant fissile constituent in spent fuel, was measured and compared to 239 Pu. The 241 Pu/ 239 Pu ratios varied between 0.5 and 1.2 for ten prominent lines in the 2700-3600 keV energy range. Such significant differences in relative peak intensities make it possible to determine relative fractions of these isotopes in a mixed sample. A method for determining fission product yields by fitting the energy and time dependence of the delayed gamma-ray emission was developed and demonstrated on a limited 235 U data set. De-convolution methods for determining fissile fractions were developed and tested on the experimental data. The use of high count-rate LaBr 3 detectors was investigated as a potential alternative to HPGe detectors. Modeling capabilities were added to an

Characterization system for Germanium detectors dedicated to gamma spectroscopy applied to nuclear waste

Energy Technology Data Exchange (ETDEWEB)

Roccaz, J.; Portella, C.; Saurel, N. [CEA, DAM, VALDUC, F-21120 Is-sur-Tille (France)

2009-07-01

CEA-Valduc produces some radioactive waste (mainly alpha emitters). Legislation requires producers to sort their waste by activity and type of isotopes, and to package them in order to forward them to the appropriate reprocessing or storage facility. Our lab LMDE (laboratory for measurements on nuclear wastes and valuation) is in charge of the characterization of the majority of waste produced by CEA-Valduc. Among non-destructive methods to characterize a radioactive object, gamma-spectroscopy is one of the most efficient. We present to this conference the method we use to characterize nuclear waste and the system we developed to characterize our germanium detectors. The goal of this system is to obtain reliable numerical models of our detectors and calculate their efficiency curves. Measurements are necessary to checks models and improve them. These measurements are made on a bench using pinpoint sources ({sup 133}Ba, {sup 152}Eu) from 60 keV to 1500 keV, with distances from 'on contact' to a few meters from the diode and variable angles between the source and the detector axis. We have demonstrated that we are able to obtain efficiency curves

High resolution gamma-ray spectroscopy applied to bulk sample analysis

International Nuclear Information System (INIS)

Kosanke, K.L.; Koch, C.D.; Wilson, R.D.

1980-01-01

A high resolution Ge(Li) gamma-ray spectrometer has been installed and made operational for use in routine bulk sample analysis by the Bendix Field Engineering Corporation (BFEC) geochemical analysis department. The Ge(Li) spectrometer provides bulk sample analyses for potassium, uranium, and thorium that are superior to those obtained by the BFEC sodium iodide spectrometer. The near term analysis scheme permits a direct assay for uranium that corrects for bulk sample self-absorption effects and is independent of the uranium/radium disequilibrium condition of the sample. A more complete analysis scheme has been developed that fully utilizes the gamma-ray data provided by the Ge(Li) spectrometer and that more properly accounts for the sample self-absorption effect. This new analysis scheme should be implemented on the BFEC Ge(Li) spectrometer at the earliest date

Gamma spectroscopy in water cooled reactors

International Nuclear Information System (INIS)

Persault, M.

1977-10-01

Gamma spectroscopy analysis of spent fuels in power reactors; study of two typical cases: determination of the power distribution by the mean of the activity of a low periodic element (Lanthanum 140) and determination of the burnup absolute rate by examining the ratio of Cesium 134 and Cesium 137 activities. Measures were realized on fuel solutions and on fuel assemblies. Development of a power distribution map of the assemblies and comparison with the results of a three dimensional calculation of core evolution [fr

Delayed Gamma-Ray Spectroscopy for Non-Destructive Assay of Nuclear Materials

Energy Technology Data Exchange (ETDEWEB)

Ludewigt, Bernhard [Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States); Mozin, Vladimir [Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States); Campbell, Luke [Pacific Northwest National Lab. (PNNL), Richland, WA (United States); Favalli, Andrea [Los Alamos National Lab. (LANL), Los Alamos, NM (United States); Hunt, Alan W. [Idaho State Univ., Pocatello, ID (United States); Reedy, Edward T. [Idaho State Univ., Pocatello, ID (United States); Seipel, Heather A. [Idaho State Univ., Pocatello, ID (United States)

2015-06-01

Modeling capabilities were added to an existing framework and codes were adapted as needed for analyzing experiments and assessing application-specific assay concepts including simulation of measurements over many short irradiation/spectroscopy cycles. The code package was benchmarked against the data collected at the IAC for small targets and assembly-scale data collected at LANL. A study of delayed gamma-ray spectroscopy for nuclear safeguards was performed for a variety of assemblies in the extensive NGSI spent fuel library. The modeling results indicate that delayed gamma-ray responses can be collected from spent fuel assemblies with statistical quality sufficient for analyzing their isotopic composition using a 10¹¹ n/s neutron generator and COTS detector instrumentation.

Feasibility study of plutonium isotopic analysis of resin beads by nondestructive gamma-ray spectroscopy

International Nuclear Information System (INIS)

Li, T.K.

1985-01-01

We have initiated a feasibility study on the use of nondestructive low-energy gamma-ray spectroscopy for plutonium isotopic analysis on resin beads. Seven resin bead samples were measured, with each sample containing an average of 9 μg of plutonium; the isotopic compositions of the samples varied over a wide range. The gamma-ray spectroscopy results, obtained from 4-h counting-time measurements, were compared with mass spectrometry results. The average ratios of gamma-ray spectroscopy to mass spectrometry were 1.014 +- 0.025 for 238 Pu/ 239 Pu, 0.996 +- 0.018 for 240 Pu/ 239 Pu, and 0.980 +- 0.038 for 241 Pu/ 239 Pu. The rapid, automated, and accurate nondestructive isotopic analysis of resin beads may be very useful to process technicians and International Atomic Energy Agency inspectors. 3 refs., 1 fig., 3 tabs

Gamma-induced Positron Spectroscopy (GiPS) at a superconducting electron linear accelerator

International Nuclear Information System (INIS)

Butterling, Maik; Anwand, Wolfgang; Cowan, Thomas E.; Hartmann, Andreas; Jungmann, Marco; Krause-Rehberg, Reinhard; Krille, Arnold; Wagner, Andreas

2011-01-01

A new and unique setup for Positron Annihilation Spectroscopy has been established and optimized at the superconducting linear electron accelerator ELBE at Helmholtz-Zentrum Dresden-Rossendorf (Germany). The intense, pulsed (26 MHz) photon source (bremsstrahlung with energies up to 16 MeV) is used to generate positrons by means of pair production throughout the entire sample volume. Due to the very short gamma bunches (< 5 ps temporal length), the facility for Gamma-induced Positron Spectroscopy (GiPS) is suitable for positron lifetime spectroscopy using the accelerator's radiofrequency as time reference. Positron lifetime and Doppler broadening Spectroscopy are employed by a coincident measurement (Age-Momentum Correlation) of the time-of-arrival and energy of the annihilation photons which in turn significantly reduces the background of scattered photons resulting in spectra with high signal to background ratios. Simulations of the setup using the GEANT4 framework have been performed to yield optimum positron generation rates for various sample materials and improved background conditions.

Gamma-induced Positron Spectroscopy (GiPS) at a superconducting electron linear accelerator

Energy Technology Data Exchange (ETDEWEB)

Butterling, Maik, E-mail: maik.butterling@googlemail.com [Martin-Luther University, Dept. of Physics, 06099 Halle (Germany); Institute of Radiation Physics, Helmholtz-Zentrum, Dresden-Rossendorf, P.O. Box 510119, 01314 Dresden (Germany); Anwand, Wolfgang; Cowan, Thomas E.; Hartmann, Andreas [Institute of Radiation Physics, Helmholtz-Zentrum, Dresden-Rossendorf, P.O. Box 510119, 01314 Dresden (Germany); Jungmann, Marco; Krause-Rehberg, Reinhard [Martin-Luther University, Dept. of Physics, 06099 Halle (Germany); Krille, Arnold; Wagner, Andreas [Institute of Radiation Physics, Helmholtz-Zentrum, Dresden-Rossendorf, P.O. Box 510119, 01314 Dresden (Germany)

2011-11-15

A new and unique setup for Positron Annihilation Spectroscopy has been established and optimized at the superconducting linear electron accelerator ELBE at Helmholtz-Zentrum Dresden-Rossendorf (Germany). The intense, pulsed (26 MHz) photon source (bremsstrahlung with energies up to 16 MeV) is used to generate positrons by means of pair production throughout the entire sample volume. Due to the very short gamma bunches (< 5 ps temporal length), the facility for Gamma-induced Positron Spectroscopy (GiPS) is suitable for positron lifetime spectroscopy using the accelerator's radiofrequency as time reference. Positron lifetime and Doppler broadening Spectroscopy are employed by a coincident measurement (Age-Momentum Correlation) of the time-of-arrival and energy of the annihilation photons which in turn significantly reduces the background of scattered photons resulting in spectra with high signal to background ratios. Simulations of the setup using the GEANT4 framework have been performed to yield optimum positron generation rates for various sample materials and improved background conditions.

Delayed Gamma-Ray Spectroscopy for Non-Destructive Assay of Nuclear Materials

Energy Technology Data Exchange (ETDEWEB)

Ludewigt, Bernhard [Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States); Mozin, Vladimir [Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States); Campbell, Luke [Pacific Northwest National Lab. (PNNL), Richland, WA (United States); Favalli, Andrea [Los Alamos National Lab. (LANL), Los Alamos, NM (United States); Hunt, Alan W. [Idaho National Lab. (INL), Idaho Falls, ID (United States); Reedy, Edward T.E. [Idaho National Lab. (INL), Idaho Falls, ID (United States); Seipel, Heather [Idaho National Lab. (INL), Idaho Falls, ID (United States)

2015-06-01

High-­energy, beta-delayed gamma-­ray spectroscopy is a potential, non-­destructive assay techniques for the independent verification of declared quantities of special nuclear materials at key stages of the fuel cycle and for directly assaying nuclear material inventories for spent fuel handling, interim storage, reprocessing facilities, repository sites, and final disposal. Other potential applications include determination of MOX fuel composition, characterization of nuclear waste packages, and challenges in homeland security and arms control verification. Experimental measurements were performed to evaluate fission fragment yields, to test methods for determining isotopic fractions, and to benchmark the modeling code package. Experimental measurement campaigns were carried out at the IAC using a photo-­neutron source and at OSU using a thermal neutron beam from the TRIGA reactor to characterize the emission of high-­energy delayed gamma rays from ²³⁵U, ²³⁹Pu, and ²⁴¹Pu targets following neutron induced fission. Data were collected for pure and combined targets for several irradiation/spectroscopy cycle times ranging from 10/10 seconds to 15/30 minutes.The delayed gamma-ray signature of ²⁴¹Pu, a significant fissile constituent in spent fuel, was measured and compared to ²³⁹Pu. The ²⁴¹Pu/²³⁹Pu ratios varied between 0.5 and 1.2 for ten prominent lines in the 2700-­3600 keV energy range. Such significant differences in relative peak intensities make it possible to determine relative fractions of these isotopes in a mixed sample. A method for determining fission product yields by fitting the energy and time dependence of the delayed gamma-­ray emission was developed and demonstrated on a limited ²³⁵U data set. De-­convolution methods for determining fissile fractions were developed and tested on the experimental data. The use of high count-­rate LaBr₃ detectors

Homogeneity of Gd-based garnet transparent ceramic scintillators for gamma spectroscopy

Science.gov (United States)

Seeley, Z. M.; Cherepy, N. J.; Payne, S. A.

2013-09-01

Transparent polycrystalline ceramic scintillators based on the composition Gd1.49Y1.49Ce0.02Ga2.2Al2.8O12 are being developed for gamma spectroscopy detectors. Scintillator light yield and energy resolution depend on the details of various processing steps, including powder calcination, green body formation, and sintering atmosphere. We have found that gallium sublimation during vacuum sintering creates compositional gradients in the ceramic and can degrade the energy resolution. While sintering in oxygen produces ceramics with uniform composition and little afterglow, light yields are reduced, compared to vacuum sintering. By controlling the atmosphere during the various process steps, we were able to minimize the gallium sublimation, resulting in a more homogeneous composition and improved gamma spectroscopy performance.

Application of gamma-ray spectroscopy in environmental monitoring

International Nuclear Information System (INIS)

Hobbs, B.B.; Kanipe, L.G.; Clayton, W.R.; Belvin, E.A.

1976-01-01

Gamma-ray spectroscopy is used as the primary analytical method in the Tennessee Valley Authority's environmental radiation monitoring program. Routine sample screening is done by means of least-squares analysis of spectra from NaI(Tl) detectors. Nonroutine or suspicious samples are analyzed by means of Ge(Li) spectral analysis. A laboratory quality control program provides internal and external checks on the reliability of analyses

Gamma Spectroscopy with Pixellated CdZnTe Gamma Detectors

International Nuclear Information System (INIS)

Shor, A.; Mardor, I.; Eisen, Y.

2002-01-01

Pixellated CdZnTe detectors are good candidates for room temperature gamma detection requiring spectroscopic performance with imaging capabilities. The CdZnTe materials possess high resistivity and good electron charge transport properties. The poor charge transport for the holes inherent in the CdZnTe material can be circumvented by fabricating the electrodes in any one of a number of structures designed for unipolar charge detection[1]. Recent interest in efficient gamma detection at relatively higher gamma energies has imposed more stringent demands on the CdZnTe material and on detector design and optimization. We developed at Soreq a technique where signals from all pixels and from the common electrode are processed, and then a correction is applied for improving the energy resolution and the photopeak efficiency. For illumination with an un-collimated 133 Ba source , we obtain a combined detector energy resolution of 5.0 % FWHM for the 81 keV peak, and 1.5 % FWHM for the 356 keV peak. We discuss the importance of detector material with high electron (μτ) e for thick Pixellated detectors

{gamma} ray spectroscopy of neutron rich nuclei around N=20; Spectroscopie {gamma} des noyaux riches en neutrons autour de N=20

Energy Technology Data Exchange (ETDEWEB)

Gelin, M

2007-09-15

There is an island of inversion around {sup 32}Mg (12 protons, 20 neutrons) in contradiction with a shell closure N=20. It means a coexistence of spherical and deformed shapes. This work is devoted to the study of {gamma}-ray spectroscopy for nuclei in this region, based on an experiment done at GANIL with a composite secondary beam produced by fragmentation. The originality of the method used here lies in the possibility to study simultaneously several nuclei, and for each of them to explore several reaction channels. The VAMOS spectrometer was used for the identification of the ejectiles. The {gamma}-rays were detected with EXOGAM, a germanium clover array. The detectors used before and after the target allowed for a unique identification and a selection of the reaction channel: inelastic scattering, transfer and fragmentation reaction. In this thesis the following nuclei were studied: {sup 28}Ne, {sup 30-32}Mg {sup 31-34}Al, {sup 33-35}Si, {sup 35}P. New {gamma}-rays have been observed. The {gamma}-ray angular distributions and {gamma}-{gamma} angular correlations have been measured for some transitions. Assignment of spins and parities has been proposed for some states. In particular, in {sup 34}Si, the 3{sup -} assignment is confirmed and a new candidate for the second 0{sup +} has been proposed. In {sup 32}Mg, the state at 2.321 MeV, for which conflicting assignment existed, is deduced from the present data as a 4{sup +}, and a 6{sup +} state is proposed. (author)

Gamma-ray spectroscopy measurements and simulations for uranium mining

Science.gov (United States)

Marchais, T.; Pérot, B.; Carasco, C.; Allinei, P.-G.; Chaussonnet, P.; Ma, J.-L.; Toubon, H.

2018-01-01

AREVA Mines and the Nuclear Measurement Laboratory of CEA Cadarache are collaborating to improve the sensitivity and precision of uranium concentration evaluation by means of gamma measurements. This paper reports gamma-ray spectra, recorded with a high-purity coaxial germanium detector, on standard cement blocks with increasing uranium content, and the corresponding MCNP simulations. The detailed MCNP model of the detector and experimental setup has been validated by calculation vs. experiment comparisons. An optimization of the detector MCNP model is presented in this paper, as well as a comparison of different nuclear data libraries to explain missing or exceeding peaks in the simulation. Energy shifts observed between the fluorescence X-rays produced by MCNP and atomic data are also investigated. The qualified numerical model will be used in further studies to develop new gamma spectroscopy approaches aiming at reducing acquisition times, especially for ore samples with low uranium content.

Gamma-ray spectroscopy of neutron-rich products of heavy-ion collisions

Energy Technology Data Exchange (ETDEWEB)

Carpenter, M.P.; Janssens, R.V.F.; Ahmad, I. [and others

1995-08-01

Thick-target {gamma}{gamma} coincidence techniques are being used to explore the spectroscopy of otherwise hard-to-reach neutron-rich products of deep-inelastic heavy ion reactions. Extensive {gamma}{gamma} coincidence measurements were performed at ATLAS using pulsed beams of {sup 80}Se, {sup 136}Xe, and {sup 238}U on lead-backed {sup 122,124}Sn targets with energies 10-15% above the Coulomb barrier. Gamma-ray coincidence intensities were used to map out yield distributions with A and Z for even-even product nuclei around the target and around the projectile. The main features of the yield patterns are understandable in terms of N/Z equilibration. We had the most success in studying the decays of yrast isomers. Thus far, more than thirty new {mu}s isomers in the Z = 50 region were found and characterized. Making isotopic assignments for previously unknown {gamma}-ray cascades proves to be one of the biggest problems. Our assignments were based (a) on rare overlaps with radioactivity data, (b) on the relative yields with different beams, and (c) on observed cross-coincidences between {gamma} rays from light and heavy reaction partners. However, the primary products of deep inelastic collisions often are sufficiently excited for subsequent neutron evaporation, so {gamma}{gamma} cross-coincidence results require careful interpretation.

Design and construction of prompt-gamma spectroscopy facility applied to the boron determination; Diseno y construccion de una facilidad de espectrometria prompt-gamma aplicada a la determinacion de boro

Energy Technology Data Exchange (ETDEWEB)

Poblete, Victor; Henriquez, Carlos; Klein, Juan; Navarro, Gustavo [Comision Chilena de Energia Nuclear, Santiago (Chile). Centro de Estudios Nucleares La Reina, Comision Chis Nucleares La Reina, Comision Chi Reina

1997-12-31

A prompt-gamma spectroscopy facility was developed using the south tangential neutron beam of the RECH-1 research reactor for boron determination. The implementation of a thermal neutron beam was performed considering different aspects such as biological protection of working area and the beam collimation for a Ge detector, design and sample holder selection, standards and sample preparation. One ppm of Boron in different samples with counting-rate of 20 minutes and a good accuracy were determined. (author). 5 refs.

In-beam gamma spectroscopy of /sup 82/Sr

CERN Document Server

Dewald, A; Gelberg, A; Kaup, U; Von Brentano, P; Zell, K O

1981-01-01

The excited levels of /sup 82/Sr have been investigated by means of in-beam gamma-ray spectroscopy via the reactions /sup 72/Ge(/sup 12/C, 2n), /sup 66/Zn(/sup 19/F, p2n), and /sup 79/Br(/sup 6/Li, 3n). Lifetimes of excited states were measured by the recoil distance method. Excitation energies and B(E2) values have been compared with calculations using the Interacting Boson Model. (19 refs).

Time dependent deadtime and pile-up corrections for gamma-ray spectroscopy

Energy Technology Data Exchange (ETDEWEB)

Roscoe, B A; Furr, A K [Virginia Polytechnic Inst. and State Univ., Blacksburg (USA)

1977-01-15

The losses of pulses in gamma spectroscopy due to the analog-to-digital (ADC) conversion process and due to pulse pile-up is a major problem in quantitative gamma ray spectroscopy. It is especially serious if the count rate varies significantly during the counting interval and if the nuclear events of interest are associated with an isotope with a half-life shorter than or comparable to the counting interval as is often the case for isotopes with half-lives of the order of 10 min or less. The count rates at which dead time losses become a problem depend upon the available equipment but, in the present work, the problem became acute at count rates in excess of 25000 cps. A technique developed at VPI and SU is discussed in the present work which very satisfactorily corrects for both ADC and pile-up losses and is dependent upon the half-life of the decaying radioisotope.

Proceeding of the workshop on gamma-ray spectroscopy utilizing heavy-ion, photon and RI beams

Energy Technology Data Exchange (ETDEWEB)

Oshima, Masumi; Sugita, Michiaki; Hayakawa, Takehito [eds.

1998-03-01

Three time since 1992, we have held the symposia entitled `Joint Spectroscopy Experiments Utilizing JAERI Tandem-Booster Accelerator` at the Tokai Research Establishment. In the symposia, we have mainly discussed the plans of experiments to be done in this joint program. The joint program started in 1994. Several experiments have been made since and some new results have already come up. This symposium `Gamma-ray Spectroscopy utilizing heavy-ion, Photon and RI beams` was held at Tokai Research Establishment of JAERI. Because this symposium is the first occasion after the program started, the first purpose of the symposium is to present and discuss the experimental results so far obtained using the JAERI Tandem-Booster. The second purpose of the symposium is to discuss new possibilities of gamma-ray spectroscopy using new resources such as RI-beam and Photon-beam. The participants from RIKEN, Tohoku University and JAERI Neutron Science Research Center presented the future plans of experiments with RI-beam at each facility. Compared with these nuclear beams, photon beam provides a completely new tool for the {gamma}-ray spectroscopy, which is achieved by inverse Compton scattering between high-energy electron and laser beams. The 23 of the presented papers are indexed individually. (J.P.N.)

Handbook of Applied Solid State Spectroscopy

CERN Document Server

Vij, D. R

2006-01-01

Solid-State spectroscopy is a burgeoning field with applications in many branches of science, including physics, chemistry, biosciences, surface science, and materials science. Handbook of Applied Solid-State Spectroscopy brings together in one volume information about various spectroscopic techniques that is currently scattered in the literature of these disciplines. This concise yet comprehensive volume covers theory and applications of a broad range of spectroscopies, including NMR, NQR, EPR/ESR, ENDOR, scanning tunneling, acoustic resonance, FTIR, auger electron emission, x-ray photoelectron emission, luminescence, and optical polarization, and more. Emphasis is placed on fundamentals and current methods and procedures, together with the latest applications and developments in the field.

Experimental investigation of silicon photomultipliers as compact light readout systems for gamma-ray spectroscopy applications in fusion plasmas

Energy Technology Data Exchange (ETDEWEB)

Nocente, M., E-mail: massimo.nocente@mib.infn.it; Gorini, G. [Dipartimento di Fisica “G. Occhialini,” Università degli Studi di Milano-Bicocca, Milano (Italy); Istituto di Fisica del Plasma “P. Caldirola,” EURATOM-ENEA-CNR Association, Milano (Italy); Fazzi, A.; Lorenzoli, M.; Pirovano, C. [Dipartimento di Energia, CeSNEF, Politecnico di Milano, Milano (Italy); Istituto Nazionale di Fisica Nucleare, Sezione di Milano, Milano (Italy); Tardocchi, M. [Istituto di Fisica del Plasma “P. Caldirola,” EURATOM-ENEA-CNR Association, Milano (Italy); Cazzaniga, C.; Rebai, M. [Dipartimento di Fisica “G. Occhialini,” Università degli Studi di Milano-Bicocca, Milano (Italy); Uboldi, C.; Varoli, V. [Dipartimento di Energia, CeSNEF, Politecnico di Milano, Milano (Italy)

2014-11-15

A matrix of Silicon Photo Multipliers has been developed for light readout from a large area 1 in. × 1 in. LaBr{sub 3} crystal. The system has been characterized in the laboratory and its performance compared to that of a conventional photo multiplier tube. A pulse duration of 100 ns was achieved, which opens up to spectroscopy applications at high counting rates. The energy resolution measured using radioactive sources extrapolates to 3%–4% in the energy range E{sub γ} = 3–5 MeV, enabling gamma-ray spectroscopy measurements at good energy resolution. The results reported here are of relevance in view of the development of compact gamma-ray detectors with spectroscopy capabilities, such as an enhanced gamma-ray camera for high power fusion plasmas, where the use of photomultiplier is impeded by space limitation and sensitivity to magnetic fields.

Random pulsing of neutron source for inelastic neutron scattering gamma ray spectroscopy

International Nuclear Information System (INIS)

Hertzog, R.C.

1981-01-01

Method and apparatus are described for use in the detection of inelastic neutron scattering gamma ray spectroscopy. Data acquisition efficiency is enhanced by operating a neutron generator such that a resulting output burst of fast neutrons is maintained for as long as practicably possible until a gamma ray is detected. Upon the detection of a gamma ray the generator burst output is terminated. Pulsing of the generator may be accomplished either by controlling the burst period relative to the burst interval to achieve a constant duty cycle for the operation of the generator or by maintaining the burst period constant and controlling the burst interval such that the resulting mean burst interval corresponds to a burst time interval which reduces contributions to the detected radiation of radiation occasioned by other than the fast neutrons

Applied spectroscopy and the science of nanomaterials

CERN Document Server

2015-01-01

This book focuses on several areas of intense topical interest related to applied spectroscopy and the science of nanomaterials. The eleven chapters in the book cover the following areas of interest relating to applied spectroscopy and nanoscience: ·         Raman spectroscopic characterization, modeling and simulation studies of carbon nanotubes, ·         Characterization of plasma discharges using laser optogalvanic spectroscopy, ·         Fluorescence anisotropy in understanding protein conformational disorder and aggregation, ·         Nuclear magnetic resonance spectroscopy in nanomedicine, ·         Calculation of Van der Waals interactions at the nanoscale, ·         Theory and simulation associated with adsorption of gases in nanomaterials, ·         Atom-precise metal nanoclusters, ·         Plasmonic properties of metallic nanostructures, two-dimensional materials, and their composites, ·         Applications of graphe...

Gamma-ray tracking - A new detector concept for nuclear spectroscopy

International Nuclear Information System (INIS)

Gast, W.

2001-01-01

In the framework of an European collaboration the nest generation of large efficiency, high resolution spectrometers for nuclear spectroscopy is under development. The new spectrometers are large volume, segmented Ge-detectors featuring 3D position sensitivity in order to allow Gamma-Ray Tracking. That is, knowing the interaction positions and the energies released at each interaction, the track each gamma-ray follows during its scattering process inside the detector volume can be reconstructed on basis of the Compton-scattering formula. The resulting high add-back efficiency an effective granularity significantly improves peak-to-total ratio, efficiency, and Doppler-broadening of the spectrometer. In this contribution the states of the project concerning detector design and development of digital signal processing techniques to achieve an optimal 3D position sensitivity is presented. (authors)

Line and continuum spectroscopy as diagnostic tools for gamma ray bursts

International Nuclear Information System (INIS)

Liang, E.P.

1990-12-01

We review the theoretical framework of both line and continuum spectra formation in gamma ray bursts. These include the cyclotron features at 10's of keV, redshifted annihilation features at ∼400 keV, as well as other potentially detectable nuclear transition lines, atomic x-ray lines, proton cyclotron lines and plasma oscillation lines. By combining the parameters derived from line and continuum modeling we can try to reconstruct the location, geometry and physical conditions of the burst emission region, thereby constraining and discriminating the astrophysical models. Hence spectroscopy with current and future generations of detectors should provide powerful diagnostic tools for gamma ray bursters. 48 refs., 10 figs., 4 tabs

Neutron-induced gamma-ray spectroscopy: simulations for chemical mapping of planetary surfaces

International Nuclear Information System (INIS)

Brueckner, J.; Waenke, H.; Reedy, R.C.

1986-01-01

Cosmic rays interact with the surface of a planetary body and produce a cascade of secondary particles, such as neutrons. Neutron-induced scattering and capture reactions play an important role in the production of discrete gamma-ray lines that can be measured by a gamma-ray spectrometer on board of an orbiting spacecraft. These data can be used to determine the concentration of many elements in the surface of a planetary body, which provides clues to its bulk composition and in turn to its origin and evolution. To investigate the gamma rays made by neutron interactions, thin targets were irradiated with neutrons having energies from 14 MeV to 0.025 eV. By means of foil activation technique the ratio of epithermal to thermal neutrons was determined to be similar to that in the Moon. Gamma rays emitted by the targets and the surrounding material were detected by a high-resolution germanium detector in the energy range of 0.1 to 8 MeV. Most of the gamma-ray lines that are expected to be used for planetary gamma-ray spectroscopy were found in the recorded spectra and the principal lines in these spectra are presented. 58 refs., 7 figs., 9 tabs

Investigations of 131I concentration in indoor air using charcoal filters and gamma spectroscopy

International Nuclear Information System (INIS)

Fischer, H.W.; Pittauerova, D.; Foschepoth, S.; Poppe, B.

2008-01-01

Full text: Radiation protection standards require the recording of staff radiation dose in nuclear medicine thyroid radiotherapy. A commonly used method measures the 131 I thyroid activity externally with a gamma detector, followed by calculation of the committed equivalent thyroid dose. The main disadvantages are the low sensitivity and the uncertainty of the time of uptake, which can only be compensated by long measurement times and short measurement intervals. The measurements have to be applied to all staff members. An alternative can be provided by the measurement of the cumulated concentration of 131 I in indoor air using charcoal filters. The filters are placed in patient rooms at representative locations, exposed for several days and then investigated for absorbed 131 I activity. Both above mentioned disadvantages can be overcome: the measurement records the cumulated concentration history of the room and the obtained value can be used for dose calculation for all staff members knowing their working history. Standard charcoal filters (PicoRad vials, Accustar Labs, normally used for indoor radon measurements) were placed into patient rooms in a thyroid therapy department and exposed to room air for 72 hours. The vials were then subjected to high resolution low level gamma spectroscopy using a high purity germanium (hpGe) detector (50% relative efficiency, 10 cm lead shielding). Absolute activity determination was based on the net count rate in the 364 keV gamma peak and absolute counting efficiency obtained mathematically from detector and vial geometry using the commercial Labsocs (Canberra Inc.) program. Using the mean air activity/vial activity calibration factor obtained in a similar study pioneering this application, but using liquid scintillation spectroscopy as detection method (F. Jimenez et al, 2nd. European IRPA Congress, Paris 2006), mean air concentrations between 0.09 and 2.01 Bq/m 3 were found. The data correlated well with patient administered

Application of neuro-fuzzy methods to gamma spectroscopy

Science.gov (United States)

Grelle, Austin L.

Nuclear non-proliferation activities are an essential part of national security activities both domestic and abroad. The safety of the public in densely populated environments such as urban areas or large events can be compromised if devices using special nuclear materials are present. Therefore, the prompt and accurate detection of these materials is an important topic of research, in which the identification of normal conditions is also of importance. With gamma-ray spectroscopy, these conditions are identified as the radiation background, which though being affected by a multitude of factors is ever present. Therefore, in nuclear non-proliferation activities the accurate identification of background is important. With this in mind, a method has been developed to utilize aggregate background data to predict the background of a location through the use of an Artificial Neural Network (ANN). After being trained on background data, the ANN is presented with nearby relevant gamma-ray spectroscopy data---as identified by a Fuzzy Inference System - to create a predicted background spectra to compare to a measured spectra. If a significant deviation exists between the predicted and measured data, the method alerts the user such that a more thorough investigation can take place. Research herein focused on data from an urban setting in which the number of false positives was observed to be 28 out of a total of 987, representing 2.94% error. The method therefore currently shows a high rate of false positives given the current configuration, however there are promising steps that can be taken to further minimize this error. With this in mind, the method stands as a potentially significant tool in urban nuclear nonproliferation activities.

Camel molar tooth enamel response to gamma rays using EPR spectroscopy.

Science.gov (United States)

El-Faramawy, N A; El-Somany, I; Mansour, A; Maghraby, A M; Eissa, H; Wieser, A

2018-03-01

Tooth enamel samples from molar teeth of camel were prepared using a combined procedure of mechanical and chemical tooth treatment. Based on electron paramagnetic resonance (EPR) spectroscopy, the dose response of tooth enamel samples was examined and compared to that of human enamel. The EPR dose response of the tooth enamel samples was obtained through irradiation to gamma doses from 1 Gy up to 100 kGy. It was found that the radiation-induced EPR signal increased linearly with gamma dose for all studied tooth enamel samples, up to about 15 kGy. At higher doses, the dose response curve leveled off. The results revealed that the location of the native signal of camel tooth enamel was similar to that of enamel from human molars at 2.00644, but different from that of enamel from cows and goats. In addition, the peak-to-peak width (ΔH pp ) for human and camel molar teeth was similar. It was also found that the response of camel enamel to gamma radiation was 36% lower than that of human enamel. In conclusion, the results indicate the suitability of camel teeth for retrospective gamma dosimetry.

Camel molar tooth enamel response to gamma rays using EPR spectroscopy

Energy Technology Data Exchange (ETDEWEB)

El-Faramawy, N.A.; El-Somany, I. [Ain Shams University, Physics Department, Faculty of Science, Cairo (Egypt); Mansour, A. [National Center for Radiation Research and Technology, Atomic Energy Authority, Cairo (Egypt); Maghraby, A.M.; Eissa, H. [National Institute of Standards (NIS), Ionizing Radiation Metrology Laboratory, Giza (Egypt); Wieser, A. [Helmholtz Zentrum Muenchen-German Research Center for Environmental Health, Department of Radiation Sciences, Institute of Radiation Protection, Neuherberg (Germany)

2018-03-15

Tooth enamel samples from molar teeth of camel were prepared using a combined procedure of mechanical and chemical tooth treatment. Based on electron paramagnetic resonance (EPR) spectroscopy, the dose response of tooth enamel samples was examined and compared to that of human enamel. The EPR dose response of the tooth enamel samples was obtained through irradiation to gamma doses from 1 Gy up to 100 kGy. It was found that the radiation-induced EPR signal increased linearly with gamma dose for all studied tooth enamel samples, up to about 15 kGy. At higher doses, the dose response curve leveled off. The results revealed that the location of the native signal of camel tooth enamel was similar to that of enamel from human molars at 2.00644, but different from that of enamel from cows and goats. In addition, the peak-to-peak width (ΔH{sub pp}) for human and camel molar teeth was similar. It was also found that the response of camel enamel to gamma radiation was 36% lower than that of human enamel. In conclusion, the results indicate the suitability of camel teeth for retrospective gamma dosimetry. (orig.)

Determination of nuclear fuel burnup by non-destructive gamma spectroscopy

International Nuclear Information System (INIS)

Soares, A.J.

1979-01-01

The determination of nuclear fuel burnup by the non-destructive gamma spectroscopy method is studied. A MTR (Materials Testing Reactor) -type fuel element is used in the measurement. The fuel element was removed from the reactor core in 1958 and, because of the long decay time, show only one peak in is gamma spectrum at 661.6 Kev. Corresponding to 137 Cs. Measurements are made at 330 points of the element using a Nal detector and the final result revealed that the quantity of 235 U consumed was 3.3 +- 0,8 milligram in the entire element. The effect of the migration of 137 Cs in the element is neglected in view of the fact that it occurs only when the temperature is above 1000 0 C, which is not the case in IEAR-1. (Author)

A large-capacity sample-changer for automated gamma-ray spectroscopy

International Nuclear Information System (INIS)

Andeweg, A.H.

1980-01-01

An automatic sample-changer has been developed at the National Institute for Metallurgy for use in gamma-ray spectroscopy with a lithium-drifted germanium detector. The sample-changer features remote storage, which prevents cross-talk and reduces background. It has a capacity for 200 samples and a sample container that takes liquid or solid samples. The rotation and vibration of samples during counting ensure that powdered samples are compacted, and improve the precision and reproducibility of the counting geometry [af

Principles of resonance-averaged gamma-ray spectroscopy

International Nuclear Information System (INIS)

Chrien, R.E.

1981-01-01

The unambiguous determination of excitation energies, spins, parities, and other properties of nuclear levels is the paramount goal of the nuclear spectroscopist. All developments of nuclear models depend upon the availability of a reliable data base on which to build. In this regard, slow neutron capture gamma-ray spectroscopy has proved to be a valuable tool. The observation of primary radiative transitions connecting initial and final states can provide definite level positions. In particular the use of the resonance-averaged capture technique has received much recent attention because of the claims advanced for this technique (Chrien 1980a, Casten 1980); that it is able to identify all states in a given spin-parity range and to provide definite spin parity information for these states. In view of the importance of this method, it is perhaps surprising that until now no firm analytical basis has been provided which delineates its capabilities and limitations. Such an analysis is necessary to establish the spin-parity assignments derived from this method on a quantitative basis; in other words a quantitative statement of the limits of error must be provided. It is the principal aim of the present paper to present such an analysis. To do this, a historical description of the technique and its applications is presented and the principles of the method are stated. Finally a method of statistical analysis is described, and the results are applied to recent measurements carried out at the filtered beam facilities at the Brookhaven National Laboratory

Combined in-beam gamma-ray and conversion electron spectroscopy with radioactive ion beams

Directory of Open Access Journals (Sweden)

Konki J.

2013-12-01

Full Text Available In-beam gamma-ray and electron spectroscopy have been widely used as tools to study the broad variety of phenomena in nuclear structure. The SPEDE spectrometer is a new device to be used in conjunction with the MINIBALL germanium detector array to enable the detection of internal conversion electrons in coincidence with gamma rays from de-exciting nuclei in radioactive ion beam experiments at the upcoming HIE-ISOLDE facility at CERN, Switzerland. Geant4 simulations were carried out in order to optimise the design and segmentation of the silicon detector to achieve good energy resolution and performance.

Digital gamma-ray spectroscopy based on FPGA technology

CERN Document Server

Bolic, M

2002-01-01

A digital pulse processing system convenient for high rate gamma-ray spectroscopy with NaI(Tl) detectors has been designed. The new programmable logic device has been used for implementation of dedicated high-speed pulse processor, as the central part of the system. The processor is capable to operate at the speed of fast ADC, preserving maximum throughput of the system. Special care has been taken to reduce the distortion of energy spectrum caused by pile-up at high-count rates. The developed system is highly flexible, and the parameters of its operation can be changed in software. The performance of the system was tested for high counting rate of 400000 s sup - sup 1.

Elastic properties of gamma-Pu by resonant ultrasound spectroscopy

Energy Technology Data Exchange (ETDEWEB)

Migliori, Albert [Los Alamos National Laboratory; Betts, J [Los Alamos National Laboratory; Trugman, A [Los Alamos National Laboratory; Mielke, C H [Los Alamos National Laboratory; Mitchell, J N [Los Alamos National Laboratory; Ramos, M [Los Alamos National Laboratory; Stroe, I [WORXESTER, MA

2009-01-01

Despite intense experimental and theoretical work on Pu, there is still little understanding of the strange properties of this metal. We used resonant ultrasound spectroscopy method to investigate the elastic properties of pure polycrystalline Pu at high temperatures. Shear and longitudinal elastic moduli of the {gamma}-phase of Pu were determined simultaneously and the bulk modulus was computed from them. A smooth linear and large decrease of all elastic moduli with increasing temperature was observed. We calculated the Poisson ratio and found that it increases from 0.242 at 519K to 0.252 at 571K.

The structure of neutron-rich nuclei explored via in-beam gamma-ray spectroscopy of fast beams

International Nuclear Information System (INIS)

Glasmacher, T.; Campbell, C.M.; Church, J.A.; Dinca, D.C.; Hansen, P.G.; Olliver, H.; Perry, B.C.; Sherrill, B.M.; Terry, J.R.; Bazin, D.; Enders, J.; Gade, A.; Hu, Z.; Mueller, W.F.

2003-01-01

In-beam gamma-ray spectroscopy with fast exotic beams provides an efficient tool to study bound states in exotic neutron-rich nuclei. Specialized experimental techniques have been developed and explore different aspects of nuclear structure. Inelastic scattering experiments with γ-ray detection can measure the response of exotic nuclei to electromagnetic (Coulomb excitation with a heavy target) or hadronic probes (proton scattering with hydrogen target). In-beam fragmentation populates higher-lying bound states to establish levels. Single- and two-nucleon knockout reactions allow for detailed wavefunction spectroscopy of individual levels and for the measurement of spectroscopic factors. Experimental programs employing these techniques are now underway at all projectile-fragmentation facilities around the world. Here we report on several successful in-beam gamma-ray spectroscopy experiments that have been performed at the Coupled Cyclotron Facility at Michigan State University with an emphasis on elucidating the evolution of nuclear structure around neutron numbers N=16, N=20, and N=28 in the π(sd) shell. (orig.)

Evaluation of Multi-Channel ADCs for Gamma-Ray Spectroscopy

Science.gov (United States)

Tan, Hui; Hennig, Wolfgang; Walby, Mark D.; Breus, Dimitry; Harris, Jackson

2013-04-01

As nuclear physicists increasingly design large scale experiments with hundreds or thousands of detector channels, there are growing needs for high density readout electronics with good timing and energy resolution that at the same time offer lower cost per channel compared to existing commercial solutions. Recent improvements in the design of commercial analog to digital converters (ADCs) have resulted in a variety of multi-channel ADCs that are natural choice for designing such high density readout modules. However, multi-channel ADCs typically are designed for medical imaging/ultrasound applications and therefore are not rated for their spectroscopic characteristics. In this work, we evaluated the gamma-ray spectroscopic performance of several multi-channel ADCs, including their energy resolution, nonlinearity, and timing resolution. Some of these ADCs demonstrated excellent energy resolution, 2.66% FWHM at 662 keV with a LaBr3 or 1.78 keV FWHM at 1332.5 keV with a high purity germanium (HPGe) detector, and sub-nanosecond timing resolution with LaBr 3. We present results from these measurements to illustrate their suitability for gamma-ray spectroscopy.

Solid state structural investigations of the bis(chalcone) compound with single crystal X-ray crystallography, DFT, gamma-ray spectroscopy and chemical spectroscopy methods

Science.gov (United States)

Yakalı, Gül; Biçer, Abdullah; Eke, Canel; Cin, Günseli Turgut

2018-04-01

A bis(chalcone), (2E,6E)-2,6-bis((E)-3phenylallidene)cyclohexanone, was characterized by 1H NMR, 13C NMR, FTIR, UV-Vis spectroscopy, gamma-ray spectroscopy and single crystal X- ray structural analysis. The optimized molecular structure of the compound is calculated using DFT/B3LYP with 6-31G (d,p) level. The calculated geometrical parameters are in good agreement with the experimental data obtained from our reported X-ray structure. The powder and single crystal compounds were gama-irradiated using clinical electron linear accelerator and 60Co gamma-ray source, respectively. Spectral studies (1H NMR, 13C NMR, FTIR and UV-Vis) of powder chalcone compound were also investigated before and after irradiation. Depending on the irradiation notable changes were observed in spectral features powder sample. Single crystal X-ray diffraction investigation shows that both unirradiated and irradiated single crystal samples crystallizes in a orthorhombic crystal system in the centrosymmetric space group Pbcn and exhibits an C-H..O intramolecular and intermolecular hydrogen bonds. The crystal packing is stabilised by strong intermolecular bifurcate C-H..O hydrogen bonds and π…π stacking interactions. The asymmetric unit of the title compound contains one-half of a molecule. The other half of the molecule is generated with (1-x,y,-3/2-z) symmetry operator. The molecule is almost planar due to having π conjugated system of chalcones. However, irradiated single crystal compound showed significant changes lattice parameters, crystal volume and density. According to results of gamma-ray spectroscopy, radioactive elements of powder compound which are 123Sb(n,g),124Sb,57Fe(g,p),56Mn, 55Mn(g,n), and 54Mn were determined using photoactivation analysis. However, the most intensive gamma-ray energy signals are 124Sb.

Determination of moisture content and natural radioactivity in soils using gamma spectroscopy

Energy Technology Data Exchange (ETDEWEB)

Abdel-Hady, E E [Department of Physics, Faculty of Science, Qater University (Qatar); El-Sayed, A M.A.; Alaa, H B [Department of Physics, Faculty of Science, El-Minia University, Minia (Egypt)

1997-12-31

The gamma-ray transmission method has been used to study the soil-water properties in the laboratory as well as in the field. The present measurements were performed using gamma-ray spectroscopy system based on a 5 x 5 cm Nal (T 1) scintillation detector and combined sources ({sup 137} Cs and {sup 241} Am). The two sources are placed in a suitable lead collimator to obtain a pin beam of 1 mm diameter. Suitable samples of clay and sandy soils obtained from the local field were prepared to determine the water content and the soil bulk densities by the combined method for different moisture stages. From the results obtained, it is clear that the soil density at both stages (saturated and after drainage) remains the same. this is because the soil particles do not rearrange during the wetting and drying process. The full results will be presented in the text. Natural radioactivity of the investigated samples was also studied using gamma-ray spectrometer having HPGe detector. Qualitative and quantitative analysis of natural gamma radiations revealed the presence of {sup 40} K, {sup 214} Bi, {sup 208} TI and {sup 228} Ac in meaningful concentrations. 3 figs.

Currie detection limits in gamma-ray spectroscopy

International Nuclear Information System (INIS)

Geer, L.-E. de

2004-01-01

Currie Hypothesis testing is applied to gamma-ray spectral data, where an optimum part of the peak is used and the background is considered well known from nearby channels. With this, the risk of making Type I errors is about 100 times lower than commonly assumed. A programme, PeakMaker, produces random peaks with given characteristics on the screen and calculations are done to facilitate a full use of Poisson statistics in spectrum analyses. Short technical note summary: The Currie decision limit concept applied to spectral data is reinterpreted, which gives better consistency between the selected error risk and the observed error rates. A PeakMaker program is described and the few count problem is analyzed

Gamma ray spectroscopy and timing using LSO and PIN photodiodes

International Nuclear Information System (INIS)

Moses, W.W.; Derenzo, S.E.; Melcher, C.L.; Manente, R.A.

1994-11-01

The high density, high light output, and short decay time of LSO (lutetium orthosilicate, Lu 2 SiO 5 :Ce) make it an attractive scintillator for gamma ray spectroscopy. The low cost, small size, high quantum efficiency, and ruggedness of silicon photodiodes make them attractive photodetectors for this same application, although their high noise (Compared to a photomultiplier tube) reduces their appeal. In this work the authors measure the gamma ray energy resolution, timing accuracy, and conversion factor from gamma energy to number of electron-hole pairs produced with a 3 x 3 x 22 mm 3 LSO scintillator crystal read out with a 3 x 3 mm 2 silicon PIN photodiode. When the detector is excited with 511 keV photons, a photopeak centered at 1,940 e - with 149 keV fwhm is observed and a timing signal with 35 ns fwhm jitter is produced. When the detector is excited with 1,275 keV photons, a photopeak centered at 4,910 e - with 149 keV fwhm is observed and a timing signal with 25 ns fwhm jitter is produced. While these performance measures are inferior to those obtained with photomultiplier tubes, they are acceptable for some applications

High-sensitivity gamma spectroscopy for extended sources. Application to activity measurements on the human body, on glass, and on soil

International Nuclear Information System (INIS)

Jouve, B.

1962-01-01

The measurement and location by gamma spectroscopy of human body internal contaminations at maximum permissible levels, and, in certain cases, at lower activities such as that due to 40 K was investigated. The characteristics of the high-sensitivity apparatus used are given, and several assemblies using large-volume NaI(Tl) scintillators are described. The relatively light shielding required for natural radioactivity permitted construction of mobile assembly. Conditions of use are described, and the results are given. All gamma emitting elements were measured in 15 min at levels lower than the tolerance dose. Gamma spectroscopy was also used to determine fission products in the earth and to study radioactive elements in the presence of other emitters. (author) [fr

Matrix Isolation Spectroscopy Applied to Positron Moderatioin in Cryogenic Solids

Science.gov (United States)

2011-07-01

Current Positron Applications • 2-γ decay exploited in Positron Emission Tomography (PET) scanners. • Positrons localize & annihilate preferentially at...Air Force  Eglin Air Force Base AFRL-RW-EG-TP-2011-024 Matrix Isolation Spectroscopy Applied to Positron Moderation in Cryogenic Solids Distribution... Spectroscopy Applied to Positron Moderation in Cryogenic Solids 5a. CONTRACT NUMBER 5b. GRANT NUMBER 62602F 5c. PROGRAM ELEMENT NUMBER 6

Effects of gamma irradiation on microhardness and Fourier Transform Infrared Spectroscopy of bovine bone

Energy Technology Data Exchange (ETDEWEB)

Dias, Derly Augusto; Pereira, Daisa L.; Gomes, Gabriela V.; Sugahara, Vanessa M.L.; Mathor, Monica B.; Zezell, Denise Maria, E-mail: zezell@usp.br [Instituto de Pesquisas Energeticas e Nucleares (IPEN/CNEN-SP), Sao Paulo, SP (Brazil). Centro para Lasers e Aplicacoes

2017-07-01

The skeletal systems with the structural arrangement of the bone are very important for load distribution, mechanical resistance and vital organs protection. The bone structure is multiphase and composed of organic, inorganic (mineral) compounds and water. Gamma radiation is an ionizing radiation that comes from gamma radiation sources or X-ray generator is commonly used in health establishments such as radio diagnostic exams, radiotherapy and sterilization of allograft. The characterization of the irradiated bone tissue can be is an important tool to study of the components that are affected and how much each dose of ionizing radiation can alter its mechanical properties. This information will be very important in in vitro and ex vivo studies where sterilization of the bone material is necessary and may still be useful in understanding the effects on the bone tissue of patients undergoing short-term radiotherapy. For this, 110 samples of bovine femur diaphysis were randomized into 11 groups: G1 untreated (control); G2 to G11 were submitted to gamma irradiation ({sup 60}Co Gammacel). Samples were polished before irradiation and submitted to a Knoop Microhardness Test to determine the hardness of bovine bone and Fourier transform Infrared spectroscopy (FTIR) to biochemical characterization. Spectra were collected in the mid-infrared range in Attenuated Total Reflectance (ATR) sampling mode associated whit PCA multivariate technique to evaluate the molecular changes in bone matrix. It was observed that hardness was not altered by gamma irradiation and FTIR spectroscopy associated with PCA is a good method to analyze the changes in bone tissue submitted to ionizing radiation. (author)

Effects of gamma irradiation on microhardness and Fourier Transform Infrared Spectroscopy of bovine bone

International Nuclear Information System (INIS)

Dias, Derly Augusto; Pereira, Daisa L.; Gomes, Gabriela V.; Sugahara, Vanessa M.L.; Mathor, Monica B.; Zezell, Denise Maria

2017-01-01

The skeletal systems with the structural arrangement of the bone are very important for load distribution, mechanical resistance and vital organs protection. The bone structure is multiphase and composed of organic, inorganic (mineral) compounds and water. Gamma radiation is an ionizing radiation that comes from gamma radiation sources or X-ray generator is commonly used in health establishments such as radio diagnostic exams, radiotherapy and sterilization of allograft. The characterization of the irradiated bone tissue can be is an important tool to study of the components that are affected and how much each dose of ionizing radiation can alter its mechanical properties. This information will be very important in in vitro and ex vivo studies where sterilization of the bone material is necessary and may still be useful in understanding the effects on the bone tissue of patients undergoing short-term radiotherapy. For this, 110 samples of bovine femur diaphysis were randomized into 11 groups: G1 untreated (control); G2 to G11 were submitted to gamma irradiation ("6"0Co Gammacel). Samples were polished before irradiation and submitted to a Knoop Microhardness Test to determine the hardness of bovine bone and Fourier transform Infrared spectroscopy (FTIR) to biochemical characterization. Spectra were collected in the mid-infrared range in Attenuated Total Reflectance (ATR) sampling mode associated whit PCA multivariate technique to evaluate the molecular changes in bone matrix. It was observed that hardness was not altered by gamma irradiation and FTIR spectroscopy associated with PCA is a good method to analyze the changes in bone tissue submitted to ionizing radiation. (author)

A silicon photomultiplier readout for time of flight neutron spectroscopy with {gamma}-ray detectors

Energy Technology Data Exchange (ETDEWEB)

Pietropaolo, A.; Gorini, G. [Dipartimento di Fisica ' ' G. Occhialini' ' and CNISM, Universita Degli Studi di Milano-Bicocca, Piazza della Scienza 3, 20126 Milano (Italy); Festa, G.; Andreani, C.; De Pascale, M. P.; Reali, E. [Dipartimento di Fisica and Centro NAST, Universita degli Studi di Roma Tor Vergata, Via della Ricerca Scientifica 1, 00133, Roma (Italy); Grazzi, F. [Istituto dei Sistemi Complessi-Consiglio Nazionale delle Ricerche, Via Madonna del Piano n.10, I-50019 Sesto Fiorentino, Firenze (Italy); Schooneveld, E. M. [ISIS Facility, Rutherford Appleton Laboratory, Chilton, Didcot, Oxfordshire, OX11 0QX (United Kingdom)

2009-09-15

The silicon photomultiplier (SiPM) is a recently developed photosensor used in particle physics, e.g., for detection of minimum ionizing particles and/or Cherenkov radiation. Its performance is comparable to that of photomultiplier tubes, but with advantages in terms of reduced volume and magnetic field insensitivity. In the present study, the performance of a gamma ray detector made of an yttrium aluminum perovskite scintillation crystal and a SiPM-based readout is assessed for use in time of flight neutron spectroscopy. Measurements performed at the ISIS pulsed neutron source demonstrate the feasibility of {gamma}-detection based on the new device.

Gamma-ray-spectroscopy following high-flux 14-MeV neutron activation

International Nuclear Information System (INIS)

Williams, R.E.

1981-01-01

The Rotating Target Neutron Source (RTNS-I), a high-intensity source of 14-MeV neutrons at the Lawrence Livermore National Laboratory (LLNL), has been used for applications in activation analysis, inertial-confinement-fusion diagnostic development, and fission decay-heat studies. The fast-neutron flux from the RTNS-I is at least 50 times the maximum fluxes available from typical neutron generators, making these applications possible. Facilities and procedures necessary for gamma-ray spectroscopy of samples irradiated at the RTNS-I were developed

Gamma-ray-spectroscopy following high-flux 14-MeV neutron activation

Energy Technology Data Exchange (ETDEWEB)

Williams, R.E.

1981-10-12

The Rotating Target Neutron Source (RTNS-I), a high-intensity source of 14-MeV neutrons at the Lawrence Livermore National Laboratory (LLNL), has been used for applications in activation analysis, inertial-confinement-fusion diagnostic development, and fission decay-heat studies. The fast-neutron flux from the RTNS-I is at least 50 times the maximum fluxes available from typical neutron generators, making these applications possible. Facilities and procedures necessary for gamma-ray spectroscopy of samples irradiated at the RTNS-I were developed.

Investigation of electric quadrupole interaction in TiO2 by means of perturbed gamma-gamma angular correlation spectroscopy

International Nuclear Information System (INIS)

Martucci, Thiago; Ramos, Juliana Marques; Carbonari, Artur Wilson; Silva, Andreia S.; Saxena, Rajendra Narain

2011-01-01

TiO 2 has called attention in both basic research and technological applications as an energy converter in solar cells, photo catalyst for water purification, sunscreen material, drug detection, and other applications. In addition TiO 2 is a candidate for use in medical devices, food preparation surfaces, air conditioning filters and sanitary ware surfaces.TiO 2 has two crystalline phases: anatase and rutile. The structural properties and hyperfine interactions in TiO 2 were investigated by perturbed gamma-gamma angular correlation (PAC) spectroscopy using 111 In and 181 Hf as probe nuclei. The PAC spectroscopy provides information on crystalline and electronic structure at an atomic scale. In the present work, PAC measurements on TiO 2 were focused on the development of a methodology to prepare bulk samples, which have been characterized by conventional techniques such as x-ray diffraction, (XRD), scanning electron microscopy (SEM) and Energy Dispersive Spectroscopy (EDS). The samples were prepared by the sol gel Pechini method. The resulting powders were annealed at different temperatures in a tubular furnace under nitrogen atmosphere. The PAC measurements were carried out at room temperature in air. The occupation fraction of the probe nuclei reached 50% when the sample was annealed at 1373K and after measured at room temperature.In this case the frequency measured in site 1 is in agreement with that found in literature for substitutional titanium site in rutile structure when 111 In were used as probe nuclei. It was measured a frequency more closely to that was found in literature[7] for the case in which 181 Hf were used as probe nuclei when the sample annealed at 1373 K and measured at 973 K. (author)

Measurement of plutonium isotopic composition by gamma-ray spectroscopy

International Nuclear Information System (INIS)

Kim, J. S.; Shin, J. S.; Ahn, J. S.

1998-01-01

The technology of the analysis of plutonium isotopic ratio is independent of the measurement geometry and applicable to samples of physical and chemical composition. Three standard plutonium samples were measured in the HPGe system. The results showed that CRM 136 and CRM 137 containing 238 Pu(0.223%) and 238 Pu(0.268%) were 18.4% and 14.2% error and CRM 138 of 238 Pu(0.01%) was 76% error. However the analysis represented less than 1.6% and 9% error in the three standard samples of highly involved 239 Pu and 240 Pu. Therefore, gamma-ray spectroscopy is very effective in the plutonium isotope analysis, having greater than 10% in content

Bismuth germanate's role in the new revolution in gamma-ray spectroscopy

International Nuclear Information System (INIS)

Johnson, N.R.; Baktash, C.; Lee, I.Y.

1983-01-01

Some of the considerations on how to effectively incorporate bismuth germanate into complex detection systems are covered, and some of these new systems now in operation or under construction are discussed. Significant achievements in gamma ray spectroscopy are reviewed as well as some recent results based on data taken with coincidence arrays of germanium detectors and Compton-suppression spectrometers. Then the first impact of bismuth germanate detectors on our understanding of the properties of nuclei that have high energy and very high angular momentum states are addressed

Positron Annihilation Ratio Spectroscopy (PsARS) Applied to Positronium Formation Studies

Science.gov (United States)

2010-03-01

Positron Annihilation Ratio Spectroscopy (PsARS). These experimental techniques have been used for a variety of military and civilian applications ... POSITRON ANNIHILATION RATIO SPECTROSCOPY (PsARS) APPLIED TO POSITRONIUM FORMATION STUDIES THESIS...of Defense, or the United States Government. AFIT/GNE/ENP/10-M07 POSITRON ANNIHILATION RATIO SPECTROSCOPY

A Modular Pipelined Processor for High Resolution Gamma-Ray Spectroscopy

Science.gov (United States)

Veiga, Alejandro; Grunfeld, Christian

2016-02-01

The design of a digital signal processor for gamma-ray applications is presented in which a single ADC input can simultaneously provide temporal and energy characterization of gamma radiation for a wide range of applications. Applying pipelining techniques, the processor is able to manage and synchronize very large volumes of streamed real-time data. Its modular user interface provides a flexible environment for experimental design. The processor can fit in a medium-sized FPGA device operating at ADC sampling frequency, providing an efficient solution for multi-channel applications. Two experiments are presented in order to characterize its temporal and energy resolution.

The Monte Carlo simulation of the neutron-induced prompt gamma ray spectroscopy of the CW abandoned by Japan

International Nuclear Information System (INIS)

Wang Bairong; Yang Zhongping; Zhan Wenzhong

2003-01-01

This paper introduced the principle of identifying the chemical weapon abandoned by Japan by neutron-induced prompt gamma ray. Using the MCNP-4C Monte Carlo program, this paper simulated and analyzed the neutron-induced prompt gamma ray spectroscopy of chemical weapon abandoned by Japan, whereby supply important datum and reference for the aftertime deeper research and disposal of Japan-abandoned chemical weapon. (authors)

Quantification of 235 U and 226 Ra in soil samples by means of Gamma spectroscopy

International Nuclear Information System (INIS)

Quintero P, E.; Rojas M, V.P.; Montes M, F.R.; Gaso P, M.I.; Cervantes N, M.L.

2000-01-01

In this work it is presented the Gamma Spectroscopy method which is realized in the Environmental Radiological Surveillance Laboratory using the option of deconvolution of a commercial software for the quantification of 235 U and 226 Ra; also is presented the method for the 226 Ra correction activity. (Author)

Design and fabrication of 4π Clover Detector Array Assembly for gamma-spectroscopy studies using thermal neutrons

International Nuclear Information System (INIS)

Kumar, Manish; Kamble, S.R.; Chaudhari, A.T.; Sabharwal, T.P.; Pathak, Kavindra; Prasad, N.K.; Kinage, L.A.; Biswas, D.C.; Bhagwat, P.V.

2017-01-01

Nuclear spectroscopy has been studied earlier from the measurement of prompt gamma rays produced in reactions with thermal neutrons from CIRUS reactor. For studying the prompt γ-spectroscopy using thermal neutrons from Dhruva Reactor, BARC, the development of a dedicated beam line (R-3001) is in progress. In this beam line a detector assembly consisting of Clover Ge detectors will be used. This experimental setup will be utilized to investigate nuclear structure using prompt (n,γ) reactions and also to study the spectroscopy of neutron-rich fission-fragment nuclei

Heavy ion deep inelastic collisions studied by discrete gamma ray spectroscopy

International Nuclear Information System (INIS)

Krolas, W.

1996-05-01

The discrete gamma ray spectroscopy has been used as a tool to investigate the heavy ion collision. It has been shown that such experimental information supplemented by results of additional of-line radioactivity measurements is complete enough to reconstruct distributions of products of very complex nuclear reactions. Three experiments have been performed in which the 208 Pb + 64 Ni, 130 Te + 64 Ni and 208 Pb + 58 Ni systems have been created. The production cross sections of fragment isotopes have been determined and compared with existing model predictions

CdZnTe detectors for gamma-ray Burst ArcSecond Imaging and Spectroscopy (BASIS)

International Nuclear Information System (INIS)

Stahle, C.M.; Palmer, D.; Bartlett, L.M.; Parsons, A.; Shi Zhiqing; Lisse, C.M.; Sappington, C.; Cao, N.; Shu, P.; Gehrels, N.; Teegarden, B.; Birsa, F.; Singh, S.; Odom, J.; Hanchak, C.; Tueller, J.; Barthelmy, S.; Krizmanic, J.; Barbier, L.

1996-01-01

A CdZnTe detector array is being developed for the proposed gamma-ray Burst ArcSecond Imaging and Spectroscopy (BASIS) spaceflight mission to accurately locate gamma-ray bursts, determine their distance scale, and measure the physical characteristics of the emission region. Two-dimensional strip detectors with 100 μm pitch have been fabricated and wire bonded to readout electronics to demonstrate the ability to localize 60 and 122 keV gamma-rays to less than 100 μm. Radiation damage studies on a CdZnTe detector exposed to MeV neutrons showed a small amount of activation but no detector performance degradation for fluences up to 10 10 neutrons/cm 2 . A 1 x 1 in. CdZnTe detector has also been flown on a balloon payload at 115 000 ft in order to measure the CdZnTe background rates. (orig.)

Proximal gamma-ray spectroscopy to predict soil properties using windows and full-spectrum analysis methods.

Science.gov (United States)

Mahmood, Hafiz Sultan; Hoogmoed, Willem B; van Henten, Eldert J

2013-11-27

Fine-scale spatial information on soil properties is needed to successfully implement precision agriculture. Proximal gamma-ray spectroscopy has recently emerged as a promising tool to collect fine-scale soil information. The objective of this study was to evaluate a proximal gamma-ray spectrometer to predict several soil properties using energy-windows and full-spectrum analysis methods in two differently managed sandy loam fields: conventional and organic. In the conventional field, both methods predicted clay, pH and total nitrogen with a good accuracy (R2 ≥ 0.56) in the top 0-15 cm soil depth, whereas in the organic field, only clay content was predicted with such accuracy. The highest prediction accuracy was found for total nitrogen (R2 = 0.75) in the conventional field in the energy-windows method. Predictions were better in the top 0-15 cm soil depths than in the 15-30 cm soil depths for individual and combined fields. This implies that gamma-ray spectroscopy can generally benefit soil characterisation for annual crops where the condition of the seedbed is important. Small differences in soil structure (conventional vs. organic) cannot be determined. As for the methodology, we conclude that the energy-windows method can establish relations between radionuclide data and soil properties as accurate as the full-spectrum analysis method.

Ultraviolet-visible and fluorescence spectroscopy can be used as a diagnostic tool for gamma irradiation detection in vivo.

Science.gov (United States)

K-Abdelhalim, Mohamed Anwar; Moussa, Sherif A-Abdelmottaleb

2016-09-01

The spectroscopic properties can indicate important features about the nature and severity of the disease. However, no earlier studies have been used the spectroscopic properties as a diagnostic tool for radiation detection. This study was aimed to use ultraviolet-visible and fluorescence spectroscopy as a diagnostic tool for gamma irradiation detection in rats in vivo. Adult male rats were exposed to 25, 50, 75 and 100 Gray as single dose, using Cobalt-60 (Co-60) source with a dose rate of 0.883 centi Gray/sec (cGy/s). Ultraviolet and fluorescence spectroscopy of rat's blood serum were measured. After gamma irradiation of rats in vivo, the blood serum absorbance peaks for 25, 50, 75 and 100 Gray (Gy) decreased and shifted towards the ultra violet wavelength. A maximal change in fluorescence intensity of blood serum at 350 nm was obtained when exciting light at 194 nm after irradiation. The fluorescence intensity also decreased with the dose. The highest radiation gamma dose might be accompanied with the highest oxidative stress. This study suggests that at the above mentioned gamma radiation doses, the blood is highly fragmented; with low aggregation at 25 Gy and with high aggregation at 50-100 Gy.

Development of a gamma ray spectroscopy capability at LANSCE

International Nuclear Information System (INIS)

Nelson, R.O.; Strottman, D.D.; Sterbenz, S.M.

1998-01-01

This is the final report of a one-year, Laboratory Directed Research and Development (LDRD) project at the Los Alamos National Laboratory (LANL). The goal of this project was to explore an upgrade to the GEANIE high-resolution gamma-ray spectrometer at the Los Alamos Neutron Science Center (LANSCE) to help build additional experimental capabilities. The improvements identified have significantly added to the capabilities of GEANIE and made the facility more attractive for studies supporting the core national security mission as well as for use by outside collaborators. These benefits apply to both basic and applied studies

Fourier transformation methods in the field of gamma spectrometry

Indian Academy of Sciences (India)

The basic principles of a new version of Fourier transformation is presented. This new version was applied to solve some main problems such as smoothing, and denoising in gamma spectroscopy. The mathematical procedures were first tested by simulated data and then by actual experimental data.

Effect of gamma-radiation on a water-insoluble arabinoxylan

International Nuclear Information System (INIS)

Ebringerová, A.; Pružinec, J.; Kačuráková, M.; Hromádková, Z.

1989-01-01

The effect of gamma radiation on a water-insoluble L-arabino-D-xylan has been studied by functional group and structural analysis using chemical methods and IR spectroscopy, by sugar composition analysis, and by viscosity measurements. The gamma irradiation has been shown to modify both sugar components of the arabinoxylan, accompanied by cleavage of the glycosidic linkages, depolymerization, and sugar decomposition, depending on the applied radiation dose, thus increasing the molecular and chemical heterogeneity of the polysaccharide. (author)

Spectroscopy

Energy Technology Data Exchange (ETDEWEB)

Hellman, Hal

1968-01-01

This booklet discusses spectroscopy, the study of absorption of radiation by matter, including X-ray, gamma-ray, microwave, mass spectroscopy, as well as others. Spectroscopy has produced more fundamental information to the study of the detailed structure of matter than any other tools.

Heavy ion deep inelastic collisions studied by discrete gamma ray spectroscopy

Energy Technology Data Exchange (ETDEWEB)

Krolas, W. [The H. Niewodniczanski Inst. of Nuclear Physics, Cracow (Poland)

1996-05-01

The discrete gamma ray spectroscopy has been used as a tool to investigate the heavy ion collision. It has been shown that such experimental information supplemented by results of additional of-line radioactivity measurements is complete enough to reconstruct distributions of products of very complex nuclear reactions. Three experiments have been performed in which the {sup 208}Pb + {sup 64}Ni, {sup 130}Te + {sup 64}Ni and {sup 208}Pb + {sup 58}Ni systems have been created. The production cross sections of fragment isotopes have been determined and compared with existing model predictions 64 refs, 59 figs, 19 tabs

Optimal digital filtering in gamma-ray spectroscopy

International Nuclear Information System (INIS)

Messai, A.; Nour, A.; Abdellani, I.

2009-01-01

In this paper, we address the subject of the digital nuclear spectroscopy as seen as a counterpart of the classic analogue approach. Consequently, we will present the design as well as the implementation on a DSP (Digital Signal Processor) board, of the various necessary digital pulse processing techniques via digital filtering in order to provide the principal tasks which often take place in a generic 'Gamma' digital spectroscopic setup. The first part will be devoted to the design of the digital IIR filter used for the charge preamplifier's slow-pole compensation. This will be followed by the practical estimation of the power spectral density relating to the electrical noise components present at the spectrometer's input. Thereafter, a very detailed attention will be given to the design of the digital optimal filter to be used for the charge measurements. We follow by another FIR filter that deals with the digital estimation of the reference line of measurements. Finally, we give a hardware implementation of the designed filters on the board: 'TMS320C6713-DSK', a DSP KIT developed by 'DIGITAL Spectrum'. (authors)

Quantification by Raman spectroscopy of the gamma radiation effects in water purification

International Nuclear Information System (INIS)

Perez C, V.M.; Santiago J, P.; Castano, V.M.

1999-01-01

The world problem about water pollution has been confronted by traditional methods such as: chlorination, filtration, etc. In this work is presented an alternative method, which consists in to radiate different concentrations of simulated polluted water (purified water + thinner) at different gamma radiation doses. The structural changes were analysed by Raman spectroscopy. Using a 52.5 Krad dose it was possible to eliminate all the thinner chemical linkages, which appear in the Raman spectra corresponding to the 87.5/12.5 water/thinner mixture. (Author)

NMR spectroscopy applied to the eye: Drugs and metabolic studies

Energy Technology Data Exchange (ETDEWEB)

Saether, Oddbjoern

2005-07-01

NMR spectroscopy has been extensively applied in biomedical research during the last decades. It has proved to be an analytical tool of great value. From being mainly used in chemistry, technological developments have expanded the application of NMR spectroscopy to a great wealth of disciplines. With this method, biochemical information can be obtained by analysing tissue extracts. Moreover, NMR spectroscopy is increasingly employed for pharmacokinetic studies and analysis of biofluids. Technological progress has provided increased sensitivity and resolution in the spectra, which enable even more of the complexity of biological samples to be elucidated. With the implementation of high-resolution magic angle spinning (HR-MAS) NMR spectroscopy in biomedicine, intact tissue samples or biopsies can be investigated. Thus, NMR spectroscopy has an ever-increasing impact in metabolic screening of human samples and in animal models, and methods are also increasingly realised in vivo. The present work, NMR spectroscopy applied to eye research, consists of two main parts. Firstly, the feasibility to monitor fluorinated ophthalmic drugs directly in the eye was assessed. Secondly, HR-MAS H1 NMR spectroscopy was applied for metabolic profiling of the anterior eye segment, specifically to analyse metabolic changes in intact corneal and lenticular samples after cataractogenic insults. This work included metabonomics with the application of pattern recognition methods to analyse HR-MAS spectra of eye tissues. Optimisation strategies were explored for F19 NMR detection of fluorinated drugs in a phantom eye. S/N gains in F19 NMR spectroscopy were achieved by implementing time-share H1 decoupling at 2.35 T. The method is advantageous for compounds displaying broad spectral coupling patterns, though detection of drugs at concentrations encountered in the anterior eye segment after topical application was not feasible. Higher magnetic fields and technological improvements could enable

NMR spectroscopy applied to the eye: Drugs and metabolic studies

International Nuclear Information System (INIS)

Saether, Oddbjoern

2005-01-01

NMR spectroscopy has been extensively applied in biomedical research during the last decades. It has proved to be an analytical tool of great value. From being mainly used in chemistry, technological developments have expanded the application of NMR spectroscopy to a great wealth of disciplines. With this method, biochemical information can be obtained by analysing tissue extracts. Moreover, NMR spectroscopy is increasingly employed for pharmacokinetic studies and analysis of biofluids. Technological progress has provided increased sensitivity and resolution in the spectra, which enable even more of the complexity of biological samples to be elucidated. With the implementation of high-resolution magic angle spinning (HR-MAS) NMR spectroscopy in biomedicine, intact tissue samples or biopsies can be investigated. Thus, NMR spectroscopy has an ever-increasing impact in metabolic screening of human samples and in animal models, and methods are also increasingly realised in vivo. The present work, NMR spectroscopy applied to eye research, consists of two main parts. Firstly, the feasibility to monitor fluorinated ophthalmic drugs directly in the eye was assessed. Secondly, HR-MAS H1 NMR spectroscopy was applied for metabolic profiling of the anterior eye segment, specifically to analyse metabolic changes in intact corneal and lenticular samples after cataractogenic insults. This work included metabonomics with the application of pattern recognition methods to analyse HR-MAS spectra of eye tissues. Optimisation strategies were explored for F19 NMR detection of fluorinated drugs in a phantom eye. S/N gains in F19 NMR spectroscopy were achieved by implementing time-share H1 decoupling at 2.35 T. The method is advantageous for compounds displaying broad spectral coupling patterns, though detection of drugs at concentrations encountered in the anterior eye segment after topical application was not feasible. Higher magnetic fields and technological improvements could enable

Modern utilization of accurate methods for gamma-ray spectral analysis detected by high pure germanium (HPGE) detectors through different applications

International Nuclear Information System (INIS)

El-Sayed, M.M.

2005-01-01

this thesis presents a novel way for application of wavelet trans-from theory in gamma -ray spectroscopy. this technique was applied for searching real and weak peaks, solving problem of multiplets, smoothing and de-noising gamma-ray spectra, and using artificial neural network for identifying peaks. a brief description about gamma-ray spectrum analysis is presented . we discussed the necessary formulas and algorithms of wavelet theory to solve these main problems in gamma ray spectrum analysis. the algorithm of peak search was applied on different types of spectra, IAEA spectra and other sources of gamma spectra. the algorithm of multiplets algorithm was applied successfully on different types of multiplets. the algorithm of denoising was applied successfully on different sources of spectra

Improvements in Applied Gamma-Ray Spectrometry with Germanium Semiconductor Detector

Energy Technology Data Exchange (ETDEWEB)

Brune, D; Hellstroem, S [AB Atomenergi, Nykoeping (Sweden); Dubois, J [Chalmers University of Technology, Goeteborg (Sweden)

1965-01-15

A germanium semi-conductor detector has in the present investigation been used in four cases of applied gamma-ray spectrometry. In one case the weak-activity contribution of Cs{sup 134} in Cs{sup 137} standard sources has been determined. The second case concerns the determination of K{sup 42} in samples of biological origin containing strong Na{sup 24} activities. In the third case the Nb{sup 94} and Nb{sup 95} activities from neutron-irradiated niobium foils used in the dosimetry of high neutron fluxes with long exposure times have been completely resolved and it has been possible to determine the ratio of the two activities with a high degree of accuracy. Finally, a Zr{sup 95} - Nb{sup 95} source has been analysed in a similar way with respect to its radiochemical composition. The resolution obtained also made possible a determination of the branching ratio of the two gamma-transitions in Zr{sup 95} and of the energies of the gamma-transitions of both nuclides.

V/V(max) test applied to SMM gamma-ray bursts

Science.gov (United States)

Matz, S. M.; Higdon, J. C.; Share, G. H.; Messina, D. C.; Iadicicco, A.

1992-01-01

We have applied the V/V(max) test to candidate gamma-ray bursts detected by the Gamma-Ray Spectrometer (GRS) aboard the SMM satellite to examine quantitatively the uniformity of the burst source population. For a sample of 132 candidate bursts identified in the GRS data by an automated search using a single uniform trigger criterion we find average V/V(max) = 0.40 +/- 0.025. This value is significantly different from 0.5, the average for a uniform distribution in space of the parent population of burst sources; however, the shape of the observed distribution of V/V(max) is unusual and our result conflicts with previous measurements. For these reasons we can currently draw no firm conclusion about the distribution of burst sources.

Dosimetry for terrestrial gamma-ray sources

International Nuclear Information System (INIS)

Abdullah, S.A.; Dickson, H.W.; Kerr, G.D.; Miah, M.F.K.; Perdue, P.T.

1975-01-01

Dose rates from natural radionuclides and 137 Cs in soils of the Oak Ridge area have been determined from in situ and core sample measurements. Information on soil composition, density, and moisture content and on the distribution of cesium in the soil was obtained from the core samples. Measurements of radionuclide concentrations in the samples were made with a 4 x 4 in. NaI detector. Gamma-ray spectroscopy using a lithium-drifted germanium (GeLi) detector has been applied to the determination of radionuclide concentrations in soil and the associated gamma dose rates above the earth plane. An unshielded GeLi detector placed about 1 m above the earth detects gamma radiation from an area of about 100 m 2 . The equipment and data processing procedure are briefly described

FY12 Final Report for PL10-Mod Separations-PD12: Electrochemically Modulated Separation of Plutonium from Dilute and Concentrated Dissolver Solutions for Analysis by Gamma Spectroscopy

Energy Technology Data Exchange (ETDEWEB)

Pratt, Sandra H.; Arrigo, Leah M.; Duckworth, Douglas C.; Cloutier, Janet M.; Breshears, Andrew T.; Schwantes, Jon M.

2013-05-01

Accurate and timely analysis of plutonium in spent nuclear fuel is critical in nuclear safeguards for detection of both protracted and rapid plutonium diversions. Gamma spectroscopy is a viable method for accurate and timely measurements of plutonium provided that the plutonium is well separated from the interfering fission and activation products present in spent nuclear fuel. Electrochemically modulated separation (EMS) is a method that has been used successfully to isolate picogram amounts of Pu from nitric acid matrices. With EMS, Pu adsorption may be turned “on” and “off” depending on the applied voltage, allowing for collection and stripping of Pu without the addition of chemical reagents. In this work, we have scaled up the EMS process to isolate microgram quantities of Pu from matrices encountered in spent nuclear fuel during reprocessing. Several challenges have been addressed including surface area limitations, radiolysis effects, electrochemical cell performance stability, and chemical interferences. After these challenges were resolved, 6 µg Pu was deposited in the electrochemical cell with approximately an 800-fold reduction of fission and activation product levels from a spent nuclear fuel sample. Modeling showed that these levels of Pu collection and interference reduction may not be sufficient for Pu detection by gamma spectroscopy. The main remaining challenges are to achieve a more complete Pu isolation and to deposit larger quantities of Pu for successful gamma analysis of Pu. If gamma analyses of Pu are successful, EMS will allow for accurate and timely on-site analysis for enhanced Pu safeguards.

Implementation of neutron-induced gamma-ray spectroscopy in industrial applications

International Nuclear Information System (INIS)

Abernethy, D. A.; Lim, C. S.

2006-01-01

Full text: Neutron based analytical techniques are commonly used in a wide variety of industrial applications, with new applications continually being found. As a result, despite popular concerns about the harmful health effects of radiation the number of these analysers is increasing. This is because neutron-induced gamma-ray techniques have the capability of combining elemental sensitivity with significant penetrating power, enabling non-intrusive and non-destructive bulk elemental measurements to be averaged over a large volume of material. Neutron induced gamma ray spectroscopy has been developed by several groups, including CSIRO Minerals, for on-line measurement of elemental composition in a range of industrial applications in vessels, pipes and on conveyor belts. Compared to those typically found in a scientific laboratory, conditions in industrial plants differ substantially in a number of ways, such as environmental variability, operator skill and training, and shielding requirements. As a result of these differences, equipment and techniques which are used as a matter of course in a laboratory often have to undergo major modification to render them suitable for use in an industrial context. This paper will discuss some of the factors that have to be considered when deciding such matters with particular emphasis on the implications of radiation safety requirements

Positron Annihilation Ratio Spectroscopy Study of Electric Fields Applied to Positronium at Material Interfaces

Science.gov (United States)

2011-03-01

from 142 ns to a few ns [3:3]. Through the application of positron annihilation lifetime spectroscopy (PALS) on a material, the o-Ps lifetime can be...Force Base, Ohio APPROVED FOR PUBLIC RELEASE; DISTRIBUTION UNLIMITED. POSITRON ANNIHILATION RATIO SPECTROSCOPY STUDY OF ELECTRIC FIELDS APPLIED TO...protection in the United States. AFIT/GNE/ENP/11-M19 POSITRON ANNIHILATION RATIO SPECTROSCOPY STUDY OF ELECTRIC FIELDS APPLIED TO POSITRONIUM AT

Advances in Molecular Rotational Spectroscopy for Applied Science

Science.gov (United States)

Harris, Brent; Fields, Shelby S.; Pulliam, Robin; Muckle, Matt; Neill, Justin L.

2017-06-01

Advances in chemical sensitivity and robust, solid-state designs for microwave/millimeter-wave instrumentation compel the expansion of molecular rotational spectroscopy as research tool into applied science. It is familiar to consider molecular rotational spectroscopy for air analysis. Those techniques for molecular rotational spectroscopy are included in our presentation of a more broad application space for materials analysis using Fourier Transform Molecular Rotational Resonance (FT-MRR) spectrometers. There are potentially transformative advantages for direct gas analysis of complex mixtures, determination of unknown evolved gases with parts per trillion detection limits in solid materials, and unambiguous chiral determination. The introduction of FT-MRR as an alternative detection principle for analytical chemistry has created a ripe research space for the development of new analytical methods and sampling equipment to fully enable FT-MRR. We present the current state of purpose-built FT-MRR instrumentation and the latest application measurements that make use of new sampling methods.

Particle-Induced Gamma-ray Emission Spectroscopy Over a Broad Range of Elements

Science.gov (United States)

Olds, Hannah; Wilkinson, John; Tighe, Meghanne; McLallen, Walter; McGuire, Patrick

2017-09-01

Ion beam analysis is a common application of nuclear physics that allows elemental and isotopic information about materials to be determined from accelerated light ion beams One of the best know ion beam analysis techniques is Particle-Induced Gamma-ray Emission (PIGE) spectroscopy, which can be used ex vacuo to identify the elements of interest in almost any solid target. The energies of the gamma-rays emitted by excited nuclei will be unique to each element and depend on its nuclear structure. For the most sensitivity, the accelerated ions should exceed the Coulomb barrier of the target, but many isotopes are known to be accessible to PIGE even below the Coulomb barrier. To explore the sensitivity of PIGE across the periodic table, PIGE measurements were made on elements with Z = 5, 9, 11-15, 17, 19-35, 37, 42, 44-48, 53, 56, 60, 62, 73, and 74 using 3.4 MeV protons. These measurements will be compared with literature values and be used as a basis for comparison with higher-energy proton beams available at the University of Notre Dame's St. Andre accelerator when it comes online this Fall. The beam normalization technique of using atmospheric argon and its 1459 keV gamma-ray to better estimate the integrated beam on target will also be discussed. Funded by the NSF REU program and the University of Notre Dame.

Gamma-ray spectroscopy of 120-130Te nuclei

International Nuclear Information System (INIS)

Vanhoy, J.R.; Champine, B.R.; Coleman, R.T.; Crandell, K.A.; Tanyi, J.A.; Hicks, S.F.; Alexander, G.K.; Burkett, P.G.; Burns, M.C.; Collard, C.J.

2000-01-01

Complete text of publication follows. Structure of the even 120-130 Te nuclei have been investigated with prompt gamma-ray spectroscopy following the 122-126,nat Te(n,n'γ) reactions and the (α,2nγ) 120,124,126 Te reactions. Gamma-ray excitation functions, angular distributions, γγ-coincidences, and Doppler shifts have been measured. Level schemes have been constructed to approximately 3.3 MeV excitation energy, and spectroscopic information including level spins and parities, branching and multipole-mixing ratios, and lifetimes have been extracted. Three different types of structure are thought to play an important role in these low-lying excitations. These are: collective, two-particle, and 4p-2h intruder excitations. Because there are seven stable even-even Te nuclei, the evolution of these excitation modes over this wide range in neutron number is investigated. Level sequences and transition rates obtained from these measurements are compared to IBM-2 model calculations both with and without intruder-state mixing by Rikovska et al. (1), and to particle-vibrational coupling model calculations by Lopac (2). The IBM-2 model calculations with intruder mixing well reproduce the level energies in the low-mass Te; however, examination of the electromagnetic transition rates reveals that there is no clear improvement in the description of these nuclei by adding the intruder configurations. Additionally, no evidence of the 2 + mixed-symmetry strength is observed in the 2 3 + and 2 4 + levels in these nuclei. The particle-vibration model calculations appear to do a good job describing both the level scheme and the transition rates in the heavier nuclei investigated. (author)

Gamma-induced positron annihilation spectroscopy and application to radiation-damaged alloys

International Nuclear Information System (INIS)

Wells, D.P.; Hunt, A.W.; Tchelidze, L.; Kumar, J.; Smith, K.; Thompson, S.; Selim, F.; Williams, J.; Harmon, J.F.; Maloy, S.; Roy, A.

2006-01-01

Radiation damage and other defect studies of materials are limited to thin samples because of inherent limitations of well-established techniques such as diffraction methods and traditional positron annihilation spectroscopy (PAS) [P. Hautojarvi, et al., Positrons in Solids, Springer, Berlin, 1979, K.G. Lynn, et al., Appl. Phys. Lett. 47 (1985) 239]. This limitation has greatly hampered industrial and in-situ applications. ISU has developed new methods that use pair-production to produce positrons throughout the volume of thick samples [F.A. Selim, D.P. Wells, et al., Nucl. Instr. and Meth. B 192 (2002) 197, F.A. Selim, D.P. Wells, et al., Nucl. Instru. Meth. A 495 (2002) 154, F.A. Selim, et al., J. Rad. Phys. Chem. 68 (2004) 427, F.A. Selim, D.P. Wells, et al., Nucl. Instr. and Meth. B 241 (2005) 253, A.W. Hunt, D.P. Wells, et al., Nucl. Instr. and Meth. B. 241 (2005) 262]. Unlike prior work at other laboratories that use bremsstrahlung beams to create positron beams (via pair-production) that are then directed at a sample of interest, we produce electron-positron pairs directly in samples of interest, and eliminate the intermediate step of a positron beam and its attendant penetrability limitations. Our methods include accelerator-based bremsstrahlung-induced pair-production in the sample for positron annihilation energy spectroscopy measurements (PAES), coincident proton-capture gamma-rays (where one of the gammas is used for pair-production in the sample) for positron annihilation lifetime spectroscopy (PALS), or photo-nuclear activation of samples for either type of measurement. The positrons subsequently annihilate with sample electrons, emitting coincident 511 keV gamma-rays [F.A. Selim, D.P. Wells, et al., Nucl. Instr. and Meth. B 192 (2002) 197, F.A. Selim, D.P. Wells, et al., Nucl. Instru. Meth. A 495 (2002) 154, F.A. Selim, et al., J. Rad. Phys. Chem. 68 (2004) 427, F.A. Selim, D.P. Wells, et al., Nucl. Instr. and Meth. B 241 (2005) 253, A.W. Hunt, D

Feasibility Study on Fiber-optic Radiation Sensor for Remote Gamma-ray Spectroscopy

International Nuclear Information System (INIS)

Jeon, Hyesu; Jang, Kyoung Won; Shin, Sang Hun and others

2014-01-01

In this study, we fabricated a fiber-optic radiation sensor using an optical fiber and various scintillators. To select an adequate inorganic scintillator for the sensing probe of fiber-optic radiation sensor, 5 types of scintillators were evaluated. The spectra of gamma-rays emitted from a Na-22 radiation source were measured by using the manufactured sensors. As a result, the BGO was suitable for the sensing probe of fiber-optic radiation sensor due to its high scintillation output and exact photoelectric peak for the gamma-ray energy. The basic principle of radiation detection is to detect the signals caused by interactions between radiations and materials. There are various types of radiation detectors depending on types of radiation to be detected and physical quantities to be measured. As one of the radiation detectors, a fiber-optic radiation sensor using a scintillator and an optical fiber has two advantages such as no space restraint and remote sensing. Moreover, in nuclear environments, this kind of sensor has immunities for electromagnetic field, temperature, and pressure. Thus, the fiber-optic radiation sensor can be used in various fields including nondestructive inspection, radioactive waste management, nuclear safety, radiodiagnosis and radiation therapy. As a fundamental study of the fiber-optic radiation sensor for remote gamma-ray spectroscopy, in this study, we fabricated a fiber-optic radiation sensor using an optical fiber and various scintillators. To select an adequate inorganic scintillator for the sensing probe of fiber-optic radiation sensor, 5 types of scintillators were evaluated. The spectra of gamma-rays emitted from a Na-22 radiation source were measured by using the manufactured sensors

The recent developments in the technology of scintillator detectors for gamma-ray spectroscopy

International Nuclear Information System (INIS)

Verdebout, J.

1988-01-01

The goal of this report is to review the recent developments in the use of high stopping power materials and solid state readout for scintillation gamma -ray spectroscopy as these techniques may give rise to a new generation of low powered portable instruments. The report is a bibliographical study based on papers published mainly these last five years. The main subject is preceded by a general introduction in which the principal characteristics of a scintillator gamma-ray spectrometer are discussed. The properties of some scintillator materials (NaI(T1), CsI(T1), CsI(Na), BGO, GSO(Ce) and CdWO 4 ) are then briefly presented. In this section, a special emphasis has been given to BGO as this material has recently received much attention and is now well documented. Finally, the results obtained by measuring the intensity of the light generated in the crystal with three types of solid-state photodetectors (Si photodiodes, HgI 2 photodetectors and avalanche Si photodiodes) are summarized

Development of a Reference Database for Particle Induced Gamma Ray Emission (PIGE) Spectroscopy

International Nuclear Information System (INIS)

2017-09-01

Ion beam analysis techniques are non-destructive analytical techniques used to identify the composition and structure of surface layers of materials. The applications of these techniques span environmental control, cultural heritage and conservation, materials and fusion technologies. The particle-induced gamma-ray emission (PIGE) spectroscopy technique in particular, is a powerful tool for detecting light elements in certain depths of surface layers. This publication describes the coordinated effort to measure and compile cross section data relevant to PIGE analysis and make these data available to the community of practice through a comprehensive online database.

modern utilization of accurate methods for gamma-ray spectral analysis detected by high pure germanium (HPGE) detectors through different applications

International Nuclear Information System (INIS)

El-Sayed, M.M.

2006-01-01

this thesis presents a novel way for application of wavelet transform theory in gamma-ray spectroscopy . this technique was applied for searching real and weak peaks, solving problem of multiplets, smoothing and de-noising gamma-ray spectra, and using artificial neural network for identifying peaks. a brief description about gamma-ray spectrum analysis is presented. we discussed the necessary formulas and algorithms of wavelet theory to solve these main problems in gamma -ray spectrum analysis. the algorithm of peak search was applied on different types of spectra, IAEA spectra and other sources of gamma spectra. the algorithm of multiplets algorithm was applied successfully on different types of multiplets. the algorithm of de noising was applied successfully on different sources of spectra.finally, a database for neutron activation laboratory is created. this data base consists of five routines, wavelet gamma spectrum analysis, peak identification, elemental concentration , neutron flux determination,and detector efficiency calculation

Gamma-ray spectroscopy of the neutron-rich Ni region through heavy-ion deep-inelastic collisions

International Nuclear Information System (INIS)

Ishii, T.; Asai, M.; Matsuda, M.; Ichikawa, S.; Makishima, A.; Hossain, I.; Kleinheinz, P.; Ogawa, M.

2002-01-01

Nuclei in the neutron-rich Ni region have been studied by γ-ray spectroscopy. Gamma-rays emitted from isomers, with T 1/2 >1 ns, produced in heavy-ion deep-inelastic collisions were measured with an isomer-scope. The nuclear structure of the doubly magic 68 Ni and its neighbor 69,71 Cu is discussed on the basis of the shell model. Future experiments for more neutron-rich Ni nuclei are also viewed. (orig.)

Gamma-ray spectroscopy of the neutron-rich Ni region through heavy-ion deep-inelastic collisions

Science.gov (United States)

Ishii, T.; Asai, M.; Makishima, A.; Hossain, I.; Kleinheinz, P.; Ogawa, M.; Matsuda, M.; Ichikawa, S.

Nuclei in the neutron-rich Ni region have been studied by γ-ray spectroscopy. Gamma-rays emitted from isomers, with T1/2 > 1 ns, produced in heavy-ion deep-inelastic collisions were measured with an isomer-scope. The nuclear structure of the doubly magic 68Ni and its neighbor 69,71Cu is discussed on the basis of the shell model. Future experiments for more neutron-rich Ni nuclei are also viewed.

Determination of natural radioactive elements in building materials by gamma spectroscopy, trace dosimetry and neutron activation analysis

International Nuclear Information System (INIS)

Perez, G.; Desdin, L.F.; Hernandez, A.T.; Gonzalez, D.; Labrada, A.; Tenreiro, J.J.; Capote, G.; Perelyguin, V.P.; Herrera, H.; Tellez, E.

1993-01-01

Five types of Cuban concretes and their main components (minerals aggregates and cement) were investigated in order to analyze the content of uranium, thorium, radium, potassium and radon 220,222, using gamma spectroscopy, trace dosimetry and neutron activation analysis. The comparative evaluation of different concretes, aggregates and two types of cements according to natural radioactivity is shown

Validating the Melusine Gamma Spectroscopy Tool

Energy Technology Data Exchange (ETDEWEB)

Erikson, Luke E.; Keillor, Martin E.; Stavenger, Timothy J.

2013-11-26

This technical report describes testing to evaluate the gamma spectroscopy tool, Melusine, under development by Pacific Northwest National Laboratory. The goal was to verify that the software can successfully be used to provide accurate results and statistical uncertainties for the detection of isotopes of interest and their activities. Of special interest were spectra similar to those produced by radionuclide stations that contribute to the Comprehensive Nuclear Test Ban Treaty Organization’s International Monitoring System. Two data sets were used to test Melusine’s capabilities. The first was the result of a multi-lab calibration effort based on neutron activations produced at the University of California at Davis. The second was taken from the Proficiency Test Exercises conducted by the CTBTO directly in 2005. In 37 of 42 cases, Melusine produced results in agreement with the best answer presently available, in most cases with calculated uncertainties comparable to or better than competing analyses. In fact, Melusine technically provided one more result than CTBTO’s PTE analyses that agreed with the “book answer” (Monte Carlo simulation). Despite these promising results, the Melusine software is still under development. Effort is especially needed to simplify its analysis process, improve stability, and provide user documentation. Some significant analysis tasks require further vetting, such as those to address summing effects. However, our test results indicate that Melusine’s calculations as presently implemented are sound and can be used to reliably analyze spectra from the CTBTO’s radionuclide stations.

Potential radionuclide emissions from stacks on the Hanford site, Part 2: Dose assessment methodology using portable low-resolution gamma spectroscopy

Energy Technology Data Exchange (ETDEWEB)

Barnett, J.M. [Westinghouse Hanford Company, Richland, WA (United States)

1995-02-01

In September 1992, the Westinghouse Hanford Company began developing an in situ measurement method to assess gamma radiation emanating from high-efficiency particulate air filters using portable low-resolution gamma spectroscopy. The purpose of the new method was to assess radioactive exhaust stack air emissions from empirical data rather than from theoretical models and to determine the potential unabated dose to an offsite theoretical maximally exposed individual. In accordance with Title 40, Code of Federal Regulations, Part 61, Subpart H, {open_quotes}National Emission Standards for Hazardous Air Pollutants{close_quotes}, stacks that have the potential to emit {ge} 1 {mu}Sv y{sup {minus}1} (0.1 mrem y{sup {minus}1}) to the maximally exposed individual are considered {open_quotes}major{close_quotes} and must meet the continuous monitoring requirements. After the method was tested and verified, the U.S. Environmental Protection Agency, Region 10, approved its use in June 1993. Of the 125 stacks operated by the Westinghouse Hanford Company, 22 were targeted for evaluation by this method, and 15 were assessed. (The method could not be applied at seven stacks because of excessive background radiation or because no gamma emitting particles appear in the emission stream.) The most significant result from this study was the redesignation of the T Plant main stack. The stack was assessed as being {open_quotes}minor{close_quotes}, and it now only requires periodic confirmatory measurements and meets federally imposed sampling requirements.

33th all-union conference on nuclear spectroscopy and atomic nucleus structure

International Nuclear Information System (INIS)

Adam, J.; Bem, P.

1984-01-01

The 33rd All-Union Conference on Nuclear Spectroscopy and the Atomic Nucleus Structure was held in Moscow from April 19 to 22. The plenary session heard 5 papers which summed up the results of extensive programmes of theoretical and experimental research. More than two thirds of the conference were held in parallel sessions: Properties of Concrete Nuclei, Nuclear Reactions (theory, experiment), Theory of the Nucleus, Mechanisms of Alpha-, Beta- and Gamma Processes, Nuclear Spectroscopy Techniques and Applied Nuclear Spectroscopy. (B.S.)

Quasi-optimum gamma and X spectroscopy based on real-time digital techniques

CERN Document Server

Pullia, Antonio; Ripamonti, G

2000-01-01

An adaptive, self-calibrated instrument for gamma- and X-ray digital spectroscopy is proposed and demonstrated. Most of the typical processing features (pole-zero cancellation, baseline restoration, and shaping) are digitally implemented and optimized. Initialization is performed through a software procedure, which makes the system particularly flexible and allows periodical adaptivity. It is shown that spectroscopy performances are achieved even while using low-cost, low-frequency (5 Ms/s), and relatively low-resolution (12-bit) AD converters. The ADC differential nonlinearity (DNL), for example, is improved of two orders of magnitude, as estimated over the Compton shoulder of a sup 6 sup 0 Co spectrum, owing to an equivalent built-in sliding-scale effect. Using the system with an high-purity germanium (HPGe) detector a resolution of 1.9 keV FWHM (1.6 per mille) is obtained on the 1.17 MeV spectral line of a sup 6 sup 0 Co source. An Integral Nonlinearity (INL) of 0.3 per mille is measured in the range from ...

Multiple Gamma-Ray Detection Capability of a CeBr3 Detector for Gamma Spectroscopy

Directory of Open Access Journals (Sweden)

A. A. Naqvi

2017-01-01

Full Text Available The newly developed cerium tribromide (CeBr3 detector has reduced intrinsic gamma-ray activity with gamma energy restricted to 1400–2200 keV energy range. This narrower region of background gamma rays allows the CeBr3 detector to detect more than one gamma ray to analyze the gamma-ray spectrum. Use of multiple gamma-ray intensities in elemental analysis instead of a single one improves the accuracy of the estimated results. Multigamma-ray detection capability of a cylindrical 75 mm × 75 mm (diameter × height CeBr3 detector has been tested by analyzing the chlorine concentration in water samples using eight chlorine prompt gamma rays over 517 to 8578 keV energies utilizing a D-D portable neutron generator-based PGNAA setup and measuring the corresponding minimum detection limit (MDC of chlorine. The measured MDC of chlorine for gamma rays with 517–8578 keV energies varies from 0.07 ± 0.02 wt% to 0.80 ± 0.24. The best value of MDC was measured to be 0.07 ± 0.02 wt% for 788 keV gamma rays. The experimental results are in good agreement with Monte Carlo calculations. The study has shown excellent detection capabilities of the CeBr3 detector for eight prompt gamma rays over 517–8578 keV energy range without significant background interference.

Terahertz spectroscopy applied to food model systems

DEFF Research Database (Denmark)

Møller, Uffe

Water plays a crucial role in the quality of food. Apart from the natural water content of a food product, the state of that water is very important. Water can be found integrated into the biological material or it can be added during production of the product. Currently it is difficult...... to differentiate between these types of water in subsequent quality controls. This thesis describes terahertz time-domain spectroscopy applied on aqueous food model systems, with particular focus on ethanol-water mixtures and confined water pools in inverse micelles....

Recoil Distance Method lifetime measurements via gamma-ray and charged-particle spectroscopy at NSCL

Science.gov (United States)

Voss, Philip Jonathan

The Recoil Distance Method (RDM) is a well-established technique for measuring lifetimes of electromagnetic transitions. Transition matrix elements derived from the lifetimes provide valuable insight into nuclear structure. Recent RDM investigations at NSCL present a powerful new model-independent tool for the spectroscopy of nuclei with extreme proton-to-neutron ratios that exhibit surprising behavior. Neutron-rich 18C is one such example, where a small B(E2; 2+1 → 0+gs) represented a dramatic shift from the expected inverse relationship between the B(E2) and 2+1 excitation energy. To shed light on the nature of this quadrupole excitation, the RDM lifetime technique was applied with the Koln/NSCL plunger. States in 18C were populated by the one-proton knockout reaction of a 19N secondary beam. De-excitation gamma rays were detected with the Segmented Germanium Array in coincidence with reaction residues at the focal plane of the S800 Magnetic Spectrometer. The deduced B(E2) and excitation energy were both well described by ab initio no-core shell model calculations. In addition, a novel extension of RDM lifetime measurements via charged-particle spectroscopy of exotic proton emitters has been investigated. Substituting the reaction residue degrader of the Koln/NSCL plunger with a thin silicon detector permits the study of short-lived nuclei beyond the proton dripline. A proof of concept measurement of the mean lifetime of the two-proton emitter 19Mg was conducted. The results indicated a sub-picosecond lifetime, one order of magnitude smaller than the published results, and validate this new technique for lifetime measurements of charged-particle emitters.

Feasibility study of performing high precision gamma spectroscopy of {lambda}{lambda} hypernuclei in the anti PANDA experiment

Energy Technology Data Exchange (ETDEWEB)

Sanchez-Lorente, Alicia

2010-09-30

Hypernuclear research will be one of the main topics addressed by the anti PANDA experiment at the planned Facility for Antiproton and Ion Research anti FAIR. Thanks to the use of stored anti p beams, copious production of double {lambda} hypernuclei is expected at the anti PANDA experiment, which will enable high precision {gamma} spectroscopy of such nuclei for the first time. At anti PANDA excited states of {xi}{sup -} hypernuclei will be used as a basis for the formation of double {lambda} hypernuclei. For their detection, a devoted hypernuclear detector setup is planned. This setup consists of a primary nuclear target for the production of {xi}{sup -}+ anti {xi} pairs, a secondary active target for the hypernuclei formation and the identification of associated decay products and a germanium array detector to perform {gamma} spectroscopy. In the present work, the feasibility of performing high precision {gamma} spectroscopy of double {lambda} hypernuclei at the anti PANDA experiment has been studied by means of a Monte Carlo simulation. For this issue, the designing and simulation of the devoted detector setup as well as of the mechanism to produce double {lambda} hypernuclei have been optimized together with the performance of the whole system. In addition, the production yields of double hypernuclei in excitedparticle stable states have been evaluated within a statistical decay model. A strategy for the unique assignment of various newly observed {gamma}-transitions to specific double hypernuclei has been successfully implemented by combining the predicted energy spectra of each target with the measurement of two pion momenta from the subsequent weak decays of a double hypernucleus. Indeed, based on these Monte Carlo simulation, the analysis of the statistical decay of {sup 13}{sub {lambda}}{sub {lambda}}B has been performed. As result, three {gamma}-transitions associated to the double hypernuclei {sup 11}{sub {lambda}}{sub {lambda}}Be and to the single

Raman spectroscopy of 2-hydroxyethyl methacrylate-acrylamide copolymer using gamma irradiation for crosslinking

International Nuclear Information System (INIS)

Goheen, Steven C.; Saunders, Rachel M.; Davis, Rachel M.; Harvey, Scott D.; Olsen, Peter C.

2006-01-01

A copolymer hydrogel was made by mixing acrylamide and 2-hydroxyethyl methacrylate monomers in water and polymerizing with gamma irradiation. The progress of polymerization and the vibrational structure of the hydrogel was examined using Raman spectroscopy. Raman spectra indicated that the co-polymer has a molecular structure different from polyacrylamide or the individual monomers. The Raman data also indicate the presence of crosslinking at the C=O, NH2 and OH side chains. The spectra further suggest the continuous lengthening of the backbone of the polymers with increasing gamma dose. This is shown as the increase in C-C modes as C=C vibrations decrease. Raman spectra changed most dramatically as the monomer mixture became a gel at a dose of approximately 320 Gy. Spectral differences were subtler with doses exceeding 640 Gy, although chain lengthening continued beyond 1500 Gy. Potential applications of the copolymer hydrogel include reconstructive tissue as well as a standard material for radiation protection dosimetry. Results are discussed in relation to other potential applications of this polymer and dose-dependent changes in the Raman spectrum

High-resolution gamma spectroscopy with whole-body and partial-body counters. Experience, recommendations. Report

International Nuclear Information System (INIS)

Sahre, P.

1997-12-01

The application of high-resolution gamma spectroscopy with whole-body and partial-body counters shows a steadily rising upward trend over the last few years. This induced the ''Arbeitskreis Inkorporationsueberwachung'' of the association ''Fachverband fuer Strahlenschutz e.V.'' to organise a meeting for joint elaboration of a guide on recommended applications of this measuring technique, based on a review of existing experience and results. A key item on the agenda of the meeting was the comparative evaluation of the Ge semiconductor detector and the NaI solid scintillation detector. (orig./CB) [de

Gamma-Ray Spectroscopy at TRIUMF-ISAC: the New Frontier of Radioactive Ion Beam Research

Science.gov (United States)

Ball, G. C.; Andreoiu, C.; Austin, R. A. E.; Bandyopadhyay, D.; Becker, J. A.; Bricault, P.; Brown, N.; Chan, S.; Churchman, R.; Colosimo, S.; Coombes, H.; Cross, D.; Demand, G.; Drake, T. E.; Dombsky, M.; Ettenauer, S.; Finlay, P.; Furse, D.; Garnsworthy, A.; Garrett, P. E.; Green, K. L.; Grinyer, G. F.; Hyland, B.; Hackman, G.; Kanungo, R.; Kulp, W. D.; Lassen, J.; Leach, K. G.; Leslie, J. R.; Mattoon, C.; Melconian, D.; Morton, A. C.; Pearson, C. J.; Phillips, A. A.; Rand, E.; Sarazin, F.; Svensson, C. E.; Sumithrarachchi, S.; Schumaker, M. A.; Triambak, S.; Waddington, J. C.; Walker, P. M.; Williams, S. J.; Wood, J. L.; Wong, J.; Zganjar, E. F.

2009-03-01

High-resolution gamma-ray spectroscopy is essential to fully exploit the unique scientific opportunities at the next generation radioactive ion beam facilities such as the TRIUMF Isotope Separator and Accelerator (ISAC). At ISAC the 8π spectrometer and its associated auxiliary detectors is optimize for β-decay studies while TIGRESS an array of segmented clover HPGe detectors has been designed for studies with accelerated beams. This paper gives a brief overview of these facilities and also presents recent examples of the diverse experimental program carried out at the 8π spectrometer.

Equipment and applications for gamma spectrometry

International Nuclear Information System (INIS)

Hemingway, J.D.

1986-01-01

In this article the theoretical aspects of gamma spectroscopy are discussed. Coaxial germanium detectors and planar detectors are described. Applications of gamma spectroscopy to the detection of the exposure of a population to naturally occuring radioactive gases and their daughter products; the accumulation of iodine isotopes in the thyroid and measuring the quantity of 239 Pu in the lungs are discussed. (UK)

ESR identification of gamma-irradiated albendazole

Science.gov (United States)

Çolak, Seyda

2010-01-01

The use of ionizing radiation for sterilization of pharmaceuticals is a well-established technology. In the present work, the spectroscopic and kinetic features of the radicals induced in gamma-irradiated solid albendazole samples is investigated at different temperatures in the dose range of 3-34 kGy by electron spin resonance (ESR) spectroscopy. Irradiation with gamma radiation produced two different radical species in albendazole. They were fairly stable at room temperature but relatively unstable above room temperature, giving rise to an unresolved ESR spectrum consisting of three resonance peaks centered at g=2.0057. Decay activation energies of the contributing radical species were calculated to be 47.8 (±13.5) and 50.5 (±9.7) kJ/mol using the signal intensity decay data derived from annealing studies performed at high temperatures. A linear function of the applied dose was found to best describe the experimental dose-response data. Albendazole does not present the characteristics of good dosimetric materials. However, the discrimination of irradiated albendazole from its unirradiated form was possible even 6 months after storage in normal conditions. Based on these findings, it is concluded that albendazole and albendazole-containing drugs can be safely sterilized by gamma radiation and that ESR spectroscopy could be successfully used as a potential technique for monitoring their radiosterilization.

A deep-level transient spectroscopy study of gamma-ray irradiation on the passivation properties of silicon nitride layer on silicon

Science.gov (United States)

Dong, Peng; Yu, Xuegong; Ma, Yao; Xie, Meng; Li, Yun; Huang, Chunlai; Li, Mo; Dai, Gang; Zhang, Jian

2017-08-01

Plasma-enhanced chemical vapor deposited silicon nitride (SiNx) films are extensively used as passivation material in the solar cell industry. Such SiNx passivation layers are the most sensitive part to gamma-ray irradiation in solar cells. In this work, deep-level transient spectroscopy has been applied to analyse the influence of gamma-ray irradiation on the passivation properties of SiNx layer on silicon. It is shown that the effective carrier lifetime decreases with the irradiation dose. At the same time, the interface state density is significantly increased after irradiation, and its energy distribution is broadened and shifts deeper with respect to the conduction band edge, which makes the interface states becoming more efficient recombination centers for carriers. Besides, C-V characteristics show a progressive negative shift with increasing dose, indicating the generation of effective positive charges in SiNx films. Such positive charges are beneficial for shielding holes from the n-type silicon substrates, i. e. the field-effect passivation. However, based on the reduced carrier lifetime after irradiation, it can be inferred that the irradiation induced interface defects play a dominant role over the trapped positive charges, and therefore lead to the degradation of passivation properties of SiNx on silicon.

Detection of gamma-irradiated peanuts by ESR spectroscopy and GC analysis of hydrocarbons

Energy Technology Data Exchange (ETDEWEB)

Wei Mingli; An Li [Institute of Agro-food Science and Technology, Chinese Academy of Agricultural Sciences, 100193 Beijing (China); Yi Mingha, E-mail: wangyilwm@163.co [Institute of Agro-food Science and Technology, Chinese Academy of Agricultural Sciences, 100193 Beijing (China); Feng Wang [Institute of Agro-food Science and Technology, Chinese Academy of Agricultural Sciences, 100193 Beijing (China); Yan Lizhang [Division of Metrology in Ionizing Radiation and Medicine, National Institute of Metrology, 100013 Beijing (China)

2011-03-15

Peanuts were analyzed by electron spin resonance (ESR) spectroscopy and gas chromatography (GC) before and after gamma irradiation. Using European protocols, the validity and effectiveness of these two techniques were compared with regard to sample preparation, sample and solvent consumption and dose-response curves after irradiation. The results showed the possibility of using ESR and GC for distinguishing between irradiated and unirradiated peanuts. A radiation dose of 0.1 kGy could be detected by ESR but not by GC. The results also indicated that GC is an effective method for qualitative analysis of irradiated peanut, while ESR is suitable for the rapid detection of irradiated peanuts.

Strong equivalence, Lorentz and CPT violation, anti-hydrogen spectroscopy and gamma-ray burst polarimetry

International Nuclear Information System (INIS)

Shore, Graham M.

2005-01-01

The strong equivalence principle, local Lorentz invariance and CPT symmetry are fundamental ingredients of the quantum field theories used to describe elementary particle physics. Nevertheless, each may be violated by simple modifications to the dynamics while apparently preserving the essential fundamental structure of quantum field theory itself. In this paper, we analyse the construction of strong equivalence, Lorentz and CPT violating Lagrangians for QED and review and propose some experimental tests in the fields of astrophysical polarimetry and precision atomic spectroscopy. In particular, modifications of the Maxwell action predict a birefringent rotation of the direction of linearly polarised radiation from synchrotron emission which may be studied using radio galaxies or, potentially, gamma-ray bursts. In the Dirac sector, changes in atomic energy levels are predicted which may be probed in precision spectroscopy of hydrogen and anti-hydrogen atoms, notably in the Doppler-free, two-photon 1s-2s and 2s-nd (n∼10) transitions

Analysis of coupled neutron-gamma radiations, applied to shieldings in multigroup albedo method

International Nuclear Information System (INIS)

Dunley, Leonardo Souza

2002-01-01

The principal mathematical tools frequently available for calculations in Nuclear Engineering, including coupled neutron-gamma radiations shielding problems, involve the full Transport Theory or the Monte Carlo techniques. The Multigroup Albedo Method applied to shieldings is characterized by following the radiations through distinct layers of materials, allowing the determination of the neutron and gamma fractions reflected from, transmitted through and absorbed in the irradiated media when a neutronic stream hits the first layer of material, independently of flux calculations. Then, the method is a complementary tool of great didactic value due to its clarity and simplicity in solving neutron and/or gamma shielding problems. The outstanding results achieved in previous works motivated the elaboration and the development of this study that is presented in this dissertation. The radiation balance resulting from the incidence of a neutronic stream into a shielding composed by 'm' non-multiplying slab layers for neutrons was determined by the Albedo method, considering 'n' energy groups for neutrons and 'g' energy groups for gammas. It was taken into account there is no upscattering of neutrons and gammas. However, it was considered that neutrons from any energy groups are able to produce gammas of all energy groups. The ANISN code, for an angular quadrature order S 2 , was used as a standard for comparison of the results obtained by the Albedo method. So, it was necessary to choose an identical system configuration, both for ANISN and Albedo methods. This configuration was six neutron energy groups and eight gamma energy groups, using three slab layers (iron aluminum - manganese). The excellent results expressed in comparative tables show great agreement between the values determined by the deterministic code adopted as standard and, the values determined by the computational program created using the Albedo method and the algorithm developed for coupled neutron-gamma

Measurement of (n,xn) reaction cross-sections using prompt {gamma} spectroscopy at neutron beams with high instantaneous flux; Mesure de sections efficaces de reaction (n,xn) par spectroscopie {gamma} prompte aupres d'un faisceau a tres haut flux instantane

Energy Technology Data Exchange (ETDEWEB)

Lukic, S

2004-10-15

The work presented in this thesis is situated in the context of the GEDEON program of neutron cross-section measurements. This program is motivated by the perspectives recently opened by projects of nuclear waste treatment and energy production. There is an obvious lack of experimental data on (n,xn) reactions in the databases, especially in the case of very radioactive isotopes. An important technique to measure cross-sections of these reactions is the prompt {gamma}-ray spectroscopy at white pulsed neutron beams with very high instantaneous flux. In this work, inelastic scattering and (n,xn) reactions cross-section measurements were performed on a lead sample from threshold to 20 MeV by prompt {gamma}-ray spectroscopy at the white neutron beam generated by GELINA facility in Geel, Belgium. Digital methods were developed to treat HPGe CLOVER detector signals and separate {gamma}-rays induced by the fastest neutrons from those belonging to the flash. Partial cross-sections for the production of several transitions in natural lead were measured and analyzed using theoretical calculations in order to separate the contributions of different reactions leading to the same residual isotope. Total cross-sections of the reactions in question were estimated. The results were compared to the TALYSS code theoretical calculations, as well as to other experimental results. This experiment has served to validate the method and it opens the way to measure (n,xn) reactions cross-sections with high instantaneous neutron flux on actinides, particularly the U{sup 233}(n,2n) reaction which is important for the thorium cycle. (author)

Experimental study of the burned of nuclear fuel by the gamma spectroscopy method

International Nuclear Information System (INIS)

Amador V, P.

2009-01-01

Accurate information on nuclear fuel burnup is of vital importance in reactor operation, fuel management and fuel-characteristics studies. Conventionally fuel management of the TRIGA III Reactor from the National Institute of Nuclear Research (ININ) is done through the thermal balance method (management) of the power generated during reactor operation, since it is known that with 1.24 grams of 235 U is possible to generate a power or 1 MW per day during the reactor operation. On the other hand, it is possible to calculate the operation time in days during a power of 1 MW with the help of the data registered in logs. With the information just mentioned one can calculate the quantity of 235 U consumed in the fuel during a complete period of irradiation. In order to compare and prove that the burnup values, calculated through the thermal balance method, are correct, the ININ implemented, for the first time, the gamma-ray spectroscopy method as an experimental technique to calculate the burnup of several fuel elements. Gamma-ray spectroscopy is a nondestructive method, so that the integrity of the fuel element is not affected which is of great importance. Since there is a direct relation between the activity of 137 Cs contained in the fuel elements and a series of constants which are unique for the radioisotope and for the high resolution system, the problem just simplifies in measuring the 137 Cs activities. Furthermore the 137 Cs concentration equation was developed theoretically and I wrote a computer program (AMAVAL) in Fortran. The task of this program is to calculate the concentrations and the activity through the use of the equation just mentioned and the history of each fuel element. The purpose of this is to compare and validate the experimental activities with the theoretical ones for each fuel element. (Author)

Gamma irradiation effect on the chemical composition and the antioxidant activity of Ipomoea batatas L

Energy Technology Data Exchange (ETDEWEB)

Tahir, D., E-mail: dtahir@fmipa.unhas.ac.id; Halide, H., E-mail: dtahir@fmipa.unhas.ac.id; Kurniawan, D. [Department of Physics, Hasanuddin University, Makassar 90245 (Indonesia); Wahab, A. W. [Department of Chemistry, Hasanuddin University, Makassar 90245 (Indonesia)

2014-09-25

The chemical composition and antioxidant activity of Ipomoea batatas L. (sweet potato) were studied by x-ray fluorescence (XRF) spectroscopy, Fourier transform infrared spectroscopy, and by the 1,1-diphenyl-2-picrylhydrazyl (DPPH) radical scavenging capacity. The irradiation treatment was performed by using Cs-137 as a gamma sources in experimental equipment. Treatment by irradiation emerges as a possible conservation technique that has been tested successfully in several food products. The amount of chemical composition was changed and resulting new chemical for absorbed dose 40 mSv. Interestingly, it was found that gamma irradiation significantly increased the antioxidant activity, as measured by DPPH radical scavenging capacity. The antioxidant activity of Ipomoea batatas L. extract was dramatically increased in the non-irradiated sample to the sample irradiated at 40 mSv. These results indicate that gamma irradiation of Ipomoea batatas L. extract can enhance its antioxidant activity through the formation of a new chemical compound. Based on these results, increased antioxidant activity of Ipomoea batatas L. extracts by gamma rays can be applied to various industries, especially cosmetics, foodstuffs, and pharmaceuticals.

Neutron counting and gamma spectroscopy with PVT detectors

International Nuclear Information System (INIS)

Mitchell, Dean James; Brusseau, Charles A.

2011-01-01

Radiation portals normally incorporate a dedicated neutron counter and a gamma-ray detector with at least some spectroscopic capability. This paper describes the design and presents characterization data for a detection system called PVT-NG, which uses large polyvinyl toluene (PVT) detectors to monitor both types of radiation. The detector material is surrounded by polyvinyl chloride (PVC), which emits high-energy gamma rays following neutron capture reactions. Assessments based on high-energy gamma rays are well suited for the detection of neutron sources, particularly in border security applications, because few isotopes in the normal stream of commerce have significant gamma ray yields above 3 MeV. Therefore, an increased count rate for high-energy gamma rays is a strong indicator for the presence of a neutron source. The sensitivity of the PVT-NG sensor to bare 252 Cf is 1.9 counts per second per nanogram (cps/ng) and the sensitivity for 252 Cf surrounded by 2.5 cm of polyethylene is 2.3 cps/ng. The PVT-NG sensor is a proof-of-principal sensor that was not fully optimized. The neutron detector sensitivity could be improved, for instance, by using additional moderator. The PVT-NG detectors and associated electronics are designed to provide improved resolution, gain stability, and performance at high-count rates relative to PVT detectors in typical radiation portals. As well as addressing the needs for neutron detection, these characteristics are also desirable for analysis of the gamma-ray spectra. Accurate isotope identification results were obtained despite the common impression that the absence of photopeaks makes data collected by PVT detectors unsuitable for spectroscopic analysis. The PVT detectors in the PVT-NG unit are used for both gamma-ray and neutron detection, so the sensitive volume exceeds the volume of the detection elements in portals that use dedicated components to detect each type of radiation.

VAT-69, a software system for gamma spectroscopy

International Nuclear Information System (INIS)

Furr, A.K.; Roscoe, B.A.; Parkinson, T.F.

1979-01-01

The software system was originally developed solely for neutron activation analysis. Its usefulness has been enhanced by adding modules that allow processing of gamma spectra from natural radioisotopes and from fission products. It allows: (1) separation of overlapping peaks, allowing retrieval of a peak of interest in the presence of an interfering peak, (2) calibration of each gamma spectrum for energy and peak width, using criteria based on gamma peak data internal to the individual spectrum, (3) correction for errors due to rapidly changing dead times during the counting interval, permitting accurate count data for samples containing mixed short-, medium-, and long-lived isotopes. One disadvantage of the original software was that it produced more output information than desired. The modifications that have been implemented to produce final concentration values include: (1) computation of a weighted-average concentration of the ith element where two or more gamma peaks are available, (2) rejection of gamma peaks when the difference in energies of the located peak and library peak exceeds a preset value, (3) rejection of concentration values based on gamma peaks which do not satisfy preselected criteria for irradiation time and wait time, (4) computation of the error in concentration of the ith element, and (5) correction of sample concentration for trace elements in the irradiation vials. Overall performance of the software system is checked periodically by analyzing standards. Several thousand spectra are processed each year with VAT-69, with typically 25 to 40 elements quantitatively determined

Experience gained in gamma spectroscopy; Experience acquise dans la spectrometrie gamma

Energy Technology Data Exchange (ETDEWEB)

Jeanmaire, L [Commissariat a l' Energie Atomique, Saclay (France).Centre d' Etudes Nucleaires

1960-07-01

There are two types of method which make it possible to estimate the internal contamination of individuals. On the one hand these are the indirect techniques based on measurements of the excreted products, on the other there are the direct techniques in which attempts are made to measure directly the radio-activity existing in the organism. We propose to give a few of the results obtained by the direct method using equipment built by the Commissariat a l'Energie Atomique. The apparatus consists of a {gamma} spectrometer. It includes: 1) A crystal of sodium iodide 20 cm in diameter and 10 cm high. The large size of this crystal ensures a good sensitivity and makes it possible to carry out rapid measurements. 2) A 25 channel type SAE 25 selector which classifies the pulses according to their amplitude. It is therefore possible to distinguish between {gamma} rays of varying energy. 3) A comparatively very light radiation protection, consisting of only 5 cm thickness of lead which diminishes the ambient {gamma} ray intensity to a sufficient level for the majority of the measurements. A certain collimation is thus obtained which makes it possible to localise the source approximately and to reduce the undesirable effects of external contamination. (author) [French] Deux types de methodes permettent d'apprecier la contamination interne d'un individu. D'une part, les techniques indirectes basees sur la mesure des produits excretes, d'autre part, les techniques directes au moyen desquelles on essaie de mesurer directement la radioactivite existant dans l'organisme. Nous nous proposons d'indiquer quelques resultats obtenus par la methode directe, au moyen d'ensembles realises par le Commissariat a l'Energie Atomique. L'appareillage est un spectrometre {gamma}. II comprend: 1) Un cristal d'iodure de sodium de 20 cm de diametre et 10 cm de hauteur. La grande taille de ce cristal assure une bonne sensibilite et permet d'effectuer des mesures rapides. 2) Un selecteur a 25 canaux

Crystal growth and thermoluminescence response of NaZr2(PO4)3 at high gamma radiation doses

International Nuclear Information System (INIS)

Ordóñez-Regil, E.; Contreras-Ramírez, A.; Fernández-Valverde, S.M.; González-Martínez, P.R.; Carrasco-Ábrego, H.

2013-01-01

Graphical abstract: -- Highlights: •NaZr 2 (PO 4 ) 3 exposed to gamma doses of 10, 30 and 50 MGy. •Gamma radiation produced growth of the crystal size of the NZP. •Morphology changes were reversible by heating. •Linear relationship between the thermoluminescence and the applied gamma dose. •This property could be useful for high-level gamma dosimetry. -- Abstract: This work describes the synthesis and characterization of NaZr 2 (PO 4 ) 3 . The stability of this material under high doses of gamma radiation was investigated in the range of 10–50 MGy. Samples of unaltered and gamma irradiated NaZr 2 (PO 4 ) 3 were characterized by X-ray diffraction, infrared spectroscopy, scanning electron microscopy, energy dispersive X-ray spectroscopy, and thermoluminescence. The results showed that while functional groups were not affected by the gamma irradiation, morphology changes were observed with increasing doses of gamma irradiation. The morphology of the non-irradiated compound is agglomerated flakes; however, irradiation at 10 MGy splits the flakes inducing the formation of well-defined cubes. Gamma irradiation induced the crystal size of the NaZr 2 (PO 4 ) 3 to grow. The heat treatment (973 K) of samples irradiated at 50 MGy resulted in the recovery of the original morphology. Furthermore, the thermoluminescence analysis of the irradiated compound is reported

Comparison of the effect of plasma treatment and gamma ray irradiation on PS-Cu nanocomposite films surface

Science.gov (United States)

Farag, O. F.

2018-06-01

Polystyrene-copper (PS-Cu) nanocomposite films were treated with DC N2 plasma and gamma rays irradiations. The plasma treatment of PS-Cu film surface was carried out at different treatment times, gas pressure 0.4 Torr and the applied power 3.5 W. On the other hand, the treatment with gamma rays irradiation were carried out at irradiation doses 10, 30 and 50 kGy. The induced changes in surface properties of PS-Cu films were investigated with UV-viss spectroscopy, scanning electron microscopy (SEM) and FTIR spectroscopy techniques. In addition, the wettability property, surface free energy, spreading coefficient and surface roughness of the treated samples were studied by measuring the contact angle. The UV-viss spectroscopy analysis revealed that the optical band gap decreases with increasing the treatment time and the irradiation dose for plasma and gamma treatments, respectively. SEM observations showed that the particle size of copper particles was increased with increasing the treatment time and the irradiation dose, but gamma treatment changes the copper particles size from nano scale to micro scale. The contact angle measurements showing that the wettability property, surface free energy, spreading coefficient and surface roughness of the treated PS-Cu samples were increased remarkably with increasing the treatment time and the irradiation dose for plasma and gamma treatments, respectively. The contact angle, surface free energy, spreading coefficient and surface roughness of the treated PS-Cu samples are more influenced by plasma treatment than gamma treatment.

Assessment of pollutants in manzala lake using gamma-ray spectroscopy

International Nuclear Information System (INIS)

Abdel-Haleem, A.S.; Zaghloul, R.; El-Abbady, W.H.; Hassan, A.M.

1996-01-01

Multielemental analysis of water samples taken from the area of manzala lake in the east-north of river Nile delta of egypt, has been performed. Prompt gamma neutron activation analysis (PGNAA) technique is applied to determine the elemental concentrations. The samples have been irradiated by means of (PGNAA) facility using a Cf 252 isotopic neutron source with a total flux of 1.5 x 10 5 n cm 2 s -1 for 300 min irradiation time. The evaluation of Cd, Gd, Sm, Pb, Zn, Co and Hg as trace elements in these samples is reported. 1 fig., 2 tabs

Testing FLUKA on neutron activation of Si and Ge at nuclear research reactor using gamma spectroscopy

Science.gov (United States)

Bazo, J.; Rojas, J. M.; Best, S.; Bruna, R.; Endress, E.; Mendoza, P.; Poma, V.; Gago, A. M.

2018-03-01

Samples of two characteristic semiconductor sensor materials, silicon and germanium, have been irradiated with neutrons produced at the RP-10 Nuclear Research Reactor at 4.5 MW. Their radionuclides photon spectra have been measured with high resolution gamma spectroscopy, quantifying four radioisotopes (28Al, 29Al for Si and 75Ge and 77Ge for Ge). We have compared the radionuclides production and their emission spectrum data with Monte Carlo simulation results from FLUKA. Thus we have tested FLUKA's low energy neutron library (ENDF/B-VIIR) and decay photon scoring with respect to the activation of these semiconductors. We conclude that FLUKA is capable of predicting relative photon peak amplitudes, with gamma intensities greater than 1%, of produced radionuclides with an average uncertainty of 13%. This work allows us to estimate the corresponding systematic error on neutron activation simulation studies of these sensor materials.

Modeling a gamma spectroscopy system and predicting spectra with Geant-4

International Nuclear Information System (INIS)

Sahin, D.; Uenlue, K.

2009-01-01

An activity predictor software was previously developed to foresee activities, exposure rates and gamma spectra of activated samples for Radiation Science and Engineering Center (RSEC), Penn State Breazeale Reactor (PSBR), Neutron Activation Analysis (NAA) measurements. With Activity Predictor it has been demonstrated that the predicted spectra were less than satisfactory. In order to obtain better predicted spectra, a new detailed model for the RSEC NAA spectroscopy system with High Purity Germanium (HPGe) detector is developed using Geant-4. The model was validated with a National Bureau of Standards certified 60 Co source and tree activated high purity samples at PSBR. The predicted spectra agreed well with measured spectra. Error in net photo peak area values were 8.6-33.6%. Along with the previously developed activity predictor software, this new model in Geant-4 provided realistic spectra prediction for NAA experiments at RSEC PSBR. (author)

Gamma-Ray Interactions for Reachback Analysts

Energy Technology Data Exchange (ETDEWEB)

Karpius, Peter Joseph [Los Alamos National Lab. (LANL), Los Alamos, NM (United States); Myers, Steven Charles [Los Alamos National Lab. (LANL), Los Alamos, NM (United States)

2016-08-02

This presentation is a part of the DHS LSS spectroscopy training course and presents an overview of the following concepts: identification and measurement of gamma rays; use of gamma counts and energies in research. Understanding the basic physics of how gamma rays interact with matter can clarify how certain features in a spectrum were produced.

Design of a software for gamma detector efficiency

International Nuclear Information System (INIS)

Lopez, G.

2011-01-01

Gamma spectroscopy with highly-pure-germanium detector is one of the most used method for qualitative and quantitative analysis of samples. Nevertheless Gamma spectroscopy results require to be corrected, first for taking into account the self-shielding effect that represents the absorption of the photons by the sample itself and secondly for correcting the fact that 2 photons emitted simultaneously with energy E 1 and E 2 are likely to be simultaneously detected and then counted as a single photon with an energy E 1 +E 2 . This effect is called gamma-gamma coincidence. A software has been designed to simulate both effect and produce correcting factors in the case of cylindrical geometries. This software has been validated on Americium 241 for the self-shielding effect and on Cesium 134 for gamma-gamma coincidence. (A.C.)

Technical Aspect for Operating Portable Prompt Gamma Neutron Activation Analysis (PGNAA) on Terengganu Inscribed Stone

International Nuclear Information System (INIS)

Rasif Mohd Zain; Hearie Hassan; Roslan Yahya

2015-01-01

Prompt Gamma Neutron Activation analysis (PGNAA) is a type of neutron activation analysis which can determined element with nearly no gamma ray decay after being irradiated by neutron sourced. Thus, element that cannot be determined by the conventional NAA for example H, B, N, Si and Cd, can be determine by PGNAA. This paper focuses on the technical working procedure for operating portable PGNAA in field work. The device is designed as a portable non-destructive investigation tool applying an isotopic neutron source (Cf-252) and a gamma-ray spectroscopy system for in-situ investigation. The studied have been carried out on Terengganu inscribed stone at Terengganu State Museum. (author)

Criteria for assembly of in vivo measuring systems using high-resolution {gamma}-spectroscopy for evaluation of incorporated radionuclides; Kriterien zum Aufbau von In Vivo Messsystemen zur hochaufloesenden {gamma}-Spektrometrie inkorporierter Radionuklide

Energy Technology Data Exchange (ETDEWEB)

Wahl, W. [GSF Forschungszentrum fuer Umwelt und Gesundheit, Neuherberg (Germany). Inst. fuer Strahlenschutz

1997-12-01

The paper reviews the available, fundamental measuring methods relying on {gamma}-spectroscopy for their possible application in whole-body and partial-body counters for detection of manifold incorporation of radionuclides. Particular emphasis is placed on the response functions of various detectors, the assembly, the differentiated radioactivity distribution in the body, the various components of background activity and the corresponding suppression mechanisms, and possible ways of using the energy dependence for optimised detection of specific {gamma} energies in a given body region. Criteria and relations as well as their advantages and drawbacks are discussed. (orig./CB) [Deutsch] Diese Arbeit prueft die zur Verfuegung stehenden grundlegenden, {gamma}-spektroskopischen Messmethoden auf deren moegliche Anwendung im Spektrum der Ganz- und Teilkoerperzaehler zum Nachweis der mannigfach inkorporierten Radionuklide. Insbesondere wird eingegangen auf die Response Funktionen verschiedener Detektoren, die Anordnung, die differenzierte Aktivitaetsverteilung im Koerper, die verschiedenen Untergrundkomponenten und deren Unterdrueckungsmechanismen sowie die Beeinflussung durch die Energieabhaengigkeit zum optimalen Nachweis spezifischer {gamma}-Energien an einem bestimmten Ort am Koerper. Kriterien und Relationen sowie deren Vor- und Nachteile werden diskutiert. (orig.)

Exploring atmospheric radon with airborne gamma-ray spectroscopy

Science.gov (United States)

Baldoncini, Marica; Albéri, Matteo; Bottardi, Carlo; Minty, Brian; Raptis, Kassandra G. C.; Strati, Virginia; Mantovani, Fabio

2017-12-01

222Rn is a noble radioactive gas produced along the 238U decay chain, which is present in the majority of soils and rocks. As 222Rn is the most relevant source of natural background radiation, understanding its distribution in the environment is of great concern for investigating the health impacts of low-level radioactivity and for supporting regulation of human exposure to ionizing radiation in modern society. At the same time, 222Rn is a widespread atmospheric tracer whose spatial distribution is generally used as a proxy for climate and pollution studies. Airborne gamma-ray spectroscopy (AGRS) always treated 222Rn as a source of background since it affects the indirect estimate of equivalent 238U concentration. In this work the AGRS method is used for the first time for quantifying the presence of 222Rn in the atmosphere and assessing its vertical profile. High statistics radiometric data acquired during an offshore survey are fitted as a superposition of a constant component due to the experimental setup background radioactivity plus a height dependent contribution due to cosmic radiation and atmospheric 222Rn. The refined statistical analysis provides not only a conclusive evidence of AGRS 222Rn detection but also a (0.96 ± 0.07) Bq/m3 222Rn concentration and a (1318 ± 22) m atmospheric layer depth fully compatible with literature data.

A triple-crystal phoswich detector with digital pulse shape discrimination for alpha/beta/gamma spectroscopy

International Nuclear Information System (INIS)

White, Travis L.; Miller, William H.

1999-01-01

Researchers at the University of Missouri - Columbia have developed a three-crystal phoswich detector coupled to a digital pulse shape discrimination system for use in alpha/beta/gamma spectroscopy. Phoswich detectors use a sandwich of scintillators viewed by a single photomultiplier tube to simultaneously detect multiple types of radiation. Separation of radiation types is based upon pulse shape difference among the phosphors, which has historically been performed with analog circuitry. The system uses a GaGe CompuScope 1012, 12 bit, 10 MHz computer-based oscilloscope that digitally captures the pulses from a phoswich detector and subsequently performs pulse shape discrimination with cross-correlation analysis. The detector, based partially on previous phoswich designs by Usuda et al., uses a 10 mg/cm 2 thick layer of ZnS(Ag) for alpha detection, followed by a 0.254 cm CaF 2 (Eu) crystal for beta detection, all backed by a 2.54 cm NaI(Tl) crystal for gamma detection. Individual energy spectra and count rate information for all three radiation types are displayed and updated periodically. The system shows excellent charged particle discrimination with an accuracy of greater than 99%. Future development will include a large area beta probe with gamma-ray discrimination, systems for low-energy photon detection (e.g. Bremsstrahlung or keV-range photon emissions), and other health physics instrumentation

High-precision gamma-ray spectroscopy for enhancing production and application of medical isotopes

Science.gov (United States)

McCutchan, E. A.; Sonzogni, A. A.; Smith, S. V.; Muench, L.; Nino, M.; Greene, J. P.; Carpenter, M. P.; Zhu, S.; Chillery, T.; Chowdhury, P.; Harding, R.; Lister, C. J.

2015-10-01

Nuclear medicine is a field which requires precise decay data for use in planning radionuclide production and in imaging and therapeutic applications. To address deficiencies in decay data, sources of medical isotopes were produced and purified at the Brookhaven Linear Isotope Producer (BLIP) then shipped to Argonne National Laboratory where high-precision, gamma-ray measurements were performed using Gammasphere. New decay schemes for a number of PET isotopes and the impact on dose calculations will be presented. To investigate the production of next-generation theranostic or radiotherapeutic isotopes, cross section measurements with high energy protons have also been explored at BLIP. The 100-200 MeV proton energy regime is relatively unexplored for isotope production, thus offering high discovery potential but at the same time a challenging analysis due to the large number of open channels at these energies. Results of cross sections deduced from Compton-suppressed, coincidence gamma-ray spectroscopy performed at Lowell will be presented, focusing on the production of platinum isotopes by irradiating natural platinum foils with 100 to 200 MeV protons. DOE Isotope Program is acknowledged for funding ST5001030. Work supported by the US DOE under Grant DE-FG02-94ER40848 and Contracts DE-AC02-98CH10946 and DE-AC02-06CH11357.

Laser spectroscopy used in nuclear physics; La spectroscopie laser appliquee a la physique nucleaire

Energy Technology Data Exchange (ETDEWEB)

Le Blanc, F

2001-04-05

The study of nuclear shapes is a basic topic since it constitutes an excellent ground for testing and validating nuclear models. Measurements of the electron quadrupolar moment, of the nuclear charge radius and of the magnetic dipolar moment shed light on the nuclear deformation. Laser spectroscopy is a specific tool for such measurements, it is based on the interaction of the nucleus with the surrounding electron cloud (hyperfine structure), it is then an external approach of the shape of the nucleus whereas the classical nuclear spectroscopy ({alpha}, {beta} or {gamma}) gives information on the deformation from the inside of the nucleus. The author describes 2 techniques of laser spectroscopy: the colinear spectroscopy directly applied to a beam issued from an isotope separator and the resonant ionization spectroscopy linked with atom desorption that allows the study of particular nuclei. In order to illustrate both methods some effective measurements are presented: - the colinear spectroscopy has allowed the achievement of the complete description of the isomeric state (T = 31 years) of hafnium-178; - The experiment Complis has revealed an unexpected even-odd zigzag effect on very neutron-deficient platinum isotopes; and - the comparison of 2 isotopes of gold and platinum with their isomers has shown that the inversion of 2 levels of neutron, that was found out by nuclear spectroscopy, is in fact a consequence of a change in the nuclear shape. (A.C.)

Toxicological studies on the Use of acid applied or combined with gamma radiation for controlling the mediterranean fruit fly Ceratitis Capitata Wied

International Nuclear Information System (INIS)

Fadel, A.M.; Othman, K.S.A.

1997-01-01

Biological studies were conducted to determine the effect of boric acid applied alone to different stages of ceratitis capitata or combined with gamma radiation of the produced treated pupae (9 days old). At a concentration range of 200-2000 ppm of boric acid per gm larval diet, larval and pupal durations were insignificantly affected. Pupation significantly decreased with increasing concentration, and adult emergence significantly increased at higher concentrations. Lc50 value of boric acid applied to the larval diet was 250 ppm. Applying boric acid as a powder mixed with pupal medium, the Lc50 was 96 mg/gm sand. Male and emergence significantly decreased. Significant mortality was obtained in adults of C capitata after applying boric acid as a thin film on the inner surface of the experimental cages where the adults were kept or when mixed with their food or as powder on the cage bottom. Applying boric acid to larval diet and gamma radiation to the produced pupae (9 days old) insignificantly affected larval and durations, percent pupation, adult emergence or adult survival. In cross-mating experiments, egg hatch ability was significantly reduced in the combination treatments of boric acid (500, 1000 ppm) and gamma radiation (90 Gy). On the other hand gamma radiation combined with boric acid treatments significantly increased male mating competitiveness at the concentration of 1000 ppm of boric acid followed by gamma irradiation (90 Gy). 2 figs., 5 tabs

Enrichment Meter Dataset from High-Resolution Gamma Spectroscopy Measurements of U3O8 Enrichment Standards and UF6 Cylinder Wall Equivalents

Energy Technology Data Exchange (ETDEWEB)

Nicholson, Andrew D. [Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States); Croft, Stephen [Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States); Shephard, Adam M. [Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)

2015-12-01

The Enrichment Meter Principle (EMP) is the basis for a commonly used standard test method for the non-destructive assay of ²³⁵U enrichment in bulk compounds [1]. The technique involves determining the net count rate in the direct 186 keV peak using medium or high energy gamma-ray spectrometry in a fixed geometry. With suitable correction for wall attenuation, compound type, rate loss (live time), and peaked background (if significant), the atom fraction of ²³⁵U may be obtained from the counting rate from a linear relationship through the origin. The widespread use of this method for field verification of enrichment [2,3] together with the fact that the response function rests on fundamental physics considerations (i.e., is not represented by a convenient but arbitrary form) makes it an interesting example of uncertainty quantification, one in which one can expect a valid measurement model can be applied. When applied using NaI(Tl) and region of interest analysis, the technique is susceptible to both interference error and bias [2-4]. When implemented using high-resolution gamma-ray spectroscopy, the spectrum interpretation is considerable simplified and more robust [5]. However, a practical challenge to studying the uncertainty budget of the EMP method (for example, to test linearity, extract wall corrections and so forth using modern methods) is the availability of quality experimental data that can be referenced and shared. To fill this gap, the research team undertook an experimental campaign [6]. A measurement campaign was conducted to produce high-resolution gamma spectroscopy enrichment meter data comparable to UF₆ cylinder measurements. The purpose of this report is to provide both an introduction to and quality assurance (QA) of the raw data produced. This report is intended for the analyst or researcher who uses the raw data. Unfortunately, the raw data (i.e., the spectra files) are too voluminous to include in this report

A digital multi-channel spectroscopy system with 100 MHz flash ADC module for the GENIUS-TF and GENIUS projects

International Nuclear Information System (INIS)

Kihm, T.; Bobrakov, V.F.; Klapdor-Kleingrothaus, H.V.

2003-01-01

In this paper we present the first results of applying a digital processing technology in low-level gamma spectroscopy with HPGE detectors. An experimental gamma spectrometer using Flash ADC module is built and tested. The test system is now under development and shows major advantages over the traditional analog technologies. It will be installed for the GENIUS-TF and GENIUS projects in Gran-Sasso in early 2003

Gamma spectrometry today

International Nuclear Information System (INIS)

Hemingway, J.

1990-01-01

This paper reviews the important advances in gamma spectroscopy made in recent years. Improvements in detectors and other components and the addition of on-line computer control systems is discussed. (UK)

Possibility of applying the gamma-gamma method to the in situ determination of uranium-ore densities

International Nuclear Information System (INIS)

Czubek, J.; Guitton, J.

1965-01-01

The principles of the gamma-gamma method are reviewed. It is shown in particular that, under certain conditions, the method makes it possible to obtain a representative measurement of the electronic density. Chemical analyses have been carried out on samples obtained from uranium deposits. The results show that an exact correlation exists between the massive and electronic densities. It is possible to consider the possibility of measuring the density of uranium-containing rocks by the gamma-gamma method. (authors) [fr

Application of gamma-ray spectroscopy to the differentiation between mobile and deposited fission products in pipes

International Nuclear Information System (INIS)

Packer, T.W.; Armitage, B.H.

1990-08-01

A method has been developed to differentiate between material flowing in pipes and deposited on the pipe walls. This has been applied to a study of fission product release from irradiated fuel under severe accident conditions. A collimation arrangement has been examined which provides good discrimination between gamma- radiation arising from flowing gases/aerosols and from stationary deposits. A systematic examination has been made of gamma- radiation obtained from gases and deposits in pipes of different diameter for a number of collimator configurations. A system of calibration has been developed based on Monte-Carlo modelling which has been found to be in broad agreement with measured values. This knowledge has been applied to the data obtained in a real-time measurement undertaken on the FALCON reactor safety facility at AEA Technology, Winfrith

Gamma ray spectroscopy of soil samples from apple orchards in Lamingo dam and Vom area in Jos, Plateau State, Nigeria

International Nuclear Information System (INIS)

Mangset, W. E.; Wilson, M. S.

2011-01-01

Five samples each were collected from the apple orchards in Lamingo dam and Vom area of Jos East and Jos South local government areas respectively. The samples were allowed to decay for three weeks to ensure efficiency in acquiring the radionuclides. The samples were analyzed using Gamma Ray spectroscopy. Barium- 204 with gamma activity energy level 1765.50keV was used to check the presence of Uranium-235 in the samples. The results showed that samples Lams 2,3,4 and Voms 1,4,5 had high gamma activity energy levels of 2436.356keV, l837.24keV 2928.37 keV and 1656.32keV, 1635.48keV, 2351.87keV respectively as compared to ( 204 B). While Lams 1,5 and Voms 2,3 had relatively lower gamma activity energy levels of 1325.23KeV, 1272.73keV and 1462.61KeV, 1183.24keV respectively. The samples with high gamma activity energy levels imply that radionuclide in the form of 235 U is present in trace amounts in the sampled areas. This can affect the output of apples cultivated in such areas as the chemical composition or structure of plants will be altered.

Standard test method for nondestructive assay of radioactive material by tomographic gamma scanning

CERN Document Server

American Society for Testing and Materials. Philadelphia

2010-01-01

1.1 This test method describes the nondestructive assay (NDA) of gamma ray emitting radionuclides inside containers using tomographic gamma scanning (TGS). High resolution gamma ray spectroscopy is used to detect and quantify the radionuclides of interest. The attenuation of an external gamma ray transmission source is used to correct the measurement of the emission gamma rays from radionuclides to arrive at a quantitative determination of the radionuclides present in the item. 1.2 The TGS technique covered by the test method may be used to assay scrap or waste material in cans or drums in the 1 to 500 litre volume range. Other items may be assayed as well. 1.3 The test method will cover two implementations of the TGS procedure: (1) Isotope Specific Calibration that uses standards of known radionuclide masses (or activities) to determine system response in a mass (or activity) versus corrected count rate calibration, that applies to only those specific radionuclides for which it is calibrated, and (2) Respo...

Computers in activation analysis and gamma-ray spectroscopy

Energy Technology Data Exchange (ETDEWEB)

Carpenter, B. S.; D' Agostino, M. D.; Yule, H. P. [eds.

1979-01-01

Seventy-three papers are included under the following session headings: analytical and mathematical methods for data analysis; software systems for ..gamma..-ray and x-ray spectrometry; ..gamma..-ray spectra treatment, peak evaluation; least squares; IAEA intercomparison of methods for processing spectra; computer and calculator utilization in spectrometer systems; and applications in safeguards, fuel scanning, and environmental monitoring. Separate abstracts were prepared for 72 of those papers. (DLC)

A Multi-Contact, Low Capacitance HPGe Detector for High Rate Gamma Spectroscopy

Energy Technology Data Exchange (ETDEWEB)

Cox, Christopher [XIA LLC, Hayward, CA (United States)

2014-12-04

The detection, identification and non-destructive assay of special nuclear materials and nuclear fission by-products are critically important activities in support of nuclear non-proliferation programs. Both national and international nuclear safeguard agencies recognize that current accounting methods for spent nuclear fuel are inadequate from a safeguards perspective. Radiation detection and analysis by gamma-ray spectroscopy is a key tool in this field, but no instrument exists that can deliver the required performance (energy resolution and detection sensitivity) in the presence of very high background count rates encountered in the nuclear safeguards arena. The work of this project addresses this critical need by developing a unique gamma-ray detector based on high purity germanium that has the previously unachievable property of operating in the 1 million counts-per-second range while achieving state-of-the-art energy resolution necessary to identify and analyze the isotopes of interest. The technical approach was to design and fabricate a germanium detector with multiple segmented electrodes coupled to multi-channel high rate spectroscopy electronics. Dividing the germanium detector’s signal electrode into smaller sections offers two advantages; firstly, the energy resolution of the detector is potentially improved, and secondly, the detector is able to operate at higher count rates. The design challenges included the following; determining the optimum electrode configuration to meet the stringent energy resolution and count rate requirements; determining the electronic noise (and therefore energy resolution) of the completed system after multiple signals are recombined; designing the germanium crystal housing and vacuum cryostat; and customizing electronics to perform the signal recombination function in real time. In this phase I work, commercial off-the-shelf electrostatic modeling software was used to develop the segmented germanium crystal geometry

A digital multi-channel spectroscopy system with 100 MHz flash ADC module for the GENIUS-TF and GENIUS projects

OpenAIRE

Kihm, T.; Bobrakov, V. F.; Klapdor-Kleingrothaus, H. V.

2003-01-01

In this paper we will present the first results of applying a digital processing technology in low-level gamma spectroscopy with HPGE detectors. An experimental gamma spectrometer using Flash ADC module is built and tested. The test system is now under development and shows major advantages over the traditional analog technologies. It will be installed for the GENIUS-TF and GENIUS projects in Gran-Sasso in early 2003.

A miniature modular multichannel analyzer system for automated, low- resolution gamma-ray spectroscopy

International Nuclear Information System (INIS)

Sprinkle, J.K. Jr.; Halbig, J.K.; Klosterbuer, S.F.; Russo, P.A.; Smith, S.E.

1992-01-01

Throughout the nuclear complex, the demand for measurements of nuclear materials holdup is increasing. Plant-wide campaigns to quantify holdup in ventilation ducts and holdup measurements in support of duct remediation are in progress at most DOE sites. Plans to satisfy more stringent requirements for holdup measurements are being developed. Facility decommissioning that accompanies downsizing the complex will require extensive holdup measurement efforts. In the early phases of planning for the modem complex, holdup measurements for new facilities are being specified at the facility design stage. Beyond the DOE, international inspection activities are relying, increasingly, on holdup measurements for verification. Developments in nondestructive assay technologies in the past decade have provided some support for measurements of this Mx. The user's requirements of ruggedness and reliability have been satisfied with compact gamma-ray detectors and spectroscopy instrumentation, but improvements are still needed in simplicity, portability, and speed. Current portable spectroscopy instruments require user sophistication as well as more than one person for transport between measurement locations. However, it is becoming clear that the real measurement need is the simultaneous operation of dozens of units, each by a single relatively unsophisticated user, to perform thousands of measurements per inventory period. The rapid and reliable conversion of measurement data to holdup quantities is essential

Detection and evaluation of uranium in different minerals by gamma spectrometry and laser induced breakdown spectroscopy

International Nuclear Information System (INIS)

Sergani, F.M.; Khedr, M.A.; Harith, M.A.; El Mongy, S.A.

2004-01-01

Analysis, detection and evaluation of source nuclear materials (e.g. uranium) in different minerals by sensitive techniques are a vital objective for uranium exploration, nuclear materials extraction, processing and verification. In this work, uranium in different geological formations was determined using gamma spectrometry and laser induced breakdown spectroscopy (LIBS). The investigated samples were collected from different regions distributed all over Egypt. The samples were then prepared for non-destructive analysis. A hyper pure germanium detector was used to measure the emitted gamma rays of uranium and its daughters in the samples. The concentrations of uranium in ppm (μg/g) in the investigated samples are given and discussed in this work. The highest uranium concentration (4354.9 ppm) was found in uranophane samples of Gattar rocks. In Laser induced breakdown spectroscopy (LIBS) technique, plasma was formed by irradiating the rock surface with focused Q-switched Nd:Yag laser pulses of 7 ns pulse duration at the fundamental wavelength (1064 nm). Atoms and ions originating from the rock surface are excited and ionized in the laser produced hot plasma (∝10 000 K). The plasma emission spectral line is characteristic of the elements present in the plasma and allows identification of the uranium in the uranophane mineral. The strong atomic line at 424.2 nm is used for the qualitative identification of uranium. It can be mentioned that the elevated levels of uranium in some of the investigated uranophane samples are of great economic feasibility to be extracted. (orig.)

Calibration of the ISOLDE acceleration voltage using a high-precision voltage divider and applying collinear fast beam laser spectroscopy

CERN Document Server

Krieger, A.; Catherall, R.; Hochschulz, F.; Kramer, J.; Neugart, R.; Rosendahl, S.; Schipper, J.; Siesling, E.; Weinheimer, Ch.; Yordanov, D.T.; Nortershauser, W.

2011-01-01

A high-voltage divider with accuracy at the ppm level and collinear laser spectroscopy were used to calibrate the highvoltage installation at the radioactive ion beam facility ISOLDE at CERN. The accurate knowledge of this voltage is particularly important for collinear laser spectroscopy measurements. Beam velocity measurements using frequencycomb based collinear laser spectroscopy agree with the new calibration. Applying this, one obtains consistent results for isotope shifts of stable magnesium isotopes measured using collinear spectroscopy and laser spectroscopy on laser-cooled ions in a trap. The long-term stability and the transient behavior during recovery from a voltage dropout were investigated for the different power supplies currently applied at ISOLDE.

Effect of gamma irradiation on nano polymer poly aniline

International Nuclear Information System (INIS)

Chan Yan Yhee

2012-01-01

Poly aniline (PANI) is a conductor polymer that investigated by a lot of researchers which display unique electric characteristic and widely applications. The objective in this research is to see the effect of gamma irradiation on PANI by using microemulsion method. Cation surfactant, cetyltrimethylammonium bromide, (CTAB) use in microemulsion method for dissolve aniline with distilled water. Mixture of aniline, ammonium persulfate (APS) as oxidizing agent and hydrochloric acid (HCL) into aqueous CTAB and magnetic bar stirrer applied at temperature of 3 degree Celsius for 3 hours to form PANI. The washing is done by using distilled water and ethanol to purify PANI. After washing the PANI are categories in two group, PANI aqueous solution and PANI powder. PANI aqueous solution irradiated with gamma irradiation from 0 kGy to 100 kGy doses in 10 kGy intervals while PANI powder are dried in oven before irradiated with gamma irradiation with same doses as PANI aqueous solution. These aqueous solution products are characterized by ultraviolet absorption spectroscopy (UV-Vis) which shows the electron transition π - π * and Microscope Electron Transmission (TEM) for morforlogy of PANI nanoparticles while PANI powder are characterized using Spectroscopy Fourier Transformation Intra-Red (FTIR) for the functional group, X-Ray Diffraction (XRD) to determine the crystalline peak and Field Emission Scanning Electron Microscope (FESEM) for morphology PANI nanoparticles. The effect of gamma irradiation nanoparticles are PANI aqueous solution produce aggregation and changing of PANI nanoparticles sizes while PANI powder produce fractures and distortion on PANI nanoparticles. (author)

Study of stability of humic acids from soil and peat irradiated by gamma rays

International Nuclear Information System (INIS)

Silva, Wilson Tadeu Lopes da

1995-01-01

Humic acids samples (one deriving from a sedimentary soil and other from a peat), in aqueous media, were irradiated with gamma rays, in doses of 10, 50 and 100 kGy, in order to understand their chemical behavior after the irradiation. The material, before and after irradiation, was analyzed by Elemental Analysis, Functional Groups (carboxylic acids and phenols), UV/Vis Spectroscopy (E 4 /E 6 ratio), IR spectroscopy, CO 2 content and Gel permeation Chromatography (GPC) ). The Elemental Analysis showed the humic acid derived from a peat had a most percentage quantity of Carbon and Hydrogen than the material from a sedimentary soil. From the UV/Vis Spectroscopy, it was observed a decrease of E 4 /E 6 ratio with an increase of the applied dose. The data from GPC are in agreement with this. The results showed that the molecular weight of the material increased by exposing it to a larger radiolitical dose. The peat material was less affected by the gamma radiation than the soil material. The carboxylic groups were responsible by radiochemical behavior of the material. (author)

Investigation of LaBr3:Ce probe for gamma-ray spectroscopy and dosimetry

Science.gov (United States)

Maghraby, Ahmed M.; Alzimami, K. S.; Alkhorayef, M. A.; Alsafi, K. G.; Ma, A.; Alfuraih, A. A.; Alghamdi, A. A.; Spyrou, N. M.

2014-02-01

The main thrust of this work is the investigation of performance of relatively new commercial LaBr3:Ce probe (Inspector 1000™ with LaBr3:Ce crystal) for gamma-ray spectroscopy and dosimetry measurements in comparison to LaCl3:Ce and NaI:Tl scintillators. The crystals were irradiated by a wide range of energies (57Co, 22Na, 18F, 137Cs and 60Co). The study involved recording of detected spectra and measurement of energy resolution, photopeak efficiency, internal radioactivity measurements as well as dose rate. The Monte Carlo package, Geant4 Application for Tomographic Emission (GATE) was used to validate the experiments. Overall results showed very good agreement between the measurements and the simulations. The LaBr3:Ce crystal has excellent energy resolution, energy resolutions of (3.37±0.05)% and (2.98±0.07)% for a 137Cs 662 keV and a 60Co 1332 keV gamma-ray point sources respectively, were recorded. The disadvantage of the lanthanum halide scintillators is their internal radioactivity. Inspector 1000™ with LaBr3:Ce scintillator has shown an accurate and quick dose measurements at Positron Emission Tomography (PET) Units which allows accurate assessment of the radiation dose received by staff members compared to the use of electronic personal dosimeters (EPD).

Dual sightline measurements of MeV range deuterons with neutron and gamma-ray spectroscopy at JET

DEFF Research Database (Denmark)

Eriksson, J.; Nocente, M.; Binda, F.

2015-01-01

Observations made in a JET experiment aimed at accelerating deuterons to the MeV range by third harmonic radio-frequency (RF) heating coupled into a deuterium beam are reported. Measurements are based on a set of advanced neutron and gamma-ray spectrometers that, for the first time, observe......-ray spectroscopy based on a one-dimensional model and by a consistency check among the individual measurement techniques. A systematic difference is seen between the two lines of sight and is interpreted to originate from the sensitivity of the oblique detectors to the pitch-angle structure of the distribution...

The PRESPEC liquid-hydrogen target for in-beam gamma spectroscopy of exotic nuclei at GSI

International Nuclear Information System (INIS)

Louchart, C.; Gheller, J.M.; Chesny, Ph.; Authelet, G.; Rousse, J.Y.; Obertelli, A.; Boutachkov, P.; Pietri, S.; Ameil, F.; Audirac, L.; Corsi, A.; Dombradi, Z.; Gerl, J.; Gillibert, A.; Korten, W.; Mailleret, C.; Merchan, E.; Nociforo, C.; Pietralla, N.; Ralet, D.

2014-01-01

We report on a new liquid hydrogen and deuterium target dedicated to in-beam γ spectroscopy experiments in inverse kinematics at relativistic incident energies at GSI/FAIR. Target thicknesses from 10 to 80 mm can be achieved for an effective diameter of 60 mm. The target-cell and entrance window are maded of 200μm thick Mylar. The design has the advantage of being free of absorbing material at forward angles and 90°, allowing the detection of photons in a wide angular range. A commissioning experiment with a 54 Cr beam at 130 MeV/nucleon has been performed at GSI, using the Rare Isotopes INvestigation at GSI (RISING) detectors. The target has been shown to behave as expected and is ready for experiments at fragmentation Radioactive-Ion Beam Facilities. -- Highlights: • We report on a new liquid hydrogen target for gamma spectroscopy experiments at FAIR. • A commissioning experiment has been performed at GSI, using the RISING detectors. • The target behaves as expected and is ready for experiments

gamma-Glutamyl dipeptides in Petiveria alliacea.

Science.gov (United States)

Kubec, Roman; Musah, Rabi A

2005-10-01

Three gamma-glutamyl dipeptides have been isolated from Petiveria alliacea L. roots. These dipeptides include (S(C2)R(C7))-gamma-glutamyl-S-benzylcysteine together with two diastereomeric sulfoxides, namely (S(C2)R(C7)R(S))- and (S(C2)R(C7)R(S))-gamma-glutamyl-S-benzylcysteine S-oxides (gamma-glutamyl-petiveriins A and B, respectively). Their structures and absolute configurations have been determined by NMR, MALDI-HRMS, IR and CD spectroscopy, and confirmed by comparison with authentic compounds obtained by synthesis.

Calibration of the ISOLDE acceleration voltage using a high-precision voltage divider and applying collinear fast beam laser spectroscopy

Energy Technology Data Exchange (ETDEWEB)

Krieger, A., E-mail: kriegea@uni-mainz.d [Institut fuer Kernchemie, Johannes Gutenberg, Universitaet Mainz, Fritz-Strassmann-Weg 2, 55128 Mainz (Germany); Geppert, Ch. [Institut fuer Kernchemie, Johannes Gutenberg, Universitaet Mainz, Fritz-Strassmann-Weg 2, 55128 Mainz (Germany); GSI Helmholtzzentrum fuer Schwerionenforschung, 64291 Darmstadt (Germany); Catherall, R. [CERN, CH-1211 Geneve 23 (Switzerland); Hochschulz, F. [Institut fuer Kernphysik, Universitaet Muenster, 48149 Muenster (Germany); Kraemer, J.; Neugart, R. [Institut fuer Kernchemie, Johannes Gutenberg, Universitaet Mainz, Fritz-Strassmann-Weg 2, 55128 Mainz (Germany); Rosendahl, S. [Institut fuer Kernphysik, Universitaet Muenster, 48149 Muenster (Germany); Schipper, J.; Siesling, E. [CERN, CH-1211 Geneve 23 (Switzerland); Weinheimer, Ch. [Institut fuer Kernphysik, Universitaet Muenster, 48149 Muenster (Germany); Yordanov, D.T. [Max-Planck-Institut fuer Kernphysik, 69117 Heidelberg (Germany); Noertershaeuser, W. [Institut fuer Kernchemie, Johannes Gutenberg, Universitaet Mainz, Fritz-Strassmann-Weg 2, 55128 Mainz (Germany); GSI Helmholtzzentrum fuer Schwerionenforschung, 64291 Darmstadt (Germany)

2011-03-11

A high-voltage divider with accuracy at the ppm level and collinear laser spectroscopy were used to calibrate the high-voltage installation at the radioactive ion beam facility ISOLDE at CERN. The accurate knowledge of this voltage is particularly important for collinear laser spectroscopy measurements. Beam velocity measurements using frequency-comb based collinear laser spectroscopy agree with the new calibration. Applying this, one obtains consistent results for isotope shifts of stable magnesium isotopes measured using collinear spectroscopy and laser spectroscopy on laser-cooled ions in a trap. The long-term stability and the transient behavior during recovery from a voltage dropout were investigated for the different power supplies currently applied at ISOLDE.

BiI₃ Crystals for High Energy Resolution Gamma-Ray Spectroscopy

Energy Technology Data Exchange (ETDEWEB)

Nino, Juan C. [Univ. of Florida, Gainesville, FL (United States); Baciak, James [Univ. of Florida, Gainesville, FL (United States); Johns, Paul [Univ. of Florida, Gainesville, FL (United States); Sulekar, Soumitra [Univ. of Florida, Gainesville, FL (United States); Totten, James [Univ. of Florida, Gainesville, FL (United States); Nimmagadda, Jyothir [Univ. of Florida, Gainesville, FL (United States)

2017-04-12

BiI₃ had been investigated for its unique properties as a layered compound semiconductor for many decades. However, despite the exceptional atomic, physical, and electronic properties of this material, good resolution gamma ray spectra had never been reported for BiI₃. The shortcomings that previously prevented BiI₃ from reaching success as a gamma ray sensor were, through this project, identified and suppressed to unlock the performance of this promising compound. Included in this work were studies on a number of methods which have, for the first time, enabled BiI₃ to exhibit spectral performance rivaling many other candidate semiconductors for room temperature gamma ray sensors. New approaches to crystal growth were explored that allow BiI₃ spectrometers to be fabricated with up to 2.2% spectral resolution at 662 keV. Fundamental studies on trap states, dopant incorporation, and polarization were performed to enhance performance of this compound. Additionally, advanced detection techniques were applied to display the capabilities of high quality BiI₃ spectrometers. Overall, through this work, BiI₃ has been revealed as a potentially transformative material for nuclear security and radiation detection sciences.

High-resolution gamma-ray spectroscopy with a microwave-multiplexed transition-edge sensor array

Energy Technology Data Exchange (ETDEWEB)

Noroozian, Omid [National Institute of Standards and Technology, Boulder, Colorado 80305 (United States); Center for Astrophysics and Space Astronomy, University of Colorado, Boulder, Colorado 80309 (United States); Mates, John A. B.; Bennett, Douglas A.; Brevik, Justus A.; Fowler, Joseph W.; Gao, Jiansong; Hilton, Gene C.; Horansky, Robert D.; Irwin, Kent D.; Schmidt, Daniel R.; Vale, Leila R.; Ullom, Joel N. [National Institute of Standards and Technology, Boulder, Colorado 80305 (United States); Kang, Zhao [Department of Physics, University of Colorado, Boulder, Colorado 80309 (United States)

2013-11-11

We demonstrate very high resolution photon spectroscopy with a microwave-multiplexed two-pixel transition-edge sensor (TES) array. We measured a {sup 153}Gd photon source and achieved an energy resolution of 63 eV full-width-at-half-maximum at 97 keV and an equivalent readout system noise of 86 pA/√(Hz) at the TES. The readout circuit consists of superconducting microwave resonators coupled to radio-frequency superconducting-quantum-interference-devices and transduces changes in input current to changes in phase of a microwave signal. We use flux-ramp modulation to linearize the response and evade low-frequency noise. This demonstration establishes one path for the readout of cryogenic X-ray and gamma-ray sensor arrays with more than 10{sup 3} elements and spectral resolving powers R=λ/Δλ>10{sup 3}.

Quantification of {sup 235} U and {sup 226} Ra in soil samples by means of Gamma spectroscopy; Cuantificacion de {sup 235} U y {sup 226} Ra en muestras de suelo por medio de espectrometria gamma

Energy Technology Data Exchange (ETDEWEB)

Quintero P, E.; Rojas M, V.P.; Montes M, F.R.; Gaso P, M.I.; Cervantes N, M.L. [Gerencia de Innovacion Tecnologica, A.P. 18-1027, C.P. 11801 Mexico D.F. (Mexico)

2000-07-01

In this work it is presented the Gamma Spectroscopy method which is realized in the Environmental Radiological Surveillance Laboratory using the option of deconvolution of a commercial software for the quantification of {sup 235} U and {sup 226} Ra; also is presented the method for the {sup 226} Ra correction activity. (Author)

Natural background gamma-ray spectrum. List of gamma-rays ordered in energy from natural radionuclides

Energy Technology Data Exchange (ETDEWEB)

Ichimiya, Tsutomu [Japan Radioisotope Association, Tokyo (Japan); Narita, Tsutomu; Kitao, Kensuke

1998-03-01

A quick index to {gamma}-rays and X-rays from natural radionuclides is presented. In the list, {gamma}-rays are arranged in order of increasing energy. The list also contains {gamma}-rays from radioactive nuclides produced in a germanium detector and its surrounding materials by interaction with cosmic neutrons, as well as direct {gamma}-rays from interaction with the neutrons. Artificial radioactive nuclides emitting {gamma}-rays with same or near energy value as that of the natural {gamma}-rays and X-rays are also listed. In appendix, {gamma}-ray spectra from a rock, uranium ore, thorium, monazite and uraninite and also background spectra obtained with germanium detectors placed in iron or lead shield have been given. The list is designed for use in {gamma}-ray spectroscopy under the conditions of highly natural background, such as in-situ environmental radiation monitoring or low-level activity measurements, with a germanium detector. (author)

Prompt gamma activation analysis (PGAA) and short-lived neutron activation analysis (NAA) applied to the characterization of legacy materials

International Nuclear Information System (INIS)

English, G.A.; Firestone, R.B.; Perry, D.L.; Reijonen, J.P.; Ka-Ngo Leung; Garabedian, G.F.; Molnar, G.L.; Revay, Zs.

2008-01-01

Without quality historical records that provide the composition of legacy materials, the elemental and/or chemical characterization of such materials requires a manual analytical strategy that may expose the analyst to unknown toxicological hazards. In addition, much of the existing legacy inventory also incorporates radioactivity, and, although radiological composition may be determined by various nuclear-analytical methods, most importantly, gamma-spectroscopy, current methods of chemical characterization still require direct sample manipulation, thereby presenting special problems with broad implications for both the analyst and the environment. Alternately, prompt gamma activation analysis (PGAA) provides a 'single-shot' in-situ, non-destructive method that provides a complete assay of all major entrained elemental constituents. Additionally, neutron activation analysis (NAA) using short-lived activation products complements PGAA and is especially useful when NAA activation surpasses the PGAA in elemental sensitivity. (author)

Prompt gamma activation analysis (PGAA) and short-lived neutron activation analysis (NAA) applied to the characterization of legacy materials

International Nuclear Information System (INIS)

Firestone, Richard B; English, G.A.; Firestone, R.B.; Perry, D.L.; Reijonen, J.P.; Leung, Ka-Ngo; Garabedian, G.F.; Molnar, G.L.; Revay, Zs.

2008-01-01

Without quality historical records that provide the composition of legacy materials, the elemental and/or chemical characterization of such materials requires a manual analytical strategy that may expose the analyst to unknown toxicological hazards. In addition, much of the existing legacy inventory also incorporates radioactivity, and, although radiological composition may be determined by various nuclear-analytical methods, most importantly, gamma-spectroscopy, current methods of chemical characterization still require direct sample manipulation, thereby presenting special problems with broad implications for both the analyst and the environment. Alternately, prompt gamma activation analysis (PGAA) provides a 'single-shot' in-situ, non-destructive method that provides a complete assay of all major entrained elemental constituents.1-3. Additionally, neutron activation analysis (NAA) using short-lived activation products complements PGAA and is especially useful when NAA activation surpasses the PGAA in elemental sensitivity

Quantification by Raman spectroscopy of the gamma radiation effects in water purification; Cuantificacion por espectroscopia Raman de los efectos de la radiacion gamma en la purificacion de agua

Energy Technology Data Exchange (ETDEWEB)

Perez C, V M; Santiago J, P; Castano, V M [Instituto Nacional de Investigaciones Nucleares, A.P. 18-1027, 11801 Mexico D.F. (Mexico)

1999-07-01

The world problem about water pollution has been confronted by traditional methods such as: chlorination, filtration, etc. In this work is presented an alternative method, which consists in to radiate different concentrations of simulated polluted water (purified water + thinner) at different gamma radiation doses. The structural changes were analysed by Raman spectroscopy. Using a 52.5 Krad dose it was possible to eliminate all the thinner chemical linkages, which appear in the Raman spectra corresponding to the 87.5/12.5 water/thinner mixture. (Author)

Application of Inverse Gamma Transport to Material Thickness Identification with SGRD Code

Directory of Open Access Journals (Sweden)

Humbert Philippe

2017-01-01

Full Text Available SGRD (Spectroscopy, Gamma rays, Rapid, Deterministic code is used to infer the dimensions of a one dimensional model of a shielded gamma ray source. The method is based on the simulation of the uncollided leakage current of discrete gamma lines that are produced by nuclear decay. Experimentally, the unscattered gamma lines leakage current is obtained by processing high precision gamma spectroscopy measurements. The material thicknesses are computed with SGRD using a fast ray-tracing algorithm embedded in a non-linear multidimensional iterative optimization procedure that minimizes the error metric between calculated and measured signatures. For verification, numerical results on a test problem are presented.

Crystal growth and thermoluminescence response of NaZr{sub 2}(PO{sub 4}){sub 3} at high gamma radiation doses

Energy Technology Data Exchange (ETDEWEB)

Ordóñez-Regil, E., E-mail: eduardo.ordonez@inin.gob.mx [Depto. de Química, Gerencia de Ciencias Básicas, Instituto Nacional de Investigaciones Nucleares, AP 18-1027, CP 11801 México D.F. (Mexico); Contreras-Ramírez, A., E-mail: aida.contreras@inin.gob.mx [Depto. de Química, Gerencia de Ciencias Básicas, Instituto Nacional de Investigaciones Nucleares, AP 18-1027, CP 11801 México D.F. (Mexico); Depto. de Tecnología de Materiales, Gerencia de Ciencias Aplicadas, Instituto Nacional de Investigaciones Nucleares, AP 18-1027, CP 11801 México D.F. (Mexico); Facultad de Ciencias, Universidad Autónoma del Estado de México, Unidad Académica el Cerrillo, Piedras Blancas, AP 2-139, CP 50000 Toluca Estado de México (Mexico); Fernández-Valverde, S.M., E-mail: suilma.fernandez@inin.gob.mx [Depto. de Química, Gerencia de Ciencias Básicas, Instituto Nacional de Investigaciones Nucleares, AP 18-1027, CP 11801 México D.F. (Mexico); González-Martínez, P.R., E-mail: pedro.gonzalez@inin.gob.mx [Depto. de Física, Gerencia de Ciencias Básicas, Instituto Nacional de Investigaciones Nucleares, AP 18-1027, CP 11801 México D.F. (Mexico); Carrasco-Ábrego, H., E-mail: hector.carrasco@inin.gob.mx [Depto. Aceleradores, Gerencia de Ciencias Ambientales, Instituto Nacional de Investigaciones Nucleares, AP 18-1027, CP 11801 México D.F. (Mexico)

2013-11-15

Graphical abstract: -- Highlights: •NaZr{sub 2}(PO{sub 4}){sub 3} exposed to gamma doses of 10, 30 and 50 MGy. •Gamma radiation produced growth of the crystal size of the NZP. •Morphology changes were reversible by heating. •Linear relationship between the thermoluminescence and the applied gamma dose. •This property could be useful for high-level gamma dosimetry. -- Abstract: This work describes the synthesis and characterization of NaZr{sub 2}(PO{sub 4}){sub 3}. The stability of this material under high doses of gamma radiation was investigated in the range of 10–50 MGy. Samples of unaltered and gamma irradiated NaZr{sub 2}(PO{sub 4}){sub 3} were characterized by X-ray diffraction, infrared spectroscopy, scanning electron microscopy, energy dispersive X-ray spectroscopy, and thermoluminescence. The results showed that while functional groups were not affected by the gamma irradiation, morphology changes were observed with increasing doses of gamma irradiation. The morphology of the non-irradiated compound is agglomerated flakes; however, irradiation at 10 MGy splits the flakes inducing the formation of well-defined cubes. Gamma irradiation induced the crystal size of the NaZr{sub 2}(PO{sub 4}){sub 3} to grow. The heat treatment (973 K) of samples irradiated at 50 MGy resulted in the recovery of the original morphology. Furthermore, the thermoluminescence analysis of the irradiated compound is reported.

Collimatorless imaging of gamma rays with help of gamma-ray tracking

CERN Document Server

Marel, J V D

2001-01-01

In many gamma-ray detector systems that are built for imaging purposes Compton scattered photons are suppressed as much as possible. However, the information from photons that scattered inside a detector system can be used to reconstruct the tracks of the photons with help of gamma-ray tracking. Estimates of the incident directions of the photons can be made and an image can be created. Examples of potential applications for this technique are the use as a gamma-camera in medical imaging (e.g. SPECT) or as a detector for PET. Due to the omission of collimators, much higher detection efficiencies can be achieved, reducing the doses required for an image. A gamma-ray tracking method, called backtracking, has been developed for nuclear spectroscopy. The method tracks gamma-rays originating from a point source in the center of a spherical detector system consisting of position-sensitive germanium detectors. This method can also be used as a tracking technique for imaging of an unknown source distribution. With he...

Dielectric spectroscopy technique applied to study the behaviour of irradiated polymer

International Nuclear Information System (INIS)

Saoud, R.; Soualmia, A.; Guerbi, C.A.; Benrekaa, N.

2006-01-01

Relaxation spectroscopy provides an excellent method for the study of motional processes in materials and has been widely applied to macromolecules and polymers. The technique is potentially of most interest when applied to irradiated systems. Application to the study of the structure beam-irradiated Teflon is thus an outstanding opportunity for the dielectric relaxation technique, particularly as this material exhibits clamping problems when subjected to dynamic mechanical relaxation studies. A very wide frequency range is necessary to resolve dipolar effects. In this paper, we discuss some significant results about the behavior and the modification of the structure of Teflon submitted to weak energy radiations

Gamma transitions in 127Te

International Nuclear Information System (INIS)

Batista, Wagner Fonseca; Zamboni, Cibele Bugno

2009-01-01

This study of the 127 Te β - decay was carried out by means of gamma spectroscopy measurements using high resolution Ge detector, in the region from 150 keV up to 1000 keV, aiming to get a better understanding of the 127 Te nuclear structure. Several gamma transitions were confirmed when compared with those published in the last compilation. These data resulting in lower uncertainty. (author)

Neutron characteristic and spectroscopy logging methods and apparatus

International Nuclear Information System (INIS)

Antkiw, S.

1977-01-01

Earth formations surrounding a well bore are irradiated with pulses of fast neutrons, and gamma rays resulting from the ensuring thermal neutron capture interactions with nuclei of the formations are detected, from which measurements of the thermal neutron decay times characterizing the respective formations are derived. The gamma ray energy spectra of the respective formations are analyzed. Gating of the gamma ray detection periods is automatically controlled, both for the decay time and the spectroscopy functions, in accrdance with the measured values of the decay times. The duration and repetition rate of the neutron pulses are also controlled as a function of the measured decay times to provide an overall optimized decay time-spectroscopy operating cycle. spectroscopy outputs representative of formation lithology, salinity, porosity and shaliness are developed to supplement and improve decay time log interpretation

GRIPS - Gamma-Ray Imaging, Polarimetry and Spectroscopy

Czech Academy of Sciences Publication Activity Database

Greiner, J.; Mannheim, K.; Hudec, René; Mészáros, A.

2012-01-01

Roč. 34, č. 2 (2012), s. 551-582 ISSN 0922-6435 Institutional research plan: CEZ:AV0Z10030501 Keywords : compton and pair creation telescope * gamma-ray bursts * nucleosynthesis Subject RIV: BN - Astronomy, Celestial Mechanics, Astrophysics Impact factor: 2.969, year: 2012

Gamma-ray spectroscopy of Λ11B

International Nuclear Information System (INIS)

Miura, Yusuke

2004-01-01

Numbers of bound states have been predicted for the hypernucleus Λ 11 B. Experiment KEK-PS E518 was performed to investigate the spin dependence of the effective ΛN interaction of p-shell hypernucleus as well as the magnetic moment of Λ particle inside nucleus by measuring B(M1) of the Λ spin-flip transition. Experiment was carried out by using Hyperball detector which consists of fourteen germanium detectors to detect γ-rays from Λ 11 B produced by 11 B(π + , K + ) Λ 11 B reaction. Six gamma ray peaks were observed from the bound state of Λ 11 B at 262, 454, 500, 564, 1482, and 2479 keV. The 2479 keV peak was revealed by applying Doppler correction. The 1482 keV peak was identified as the Λ 11 B (E2;1/2 + → 5/2 + ) due to the short γ-transition life, good yield and the closeness of the γ-ray emission level to the ground state. Statistics were too poor for the rest five peaks to identify their origin without γ-γ coincidence measurement. The result shows that discrepancy between the experiment and theoretical prediction is large compared with other hypernuclei. Upgrading of the Hyperball and the γ-γ coincidence are considered for the future experiment. (S. Funahashi)

The efficiency calibration and development of environmental correction factors for an in situ high-resolution gamma spectroscopy well logging system

International Nuclear Information System (INIS)

Giles, J.R.

1996-05-01

A Gamma Spectroscopy Logging System (GSLS) has been developed to study sub-surface radionuclide contamination. Absolute efficiency calibration of the GSLS was performed using simple cylindrical borehole geometry. The calibration source incorporated naturally occurring radioactive material (NORM) that emitted photons ranging from 186-keV to 2,614-keV. More complex borehole geometries were modeled using commercially available shielding software. A linear relationship was found between increasing source thickness and relative photon fluence rates at the detector. Examination of varying porosity and moisture content showed that as porosity increases, relative photon fluence rates increase linearly for all energies. Attenuation effects due to iron, water, PVC, and concrete cylindrical shields were found to agree with previous studies. Regression analyses produced energy-dependent equations for efficiency corrections applicable to spectral gamma-ray well logs collected under non-standard borehole conditions

comparative studies on pyriproxyfen and fenoxycarb as juvenile hormones applied separately or combined with gamma radiation for controlling the mediterranean fruit fly, ceratitis capitata (Wied)

International Nuclear Information System (INIS)

Fadel, A.M.; Othman, K.S.A.

1998-01-01

Comparative studies on pyriproxyfen and fenoxycarb as juvenile hormones applied separately or combined with gamma radiation were carried out for controlling ceratitis capitata. Lc 50's of the two juvenile hormones, pyriproxfen and fenoxycarb, were determined against ceratitis capitata in treated diet by continuous contact of eggs and larvae using various concentrations. The Lc 50 were 32 and 140 ppm for pyriproxyfen and fenoxycarb, respectively. The resulting pupae were gamma irradiated with 90 Gy. Larval and pupal durations were insignificantly affected, pupation and adult emergence were significantly affected while adult survival was insignificantly affected when applying the two JH's. Applying pyriproxyfen alone insignificantly increased egg hatch at the concentrations used (12.5 and 25 ppm) while when fenoxycarb was applied alone egg hatch was significantly decreased at the concentration used (100 ppm). Applying both juvenile hormones each combined with gamma radiation significantly reduced egg hatch. Male mating competitiveness was significantly increased when applying pyriproxyfen at the concentration 25 Ppm. Results indicated that pyriproxyfen was more effective than fenoxycarb against the mediterranean fruit fly ceratitis capitata.1 figs., 3 tabs

{sup 1}H MR spectroscopy of mesial temporal lobe epilepsies treated with Gamma knife

Energy Technology Data Exchange (ETDEWEB)

Hajek, Milan; Dezortova, Monika [MR Unit, Department of Diagnostic and Interventional Radiology, Institute for Clinical and Experimental Medicine, Videnska 1958/9, 140 21 Prague (Czech Republic); Center for Cell Therapy and Tissue Repair, V Uvalu 84, 150 00 Prague (Czech Republic); Liscak, Roman; Vymazal, Josef; Vladyka, Vilibald [Department of Stereotactic and Radiation Neurosurgery, Hospital Na Homolce, 151 19, Prague (Czech Republic)

2003-05-01

Proton MR spectroscopy was used to observe long-term post-irradiation metabolic changes in epileptogenic tissue and in the contralateral parts of the brain which are not available with conventional imaging methods. We studied these changes in the temporal lobe in six patients, following radiosurgery on the amygdala and hippocampus. {sup 1}H MR spectroscopy at 1.5 T with short and long echo times (TE=10 and 135 ms) were used together with standard MR imaging sequences (T1-, T2-weighted). The treatment was performed by Leksell Gamma Knife with a dose of 50 Gy to the center and a 50% isodose to the margin of the target, represented by the mean volume of approximately 7.5 ml. Magnetic resonance imaging and MR spectroscopy examinations were performed at least once per year for 3 years. The most significant changes in spectra were observed approximately 1 year after the irradiation when edema in irradiated area was observed and strong signal of lipids was identified. Later, edema and lipid signals disappeared and follow-up was characterized by a decrease of NAA, Cr, and Cho concentrations in the ipsilateral region of the brain to the irradiation (LCModel calculation from voxel of interest 3.8-4.5 ml positioned into the centrum of target volume). The concentration of NAA, Cr, and Cho after radiosurgery was significantly different from control values (p<0.05) and also from concentrations in the contralateral part of the brain (p<0.05). In the contralateral part, the concentration of NAA was significantly increased (p<0.05) (NAA: before treatment 8.81, after treatment 11.33 mM). No radiotoxic changes were observed in the contralateral part of the brain or behind the area of target volume. The MR spectroscopy findings precluded MRI observation and MRS results completed data about the development of radiotoxic changes in the target volume. (orig.)

Preservation of photographic and cinematographic films by gamma radiation: Preliminary analyses

Energy Technology Data Exchange (ETDEWEB)

Nagai, Maria Luiza E.; Santos, Paulo S.; Otubo, Larissa; Oliveira, Maria José A.; Vasquez, Pablo A.S., E-mail: malunagai@usp.br, E-mail: pavsalva@ipen.br [Instituto de Pesquisas Energéticas e Nucleares (IPEN/CNEN-SP), São Paulo, SP (Brazil)

2017-07-01

Brazilian weather conditions affect directly tangible materials causing deterioration notably getting worse by insects and fungi attack. In this sense, gamma radiation provided from the cobalt-60 is an excellent alternative tool to the traditional preservation process mainly because it has biocidal action. Radiation processing using gamma radiation for cultural heritage materials for disinfection has been widely used around the world in the last decades. Many cultural heritage objects especially made on paper and wood were studied in scientific publications aiming mechanical, physical and chemical properties changes. Over the last fifteen years, the Multipurpose Gamma Irradiation Facility of the Nuclear and Energy Research Institute located inside the Sao Paulo University campus has been irradiated many collections of archived materials, books, paintings and furniture. Adequate storage of photographic and cinematographic materials is a challenge for conservators from preservation institutions. Contamination by fungi is one of leading causes of problem in photographic and cinematographic collections. Several Sao Paulo University libraries have been affected by fungi in their photographic and cinematographic collections making it impossible to research on these materials either manipulate them for health and safety reasons. In this work are presented preliminary results of effects of the ionizing radiation in photographic and cinematographic films. Selected film samples made on cellulose acetate were prepared and characterized by FTIR-ATR spectroscopy. Samples were irradiated by gamma rays with absorbed dose between 2 kGy and 50 kGy. Irradiated samples were analyzed by UV-VIS spectroscopy and electron microscopy techniques. Results shown that disinfection by gamma radiation can be achieved safely applying the disinfection dose between 6 kGy to 15 kGy with no significant change or modification of main properties of the constitutive materials. (author)

Preservation of photographic and cinematographic films by gamma radiation: Preliminary analyses

International Nuclear Information System (INIS)

Nagai, Maria Luiza E.; Santos, Paulo S.; Otubo, Larissa; Oliveira, Maria José A.; Vasquez, Pablo A.S.

2017-01-01

Brazilian weather conditions affect directly tangible materials causing deterioration notably getting worse by insects and fungi attack. In this sense, gamma radiation provided from the cobalt-60 is an excellent alternative tool to the traditional preservation process mainly because it has biocidal action. Radiation processing using gamma radiation for cultural heritage materials for disinfection has been widely used around the world in the last decades. Many cultural heritage objects especially made on paper and wood were studied in scientific publications aiming mechanical, physical and chemical properties changes. Over the last fifteen years, the Multipurpose Gamma Irradiation Facility of the Nuclear and Energy Research Institute located inside the Sao Paulo University campus has been irradiated many collections of archived materials, books, paintings and furniture. Adequate storage of photographic and cinematographic materials is a challenge for conservators from preservation institutions. Contamination by fungi is one of leading causes of problem in photographic and cinematographic collections. Several Sao Paulo University libraries have been affected by fungi in their photographic and cinematographic collections making it impossible to research on these materials either manipulate them for health and safety reasons. In this work are presented preliminary results of effects of the ionizing radiation in photographic and cinematographic films. Selected film samples made on cellulose acetate were prepared and characterized by FTIR-ATR spectroscopy. Samples were irradiated by gamma rays with absorbed dose between 2 kGy and 50 kGy. Irradiated samples were analyzed by UV-VIS spectroscopy and electron microscopy techniques. Results shown that disinfection by gamma radiation can be achieved safely applying the disinfection dose between 6 kGy to 15 kGy with no significant change or modification of main properties of the constitutive materials. (author)

High-sensitivity gamma spectroscopy for extended sources. Application to activity measurements on the human body, on glass, and on soil; Spectrographie gamma a grande sensibilite pour sources etendues. Application a la mesure de l'activite du corps humain, du verre et du sol

Energy Technology Data Exchange (ETDEWEB)

Jouve, B

1962-07-01

The measurement and location by gamma spectroscopy of human body internal contaminations at maximum permissible levels, and, in certain cases, at lower activities such as that due to {sup 40}K was investigated. The characteristics of the high-sensitivity apparatus used are given, and several assemblies using large-volume NaI(Tl) scintillators are described. The relatively light shielding required for natural radioactivity permitted construction of mobile assembly. Conditions of use are described, and the results are given. All gamma emitting elements were measured in 15 min at levels lower than the tolerance dose. Gamma spectroscopy was also used to determine fission products in the earth and to study radioactive elements in the presence of other emitters. (author) [French] La spectrographie gamma du corps humain permet la mesure et la localisation des contaminations internes au niveau des doses de tolerance et, dans certains cas, celle d'activites plus faibles comme la radioactivite naturelle due principalement au potassium 40. Les caracteristiques des appareils a grande sensibilite permettant ces mesures sont exposees et on decrit plusieurs realisations originales utilisant un scintillateur NaI(Tl) de grand volume. L'epaisseur du blindage a ete limitee a 5 cm de plomb, ainsi, pour une protection suffisante contre les rayonnements ambiants, les appareils sont relativement legers et l'une des realisations a pu etre installee dans un laboratoire mobile. Les conditions d'utilisation (mouvement propre, etalonnage) et les resultats obtenus sont donnes; tous les radioelements emetteurs gamma sont mesurables en 15 minutes a un niveau inferieur a la dose de tolerance. On presente enfin des applications a la spectrographie gamma d'echantillons volumineux (poudres ou liquides) et de tres faible activite: elles interessent des domaines tres varies comme, par exemple, la geophysique (etude des retombees radioactives) ou l'industrie chimique (dosage du potassium dans les

Advanced gamma spectrum processing technique applied to the analysis of scattering spectra for determining material thickness

International Nuclear Information System (INIS)

Hoang Duc Tam; VNUHCM-University of Science, Ho Chi Minh City; Huynh Dinh Chuong; Tran Thien Thanh; Vo Hoang Nguyen; Hoang Thi Kieu Trang; Chau Van Tao

2015-01-01

In this work, an advanced gamma spectrum processing technique is applied to analyze experimental scattering spectra for determining the thickness of C45 heat-resistant steel plates. The single scattering peak of scattering spectra is taken as an advantage to measure the intensity of single scattering photons. Based on these results, the thickness of steel plates is determined with a maximum deviation of real thickness and measured thickness of about 4 %. Monte Carlo simulation using MCNP5 code is also performed to cross check the results, which yields a maximum deviation of 2 %. These results strongly confirm the capability of this technique in analyzing gamma scattering spectra, which is a simple, effective and convenient method for determining material thickness. (author)

Self-absorption theory applied to rocket measurements of the nitric oxide (1, 0) gamma band in the daytime thermosphere

Science.gov (United States)

Eparvier, F. G.; Barth, C. A.

1992-01-01

Observations of the UV fluorescent emissions of the NO (1, 0) and (0, 1) gamma bands in the lower-thermospheric dayglow, made with a sounding rocket launched on March 7, 1989 from Poker Flat, Alaska, were analyzed. The resonant (1, 0) gamma band was found to be attenuated below an altitude of about 120 km. A self-absorption model based on Holstein transmission functions was developed for the resonant (1, 0) gamma band under varying conditions of slant column density and temperature and was applied for the conditions of the rocket flight. The results of the model agreed with the measured attenuation of the band, indicating the necessity of including self-absorption theory in the analysis of satellite and rocket limb data of NO.

Nuclear γ-ray spectroscopy of cool free atoms

International Nuclear Information System (INIS)

Rivlin, Lev A

1999-01-01

Consideration is given to the capabilities of gamma-ray spectroscopy of the nuclei of free neutral atoms cooled employing modern laser light-pressure techniques. This spectroscopy is comparable with the Mossbauer spectroscopy in respect of the expected resolving power. (laser applications and other topics in quantum electronics)

Tangential channel for nuclear gamma-resonance spectroscopy in thermal neutron capture

International Nuclear Information System (INIS)

Belogurov, V.N.; Bondars, H.Ya.; Lapenas, A.A.; Reznikov, R.S.; Senkov, P.E.

1979-01-01

Design of a tangential reactor channel which has been made to replace the radial one in the pulsed research reactor IRT-2000 is described. It allows to use the same hole in biological reactor schielding. Characteristics of neutron and gamma-background spectra at the excit of the channel are given and compared with analogous characteristics of the radial one. The gamma background in the tangential channel is lower than in the radial channel. The gamma spectra in the Gd 155 (n, γ)Gd 156 , Gd 157 (n, γ)Gd 158 , Er 167 (n, γ)Er 168 and Hf 177 (n, γ)Hf 178 reactions show that the application of X-ray detection units BDR with the tangential channel allows to carry out the gamma spectrometry of gamma quanta emitted in the thermal neutron capture by both high and low neutron capture cross section nuclei (e.g., Gdsup(157, 155) and Er 167 , Hf 177 , respectively)

Gamma-ray scatter methods applied to industrial measurement systems

Energy Technology Data Exchange (ETDEWEB)

Holstad, Marie Bueie

2004-09-01

Throughout the work presented in this dissertation it has been confirmed that the use of scattered gamma-radiation is a complex but useful tool in industrial measurement science. Scattered radiation has shown to be useful both when traditional measurement principles cannot be used (Chapter 4) and when more information about a system is needed than what is obtained with transmission measurements (Chapter 6). All three main projects (Chapters 4, 5 and 6) confirm that the sensitivity and accuracy of systems based on scattered gamma-radiation depends strongly on the geometry of the setup and that that presence of multiple scattered radiation makes the problems complex. Chapter 4 shows that multiple scattered gamma-radiation can be used for detection of changes in density where the dimensions are too large to use transmitted radiation. There is, however, an upper limit on the thickness of the absorbing medium also when scattered radiation is utilized. As seen in Chapter 5, multiple scattered gamma-radiation can in principle also be used in level gauges with very compact measurement geometries. The main challenges are the sensitivity to interfaces between materials with similar densities and low count rate. These challenges could not be overcome for level measurements in gravitational separator tanks. The results presented in Chapter 6 show that it is feasible to combine transmission and scatter measurements to characterize produced water in the oil and gas industry. (Author)

An application of the coincidence Doppler spectroscopy for substances of chemical interest: phthalocyanine and acetylacetonate complexes

International Nuclear Information System (INIS)

Ito, Y.; Suzuki, T.

2000-01-01

Coincidence Doppler spectroscopy, which is particularly powerful when one is concerned with high momentum components of positron annihilation gamma-rays, has been applied to two different kinds of organo-metallic ligands: metal phthalocyanines and metal acetylacetonates. The energy (momentum) profiles of the annihilation gamma-rays were the same for metal phthalocyanines indicating that positron and/or positronium are not interacting with the metal ions. However, the profiles for the metal acetylacetonates evidently showed a dependence on the kind of metal ions. Discussion is made on the features of positron interaction which are different for phthalocyanines and acetylacetonates.

FTIR spectroscopy as an alternative tool for high gamma dose dosimetry using P(VDF-TrFE) fluorinated copolymers

Energy Technology Data Exchange (ETDEWEB)

Medeiros, Adriana S.; Liz, Otavio S., E-mail: asm@cdtn.b [Universidade Federal de Minas Gerais (DEN/UFMG), Belo Horizonte, MG (Brazil). Dept. de Engenharia Nuclear; Faria, Luiz O., E-mail: farialo@cdtn.b [Centro de Desenvolvimento da Tecnologia Nuclear (CDTN/CNEN-MG), Belo Horizonte, MG (Brazil)

2011-07-01

Poly(vinylidene fluoride) [PVDF] is a semicrystalline homopolymer and some of its fluorinated copolymer has demonstrated to have sensitiveness to high doses of ionizing radiation. We have recently proposed a semicrystalline fluorinated PVDF copolymer, the poly(vinylidene-trifluorethylene) [P(VDF-TrFE], as a candidate for measuring larger dose ranges. In fact, in these copolymers the optical absorption peak at 274 nm has been used to measure gamma doses ranging from 1.0 to 100.0 kGy and the melting latent heat, collected by differential scanning calorimetry (DSC), have been used to measure gamma doses from 1.0 to 1,000.0 kGy. In this paper, the infrared stretching vibration of radio-induced in-chain unsaturations (CH=CF) in P(VDF-TrFE) copolymers has been considered as an alternative tool for high dose dosimetric purposes. FTIR spectroscopic data revealed two optical absorption bands at 1754 cm{sup -1} and 1854 cm{sup -1} whose intensities are unambiguously related to gamma delivered doses ranging from 100.0 kGy to 1,000.0 kGy. Fading was evaluated one month after irradiation. The results indicate that the sample dose evaluation should be performed in the first two hours after being exposed to the radiation beam. The radio-induced formation of unsaturations was also investigated by ultraviolet and visible spectroscopy, which has confirmed the gradual increase of conjugated C=C bonds with the absorbed dose. Our results indicate that quantitative analysis of FTIR absorption bands is a useful tool to perform a product end-point dosimetry in radiation processing facilities that use high gamma dose irradiation. (author)

Gamma-Ray Imaging Spectrometer (GRIS): a new balloon-borne experiment for gamma-ray line astronomy

International Nuclear Information System (INIS)

Teegarden, B.J.; Cline, T.L.; Gehrels, N.; Porreca, G.; Tueller, J.; Leventhal, M.; Huters, A.F.; Maccallum, C.J.; Stang, P.D.; Sandia Labs., Albuquerque, NM)

1985-01-01

High resolution gamma-ray spectroscopy is a relatively new field that holds great promise for further understanding of high energy astrophysical processes. When the high resolution gamma-ray spectrometer (GRSE) was removed from the GRO payload, a balloon program was initiated to permit continued development and improvement of instrumentation in this field, as well as continued scientific observations. The Gamma-Ray Imaging Spectrometer (GRIS) is one of the experiments selected as part of this program. The instrument contains a number of new and innovative features that are expected to produce a significant improvement in source location accuracy and sensitivity over previous balloon and satellite experiments

Standard test method for nondestructive assay of special nuclear material in low density scrap and waste by segmented passive gamma-Ray scanning

CERN Document Server

American Society for Testing and Materials. Philadelphia

2010-01-01

1.1 This test method covers the transmission-corrected nondestructive assay (NDA) of gamma-ray emitting special nuclear materials (SNMs), most commonly 235U, 239Pu, and 241Am, in low-density scrap or waste, packaged in cylindrical containers. The method can also be applied to NDA of other gamma-emitting nuclides including fission products. High-resolution gamma-ray spectroscopy is used to detect and measure the nuclides of interest and to measure and correct for gamma-ray attenuation in a series of horizontal segments (collimated gamma detector views) of the container. Corrections are also made for counting losses occasioned by signal processing limitations (1-3). 1.2 There are currently several systems in use or under development for determining the attenuation corrections for NDA of radioisotopic materials (4-8). A related technique, tomographic gamma-ray scanning (TGS), is not included in this test method (9, 10, 11). 1.2.1 This test method will cover two implementations of the Segmented Gamma Scanning ...

Gamma-ray spectra from the age of the dinosaurs

International Nuclear Information System (INIS)

Johnson, M.W.

1994-01-01

Gamma-ray spectroscopy has been tested as a technique for assisting in the excavation of paleontological sites in the Morrison Formation of western New Mexico. Excavation of these sites is difficult, owing to remoteness and to environmental concerns that militate against wholesale removal of overburden. Various researchers have used remote-sensing techniques to attempt to locate sub-surface bone near known, exposed fossils, thereby to confine excavation to areas where success in finding bone is most likely. Bones accumulate uranium from surrounding rock during fossilization; accordingly, in-situ gamma-ray spectroscopy might serve to locate bone, by detecting the 609- and 1764-keV gamma rays from uranium daughters. Because of the high uranium content of fossils in the Morrison Formation, calculations suggest the feasibility of locating bone despite the presence of several cm of rock and soil overburden. Investigations at several sites with fossils of large sauropods have revealed increased count rates for the key gamma rays near exposed bone, possibly implying the presence of additional fossils beneath the surface of the ground. However, attempts to use spectroscopy inside shafts drilled into possible fossil-bearing rock have been less successful. Results are presented and prospects for additional work discussed

High-sensitivity gamma spectroscopy for extended sources. Application to activity measurements on the human body, on glass, and on soil; Spectrographie gamma a grande sensibilite pour sources etendues. Application a la mesure de l'activite du corps humain, du verre et du sol

Energy Technology Data Exchange (ETDEWEB)

Jouve, B

1962-07-01

The measurement and location by gamma spectroscopy of human body internal contaminations at maximum permissible levels, and, in certain cases, at lower activities such as that due to {sup 40}K was investigated. The characteristics of the high-sensitivity apparatus used are given, and several assemblies using large-volume NaI(Tl) scintillators are described. The relatively light shielding required for natural radioactivity permitted construction of mobile assembly. Conditions of use are described, and the results are given. All gamma emitting elements were measured in 15 min at levels lower than the tolerance dose. Gamma spectroscopy was also used to determine fission products in the earth and to study radioactive elements in the presence of other emitters. (author) [French] La spectrographie gamma du corps humain permet la mesure et la localisation des contaminations internes au niveau des doses de tolerance et, dans certains cas, celle d'activites plus faibles comme la radioactivite naturelle due principalement au potassium 40. Les caracteristiques des appareils a grande sensibilite permettant ces mesures sont exposees et on decrit plusieurs realisations originales utilisant un scintillateur NaI(Tl) de grand volume. L'epaisseur du blindage a ete limitee a 5 cm de plomb, ainsi, pour une protection suffisante contre les rayonnements ambiants, les appareils sont relativement legers et l'une des realisations a pu etre installee dans un laboratoire mobile. Les conditions d'utilisation (mouvement propre, etalonnage) et les resultats obtenus sont donnes; tous les radioelements emetteurs gamma sont mesurables en 15 minutes a un niveau inferieur a la dose de tolerance. On presente enfin des applications a la spectrographie gamma d'echantillons volumineux (poudres ou liquides) et de tres faible activite: elles interessent des domaines tres varies comme, par exemple, la geophysique (etude des retombees radioactives) ou l'industrie chimique

Bismuth- and lithium-loaded plastic scintillators for gamma and neutron detection

International Nuclear Information System (INIS)

Cherepy, Nerine J.; Sanner, Robert D.; Beck, Patrick R.; Swanberg, Erik L.; Tillotson, Thomas M.; Payne, Stephen A.; Hurlbut, Charles R.

2015-01-01

Transparent plastic scintillators based on polyvinyltoluene (PVT) have been fabricated with high loading of bismuth carboxylates for gamma spectroscopy, and with lithium carboxylates for neutron detection. When activated with a combination of standard fluors, 2,5-diphenyloxazole (PPO) and tetraphenylbutadiene (TPB), gamma light yields with 15 wt% bismuth tripivalate of 5000 Ph/MeV are measured. A PVT plastic formulation including 30 wt% lithium pivalate and 30 wt% PPO offers both pulse shape discrimination, and a neutron capture peak at ~400 keVee. In another configuration, a bismuth-loaded PVT plastic is coated with ZnS( 6 Li) paint, permitting simultaneous gamma and neutron detection via pulse shape discrimination with a figure-of-merit of 3.8, while offering gamma spectroscopy with energy resolution of R(662 keV)=15%

Comparisons between digital gamma-ray spectrometer (DSPec) and standard nuclear instrumentation methods (NIM) systems

International Nuclear Information System (INIS)

Vo, D.T.; Russo, P.A.; Sampson, T.E.

1998-03-01

Safeguards isotopic measurements require the best spectrometer systems with excellent resolution, stability and throughput. Up until about a year ago, gamma ray spectroscopy has always been done using the analog amplifier, which processes the pulses from the preamplifier to remove the noise, reject the pile up signals, and shape the signals into some desirable form before sending them to the analog to digital converter (ADC) to be digitized. In late 1996, EG and G Ortec introduced a digital gamma ray spectrometer (DSPec) which uses digital technology to analyze the preamplifiers' pulses from all types of germanium and silicon detectors. Considering its performance, digital based spectroscopy may become the way of future gamma ray spectroscopy

Determination of Ethanol in Blood Samples Using Partial Least Square Regression Applied to Surface Enhanced Raman Spectroscopy.

Science.gov (United States)

Açikgöz, Güneş; Hamamci, Berna; Yildiz, Abdulkadir

2018-04-01

Alcohol consumption triggers toxic effect to organs and tissues in the human body. The risks are essentially thought to be related to ethanol content in alcoholic beverages. The identification of ethanol in blood samples requires rapid, minimal sample handling, and non-destructive analysis, such as Raman Spectroscopy. This study aims to apply Raman Spectroscopy for identification of ethanol in blood samples. Silver nanoparticles were synthesized to obtain Surface Enhanced Raman Spectroscopy (SERS) spectra of blood samples. The SERS spectra were used for Partial Least Square (PLS) for determining ethanol quantitatively. To apply PLS method, 920~820 cm -1 band interval was chosen and the spectral changes of the observed concentrations statistically associated with each other. The blood samples were examined according to this model and the quantity of ethanol was determined as that: first a calibration method was established. A strong relationship was observed between known concentration values and the values obtained by PLS method (R 2 = 1). Second instead of then, quantities of ethanol in 40 blood samples were predicted according to the calibration method. Quantitative analysis of the ethanol in the blood was done by analyzing the data obtained by Raman spectroscopy and the PLS method.

High rate gamma spectroscopy system for activation analysis of short-lived isomeric transitions

Energy Technology Data Exchange (ETDEWEB)

Westphall, G P [Atominstitut der Oesterreichischen Hochschulen, Vienna

1976-07-15

A high rate spectroscopy system specially suited for measurement of short-lived isomeric transitions is described, which, as part of a fast activation analysis facility at the TRIGA Mark II reactor, provides for automatic recording and immediate evaluation of gamma spectra taken from nuclides activated at stationary or pulsed reactor power. The system consists of a commercial de-coupled Ge(Li)-detector of 70 cm/sup 3/ modified for recycling operation for input rates in excess of 500000 c/s /sup 60/Co, a time variant trapezoidal shaping section and a fast constant dead-time ADC coupled to a programmed multichannel analyzer. Novel circuits for efficient pile-up rejection and time variant base line restoration extend the concept of gated integration up to count rates of more than 200000 c/s /sup 60/Co. Time-sequenced recording of spectra is performed by a minicomputer operated as a front-end processor of a larger laboratory computer, where final data processing takes place. New concepts for very simple and cost-effective implementation of multichannel analyzers by means of general purpose small computers are described.

Photon Activation Analysis Of Light Elements Using 'Non-Gamma' Radiation Spectroscopy - The Instrumental Determination Of Phosphorus

International Nuclear Information System (INIS)

Segebade, Christian; Goerner, Wolf

2011-01-01

Unlike metal determinations the analysis of light elements (e.g., carbon, oxygen, phosphorus) is frequently problematic, in particular if analysed instrumentally. In photon activation analysis (PAA) the respective activation products do not emit gamma radiation in the most cases. Usually, annihilation quanta counting and subsequent decay curve analysis have been used for determinations of C, N, O, and F. However, radiochemical separation of the respective radioisotopes mostly is indispensable. For several reasons, some of the light elements cannot be analysed following this procedure, e.g. phosphorus. In this contribution the instrumental PAA of phosphorus in organic matrix by activation with bremsstrahlung of an electron linear accelerator and subsequent beta spectroscopy is described. The accuracy of the results was excellent as obtained by analysis of a BCR Reference Material.

New enhanced sensitivity infrared laser spectroscopy techniques applied to reactive plasmas and trace gas detection

NARCIS (Netherlands)

Welzel, S.

2009-01-01

Infrared laser absorption spectroscopy (IRLAS) employing both tuneable diode and quantum cascade lasers (TDLs, QCLs) has been applied with both high sensitivity and high time resolution to plasma diagnostics and trace gas measurements. TDLAS combined with a conventional White type multiple pass cell

Evaluation of gamma spectroscopy gauge for uranium-plutonium assay

International Nuclear Information System (INIS)

Notea, A.; Segal, Y.

1975-01-01

A procedure is presented for the characterization of a gamma passive method for nondestructive analysis of nuclear fuel. The approach provides an organized and systematic way for optimizing the assay system. The key function is the relative resolving power defined as the smallest relative change in the Quantity of radionuclide measured, that may be detected within a certain confidence level. This function is derived for nuclear fuel employing a model based on empirical parameters. The ability to detect changes in fuels of binary and trinary compositions with a 50 cc Ge(Li) at a 1 min counting period is discussed. As an example to a binary composition, an enriched uranium fuel was considered. The 185 keV and 1001 keV gamma lines are used for the assay of 235 U and 238 U respectively. As a trinary composition a plutonium-containing gamma line. The interference of the high energy lines is carefully analyzed, and numerical results are presented. For both cases the range of measurement under specific accuracy demands is determined. The approach described is suitable also for evaluation of other passive as well as active assay methods. (author)

Gamma-radiography techniques applied to quality control of welds in water pipe lines

International Nuclear Information System (INIS)

Sanchez, W.; Oki, H.

1974-01-01

Non-destructive testing of welds may be done by the gamma-radiography technique, in order to detect the presence or absence of discontinuities and defects in the bulk of deposited metal and near the base metal. Gamma-radiography allows the documentation of the test with a complete inspection record, which is a fact not common in other non-destructive testing methods. In the quality control of longitudinal or transversal welds in water pipe lines, two exposition techniques are used: double wall and panoramic exposition. Three different water pipe lines systems have analysed for weld defects, giving a total of 16,000 gamma-radiographies. The tests were made according to the criteria established by the ASME standard. The principal metallic discontinuites found in the weld were: porosity (32%), lack of penetration (29%), lack of fusion (20%), and slag inclusion (19%). The percentage of gamma-radiographies showing welds without defects was 39% (6168 gamma-radiographies). On the other hand, 53% (8502 gamma-radiographies) showed the presence of acceptable discontinuities and 8% (1330 gamma-radiographies) were rejected according to the ASME standards [pt

ZnO Luminescence and scintillation studied via photoexcitation, X-ray excitation, and gamma-induced positron spectroscopy

Science.gov (United States)

Ji, J.; Colosimo, A. M.; Anwand, W.; Boatner, L. A.; Wagner, A.; Stepanov, P. S.; Trinh, T. T.; Liedke, M. O.; Krause-Rehberg, R.; Cowan, T. E.; Selim, F. A.

2016-08-01

The luminescence and scintillation properties of ZnO single crystals were studied by photoluminescence and X-ray-induced luminescence (XRIL) techniques. XRIL allowed a direct comparison to be made between the near-band emission (NBE) and trap emissions providing insight into the carrier recombination efficiency in the ZnO crystals. It also provided bulk luminescence measurements that were not affected by surface states. The origin of a green emission, the dominant trap emission in ZnO, was then investigated by gamma-induced positron spectroscopy (GIPS) - a unique defect spectroscopy method that enables positron lifetime measurements to be made for a sample without contributions from positron annihilation in the source materials. The measurements showed a single positron decay curve with a 175 ps lifetime component that was attributed to Zn vacancies passivated by hydrogen. Both oxygen vacancies and hydrogen-decorated Zn vacancies were suggested to contribute to the green emission. By combining scintillation measurements with XRIL, the fast scintillation in ZnO crystals was found to be strongly correlated with the ratio between the defect luminescence and NBE. This study reports the first application of GIPS to semiconductors, and it reveals the great benefits of the XRIL technique for the study of emission and scintillation properties of materials.

Development of gamma spectrometer using silicon photomultiplier (SiPM)

International Nuclear Information System (INIS)

Kim, Chan Kyu

2011-02-01

Gamma spectroscopy is used to determine the identity and quantity of gamma-emitters in nuclear physics, geochemistry and astrophysics. The scintillation detectors are being used as a gamma spectrometer generally, because of their higher gamma-ray detection efficiency and cheaper price than germanium semi-conductor detectors. A typical scintillation detector is composed of a scintillator, a window, and a photodetector. The photomultiplier (PM) tube has been the most widely used as a photodetector because of its advantages like high sensitivity, high signal-to-noise ratio, and wide dynamic range. Recently, the Silicon Photomultiplier (SiPM) is being studied as a substitute of PM tube. The SiPM has almost same performance compared to PM tube but it has additional advantages; low operating voltage, small volume, and cheap production cost. In this research, the gamma spectrometer using SiPM instead of PM tube is developed. The use of SiPM as a photodetector makes the gamma spectrometer smaller, cheaper, easier to use. For photon transport and collection from the large area scintillator to the small area SiPM, a light guide is applied in this gamma spectrometer system. Before fabrication of light guide, DETECT simulation is performed to study and prospect characteristics of light guide structure. And actual light guides are fabricated on the basis of this simulation result. Poly(methyl methacrylate) (PMMA) is chosen as material of light guide, 5 sample light guides are fabricated in different lengths and coatings. As a scintillator crystal, same NaI(Tl) crystal is chosen. For measurement and analysis of gamma spectrometer system, 3 gamma spectrometer systems are composed: PM tube-based system, PM tube-based system with the light guide, SiPM-based system with the light guide. Through comparison between the results of each gamma spectrometer, the performances of gamma spectrometer system are analyzed by each component. Measurement results of the second system is well

Studies of. gamma. -ray irradiation effects on tris(. beta. -diketonato)iron(III) and cobalt(III) coordination compounds by means of Moessbauer spectroscopy and magnetic susceptibility measurements

Energy Technology Data Exchange (ETDEWEB)

Sakai, Y.; Endo, K.; Sano, H. (Tokyo Metropolitan Univ. (Japan). Faculty of Science)

1981-06-01

Both absorption Moessbauer spectroscopy and magnetic susceptibility measurements on tris(..beta..-diketonato)iron(III) and cobalt(III) compounds indicate that ligands which have phenyl group as a substituent are more stable to ..gamma..-ray radiolysis, in accordance with previous results of emission Moessbauer spectroscopic studies of /sup 57/Co-labelled tris (..beta..-diketonato)cobalt(III) compounds.

7T Proton Magnetic Resonance Spectroscopy of Gamma-Aminobutyric Acid, Glutamate, and Glutamine Reveals Altered Concentrations in Patients With Schizophrenia and Healthy Siblings

DEFF Research Database (Denmark)

Thakkar, Katharine N; Rösler, Lara; Wijnen, Jannie P

2017-01-01

BACKGROUND: The N-methyl-D-aspartate receptor hypofunction model of schizophrenia predicts dysfunction in both glutamatergic and gamma-aminobutyric acidergic (GABAergic) transmission. We addressed this hypothesis by measuring GABA, glutamate, glutamine, and the sum of glutamine plus glutamate...... concentrations in vivo in patients with schizophrenia using proton magnetic resonance spectroscopy at 7T, which allows separation of metabolites that would otherwise overlap at lower field strengths. In addition, we investigated whether altered levels of GABA, glutamate, glutamine, and the sum of glutamine plus...... glutamate reflect genetic vulnerability to schizophrenia by including healthy first-degree relatives. METHODS: Proton magnetic resonance spectroscopy at 7T was performed in 21 patients with chronic schizophrenia who were taking medication, 23 healthy first-degree relatives of patients with schizophrenia...

Development of a low-level setup for gamma spectroscopy: Application for nuclear astrophysics using reverse kinematics

International Nuclear Information System (INIS)

Genard, G.; Nuttens, V.E.; Bouchat, V.; Terwagne, G.

2010-01-01

It is more and more necessary to improve the sensitivity of gamma-ray spectroscopy systems, especially in nuclear astrophysics. In the case of radiative proton capture reactions, one means is to avoid the reactions on the target impurities by using reverse kinematics. This technique is possible with the LARN accelerator and can provide very clean cross-section measurements. For that purpose, a hydrogen standard has been carried out by means of ion implantation in silicon. In addition, a low-level setup has been put in place on a new beam line of the accelerator. A high efficiency and high resolution germanium detector is used conjointly with a double shielding. A passive lead castle shielding system is used to reduce the natural radioactivity and an active shielding consisting of an anti-cosmic veto is provided by an anticoincidence between the plastic scintillator and the gamma-ray detector. The setup allows a reduction of 70% of the background interference and provides an approximately 200 fold sensitivity gain of between 600 and 3000 keV. Some other developments have also been carried out to optimize the setup. The entire setup and the reverse kinematics have been validated by measuring the cross-section of the 13 C(p,γ) 14 N and 15 N(p,γ) 16 O reactions that present some astrophysical interest.

Innovative Applications of In Situ Gamma Spectroscopy for Non-destructive Assay of Transuranic Wastes

International Nuclear Information System (INIS)

Watters, D.J.; Weismann, J.J.; Duke, S.J.; Nicosia, W.C.

2009-01-01

Cabrera Services (CABRERA), under contract to National Security Technologies, LLC (NSTec), supported the transuranic (TRU) waste reduction initiative at the Radioactive Waste Management Complex of the Nevada Test Site (NTS). CABRERA developed advanced NDA techniques for oversized boxes (OSB) and drums using in situ gamma spectroscopy during several phases of the project. A more thorough characterization method was employed during the planning phase of the project to better understand the TRU content and distribution within each container, while a comprehensive NDA program was designed and implemented during the intrusive phase that guided waste segregation and re-packaging of both TRU and low-level wastes (LLW). NSTec took receipt of 58 oversized boxes of suspect TRU waste from Lawrence Livermore National Lab (LLNL). TRU waste is defined as greater than 3.7 kilobecquerels per gram [kBq/g] (100 nanocuries (nCi)/g) activity from alpha-emitting radionuclides with atomic number greater than 92 having a half-life greater than 20 years. Each box was custom-made to house a variety of suspect TRU wastes resulting from years of weapons program research, development, and testing. Since their arrival at NTS, the boxes have undergone several iterations of non-destructive assay (NDA) in preparation for the comprehensive repackaging effort. NDA has included two rounds of in situ gamma spectroscopy and real-time radiography (RTR) scans that were videotaped. Contents have been confirmed to include glove boxes, HEPA filters and their housings, and assorted process equipment and piping. TRU content was determined via directly measuring plutonium-239 (Pu-239), americium-241 (Am-241), and other radionuclides, while adding calculated results for non-measurable nuclides using reliable scaling factors developed from acceptable knowledge (AK). Advantages of CABRERA's NDA methods included: - More NDA information is available in the same amount of counting time, allowing NSTec to make more

Anthracene as a Non-hygroscopic Diluting Agent for Moessbauer Spectroscopy of Silicate Samples in Moisture-Uptake Studies

International Nuclear Information System (INIS)

Hoffman, E. J.; Bickraj, K.; Denalli, C.

2004-01-01

Anthracene gained no mass when held in a humid chamber and showed no gamma absorption and so appears to be suitable as a replacement for sugars for dilution of moisture-sensitive 57 Fe-Moessbauer spectroscopy samples. Applied to studies of moisture effects on a circumstellar silicate dust simulant, anthracene permitted preparation of sample series for experimental determination of optimal 57 Fe-Moessbauer areal density.

Prototype of an expert system to help nuclide identification in gamma spectrum analysis

International Nuclear Information System (INIS)

Jayanthi, Kasi Annapurna; Corcuera, Raquel Paviotti; Oliveira, Gina Maira B.

1995-01-01

This report describes the development and use of IDENT, prototype of an expert system that helps the researcher to identify radionuclides in gamma-ray spectroscopy. Normally the method adopted by the researcher is iterative, time consuming and becomes complicated in the analysis of large and complex gamma-ray spectra. The present expert system is based on the knowledge transmitted by expert and specialists in this area and the results show that it is helpful for researches who perform nuclide identification through gamma-ray spectroscopy. The gamma-ray spectrum of a material sample with about 140 peaks would take about a week or two be analysed by a specialist. The same task can be done in a few minutes using this expert system. (author). 14 refs., 2 figs

The effect of gamma ray irradiation on PAN-based intermediate modulus carbon fibers

International Nuclear Information System (INIS)

Li, Bin; Feng, Yi; Qian, Gang; Zhang, Jingcheng; Zhuang, Zhong; Wang, Xianping

2013-01-01

Raman spectroscopy, X-ray photoelectron spectroscopy (XPS), X-ray diffraction (XRD) and field emission scanning electron microscopy (FESEM) were conducted on PAN-based intermediate modulus carbon fibers to investigate the structure and surface hydrophilicity of the carbon fibers before and after gamma irradiation. Two methods were used to determine Young’s modulus of the carbon fibers. The results show that gamma ray irradiation improved the degree of graphitization and introduced compressive stress into carbon fiber surface. Gamma ray also improved the carbon fiber surface hydrophilicity through increasing the value of O/C and enhancing the quantity of oxygen functional groups on carbon fibers. No distinct morphology change was observed after gamma ray irradiation. The Young’s modulus of the fibers increased with increasing irradiation dose

Opto-structural characterization of gamma irradiated Bayfol polymer track detector

Energy Technology Data Exchange (ETDEWEB)

Tayel, A. [Physics Department, Faculty of Industrial Education, Helwan University, Cairo (Egypt); Zaki, M.F., E-mail: moha1016@yahoo.com [Experimental Nuclear Physics Department, Nuclear Research Center, Atomic Energy Authority, P.O. 13759, Abu Zaabal, Cairo (Egypt); El Basaty, A.B. [Physics Department, Faculty of Industrial Education, Helwan University, Cairo (Egypt); Hegazy, Tarek M. [Physics Department, College of Women for Arts, Science and Education, Ain Shams University, Cairo (Egypt)

2013-11-15

Bayfol CR 1-4 is one of polymeric solid state nuclear track detector which has numerous applications due to its outstanding optical, mechanical, thermal and electrical properties. In the present study, Bayfol polymer is irradiated with different doses of gamma rays ranging from 0 to 1000 KGy. The effects of gamma irradiations on the optical, structural and chemical properties of Bayfol were studied using Ultraviolet and visible (UV/Vis) spectroscopy, X-ray diffraction (XRD) and Fourier transform infrared (FTIR) spectroscopy. The UV–Vis spectra of irradiated samples show that the absorption edge is shifted towards longer wavelength comparing to pristine sample spectrum. This behavior indicates that there is a decrease in the band gap after irradiation. The maximum decrease in the band gap is about 0.8 eV. The XRD patterns of amorphous halo of pristine and irradiated samples show a fluctuation of integrated intensity of amorphous halo. This indicates a change in the structure due to gamma irradiation. In order to understand that structure change mechanism, we used the FTIR spectroscopy.

Permitting of the accuracy in location of tumours and the accuracy in applying a precise dose covering in stereotactic gamma-knife treatments

International Nuclear Information System (INIS)

Ertl, A. G.

1997-01-01

The gamma-knife is a Co-60 irradiation device, permitting the location of a lesion with an accuracy of millimeters. Moreover, with the Gamma Knife it is possible to apply a precise dose covering the entire area inside the head. In order to visualize a lesion, we mostly have to resort to imaging techniques such as the MR tomography. The accuracy of locating the specific area for the stereotactic treatment was achieved with the help of a special screen plate which we designed ourselves. For determining the precise dose to be applied at the Gamma Knife, the central dose for all four collimator helmets as well as the dose distribution of the combined collimators had to be measured. In case of irradiations in prone position there may be considerable deviations compared to the dose-planning program; this we were able to demonstrate by a TLD array designed by ourselves. A more sophisticated evaluation of new dosimetry techniques - GafChromic films and BANG polymer gel - enabled us to investigate more complex irradiation patterns. (author)

Application of airborne gamma-ray spectrometry in soil/regolith mapping and applied geomorphology

International Nuclear Information System (INIS)

Wilford, J.R.; Bierwirth, P.N.; Craig, M.A.

1997-01-01

Gamma-ray spectrometric surveys are an important source of information for soil, regolith and geomorphological studies, as demonstrated by the interpretation of airborne surveys in Western Australia, central New South Wales and north Queensland. Gamma-rays emitted from the ground surface relate to the primary mineralogy and geochemistry of the bedrock, and the secondary weathered materials. Weathering modifies the distribution and concentration of radioelements from the original bedrock source. Once the radioelement response of bedrock and weathered materials is understood, the gamma-ray data can provide information on geomorphic processes and soil/regolith properties, including their mineralogy, texture, chemistry and style of weathering. This information can contribute significantly to an understanding of the weathering and geomorphic history of a region and, therefore, has the potential to be used in developing more effective land-management strategies and refining geochemical models in support of mineral exploration. Gamma-ray imagery is enhanced when combined with Landsat TM bands and digital elevation models (DEM). This synergy enables geochemical information derived from the gamma-ray data to be interpreted within a geomorphic framework. Draping gamma-ray images over DEMs as 3D landscape perspective views aids interpretation and allows the interpreter to visualise complex relationships between the gamma-ray response and landform features. 44 refs.,1 tab., 11 figs

Application of high resolution NMR, ESR, and gamma-ray scintillation spectroscopy to the study of ligand binding in proteins

International Nuclear Information System (INIS)

Lancione, G.V.

1982-01-01

Electron spin resonance spectroscopy has been employed to study the nature of the ligand binding site of alpha-1-antitrypsin. Spectra of spin-labeled alpha-1-antitrypsin were recorded at pH's ranging from 2.4 to 12.5. This data demonstrates the tight binding of the spin-label to the protease, and the sensitivity of the bound spin-label to informational changes in the protease inhibitor. A molecular dipstick approach has also been applied to this system and has yielded information on the geometry of the cleft accommodating the spin-label. 160 Terbium(III) exchange experiments have been performed on the acetylcholine receptor protein isolated from Torpedo californica, employing a specially designed flow dialysis apparatus constructed in the laboratory. The apparatus is designed to allow continuous monitoring of 160 Tb(III) gamma-ray emission from the protein compartment of the flow dialysis cell. Nicotinic ligand-induced displacement of 160 Tb(III) from the nicotinic binding site of the receptor was monitored as a funtion of (1) the concentration of nicotinic ligand in the washout buffer, and (2) the nature of the nicotinic ligand in the buffer. Measured 160 Tb(III) exchange half-lives indicate (1) a direct relationship between 160 Tb(III) displacement and nicotinic ligand concentration in the wash-out buffer, and (2) an enhanced 160 Tb(III) displacement for nicotinic agents possessing quaternary ammonium functions

COMPLIS: COllinear spectroscopy Measurements using a Pulsed Laser Ion Source

CERN Multimedia

2002-01-01

A Pulsed Laser spectroscopy experiment has been installed for the study of hyperfine structure and isotope shift of refractory and daughter elements from ISOLDE beams. It includes decelerated ion-implantation, element-selective laser ionization, magnetic and time-of-flight mass separation. The laser spectroscopy has been performed on the desorbed atoms in a set-up at ISOLDE-3 but later on high resolution laser collinear spectroscopy with the secondary pulsed ion beam is planned for the Booster ISOLDE set-up. During the first operation time of ISOLDE-3 we restricted our experiments to Doppler-limited resonant ionization laser and $\\gamma$-$\\gamma$ nuclear spectroscopy on neutron deficient platinum isotopes of even mass number down to A~=~186 and A~=~179 respectively. These isotopes have been produced by implantation of radioactive Hg and their subsequent $\\beta$-decay.

Gamma spectrometry of infinite 4Π geometry

International Nuclear Information System (INIS)

Nordemann, D.J.R.

1987-07-01

Owing to the weak absorption og gamma radiation by matter, gamma-ray spectrometry may be applied to samples of great volume. A very interesting case is that of the gamma-ray spectrometry applied with 4Π geometry around the detector on a sample assumed to be of infinite extension. The determination of suitable efficiencies allows this method to be quantitative. (author) [pt

Sixth symposium on x- and gamma ray sources and applications. Abstracts

International Nuclear Information System (INIS)

1985-01-01

Abstracts are provided for technical presentations in the areas of: gamma and x-ray sources, kinds of detectors, characterization of detectors and detector systems, models and data analysis, gamma spectroscopy, instrumentation, x-ray fluorescence, tomography, x-ray absorption, and pion induced x-ray emission

Gamma-ray burst spectra

International Nuclear Information System (INIS)

Teegarden, B.J.

1982-01-01

A review of recent results in gamma-ray burst spectroscopy is given. Particular attention is paid to the recent discovery of emission and absorption features in the burst spectra. These lines represent the strongest evidence to date that gamma-ray bursts originate on or near neutron stars. Line parameters give information on the temperature, magnetic field and possibly the gravitational potential of the neutron star. The behavior of the continuum spectrum is also discussed. A remarkably good fit to nearly all bursts is obtained with a thermal-bremsstrahlung-like continuum. Significant evolution is observed of both the continuum and line features within most events

Environmental monitoring with in-situ gamma spectrometer; Umweltueberwachung mit in-situ-Gamma-Spektrometer

Energy Technology Data Exchange (ETDEWEB)

Reinhardt, S. [ENVINET GmbH, Haar (Germany)

2014-01-20

The in-situ gamma spectroscopy allows large area and continuous monitoring of the radio nuclides and there composition in the environment. In comparison to the gamma dose rate measurement the additional spectral information gives the possibility for a quick and effective action in the case of a man-made radiation exposition in the environment. The knowledge respectively localization of the possible nuclides, which a responsible for the increased dose rate, supports responsible organization in the quick identification of the situation, definition of the actions and tracking of the temporal and local process of the radiation exposition. Due to dedicate actions the risk for people and environment is reduced.

Gamma-Ray Background Variability in Mobile Detectors

Science.gov (United States)

Aucott, Timothy John

Gamma-ray background radiation significantly reduces detection sensitivity when searching for radioactive sources in the field, such as in wide-area searches for homeland security applications. Mobile detector systems in particular must contend with a variable background that is not necessarily known or even measurable a priori. This work will present measurements of the spatial and temporal variability of the background, with the goal of merging gamma-ray detection, spectroscopy, and imaging with contextual information--a "nuclear street view" of the ubiquitous background radiation. The gamma-ray background originates from a variety of sources, both natural and anthropogenic. The dominant sources in the field are the primordial isotopes potassium-40, uranium-238, and thorium-232, as well as their decay daughters. In addition to the natural background, many artificially-created isotopes are used for industrial or medical purposes, and contamination from fission products can be found in many environments. Regardless of origin, these backgrounds will reduce detection sensitivity by adding both statistical as well as systematic uncertainty. In particular, large detector arrays will be limited by the systematic uncertainty in the background and will suffer from a high rate of false alarms. The goal of this work is to provide a comprehensive characterization of the gamma-ray background and its variability in order to improve detection sensitivity and evaluate the performance of mobile detectors in the field. Large quantities of data are measured in order to study their performance at very low false alarm rates. Two different approaches, spectroscopy and imaging, are compared in a controlled study in the presence of this measured background. Furthermore, there is additional information that can be gained by correlating the gamma-ray data with contextual data streams (such as cameras and global positioning systems) in order to reduce the variability in the background

Delayed Gamma-Ray Spectroscopy for Non-Destructive Assay of Nuclear Materials

Energy Technology Data Exchange (ETDEWEB)

Ludewigt, Bernhard [Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States); Mozin, Vladimir [Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States); Campbell, Luke [Pacific Northwest National Lab. (PNNL), Richland, WA (United States); Favalli, Andrea [Los Alamos National Lab. (LANL), Los Alamos, NM (United States); Hunt, Alan W. [Iowa State Univ., Ames, IA (United States); Reedy, Edward T.E. [Iowa State Univ., Ames, IA (United States); Seipel, Heather A. [Iowa State Univ., Ames, IA (United States)

2015-09-28

This project has been a collaborative effort of researchers from four National Laboratories, Lawrence Berkley National Laboratory (LBNL), Lawrence Livermore National Laboratory (LLNL), Los Alamos National Laboratory (LANL), Pacific Northwest National Laboratory (PNNL), and Idaho State University’s (ISU) Idaho Accelerator Center (IAC). Experimental measurements at the Oregon State University (OSU) were also supported. The research included two key components, a strong experimental campaign to characterize the delayed gamma-ray signatures of the isotopes of interests and of combined targets, and a closely linked modeling effort to assess system designs and applications. Experimental measurements were performed to evaluate fission fragment yields, to test methods for determining isotopic fractions, and to benchmark the modeling code package. Detailed signature knowledge is essential for analyzing the capabilities of the delayed gamma technique, optimizing measurement parameters, and specifying neutron source and gamma-ray detection system requirements. The research was divided into three tasks: experimental measurements, characterization of fission yields, and development of analysis methods (task 1), modeling in support of experiment design and analysis and for the assessment of applications (task 2), and high-rate gamma-ray detector studies (task 3).

Parallel processing method for high-speed real time digital pulse processing for gamma-ray spectroscopy

International Nuclear Information System (INIS)

Fernandes, A.M.; Pereira, R.C.; Sousa, J.; Neto, A.; Carvalho, P.; Batista, A.J.N.; Carvalho, B.B.; Varandas, C.A.F.; Tardocchi, M.; Gorini, G.

2010-01-01

A new data acquisition (DAQ) system was developed to fulfil the requirements of the gamma-ray spectrometer (GRS) JET-EP2 (joint European Torus enhancement project 2), providing high-resolution spectroscopy at very high-count rate (up to few MHz). The system is based on the Advanced Telecommunications Computing Architecture TM (ATCA TM ) and includes a transient record (TR) module with 8 channels of 14 bits resolution at 400 MSamples/s (MSPS) sampling rate, 4 GB of local memory, and 2 field programmable gate array (FPGA) able to perform real time algorithms for data reduction and digital pulse processing. Although at 400 MSPS only fast programmable devices such as FPGAs can be used either for data processing and data transfer, FPGA resources also present speed limitation at some specific tasks, leading to an unavoidable data lost when demanding algorithms are applied. To overcome this problem and foreseeing an increase of the algorithm complexity, a new digital parallel filter was developed, aiming to perform real time pulse processing in the FPGAs of the TR module at the presented sampling rate. The filter is based on the conventional digital time-invariant trapezoidal shaper operating with parallelized data while performing pulse height analysis (PHA) and pile up rejection (PUR). The incoming sampled data is successively parallelized and fed into the processing algorithm block at one fourth of the sampling rate. The following data processing and data transfer is also performed at one fourth of the sampling rate. The algorithm based on data parallelization technique was implemented and tested at JET facilities, where a spectrum was obtained. Attending to the observed results, the PHA algorithm will be improved by implementing the pulse pile up discrimination.

Achieving Higher Accuracy in the Gamma-Ray Spectrocopic Assay of Holdup

International Nuclear Information System (INIS)

Russo, P.A.; Wenz, T.R.; Smith, S.E.; Harris, J.F.

2000-01-01

Gamma-ray spectroscopy is an important technique for the measurement of quantities of nuclear material holdup in processing equipment. Because the equipment in large facilities dedicated to uranium isotopic enrichment, uranium/plutonium scrap recovery or various stages of fuel fabrication is extensive, the total holdup may be large by its distribution alone, even if deposit thicknesses are small. Good accountability practices require unbiased measurements with uncertainties that are as small as possible. This paper describes new procedures for use with traditional holdup analysis methods based on gamma-ray spectroscopy. The procedures address the two sources of bias inherent in traditional gamma-ray measurements of holdup. Holdup measurements are performed with collimated, shielded gamma-ray detectors. The measurement distance is chosen to simplify the deposit geometry to that of a point, line or area. The quantitative holdup result is based on the net count rate of a representative gamma ray. This rate is corrected for contributions from room background and for attenuation by the process equipment. Traditional holdup measurements assume that the width of the point or line deposit is very small compared to the measurement distance, and that the self-attenuation effects can be neglected. Because each point or line deposit has a finite width and because self-attenuation affects all measurements, bias is incurred in both assumptions. In both cases the bias is negative, explaining the systematically low results of gamma-ray holdup measurements. The new procedures correct for bias that arises from both the finite-source effects and the gamma-ray self-attenuation. The procedures used to correct for both of these effects apply to the generalized geometries. One common empirical parameter is used for both corrections. It self-consistently limits the total error incurred (from uncertain knowledge of this parameter) in the combined correction process, so that it is

Gamma-Ray Imager With High Spatial And Spectral Resolution

Science.gov (United States)

Callas, John L.; Varnell, Larry S.; Wheaton, William A.; Mahoney, William A.

1996-01-01

Gamma-ray instrument developed to enable both two-dimensional imaging at relatively high spatial resolution and spectroscopy at fractional-photon-energy resolution of about 10 to the negative 3rd power in photon-energy range from 10 keV to greater than 10 MeV. In its spectroscopic aspect, instrument enables identification of both narrow and weak gamma-ray spectral peaks.

Gamma-Ray Instrument for Polarimetry, Spectroscopy and Imaging (GIPSI)

National Research Council Canada - National Science Library

Kroeger, R. A; Johnson, W. N; Kinzer, R. L; Kurfess, J. D; Inderhees, S. E; Phlips, B. F; Graham, B. L

1996-01-01

.... Gamma-ray polarimetry in the energy band around 60-300 keV is an interesting area of high energy astrophysics where observations have not been possible with the technologies employed in current and past space missions...

Gamma-spectrometry of extended sources for analysing environmental samples

International Nuclear Information System (INIS)

Jarosievitz, B.

1996-01-01

Measurements of the environmental activity concentration by gamma spectrometers require the determination of the full-energy-peak efficiency as a function of photon energy over the detector range. This can be done by experiments or by calculation. For simple cases, experiments are straightforward, but if the decay scheme is complex, cascade effects modify detection efficiency. Also, actual detection efficiency depends on the detection geometry. All these effects are treated as corrections or modifications of the simple value cases which are especially relevant when applied to large volume of environmental samples. In this thesis calculations are made, using the GEANT MC program, for realistic experimental situations that have been performed, and these calculations are validated. The calculational and experimental results have been compared, and if it proves to be satisfactory, the results can be relied on even for cases when no direct experimental observation is possible. The general problems of gamma spectroscopy and correction problems are discussed. The two main tools, the experimental setup and the simulation program are described. A careful checking of the simulation results and the consequences are presented. (R.P.)

General Remarks about mossbauer spectroscopy

International Nuclear Information System (INIS)

Mirzababayev, R.M.

2001-01-01

More than forty years have passed since the discovery of Mossbauer effect; one of the most brilliant findings in modern physics. This effect proved itself to be the powerful tool in almost all disciplines of the natural sciences and technology. Its unique feature is that it gives the possibility to get the results which cannot be obtained by any other physical methods. Mossbauer effect has been used as a key to unlock some basic physical, chemical and biological phenomena, as a guide for finding the new ways of solving applied scientific and technical problems of electronics, metallurgy, civil engineering, and even fine arts and archaeology. Very few scientific techniques can claim entry into as many countries as Mossbauer spectroscopy. Due to its wide application in an education and research processes the community of Mossbauer spectroscopists extends to almost 100 different countries. Laboratory equipment necessary for conducting gamma resonance spectroscopy, do not require large investments, premises, personnel. The spectrometer is rather small in size and could be installed on the ordinary laboratory table. That is why Mossbauer effect is widely used at numerous Universities all over the world as an universal instrument for tuition and research

Study of radioactivity levels in detergent powders samples by gamma spectroscopy

Directory of Open Access Journals (Sweden)

Ali A. Abojassim

2014-10-01

Full Text Available This study focuses on the evaluation of the natural radioactivity levels in ten samples of the detergent powders that available in Iraqi markets. We have determined the specific activities of uranium, thorium and potassium using gamma spectroscopy and calculation of radiation hazard indices. The results of the activities of radionuclides (238U, 232Th, 40K for detergent powders samples, are found that the 238U specific activities were varied from (11.489 ± 2.089 Bq/kg to (36.062 ± 2.478 Bq/kg, while the 232th specific activities were varied from (1.411 ± 0.609 Bq/kg to (9.272 ± 1.642 Bq/kg and 40K were varied from (8.189 ± 2.339 Bq/kg to (91.888 ± 4.164 Bq/kg. These values are always lower than those of raw materials, what is explained by the conservation of radioactive material throughout the manufacturing process. The radium equivalent activity Raeq, the external hazard index Hex and the internal hazard index Hin dose due to natural radioactivity estimated below the regulatory standard recommended which are (370 Bq/kg, 1 and 1 according to OECD 1979 and ICRP 2000, allows us to show that Detergent powders samples products are not contaminated by radioactivity, are healthy and do not have harmful radiological impact on the consumer.

Monte Carlo simulation of determining porosity by using dual gamma detectors

International Nuclear Information System (INIS)

Zhang Feng; Liu Juntao; Yu Huawei; Yuan Chao; Jia Yan

2013-01-01

Current formation elements spectroscopy logging technology utilize 241 Am-Be neutron source and single BGO detector to determine elements contents. It plays an important role in mineral analysis and lithology identification of unconventional oil and gas exploration, but information measured is relatively ld. Measured system based on 241 Am-Be neutron and dual detectors can be developed to realize the measurement of elements content as well as determine neutron gamma porosity by using ratio of gamma count between near and far detectors. Calculation model is built by Monte Carlo method to study neutron gamma porosity logging response with different spacing and shields. And it is concluded that measuring neutron gamma have high counts and good statistical property contrasted with measuring thermal neutron, but the sensitivity of porosity decrease. Sensitivity of porosity will increase as the spacing of dual detector increases. Spacing of far and near detectors should be around 62 cm and 35 cm respectively. Gamma counts decrease and neutron gamma porosity sensitivity increase when shield is fixed between neutron and detector. The length of main shield should be greater than 10 cm and associated shielding is about 5 cm. By Monte Carlo Simulation study, the result provides technical support for determining porosity in formation elements spectroscopy logging using 241 Am-Be neutron and gamma detectors. (authors)

Gamma Ray Imaging for Environmental Remediation

Energy Technology Data Exchange (ETDEWEB)

B.F. Philips; R.A. Kroeger: J.D. Kurfess: W.N. Johnson; E.A. Wulf; E. I. Novikova

2004-11-12

This program is the development of germanium strip detectors for environmental remediation. It is a collaboration between the Naval Research Laboratory and Lawrence Berkeley National Lab. The goal is to develop detectors that are simultaneously capable of excellent spectroscopy and imaging of gamma radiation.

The spectroscopy of fission fragments

Energy Technology Data Exchange (ETDEWEB)

Phillips, W.R. [Department of Physics and Astronomy, University of Manchester, Manchester, M13 9PL (United Kingdom); Collaboration: La Direction des Sciences de la Matiere du CEA (FR); Le Fonds National de la Recherche Scientifique de Belgique (BE)

1998-12-31

High-resolution measurements on {gamma} rays from fission fragments have provided a rich source of information, unobtainable at the moment in any other way, on the spectroscopy of neutron-rich nuclei. In recent years important data have been obtained on the yrast- and near yrast-structure of neutron-rich fission fragments. We discuss the scope of measurements which can be made on prompt gamma rays from secondary fission fragments, the techniques used in the experiments and some results recently obtained. (author) 24 refs., 8 figs., 1 tab.

The alterations in high density polyethylene properties with gamma irradiation

Science.gov (United States)

Zaki, M. F.; Elshaer, Y. H.; Taha, Doaa. H.

2017-10-01

In the present investigation, high density polyethylene (HDPE) polymer has been used to study the alterations in its properties under gamma-irradiation. Physico-chemical properties have been investigated with different spectroscopy techniques, Fourier Transform Infrared spectroscopy (FTIR), X-ray diffraction (XRD), biocompatibility properties, as well as, mechanical properties change. The FT-IR analysis shows the formation of new band at 1716 cm-1 that is attributed to the oxidation of irradiated polymer chains, which is due to the formation of carbonyl groups (C˭O). XRD patterns show that a decrease in the crystallite size and increase in the Full Width at Half Maximum (FWHM). This means that the crystallinity of irradiated samples is decreased with increase in gamma dose. The contact angle measurements show an increase in the surface free energy as the gamma irradiation increases. The measurements of mechanical properties of irradiated HDPE samples were discussed.

A maximum-likelihood reconstruction algorithm for tomographic gamma-ray nondestructive assay

International Nuclear Information System (INIS)

Prettyman, T.H.; Estep, R.J.; Cole, R.A.; Sheppard, G.A.

1994-01-01

A new tomographic reconstruction algorithm for nondestructive assay with high resolution gamma-ray spectroscopy (HRGS) is presented. The reconstruction problem is formulated using a maximum-likelihood approach in which the statistical structure of both the gross and continuum measurements used to determine the full-energy response in HRGS is precisely modeled. An accelerated expectation-maximization algorithm is used to determine the optimal solution. The algorithm is applied to safeguards and environmental assays of large samples (for example, 55-gal. drums) in which high continuum levels caused by Compton scattering are routinely encountered. Details of the implementation of the algorithm and a comparative study of the algorithm's performance are presented

Measurement of actinide concentration in solution samples from the NUCEF reprocessing facility by X-ray and low energy gamma-ray spectroscopy

International Nuclear Information System (INIS)

Howarth, P.J.A.; Uchiyama, Gunzo; Asakura, Toshihide; Sawada, Mutsumi; Hagiya, Hiromichi; Fujine, Sachio

1999-01-01

X-ray and low-energy gamma-ray spectroscopy has been used to measure actinide concentration within the backend nuclear fuel reprocessing research facility at NUCEF. Research on advanced reprocessing techniques at NUCEF is based on the PARC refinement of the PUREX process which aims to recover Am and Cm from the highly active waste stream and to control and partition Np and Tc. It is hoped that the PARC process will mitigate the environmental impact of the wastes and improve the economy of reprocessing. The main actinides for which assay is required are U, Pu, Np and Am and knowledge of these concentrations will enable the following to be determined: i.) evaluation of the distribution of actinides throughout the reprocessing facility ii.) verification of the simulated actinide distribution from chemical kinetic simulations of the PARC process and iii.) assurance of safety and control over migrant radioactive species. The research presented here shows that passive measurement of x-rays and low-energy gamma-rays from solution samples provides an accurate and non-destructive means for assaying the concentration. The measurement technique is based on the use of the characteristic low energy gamma-rays and internal conversion x-ray emission from actinides (11 keV to 22 keV). The x-ray emission is a few orders of magnitude more intense than the characteristic gamma-ray emission and can be easily detected from solutions. The experimental system described here can be used for solution monitoring to a minimum concentration of typically 10-6 M for Pu, 10-10 M for Am and 10-6 M for Np. (author)

Efficiency calibration and measurement of self-absorption correction of environmental gamma spectroscopy of soils samples using Marinelli beaker

International Nuclear Information System (INIS)

Abdi, M. R.; Mostajaboddavati, M.; Hassanzadeh, S.; Faghihian, H.; Rezaee, Kh.; Kamali, M.

2006-01-01

A nonlinear function in combination with the method of mixing activity calibrated is applied for fitting the experimental peak efficiency of HPGe spectrometers in 59-2614 keV energy range. The preparation of Marinelli beaker standards of mixed gamma and RG-set at secular equilibrium with its daughter radionuclides was studied. Standards were prepared by mixing of known amounts of 13B a, 241 Am, 152 Eu, 207 Bi, 24 Na, Al 2 O 3 powder and soil. The validity of these standards was checked by comparison with certified standard reference material RG-set and IAEA-Soil-6 Self-absorption was measured for the activity calculation of the gamma-ray lines about series of 238 U daughter, 232 Th series, 137 Cs and 40 K in soil samples. Self-absorption in the sample will depend on a number of factor including sample composition, density, sample size and gamma-ray energy. Seven Marinelli beaker standards were prepared in different degrees of compaction with bulk density ( ρ) of 1.000 to 1.600 g cm -3 . The detection efficiency versus density was obtained and the equation of self-absorption correction factors calculated for soil samples

Irradiation effects detected by Moessbauer spectroscopy in iron complexes

International Nuclear Information System (INIS)

Ladriere, J.

1998-01-01

The nature and the extent of the 60 Co gamma radiolysis of several iron coordination compounds have been analysed by Moessbauer absorption spectroscopy. The comparison of the radiolytic yields with the after effects observed by Moessbauer emission spectroscopy in similar 57 Co-doped compounds, supports the self-radiolysis model

Possibility of applying the gamma-gamma method to the in situ determination of uranium-ore densities; Les possibilites d'application de la methode gamma-gamma a la determination en place de la densite des minerais d'uranium

Energy Technology Data Exchange (ETDEWEB)

Czubek, J; Guitton, J [Commissariat a l' Energie Atomique, Saclay (France). Centre d' Etudes Nucleaires

1965-07-01

The principles of the gamma-gamma method are reviewed. It is shown in particular that, under certain conditions, the method makes it possible to obtain a representative measurement of the electronic density. Chemical analyses have been carried out on samples obtained from uranium deposits. The results show that an exact correlation exists between the massive and electronic densities. It is possible to consider the possibility of measuring the density of uranium-containing rocks by the gamma-gamma method. (authors) [French] Les principes de la methode gamma-gamma sont rappeles. En particulier, il est montre que, dans certaines conditions, la methode permet une mesure representative de la densite electronique. Des analyses chimiques ont ete effectuees sur des echantillons provenant de gisements uraniferes. Les resultats indiquent qu'il existe une correlation precise entre leur densite massique et leur densite electronique. Il est possible d'envisager la mesure de la densite des roches uraniferes par la methode gamma-gamma.

An optimum analysis sequence for environmental gamma-ray spectrometry

International Nuclear Information System (INIS)

De la Torre, F.; Rios M, C.; Ruvalcaba A, M. G.; Mireles G, F.; Saucedo A, S.; Davila R, I.; Pinedo, J. L.

2010-10-01

This work aims to obtain an optimum analysis sequence for environmental gamma-ray spectroscopy by means of Genie 2000 (Canberra). Twenty different analysis sequences were customized using different peak area percentages and different algorithms for: 1) peak finding, and 2) peak area determination, and with or without the use of a library -based on evaluated nuclear data- of common gamma-ray emitters in environmental samples. The use of an optimum analysis sequence with certified nuclear information avoids the problems originated by the significant variations in out-of-date nuclear parameters of commercial software libraries. Interference-free gamma ray energies with absolute emission probabilities greater than 3.75% were included in the customized library. The gamma-ray spectroscopy system (based on a Ge Re-3522 Canberra detector) was calibrated both in energy and shape by means of the IAEA-2002 reference spectra for software intercomparison. To test the performance of the analysis sequences, the IAEA-2002 reference spectrum was used. The z-score and the reduced χ 2 criteria were used to determine the optimum analysis sequence. The results show an appreciable variation in the peak area determinations and their corresponding uncertainties. Particularly, the combination of second derivative peak locate with simple peak area integration algorithms provides the greater accuracy. Lower accuracy comes from the combination of library directed peak locate algorithm and Genie's Gamma-M peak area determination. (Author)

Evaluation of peak-fitting software for gamma spectrum analysis

International Nuclear Information System (INIS)

Zahn, Guilherme S.; Genezini, Frederico A.; Moralles, Mauricio

2009-01-01

In all applications of gamma-ray spectroscopy, one of the most important and delicate parts of the data analysis is the fitting of the gamma-ray spectra, where information as the number of counts, the position of the centroid and the width, for instance, are associated with each peak of each spectrum. There's a huge choice of computer programs that perform this type of analysis, and the most commonly used in routine work are the ones that automatically locate and fit the peaks; this fit can be made in several different ways - the most common ways are to fit a Gaussian function to each peak or simply to integrate the area under the peak, but some software go far beyond and include several small corrections to the simple Gaussian peak function, in order to compensate for secondary effects. In this work several gamma-ray spectroscopy software are compared in the task of finding and fitting the gamma-ray peaks in spectra taken with standard sources of 137 Cs, 60 Co, 133 Ba and 152 Eu. The results show that all of the automatic software can be properly used in the task of finding and fitting peaks, with the exception of GammaVision; also, it was possible to verify that the automatic peak-fitting software did perform as well as - and sometimes even better than - a manual peak-fitting software. (author)

Gamma ray degradation of electrolytes containing alkylcarbonate solvents and a lithium salt

Energy Technology Data Exchange (ETDEWEB)

Caillon-Caravanier, Magaly; Jones, Jennifer; Anouti, Meriem; Lemordant, Daniel [Laboratoire CIME/PCMB (EA4244), Universite F. Rabelais, Faculte des Sciences et Techniques, Parc de Grandmont, 37200 Tours (France); Montigny, Frederic [Plateau d' Analyse Chimique, Universite F. Rabelais, Faculte de Pharmacie, 31 avenue Monge 37200 Tours (France); Willmann, Patrick [CNES, 18 avenue E. Belin, 31055 Toulouse (France); David, Jean-Pierre; Soonckindt, Sabine [Departement Environnement Spatial DSEP/ONERA, 2, avenue E. Belin, 31055 Toulouse (France)

2010-01-15

Lithium-ion batteries for space applications, such as satellites, are subjected to cosmic radiations, in particular, {gamma}-irradiation. In this study, the effects of this radiation on electrolytes and their components used in the lithium-ion batteries are investigated. The conductivity and viscosity of the samples have been measured before and after the irradiation. The modifications are evaluated by spectral analyses such as Fourier transform infrared spectroscopy (FTIR), nuclear magnetic resonance spectroscopy ({sup 1}H and {sup 13}C NMR), solid phase microextraction-gas chromatography (SPME-GC) and gas chromatography-mass spectroscopy (GC-MS). The experimental results show that only the samples containing vinylene carbonate and/or the lithium salt LiPF{sub 6} are degraded by {gamma}-radiation. (author)

Investigation of radiosterilization feasibility of sulfamethoxazole by ESR spectroscopy

Science.gov (United States)

Çolak, Şeyda

2017-12-01

In the present study, the spectroscopic features of the radiolytic intermediates that were produced in gamma-irradiated (5, 10, 25 and 50 kGy) sulfamethoxazole (SMX) have been investigated by electron spin resonance (ESR) spectroscopy and the radiation sterilization feasibility of SMX by ionizing radiation was examined. Gamma-irradiated SMX exhibited a complex ESR spectrum consisting of 13 resonance lines where spectral parameters for the central resonance line were found to be g = 2.0062 and ΔHpp = 0.6 mT. The radiation yield of SMX was calculated to be relatively low (G = 0.1) by ESR spectroscopy and no meaningful difference was observed in the comparison of unirradiated and 50 kGy gamma irradiated SMX by the Fourier transform infrared (FT-IR) technique, confirming that SMX is a radioresistive material. Although SMX could not be accepted to be a good dosimetric material, the identification of irradiated SMX from the unirradiated sample was possible even for the low absorbed radiation doses and for a relatively long time (three months) after the irradiation process. Decay activation energy of the radical species, which is mostly responsible for the central intense resonance line, is calculated to be 45.15 kJ/mol by using the signal intensity decay data derived from annealing studies. Four radical species with different spectroscopic properties were accepted to be responsible for the ESR spectra of gamma-irradiated SMX, by simulation calculations. It is concluded that SMX and SMX-containing drugs can be sterilized by gamma radiation and ESR spectroscopy is an appropriate technique for the characterization of these induced radical intermediates during the gamma irradiation process of SMX. Toxicology tests should also be done for its safe usage.

Using gamma distribution to determine half-life of rotenone, applied in freshwater

Energy Technology Data Exchange (ETDEWEB)

Rohan, Maheswaran, E-mail: mrohan@aut.ac.nz [Department of Biostatistics and Epidemiology, Auckland University of Technology, Auckland (New Zealand); Fairweather, Alastair; Grainger, Natasha [Science and Capability, Department of Conservation, Hamilton (New Zealand)

2015-09-15

Following the use of rotenone to eradicate invasive pest fish, a dynamic first-order kinetic model is usually used to determine the half-life and rate at which rotenone dissipated from the treated waterbody. In this study, we investigate the use of a stochastic gamma model for determining the half-life and rate at which rotenone dissipates from waterbodies. The first-order kinetic and gamma models produced similar values for the half-life (4.45 days and 5.33 days respectively) and days to complete dissipation (51.2 days and 52.48 days respectively). However, the gamma model fitted the data better and was more flexible than the first-order kinetic model, allowing us to use covariates and to predict a possible range for the half-life of rotenone. These benefits are particularly important when examining the influence that different environmental factors have on rotenone dissipation and when trying to predict the rate at which rotenone will dissipate during future operations. We therefore recommend that in future the gamma distribution model is used when calculating the half-life of rotenone in preference to the dynamic first-order kinetics model. - Highlights: • We investigated the use of the gamma model to calculate the half-life of rotenone. • Physical and environmental variables can be incorporated into the model. • A method for calculating the range around a mean half-life is presented. • The model is more flexible than the traditionally used first-order kinetic model.

Observation of neutron standing waves at total reflection by precision gamma spectroscopy

International Nuclear Information System (INIS)

Aksenov, V.L.; Gundorin, N.A.; Nikitenko, Yu.V.; Popov, Yu.P.; Cser, L.

1998-01-01

Total reflection of polarized neutrons from the layered structure glass/Fe (1000 A Angstrom)/Gd (50 A Angstrom) is investigated by registering neutrons and gamma-quanta from thermal neutron capture. The polarization ratio of gamma counts of neutron beams polarized in and opposite the direction of the magnetic field is measured. The polarization ratio is larger than unity for the neutron wavelengths λ 2.2 A Angstrom. Such behaviour of the wavelength dependence of the gamma-quanta polarization ratio points to the fact that over the surface of the Fe Layer a neutron standing wave caused by the interference of the incident neutron wave and the wave refracted from the magnetized Fe layer is formed

Impurities in radioactive solutions for gamma spectroscopy

International Nuclear Information System (INIS)

Delgado, J.U.

1990-01-01

The absolute and relative methods for radioactive sources calibration, like 4 Πβ-γ and 4Πγ ionization chamber respectively, allows to reach 0,1% of exactiness in activity measurement, but cannot distinguish radioactive impurities that interfere in the activity. Then, one of the problems associated to a quality control of calibrated sources furnished to users is the identification and quantification of the impurities. In this work, a routine technical procedure, using the facilities of gamma spectrometry method that allows to identify and to determine the impurities relative contribution to the source main radionuclide activity, is described. (author) [pt

Isomer-delayed gamma-ray spectroscopy of neutron-rich 166Tb

Directory of Open Access Journals (Sweden)

Gurgi L.A.

2017-01-01

Full Text Available This short paper presents the identification of a metastable, isomeric-state decay in the neutron-rich odd-odd, prolate-deformed nucleus 166Tb. The nucleus of interest was formed using the in-flight fission of a 345 MeV per nucleon 238U primary beam at the RIBF facility, RIKEN, Japan. Gamma-ray transitions decaying from the observed isomeric states in 166Tb were identified using the EURICA gamma-ray spectrometer, positioned at the final focus of the BigRIPS fragments separator. The current work identifies a single discrete gamma-ray transition of energy 119 keV which de-excites an isomeric state in 166Tb with a measured half-life of 3.5(4 μs. The multipolarity assignment for this transition is an electric dipole and is made on the basis internal conversion and decay lifetime arguments. Possible two quasi-particle Nilsson configurations for the initial and final states which are linked by this transition in 166Tb are made on the basis of comparison with Blocked BCS Nilsson calculations, with the predicted ground state configuration for this nucleus arising from the coupling of the v(1-/2[521] and π(3+/2 Nilsson orbitals.

Evaluation of a gamma-spectroscopy gauge for uranium-plutonium assay

International Nuclear Information System (INIS)

Notea, A.; Segal, Y.

1976-01-01

A procedure is presented for the characterization of a gamma passive method for non-destructive analysis of nuclear fuel. The approachh provides an organized and systematic way for optimizing the assay system. The key function is the relative resolving power defined as the smallest relative change in the quantity of radionuclide measured that may be detected within a certain confidence level. This function is derived for nuclear fuel employing a model based on empirical parameters. The ability to detect changes in fuels of binary and trinary compositions with a 50-cm 3 Ge(Li) at a 1-min counting period is discussed. As an example to a binary composition, an enriched uranium fuel was considered. The 185-keV and 1001-keV gamma lines are used for the assay of 235 U and 238 U, respectively. As a trinary composition a plutonium-containing fuel was examined. The plutonium was identified by the 414-keV gamma line. The interference of the high-energy lines is carefully analysed, and numerical results are presented. For both cases the range of measurement under specific accuracy demands is determined. The approac described is suitable also for evaluation of other passive as well as active assay methods. (author)

Total absorption gamma-ray spectroscopy (TAGS): Current status of measurement programmes for decay heat calculations and other applications. Summary report of consultants' meeting

International Nuclear Information System (INIS)

Nichols, A.L.; Nordborg, C.

2009-02-01

A Consultants' Meeting on 'Total Absorption Gamma-ray Spectroscopy (TAGS)' was held on 27-28 January 2009 at the IAEA Headquarters, Vienna, Austria. All presentations, discussions and recommendations of this meeting are contained within this report. The purpose of the meeting was to report and discuss progress and plans to measure total gamma-ray spectra in order to derive mean beta and gamma decay data for decay heat calculations and other applications. This form of review had been recommended by contributors to Subgroup 25 of the OECD-NEA Working Party on International Evaluation Cooperation of the Nuclear Science Committee, for implementation in 2008/09. Hence, relevant specialists were invited to discuss their recently performed and planned TAGS studies, along with experimentalists proposing to assemble and operate such dedicated facilities. Knowledge and quantification of antineutrino spectra is believed to be a significant asset in the non-invasive monitoring of reactor operations and possible application in safeguards, as well as fundamental in the study of neutrino oscillations - these data needs were also debated in terms of appropriate TAGS measurements. A re-assessment of the current request list for TAGS studies is merited and was undertaken in the context of decay heat calculations, and agreement was reached to extend these requirements to the derivation of antineutrino spectra. (author)

Differential sensitivity of Chironomus and human hemoglobin to gamma radiation

Energy Technology Data Exchange (ETDEWEB)

Gaikwad, Pallavi S. [Stress Biology Research Laboratory, Department of Zoology, Savitribai Phule University, Pune, 411007 (India); Molecular Biology Division, Bhabha Atomic Research Centre, Trombay, Mumbai, 400085 (India); Panicker, Lata [Solid State Physics Division, Bhabha Atomic Research Centre, Trombay, Mumbai, 400085 (India); Mohole, Madhura; Sawant, Sangeeta [Bioinformatics Center, Savitribai Phule Pune University, Pune, 411007 (India); Mukhopadhyaya, Rita [Molecular Biology Division, Bhabha Atomic Research Centre, Trombay, Mumbai, 400085 (India); Nath, Bimalendu B., E-mail: bbnath@gmail.com [Stress Biology Research Laboratory, Department of Zoology, Savitribai Phule University, Pune, 411007 (India)

2016-08-05

Chironomus ramosus is known to tolerate high doses of gamma radiation exposure. Larvae of this insect possess more than 95% of hemoglobin (Hb) in its circulatory hemolymph. This is a comparative study to see effect of gamma radiation on Hb of Chironomus and humans, two evolutionarily diverse organisms one having extracellular and the other intracellular Hb respectively. Stability and integrity of Chironomus and human Hb to gamma radiation was compared using biophysical techniques like Dynamic Light Scattering (DLS), UV-visible spectroscopy, fluorescence spectrometry and CD spectroscopy after exposure of whole larvae, larval hemolymph, human peripheral blood, purified Chironomus and human Hb. Sequence- and structure-based bioinformatics methods were used to analyze the sequence and structural similarities or differences in the heme pockets of respective Hbs. Resistivity of Chironomus Hb to gamma radiation is remarkably higher than human Hb. Human Hb exhibited loss of heme iron at a relatively low dose of gamma radiation exposure as compared to Chironomus Hb. Unlike human Hb, the heme pocket of Chironomus Hb is rich in aromatic amino acids. Higher hydophobicity around heme pocket confers stability of Chironomus Hb compared to human Hb. Previously reported gamma radiation tolerance of Chironomus can be largely attributed to its evolutionarily ancient form of extracellular Hb as evident from the present study. -- Highlights: •Comparison of radiation tolerant Chironomus Hb and radiation sensitive Human Hb. •Amino acid composition of midge and human heme confer differential hydrophobicity. •Heme pocket of evolutionarily ancient midge Hb provide gamma radiation resistivity.

Differential sensitivity of Chironomus and human hemoglobin to gamma radiation

International Nuclear Information System (INIS)

Gaikwad, Pallavi S.; Panicker, Lata; Mohole, Madhura; Sawant, Sangeeta; Mukhopadhyaya, Rita; Nath, Bimalendu B.

2016-01-01

Chironomus ramosus is known to tolerate high doses of gamma radiation exposure. Larvae of this insect possess more than 95% of hemoglobin (Hb) in its circulatory hemolymph. This is a comparative study to see effect of gamma radiation on Hb of Chironomus and humans, two evolutionarily diverse organisms one having extracellular and the other intracellular Hb respectively. Stability and integrity of Chironomus and human Hb to gamma radiation was compared using biophysical techniques like Dynamic Light Scattering (DLS), UV-visible spectroscopy, fluorescence spectrometry and CD spectroscopy after exposure of whole larvae, larval hemolymph, human peripheral blood, purified Chironomus and human Hb. Sequence- and structure-based bioinformatics methods were used to analyze the sequence and structural similarities or differences in the heme pockets of respective Hbs. Resistivity of Chironomus Hb to gamma radiation is remarkably higher than human Hb. Human Hb exhibited loss of heme iron at a relatively low dose of gamma radiation exposure as compared to Chironomus Hb. Unlike human Hb, the heme pocket of Chironomus Hb is rich in aromatic amino acids. Higher hydophobicity around heme pocket confers stability of Chironomus Hb compared to human Hb. Previously reported gamma radiation tolerance of Chironomus can be largely attributed to its evolutionarily ancient form of extracellular Hb as evident from the present study. -- Highlights: •Comparison of radiation tolerant Chironomus Hb and radiation sensitive Human Hb. •Amino acid composition of midge and human heme confer differential hydrophobicity. •Heme pocket of evolutionarily ancient midge Hb provide gamma radiation resistivity.

Xe isotope detection and discrimination using beta spectroscopy with coincident gamma spectroscopy

Science.gov (United States)

Reeder, P. L.; Bowyer, T. W.

1998-02-01

Beta spectroscopic techniques show promise of significant improvements for a beta-gamma coincidence counter that is part of a system for analyzing Xe automatically separated from air. The previously developed counting system for 131mXe, 133mXe, 133gXe, and 135gXe can be enhanced to give additional discrimination between these Xe isotopes by using the plastic scintillation sample cell as a beta spectrometer to resolve the conversion electron peaks. The automated system will be a key factor in monitoring the Comprehensive Test Ban Treaty.

The effect of gamma irradiation on rice protein aqueous solution

Science.gov (United States)

Baccaro, Stefania; Bal, Oya; Cemmi, Alessia; Di Sarcina, Ilaria

2018-05-01

The use of proteins as natural biopolymers are sensibly increasing in several application fields such as food industry, packaging and environment protection. In particular, rice proteins (RP) present good nutritional, hypoallergenic and healthful properties very interesting for human consumption. Since ionizing radiation can be successfully applied on protein containing systems involved in different industrial processes, this work aims to determine the effect of gamma radiation on 5 wt%-7.5 wt% RP aqueous solutions in a wide range of absorbed doses up to around 40 kGy. The changes of RP secondary and tertiary structures and their chemical composition were followed by UV-VIS absorbance spectroscopy, luminescence analysis and pH measurements. The experimental data showed the occurrence of the unfolding of RP chains with the increase of the absorbed dose and the formation of new molecules, due to the reaction among tryptophane and tyrosine amino acids and the radical species induced by gamma radiation. The results are also confirmed by the modification of the pH values measured for the irradiated solutions.

Modifications induced by gamma irradiation to Makrofol polymer nuclear track detector

Directory of Open Access Journals (Sweden)

A. Tayel

2015-03-01

Full Text Available The aim of the present study was extended from obtaining information about the interaction of gamma rays with Makrofol DE 7-2 track detector to introduce the basis that can be used in concerning simple sensor for gamma irradiation and bio-engineering applications. Makrofol polymer samples were irradiated with 1.25 MeV 60Co gamma radiations at doses ranging from 20 to 1000 kG y. The modifications of irradiated samples so induced were analyzed using UV–vis spectrometry, photoluminescence spectroscopy, and the measurements of Vickers’ hardness. Moreover, the change in wettability of irradiated Makrofol was investigated by the contact angle determination of the distilled water. UV–vis spectroscopy shows a noticeable decrease in the energy band gap due to gamma irradiation. This decrease could be attributed to the appearance of a shift to UV spectra toward higher wavelength region after irradiation. Photoluminescence spectra reveal a remarkable change in the integrated photoluminescence intensity with increasing gamma doses, which may be resulted from some matrix disorder through the creation of some defected states in the irradiated polymer. The hardness was found to increase from 4.78 MPa for the unirradiated sample to 23.67 MPa for the highest gamma dose. The contact angle investigations show that the wettability of the modified samples increases with increasing the gamma doses. The result obtained from present investigation furnishes evidence that the gamma irradiations are a successful technique to modify the Makrofol DE 7-2 polymer properties to use it in suitable applications.

X-ray emission spectroscopy applied to glycine adsorbed on Cu(110): An atom and symmetry projected view

Energy Technology Data Exchange (ETDEWEB)

Hasselstroem, J.; Karis, O.; Weinelt, M. [Uppsala Univ. (Sweden)] [and others

1997-04-01

When a molecule is adsorbed on a metal surface by chemical bonding new electronic states are formed. For noble and transition metals these adsorption-induced states overlap with the much more intense metal d-valence band, making them difficult to probe by for instance direct photoemission. However, it has recently been shown that X-ray emission spectroscopy (XES) can be applied to adsorbate systems. Since the intermediate state involves a core hole, this technique has the power to project out the partial density of states around each atomic site. Both the excitation and deexcitation processes are in general governed by the dipole selection rules. For oriented system, it is hence possible to obtain a complete separation into 2p{sub x}, 2p{sub y} and 2p{sub z} contributions using angular resolved measurements. The authors have applied XES together with other core level spectroscopies to glycine adsorption on Cu(110). Glycine (NH{sub 2}CH{sub 2}COOH) is the smallest amino acid and very suitable to study by core level spectroscopy since it has several functional groups, all well separated in energy by chemical shifts. Its properties are futhermore of biological interest. In summary, the authors have shown that it is possible to apply XES to more complicated molecular adsorbates. The assignment of different electronic states is however not as straight forward as for simple diatomic molecules. For a complete understanding of the redistribution and formation of new electronic states associated with the surface chemical bond, experimental data must be compared to theoretical calculations.

Raman spectroscopy and capillary electrophoresis applied to forensic colour inkjet printer inks analysis.

Science.gov (United States)

Król, Małgorzata; Karoly, Agnes; Kościelniak, Paweł

2014-09-01

Forensic laboratories are increasingly engaged in the examination of fraudulent documents, and what is important, in many cases these are inkjet-printed documents. That is why systematic approaches to inkjet printer inks comparison and identification have been carried out by both non-destructive and destructive methods. In this study, micro-Raman spectroscopy and capillary electrophoresis (CE) were applied to the analysis of colour inkjet printer inks. Micro-Raman spectroscopy was used to study the chemical composition of colour inks in situ on a paper surface. It helps to characterize and differentiate inkjet inks, and can be used to create a spectra database of inks taken from different cartridge brands and cartridge numbers. Capillary electrophoresis in micellar electrophoretic capillary chromatography mode was applied to separate colour and colourless components of inks, enabling group identification of those components which occur in a sufficient concentration (giving intensive peaks). Finally, on the basis of the obtained results, differentiation of the analysed inks was performed. Twenty-three samples of inkjet printer inks were examined and the discriminating power (DP) values for both presented methods were established in the routine work of experts during the result interpretation step. DP was found to be 94.0% (Raman) and 95.6% (CE) when all the analysed ink samples were taken into account, and it was 96.7% (Raman) and 98.4% (CE), when only cartridges with different index numbers were considered. Copyright © 2014 Elsevier Ireland Ltd. All rights reserved.

High resolution gamma-ray spectroscopy and the fascinating angular momentum realm of the atomic nucleus

International Nuclear Information System (INIS)

Riley, M A; Simpson, J; Paul, E S

2016-01-01

In 1974 Aage Bohr and Ben Mottelson predicted the different ‘phases’ that may be expected in deformed nuclei as a function of increasing angular momentum and excitation energy all the way up to the fission limit. While admitting their picture was highly conjectural they confidently stated ‘...with the ingenious experimental approaches that are being developed, we may look forward with excitement to the detailed spectroscopic studies that will illuminate the behaviour of the spinning quantised nucleus’ . High resolution gamma-ray spectroscopy has indeed been a major tool in studying the structure of atomic nuclei and has witnessed numerous significant advances over the last four decades. This article will select highlights from investigations at the Niels Bohr Institute, Denmark, and Daresbury Laboratory, UK, in the late 1970s and early 1980s, some of which have continued at other national laboratories in Europe and the USA to the present day. These studies illustrate the remarkable diversity of phenomena and symmetries exhibited by nuclei in the angular momentum–excitation energy plane that continue to surprise and fascinate scientists. (invited comment)

High resolution gamma-ray spectroscopy and the fascinating angular momentum realm of the atomic nucleus

Science.gov (United States)

Riley, M. A.; Simpson, J.; Paul, E. S.

2016-12-01

In 1974 Aage Bohr and Ben Mottelson predicted the different ‘phases’ that may be expected in deformed nuclei as a function of increasing angular momentum and excitation energy all the way up to the fission limit. While admitting their picture was highly conjectural they confidently stated ‘...with the ingenious experimental approaches that are being developed, we may look forward with excitement to the detailed spectroscopic studies that will illuminate the behaviour of the spinning quantised nucleus’. High resolution gamma-ray spectroscopy has indeed been a major tool in studying the structure of atomic nuclei and has witnessed numerous significant advances over the last four decades. This article will select highlights from investigations at the Niels Bohr Institute, Denmark, and Daresbury Laboratory, UK, in the late 1970s and early 1980s, some of which have continued at other national laboratories in Europe and the USA to the present day. These studies illustrate the remarkable diversity of phenomena and symmetries exhibited by nuclei in the angular momentum-excitation energy plane that continue to surprise and fascinate scientists.

A high rate gamma spectroscopy system for activation analysis of short lived isomeric transitions

Energy Technology Data Exchange (ETDEWEB)

Westphal, G P [Atominstitut, Vienna (Austria)

1976-07-01

A high rate spectroscopy system specially suited for measurement of short-lived isomeric transitions is described, which, as part of a fast activation analysis facility at the TRIGA Mark II reactor, provides for automatic recording and immediate evaluation of gamma spectra taken from nuclides activated at stationary or pulsed reactor power. The system consists of a commercial DC-coupled Ge(Li)-detector of 70 cm{sup 3} modified for recycling operation for input rates in excess of 500,000 c/s Co-60, a time variant trapezoidal shaping section and a fast constant dead-time ADC coupled to a programmed multi-channel analyzer. Novel circuits for efficient pile-up rejection and time variant base line restoration extend the concept of gated integration up to count rates of more than 300,000 c/s Co-60. Time-sequenced recording of spectra is performed by a mini computer operated as a front-end processor of a larger laboratory computer, where final data processing takes place. New concepts for very simple and cost-effective implementation of multi-channel analyzers by means of general purpose small computers are described. (author)

Summary report of the first research coordination meeting on development of a reference database for particle-induced gamma ray emission (PIGE) spectroscopy

International Nuclear Information System (INIS)

Abriola, D.; Pedro de Jesus, A.

2011-07-01

The First Research Coordination Meeting (RCM) of the IAEA Coordinated Research Project (CRP) on 'Development of a Reference Database for Particle-Induced Gamma-ray Emission (PIGE) Spectroscopy' was held at the IAEA, Vienna, from 16-20 May 2011. A summary of the participants' presentations is given as well as background information, objectives and recommendations concerning approach and methodology. The extension of the IBANDL database format to include PIGE data was discussed. The different tasks to achieve the CRP objectives were assigned to participants. A list of priority measurements was produced and the individual sets of measurements assigned to participants. (author)

Alternative Measuring Approaches in Gamma Scanning on Spent Nuclear Fuel

Energy Technology Data Exchange (ETDEWEB)

Sihm Kvenangen, Karen

2007-06-15

In the future, the demand for energy is predicted to grow and more countries plan to utilize nuclear energy as their source of electric energy. This gives rise to many important issues connected to nuclear energy, such as finding methods that can verify that the spent nuclear fuel has been handled safely and used in ordinary power producing cycles as stated by the operators. Gamma ray spectroscopy is one method used for identification and verification of spent nuclear fuel. In the specific gamma ray spectroscopy method called gamma scanning the gamma radiation from the fission products Cs-137, Cs-134 and Eu-154 are measured in a spent fuel assembly. From the results, conclusions can be drawn about the fuels characteristics. This degree project examines the possibilities of using alternative measuring approaches when using the gamma scanning method. The focus is on examining how to increase the quality of the measured data. How to decrease the measuring time as compared with the present measuring strategy, has also been investigated. The main part of the study comprises computer simulations of gamma scanning measurements. The simulations have been validated with actual measurements on spent nuclear fuel at the central interim storage, Clab. The results show that concerning the quality of the measuring data the conventional strategy is preferable, but with other starting positions and with a more optimized equipment. When focusing on the time aspect, the helical measuring strategy can be an option, but this needs further investigation.

Alternative Measuring Approaches in Gamma Scanning on Spent Nuclear Fuel

International Nuclear Information System (INIS)

Sihm Kvenangen, Karen

2007-06-01

In the future, the demand for energy is predicted to grow and more countries plan to utilize nuclear energy as their source of electric energy. This gives rise to many important issues connected to nuclear energy, such as finding methods that can verify that the spent nuclear fuel has been handled safely and used in ordinary power producing cycles as stated by the operators. Gamma ray spectroscopy is one method used for identification and verification of spent nuclear fuel. In the specific gamma ray spectroscopy method called gamma scanning the gamma radiation from the fission products Cs-137, Cs-134 and Eu-154 are measured in a spent fuel assembly. From the results, conclusions can be drawn about the fuels characteristics. This degree project examines the possibilities of using alternative measuring approaches when using the gamma scanning method. The focus is on examining how to increase the quality of the measured data. How to decrease the measuring time as compared with the present measuring strategy, has also been investigated. The main part of the study comprises computer simulations of gamma scanning measurements. The simulations have been validated with actual measurements on spent nuclear fuel at the central interim storage, Clab. The results show that concerning the quality of the measuring data the conventional strategy is preferable, but with other starting positions and with a more optimized equipment. When focusing on the time aspect, the helical measuring strategy can be an option, but this needs further investigation

A 3D simulation look-up library for real-time airborne gamma-ray spectroscopy

Science.gov (United States)

Kulisek, Jonathan A.; Wittman, Richard S.; Miller, Erin A.; Kernan, Warnick J.; McCall, Jonathon D.; McConn, Ron J.; Schweppe, John E.; Seifert, Carolyn E.; Stave, Sean C.; Stewart, Trevor N.

2018-01-01

A three-dimensional look-up library consisting of simulated gamma-ray spectra was developed to leverage, in real-time, the abundance of data provided by a helicopter-mounted gamma-ray detection system consisting of 92 CsI-based radiation sensors and exhibiting a highly angular-dependent response. We have demonstrated how this library can be used to help effectively estimate the terrestrial gamma-ray background, develop simulated flight scenarios, and to localize radiological sources. Source localization accuracy was significantly improved, particularly for weak sources, by estimating the entire gamma-ray spectra while accounting for scattering in the air, and especially off the ground.

Application of a gamma spectroscopy system to the measurement of neutron cross sections necessary to the development of nuclear energy; Mise au point d'un systeme de spectroscopie pour mesurer des sections efficaces neutroniques applicables a un possible developpement du nucleaire comme source d'energie

Energy Technology Data Exchange (ETDEWEB)

Deruelle, O

2002-09-01

This work concerns the development of nuclear energy and nuclear waste management in particular. Two parts of this study can be distinguished. In the first part (theoretical), a thorium-plutonium fuel based on MOX and dedicated for PWR was investigated in order to transmute plutonium in a potentially low waste fuel cycle. It was shown that this type of fuel is not regenerative but could be used for a transition to the industrial thorium fuel cycle without building new reactors. Thanks to moderated neutron spectra and high loaded actinide mass in the core, U-233 is quickly created ({approx}300 kg/y) for a loss of about {approx}1200 kg of fissile plutonium. In the second part (experimental), we have developed and built a new reaction chamber to measure neutron cross sections of actinides by alpha-gamma spectroscopy. This experimental device (in principle transportable) was commissioned in the high flux reactor of ILL Grenoble. Neutron flux was measured by gamma spectroscopy of irradiated Al and Co samples and was found to be of the order of 6,0. 10{sup 14} n.cm{sup -2}.s{sup -1} (4%). By the irradiation of 11{mu}g of Am-243 and Pu-242, corresponding capture cross sections were measured in the thermal neutron flux at 50 deg C. These are the results: {sup 243}Am(n,{gamma}) {sup 244fond.}Am = 4,72{+-}1,42b; {sup 243}Am(n,{gamma}) {sup 244total}Am = 74,8{+-}3,25b; {sup 242}Pu (n,{gamma}){sup 243}Pu = 22,7{+-}1,09b. Uncertainties of the measurements are mostly due to the determination of the neutron flux, efficiency of the electronics and ambiguities related to the definition of the area under {alpha}-{gamma} spectra. Although our measured cross sections deviate (by 10-30%) from the corresponding values widely used in evaluated data libraries such as ENDF, JEF and JENDL, in this work we have demonstrated the feasibility and principle of our experimental method. Furthermore, the value for the 243-americium capture cross-section is in very good agreement with the last two

Portable gamma-ray holdup and attributes measurements of high- and variable-burnup plutonium

International Nuclear Information System (INIS)

Wenz, T.R.; Russo, P.A.; Miller, M.C.; Menlove, H.O.; Takahashi, S.; Yamamoto, Y.; Aoki, I.

1991-01-01

High burnup-plutonium holdup has been assayed quantitatively by low resolution gamma-ray spectrometry. The assay was calibrated with four plutonium standards representing a range of fuel burnup and 241 Am content. Selection of a calibration standard based on its qualitative spectral similarity to gamma-ray spectra of the process material is partially responsible for the success of these holdup measurements. The spectral analysis method is based on the determination of net counts in a single spectral region of interest (ROI). However, the low-resolution gamma-ray assay signal for the high-burnup plutonium includes unknown amounts of contamination from 241 Am. For most needs, the range of calibration standards required for this selection procedure is not available. A new low-resolution gamma-ray spectral analysis procedure for assay of 239 Pu has been developed. The procedure uses the calculated isotope activity ratios and the measured net counts in three spectral ROIs to evaluate and remove the 241 Am contamination from the 239 Pu assay signal on a spectrum-by-spectrum basis. The calibration for the new procedure requires only a single plutonium standard. The procedure also provides a measure of the burnup and age attributes of holdup deposits. The new procedure has been demonstrated using portable gamma-ray spectroscopy equipment for a wide range of plutonium standards and has also been applied to the assay of 239 Pu holdup in a mixed oxide fuel fabrication facility. 10 refs., 5 figs., 3 tabs

High-resolution gamma spectroscopy with whole-body and partial-body counters. Experience, recommendations. Report; Hochaufloesende Gamma-Spektrometrie an Ganz- und Teilkoerperzaehlern. Erfahrungen, Empfehlungen. Bericht

Energy Technology Data Exchange (ETDEWEB)

Sahre, P. [comp.

1997-12-01

The application of high-resolution gamma spectroscopy with whole-body and partial-body counters shows a steadily rising upward trend over the last few years. This induced the ``Arbeitskreis Inkorporationsueberwachung`` of the association ``Fachverband fuer Strahlenschutz e.V.`` to organise a meeting for joint elaboration of a guide on recommended applications of this measuring technique, based on a review of existing experience and results. A key item on the agenda of the meeting was the comparative evaluation of the Ge semiconductor detector and the NaI solid scintillation detector. (orig./CB) [Deutsch] Der Einsatz der hochaufloesenden Gammaspektroskopie in Ganz- und Teilkoerperzaehlern hat in den letzten Jahren stetig zugenommen. Der ``Arbeitskreis Inkorporationsueberwachung`` des Fachverbandes fuer Strahlenschutz e.V. hat darum bisherige Erfahrungen zusammengetragen und Empfehlungen fuer den Einsatz dieser Messtechnik erarbeitet. Der Schwerpunkt der Tagung lag beim Vergleich von Germaniumhalbleiter- mit Natriumjodid-Festszintillationsdetektoren.Tl-Detektoren eignen sich v.a. beim Vorhandensein bekannter und zeitlich konstanter Nuklidvektoren (Kernkraftwerke, Nuklearmedizin). Bei unbekanntem bzw. variablem Nuklidvektor (Stoerfall, Unfall, Forschung) sollen Ge-Detektoren benutzt werden (orig./ABI)

Fermi GBM Observations of Terrestrial Gamma Flashes

Science.gov (United States)

Wilson-Hodge, Colleen A.; Briggs, M. S.; Connaughton, V.; Fishman, G. J.; Bhat, P. N.; Paciesas, W. S.; Preece, R. D.; Kippen, R. M.; vonKienlin, A.; Dwyer, J. R.;

Applying ISO 11929:2010 Standard to detection limit calculation in least-squares based multi-nuclide gamma-ray spectrum evaluation

Energy Technology Data Exchange (ETDEWEB)

Kanisch, G., E-mail: guenter.kanisch@hanse.net

2017-05-21

The concepts of ISO 11929 (2010) are applied to evaluation of radionuclide activities from more complex multi-nuclide gamma-ray spectra. From net peak areas estimated by peak fitting, activities and their standard uncertainties are calculated by weighted linear least-squares method with an additional step, where uncertainties of the design matrix elements are taken into account. A numerical treatment of the standard's uncertainty function, based on ISO 11929 Annex C.5, leads to a procedure for deriving decision threshold and detection limit values. The methods shown allow resolving interferences between radionuclide activities also in case of calculating detection limits where they can improve the latter by including more than one gamma line per radionuclide. The co'mmon single nuclide weighted mean is extended to an interference-corrected (generalized) weighted mean, which, combined with the least-squares method, allows faster detection limit calculations. In addition, a new grouped uncertainty budget was inferred, which for each radionuclide gives uncertainty budgets from seven main variables, such as net count rates, peak efficiencies, gamma emission intensities and others; grouping refers to summation over lists of peaks per radionuclide.

Synthesis, characterization and behaviour to gamma radiation of the bis-L-alaninato-copper (II)

International Nuclear Information System (INIS)

Passos, B.F.T.

1985-01-01

The behaviour of coordinated compound obtained from the copper (II) and the L-(+)- alanine to gamma radiation was determined. A study of synthesis and characterization of this complex was made with elementary analysis, ultraviolet and visible electronic spectroscopy, infrared vibrational spectroscopy, proton magnetic resonance spectroscopy and thermo-gravimetric analysis. (C.G.C.)

Gamma-ray imaging spectrometer (GRIS): a new balloon-borne experiment for gamma-ray line astronomy

International Nuclear Information System (INIS)

Teegarden, B.J.; Cline, T.L.; Gehrels, N.; Porreca, G.; Tueller, J.; Leventhal, M.; Huters, A.F.; MacCallum, C.J.; Stang, P.D.

1985-01-01

High resolution gamma-ray spectroscopy is a relatively new field that holds great promise for further understanding of high energy astrophysical processes. Preliminary results such as the annihilation radiation from the galactic center, the 26 Al line from the galactic plane and cyclotron lines from neutron stars may well be just the initial discoveries of a rich and as yet undeveloped field. When the high resolution gamma-ray spectrometer (GRSE) was removed from the GRO payload NASA decided to initiate a balloon program to permit continued development and improvement of instrumentation in this field, as well as continued scientific observations. The Gamma-Ray Imaging Spectrometer (GRIS) is one of the experiments selected as part of this program. The instrument contains a number of new and innovative features that are expected to produce a significant improvement in source location accuracy and sensitivity over previous balloon and satellite experiments. 6 refs., 2 figs

Spectroscopy of {sup 189,187}Pb from gamma-FMA coincidences

Energy Technology Data Exchange (ETDEWEB)

Janssens, R.V.F.; Davids, C.N.; Blumenthal, D. [and others

1995-08-01

The very neutron-deficient Pb isotopes are of much current interest because they exhibit shape coexistence between a spherical groundstate and a deformed prolate excited configuration located very low in excitation energy. Last year the nucleus {sup 186}Pb was studied at the FMA in an FMA-{gamma}-{gamma} coincidence experiment. The purpose of the present measurement was to delineate, for the first time, the groundstate and near groundstate excitations in the odd Pb isotopes {sup 189,187}Pb in order to identify the orbitals which have an important role in driving the nuclear shape. The experiment was performed only very recently at the FMA with 10 Compton-suppressed Ge detectors from the Argonne Notre Dame BGO Gamma-Ray facility. {sup 187}Pb was studied with the {sup 155}Gd({sup 36}Ar,4n) reaction at 179 MeV, while {sup 189}Pb was reached with the {sup 158}Gd({sup 36}Ar,5n) reaction at the same beam energy. The analysis just began. It can already be stated that transitions in both Pb isotopes were identified and that it should be possible to establish level schemes. The presence of possible isomeric states in {sup 189}Pb will be checked in a follow-up experiment planned in Canberra. A similar measurement on {sup 187}Pb appears very difficult because of the very small cross section involved.

Gamma irradiation effect on polymers derived of pyrrole synthesized by plasma

International Nuclear Information System (INIS)

Lopez G, O. G.

2013-01-01

This work studies the effect of gamma irradiation at doses of 50, 100, 200, 400 and 800 kGy on polymers obtained from pyrrole synthesized by plasma. The evolution of the structure was studied by Fourier transform infrared spectroscopy (Ftir) and X-ray photoelectron spectroscopy (XPS). The Ftir spectra show that poly pyrroles have N-H, C-H, C=O, triple and consecutive double bonds in their structure. The irradiated polymers show the same chemical groups in their structure without significant changes. Nevertheless, a more detailed analysis by XPS allows the identification of superficial chemical states, such as: C=CH-C, C=CC-C, C-NH-C, C-NC-C, etc., and shows that most of these states are present in all polymers but with different participation. One possible mechanism indicates that as the irradiation dose increases, dehydrogenation processes are performed increasing fragmentation, crosslinking and formation of multiple bonds. The fragmentation and thermal degradation were studied by thermogravimetric analysis, indicating that the loss of moisture and light compounds formed during gamma irradiation occurs in the firsts 100 grades C. The main degradation of all polymers occurs from 150 to 700 grades C, suggesting that the thermal stability is independent of the irradiation dose in the interval studied. Morphology was studied using scanning electron microscopy techniques. Before irradiation, the polymer presented a uniform and practically smooth surface, however, after gamma irradiation, the applied energy increased roughness and macro fragmentation. The roughness and functional groups on the surface reduced the contact angle with water as the irradiation dose increased. However, the polymers are hydrophilic, because for all doses that contact angle is smaller than 90 grades C. Electrical conductivity was calculated respect to temperature in the interval from 25 to 100 grades C. Conductivity increases with temperature and is slightly greater in the irradiated polymers

An optimum analysis sequence for environmental gamma-ray spectrometry

Energy Technology Data Exchange (ETDEWEB)

De la Torre, F.; Rios M, C.; Ruvalcaba A, M. G.; Mireles G, F.; Saucedo A, S.; Davila R, I.; Pinedo, J. L., E-mail: fta777@hotmail.co [Universidad Autonoma de Zacatecas, Centro Regional de Estudis Nucleares, Calle Cipres No. 10, Fracc. La Penuela, 98068 Zacatecas (Mexico)

2010-10-15

This work aims to obtain an optimum analysis sequence for environmental gamma-ray spectroscopy by means of Genie 2000 (Canberra). Twenty different analysis sequences were customized using different peak area percentages and different algorithms for: 1) peak finding, and 2) peak area determination, and with or without the use of a library -based on evaluated nuclear data- of common gamma-ray emitters in environmental samples. The use of an optimum analysis sequence with certified nuclear information avoids the problems originated by the significant variations in out-of-date nuclear parameters of commercial software libraries. Interference-free gamma ray energies with absolute emission probabilities greater than 3.75% were included in the customized library. The gamma-ray spectroscopy system (based on a Ge Re-3522 Canberra detector) was calibrated both in energy and shape by means of the IAEA-2002 reference spectra for software intercomparison. To test the performance of the analysis sequences, the IAEA-2002 reference spectrum was used. The z-score and the reduced {chi}{sup 2} criteria were used to determine the optimum analysis sequence. The results show an appreciable variation in the peak area determinations and their corresponding uncertainties. Particularly, the combination of second derivative peak locate with simple peak area integration algorithms provides the greater accuracy. Lower accuracy comes from the combination of library directed peak locate algorithm and Genie's Gamma-M peak area determination. (Author)

A Review on Microbial Mutagenesis through Gamma Irradiation for Agricultural Applications

International Nuclear Information System (INIS)

Hoe, P.C.K.; Khairuddin Abdul Rahim

2016-01-01

Gamma irradiation is widely used in sterilization and mutagenesis, especially for plant breeding and crop protection. Microbial mutagenesis through gamma irradiation is mainly applied in fermentation industry. In agriculture, gamma irradiation is mostly applied in crop improvement. Microbial mutagenesis is mainly applied against fungus and spore-forming bacteria, which are resistant to gamma irradiation. Response of microbes to gamma irradiation varies and depends on various factors. Review of previous works on gamma irradiation for microbial mutagenesis in agriculture may provide some information for the use of this method. The general view on gamma irradiation, its application, and mutagenesis are discussed in this paper. Further investigation on microbial mutagenesis should consider molecular changes, information on which is lacking in previous works. Moreover, studies on microbial mutagenesis are still lacking in Malaysia despite having several gamma irradiation facilities. Therefore, further studies on microbial mutagenesis should be conducted. (author)

Internet accessible hot cell with gamma spectroscopy at the Missouri S and T nuclear reactor

Energy Technology Data Exchange (ETDEWEB)

Grant, Edwin [Nuclear Engineering, Missouri University of Science and Technology, 203 Fulton Hall, 300 W. 13th St., Rolla, MO 65409 (United States); Mueller, Gary, E-mail: gmueller@mst.edu [Nuclear Engineering, Missouri University of Science and Technology, 203 Fulton Hall, 300 W. 13th St., Rolla, MO 65409 (United States); Castano, Carlos; Usman, Shoaib; Kumar, Arvind [Nuclear Engineering, Missouri University of Science and Technology, 203 Fulton Hall, 300 W. 13th St., Rolla, MO 65409 (United States)

2011-08-15

Highlights: > A dual-chambered internet-accessible heavily shielded facility has been built. > The facility allows distance users to analyze neutron irradiated samples remotely. > The Missouri S and T system uses computer automation with user feedback. > The system can analyze multiple samples and assist several researchers concurrently. - Abstract: A dual-chambered internet-accessible heavily shielded facility with pneumatic access to the University of Missouri Science and Technology (Missouri S and T) 200 kW Research Nuclear Reactor (MSTR) core has been built and is currently available for irradiation and analysis of samples. The facility allows authorized distance users engaged in collaborative activities with Missouri S and T to remotely manipulate and analyze neutron irradiated samples. The system consists of two shielded compartments, one for multiple sample storage, and the other dedicated exclusively for radiation measurements and spectroscopy. The second chamber has multiple detector ports, with graded shielding, and has the capability to support gamma spectroscopy using radiation detectors such as an HPGe detector. Both these chambers are connected though a rapid pneumatic system with access to the MSTR nuclear reactor core. This new internet-based system complements the MSTR's current bare pneumatic tube (BPT) and cadmium lined pneumatic tube (CPT) facilities. The total transportation time between the core and the hot cell, for samples weighing 10 g, irradiated in the MSTR core, is roughly 3.0 s. This work was funded by the DOE grant number DE-FG07-07ID14852 and expands the capabilities of teaching and research at the MSTR. It allows individuals who do not have on-site access to a nuclear reactor facility to remotely participate in research and educational activities.

Internet accessible hot cell with gamma spectroscopy at the Missouri S and T nuclear reactor

International Nuclear Information System (INIS)

Grant, Edwin; Mueller, Gary; Castano, Carlos; Usman, Shoaib; Kumar, Arvind

2011-01-01

Highlights: → A dual-chambered internet-accessible heavily shielded facility has been built. → The facility allows distance users to analyze neutron irradiated samples remotely. → The Missouri S and T system uses computer automation with user feedback. → The system can analyze multiple samples and assist several researchers concurrently. - Abstract: A dual-chambered internet-accessible heavily shielded facility with pneumatic access to the University of Missouri Science and Technology (Missouri S and T) 200 kW Research Nuclear Reactor (MSTR) core has been built and is currently available for irradiation and analysis of samples. The facility allows authorized distance users engaged in collaborative activities with Missouri S and T to remotely manipulate and analyze neutron irradiated samples. The system consists of two shielded compartments, one for multiple sample storage, and the other dedicated exclusively for radiation measurements and spectroscopy. The second chamber has multiple detector ports, with graded shielding, and has the capability to support gamma spectroscopy using radiation detectors such as an HPGe detector. Both these chambers are connected though a rapid pneumatic system with access to the MSTR nuclear reactor core. This new internet-based system complements the MSTR's current bare pneumatic tube (BPT) and cadmium lined pneumatic tube (CPT) facilities. The total transportation time between the core and the hot cell, for samples weighing 10 g, irradiated in the MSTR core, is roughly 3.0 s. This work was funded by the DOE grant number DE-FG07-07ID14852 and expands the capabilities of teaching and research at the MSTR. It allows individuals who do not have on-site access to a nuclear reactor facility to remotely participate in research and educational activities.

Next Generation Gamma/Neutron Detectors for Planetary Science., Phase I

Data.gov (United States)

National Aeronautics and Space Administration — Gamma ray and neutron spectroscopy are well established techniques for determining the chemical composition of planetary surfaces, and small cosmic bodies such as...

A twin Frisch-grid ionization chamber as a selective detector for the delayed gamma-spectroscopy of fission fragments

Energy Technology Data Exchange (ETDEWEB)

Gaudefroy, L., E-mail: laurent.gaudefroy@cea.fr [CEA, DAM, DIF, F-91297 Arpajon (France); Roger, T., E-mail: roger@ganil.fr [GANIL, CEA/DSM-CNRS/IN2P3, BP 55027, F-14076 Caen (France); Pancin, J., E-mail: pancin@ganil.fr [GANIL, CEA/DSM-CNRS/IN2P3, BP 55027, F-14076 Caen (France); Spitaels, C. [GANIL, CEA/DSM-CNRS/IN2P3, BP 55027, F-14076 Caen (France); Aupiais, J. [CEA, DAM, DIF, F-91297 Arpajon (France); Mottier, J. [Institut de Physique Nucléaire, Université Paris-Sud-11-CNRS-IN2P3, F-91406 Orsay (France)

2017-05-21

We present a twin Frisch-grid ionization chamber. The detector is meant to provide high selective power for the study of delayed gamma-ray spectroscopy of fission fragments produced via {sup 252}Cf spontaneous fission. A mean energy resolution on the kinetic energy of fission fragments of 675 keV (FWHM) is achieved and allows us to resolve masses of fragments for fission events where neutron emission is not energetically possible. The mean mass resolution measured for these particular events amounts to 0.54 mass units (FWHM). For fission events with neutron emission a resolution of 4 mass units (FWHM) is reported. Information on fragment emission angle is measured with a resolution of 0.1 on the difference of the cosines determined for both halves of the detector. A charge resolution of 4.5 charge units (FWHM) is also demonstrated.

Establishment of Imaging Spectroscopy of Nuclear Gamma-Rays based on Geometrical Optics.

Science.gov (United States)

Tanimori, Toru; Mizumura, Yoshitaka; Takada, Atsushi; Miyamoto, Shohei; Takemura, Taito; Kishimoto, Tetsuro; Komura, Shotaro; Kubo, Hidetoshi; Kurosawa, Shunsuke; Matsuoka, Yoshihiro; Miuchi, Kentaro; Mizumoto, Tetsuya; Nakamasu, Yuma; Nakamura, Kiseki; Parker, Joseph D; Sawano, Tatsuya; Sonoda, Shinya; Tomono, Dai; Yoshikawa, Kei

2017-02-03

Since the discovery of nuclear gamma-rays, its imaging has been limited to pseudo imaging, such as Compton Camera (CC) and coded mask. Pseudo imaging does not keep physical information (intensity, or brightness in Optics) along a ray, and thus is capable of no more than qualitative imaging of bright objects. To attain quantitative imaging, cameras that realize geometrical optics is essential, which would be, for nuclear MeV gammas, only possible via complete reconstruction of the Compton process. Recently we have revealed that "Electron Tracking Compton Camera" (ETCC) provides a well-defined Point Spread Function (PSF). The information of an incoming gamma is kept along a ray with the PSF and that is equivalent to geometrical optics. Here we present an imaging-spectroscopic measurement with the ETCC. Our results highlight the intrinsic difficulty with CCs in performing accurate imaging, and show that the ETCC surmounts this problem. The imaging capability also helps the ETCC suppress the noise level dramatically by ~3 orders of magnitude without a shielding structure. Furthermore, full reconstruction of Compton process with the ETCC provides spectra free of Compton edges. These results mark the first proper imaging of nuclear gammas based on the genuine geometrical optics.

Mixed gamma emitting gas standard and method

International Nuclear Information System (INIS)

McFarland, R.C.; McFarland, P.A.

1986-01-01

The invention in one aspect pertains to a method of calibrating gamma spectroscopy systems for gas counting in a variety of counting containers comprising withdrawing a precision volume of a mixed gamma-emitting gas standard from a precision volume vial and delivering the withdrawn precision volume of the gas standard to the interior of a gas counting container. Another aspect of the invention pertains to a mixed gamma-emitting gas standard, comprising a precision spherical vial of predetermined volume, multiple mixed emitting gas components enclosed within the vial, and means for withdrawing from the vial a predetermined amount of the components wherein the gas standard is used to calibrate a gamma spectrometer system for gas counting over a wide energy range without the use of additional standards. A third aspect comprehends a gamma spectrometer calibration system for gas counting, comprising a precision volume spherical glass vial for receiving mixed multiisotope gas components, and two tubular arms extending from the vial. A ground glass stopcock is positioned on each arm, and the outer end of one arm is provided with a rubber septum port

Applying a low energy HPGe detector gamma ray spectrometric technique for the evaluation of Pu/Am ratio in biological samples.

Science.gov (United States)

Singh, I S; Mishra, Lokpati; Yadav, J R; Nadar, M Y; Rao, D D; Pradeepkumar, K S

2015-10-01

The estimation of Pu/(241)Am ratio in the biological samples is an important input for the assessment of internal dose received by the workers. The radiochemical separation of Pu isotopes and (241)Am in a sample followed by alpha spectrometry is a widely used technique for the determination of Pu/(241)Am ratio. However, this method is time consuming and many times quick estimation is required. In this work, Pu/(241)Am ratio in the biological sample was estimated with HPGe detector based measurements using gamma/X-rays emitted by these radionuclides. These results were compared with those obtained from alpha spectroscopy of sample after radiochemical analysis and found to be in good agreement. Copyright © 2015 Elsevier Ltd. All rights reserved.

Plutonium isotopic measurements by gamma-ray spectroscopy

International Nuclear Information System (INIS)

Gunnink, R.

1973-11-01

A method is reported for analysis of isotopic and total plutonium by detecting and analyzing gamma rays emitted by the sample. A computerized prototype-system was developed and is now being routinely used at the Savannah River Plant for the nondestructive assay of solution samples. The analyses for 238 Pu, 239 Pu, 240 Pu, 241 Pu, and for 241 Am, when it is present, can be made in counting times as short as 10 to 15 minutes under optimum conditions. Comparison of isotopic ratio values with mass spectrometry generally shows agreement within 0.1 percent for 239 Pu and about 1 percent for 240 Pu and 241 Pu. Some preliminary isotopic measurements on solids are also discussed. (U.S.)

Feasibility of applying gamma irradiation as disinfestation technique on date fruits in respect to nutritional value that is affected by disinfesting gamma ray doses

International Nuclear Information System (INIS)

Ahmed, El-Sayed S.

1976-01-01

Infested and non-infested dry date fruits (Phonex dactylifera), Abrimi variety (9.2% moisture), with Ephestia cautella Walker were irradiated for 0, 15, 20 and 40 Krad gamma ray doses emitted from Co-60 source with 1.36 x 10-rad/h. as a dose rate. Irradiated fruits were stored at room temperature, at 20-25 0 C and 85-95% R.H., in packages to avoid reinfestation. A dose of 20 Krad is 100 percent effective in preventing the emergency of eggs, larva, and pupae in fruits as reflected by zero per cent emergency count for live adults. Also, this dose was found to be lethal for adult stage of the insect. On the other hand, 2 Krad dose does not produce significant changes in the nutritional qualities of fruits, as measured by chemical analytical means for carbohydrates, protein and amino acids, directly after irradiation as well as at 2, 4 and 6 months storage. The triangular tests show that irradiation treatments even with 4 Krad exerted no determinal effect upon the sensory qualities of stored irradiated date fruits. These results point out the feasibility of applying gamma irradiation, 20 Krad, as disinfestation technique against Ephestia cautella Walker in dry date fruits without exerting any effect on the nutritional value

Nuclear structure studies on 178Hf by means of neutron induced gamma and electron spectroscopy

International Nuclear Information System (INIS)

Al Mamun Imtiazul Haque.

1985-01-01

By means of thermal and epithermal neutron captures the nucleus 178 Hf was studied. With high-resolution spectrometers the gamma transitions and conversion electrons were measured. By the found energies, intensities, and multipolarities the level scheme of 178 Hf could be essentially improved and extended. Totally 270 secondary (from 600 gamma lines) and 39 primary gamma transitions were used in order to establish the level scheme with 66 levels in 18 rotational bands. For this 92% of all gamma intensities were used. Several new rotational bands were established. By improved gamma energies the level scheme below 2 MeV for spins between 0 and 6 is well confirmed. Moreover by the resolution of several multiplets the decay structure of the levels could be explained. The thermal neutron capture state results from the primary gamma transitions to Q n =7626.34 (23) keV. Electrical monopole transitions from several states were studied in order to determine the X(E0/E2) values. (orig./HSI) [de

A Framework for the Relative and Absolute Performance Evaluation of Automated Spectroscopy Systems

International Nuclear Information System (INIS)

Portnoy, David; Heimberg, Peter; Heimberg, Jennifer; Feuerbach, Robert; McQuarrie, Allan; Noonan, William; Mattson, John

2009-01-01

The development of high-speed, high-performance gamma-ray spectroscopy algorithms is critical to the success of many automated threat detection systems. In response to this need a proliferation of such algorithms has taken place. With this proliferation comes the necessary and non-trivial task of validation. There is (and always will be) insufficient experimental data to determine performance of spectroscopy algorithms over the relevant factor space at any reasonable precision. In the case of gamma-ray spectroscopy, there are hundreds of radioisotopes of interest, which may come in arbitrary admixtures, there are many materials of unknown quantity, which may be found in the intervening space between the source and the detection system, and there are also irregular variations in the detector systems themselves. All of these factors and more should be explored to determine algorithm/system performance. This paper describes a statistical framework for the performance estimation and comparison of gamma-ray spectroscopy algorithms. The framework relies heavily on data of increasing levels of artificiality to sufficiently cover the factor space. At each level rigorous statistical methods are employed to validate performance estimates.

Future perspective of meson spectroscopy studies at KEK-PS

International Nuclear Information System (INIS)

Tsuru, T.

1992-01-01

Physics of light-quark meson spectroscopy at present is simply reviewed and a direction of next generation experiment is investigated. A new charge and gamma spectrometer is proposed to push forward next generation physics at KEK-PS. It should have almost 4π acceptance for both charged particles and gamma's and have options of π/K separation and good π 0 /γ separation. (author)

Application of gamma-gamma logging in predicting anomalous geodynamic phenomena in hard coal mines

International Nuclear Information System (INIS)

Blaha, F.; Keclik, L.

1980-01-01

The application is discussed of gamma-gamma logging in the prediction of dynamic events like coal and gas bursts, coal sliding in medium dip seams and rock bumps. The overall analysis of the applied rock characterization method and of the measurement results shows that the prediction possibilities of dynamic events are partly limited due to specific effects of the rock massive. In these cases, however, unambiguous results may be obtained by other geophysical methods such as seismoacoustic testing etc. In most cases, however, the gamma-gamma logging results may be used for estimating the degree of dynamic events or checking the efficiency of preventive measures in the locality under investigation. (author)

OBSERVATION OF CORRELATED OPTICAL AND GAMMA EMISSIONS FROM GRB 081126

International Nuclear Information System (INIS)

Klotz, A.; Boer, M.; Gendre, B.; Atteia, J. L.; Coward, D. M.; Imerito, A. C.

2009-01-01

We present an analysis of time-resolved optical emissions observed from the gamma-ray burst GRB 081126 during the prompt phase. The analysis employed time-resolved photometry using optical data obtained by the TAROT telescope, using BAT data from the Swift spacecraft, and time-resolved spectroscopy at high energies from the GBM instrument onboard the Fermi spacecraft. The optical emission of GRB 081126 is found to be compatible with the second gamma emission pulse shifted by a positive time lag of 8.4 ± 3.9 s. This is the first well-resolved observation of a time lag between optical and gamma emissions during a gamma-ray burst. Our observations could potentially provide new constraints on the fireball model for gamma-ray burst early emissions. Furthermore, observations of time lags between optical and gamma ray photons provides an exciting opportunity to constrain quantum gravity theories.

A Correlated Optical and Gamma Emission from GRB 081126A

International Nuclear Information System (INIS)

Gendre, B.; Klotz, A.; Atteia, J. L.; Boeer, M.; Coward, D. M.; Imerito, A. C.

2010-01-01

We present an analysis of time-resolved optical emissions observed from the gamma-ray burst GRB 081126 during the prompt phase. The analysis employed time-resolved photometry using optical data obtained by the TAROT telescope, BAT data from the Swift spacecraft and time-resolved spectroscopy at high energies from the GBM instrument onboard the Fermi spacecraft. The optical emission of GRB 081126 is found to be compatible with the second gamma emission pulse shifted by a positive time-lag of 8.4±3.9 sec. This is the first well resolved observation of a time lag between optical and gamma emissions during a gamma-ray burst. Our observations could potentially provide new constraints on the fireball model for gamma ray burst early emissions. Furthermore, observations of time-lags between optical and gamma ray photons provides an exciting opportunity to constrain quantum gravity theories.

In vivo magnetic resonance spectroscopy measurement of gray-matter and white-matter gamma-aminobutyric acid concentration in sensorimotor cortex using a motion-controlled MEGA point-resolved spectroscopy sequence.

Science.gov (United States)

Bhattacharyya, Pallab K; Phillips, Micheal D; Stone, Lael A; Lowe, Mark J

2011-04-01

Gamma-aminobutyric acid (GABA) is a major inhibitory neurotransmitter in the brain. Understanding the GABA concentration, in vivo, is important to understand normal brain function. Using MEGA point-resolved spectroscopy sequence with interleaved water scans to detect subject motion, GABA level of sensorimotor cortex was measured using a voxel identified from a functional magnetic resonance imaging scan. The GABA level in a 20×20×20-mm(3) voxel consisting of 37%±7% gray matter, 52%±12% white matter and 11%±8% cerebrospinal fluid in the sensorimotor region was measured to be 1.43±0.48 mM. In addition, using linear regression analysis, GABA concentrations within gray and white matter were calculated to be 2.87±0.61 and 0.33±0.11 mM, respectively. Copyright © 2011 Elsevier Inc. All rights reserved.

{sup 41}K(n, {gamma}){sup 42}K thermal and resonance integral cross section measurements

Energy Technology Data Exchange (ETDEWEB)

Ferreira, F.A. Jr.; Maidana, N.L.; Vanin, V.R. [Sao Paulo Univ., SP (Brazil). Lab. do Acelerador Linear; Dias, M.S.; Koskinas, M.F. [IPEN-CNEN, Sao Paulo, SP (Brazil). Lab. de Metrolgia Nuclear; Lopez-Pino, N. [Instituto Superior de Tecnolgias y Ciencias Aplicadas (InSTEC), Habana (Cuba)

2012-07-01

We measured the {sup 41}K thermal neutron absorption and resonance integral cross sections after the irradiation of KNO{sub 3} samples near the core of the IEA-R1 IPEN pool-type research reactor. Bare and cadmium-covered targets were irradiated in pairs with Au-Al alloy flux-monitors. The residual activities were measured by gamma-ray spectroscopy with a HPGe detector, with special care to avoid the {sup 42}K decay {beta}{sup -} emission effects on the spectra. The gamma-ray self-absorption was corrected with the help of MCNP simulations. We applied the Westcott formalism in the average neutron flux determination and calculated the depression coefficients for thermal and epithermal neutrons due to the sample thickness with analytical approximations. We obtained 1.57(4) b and 1.02(4) b, for thermal and resonance integral cross sections, respectively, with correlation coefficient equal to 0.39.

Application of a gamma spectroscopy system to the measurement of neutron cross sections necessary to the development of nuclear energy; Mise au point d'un systeme de spectroscopie pour mesurer des sections efficaces neutroniques applicables a un possible developpement du nucleaire comme source d'energie

Energy Technology Data Exchange (ETDEWEB)

Deruelle, O

2002-09-01

This work concerns the development of nuclear energy and nuclear waste management in particular. Two parts of this study can be distinguished. In the first part (theoretical), a thorium-plutonium fuel based on MOX and dedicated for PWR was investigated in order to transmute plutonium in a potentially low waste fuel cycle. It was shown that this type of fuel is not regenerative but could be used for a transition to the industrial thorium fuel cycle without building new reactors. Thanks to moderated neutron spectra and high loaded actinide mass in the core, U-233 is quickly created ({approx}300 kg/y) for a loss of about {approx}1200 kg of fissile plutonium. In the second part (experimental), we have developed and built a new reaction chamber to measure neutron cross sections of actinides by alpha-gamma spectroscopy. This experimental device (in principle transportable) was commissioned in the high flux reactor of ILL Grenoble. Neutron flux was measured by gamma spectroscopy of irradiated Al and Co samples and was found to be of the order of 6,0. 10{sup 14} n.cm{sup -2}.s{sup -1} (4%). By the irradiation of 11{mu}g of Am-243 and Pu-242, corresponding capture cross sections were measured in the thermal neutron flux at 50 deg C. These are the results: {sup 243}Am(n,{gamma}) {sup 244fond.}Am = 4,72{+-}1,42b; {sup 243}Am(n,{gamma}) {sup 244total}Am = 74,8{+-}3,25b; {sup 242}Pu (n,{gamma}){sup 243}Pu = 22,7{+-}1,09b. Uncertainties of the measurements are mostly due to the determination of the neutron flux, efficiency of the electronics and ambiguities related to the definition of the area under {alpha}-{gamma} spectra. Although our measured cross sections deviate (by 10-30%) from the corresponding values widely used in evaluated data libraries such as ENDF, JEF and JENDL, in this work we have demonstrated the feasibility and principle of our experimental method. Furthermore, the value for the 243-americium capture cross-section is in very good agreement with the last two

Numerical study on determining formation porosity using a boron capture gamma ray technique and MCNP.

Science.gov (United States)

Liu, Juntao; Zhang, Feng; Wang, Xinguang; Han, Fei; Yuan, Zhelong

2014-12-01

Formation porosity can be determined using the boron capture gamma ray counting ratio with a near to far detector in a pulsed neutron-gamma element logging tool. The thermal neutron distribution, boron capture gamma spectroscopy and porosity response for formations with different water salinity and wellbore diameter characteristics were simulated using the Monte Carlo method. We found that a boron lining improves the signal-to-noise ratio and that the boron capture gamma ray counting ratio has a higher sensitivity for determining porosity than total capture gamma. Copyright © 2014 Elsevier Ltd. All rights reserved.

Study of 16O-induced deep inelastic nuclear reactions on 27Al, 48Ti, and 58Ni by spectroscopy of the gamma radiation from the reaction products

International Nuclear Information System (INIS)

Puchta, H.

1980-01-01

The present thesis deals with the spectroscopy of the gamma radiation from the reaction fragments after binary reactions in the systems 16 O + 27 Al, 48 Ti, and 58 Ni at incident energies from 90 to 100 MeV, i.e. far above the Coulomb threshold. ΔE-E telescopes, which were located at 35 0 to the beam direction, detected the projectile-like fragments and defined the reaction channel and the scattering plane. In coincidence to this the gamma quanta in a 120-cm 3 -Ge(Li)-diode and a 27 x 33-cm-NaI-spectrometer were observed. The gamma spectra are equal to those observed hitherto in fusion reactions except for the high energetic gamma lines from the ejectiles, which are raised from the gamma continuum of the heavy fragments. From the spectroscoped gamma radiation for the light as for the heavy fragments the excitation energy, the value of the fragment angular momentum, as well as the occupation of the magnetic sublevels could be determined. The hard projectile 16 O transfers the dissipated energy and the angular momentum transferred by the spin of the fragments nearly completely into the residue nucleus. The probability for the observation of a ground state transition in one of the heavy fragments extends to (0.85 +- 0.10) per carbon ejectile in the system 16 O + 48 Ti. The residue nucleus distribution corresponds to that expected by the statistical model from the decay of the compound-nucleus 52 Cr belonging to the ejectile 12 C, the excitation energy of which corresponds to the reaction Q-value. (orig./HSI) [de

A segmented detector for airbone gamma ray spectroscopy

Energy Technology Data Exchange (ETDEWEB)

Burgada, G.; Iovene, A.; Petrucci, S.; Tintori, C., E-mail: g.burgada@caen.it [Costruzioni Apparecchiature Elettroniche Nucleari S.p.A. (CAEN), Viareggio (Italy); Alvarez, M.A.G., E-mail: malvarez@if.usp.br [Universidade de Sao Paulo (IF/USP), Sao Paulo, SP (Brazil). Instituto de Fisica; Baldoncini, M.; Xhixha, G.; Strati, V., E-mail: gerti.xhixha@unife.it [University of Ferrara, Department of Physics and Earth Sciences, Ferrara (Italy); Mantovani, F., E-mail: mantovani@fe.infn.it [Istituto Nazionale di Fisica Nucleare (INFN), Ferrara (Italy); Garosi, P.; Mou, L., E-mail: li.mou@libero.it [University of Siena (Italy); Alvarez, C. Rossi, E-mail: rossialvarez@pd.infn.it [Istituto Nazionale di Fisica Nucleare (INFN), Legnaro (Italy)

2014-07-01

The airborne gamma-ray spectrometry (AGRS) is widely acknowledged as a very efficient technique for large areas monitoring. The detector system mounted on a helicopter allows for an extensive survey in a single flight time, thus reducing the exposure risk for the operator. Results from AGRS techniques are exploited in many fields, from the geological research to the homeland security for the search of orphan radioactive sources, from the mining and hydrocarbon exploration to the construction industry. The new generation of compact digital data acquisition and online processing equipment allows for faster airborne survey campaigns, and enhances the flexibility of operations. In addition, the algorithm for the extrapolation of the nuclide concentrations from the acquired gamma spectra is a challenging step of the entire technique. We are going to present a new device for advanced AGRS measurements, with an innovative detector configuration and data processing algorithms for optimizing the source localization and the on-line response capabilities. The new compact structure makes the system easily portable by a single operator, and rapidly mountable on most common helicopters. Preliminary feasibility studies have been performed to test the mechanics and the hardware of the whole system, which is intended to work without any human attendance. The first flights are planned by the end of 2014, with the aim of detecting artificial point sources having intensities on the order of 10^8 Bq and natural enriched fields already monitored. (author)

A segmented detector for airbone gamma ray spectroscopy

International Nuclear Information System (INIS)

Burgada, G.; Iovene, A.; Petrucci, S.; Tintori, C.; Alvarez, M.A.G.; Mantovani, F.; Garosi, P.; Mou, L.; Alvarez, C. Rossi

2014-01-01

The airborne gamma-ray spectrometry (AGRS) is widely acknowledged as a very efficient technique for large areas monitoring. The detector system mounted on a helicopter allows for an extensive survey in a single flight time, thus reducing the exposure risk for the operator. Results from AGRS techniques are exploited in many fields, from the geological research to the homeland security for the search of orphan radioactive sources, from the mining and hydrocarbon exploration to the construction industry. The new generation of compact digital data acquisition and online processing equipment allows for faster airborne survey campaigns, and enhances the flexibility of operations. In addition, the algorithm for the extrapolation of the nuclide concentrations from the acquired gamma spectra is a challenging step of the entire technique. We are going to present a new device for advanced AGRS measurements, with an innovative detector configuration and data processing algorithms for optimizing the source localization and the on-line response capabilities. The new compact structure makes the system easily portable by a single operator, and rapidly mountable on most common helicopters. Preliminary feasibility studies have been performed to test the mechanics and the hardware of the whole system, which is intended to work without any human attendance. The first flights are planned by the end of 2014, with the aim of detecting artificial point sources having intensities on the order of 10^8 Bq and natural enriched fields already monitored. (author)

Characterization of Campylobacter jejuni applying flaA short variable region sequencing, multilocus sequencing and Fourier transform infrared spectroscopy

DEFF Research Database (Denmark)

Josefsen, Mathilde Hartmann; Bonnichsen, Lise; Larsson, Jonas

flaA short variable region sequencing and phenetic Fourier transform infrared (FTIR) spectroscopy was applied on a collection of 102 Campylobacter jejuni isolated from continuous sampling of organic, free range geese and chickens. FTIR has been shown to serve as a valuable tool in typing...

Inverse Compton gamma-rays from pulsars

International Nuclear Information System (INIS)

Morini, M.

1983-01-01

A model is proposed for pulsar optical and gamma-ray emission where relativistic electrons beams: (i) scatter the blackbody photons from the polar cap surface giving inverse Compton gamma-rays and (ii) produce synchrotron optical photons in the light cylinder region which are then inverse Compton scattered giving other gamma-rays. The model is applied to the Vela pulsar, explaining the first gamma-ray pulse by inverse Compton scattering of synchrotron photons near the light cylinder and the second gamma-ray pulse partly by inverse Compton scattering of synchrotron photons and partly by inverse Compton scattering of the thermal blackbody photons near the star surface. (author)

The influence of gamma irradiation on natural dyeing properties of cotton and flax fabrics

Science.gov (United States)

Chirila, Laura; Popescu, Alina; Cutrubinis, Mihalis; Stanculescu, Ioana; Moise, Valentin Ioan

2018-04-01

Fabrics made of 100% cotton and 100% flax respectively were exposed at ambient temperature to gamma radiation doses, from 5 to 40 kGy, using a Co-60 research irradiator. After the irradiation treatment the fabrics were subjected to dyeing process with Itodye Nat Pomegranate commercial natural dye. The influence of gamma irradiation treatment on the physical-mechanical properties, dyeing and surface morphology of natural fibres were investigated. Gamma ray treatment of 40 kGy was the most effective in the case of fabrics made from 100% cotton, enhancing the colour strength as evidenced by K/S value. The results obtained from the mechanical properties of fabrics made of 100% flax indicated that the dose of 40 kGy leads to a decrease of tensile strength up of to 41.5%. Infrared spectroscopy was used to monitor chemical and structural changes in cellulosic fibres induced during processing. Crystallinity indices calculated from various bands ratio showed insignificant variations for cotton and small variations in the case of flax. The surface morphology of irradiated cotton fabrics did not show significant changes even at the highest dose of 40 kGy, while the low doses applied on flax fabrics led to an appearance of small changes of surface morphology. The gamma irradiation increased the uptake of natural dyes on natural cellulosic fibres.

About cosmic gamma ray lines

Science.gov (United States)

Diehl, Roland

2017-06-01

Gamma ray lines from cosmic sources convey the action of nuclear reactions in cosmic sites and their impacts on astrophysical objects. Gamma rays at characteristic energies result from nuclear transitions following radioactive decays or high-energy collisions with excitation of nuclei. The gamma-ray line from the annihilation of positrons at 511 keV falls into the same energy window, although of different origin. We present here the concepts of cosmic gamma ray spectrometry and the corresponding instruments and missions, followed by a discussion of recent results and the challenges and open issues for the future. Among the lessons learned are the diffuse radioactive afterglow of massive-star nucleosynthesis in 26Al and 60Fe gamma rays, which is now being exploited towards the cycle of matter driven by massive stars and their supernovae; large interstellar cavities and superbubbles have been recognised to be of key importance here. Also, constraints on the complex processes making stars explode as either thermonuclear or core-collapse supernovae are being illuminated by gamma-ray lines, in this case from shortlived radioactivities from 56Ni and 44Ti decays. In particular, the three-dimensionality and asphericities that have recently been recognised as important are enlightened in different ways through such gamma-ray line spectroscopy. Finally, the distribution of positron annihilation gamma ray emission with its puzzling bulge-dominated intensity disctribution is measured through spatially-resolved spectra, which indicate that annihilation conditions may differ in different parts of our Galaxy. But it is now understood that a variety of sources may feed positrons into the interstellar medium, and their characteristics largely get lost during slowing down and propagation of positrons before annihilation; a recent microquasar flare was caught as an opportunity to see positrons annihilate at a source.

Optimal Shape of a Gamma-ray Collimator: single vs double knife edge

Science.gov (United States)

Metz, Albert; Hogenbirk, Alfred

2017-09-01

Gamma-ray collimators in nuclear waste scanners are used for selecting a narrow vertical segment in activity measurements of waste vessels. The system that is used by NRG uses tapered slit collimators of both the single and double knife edge type. The properties of these collimators were investigated by means of Monte Carlo simulations. We found that single knife edge collimators are highly preferable for a conservative estimate of the activity of the waste vessels. These collimators show much less dependence on the angle of incidence of the radiation than double knife edge collimators. This conclusion also applies to cylindrical collimators of the single knife edge type, that are generally used in medical imaging spectroscopy.

Synthesis, characterization and behaviour of trans-bis (argininate) copper (II) to gamma radiation

International Nuclear Information System (INIS)

Pereira, A.B.

1984-01-01

The synthesis, the characterization and the behaviour to gamma radiation of trans-bis (argininate) copper (II) are presented. The synthesis is made from copper sulfate, sodium hydroxide and hydrochloride of L (+) arginine, in aqueous medium, and the characterization by infrared spectroscopy, visible and ultraviolet spectroscopy and elementary analysis. (C.G.C.)

$\\gamma$- spectroscopy of n-rich $^{95,96}$Rb nuclei by the incomplete fusion reaction of $^{94}$Kr on $^{7}$Li: Introduction to HIE-ISOLDE studies of n-rich Sb and Tl isotopes with Sn and Hg radioactive beams.

CERN Document Server

Fornal, B; Bednarczyk, P; Cieplicka, N; Krolas, W; Maj, A; Leoni, S; Benzoni, G; Blasi, N; Bottoni, S; Bracco, A; Camera, F; Crespi, F; Million, B; Morales, A; Wieland, O; Rusek, K; Lunardi, S; Mengoni, D; Recchia, F; Ur, CA; Valiente-Dobon, J; de France, G; Clement, E; Elseviers, J; Flavigny, F; Huyse, M; Raabe, R; Sambi, S; Van Duppen, P; Sferrazza, M; Simpson, G; Georgiev, G; Sotty, C; Blazhev, A; German, R; Siebeck, B; Seidlitz, M; Reiter, P; Warr, N; Boenig, S; Ilieva, S; Kroell, T; Scheck, M; Thurauf, M; Gernhaeuser, R; Mucher, D; Janssens, R; Carpenter, MP; Zhu, S; Marginean, NM; Balabanski, D; Kowalska, M

2012-01-01

$\\gamma$- spectroscopy of n-rich $^{95,96}$Rb nuclei by the incomplete fusion reaction of $^{94}$Kr on $^{7}$Li: Introduction to HIE-ISOLDE studies of n-rich Sb and Tl isotopes with Sn and Hg radioactive beams.

Observation of immobile regions in natural rubber at ambient temperature by solid-state C-13 CP/MAS NMR spectroscopy

DEFF Research Database (Denmark)

Larsen, F.H.; Rasmussen, T.; Pedersen, Walther Batsberg

1999-01-01

Employing C-13 CP/MAS NMR spectroscopy, the existence of immobile regions in natural rubber (cis-1,4-polyisoprene) corresponding to a few percent of the monomer units has been detected at ambient temperature. For synthetic rubbers no immobile regions have been detected at all. Applying different...... physical and chemical treatments to natural rubber it is shown that mastication, gamma-irradiation, and increasing the temperature, slightly above the ambient, reduce the amount of immobile regions. (C) 1999 Elsevier Science Ltd. All rights reserved....

Shaly sand evaluation using gamma ray spectrometry, applied to the North Sea Jurassic

International Nuclear Information System (INIS)

Marett, G.; Chevalier, P.; Souhaite, P.; Suau, J.

1976-01-01

In formations where radioactive minerals other than clay are present, their effects on log responses result in a reduction of the accuracy of determination of the shale fraction. The gamma ray log, which is one of the primary indicators for shaliness determination, is the most affected; other logs used in shaliness indicators are also influenced, particularly when heavy minerals are present, such as those encountered in the micaceous sandstones of the North Sea Jurassic. For comparison purposes, possible ways to correct for heavy radioactive minerals using a conventional logging suite are described. Computer processed examples illustrate the results obtained. A different approach is through an analysis of the natural gamma ray spectrum of the formation, as determined with the gamma ray spectrometry tool. Natural gamma rays originate from the radioactive isotope of potassium and the radioactive elements of the uranium and thorium series. Each of these three elements contributes its distinctive spectrum to that of the formation in proportion to its abundance. Thus, by analysis of the formation spectrum, the presence of each can be detected and its amount estimated. This makes possible quantitative corrections to the shaliness indicators. A computer program which performs the necessary computations is described, and several log examples using this technique are presented

Pulser injection with subsequent removal for gamma-ray spectrometry

International Nuclear Information System (INIS)

Hartwell, J.K.; Goodwin, S.G.; Johnson, L.O.; Killian, E.W.

1990-01-01

This patent describes a module for use with a gamma-ray spectroscopy system. The system includes a gamma-ray detector for detecting gamma-ray events and producing a signal representing the gamma-ray events, a converter responsive to the detector and capable of converting the signal to a spectrum, a storage memory responsive to the converter and capable of storing the spectrum at address locations in memory, and a pulser capable of injecting pulses into the signal produced by the detector. The module comprises: means for generating a logic pulse for controlling the pulser, the controlling means adapted for coupling to the pulser; means for generating separation of events logic to isolate the components of a combined gamma-ray---pulse spectrum, the separation of events logic means adapted for coupling to the converter and the storage memory with the capability of storing pulses at address locations in the storage memory separate from the gamma-ray events; means for receiving an imitating signal from the converter to generate a plurality of operations by the module; means for tracking variations in a gamma-ray---pulse spectrum brought on by external parameter changes; and means for interfacing with commercially developed gamma-ray spectrometry equipment

Pulsed EPR analysis of tooth enamel samples exposed to UV and {gamma}-radiations

Energy Technology Data Exchange (ETDEWEB)

Marrale, M., E-mail: marrale@unipa.it [Dipartimento di Fisica, Universita di Palermo, Viale delle Scienze, Edificio 18, 90128 Palermo (Italy); Gruppo V Sezione INFN, Catania, Italy and Unita CNISM, Palermo (Italy); Longo, A.; Brai, M. [Dipartimento di Fisica, Universita di Palermo, Viale delle Scienze, Edificio 18, 90128 Palermo (Italy); Gruppo V Sezione INFN, Catania (Italy) and Unita CNISM, Palermo (Italy); Barbon, A.; Brustolon, M. [Dipartimento di Scienze Chimiche, Universita degli Studi di Padova, Via Marzolo 1, 35131 Padova (Italy); Fattibene, P. [Istituto Superiore di Sanita, Viale Regina Elena 299, 00161 Rome (Italy)

2011-09-15

The electron paramagnetic resonance (EPR) spectroscopy is widely applied for retrospective dosimetric purposes by means of quantitative detection of radicals in tooth enamel and bone samples. In this work we report a study by cw and pulsed EPR on two samples of human tooth enamel respectively irradiated by UV (254 nm) and {gamma}-exposed. The continuous wave (cw) EPR spectra have shown the usual presence in both samples of two types of CO{sub 2}{sup -} radicals, with axial and orthorombic g tensors. We have obtained the electron spin echo detected EPR (ED-EPR) spectra at 80 K of the two samples, and we have shown that they are suitable to mark the difference between the effects produced by the different irradiations. At low temperature the contribution to the ED-EPR spectrum of the mobile radical with the axial g tensor is still present in the UV irradiated sample, but not in the {gamma}-irradiated one, where its dynamics is too slow to average the g tensor. We have moreover studied the two-pulse electron spin echo decay on varying the microwave power, a well established method for measuring the Instantaneous Diffusion. We have found that the spectral diffusion parameter is almost the same for both radiation types, whereas the Instantaneous Diffusion is significantly larger for {gamma}-exposed samples than for UV irradiated ones. This difference is due to a higher local microscopic concentration of free radicals for samples irradiated with {gamma} photons.

Copper doping of ZnO crystals by transmutation of 64Zn to 65Cu: An electron paramagnetic resonance and gamma spectroscopy study

Science.gov (United States)

Recker, M. C.; McClory, J. W.; Holston, M. S.; Golden, E. M.; Giles, N. C.; Halliburton, L. E.

2014-06-01

Transmutation of 64Zn to 65Cu has been observed in a ZnO crystal irradiated with neutrons. The crystal was characterized with electron paramagnetic resonance (EPR) before and after the irradiation and with gamma spectroscopy after the irradiation. Major features in the gamma spectrum of the neutron-irradiated crystal included the primary 1115.5 keV gamma ray from the 65Zn decay and the positron annihilation peak at 511 keV. Their presence confirmed the successful transmutation of 64Zn nuclei to 65Cu. Additional direct evidence for transmutation was obtained from the EPR of Cu2+ ions (where 63Cu and 65Cu hyperfine lines are easily resolved). A spectrum from isolated Cu2+ (3d9) ions acquired after the neutron irradiation showed only hyperfine lines from 65Cu nuclei. The absence of 63Cu lines in this Cu2+ spectrum left no doubt that the observed 65Cu signals were due to transmuted 65Cu nuclei created as a result of the neutron irradiation. Small concentrations of copper, in the form of Cu+-H complexes, were inadvertently present in our as-grown ZnO crystal. These Cu+-H complexes are not affected by the neutron irradiation, but they dissociate when a crystal is heated to 900 °C. This behavior allowed EPR to distinguish between the copper initially in the crystal and the copper subsequently produced by the neutron irradiation. In addition to transmutation, a second major effect of the neutron irradiation was the formation of zinc and oxygen vacancies by displacement. These vacancies were observed with EPR.

Spectrometric gamma radiation of shale cores applied to sweet spot discrimination in Eastern Pomerania, Poland

Science.gov (United States)

Skupio, Rafal; de Alemar Barberes, Gabriel

2017-12-01

This paper describes the application and calculation of hydrocarbon anomalies in two different boreholes located in Eastern Pomerania (northern Poland). Spectrometric data from borehole geophysical probe (borehole 1) and portable gamma logger (borehole 2) were used to analyze shale formations. The results from borehole 1 presented a statistically significant, moderate correlation between calculated hydrocarbon anomalies and hydrocarbon saturation data obtained from well log interpretation. Borehole 2 has been analyzed focusing on the gamma radiation of the core samples, and the positive results of borehole 1. Hydrocarbon anomalies calculated from spectral gamma radiation are reliable indicators of sweet spots, based solely on a cursory evaluation of core measurements. These preliminary information acquired from gamma-ray measurements could help increase sampling precision of further geochemical analysis.

Impact of detector efficiency and energy resolution on gamma-ray background rejection in mobile spectroscopy and imaging systems

Energy Technology Data Exchange (ETDEWEB)

Aucott, Timothy J., E-mail: Timothy.Aucott@SRS.gov [Lawrence Berkeley National Laboratory, Nuclear Science Division, Berkeley, CA (United States); Bandstra, Mark S. [Lawrence Berkeley National Laboratory, Nuclear Science Division, Berkeley, CA (United States); Negut, Victor; Curtis, Joseph C. [University of California, Berkeley, Department of Nuclear Engineering, Berkeley, CA (United States); Meyer, Ross E.; Chivers, Daniel H. [Lawrence Berkeley National Laboratory, Nuclear Science Division, Berkeley, CA (United States); Vetter, Kai [University of California, Berkeley, Department of Nuclear Engineering, Berkeley, CA (United States); Lawrence Berkeley National Laboratory, Nuclear Science Division, Berkeley, CA (United States)

2015-07-21

The presence of gamma-ray background significantly reduces detection sensitivity when searching for radioactive sources in the field, and the systematic variability in the background will limit the size and energy resolution of systems that can be used effectively. An extensive survey of the background was performed using both sodium iodide and high-purity germanium. By using a bivariate negative binomial model for the measured counts, these measurements can be resampled to simulate the performance of a detector array of arbitrary size and resolution. The response of the system as it moved past a stationary source was modeled for spectroscopic and coded aperture imaging algorithms and used for source injection into the background. The performance of both techniques is shown for various sizes and resolutions, as well as the relative performance for sodium iodide and germanium. It was found that at smaller detector sizes or better energy resolution, spectroscopy has higher detection sensitivity than imaging, while imaging is better suited to larger or poorer resolution detectors.

GammaSem Proceedings. A Nordic seminar for users of gamma spectrometry

Energy Technology Data Exchange (ETDEWEB)

Straalberg, E. (ed.) (Institute for Energy Technolgy (Norway)); Berg, K. (National Institute of Radiation Protection (Denmark)); Dowdall, M. (Norwegian Radiation Protection Authority (Norway)) (and others)

2010-11-15

The project GammaSem was proposed to the NKS in 2008. The aim of the project was to arrange two seminars for users of gamma spectrometry, in 2009 and 2010. The seminars were meant to provide a forum for discussions and sharing of information on practical issues concerning gamma spectrometry and initiate a network of gamma spectrometry users in the Nordic countries. Such a Nordic network should strengthen the collaboration between laboratories and improve all participants' competence in practical gamma spectrometry. Both seminars' focus was practical challenges met by the users themselves, rather than theoretical matters. Scientists and users of gamma spectrometry from all five Nordic countries were invited to the seminar, as well as scientist from the Baltic countries. A total of 65 people signed up for GammaSem 2010; representing 30 different universities, commercial companies, research institutes and authorities. The working group concept as presented at last year's GammaSem, has not worked out as intended. The reason for this is probably because most of the laboratories that signed up to join the working groups, signed up because they wanted to learn more about the different subjects. In combination with the fact that no funding was made available for the working groups, it was difficult to establish goals on what to achieve. None of the working groups applied for funding from the NKS (or elsewhere) to establish separate projects. There is a big need for more cooperation and for training within the field of gamma spectrometry. This fact has been proved through these two seminars, both by the many different topics that have been discussed, but also by the huge interest for participating in the suggested series of workshop. The GammaSem seminars have thus provided a much welcomed starting point for a broader Nordic collaboration. (Author)

GammaSem Proceedings. A Nordic seminar for users of gamma spectrometry

International Nuclear Information System (INIS)

Straelberg, E.; Berg, K.; Dowdall, M.

2010-11-01

The project GammaSem was proposed to the NKS in 2008. The aim of the project was to arrange two seminars for users of gamma spectrometry, in 2009 and 2010. The seminars were meant to provide a forum for discussions and sharing of information on practical issues concerning gamma spectrometry and initiate a network of gamma spectrometry users in the Nordic countries. Such a Nordic network should strengthen the collaboration between laboratories and improve all participants' competence in practical gamma spectrometry. Both seminars' focus was practical challenges met by the users themselves, rather than theoretical matters. Scientists and users of gamma spectrometry from all five Nordic countries were invited to the seminar, as well as scientist from the Baltic countries. A total of 65 people signed up for GammaSem 2010; representing 30 different universities, commercial companies, research institutes and authorities. The working group concept as presented at last year's GammaSem, has not worked out as intended. The reason for this is probably because most of the laboratories that signed up to join the working groups, signed up because they wanted to learn more about the different subjects. In combination with the fact that no funding was made available for the working groups, it was difficult to establish goals on what to achieve. None of the working groups applied for funding from the NKS (or elsewhere) to establish separate projects. There is a big need for more cooperation and for training within the field of gamma spectrometry. This fact has been proved through these two seminars, both by the many different topics that have been discussed, but also by the huge interest for participating in the suggested series of workshop. The GammaSem seminars have thus provided a much welcomed starting point for a broader Nordic collaboration. (Author)

Applying Quantum Cascade Laser Spectroscopy in Plasma Diagnostics

Directory of Open Access Journals (Sweden)

Jürgen Röpcke

2016-07-01

Full Text Available The considerably higher power and wider frequency coverage available from quantum cascade lasers (QCLs in comparison to lead salt diode lasers has led to substantial advances when QCLs are used in pure and applied infrared spectroscopy. Furthermore, they can be used in both pulsed and continuous wave (cw operation, opening up new possibilities in quantitative time resolved applications in plasmas both in the laboratory and in industry as shown in this article. However, in order to determine absolute concentrations accurately using pulsed QCLs, careful attention has to be paid to features like power saturation phenomena. Hence, we begin with a discussion of the non-linear effects which must be considered when using short or long pulse mode operation. More recently, cw QCLs have been introduced which have the advantage of higher power, better spectral resolution and lower fluctuations in light intensity compared to pulsed devices. They have proved particularly useful in sensing applications in plasmas when very low concentrations have to be monitored. Finally, the use of cw external cavity QCLs (EC-QCLs for multi species detection is described, using a diagnostics study of a methane/nitrogen plasma as an example. The wide frequency coverage of this type of QCL laser, which is significantly broader than from a distributed feedback QCL (DFB-QCL, is a substantial advantage for multi species detection. Therefore, cw EC-QCLs are state of the art devices and have enormous potential for future plasma diagnostic studies.

A NIM (Nuclear Instrumentation Module) system conjugated with optional input for pHEMT amplifier for beta and gamma spectroscopy

International Nuclear Information System (INIS)

Konrad, Barbara; Lüdke, Everton

2014-01-01

This work presents a high speed NIM module (Nuclear Instrumentation Module) to detect radiation, gamma and muons, as part of a system for natural radiation monitoring and of extraterrestrial origin. The subsystem developed consists of a preamplifier and an integrated SCA (Single Channel Analyzer), including power supplies of ± 12 and ± 24V with derivations of +3.6 and ± 5V. The single channel analyzer board, consisting of discrete logic components, operating in window modes, normal and integral. The pulse shaping block is made up of two voltage comparators working at 120 MHz with a response time > 60 ns and a logic anticoincidence system. The preamplifier promotes a noise reduction and introduces the impedance matching between the output of anode / diode photomultiplier tubes (PMTs) and subsequent equipment, providing an input impedance of 1MΩ and output impedance of 40 to 140Ω. The shaper amplifier is non-inverting and has variable input capacitance of 1000 pF. The upper and lower thresholds of the SCA are adjustable from 0 to ± 10V, and the equipment is compatible with various types of detectors, like PMTs coupled to sodium iodide crystals. For use with liquid scintillators and photodiodes with crystals (CsI: Tl) is proposed to include a preamplifier circuit pHEMT (pseudomorphic High Electron Mobility Transistor) integrated. Yet, the system presents the possibility of applications for various purposes of gamma spectroscopy and automatic detection of events producing of beta particles

A trio of gamma-ray burst supernovae

DEFF Research Database (Denmark)

Cano, Z.; Ugarte Postigo, Antonio de; Pozanenko, A.

2014-01-01

We present optical and near-infrared (NIR) photometry for three gamma-ray burst supernovae (GRB-SNe): GRB 120729A, GRB 130215A / SN 2013ez and GRB 130831A / SN 2013fu. In the case of GRB 130215A / SN 2013ez, we also present optical spectroscopy at t-t0=16.1 d, which covers rest-frame 3000...

Gamma spectrum analysis including NAA with SAMPO for Windows

International Nuclear Information System (INIS)

Aarnio, P.A.; Nikkinen, M.T.; Routti, J.T.

1995-01-01

SAMPO for Windows is a high performance gamma spectrum analysis program. All the measurement, analysis and NAA phases can be done either under full interactive use control or user defined tasks can be used for automated measurement and analysis sequences including control of MCAs and sample changers. High resolution gamma-ray spectroscopy together with the possibility to resolve complex multiplets with high accuracy makes SAMPO very suitable for INAA. On the other hand, the possibility to automate analysis sequences allows it use effectively also in all routine NAA measurements. NAA in SAMPO is accomplished using comparative methods. Spectra of standards, flux monitors, controls and actual samples are analyzed normally to obtain the peak areas which are optionally corrected for decay. In the comparison the flux monitor results are used to correct for variations in the effective neutron flux. An optional irradiation position correction can also be applied. The controls are used to alarm for possible deviations in the results. The sophisticated spectrum analysis methods used together with the comparative NAA and monitors give accurate results limited by the systematic effects only. The Windows environment provides ease of use and further processing power is available through the interface to expert system identification of nuclides. (author) 19 refs.; 1 tab

Gamma-ray spectroscopy of nuclei near {sup 100}Sn

Energy Technology Data Exchange (ETDEWEB)

Seweryniak, D; Nyberg, J; Fahlander, C [Uppsala Univ. (Sweden). Dept. of Radiation Sciences; Cederwall, B; Norline, L; Johnson, A; Kerek, A [Manne Siegbahn Inst. of Physics, Stockholm (Sweden); [Royal Inst. of Tech., Stockholm (Sweden); Adamides, E [National Centre for Scientific Research, Ag. Paraskevi, Attiki (Greece); Atac, A; Piiparinen, M; Sletten, G [Niels Bohr Inst., Copenhagen (Denmark); Angelis, G de [Laboratori Nazionali di legnaro (Italy); Grawe, H; Schubart, R [Hahn-Meitner-Institut Berlin GmbH (Germany); Ideguchi, E; Mitarai, S [Kyushu Univ., Fukuoka (Japan). Dept. of Physics; Julin, R; Juutinen, S; Tormanen, S; Virtanen, A [Jyvaeskylae Univ. (Finland). Dept. of Physics; Karczmarczyk, W; Kownacki, J [Warsaw Univ. (Poland)

1992-08-01

Proton rich nuclei close to {sup 100}Sn have been investigated in an in-beam {gamma}-ray spectroscopic study using the NORDBALL detector array, including arrays of charged particle and neutron detectors. Excited states were identified for the first time in {sup 102}In, {sup 106,107,108}Sb and tentatively in {sup 108,109}Te. The nucleus {sup 110}Te was also populated and studied for the first time in an in-beam experiment. (author). 4 figs.

Study of different filtering techniques applied to spectra from airborne gamma spectrometry

Energy Technology Data Exchange (ETDEWEB)

Wilhelm, Emilien; Gutierrez, Sebastien; Reboli, Anne; Menard, Stephanie; Nourreddine, Abdel-Mjid [Commissariat a l' Energie Atomique et aux energies alternatives - CEA, DAM, DIF F-91297 Arpajon (France); Arbor, Nicolas [Institut Pluridisciplinaire Hubert Curien, UMR 7178 Universite de Strasbourg-CNRS, 23 rue du Loess, BP 28, F-67037 Strasbourg Cedex 2 (France)

2015-07-01

One of the features of spectra obtained by airborne gamma spectrometry is low counting statistics due to the short acquisition time (1 s) and the large source-detector distance (40 m). It leads to considerable uncertainty in radionuclide identification and determination of their respective activities from the windows method recommended by the IAEA, especially for low-level radioactivity. The present work compares the results obtained with filters in terms of errors of the filtered spectra with the window method and over the whole gamma energy range. The results are used to determine which filtering technique is the most suitable in combination with some method for total stripping of the spectrum. (authors)

Gamma-ray spectroscopy in the decay of (83)Se to levels of (83)Br.

Science.gov (United States)

Krane, K S

2015-03-01

High-resolution γ ray spectroscopy experiments have been done to study the emissions from the radioactive decay of 22-min (83g)Se produced from neutron capture using samples of enriched (82)Se. Energy and intensity values have been obtained to roughly an order of magnitude greater precision than in previous studies. Based on energy sums, 2 new levels are proposed in the daughter (83)Br and one previously proposed level is shown to be doubtful. Some 25 new transitions appear to decay with the (83)Se halflife, about half of which can be accommodated among the previous or newly proposed levels. Several previous γ ray placements are shown to be inconsistent with the new determinations of the (83)Br energy levels, but cannot be accommodated anywhere else among the known levels. As a result of the missing γ ray placements, some of the β branchings in the decay to levels of (83)Br appear to be negative. Gamma rays from the 2.4-h decay of the daughter (83)Br to levels of (83)Kr have also been observed, along with decays of (81g)(,m)Se present as a small impurity in the enriched samples and also as a strong component in irradiated samples of natural Se. Copyright © 2014 Elsevier Ltd. All rights reserved.

Solved problems in analysis as applied to gamma, beta, Legendre and Bessel functions

CERN Document Server

Farrell, Orin J

2013-01-01

Nearly 200 problems, each with a detailed, worked-out solution, deal with the properties and applications of the gamma and beta functions, Legendre polynomials, and Bessel functions. The first two chapters examine gamma and beta functions, including applications to certain geometrical and physical problems such as heat-flow in a straight wire. The following two chapters treat Legendre polynomials, addressing applications to specific series expansions, steady-state heat-flow temperature distribution, gravitational potential of a circular lamina, and application of Gauss's mechanical quadrature

Uranium, radium and thorium in soils with high-resolution gamma spectroscopy, MCNP-generated efficiencies, and VRF non-linear full-spectrum nuclide shape fitting

Directory of Open Access Journals (Sweden)

Metzger Robert

2017-01-01

Full Text Available A new method for analysis of uranium and radium in soils by gamma spectroscopy has been developed using VRF (“Visual RobFit” which, unlike traditional peak-search techniques, fits full-spectrum nuclide shapes with non-linear least-squares minimization of the chi-squared statistic. Gamma efficiency curves were developed for a 500 mL Marinelli beaker geometry as a function of soil density using MCNP. Collected spectra were then analyzed using the MCNP-generated efficiency curves and VRF to deconvolute the 90 keV peak complex of uranium and obtain 238U and 235U activities. 226Ra activity was determined either from the radon daughters if the equilibrium status is known, or directly from the deconvoluted 186 keV line. 228Ra values were determined from the 228Ac daughter activity. The method was validated by analysis of radium, thorium and uranium soil standards and by inter-comparison with other methods for radium in soils. The method allows for a rapid determination of whether a sample has been impacted by a man-made activity by comparison of the uranium and radium concentrations to those that would be expected from a natural equilibrium state.

Uranium, radium and thorium in soils with high-resolution gamma spectroscopy, MCNP-generated efficiencies, and VRF non-linear full-spectrum nuclide shape fitting

Science.gov (United States)

Metzger, Robert; Riper, Kenneth Van; Lasche, George

2017-09-01

A new method for analysis of uranium and radium in soils by gamma spectroscopy has been developed using VRF ("Visual RobFit") which, unlike traditional peak-search techniques, fits full-spectrum nuclide shapes with non-linear least-squares minimization of the chi-squared statistic. Gamma efficiency curves were developed for a 500 mL Marinelli beaker geometry as a function of soil density using MCNP. Collected spectra were then analyzed using the MCNP-generated efficiency curves and VRF to deconvolute the 90 keV peak complex of uranium and obtain 238U and 235U activities. 226Ra activity was determined either from the radon daughters if the equilibrium status is known, or directly from the deconvoluted 186 keV line. 228Ra values were determined from the 228Ac daughter activity. The method was validated by analysis of radium, thorium and uranium soil standards and by inter-comparison with other methods for radium in soils. The method allows for a rapid determination of whether a sample has been impacted by a man-made activity by comparison of the uranium and radium concentrations to those that would be expected from a natural equilibrium state.

Advances in gamma ray resonant scattering and absorption long-lived isomeric nuclear states

CERN Document Server

Davydov, Andrey V

2015-01-01

This book presents the basics and advanced topics of research of gamma ray physics. It describes measuring of  Fermi surfaces with gamma resonance spectroscopy and the theory of angular distributions of resonantly scattered gamma rays. The dependence of excited-nuclei average lifetime on the shape of the exciting-radiation spectrum and electron binding energies in the spectra of scattered gamma rays is described. Resonant excitation by gamma rays of nuclear isomeric states with long lifetime leads to the emission and absorption lines. In the book, a new gamma spectroscopic method, gravitational gamma spectrometry, is developed. It has a resolution hundred million times higher than the usual Mössbauer spectrometer. Another important topic of this book is resonant scattering of annihilation quanta by nuclei with excited states in connection with positron annihilation. The application of the methods described is to explain the phenomenon of Coulomb fragmentation of gamma-source molecules and resonant scatt...

Gamma-ray tracking: Characterisation of the AGATA symmetric prototype detectors

International Nuclear Information System (INIS)

Boston, A.J.; Boston, H.C.; Cresswell, J.R.; Dimmock, M.R.; Nelson, L.; Nolan, P.J.; Rigby, S.; Lazarus, I.; Simpson, J.; Medina, P.; Santos, C.; Parisel, C.

2007-01-01

Each major technical advance in gamma-ray detection devices has resulted in significant new insights into the structure of atomic nuclei. The next major step in gamma-ray spectroscopy involves achieving the goal of a 4pi ball of Germanium detectors by using the technique of gamma-ray energy tracking in electrically segmented Germanium crystals. The resulting spectrometer will have an unparalleled level of detection power for nuclear electromagnetic radiation. Collaborations have been established in Europe (AGATA) [J. Simpson, Acta Phys. Pol. B 36 (2005) 1383. ] and the USA (GRETA/GRETINA) to build gamma-ray tracking spectrometers. This paper discusses the performance of the AGATA (Advanced Gamma Tracking Array) symmetric prototype detectors that have been tested at University of Liverpool. The use of a fully digital data acquisition system has allowed detector charge pulse shapes from a selection of well defined photon interaction positions to be analysed, yielding important information on the position sensitivity of the detector

Gamma-ray tracking: Characterisation of the AGATA symmetric prototype detectors

Energy Technology Data Exchange (ETDEWEB)

Boston, A.J. [Oliver Lodge Laboratory, University of Liverpool, Oxford Street, Liverpool L69 7ZE (United Kingdom)]. E-mail: ajboston@liv.ac.uk; Boston, H.C. [Oliver Lodge Laboratory, University of Liverpool, Oxford Street, Liverpool L69 7ZE (United Kingdom); Cresswell, J.R. [Oliver Lodge Laboratory, University of Liverpool, Oxford Street, Liverpool L69 7ZE (United Kingdom); Dimmock, M.R. [Oliver Lodge Laboratory, University of Liverpool, Oxford Street, Liverpool L69 7ZE (United Kingdom); Nelson, L. [Oliver Lodge Laboratory, University of Liverpool, Oxford Street, Liverpool L69 7ZE (United Kingdom); Nolan, P.J. [Oliver Lodge Laboratory, University of Liverpool, Oxford Street, Liverpool L69 7ZE (United Kingdom); Rigby, S. [Oliver Lodge Laboratory, University of Liverpool, Oxford Street, Liverpool L69 7ZE (United Kingdom); Lazarus, I. [STFC Daresbury Laboratory, Daresbury, Warrington WA4 4AD (United Kingdom); Simpson, J. [STFC Daresbury Laboratory, Daresbury, Warrington WA4 4AD (United Kingdom); Medina, P. [Institut de Recherches Subatomiques, Strasbourg BP28 67037 (France); Santos, C. [Institut de Recherches Subatomiques, Strasbourg BP28 67037 (France); Parisel, C. [Institut de Recherches Subatomiques, Strasbourg BP28 67037 (France)

2007-08-15

Each major technical advance in gamma-ray detection devices has resulted in significant new insights into the structure of atomic nuclei. The next major step in gamma-ray spectroscopy involves achieving the goal of a 4pi ball of Germanium detectors by using the technique of gamma-ray energy tracking in electrically segmented Germanium crystals. The resulting spectrometer will have an unparalleled level of detection power for nuclear electromagnetic radiation. Collaborations have been established in Europe (AGATA) [J. Simpson, Acta Phys. Pol. B 36 (2005) 1383. ] and the USA (GRETA/GRETINA) to build gamma-ray tracking spectrometers. This paper discusses the performance of the AGATA (Advanced Gamma Tracking Array) symmetric prototype detectors that have been tested at University of Liverpool. The use of a fully digital data acquisition system has allowed detector charge pulse shapes from a selection of well defined photon interaction positions to be analysed, yielding important information on the position sensitivity of the detector.

Terahertz time-domain attenuated total reflection spectroscopy applied to the rapid discrimination of the botanical origin of honeys

Science.gov (United States)

Liu, Wen; Zhang, Yuying; Yang, Si; Han, Donghai

2018-05-01

A new technique to identify the floral resources of honeys is demanded. Terahertz time-domain attenuated total reflection spectroscopy combined with chemometrics methods was applied to discriminate different categorizes (Medlar honey, Vitex honey, and Acacia honey). Principal component analysis (PCA), cluster analysis (CA) and partial least squares-discriminant analysis (PLS-DA) have been used to find information of the botanical origins of honeys. Spectral range also was discussed to increase the precision of PLS-DA model. The accuracy of 88.46% for validation set was obtained, using PLS-DA model in 0.5-1.5 THz. This work indicated terahertz time-domain attenuated total reflection spectroscopy was an available approach to evaluate the quality of honey rapidly.

On the incomparability of Gamma and Linda

NARCIS (Netherlands)

G. Zavattaro (Gianluigi)

1998-01-01

htmlabstractWe compare Gamma and Linda, two of the most prominent coordination languages based on generative communication via a shared data space. In Gamma computation is obtained by applying multiset rewriting rules, reminiscent of the way chemical reactions happen in a solution. On the other

Transmission and signal loss in mask designs for a dual neutron and gamma imager applied to mobile standoff detection

International Nuclear Information System (INIS)

Ayaz-Maierhafer, Birsen; Hayward, Jason P.; Ziock, Klaus P.; Blackston, Matthew A.; Fabris, Lorenzo

2013-01-01

In order to design a next-generation, dual neutron and gamma imager for mobile standoff detection which uses coded aperture imaging as its primary detection modality, the following design parameters have been investigated for gamma and neutron radiation incident upon a hybrid, coded mask: (1) transmission through mask elements for various mask materials and thicknesses; and (2) signal attenuation in the mask versus angle of incidence. Each of these parameters directly affects detection significance, as quantified by the signal-to-noise ratio. The hybrid mask consists of two or three layers: organic material for fast neutron attenuation and scattering, Cd for slow neutron absorption (if applied), and one of three of the following photon or photon and slow neutron attenuating materials—Linotype alloy, CLYC, or CZT. In the MCNP model, a line source of gamma rays (100–2500 keV), fast neutrons (1000–10,000 keV) or thermal neutrons was positioned above the hybrid mask. The radiation penetrating the mask was simply tallied at the surface of an ideal detector, which was located below the surface of the last mask layer. The transmission was calculated as the ratio of the particles transmitted through the fixed aperture to the particles passing through the closed mask. In order to determine the performance of the mask considering relative motion between the source and detector, simulations were used to calculate the signal attenuation for incident radiation angles of 0–50°. The results showed that a hybrid mask can be designed to sufficiently reduce both transmission through the mask and signal loss at large angles of incidence, considering both gamma ray and fast neutron radiations. With properly selected material thicknesses, the signal loss of a hybrid mask, which is necessarily thicker than the mask required for either single mode imaging, is not a setback to the system's detection significance

Analysis of the gamma spectra of the uranium, actinium, and thorium decay series

International Nuclear Information System (INIS)

Momeni, M.H.

1981-09-01

This report describes the identification of radionuclides in the uranium, actinium, and thorium series by analysis of gamma spectra in the energy range of 40 to 1400 keV. Energies and absolute efficiencies for each gamma line were measured by means of a high-resolution germanium detector and compared with those in the literature. A gamma spectroscopy method, which utilizes an on-line computer for deconvolution of spectra, search and identification of each line, and estimation of activity for each radionuclide, was used to analyze soil and uranium tailings, and ore

Procedural and developmental aspects of a multielement automatic radiochemical machine, applied to neutron irradiated biomedical samples

International Nuclear Information System (INIS)

Iyengar, G.V.

1976-06-01

This report is intended to serve as a practical guide, elaborately describing the working details and some developmental work connected with an automatic multielement radiochemical machine based on thermal neutron activation analysis using ion exchange and partition chromatography. Some of the practical aspects and personal observations after much experience with this versatile multielement method, applied to investigate the elemental composition of different biomedical matrices, are summarized. Standard reference materials are analyzed, and the data are presented with a set of gamma-spectra obtained before and after chemical separation into convenient groups suitable for gamma spectroscopy. The samples analyzed included various human and animal tissues, body fluids, IAEA biological standard reference materials, and samples from the WHO/IAEA project on 'Trace elements in relation to cardiovascular diseases'. Simplified modifications of the radiochemical processing, suitable for fast and routine analysis of clinical samples have also been discussed. (orig.) [de

FTR europia gamma heating

International Nuclear Information System (INIS)

Ward, J.T. Jr.

1975-01-01

Calculated and experimental gamma heating rates of europia in the Engineering Mockup Critical Assembly (EMC) were correlated. A calculated to experimental (C/E) ratio of 1.086 was established in validating the theoretical approach and computational technique applied in the calculations. Gamma heat deposition rates in the FTR with Eu 2 O 3 control absorbers were determined from three-dimensional calculations. Maximum gamma heating was found to occur near the tip of a half-inserted row 5 control rod assembly--12.8 watts/gm of europia. Gamma heating profiles were established for a single half-inserted europia absorber assembly. Local heat peaking was found not to alter significantly heating rates computed in the FTR core model, where larger mesh interval sizes precluded examination of spatially-limited heating gradients. These computations provide the basis for thermal-hydraulic analyses to ascertain temperature profiles in the FTR under europia control

Study of stability of humic acids from soil and peat irradiated by gamma rays; Estudo da estabilidade de acidos humicos extraidos de solo e turfa, frente a radiacao ionizante gama

Energy Technology Data Exchange (ETDEWEB)

Silva, Wilson Tadeu Lopes da

1995-07-01

Humic acids samples (one deriving from a sedimentary soil and other from a peat), in aqueous media, were irradiated with gamma rays, in doses of 10, 50 and 100 kGy, in order to understand their chemical behavior after the irradiation. The material, before and after irradiation, was analyzed by Elemental Analysis, Functional Groups (carboxylic acids and phenols), UV/Vis Spectroscopy (E{sub 4}/E{sub 6} ratio), IR spectroscopy, CO{sub 2} content and Gel permeation Chromatography (GPC) ). The Elemental Analysis showed the humic acid derived from a peat had a most percentage quantity of Carbon and Hydrogen than the material from a sedimentary soil. From the UV/Vis Spectroscopy, it was observed a decrease of E{sub 4}/E{sub 6} ratio with an increase of the applied dose. The data from GPC are in agreement with this. The results showed that the molecular weight of the material increased by exposing it to a larger radiolitical dose. The peat material was less affected by the gamma radiation than the soil material. The carboxylic groups were responsible by radiochemical behavior of the material. (author)

Evaluation of Shifted Excitation Raman Difference Spectroscopy and Comparison to Computational Background Correction Methods Applied to Biochemical Raman Spectra.

Science.gov (United States)

Cordero, Eliana; Korinth, Florian; Stiebing, Clara; Krafft, Christoph; Schie, Iwan W; Popp, Jürgen

2017-07-27

Raman spectroscopy provides label-free biochemical information from tissue samples without complicated sample preparation. The clinical capability of Raman spectroscopy has been demonstrated in a wide range of in vitro and in vivo applications. However, a challenge for in vivo applications is the simultaneous excitation of auto-fluorescence in the majority of tissues of interest, such as liver, bladder, brain, and others. Raman bands are then superimposed on a fluorescence background, which can be several orders of magnitude larger than the Raman signal. To eliminate the disturbing fluorescence background, several approaches are available. Among instrumentational methods shifted excitation Raman difference spectroscopy (SERDS) has been widely applied and studied. Similarly, computational techniques, for instance extended multiplicative scatter correction (EMSC), have also been employed to remove undesired background contributions. Here, we present a theoretical and experimental evaluation and comparison of fluorescence background removal approaches for Raman spectra based on SERDS and EMSC.

Copper doping of ZnO crystals by transmutation of 64Zn to 65Cu: An electron paramagnetic resonance and gamma spectroscopy study

International Nuclear Information System (INIS)

Recker, M. C.; McClory, J. W.; Holston, M. S.; Golden, E. M.; Giles, N. C.; Halliburton, L. E.

2014-01-01

Transmutation of 64 Zn to 65 Cu has been observed in a ZnO crystal irradiated with neutrons. The crystal was characterized with electron paramagnetic resonance (EPR) before and after the irradiation and with gamma spectroscopy after the irradiation. Major features in the gamma spectrum of the neutron-irradiated crystal included the primary 1115.5 keV gamma ray from the 65 Zn decay and the positron annihilation peak at 511 keV. Their presence confirmed the successful transmutation of 64 Zn nuclei to 65 Cu. Additional direct evidence for transmutation was obtained from the EPR of Cu 2+ ions (where 63 Cu and 65 Cu hyperfine lines are easily resolved). A spectrum from isolated Cu 2+ (3d 9 ) ions acquired after the neutron irradiation showed only hyperfine lines from 65 Cu nuclei. The absence of 63 Cu lines in this Cu 2+ spectrum left no doubt that the observed 65 Cu signals were due to transmuted 65 Cu nuclei created as a result of the neutron irradiation. Small concentrations of copper, in the form of Cu + -H complexes, were inadvertently present in our as-grown ZnO crystal. These Cu + -H complexes are not affected by the neutron irradiation, but they dissociate when a crystal is heated to 900 °C. This behavior allowed EPR to distinguish between the copper initially in the crystal and the copper subsequently produced by the neutron irradiation. In addition to transmutation, a second major effect of the neutron irradiation was the formation of zinc and oxygen vacancies by displacement. These vacancies were observed with EPR.

Laser spectroscopy applied to environmental, ecological, food safety, and biomedical research.

Science.gov (United States)

Svanberg, Sune; Zhao, Guangyu; Zhang, Hao; Huang, Jing; Lian, Ming; Li, Tianqi; Zhu, Shiming; Li, Yiyun; Duan, Zheng; Lin, Huiying; Svanberg, Katarina

2016-03-21

Laser spectroscopy provides many possibilities for multi-disciplinary applications in environmental monitoring, in the ecological field, for food safety investigations, and in biomedicine. The paper gives several examples of the power of multi-disciplinary applications of laser spectroscopy as pursued in our research group. The studies utilize mostly similar and widely applicable spectroscopic approaches. Air pollution and vegetation monitoring by lidar techniques, as well as agricultural pest insect monitoring and classification by elastic scattering and fluorescence spectroscopy are described. Biomedical aspects include food safety applications and medical diagnostics of sinusitis and otitis, with strong connection to the abatement of antibiotics resistance development.

CEBAF at higher energies: Working group report on hadron spectroscopy and production

Energy Technology Data Exchange (ETDEWEB)

Barnes, T. [Oak Ridge National Laboratory, TN (United States)]| [Univ. of Tennessee, Knoxville (United States); Napolitano, J. [Rensselaer Polytechnic Inst., Troy, NY (United States)

1994-04-01

This report summarizes topics in hadron spectroscopy and production which could be addressed at CEBAF with an energy upgrade to E{sub {gamma}} = 8 GeV and beyond. The topics discussed include conventional meson and baryon spectrocopy, spectroscopy of exotica (especially molecules and hybrids), CP and CPT tests using {phi} mesons, and new detector and accelerator options.

In situ gamma ray measurements of radionuclides at a disused phosphate mine on the West Coast of South Africa

International Nuclear Information System (INIS)

Bezuidenhout, Jacques

2015-01-01

High levels of uranium and its radioactive progeny like radium is normally associated with phosphate mining. In Situ gamma ray spectroscopy as a survey tool has been successfully applied to assess radionuclide concentrations in various geographical environments. A transportable and robust gamma ray detection system (GISPI) was therefore employed to determine the concentrations of naturally occurring radionuclides at a disused phosphate mine on the West Coast of South Africa. The concentrations of radium, thorium and potassium were measured and plotted. The measurements showed fairly high concentrations with medians of 320 Bq/kg for "2"2"6Ra, 64 Bq/kg for "2"3"2Th and 390 Bq/kg for "4"0K. The highest concentrations were however confined to specific areas of the mine. The effective dose due to gamma irradiation for the various areas of the mine was also estimated and the highest estimated level was 0.45 mSv/y. The article finally draws conclusions as to the origins and impact of the radiation. - Highlights: • A self-developed transportable and robust gamma ray detection system (the GISPI) was employed in the measurements. • A different mathematical analysis method was used. • QGIS was used extensively. • The results is important for current developments in infrastructure and mining.

Detection of explosive substances by tomographic inspection using neutron and gamma-ray spectroscopy

International Nuclear Information System (INIS)

Farahmand, M.; Boston, A.J.; Grint, A.N.; Nolan, P.J.; Joyce, M.J.; Mackin, R.O.; D'Mellow, B.; Aspinall, M.; Peyton, A.J.; Silfhout, R. van

2007-01-01

In recent years the detection and identification of hazardous materials has become increasingly important. This work discusses research and development of a technique which is capable of detecting and imaging hidden explosives. It is proposed to utilise neutron interrogation of the substances under investigation facilitating the detection of emitted gamma radiation and scattered neutrons. Pulsed fast neutron techniques are attractive because they can be used to determine the concentrations of the light elements (hydrogen, carbon, nitrogen, and oxygen) which can be the primary components of explosive materials. Using segmented High Purity Ge (HPGe) detectors and digital pulse processing [R.J. Cooper, G. Turk, A.J. Boston, H.C. Boston, J.R. Cresswell, A.R. Mather, P.J. Nolan, C.J. Hall, I. Lazarus, J. Simpson, A. Berry, T. Beveridge, J. Gillam, R.A. Lewis, in: Proceedings of the 7th International Conference on Position Sensitive Detectors, Nuclear Instruments and Methods A, in press; I. Lazarus, D.E. Appelbe, A. J. Boston, P.J. Coleman-Smith, J.R. Cresswell, M. Descovich, S.A.A. Gros, M. Lauer, J. Norman, C.J. Pearson, V.F.E. Pucknell, J.A. Sampson, G. Turk, J.J. Valiente-Dobon, IEEE Trans. Nucl. Sci., 51 (2004) 1353; R.J. Cooper, A.J. Boston, H.C. Boston, J.R. Cresswell, A.N. Grint, A.R. Mather, P.J. Nolan, D.P. Scraggs, G. Turk, C.J. Hall, I. Lazarus, A. Berry, T. Beveridge, J. Gillam, R.A. Lewis, in: Proceedings of the 11th International Symposium on Radiation Measurements and Application, 2006. ] the scatter path of incident photons can be reconstructed to determine the origin of the gamma-rays without the need for mechanical collimation by applying the Compton camera principle [V. Schonfelder, A. Hirner, K. Schneider, Nucl. Instr. and Meth. 107 (1973) 385; R.W. Todd, J.M. Nightingale, D.B. Everett, Nature 251 (1974) 132. ]. In addition, it is proposed to utilise the scattered neutrons which recoil from the materials being assayed, detecting them with a fast

[Gamma scattering in condensed matter with high intensity Moessbauer radiation

International Nuclear Information System (INIS)

1989-01-01

There are four areas where major progress has occurred this year. We have applied the Fourier-transform method of describing and analyzing Moessbauer effect (ME) line shapes to make measurements of the temperature dependence of the recoilless fraction in tungsten. We have carried out quasi-elastic measurements of the gamma scattering from viscous liquids, learning about diffusive motion in polydimethylsiloxane, pentadecane, and glycerol. We have made major progress in fundamental physics, having shown for the first time how to determine precise quantum interference parameters, obtaining experimental results on the 46.5 keV line of 183 W and the 129 keV line of 191 Ir. Finally, we have continued our development of MICE detectors, with a theoretical analysis of the MICE lineshape and its relation to the lineshape of conventional transmission ME spectroscopy. 12 refs

Burnup Measurement of Spent Fuel Assembly by CZT-based Gamma-ray Spectroscopy for Input Nuclear Material Accountancy of Pyroprocessing

International Nuclear Information System (INIS)

Seo, Hee; Oh, Jong-Myeong; Shin, Hee-Sung; Kim, Ho-Dong; Lee, Seung-Kyu; Park, Se-Hwan

2013-06-01

Input nuclear material accountancy is crucial for a pyroprocessing facility safeguards. Until a direct Pu measurement technique is established, an indirect method based on code calculations with burnup measurement and neutron counting for 244 Cm could be a practical option. Burnup can be determined by destructive analysis (DA) for final dispositive accuracy or by nondestructive assay (NDA) for near-real time accountancy. In the present study, an underwater burnup measurement system based on gamma-ray spectroscopy with the CZT detector was developed and tested on a spent fuel assembly. Burnup was determined according to the 134 Cs/ 137 Cs activity ratio with efficiency correction by Geant4 Monte Carlo simulations. The activity ratio as a function of burnup was obtained by ORIGEN calculations. The measured burnup error was 8.6%, which was within the measurement uncertainty. It is expected that the underwater burnup measurement system could fulfill an important role as a means of near-real time accountancy at a future pyroprocessing facility. (authors)

Performance of the prototype LaBr{sub 3} spectrometer developed for the JET gamma-ray camera upgrade

Energy Technology Data Exchange (ETDEWEB)

Rigamonti, D., E-mail: davide.rigamonti@mib.infn.it; Nocente, M.; Gorini, G. [Dipartimento di Fisica “G. Occhialini,” Università degli Studi di Milano-Bicocca, Milano (Italy); Istituto di Fisica del Plasma “P. Caldirola,” CNR, Milano (Italy); Muraro, A.; Giacomelli, L.; Cippo, E. P.; Tardocchi, M. [Istituto di Fisica del Plasma “P. Caldirola,” CNR, Milano (Italy); Perseo, V. [Dipartimento di Fisica “G. Occhialini,” Università degli Studi di Milano-Bicocca, Milano (Italy); Boltruczyk, G.; Gosk, M.; Korolczuk, S.; Mianowski, S.; Zychor, I. [Narodowe Centrum Badań Jądrowych (NCBJ), 05-400 Otwock-Swierk (Poland); Fernandes, A.; Pereira, R. C. [Instituto de Plasmas e Fusão Nuclear, Instituto Superior Técnico, Universidade de Lisboa, Lisboa (Portugal); Figueiredo, J. [Instituto de Plasmas e Fusão Nuclear, Instituto Superior Técnico, Universidade de Lisboa, Lisboa (Portugal); EUROfusion Programme Management Unit, Culham Science Centre, OX14 3DB Abingdon (United Kingdom); Kiptily, V. [Culham Science Centre for Fusion Energy, Culham (United Kingdom); Murari, A. [EUROfusion Programme Management Unit, Culham Science Centre, OX14 3DB Abingdon (United Kingdom); Consorzio RFX (CNR, ENEA, INFN, Universita’ di Padova, Acciaierie Venete SpA), Padova (Italy); Collaboration: EUROfusion Consortium, JET, Culham Science Centre, Abingdon OX14 3DB (United Kingdom)

2016-11-15

In this work, we describe the solution developed by the gamma ray camera upgrade enhancement project to improve the spectroscopic properties of the existing JET γ-ray camera. Aim of the project is to enable gamma-ray spectroscopy in JET deuterium-tritium plasmas. A dedicated pilot spectrometer based on a LaBr{sub 3} crystal coupled to a silicon photo-multiplier has been developed. A proper pole zero cancellation network able to shorten the output signal to a length of 120 ns has been implemented allowing for spectroscopy at MHz count rates. The system has been characterized in the laboratory and shows an energy resolution of 5.5% at E{sub γ} = 0.662 MeV, which extrapolates favorably in the energy range of interest for gamma-ray emission from fast ions in fusion plasmas.

Application of a gamma spectroscopy system to the measurement of neutron cross sections necessary to the development of nuclear energy

International Nuclear Information System (INIS)

Deruelle, O.

2002-09-01

This work concerns the development of nuclear energy and nuclear waste management in particular. Two parts of this study can be distinguished. In the first part (theoretical), a thorium-plutonium fuel based on MOX and dedicated for PWR was investigated in order to transmute plutonium in a potentially low waste fuel cycle. It was shown that this type of fuel is not regenerative but could be used for a transition to the industrial thorium fuel cycle without building new reactors. Thanks to moderated neutron spectra and high loaded actinide mass in the core, U-233 is quickly created (∼300 kg/y) for a loss of about ∼1200 kg of fissile plutonium. In the second part (experimental), we have developed and built a new reaction chamber to measure neutron cross sections of actinides by alpha-gamma spectroscopy. This experimental device (in principle transportable) was commissioned in the high flux reactor of ILL Grenoble. Neutron flux was measured by gamma spectroscopy of irradiated Al and Co samples and was found to be of the order of 6,0. 10 14 n.cm -2 .s -1 (4%). By the irradiation of 11μg of Am-243 and Pu-242, corresponding capture cross sections were measured in the thermal neutron flux at 50 deg C. These are the results: 243 Am(n,γ) 244fond. Am = 4,72±1,42b; 243 Am(n,γ) 244total Am = 74,8±3,25b; 242 Pu (n,γ) 243 Pu = 22,7±1,09b. Uncertainties of the measurements are mostly due to the determination of the neutron flux, efficiency of the electronics and ambiguities related to the definition of the area under α-γ spectra. Although our measured cross sections deviate (by 10-30%) from the corresponding values widely used in evaluated data libraries such as ENDF, JEF and JENDL, in this work we have demonstrated the feasibility and principle of our experimental method. Furthermore, the value for the 243-americium capture cross-section is in very good agreement with the last two measurements done in 1975 and 1997. These facts allowed us to think of new experiments

gamma-ray tracking in germanium the backtracking method

CERN Document Server

Marel, J V D

2002-01-01

In the framework of a European TMR network project the concept for a gamma-ray tracking array is being developed for nuclear physics spectroscopy in the energy range of approx 10 keV up to several MeV. The tracking array will consist of a large number of position-sensitive germanium detectors in a spherical geometry around a target. Due to the high segmentation, a Compton scattered gamma-ray will deposit energy in several different segments. A method has been developed to reconstruct the tracks of multiple coincident gamma-rays and to find their initial energies. By starting from the final point the track can be reconstructed backwards to the origin with the help of the photoelectric and Compton cross-sections and the Compton scatter formula. Every reconstructed track is given a figure of merit, thus allowing suppression of wrongly reconstructed tracks and gamma-rays that have scattered out of the detector system. This so-called backtracking method has been tested on simulated events in a shell-like geometry ...

Nuclear spectroscopy with lithium ions

International Nuclear Information System (INIS)

Heiser, C.

1977-02-01

A survey of the state of nuclear spectroscopy with lithium ions is given. Proceeding from the physical and nuclear properties the specific topics arising by the acceleration of these ions are discussed. The results obtained from measurements of excitation functions of different lithium reactions, particularly of compound reactions, with several target nuclei are summarized. Besides compound reactions direct reactions are important, especially transfer reactions, elastic and inelastic scattering and exchange reactions. The results on high spin states obtained by in-beam gamma-spectroscopy are discussed in detail. Finally the possibilities are considered for accelerating lithium ions in the cyclotron U-120 and in the tandem generator EGP-10 of the ZfK. (author)

Development of gamma camera and application to decontamination

International Nuclear Information System (INIS)

Yoshida, Akira; Moro, Eiji; Takahashi, Isao

2013-01-01

A gamma camera has been developed to support recovering from the contamination caused by the accident of Fukushima Dai-ichi Nuclear Power Plant of Tokyo Electric Power Company. The gamma camera enables recognition of the contamination by visualizing radioactivity. The gamma camera has been utilized for risk communication (explanation to community resident) at local governments in Fukushima. From now on, the gamma camera will be applied to solve decontaminations issues; improving efficiency of decontamination, visualizing the effect of decontamination work and reducing radioactive waste. (author)

AGILE: A gamma-ray mission

International Nuclear Information System (INIS)

Tavani, M.; Caraveo, P.; Mereghetti, S.; Perotti, F.; Vercellone, S.; Barbiellini, G.; Budini, G.; Longo, F.; Prest, M.; Vallazza, E.; Cocco, V.; Morselli, A.; Picozza, P.; Pittori, C.; Costa, E.; Feroci, M.; Lapshov, I.; Morelli, E.; Rubini, A.; Soffitta, P.

2000-01-01

AGILE is an innovative, cost-effective gamma-ray mission selected by the Italian Space Agency for a Program of Small Scientific Missions. The AGILE gamma-ray imaging detector (GRID, made of a Silicon tracker and CsI Mini-Calorimeter) is designed to detect and image photons in the 30 MeV-50 GeV energy band with good sensitivity and very large field of view (FOV ∼3 sr). The X-ray detector, Super-AGILE, sensitive in the 10-40 keV band and integrated on top of the GRID gamma-ray tracker will provide imaging (1-3 arcmin) and moderate spectroscopy. For selected sky areas, AGILE might achieve a flux sensitivity (above 100 MeV) better than 5x10 -8 ph cm 2 s -1 at the completion of its scientific program. AGILE will operate as an Observatory open to the international community and is planned to be operational during the year 2002 for a nominal 2-year mission. It will be an ideal 'bridge' between EGRET and GLAST, and the only mission entirely dedicated to high-energy astrophysics above 30 MeV during that period

Dedicated detectors for surface studies by Moessbauer spectroscopy

International Nuclear Information System (INIS)

Bibicu, I.; Rogalski, M.S.; Nicolescu, G.

2001-01-01

Moessbauer spectroscopy is a nuclear resonance method largely utilized in solid state studies. Following resonant nuclear absorption, gamma radiations, conversion X-rays, conversion or Auger electrons are emitted. By detection of gamma radiations information about the sample as a whole are obtained while by detection of electrons or X radiation one obtains data on the surface layer. Our laboratory was among the firsts to produce and use flow gas proportional detectors for surface studies by Moessbauer spectroscopy. Four types of detectors were devised: - detectors for electron detection (90% He + 10% CH 4 ); - detectors for conversion X-ray detection (90% Ar + 10% CH 4 ); - detectors for electrons or internal conversion X rays; - detectors for simultaneous detection of electrons and conversion X rays emitted from the same source. All detectors allow simultaneous Moessbauer measurements both for surface and volume for a given sample. Details of construction are presented for the four types of detectors

Validation of an advanced analytical procedure applied to the measurement of environmental radioactivity.

Science.gov (United States)

Thanh, Tran Thien; Vuong, Le Quang; Ho, Phan Long; Chuong, Huynh Dinh; Nguyen, Vo Hoang; Tao, Chau Van

2018-04-01

In this work, an advanced analytical procedure was applied to calculate radioactivity in spiked water samples in a close geometry gamma spectroscopy. It included MCNP-CP code in order to calculate the coincidence summing correction factor (CSF). The CSF results were validated by a deterministic method using ETNA code for both p-type HPGe detectors. It showed that a good agreement for both codes. Finally, the validity of the developed procedure was confirmed by a proficiency test to calculate the activities of various radionuclides. The results of the radioactivity measurement with both detectors using the advanced analytical procedure were received the ''Accepted'' statuses following the proficiency test. Copyright © 2018 Elsevier Ltd. All rights reserved.

High-resolution imaging gamma-ray spectroscopy with externally segmented germanium detectors

Science.gov (United States)

Callas, J. L.; Mahoney, W. A.; Varnell, L. S.; Wheaton, W. A.

1993-01-01

Externally segmented germanium detectors promise a breakthrough in gamma-ray imaging capabilities while retaining the superb energy resolution of germanium spectrometers. An angular resolution of 0.2 deg becomes practical by combining position-sensitive germanium detectors having a segment thickness of a few millimeters with a one-dimensional coded aperture located about a meter from the detectors. Correspondingly higher angular resolutions are possible with larger separations between the detectors and the coded aperture. Two-dimensional images can be obtained by rotating the instrument. Although the basic concept is similar to optical or X-ray coded-aperture imaging techniques, several complicating effects arise because of the penetrating nature of gamma rays. The complications include partial transmission through the coded aperture elements, Compton scattering in the germanium detectors, and high background count rates. Extensive electron-photon Monte Carlo modeling of a realistic detector/coded-aperture/collimator system has been performed. Results show that these complicating effects can be characterized and accounted for with no significant loss in instrument sensitivity.

Multi-isotopic gamma-ray assay system for alpha-contaminated waste

International Nuclear Information System (INIS)

Close, D.A.; Pratt, J.C.; Caldwell, J.T.; Kunz, W.E.; Schultz, F.J.; Haff, K.W.

1983-01-01

The capability of an existing segmented gamma-ray system is being expanded for the analysis of alpha-contaminated waste drums. A cursory assay of 114 transuranic waste drums of 208-l capacity has been made. Analysis of these data indicates a detection limit better than 100 nCi/g of waste for 237 Np/ 233 Pa, 239 Pu, 241 Am, 243 Am/ 239 Np, 60 Co, 125 Sb, 134 137 Cs, and 154 Eu. A pending Code of Federal Regulation (10CFR61) stipulates that the nuclear industry quantify not only its transuranic waste, but also certain beta- and gamma-ray-emitting fission products. An assay system based on gamma-ray spectroscopy is the only system that can meet this requirement for the fission products

Structural evolution of defective graphene under heat treatment and gamma irradiation

Science.gov (United States)

Zhang, Yifei; Shi, Jie; Chen, Cheng; Li, Nan; Xu, Zhiwei; Liu, Liangsen; Zhao, Lihuan; Li, Jing; Jing, Miaolei

2018-03-01

We have studied the structural change of defective graphene built by annealing in different temperature under the condition of gamma irradiation. Firstly, we found the heat treatment not only reduced but also striped the graphene. This behavior made defects become more firstly and then become less with the increase of temperature. And then gamma irradiation removed some oxygen-containing groups, by a simultaneous changed over carbon in the graphitic lattice from sp3 to sp2. Also, the gamma irradiation decreased the interlayer spacing between graphene lowest to 3.391 Å and made a crosslink which resulting in the size of the ordered gaining. A variation was detected by Raman spectroscopy that the amorphous carbon was declined after gamma irradiation. Furtherly we found the degree of this decline raised first and then diminished with the increase in the number of defects. The change in repair capacity of gamma irradiation presented a strategy for repairing the defects of graphene.

gamma-induced modification on optical band gap of CR-39 SSNTD

International Nuclear Information System (INIS)

Zaki, M.F.

2010-01-01

effect of gamma irradiation on optical absorption of nuclear track detectors like CR-39 was studied at different absorbed doses using ultraviolet-visible (UV-VIS)spectroscopy. the existence of the peaks, their shifting and broadening as a result of gamma irradiation has been discussed. the width of the tail of localized states in the band gap (E u )was evaluated using the Urbach edge method. finally the indirect and direct band gap in pristine and gamma irradiated CR-39 have been determined. the values of indirect band gap have been found to be lower than the corresponding values of direct band gap. a decrease in the optical energy gap with increasing the gamma absorbed dose can be discussed on the basis of gamma-irradiation-induced defects in the CR-39. the correlation between optical band gap and the number of carbon atoms in a cluster with modified Tauc's equation has been discussed in case of CR-39.

Development of a Reference Database for Particle-Induced Gamma-ray Emission spectroscopy

Energy Technology Data Exchange (ETDEWEB)

Dimitriou, P., E-mail: P.Dimitriou@iaea.org [International Atomic Energy Agency, Wagramerstrasse 5, A-1400 Vienna (Austria); Becker, H.-W. [Ruhr Universität Bochum, Gebäude NT05/130, Postfach 102148, Bochum 44721 (Germany); Bogdanović-Radović, I. [Department of Experimental Physics, Institute Rudjer Boskovic, Bijenicka Cesta 54, 10000 Zagreb (Croatia); Chiari, M. [Istituto Nazionale di Fisica Nucleare, Via Sansone 1, Sesto Fiorentino, 50019 Firenze (Italy); Goncharov, A. [Kharkov Institute of Physics and Technology, National Science Center, Akademicheskaya Str.1, Kharkov 61108 (Ukraine); Jesus, A.P. [Departamento de Física, Faculdade de Ciências e Tecnologia da Universidade Nova de Lisboa (Portugal); Kakuee, O. [Nuclear Science and Technology Research Institute, End of North Karegar Ave., PO Box 14395-836, Tehran (Iran, Islamic Republic of); Kiss, A.Z. [Institute of Nuclear Research (ATOMKI), Bem ter 18/c, PO Box 51, 4001 Debrecen (Hungary); Lagoyannis, A. [National Center of Scientific Research “Demokritos”, Agia Paraskevi, P.O. Box 60228, 15310 Athens (Greece); Räisänen, J. [Division of Materials Physics, Department of Physics, University of Helsinki, PO Box 43, 00014 University of Helsinki (Finland); Strivay, D. [Institut de Physique Nucleaire, Atomique et de Spectroscopie, Universite de Liège, Sart Tilman, B15 4000 Liège (Belgium); Zucchiatti, A. [Centro de Micro Análisis de Materiales, Universidad Autónoma de Madrid, Faraday 3, Madrid 28049 (Spain)

2016-03-15

Particle-Induced Gamma-ray Emission (PIGE) is a powerful analytical technique that exploits the interactions of rapid charged particles with nuclei located near a sample surface to determine the composition and structure of the surface regions of solids by measurement of characteristic prompt γ rays. The potential for depth profiling of this technique has long been recognized, however, the implementation has been limited owing to insufficient knowledge of the physical data and lack of suitable user-friendly computer codes for the applications. Although a considerable body of published data exists in the nuclear physics literature for nuclear reaction cross sections with γ rays in the exit channel, there is no up-to-date, comprehensive compilation specifically dedicated to IBA applications. A number of PIGE cross-section data had already been uploaded to the Ion Beam Analysis Nuclear Data Library (IBANDL) ( (http://www-nds.iaea.org/ibandl)) by members of the IBA community by 2011, however a preliminary survey of this body of unevaluated experimental data has revealed numerous discrepancies beyond the uncertainty limits reported by the authors. Using the resources and coordination provided by the IAEA, a concerted effort to improve the situation was made within the Coordinated Research Project on the Development of a Reference Database for PIGE spectroscopy, from 2011 to 2015. The aim of the CRP was to create a data library for Ion Beam Analysis that contains reliable and usable data on charged particle γ-ray emission cross sections that would be made freely available to the user community. As the CRP has reached its completion, we shall present its main achievements, including the results of nuclear cross-section evaluations and the development of a computer code that will become available to the public allowing for the implementation of a standardless PIGE technique.

Scientific prospects for spectroscopy of the gamma-ray burst prompt emission with SVOM

Science.gov (United States)

Bernardini, M. G.; Xie, F.; Sizun, P.; Piron, F.; Dong, Y.; Atteia, J.-L.; Antier, S.; Daigne, F.; Godet, O.; Cordier, B.; Wei, J.

2017-10-01

SVOM (Space-based multi-band astronomical Variable Objects Monitor) is a Sino-French space mission dedicated to the study of Gamma-Ray Bursts (GRBs) in the next decade, capable to detect and localise the GRB emission, and to follow its evolution in the high-energy and X-ray domains, and in the visible and NIR bands. The satellite carries two wide-field high-energy instruments: a coded-mask gamma-ray imager (ECLAIRs; 4-150 keV), and a gamma-ray spectrometer (GRM; 15-5500 keV) that, together, will characterise the GRB prompt emission spectrum over a wide energy range. In this paper we describe the performances of the ECLAIRs and GRM system with different populations of GRBs from existing catalogues, from the classical ones to those with a possible thermal component superimposed to their non-thermal emission. The combination of ECLAIRs and the GRM will provide new insights also on other GRB properties, as for example the spectral characterisation of the subclass of short GRBs showing an extended emission after the initial spike.

The design and performance of a large-volume spherical CsI(Tl) scintillation counter for gamma-ray spectroscopy

CERN Document Server

Meng, L J; Chirkin, V M; Potapov, V N; Ivanov, O P; Ignatov, S M

2002-01-01

This paper presents details of the design and performance of a prototype large-volume scintillation detector used for gamma-ray spectroscopy. In this detector, a spherical CsI(Tl) scintillation crystal having a diameter of 5.7 cm was polished and packed in dry MgO powder. The scintillation light from the crystal was viewed using a single 1x1 cm sup 2 silicon PIN diode. A low-noise preamplifier was also integrated within the detector housing. The measured noise level was equivalent to approx 800 electrons (FWHM). Such a configuration provided a very good light collection efficiency, which resulted in an average of 20 electrons being generated per keV of energy deposited in the crystal. One of the key features of the detector design is that it minimises spatial variations in the light collection efficiency throughout the detector. Compared with a standard 3 in. NaI scintillation counter, this feature leads to a much-improved energy resolution, particularly for photon energies above 1 MeV. The results presented ...

Development of FPGA-based digital signal processing system for radiation spectroscopy

International Nuclear Information System (INIS)

Lee, Pil Soo; Lee, Chun Sik; Lee, Ju Hahn

2013-01-01

We have developed an FPGA-based digital signal processing system that performs both online digital signal filtering and pulse-shape analysis for both particle and gamma-ray spectroscopy. Such functionalities were made possible by a state-of-the-art programmable logic device and system architectures employed. The system performance as measured, for example, in the system dead time and accuracy for pulse-height and rise-time determination, was evaluated with standard alpha- and gamma-ray sources using a CsI(Tl) scintillation detector. It is resulted that the present system has shown its potential application to various radiation-related fields such as particle identification, radiography, and radiation imaging. - Highlights: ► An FPGA-based digital processing system was developed for radiation spectroscopy. ► Our digital system has a 14-bit resolution and a 100-MHz sampling rate. ► The FPGA implements the online digital filtering and pulse-shape analysis. ► The pileup rejection is implemented in trigger logic before digital filtering process. ► Our digital system was verified in alpha-gamma measurements using a CsI detector

Noise-spectroscopy of multiqubit systems: Determining all their parameters by applying an external classical noise

Energy Technology Data Exchange (ETDEWEB)

Savel' ev, S., E-mail: S.Saveliev@lboro.ac.uk [Department of Physics, Loughborough University, Leicestershire LE11 3TU (United Kingdom); Advanced Science Institute, RIKEN, Wako-shi, Saitama 351-0198 (Japan); Zagoskin, A.M. [Department of Physics, Loughborough University, Leicestershire LE11 3TU (United Kingdom); Advanced Science Institute, RIKEN, Wako-shi, Saitama 351-0198 (Japan); Omelyanchouk, A.N. [Advanced Science Institute, RIKEN, Wako-shi, Saitama 351-0198 (Japan); B. Verkin Institute for Low Temperature Physics and Engineering, 61103 Kharkov (Ukraine); Nori, Franco [Advanced Science Institute, RIKEN, Wako-shi, Saitama 351-0198 (Japan); Physics Department, University of Michigan, Ann Arbor, MI 48109-1040 (United States)

2010-10-05

Imagine that you have several sets of two coupled qubits, but you do not know the parameters of their Hamitonians. How to determine these without resorting to the usual spectroscopy approach to the problem? Based on numerical modeling, we show that all the parameters of a system of two coupled qubits can be determined by applying to it an external classical noise and analyzing the Fourier spectrum of the elements of the system's density matrix. In particular, the interlevel spacings as well as the strength and sign of the qubit-qubit coupling can be determined this way.

Study of neutron-rich nuclei structure around the N=28 shell closure using the in-beam gamma spectroscopy technique; Etude de la structure des noyaux riches en neutrons autour de la fermeture de couches N=28 par spectroscopie gamma en ligne

Energy Technology Data Exchange (ETDEWEB)

Bastin, B

2007-10-15

For a few years now, a loss of magicity in neutron-rich nuclei near the neutron drip-line at N=28 has been suggested and observed. Deformation in these nuclei has been observed. The deformation was explained in S isotopes as being due to a moderate reduction of the N=28 shell closure together with a proton induced collectivity originating from the near degeneracy of the proton d3/2 and s1/2 orbitals. As a consequence, the observed deformation seems to result from a subtle interplay between neutron and proton excitations. Since the proton configuration in the Si isotopes is expected to be more stable due to the Z=14 sub-shell gap, {sup 42}Si was considered as a key nucleus in order to distinguish the different effects responsible for the structural changes observed at N=28. Even if it is at the limits of our technical possibilities, an in-beam gamma-spectroscopy experiment using two-step fragmentation and one or several nucleons knockout reaction mechanisms was performed at GANIL. The measurement of the energy of the first excited state in {sup 42}Si, combined with the observation of {sup 38,40}Si and the spectroscopy of {sup 41,43}P, has given evidence for the loss of magicity at N=28 far from stability. Modifications of the effective interaction used in modern shell model calculations have been completed following this investigation, increasing its predictive character. This study confirms the role of the tensor force and the density dependence of the spin-orbit interaction in the collapse of the N=28 shell closure. (author)

Preparation of graphene/polyaniline nanocomposites by gamma radiation for supercapacitor

International Nuclear Information System (INIS)

Cai Xiaosheng; Zhang Qilu; Peng Jing; Li Jiuqiang; Zhai Maolin

2014-01-01

Graphene was prepared from graphite oxide (GO) with surfactants by gamma irradiation, and then mixed with polyaniline to produce the composites. The structure characterization was investigated using (FTIR), thermalgravimetric analysis (TGA), Raman spectroscopy and X-ray photoelectron spectroscopy (XPS), and the electrochemical properties of the composites were measured. The results show that the cationic surfactant can promote the reduction of GO. The specific capacitance of the composite materials reaches 435 F/g at 0.1 A/g showing potential for use in supercapacitors. (authors)

Study and optimisation of the high energy detector in Cd(Zn)Te of the Simbol-X space mission for X and gamma astronomy; Etude et optimisation du plan de detection de haute energie en Cd(Zn)Te pour la mission spatiale d'observation astronomie X et gamma SIMBOL-X

Energy Technology Data Exchange (ETDEWEB)

Meuris, A.

2009-09-15

Stars in final phases of evolution are sites of highest energetic phenomena of the Universe. The understanding of their mechanisms is based on the observation of the X and gamma rays from the sources. The Simbol-X French-Italian project is a novel concept of telescope with two satellites flying in formation. This space mission combines upgraded optics from X-ray telescopes with detection Systems from gamma-ray telescopes. CEA Saclay involved in major space missions for gamma astronomy is in charge of the definition and the design of the High Energy Detector (HED) of Simbol-X to cover the spectral range from 8 to 80 keV. Two generations of micro-cameras called Caliste have been designed, fabricated and tested. They integrate cadmium telluride (CdTe) crystals and optimised front-end electronics named Idef-X. The hybridization technique enables to put them side by side as a mosaic to achieve for the first time a CdTe detection plane with fine spatial resolution (600 {mu}m) and arbitrarily large surface. By setting up test benches and leading test campaigns, I was involved in the fabrication of Caliste prototypes and I assessed temporal, spatial and spectral resolutions. At the conclusion of experiments and simulations, I propose a detector type, operating conditions and digital processing on board the spacecraft to optimise HED performance. The best detector candidate is CdTe Schottky, well suited to high resolution spectroscopy; however, it suffers from lost in stability during biasing. Beyond Simbol-X mission, I studied theoretically and experimentally this kind of detector to build an updated model that can apply to other projects of gamma spectroscopy and imaging. (author)

Oasis-an innovative system for alpha spectroscopy

Energy Technology Data Exchange (ETDEWEB)

Seymour, R; Richards, W; Knight, K; El-Sayad, G [Oxford Instruments Inc., P.O. Box 2560, Oak Ridge, TN 37831-2560 (United States)

1995-10-01

Until recently, instrumental alpha spectroscopy has behind the technical developments of instrumentation and software that are available for low background o c/ counting, liquid scintillation, and gamma spectroscopy instruments. We report in this paper, the development of Oasis, a new family of alpha spectroscopy systems from oxford instruments Inc., Nuclear measurements Group. The Oasis instruments incorporate many hardware and software innovations providing an automated and integrated production environment for alpha spectroscopy. These instruments are needed because of the large number of samples to be measured and the required throughput of production laboratories processing these samples. Oasis is also useful for facilities because of their sophisticated vacuum control, management, and analysis features. One of the most important innovations is the electronic vacuum system and cartesian diver. Many additional features contribute to improving accuracy, lowering cost per sample, improving sample throughput, and ensuring accountability of laboratory results. 5 figs.

Oasis-an innovative system for alpha spectroscopy

International Nuclear Information System (INIS)

Seymour, R.; Richards, W.; Knight, K.; El-Sayad, G.

1995-01-01

Until recently, instrumental alpha spectroscopy has behind the technical developments of instrumentation and software that are available for low background o c/ counting, liquid scintillation, and gamma spectroscopy instruments. We report in this paper, the development of Oasis, a new family of alpha spectroscopy systems from oxford instruments Inc., Nuclear measurements Group. The Oasis instruments incorporate many hardware and software innovations providing an automated and integrated production environment for alpha spectroscopy. These instruments are needed because of the large number of samples to be measured and the required throughput of production laboratories processing these samples. Oasis is also useful for facilities because of their sophisticated vacuum control, management, and analysis features. One of the most important innovations is the electronic vacuum system and cartesian diver. Many additional features contribute to improving accuracy, lowering cost per sample, improving sample throughput, and ensuring accountability of laboratory results. 5 figs

A wavelet filtering method for cumulative gamma spectroscopy used in wear measurements

International Nuclear Information System (INIS)

Bianchi, Davide; Lenauer, Claudia; Betz, Gerhard; Vernes, András

2017-01-01

Continuous ultra-mild wear quantification using radioactive isotopes involves measuring very low amounts of activity in limited time intervals. This results in gamma spectra with poor signal-to-noise ratio and hence very scattered wear data, especially during running-in, where wear is intrinsically low. Therefore, advanced filtering methods reducing the wear data scattering and making the calculation of the main peak area more accurate are mandatory. An energy-time dependent threshold for wavelet detail coefficients based on Poisson statistics and using a combined Barwell law for the estimation of the average photon counting rate is then introduced. In this manner, it was shown that the accuracy of running-in wear quantification is enhanced. - Highlights: • Time-dependent Poisson statistics. • Wavelet-based filtering of cumulative gamma spectra. • Improvement of low wear analysis.

Study and optimisation of the high energy detector in Cd(Zn)Te of the Simbol-X space mission for X and gamma astronomy

International Nuclear Information System (INIS)

Meuris, A.

2009-09-01

Stars in final phases of evolution are sites of highest energetic phenomena of the Universe. The understanding of their mechanisms is based on the observation of the X and gamma rays from the sources. The Simbol-X French-Italian project is a novel concept of telescope with two satellites flying in formation. This space mission combines upgraded optics from X-ray telescopes with detection Systems from gamma-ray telescopes. CEA Saclay involved in major space missions for gamma astronomy is in charge of the definition and the design of the High Energy Detector (HED) of Simbol-X to cover the spectral range from 8 to 80 keV. Two generations of micro-cameras called Caliste have been designed, fabricated and tested. They integrate cadmium telluride (CdTe) crystals and optimised front-end electronics named Idef-X. The hybridization technique enables to put them side by side as a mosaic to achieve for the first time a CdTe detection plane with fine spatial resolution (600 μm) and arbitrarily large surface. By setting up test benches and leading test campaigns, I was involved in the fabrication of Caliste prototypes and I assessed temporal, spatial and spectral resolutions. At the conclusion of experiments and simulations, I propose a detector type, operating conditions and digital processing on board the spacecraft to optimise HED performance. The best detector candidate is CdTe Schottky, well suited to high resolution spectroscopy; however, it suffers from lost in stability during biasing. Beyond Simbol-X mission, I studied theoretically and experimentally this kind of detector to build an updated model that can apply to other projects of gamma spectroscopy and imaging. (author)

Time resolved spectroscopy of GRB 030501 using INTEGRAL

DEFF Research Database (Denmark)

Beckmann, V.; Borkowski, J.; Courvoisier, T.J.L.

2003-01-01

The gamma-ray instruments on-board INTEGRAL offer an unique opportunity to perform time resolved analysis on GRBs. The imager IBIS allows accurate positioning of GRBs and broad band spectral analysis, while SPI provides high resolution spectroscopy. GRB 030501 was discovered by the INTEGRAL Burst...... the Ulysses and RHESSI experiments....

Spectroscopic study of gamma irradiated bovine hemoglobin

International Nuclear Information System (INIS)

Maghraby, Ahmed Mohamed; Ali, Maha Anwar

2007-01-01

In the present study, the effects of ionizing radiation of Cs-137 and Co-60 from 4.95 to 743.14 Gy and from 40 Gy to 300 kGy, respectively, on some bovine hemoglobin characteristics were studied. Such an effect was evaluated using electron paramagnetic resonance (EPR) spectroscopy, and infra-red (IR) spectroscopy. Bovine hemoglobin EPR spectra were recorded and analyzed before and after irradiation and changes were explained in detail. IR spectra of unirradiated and irradiated Bovine hemoglobin were recorded and analyzed also. It was found that ionizing radiation may lead to the increase of free radicals production, the decrease in α-helices contents, which reflects the degradation of hemoglobin molecular structure, or at least its incomplete performance. Results also show that the combined application of EPR and FTIR spectroscopy is a powerful tool for determining structural modification of bovine hemoglobin samples exposed to gamma irradiation

Reduction of Graphene Oxide to Graphene by Using Gamma Irradiation

International Nuclear Information System (INIS)

Shamellia Sharin; Irman Abdul Rahman; Ainee Fatimah Ahmad

2015-01-01

This research aims to gauge the ability of gamma radiation to induce the reduction of graphene oxide to graphene. Graphene oxide powders were dispersed into a mixture of alcohol and deionized water, and the mixture was then irradiated with a "6"0Co source using a GammaCell 220 Excel irradiator at absorbed doses of 0, 5, 15, 20 and 35 kGy. According to characterization using Fourier Transformed Infrared Spectroscopy (FTIR), it can be seen that almost every oxygen-containing functional group has been removed after irradiation of the graphene oxide mixture. Reduction of graphene oxide was also proven from the characterization using UV-Vis Spectroscopy, in which the wavelength of graphene oxide at 237 nm was red-shifted to 277 nm after being irradiated and the peak at 292 nm, (indicating the carboxyl group) disappears in the UV-Vis spectrum of reduced graphene oxide. Morphology of graphene oxide also changed from a smooth and flat surface to crumpled. The ratio of carbon/ oxygen in the graphene oxide was lower than the carbon/ oxygen of reduced graphene oxide. At the end of the experiment, it can be deduced that graphene oxide underwent reduction, characterized before and after irradiation using Emission Scanned Electron Microscopy and Energy Dispersive X-ray, Fourier Transformed Infrared Spectroscopy and UV-Vis Spectroscopy. Therefore, we postulate that the irradiation technique that induces reduction, can be used to obtain reduced graphene oxide from graphene oxide. (author)

Validation of gamma spectrometer in spectroscopy laboratory of education and training center BATAN

International Nuclear Information System (INIS)

Sugino; Tulisna; Anda Sanusi; Sugito

2010-01-01

Gamma spectrometer used to determine the type and activity of gamma emitting radionuclides, such as the measurement of environmental radioactivity and neutron activation analysis (NAA). In order to obtain precise and accurate qualitative and quantitative analysis, the gamma spectrometer should be validated. Validation of the gamma spectrometer was conducted on the confirmation of identity, differential linearity, performance, efficiency calibration, precision test, and accuracy test. Confirmation of identity conducted by energy calibration testing conducted and showed the largest energy deviation of 0.3 keV. Differential linearity testing showed the highest count difference of 6.9 %. Test Results for 1 year showed the lowest resolution of 1.82 keV, in accordance with the initial resolution of 1.8 keV. Value of lowest P/C is 59.8, according to the first P/C of 60. The lowest relative efficiency of 28.6 %, according to the initial efficiency of 30 %. Calibration curve shows that for more than 200 keV energy, the relationship of Ln Energy vs Ln Efficiency is a straight line with equation Ln(ε) = 7.211-0.8173 Ln(E), while for less than 100 keV energy the the equation Ln(ε) = -13.34+6.712Ln(E)+0.06894 Ln(E)"2, in accordance with the theory and references. Precision test conducted by chi square value of 10.6, according to probability of 5 % to 95 %. Testing the accuracy is shown from the results of comparative tests of measuring I-131 activity in 2009 with good results, the difference in the results of 2.35 % with the uncertainty of 6 %. (author)

Study of the Nuclear Structure of 39P Using Beta-Delayed Gamma Spectroscopy

Science.gov (United States)

Abromeit, Brittany; NSCL Experiment E14063 Team Team

2016-03-01

Investigation of nuclei with neutron and proton imbalance is at the forefront of nuclear physics research today. This is driven by the fact that the structure in these regimes may vary with that seen near the valley of stability. With eight neutrons more than the stable isotope of phosphorous, 39P is a neutron-rich exotic nucleus that has very limited information on it: previous studies of 39P produce only three known energy levels and gamma rays. The fragmentation of a 48Ca primary beam on a 564mg/cm2 thick Be target at the National Superconducting Cyclotron Laboratory (NSCL) was used to produce exotic 39Si. Using the NSCL Beta Counting System (BCS), consisting of a thick planner germanium double-sided strip detector (GeDSSD) and 16 High-purity germanium detectors in an array, SeGA, the beta-gamma coincidences from the decay of 39Si to 39P were analyzed. The resulting level scheme of 39P, including over 12 new gamma rays and energy states, confirmation of the previously measured half-life, and first-time logft values will be presented. This work was supported by the NSF under Grant No. 1401574.

Stability Studies of Certain Chemotherapeutic Agents Following Gamma Irradiation and Silver Nanoparticles Conjugation

International Nuclear Information System (INIS)

El-Sayyad, Gh.E.S.M.

2014-01-01

The Chemical stability of drug is of great importance since it becomes less effective as it undergoes degradation in case of applied of gamma irradiation process. The application of gamma irradiation for different chemotherapeutic agents Such as (ofloxacin, sodium ampicillin, sodium cefotaxime, gentamycin and amoxicillin) and studying the effect of applied doses on chemical structure and biological activity of the irradiated antibiotics compared to unirradiated ones was studied by ultraviolet-Visible spectrophotometer (UV-Visible), Fourier transform infrared spectroscopy measurements (FTIR spectra) and high performance liquid chromatography (HPLC) in addition to microbiological assay were run before and after irradiation to probe any change after irradiation. The results showed that all of the irradiated compounds remain stable and radio resistant; retaining their structure and activity unchanged up to 25 KGy. The radiation-induced AgNPs synthesis is a simple, clean which involves radiolysis of aqueous solution that provides an efficient method to reduce metal ions. Also, in this study, Bacillus megaterium was found to be an effective biological tool for the extracellular biosynthesis of stable AgNPs which are highly stable and this method has advantages over other methods as the organism used here is safe. This study would therefore lead to an easy procedure for producing silver nanoparticles with the added advantage of bio safety. The Synthesized AgNPs exhibit remarkable antimicrobial activity against both Gram-positive and Gram negative bacterial strains regardless of their drug-resistant mechanisms. The bactericidal activity have proved that AgNPs kill bacteria at such low concentrations (units of ppm), which Stability Studies of Certain Chemotherapeutic Agents Following Gamma Irradiation and Silver Nanoparticles Conjugation. do not reveal acute toxic effects on human cell, in addition to overcoming resistance, and lowering cost when compared to conventional

ESR spectroscopy for detecting gamma-irradiated dried vegetables and estimating absorbed doses

Energy Technology Data Exchange (ETDEWEB)

Kwon, Joong-Ho; Chung, Hyung-Wook; Byun, Myung-Woo

2000-03-01

In view of an increasing demand for food irradiation technology, the development of a reliable means of detection for the control of irradiated foods has become necessary. Various vegetable food materials (dried cabbage, carrot, chunggyungchae, garlic, onion, and green onion), which can be legally irradiated in Korea, were subjected to a detection study using ESR spectroscopy. Correlation coefficients (R{sup 2}) between absorbed doses (2.5-15 kGy) and their corresponding ESR signals were identified from ESR signals. Pre-established threshold values were successfully applied to the detection of 54 coded unknown samples of dried clean vegetables (chunggyungchae, Brassica camestris var. chinensis), both non-irradiated and irradiated. The ESR signals of irradiated chunggyungchae decreased over a longer storage time, however, even after 6 months of ambient storage, these signals were still distinguishable from those of non-irradiated samples. The most successful estimates of absorbed dose (5 and 8 kGy) were obtained immediately after irradiation using a quadratic fit with average values of 4.85 and 8.65 kGy being calculated. (author)

Production of modified starches by gamma irradiation

International Nuclear Information System (INIS)

Kang, Il-Jun; Byun, Myung-Woo; Yook, Hong-Sun; Bae, Chun-Ho; Lee, Hyun-Soo; Kwon, Joong-Ho; Chung, Cha-Kwon

1999-01-01

As a new processing method for the production of modified starch, gamma irradiation and four kinds of inorganic peroxides were applied to commercial corn starch. The addition of inorganic peroxides without gamma irradiation or gamma irradiation without the addition of inorganic peroxides effectively decreased initial viscosity, but did not sufficiently keep viscosity stable. The combination of adding ammonium persulfate (APS) and gamma irradiation showed the lowest initial viscosity and the best stability out of the tested four kinds of inorganic peroxides. Among the tested mixing methods of APS, soaking was found to be more effective than dry blending or spraying. Therefore, the production of modified starch with low viscosity as well as with sufficient viscosity stability became feasible by the control of gamma irradiation dose levels and the amount of added APS to starch

SNM gamma-ray fingerprint monitor functional requirements and design specifications

International Nuclear Information System (INIS)

Bieber, A.M. Jr.; Kane, W.R.

1994-07-01

A number of DOE facilities need to perform confirmatory inventory measurements on items of special nuclear material (SNM). The DOE Office of Safeguards and Security (OSS) has tasked the Safeguards, Safety and Nonproliferation Division (SSN) of the Department of Advanced Technology at Brookhaven National Laboratory (BNL) to develop a high-resolution gamma-ray-spectroscopy-based instrument for performing confirmatory inventory measurements on such materials, a ''gamma-ray fingerprint monitor'' (GRFM). This document is a conceptual design for the SSN GRFM system. This conceptual design is based on previous experience with measurements of plutonium-bearing materials and comparison of gamma-ray spectrum features, not on actual tests of the procedures or hardware described. As a result, modifications may be necessary when actual prototype hardware and software are tested in realistic circumstances on actual materials of interest

Study of neutron-rich nuclei structure around the N=28 shell closure using the in-beam gamma spectroscopy technique

International Nuclear Information System (INIS)

Bastin, B.

2007-10-01

For a few years now, a loss of magicity in neutron-rich nuclei near the neutron drip-line at N=28 has been suggested and observed. Deformation in these nuclei has been observed. The deformation was explained in S isotopes as being due to a moderate reduction of the N=28 shell closure together with a proton induced collectivity originating from the near degeneracy of the proton d3/2 and s1/2 orbitals. As a consequence, the observed deformation seems to result from a subtle interplay between neutron and proton excitations. Since the proton configuration in the Si isotopes is expected to be more stable due to the Z=14 sub-shell gap, 42 Si was considered as a key nucleus in order to distinguish the different effects responsible for the structural changes observed at N=28. Even if it is at the limits of our technical possibilities, an in-beam gamma-spectroscopy experiment using two-step fragmentation and one or several nucleons knockout reaction mechanisms was performed at GANIL. The measurement of the energy of the first excited state in 42 Si, combined with the observation of 38,40 Si and the spectroscopy of 41,43 P, has given evidence for the loss of magicity at N=28 far from stability. Modifications of the effective interaction used in modern shell model calculations have been completed following this investigation, increasing its predictive character. This study confirms the role of the tensor force and the density dependence of the spin-orbit interaction in the collapse of the N=28 shell closure. (author)

Modelling rainfall amounts using mixed-gamma model for Kuantan district

Science.gov (United States)

Zakaria, Roslinazairimah; Moslim, Nor Hafizah

2017-05-01

An efficient design of flood mitigation and construction of crop growth models depend upon good understanding of the rainfall process and characteristics. Gamma distribution is usually used to model nonzero rainfall amounts. In this study, the mixed-gamma model is applied to accommodate both zero and nonzero rainfall amounts. The mixed-gamma model presented is for the independent case. The formulae of mean and variance are derived for the sum of two and three independent mixed-gamma variables, respectively. Firstly, the gamma distribution is used to model the nonzero rainfall amounts and the parameters of the distribution (shape and scale) are estimated using the maximum likelihood estimation method. Then, the mixed-gamma model is defined for both zero and nonzero rainfall amounts simultaneously. The formulae of mean and variance for the sum of two and three independent mixed-gamma variables derived are tested using the monthly rainfall amounts from rainfall stations within Kuantan district in Pahang Malaysia. Based on the Kolmogorov-Smirnov goodness of fit test, the results demonstrate that the descriptive statistics of the observed sum of rainfall amounts is not significantly different at 5% significance level from the generated sum of independent mixed-gamma variables. The methodology and formulae demonstrated can be applied to find the sum of more than three independent mixed-gamma variables.

Time-of-flight discrimination between gamma-rays and neutrons by using artificial neural networks

International Nuclear Information System (INIS)

Akkoyun, S.

2013-01-01

Highlights: ► Time-of-flight (tof) is an obvious method for separation between gamma and neutron particles. ► tof distributions are obtained by neural networks. ► Neural network method is consistent with the experimental results. ► Neural networks can classify different events for discrimination. - Abstract: In gamma-ray spectroscopy, a number of neutrons are emitted from the nuclei together with the gamma-rays. These neutrons influence gamma-ray spectra. An obvious method for discrimination between neutrons and gamma-rays is based on the time-of-flight (tof) technique. In this work, the tof distributions of gamma-rays and neutrons were obtained both experimentally and by using artificial neural networks (ANNs). It was shown that, ANN can correctly classify gamma-ray and neutron events. Also, for highly nonlinear detector response for tof, we have constructed consistent empirical physical formulas (EPFs) by appropriate ANNs. These ANN–EPFs can be used to derive further physical functions which could be relevant to discrimination between gamma-rays and neutrons

Separate and combined effects of 1-pentanol applied to the eggs and gamma radiation applied to the pupae on some biological aspects of the medfly, ceratitis capitata Wied

International Nuclear Information System (INIS)

Wakid, A.M.; Fadel, A.M.

1996-01-01

Laboratory experiments were conducted on the medfly, ceratitis capitata (Wied) to study the separate and combined effects of the alcohol, l-pentanol (1-3%), applied to the eggs and gamma radiation (50 and 90 Gy) applied to the pupae on egg hatch, pupation, adult emergence. sex ration, adult survival, sterility and male mating competitiveness. The concentrations 1,2 and 3% of 1-pentanol applied to eggs for one or two days did not affect neither egg hatch, pupation, adult emergence nor sec ratio. Also there were no clear differences in adult emergence, sex ration or male and female survival, in different treatments studied (Irradiated, treated and treated irradiated). Male sterility, treated as eggs with 2% 1-pentanol for one or two days and irradiated as pupae (8-9 days), was increased significantly at 90 Gy compared to 50 Gy or the control. Moreover male competitiveness was increased significantly at 50 Gy compared to 90 Gy whether when eggs were treated with the alcohol or not. Treating eggs with the alcohol produced more competitive males especially when treatment was achieved for one day. 2 figs., 3 tabs

Gamma spectroscopy analysis of archived Marshall Island soil samples

International Nuclear Information System (INIS)

Herman, S.; Hoffman, K.; Lavelle, K.; Trauth, A.; Glover, S.E.; Connick, W.; Spitz, H.; LaMont, S.P.; Hamilton, T.

2016-01-01

Four samples of archival Marshall Islands soil were subjected to non-destructive, broad energy (17 keV-2.61 MeV) gamma-ray spectrometry analysis using a series of different high-resolution germanium detectors. These archival samples were collected in 1967 from different locations on Bikini Atoll and were contaminated with a range of fission and activation products, and other nuclear material from multiple weapons tests. Unlike samples collected recently, these samples have been stored in sealed containers and have been unaffected by approximately 50 years of weathering. Initial results show that the samples contained measurable but proportionally different concentrations of plutonium, 241 Am, and 137 Cs, and 60 Co. (author)

Thermally stimulated capacitance in gamma irradiated epitaxial 4H-SiC Schottky barrier diodes

Science.gov (United States)

Vigneshwara Raja, P.; Narasimha Murty, N. V. L.

2018-04-01

Deep level defects in 4H-SiC Schottky barrier diodes (SBDs) fabricated on n-type epitaxial 4H-SiC have been identified by thermally stimulated capacitance (TSCAP) spectroscopy prior to and after 60Co-gamma irradiation. The TSCAP measurements on the non-irradiated SBDs reveal two electron traps at Ec-0.63 eV (˜250 K) and Ec-1.13 eV (˜525 K), whereas only one trap at Ec-0.63 eV is identified by conventional thermally stimulated current (TSC) measurements. Hence, TSCAP spectroscopy is more effective in identifying deep level defects in epitaxial 4 H-SiC SBDs as compared to the TSC spectroscopy. Upon exposure to 60Co-gamma rays up to a dose of 100 Mrad, significant changes in the concentration of the traps at Ec-0.63 eV, Ec-1.13 eV, and one new trap at Ec-0.89 eV (˜420 K) are observed. The electrical characteristics of the SBDs are considerably changed after gamma irradiation. The dominant mechanisms responsible for the irradiation induced changes in the SBD electrical characteristics are analyzed by incorporating the trap signatures in the commercial Silvaco® TCAD device simulator. The extracted trap parameters of the irradiated SBDs may be helpful in predicting the survival of 4H-SiC SBD detectors at higher irradiation levels.

Optical study of gamma irradiated sodium metaphosphate glasses containing divalent metal oxide MO (ZnO or CdO

Directory of Open Access Journals (Sweden)

E. Nabhan

Full Text Available Sodium metaphosphate glasses containing divalent metal oxide, ZnO or CdO with composition 50 P2O5 – (50 − x Na2O – x MO (ZnO, or CdO where x = 0, 10, 20 (mol% were prepared by conventional melt method. UV/visible spectroscopy and FTIR spectroscopy are measured before and after exposing to successive gamma irradiation doses (5–80 kGy. The optical absorption spectra results of the samples before irradiation reveal a strong UV absorption band at (∼230 nm which is related to unavoided iron impurities. The effects of gamma irradiation on the optical spectral properties of the various glasses have been compared. From the optical absorption spectral data, the optical band gap is evaluated. The main structural groups and the influence of both divalent metal oxide and gamma irradiation effect on the structural vibrational groups are realized through IR spectroscopy. The FTIR spectra of γ-irradiated samples are characterized by the stability of the number and position for the main characteristic band of phosphate groups. To better understood the structural changes during γ-irradiation, a deconvolution of FTIR spectra in the range 650–1450 cm−1 is made. The FTIR deconvolution results found evidence that, the changes occurring after gamma irradiation have been related to irradiation induced structural defects and compositional changes. Keywords: Sodium metaphosphate glass, UV–visible spectra, IR spectra, Deconvolution, Optical band gap, Gamma ray

Quality assurance system in gamma spectrometry laboratory

International Nuclear Information System (INIS)

Mielnikow, A.; Michalik, B.; Chalupnik, S.; Lebecka, J.

1996-01-01

On basis of guidelines for development of QUALITY SYSTEM for a testing laboratory (European Standard Series EN 45000) a quality assurance system was implemented in gamma spectroscopy laboratory, where routine measurements of natural (mainly Ra-226, Ra-228, Ra-224, K-40) and artificial (mainly Cs-137 and Cs-134) isotopes are performed. We measure a variety of samples, but mainly coal, vaste rock, ashe, deposits, vegetation and air filters. Laboratory of gamma spectroscopy in Central Mining Institute has three HPGe detectors. There is one coaxial detector with 45% relative efficiency, one detector for low energy region and one detector with extended range). We have also two Ge(Li) detectors from former Czechoslovakia. Shielding is made mainly of steel (40 cm) with the interior covered with lead and copper. The electronics and software (Genie-PC) was bought at 'Canberra' and 'Silena'. The paper describes not only the system of quality assurance but also main problems met by its implementation and results of intercomparison measurements. The QAS has been introduced in 1992. In 1993 the Accreditation Certificate of Testing Laboratory for our Laboratory has been obtained from the Polish Bureau of Research and Certification as a fifth laboratory in Poland. (author)

Gamma Irradiation Induced Degradation of Orange Peels

Directory of Open Access Journals (Sweden)

Jaime Saucedo Luna

2012-08-01

Full Text Available In this study, gamma irradiation induced degradation of orange peels (OP was investigated. The lignocellulosic biomass degradation was carried out at doses of 0 (control, 600, 1800 and 3500 kGy using a Co-60 gamma radiation source. The samples were tested for total and reducing sugars. The concentrations of total sugars ranged from 0.530 g∙g⁻¹ in control sample to 0.382 g∙g⁻¹ of dry weight in the sample which received the highest radiation dose. The reducing sugars content varying from 0.018 to 0.184 g∙g⁻¹ of dry weight with the largest rise occurring in the sample irradiated at 3500 kGy. The concentrations of sucrose, glucose and fructose were determined. The changes generated in physico-chemical properties were determined by Fourier Transform Infrared Spectroscopy (FTIR and termogravimetric analysis (TG-DTG. The results show that OP was affected, but not significantly, which suggests that lignocellulose and sugars profiles were partially degraded after gamma irradiation.

An Overview of the Evolution of Infrared Spectroscopy Applied to Bacterial Typing.

Science.gov (United States)

Quintelas, Cristina; Ferreira, Eugénio C; Lopes, João A; Sousa, Clara

2018-01-01

The sustained emergence of new declared bacterial species makes typing a continuous challenge for microbiologists. Molecular biology techniques have a very significant role in the context of bacterial typing, but they are often very laborious, time consuming, and eventually fail when dealing with very closely related species. Spectroscopic-based techniques appear in some situations as a viable alternative to molecular methods with advantages in terms of analysis time and cost. Infrared and mass spectrometry are among the most exploited techniques in this context: particularly, infrared spectroscopy emerged as a very promising method with multiple reported successful applications. This article presents a systematic review on infrared spectroscopy applications for bacterial typing, highlighting fundamental aspects of infrared spectroscopy, a detailed literature review (covering different taxonomic levels and bacterial species), advantages, and limitations of the technique over molecular biology methods and a comparison with other competing spectroscopic techniques such as MALDI-TOF MS, Raman, and intrinsic fluorescence. Infrared spectroscopy possesses a high potential for bacterial typing at distinct taxonomic levels and worthy of further developments and systematization. The development of databases appears fundamental toward the establishment of infrared spectroscopy as a viable method for bacterial typing. © 2017 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

Radiosurgery with the gamma knife; Radiochirurgie mit dem Gamma-Knife

Energy Technology Data Exchange (ETDEWEB)

Wowra, B.; Reulen, H.J.

1996-05-10

Radiosurgery is a novel modality introduced by the neurosurgeon Lars Leksell. For the most important lesions, (arteriovenous angiomas, benign tumors in the base of the skull, formation of metastases in the brain), radiosurgery is a valuable additional tool in the range of therapies available to the benefit of patients. The gamma knife has been gaining a leading rank in the range of therapies applied in Germany. (orig.) [Deutsch] Radiochirurgie ist ein neues, von dem Neurochirurgen Lars Leksell konzipiertes Prinzip. Bei den wichtigsten Indikationen (arteriovenoese Angiome, gutartige Tumoren der Schaedelbasis, Hirnmetastasen etc.) bereichert und ergaenzt die Radiochirurgie das therapeutische Arsenal der Neurochirurgie zum Vorteil der Patienten betraechtlich. Dem Gamma-Knife kommt jetzt auch in Deutschland ein prominenter Platz unter den verschiedenen radiochirurgischen Verfahren zu. (orig.)

The optimization of gamma spectra processing in prompt gamma neutron activation analysis (PGNAA)

Energy Technology Data Exchange (ETDEWEB)

Pinault, Jean-Louis [IAEA Expert, 96 rue du Port David, 45370 Dry (France)], E-mail: jeanlouis_pinault@hotmail.fr; Solis, Jose [Instituto Peruano de Energia Nuclear, Av. Canada No. 1470, San Borja, Lima 41 (Peru)

2009-04-15

The uncertainty of the elemental analysis is one of the major factors governing the utility of on-line Prompt Gamma Neutron Activation Analysis (PGNAA) in the blending and sorting of bulk materials. In this paper, a general method applicable to Gamma spectra processing is presented and applied to PGNAA in mineral industry. Based on the Fourier transform of spectra and their de-correlation in the Fourier space (the improvement of the conditioning of the correlation matrix), processing of overlapping of characteristic peaks minimizes the propagation of random errors, which optimizes the accuracy and decreases the detection limits of elemental analyses. In comparison with classical methods based on the linear combinations of relevant regions of spectra the improvement may be considerable, especially when several elements are interfering. The method is applied to four case stories covering both borehole logging and on-line analysis on conveyor belt of raw materials.

Investigation of gamma spectra analysis

International Nuclear Information System (INIS)

Wu Huailong; Liu Suping; Hao Fanhua; Gong Jian; Liu Xiaoya

2006-01-01

In the investigation of radiation fingerprint comparison, it is found out that some of the popular gamma spectra analysis software have shortcomings, which decrease the radiation fingerprint comparison precision. So a new analysis software is developed for solving the problems. In order to display the advantage of developed program, some typical simulative warhead gamma spectra are analyzed respectively by present software and GAMMAVISION and GENNIE2000. Present software can be applied not only in nuclear warheads deep-cuts verification, but also in any radiation measurement field. (authors)

High-energy emission from gamma-ray bursts

International Nuclear Information System (INIS)

Nolan, P.L.; Share, G.H.; Matz, S.; Chupp, E.L.; Forrest, D.J.; Rieger, E.

1984-01-01

We discuss broad-band continuum spectroscopy of 17 gamma-ray bursts above 0.3 MeV. The spectra were fitted by 3 trial functions, none of which provided an adequate fit to all the spectra. Most were too hard for a thermal bremsstarhlung function. Harder functional forms, such as thermal synchrotron or power-law, provide better fits for most of the spectra. The strong emission observed above 1 MeV raises some interesting theoretical questions

$\\beta$-decay studies using total-absorption spectroscopy

CERN Document Server

Algora, A; García-Borge, M J; Cano-Ott, D; Collatz, R; Courtin, S; Dessagne, P; Fraile-Prieto, L M; Gadea, A; Gelletly, W; Hellström, M; Janas, Z; Jungclaus, A; Kirchner, R; Karny, M; Le Scornet, G; Miehé, C; Maréchal, F; Moroz, F; Nacher, E; Poirier, E; Roeckl, E; Rubio, B; Rykaczewski, K; Taín, J L; Tengblad, O; Wittmann, V

2004-01-01

$\\beta$-decay experiments are a primary source of information for nuclear-structure studies and at the same time complementary to in- beam investigations of nuclei far from stability. Although both types of experiment are mainly based on $\\gamma$-ray spectroscopy, they face different experimental problems. The so-called " Pandemonium effect " is a critical problem in $\\beta$-decay if we are to test theoretically calculated transition probabilities. In this contribution we will present a solution to this problem using total absorption spectroscopy methods. We will also present some examples of experiments carried out with the Total Absorption Spectrometer (TAS) at GSI and describe a new device LUCRECIA recently installed at CERN.

UV spectroscopy applied to stratospheric chemistry, methods and results

Energy Technology Data Exchange (ETDEWEB)

Karlsen, K.

1996-03-01

The publication from the Norwegian Institute for Air Research (NILU) deals with an investigation done on stratospheric chemistry by UV spectroscopy. The scientific goals are briefly discussed, and it gives the results from the measuring and analysing techniques used in the investigation. 6 refs., 11 figs.

Prompt gamma cold neutron activation analysis applied to biological materials

International Nuclear Information System (INIS)

Rossbach, M.; Hiep, N.T.

1992-01-01

Cold neutrons at the external neutron guide laboratory (ELLA) of the KFA Juelich are used to demonstrate their profitable application for multielement characterization of biological materials. The set-up and experimental conditions of the Prompt Gamma Cold Neutron Activation Analysis (PGCNAA) device is described in detail. Results for C, H, N, S, K, B, and Cd using synthetic standards and the 'ratio' technique for calculation are reported for several reference materials and prove the method to be reliable and complementary with respect to the elements being determined by INAA. (orig.)

Self-attenuation of gamma rays during radioactivity concentration analysis of environmental samples

International Nuclear Information System (INIS)

Watson, D.; Dharmasiri, J.; Akber, R.

2001-01-01

Gamma spectroscopy using HPGe detector systems is a readily used technique for routine analysis of radioactivity in environmental samples. The systems are generally calibrated using standards of known radioactivity and composition. Radioactivity in environmental samples is generally distributed in the bulk of the material. When a sample of finite thickness is analysed through gamma spectroscopy, a proportion of the gamma rays emitted from the sample is either stopped or scattered from the sample material itself. These processes of self-absorption and self-attenuation depend upon the physical and elemental composition of the sample and the energy of the gamma radiation. Since environmental samples vary in composition, instrument calibration using a fixed matrix composition may not be valid for a diversity of samples. We selected and analysed five sample matrices to investigate the influence of self-absorption and self-attenuation in environmental samples. Our selection consisted of bentonite and kaolin representing clay, quartz representing silica, ash representing prepared biota, and analytical grade MnO 2 representing a co-precipitant used for extractive radioactivity from aqueous samples. Our findings show that within 5% of uncertainty the silica based standards can be used to cover the environmental samples of varying clay (silica content). The detection efficiency for ash and MnO 2 could be different particularly in the 30 - 100 keV energy range. The differences in sample behaviour can be explained on the basis of atomic number, mass number and density

Radiation-induced defects in chalcogenide glasses characterized by combined optical spectroscopy, XPS and PALS methods

Energy Technology Data Exchange (ETDEWEB)

Shpotyuk, O. [Institute of Physics of Jan Dlugosz University, 13/15 al. Armii Krajowej, Czestochowa 42201 (Poland); Lehigh University, 5 East Packer Avenue, Bethlehem, PA 18015-3195 (United States); Lviv Institute of Materials of SRC ' ' Carat' ' , 202, Stryjska str., 79031 Lviv (Ukraine); Kovalskiy, A.; Jain, H. [Lehigh University, 5 East Packer Avenue, Bethlehem, PA 18015-3195 (United States); Golovchak, R. [Lehigh University, 5 East Packer Avenue, Bethlehem, PA 18015-3195 (United States); Lviv Institute of Materials of SRC ' ' Carat' ' , 202, Stryjska str., 79031 Lviv (Ukraine); Zurawska, A. [Opole University of Technology, 75, Ozimska str., Opole 45370 (Poland)

2007-03-15

Temperature-dependent optical absorption spectroscopy, high-resolution X-ray photoelectron spectroscopy and positron annihilation lifetimes spectroscopy are utilized to understand radiation-induced changes in Ge-Sb-S chalcogenide glasses. Theoretically predicted topological scheme of {gamma}-induced coordination defect formation in stoichiometric Ge{sub 23.5}Sb{sub 11.8}S{sub 64.7} glass composition is supported by these measurements. (copyright 2007 WILEY-VCH Verlag GmbH and Co. KGaA, Weinheim) (orig.)

GRB 080517: a local, low-luminosity gamma-ray burst in a dusty galaxy at z = 0.09

NARCIS (Netherlands)

Stanway, E.R.; Levan, A.J.; Tanvir, N.; Wiersema, K.; van der Horst, A.; Mundell, C.G.; Guidorzi, C.

2015-01-01

We present an analysis of the photometry and spectroscopy of the host galaxy of Swift-detected GRB 080517. From our optical spectroscopy, we identify a redshift of z = 0.089 ± 0.003, based on strong emission lines, making this a rare example of a very local, low-luminosity, long gamma-ray burst. The

Study on gamma radiation-induced synthesis of gold nanoparticles stabilized by hyaluronan

International Nuclear Information System (INIS)

Dang Van Phu; Nguyen Ngoc Duy; Nguyen Tue Anh; Nguyen Quoc Hien

2011-01-01

Gold nanoparticles (AuNPs) with diameter from 4 to 10 nm were synthesized in hyaluronan (HA) solution without usage of any reductant and *OH radical scavenger by gamma irradiation reduction. The size and size distribution of AuNPs were determined by TEM images. The λ max (517 - 525 nm) of colloidal AuNPs solutions as prepared were measured by UV-Vis spectroscopy. The influence factors on the size of AuNPs particularly the concentration of Au 3+ , HA and dose rate were investigated. The stability of AuNPs/HA as synthesized was more than 6 months in storage under atmospheric condition. AuNPs with the size less than 10 nm and narrow size distribution stabilized by HA which is biocompatible natural polysaccharide so that AuNPs/HA can potentially be applied in biomedicine and cosmetic. (author)

Mössbauer study of the effect of gamma irradiation on the removal of pyrite from Colombian coals

International Nuclear Information System (INIS)

Mejía, J A; Palacio, C A; Caballero, F Reyes; Dávila, H Olaya; Ovalle, S A Martínez; De Grave, E

2014-01-01

The removal of sulfur from the coals is necessary before using it. It is due to the environmental and technological problems that it causes. In this work, the results of the study by Mössbauer spectroscopy of the gamma-irradiation effect on the pyrite in three Colombian coals are analyzed. They were exposed to different gamma-irradiation doses using a 60 Co source

Synthesis and characterization of the silver methacrylate and its polymerization with gamma radiation

International Nuclear Information System (INIS)

Figueroa de Paz, Y. M.

2014-01-01

One of the traditional objectives in research has been the development of new and useful materials that combine the properties of polymers with metals. Synthesis of monomers containing metal, followed by a polymerization process, is a method to introduce metal ions in the structure of a polymer, and the gamma radiation was easily applied to initiate polymerization. The coordination polymers have high insolubility, which is a general problem of these materials, besides the lack of structural information available. Also, due to the difficulty of obtaining single crystals, it has hindered the identification of the structures of some coordination polymers, requiring the use of indirect methods for structural characterization. In this work the synthesis of silver poly-methacrylate (PMAAg), was performed using the gamma radiation as polymerization initiator, having as precursor to silver methacrylate monomer (MAAg). The combination of spectroscopic methods revealed structural changes in the coordination polymers. With scanning electron microscopy, it was observed that the morphology of the monomer and its polymers is fiber, which grows with increasing radiation dose; furthermore, this increase in size is related to Bet analysis result, since the monomer has a bigger superficial area to the irradiated polymers. In monomer and irradiated polymers the crystalline structure CCC was observed by X-ray diffraction. By thermogravimetric analysis the decomposition temperature of the products was determined, finding around 150 degrees C. The infrared spectroscopy confirmed the silver methacrylate polymerization, as with increasing radiation dose, also increases the degree of polymerization; likewise the form of coordination of the monomer was determined and its irradiated polymers which corresponds to a bi-dentate chelate, confirmed by X-ray photoelectron spectroscopy. (Author)

The measurement of gamma ray induced heating in a mixed neutron and gamma ray environment

International Nuclear Information System (INIS)

Chiu, H.K.

1991-10-01

The problem of measuring the gamma heating in a mixed DT neutron and gamma ray environment was explored. A new detector technique was developed to make this measurement. Gamma heating measurements were made in a low-Z assembly irradiated with 14-Mev neutrons and (n, n') gammas produced by a Texas Nuclear Model 9400 neutron generator. Heating measurements were made in the mid-line of the lattice using a proportional counter operating in the Continuously-varied Bias-voltage Acquisition mode. The neutron-induced signal was separated from the gamma-induced signal by exploiting the signal rise-time differences inherent to radiations of different linear energy transfer coefficient, which are observable in a proportional counter. The operating limits of this measurement technique were explored by varying the counter position in the low-Z lattice, hence changing the irradiation spectrum observed. The experiment was modelled numerically to help interpret the measured results. The transport of neutrons and gamma rays in the assembly was modelled using the one- dimensional radiation transport code ANISN/PC. The cross-section set used for these calculations was derived from the ENDF/B-V library using the code MC 2 -2 for the case of DT neutrons slowing down in a low-Z material. The calculated neutron and gamma spectra in the slab and the relevant mass-stopping powers were used to construct weighting factors which relate the energy deposition in the counter fill-gas to that in the counter wall and in the surrounding material. The gamma energy deposition at various positions in the lattice is estimated by applying these weighting factors to the measured gamma energy deposition in the counter at those locations

CeBr3 as a room-temperature, high-resolution gamma-ray detector

International Nuclear Information System (INIS)

Guss, Paul; Reed, Michael; Yuan Ding; Reed, Alexis; Mukhopadhyay, Sanjoy

2009-01-01

Cerium bromide (CeBr 3 ) has become a material of interest in the race for high-resolution gamma-ray spectroscopy at room temperature. This investigation quantified the potential of CeBr 3 as a room-temperature, high-resolution gamma-ray detector. The performance of CeBr 3 crystals was compared to other scintillation crystals of similar dimensions and detection environments. Comparison of self-activity of CeBr 3 to cerium-doped lanthanum tribromide (LaBr 3 :Ce) was performed. Energy resolution and relative intrinsic efficiency were measured and are presented.

Advantages of GSO Scintillator in Imaging and Law Level Gamma-ray Spectroscopy

CERN Document Server

Sharaf, J

2002-01-01

The single GSO crystal is an excellent scintillation material featuring a high light yield and short decay time for gamma-ray detection. Its performance characteristics were investigated and directly compared to those of BGO. For this purpose, the two scintillators are cut into small crystals of approximately 4*4*10 mm sup 3 and mounted on a PMT. Energy resolution, detection efficiency and counting precision have been measured for various photon energies. In addition to this spectroscopic characterization, the imaging performance of GSO was studied using a scanning rig. The modulation transfer function was calculated and the spatial resolution evaluated by measurements of the detector's point spread function. It is shown that there exists some source intensity for which the two scintillators yield identical precision for identical count time. Below this intensity, the GSO is superior to the BGO detector. The presented properties of GSO suggest potential applications of this scintillator in gamma-ray spectrosc...

Assessment of the toxicity level of gamma-irradiated snake (Naja naja oxiana) venom by photoacoustic spectroscopy

International Nuclear Information System (INIS)

Vidyasagar, P.B.; Pal, Saumen

1991-01-01

Immunization is the only answer to the challenge of the diseases for which it is extremely difficult to institute timely and proper treatment following the inset. Various antigenic agents responsible for such diseases are used for the purpose of immunization to overcome this difficulty. To make safe use of the antigens it is required to reduce their toxicity level keeping the antigenicity intact and develop a suitable way to detect it. To ensure this, toxoids are produced from the toxic antigens by using different physical and chemical methods. Snake venoms are some important antigens which deserve more attention to be used for immunization because bites by poisonous snakes require instant treatment which is difficult to install. Toxoids used in the present study were produced by irradiating oxus cobra (Naja naja oxiana) venom under cobalt-60 gamma-ray source. The toxocity level of thus produced venom toxoid was assessed by photoacoustic (PA) spectroscopy. In support of the PA observations, optical absorption and fluorescence spectra of the venom in solution were also studied. Percentile change in PA signal intensity was taken as the parameter for toxocity level which was then correlated to the percentile residual toxocity of the venom obtained by direct method of injecting the venom in mice. Efforts were also made to find out the possible effects of the radiation on the venom. (author). 29 refs., 7 figs

Study of radiation damage in ODS steels by positron annihilation spectroscopy

International Nuclear Information System (INIS)

Bartošová, I; Bouhaddane, A; Slugeň, V; Dománková, M; Wall, D; Selim, F A

2016-01-01

Microstructure of various oxide-dispersion-strengthened (ODS) steels with 15% chromium content was studied in term of vacancy defects presence and their accumulation after defined irradiation treatment, respectively. Studied materials originated from Kyoto University and studied via IAEA collaborative project. Samples were characterized “as received” by positron annihilation lifetime spectroscopy and their microstructure was examined by transmission electron microscopy as well. Samples were afterwards irradiated in Washington State University Nuclear Radiation Center via a strong gamma source (6TBq). Damage induced by gamma irradiation was evaluated by positron lifetime measurements in emphasis on defect accumulation in the materials. We have demonstrated strong defect production induced by gamma irradiation which results from positron measurement data. (paper)

Gamma-ray spectroscopy applications in radiation control and environmental monitoring

Energy Technology Data Exchange (ETDEWEB)

Manushev, B [Sofia Univ. (Bulgaria). Fizicheski Fakultet; Koleva, K [National Metrology Centre, Sofia (Bulgaria)

1996-12-31

A method for stabilization of gamma-ray spectrometers energy calibration is proposed. It is based on recalibration of the spectrum by numerical filtration. The possibility of efficiency auto-calibration is considered in the case when a reference source with appropriate shape is unavailable. The method is tested by estimation of the effective thickness of a lead plate (self-absorption). Potential applications include the evaluation of surface pollution infiltration depth as well as the development of pure beta sources (e.g. Sr-90) using the registration of their Bremsstrahlung. 6 refs.

Investigation of gamma spectra analysis

International Nuclear Information System (INIS)

Wu Huailong; Liu Suping; Hao Fanhua

2006-12-01

During the investigation of radiation fingerprint comparison, it is found out that the popular gamma spectra analysis softwares are faultful, which decrease the precision of radiation fingerprint comparison. So a new analysis software is development for solving the problems. In order to display the advantage of new program, some typical simulative gamma spectra of radiation source are analyzed respectively by our software and GAMMAVISION and GENNIE2000. The software can be applied not only in nuclear warheads deep-cuts verification, but also in any radiation measurement field. (authors)

Special Nuclear Material Gamma-Ray Signatures for Reachback Analysts

Energy Technology Data Exchange (ETDEWEB)

Karpius, Peter Joseph [Los Alamos National Lab. (LANL), Los Alamos, NM (United States); Myers, Steven Charles [Los Alamos National Lab. (LANL), Los Alamos, NM (United States)

2016-08-29

These are slides on special nuclear material gamma-ray signatures for reachback analysts for an LSS Spectroscopy course. The closing thoughts for this presentation are the following: SNM materials have definite spectral signatures that should be readily recognizable to analysts in both bare and shielded configurations. One can estimate burnup of plutonium using certain pairs of peaks that are a few keV apart. In most cases, one cannot reliably estimate uranium enrichment in an analogous way to the estimation of plutonium burnup. The origin of the most intense peaks from some SNM items may be indirect and from ‘associated nuclides.' Indirect SNM signatures sometimes have commonalities with the natural gamma-ray background.

In vivo Raman spectroscopy detects increased epidermal antioxidative potential with topically applied carotenoids

International Nuclear Information System (INIS)

Lademann, J; Richter, H; Patzelt, A; Darvin, M; Sterry, W; Fluhr, J W; Caspers, P J; Van der Pol, A; Zastrow, L

2009-01-01

In the present study, the distribution of the carotenoids as a marker for the complete antioxidative potential in human skin was investigated before and after the topical application of carotenoids by in vivo Raman spectroscopy with an excitation wavelength of 785 nm. The carotenoid profile was assessed after a short term topical application in 4 healthy volunteers. In the untreated skin, the highest concentration of natural carotenoids was detected in different layers of the stratum corneum (SC) close to the skin surface. After topical application of carotenoids, an increase in the antioxidative potential in the skin could be observed. Topically applied carotenoids penetrate deep into the epidermis down to approximately 24 μm. This study supports the hypothesis that antioxidative substances are secreted via eccrine sweat glands and/or sebaceous glands to the skin surface. Subsequently they penetrate into the different layers of the SC

Fourier transform infrared spectroscopic study of gamma irradiated SiO2 nanoparticles

Science.gov (United States)

Huseynov, Elchin; Garibov, Adil; Mehdiyeva, Ravan; Huseynova, Efsane

2018-03-01

In the present work, nano SiO2 particles are investigated before and after gamma irradiation (25, 50, 75, 100 and 200 kGy) using Fourier transform infrared (FTIR) spectroscopy method for the wavenumber between 400-4000 cm-1. It is found that as a result of spectroscopic analysis, five new peaks have appeared after gamma radiation. Two of new obtained peaks (which are located at 687 cm-1 and 2357 cm-1 of wavenumber) were formed as a result of gamma radiation interaction with Si-O bonds. Another three new peaks (peaks appropriate to 941, 2052 and 2357 cm-1 values of wavenumber) appear as a result of interaction of water with nano SiO2 particles after gamma irradiation. It has been defined as asymmetrical bending vibration, symmetrical bending vibration, symmetrical stretching vibration and asymmetrical stretching vibration of Si-O bonds appropriate to peaks.

Determination of curie content and 134/137cesium ratios by gamma spectroscopy of high burnup plutonium-aluminum fuel assemblies

International Nuclear Information System (INIS)

Haggard, D.L.; Tanner, J.E.

1997-06-01

Nondestructive assay (NDA) gamma spectroscopy techniques were used to measure 134/137 Cs ratios on nine PuAl Mark 42 fuel assemblies. The purpose of the ratio measurement was to confirm theoretical burnup calculations. 134/137 Cs ratios were determined from the measured activity based on corrected net peak area counts for the 605 keV peak from 134 Cs and the 662 keV peak from 137 Cs/ 137m Ba. Assembly No. 2 134/137 Cs ratio measured on 4-15-92 was 0.19. The measured 134/137 Cs ratio was decay corrected to be 2.11 on 8-1-84 based on the half lives of 134 Cs and 137 Cs. The measured 134/137 Cs ratio range was 1.90--2.14 for all nine assemblies. These measured values compare to a theoretical ratio of 1.7 on 8-1-84 determined by burnup calculations. Total cesium curie content was also requested and determined using the NDA direct measurements. Gamma spectral data were measured on the nine sectioned Mark 42 fuel assemblies. Measured cesium curie content, decay corrected to 8-1-84, ranged from 18170--24480 curies of 134 Cs and 8620--11646 curies of 137 Cs. Theoretical cesium curie content of 8-1-84 was 15200 curies 134 Cs and 8973 curies 137 Cs. Direct assay cesium ratio is 12% to 26% higher than the predicted ratio of 1.7. The measured 134 Cs data indicate between 20%--61% more activity than that predicted by the burnup code, whereas the measured 137 Cs activity is between 4% less to 30% more than the predicted activity. This information may be used to address issues concerning criticality safety, storage, and shipping of this type of material

Application of Principal Component Analysis in Prompt Gamma Spectra for Material Sorting

Energy Technology Data Exchange (ETDEWEB)

Im, Hee Jung; Lee, Yun Hee; Song, Byoung Chul; Park, Yong Joon; Kim, Won Ho

2006-11-15

For the detection of illicit materials in a very short time by comparing unknown samples' gamma spectra to pre-programmed material signatures, we at first, selected a method to reduce the noise of the obtained gamma spectra. After a noise reduction, a pattern recognition technique was applied to discriminate the illicit materials from the innocuous materials in the noise reduced data. Principal component analysis was applied for a noise reduction and pattern recognition in prompt gamma spectra. A computer program for the detection of illicit materials based on PCA method was developed in our lab and can be applied to the PGNAA system for the baggage checking at all ports of entry at a very short time.

$\\gamma$-$\\gamma$ and $\\gamma$-p events at high energies

CERN Document Server

Schuler, Gerhard A.; Gerhard A Schuler; Torbjorn Sjostrand

1994-01-01

A real photon has a complicated nature, whereby it may remain unresolved or fluctuate into a vector meson or a perturbative q-qbar pair. Based on this picture, we previously presented a model for gamma-p events that is based on the presence of three main event classes: direct, VMD and anomalous. In gamma-gamma events, a natural generalization gives three-by-three combinations of the nature of the two incoming photons, and thus six distinct event classes. The properties of these classes are constrained by the choices already made, in the gamma-p model, of cut-off procedures and other aspects. It is therefore possible to predict the energy-dependence of the cross section for each of the six components separately. The total cross section thus obtained is in good agreement with data, and also gives support to the idea that a simple factorized ansatz with a pomeron and a reggeon term can be a good approximation. Event properties undergo a logical evolution from p-p to gamma-p to gamma-gamma events, with larger cha...

Efficiency of cement - based low - weight shielding materials for Cs-137 gamma rays

International Nuclear Information System (INIS)

Satty, H. E. M.

2014-10-01

Due to the development of nuclear technology and use of technologies in various field of industry, medicine and research against ionizing radiation is one of the most important topics in this field. The purpose of this work is to reduce the dose rate from radioactive sources. The exposure to gamma radiation is leading to several health effects as the result of absorption by the human body. The frequently used shielding material for gamma rays is lead. In spite of its effectiveness and high mass attenuation coefficient, lower weight gamma shielding materials are required. In this effectiveness of three materials: carbon and mixture (50% carbon + 50% cement) was studied and compared to that of lead. The results were obtained in terms of the variations of the transmitted intensity. This is done using a gamma spectroscopy system.(Author)

The spectroscopy of fission fragments

International Nuclear Information System (INIS)

Phillips, W.R.

1998-01-01

High-resolution measurements on γ rays from fission fragments have provided a rich source of information, unobtainable at the moment in any other way, on the spectroscopy of neutron-rich nuclei. In recent years important data have been obtained on the yrast- and near yrast-structure of neutron-rich fission fragments. We discuss the scope of measurements which can be made on prompt gamma rays from secondary fission fragments, the techniques used in the experiments and some results recently obtained. (author)

Gamma ray energy tracking in GRETINA

Science.gov (United States)

Lee, I. Y.

2011-10-01

The next generation of stable and exotic beam accelerators will provide physics opportunities to study nuclei farther away from the line of stability. However, these experiments will be more demanding on instrumentation performance. These come from the lower production rate for more exotic beams, worse beam impurities, and large beam velocity from the fragmentation and inverse reactions. Gamma-ray spectroscopy will be one of the most effective tools to study exotic nuclei. However, to fully exploit the physics reach provided by these new facilities, better gamma-ray detector will be needed. In the last 10 years, a new concept, gamma-ray energy tracking array, was developed. Tracking arrays will increase the detection sensitivity by factors of several hundred compared to current arrays used in nuclear physics research. Particularly, the capability of reconstructing the position of the interaction with millimeters resolution is needed to correct the Doppler broadening of gamma rays emitted from high velocity nuclei. GRETINA is a gamma-ray tracking array which uses 28 Ge crystals, each with 36 segments, to cover ¼ of the 4 π of the 4 π solid angle. The gamma ray tracking technique requires detailed pulse shape information from each of the segments. These pulses are digitized using 14-bit 100 MHz flash ADCs, and digital signal analysis algorithms implemented in the on-board FPGAs provides energy, time and selection of pulse traces. A digital trigger system, provided flexible trigger functions including a fast trigger output, and also allows complicated trigger decisions to be made up to 20 microseconds. Further analyzed, carried out in a computer cluster, determine the energy, time, and three-dimensional positions of all gamma-ray interactions in the array. This information is then utilized, together with the characteristics of Compton scattering and pair-production processes, to track the scattering sequences of the gamma rays. GRETINA construction is completed in

Gamma Large Area Silicon Telescope (GLAST): Applying silicon strip detector technology to the detection of gamma rays in space

International Nuclear Information System (INIS)

Atwood, W.B.

1993-06-01

The recent discoveries and excitement generated by space satellite experiment EGRET (presently operating on Compton Gamma Ray Observatory -- CGRO) have prompted an investigation into modern detector technologies for the next generation space based gamma ray telescopes. The GLAST proposal is based on silicon strip detectors as the open-quotes technology of choiceclose quotes for space application: no consumables, no gas volume, robust (versus fragile), long lived, and self triggerable. The GLAST detector basically has two components: a tracking module preceding a calorimeter. The tracking module has planes of crossed strip (x,y) 300 μm pitch silicon detectors coupled to a thin radiator to measure the coordinates of converted electron-positron pairs. The gap between the layers (∼5 cm) provides a lever arm for track fitting resulting in an angular resolution of <0.1 degree at high energy. The status of this R ampersand D effort is discussed including details on triggering the instrument, the organization of the detector electronics and readout, and work on computer simulations to model this instrument

Ultrasonography X gamma radiography

International Nuclear Information System (INIS)

Mello Campos, A.M. de

1989-01-01

The accumulated experience in the last ten years of substitution to essays by gamma radiography to essay by ultrasonography, starting of the systematic comparison and tabulation of the results obtained by both essays applied in welding joints, in field, in steel pipelines of the SABESP. (V.R.B.)

Multiple gamma lines from semi-annihilation

International Nuclear Information System (INIS)

D'Eramo, Francesco; McCullough, Matthew; Thaler, Jesse

2013-01-01

Hints in the Fermi data for a 130 GeV gamma line from the galactic center have ignited interest in potential gamma line signatures of dark matter. Explanations of this line based on dark matter annihilation face a parametric tension since they often rely on large enhancements of loop-suppressed cross sections. In this paper, we pursue an alternative possibility that dark matter gamma lines could arise from ''semi-annihilation'' among multiple dark sector states. The semi-annihilation reaction ψ i ψ j → ψ k γ with a single final state photon is typically enhanced relative to ordinary annihilation ψ i ψ-bar i → γγ into photon pairs. Semi-annihilation allows for a wide range of dark matter masses compared to the fixed mass value required by annihilation, opening the possibility to explain potential dark matter signatures at higher energies. The most striking prediction of semi-annihilation is the presence of multiple gamma lines, with as many as order N 3 lines possible for N dark sector states, allowing for dark sector spectroscopy. A smoking gun signature arises in the simplest case of degenerate dark matter, where a strong semi-annihilation line at 130 GeV would be accompanied by a weaker annihilation line at 173 GeV. As a proof of principle, we construct two explicit models of dark matter semi-annihilation, one based on non-Abelian vector dark matter and the other based on retrofitting Rayleigh dark matter

Inactivation of fungal contaminants on Korean traditional cashbox by gamma irradiation

Science.gov (United States)

Choi, Jong-il; Lim, Sangyong

2016-01-01

In this study, gamma irradiation was applied to decontaminate a Korean cultural artifact, a wooden cashbox stored in local museum. Fungi isolated from the wooden cashbox were identified by 18S rDNA sequencing methods. It was observed that the isolated fungi exhibited high similarity to Aspergillus niger, Penicillium verruculosum, and Trichoderma viride. Each strain was tested for sensitivity to gamma irradiation, and was inactivated by the irradiation at a dose of 5 kGy. The wooden cashbox was thus gamma-irradiated at this dose (5 kGy), and consequently decontaminated. Two months after the irradiation, when the wooden cashbox was retested to detect biological contamination, no fungi were found. Therefore, these results suggest that gamma irradiation at a low dose of 5 kGy can be applied for successful decontamination of wooden artifacts.

Twenty years of experience in applying gamma spectrometry for NDT

International Nuclear Information System (INIS)

Meenakshisundaram, V.; Raghunath, V.M.

1996-01-01

A NDT technique using NaI(Tl) detector and Single Channel Analyser (SCA) based gamma ray spectrometer was developed to check the shielding integrity of lead poured vessels, for as low a specification as 2% tolerance. The method in detail, its advantages, and some of the interesting findings are described. This paper also highlights other possible in-situ applications like i) identifying cracks propagating in end shield of a Pressurised Heavy Water Reactor (PHWR) in the presence of high radiation field and ii) level estimation for liquids such as Na and NaK used in fast reactor storage tanks. (author)

Chemometric methods and near-infrared spectroscopy applied to bioenergy production

International Nuclear Information System (INIS)

Liebmann, B.

2010-01-01

The present work examines bioenergy production from different viewpoints. The three main objectives are: (1) to reveal the relation of technology, sustainability and economy in bioenergy processes; (2) to investigate spectroscopic methods as a tool for analytical monitoring of bioenergy processes; and (3) to develop new chemometric methods for advanced analysis of spectroscopic data. At the first stage, this thesis investigates the technological, ecological, and economic features of renewable-resource-based and de-centralized bioenergy production systems. In different scenarios, small-scale bioethanol production is combined with other technologies that provide renewable energy from residuals of the bioethanol process. The general aim is to substitute fossil energy conventionally used within the bioethanol process. The investigated technologies are biogas production and straw incineration. Agricultural aspects are introduced by sustainable crop rotation concepts that reconcile food, feed, and biofuel production. The sustainability of small-scale bioethanol production in the different scenarios is quantified by an ecological footprint method, the sustainable process index, SPI, and compared to conventional fuels. The main findings are: (i) small-scaled bioethanol production can be operated with 100 % renewable energy supply, (ii) the SPI of bioethanol can be reduced up to 92 % compared to conventional fuels, (iii) a complex trade-off between ecology-of-scale and economy-of-scale is necessary. At the second stage, this thesis approaches bioenergy production processes from an analytical perspective, and presents near-infrared spectroscopy (NIR) as promising method for fast process monitoring of bioethanol production and biomass characterization. In addition, new analytical methods are presented for a fast determination of the heating value of solid biomass fuel, based on IR and NIR spectroscopy. The main findings are that NIR spectroscopy and appropriate chemometric

GABA level, gamma oscillation, and working memory performance in schizophrenia.

Science.gov (United States)

Chen, Chi-Ming A; Stanford, Arielle D; Mao, Xiangling; Abi-Dargham, Anissa; Shungu, Dikoma C; Lisanby, Sarah H; Schroeder, Charles E; Kegeles, Lawrence S

2014-01-01

A relationship between working memory impairment, disordered neuronal oscillations, and abnormal prefrontal GABA function has been hypothesized in schizophrenia; however, in vivo GABA measurements and gamma band neural synchrony have not yet been compared in schizophrenia. This case-control pilot study (N = 24) compared baseline and working memory task-induced neuronal oscillations acquired with high-density electroencephalograms (EEGs) to GABA levels measured in vivo with magnetic resonance spectroscopy. Working memory performance, baseline GABA level in the left dorsolateral prefrontal cortex (DLPFC), and measures of gamma oscillations from EEGs at baseline and during a working memory task were obtained. A major limitation of this study is a relatively small sample size for several analyses due to the integration of diverse methodologies and participant compliance. Working memory performance was significantly lower for patients than for controls. During the working memory task, patients (n = 7) had significantly lower amplitudes in gamma oscillations than controls (n = 9). However, both at rest and across working memory stages, there were significant correlations between gamma oscillation amplitude and left DLPFC GABA level. Peak gamma frequency during the encoding stage of the working memory task (n = 16) significantly correlated with GABA level and working memory performance. Despite gamma band amplitude deficits in patients across working memory stages, both baseline and working memory-induced gamma oscillations showed strong dependence on baseline GABA levels in patients and controls. These findings suggest a critical role for GABA function in gamma band oscillations, even under conditions of system and cognitive impairments as seen in schizophrenia.

In-beam {gamma}-ray spectroscopy of two-step fragmentation reactions at relativistic energies. The case of {sup 36}Ca

Energy Technology Data Exchange (ETDEWEB)

Doornenbal, P.

2007-10-23

A two-step fragmentation experiment has been performed at GSI with the RISING setup. It combines the fragment separator FRS, which allows for the production of radioactive heavy ions at relativistic energies, with a high resolution {gamma}-spectrometer. This combination offers unique possibilities for nuclear structure investigations like the test of shell model predictions far from stability. Within the present work the question if the N=14(16) shell stabilisation in Z=8 oxygen isotopes and the N=20 shell quenching in {sup 32}Mg are symmetric with respect to the isospin projection quantum number Tz has been addressed. New {gamma}-ray decays were found in the neutron deficient {sup 36}Ca and {sup 36}K by impinging a radioactive ion beam of {sup 37}Ca on a secondary {sup 9}Be target. The fragmentation products were selected with the calorimeter telescope CATE and the emitted {gamma}-rays were measured with Ge Cluster, MINIBALL, and BaF{sub 2} HECTOR detectors. For {sup 36}Ca the 2{sub 1}{sup +}{yields}0{sub g.s.}{sup +} transition energy was determined to be 3015(16) keV, which is the heaviest T=2 nucleus from which {gamma}-spectroscopic information has been obtained so far. A comparison between the experimental 2{sub 1}{sup +} energies of {sup 36}Ca and its mirror nucleus {sup 36}S yielded a mirror energy difference of {delta}E{sub M}=-276(16) keV. In order to understand the large {delta}E{sub M} value, the experimental single-particle energies from the A=17, T=1/2 mirror nuclei were taken and applied onto modified isospin symmetric USD interactions in shell model calculations. These calculations were in agreement with the experimental result and showed that the experimental single-particle energies may account empirically for the one body part of Thomas-Ehrman and/or Coulomb effects. A method to extract the lifetime of excited states in fragmentation reactions was investigated. Therefore, the dependence between the lifetime of an excited state and the average de

Precise measurement of {gamma}(K{yields}e {nu}({gamma}))/{gamma}(K{yields}{mu} {nu}({gamma})) and study of K{yields}e {nu} {gamma}

Energy Technology Data Exchange (ETDEWEB)

Ambrosino, F.; Massarotti, P.; Meola, S.; Napolitano, M. [Dipartimento di Scienze Fisiche dell' Universita ' ' Federico II' ' , Napoli (Italy); INFN Sezione di Napoli, Napoli (Italy); Antonelli, A.; Antonelli, M.; Bencivenni, G.; Bloise, C.; Bossi, F.; Capon, G.; Capussela, T.; Ciambrone, P.; De Lucia, E.; De Simone, P.; Dreucci, M.; Felici, G.; Gatti, C.; Giovannella, S.; Jacewicz, M.; Lanfranchi, G.; Miscetti, S.; Moulson, M.; Murtas, F.; Palutan, M.; Santangelo, P.; Sciascia, B.; Sibidanov, A.; Spadaro, T.; Venanzoni, G. [Laboratori Nazionali di Frascati dell' INFN, Frascati (Italy); Archilli, F. [Dipartimento di Fisica dell' Universita ' ' Tor Vergata' ' , Rome (Italy); INFN Sezione di Roma Tor Vergata, Rome (Italy); Beltrame, P.; Denig, A.; Mueller, S. [Johannes Gutenberg-Universitaet, Institut fuer Kernphysik, Mainz (Germany); Bini, C.; De Santis, A.; De Zorzi, G.; Di Domenico, A.; Fiore, S.; Franzini, P.; Gauzzi, P. [Dipartimento di Fisica dell' Universita ' ' La Sapienza' ' , Rome (Italy); INFN Sezione di Roma, Rome (Italy); Bocchetta, S.; Ceradini, F.; Di Micco, B.; Nguyen, F. [Dipartimento di Fisica dell' Universita ' ' Roma Tre' ' , Rome (Italy); INFN Sezione di Roma Tre, Rome (Italy); Branchini, P.; Graziani, E.; Passeri, A.; Tortora, L. [INFN Sezione di Roma Tre, Rome (Italy); Capriotti, D. [Dipartimento di Fisica dell' Universita ' ' Roma Tre' ' , Rome (Italy); Di Donato, C. [INFN Sezione di Napoli, Napoli (Italy); Kulikov, V. [Institute for Theoretical and Experimental Physics, Moscow (Russian Federation); Lee-Franzini, J. [Laboratori Nazionali di Frascati dell' INFN, Frascati (Italy); State University of New York, Physics Department, Stony Brook (United States); Martini, M.; Patera, V.; Versaci, R. [Laboratori Nazionali di Frascati dell' INFN, Frascati (Italy); Dipartimento di Energetica dell' Universita ' ' La Sapienza' ' , Rome (Italy); Valente, P. [INFN Sezione di Roma, Rome (Italy)

2009-12-15

We present a precise measurement of the ratio R{sub K}={gamma}(K{yields}e{nu}({gamma}))/{gamma}(K{yields}{mu}{nu}({gamma})) and a study of the radiative process K{yields}e{nu}{gamma}, performed with the KLOE detector. The results are based on data collected at the Frascati e{sup +}e{sup -} collider DA {phi}NE for an integrated luminosity of 2.2 fb{sup -1}. We find R{sub K}=(2.493{+-}0.025{sub stat}{+-}0.019{sub syst}) x 10{sup -5}, in agreement with the Standard Model expectation. This result is used to improve constraints on parameters of the Minimal Supersymmetric Standard Model with lepton flavor violation. We also measured the differential decay rate d {gamma}(K{yields}e{nu}{gamma})/dE{sub {gamma}} for photon energies 10gamma}}<250 MeV. Results are compared with predictions from theory. (orig.)

Studies of natural radioactivity in cement products using gamma ray spectroscopy

International Nuclear Information System (INIS)

Ibrahim, N.; Periasamy, V.

2000-01-01

Evidence from our earlier study on several types of building materials has shown that cement contains a substantial amount of natural occurring radioactive materials. There are many brands of cement products available in Malaysia. Although the basic ingredients of cement are similar across brand, their proportion varies. In this study we have selected twelve brands of cement products which are analysed for natural radioactivity (U,Th,K) using gamma ray spectrometry. The gamma energies of interest are 583.1 keV, 609.3 keV and 1460 keV for nuclides 208 Tl, 214 Bi and 40 K respectively. Our findings show a relatively high activity of 40 K for all cement brands, ranging from 33 Bq/kg to as high as 3010 Bq/kg. Uranium activity ranges from 9Bq/kg to 672 Bq/kg while thorium activity was found range from 6Bq/kg to 94 Bq/kg. The radium equivalent activity is calculated for all brands and the values obtained range between 24 Bq/kg to 879 Bq/kg. Eight out of twelve products possess radium equivalent greater than 370 Bq/kg, a threshold limit for radiation dose equivalent to 1.5 mSv per annum. (author)

Determination of natural radioactive elements in Abo Zaabal, Egypt by means of gamma spectroscopy

International Nuclear Information System (INIS)

Morsy, Zeinab; Abd El-Wahab, Magda; El-Faramawy, Nabil

2012-01-01

Highlights: ► We examined the radioactivity of different type samples from Abo Zaabaal Lake. ► We evaluated the natural nuclide gamma-ray activities and their annual dose rates. ► We evaluated the concentrations of 226 Ra and its hazard indices. ► We assessed the absorbed dose in human. ► All results are within normal ranges. - Abstract: The natural nuclide gamma-ray activities and their respective annual effective dose rates, produced by 238 U, 232 Th, 40 K and 226 Ra, are determined for 10 different natural samples (soil–plant–water) from Abo Zaabaal Lake. This lake is located very close to the Egyptian reactors. The gamma spectra analysis indicates that the photo-gamma lines represent ten radioactive nuclides 234 Th, 239 Pu, 228 Ac, 226 Ra, 212 Pb, 214 Pb, 208 Tl, 212 Bi, 214 Bi and 40 K. These nuclides represent the daughters of the natural radioactive series 238 U and 232 Th with 40 K. The mean activity concentration of 238 U was found to be 6.57, 10.16 and 5.44 Bq kg −1 for (soil–plant–water); 8.46, 8.33 and 6.04 Bq kg −1 of 232 Th, and 136.3, 216.8 and 119.2 Bq kg −1 of 40 K respectively. The mean activity concentrations of 226 Ra were obtained which help to evaluate the radiation hazard indices as radium equivalent, internal and external hazard indices. In addition, to assess the radiation risk to a biosystem, the annual effective dose rate, the absorbed dose in human and the absorbed dose outdoor are also evaluated.

Characterization of Compton-suppressed TIGRESS detectors for high energy gamma-rays

International Nuclear Information System (INIS)

Kshetri, R.; Andreoiu, C.; Cross, D.S.; Galinski, N.; Ball, G.C.; Djongolov, M.; Garnsworthy, A.B.; Hackman, G.; Orce, J.N.; Pearson, C.; Triambak, S.; Williams, S.J.; Drake, T.; Smalley, D.; Svensson, C.E.

2009-01-01

The TRIUMF-ISAC Gamma-Ray Escape- Suppressed Spectrometer (TIGRESS) will consist of 12 large-volume, 32-fold segmented HPGe clover detectors. Each detector is shielded by a 20-fold segmented Compton suppression shield. For performing discrete gamma-ray spectroscopy of light mass nuclei with TIGRESS, we need information about full energy peak efficiency, resolution and lineshape of full energy peaks for high energy gamma-rays. However, suitable radioactive sources having decay gamma-rays of energies greater than ∼ 3.5 MeV are not easily available. So the characteristics of gamma spectrometers at energies higher than 3.5 MeV are usually determined from simulation data. Predictions from GEANT4 simulations (experimentally validated from 0.3 to 3 MeV) indicate that TIGRESS will be capable for single 10 MeV gamma-rays of absolute detection efficiency of 1.5% for backward configuration of the array. It has been observed experimentally that simulation results work well up to certain energies and might deviate at higher energies. So, it is essential to check the validity of simulation results for energies above 3.3 MeV. We have investigated the high energy performance of seven TIGRESS detectors up to 8 MeV

Population doses from terrestrial gamma exposure in China

International Nuclear Information System (INIS)

Ren, T.; Wang, Z.; Zhu, C.

1992-01-01

In order to estimate terrestrial gamma radiation exposure three nationwide surveys have been completed since 1981. The population-weighted outdoor and indoor arithmetic means of gamma dose rate based on momentary dose rate measurements using a NaI(Tl) environmental radiation meter and high-pressure ionisation chamber are, respectively, 80.3 nGy.h -1 and 120 nGy.h -1 . Based on integrating dose measurement using TLD CaSO 4 /Dy they are 67 nGy.h -1 and 89 nGy.h -1 respectively, and based on natural radionuclides concentrations in soil, determined by gamma spectroscopy analyses, they are 72.8 nGy.h -1 and 102 nGy.h -1 , respectively. These surveys were conducted independently by different groups. The best estimations of population-weighted gamma dose rates in China, based on all these surveys, would be 70 nGy.h -1 and 98 nGy.h -1 for outdoors and indoors, respectively. The annual average of effective dose equivalent is 0.56 mSv. These values are higher than the world averages estimated by UNSCEAR. The main reason is that the concentrations of 232 Th and 40 K in the soil of China are much higher than the world average estimated. (author)

Comparative studies on PADC polymeric detector treated by gamma radiation and Ar ion beam

International Nuclear Information System (INIS)

El-Saftawy, A.A.; Abdel Reheem, A.M.; Kandil, S.A.; Abd El Aal, S.A.; Salama, S.

2016-01-01

Highlights: • The induced defects on PADC polymer by low energy Ar ions bombardments have been investigated and evaluated with respect to gamma rays. • Low energy ions in the range of 3 keV is not examined elsewhere. And offers a competitive irradiation tool to gamma. • The structure, hardness and wear resistance enhanced after irradiation. • The optical properties changed, the optical band gap decreased and the refractive index enhanced. • The used ion source proves efficiency in improving surface properties of PADC polymer in comparison to the obtained results by the powerful energy source, gamma rays. - Abstract: In the present study, a comparative analysis and evaluation of the induced defects in polyallyl diglycol carbonate (PADC) polymeric detector exposed to Ar+ and gamma radiation were made. To get insight into the structure defects due to irradiation, X-ray diffraction (XRD) technique was employed. The PADC surface structure changed after irradiation due to the reduction in the surface crystalline structure and the formation of disordered systems. Also, surface morphology changes were traced using scanning electron microscopy (SEM) and showed minor surface irregularities after gamma irradiation and large changes upon Ar+ irradiation. Additionally, micro-hardness and friction coefficient of the irradiated samples were investigated and found to increase after irradiation. UV–vis spectroscopy was used to estimate the optical band gap energy which considered as the basis for calculating the number of conjugated carbon atoms responsible for the blackening effect and color changes took place over the PADC surface. It was found that as the applied dose increased, the band gap decreased and the number of carbon clusters get larger. The refractive index and the dispersion parameters for the studied polymer were calculated and discussed. Also, the induced defects on the polymer surface which serve as a non-radiative centers resulting in reduced

Comparative studies on PADC polymeric detector treated by gamma radiation and Ar ion beam

Energy Technology Data Exchange (ETDEWEB)

El-Saftawy, A.A., E-mail: aama1978@yahoo.com [Accelerators & Ion Sources Department, Nuclear Research Center, Atomic Energy Authority, P.O. 13759, Cairo (Egypt); Abdel Reheem, A.M. [Accelerators & Ion Sources Department, Nuclear Research Center, Atomic Energy Authority, P.O. 13759, Cairo (Egypt); Kandil, S.A. [Cyclotron project, Nuclear Research Center, Atomic Energy Authority, P.O. 13759, Cairo (Egypt); Abd El Aal, S.A. [Central Lab. for Elemental & Isotopic Analysis, Nuclear Research Center, Atomic Energy Authority, P.O. 13759, Cairo (Egypt); Salama, S. [Radiation Protection & Civil Defense Department, Nuclear Research Center, Atomic Energy Authority, P.O. 13759, Cairo (Egypt)

2016-05-15

Highlights: • The induced defects on PADC polymer by low energy Ar ions bombardments have been investigated and evaluated with respect to gamma rays. • Low energy ions in the range of 3 keV is not examined elsewhere. And offers a competitive irradiation tool to gamma. • The structure, hardness and wear resistance enhanced after irradiation. • The optical properties changed, the optical band gap decreased and the refractive index enhanced. • The used ion source proves efficiency in improving surface properties of PADC polymer in comparison to the obtained results by the powerful energy source, gamma rays. - Abstract: In the present study, a comparative analysis and evaluation of the induced defects in polyallyl diglycol carbonate (PADC) polymeric detector exposed to Ar+ and gamma radiation were made. To get insight into the structure defects due to irradiation, X-ray diffraction (XRD) technique was employed. The PADC surface structure changed after irradiation due to the reduction in the surface crystalline structure and the formation of disordered systems. Also, surface morphology changes were traced using scanning electron microscopy (SEM) and showed minor surface irregularities after gamma irradiation and large changes upon Ar+ irradiation. Additionally, micro-hardness and friction coefficient of the irradiated samples were investigated and found to increase after irradiation. UV–vis spectroscopy was used to estimate the optical band gap energy which considered as the basis for calculating the number of conjugated carbon atoms responsible for the blackening effect and color changes took place over the PADC surface. It was found that as the applied dose increased, the band gap decreased and the number of carbon clusters get larger. The refractive index and the dispersion parameters for the studied polymer were calculated and discussed. Also, the induced defects on the polymer surface which serve as a non-radiative centers resulting in reduced

Gamma signatures of the C-BORD Tagged Neutron Inspection System

Directory of Open Access Journals (Sweden)

Sardet A.

2018-01-01

Full Text Available In the frame of C-BORD project (H2020 program of the EU, a Rapidly relocatable Tagged Neutron Inspection System (RRTNIS is being developed to non-intrusively detect explosives, chemical threats, and other illicit goods in cargo containers. Material identification is performed through gamma spectroscopy, using twenty NaI detectors and four LaBr3 detectors, to determine the different elements composing the inspected item from their specific gamma signatures induced by fast neutrons. This is performed using an unfolding algorithm to decompose the energy spectrum of a suspect item, selected by X-ray radiography and on which the RRTNIS inspection is focused, on a database of pure element gamma signatures. This paper reports on simulated signatures for the NaI and LaBr3 detectors, constructed using the MCNP6 code. First experimental spectra of a few elements of interest are also presented.

Yrast spectroscopy in {sup 49-51}Ti via fusion-evaporation reaction induced by a radioactive beam

Energy Technology Data Exchange (ETDEWEB)

Niikura, M.; Ideguchi, E.; Michimasa, S.; Ota, S.; Shimoura, S.; Wakabayashi, Y. [University of Tokyo, Center for Nuclear Study, Wako, Saitama (Japan); Aoi, N.; Baba, H.; Fukuchi, T.; Ichikawa, Y.; Kubo, T.; Kurokawa, M.; Ohnishi, T.; Suzuki, H.; Yoshida, K. [RIKEN Nishina Center, Wako, Saitama (Japan); Iwasaki, H.; Onishi, T.K.; Suzuki, D. [University of Tokyo, Department of Physics, Tokyo (Japan); Liu, M.; Zheng, Y. [Chinese Academy of Sciences, Institute of Modern Physics, Lanzhou (China)

2009-12-15

In-beam {gamma} -ray spectroscopy of high-spin states in {sup 49-51}Ti was performed via the fusion-evaporation reaction using a radioactive beam. By excitation function and {gamma} - {gamma} coincidence analysis, yrast high-spin levels up to I=(21/2{sup -}),(11{sup +}),(17/2{sup -}) in {sup 49-51}Ti were determined. The levels were compared with full-pf -shell model calculation. The level structure indicates the persistency of the N=28 shell gap at yrast states in {sup 49-51}Ti. (orig.)

Energy loss spectroscopy applied to surface studies

International Nuclear Information System (INIS)

Lecante, J.

1975-01-01

The analysis of energy losses suffered by slow electrons (5 eV to 300 eV) back-scattered by single crystal surfaces appears to be a powerful method for surfaces studies. The inelastic scattering of these slow electrons limits their escape depth to the surface region which is defined here. After a review of the basic excitation processes due to the interaction between electrons and surfaces (phonons, plasmons and electronic transitions) a brief discussion is given about the instruments needed for this electron spectroscopy. Finally some experimental results are listed and it is shown that the comparison of the results given by ELS with other surface sensitive methods such as UPS is very fruitful and new information can be obtained [fr

Gamma irradiation effects on poly(vinylidene fluoride) films

International Nuclear Information System (INIS)

Ribeiro, Geise; Zen, Heloisa A.; Geraldes, Adriana N.; Souza, Camila P.; Parra, Duclerc F.; Lima, Luis Filipe C.P.; Lugao, Ademar B.

2009-01-01

In this work, the properties of Poly(vinylidene fluoride) PVDF films after exposing to gamma radiation at different doses (5, 10 and 15 kGy) were investigated. PVDF is a semicrystalline polymer that shows good properties in terms of chemical, thermal and electrical stabilities. The gamma radiation is a convenient and effective way of modification perfluorinated and partially fluorinated polymers such as PVDF. The properties of the pristine and irradiated PVDF films were studied by infrared spectroscopy, thermal analysis (TGA and DSC) and mechanical measurements at room temperature and at melting temperature of the PVDF. The infrared spectra of the irradiated PVDF samples do not present significant alterations in the absorption bands at all irradiated doses. The results obtained by thermal analysis indicate that the radiation does not alter significantly the decomposition temperature of the pristine PVDF film. Tensile strength measurements at room temperature before and after exposition to gamma radiation showed decrease of elongation at rupture in relation of pristine PVDF, suggesting that the radiation caused the crosslinking or chain scission of the PVDF film. (author)

Copper doping of ZnO crystals by transmutation of {sup 64}Zn to {sup 65}Cu: An electron paramagnetic resonance and gamma spectroscopy study

Energy Technology Data Exchange (ETDEWEB)

Recker, M. C.; McClory, J. W., E-mail: John.McClory@afit.edu; Holston, M. S.; Golden, E. M.; Giles, N. C. [Department of Engineering Physics, Air Force Institute of Technology, Wright-Patterson Air Force Base, Ohio 45433 (United States); Halliburton, L. E. [Department of Physics and Astronomy, West Virginia University, Morgantown, West Virginia 26506 (United States)

2014-06-28

Transmutation of {sup 64}Zn to {sup 65}Cu has been observed in a ZnO crystal irradiated with neutrons. The crystal was characterized with electron paramagnetic resonance (EPR) before and after the irradiation and with gamma spectroscopy after the irradiation. Major features in the gamma spectrum of the neutron-irradiated crystal included the primary 1115.5 keV gamma ray from the {sup 65}Zn decay and the positron annihilation peak at 511 keV. Their presence confirmed the successful transmutation of {sup 64}Zn nuclei to {sup 65}Cu. Additional direct evidence for transmutation was obtained from the EPR of Cu{sup 2+} ions (where {sup 63}Cu and {sup 65}Cu hyperfine lines are easily resolved). A spectrum from isolated Cu{sup 2+} (3d{sup 9}) ions acquired after the neutron irradiation showed only hyperfine lines from {sup 65}Cu nuclei. The absence of {sup 63}Cu lines in this Cu{sup 2+} spectrum left no doubt that the observed {sup 65}Cu signals were due to transmuted {sup 65}Cu nuclei created as a result of the neutron irradiation. Small concentrations of copper, in the form of Cu{sup +}-H complexes, were inadvertently present in our as-grown ZnO crystal. These Cu{sup +}-H complexes are not affected by the neutron irradiation, but they dissociate when a crystal is heated to 900 °C. This behavior allowed EPR to distinguish between the copper initially in the crystal and the copper subsequently produced by the neutron irradiation. In addition to transmutation, a second major effect of the neutron irradiation was the formation of zinc and oxygen vacancies by displacement. These vacancies were observed with EPR.

Effect of gamma irradiation on the structural, mechanical and optical properties of polytetrafluoroethylene sheet

Science.gov (United States)

Mohammadian-Kohol, M.; Asgari, M.; Shakur, H. R.

2018-04-01

In this study, the effects of gamma radiation on the chemical structure, mechanical and optical properties of polytetrafluoroethylene (PTFE) sheet were investigated with various doses up to 12 kGy. The chemical changes in the structure were studied by FTIR spectroscopy. Also, effects of radiation on the different mechanical parameters such as Young's modulus, toughness, strain, and stress were studied at the maximum tolerable force and the fracture points. Furthermore, changing the various optical parameters such as absorption coefficient, Urbach energy, optical band gaps, refractive index, optical dispersion parameters and plasma resonance frequency were studied by UV-visible spectroscopy. Formation of a band at 1594 cm-1, which was belonged to double carbon bonds, indicated that chain-scission was occurred at 12 kGy gamma irradiation dose. As well, the mechanical results showed an increase in the elastic behavior of PTFE sheets and a decrease in the plastic behavior of it with absorbed dose increasing. Moreover, the results showed that gamma irradiation can effectively change the various optical properties of PTFE sheets due to different phenomena such as degradation of the main chains, occurring chain-scission, formation of free radicals and cross-linking in the polymer structure.

Study of X-rays and nuclear gamma -rays in muonic thallium

CERN Document Server

Backe, H; Jahnke, U; Kankeleit, E; Pearce, R M; Petitjean, C; Schellenberg, L; Schneuwly, H; Schröder, W U; Walter, H K; Zehnder, A

1972-01-01

Energies and intensities of muonic X-rays, nuclear gamma -rays and mu -capture gamma -rays were measured in natural muonic thallium with Ge (Li) detectors. The absolute intensities of higher mu X-rays were reproduced by a cascade calculation starting with a statistical population at n=20 including K-, L- and M-conversion. The electron screening effect was deduced from energies of higher mu X-rays. Eight prompt nuclear gamma -rays were found. This excitation explains the anomalous intensity ratios of the 2p-1s and 3d-2p fine structure components. From the nuclear gamma -rays of the first excited states were deduced: the magnetic h.f. splittings, muonic isomer shifts E2/M1 mixing ratios and the half-life in the presence of the muon in /sup 205/Tl. Evidence for a magnetic nuclear polarization was found. An isotope shift of Delta E=10.35+or-0.25 keV was measured for the 1s/sub 1/2/ state which is compared with data from optical spectroscopy. From an analysis of the time distribution of delayed gamma -rays from mu...

Photoacoustic spectroscopy applied to the optical characterization of calcium phosphates for biomedical use

Energy Technology Data Exchange (ETDEWEB)

Mendez G, M. [ESFM-IPN, 07738 Mexico D.F. (Mexico); Cruz O, A. [CINVESTAV, Dept. of Physics, 07360 Mexico D.F. (Mexico)

2007-07-01

Full text: Photoacoustic Spectroscopy (PAS), based on the Rosencwaig and Gersho model, has been used for thermal and optical characterization of diverse materials. The use of PAS has become an important tool because is a nondestructive and no contact analytical technique. Furthermore its use to measure optical absorption spectra has advantages over the usual transmission measurements due to important features as the fact that scattered light does not disturb the measurements significantly and also the sample don't need to be prepared to have good quality surfaces. Then the optical properties of biological samples can be easily investigated with this technique. In the present study PAS is applied to obtain the optical absorption spectra of hydroxyapatite (HAp) [Ca{sub 10} (PO{sub 4} ){sub 6} (OH ){sub 2}] and bioactive calcium phosphates. The spectra of these samples ranged from 300 to 800 nm. All samples were prepared in a power form with particle size < 741m. Complementary studies X-ray diffraction and EDC were performed. (Author)

Characterization and Identification of Gamma-Irradiated Kimchi Cabbage and Broccoli by Electron Spin Resonance Spectroscopy using Different Sample Pre-treatments

International Nuclear Information System (INIS)

Kwak, J.Y.; Ahn, J.J.; Kashif Akram; Kim, G.R.; Kwon, J.H.

2012-01-01

Electron spin resonance (ESR) spectroscopy of gamma-irradiated fresh broccoli and kimchi cabbage was conducted to identify their irradiation history. Different pretreatments, such as freeze-drying (FD), oven-drying (OD), alcoholic-drying (ALD), and water-washing and alcoholic-drying (WAD) were used to lower the moisture contents of the samples prior to ESR analysis. The non-irradiated samples exhibited a single central signal (g 0 = 2.0007) with clear effect of Mn 2+ , especially in kimchi cabbage. Upon irradiation, there was an increase in the intensity of the central signal, and two side peaks, mutually spaced at 6 mT, were also observed. These side peaks with g 1 (left) = 2.023 and g 2 (right) = 1.985 were attributed to radiation-induced cellulose radicals. Leaf and stem in broccoli, and root and stem in kimchi cabbage provided good ESR signal responses upon irradiation. The signal noise was reduced in case of ALD and WAD pretreatments, particularly due to Mn 2+ signals. The ALD treatment was found most feasible to detect the improved ESR spectra in the irradiated samples. (author)

$\\gamma$ -spectroscopy of n-rich $^{95,96}$Rb nuclei by the incomplete fusion reaction of $^{94}$Kr on $^{7}$Li

CERN Multimedia

We propose an experiment with MINIBALL coupled to T-REX to investigate n-rich $^{95,96}$Rb nuclei by the incomplete fusion reaction of $^{94}$Kr on $^{7}$Li. The nuclei of interest will be populated by transfer of a triton into $^{94}$Kr, forming the excited $^{97}$Rb nucleus, followed by the emission of an alpha particle, which will be detected in the Si telescopes of T-REX. The $^{97}$Rb product will evaporate 1 or 2 (with the highest probability) neutrons leading to $^{96}$Rb or $^{95}$Rb, respectively. The aim of the experiment is twofold: \\\\ i) to perform a $\\gamma$- spectroscopy study of $^{95,96}$Rb nuclei with N=58,59, the structure of which is of particular interest in investigating the transition towards stable deformation at N=60, \\\\ ii) to acquire experience in using incomplete fusion reactions with the weakly bound $^{7}$Li target, in order to perform, at a later stage with HIE-ISOLDE, similar measurements induced by n-rich radioactive beams of Sn and Hg, for which at least 5 MeV/nucleon are need...

Study of the Neutron Deficient Pb and Bi Isotopes by Simultaneous Atomic- and Nuclear-Spectroscopy

CERN Multimedia

Kessler, T

2002-01-01

We propose to study systematically nuclear properties of the neutron deficient lead $^{183-189}$Pb, $^{191g}$Pb, $^{193g}$Pb and bismuth isotopes $^{188-200}$Bi by atomic spectroscopy with the ISOLDE resonance ionisation laser ion source (RILIS) combined with simultaneous nuclear spectroscopy at the detection set-up. The main focus is the determination of the mean square charge radii of $^{183-190}$Pb and $^{188-193}$Bi from which the influence of low-lying intruder states should become obvious. Also the nuclear spin and magnetic moments of ground-states and long-lived isomers will be determined unambiguously through evaluation of the hyperfine structure, and new isomers could be discovered. The decay properties of these nuclei can be measured by $\\alpha$-$\\gamma$ and $\\beta$-$\\gamma$ spectroscopy. With this data at hand, possible shape transitions around mid-shell at N$\\sim$104 will be studied. This data is crucial for the direct test of nuclear theory in the context of intruder state influence (e.g. energy ...

Gamma irradiation versus microbial contamination of Thai medicinal herbs

Directory of Open Access Journals (Sweden)

Wannipa Phianphak

2007-03-01

Full Text Available Seventeen species of herbs established in Thai traditional remedies were microbially decontaminated by gamma-irradiation doses of 7.7 and 8.8 kGy. The herb samples were randomly collected four times from producers in Chiangmai during a 1-year period. These were tested, qualitatively and quantitatively, for total aerobic bacteria, Staphylococcus spp., Salmonella spp., coliform bacteria, and fungi before and after gamma treatment. No microorganisms were found after gamma treatment; and the color, aroma, and texture of the herbs remained normal. The applied dose of gamma irradiation was within the regulatory limits in Thailand (<10 kGy and the main export country (USA< 30 kGy. Gamma irradiation is an effective treatment for microbial decontamination of Thai export herbs.

Characterization of crumb rubber modified by gamma radiation

Energy Technology Data Exchange (ETDEWEB)

Faldini, Sonia B.; Terence, Mauro C.; Miranda, Leila F.; Munhoz, Antonio H.; Domingues, Leandro S.; Coghetto, Gregory, E-mail: sfaldini@yahoo.com.br, E-mail: mauroterence@yahoo.com.br [Universidade Presbiteriana Mackenzie (UPM), Sao Paulo, SP (Brazil). Escola de Engenharia. Engenharia de Materiais

2013-07-01

The use of crumb rubber from scrap tires has become a common practice in the construction of roads, leading to improved properties of the asphalt and decreasing the environmental pollution. In this study, crumb rubber was modified by gamma radiation to eventually incorporate it into the asphalt and verify potential improvements of their properties. The crumb rubber modified by gamma radiation in the dose 500 kGy and 1000kGy was characterized by thermal analysis, infrared spectroscopy and scanning electron microscopy. The dose of radiation used has no effect on degradation temperatures. It is observed that the IV spectra of untreated rubbers and rubbers irradiated have substantially the same profile. The results indicate that despite small morphological changes in the irradiated rubber, they do not influence its degradation temperature and composition. (author)

Characterization of crumb rubber modified by gamma radiation

International Nuclear Information System (INIS)

Faldini, Sonia B.; Terence, Mauro C.; Miranda, Leila F.; Munhoz, Antonio H.; Domingues, Leandro S.; Coghetto, Gregory

2013-01-01

The use of crumb rubber from scrap tires has become a common practice in the construction of roads, leading to improved properties of the asphalt and decreasing the environmental pollution. In this study, crumb rubber was modified by gamma radiation to eventually incorporate it into the asphalt and verify potential improvements of their properties. The crumb rubber modified by gamma radiation in the dose 500 kGy and 1000kGy was characterized by thermal analysis, infrared spectroscopy and scanning electron microscopy. The dose of radiation used has no effect on degradation temperatures. It is observed that the IV spectra of untreated rubbers and rubbers irradiated have substantially the same profile. The results indicate that despite small morphological changes in the irradiated rubber, they do not influence its degradation temperature and composition. (author)

Review of superconducting transition-edge sensors for x-ray and gamma-ray spectroscopy

International Nuclear Information System (INIS)

Ullom, Joel N; Bennett, Douglas A

2015-01-01

We present a review of emerging x-ray and gamma-ray spectrometers based on arrays of superconducting transition-edge sensors (TESs). Special attention will be given to recent progress in TES applications and in understanding TES physics. (paper)

A matrix-inversion method for gamma-source mapping from gamma-count data - 59082

International Nuclear Information System (INIS)

Bull, Richard K.; Adsley, Ian; Burgess, Claire

2012-01-01

Gamma ray counting is often used to survey the distribution of active waste material in various locations. Ideally the output from such surveys would be a map of the activity of the waste. In this paper a simple matrix-inversion method is presented. This allows an array of gamma-count data to be converted to an array of source activities. For each survey area the response matrix is computed using the gamma-shielding code Microshield [1]. This matrix links the activity array to the count array. The activity array is then obtained via matrix inversion. The method was tested on artificially-created arrays of count-data onto which statistical noise had been added. The method was able to reproduce, quite faithfully, the original activity distribution used to generate the dataset. The method has been applied to a number of practical cases, including the distribution of activated objects in a hot cell and to activated Nimonic springs amongst fuel-element debris in vaults at a nuclear plant. (authors)

The gamma ray spectrometer GA.SP

Energy Technology Data Exchange (ETDEWEB)

Bazzacco, D [Instituto Nazionale di Fisica Nucleare, Sezione di Padova, Padova (Italy)

1992-08-01

GA.SP is a general purpose 4{pi} detector array for advanced {gamma}-spectroscopy and, in the same time, a suitable system for reaction mechanism studies. The detector is sited at the LNL Tandem+Linac accelerator and has been built as a joint project of INFN Padova, LNL, Milano and Firenze. The array consists of 40 Compton suppressed HPGe detectors and of a 4{pi} calorimeter composed of 80 BGO crystals. The detector houses a reaction chamber of 34 cm diameter where a charged particles multiplicity filter composed of 40 Si detectors is going to be installed. Evaporation residues produced in the centre of GA.SP can be injected into the recoil mass spectrometer (RMS, named CAMEL) in use at LNL, without the need to remove any of the gamma detectors. The coupled operation of GA.SP, RMS and Si ball will give a unique instrument for identification and study of weak reaction channels. (author). 6 figs.

Nonlinear resonant ultrasound spectroscopy (NRUS) applied to damage assessment in bone

Science.gov (United States)

Muller, Marie; Sutin, Alexander; Guyer, Robert; Talmant, Maryline; Laugier, Pascal; Johnson, Paul A.

2005-12-01

Nonlinear resonant ultrasound spectroscopy (NRUS) is a resonance-based technique exploiting the significant nonlinear behavior of damaged materials. In NRUS, the resonant frequency(ies) of an object is studied as a function of the excitation level. As the excitation level increases, the elastic nonlinearity is manifest by a shift in the resonance frequency. This study shows the feasibility of this technique for application to damage assessment in bone. Two samples of bovine cortical bone were subjected to progressive damage induced by application of mechanical cycling. Before cycling commenced, and at each step in the cycling process, NRUS was applied for damage assessment. For independent assessment of damage, high-energy x-ray computed tomography imaging was performed but was only useful in identifying the prominent cracks. As the integral quantity of damage increased, NRUS revealed a corresponding increase in the nonlinear response. The measured change in nonlinear response is much more sensitive than the change in linear modulus. The results suggest that NRUS could be a potential tool for micro-damage assessment in bone. Further work must be carried out for a better understanding of the physical nature of damaged bone and for the ultimate goal of the challenging in vivo implementation of the technique.

Studies of P(VDF-HFP) copolymer applied to gamma dosimetry

International Nuclear Information System (INIS)

Liz, Otavio S.R.; Medeiros, Adriana S.

2011-01-01

When polymeric materials are irradiated by ionizing radiation, the effects are roughly divided into two types, degradation (chain scission) and chain link (crosslinking). These effects are normally identified by spectroscopic analysis in the UV-Vis and Infrared region. Recently, the intensities of optical absorption in the ultraviolet visible region (273 nm) due to radio-induction of conjugated C = C bonds in P(VDF-TrFE) copolymers have been successfully used for high dose gamma dosimetry, for doses ranging from 0.1 to 200 kGy. In this context, there is now an interest to conduct a similar systematic investigation of another fluorinated copolymer of PVDF, the poly(fluorovinylidene-co-hexafluoropropylene) [P(VDF-HFP)], not only in the UV-VIS region but also in the near and mid-infrared region. The copolymer used was obtained by randomly adding 10% molar of [CF2- CF-CF3] monomers in the [CH2-CF2]n main chain of PVDF homopolymer. Preliminary results have shown that the irradiated copolymer has characteristic absorption bands originated by irradiation in the FTIR spectrum. It was found that the 1852 cm -1 band, associated with C = O bonds, have a linear correlation with the absorbed dose for doses ranging from 10 to 750 kGy. The absorption band at 1729 cm -1 , associated to chain oxidation (C = O), has shown a similar behavior and can be used to measure doses from 100 to 1000 kGy. These results indicate that the FTIR absorption bands of gamma irradiated P (VDF-HFP) have great potential to be used in high dose dosimetry, without the addition of dyes. (author)